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Sample records for two-photon transition amplitudes

  1. Adiabatic following in two-photon transition

    Energy Technology Data Exchange (ETDEWEB)

    Nayfeh, M.H.; Nayfeh, A.H.

    1977-01-01

    There has been much interest recently in coherent multiphoton transitions in many-level systems. The present work considers the effect of relaxation in the response of a three-level system to a smoothly varying, near-resonant, two-photon field. The relaxation-dependent contributions to the nonlinear refractive index are calculated. It is shown that the coherent interaction of two smoothly varying, near-resonant, two-photon pulses with a three-level system can be described by ''two-photon damped Bloch equations'' which are analogous to those for a one-photon transition in a two-level system except for the presence of a two-photon coupling and a frequency shift. 1 figure. (RWR)

  2. Adiabatic following in two-photon transition

    Energy Technology Data Exchange (ETDEWEB)

    Nayfeh, M.H.; Nayfeh, A.H.

    1977-03-01

    The coherent interaction of two smoothly varying, near-resonant, two-photon pulses with a three-level system can be described by ''two-photon damped Bloch equations'' which are analogous to those for a one-photon transition in a two-level system except for the presence of a two-photon coupling and a frequency shift. These equations are solved for the cases ..gamma../sub 1/, ..gamma../sub 2/ very-much-less-than ..cap omega.., ..gamma../sub 1/ = ..gamma../sub 2/, and ..gamma../sub 2/k/sup 2/epsilon/sup 4//..cap omega../sup 2/, ..gamma../sub 1/ very-much-less-than ..cap omega.., where ..gamma../sub 1/ and ..gamma../sub 2/ are the atomic energy and phase relaxation widths, respectively, and ..cap omega.. is the Rabi frequency. The leading contribution to the refractive index is intensity dependent, caused by the level shifts inherent in multiphoton processes; it includes a relaxation dependent part which is important at times shorter than ..gamma../sup -1//sub 1/. The second-order contributions depend on the square of the intensity and the time-integrated square of the intensity. The latter contribution, which is relaxation dependent, causes line asymmetry at the long-wavelength wing; it consists of a term proportional to ..gamma../sub 2/-..gamma../sub 1/ and only important at early times and a term proportional to 2..gamma../sub 2/-..gamma../sub 1/.

  3. Modulation of attosecond beating by resonant two-photon transition

    CERN Document Server

    Galán, Álvaro Jiménez; Martín, Fernando

    2015-01-01

    We present an analytical model that characterizes two-photon transitions in the presence of autoionising states. We applied this model to interpret resonant RABITT spectra, and show that, as a harmonic traverses a resonance, the phase of the sideband beating significantly varies with photon energy. This phase variation is generally very different from the $\\pi$ jump observed in previous works, in which the direct path contribution was negligible. We illustrate the possible phase profiles arising in resonant two-photon transitions with an intuitive geometrical representation.

  4. Long vs. short distance dispersive two-photon $K_{L} \\to \\mu^{+} \\mu^{-}$ amplitude

    CERN Document Server

    Eeg, Jan O; Picek, I

    1999-01-01

    We report on the calculation of the two-loop electroweak, two-photon mediated short-distance dispersive K_L \\to \\mu^+\\mu^- decay amplitude. QCD corrections change the sign of this contribution and reduce it by an order of magnitude. The resulting amplitude enables us to provide a constraint on the otherwise uncertain long-distance dispersive amplitude.

  5. Temporal behavior of low-amplitude two-photon screening-photovoltaic grey spatial solitons

    Institute of Scientific and Technical Information of China (English)

    JI Xuan-mang; JIANG Qi-chang; WANG Jin-lai; LIU Jin-song

    2011-01-01

    The time-dependent formation of one-dimensional two-photon screening-photovoltaic (PV) grey spatial solitons under low-amplitude conditions is presented theoretically. The time-dependent propagation equation of two-photon screening- photovoltaic solitons is obtained by the numerical method. The results indicate that as the time evolves, the intensity width of grey screening-photovoltaic spatial solitons decreases monotonously to a minimum value towards the steady state. The higher the ratio of soliton peak intensity to the dark irradiation intensity, the narrower the width of grey solitons within the propagation time.

  6. Two-photon transition form factor of c ¯ quarkonia

    Science.gov (United States)

    Chen, Jing; Ding, Minghui; Chang, Lei; Liu, Yu-xin

    2017-01-01

    The two-photon transition of c ¯c quarkonia are studied within a covariant approach based on the consistent truncation scheme of the quantum chromodynamics Dyson-Schwinger equation for the quark propagator and the Bethe-Salpeter equation for the mesons. We find the decay widths of ηc→γ γ and χc 0 ,2→γ γ in good agreement with experimental data. The obtained transition form factor of ηc→γ γ* for a wide range of spacelike photon-momentum-transfer squared is also in agreement with the experimental findings of the BABAR experiment. As a by-product, the decay widths of ηb,χb 0 ,2→γ γ and the transition form factor of ηb,χc 0 ,b 0→γ γ* are predicted, which await experimental testing.

  7. Nonresonant two-photon transitions in length and velocity gauges

    Science.gov (United States)

    Jentschura, U. D.

    2016-08-01

    We reexamine the invariance of two-photon transition matrix elements and corresponding two-photon Rabi frequencies under the "gauge" transformation from the length to the velocity gauge. It is shown that gauge invariance, in the most general sense, only holds at exact resonance, for both one-color as well as two-color absorption. The arguments leading to this conclusion are supported by analytic calculations which express the matrix elements in terms of hypergeometric functions, and ramified by a "master identity" which is fulfilled by off-diagonal matrix elements of the Schrödinger propagator under the transformation from the velocity to the length gauge. The study of the gauge dependence of atomic processes highlights subtle connections between the concept of asymptotic states, the gauge transformation of the wave function, and infinitesimal damping parameters for perturbations and interaction Hamiltonians that switch off the terms in the infinite past and future [of the form exp(-ɛ |t |)] . We include a pertinent discussion.

  8. Nuclear two-photon decay in 0 +→0 + transitions

    Science.gov (United States)

    Kramp, J.; Habs, D.; Kroth, R.; Music, M.; Schirmer, J.; Schwalm, D.; Broude, C.

    1987-11-01

    The two-photon decay of the first excited 0 + state of 16O has been measured using the Heidelberg-Darmstadt crystal ball. A branching ratio of {Γ γγ}/{Γ tot} = (6.6±0.5) · 10 -4 was obtained. As in the cases of 40Ca and 90Zr previously reported by us, the 2γ decay of 16O proceeds via double E1 and M1 transitions of similar strength; the evidence is the observed interference term in the 2γ angular correlation. The ratio of the matrix elements {α E1 }/{χ} for 16O was restricted to the two inverse values (-6.2±1.5) or (-0.16±0.04). An interpretation of 2γ matrix elements observed for 16O, 40Ca and 90Zr in terms of the electric polarizabilities and magnetic susceptibility is given leading to a qualitative understanding of this decay mode.

  9. Polarization Effects in Two-Photon Free-Free Transitions in Laser-Assisted Electron-Hydrogen Collisions

    CERN Document Server

    Cionga, Aurelia

    2013-01-01

    Two-photon free-free transitions in elastic laser-assisted electron-hydrogen collisions are studied in the domain of high scattering energies and low or moderate field intensities, in the third order of perturbation theory, taking into account all the involved Feynman diagrams. Based on the analytical expressions of the transition amplitudes, the differential cross sections for two-photon absorption/emission are computed at impact energy $E_i=100$ eV. The effect of field polarizations on the angular distribution and on the frequency dependence of the differential cross section is analyzed.

  10. Absolute Frequency Measurement of Rubidium 5S-7S Two-Photon Transitions

    CERN Document Server

    Morzynski, Piotr; Ablewski, Piotr; Gartman, Rafal; Gawlik, Wojciech; Maslowski, Piotr; Nagorny, Bartlomiej; Ozimek, Filip; Radzewicz, Czeslaw; Witkowski, Marcin; Ciurylo, Roman; Zawada, Michal

    2013-01-01

    We report the absolute frequency measurements of rubidium 5S-7S two-photon transitions with a cw laser digitally locked to an atomic transition and referenced to an optical frequency comb. The narrow, two-photon transition, 5S-7S (760 nm) insensitive to first order in a magnetic field, is a promising candidate for frequency reference. The performed tests yield the transition frequency with accuracy better than reported previously.

  11. Coherent control of non-resonant two-photon transition in molecular system

    Institute of Scientific and Technical Information of China (English)

    Zhang Hui; Zhang Shi-An; Wang Zu-Geng; Sun Zhen-Rong

    2010-01-01

    In this paper,we study theoretically and experimentally the coherent control of non-resonant two-photon transition in a molecular system (Perylene dissolved in chloroform solution) by shaping the femtosecond pulses with simple phase patterns (cosinusoidal and π phase step-function shape).The control efficiency of the two-photon transition probability is correlated with both the laser field and the molecular absorption bandwidth.Our results demonstrate that,the two-photon transition probability in a molecular system can be reduced but not completely eliminated by manipulating the laser field,and the control efficiency is minimal when the molecular absorption bandwidth is larger than twice the laser spectral bandwidth.

  12. Efficient two-photon sensitized luminescence of europium (Ⅲ) complex based on hypersensitive transitions

    Institute of Scientific and Technical Information of China (English)

    Meng Shi; Hua Li; Mei Pan; Fufang Su; Lili Ma; Peigao Han; Hezhou Wang

    2011-01-01

    Red frequency-upconversion fluorescence emission is observed in europium(Ⅲ) complex with encapsulating polybenzimidazole tripodal ligands, pumped with 930- and 1070-nm picosecond laser pulses. The luminescence of transition 5D0 →7F2 (612 nm) is induced by two-photon absorption of hypersensitive transitions 7F0 →5D2 (465 nm) and 7F1 →5D1 (535 nm). Analysis results suggest that the two-photon excitation strength of these hypersensitive transitions is increased dramatically owing to the C3 symmetry of the coordination field.%@@ Red frequency-upconversion fluorescence emission is observed in europium(Ⅲ) complex with encapsulating polybenzimidazole tripodal ligands, pumped with 930- and 1070-nm picosecond laser pulses.The luminescence of transition 5D0 →7F2 (612 nm) is induced by two-photon absorption of hypersensitive transitions 7F0 →5D2 (465 nm) and 7F1 →5D1 (535 nm).Analysis results suggest that the two-photon excitation strength of these hypersensitive transitions is increased dramatically owing to the Ca symmetry of the coordination field.

  13. A direct frequency comb for two-photon transition spectroscopy in a cesium vapor

    Institute of Scientific and Technical Information of China (English)

    Zhang Yi-Chi; Wu Ji-Zhou; Li Yu-Qing; Jin Li; Ma Jie; Wang Li-Rong; Zhao Yan-Ting; Xiao Lian-Tuan; Jia Suo-Tang

    2012-01-01

    A phase-stabilized femtosecond frequency comb is used to measure high-resolution spectra of two-photon transition 62S1/2-62P1/2,3/2-82S1/2 in a cesium vapor.The broadband laser output from a femtosecond frequency comb is split into counter-propagating parts,shaped in an original way,and focused into a room-temperature cesium vapor.We obtain high-resolution two-photon spectroscopy by scanning the repetition rate of femtosecond frequency comb,and through absolute frequency measurements.

  14. Transition probabilities for two-photon H(1-2) and He(11-21) transitions: A partial-closure approach

    Indian Academy of Sciences (India)

    Monika Bassi; K L Baluja

    2000-03-01

    Transition amplitudes and transition probabilities for the two-photon 1-2 transition in the hydrogen atom and 11-21 transition in helium atom have been calculated using a partialclosure approach. The dominant term is calculated exactly and the remaining sum over intermediate states is calculated using a mean excitation energy. Our value of the transition amplitudes agree within 2% with the exact results for the hydrogen case. Our value of the transition probability for hydrogen is 8.50 -1 which is in good accord with its known value 8.226 s-1. For helium, the photon energy distribution of the metastable 21 state is in good agreement with the accurate values. The corresponding transition probability is 53.7 s-1 which is in good agreement with the accurate value 51.3 s-1.

  15. Evidence for the Direct Two-Photon Transition from $\\psi'$ to $J/\\psi$

    CERN Document Server

    Ablikim, M; Ambrose, D J; An, F F; An, Q; An, Z H; Bai, J Z; Ferroli, R B; Ban, Y; Becker, J; Berger, N; Bertani, M B; Bian, J M; Boger, E; Bondarenko, O; Boyko, I; Briere, R A; Bytev, V; Cai, X; Calcaterra, A C; Cao, G F; Chang, J F; Chelkov, G; Chen, G; Chen, H S; Chen, J C; Chen, M L; Chen, S J; Chen, Y; Chen, Y B; Cheng, H P; Chu, Y P; Cronin-Hennessy, D; Dai, H L; Dai, J P; Dedovich, D; Deng, Z Y; Denig, A; Denysenko, I; Destefanis, M; Ding, W M; Ding, Y; Dong, L Y; Dong, M Y; Du, S X; Fang, J; Fang, S S; Fava, L; Feldbauer, F; Feng, C Q; Fu, C D; Fu, J L; Gao, Y; Geng, C; Goetzen, K; Gong, W X; Gradl, W; Greco, M; Gu, M H; Gu, Y T; Guan, Y H; Guo, A Q; Guo, L B; Guo, Y P; Han, Y L; Hao, X Q; Harris, F A; He, K L; He, M; He, Z Y; Held, T; Heng, Y K; Hou, Z L; Hu, H M; Hu, J F; Hu, T; Huang, B; Huang, G M; Huang, J S; Huang, X T; Huang, Y P; Hussain, T; Ji, C S; Ji, Q; Ji, X B; Ji, X L; Jia, L K; Jiang, L L; Jiang, X S; Jiao, J B; Jiao, Z; Jin, D P; Jin, S; Jing, F F; Kalantar-Nayestanaki, N; Kavatsyuk, M; Kuehn, W; Lai, W; Lange, J S; Leung, J K C; Li, C H; Li, Cheng; Li, Cui; Li, D M; Li, F; Li, G; Li, H B; Li, J C; Li, K; Li, Lei; Li, N B; Li, Q J; Li, S L; Li, W D; Li, W G; Li, X L; Li, X N; Li, X Q; Li, X R; Li, Z B; Liang, H; Liang, Y F; Liang, Y T; Liao, G R; Liao, X T; Liu, B J; Liu, B J; Liu, C L; Liu, C X; Liu, C Y; Liu, F H; Liu, Fang; Liu, Feng; Liu, H; Liu, H B; Liu, H H; Liu, H M; Liu, H W; Liu, J P; Liu, Kun; Liu, Kai; Liu, K Y; Liu, P L; Liu, S B; Liu, X; Liu, X H; Liu, Y B; Liu, Y; Liu, Z A; Liu, Zhiqiang; Liu, Zhiqing; Loehner, H; Lu, G R; Lu, H J; Lu, J G; Lu, Q W; Lu, X R; Lu, Y P; Luo, C L; Luo, M X; Luo, T; Luo, X L; Lv, M; Ma, C L; Ma, F C; Ma, H L; Ma, Q M; Ma, S; Ma, T; Ma, X Y; Ma, Y; Maas, F E; Maggiora, M; Malik, Q A; Mao, H; Mao, Y J; Mao, Z P; Messchendorp, J G; Min, J; Min, T J; Mitchell, R E; Mo, X H; Morales, C Morales; Motzko, C; Muchnoi, N Yu; Nefedov, Y; Nicholson, C; Nikolaev, I B; Ning, Z; Olsen, S L; Ouyang, Q; Pacetti, S P; Park, J W; Pelizaeus, M; Peters, K; Ping, J L; Ping, R G; Poling, R; Prencipe, E; Pun, C S J; Qi, M; Qian, S; Qiao, C F; Qin, X S; Qin, Y; Qin, Z H; Qiu, J F; Rashid, K H; Rong, G; Ruan, X D; Sarantsev, A; Schulze, J; Shao, M; Shen, C P; Shen, X Y; Sheng, H Y; Shepherd, M R; Song, X Y; Spataro, S; Spruck, B; Sun, D H; Sun, G X; Sun, J F; Sun, S S; Sun, X D; Sun, Y J; Sun, Y Z; Sun, Z J; Sun, Z T; Tang, C J; Tang, X; Thorndike, E H; Tian, H L; Toth, D; Ulrich, M U; Varner, G S; Wang, B; Wang, B Q; Wang, K; Wang, L L; Wang, L S; Wang, M; Wang, P; Wang, P L; Wang, Q; Wang, Q J; Wang, S G; Wang, X F; Wang, X L; Wang, Y D; Wang, Y F; Wang, Y Q; Wang, Z; Wang, Z G; Wang, Z Y; Wei, D H; Weidenkaff, P; Wen, Q G; Wen, S P; Werner, M W; Wiedner, U; Wu, L H; Wu, N; Wu, S X; Wu, W; Wu, Z; Xia, L G; Xiao, Z J; Xie, Y G; Xiu, Q L; Xu, G F; Xu, G M; Xu, H; Xu, Q J; Xu, X P; Xu, Y; Xu, Z R; Xue, F; Xue, Z; Yan, L; Yan, W B; Yan, Y H; Yang, H X; Yang, T; Yang, Y; Yang, Y X; Ye, H; Ye, M; Ye, M H; Yu, B X; Yu, C X; Yu, J S; Yu, S P; Yuan, C Z; Yuan, W L; Yuan, Y; Zafar, A A; Zallo, A Z; Zeng, Y; Zhang, B X; Zhang, B Y; Zhang, C C; Zhang, D H; Zhang, H H; Zhang, H Y; Zhang, J; Zhang, J G; Zhang, J Q; Zhang, J W; Zhang, J Y; Zhang, J Z; Zhang, L; Zhang, S H; Zhang, T R; Zhang, X J; Zhang, X Y; Zhang, Y; Zhang, Y H; Zhang, Y S; Zhang, Z P; Zhang, Z Y; Zhao, G; Zhao, H S; Zhao, J W; Zhao, K X; Zhao, Lei; Zhao, Ling; Zhao, M G; Zhao, Q; Zhao, S J; Zhao, T C; Zhao, X H; Zhao, Y B; Zhao, Z G; Zhemchugov, A; Zheng, B; Zheng, J P; Zheng, Y H; Zheng, Z P; Zhong, B; Zhong, J; Zhou, L; Zhou, X K; Zhou, X R; Zhu, C; Zhu, K; Zhu, K J; Zhu, S H; Zhu, X L; Zhu, X W; Zhu, Y M; Zhu, Y S; Zhu, Z A; Zhuang, J; Zou, B S; Zou, J H; Zuo, J X

    2012-01-01

    The two-photon transition $\\psi' \\to \\gamma\\gamma J/\\psi$ is studied in a sample of 106 million $\\psi'$ decays collected by the BESIII detector. The branching fraction is measured to be $(3.3\\pm0.6(\\unit{stat})^{+0.8}_{-1.1}(\\unit{syst})) \\times10^{-4}$ using $J/\\psi \\to e^+e^-$ and $J/\\psi \\to \\mu^+\\mu^-$decays. This work represents the first measurement of a two-photon transition among charmonium states. The orientation of the $\\psi'$ decay plane and the $J/\\psi$ polarization in this decay are also studied. In addition, the product branching fractions of sequential $E1$ transitions $\\psi'\\to\\gamma\\chi_{cJ}$, $\\chi_{cJ}\\to\\gamma J/\\psi (J=0,1,2)$ are reported.

  16. A superradiant laser based on two-photon Raman transition of caesium atoms

    CERN Document Server

    Liu, Pengfei

    2013-01-01

    We propose a superradiant laser based on two-photon Raman transition of caesium-133 atoms which collectively emit photons on an ultra narrow transition into the mode of a low Q resonator known as optical bad-cavity regime. The spin-spin correlation which characterizes the collective effect is demonstrated. We theoretically predict that the optical radiation has an extremely narrow linewidth in the 98 (1) *10-2 mHz range, smaller than the transition itself due to collective effects, and a power level of 7 (1)*10-10 W is possible, which can provide a possible new way to realize an optical clock with a millihertz linewidth.

  17. Direct two-photon excitation of isomeric transition in thorium-229 nucleus

    CERN Document Server

    Romanenko, V I; Yatsenko, L P; Romanenko, A V; Litvinov, A N; Kazakov, G A

    2012-01-01

    A possibility of the two-photon excitation of an isomeric state in a nucleus of thorium-229 has been discussed. The fluorescence intensity of the excitation is demonstrated to be identical for the irradiation of nuclei with either monochromatic light or polychromatic radiation consisting of a sequence of short light pulses of the same intensity. The two-photon excitation of Th^{3+} ion in an electromagnetic trap with a focused laser beam with a wavelength of about 320 nm and power of 100 mW can lead to the absorption saturation, at which the fluorescence emission with the frequency of the transition in a nucleus is maximal. In crystals doped with Th^{4+} to a concentration of about 10^{18} cm^{-3} and irradiated with a laser radiation 10 W in power, the emission of several photons per second with a wavelength of about 160 nm becomes possible.

  18. Two-photon frequency comb spectroscopy of the 6s-8s transition in cesium.

    Science.gov (United States)

    Fendel, P; Bergeson, S D; Udem, Th; Hänsch, T W

    2007-03-15

    We report a new absolute frequency measurement of the Cs 6s-8s two-photon transition measured using frequency comb spectroscopy. The fractional frequency uncertainty is 5x10(-11), a factor of 6 better than previous results. The comb is derived from a stabilized picosecond laser and referenced to an octave-spanning femtosecond frequency comb. The relative merits of picosecond-based frequency combs are discussed, and it is shown that the AC Stark shift of the transition is determined by the average rather than the much larger peak intensity.

  19. Two-photon finite-pulse model for resonant transitions in attosecond experiments

    CERN Document Server

    Galán, Álvaro Jiménez; Argenti, Luca

    2015-01-01

    We present an analytical model capable of describing two-photon ionization of atoms with attosecond pulses in the presence of intermediate and final isolated autoionizing states. The model is based on the finite-pulse formulation of second-order time-dependent perturbation theory. It approximates the intermediate and final states with Fano's theory for resonant continua, and it depends on a small set of atomic parameters that can either be obtained from separate \\emph{ab initio} calculations, or be extracted from few selected experiments. We use the model to compute the two-photon resonant photoelectron spectrum of helium below the N=2 threshold for the RABITT (Reconstruction of Attosecond Beating by Interference of Two-photon Transitions) pump-probe scheme, in which an XUV attosecond pulse train is used in association to a weak IR probe, obtaining results in quantitative agreement with those from accurate \\emph{ab initio} simulations. In particular, we show that: i) Use of finite pulses results in a homogene...

  20. Spectral distribution of the 2 → 1 two-photon transition in atoms and few-electron ions

    Indian Academy of Sciences (India)

    Ajay Kumar; S Trotsenko; A V Volotka; D Banaś; H F Beyer; H Bräuning; S Fritzsche; A Gumberidze; S Hagmann; S Hess; C Kozhuharov; R Reuschl; U Spillmann; M Trassinelli; G Weber; Th Stöhlker

    2011-02-01

    The two-photon decay of the 2 state to the ground state in dressed atoms and oneor two-electron ions has been studied for several decades. Relativistic calculations have shown an -dependence of the spectral shape of this two-photon transition in one- or two-electron ions. We have measured the spectral distribution of the 121 0 → 12 1 0 two-photon transition in He-like tin at the ESR storage ring using a new approach for such experiments. In this method, relativistic collisions of initially Li-like projectiles with a gaseous target were used to populate exclusively the first excited state, 12, of He-like tin, which provided a clean two-photon spectrum. The measured two-photon spectral distribution was compared with fully relativistic calculations. The obtained results show very good agreement with the calculations for He-like tin

  1. Two Photon Transition Form Factor of $\\bar{c}c $ Quarkonia

    CERN Document Server

    Chen, Jing; Chang, Lei; Liu, Yu-xin

    2016-01-01

    The two photon transition of $\\bar{c}c$ quarkonia are studied within a covariant approach based on the consistent truncation scheme of the quantum chromodynamics Dyson-Schwinger equation for the quark propagator and the Bethe--Salpeter equation for the mesons. We find the decay widths of $\\eta_{c}^{} \\to \\gamma\\gamma$ and $\\chi_{c0,2}^{} \\to \\gamma\\gamma$ in good agreement with experimental data. The obtained transition form factor of $\\eta_{c}^{} \\to \\gamma\\gamma^{\\ast}$ for a wide range of space-like photon momentum transfer squared is also in agreement with the experimental findings of the BABAR experiment. As a by-product, the decay widths of $\\eta_{b}^{},\\chi_{b0,2}^{} \\to \\gamma\\gamma$ and the transition form factor of $\\eta_{b}^{}, \\chi_{c0,b0}^{} \\to\\gamma\\gamma^{\\ast}$ are predicted, which await for experimental test.

  2. Efficient photoionization for barium ion trapping using a dipole-allowed resonant two-photon transition

    CERN Document Server

    Leschhorn, G; Schaetz, T

    2011-01-01

    Two efficient and isotope-selective resonant two-photon ionization techniques for loading barium ions into radio-frequency (RF)-traps are demonstrated. The scheme of using a strong dipole-allowed transition at \\lambda=553 nm as a first step towards ionization is compared to the established technique of using a weak intercombination line (\\lambda=413 nm). An increase of two orders of magnitude in the ionization efficiency is found favoring the transition at 553 nm. This technique can be implemented using commercial all-solid-state laser systems and is expected to be advantageous compared to other narrowband photoionization schemes of barium in cases where highest efficiency and isotope-selectivity are required.

  3. Electric field allowed molecular transitions for one and two photon excitation microscopy.

    Science.gov (United States)

    Mondal, Partha Pratim; Diaspro, Alberto

    2008-07-01

    We propose an excitation technique for observing single and two photon excitation in those molecules for which such transitions are forbidden by the selection rules. This is possible by the application of an external electric field that perturbs the molecular orbitals, thereby resulting in a significant shift of energy levels. Such a shift of energy levels may bring those levels in resonance with the radiation field which is normally forbidden by selection rules. Further, parity of the these states may significantly improve the emission process. The external electric field results in the mixing of excited (short lifetime) and metastable states (long lifetime), thus reducing the lifetime of metastable (or near metastable) states. This may provide an effective channel for allowing transition from the metastable states. An application of electric field may result in the excitation of poorly excitable biomolecules. This excitation technique may find applications in single- and multi-photon fluorescence microscopy, bioimaging and optical devices.

  4. Theory of two-photon micromaser: competition among different transition processes

    Institute of Scientific and Technical Information of China (English)

    Sun Wei-Hui; Du Si-De; Chen Xiao-Shuang

    2006-01-01

    We have investigated the steady-state cavity-field properties of a single-mode two-photon micromaser when the atoms in a cascade three-level configuration are initially prepared in a mixture of the upper and intermediate states. The mean photon number, trapping state and sub-Poissonian effect are discussed with upper (intermediate)-state population changing from 1(0) to 0(1). These properties are very different from those in a pure two- or one-photon transition process, due to the competition among different transition processes. In particular, the trapping states of nonzero photons are discovered in this system under some conditions, which is contrary to the previous findings.

  5. Two-photon transitions driven by a combination of diode and femtosecond lasers

    CERN Document Server

    Moreno, Marco P; Felinto, Daniel; Vianna, Sandra S

    2012-01-01

    We report on the combined action of a cw diode laser and a train of ultrashort pulses when each of them drives one step of the 5S-5P-5D two-photon transition in rubidium vapor. The fluorescence from the 6P_{3/2} state is detected for a fixed repetition rate of the femtosecond laser while the cw-laser frequency is scanned over the rubidium D_{2} lines. This scheme allows for a velocity selective spectroscopy in a large spectral range including the 5D_{3/2} and 5D_{5/2} states. The results are well described in a simplified frequency domain picture, considering the interaction of each velocity group with the cw laser and a single mode of the frequency comb.

  6. Polarization dependence of the direct two photon transitions of 87Rb atoms by erbium: Fiber laser frequency comb

    Science.gov (United States)

    Dai, Shaoyang; Xia, Wei; Zhang, Yin; Zhao, Jianye; Zhou, Dawei; Wang, Qing; Yu, Qi; Li, Kunqian; Qi, Xianghui; Chen, Xuzong

    2016-11-01

    The femtosecond fiber-based optical frequency combs have been proved to be powerful tools for investigating the energy levels of atoms and molecules. In this paper, an Er-doped fiber femtosecond optical frequency comb has been implemented for studying the polarization dependence of 5S-5D two-photon transitions in thermal gas of atomic rubidium 87 using an entirely symmetrical optical configuration. By changing the polarization states of the counter-propagating light beams, the polarization dependence of direct two photon transition spectrum is demonstrated, and a dramatic variation (up to 5.5 times) of the two-photon transitions strength has been observed. The theory for the polarization dependence of two photon transition based on the second-order perturbation was established, which is in good agreement with the experimental results. The measurement results indicate that the polarization state manipulation with the existing frequency comb is used for femtosecond optical frequency comb based two photon transition spectroscopic purposes, which will improve the precision measurement of the absolute transition frequency and related applications.

  7. Nuclear two-photon decay in 0/sup +/ -> 0/sup +/ transitions

    Energy Technology Data Exchange (ETDEWEB)

    Kramp, J.; Habs, D.; Kroth, R.; Music, M.; Schirmer, J.; Schwalm, D.; Broude, C.

    1987-11-23

    The two-photon decay of the first excited 0/sup +/ state of /sup 16/O has been measured using the Heidelberg-Darmstadt crystal ball. A branching ratio of GAMMA/sub ..gamma gamma..//GAMMA/sub tot/ = (6.6+-0.5).10/sup -4/ was obtained. As in the cases of /sup 40/Ca and /sup 90/Zr previously reported by us, the 2..gamma.. decay of /sup 16/O proceeds via double E1 and M1 transitions of similar strength; the evidence is the observed interference term in the 2..gamma.. angular correlation. The ratio of the matrix elements ..cap alpha../sub E1//chi for /sup 16/O was restricted to the two inverse values (-6.2+-1.5) or (-0.16+-0.04). An interpretation of 2..gamma.. matrix elements observed for /sup 16/O, /sup 40/Ca and /sup 90/Zr in terms of the electric polarizabilities and magnetic susceptibility is given leading to a qualitative understanding of this decay mode.

  8. Two-photon absorption and spectroscopy of the lowest two-photon transition in small donor-acceptor-substituted organic molecules

    Science.gov (United States)

    Beels, Marten T.; Biaggio, Ivan; Reekie, Tristan; Chiu, Melanie; Diederich, François

    2015-04-01

    We determine the dispersion of the third-order polarizability of small donor-acceptor substituted organic molecules using wavelength-dependent degenerate four-wave mixing experiments in solutions with varying concentrations. We find that donor-acceptor-substituted molecules that are characterized by extremely efficient off-resonant nonlinearities also have a correspondingly high two-photon absorption cross section. The width and shape of the first two-photon resonance for these noncentrosymmetric molecules follows what is expected from their longest wavelength absorption peak, and the observed two-photon absorption cross sections are record high when compared to the available literature data, the size of the molecule, and the fundamental limit for two-photon absorption to the lowest excited state, which is essentially determined by the number of conjugated electrons and the excited-state energies. The two-photon absorption of the smallest molecule, which only has 16 electrons in its conjugated system, is one order of magnitude larger than for the molecule called AF-50, a reference molecule for two-photon absorption [O.-K. Kim et al., Chem. Mater. 12, 284 (2000), 10.1021/cm990662r].

  9. Partonic structure of neutral pseudoscalars via two photon transition form factors

    CERN Document Server

    Raya, Khepani; Bashir, Adnan; Chang, Lei; Roberts, Craig D

    2016-01-01

    The $\\gamma \\gamma^\\ast \\to \\eta_{c,b}$ transition form factors are computed using a continuum approach to the two valence-body bound-state problem in relativistic quantum field theory, and thereby unified with equivalent calculations of electromagnetic pion elastic and transition form factors. The resulting $\\gamma \\gamma^\\ast \\to \\eta_c$ form factor, $G_{\\eta_c}(Q^2)$, is consistent with available data: significantly, at accessible momentum transfers, $Q^2 G_{\\eta_c}(Q^2)$ lies well below its conformal limit. These observations confirm that the leading-twist parton distribution amplitudes (PDAs) of heavy-heavy bound-states are compressed relative to the conformal limit. A clear understanding of the distribution of valence-quarks within mesons thus emerges; a picture which connects Goldstone modes, built from the lightest-quarks in Nature, with systems containing the heaviest valence-quarks that can now be studied experimentally, and highlights basic facts about manifestations of mass within the Standard Mod...

  10. The controlled excitation of forbidden transitions in the two-photon spectrum of strontium by using collisions and electric fields

    Science.gov (United States)

    Philip, G.; Connerade, J.-P.

    2007-11-01

    We present experimental results involving controlled configuration mixing in two-photon spectroscopy of highly-excited states by exploiting a weak external electric field and collisions. The method has allowed new extensions to high members of the two-photon forbidden J = 3 odd-parity 5snf 1F 3 and the J = 0, even-parity 5sns 1S 0 Rydberg series of neutral strontium to be observed. We achieve resonant two-photon transverse excitation of a high density atomic jet by using a narrow bandwidth tunable dye laser in a heat pipe setup with sensitive ionization detection. Experimental term values are extended for the 5sns 1S 0 series up to n = 46. By suitable exploitation of the composition and pressure of the buffer gases in conjunction with the electric field strength in the excitation region and the exciting laser beam intensity we have also extended observations up to n = 44 for the 5snf 1F 3 series and up to n = 46 for the 5snp 1P 1 series. Our results demonstrate a novel and remarkably simple experimental method to access high Rydberg states to which transitions are forbidden from the ground state by parity and other selection rules.

  11. Two-photon exchange corrections to the 2p(1/2)-2s transition energy in Li-like high- Z ions

    Science.gov (United States)

    Yerokhin; Artemyev; Shabaev; Sysak; Zherebtsov; Soff

    2000-11-27

    A rigorous QED calculation of the two-photon exchange corrections to the 2p(1/2)- 2s transition energy in Li-like high- Z ions is presented. The contribution due to an exchange by more than two photons is evaluated within the Breit approximation. The resulting theoretical value of the 2p(1/2)- 2s transition energy in Li-like uranium is found to be 280.44(20) eV.

  12. Visualizing the Contributions of Virtual States to Two-Photon Absorption Cross Sections by Natural Transition Orbitals of Response Transition Density Matrices.

    Science.gov (United States)

    Nanda, Kaushik D; Krylov, Anna I

    2017-07-20

    Observables such as two-photon absorption cross sections cannot be computed from the wave functions of initial and final states alone because of their nonlinear nature. Rather, they depend on the entire manifold of the excited states, which follows from the familiar sum-over-states expressions of second- and higher-order properties. Consequently, the interpretation of the computed nonlinear optical properties in terms of molecular orbitals is not straightforward and usually relies on approximate few-states models. Here, we show that the two-photon absorption (2PA) transitions can be visualized using response one-particle transition density matrices, which are defined as transition density matrices between the zero-order and first-order perturbed states. We also extend the concept of natural transition orbitals to 2PA transitions. We illustrate the utility of this new tool, which provides a rigorous black box alternative to traditional qualitative few-states analysis, by considering 2PA transitions in ethylene, trans-stilbene, and para-nitroaniline.

  13. The influence of atomic coherence and dipole–dipole interaction on entanglement of two qubits with nondegenerate two-photon transitions

    Indian Academy of Sciences (India)

    E K Bashkirov; M S Mastyugin

    2015-01-01

    Considering two artificial identical atoms interacting with two-mode thermal field through non-degenerate two-photon transitions, this paper studies the influence of atomic coherence and dipole–dipole interaction on the entanglement of two qubits. It is found that the entanglement is greatly enhanced by these mechanisms.

  14. Higgs Decay to Two Photons

    OpenAIRE

    Marciano, William J.; Zhang, Cen; Willenbrock, Scott

    2011-01-01

    The amplitude for Higgs decay to two photons is calculated in renormalizable and unitary gauges using dimensional regularization at intermediate steps. The result is finite, gauge independent, and in agreement with previously published results. The large Higgs mass limit is examined using the Goldstone-boson equivalence theorem as a check on the use of dimensional regularization and to explain the absence of decoupling.

  15. Transition Distribution Amplitudes for gamma* gamma collisions

    CERN Document Server

    Lansberg, J P; Szymanowski, L

    2008-01-01

    We study the exclusive production of pi-pi and rho-pi in hard gamma* gamma scattering in the forward kinematical region where the virtuality of one photon provides us with a hard scale in the process. The newly introduced concept of Transition Distribution Amplitudes (TDA) is used to perform a QCD calculation of these reactions thanks to two simple models for TDAs. The sizable cross sections for rho-pi and pi-pi production may be tested at intense electron-positron colliders such as CLEO and B factories (Belle and BaBar).

  16. Exact steady-state of a Kerr resonator with one- and two-photon driving-dissipation: controllable Wigner-function multimodality and dissipative phase transitions

    CERN Document Server

    Bartolo, Nicola; Casteels, Wim; Ciuti, Cristiano

    2016-01-01

    We present exact results for the steady-state density matrix of a general class of driven-dissipative systems consisting of a nonlinear Kerr resonator in the presence of both coherent (one-photon) and parametric (two-photon) driving and dissipation. Thanks to the analytical solution, obtained via the complex P-representation formalism, we are able to explore any regime, including photon blockade, multi-photon resonant effects, and a mesoscopic regime with large photon density and quantum correlations. We show how the interplay between one- and two-photon driving provides a way to control the multi-modality of the Wigner function in regimes where the semiclassical theory exhibits multistability. We also study the emergence of dissipative phase transitions in the thermodynamic limit of large photon numbers.

  17. Two-photon physics

    Energy Technology Data Exchange (ETDEWEB)

    Bardeen, W.A.

    1981-10-01

    A new experimental frontier has recently been opened to the study of two photon processes. The first results of many aspects of these reactions are being presented at this conference. In contrast, the theoretical development of research ito two photon processes has a much longer history. This talk reviews the many different theoretical ideas which provide a detailed framework for our understanding of two photon processes.

  18. Accessing the $\\rm 5S_{1/2} \\rightarrow 5D_{5/2}$ two-photon transition in Rb using a diode laser system

    CERN Document Server

    Rathod, Ketan D

    2015-01-01

    We report observation of the $\\rm 5S_{1/2} \\rightarrow 5D_{5/2}$ two-photon transition in Rb vapor at 778 nm, using an external cavity diode laser system and a heated vapor cell. The spectra in the two isotopes show well-resolved hyperfine transitions. The peaks are Doppler free, and have a Lorentzian lineshape with a typical linewidth of 2.2 MHz. This linewidth is larger than the natural linewidth of 300 kHz, but is still 5--10 times smaller than the linewidth for single-photon transitions in the D$_2$ line. Since the absolute frequency of this transition is measured with 8 kHz precision, it can form a better secondary reference in the optical regime compared to the D$_2$ line.

  19. Atomic frequency reference at 1033 nm for ytterbium (Yb)-doped fiber lasers and applications exploiting a rubidium (Rb) 5S_1/2 to 4D_5/2 one-colour two-photon transition

    Science.gov (United States)

    Roy, Ritayan; Condylis, Paul C.; Johnathan, Yik Jinen; Hessmo, Björn

    2017-04-01

    We demonstrate a two-photon transition of rubidium (Rb) atoms from the ground state (5$S_{1/2}$) to the excited state (4$D_{5/2}$), using a home-built ytterbium (Yb)-doped fiber amplifier at 1033 nm. This is the first demonstration of an atomic frequency reference at 1033 nm as well as of a one-colour two-photon transition for the above energy levels. A simple optical setup is presented for the two-photon transition fluorescence spectroscopy, which is useful for frequency stabilization for a broad class of lasers. This spectroscopy has potential applications in the fiber laser industry as a frequency reference, particularly for the Yb-doped fiber lasers. This two-photon transition also has applications in atomic physics as a background- free high- resolution atom detection and for quantum communication, which is outlined in this article.

  20. Observation of Distinct Two-Photon Transition Channels in CdTe Quantum Dots in a Regime of Very Strong Confinement

    Directory of Open Access Journals (Sweden)

    Marcelo Gonçalves Vivas

    2017-03-01

    Full Text Available We report here on the direct observation of distinct two-photon transition channels in glutathione-capped (GSH CdTe quantum dots (QDs in a very strong confinement regime. CdTe-GSH QDs with different average diameters (2.5, 3.0, and 3.3 nm were synthesized through the one-pot method and their two-photon absorption (2PA spectrum determined by a femtosecond wavelength-tunable Z-scan. Our results show that the two lower-energy one-photon-allowed excitonic transitions, 1S3/2(h → 1S(e and 2S3/2(h → 1S(e, are also accessed via 2PA. These results were ascribed to the relaxation of the parity selection rules due to the noncentrosymmetric structure of the CdTe QDs (zinc-blended structure, whose magnitude are determined by surface defects and structural irregularities present in CdTe-GSH QDs, in the strong confinement regime.

  1. Phase Effects in Two-Photon Free-Free Transitions in a Bichromatic Field of Frequencies $\\omega$ and $3\\omega$

    CERN Document Server

    Cionga, Aurelia

    2013-01-01

    The effect of the relative phase between the components of a bichromatic field of frequencies $\\omega$ and $3\\omega $ is discussed in the case of free-free transitions in laser-assisted electron-hydrogen scattering. For fast projectile and low field intensities, the role of target dressing is pointed out.

  2. Two-photon cryomicroscope

    Science.gov (United States)

    Breunig, H. G.; Köhler, C.; König, K.

    2012-03-01

    We report on a new two-photon cryomicroscope which consist of a compact laser-scanning microscope combined with a motorized heating and freezing stage. Samples can be cooled down to -196 °C (77 K) and heated up to 600 °C (873 K) with adjustable heating/freezing rates between 0.01 K / min and 150 K / min. Two-photon imaging is realized by near infrared femtosecond-laser pulse excitation. The abilities of the two-photon cryomicroscope are illustrated in several measurements: imaging of fluorescent microspheres inside a piece of ice illustrates the feasibility of deep-microscopic imaging inside frozen sample. The temperature-dependent structural integrity of collagen is monitored by detection of second harmonic generation signals from porcine cornea. The measurements reveal also the dependence of the collagendenaturation temperature on hydration state of the cornea collagen. Furthermore, the potential of the two-photon cryomicroscope for optimization of freezing and thawing procedures as well as to evaluate the viability of frozen cells and tissue is discussed.

  3. Nonclassical effects of a two-level spin system interacting with a two-mode cavity field via two-photon transition.

    Science.gov (United States)

    Grinberg, Horacio

    2008-12-18

    The interaction of a two-level cyclic XY n-spin model with a two-mode cavity field involving two-photon transitions is investigated through a generalized Jaynes-Cummings model in the rotating-wave approximation. The two-photon interacting Hamiltonian becomes from the replacement of each single-mode field in the one-photon interacting Hamiltonian with the second-harmonic generation. It was assumed that initially the correlated field modes are in disentangled coherent states having the same photon distribution and that the spin system is in an excited state. At any time t > 0, the spin system and the field are in an entangled state, in this case, via a unitary time evolution operator. Thus, the spontaneous decay of a spin level was treated by considering the interaction of the two-level spin system with the modes of the universe in the vacuum state. The different cases of interest, characterized in terms of a detuning parameter for each mode, which emerge from nonvanishing commutation relations, were analytically implemented and numerically discussed for various values of the initial mean photon number and spin-photon coupling constants. Photon distribution, time evolution of the spin population inversion, as well as the statistical properties of the field leading to the possible production of nonclassical states, such as antibunched light, violations of the Cauchy-Schwartz inequality, and second- and fourth-order squeezing, are examined. The case of zero detuning of both modes was treated in terms of a linearization of the expansion of the time evolution operator, while in other three cases, the computations were conducted via second- and third-order Dyson perturbation expansion of the time evolution operator matrix elements for the excited and ground states of the spin system, respectively.

  4. Two-Photon Physics in Hadronic Processes

    Energy Technology Data Exchange (ETDEWEB)

    Carl Carlson; Marc Vanderhaeghen

    2007-11-01

    Two-photon exchange contributions to elastic electron-scattering are reviewed. The apparent discrepancy in the extraction of elastic nucleon form factors between unpolarized Rosenbluth and polarization transfer experiments is discussed, as well as the understanding of this puzzle in terms of two-photon exchange corrections. Calculations of such corrections both within partonic and hadronic frameworks are reviewed. In view of recent spin-dependent electron scattering data, the relation of the two-photon exchange process to the hyperfine splitting in hydrogen is critically examined. The imaginary part of the two-photon exchange amplitude as can be accessed from the beam normal spin asymmetry in elastic electron-nucleon scattering is reviewed. Further extensions and open issues in this field are outlined.

  5. Sideband-Induced Two-Photon Transparency

    Institute of Scientific and Technical Information of China (English)

    CHENG Guang-Ling; HU Xiang-Ming

    2006-01-01

    @@ We show that it is possible to use a single sideband to induce two-photon transparency in a three-level cascade medium. The medium simultaneously absorbs two photons as a one-step process when the middle level is far off one-photon resonance. A resonant sideband coupling on the upper transition and the two-photon one-step process drive the medium into a trapped state, and the dominant component is the ground state. Thus almost all population is trapped in the ground state and the two-photon absorption is dramatically suppressed. We present a numerical calculation for arbitrary values of the atomic and field parameters and also provide an analytic description for the required conditions.

  6. Convergence of transition amplitudes obtained with the Schwinger variational principle

    CERN Document Server

    Rodríguez, V D

    2016-01-01

    An exactly solvable time-dependent quantum mechanical problem is employed to study the convergence properties of transition amplitudes calculated by using the Schwinger variational principle. A detailed comparison between the amplitudes approximated by the perturbative series and by their associated Schwinger variational principles is performed. The much better performance obtained by the variational principle is documented through different case studies. For a given order of the Schwinger principle, it is observed that the transition amplitudes do not converge to the exact one for large perturbations. The latter is true even though large combinations of unperturbed states with constant coefficients are taken as trial wave functions. As a matter of fact, it is shown that the improvement of the method comes from using better trial wave functions and increasing the order of the Schwinger principle employed.

  7. Baryon-to-meson transition distribution amplitudes: formalism and models

    CERN Document Server

    Pire, B; Szymanowski, L

    2016-01-01

    In specific kinematics, hard exclusive amplitudes may be factorized into a short distance dominated part computable in a perturbative way on the one hand, and universal, confinement related hadronic matrix elements on the other hand. The extension of this description to processes such as backward meson electroproduction and forward meson production in antiproton-nucleon scattering leads to define new hadronic matrix elements of three quark operators on the light cone, the nucleon-to-meson transition distribution amplitudes, which shed a new light on the nucleon structure.

  8. Baryon-to-Meson Transition Distribution Amplitudes: Formalism and Models

    Science.gov (United States)

    Pire, B.; Semenov-Tian-Shansky, K.; Szymanowski, L.

    2017-03-01

    In specific kinematics, hard exclusive amplitudes may be factorized into a short distance dominated part computable in a perturbative way on the one hand, and universal, confinement related hadronic matrix elements on the other hand. The extension of this description to processes such as backward meson electroproduction and forward meson production in antiproton-nucleon scattering leads to define new hadronic matrix elements of three quark operators on the light cone, the nucleon-to-meson transition distribution amplitudes, which shed a new light on the nucleon structure.

  9. Baryon to meson transition distribution amplitudes and their spectral representation

    CERN Document Server

    Pire, Bernard; Szymanowski, Lech

    2011-01-01

    We consider the problem of construction of a spectral representation for nucleon to meson transition distribution amplitudes (TDAs), non-diagonal matrix elements of nonlocal three quark light-cone operators between a nucleon and a meson states. We introduce the notion of quadruple distributions and generalize Radyshkin's factorized Ansatz for this issue. Modelling of baryon to meson TDAs in the complete domain of their definition opens the way to quantitative estimates of cross-sections for various hard exclusive reactions.

  10. 中心对称双光子低振幅亮屏蔽孤子的时间特性%Temporal behavior of the low-amplitude bright spatial soliton in two-photon centrosymmetric photorefractive media

    Institute of Scientific and Technical Information of China (English)

    吉选芒; 王金来; 姜其畅; 刘劲松

    2011-01-01

    To study the temporal properties of the low-amplitude bright spatial solitons in biased two-photon centrosymmetric photorefractive crystals,we present the expressions of the time-dependent spatial charge field and the equation of the spatial profile for the bright solitons as time evolve.The numerical results show that solitons width decreases monotonically to a minimum value toward steady state with the increasing of time.The higher the ratio of soliton peak intensity to the dark irradiation intensity,the narrower the width of bright solitons under within propagation time.The input beam can evolve the steady spatial solitons under different time.The results are benefit for improving the theory of spatial photorefractive solitons.%为了得到中心对称双光子光折变晶体中低振幅亮屏蔽孤子的时间特性的结果,推导出了晶体中空间电荷场的时间特性,得到了亮孤子的归一化空间包络随时间变化的方程.采用数值分析的方法对亮孤子的归一化空间包络及其在晶体中的时间演化特性进行了理论分析.结果表明:孤子的空间包络宽度随时间的演化单调递减一个最小值直至稳态孤子的形成;在相同的演化时间下,孤子的半峰全宽随着孤子峰值强度和暗辐射比值的增大而变小.在不同的时刻,入射光束都可在中心对称双光子光折变晶体中演化成空间孤子.所得结果对完善光折变空间孤子的理论有十分重要的意义.

  11. Two-photon excitation of the 2Π(4p)-X2Π(3p) transition of AlAr

    Science.gov (United States)

    Mascaritolo, Kyle J.; Antonov, Ivan O.; Heaven, Michael C.

    2014-03-01

    The 2Π(4p)-X2Π(3p) band system of AlAr has been observed using two-photon excitation. The spectrum consists of a short progression of doublet bands, with spin-orbit intervals that are close to that of Al(4p). Potential energy curve fitting yielded a bond dissociation energy for 2Π(4p) of De = 495(5) cm-1 and an approximate bond length of Re = 3.33(4) Å.

  12. Two photon physics. Personal recollection

    CERN Document Server

    Ginzburg, Ilya F

    2015-01-01

    The term two--photon processes is used for the reactions in which some system of particles is produced in collision of two photons, either real or virtual. In the study of these processes our main goal was to suggest approach, allowing to extract from the data information on proper two--photon process separating it from mechanism which responsible for the production of photons. Here I present my view for history of two--photon physics. I don't try to give complete review, concentrating mainly on works of our team (which cover essential part of the topic) and some colleagues. My citation is strongly incomplete. I cite here only papers which were essential in our understanding of the problems. The choice of presented details is the result of my discussions with Gleb Kotkin and Valery Serbo. 1. Prehistory. 2. Two photon processes at e^+e^- colliders. 3. Photon colliders. 4. Notes on physical program.

  13. Two-photon physics

    Energy Technology Data Exchange (ETDEWEB)

    Mark Vanderhaeghen

    2005-10-22

    It is reviewed how Compton scattering sum rules relate low-energy nucleon structure quantities to the nucleon excitation spectrum. In particular, the GDH sum rule and recently proposed extensions of it will be discussed. These extensions are sometimes more calculationally robust, which may be an advantage when estimating the chiral extrapolations of lattice QCD results, such as for anomalous magnetic moments. Subsequently, new developments in our description of the nucleon excitation spectrum will be discussed, in particular a recently developed chiral effective field theory framework for the {Delta}(1232)-resonance region. Within this framework, we discuss results on N and {Delta} masses, the {gamma} N {Delta} transition and the {Delta} magnetic dipole moment.

  14. Two-photon cooling of magnesium atoms

    DEFF Research Database (Denmark)

    Malossi, N.; Damkjær, S.; Hansen, P. L.

    2005-01-01

    A two-photon mechanism for cooling atoms below the Doppler temperature is analyzed. We consider the magnesium ladder system (3s2)S01¿(3s3p)P11 at 285.2nm followed by the (3s3p)P11¿(3s3d)D21 transition at 880.7nm . For the ladder system quantum coherence effects may become important. Combined...... with the basic two-level Doppler cooling process this allows for reduction of the atomic sample temperature by more than a factor of 10 over a broad frequency range. First experimental evidence for the two-photon cooling process is presented and compared to model calculations. Agreement between theory...... and experiment is excellent. In addition, by properly choosing the Rabi frequencies of the two optical transitions a velocity independent atomic dark state is observed....

  15. Two-photon cooling of magnesium atoms

    DEFF Research Database (Denmark)

    Malossi, N.; Damkjær, S.; Hansen, P. L.;

    2005-01-01

    A two-photon mechanism for cooling atoms below the Doppler temperature is analyzed. We consider the magnesium ladder system (3s2)S01¿(3s3p)P11 at 285.2nm followed by the (3s3p)P11¿(3s3d)D21 transition at 880.7nm . For the ladder system quantum coherence effects may become important. Combined...

  16. BRIEF COMMUNICATIONS: Parametric noise in a nonlinear frequency up-converter of infrared signals by two-photon pumping of 3S-3D and 3S-5S transitions in sodium vapor

    Science.gov (United States)

    Galaĭchuk, Yu A.; Kudryashov, V. A.; Strizhevskiĭ, V. L.; Fontaniĭ, V. A.; Yashkir, Yu N.

    1985-07-01

    A systematic analysis was made of the spectral characteristics of resonance four-photon parametric conversion of infrared radiation as a result of two-photon resonance pumping of the 3S-3D and 3S-5S transitions in sodium and the influence of these characteristics on the threshold sensitivity of a parametric conversion detector was investigated. An experimental study was made of the characteristics of the noise radiation generated as a result of hyperparametric scattering. The results obtained can be used to select the optimal parameters of high-sensitivity detectors of weak infrared signals by parametric conversion in alkali metal vapors.

  17. Two-Photon Collective Atomic Recoil Lasing

    Directory of Open Access Journals (Sweden)

    James A. McKelvie

    2015-11-01

    Full Text Available We present a theoretical study of the interaction between light and a cold gasof three-level, ladder configuration atoms close to two-photon resonance. In particular, weinvestigate the existence of collective atomic recoil lasing (CARL instabilities in differentregimes of internal atomic excitation and compare to previous studies of the CARL instabilityinvolving two-level atoms. In the case of two-level atoms, the CARL instability is quenchedat high pump rates with significant atomic excitation by saturation of the (one-photoncoherence, which produces the optical forces responsible for the instability and rapid heatingdue to high spontaneous emission rates. We show that in the two-photon CARL schemestudied here involving three-level atoms, CARL instabilities can survive at high pump rateswhen the atoms have significant excitation, due to the contributions to the optical forces frommultiple coherences and the reduction of spontaneous emission due to transitions betweenthe populated states being dipole forbidden. This two-photon CARL scheme may form thebasis of methods to increase the effective nonlinear optical response of cold atomic gases.

  18. The twistorial structure of loop-gravity transition amplitudes

    CERN Document Server

    Speziale, Simone

    2012-01-01

    The spin foam formalism provides transition amplitudes for loop quantum gravity. Important aspects of the dynamics are understood, but many open questions are pressing on. In this paper we address some of them using a twistorial description, which brings new light on both classical and quantum aspects of the theory. At the classical level, we clarify the covariant properties of the discrete geometries involved, and the role of the simplicity constraints in leading to SU(2) Ashtekar-Barbero variables. We identify areas and Lorentzian dihedral angles in twistor space, and show that they form a canonical pair. The primary simplicity constraints are solved by simple twistors, parametrized by SU(2) spinors and the dihedral angles. We construct an SU(2) holonomy and prove it to correspond to the Ashtekar-Barbero connection. We argue that the role of secondary constraints is to provide a non trivial embedding of the cotangent bundle of SU(2) in the space of simple twistors. At the quantum level, a Schroedinger repre...

  19. From 3-geometry transition amplitudes to graviton states

    CERN Document Server

    Mattei, F; Speziale, S; Testa, M; Mattei, Federico; Rovelli, Carlo; Speziale, Simone; Testa, Massimo

    2006-01-01

    In various background independent approaches, quantum gravity is defined in terms of a field propagation kernel: a sum over paths interpreted as a transition amplitude between 3-geometries, expected to project quantum states of the geometry on the solutions of the Wheeler-DeWitt equation. We study the relation between this formalism and conventional quantum field theory methods. We consider the propagation kernel of 4d Lorentzian general relativity in the temporal gauge, defined by a conventional formal Feynman path integral, gauge fixed a' la Fadeev--Popov. If space is compact, this turns out to depend only on the initial and final 3--geometries, while in the asymptotically flat case it depends also on the asymptotic proper time. We compute the explicit form of this kernel at first order around flat space, and show that it projects on the solutions of all quantum constraints, including the Wheeler-DeWitt equation, and yields the correct vacuum and n-graviton states. We also illustrate how the Newtonian inter...

  20. From 3-geometry transition amplitudes to graviton states

    Science.gov (United States)

    Mattei, Federico; Rovelli, Carlo; Speziale, Simone; Testa, Massimo

    2006-04-01

    In various background independent approaches, quantum gravity is defined in terms of a field propagation kernel: a sum over paths interpreted as a transition amplitude between 3-geometries, expected to project quantum states of the geometry on the solutions of the Wheeler-deWitt equation. We study the relation between this formalism and conventional quantum field theory methods. We consider the propagation kernel of 4d Lorentzian general relativity in the temporal gauge, defined by a conventional formal Feynman path integral, gauge fixed à la Faddeev-Popov. If space is compact, this turns out to depend only on the initial and final 3-geometries, while in the asymptotically flat case it depends also on the asymptotic proper time. We compute the explicit form of this kernel at first order around flat space, and show that it projects on the solutions of all quantum constraints, including the Wheeler-DeWitt equation, and yields the correct vacuum and n-graviton states. We also illustrate how the Newtonian interaction is coded into the propagation kernel, a key open issue in the spinfoam approach.

  1. Two-photon processes in highly charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Jahrsetz, Thorsten

    2015-03-05

    Two-photon processes are atomic processes in which an atom interacts simultaneously with two photons. Such processes describe a wide range of phenomena, such as two-photon decay and elastic or inelastic scattering of photons. In recent years two-photon processes involving highly charged heavy ions have become an active area of research. Such studies do not only consider the total transition or scattering rates but also their angular and polarization dependence. To support such examinations in this thesis I present a theoretical framework to describe these properties in all two-photon processes with bound initial and final states and involving heavy H-like or He-like ions. I demonstrate how this framework can be used in some detailed studies of different two-photon processes. Specifically a detailed analysis of two-photon decay of H-like and He-like ions in strong external electromagnetic fields shows the importance of considering the effect of such fields for the physics of such systems. Furthermore I studied the elastic Rayleigh as well as inelastic Raman scattering by heavy H-like ions. I found a number of previously unobserved phenomena in the angular and polarization dependence of the scattering cross-sections that do not only allow to study interesting details of the electronic structure of the ion but might also be useful for the measurement of weak physical effects in such systems.

  2. Amplitude analysis without ambiguity in the transition NN {yields} {Delta}N; Analyse en amplitudes sans ambiguite de la transition NN {yields} {Delta}N

    Energy Technology Data Exchange (ETDEWEB)

    Auger, J.P. [Orleans Univ., 45 Orleans (France); Lazard, C. [Theoretical Physics Division, Inst. de Physique Nucleaire, Paris-11 Univ., 91 - Orsay (France)

    1999-10-01

    A three step method is developed for determining without ambiguity the NN {yields} {Delta}N transition amplitudes. The purpose of the study is to select a set of observables, which determines, first, the 16 values of the amplitudes, secondly, the 15 independent relative phases, and thirdly, some dependent relative phases for resolving the remaining ambiguities. For determining NN {yields} (N{pi})N experiments needed to such an amplitude analysis, the decay distribution is expressed in the density matrix formalism. For particular {Delta} - production angles, an unambiguously amplitude analysis is performed with experiments involving polarized beam and target, only, avoiding the detection of the polarization of the outgoing nucleons. (authors) 2 refs.

  3. Transition to Amplitude Death in Coupled System with Small Number of Nonlinear Oscillators

    Institute of Scientific and Technical Information of China (English)

    CHEN Hai-Ling; YANG Jun-Zhong

    2009-01-01

    In this work, we investigate the amplitude death in coupled system with small number of nonlinear oscillators. We show how the transitions to the partial and the complete amplitude deathes happen. We also show that the partial amplitude death can be found in globally coupled oscillators either.

  4. Two-Photon-Exchange Effects and $\\Delta(1232)$ Deformation

    CERN Document Server

    Zhou, Hai-Qing

    2016-01-01

    The two-photon-exchange (TPE) contribution in $ep\\rightarrow ep\\pi ^0$ with $W=M_{\\Delta}$ and small $Q^2$ is calculated and its corrections to the ratios of electromagnetic transition form factors $R_{EM} = E_{1+}^{(3/2)}/M_{1+}^{(3/2)} $ and $R_{SM} = S_{1+}^{(3/2)}/M_{1+}^{(3/2)}$, are analysed. A simple hadronic model is used to estimate the TPE amplitude. Two phenomenological models, MAID2007 and SAID, are used to approximate the full $ep\\rightarrow ep\\pi ^0$ cross sections which contain both the TPE and the one-photon-exchange (OPE) contributions. The genuine the OPE amplitude is then extracted from an integral equation by iteration. We find that the TPE contribution is not sensitive to whether MAID or SAID is used as input in the region with $Q^2<2$ GeV$^2$. It gives small correction to $R_{EM}$ while for $R_{SM}$, the correction is about -10\\% at small $\\epsilon$ and about $1\\%$ at large $\\epsilon$ for $Q^2\\approx2.5$ GeV$^2$. The large correction from TPE at small $\\epsilon$ must be included in th...

  5. Two-Photon Flow Cytometry

    Science.gov (United States)

    Zhog, Cheng Frank; Ye, Jing Yong; Norris, Theodore B.; Myc, Andrzej; Cao, Zhengyl; Bielinska, Anna; Thomas, Thommey; Baker, James R., Jr.

    2004-01-01

    Flow cytometry is a powerful technique for obtaining quantitative information from fluorescence in cells. Quantitation is achieved by assuring a high degree of uniformity in the optical excitation and detection, generally by using a highly controlled flow such as is obtained via hydrodynamic focusing. In this work, we demonstrate a two-beam, two- channel detection and two-photon excitation flow cytometry (T(sup 3)FC) system that enables multi-dye analysis to be performed very simply, with greatly relaxed requirements on the fluid flow. Two-photon excitation using a femtosecond near-infrared (NIR) laser has the advantages that it enables simultaneous excitation of multiple dyes and achieves very high signal-to-noise ratio through simplified filtering and fluorescence background reduction. By matching the excitation volume to the size of a cell, single-cell detection is ensured. Labeling of cells by targeted nanoparticles with multiple fluorophores enables normalization of the fluorescence signal and thus ratiometric measurements under nonuniform excitation. Quantitative size measurements can also be done even under conditions of nonuniform flow via a two-beam layout. This innovative detection scheme not only considerably simplifies the fluid flow system and the excitation and collection optics, it opens the way to quantitative cytometry in simple and compact microfluidics systems, or in vivo. Real-time detection of fluorescent microbeads in the vasculature of mouse ear demonstrates the ability to do flow cytometry in vivo. The conditions required to perform quantitative in vivo cytometry on labeled cells will be presented.

  6. Measurement of the I =1 /2 K π S -wave amplitude from Dalitz plot analyses of ηc→K K ¯π in two-photon interactions

    Science.gov (United States)

    Lees, J. P.; Poireau, V.; Tisserand, V.; Grauges, E.; Palano, A.; Eigen, G.; Brown, D. N.; Kolomensky, Yu. G.; Koch, H.; Schroeder, T.; Hearty, C.; Mattison, T. S.; McKenna, J. A.; So, R. Y.; Blinov, V. E.; Buzykaev, A. R.; Druzhinin, V. P.; Golubev, V. B.; Kravchenko, E. A.; Onuchin, A. P.; Serednyakov, S. I.; Skovpen, Yu. I.; Solodov, E. P.; Todyshev, K. Yu.; Lankford, A. J.; Gary, J. W.; Long, O.; Eisner, A. M.; Lockman, W. S.; Panduro Vazquez, W.; Chao, D. S.; Cheng, C. H.; Echenard, B.; Flood, K. T.; Hitlin, D. G.; Kim, J.; Miyashita, T. S.; Ongmongkolkul, P.; Porter, F. C.; Röhrken, M.; Huard, Z.; Meadows, B. T.; Pushpawela, B. G.; Sokoloff, M. D.; Sun, L.; Smith, J. G.; Wagner, S. R.; Bernard, D.; Verderi, M.; Bettoni, D.; Bozzi, C.; Calabrese, R.; Cibinetto, G.; Fioravanti, E.; Garzia, I.; Luppi, E.; Santoro, V.; Calcaterra, A.; de Sangro, R.; Finocchiaro, G.; Martellotti, S.; Patteri, P.; Peruzzi, I. M.; Piccolo, M.; Zallo, A.; Passaggio, S.; Patrignani, C.; Bhuyan, B.; Mallik, U.; Chen, C.; Cochran, J.; Prell, S.; Ahmed, H.; Pennington, M. R.; Gritsan, A. V.; Arnaud, N.; Davier, M.; Le Diberder, F.; Lutz, A. M.; Wormser, G.; Lange, D. J.; Wright, D. M.; Coleman, J. P.; Gabathuler, E.; Hutchcroft, D. E.; Payne, D. J.; Touramanis, C.; Bevan, A. J.; Di Lodovico, F.; Sacco, R.; Cowan, G.; Banerjee, Sw.; Brown, D. N.; Davis, C. L.; Denig, A. G.; Fritsch, M.; Gradl, W.; Griessinger, K.; Hafner, A.; Schubert, K. R.; Barlow, R. J.; Lafferty, G. D.; Cenci, R.; Jawahery, A.; Roberts, D. A.; Cowan, R.; Cheaib, R.; Robertson, S. H.; Dey, B.; Neri, N.; Palombo, F.; Cremaldi, L.; Godang, R.; Summers, D. J.; Taras, P.; De Nardo, G.; Sciacca, C.; Raven, G.; Jessop, C. P.; LoSecco, J. M.; Honscheid, K.; Kass, R.; Gaz, A.; Margoni, M.; Posocco, M.; Rotondo, M.; Simi, G.; Simonetto, F.; Stroili, R.; Akar, S.; Ben-Haim, E.; Bomben, M.; Bonneaud, G. R.; Calderini, G.; Chauveau, J.; Marchiori, G.; Ocariz, J.; Biasini, M.; Manoni, E.; Rossi, A.; Batignani, G.; Bettarini, S.; Carpinelli, M.; Casarosa, G.; Chrzaszcz, M.; Forti, F.; Giorgi, M. A.; Lusiani, A.; Oberhof, B.; Paoloni, E.; Rama, M.; Rizzo, G.; Walsh, J. J.; Smith, A. J. S.; Anulli, F.; Faccini, R.; Ferrarotto, F.; Ferroni, F.; Pilloni, A.; Piredda, G.; Bünger, C.; Dittrich, S.; Grünberg, O.; Heß, M.; Leddig, T.; Voß, C.; Waldi, R.; Adye, T.; Wilson, F. F.; Emery, S.; Hamel de Monchenault, G.; Vasseur, G.; Aston, D.; Cartaro, C.; Convery, M. R.; Dorfan, J.; Dunwoodie, W.; Ebert, M.; Field, R. C.; Fulsom, B. G.; Graham, M. T.; Hast, C.; Innes, W. R.; Kim, P.; Leith, D. W. G. S.; Luitz, S.; Luth, V.; MacFarlane, D. B.; Muller, D. R.; Neal, H.; Ratcliff, B. N.; Roodman, A.; Sullivan, M. K.; Va'vra, J.; Wisniewski, W. J.; Purohit, M. V.; Wilson, J. R.; Randle-Conde, A.; Sekula, S. J.; Bellis, M.; Burchat, P. R.; Puccio, E. M. T.; Alam, M. S.; Ernst, J. A.; Gorodeisky, R.; Guttman, N.; Peimer, D. R.; Soffer, A.; Spanier, S. M.; Ritchie, J. L.; Schwitters, R. F.; Izen, J. M.; Lou, X. C.; Bianchi, F.; De Mori, F.; Filippi, A.; Gamba, D.; Lanceri, L.; Vitale, L.; Martinez-Vidal, F.; Oyanguren, A.; Albert, J.; Beaulieu, A.; Bernlochner, F. U.; King, G. J.; Kowalewski, R.; Lueck, T.; Nugent, I. M.; Roney, J. M.; Tasneem, N.; Gershon, T. J.; Harrison, P. F.; Latham, T. E.; Prepost, R.; Wu, S. L.; BaBar Collaboration

    2016-01-01

    We study the processes γ γ →KS0K±π∓ and γ γ →K+K-π0 using a data sample of 519 fb-1 recorded with the BABAR detector operating at the SLAC PEP-II asymmetric-energy e+e- collider at center-of-mass energies at and near the Υ (n S ) (n =2 , 3, 4) resonances. We observe ηc decays to both final states and perform Dalitz plot analyses using a model-independent partial wave analysis technique. This allows a model-independent measurement of the mass-dependence of the I =1 /2 K π S -wave amplitude and phase. A comparison between the present measurement and those from previous experiments indicates similar behavior for the phase up to a mass of 1.5 GeV /c2. In contrast, the amplitudes show very marked differences. The data require the presence of a new a0(1950 ) resonance with parameters m =1931 ±14 ±22 MeV /c2 and Γ =271 ±22 ±29 MeV .

  7. The variation of transition location in response to the variation of the amplitudes of initial disturbances

    Institute of Scientific and Technical Information of China (English)

    2010-01-01

    The transition location of a boundary layer depends on the amplitude and characteristic of initial disturbances. The larger the amplitude and the amplification rate of the initial disturbances are,the more upstream the transition location is. However,the environment surrounding the flying vehicle is variable,so the amplitude and characteristic of the disturbances triggered in the boundary layer through receptivity are also variable. In this paper,how the transition location varies in response to the variation of the initial disturbance amplitudes is studied by using direct numerical simulation. The results show that if the initial disturbance amplitudes become smaller,the transition location moves downstream correspondingly,but there is a time delay compared to the time of arrival of the disturbances with reduced amplitudes. Moreover,the speed of moving downstream is appreciably lower than the propagation speed of the disturbances. On the other hand,if the amplitudes of the initial disturbances recover their original value,the transition would immediately take place whenever the disturbances reach the former transition location,but the laminar flow between the new and old transition locations would not become turbulent immediately. Theoretical explanations are provided based on the transition mechanism found by our group.

  8. Two-photon approximation in the theory of the electron recombination in hydrogen

    OpenAIRE

    Solovyev, D.; Labzowsky, L.

    2010-01-01

    A rigorous QED theory of the multiphoton decay of excited states in hydrogen atom is presented. The "two-photon" approximation is formulated which is limited by the one-photon and two-photon transitions including cascades transitions with two-photon links. This may be helpful for the strict description of the recombination process in hydrogen atom and, in principle, for the history of the hydrogen recombination in the early Universe.

  9. (Un)determined finite regularization dependent quantum corrections: the Higgs decay into two photons and the two photon scattering examples

    CERN Document Server

    Cherchiglia, A L; Nemes, M C; Sampaio, Marcos

    2012-01-01

    We investigate the appearance of arbitrary, regularization dependent parameters introduced by divergent integrals in two a priori finite but superficially divergent amplitudes: the Higgs decay into two photons and the two photon scattering. We use a general parametrization of ultraviolet divergences which explicitates such ambiguities. Thus we separate in a consistent way using Implicit Regularization the divergent, finite and regularization dependent parts of the amplitudes which in turn are written as surface terms. We find that, although finite, these amplitudes are ambiguous before the imposition of physical conditions namely momentum routing invariance in the loops of Feynman diagrams. In the examples we study momentum routing invariance turns out to be equivalent to gauge invariance. We also discuss the results obtained by different regularizations and show how they can be reproduced within our framework allowing for a clear view on the origin of regularization ambiguities.

  10. Multichannel 1 → 2 transition amplitudes in a finite volume

    Energy Technology Data Exchange (ETDEWEB)

    Briceno, Raul A. [Thomas Jefferson National Accelerator Facility, Newport News, VA (United States); Hansen, Maxwell T. [Univ. of Washington, Seattle, WA (United States); Walker-Loud, Andre [Thomas Jefferson National Accelerator Facility, Newport News, VA (United States); College of William and Mary, Williamsburg, VA (United States)

    2015-02-03

    We perform a model-independent, non-perturbative investigation of two-point and three-point finite-volume correlation functions in the energy regime where two-particle states can go on-shell. We study three-point functions involving a single incoming particle and an outgoing two-particle state, relevant, for example, for studies of meson decays (e.g., B⁰ → K*l⁺l⁻) or meson photo production (e.g., πγ* → ππ). We observe that, while the spectrum solely depends upon the on-shell scattering amplitude, the correlation functions also depend upon off-shell amplitudes. The main result of this work is a non-perturbative generalization of the Lellouch-Luscher formula relating matrix elements of currents in finite and infinite spatial volumes. We extend that work by considering a theory with multiple, strongly-coupled channels and by accommodating external currents which inject arbitrary four-momentum as well as arbitrary angular-momentum. The result is exact up to exponentially suppressed corrections governed by the pion mass times the box size. We also apply our master equation to various examples, including two processes mentioned above as well as examples where the final state is an admixture of two open channels.

  11. Holographic Two-Photon Induced Photopolymerization

    Data.gov (United States)

    Federal Laboratory Consortium — Holographic two-photon-induced photopolymerization (HTPIP) offers distinct advantages over conventional one-photon-induced photopolymerization and current techniques...

  12. Precision two-photon spectroscopy of alkali elements

    Indian Academy of Sciences (India)

    P V Kiran Kumar; M V Suryanarayana

    2014-08-01

    In this paper, we have briefly reviewed the work on two-photon spectroscopy of alkali elements and its applications. The technique of Doppler-free two-photon spectroscopy is briefly summarized. A review of various techniques adopted for measuring absolute frequencies of the atomic transitions and precision measurements of isotope shifts and hyperfine structures (HFS) is presented. Some of the recent works on precision measurements of HFS constants of 6 ${}^2S_{1/2}$ level of ${}^{39}$K and ${}^{41}$K, 9 ${}^2S_{1/2}$ level and 7 ${}^2D_{3/2}$ level of 133Cs are also discussed.

  13. Approach to Perturbative QCD Results in Transition Amplitudes of Nucleon Negative-Parity Resonances

    Institute of Scientific and Technical Information of China (English)

    DONG Yu-Bing

    2004-01-01

    The scaling behaviors of the nucleon resonance transition amplitudes from perturbative QCD (PQCD) are utilized to parametrize the amplitudes of the first negative-parity nucleon resonance S11 (1535). Our analysis indicates that the constraints of the transition amplitude for the S11 resonance at the limit Q2 →∞ by QCD sum rule calculations are not applicable at a moderate Q2 range of 2.5 ~ 4 Ge V2 compared with the present available data if the contribution of S11 is dominant in the Q2 limit.

  14. Testing ultrafast two-photon spectral amplitudes via optical fibres.

    Science.gov (United States)

    Brida, G; Caricato, V; Chekhova, M V; Genovese, M; Gramegna, M; Iskhakov, T Sh

    2010-06-07

    We test two-dimensional TPSA of biphoton light emitted via ultrafast spontaneous parametric down-conversion (SPDC) using the effect of group-velocity dispersion in optical fibres. Further, we apply this technique to demonstrate the engineering of biphoton spectral properties by acting on the pump pulse shape.

  15. Diffusion-induced periodic transition between oscillatory modes in amplitude-modulated patterns

    Energy Technology Data Exchange (ETDEWEB)

    Tang, Xiaodong; He, Yuxiu; Wang, Shaorong; Gao, Qingyu, E-mail: gaoqy@cumt.edu.cn [College of Chemical Engineering, China University of Mining and Technology, Xuzhou 221008 (China); Epstein, Irving R., E-mail: epstein@brandeis.edu [Department of Chemistry and Volen Center for Complex Systems, MS 015, Brandeis University, Waltham, Massachusetts 02454-9110 (United States); Wang, Qun [School of Physics and Electronic Engineering, Jiangsu Normal University, Xuzhou 221116 (China)

    2014-06-15

    We study amplitude-modulated waves, e.g., wave packets in one dimension, overtarget spirals and superspirals in two dimensions, under mixed-mode oscillatory conditions in a three-variable reaction-diffusion model. New transition zones, not seen in the homogeneous system, are found, in which periodic transitions occur between local 1{sup N−1} and 1{sup N} oscillations. Amplitude-modulated complex patterns result from periodic transition between (N − 1)-armed and N-armed waves. Spatial recurrence rates provide a useful guide to the stability of these modulated patterns.

  16. Direct frequency comb two-photon laser cooling and trapping

    Science.gov (United States)

    Jayich, Andrew; Long, Xueping; Campbell, Wesley C.

    2016-05-01

    Generating and manipulating high energy photons for spectroscopy on electric dipole transitions of atoms and molecules with deeply bound valence electrons is difficult. Further, laser cooling of such species is even more challenging for lack of laser power. A possible solution is to drive two-photon transitions. This may alleviate the photon energy problem and open the door to cold, trapped samples of highly desirable species with tightly bound electrons. We perform a proof of principle experiment with rubidium by driving a two-photon transition with an optical frequency comb. We perform optical cooling and extend this technique to trapping, where we are able to make a magneto-optical trap in one dimension. This work is supported by the National Science Foundation CAREER program.

  17. Fano interference in two-photon transport

    Science.gov (United States)

    Xu, Shanshan; Fan, Shanhui

    2016-10-01

    We present a general input-output formalism for the few-photon transport in multiple waveguide channels coupled to a local cavity. Using this formalism, we study the effect of Fano interference in two-photon quantum transport. We show that the physics of Fano interference can manifest as an asymmetric spectral line shape in the frequency dependence of the two-photon correlation function. The two-photon fluorescence spectrum, on the other hand, does not exhibit the physics of Fano interference.

  18. Correlations of two photons at hadron colliders

    OpenAIRE

    Kozlov, G. A.

    2011-01-01

    We study the Bose-Einstein correlations of two photons and their coherent properties that can provide the information about the space-time structure of the emitting source through the Higgs-boson decays into two photons. We argue that such an investigation could probe the Higgs-boson mass. The model is rather sensitive to the temperature of the environment and to the external distortion effect in medium.

  19. Platinum Acetylide Two-Photon Chromophores (Preprint)

    Science.gov (United States)

    2007-04-01

    the higher energy range that lead to its photodegradation . Secondly, because there is a quadratic dependence of two-photon absorption (2PA) on the...to either an electron donating amino- fluorenyl or electron withdrawing benzothiazolyl-fluorene that are themselves known as two-photon absorbing dyes ...groups in place of phenyl groups have shown a doubling of the intrinsic cr2value at 740 nm.40,41In this paper we describe novel platinum dyes that

  20. Using the Single Quark Transition Model to predict nucleon resonance amplitudes

    CERN Document Server

    Ramalho, G

    2014-01-01

    We present predictions for the $\\gamma^\\ast N \\to N^\\ast$ helicity amplitudes, where $N^\\ast$ is a member of the $[70,1^-]$ supermultiplet. We combine the results from the single quark transition model for the helicity amplitudes with the results of the covariant spectator quark model for the $\\gamma^\\ast N \\to N^\\ast(1535)$ and $\\gamma^\\ast N \\to N^\\ast(1520)$ transitions. The theoretical estimations from the covariant spectator quark model are used to calculate three independent functions $A,B$, and $C$ of $Q^2$, where $Q^2=-q^2$ and $q$ is the momentum transfer. With the knowledge of the functions $A,B$, and $C$ we estimate the helicity amplitudes for the transitions $\\gamma^\\ast N \\to N^\\ast(1650)$, $\\gamma^\\ast N \\to N^\\ast(1700)$, $\\gamma^\\ast N \\to \\Delta(1620)$, and $\\gamma^\\ast N \\to \\Delta(1700)$. The analysis is restricted to reactions with proton targets. The predictions for the transition amplitudes are valid for $Q^2 > 2$ GeV$^2$.

  1. A new approach to dual-color two-photon microscopy with fluorescent proteins

    Directory of Open Access Journals (Sweden)

    Rebane Aleks

    2010-02-01

    Full Text Available Abstract Background Two-photon dual-color imaging of tissues and cells labeled with fluorescent proteins (FPs is challenging because most two-photon microscopes only provide one laser excitation wavelength at a time. At present, methods for two-photon dual-color imaging are limited due to the requirement of large differences in Stokes shifts between the FPs used and their low two-photon absorption (2PA efficiency. Results Here we present a new method of dual-color two-photon microscopy that uses the simultaneous excitation of the lowest-energy electronic transition of a blue fluorescent protein and a higher-energy electronic transition of a red fluorescent protein. Conclusion Our method does not require large differences in Stokes shifts and can be extended to a variety of FP pairs with larger 2PA efficiency and more optimal imaging properties.

  2. The two-photon exchange contribution to elastic electron-nucleon scattering at large momentum transfer

    Energy Technology Data Exchange (ETDEWEB)

    Andrei V. Afanasev; Stanley J. Brodsky; Carl E. Carlson; Yu-Chun Chen; Marc Vanderhaeghen

    2005-01-01

    We estimate the two-photon exchange contribution to elastic electron-proton scattering at large momentum transfer by using a quark-parton representation of virtual Compton scattering. We thus can relate the two-photon exchange amplitude to the generalized parton distributions which also enter in other wide angle scattering processes. We find that the interference of one- and two-photon exchange contribution is able to substantially resolve the difference between electric form factor measurements from Rosenbluth and polarization transfer experiments.

  3. The effects of dual-channel coupling on the transition from amplitude death to oscillation death

    Science.gov (United States)

    Chen, Jiangnan; Liu, Weiqing; Zhu, Yun; Xiao, Jinghua

    2016-07-01

    Oscillation quenching including amplitude death (AD) and oscillation death (OD) in addition to the transition processes between them have been hot topics in aspect of chaos control, physical and biological applications. The effects of dual-channel coupling on the AD and OD dynamics regimes, and their transition processes in coupled nonidentical oscillators are explored numerically and theoretically. Our results indicate that an additional repulsive coupling tends to shrink the AD domain while it enlarges the OD domain, however, an additional attractive coupling acts inversely. As a result, the transitions from AD to OD are replaced by transitions from oscillation state (OS) to AD or from OS to OD in the dual-channel coupled oscillators with different frequency mismatches. Our results are helpful to better understand the control of AD and OD and their transition processes.

  4. Medical prototyping using two photon polymerization

    Directory of Open Access Journals (Sweden)

    Roger J Narayan

    2010-12-01

    Full Text Available Two photon polymerization involves nearly simultaneous absorption of ultrashort laser pulses for selective curing of photosensitive material. This process has recently been used to create small-scale medical devices out of several classes of photosensitive materials, such as acrylate-based polymers, organically-modified ceramic materials, zirconium sol-gels, and titanium-containing hybrid materials. In this review, the use of two photon polymerization for fabrication of several types of small-scale medical devices, including microneedles, artificial tissues, microfluidic devices, pumps, sensors, and valves, from computer models is described. Necessary steps in the development of two photon polymerization as a commercially viable medical device manufacturing method are also considered.

  5. Two Photon Couplings of Hybrid Mesons

    CERN Document Server

    Page, P R

    1996-01-01

    A new formalism is developed for the two photon production of hybrid mesons via intermediate hadronic decays. In an adiabatic and non--relativistic context with spin 1 pair creation we obtain the first absolute estimates of unmixed hybrid production strengths to be small (0.03 - 3 eV) in relation to experimental meson widths (0.1 - 5 keV). Within this context, two photon collisions therefore strongly discriminate between hybrid and conventional meson wave function components at BaBar, Cleo II, LEP2 and LHC, filtering out non--gluonic components. Decay widths of unmixed hybrids are tiny. The formalism also induces conventional meson two photon widths roughly in agreement with experiment.

  6. Two-photon quantum interference in plasmonics: theory and applications.

    Science.gov (United States)

    Gupta, S Dutta; Agarwal, G S

    2014-01-15

    We report perfect two-photon quantum interference with near-unity visibility in a resonant tunneling plasmonic structure in folded Kretschmann geometry. This is despite absorption-induced loss of unitarity in plasmonic systems. The effect is traced to perfect destructive interference between the squares of amplitude reflection and transmission coefficients. We further highlight yet another remarkable potential of coincidence measurements as a probe with better resolution as compared to standard spectroscopic techniques. The finer features show up in both angle resolved and frequency resolved studies.

  7. Modulation of attosecond beating in resonant two-photon ionization

    CERN Document Server

    Galán, Álvaro J; Martín, Fernando

    2014-01-01

    We present a theoretical study of the photoelectron attosecond beating at the basis of RABBIT (Reconstruction of Attosecond Beating By Interference of Two-photon transitions) in the presence of autoionizing states. We show that, as a harmonic traverses a resonance, its sidebands exhibit a peaked phase shift as well as a modulation of the beating frequency itself. Furthermore, the beating between two resonant paths persists even when the pump and the probe pulses do not overlap, thus providing a sensitive non-holographic interferometric means to reconstruct coherent metastable wave packets. We characterize these phenomena quantitatively with a general finite-pulse analytical model that accounts for the effect of both intermediate and final resonances on two-photon processes, at a negligible computational cost. The model predictions are in excellent agreement with those of accurate ab initio calculations for the helium atom in the region of the N=2 doubly excited states.

  8. Adiabatic quenches and characterization of amplitude excitations in a continuous quantum phase transition

    Science.gov (United States)

    Hoang, Thai M.; Bharath, Hebbe M.; Boguslawski, Matthew J.; Anquez, Martin; Robbins, Bryce A.; Chapman, Michael S.

    2016-01-01

    Spontaneous symmetry breaking occurs in a physical system whenever the ground state does not share the symmetry of the underlying theory, e.g., the Hamiltonian. This mechanism gives rise to massless Nambu–Goldstone modes and massive Anderson–Higgs modes. These modes provide a fundamental understanding of matter in the Universe and appear as collective phase or amplitude excitations of an order parameter in a many-body system. The amplitude excitation plays a crucial role in determining the critical exponents governing universal nonequilibrium dynamics in the Kibble–Zurek mechanism (KZM). Here, we characterize the amplitude excitations in a spin-1 condensate and measure the energy gap for different phases of the quantum phase transition. At the quantum critical point of the transition, finite-size effects lead to a nonzero gap. Our measurements are consistent with this prediction, and furthermore, we demonstrate an adiabatic quench through the phase transition, which is forbidden at the mean field level. This work paves the way toward generating entanglement through an adiabatic phase transition. PMID:27503886

  9. Adiabatic quenches and characterization of amplitude excitations in a continuous quantum phase transition

    Science.gov (United States)

    Hoang, Thai M.; Bharath, Hebbe M.; Boguslawski, Matthew J.; Anquez, Martin; Robbins, Bryce A.; Chapman, Michael S.

    2016-08-01

    Spontaneous symmetry breaking occurs in a physical system whenever the ground state does not share the symmetry of the underlying theory, e.g., the Hamiltonian. This mechanism gives rise to massless Nambu-Goldstone modes and massive Anderson-Higgs modes. These modes provide a fundamental understanding of matter in the Universe and appear as collective phase or amplitude excitations of an order parameter in a many-body system. The amplitude excitation plays a crucial role in determining the critical exponents governing universal nonequilibrium dynamics in the Kibble-Zurek mechanism (KZM). Here, we characterize the amplitude excitations in a spin-1 condensate and measure the energy gap for different phases of the quantum phase transition. At the quantum critical point of the transition, finite-size effects lead to a nonzero gap. Our measurements are consistent with this prediction, and furthermore, we demonstrate an adiabatic quench through the phase transition, which is forbidden at the mean field level. This work paves the way toward generating entanglement through an adiabatic phase transition.

  10. \\pi N transition distribution amplitudes: their symmetries and constraints from chiral dynamics

    CERN Document Server

    Pire, Bernard; Szymanowski, Lech

    2011-01-01

    Baryon to meson Transition Distribution Amplitudes (TDAs) extend the concept of generalized parton distributions. Baryon to meson TDAs appear as building blocks in the colinear factorized description of amplitudes for a class of hard exclusive reactions, prominent examples of which being hard exclusive meson electroproduction off a nucleon in the backward region and baryon-antibaryon annihilation into a meson and a lepton pair. We study general properties of these objects following from the underlying symmetries of QCD. In particular, the Lorentz symmetry results in the polynomiality property of the Mellin moments in longitudinal momentum fractions. We present a detailed account of isotopic and permutation symmetry properties of nucleon to pion (\\pi N) TDAs. This restricts the number of independent leading twist \\pi N TDAs to eight functions providing description of all isotopic channels. Using chiral symmetry and the crossing relation between \\pi N TDAs and \\pi N generalized distribution amplitudes we establ...

  11. A ``Master'' perturbation series for the transition amplitude in a light field

    Science.gov (United States)

    Faisal, F. H. M.

    2009-08-01

    We derive a “master” perturbation series for the quantum amplitude for a given transition process induced by laser-matter interaction. The result is derived using a complete set of basis functions depending on a real parameter λ. It provides a one-parameter (λ) family of infinitely many equivalent series representations of one and the same transition amplitude defined in the minimal coupling (MC) “velocity gauge”. As a first application of the master series we put λ = 0 and 1 in the formula and immediately obtain the two well-known perturbation series, traditionally derived in the “velocity” and “length” gauges. The master formula can be used to obtain any number of equivalent perturbation series by simply choosing a real number for λ; e.g., a “hybrid perturbation” series follows from putting λ = 1/2 in the formula.

  12. Two-photon physics at LEP2

    Energy Technology Data Exchange (ETDEWEB)

    Cartwright, Susan; Lehto, Mark [University of Sheffield Department of Physics, Sheffield S3 7RH (United Kingdom); Seymour, Michael H.; Close, Frank; Wright, Alison [Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire OX11 0QX (United Kingdom); Affholderbach, Klaus; Cowan, Glen [Universitaet Siegen, Fachbereich Physik, D-57068 Siegen (Germany); Finch, Alex [University of Lancaster, Lancaster LA1 4YB (United Kingdom); Lauber, Jan [University College London, Gower Street, London WC1E 6BT (United Kingdom)

    1998-02-01

    The working group on two-photon physics concentrated on three main subtopics: modelling the hadronic final state of deep inelastic scattering on a photon; unfolding the deep inelastic scattering data to obtain the photon structure function; and resonant production of exclusive final states, particularly of glueball candidates. In all three areas, new results were presented. (author)

  13. Two-photon microscopy for chemical neuroscience.

    Science.gov (United States)

    Ellis-Davies, Graham C R

    2011-04-20

    Microscopes using non-linear excitation of chromophores with pulsed near-IR light can generate highly localized foci of molecules in the electronic singlet state that are concentrated in volumes of less than one femtoliter. The three-dimensional confinement of excitation arises from the simultaneous absorption of two IR photons of approximately half the energy required for linear excitation. Two-photon microscopy is especially useful for two types of interrogation of neural processes. First, uncaging of signaling molecules such as glutamate, as stimulation is so refined it can be used to mimic normal unitary synaptic levels. In addition, uncaging allows complete control of the timing and position of stimulation, so the two-photon light beam provides the chemical neuroscientist with an "optical conductor's baton" which can command synaptic activity at will. A second powerful feature of two-photon microscopy is that when used for fluorescence imaging it enables the visualization of cellular structure and function in living animals at depths far beyond that possible with normal confocal microscopes. In this review I provide a survey of the many important applications of two-photon microscopy in these two fields of neuroscience, and suggest some areas for future technical development.

  14. Two-photon production of charged pion and kaon pairs

    CERN Document Server

    Dominick, J; Sanghera, S; Shelkov, V; Skwarnicki, T; Stroynowski, R; Volobuev, I P; Wei, G; Zadorozhny, P; Artuso, M; Goldberg, M; He, D; Horwitz, N; Kennett, R; Mountain, R; Moneti, G C; Muheim, F; Mukhin, Y; Playfer, S; Rozen, Y; Stone, S; Thulasidas, M; Vasseur, G; Zhu, G; Bartelt, J; Csorna, S E; Egyed, Z; Jain, V; Kinoshita, K; Edwards, K W; Ogg, M; Britton, D I; Hyatt, E R F; MacFarlane, D B; Patel, P M; Akerib, D S; Barish, B C; Chadha, M; Chan, S; Cowen, D F; Eigen, G; Miller, J S; O'Grady, C; Urheim, J; Weinstein, A J; Acosta, D; Athanas, M; Masek, G E; Paar, H P; Sivertz, M; Gronberg, J B; Kutschke, R; Menary, S R; Morrison, R J; Nakanishi, S; Nelson, H N; Nelson, T K; Qiao, C; Richman, J D; Ryd, A; Tajima, H; Sperka, D; Witherell, M S; Procario, M; Balest, R; Cho, K; Daoudi, M; Ford, W T; Johnson, D R; Lingel, K; Lohner, M; Rankin, P; Smith, J G; Alexander, J P; Bebek, C; Berkelman, K; Bloom, K; Browder, T E; Cassel, David G; Cho, H A; Coffman, D M; Drell, P S; Ehrlich, R; Gaidarev, P B; Galik, R S; García-Sciveres, M; Geiser, B; Gittelman, B; Gray, S W; Hartill, D L; Heltsley, B K; Jones, C D; Jones, S L; Kandaswamy, J; Katayama, N; Kim, P C; Kreinick, D L; Ludwig, G S; Masui, J; Mevissen, J; Mistry, N B; Ng, C R; Nordberg, E; Patterson, J R; Peterson, D; Riley, D; Salman, S; Sapper, M; Würthwein, F; Avery, P; Freyberger, A P; Rodríguez, J; Stephens, R; Yang, S; Yelton, J; Cinabro, D; Henderson, S; Liu, T; Saulnier, M; Wilson, R; Yamamoto, H; Bergfeld, T; Eisenstein, B I; Gollin, G; Ong, B; Palmer, M; Selen, M; Thaler, J J; Sadoff, A J; Ammar, R; Ball, S; Baringer, P; Bean, A; Besson, D; Coppage, D; Copty, N K; Davis, R; Hancock, N; Kelly, M; Kwak, N; Lam, H; Kubota, Y; Lattery, M; Nelson, J K; Patton, S; Perticone, D; Poling, R A; Savinov, V; Schrenk, S; Wang, R; Alam, M S; Kim, I J; Nemati, B; O'Neill, J J; Severini, H; Sun, C R; Zoeller, M M; Crawford, G; Daubenmier, C M; Fulton, R; Fujino, D; Gan, K K; Honscheid, K; Kagan, H; Kass, R; Lee, J; Malchow, R L; Skovpen, Y; Sung, M; White, C; Butler, F; Fu, X; Kalbfleisch, G R; Ross, W R; Skubic, P L; Snow, J; Wang, P L; Wood, M; Brown, D N; Fast, J; McIlwain, R L; Miao, T; Miller, D H; Modesitt, M; Payne, D; Shibata, E I; Shipsey, I P J; Wang Pei Ning; Battle, M; Ernst, J; Kwon, Y; Roberts, S; Thorndike, E H; Wang, C H

    1994-01-01

    A measurement of the cross section for the combined two-photon production of charged pion and kaon pairs is performed using 1.2~\\rm fb^{-1} of data collected by the CLEO II detector at the Cornell Electron Storage Ring. The cross section is measured at invariant masses of the two-photon system between 1.5 and 5.0~GeV/c^2, and at scattering angles more than 53^\\circ away from the \\gamma\\gamma collision axis in the \\gamma\\gamma center-of-mass frame. The large background of leptonic events is suppressed by utilizing the CsI calorimeter in conjunction with the muon chamber system. The reported cross section is compared with leading order QCD models as well as previous experiments. In particular, although the functional dependence of the measured cross section disagrees with leading order QCD at small values of the two-photon invariant mass, the data show a transition to perturbative behavior at an invariant mass of approximately 2.5~GeV/c^2. hardcopies with figures can be obtained by writing to to: Pam Morehouse ...

  15. Transparency induced by two photon interference in a beam splitter

    Institute of Scientific and Technical Information of China (English)

    Wang Kai-Ge; Yang Guo-Jian

    2004-01-01

    We propose a special two-photon state which is completely transparent in a 50/50 beam splitter. This effect is caused by the destructive two-photon interference and shows the signature of photon entanglement. We find that the symmetry of the two-photon spectrum plays the key role for the properties of two-photon interference.

  16. Magnetic two-photon scattering and two-photon emission - Cross sections and redistribution functions

    Science.gov (United States)

    Alexander, S. G.; Meszaros, P.

    1991-01-01

    The magnetic two-photon scattering cross section is discussed within the framework of QED, and the corresponding scattering redistribution function for this process and its inverse, as well as the scattering source function are calculated explicitly. In a similar way, the magnetic two-photon emission process which follows the radiative excitation of Landau levels above ground is calculated. The two-photon scattering and two-photon emission are of the same order as the single-photon magnetic scattering. All three of these processes, and in optically thick cases also their inverses, are included in radiative transport calculations modeling accreting pulsars and gamma-ray bursters. These processes play a prominent role in determining the relative strength of the first two cyclotron harmonics, and their effects extend also to the higher harmonics.

  17. Two-photon ionization of colliding atoms

    Energy Technology Data Exchange (ETDEWEB)

    Nayfeh, M.H.

    1977-09-01

    Semiclassical expressions of two-photon ionization of two colliding atoms are derived for a wide range of electromagnetic field intensity and detunings from the isolated atom line. The dependence of the ionization yield on the details of the interaction potential of the system is derived. This process promises an extremely sensitive method for studying line broadening on the far wing, especially when absorption or fluorescence becomes very weak.

  18. Two Photon Decays of Charmonia from Lattice QCD

    Energy Technology Data Exchange (ETDEWEB)

    Jozef Dudek; Robert Edwards

    2006-07-12

    We make the first calculation in lattice QCD of two-photon decays of mesons. Working in the charmonium sector, using the LSZ reduction to relate a photon to a sum of hadronic vector eigenstates, we compute form-factors in both the space-like and time-like domains for the transitions {eta}{sub c} {yields} {gamma}*{gamma}* and {chi}{sub c0} {yields} {gamma}*{gamma}*. At the on-shell point we find approximate agreement with experimental world-average values.

  19. Two-photon photoassociative spectroscopy of ultracold 88-Sr

    CERN Document Server

    de Escobar, Y N Martinez; Pellegrini, P; Nagel, S B; Traverso, A; Yan, M; Côté, R; Killian, T C

    2008-01-01

    We present results from two-photon photoassociative spectroscopy of the least-bound vibrational level of the X$^1\\Sigma_g^+$ state of the $^{88}$Sr$_2$ dimer. Measurement of the binding energy allows us to determine the s-wave scattering length, $a_{88}=-1.4(6) a_0$. For the intermediate state, we use a bound level on the metastable $^1S_0$-$^3P_1$ potential, which provides large Franck-Condon transition factors and narrow one-photon photoassociative lines that are advantageous for observing quantum-optical effects such as Autler-Townes resonance splittings.

  20. Two-photon photoassociative spectroscopy of ultracold Sr88

    Science.gov (United States)

    Martinez de Escobar, Y. N.; Mickelson, P. G.; Pellegrini, P.; Nagel, S. B.; Traverso, A.; Yan, M.; Côté, R.; Killian, T. C.

    2008-12-01

    We present results from two-photon photoassociative spectroscopy of the least-bound vibrational level of the XΣg+1 state of the Sr288 dimer. Measurement of the binding energy allows us to determine the s -wave scattering length a88=-1.4(6)a0 . For the intermediate state, we use a bound level on the metastable S01-P13 potential, which provides large Franck-Condon transition factors and narrow one-photon photoassociative lines that are advantageous for observing quantum-optical effects such as Autler-Townes resonance splittings.

  1. Two-photon super bunching of thermal light via multiple two-photon-path interference

    CERN Document Server

    Hong, Peilong; Zhang, Guoquan

    2012-01-01

    We propose a novel scheme to achieve two-photon super bunching of thermal light through multiple two-photon-path interference, in which two mutually first-order incoherent optical channels are introduced by inserting a modified Michelson interferometer into a traditional two-photon HBT interferometer, and the bunching peak-to-background ratio can reach 3 theoretically. Experimentally, the super bunching peak-to-background ratio was measured to be 2.4, much larger than the ratio 1.7 measured with the same thermal source in a traditional HBT interferometer. The peak-to-background ratio of two-photon super bunching of thermal light can be increased up to $2\\times1.5^n$ by inserting cascadingly $n$ pairs of mutually first-order incoherent optical channels into the traditional two-photon HBT interferometer. The two-photon super bunching of thermal light should be of great significance in improving the visibility of classical ghost imaging.

  2. Experimental access to transition distribution amplitudes with the PANDA experiment at FAIR

    Energy Technology Data Exchange (ETDEWEB)

    Zambrana, Manuel; Ahmed, Samer; Deiseroth, Malte; Froehlich, Bertold; Khaneft, Dmitry; Lin, Dexu; Noll, Oliver; Valente, Roserio; Zimmermann, Iris [Institut fuer Kernphysik, Johannes Gutenberg Universitaet, Mainz (Germany); Helmholtz-Institut Mainz (Germany); Mora Espi, Maria Carmen; Ahmadi, Heybat; Capozza, Luigi; Dbeyssi, Alaa; Morales, Cristina; Rodriguez Pineiro, David [Helmholtz-Institut Mainz (Germany); Maas, Frank [Institut fuer Kernphysik, Johannes Gutenberg Universitaet, Mainz (Germany); Helmholtz-Institut Mainz (Germany); Prisma Cluster of Excellence, Mainz (Germany)

    2015-07-01

    We address the feasibility of accessing proton to pion Transition Distribution Amplitudes with the future PANDA detector at the FAIR facility. At high center of mass energy and four-momentum transfer, the amplitude of signal channel anti pp → e{sup +}e{sup -}π{sup 0} admits a QCD factorized description in terms of Distribution Amplitudes and Transition Distribution Amplitudes in the forward and backward regions. Assuming a factorized cross section, feasibility studies of measuring anti pp → e{sup +}e{sup -}π{sup 0} with PANDA have been performed at the center of mass energy squared s=5 GeV{sup 2} and s=10 GeV{sup 2}, in the kinematic region of four-momentum transfer 3.0 < q{sup 2} < 4.3 GeV{sup 2} and 5 < q{sup 2} < 9 GeV{sup 2}, respectively, with a neutral pion scattered in the forward or backward cone cosθ{sub π{sup 0}} > 0.5 in the anti pp center of mass frame. These include detailed simulations on signal reconstruction efficiency, rejection of the most severe background channel, i.e. anti pp → π{sup +}π{sup -}π{sup 0}, and the feasibility of the measurement using a sample of 2 fb{sup -1} of integrated luminosity. Results of the simulations show that a background rejection factor from 10{sup 7} at s=5 GeV{sup 2} to 10{sup 8} at s=10 GeV{sup 2} can be achieved, while keeping the signal reconstruction efficiency at the level of 40%, and that a clean lepton signal can be reconstructed with 2 fb{sup -1} of integrated luminosity at both energies. The ''measured'' cross sections with the simulations are used to test QCD factorization at the leading order by measuring scaling laws and fitting angular distributions.

  3. The Pion-Photon Transition Distribution Amplitudes in the Nambu-Jona Lasinio Model

    CERN Document Server

    Courtoy, A

    2007-01-01

    We define the pion-photon Transition Distribution Amplitudes (TDA) in a field theoretic formalism from a covariant Bethe-Salpeter approach for the determination of the bound state. We apply our formalism to the Nambu - Jona Lasinio model, as a realistic theory of the pion. The obtained vector and axial TDAs satisfy all features required by general considerations. In particular, sum rules and polynomiality condition are explicitly verified. We have numerically proved that the odd coefficients in the polynomiality expansion of the vector TDA vanish in the chiral limit. The role of PCAC and the presence of a pion pole are explicitly showed.

  4. Pion-to-photon transition distribution amplitudes in the non-local chiral quark model

    CERN Document Server

    Kotko, Piotr

    2008-01-01

    We apply the non-local chiral quark model to study vector and axial pion-to-photon transition amplitudes that are needed as a nonperturbative input to estimate the cross section of pion annihilation into the real and virtual photon. We use a simple form of the non-locality that allows to perform all calculations in the Minkowski space and guaranties polynomiality of the TDA's. We note only residual dependence on the precise form of the cut-off function, however vector TDA that is symmetric in skewedness parameter in the local quark model is no longer symmetric in the non-local case. We calculate also the transition form-factors and compare them with existing experimental parametrizations.

  5. Relativistic coupled cluster calculations on hyperfine structures and electromagnetic transition amplitudes of In III

    CERN Document Server

    Roy, Sourav; Majumder, Sonjoy

    2014-01-01

    Hyperfine constants and anomalies of ground as well as few low lying excited states of $^{113,115,117}$In III are studied with highly correlated relativistic coupled-cluster theory. The ground state hyperfine splitting of $^{115}$In III is estimated to be 106.8 GHz. A shift of almost 1.9 GHz of the above frequency has been calculated due to modified nuclear dipole moment. This splitting result shows its applicability as communication band and frequency standards at $10^{-11}$ sec. Correlations study of hyperfine constants indicates a few distinct features of many-body effects in the wave-functions in and near the nuclear region of this ion. Astrophysically important forbidden transition amplitudes are estimated for the first time in the literature to our knowledge. The calculated oscillator strengths of few allowed transitions are compared with recent experimental and theoretical results wherever available.

  6. A spectral representation for baryon to meson and baryon to photon transition distribution amplitudes

    CERN Document Server

    Pire, Bernard; Szymanowski, Lech

    2010-01-01

    We construct a spectral representation for the transition distribution amplitudes (TDAs), i.e. matrix elements of three quark correlators which arise e.g. in the description of baryon to meson and baryon to photon transitions within the factorization approach to hard exclusive reactions. We generalize for these quantities the notion of double distributions introduced in the context of generalized parton distributions. We propose the generalization of A.Radyushkin's factorized Ansatz for the case of baryon to meson and baryon to photon TDAs. Our construction opens the way to modeling of baryon to meson and baryon to photon TDAs in their complete domain of definition and quantitative estimates of cross-sections for various hard exclusive reactions.

  7. Denoising two-photon calcium imaging data.

    Science.gov (United States)

    Malik, Wasim Q; Schummers, James; Sur, Mriganka; Brown, Emery N

    2011-01-01

    Two-photon calcium imaging is now an important tool for in vivo imaging of biological systems. By enabling neuronal population imaging with subcellular resolution, this modality offers an approach for gaining a fundamental understanding of brain anatomy and physiology. Proper analysis of calcium imaging data requires denoising, that is separating the signal from complex physiological noise. To analyze two-photon brain imaging data, we present a signal plus colored noise model in which the signal is represented as harmonic regression and the correlated noise is represented as an order autoregressive process. We provide an efficient cyclic descent algorithm to compute approximate maximum likelihood parameter estimates by combing a weighted least-squares procedure with the Burg algorithm. We use Akaike information criterion to guide selection of the harmonic regression and the autoregressive model orders. Our flexible yet parsimonious modeling approach reliably separates stimulus-evoked fluorescence response from background activity and noise, assesses goodness of fit, and estimates confidence intervals and signal-to-noise ratio. This refined separation leads to appreciably enhanced image contrast for individual cells including clear delineation of subcellular details and network activity. The application of our approach to in vivo imaging data recorded in the ferret primary visual cortex demonstrates that our method yields substantially denoised signal estimates. We also provide a general Volterra series framework for deriving this and other signal plus correlated noise models for imaging. This approach to analyzing two-photon calcium imaging data may be readily adapted to other computational biology problems which apply correlated noise models.

  8. Experimental access to Transition Distribution Amplitudes with the \\={P}ANDA experiment at FAIR

    CERN Document Server

    Singh, B P; Keshelashvili, I; Krusche, B; Steinacher, M; Liu, B; Liu, H; Liu, Z; Shen, X; Wang, C; Zhao, J; Albrecht, M; Fink, M; Heinsius, F H; Held, T; Holtmann, T; Koch, H; Kopf, B; Kümmel, M; Kuhl, G; Kuhlmann, M; Leyhe, M; Mikirtychyants, M; Musiol, P; Mustafa, A; Pelizäus, M; Pychy, J; Richter, M; Schnier, C; Schröder, T; Sowa, C; Steinke, M; Triffterer, T; Wiedner, U; Beck, R; Hammann, C; Kaiser, D; Ketzer, B; Kube, M; Mahlberg, P; Rossbach, M; Schmidt, C; Schmitz, R; Thoma, U; Walther, D; Wendel, C; Wilson, A; Bianconi, A; Bragadireanu, M; Caprini, M; Pantea, D; Pietreanu, D; Vasile, M E; Patel, B; Kaplan, D; Brandys, P; Czyzewski, T; Czyzycki, W; Domagala, M; Hawryluk, M; Filo, G; Krawczyk, M; Kwiatkowski, D; Lisowski, E; Lisowski, F; Fiutowski, T; Idzik, M; Mindur, B; Przyborowski, D; Swientek, K; Czech, B; Kliczewski, S; Korcyl, K; Kozela, A; Kulessa, P; Lebiedowicz, P; Malgorzata, K; Pysz, K; Schäfer, W; Siudak, R; Szczurek, A; Biernat, J; Jowzaee, S; Kamys, B; Kistryn, S; Korcyl, G; Krzemien, W; Magiera, A; Moskal, P; Palka, M; Psyzniak, A; Rudy, Z; Salabura, P; Smyrski, J; Strzempek, P; Wrońska, A; Augustin, I; Lehmann, I; Nicmorus, D; Schepers, G; Schmitt, L; Al-Turany, M; Cahit, U; Capozza, L; Dbeyssi, A; Deppe, H; Dzhygadlo, R; Ehret, A; Flemming, H; Gerhardt, A; Götzen, K; Karabowicz, R; Kliemt, R; Kunkel, J; Kurilla, U; Lehmann, D; Lühning, J; Maas, F; Morales, C Morales; Espí, M C Mora; Nerling, F; Orth, H; Peters, K; Piñeiro, D Rodríguez; Saito, N; Saito, T; Lorente, A Sánchez; Schmidt, C J; Schwarz, C; Schwiening, J; Traxler, M; Valente, R; Voss, B; Wieczorek, P; Wilms, A; Zühlsdorf, M; Abazov, V M; Alexeev, G; Arefiev, A; Astakhov, V I; Barabanov, M Yu; Batyunya, B V; Davydov, Yu I; Dodokhov, V Kh; Efremov, A A; Fedunov, A G; Festchenko, A A; Galoyan, A S; Grigoryan, S; Karmokov, A; Koshurnikov, E K; Lobanov, V I; Lobanov, Yu Yu; Makarov, A F; Malinina, L V; Malyshev, V L; Mustafaev, G A; Olshevskiy, A; Pasyuk, M A; Perevalova, E A; Piskun, A A; Pocheptsov, T A; Pontecorvo, G; Rodionov, V K; Rogov, Yu N; Salmin, R A; Samartsev, A G; Sapozhnikov, M G; Shabratova, G S; Skachkov, N B; Skachkova, A N; Strokovsky, E A; Suleimanov, M K; Teshev, R Sh; Tokmenin, V V; Uzhinsky, V V; Vodopyanov, A S; Zaporozhets, S A; Zhuravlev, N I; Zorin, A G; Branford, D; Glazier, D; Watts, D; Woods, P; Britting, A; Eyrich, W; Lehmann, A; Uhlig, F; Dobbs, S; Seth, K; Tomaradze, A; Xiao, T; Bettoni, D; Carassiti, V; Ramusino, A Cotta; Dalpiaz, P; Drago, A; Fioravanti, E; Garzia, I; Savriè, M; Stancari, G; Akishina, V; Kisel, I; Kulakov, I; Zyzak, M; Arora, R; Bel, T; Gromliuk, A; Kalicy, G; Krebs, M; Patsyuk, M; Zuehlsdorf, M; Bianchi, N; Gianotti, P; Guaraldo, C; Lucherini, V; Pace, E; Bersani, A; Bracco, G; Macri, M; Parodi, R F; Bianco, S; Bremer, D; Brinkmann, K T; Diehl, S; Dormenev, V; Drexler, P; Düren, M; Eissner, T; Etzelmüller, E; Föhl, K; Galuska, M; Gessler, T; Gutz, E; Hayrapetyan, A; Hu, J; Kröck, B; Kühn, W; Kuske, T; Lange, S; Liang, Y; Merle, O; Metag, V; Mülhheim, D; Münchow, D; Nanova, M; Novotny, R; Pitka, A; Quagli, T; Rieke, J; Rosenbaum, C; Schnell, R; Spruck, B; Stenzel, H; Thöring, U; Ullrich, T; Wasem, T; Werner, M; Zaunick, H G; Ireland, D; Rosner, G; Seitz, B; Deepak, P N; Kulkarni, A V; Apostolou, A; Babai, M; Kavatsyuk, M; Lemmens, P; Lindemulder, M; Löhner, H; Messchendorp, J; Schakel, P; Smit, H; van der Weele, J C; Veenstra, R; Tiemens, M; Vejdani, S; Kalita, K; Mohanta, D P; Kumar, A; Roy, A; Sahoo, R; Sohlbach, H; Büscher, M; Cao, L; Cebulla, A; Deermann, D; Dosdall, R; Esch, S; Georgadze, I; Gillitzer, A; Goerres, A; Goldenbaum, F; Grunwald, D; Herten, A; Hu, Q; Kemmerling, G; Kleines, H; Kozlov, V; Lehrach, A; Leiber, S; Maier, R; Nellen, R; Ohm, H; Orfanitski, S; Prasuhn, D; Prencipe, E; Ritman, J; Schadmand, S; Schumann, J; Sefzick, T; Serdyuk, V; Sterzenbach, G; Stockmanns, T; Wintz, P; Wüstner, P; Xu, H; Li, S; Li, Z; Sun, Z; Rigato, V; Fissum, S; Hansen, K; Isaksson, L; Lundin, M; Schröder, B; Achenbach, P; Bleser, S; Cardinali, M; Corell, O; Deiseroth, M; Denig, A; Distler, M; Feldbauer, F; Fritsch, M; Jasinski, P; Hoek, M; Kangh, D; Karavdina, A; Lauth, W; Leithoff, H; Merkel, H; Michel, M; Motzko, C; Müller, U; Noll, O; Plueger, S; Pochodzalla, J; Sanchez, S; Schlimme, S; Sfienti, C; Steinen, M; Thiel, M; Weber, T; Zambrana, M; Dormenev, V I; Fedorov, A A; Korzihik, M V; Missevitch, O V; Balanutsa, P; Balanutsa, V; Chernetsky, V; Demekhin, A; Dolgolenko, A; Fedorets, P; Gerasimov, A; Goryachev, V; Varentsov, V; Boukharov, A; Malyshev, O; Marishev, I; Semenov, A; Konorov, I; Paul, S; Grieser, S; Hergemöller, A K; Khoukaz, A; Köhler, E; Täschner, A; Wessels, J; Dash, S; Jadhav, M; Kumar, S; Sarin, P; Varma, R; Chandratre, V B; Datar, V; Dutta, D; Jha, V; Kumawat, H; Mohanty, A K; Roy, B; Yan, Y; Chinorat, K; Khanchai, K; Ayut, L; Pornrad, S; Barnyakov, A Y; Blinov, A E; Blinov, V E; Bobrovnikov, V S; Kononov, S A; Kravchenko, E A; Kuyanov, I A; Onuchin, A P; Sokolov, A A; Tikhonov, Y A; Atomssa, E; Hennino, T; Imre, M; Kunne, R; Galliard, C Le; Ma, B; Marchand, D; Ong, S; Ramstein, B; Rosier, P; Tomasi-Gustafsson, E; Van de Wiele, J; Boca, G; Costanza, S; Genova, P; Lavezzi, L; Montagna, P; Rotondi, A; Abramov, V; Belikov, N; Bukreeva, S; Davidenko, A; Derevschikov, A; Goncharenko, Y; Grishin, V; Kachanov, V; Kormilitsin, V; Melnik, Y; Levin, A; Minaev, N; Mochalov, V; Morozov, D; Nogach, L; Poslavskiy, S; Ryazantsev, A; Ryzhikov, S; Semenov, P; Shein, I; Uzunian, A; Vasiliev, A; Yakutin, A; Yabsley, B; Bäck, T; Cederwall, B; Makónyi, K; Tegnér, P E; von Würtemberg, K M; Belostotski, S; Gavrilov, G; Izotov, A; Kashchuk, A; Levitskaya, O; Manaenkov, S; Miklukho, O; Naryshkin, Y; Suvorov, K; Veretennikov, D; Zhadanov, A; Rai, A K; Godre, S S; Duchat, R; Amoroso, A; Bussa, M P; Busso, L; De Mori, F; Destefanis, M; Fava, L; Ferrero, L; Greco, M; Maggiora, M; Maniscalco, G; Marcello, S; Sosio, S; Spataro, S; Zotti, L; Calvo, D; Coli, S; De Remigis, P; Filippi, A; Giraudo, G; Lusso, S; Mazza, G; Mingnore, M; Rivetti, A; Wheadon, R; Balestra, F; Iazzi, F; Introzzi, R; Lavagno, A; Younis, H; Birsa, R; Bradamante, F; Bressan, A; Martin, A; Clement, H; Gålnander, B; Balkeståhl, L Caldeira; Calén, H; Fransson, K; Johansson, T; Kupsc, A; Marciniewski, P; Pettersson, J; Schönning, K; Wolke, M; Zlomanczuk, J; Díaz, J; Ortiz, A; Vinodkumar, P C; Parmar, A; Chlopik, A; Melnychuk, D; Slowinski, B; Trzcinski, A; Wojciechowski, M; Wronka, S; Zwieglinski, B; Bühler, P; Marton, J; Suzuki, K; Widmann, E; Zmeskal, J; Fröhlich, B; Khaneft, D; Lin, D; Zimmermann, I; Semenov-Tian-Shansky, K

    2014-01-01

    We address the possibility of accessing nucleon-to-pion ($\\pi N$) Transition Distribution Amplitudes (TDAs) from $\\bar{p}p \\to e^+e^- \\pi^0$ reaction with the future \\={P}ANDA detector at the FAIR facility. At high center of mass energy and high invariant mass of the lepton pair $q^2$, the amplitude of the signal channel $\\bar{p}p \\to e^+e^- \\pi^0$ admits a QCD factorized description in terms of $\\pi N$ TDAs and nucleon Distribution Amplitudes (DAs) in the forward and backward kinematic regimes. Assuming the validity of this factorized description, we perform feasibility studies for measuring $\\bar{p}p \\to e^+e^- \\pi^0$ with the \\={P}ANDA detector. Detailed simulations on signal reconstruction efficiency as well as on rejection of the most severe background channel, {\\it i.e.} $\\bar{p}p \\to \\pi^+\\pi^- \\pi^0$ were performed for the center of mass energy squared $s = 5$ GeV$^2$ and $s = 10$ GeV$^2$, in the kinematic regions $3.0 0.5 $ in the proton-antiproton center of mass frame. Results of the simulation sho...

  9. Two-photon vibrational excitation of air by long-wave infrared laser pulses

    CERN Document Server

    Palastro, J P; Johnson, L A; Hafizi, B; Wahlstrand, J K; Milchberg, H M

    2016-01-01

    Ultrashort long-wave infrared (LWIR) laser pulses can resonantly excite vibrations in N2 and O2 through a two-photon transition. The absorptive, vibrational component of the ultrafast optical nonlinearity grows in time, starting smaller than, but quickly surpassing, the electronic, rotational, and vibrational refractive components. The growth of the vibrational component results in a novel mechanism of 3rd harmonic generation, providing an additional two-photon excitation channel, fundamental + 3rd harmonic. The original and emergent two-photon excitations drive the resonance exactly out of phase, causing spatial decay of the absorptive, vibrational nonlinearity. This nearly eliminates two-photon vibrational absorption. Here we present simulations and analytical calculations demonstrating how these processes modify the ultrafast optical nonlinearity in air. The results reveal nonlinear optical phenomena unique to the LWIR regime of ultrashort pulse propagation in atmosphere.

  10. Higgs boson decay into two photons in an electromagnetic background field

    DEFF Research Database (Denmark)

    Nielsen, N. K.

    2014-01-01

    The amplitude for Higgs boson decay into two photons in a homogeneous and time-independent magnetic field is investigated by proper-time regularization in a gauge-invariant manner and is found to be singular at large field values. The singularity is caused by the component of the charged vector...

  11. Experimental method for the determination of two-photon cross sections using four-wave mixing

    Science.gov (United States)

    Burris, J.; Mcilrath, T. J.

    1985-01-01

    The two-photon absorption cross section for the R22 + S12(J double prime = 9 1/2) transition in nitric oxide's gamma band has been determined. The value is in good agreement with previous measurements on several other NO transitions. The technique described here can be used to obtain accurate cross sections for other diatomic molecules.

  12. Experimental method for the determination of two-photon cross sections using four-wave mixing

    Science.gov (United States)

    Burris, J.; Mcilrath, T. J.

    1985-01-01

    The two-photon absorption cross section for the R22 + S12(J double prime = 9 1/2) transition in nitric oxide's gamma band has been determined. The value is in good agreement with previous measurements on several other NO transitions. The technique described here can be used to obtain accurate cross sections for other diatomic molecules.

  13. Two-photon absorption and two-photon circular dichroism of L-tryptophan in the near to far UV region

    Science.gov (United States)

    Vesga, Yuly; Hernandez, Florencio E.

    2017-09-01

    Herein we report on the first measurements of the two-photon absorption (TPA) spectrum of L-tryptophan in DMSO solution in the near to far UV region and the two-photon circular dichroism (TPCD) signal corresponding to a transition at 200 nm. We demonstrate the application of the Double L-scan technique in the near to far UV region to perform polarization dependent TPA measurements of chiral molecules. TPCD measurements below 400 nm reveal that chiral molecules in solution, such as tryptophan/DMSO, can undergo photochemical reactions in front of prolonged exposure to UV radiation.

  14. Experimental investigation of a low-amplitude transition in pipe flow

    Science.gov (United States)

    Mehta, V.; Cohen, J.

    2016-12-01

    The vast majority of experiments on transition in pipe flow have been concerned with high-amplitude disturbance (of ≈ 10 % of the centerline velocity) at Reynolds numbers around 2000 and above. In this experimental study, we concentrate on the transition process in water pipe flow where the level of the disturbance is at least an order of magnitude smaller. We follow the sequence of transitional events while varying gradually the disturbance level from a laminar state to an almost fully turbulent one, using flow visualization, pressure-drop and hot-wire measurements. This is accomplished by injection of a very small diameter jet perpendicular to the main stream at a controllable flow rate, in a downstream distance where the flow is approximately fully developed. The injection flow rate normalized by the main stream rate is of O(0.001). With increasing injection flow rates the friction coefficient (λ) increases along with changes in the nature of the flow structures. The transition begins with the generation of a streamwise counter-rotating vortex pair, followed by the formation of a packet of hairpins and their breakdown. As the injection level is increased, the separation distance between two consecutive bursts (wavelength) decreases and the breakdown to turbulence begins further upstream and consequently the value of the friction coefficient λ increases. Above and below a certain threshold of the disturbance level, turbulence is either triggered or the flow is relaminarized, respectively. Finally, it is established that the evolution of the packet of hairpins is a key element during this transition scenario, and is well explained by the three-element model recently proposed by Cohen et al (2014).

  15. Two-photon interference : spatial aspects of two-photon entanglement, diffraction, and scattering

    NARCIS (Netherlands)

    Peeters, Wouter Herman

    2010-01-01

    This dissertation contains scientific research within the realm of quantum optics, which is a branch of physics. An experimental and theoretical study is made of two-photon interference phenomena in various optical systems. Spatially entangled photon pairs are produced via the nonlinear optical proc

  16. Two-photon imaging of stem cells

    Science.gov (United States)

    Uchugonova, A.; Gorjup, E.; Riemann, I.; Sauer, D.; König, K.

    2008-02-01

    A variety of human and animal stem cells (rat and human adult pancreatic stem cells, salivary gland stem cells, dental pulpa stem cells) have been investigated by femtosecond laser 5D two-photon microscopy. Autofluorescence and second harmonic generation have been imaged with submicron spatial resolution, 270 ps temporal resolution, and 10 nm spectral resolution. In particular, NADH and flavoprotein fluorescence was detected in stem cells. Major emission peaks at 460nm and 530nm with typical mean fluorescence lifetimes of 1.8 ns and 2.0 ns, respectively, were measured using time-correlated single photon counting and spectral imaging. Differentiated stem cells produced the extracellular matrix protein collagen which was detected by SHG signals at 435 nm.

  17. THE TWO-PHOTON DEGENERATE JAYNES-CUMMINGS MODEL WITH AND WITHOUT ROTATING-WAVE APPROXIMATION

    Institute of Scientific and Technical Information of China (English)

    ZHOU LING; SONG HE-SHAN; YAO LI

    2001-01-01

    We take into account the two-photon process and generalize the Jaynes-Cummings (JC) model to the case of atomic level degenerate in the projections of the angular momenta, and we establish two-photon degenerate JC models with and without the rotating-wave approximation (RWA) quantum theory. Comparing the atom population inversion of the generalized JC model with that of the original JC model, we found that the revival period of the degenerate JC model becomes longer and the maximum amplitude of atomic inversion decreases with RWA. Without RWA, the quantum chaos of the generalized JC model is much weaker than that of the original JC model

  18. Feasibility study for the measurement of πN transition distribution amplitudes with PANDA

    Science.gov (United States)

    Atomssa, Ermias

    2016-05-01

    Transition Distribution Amplitudes (TDA) are parametrizations of the hadronic matrix elements that occur in the perturbative Quantum Chromo Dynamics (QCD) calculations of a certain family of reactions within the framework of collinear factorization. We propose a complete feasibility study of the measurement of one of the reactions covered by the TDA models p ¯p →π0J /ψ (J /ψ →e+e-) at PANDA (AntiProton ANnihilation at DArmstadt) experiment currently under construction at the future FAIR (Facility for Antiproton and Ion Research). We show that PANDA will be ideally suited to access the relevant observables, in particular the pion-to-nucleon TDAs (πN TDAs) which are important for the understanding of the pion cloud contribution in the nucleon wave function.

  19. A second look at transition amplitudes in (2+1)-dimensional causal dynamical triangulations

    CERN Document Server

    Cooperman, Joshua H; Miller, Jonah M

    2016-01-01

    Studying transition amplitudes in (2+1)-dimensional causal dynamical triangulations, Cooperman and Miller discovered speculative evidence for Lorentzian quantum geometries emerging from its Euclidean path integral. On the basis of this evidence, Cooperman and Miller conjectured that Lorentzian de Sitter spacetime, not Euclidean de Sitter space, dominates the ground state of the quantum geometry of causal dynamical triangulations on large scales, a scenario akin to that of the Hartle-Hawking no-boundary proposal in which Lorentzian spacetimes dominate a Euclidean path integral. We argue against this conjecture: we propose a more straightforward explanation of their findings, and we proffer evidence for the Euclidean nature of these seemingly Lorentzian quantum geometries. This explanation reveals another manner in which the Euclidean path integral of causal dynamical triangulations behaves correctly in its semiclassical limit--the implementation and interaction of multiple constraints.

  20. A consistent model for \\pi N transition distribution amplitudes and backward pion electroproduction

    CERN Document Server

    Lansberg, J P; Semenov-Tian-Shansky, K; Szymanowski, L

    2011-01-01

    The extension of the concept of generalized parton distributions leads to the introduction of baryon to meson transition distribution amplitudes (TDAs), non-diagonal matrix elements of the nonlocal three quark operator between a nucleon and a meson state. We present a general framework for modelling nucleon to pion ($\\pi N$) TDAs. Our main tool is the spectral representation for \\pi N TDAs in terms of quadruple distributions. We propose a factorized Ansatz for quadruple distributions with input from the soft-pion theorem for \\pi N TDAs. The spectral representation is complemented with a D-term like contribution from the nucleon exchange in the cross channel. We then study backward pion electroproduction in the QCD collinear factorization approach in which the non-perturbative part of the amplitude involves \\pi N TDAs. Within our two component model for \\pi N TDAs we update previous leading-twist estimates of the unpolarized cross section. Finally, we compute the transverse target single spin asymmetry as a fu...

  1. Calculation of hadronic transition amplitudes in charm physics; Berechnung hadronischer Uebergangsamplituden in der Charm-Physik

    Energy Technology Data Exchange (ETDEWEB)

    Klein, Christoph

    2011-09-23

    Transitions of charmed hadrons are of significant importance, since they provide possibilities to extract the CKM matrix elements V{sub cd} and V{sub cs} from experimental data as well as interesting channels to search for new physics effects. However, quarks are bound in hadrons, and it is necessary to describe this effect in a reliable way, to study the underlying flavour dynamics. For this, one has to use nonperturbative tools, to determine the corresponding transition amplitudes. The results of such calculations can furthermore be of use, to test the predictions of QCD and to contribute to a deeper understanding of the structure of hadrons. In this thesis two topics are investigated using the method of QCD light-cone sum rules (LCSRs). The first topic consists in the form factors of the semileptonic decays D {yields} {pi}l{nu}{sub l} and D {yields} Kl{nu}{sub l}, for which new results are calculated using up-to-date input values. Since LCSRs are not applicable in the whole range of kinematics, they are extrapolated by the use of appropriate parametrisations and the results agree well with experimental data. The second topic are the transitions of charmed baryons to a nucleon. Here the corresponding transition form factors and in addition the hadronic {lambda}{sub c}D{sup (*)}N and {sigma}{sub c}D{sup (*)}N coupling constants are calculated - the latter by the consideration of double dispersion relations. These coupling constants are of special interest for the description of hadronic interactions, like open charm production in proton-antiprotoncollisions. Furthermore there appears the problem, that both parity states of a baryon contribute to the considered functional representation, for which a consistent way to separate them is presented. (orig.)

  2. Two-photon Interference with Non-identical Photons

    CERN Document Server

    Liu, Jianbin; Zheng, Huaibin; Chen, Hui; Li, Fu-Li; Xu, Zhuo

    2014-01-01

    The indistinguishability of non-identical photons is dependent on detection system in quantum physics. If two photons with different wavelengths are indistinguishable for a detection system, there can be two-photon interference when these two photons are incident to two input ports of a Hong-Ou-Mandel interferometer, respectively. The reason why two-photon interference phenomena are different for classical and nonclassical light is not due to interference, but due to the properties of light and detection system. These conclusions are helpful to understand the physics and applications of two-photon interference.

  3. Two-Photon Micromaser with Initial Atomic Coherence

    Institute of Scientific and Technical Information of China (English)

    SUN Wei-Hui; DU Si-De; CHEN Xiao-Shuang

    2005-01-01

    @@ We investigate the quantum dynamics ora two-photon micromaser pumped by atoms injected in the superpositionstate of the upper and intermediate levels. We simulate a master equation governing the system by the MonteCarlo wavefunction approach and analyse the steady-state behaviour as a function of the atomic transit time.The atomic coherence can effectively enhance the intensity and sub-Poissonian of the cavity field as comparedwith the atomic mixture. It is also discovered that the phase of the cavity field can be shifted by adjusting thedetuning between the atom and field. This result shows that it is possible to manipulate the phase of the cavityfield by detuning, due to atomic coherence.

  4. Anomalous two-photon spectral features in warm rubidium vapor

    Science.gov (United States)

    Perrella, C.; Light, P. S.; Milburn, T. J.; Kielpinski, D.; Stace, T. M.; Luiten, A. N.

    2016-09-01

    We report observation of anomalous fluorescence spectral features in the environs of a two-photon transition in a rubidium vapor when excited with two different wavelength lasers that are both counterpropagating through the vapor. These features are characterized by an unusual trade-off between the detunings of the driving fields. Three different hypothetical processes are presented to explain the observed spectra: a simultaneous three-atom and four-photon collision, a four-photon excitation involving a light field produced via amplified spontaneous emission, and population pumping perturbing the expected steady-state spectra. Numerical modeling of each hypothetical process is presented, supporting the population pumping process as the most plausible mechanism.

  5. Polarization properties of optical phase conjugation by two-photon resonant degenerate four-wave mixing

    Science.gov (United States)

    Kauranen, Martti; Gauthier, Daniel J.; Malcuit, Michelle S.; Boyd, Robert W.

    1989-08-01

    We develop a semiclassical theory of the polarization properties of phase conjugation by two-photon resonant degenerate four-wave mixing. The theory includes the effects of saturation by the pump waves. We solve the density-matrix equations of motion in steady state for a nonlinear medium consisting of stationary atoms with a ground and excited state connected by two-photon transitions. As an illustration of the general results, we consider an S0-->S0 two-photon transition, which is known to lead to perfect polarization conjugation in the limit of third-order theory. We show that the fidelity of the polarization-conjugation process is degraded for excessively large pump intensities. The degradation can occur both due to transfer of population to the excited state and due to nonresonant Stark shifts. Theoretical results are compared to those of a recent experiment [Malcuit, Gauthier, and Boyd, Opt. Lett. 13, 663 (1988)].

  6. Higgs decay into two photons in a warped extra dimension

    Energy Technology Data Exchange (ETDEWEB)

    Hahn, Juliane; Hoerner, Clara; Malm, Raoul; Novotny, Kristiane; Schmell, Christoph [Johannes Gutenberg University, PRISMA Cluster of Excellence and Mainz Institute for Theoretical Physics, Mainz (Germany); Neubert, Matthias [Johannes Gutenberg University, PRISMA Cluster of Excellence and Mainz Institute for Theoretical Physics, Mainz (Germany); Cornell University, Department of Physics, LEPP, Ithaca, NY (United States)

    2014-05-15

    A detailed five-dimensional calculation of the Higgs-boson decay into two photons is performed in both the minimal and the custodially protected Randall-Sundrum (RS) model, where the Standard Model (SM) fields propagate in the bulk and the scalar sector lives on or near the IR brane. It is explicitly shown that the R{sub ξ} gauge invariance of the sum of diagrams involving bosonic fields in the SM also applies to the case of these RS scenarios. An exact expression for the h → γγ amplitude in terms of the five-dimensional (5D) gauge-boson and fermion propagators is presented, which includes the full dependence on the Higgs-boson mass. Closed expressions for the 5D W-boson propagators in theminimal and the custodial RS model are derived, which are valid to all orders in v{sup 2}/M{sup 2}{sub KK}. In contrast to the fermion case, the result for the bosonic contributions to the h → γγ amplitude is insensitive to the details of the localization of the Higgs profile on or near the IR brane. The various RS predictions for the rate of the pp → h → γγ process are compared with the latest LHC data, and exclusion regions for the RS model parameters are derived. (orig.)

  7. Experimental access to Transition Distribution Amplitudes with the P¯ANDA experiment at FAIR

    Science.gov (United States)

    Singh, B. P.; Erni, W.; Keshelashvili, I.; Krusche, B.; Steinacher, M.; Liu, B.; Liu, H.; Liu, Z.; Shen, X.; Wang, C.; Zhao, J.; Albrecht, M.; Fink, M.; Heinsius, F. H.; Held, T.; Holtmann, T.; Koch, H.; Kopf, B.; Kümmel, M.; Kuhl, G.; Kuhlmann, M.; Leyhe, M.; Mikirtychyants, M.; Musiol, P.; Mustafa, A.; Pelizäus, M.; Pychy, J.; Richter, M.; Schnier, C.; Schröder, T.; Sowa, C.; Steinke, M.; Triffterer, T.; Wiedner, U.; Beck, R.; Hammann, C.; Kaiser, D.; Ketzer, B.; Kube, M.; Mahlberg, P.; Rossbach, M.; Schmidt, C.; Schmitz, R.; Thoma, U.; Walther, D.; Wendel, C.; Wilson, A.; Bianconi, A.; Bragadireanu, M.; Caprini, M.; Pantea, D.; Pietreanu, D.; Vasile, M. E.; Patel, B.; Kaplan, D.; Brandys, P.; Czyzewski, T.; Czyzycki, W.; Domagala, M.; Hawryluk, M.; Filo, G.; Krawczyk, M.; Kwiatkowski, D.; Lisowski, E.; Lisowski, F.; Fiutowski, T.; Idzik, M.; Mindur, B.; Przyborowski, D.; Swientek, K.; Czech, B.; Kliczewski, S.; Korcyl, K.; Kozela, A.; Kulessa, P.; Lebiedowicz, P.; Malgorzata, K.; Pysz, K.; Schäfer, W.; Siudak, R.; Szczurek, A.; Biernat, J.; Jowzaee, S.; Kamys, B.; Kistryn, S.; Korcyl, G.; Krzemien, W.; Magiera, A.; Moskal, P.; Palka, M.; Psyzniak, A.; Rudy, Z.; Salabura, P.; Smyrski, J.; Strzempek, P.; Wrońska, A.; Augustin, I.; Lehmann, I.; Nicmorus, D.; Schepers, G.; Schmitt, L.; Al-Turany, M.; Cahit, U.; Capozza, L.; Dbeyssi, A.; Deppe, H.; Dzhygadlo, R.; Ehret, A.; Flemming, H.; Gerhardt, A.; Götzen, K.; Karabowicz, R.; Kliemt, R.; Kunkel, J.; Kurilla, U.; Lehmann, D.; Lühning, J.; Maas, F.; Morales Morales, C.; Mora Espí, M. C.; Nerling, F.; Orth, H.; Peters, K.; Rodríguez Piñeiro, D.; Saito, N.; Saito, T.; Sánchez Lorente, A.; Schmidt, C. J.; Schwarz, C.; Schwiening, J.; Traxler, M.; Valente, R.; Voss, B.; Wieczorek, P.; Wilms, A.; Zühlsdorf, M.; Abazov, V. M.; Alexeev, G.; Arefiev, A.; Astakhov, V. I.; Barabanov, M. Yu.; Batyunya, B. V.; Davydov, Yu. I.; Dodokhov, V. Kh.; Efremov, A. A.; Fedunov, A. G.; Festchenko, A. A.; Galoyan, A. S.; Grigoryan, S.; Karmokov, A.; Koshurnikov, E. K.; Lobanov, V. I.; Lobanov, Yu. Yu.; Makarov, A. F.; Malinina, L. V.; Malyshev, V. L.; Mustafaev, G. A.; Olshevskiy, A.; Pasyuk, M. A.; Perevalova, E. A.; Piskun, A. A.; Pocheptsov, T. A.; Pontecorvo, G.; Rodionov, V. K.; Rogov, Yu. N.; Salmin, R. A.; Samartsev, A. G.; Sapozhnikov, M. G.; Shabratova, G. S.; Skachkov, N. B.; Skachkova, A. N.; Strokovsky, E. A.; Suleimanov, M. K.; Teshev, R. Sh.; Tokmenin, V. V.; Uzhinsky, V. V.; Vodopyanov, A. S.; Zaporozhets, S. A.; Zhuravlev, N. I.; Zorin, A. G.; Branford, D.; Glazier, D.; Watts, D.; Woods, P.; Britting, A.; Eyrich, W.; Lehmann, A.; Uhlig, F.; Dobbs, S.; Seth, K.; Tomaradze, A.; Xiao, T.; Bettoni, D.; Carassiti, V.; Cotta Ramusino, A.; Dalpiaz, P.; Drago, A.; Fioravanti, E.; Garzia, I.; Savriè, M.; Stancari, G.; Akishina, V.; Kisel, I.; Kulakov, I.; Zyzak, M.; Arora, R.; Bel, T.; Gromliuk, A.; Kalicy, G.; Krebs, M.; Patsyuk, M.; Zuehlsdorf, M.; Bianchi, N.; Gianotti, P.; Guaraldo, C.; Lucherini, V.; Pace, E.; Bersani, A.; Bracco, G.; Macri, M.; Parodi, R. F.; Bianco, S.; Bremer, D.; Brinkmann, K. T.; Diehl, S.; Dormenev, V.; Drexler, P.; Düren, M.; Eissner, T.; Etzelmüller, E.; Föhl, K.; Galuska, M.; Gessler, T.; Gutz, E.; Hayrapetyan, A.; Hu, J.; Kröck, B.; Kühn, W.; Kuske, T.; Lange, S.; Liang, Y.; Merle, O.; Metag, V.; Mülhheim, D.; Münchow, D.; Nanova, M.; Novotny, R.; Pitka, A.; Quagli, T.; Rieke, J.; Rosenbaum, C.; Schnell, R.; Spruck, B.; Stenzel, H.; Thöring, U.; Ullrich, M.; Wasem, T.; Werner, M.; Zaunick, H. G.; Ireland, D.; Rosner, G.; Seitz, B.; Deepak, P. N.; Kulkarni, A. V.; Apostolou, A.; Babai, M.; Kavatsyuk, M.; Lemmens, P.; Lindemulder, M.; Löhner, H.; Messchendorp, J.; Schakel, P.; Smit, H.; van der Weele, J. C.; Tiemens, M.; Veenstra, R.; Vejdani, S.; Kalita, K.; Mohanta, D. P.; Kumar, A.; Roy, A.; Sahoo, R.; Sohlbach, H.; Büscher, M.; Cao, L.; Cebulla, A.; Deermann, D.; Dosdall, R.; Esch, S.; Georgadze, I.; Gillitzer, A.; Goerres, A.; Goldenbaum, F.; Grunwald, D.; Herten, A.; Hu, Q.; Kemmerling, G.; Kleines, H.; Kozlov, V.; Lehrach, A.; Leiber, S.; Maier, R.; Nellen, R.; Ohm, H.; Orfanitski, S.; Prasuhn, D.; Prencipe, E.; Ritman, J.; Schadmand, S.; Schumann, J.; Sefzick, T.; Serdyuk, V.; Sterzenbach, G.; Stockmanns, T.; Wintz, P.; Wüstner, P.; Xu, H.; Li, S.; Li, Z.; Sun, Z.; Xu, H.; Rigato, V.; Fissum, S.; Hansen, K.; Isaksson, L.; Lundin, M.; Schröder, B.; Achenbach, P.; Bleser, S.; Cardinali, M.; Corell, O.; Deiseroth, M.; Denig, A.; Distler, M.; Feldbauer, F.; Fritsch, M.; Jasinski, P.; Hoek, M.; Kangh, D.; Karavdina, A.; Lauth, W.; Leithoff, H.; Merkel, H.; Michel, M.; Motzko, C.; Müller, U.; Noll, O.; Plueger, S.; Pochodzalla, J.; Sanchez, S.; Schlimme, S.; Sfienti, C.; Steinen, M.; Thiel, M.; Weber, T.; Zambrana, M.; Dormenev, V. I.; Fedorov, A. A.; Korzihik, M. V.; Missevitch, O. V.; Balanutsa, P.; Balanutsa, V.; Chernetsky, V.; Demekhin, A.; Dolgolenko, A.; Fedorets, P.; Gerasimov, A.; Goryachev, V.; Varentsov, V.; Boukharov, A.; Malyshev, O.; Marishev, I.; Semenov, A.; Konorov, I.; Paul, S.; Grieser, S.; Hergemöller, A. K.; Khoukaz, A.; Köhler, E.; Täschner, A.; Wessels, J.; Dash, S.; Jadhav, M.; Kumar, S.; Sarin, P.; Varma, R.; Chandratre, V. B.; Datar, V.; Dutta, D.; Jha, V.; Kumawat, H.; Mohanty, A. K.; Roy, B.; Yan, Y.; Chinorat, K.; Khanchai, K.; Ayut, L.; Pornrad, S.; Barnyakov, A. Y.; Blinov, A. E.; Blinov, V. E.; Bobrovnikov, V. S.; Kononov, S. A.; Kravchenko, E. A.; Kuyanov, I. A.; Onuchin, A. P.; Sokolov, A. A.; Tikhonov, Y. A.; Atomssa, E.; Hennino, T.; Imre, M.; Kunne, R.; Le Galliard, C.; Ma, B.; Marchand, D.; Ong, S.; Ramstein, B.; Rosier, P.; Tomasi-Gustafsson, E.; Van de Wiele, J.; Boca, G.; Costanza, S.; Genova, P.; Lavezzi, L.; Montagna, P.; Rotondi, A.; Abramov, V.; Belikov, N.; Bukreeva, S.; Davidenko, A.; Derevschikov, A.; Goncharenko, Y.; Grishin, V.; Kachanov, V.; Kormilitsin, V.; Melnik, Y.; Levin, A.; Minaev, N.; Mochalov, V.; Morozov, D.; Nogach, L.; Poslavskiy, S.; Ryazantsev, A.; Ryzhikov, S.; Semenov, P.; Shein, I.; Uzunian, A.; Vasiliev, A.; Yakutin, A.; Yabsley, B.; Bäck, T.; Cederwall, B.; Makónyi, K.; Tegnér, P. E.; von Würtemberg, K. M.; Belostotski, S.; Gavrilov, G.; Izotov, A.; Kashchuk, A.; Levitskaya, O.; Manaenkov, S.; Miklukho, O.; Naryshkin, Y.; Suvorov, K.; Veretennikov, D.; Zhadanov, A.; Rai, A. K.; Godre, S. S.; Duchat, R.; Amoroso, A.; Bussa, M. P.; Busso, L.; De Mori, F.; Destefanis, M.; Fava, L.; Ferrero, L.; Greco, M.; Maggiora, M.; Maniscalco, G.; Marcello, S.; Sosio, S.; Spataro, S.; Zotti, L.; Calvo, D.; Coli, S.; De Remigis, P.; Filippi, A.; Giraudo, G.; Lusso, S.; Mazza, G.; Mingnore, M.; Rivetti, A.; Wheadon, R.; Balestra, F.; Iazzi, F.; Introzzi, R.; Lavagno, A.; Younis, H.; Birsa, R.; Bradamante, F.; Bressan, A.; Martin, A.; Clement, H.; Gålnander, B.; Caldeira Balkeståhl, L.; Calén, H.; Fransson, K.; Johansson, T.; Kupsc, A.; Marciniewski, P.; Pettersson, J.; Schönning, K.; Wolke, M.; Zlomanczuk, J.; Díaz, J.; Ortiz, A.; Vinodkumar, P. C.; Parmar, A.; Chlopik, A.; Melnychuk, D.; Slowinski, B.; Trzcinski, A.; Wojciechowski, M.; Wronka, S.; Zwieglinski, B.; Bühler, P.; Marton, J.; Suzuki, K.; Widmann, E.; Zmeskal, J.; Fröhlich, B.; Khaneft, D.; Lin, D.; Zimmermann, I.; Semenov-Tian-Shansky, K.

    2015-08-01

    Baryon-to-meson Transition Distribution Amplitudes (TDAs) encoding valuable new information on hadron structure appear as building blocks in the collinear factorized description for several types of hard exclusive reactions. In this paper, we address the possibility of accessing nucleon-to-pion ( πN) TDAs from reaction with the future P¯ANDA detector at the FAIR facility. At high center-of-mass energy and high invariant mass squared of the lepton pair q 2, the amplitude of the signal channel admits a QCD factorized description in terms of πN TDAs and nucleon Distribution Amplitudes (DAs) in the forward and backward kinematic regimes. Assuming the validity of this factorized description, we perform feasibility studies for measuring with the P¯ANDA detector. Detailed simulations on signal reconstruction efficiency as well as on rejection of the most severe background channel, i.e. were performed for the center-of-mass energy squared s = 5 GeV2 and s = 10 GeV2, in the kinematic regions 3.0 < q 2 < 4.3 GeV2 and 5 < q 2 GeV2, respectively, with a neutral pion scattered in the forward or backward cone in the proton-antiproton center-of-mass frame. Results of the simulation show that the particle identification capabilities of the P¯ANDA detector will allow to achieve a background rejection factor of 5 · 107 (1 · 107) at low (high) q 2 for s = 5 GeV2, and of 1 · 108 (6 · 106) at low (high) q 2 for s = 10 GeV2, while keeping the signal reconstruction efficiency at around 40%. At both energies, a clean lepton signal can be reconstructed with the expected statistics corresponding to 2 fb-1 of integrated luminosity. The cross sections obtained from the simulations are used to show that a test of QCD collinear factorization can be done at the lowest order by measuring scaling laws and angular distributions. The future measurement of the signal channel cross section with P¯ANDA will provide a new test of the perturbative QCD description of a novel class of hard

  8. Photon-to-pion transition form factor and pion distribution amplitude from holographic QCD

    Energy Technology Data Exchange (ETDEWEB)

    Zuo, Fen [Chinese Academy of Sciences, Institute of High Energy Physics, Beijing (China); Chinese Academy of Sciences, Theoretical Physics Research Center for Science Facilities, Beijing (China); Istituto Nazionale di Fisica Nucleare, Secione di Bari, Bari (Italy); Huang, Tao [Chinese Academy of Sciences, Institute of High Energy Physics, Beijing (China); Chinese Academy of Sciences, Theoretical Physics Research Center for Science Facilities, Beijing (China)

    2012-01-15

    We try to understand the recently observed anomalous behavior of the photon-to-pion transition form factor in the holographic QCD approach. First the holographic description of the anomalous {gamma}{sup *}{gamma}{sup *}{pi}{sup 0} form factor is reviewed and applied to various models. It is pointed out that the holographic identification of the pion mode from the 5D gauge field strength rather than the gauge potential, as first made by Sakai and Sugimoto, naturally reproduces the scaling behavior of various pion form factors. It is also illustrated that in describing the anomalous form factor, the holographic approach is asymptotically dual to the perturbative QCD (pQCD) framework, with the pion mode {pi}(z){proportional_to}z corresponding to the asymptotic pion distribution amplitude. This indicates some inconsistency in light-front holography, since {pi}(z){proportional_to}z would be dual to {phi}(x){proportional_to}{radical}(x(1-x)) there. This apparently contradictory can be attributed to the fact that the holographic wave functions are effective ones, as observed early by Radyushkin. After clarifying these subtleties, we employ the relation between the holographic and the perturbative expressions to study possible asymptotic violation of the transition form factor. It is found that if one require that the asymptotic form factor possess a pQCD-like expression, the pion mode can only be ultraviolet-enhanced by logarithmic factors. The minimally deformed pion mode will then be of the form {pi}(z){proportional_to}zln(z{lambda}){sup -1}. We suppose that this deformation may be due to the coupling of the pion with a nontrivial open string tachyon field, and then the parameter {lambda} will be related to the quark condensate. Interestingly, this pion mode leads immediately to Radyushkin's logarithmic model, which fitted very well the experimental data in the large-Q{sup 2} region. On the other side, the pQCD interpretation with a flat-like pion distribution

  9. Coincidence in the two-photon spectra of Li and Li2 at 735 nm

    Science.gov (United States)

    DeGraffenreid, W.; Sansonetti, Craig J.

    2005-02-01

    A coincidence between the 22S1/2-32S1/2 two-photon transition in the atomic spectrum of 6Li and the X 1Σ+g→ E 1Σ+g two-photon ro-vibrational series of 7Li2 was observed near 735 nm in a heat pipe oven using a tunable laser and thermionic diode detection scheme. The molecular transition obscures one component of the 6Li atomic transition. Selective detection of the atomic transition was obtained by adding an intensity-modulated laser that drives atoms from the 3S to 16P state. The coincident molecular transition and four nearby molecular lines were identified using previously determined Dunham coefficients.

  10. Terahertz-visible two-photon rotational spectroscopy of cold OD-

    CERN Document Server

    Lee, Seunghyun; Lakhmanskaya, Olga; Spieler, Steffen; Endres, Eric S; Geistlinger, Katharina; Kumar, Sunil S; Wester, Roland

    2016-01-01

    We present a method to measure rotational transitions of molecular anions in the terahertz domain by sequential two-photon absorption. Ion excitation by bound-bound terahertz absorption is probed by absorption in the visible on a bound-free transition. The visible frequency is tuned to a state-selective photodetachment transition of the excited anions. This provides a terahertz action spectrum for just few hundred molecular ions. To demonstrate this we measure the two lowest rotational transitions, J=1<-0 and J =2<-1 of OD- anions in a cryogenic 22-pole trap. We obtain rotational transition frequencies of 598596.08(19) MHz for J=1<-0 and 1196791.57(27) MHz for J=2<-1 of OD-, in good agreement with their only previous measurement. This two-photon scheme opens up terahertz rovibrational spectroscopy for a range of molecular anions, in particular for polyatomic and cluster anions.

  11. Two-photon excitation spectra of Cr3 :K2NaScF6

    Science.gov (United States)

    Bartram, R. H.; Wein, G. R.; Hamilton, D. S.; Sliwczuk, U.; Rinzler, A. G.

    Two-photon excitation (TPE) spectra of Cr3+:K2NaScF6 exhibit unexpected features including a forbidden transition, extended progressions, a split zero-phonon line and anomalous polarization anisotropy. These features are explained by departures from standard approximations.

  12. Giant-amplitude, high-work density microactuators with phase transition activated nanolayer bimorphs.

    Science.gov (United States)

    Liu, Kai; Cheng, Chun; Cheng, Zhenting; Wang, Kevin; Ramesh, Ramamoorthy; Wu, Junqiao

    2012-12-12

    Various mechanisms are currently exploited to transduce a wide range of stimulating sources into mechanical motion. At the microscale, simultaneously high amplitude, high work output, and high speed in actuation are hindered by limitations of these actuation mechanisms. Here we demonstrate a set of microactuators fabricated by a simple microfabrication process, showing simultaneously high performance by these metrics, operated on the structural phase transition in vanadium dioxide responding to diverse stimuli of heat, electric current, and light. In both ambient and aqueous conditions, the actuators bend with exceedingly high displacement-to-length ratios up to 1 in the sub-100 μm length scale, work densities over 0.63 J/cm(3), and at frequencies up to 6 kHz. The functionalities of actuation can be further enriched with integrated designs of planar as well as three-dimensional geometries. Combining the superior performance, high durability, diversity in responsive stimuli, versatile working environments, and microscale manufacturability, these actuators offer potential applications in microelectromechanical systems, microfluidics, robotics, drug delivery, and artificial muscles.

  13. Two-Photon Activation of p-Hydroxyphenacyl Phototriggers: Toward Spatially Controlled Release of Diethyl Phosphate and ATP.

    Science.gov (United States)

    Houk, Amanda L; Givens, Richard S; Elles, Christopher G

    2016-03-31

    Two-photon activation of the p-hydroxyphenacyl (pHP) photoactivated protecting group is demonstrated for the first time using visible light at 550 nm from a pulsed laser. Broadband two-photon absorption measurements reveal a strong two-photon transition (>10 GM) near 4.5 eV that closely resembles the lowest-energy band at the same total excitation energy in the one-photon absorption spectrum of the pHP chromophore. The polarization dependence of the two-photon absorption band is consistent with excitation to the same S3 ((1)ππ*) excited state for both one- and two-photon activation. Monitoring the progress of the uncaging reaction under nonresonant excitation at 550 nm confirms a quadratic intensity dependence and that two-photon activation of the uncaging reaction is possible using visible light in the range 500-620 nm. Deprotonation of the pHP chromophore under mildly basic conditions shifts the absorption band to lower energy (3.8 eV) in both the one- and two-photon absorption spectra, suggesting that two-photon activation of the pHP chromophore may be possible using light in the range 550-720 nm. The results of these measurements open the possibility of spatially and temporally selective release of biologically active compounds from the pHP protecting group using visible light from a pulsed laser.

  14. Manipulation of multiple electromagnetically induced two-photon transparency in a six-level atomic system

    Institute of Scientific and Technical Information of China (English)

    Jia Wen-Zhi; Wang Shun-Jin

    2009-01-01

    In the five-level K-type atomic system, by using another control field to couple the excited level of the coupling transition to the sixth higher excited level, a six-level atomic system is constructed. In this system, the multiple electromagnetically induced two-photon transparency has been investigated. What is more, if choosing the parameters of the control fields properly the triple transparency window will reduce to a double one which means that the multiple electromagnetically induced two-photon transparency can be manipulated in this system. The physical interpretation of these phenomena is given in terms of the dressed states and the dark states.

  15. Two Photon Exchange in Impact Parameter Space in the Relativistic Eikonal Approximation for Elastic e - N Scattering

    CERN Document Server

    Alhalholy, Tareq

    2016-01-01

    Using the relativistic Eikonal approximation, we study the one and two photon exchange amplitudes in elastic electron-nucleon scattering for the case of transversely polarized nucleons with unpolarized electrons beam. In our approach, we utilize the convolution theory of Fourier transforms and the transverse charge density in transverse momentum space to evaluate the one and two photon exchange Eikonal amplitudes. The results obtained for the $2\\gamma$ amplitude in impact parameter space are compared to the corresponding 4D case. We show that while the one and two photon cross sections are azimuthally symmetric, the interference term between them is azimuthally asymmetric, which is an indication of an azimuthal single spin asymmetry for proton and neutron which can be attributed to the fact that the nucleon charge density is transversely (azimuthally) distorted in the transverse plane for transversely polarized nucleons. In addition, the calculations of the interference term for proton and neutron show agreem...

  16. Resummation of target mass corrections in two-photon processes twist-two sector

    CERN Document Server

    Belitsky, A V

    2001-01-01

    We develop a formalism for the resummation of target mass corrections in off-forward two-photon amplitudes given by a chronological product of electromagnetic currents, arising in e.g. deeply virtual Compton scattering. The method is based on a relation of composite operators with a definite twist to harmonic tensors, which form an irreducible representation of the Lorentz group. We give an application of the framework for the matrix elements of twist-two operators.

  17. Experimental access to Transition Distribution Amplitudes with the PANDA experiment at FAIR

    Energy Technology Data Exchange (ETDEWEB)

    Singh, B.P. [Aligarh Muslim Univ. (India). Physics Dept.; Erni, W.; Keshelashvili, I. [Basel Univ. (Switzerland); Collaboration: The PANDA Collaboration; and others

    2015-08-15

    Baryon-to-meson Transition Distribution Amplitudes (TDAs) encoding valuable new information on hadron structure appear as building blocks in the collinear factorized description for several types of hard exclusive reactions. In this paper, we address the possibility of accessing nucleon-to-pion (πN) TDAs from anti pp → e{sup +}e{sup -}π{sup 0} reaction with the future PANDA detector at the FAIR facility. At high center-of-mass energy and high invariant mass squared of the lepton pair q{sup 2}, the amplitude of the signal channel anti pp → e{sup +}e{sup -}π{sup 0} admits a QCD factorized description in terms of πN TDAs and nucleon Distribution Amplitudes (DAs) in the forward and backward kinematic regimes. Assuming the validity of this factorized description, we perform feasibility studies for measuring anti pp → e{sup +}e{sup -}π{sup 0} with the PANDA detector. Detailed simulations on signal reconstruction efficiency as well as on rejection of the most severe background channel, i.e. anti pp → π{sup +}π{sup -}π{sup 0} were performed for the center-of-mass energy squared s = 5 GeV{sup 2} and s = 10 GeV{sup 2}, in the kinematic regions 3.0 < q{sup 2} < 4.3 GeV{sup 2} and 5 < q{sup 2} GeV{sup 2}, respectively, with a neutral pion scattered in the forward or backward cone vertical stroke cos θ{sub π{sup 0}} vertical stroke > 0.5 in the proton-antiproton center-of-mass frame. Results of the simulation show that the particle identification capabilities of the PANDA detector will allow to achieve a background rejection factor of 5 . 10{sup 7} (1 . 10{sup 7}) at low (high) q{sup 2} for s = 5 GeV{sup 2}, and of 1 . 10{sup 8} (6 . 10{sup 6}) at low (high) q{sup 2} for s = 10 GeV{sup 2}, while keeping the signal reconstruction efficiency at around 40%. At both energies, a clean lepton signal can be reconstructed with the expected statistics corresponding to 2 fb{sup -1} of integrated luminosity. The cross sections obtained from the simulations are used to

  18. Two-Photon Absorption in Conjugated Energetic Molecules.

    Science.gov (United States)

    Bjorgaard, Josiah A; Sifain, Andrew E; Nelson, Tammie; Myers, Thomas W; Veauthier, Jacqueline M; Chavez, David E; Scharff, R Jason; Tretiak, Sergei

    2016-07-07

    Time-dependent density functional theory (TD-DFT) was used to investigate the relationship between molecular structure and the one- and two-photon absorption (OPA and TPA, respectively) properties of novel and recently synthesized conjugated energetic molecules (CEMs). The molecular structures of CEMs can be strategically altered to influence the heat of formation and oxygen balance, two factors that can contribute to the sensitivity and strength of an explosive material. OPA and TPA are sensitive to changes in molecular structure as well, influencing the optical range of excitation. We found calculated vertical excitation energies to be in good agreement with experiment for most molecules. Peak TPA intensities were found to be significant and on the order of 10(2) GM. Natural transition orbitals for essential electronic states defining TPA peaks of relatively large intensity were used to examine the character of relevant transitions. Modification of molecular substituents, such as additional oxygen or other functional groups, produces significant changes in electronic structure, OPA, and TPA and improves oxygen balance. The results show that certain molecules are apt to undergo nonlinear absorption, opening the possibility for controlled, direct optical initiation of CEMs through photochemical pathways.

  19. Several Organic Salts with High Two-Photon Active

    Institute of Scientific and Technical Information of China (English)

    TIAN, Yu-Peng; JIANG, Min-Hua; WANG, He-Zhou; FANG, Qi

    2001-01-01

    Several organic salts with D-A molecular structure and different counterion have been prepared and experimentally investigated. The two-photon induced frequency-upconverted spectra and two-photon pumped lasing are measured for the organic salt solutions in various solvents. The results indicate that counterions have influence on their stability and lasing property.

  20. Two-photon absorption in arsenic sulfide glasses

    Science.gov (United States)

    Chunaev, D. S.; Snopatin, G. E.; Plotnichenko, V. G.; Karasik, A. Ya.

    2016-10-01

    The two-photon absorption coefficient of 1047-{\\text{nm}} light in {\\text{As}}35{\\text{S}}65 chalcogenide glass has been measured. CW probe radiation has been used to observe the linear absorption in glass induced by two-photon excitation. The induced absorption lifetime was found to be ∼ 2 {\\text{ms}}.

  1. The development of efficient two-photon singlet oxygen sensitizers

    DEFF Research Database (Denmark)

    Nielsen, Christian Benedikt

    The development of efficient two-photon singlet oxygen sensitizers is addressed focusing on organic synthesis. Photophysical measurements were carried out on new lipophilic molecules, where two-photon absorption cross sections and singlet oxygen quantumyields were measured. Design principles...... for making efficient two-photon singlet oxygen sensitizers were then constructed from these results. Charge-transfer in the excited state of the prepared molecules was shown to play a pivotal role in the generationof singlet oxygen. This was established through studies of substituent effects on both...... the singlet oxygen yield and the two-photon absorption cross section, where it was revealed that a careful balancing of the amount of charge transfer present in theexcited state of the sensitizer is necessary to obtain both a high singlet oxygen quantum yield and a high two-photon cross section. An increasing...

  2. Direct Evaluation of Transition Amplitude Using Determinant of Wave Operator in One-Dimensional Potential Scattering System

    Institute of Scientific and Technical Information of China (English)

    Itsuki Banno; Kazumi Fujima

    2007-01-01

    A determinantal formula is developed for direct evaluation of transition amplitude without solving the wave equation in a one-dimensional potential scattering system. Our formulation is based on the principle that a desired quantity can be extracted from the wave operator, which is the master operator maintaining all the information of the system. This principle is tested in a simplified system, I.e., in a one-dimensional potential scattering system. We are now developing a formula for direct evaluation of near-field amplitude to design a system, in which local Geld enhancement is desired.

  3. Synthesis of Two-Photon Materials and Two-Photon Liquid Crystals

    Science.gov (United States)

    Subramaniam, Girija

    2001-01-01

    The duration of the grant was interrupted by two major accidents that the PI met with-- an auto accident in Pasadena, CA during her second summer at JPL which took almost eight months for recovery and a second accident during Fall 2000 that left her in crutches for the entire semester. Further, the time released agreed by the University was not given in a timely fashion. The candidate has been given post-grant expire time off. In spite of all these problems, the PI synthesized a number of new two-photon materials and studied the structure-activity correlation to arrive at the best-optimized structure. The PI's design proved to be one of the best in the sense that these materials has a hitherto unreported two-photon absorption cross section. Many materials based on PI's design was later made by the NASA colleague. This is Phase 1. Phase II of this grant is to orate liquid crystalline nature into this potentially useful materials and is currently in progress. Recent observations of nano- and pico-second response time of homeotropically aligned liquid crystals suggest their inherent potentials to act as laser hardening materials, i.e., as protective devices against short laser pulses. The objective of the current project is to exploit this potential by the synthesis of liquid crystals with high optical nonlinearity and optimizing their performance. The PI is trying structural variations to bring in liquid crystalline nature without losing the high two-photon cross section. Both Phase I and Phase II led to many invited presentations and publications in reputed journals like 'Science' and 'Molecular Crystals'. The list of presentations and reprints are enclosed. Another important and satisfying outcome of this grant is the opportunity that this grant offered to the budding undergraduate scientists to get involved in a visible research of international importance. All the students had a chance to learn a lot during research, had the opportunity to present their work at

  4. Two-photon interference of temporally separated photons

    Science.gov (United States)

    Kim, Heonoh; Lee, Sang Min; Moon, Han Seb

    2016-10-01

    We present experimental demonstrations of two-photon interference involving temporally separated photons within two types of interferometers: a Mach-Zehnder interferometer and a polarization-based Michelson interferometer. The two-photon states are probabilistically prepared in a symmetrically superposed state within the two interferometer arms by introducing a large time delay between two input photons; this state is composed of two temporally separated photons, which are in two different or the same spatial modes. We then observe two-photon interference fringes involving both the Hong-Ou-Mandel interference effect and the interference of path-entangled two-photon states simultaneously in a single interferometric setup. The observed two-photon interference fringes provide simultaneous observation of the interferometric properties of the single-photon and two-photon wavepackets. The observations can also facilitate a more comprehensive understanding of the origins of the interference phenomena arising from spatially bunched/anti-bunched two-photon states comprised of two temporally separated photons within the interferometer arms.

  5. Quantum homodyne tomography of a two-photon Fock state

    CERN Document Server

    Ourjoumtsev, A; Grangier, P; Ourjoumtsev, Alexei; Tualle-Brouri, Rosa; Grangier, Philippe

    2006-01-01

    We present a continuous-variable experimental analysis of a two-photon Fock state of free-propagating light. This state is obtained from a pulsed non-degenerate parametric amplifier, which produces two intensity-correlated twin beams. Counting two photons in one beam projects the other beam in the desired two-photon Fock state, which is analyzed by using a pulsed homodyne detection. The Wigner function of the measured state is clearly negative. We developed a detailed analytic model which allows a fast and efficient analysis of the experimental results.

  6. Quantum homodyne tomography of a two-photon Fock state.

    Science.gov (United States)

    Ourjoumtsev, Alexei; Tualle-Brouri, Rosa; Grangier, Philippe

    2006-06-02

    We present a continuous-variable experimental analysis of a two-photon Fock state of free-propagating light. This state is obtained from a pulsed nondegenerate parametric amplifier, which produces two intensity-correlated twin beams. Counting two photons in one beam projects the other beam in the desired two-photon Fock state, which is analyzed by using a pulsed homodyne detection. The Wigner function of the measured state is clearly negative. We developed a detailed analytic model which allows a fast and efficient analysis of the experimental results.

  7. Scattering of two photons from two distant qubits: exact solution

    Energy Technology Data Exchange (ETDEWEB)

    Laakso, Matti; Pletyukhov, Mikhail [Institute for Theory of Statistical Physics, RWTH Aachen, 52056 Aachen (Germany)

    2015-07-01

    We consider the inelastic scattering of two photons from two qubits separated by an arbitrary distance and coupled to a one-dimensional transmission line. We present an exact, analytical solution to the problem, and use it to explore a particular configuration of qubits which is transparent to single-photon scattering, thus highlighting non-Markovian effects of inelastic two-photon scattering: Strong two-photon interference and momentum dependent photon (anti)bunching. This latter effect can be seen as an inelastic generalization of the Hong-Ou-Mandel effect.

  8. NLO Electroweak Corrections to Higgs Decay to Two Photons

    OpenAIRE

    Actis, Stefano

    2009-01-01

    The recent calculation of the next-to-leading order electroweak corrections to the decay of the Standard Model Higgs boson to two photons in the framework of the complex-mass scheme is briefly summarized.

  9. Standard Model Higgs decay for two Photons in CMS

    CERN Multimedia

    Daniel Denegri

    2000-01-01

    Simulated two-photon mass distribution for SM Higgs and expected background in the CMS PbW04 crystal calorimeter for an integrated luminosity of 10 . 5 pb-1, with detailed simulation of calorimeter response.

  10. Two-photon pumped lead halide perovskite nanowire lasers

    CERN Document Server

    Gu, Zhiyuan; Sun, Wenzhao; Li, Jinakai; Liu, Shuai; Song, Qinghai; Xiao, Shumin

    2015-01-01

    Solution-processed lead halide perovskites have shown very bright future in both solar cells and microlasers. Very recently, the nonlinearity of perovskites started to attract considerable research attention. Second harmonic generation and two-photon absorption have been successfully demonstrated. However, the nonlinearity based perovskite devices such as micro- & nano- lasers are still absent. Here we demonstrate the two-photon pumped nanolasers from perovskite nanowires. The CH3NH3PbBr3 perovskite nanowires were synthesized with one-step solution self-assembly method and dispersed on glass substrate. Under the optical excitation at 800 nm, two-photon pumped lasing actions with periodic peaks have been successfully observed at around 546 nm. The obtained quality (Q) factors of two-photon pumped nanolasers are around 960, and the corresponding thresholds are about 674?J=cm2. Both the Q factors and thresholds are comparable to conventional whispering gallery modes in two-dimensional polygon microplates. Ou...

  11. Pulse-shaping based two-photon FRET stoichiometry.

    Science.gov (United States)

    Flynn, Daniel C; Bhagwat, Amar R; Brenner, Meredith H; Núñez, Marcos F; Mork, Briana E; Cai, Dawen; Swanson, Joel A; Ogilvie, Jennifer P

    2015-02-09

    Förster Resonance Energy Transfer (FRET) based measurements that calculate the stoichiometry of intermolecular interactions in living cells have recently been demonstrated, where the technique utilizes selective one-photon excitation of donor and acceptor fluorophores to isolate the pure FRET signal. Here, we present work towards extending this FRET stoichiometry method to employ two-photon excitation using a pulse-shaping methodology. In pulse-shaping, frequency-dependent phases are applied to a broadband femtosecond laser pulse to tailor the two-photon excitation conditions to preferentially excite donor and acceptor fluorophores. We have also generalized the existing stoichiometry theory to account for additional cross-talk terms that are non-vanishing under two-photon excitation conditions. Using the generalized theory we demonstrate two-photon FRET stoichiometry in live COS-7 cells expressing fluorescent proteins mAmetrine as the donor and tdTomato as the acceptor.

  12. Synthesis of a Series of Novel Organic Compounds with Two-photon Absorption and Two-photon pumped Lasing

    Institute of Scientific and Technical Information of China (English)

    2001-01-01

    A series of novel organic compounds named as CSPI, DPASPI, PSPI DEASPI and HEASPI respectively, with large two-photon absorption has been synthesized and their structures have been determined by 1HNMR and elemental analysis. The highest two-photon pumped (TPP) output /input efficiency is as high as 13.4% for PSPI in DMF with d0 = 0.03 mol/L and the effective two-photon absorption cross section is 8.8′10-48 cm4×s/photon for DPASPI in DMF with d0= 0.05mol/L.

  13. Mass distribution for the two-photon channel

    CERN Multimedia

    ATLAS, collaboration

    2012-01-01

    Mass distribution for the two-photon channel. The strongest evidence for this new particle comes from analysis of events containing two photons. The smooth dotted line traces the measured background from known processes. The solid line traces a statistical fit to the signal plus background. The new particle appears as the excess around 126.5 GeV. The full analysis concludes that the probability of such a peak is three chances in a million.

  14. Generalized Kramers-Heisenberg expressions for stimulated Raman scattering and two-photon absorption

    Science.gov (United States)

    Roslyak, Oleksiy; Marx, Christoph A.; Mukamel, Shaul

    2010-01-01

    The frequency-domain pump-probe signal of a material system interacting with two quantum modes of the radiation field is recast in terms of products of scattering amplitudes (T matrix elements) rather than the third-order susceptibility Im χ(3). The resulting expression offers a more intuitive physical picture for the optical process compared with the semiclassical approach which treats the radiation field as classical. It can be derived and interpreted using closed-time-path-loop diagrams which represent the joint state of the matter and the field for each contribution to the signal. The signal has two components representing stimulated Raman scattering ω1 − ω2 and two-photon absorption ω1 + ω2 two-photon resonances. Both are expressed as nonequi-librium steady-state photon and matter fluxes, as is common in the description of dissipative processes in open quantum systems. PMID:20613889

  15. The effect of large amplitude motions on the transition frequency redshift in hydrogen bonded complexes

    DEFF Research Database (Denmark)

    Mackeprang, Kasper; Kjærgaard, Henrik Grum; Salmi, Teemu

    2014-01-01

    -stretching transition. The model accurately predicts the transition wavenumbers of the vibrations in water dimer compared to experimental values and provides a physical picture that explains the redshift of the hydrogen bonded OH-oscillator. We find that it is unnecessary to include all six intermolecular modes...

  16. Two-Photon Absorption of Metal-Assisted Chromophores.

    Science.gov (United States)

    Li, Xin; Rinkevicius, Zilvinas; Ågren, Hans

    2014-12-09

    Aiming to understand the effect of a metal surface on nonlinear optical properties and the combined effects of surface and solvent environments on such properties, we present a multiscale response theory study, integrated with dynamics of the two-photon absorption of 4-nitro-4'-amino-trans-stilbene physisorbed on noble metal surfaces, considering two such surfaces, Ag(111) and Au(111), and two solvents, cyclohexane and water, as cases for demonstration. A few conclusions of general character could be drawn: While the geometrical change of the chromophore induced by the environment was found to notably alter (diminish) the two-photon absorption cross section in the polar medium, the effects of the metal surface and solvent on the electronic structure of the chromophore surpasses the geometrical effects and leads to a considerably enhanced two-photon absorption cross section in the polar solvent. This enhancement of two-photon absorption arises essentially from the metal charge image induced enlargement of the difference between the dipole moment of the excited state and the ground state. The orientation-dependence of the two-photon absorption is found to connect with the lateral rotation of the chromophore, where the two-photon absorption reaches its maximum when the polarization of the incident light coincides with the long-axis of the chromophore. Our results demonstrate a distinct enhancement of the two-photon absorption by a metal surface and a polar medium and envisage the employment of metal-chromophore composite materials for future development of nonlinear optical materials with desirable properties.

  17. Improved empirical parametrizations of the $\\gamma^\\ast N \\to N(1535)$ transition amplitudes and the Siegert's theorem

    CERN Document Server

    Ramalho, G

    2016-01-01

    Some empirical parametrizations of the $\\gamma^\\ast N \\to N(1535)$ transition amplitudes violates the Siegert's theorem, that relates the longitudinal and the transverse amplitudes, in the pseudo-threshold limit (nucleon and resonance at rest). In the case of the electromagnetic transition from the nucleon (mass $M$) to the resonance $N(1525)$ (mass $M_R$), the Siegert's theorem is sometimes expressed by the relation $|{\\bf q}| A_{1/2}= \\lambda S_{1/2}$ in the pseudo-threshold limit, when the photon momentum $|{\\bf q}|$ vanishes, and $\\lambda = \\sqrt{2} (M_R -M)$. In this article, we argue that the Siegert's theorem should be expressed by the relation $A_{1/2} = \\lambda \\frac{S_{1/2}}{ |{\\bf q}|}$, in the limit $|{\\bf q}| \\to 0$. This result is a consequence of the relation $S_{1/2} \\propto |{\\bf q}|$, when $|{\\bf q}| \\to 0$, as suggested by the analysis of the transition form factors and by the orthogonality between the nucleon and $N(1535)$ states. We propose then new empirical parametrizations for the $\\ga...

  18. Three-dimensional microfabrication using two-photon polymerization

    Science.gov (United States)

    Cumpston, Brian H.; Ehrlich, Jeffrey E.; Kuebler, Stephen M.; Lipson, Matthew; Marder, Seth R.; McCord-Maughon, D.; Perry, Joseph W.; Roeckel, Harold; Rumi, Maria Cristina

    1998-09-01

    Photopolymerization initiated by the simultaneous absorption of two photons is unique in its ability to produce complex three-dimensional (3D) structures from a single, thick photopolymer film. Strong 3D confinement of the polymerization process is not possible in other polymer microfabrication techniques such as LIGA, rapid prototyping, and conventional photoresist technology. Two-photon polymerization also permits the fabrication of 3D structures and the definition of lithographic features on non-planar surfaces. We have developed a wide array of chromophores which hold great promise for 3D microfabrication, as well as other applications, such as two-photon fluorescence imaging and 3D optical data storage. These materials are based on a donor- (pi) -donor, donor-acceptor-donor, or acceptor-donor-acceptor structural motif. The magnitude of the two-photon absorption cross-section, (delta) , and the position of the two-photon absorption maximum, (lambda) (2)max, can be controlled by varying the length of the conjugated bridge and by varying the strength of the donor/acceptor groups. In this way, chromophores have been developed which exhibit strong two- photon absorption in the range of 500 - 975 nm, in some cases as high as 4400 X 10-50 cm4 s/photon-molecule. In the case of donor-(pi) -donor structures, quantum-chemical calculations show that the large absorption cross-sections arise from the symmetric re-distribution of charge from the donor end-groups to the conjugated bridge, resulting in an electronic excited-state which is more delocalized than the ground state. For many of these molecules, two-photon excitation populates a state which is sufficiently reducing that a charge transfer reaction can occur with acrylate monomers. The efficiency of these processes can be described using Marcus theory. Under suitable conditions, such reactions can induce radical polymerization of acrylate resins. Polymerization rates have been measured, and we show that these two-photon

  19. Two-photon flow cytometer with laser scanning Bessel beams

    Science.gov (United States)

    Wang, Yongdong; Ding, Yu; Ray, Supriyo; Paez, Aurelio; Xiao, Chuan; Li, Chunqiang

    2016-03-01

    Flow cytometry is an important technique in biomedical discovery for cell counting, cell sorting and biomarker detection. In vivo flow cytometers, based on one-photon or two-photon excited fluorescence, have been developed for more than a decade. One drawback of laser beam scanning two-photon flow cytometer is that the two-photon excitation volume is fairly small due to the short Rayleigh range of a focused Gaussian beam. Hence, the sampling volume is much smaller than one-photon flow cytometry, which makes it challenging to count or detect rare circulating cells in vivo. Bessel beams have narrow intensity profiles with an effective spot size (FWHM) as small as several wavelengths, making them comparable to Gaussian beams. More significantly, the theoretical depth of field (propagation distance without diffraction) can be infinite, making it an ideal solution as a light source for scanning beam flow cytometry. The trade-off of using Bessel beams rather than a Gaussian beam is the fact that Bessel beams have small concentric side rings that contribute to background noise. Two-photon excitation can reduce this noise, as the excitation efficiency is proportional to intensity squared. Therefore, we developed a two-photon flow cytometer using scanned Bessel beams to form a light sheet that intersects the micro fluidic channel.

  20. Confocal and Two-Photon Microscopy: Foundations, Applications and Advances

    Science.gov (United States)

    Diaspro, Alberto

    2001-11-01

    Confocal and Two-Photon Microscopy Foundations, Applications, and Advances Edited by Alberto Diaspro Confocal and two-photon fluorescence microscopy has provided researchers with unique possibilities of three-dimensional imaging of biological cells and tissues and of other structures such as semiconductor integrated circuits. Confocal and Two-Photon Microscopy: Foundations, Applications, and Advances provides clear, comprehensive coverage of basic foundations, modern applications, and groundbreaking new research developments made in this important area of microscopy. Opening with a foreword by G. J. Brakenhoff, this reference gathers the work of an international group of renowned experts in chapters that are logically divided into balanced sections covering theory, techniques, applications, and advances, featuring: In-depth discussion of applications for biology, medicine, physics, engineering, and chemistry, including industrial applications Guidance on new and emerging imaging technology, developmental trends, and fluorescent molecules Uniform organization and review-style presentation of chapters, with an introduction, historical overview, methodology, practical tips, applications, future directions, chapter summary, and bibliographical references Companion FTP site with full-color photographs The significant experience of pioneers, leaders, and emerging scientists in the field of confocal and two-photon excitation microscopy Confocal and Two-Photon Microscopy: Foundations, Applications, and Advances is invaluable to researchers in the biological sciences, tissue and cellular engineering, biophysics, bioengineering, physics of matter, and medicine, who use these techniques or are involved in developing new commercial instruments.

  1. Single-cycle Terahertz Pulses with >0.2 V/A Field Amplitudes via Coherent Transition Radiation

    Energy Technology Data Exchange (ETDEWEB)

    Daranciang, Dan; /Stanford U., Chem. Dept.; Goodfellow, John; /Stanford U. Materials Sci. Dept.; Fuchs, Matthias; /SIMES, Stanford /SLAC, PULSE; Wen, Haidan; /ANL, APS; Ghimire, Shambhu; /SLAC, PULSE; Reis, David A.; /SIMES, Sanford /SLAC, PULSE /Stanford U., Appl. Phys. Dept.; Loos, Henrik; Fisher, Alan S.; /SLAC, LCLS; Lindenberg, Aaron M.; /Stanford U. Materials Sci. Dept. /SIMES, Stanford /SLAC, PULSE

    2012-02-15

    We demonstrate terahertz pulses with field amplitudes exceeding 0.2 V/{angstrom} generated by coherent transition radiation. Femtosecond, relativistic electron bunches generated at the Linac Coherent Light Source are passed through a beryllium foil, and the emitted radiation is characterized as a function of the bunch duration and charge. Broadband pulses centered at a frequency of 10 THz with energies of 140 {mu}J are measured. These far-below-bandgap pulses drive a nonlinear optical response in a silicon photodiode, with which we perform nonlinear autocorrelations that yield information regarding the terahertz temporal profile. Simulations of the spatiotemporal profile agree well with experimental results.

  2. Nonlinear quantitative photoacoustic tomography with two-photon absorption

    CERN Document Server

    Ren, Kui

    2016-01-01

    Two-photon photoacoustic tomography (TP-PAT) is a non-invasive optical molecular imaging modality that aims at inferring two-photon absorption property of heterogeneous media from photoacoustic measurements. In this work, we analyze an inverse problem in quantitative TP-PAT where we intend to reconstruct optical coefficients in a semilinear elliptic PDE, the mathematical model for the propagation of near infra-red photons in tissue-like optical media with two-photon absorption, from the internal absorbed energy data. We derive uniqueness and stability results on the reconstructions of single and multiple optical coefficients, and present some numerical reconstruction results based on synthetic data to complement the theoretical analysis.

  3. Two-photon interference between disparate sources for quantum networking

    Science.gov (United States)

    McMillan, A. R.; Labonté, L.; Clark, A. S.; Bell, B.; Alibart, O.; Martin, A.; Wadsworth, W. J.; Tanzilli, S.; Rarity, J. G.

    2013-06-01

    Quantum networks involve entanglement sharing between multiple users. Ideally, any two users would be able to connect regardless of the type of photon source they employ, provided they fulfill the requirements for two-photon interference. From a theoretical perspective, photons coming from different origins can interfere with a perfect visibility, provided they are made indistinguishable in all degrees of freedom. Previous experimental demonstrations of such a scenario have been limited to photon wavelengths below 900 nm, unsuitable for long distance communication, and suffered from low interference visibility. We report two-photon interference using two disparate heralded single photon sources, which involve different nonlinear effects, operating in the telecom wavelength range. The measured visibility of the two-photon interference is 80 +/- 4%, which paves the way to hybrid universal quantum networks.

  4. Enhanced two-photon absorption using true thermal light

    CERN Document Server

    Jechow, Andreas; Kurzke, Henning; Heuer, Axel; Menzel, Ralf

    2013-01-01

    Two-photon excited fluorescence (TPEF) is a standard technique in modern microscopy but still affected by photo-damage of the probe. It was proposed that TPEF can be enhanced by using entangled photons, but has proven to be challenging. Recently it was shown that some features of entangled photons can be mimicked with thermal light, which finds application in ghost imaging, sub-wavelength lithography and metrology. Here, we utilize true thermal light from a super-luminescence diode to demonstrate enhanced TPEF compared to coherent light using two common fluorophores and luminescent quantum dots. We find that the two-photon absorption rate is directly proportional to the measured degree of second-order coherence, as predicted by theory. Our results show that photon bunching can be exploited in two-photon microscopy with the photon statistic providing a new degree of freedom.

  5. Two-photon entanglement generation: different Bell states within the linewidth of phase-matching.

    Science.gov (United States)

    Brida, G; Chekhova, M V; Genovese, M; Krivitsky, L A

    2007-08-06

    It is shown that for a phase-matched nonlinear process producing entangled states, different Bell states are generated for different mismatch values. In particular, generation of the singlet Bell state is demonstrated within the natural linewidth of collinear frequency-degenerate type-II spontaneous parametric down-conversion (SPDC) without the o-e delay compensation. The singlet state can be filtered out by spectral selection or by the time selection of the two-photon amplitude at the output of a dispersive fibre. The effect is of considerable importance for fibre quantum communication.

  6. Coherence Loss of Two-Photon Jaynes-Cummings Model in Dispersive Approximation

    Institute of Scientific and Technical Information of China (English)

    ZHOU Ling; GUO Yan-Qing; SONG He-Shan; LI Chong

    2004-01-01

    Completely solving the dissipative dynamics of nonlinear Jaynes-Cumming model is a very difficult task.In our recent work (Phys. Lett. A284 (2001) 156), we just obtained analytical results of the field dissipative dynamics of the nonlinear JCM. In the present paper, employing the perturbative expansion of master equation, we obtain the density operator of the system (field +atom). The coherence losses of the system and of the atom are investigated when two-photon process is involved. We also study the effect of different atomic initial states and the influence of the field amplitude on the atomic coherence loss.

  7. Enhancement of Two-photon Absorption by Ce3+ Sensitization in Organic Dyes

    Institute of Scientific and Technical Information of China (English)

    LI Jian-fu; SUN Cheng-lin; ZHOU Hai-ling; XU Li-hua; YANG Qing-xin; JIANG Zhan-kui

    2007-01-01

    The two-photon absorption (TPA) and TPA-induced frequency upconversion emission properties of the dyes4-[P-(dicyanoethylamino) crystal]-N-methypyrdinium iodide and the complex of 4-[ P-(dicyanoethylamino) crystal]-N-methypyrdinium iodide and Ce( NO3 )3 were experimentally studied. It was found that the TPA cross section for the dye sensitized by Ce3+ is two factors larger than that of the dye without being sensitized. A three-level system model of the dye molecules was used to analyze the enhancement of TPA by the sensitizer Ce3+, which indicated that the sensitizer results in the increase of the transition dipole moment from the one-photon allowed excited state(1Bu)to the two-photon allowed excited state(2Ag).

  8. Cascaded two-photon spectroscopy of Yb atoms with a transportable effusive atomic beam apparatus.

    Science.gov (United States)

    Song, Minsoo; Yoon, Tai Hyun

    2013-02-01

    We present a transportable effusive atomic beam apparatus for cascaded two-photon spectroscopy of the dipole-forbidden transition (6s(2)(1)S0↔ 6s7s (1)S0) of Yb atoms. An ohmic-heating effusive oven is designed to have a reservoir volume of 1.6 cm(3) and a high degree of atomic beam collimation angle of 30 mrad. The new atomic beam apparatus allows us to detect the spontaneously cascaded two-photons from the 6s7s(1)S0 state via the intercombination 6s6p(3)P1 state with a high signal-to-noise ratio even at the temperature of 340 °C. This is made possible in our apparatus because of the enhanced atomic beam flux and superior detection solid angle.

  9. Two-photon interference with non-identical photons

    Science.gov (United States)

    Liu, Jianbin; Zhou, Yu; Zheng, Huaibin; Chen, Hui; Li, Fu-li; Xu, Zhuo

    2015-11-01

    Two-photon interference with non-identical photons is studied based on the superposition principle in Feynman's path integral theory. The second-order temporal interference pattern is observed by superposing laser and pseudothermal light beams with different spectra. The reason why there is two-photon interference for photons of different spectra is that non-identical photons can be indistinguishable for the detection system when Heisenberg's uncertainty principle is taken into account. These studies are helpful to understand the second-order interference of light in the language of photons.

  10. Two-Photon Total Annihilation of Molecular Positronium

    CERN Document Server

    Pérez-Ríos, Jesús; Greene, Chris H

    2014-01-01

    The rate for complete two-photon annihilation of molecular positronium Ps$_{2}$ is reported. This decay channel involves a four-body collision among the fermions forming Ps$_{2}$, and two photons of 1.022 MeV, each, as the final state. The quantum electrodynamics result for the rate of this process is found to be $\\Gamma_{Ps_{2} \\rightarrow \\gamma\\gamma}$ = 9.0 $\\times 10^{-12}$ s$^{-1}$. This decay channel completes the most comprehensive decay chart for Ps$_{2}$ up to date.

  11. Two-photon Compton process in pulsed intense laser fields

    CERN Document Server

    Seipt, D

    2012-01-01

    Based on strong-field QED in the Furry picture we use the Dirac-Volkov propagator to derive a compact expression for the differential emission probability of the two-photon Compton process in a pulsed intense laser field. The relation of real and virtual intermediate states is discussed, and the natural regularization of the on-shell contributions due to the finite laser pulse is highlighted. The inclusive two-photon spectrum is two orders of magnitude stronger than expected from a perturbative estimate.

  12. A fluorescent benzothiazole probe with efficient two-photon absorption

    Science.gov (United States)

    Echevarria, Lorenzo; Moreno, Iván; Camacho, José; Salazar, Mary Carmen; Hernández, Antonio

    2012-11-01

    In this work, we report the two-photon absorption of 2-[4-(dimethylamino)phenyl]-1,3-benzothiazole-6-carbonitrile (DBC) in DMSO solution pumping at 779 nm with a 10 ns pulse laser-Nd:YAG system. The obtained two-photon absorption cross-section in DBC (407 ± 18 GM) is considerably high. Because DBC is a novel compound and have high values of fluorescence quantum yield, this result is expected to have an impact in biomolecules detection, diagnosis and treatment of cancer. Similar structures have previously been reported to show remarkable antitumour effects.

  13. Two-photon rotational action spectroscopy of cold OH- at 1 ppb accuracy.

    Science.gov (United States)

    Jusko, Pavol; Asvany, Oskar; Wallerstein, Ann-Christin; Brünken, Sandra; Schlemmer, Stephan

    2014-06-27

    The fundamental rotational transition J = 1←0 of the anion OH(-) has been measured by cooling mass-selected OH(-) ions to 10 K in a 22-pole ion trap and applying a novel rotational-rovibrational two-photon scheme. A transition frequency of (1  123 101.0410 ± 0.0014)  MHz was obtained with so far unprecedented accuracy. The general application of the presented action-spectroscopy scheme to other anions and cations is discussed.

  14. Quantum manifestation of systems on the macro-scale – the concept of transition state and transition amplitude wave

    Indian Academy of Sciences (India)

    Ram K Varma

    2007-06-01

    Quantum effects which have usually been associated with micro-scale phenomena can also arise on the macro-scale in situations other than the well-known macro-quantum phenomena of superconductivity and superfluidity. Such situations have been shown here to arise in processes involving inelastic scattering with bound or partially bound systems (not bound in all degrees of freedom), and the macro-quantum behaviour is associated with the state of the total system in transition in the process of scattering. Such a state is designated as a `transition-state'. It is pointed out that we have already observed such manifestations for a particular system, the charged particles in a magnetic field where interference effects involving macro-scale matter waves along the magnetic field have been reported [R K Varma et al, Phys. Rev. E65, 026503 (2002)].

  15. Finite Amplitude Method for Charge-Changing Transitions in Axially-Deformed Nuclei

    CERN Document Server

    Mustonen, M T; Zenginerler, Z; Engel, J

    2014-01-01

    We describe and apply a version of the finite amplitude method for obtaining the charge-changing nuclear response in the quasiparticle random phase approximation. The method is suitable for calculating strength functions and beta-decay rates, both allowed and forbidden, in axially-deformed open-shell nuclei. We demonstrate the speed and versatility of the code through a preliminary examination of the effects of tensor terms in Skyrme functionals on beta decay in a set of spherical and deformed open-shell nuclei. Like the isoscalar pairing interaction, the tensor terms systematically increase allowed beta-decay rates. This finding generalizes previous work in semimagic nuclei and points to the need for a comprehensive study of time-odd terms in nuclear density functionals.

  16. System Size Dependence of Finite-Amplitude Thresholds for Transition to Turbulence in Taylor-Couette Flow

    Science.gov (United States)

    Borrero-Echeverrry, Daniel; Morrison, Benjamin; Peairs, Evan

    2015-11-01

    Despite centuries of study, fluid dynamicists are still unable to explain why a large class of flows, including pipe flow and plane Couette flow, become turbulent. Hydrodynamic stability theory predicts these flows should be stable to infinitesimal perturbations, which means finite-amplitude perturbations need to be applied to destabilize them. We present the results of a series of experiments studying such subcritical transitions to turbulence in linearly-stable configurations of Taylor-Couette flow. In particular, we discuss how the stability of these flows depends on the size and duration of the applied perturbation as the aspect ratio of the experimental apparatus is varied. We show that for experimental configurations where the end caps rotate with the outer cylinder, the stability of the flow is enhanced at small aspect ratios. We find that at sufficiently high Reynolds numbers, perturbations must exceed a critical amplitude before the transition to turbulence can be triggered. The scaling of this threshold with Re appears to be different than that which has been reported for other linearly-stable shear flows. This work was supported by Reed College's Summer Scholarship Fund, the James Borders Physics Student Fellowship, and the Reed College Science Research Fellowship. We also thank H.L. Swinney, who kindly donated the apparatus used in these experiments.

  17. Wave structure and flow amplitude-frequency characteristics in the turbine nozzle lattice in the presence of phase transition

    Science.gov (United States)

    Gribin, V. G.; Gavrilov, I. Yu.; Tishchenko, A. A.; Tishchenko, V. A.; Alekseev, R. A.

    2017-05-01

    This paper is devoted to the wave structure of a flow at its near- and supersonic velocities in a flat turbine cascade of profiles in the zone of phase transitions. The main task was investigation of the mechanics of interaction of the condensation jump with the adiabatic jumps of packing in a change of the initial condition of the flow. The obtained results are necessary for verification of the calculation models of the moisture-steam flow in the elements of lotic parts of the steam turbines. The experimental tests were made on a stand of the wet steam contour (WSC-2) in the Moscow Power Engineering Institute (MPEI, National Research University) at various initial states of steam in a wide range of Mach numbers. In the investigation of the wave structure, use was made of an instrument based on the Schlieren-method principle. The amplitude-frequency characteristics of the flow was found by measurement of static pressure pulsations by means of the piezo resistive sensors established on a bandage plate along the bevel cut of the cascade. It is shown that appearance of phase transitions in the bevel cut of the nozzle turbine cascade leads to a change in the wave structure of the flow. In case of condensation jump, the system of adiabatic jumps in the bevel cut of the cascade becomes nonstationary, and the amplitude-frequency characteristics of static pressure pulsations are restructured. In this, a change in the frequency pulsations of pressure and amplitude takes place. It is noted that, at near-sonic speeds of the flow and the state of saturation at the input, the low-frequency pulsations of static pressure appear that lead to periodic disappearance of the condensation jump and of the adiabatic jump. As a result, in this mode, the flow discharge variations take place.

  18. Internal conversions in Higgs decays to two photons

    OpenAIRE

    Firan, Ana; Stroynowski, Ryszard

    2007-01-01

    We evaluate the partial widths for internal conversions in the Higgs decays to two photons. For the Higgs masses of interest at LHC in the range of 100-150 GeV, the conversions to pairs of fermions represent significant fraction of Higgs decays.

  19. Two-Photon-Pumped Perovskite Semiconductor Nanocrystal Lasers.

    Science.gov (United States)

    Xu, Yanqing; Chen, Qi; Zhang, Chunfeng; Wang, Rui; Wu, Hua; Zhang, Xiaoyu; Xing, Guichuan; Yu, William W; Wang, Xiaoyong; Zhang, Yu; Xiao, Min

    2016-03-23

    Two-photon-pumped lasers have been regarded as a promising strategy to achieve frequency up-conversion for situations where the condition of phase matching required by conventional approaches cannot be fulfilled. However, their practical applications have been hindered by the lack of materials holding both efficient two-photon absorption and ease of achieving population inversion. Here, we show that this challenge can be tackled by employing colloidal nanocrystals of perovskite semiconductors. We observe highly efficient two-photon absorption (with a cross section of 2.7 × 10(6) GM) in toluene solutions of CsPbBr3 nanocrystals that can excite large optical gain (>500 cm(-1)) in thin films. We have succeeded in demonstrating stable two-photon-pumped lasing at a remarkable low threshold by coupling CsPbBr3 nanocrystals with microtubule resonators. Our findings suggest perovskite nanocrystals can be used as excellent gain medium for high-performance frequency-up-conversion lasers toward practical applications.

  20. Two-photon absorbing porphyrins for oxygen microscopy (Conference Presentation)

    Science.gov (United States)

    Esipova, Tatiana V.; Vinogradov, Sergei A.

    2016-03-01

    The ability to quantify oxygen in vivo in 3D with high spatial and temporal resolution is invaluable for many areas of the biomedical science, including ophthalmology, neuroscience, cancer and stem biology. An optical method based on oxygen-dependent quenching of phosphorescence is being developed, that allows quantitative minimally invasive real-time imaging of partial pressure of oxygen (pO2) in tissue. In the past, dendritically protected phosphorescent oxygen probes with controllable quenching parameters and defined bio-distributions have been developed. More recently our probe strategy has extended to encompass two-photon excitable oxygen probes, which brought about first demonstrations of two-photon phosphorescence lifetime microscopy (2PLM) of oxygen in vivo, providing new valuable information for neuroscience and stem cell biology. However, current two-photon oxygen probes suffer from a number of limitations, such as low brightness and high cost of synthesis, which dramatically reduce imaging performance and limit usability of the method. Here we present an approach to new bright phosphorescent chromophores with internally enhanced two-photon absorption cross-sections, which pave a way to novel proves for 2PLM. In addition to substantial increase in performance, the new probes can be synthesized by much more efficient methods, thereby greatly reducing the cost of the synthesis and making the technique accessible to a broader range of researchers across different fields.

  1. Direct Writing of Photonic Structures by Two-Photon Polymerization

    Directory of Open Access Journals (Sweden)

    Li Yan

    2013-11-01

    Full Text Available Single-mode dielectric-loaded surface plasmon-polariton nanowaveguides with strong mode confinement at excitation wavelength of 830 nm and high-Q polymer whispering gallery mode microcavities with surface roughness less than 12 nm have been directly written by two-photon polymerization, which pave the way to fabricate 3D plasmonic photonic structures by direct laser writing.

  2. Coincidence in the two-photon spectra of Li and Li{sub 2} at 735 nm

    Energy Technology Data Exchange (ETDEWEB)

    DeGraffenreid, W [Department of Physics and Astronomy, California State University, Sacramento, Sacramento, CA 95819-6041 (United States); Sansonetti, Craig J [National Institute of Standards and Technology, Gaithersburg, MD 20899-8422 (United States)

    2005-02-28

    A coincidence between the 2{sup 2}S{sub 1/2}-3{sup 2}S{sub 1/2} two-photon transition in the atomic spectrum of {sup 6}Li and the X {sup 1}{sigma}{sup +}{sub g}{yields} E {sup 1}{sigma}{sup +}{sub g} two-photon ro-vibrational series of {sup 7}Li{sub 2} was observed near 735 nm in a heat pipe oven using a tunable laser and thermionic diode detection scheme. The molecular transition obscures one component of the {sup 6}Li atomic transition. Selective detection of the atomic transition was obtained by adding an intensity-modulated laser that drives atoms from the 3S to 16P state. The coincident molecular transition and four nearby molecular lines were identified using previously determined Dunham coefficients.

  3. Antiproton–to–electron mass ratio determined by two-photon laser spectroscopy of antiprotonic helium atoms

    Directory of Open Access Journals (Sweden)

    Sótér A.

    2014-03-01

    Full Text Available The ASACUSA collaboration of CERN has recently carried out two-photon laser spectroscopy of antiprotonic helium atoms. Three transition frequencies were determined with fractional precisions of 2.3–5 parts in 109. By comparing the results with three-body QED calculations, the antiproton-to-electron mass ratio was determined as 1836.1526736(23.

  4. Calculation of the spatial resolution in two-photon absorption spectroscopy applied to plasma diagnosis

    Energy Technology Data Exchange (ETDEWEB)

    Garcia-Lechuga, M. [Departamento de Física Teórica, Atómica y Óptica, Universidad de Valladolid, 47011-Valladolid (Spain); Laser Processing Group, Instituto de Óptica “Daza de Valdés,” CSIC, 28006-Madrid (Spain); Fuentes, L. M. [Departamento de Física Aplicada, Universidad de Valladolid, 47011-Valladolid (Spain); Grützmacher, K.; Pérez, C., E-mail: concha@opt.uva.es; Rosa, M. I. de la [Departamento de Física Teórica, Atómica y Óptica, Universidad de Valladolid, 47011-Valladolid (Spain)

    2014-10-07

    We report a detailed characterization of the spatial resolution provided by two-photon absorption spectroscopy suited for plasma diagnosis via the 1S-2S transition of atomic hydrogen for optogalvanic detection and laser induced fluorescence (LIF). A precise knowledge of the spatial resolution is crucial for a correct interpretation of measurements, if the plasma parameters to be analysed undergo strong spatial variations. The present study is based on a novel approach which provides a reliable and realistic determination of the spatial resolution. Measured irradiance distribution of laser beam waists in the overlap volume, provided by a high resolution UV camera, are employed to resolve coupled rate equations accounting for two-photon excitation, fluorescence decay and ionization. The resulting three-dimensional yield distributions reveal in detail the spatial resolution for optogalvanic and LIF detection and related saturation due to depletion. Two-photon absorption profiles broader than the Fourier transform-limited laser bandwidth are also incorporated in the calculations. The approach allows an accurate analysis of the spatial resolution present in recent and future measurements.

  5. Study of Two-Photon Transistions in CLEO III Upsilon(3S) Data

    CERN Document Server

    Cinabro, D; McGee, S; Bornheim, A; Lipeles, E; Pappas, S P; Shapiro, A; Sun, W M; Weinstein, A J; Mahapatra, R; Briere, R A; Chen, G P; Ferguson, T; Tatishvili, G T; Vogel, H; Adam, N E; Alexander, J P; Berkelman, K; Boisvert, V; Cassel, David G; Drell, P S; Duboscq, J E; Ecklund, K M; Ehrlich, R; Galik, R S; Gibbons, L; Gittelman, B; Gray, S W; Hartill, D L; Heltsley, B K; Hsu, L; Jones, C D; Kandaswamy, J; Kreinick, D L; Magerkurth, A; Mahlke-Krüger, H; Meyer, T O; Mistry, N B; Nordberg, E; Patterson, J R; Peterson, D; Pivarski, J; Riley, D; Sadoff, A J; Schwarthoff, H; Shepherd, M R; Thayer, J G; Urner, D; Viehhauser, G; Warburton, A; Weinberger, M; Athar, S B; Avery, P; Breva-Newell, L; Potlia, V; Stöck, H; Yelton, J; Brandenburg, G; Kim, D Y J; Wilson, R; Benslama, K; Eisenstein, B I; Ernst, J; Gollin, G D; Hans, R M; Karliner, I; Lowrey, N; Plager, C; Sedlack, C; Selen, M; Thaler, J J; Williams, J; Edwards, K W; Ammar, R; Besson, D; Zhao, X; Anderson, S; Frolov, V V; Kubota, Y; Lee, S J; Li, S Z; Poling, R A; Smith, A; Stepaniak, C J; Urheim, J; Metreveli, Z V; Seth, K K; Tomaradze, A G; Zweber, P; Ahmed, S; Alam, M S; Jian, L; Saleem, M; Wappler, F; Eckhart, E; Gan, K K; Gwon, C; Hart, T; Honscheid, K; Hufnagel, D; Kagan, H; Kass, R; Pedlar, T K; Thayer, J B; Von Törne, E; Wilksen, T; Zoeller, M M; Muramatsu, H; Richichi, S J; Severini, H; Skubic, P L; Dytman, S A; Müller, J A; Nam, S; Savinov, V; Chen, S; Hinson, J W; Lee, J; Miller, D H; Pavlunin, V; Shibata, E I; Shipsey, I P J; Cronin-Hennessy, D; Lyon, A L; Park, C S; Park, W; Thorndike, E H; Coan, T E; Gao, Y S; Liu, F; Maravin, Y; Stroynowski, R; Artuso, M; Boulahouache, C; Bukin, K; Dambasuren, E; Khroustalev, K; Mountain, R; Nandakumar, R; Skwarnicki, T; Stone, S; Wang, J C; Mahmood, A H; Csorna, S E; Danko, I

    2002-01-01

    We have studied two-photon transitions from Upsilon(3S) decays recorded by the CLEO-III detector in exclusive events with two photons and either two electrons or two muons. We obtain precision measurements of the chi_b(2P_J) masses for J=2 and J=1. The transition rates for all three spin states of the 2P triplet are measured with improved precision which leads to a better determination of their hadronic width ratios. We also observe rare transitions via the chi_b(1P) states. The measured rates for these transitions allow a determination of , the E1 matrix element, which is more sensitive to the structure of the bb states than the matrix element which dominates the radiative decays of the Upsilon(3S) state. We also present first upper limits on the branching ratios for Upsilon(3S)-> pi0 Upsilon(2S) Upsilon(3S) -> pi0 Upsilon(1S) and a new limit for the branching ratio for Upsilon(3S) -> eta Upsilon(1S).

  6. Transition to kinetic turbulence at proton scales driven by large-amplitude kinetic Alfvén fluctuations

    Science.gov (United States)

    Valentini, F.; Vásconez, C. L.; Pezzi, O.; Servidio, S.; Malara, F.; Pucci, F.

    2017-02-01

    Space plasmas are dominated by the presence of large-amplitude waves, large-scale inhomogeneities, kinetic effects and turbulence. Beside the homogeneous turbulence, the generation of small scale fluctuations can take place also in other realistic configurations, namely, when perturbations superpose to an inhomogeneous background magnetic field. When an Alfvén wave propagates in a medium where the Alfvén speed varies in a direction transverse to the mean field, it undergoes phase-mixing, which progressively bends wavefronts, generating small scales in the transverse direction. As soon as transverse scales become of the order of the proton inertial length dp, kinetic Alfvén waves (KAWs) are naturally generated. KAWs belong to the branch of Alfvén waves and propagate almost perpendicularly to the ambient magnetic field, at scales close to dp. Many numerical, observational and theoretical works have suggested that these fluctuations may play a determinant role in the development of the solar-wind turbulent cascade. In the present paper, the generation of large amplitude KAW fluctuations in inhomogeneous background, as well as their effect on the protons, have been investigated by means of hybrid Vlasov-Maxwell direct numerical simulations. Imposing a pressure balanced magnetic shear, the kinetic dynamics of protons has been investigated by varying both the magnetic configuration and the amplitude of the initial perturbations. Of particular interest here is the transition from quasi-linear to turbulent regimes, focusing in particular on the development of important non-Maxwellian features in the proton distribution function driven by KAW fluctuations. Several indicators to quantify the deviations of the protons from thermodynamic equilibrium are presented. These numerical results might help to explain the complex dynamics of inhomogeneous and turbulent astrophysical plasmas, such as the heliospheric current sheet, the magnetospheric boundary layer, and the solar

  7. Two-photon absorption of Zn(II) octupolar molecules.

    Science.gov (United States)

    Mazzucato, Simone; Fortunati, Ilaria; Scolaro, Sara; Zerbetto, Michele; Ferrante, Camilla; Signorini, Raffaella; Pedron, Danilo; Bozio, Renato; Locatelli, Danika; Righetto, Stefania; Roberto, Dominique; Ugo, Renato; Abbotto, Alessandro; Archetti, Graziano; Beverina, Luca; Ghezzi, Sergio

    2007-06-21

    In this work we present an investigation of the non-linear optical (NLO) properties of two octupolar chromophores: [Zn(4,4'-bis(dibutylaminostyryl)-[2,2']-bipyridine)(3)](2+) and [Zn(4,4'-bis((E)-2-(N-(TEG)pyrrol-2-yl)vinyl)-[2,2']-bipyridine)(3)](2+) with Zn(ii) as the coordination center, using two-photon emission technique (TPE) in fs-pulse temporal regime. Compared to the free ligands, our results do not show a net increase in the two-photon absorption (TPA) cross-section for the octupolar complexes, once normalized to the ligand unit. This is in partial disagreement with a previous theoretical study investigating the first molecule where a significant increase of the TPA cross-section was predicted (X. J. Liu, et al., J. Chem. Phys., 2004, 120, 11 493).

  8. Synthesizing arbitrary two-photon polarization mixed states

    CERN Document Server

    Wei, T C; Branning, D; Goldbart, P M; James, D F V; Jeffrey, E; Kwiat, P G; Mukhopadhyay, S; Peters, N A; Wei, Tzu-Chieh; Altepeter, Joseph B.; Branning, David; Goldbart, Paul M.; Jeffrey, Evan; Kwiat, Paul G.; Mukhopadhyay, Swagatam; Peters, Nicholas A.

    2005-01-01

    Two methods for creating arbitrary two-photon polarization pure states are introduced. Based on these, four schemes for creating two-photon polarization mixed states are proposed and analyzed. The first two schemes can synthesize completely arbitrary two-qubit mixed states, i.e., control all 15 free parameters: Scheme I requires several sets of crystals, while Scheme II requires only a single set, but relies on decohering the pump beam. Additionally, we describe two further schemes which are much easier to implement. Although the total capability of these is still being studied, we show that they can synthesize all two-qubit Werner states, maximally entangled mixed states, Collins-Gisin states, and arbitrary Bell-diagonal states.

  9. Two-photon excited ultraviolet photoluminescence of zinc oxide nanorods.

    Science.gov (United States)

    Zhu, Guangping; Xu, Chunxiang; Zhu, Jing; Lu, Changgui; Cui, Yiping; Sun, Xiaowei

    2008-11-01

    High density zinc oxide nanorods with uniform size were synthesized on (100) silicon substrate by vapor-phase transport method. The scanning electron microscopy images reveal that the nanorods have an average diameter of about 400 nm. The X-ray diffraction pattern demonstrates the wurtzite crystalline structure of the ZnO nanorods growing along [0001] direction. The single-photon excited photoluminescence presents a strong ultraviolet emission band at 394 nm and a weak visible emission band at 600 nm. When the ZnO nanorods were respectively pumped by various wavelength lasers from 520 nm to 700 nm, two-photon excited ultraviolet photoluminescence was observed. The dependence of the two-photon excited photoluminescence intensity on the excitation wavelength and power was investigated in detail.

  10. High-order dispersion effects in two-photon interference

    CERN Document Server

    Mazzotta, Z; Cipriani, D; Olivares, S; Paris, M G A

    2016-01-01

    Two-photon interference and Hong-Ou-Mandel (HOM) effect are relevant tools for quantum metrology and quantum information processing. In optical coherence tomography, HOM effect is exploited to achieve high-resolution measurements with the width of the HOM dip being the main parameter. On the other hand, applications like dense coding require high-visibility performances. Here we address high-order dispersion effects in two-photon interference and study, theoretically and experimentally, the dependence of the visibility and the width of the HOM dip on both the pump spectrum and the downconverted photon spectrum. In particular, a spatial light modulator is exploited to experimentally introduce and manipulate a custom phase function to simulate the high-order dispersion effects.

  11. Two-photon interference from two blinking quantum emitters

    Science.gov (United States)

    Jöns, Klaus D.; Stensson, Katarina; Reindl, Marcus; Swillo, Marcin; Huo, Yongheng; Zwiller, Val; Rastelli, Armando; Trotta, Rinaldo; Björk, Gunnar

    2017-08-01

    We investigate the effect of blinking on the two-photon interference measurement from two independent quantum emitters. We find that blinking significantly alters the statistics in the Hong-Ou-Mandel second-order intensity correlation function g(2 )(τ ) and the outcome of two-photon interference measurements performed with independent quantum emitters. We theoretically demonstrate that the presence of blinking can be experimentally recognized by a deviation from the gD(2 )(0 ) =0.5 value when distinguishable photons from two emitters impinge on a beam splitter. Our findings explain the significant differences between linear losses and blinking for correlation measurements between independent sources and are experimentally verified using a parametric down-conversion photon-pair source. We show that blinking imposes a mandatory cross-check measurement to correctly estimate the degree of indistinguishability of photons emitted by independent quantum emitters.

  12. Two-photon interaction between trapped ions and cavity fields

    CERN Document Server

    Semião, F L

    2006-01-01

    In this paper, we generalize the ordinary two-photon Jaynes-Cummings model (TPJCM) by considering the atom (or ion) to be trapped in a simple harmonic well. A typical setup would be an optical cavity containing a single ion in a Paul trap. Due to the inclusion of atomic vibrational motion, the atom-field coupling becomes highly nonlinear what brings out quite different behaviors for the system dynamics when compared to the ordinary TPJCM. In particular, we derive an effective two-photon Hamiltonian with dependence on the number operator of the ion's center-of-mass motion. This dependence occurs both in the cavity induced Stark-shifs and in the ion-field coupling, and its role in the dynamics is illustrated by showing the time evolution of the probability of occupation of the electronic levels for simple initial preparations of the state of the system.

  13. Two-photon microscopy using fiber-based nanosecond excitation.

    Science.gov (United States)

    Karpf, Sebastian; Eibl, Matthias; Sauer, Benjamin; Reinholz, Fred; Hüttmann, Gereon; Huber, Robert

    2016-07-01

    Two-photon excitation fluorescence (TPEF) microscopy is a powerful technique for sensitive tissue imaging at depths of up to 1000 micrometers. However, due to the shallow penetration, for in vivo imaging of internal organs in patients beam delivery by an endoscope is crucial. Until today, this is hindered by linear and non-linear pulse broadening of the femtosecond pulses in the optical fibers of the endoscopes. Here we present an endoscope-ready, fiber-based TPEF microscope, using nanosecond pulses at low repetition rates instead of femtosecond pulses. These nanosecond pulses lack most of the problems connected with femtosecond pulses but are equally suited for TPEF imaging. We derive and demonstrate that at given cw-power the TPEF signal only depends on the duty cycle of the laser source. Due to the higher pulse energy at the same peak power we can also demonstrate single shot two-photon fluorescence lifetime measurements.

  14. Two-photon-induced cycloreversion reaction of chalcone photodimers

    Science.gov (United States)

    Träger, J.; Härtner, S.; Heinzer, J.; Kim, H.-C.; Hampp, N.

    2008-04-01

    The photocleavage reaction of chalcone photodimers has been studied using a two-photon process. For this purpose, a novel chalcone dimer has been synthesized as a low molecular weight model substance for polymer bound chalcones and its photochemistry triggered by two-photon-absorption (2PA) has been investigated using a pulsed frequency-doubled Nd:YAG-laser. The 2PA-induced cycloreversion reaction selectively leads to the cleavage of the chalcone photodimers resulting in the formation of monomeric chalcone molecules. Hence, as an application chalcones can be used as a photosensitive linker which can be cleaved beyond an UV-absorbing barrier. The 2PA cross section of the chalcone photodimer was determined to be of 1.1 × 10 -49 cm 4 s photon -1 (11 GM).

  15. Four-dimensional multi-site two-photon excitation

    CERN Document Server

    Daria, Vincent Ricardo; Bowman, Richard; Redman, Stephen; Bachor, Hans-A

    2009-01-01

    We report the first demonstration of dynamic and arbitrary multi-site two-photon excitation in three-dimensional (3D) space using the holographic projection method. Rapid temporal response (fourth dimension) is achieved through high-speed non-iterative and non-optimized calculation of the hologram using a video graphics accelerator board. We verify that the projected asymmetric spot configurations have sufficient spatiotemporal photon density for localized two-photon excitation. This system is a significant advance and ready for applications such as time-resolved 3D photolysis of complex biological cell and neuronal networks, 3D microscopy, non-linear micro-fabrication and volume holographic optical storage.

  16. Simultaneous two-photon excitation of photodynamic therapy agents

    Energy Technology Data Exchange (ETDEWEB)

    Wachter, E.A.; Fisher, W.G. [Oak Ridge National Lab., TN (United States)]|[Photogen, Inc., Knoxville, TN (United States); Partridge, W.P. [Oak Ridge National Lab., TN (United States); Dees, H.C. [Photogen, Inc., Knoxville, TN (United States); Petersen, M.G. [Univ. of Tennessee, Knoxville, TN (United States). College of Veterinary Medicine

    1998-01-01

    The spectroscopic and photochemical properties of several photosensitive compounds are compared using conventional single-photon excitation (SPE) and simultaneous two-photon excitation (TPE). TPE is achieved using a mode-locked titanium:sapphire laser, the near infrared output of which allows direct promotion of non-resonant TPE. Excitation spectra and excited state properties of both type 1 and type 2 photodynamic therapy (PDT) agents are examined.

  17. Giant Two-photon Absorption in Circular Graphene Quantum Dots in Infrared Region

    Science.gov (United States)

    Feng, Xiaobo; Li, Zhisong; Li, Xin; Liu, Yingkai

    2016-01-01

    We investigate theoretically the two-photon absorption (TPA) for circular graphene quantum dots (GQDs) with the edge of armchair and zigzag on the basis of electronic energy states obtained by solving the Dirac-Weyl equation numerically under finite difference method. The expressions for TPA cross section are derived and the transition selection rules are obtained. Results reveal that the TPA is significantly greater in GQDs than conventional semiconductor QDs in infrared spectrum (2–6 um) with a resonant TPA cross section of up to 1011 GM. The TPA peaks are tuned by the GQDs’ size, edge and electron relaxation rate. PMID:27629800

  18. Polarised two-photon excitation of quantum well excitons for manipulation of optically pumped terahertz lasers

    Energy Technology Data Exchange (ETDEWEB)

    Slavcheva, G., E-mail: gsk23@bath.ac.uk [Blackett Laboratory, Imperial College London, Prince Consort Road, London SW7 2AZ (United Kingdom); Kavokin, A.V., E-mail: A.Kavokin@soton.ac.uk [School of Physics and Astronomy, University of Southampton, Highfield, Southampton SO17 1BJ (United Kingdom); Spin Optics Laboratory, St. Petersburg State University, 1, Ulyanovskaya 198504 (Russian Federation)

    2014-11-15

    Optical pumping of excited exciton states in a semiconductor quantum well embedded in a microcavity is a tool for realisation of ultra-compact terahertz (THz) lasers based on stimulated optical transition between excited (2p) and ground (1s) exciton state. We show that the probability of two-photon absorption by a 2p-exciton is strongly dependent on the polarisation of both pumping photons. Five-fold variation of the threshold power for terahertz lasing by switching from circular to co-linear pumping is predicted. We identify photon polarisation configurations for achieving maximum THz photon generation quantum efficiency.

  19. Two-photon Photo-emission of Ultrathin Film PTCDA Morphologies on Ag(111)

    Energy Technology Data Exchange (ETDEWEB)

    Yang, Aram; Yang, Aram; Shipman, Steven T.; Garrett-Roe, Sean; Johns, James; Strader, Matt; Szymanski, Paul; Muller, Eric; Harris, Charles B.

    2007-11-29

    Morphology- and layer-dependent electronic structure and dynamics at the PTCDA/Ag(111) interface have been studied with angle-resolved two-photon photoemission. In Stranski-Krastanov growth modes, the exposed wetting layer inhibited the evolution of the vacuum level and valence band to bulk values. For layer-by-layer growth, we observed the transition of electron structure from monolayer to bulk values within eight monolayers. Effective masses and lifetimes of the conduction band and the n=1 image potential state were measured to be larger for disordered layers. The effective mass was interpreted in the context of charge mobility measurements.

  20. Giant Two-photon Absorption in Circular Graphene Quantum Dots in Infrared Region

    Science.gov (United States)

    Feng, Xiaobo; Li, Zhisong; Li, Xin; Liu, Yingkai

    2016-09-01

    We investigate theoretically the two-photon absorption (TPA) for circular graphene quantum dots (GQDs) with the edge of armchair and zigzag on the basis of electronic energy states obtained by solving the Dirac-Weyl equation numerically under finite difference method. The expressions for TPA cross section are derived and the transition selection rules are obtained. Results reveal that the TPA is significantly greater in GQDs than conventional semiconductor QDs in infrared spectrum (2-6 um) with a resonant TPA cross section of up to 1011 GM. The TPA peaks are tuned by the GQDs’ size, edge and electron relaxation rate.

  1. Multichannel 0-to-2 and 1-to-2 transition amplitudes for arbitrary spin particles in a finite volume

    CERN Document Server

    Briceño, Raúl A

    2015-01-01

    We present a model-independent, non-perturbative relation between finite-volume matrix elements and infinite-volume $\\textbf{0}\\rightarrow\\textbf{2}$ and $\\textbf{1}\\rightarrow\\textbf{2}$ transition amplitudes. Our result accommodates theories in which the final two-particle state is coupled to any number of other two-body channels, with all angular momentum states included. The derivation uses generic, fully relativistic field theory, and is exact up to exponentially suppressed corrections in the lightest particle mass times the box size. This work distinguishes itself from previous studies by accommodating particles with any intrinsic spin. To illustrate the utility of our general result, we discuss how it can be implemented for studies of $N+\\mathcal{J}~\\rightarrow~(N\\pi,N\\eta,N\\eta',\\Sigma K,\\Lambda K)$ transitions, where $\\mathcal{J}$ is a generic external current. The reduction of rotational symmetry, due to the cubic finite volume, manifests in this example through the mixing of S- and P-waves when the...

  2. Two-photon imaging through a multimode fiber

    CERN Document Server

    Morales-Delgado, Edgar E; Moser, Christophe

    2015-01-01

    In this work we demonstrate 3D imaging using two-photon excitation through a 20 cm long multimode optical fiber (MMF) of 350 micrometers diameter. The imaging principle is similar to single photon fluorescence through a MMF, except that a focused femtosecond pulse is delivered and scanned over the sample. In our approach, focusing and scanning through the fiber is accomplished by digital phase conjugation using mode selection by time gating with an ultra-fast reference pulse. The excited two-photon emission is collected through the same fiber. We demonstrate depth sectioning by scanning the focused pulse in a 3D volume over a sample consisting of fluorescent beads suspended in a polymer. The achieved resolution is 1 micrometer laterally and 15 micrometers axially. Scanning is performed over an 80x80 micrometers field of view. To our knowledge, this is the first demonstration of high-resolution three-dimensional imaging using two-photon fluorescence through a multimode fiber.

  3. Two photon exchange in elastic electron-nucleon scattering

    Energy Technology Data Exchange (ETDEWEB)

    Peter Blunden; Wolodymyr Melnitchouk; John Tjon

    2005-06-01

    A detailed study of two-photon exchange in unpolarized and polarized elastic electron-nucleon scattering is presented, taking particular account of nucleon finite size effects. Contributions from nucleon elastic intermediate states are found to have a strong angular dependence, which leads to a partial resolution of the discrepancy between the Rosenbluth and polarization transfer measurements of the proton electric to magnetic form factor ratio. The two-photon exchange contribution to the longitudinal polarization transfer ratio P{sub L} is small, whereas the contribution to the transverse polarization transfer ratio P{sub T} is enhanced at backward angles by several percent, increasing with Q{sup 2}. This gives rise to a several percent enhancement of the polarization transfer ratio P{sub T}/P{sub l} at large Q{sup 2} and backward angles. We compare the two-photon exchange effects with data on the ratio of e{sup +p} to e{sup -p} cross sections, which is predicted to be enhanced at backward angles. Finally, we evaluate the corrections to the form factors of the neutron, and estimate the elastic intermediate state contribution to the {sup 3}He form factors.

  4. Recent two-photon physics results from ARGUS

    Science.gov (United States)

    Živko Representing Argus Collaboration, Tomi

    1995-07-01

    Two photon production of π+π+π0π-π-, K+K-π+π-, K+K-π+π0π-, π+π0π-, and π+π- has been studied using the ARGUS detector at the e+e- storage ring DORIS II at DESY. A partial wave analysis was performed on the five-pion and three-pion final states. In the reaction γγ→ωρ0 is showed that the partial-wave with spin and parity (JP,Jz)=(2+,±2) dominates. The cross section and angular distributions of the reaction γγ→φρ0→K+K-π+π- were measured for the first time. The production of the vector-meson pair φω is observed in the two-photon reaction γγ→K+K-π+π0π-. The two-photon width of the tensor meson a2(1320) was measured in the decay channel π+π0π-. An upper limit, significantly lower than indicated by previous experiments was set on the radiative width of the π2(1670) meson. An upper limit was set on the radiative width of the f0(975)in the decay channel π+π-.

  5. Two-Photon Absorption in Organometallic Bromide Perovskites

    KAUST Repository

    Walters, Grant

    2015-07-21

    Organometallic trihalide perovskites are solution processed semiconductors that have made great strides in third generation thin film light harvesting and light emitting optoelectronic devices. Recently it has been demonstrated that large, high purity single crystals of these perovskites can be synthesized from the solution phase. These crystals’ large dimensions, clean bandgap, and solid-state order, have provided us with a suitable medium to observe and quantify two-photon absorption in perovskites. When CH3NH3PbBr3 single crystals are pumped with intense 800 nm light, we observe band-to-band photoluminescence at 572 nm, indicative of two-photon absorption. We report the nonlinear absorption coefficient of CH3NH3PbBr3 perovskites to be 8.6 cm GW-1 at 800 nm, comparable to epitaxial single crystal semiconductors of similar bandgap. We have leveraged this nonlinear process to electrically autocorrelate a 100 fs pulsed laser using a two-photon perovskite photodetector. This work demonstrates the viability of organometallic trihalide perovskites as a convenient and low-cost nonlinear absorber for applications in ultrafast photonics.

  6. Exploring control parameters of two photon processes in solutions

    Indian Academy of Sciences (India)

    Debabrata Goswami; Amit Nag

    2012-01-01

    Two-photon microscopy depends extensively on the two-photon absorption cross-sections of biologically relevant chromophores. High repetition rate (HRR) lasers are essential in multiphoton microscopy for generating satisfactory signal to noise at low average powers. However, HRR lasers generate thermal distortions in samples even with the slightest single photon absorption. We use an optical chopper with HRR lasers to intermittently `blank’ irradiation and effectively minimize thermal effects to result in a femtosecond z-scan setup that precisely measures the two-photon absorption (TPA) cross-sections of chromophores. Though several experimental factors impact such TPA measurements, a systematic effort to modulate and influence TPA characteristics is yet to evolve. Here, we present the effect of several control parameters on the TPA process that are independent of chromophore characteristics for femtosecond laser pulse based measurements; and demonstrate how the femtosecond laser pulse repetition rate, chromophore environment and incident laser polarization can become effective control parameters for such nonlinear optical properties.

  7. Two-Photon Absorption in Organometallic Bromide Perovskites.

    Science.gov (United States)

    Walters, Grant; Sutherland, Brandon R; Hoogland, Sjoerd; Shi, Dong; Comin, Riccardo; Sellan, Daniel P; Bakr, Osman M; Sargent, Edward H

    2015-09-22

    Organometallic trihalide perovskites are solution-processed semiconductors that have made great strides in third-generation thin film light-harvesting and light-emitting optoelectronic devices. Recently, it has been demonstrated that large, high-purity single crystals of these perovskites can be synthesized from the solution phase. These crystals' large dimensions, clean bandgap, and solid-state order have provided us with a suitable medium to observe and quantify two-photon absorption in perovskites. When CH3NH3PbBr3 single crystals are pumped with intense 800 nm light, we observe band-to-band photoluminescence at 572 nm, indicative of two-photon absorption. We report the nonlinear absorption coefficient of CH3NH3PbBr3 perovskites to be 8.6 cm GW(-1) at 800 nm, comparable to epitaxial single-crystal semiconductors of similar bandgap. We have leveraged this nonlinear process to electrically autocorrelate a 100 fs pulsed laser using a two-photon perovskite photodetector. This work demonstrates the viability of organometallic trihalide perovskites as a convenient and low-cost nonlinear absorber for applications in ultrafast photonics.

  8. The $\\pi\\pi\\to\\pi\\gamma^\\star$ amplitude and the resonant $\\rho\\to\\pi\\gamma^\\star$ transition from lattice QCD

    CERN Document Server

    Briceño, Raúl A; Edwards, Robert G; Shultz, Christian J; Thomas, Christopher E; Wilson, David J

    2016-01-01

    We present a determination of the $P$-wave $\\pi\\pi\\to\\pi\\gamma^\\star$ transition amplitude from lattice quantum chromodynamics. Matrix elements of the vector current in a finite-volume are extracted from three-point correlation functions, and from these we determine the infinite-volume amplitude using a generalization of the Lellouch-L\\"uscher formalism. We determine the amplitude for a range of discrete values of the $\\pi\\pi$ energy and virtuality of the photon, and observe the expected dynamical enhancement due to the $\\rho$ resonance. Describing the energy dependence of the amplitude, we are able to analytically continue into the complex energy plane and from the residue at the $\\rho$ pole extract the $\\rho\\to \\pi \\gamma^\\star$ transition form factor. This calculation, at $m_\\pi\\approx 400$ MeV, is the first to determine the form factor of an unstable hadron within a first principles approach to QCD.

  9. Two-Photon Absorption Spectroscopy of Rubidium with a Dual-Comb Tequnique

    Science.gov (United States)

    Nishiyama, Akiko; Yoshida, Satoru; Hariki, Takuya; Nakajima, Yoshiaki; Minoshima, Kaoru

    2017-06-01

    Dual-comb spectroscopies have great potential for high-resolution molecular and atomic spectroscopies, thanks to the broadband comb spectrum consisting of dense narrow modes. In this study, we apply the dual-comb system to Doppler-free two-photon absorption spectroscopy. The outputs of two frequency combs excite several two-photon transitions of rubidium, and we obtained broadband Doppler-free spectra from dual-comb fluorescence signals. The fluorescence detection scheme circumvents the sensitivity limit which is effectively determined by the dynamic range of photodetectors in absorption-based dual-comb spectroscopies. Our system realized high-sensitive, Doppler-free high-resolution and broadband atomic spectroscopy. A part of observed spectra of 5S_{1/2} - 5D_{5/2} transition is shown in the figure. The hyperfine structures of the F" = 1 - F' = 3,2,1 transitions are fully-resolved and the spectral widths are approximately 5 MHz. The absolute frequency axis is precisely calibrated from comb mode frequencies which were stabilized to a GPS-disciplined clock. This work was supported by JST through the ERATO MINOSHIMA Intelligent Optical Synthesizer Project and Grant-in-Aid for JSPS Fellows (16J02345). A. Nishiyama, S. Yoshida, Y. Nakajima, H. Sasada, K. Nakagawa, A. Onae, K. and Minoshima, Opt. Express 24, 25894 (2016). A. Hipke, S. A. Meek, T. Ideguchi, T.W. Hänsch, and N. Picqué, Phys. Rev. A 90, 011805(R) (2014).

  10. Confined optical-phonon-assisted cyclotron resonance in quantum wells via two-photon absorption process

    Science.gov (United States)

    Phuc, Huynh Vinh; Hien, Nguyen Dinh; Dinh, Le; Phong, Tran Cong

    2016-06-01

    The effect of confined phonons on the phonon-assisted cyclotron resonance (PACR) via both one and two photon absorption processes in a quantum well is theoretically studied. We consider cases when electrons are scattered by confined optical phonons described by the Fuchs-Kliewer slab, Ridley's guided, and Huang-Zhu models. The analytical expression of the magneto-optical absorption coefficient (MOAC) is obtained by relating it to the transition probability for the absorption of photons. It predicts resonant peaks caused by transitions between Landau levels and electric subband accompanied by confined phonons emission in the absorption spectrum. The MOAC and the full-width at half-maximum (FWHM) for the intra- and inter-subband transitions are given as functions of the magnetic field, temperature, and quantum well width. In narrow quantum wells, the phonon confinement becomes more important and should be taken into account in studying FWHM.

  11. Magneto-Photoluminescence Based on Two-Photon Excitation in Lanthanide-Doped Up-Conversion Crystal Particles.

    Science.gov (United States)

    Xu, Hengxing; Qin, Wei; Li, Mingxing; Wu, Ting; Hu, Bin

    2017-04-01

    Experimental studies on magneto-photoluminescence based on two-photon excitation in up-conversion Y2 O2 S:Er, Yb crystal particles are reported. It is found that the up-conversion photoluminescence generated by two-photon excitation exhibits magnetic field effects at room temperature, leading to a two-photon excitation-induced magneto-photoluminescence, when the two-photon excitation exceeds the critical intensity. By considering the spin selection rule in electronic transitions, it is proposed that spin-antiparallel and spin-parallel transition dipoles with spin mixing are accountable for the observed magneto-photoluminescence. Specifically, the two-photon excitation generates spin-antiparallel electric dipoles between (4) S3/2 -(4) I15/2 in Er(3+) ions. The antiparallel spins are conserved by exchange interaction within dipoles. When the photoexcitation exceeds the critical intensity, the Coulomb screening can decrease the exchange interaction. Consequently, the spin-orbital coupling can partially convert the antiparallel dipoles into parallel dipoles, generating a spin mixing. Eventually, the populations between antiparallel and parallel dipoles reach an equilibrium established by the competition between exchange interaction and spin-orbital coupling. Applying a magnetic field can break the equilibrium by disturbing spin mixing through introducing spin precessions, changing the spin populations on antiparallel and parallel dipoles and leading to the magneto-photoluminescence. Therefore, spin-dependent transition dipoles present a convenient mechanism to realize magneto-photoluminescence in multiphoton up-conversion crystal particles. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  12. On the origin of large two-photon activity of DANS molecule.

    Science.gov (United States)

    Alam, Md Mehboob; Chattopadhyaya, Mausumi; Chakrabarti, Swapan

    2012-11-15

    In this work, using the quadratic response theory and two-state model approach, we have explained the origin of high two-photon activity and the corresponding solvent dependence of 4,4'-dimethyl-amino-nitro-stilbene (DANS) molecule. For this purpose, we have made two structural modifications in the DANS molecule (1) at the donor-acceptor part and (2) at the unsaturated bridge between the two rings and calculated the one- and two-photon (OP and TP) absorption parameters of all the systems in gas phase and in three different solvents, viz., MeCN, THF, and toluene. We found that the removal of donor-acceptor groups from the original DANS molecule vanishes the transition moment between the ground and excited states and also the corresponding dipole moment difference, and the saturation of the π-conjugation bridge between the two rings keeping the donor-acceptor groups intact causes a large decrease in the ground to excited state transition moment. These changes, in turn, decrease the overall TP activity of the molecules as compared to DANS. On the basis of our analysis, we have concluded that neither the donor-acceptor pair nor the π-conjugation bridge between the two, rather their cooperative involvement leads to a large overlap between the ground and virtual and also the virtual and charge-transfer states, which are eventually responsible for the very large TP activity of DANS.

  13. Quantum correlations in the two-photon decay of few-electron ions

    CERN Document Server

    Fratini, Filippo; Jahrsetz, Thorsten; Buchleitner, Andreas; Fritzsche, Stephan; Surzhykov, Andrey

    2010-01-01

    A theoretical study of the polarization entanglement of two photons emitted in the decay of metastable ionic states is performed within the framework of density matrix theory and second--order perturbative approach. Particular attention is paid to relativistic and non--dipole effects that become important for medium-- and high--$Z$ ions. To analyze these effects, the degree of entanglement is evaluated both in the dipole approximation and within the rigorous relativistic theory. Detailed calculations are performed for the two--photon $2s_{1/2}\\to 1s_{1/2}$ transition in hydrogen--like, as well as for the $1s_{1/2}\\, 2s_{1/2} \\; {}^1S_0 \\to 1s_{1/2}^2 \\; {}^1S_0$, $1s_{1/2} \\, 2s_{1/2} \\; {}^3S_1\\to 1s_{1/2}^2 \\; {}^1S_0$ and $1s_{1/2} \\, 2p_{1/2} \\; {}^3P_0\\to 1s_{1/2}^2 \\; {}^1S_0$ transitions in helium--like ions.

  14. Two-photon imaging and analysis of neural network dynamics

    Science.gov (United States)

    Lütcke, Henry; Helmchen, Fritjof

    2011-08-01

    The glow of a starry night sky, the smell of a freshly brewed cup of coffee or the sound of ocean waves breaking on the beach are representations of the physical world that have been created by the dynamic interactions of thousands of neurons in our brains. How the brain mediates perceptions, creates thoughts, stores memories and initiates actions remains one of the most profound puzzles in biology, if not all of science. A key to a mechanistic understanding of how the nervous system works is the ability to measure and analyze the dynamics of neuronal networks in the living organism in the context of sensory stimulation and behavior. Dynamic brain properties have been fairly well characterized on the microscopic level of individual neurons and on the macroscopic level of whole brain areas largely with the help of various electrophysiological techniques. However, our understanding of the mesoscopic level comprising local populations of hundreds to thousands of neurons (so-called 'microcircuits') remains comparably poor. Predominantly, this has been due to the technical difficulties involved in recording from large networks of neurons with single-cell spatial resolution and near-millisecond temporal resolution in the brain of living animals. In recent years, two-photon microscopy has emerged as a technique which meets many of these requirements and thus has become the method of choice for the interrogation of local neural circuits. Here, we review the state-of-research in the field of two-photon imaging of neuronal populations, covering the topics of microscope technology, suitable fluorescent indicator dyes, staining techniques, and in particular analysis techniques for extracting relevant information from the fluorescence data. We expect that functional analysis of neural networks using two-photon imaging will help to decipher fundamental operational principles of neural microcircuits.

  15. Two-photon imaging and analysis of neural network dynamics

    Energy Technology Data Exchange (ETDEWEB)

    Luetcke, Henry; Helmchen, Fritjof [Brain Research Institute, University of Zurich, Winterthurerstrasse 190, CH-8057 Zurich (Switzerland)

    2011-08-15

    The glow of a starry night sky, the smell of a freshly brewed cup of coffee or the sound of ocean waves breaking on the beach are representations of the physical world that have been created by the dynamic interactions of thousands of neurons in our brains. How the brain mediates perceptions, creates thoughts, stores memories and initiates actions remains one of the most profound puzzles in biology, if not all of science. A key to a mechanistic understanding of how the nervous system works is the ability to measure and analyze the dynamics of neuronal networks in the living organism in the context of sensory stimulation and behavior. Dynamic brain properties have been fairly well characterized on the microscopic level of individual neurons and on the macroscopic level of whole brain areas largely with the help of various electrophysiological techniques. However, our understanding of the mesoscopic level comprising local populations of hundreds to thousands of neurons (so-called 'microcircuits') remains comparably poor. Predominantly, this has been due to the technical difficulties involved in recording from large networks of neurons with single-cell spatial resolution and near-millisecond temporal resolution in the brain of living animals. In recent years, two-photon microscopy has emerged as a technique which meets many of these requirements and thus has become the method of choice for the interrogation of local neural circuits. Here, we review the state-of-research in the field of two-photon imaging of neuronal populations, covering the topics of microscope technology, suitable fluorescent indicator dyes, staining techniques, and in particular analysis techniques for extracting relevant information from the fluorescence data. We expect that functional analysis of neural networks using two-photon imaging will help to decipher fundamental operational principles of neural microcircuits.

  16. Chromophore design for large two-photon absorption

    Science.gov (United States)

    Dudley, Christopher

    2014-11-01

    Conjugated oligothiophene chromophores are compared and studied for designing large linear and nonlinear absorption cross-sections. Optical properties of chromophores synthesized by the Naval Research Laboratory are modeled to construct a design factor of merit to predict and understand two-photon absorption (TPA) designs. Computer modeling to optimize parameters to produce photo active chromophores is conducted. Geometry, π-center (electron relay) and the electron donor or acceptor groups attached to the π-centers are considered for importance in TPA. This work could serve equally well as guide for quick back of the envelop research or industrial design verifications as well as an outline for introducing computation methods to students.

  17. New two-photon based nanoscopic modalities and optogenetics

    DEFF Research Database (Denmark)

    Glückstad, Jesper

    -matter interaction on these scales involves the combination of optimal light-sculpting [4] with the use of optimized shapes in micro-robotics structures [5]. Microfabrication processes such as two-photon photo-polymerization offer three-dimensional resolutions for creating custom-designed monolithic microstructures...... that can be equipped with optical trapping handles for convenient mechanical control using only optical forces [6]. These microstructures illustrated above can be effectively handled with simultaneous top- and side-view on our BioPhotonics Workstation to undertake six-degree-of-freedom optical actuation...

  18. Two-photon polymerization of immune cell scaffolds

    DEFF Research Database (Denmark)

    Olsen, Mark Holm

    and easy to use chip integrated migration platform. Free-form constructs with three-dimensional (3D) microporosity were fabricated by two-photon polymerization inside the closed microchannel of an injection molded commercially available polymer chip for analysis of directed cell migration. Acrylate...... also present a poly (ethylene glycol) diacrylate (PEGDA) based strategy to fabricate soft 3D hydrogel scaffolds. Our experiments with the hydrogel confirm we can control the mechanical properties and introduce biochemical cues on the surface that are recognized by fibroblast cells. Finally we present...

  19. The Nelson Model with Less Than Two Photons

    CERN Document Server

    Galtbayar, A; Yajima, K

    2002-01-01

    We study the spectral and scattering theory of the Nelson model for an atom interacting with a photon field in the subspace with less than two photons. For the free electron-photon system, the spectral property of the reduced Hamiltonian in the center of mass coordinates and the large time dynamics are determined. If the electron is under the influence of the nucleus via spatially decaying potentials, we locate the essential spectrum, prove the absence of singular continuous spectrum and the existence of the ground state, and construct wave operators giving the asymptotic dynamics.

  20. Two-photon tomography using on-chip quantum walks

    CERN Document Server

    Titchener, James; Sukhorukov, Andrey

    2016-01-01

    We present a conceptual approach to quantum tomography based on first expanding a quantum state across extra degrees of freedom and then exploiting the introduced sparsity to perform reconstruction. We formulate its application to photonic circuits, and show that measured spatial photon correlations at the output of a specially tailored discrete-continuous quantum-walk can enable full reconstruction of any two-photon spatially entangled and mixed state at the input. This approach does not require any tunable elements, so is well suited for integration with on-chip superconducting photon detectors.

  1. Quantum teleportation of one- and two-photon superposition states

    Institute of Scientific and Technical Information of China (English)

    李英; 张天才; 张俊香; 谢常德

    2003-01-01

    Quantum teleportation of one- and two-photon superposition states based on EPR entanglement of continuouswave two-mode squeezed state is discussed. The fidelities of teleportation are deduced for two different input quantum states. The dependence of the fidelity on the parameters of EPR entanglement and the gain of the classical channels are shown numerically. Comparing with the teleportation of Fock state and coherent state, it is pointed out that for given EPR entanglement and classical gain, the higher the nonclassicality of the input state, the lower the accessible fidelity of teleportation.

  2. Spectral Features of FM Spectroscopy of Two-Photon Interactions

    Institute of Scientific and Technical Information of China (English)

    夏慧荣; JohnL.Hall

    1994-01-01

    The spectral features of FM two-photon resonant interaction processes have been calculated for five different frequency modulation versions of counter-propagating incident fields. It is found that the proposed new modulation version (case b in the text) provides novel spectral features for a completely canceled absorption and a sharp dispersion shape at the fundamental beat note. Moreover, its absorption feature appears at the second harmonic of the RF modulation frequency generated by the joint modes via six interaction pathways without mutual phase shift. Such features persist even when the effects of the second-order sidebands of the incident fields are taken into account. Application potentials are emphasized.

  3. Inclusive $D*^{+-}$ Production in Two-Photon Collisions at LEP

    CERN Document Server

    Achard, P; Aguilar-Benítez, M; Alcaraz, J; Alemanni, G; Allaby, James V; Aloisio, A; Alviggi, M G; Anderhub, H; Andreev, V P; Anselmo, F; Arefev, A; Azemoon, T; Aziz, T; Bagnaia, P; Bajo, A; Baksay, G; Baksay, L; Baldew, S V; Banerjee, S; Banerjee, Sw; Barczyk, A; Barillère, R; Bartalini, P; Basile, M; Batalova, N; Battiston, R; Bay, A; Becattini, F; Becker, U; Behner, F; Bellucci, L; Berbeco, R; Berdugo, J; Berges, P; Bertucci, B; Betev, B L; Biasini, M; Biglietti, M; Biland, A; Blaising, J J; Blyth, S C; Bobbink, Gerjan J; Böhm, A; Boldizsar, L; Borgia, B; Bottai, S; Bourilkov, D; Bourquin, Maurice; Braccini, S; Branson, J G; Brochu, F; Burger, J D; Burger, W J; Cai, X D; Capell, M; Cara Romeo, G; Carlino, G; Cartacci, A M; Casaus, J; Cavallari, F; Cavallo, N; Cecchi, C; Cerrada, M; Chamizo-Llatas, M; Chang, Y H; Chemarin, M; Chen, A; Chen, G; Chen, G M; Chen, H F; Chen, H S; Chiefari, G; Cifarelli, Luisa; Cindolo, F; Clare, I; Clare, R; Coignet, G; Colino, N; Costantini, S; de la Cruz, B; Cucciarelli, S; van Dalen, J A; De Asmundis, R; Déglon, P L; Debreczeni, J; Degré, A; Deiters, K; Della Volpe, D; Delmeire, E; Denes, P; De Notaristefani, F; De Salvo, A; Diemoz, M; Dierckxsens, M; Dionisi, C; Dittmar, Michael; Doria, A; Dova, M T; Duchesneau, D; Echenard, B; Eline, A; El-Mamouni, H; Engler, A; Eppling, F J; Ewers, A; Extermann, Pierre; Falagán, M A; Falciano, S; Favara, A; Fay, J; Fedin, O; Felcini, Marta; Ferguson, T; Fesefeldt, H S; Fiandrini, E; Field, J H; Filthaut, Frank; Fisher, P H; Fisher, W; Fisk, I; Forconi, G; Freudenreich, Klaus; Furetta, C; Galaktionov, Yu; Ganguli, S N; García-Abia, P; Gataullin, M; Gentile, S; Giagu, S; Gong, Z F; Grenier, G; Grimm, O; Grünewald, M W; Guida, M; van Gulik, R; Gupta, V K; Gurtu, A; Gutay, L J; Haas, D; Hakobyan, R S; Hatzifotiadou, D; Hebbeker, T; Hervé, A; Hirschfelder, J; Hofer, H; Hohlmann, M; Holzner, G; Hou, S R; Hu, Y; Jin, B N; Jones, L W; de Jong, P; Josa-Mutuberria, I; Käfer, D; Kaur, M; Kienzle-Focacci, M N; Kim, J K; Kirkby, Jasper; Kittel, E W; Klimentov, A; König, A C; Kopal, M; Koutsenko, V F; Kräber, M H; Krämer, R W; Krenz, W; Krüger, A; Kunin, A; Ladrón de Guevara, P; Laktineh, I; Landi, G; Lebeau, M; Lebedev, A; Lebrun, P; Lecomte, P; Lecoq, P; Le Coultre, P; Le Goff, J M; Leiste, R; Levtchenko, M; Levchenko, P M; Li, C; Likhoded, S A; Lin, C H; Lin, W T; Linde, Frank L; Lista, L; Liu, Z A; Lohmann, W; Longo, E; Lü, Y S; Lübelsmeyer, K; Luci, C; Luminari, L; Lustermann, W; Ma Wen Gan; Malgeri, L; Malinin, A; Maña, C; Mangeol, D J J; Mans, J; Martin, J P; Marzano, F; Mazumdar, K; McNeil, R R; Mele, S; Merola, L; Meschini, M; Metzger, W J; Mihul, A; Milcent, H; Mirabelli, G; Mnich, J; Mohanty, G B; Muanza, G S; Muijs, A J M; Musicar, B; Musy, M; Nagy, S; Natale, S; Napolitano, M; Nessi-Tedaldi, F; Newman, H; Niessen, T; Nisati, A; Nowak, H; Ofierzynski, R A; Organtini, G; Palomares, C; Pandoulas, D; Paolucci, P; Paramatti, R; Passaleva, G; Patricelli, S; Paul, T; Pauluzzi, M; Paus, C; Pauss, Felicitas; Pedace, M; Pensotti, S; Perret-Gallix, D; Petersen, B; Piccolo, D; Pierella, F; Pioppi, M; Piroué, P A; Pistolesi, E; Plyaskin, V; Pohl, M; Pozhidaev, V; Pothier, J; Prokofiev, D O; Prokofev, D; Quartieri, J; Rahal-Callot, G; Rahaman, M A; Raics, P; Raja, N; Ramelli, R; Rancoita, P G; Ranieri, R; Raspereza, A V; Razis, P A; Ren, D; Rescigno, M; Reucroft, S; Riemann, S; Riles, K; Roe, B P; Romero, L; Rosca, A; Rosier-Lees, S; Roth, S; Rosenbleck, C; Roux, B; Rubio, Juan Antonio; Ruggiero, G; Rykaczewski, H; Sakharov, A; Saremi, S; Sarkar, S; Salicio, J; Sánchez, E; Sanders, M P; Schäfer, C; Shchegelskii, V; Schmidt-Kärst, S; Schmitz, D; Schopper, Herwig Franz; Schotanus, D J; Schwering, G; Sciacca, C; Servoli, L; Shevchenko, S; Shivarov, N; Shoutko, V; Shumilov, E; Shvorob, A V; Siedenburg, T; Son, D; Spillantini, P; Steuer, M; Stickland, D P; Stoyanov, B; Strässner, A; Sudhakar, K; Sultanov, G G; Sun, L Z; Sushkov, S V; Suter, H; Swain, J D; Szillási, Z; Tang, X W; Tarjan, P; Tauscher, Ludwig; Taylor, L; Tellili, B; Teyssier, D; Timmermans, C; Ting, Samuel C C; Ting, S M; Tonwar, S C; Tóth, J; Tully, C; Tung, K L; Ulbricht, J; Valente, E; Van, R T; De Walle, M; Veszpremi, V; Vesztergombi, G; Vetlitskii, I; Vicinanza, D; Viertel, Gert M; Villa, S; Vivargent, M; Vlachos, S; Vodopyanov, I; Vogel, H; Vogt, H; Vorobev, I; Vorobyov, A A; Wadhwa, M; Wallraff, W; Wang, X L; Wang, Z M; Weber, M; Wienemann, P; Wilkens, H; Wynhoff, S; Xia, L; Xu, Z Z; Yamamoto, J; Yang, B Z; Yang, C G; Yang, H J; Yang, M; Yeh, S C; Zalite, A; Zalite, Yu; Zhang, Z P; Zhao, J; Zhu, G Y; Zhu, R Y; Zhuang, H L; Zichichi, A; Zilizi, G; Zimmermann, B; Zöller, M

    2002-01-01

    Inclusive D^{*+-} production in two-photon collisions is studied with the L3 detector at LEP, using 683 pb^{-1} of data collected at centre-of-mass energies from 183 to 208 GeV. Differential cross sections are determined as functions of the transverse momentum and pseudorapidity of the D^{*+-} mesons in the kinematic region 1 GeV e^+e^-D^{*+-}X)$ in this kinematical region is measured and the sigma(e^+e^- ---> e^+e^- cc{bar}X) cross section is derived. The measurements are compared with next-to-leading order perturbative QCD calculations.

  4. Measurement of the isotope shift of the 2{{\\rm{p}}}^{4}{}^{3}{{P}}_{2} \\rightarrow 2{{\\rm{p}}}^{3}3{\\rm{p}}{}^{3}{{P}}_{2} two-photon transition of O I and a revision of the triplet energy levels of atomic oxygen

    Science.gov (United States)

    Marinov, D.; Booth, J.-P.; Drag, C.; Blondel, C.

    2017-03-01

    Two-photon induced fluorescence of atomic oxygen, which is routinely used for plasma and flame diagnostics, is implemented with two counterpropagating laser beams of sufficient monochromaticity to permit Doppler-free spectroscopy. A single-mode injection-seeded pulsed Ti:sapphire laser has been frequency-doubled twice to produce narrow-band pulsed radiation at wavelengths around 225.6 nm, suitable to excite the ground-state-to-2{{{p}}}33{{p}}{}3{P} two-photon resonance line of oxygen. Accurate measurement of the injection-seeding wavelength provides new data on the excitation energy of the 3{{p}}{}3{P} states. The experiment was done both sequentially and simultaneously on 16O and 18O, which makes it possible to test recent calculations of the isotope shift. Having an absolute measurement of the excitation wave-number from the ground level, which has been the case only twice in previous spectroscopic studies of O I, we can re-examine the energy levels of the subset of triplet states and present an updated set of optimised energy values.

  5. Two-Photon Holographic Stimulation of ReaChR

    Science.gov (United States)

    Chaigneau, Emmanuelle; Ronzitti, Emiliano; Gajowa, Marta A.; Soler-Llavina, Gilberto J.; Tanese, Dimitrii; Brureau, Anthony Y. B.; Papagiakoumou, Eirini; Zeng, Hongkui; Emiliani, Valentina

    2016-01-01

    Optogenetics provides a unique approach to remotely manipulate brain activity with light. Reaching the degree of spatiotemporal control necessary to dissect the role of individual cells in neuronal networks, some of which reside deep in the brain, requires joint progress in opsin engineering and light sculpting methods. Here we investigate for the first time two-photon stimulation of the red-shifted opsin ReaChR. We use two-photon (2P) holographic illumination to control the activation of individually chosen neurons expressing ReaChR in acute brain slices. We demonstrated reliable action potential generation in ReaChR-expressing neurons and studied holographic 2P-evoked spiking performances depending on illumination power and pulse width using an amplified laser and a standard femtosecond Ti:Sapphire oscillator laser. These findings provide detailed knowledge of ReaChR's behavior under 2P illumination paving the way for achieving in depth remote control of multiple cells with high spatiotemporal resolution deep within scattering tissue. PMID:27803649

  6. Inclusive D*(+/-) production in two photon collisions at LEP

    CERN Document Server

    Prokofiev, Denis Olegovich

    2001-01-01

    In this thesis I present my results on the measurement of the open charm production in two-photon collision events done with the L3 detector at Large Electron Positron machine (LEP). The data sample was collected from 1997 through 2000 at center-of-mass energies ranging from 183 GeV to 209 GeV, corresponding to a total integrated luminosity of 683.4pb −1. The open charm production in two-photon collision events extrapolated to the full phase space is estimated to be: s&parl0;e+e-&rarrr;e +e-cc&d1;X&parr0;=9 23±69±109±222pb. The differential cross sections d s /dpT(D*±) and d s /d:η(D*±): are also measured as functions of transverse momentum pT(D*±) and the absolute value of pseudorapidity :η(D*±):, respectively. A fit to the data estimating the relative contributions of Direct and Resolved open charm production mechanisms is performed, giving (28.7 ± 5.6)% and (71.3 ± 8.8)%, respectively. Using those relative fractions, the Direct and Resolved process cross sections yield: s&p...

  7. High-order dispersion effects in two-photon interference

    Science.gov (United States)

    Mazzotta, Zeudi; Cialdi, Simone; Cipriani, Daniele; Olivares, Stefano; Paris, Matteo G. A.

    2016-12-01

    Two-photon interference and Hong-Ou-Mandel (HOM) effect are relevant tools for quantum metrology and quantum information processing. In optical coherence tomography, the HOM effect is exploited to achieve high-resolution measurements with the width of the HOM dip being the main parameter. On the other hand, applications like dense coding require high-visibility performance. Here we address high-order dispersion effects in two-photon interference and study, theoretically and experimentally, the dependence of the visibility and the width of the HOM dip on both the pump spectrum and the downconverted photon spectrum. In particular, a spatial light modulator is exploited to experimentally introduce and manipulate a custom phase function to simulate the high-order dispersion effects. Overall, we show that it is possible to effectively introduce high-order dispersion effects on the propagation of photons and also to compensate for such effect. Our results clarify the role of the different dispersion phenomena and pave the way for optimization procedures in quantum technological applications involving PDC photons and optical fibers.

  8. Theory of Two-Photon Absorptions in Graphene Fragments

    Science.gov (United States)

    Aryanpour, K.; Shukla, A.; Mazumdar, S.; Sandhu, A.; Roberts, A.

    2012-02-01

    Electron-electron correlations in graphene is currently an active field of research [1-3]. The carbon atoms in graphene have the same sp^2 hybridization as in strongly correlated π-conjugated polymer systems. The low energy behavior in graphene however appears to be reasonably described within the one-electron Dirac massless fermions model. Historically, the occurrence of the lowest two-photon state below the optical one-photon state provided the strongest proof for strong electron correlations in linear polyenes [4]. We systematically study the Coulomb interaction effects on the ground state and nonlinear absorptions in graphene fragments as a function of system size, beginning from the smallest stable fragment coronene. We report high order calculations of one- vs two-photon spin singlet and triplet states, in coronene, hexabenzocoronene and other molecular fragments that clearly indicate the strong role of electron-electron interactions. We will discuss the implications of our work on molecular systems for the thermodynamic limit of graphene. [4pt] [1] Siegel David A.; et al., PNAS, v108, 28, 11365-11369 (2011)[0pt] [2] Gr"onqvist J. H.; et al., arXiv: 1107.5653v1[0pt] [3] Uchoa B.; et al., arXiv: 1109.1577v1[0pt] [4] Ramasesha S.; et al., J. Chem. Phys. 80, 3278 (1984)

  9. Simultaneous two-photon excitation of photodynamic therapy agents

    Science.gov (United States)

    Wachter, Eric A.; Partridge, W. P., Jr.; Fisher, Walter G.; Dees, Craig; Petersen, Mark G.

    1998-07-01

    The spectroscopic and photochemical properties of several photosensitive compounds are compared using conventional single-photon excitation (SPE) and simultaneous two-photon excitation (TPE). TPE is achieved using a mode-locked titanium:sapphire laser, the near infrared output of which allows direct promotion of non-resonant TPE. Excitation spectra and excited state properties of both type I and type II photodynamic therapy (PDT) agents are examined. In general, while SPE and TPE selection rules may be somewhat different, the excited state photochemical properties are equivalent for both modes of excitation. In vitro promotion of a two-photon photodynamic effect is demonstrated using bacterial and human breast cancer models. These results suggest that use of TPE may be beneficial for PDT, since the technique allows replacement of visible or ultraviolet excitation with non- damaging near infrared light. Further, a comparison of possible excitation sources for TPE indicates that the titanium:sapphire laser is exceptionally well suited for non- linear excitation of PDT agents in biological systems due to its extremely short pulse width and high repetition rate; these features combine to effect efficient PDT activation with minimal potential for non-specific biological damage.

  10. Two-Photon Widths of the chi_cJ States of Charmonium

    CERN Document Server

    Ecklund, K M; Savinov, V; López, A; Méndez, H; Ramírez, J; Ge, J Y; Miller, D H; Shipsey, I P J; Xin, B; Adams, G S; Anderson, M; Cummings, J P; Danko, I; Hu, D; Moziak, B; Napolitano, J; He, Q; Insler, J; Muramatsu, H; Park, C S; Thorndike, E H; Yang, F; Artuso, M; Blusk, S; Khalil, S; Li, J; Mountain, R; Nisar, S; Randrianarivony, K; Sultana, N; Skwarnicki, T; Stone, S; Wang, J C; Zhang, L M; Bonvicini, G; Cinabro, D; Dubrovin, M; Lincoln, A; Naik, P; Rademacker, J; Asner, D M; Edwards, K W; Reed, J; Briere, R A; Ferguson, T; Tatishvili, G; Vogel, H; Watkins, M E; Rosner, J L; Alexander, J P; Cassel, D G; Duboscq, J E; Ehrlich, R; Fields, L; Galik, R S; Gibbons, L; Gray, R; Gray, S W; Hartill, D L; Hertz, D; Hunt, J M; Kandaswamy, J; Kreinick, D L; Kuznetsov, V E; Ledoux, J; Mahlke-Krüger, H; Mohapatra, D; Onyisi, P U E; Patterson, J R; Peterson, D; Riley, D; Ryd, A; Sadoff, A J; Shi, X; Stroiney, S; Sun, W M; Wilksen, T; Athar, S B; Patel, R; Yelton, J; Rubin, P; Eisenstein, B I; Karliner, I; Mehrabyan, S; Lowrey, N; Selen, M; White, E J; Wiss, J; Mitchell, R E; Shepherd, M R; Besson, D; Pedlar, T K; Cronin-Hennessy, D; Gao, K Y; Hietala, J; Kubota, Y; Klein, T; Lang, B W; Poling, R; Scott, A W; Zweber, P; Dobbs, S; Metreveli, Z; Seth, K K; Tomaradze, A G; Libby, J; Powell, A; Wilkinson, G

    2008-01-01

    Using a data sample of 24.5 million psi(2S) the reactions psi(2S)->gamma chi_cJ, chi_cJ->gamma gamma have been studied for the first time to determine the two-photon widths of the chi_cJ states of charmonium in their decay into two photons. The measured quantities are B(psi(2S)->gamma chi_c0)xB(chi_c0->gamma gamma)=(2.22+-0.32+-0.10)x10^-5, and B(psi(2S)->gamma chi_c2)xB(chi_c2->gamma gamma)=(2.70+-0.28+-0.15)x10^-5. Using values for B(psi(2S)->gamma chi_c0,c2) and \\Gamma(chi_c0,c2) from the literature the two-photon widths are derived to be \\Gamma_{gamma gamma}(chi_c0)=(2.53+-0.37+-0.26) keV, \\Gamma_{gamma gamma}(chi_c2)=(0.60+-0.06+-0.06) keV, and R=\\Gamma_{gamma gamma}(chi_c2)/\\Gamma_{gamma gamma}(chi_c0)= 0.237+-0.043+-0.034. The importance of the measurement of R is emphasized. For the forbidden transition, chi_c1->gamma gamma, an upper limit of \\Gamma_{gamma gamma}(chi_c1)<0.03 keV is established.

  11. Free electron laser induced two-photon photoconductivity in Hg1-xCdxTe

    Institute of Scientific and Technical Information of China (English)

    YUAN; Xianzhang

    2001-01-01

    [1]Nathan, V., Guenther, A. H., Mitra, S. S., Review of multiphoton absortion in crystalline solids, J. Opt. Soc. Am. B, 1985, 2: 294—316.[2]Gibson, A. F., Hatch, C. B., Maggs, P. N. D. et al., Two-photon absorption in indium antimonide and germanium, J. Phys., C, 1976, 9: 3259—3275.[3]Miller, A., Johnston, A., Dempsey, J. et al., Two-photon absorption in InSb and Hg1-xCdxTe, J. Phys. C, 1929, 12: 4839—4849.[4]Burghoorn, J., Anderegg, V. F., Klaassen, T. O. et al., Free electron laser induced two-photon absorption in Hg1-xCdxTe, Appl. Phys. Lett., 1992, 61(19): 2320—2322.[5]Hui, Z. X., Yang, Z. H., Free Electron Laser (in Chinese), Beijing: National Defense Industry Press, 1995, 7—8.[6]Matter, J. C., Smirt, A. L., Scully, M. O., Saturable transmission in mercury cadmium telluride, Appl. Phys. Lett., 1976, 28(9): 507—509.[7]Nurmikko, A. V., Nonlinear absorption at 10.6 μm in Hg1-xCdxTe, Optics Communications, 1976, 18(4): 522—524.[8]Catalano, I. M., Cingolani, A., Minafra, A., Multiphoton transitions in ionic crystals, Phys. Rev. B, 1972, 5(4): 1629—1632.[9]Blakemore, J. S., Semiconductor Statistics, Oxford: Pergamon, 1962, 221—222.[10]Shen, S. C., Optical Property of Semiconductor (in Chinese), Beijing: Science Press, 1992, 392—394.

  12. Theoretical analysis and system design of two-photon based optical frequency standards

    Science.gov (United States)

    Burger, J. P.; Jivan, P.; Matthee, C.; Kritzinger, R.; Hussein, H.; Terra, O.

    2014-06-01

    The National Metrology Institute of South Africa (NMISA) is developing a new optical frequency standard based on the Rubidium two-photon transition in collaboration with the National Institute of Standards (NIS, Egypt) that will use both bulk and fiber optics in the system. This is system is called A-POD; an acronym for a portable photonic oscillator device. Rubidium two-photon standards can yield relatively simple and precise standards that are compatible with standard Ti:Sapphire optical frequency combs, as well as the need for a precise frequency standard in the optical telecommunication domain and for measurement of length with a visible beam. The robustness and transportability of the standard are important considerations for the optical frequency standard. This projects implements a framework for better two-photon standards that can be highly accurate, and possibly compete with much more complex clocks in the metrology environment, and especially so in the smaller national metrology institutes found in the developing world. This paper discusses the design constraints and the development considerations towards the optical setup. The robustness and transportability was greatly improved via the usage of optical fiber in the light source of the system, or even in atom-light interaction region. Of particular importance are the beam parameters inside the atomic interaction area. The extent of Doppler broadening and the intensity dependent line shift have to be optimized within practical extents, where both these aspects are affected by the beam shape and optical geometry. A way to fully treat the optical beam effects together with atomic movement is proposed. Furthermore a method is proposed to do real time compensation of intensity dependent light shift, which could have major applicability to frequency standards in general - the complexity is shifted from physical setups to digital signal processing, which is easily adaptable and stable.

  13. A [111]-Cut Si Hemisphere Two-Photon Response Photodetector

    Institute of Scientific and Technical Information of China (English)

    LIU Xiu-Huan; CHEN Zhan-Guo; JIA Gang; WANG Hai-Yan; GAO Yan-Jun; LI Yi1

    2011-01-01

    Properties of two-photon response in a [lll]-cut nearly-intrinsic Si hemisphere photodetector are studied. The measured photocurrent of the photodetector responding to the 1.32μm continuous wave laser shows a quadratic dependence on the coupled optical power and is saturated with the bias voitage. Also, the photocurrent is independent of polarization. Such properties are in good agreement with the theory of two-photon absorption. The isotropic photocurrent generated from the [lll]-cut Si hemisphere is compared to the anisotropic one induced in the [110]-cut Si sample and the ratio of Xxxxx /Xxxyy for silicon performing at 1.32μm is calculated to be 2.4 via the fitted function of the anisotropic photocurrent from the [110]-cut sample.%Properties of two-photon response in a [111]-cut nearly-intrinsic Si hemisphere photodetector are studied.The measured photocurrent of the photodetector responding to the 1.32 μm continuous wave laser shows a quadratic dependence on the coupled optical power and is saturated with the bias voltage.Also,the photocurrent is independent of polarization.Such properties are in good agreement with the theory of two-photon absorption.The isotropic photocurrent generated from the [111]-cut Si hemisphere is compared to the anisotropic one induced in the [110]-cut Si sample and the ratio of Xxxxx /Xxxyy for silicon performing at 1.32μm is calculated to be 2.4via the fitted function of the anisotropic photocurrent from the [110]-cut sample.Silicon materials have a variety of applications in microelectronics and silicon optoelectronics and are still attractive to relevant researchers.Commercial Si photodetectors are largely designed based on singlephoton absorption (SPA).However,nonlinear characteristics have been exhibited in silicon devices.Specifically,two-photon absorption (TPA) has attracted much attention in such devices of Si p-n and p-i-n photodiodes,Si waveguides and Si avalanche diodes,etc.for the autocorrelation measurements of

  14. Remote preparation of complex spatial states of single photons and verification by two-photon coincidence experiment.

    Science.gov (United States)

    Kang, Yoonshik; Cho, Kiyoung; Noh, Jaewoo; Vitullo, Dashiell L P; Leary, Cody; Raymer, M G

    2010-01-18

    We propose and provide experimental evidence in support of a theory for the remote preparation of a complex spatial state of a single photon. An entangled two-photon source was obtained by spontaneous parametric down-conversion, and a double slit was placed in the path of the signal photon as a scattering object. The signal photon was detected after proper spatial filtering so that the idler photon was prepared in the corresponding single-photon state. By using a two-photon coincidence measurement, we obtained the Radon transform, at several longitudinal distances, of the single-photon Wigner distribution function modified by the double slit. The experimental results are consistent with the idler photon being in a pure state. An inverse Radon transformation can, in principle, be applied to the measured data to reconstruct the modified single-photon Wigner function, which is a complete representation of the amplitude and phase structure of the scattering object.

  15. Measurement of Ultra-Short Single-Photon Pulse Duration with Two-Photon Interference

    Institute of Scientific and Technical Information of China (English)

    LV Fan; SUN Fang-Wen; ZOU Chang-Ling; HAN Zheng-Fu; GUO Guang-Can

    2011-01-01

    We proposed a protocol of measuring the duration of ultra-short single-photon pulse with two-photon interference.The pulse duration can be obtained from the width of the visibility of two-photon Hong-Ou-Mandel interference or the indistinguishability of the two photons. Moreover, the shape of a single-photon pulse can be measured with ultra-short single-photon pulses through the two-photon interference.%@@ We proposed a protocol of measuring the duration of ultra-short single-photon pulse with two-photon interference.The pulse duration can be obtained from the width of the visibility of two-photon Hong-Ou-Mandel interference or the indistinguishability of the two photons.Moreover, the shape of a single-photon pulse can be measured with ultra-short single-photon pulses through the two-photon interference.

  16. Observation of Rydberg Series in Sodium Vapour by Two-Photon Resonant Nondegenerate Four-Wave Mixing

    Institute of Scientific and Technical Information of China (English)

    王延帮; 姜谦; 李隆; 米辛; 俞祖和; 傅盘铭

    2001-01-01

    We apply two-photon resonant nondegenerate four-wave mixing with a resonant intermediate state for the obser- vation of Rydberg states in sodium vapour. The broadening and shift of the sodium 3S- 11D transition perturbed by argon are investigated. This technique can achieve Doppler-free resolution of narrow spectral structures of Rydberg levels if lasers with narrow bandwidths are employed.

  17. Suppression and Enhancement in Parametric Two-Photon Resonant Nondegenerate Four-Wave Mixing via Quantum Interference

    Institute of Scientific and Technical Information of China (English)

    SUN Jiang; MI Xin; YU Zu-He; JIANG Qian; ZUO Zhan-Chun; WANG Yan-Bang; WU Ling-An; FU Pan-Ming

    2004-01-01

    @@ Quantum interference may lead to suppression and enhancement of the two-photon resonant nondegenerate fourwave mixing signal in a cascade four-level system. Such phenomena are demonstrated in Ba through inducing atomic coherence between the ground state 6s2 and the doubly excited autoionizing Rydberg state 6pnd. This method can be used as a new spectroscopic tool for measuring the transition dipole moment between two highly excited atomic states.

  18. Electromagnetically induced absorption and transparency in an optical-rf two-photon coupling configuration

    Energy Technology Data Exchange (ETDEWEB)

    Fu Guangsheng [College of Physical Science and Technology, Hebei University, Baoding 071002 (China); Li Xiaoli [College of Physical Science and Technology, Hebei University, Baoding 071002 (China)], E-mail: xiaolixiaoli001@yahoo.com.cn; Zhuang Zhonghong; Zhang Lianshui; Yang Lijun; Li Xiaowei; Han Li [College of Physical Science and Technology, Hebei University, Baoding 071002 (China); Manson, Neil B.; Wei Changjiang [Laser Physics Center, Research School of Physical Sciences and Engineering, Australian Nation University, Canberra, ACT 0200 (Australia)

    2008-01-07

    We study electromagnetically induced absorption (EIA) and transparency (EIT) in an optical-rf two-photon coupling configuration. It is shown that the interference effect due to interacting dark resonances results in an EIA for a resonant two-photon coupling and this EIA is observed to evolve into an EIT when there is a detuning in the two-photon coupling.

  19. Effect of heat-induced pain stimuli on pulse transit time and pulse wave amplitude in healthy volunteers.

    Science.gov (United States)

    van Velzen, Marit H N; Loeve, Arjo J; Kortekaas, Minke C; Niehof, Sjoerd P; Mik, Egbert G; Stolker, Robert J

    2016-01-01

    Pain is commonly assessed subjectively by interpretations of patient behaviour and/or reports from patients. When this is impossible the availability of a quantitative objective pain assessment tool based on objective physiological parameters would greatly benefit clinical practice and research beside the standard self-report tests. Vasoconstriction is one of the physiological responses to pain. The aim of this study was to investigate whether pulse transit time (PTT) and pulse wave amplitude (PWA) decrease in response to this vasoconstriction when caused by heat-induced pain. The PTT and PWA were measured in healthy volunteers, on both index fingers using photoplethysmography and electrocardiography. Each subject received 3 heat-induced pain stimuli using a Temperature-Sensory Analyzer thermode block to apply a controlled, increasing temperature from 32.0 °C to 50.0 °C to the skin. After reaching 50.0 °C, the thermode was immediately cooled down to 32.0 °C. The study population was divided into 2 groups with a time-interval between the stimuli 20s or 60s. The results showed a significant (p  <  0.05) decrease of both PTT and PWA on the stimulated and contralateral side. Moreover, there was no significant difference between the stimulated and contralateral side. The time-interval of 20s was too short to allow PTT and PWA to return to baseline values and should exceed 40s in future studies. Heat-induced pain causes a decrease of PTT and PWA. Consequently, it is expected that, in the future, PTT and PWA may be applied as objective indicators of pain, either beside the standard self-report test, or when self-report testing is impossible.

  20. One- and two-photon absorption properties of two metalloporphyrin complexes

    Institute of Scientific and Technical Information of China (English)

    Sun Yuan-Hong; Wang Chuan-Kui

    2011-01-01

    The linear and nonlinear optical properties of two metalloporphyrin complexes formed by the complementary coordination of central zinc or magnesium ions to the ligand 5,10,15-tri-(p-tolyl)-20-phenylethynylporphyrin are theoretically investigated by using the analytic response theory at the density functional theory level.The results indicate that the studied complexes present more symmetric geometry structures than the ligand.The charge-transfer states of the two complexes in the lower energy region are all almost degenerate but those of the ligand are well separated.The ratio of the two-photon absorption cross sections of the ligand,zinc-porphyrin and magnesium-porphyrin complexes is 1.0:1.5:1.8,demonstrating that the two-photon absorption capability can be greatly increased when the ligand is coordinated with a metal ion.Moreover,several physical micro-mechanisms including electron transitions and intramolecular charge-transfer processes are discussed to explore the differences in optical property between the ligand and two complexes.

  1. Controlling nonclassical properties of the two-photon process by a time-varying field

    Institute of Scientific and Technical Information of China (English)

    Jia Fei; Xie Shuang-Yuan; Yang Ya-Ping

    2009-01-01

    The interactions between a two-level atom and a field via two-photon transition without rotating wave approx imation have been investigated.We emphasize the dynamic behaviors of the atomic population inversion,the field squeezing,and the atomic dipole squeezing numerically when the field frequency varies with time in the forms of sine and rectangle.Some interesting phenomena axe discovered and discussed.The good periodic character of the atomic population inversion in the standard two-photon Jaynes-Cummings model is weakened by the influence of the sine field frequency modulation.The rectangular field frequency modulation can change the correlation among different oscillations suddenly and induce new collapse-revival processes of the atomic population inversion.The field squeezing increases at the beginning of time,but then decreases and loses as the time increases after it reaches the maximum due to the sine modulation.The effects of the rectangular modulation on the field squeezing depend mostly on the appear ance time of the modulation.The atomic dipole squeezing is weakened under the influence of the sine or rectangular modulation.Our results indicate that it is possible to perform the dynamic controlling of the system properties by changing the parameters of the system with time.This implies that one can dynamically control a quantum information process by choosing the system modulation properly.

  2. Clinical multiphoton tomography and clinical two-photon microendoscopy

    Science.gov (United States)

    König, Karsten; Bückle, Rainer; Weinigel, Martin; Elsner, Peter; Kaatz, Martin

    2009-02-01

    We report on applications of high-resolution clinical multiphoton tomography based on the femtosecond laser system DermaInspectTM with its flexible mirror arm in Australia, Asia, and Europe. Applications include early detection of melanoma, in situ tracing of pharmacological and cosmetical compounds including ZnO nanoparticles in the epidermis and upper dermis, the determination of the skin aging index SAAID as well as the study of the effects of anti-aging products. In addition, first clinical studies with novel rigid high-NA two-photon 1.6 mm GRIN microendoscopes have been conducted to study the effect of wound healing in chronic wounds (ulcus ulcera) as well as to perform intrabody imaging with subcellular resolution in small animals.

  3. Two-photon resonant, stimulated processes in krypton and xenon

    Energy Technology Data Exchange (ETDEWEB)

    Miller, J.C.

    1988-11-01

    Both on-axis and conical emissions have been observed following two-photon pumping of the 5p states of krypton and the 6p', 7p, 8p, and 4f states of xenon. In the former case, coherent emissions from the 5p states to the 5s are observed, and in the latter case, many p..-->..s, d..-->..p, and f..-->..d cascade emissions are observed. By analogy to the well-studied alkali and alkaline earth examples, the emissions are discussed in terms of amplified spontaneous emission (ASE), stimulated hyper-Raman scattering, and parametric four-wave mixing. The physical processes responsible for the conical emission and for intensity anomalies in the xenon p..-->..s emissions are not understood at present. Interference effects due to coherent cancellation between competing excitation pathways may be occurring. 4 refs., 3 figs.

  4. Whole brain imaging with Serial Two-Photon Tomography

    Directory of Open Access Journals (Sweden)

    Stephen P Amato

    2016-03-01

    Full Text Available Imaging entire mouse brains at submicron resolution has historically been a challenging undertaking and largely confined to the province of dedicated atlasing initiatives. The has limited systematic investigations into important areas of neuroscience, such as neural circuits, brain mapping and neurodegeneration. In this paper, we describe in detail Serial Two-Photon (STP tomography, a robust, reliable method for imaging entire brains with histological detail. We provide examples of how the basic methodology can be extended to other imaging modalities, such as optical coherence tomography, in order to provide unique contrast mechanisms. Furthermore we provide a survey of the research that STP tomography has enabled in the field of neuroscience, provide examples of how this technology enables quantitative whole brain studies, and discuss the current limitations of STP tomography-based approaches

  5. Two-photon assisted clock comparison to picosecond precision

    CERN Document Server

    Zhang, Shi-Wei; Yao, Yin-Ping; Wan, Ren-Gang; Zhang, Tong-Yi

    2015-01-01

    We have experimentally demonstrated a clock comparison scheme utilizing time-correlated photon pairs generated from the spontaneous parametric down conversion process of a laser pumped beta-barium borate crystal. The coincidence of two-photon events are analyzed by the cross correlation of the two time stamp sequences. Combining the coarse and fine part of the time differences at different resolutions, a 64 ps precision for clock synchronization has been realized. We also investigate the effects of hardware devices used in the system on the precision of clock comparison. The results indicate that the detector's time jitter and the background noise will degrade the system performance. With this method, comparison and synchronization of two remote clocks could be implemented with a precision at the level of a few tens of picoseconds.

  6. Measurement of bottom quark production in two photon collisions

    CERN Document Server

    Saremi, Sepehr

    2001-01-01

    The cross section for bottom quark production in two-photon collisions, sigma( e+e- → e+e- bb¯X), is measured for the first time. The measurement is performed with the L3 detector at the Large Electron Positron (LEP) collider at the European Center for Nuclear and Particle Physics (CERN). The data corresponds to 410 pb-1 taken at center-of-mass energies from 189 GeV to 202 GeV. Hadrons containing a bottom quark are identified by detecting electrons or muons from their semi-leptonic decays. The measured cross section is in excess of the Next to Leading Order QCD prediction by a factor of three.

  7. High contrast two-photon imaging of fingermarks

    Science.gov (United States)

    Stoltzfus, Caleb R.; Rebane, Aleksander

    2016-04-01

    Optically-acquired fingermarks are widely used as evidence across law enforcement agencies as well as in the courts of law. A common technique for visualizing latent fingermarks on nonporous surfaces consists of cyanoacrylate fuming of the fingerprint material, followed by impregnation with a fluorescent dye, which under ultra violet (UV) illumination makes the fingermarks visible and thus accessible for digital recording. However, there exist critical circumstances, when the image quality is compromised due to high background scattering, high auto-fluorescence of the substrate material, or other detrimental photo-physical and photo-chemical effects such as light-induced damage to the sample. Here we present a novel near-infrared (NIR), two-photon induced fluorescence imaging modality, which significantly enhances the quality of the fingermark images, especially when obtained from highly reflective and/or scattering surfaces, while at the same time reducing photo-damage to sensitive forensic samples.

  8. Optically Pumped Atomic Rubidium Lasers: Two-Photon and Exciplex Excitation Mechanisms

    Science.gov (United States)

    Gallagher, Jeffrey E.

    The Doppler-broadened two-photon absorption (TPA) cross-section for the 52S1/2 → 52 D5/2 transition in Rb is measured using direct absorption methods. The selection rule |DeltaF| ≤ 2 applied to both isotopes yields 17 transitions in 3 Doppler limited lines. A detailed model of the intensity profile was also developed to account for a focused Gaussian beam (with an M2 value of 1.09) propagating through a two-photon absorption medium. A peak absorbance of 24% was observed for an intensity of 6.28 kWcm2 at the focus, a Rb density of 4.6x1015 cm-3 , and a path length of 15 cm. Alkali concentrations from 1.61 - 8.52x1015 cm -3 were monitored in the far wing of the D 2 line. Extracting the hyperfine-broadened TPA cross-section from 87 test configurations, while varying the pump power, alkali concentration and focal length, yielded an error-weighted average of 6.75x10^-21 cm4W with a standard deviation of 3.61x10-21 cm4W. This cross-section is sufficient for a pulsed dye laser to bleach the pump transition in the Two-Photon Pumped Alkali Laser (TPAL) that lases at 420 nm and 5.2 microm. Optically pumped atomic rubidium lasers pumped in the blue satellite of the D2 line from the ground Rb-Ar or Rb-Kr collision pair to the dissociative B2S+1/2 state produce laser emission at 780.2 nm. Lasing is achieved for pump wavelengths of 752.3 to greater than 760 nm for the Rb-Ar system and 757.1 -- 760.4 nm for the Rb-Kr system. Slope efficiencies increase with both Rb and Ar concentrations and exceed 0.25% using a heat pipe configuration. The gain is very high with photon build-up times of 1--3.7 ns. Laser induced heating and subsequent condensation of alkali vapor in the heat pipe configuration currently limits operation to less than 2500 Torr.

  9. Theoretical analysis on two-photon absorption spectroscopy in a confined four-level atomic system

    Institute of Scientific and Technical Information of China (English)

    Yuanyuan Li; Jintao Bai; Li Li; Yanpeng Zhang; Xun Hou

    2009-01-01

    We investigate theoretically two-photon absorption spectroscopy modified by a control field in a confined Y-type four-level system. Dicke-narrowing effect occurs both in two-photon absorption lines and the dips of transparency against two-photon absorption due to enhanced contribution of slow atoms. We also find that the suppression and the enhancement of two-photon absorption can be modified by changing the strength of the control field and the detuning of three laser fields. This control of two-photon absorption may have some applications in information processing and optical devices.

  10. Two-photon STED spectral determination for a new V-shaped organic fluorescent probe with efficient two-photon absorption.

    Science.gov (United States)

    Belfield, Kevin D; Bondar, Mykhailo V; Morales, Alma R; Padilha, Lazaro A; Przhonska, Olga V; Wang, Xuhua

    2011-10-24

    Two-photon stimulated emission depletion (STED) cross sections were determined over a broad spectral range for a novel two-photon absorbing organic molecule, representing the first such report. The synthesis, comprehensive linear photophysical, two-photon absorption (2PA), and stimulated emission properties of a new fluorene-based compound, (E)-2-{3-[2-(7-(diphenylamino)-9,9-diethyl-9H-fluoren-2-yl)vinyl]-5-methyl-4-oxocyclohexa-2,5-dienylidene} malononitrile (1), are presented. Linear spectral parameters, including excitation anisotropy and fluorescence lifetimes, were obtained over a broad range of organic solvents at room temperature. The degenerate two-photon absorption (2PA) spectrum of 1 was determined with a combination of the direct open-aperture Z-scan and relative two-photon-induced fluorescence methods using 1 kHz femtosecond excitation. The maximum value of the 2PA cross section ~1700 GM was observed in the main, long wavelength, one-photon absorption band. One- and two-photon stimulated emission spectra of 1 were obtained over a broad spectral range using a femtosecond pump-probe technique, resulting in relatively high two-photon stimulated emission depletion cross sections (~1200 GM). A potential application of 1 in bioimaging was demonstrated through one- and two-photon fluorescence microscopy images of HCT 116 cells incubated with micelle-encapsulated dye.

  11. New design strategy for the two-photon active material based on push-pull substituted bisanthene molecule.

    Science.gov (United States)

    Chattopadhyaya, Mausumi; Alam, Md Mehboob; Chakrabarti, Swapan

    2011-03-31

    In the present work, we have critically examined the origin of strong two-photon transition probability of a donor-acceptor substituted bisanthene molecule that imitates a small piece of edge passivated (4, 4) graphene nanoribbon. In our calculations, we have considered -OMe, and -NH(2) as donors and -NO(2) as an acceptor. The one- and two-photon absorption parameters are evaluated using state-of-the-art linear and quadratic response theory, respectively, and all these calculations are carried out within the framework of time dependent density functional theory. To give a proper judgment on our findings, we have used the long-range corrected CAMB3LYP functional for all of the time dependent calculations. The present investigation reveals that the bisanthene molecule with three pairs of donor/acceptor moiety has a lower two-photon transition probability than that of a suitably designed bisanthene with only a single pair of donor/acceptor moiety. This in silico observation is consistent for all of the donor/acceptor moieties chosen in the present work. A comprehensive analysis at the two state model level of theory clearly offers us a verdict that by placing the donor/acceptor moiety in a suitable position of bisanthene, we can create a significant asymmetry in the electron density in the first excited state, which eventually leads to a significant difference in the ground and excited state dipole moment and is attributed to the higher two-photon transition probability of a particular bisanthene with a single pair of donor/acceptor moiety than bisanthene with three pairs of donor/acceptor.

  12. Coherent blue emission generated by Rb two-photon excitation using diode and femtosecond lasers

    Science.gov (United States)

    Lopez, Jesus P.; Moreno, Marco P.; de Miranda, Marcio H. G.; Vianna, Sandra S.

    2017-04-01

    The coherent blue light generated in rubidium vapor due to the combined action of an ultrashort pulse train and a continuous wave diode laser is investigated. Each step of the two-photon transition 5S-5P{}3/2-5D is excited by one of the lasers, and the induced coherence between the 5S and 6P{}3/2 states is responsible for generating the blue beam. Measurements of the excitation spectrum reveal the frequency comb structure and allow us to identify the resonant modes responsible for inducing the nonlinear process. Further, each resonant mode excites a different group of atoms, making the process selective in atomic velocity. The signal dependency on the atomic density is characterized by a sharp growth and a rapid saturation. We also show that for high intensity of the diode laser, the Stark shift at resonance causes the signal suppression observed at low atomic density.

  13. Two-Photon Ghost Image and Interference-Diffraction

    Science.gov (United States)

    Shih, Y. H.; Sergienko, A. V.; Pittman, T. B.; Strekalov, D. V.; Klyshko, D. N.

    1996-01-01

    One of the most surprising consequences of quantum mechanics is entanglement of two or more distance particles. The two-particle entangled state was mathematically formulated by Schrodinger. Based on this unusual quantum behavior, EPR defined their 'physical reality' and then asked the question: 'Can Quantum-Mechanical Description of Physical Reality Be Considered Complete?' One may not appreciate EPR's criterion of physical reality and insist that 'no elementary quantum phenomenon is a phenomenon until it is a recorded phenomenon'. Optical spontaneous parametric down conversion (SPDC) is the most effective mechanism to generate an EPR type entangled two-photon state. In SPDC, an optical beam, called the pump, is incident on a birefringent crystal. The pump is intense enough so that nonlinear effects lead to the conversion of pump photons into pairs of photons, historically called signal and idler. Technically, the SPDC is said to be type-1 or type-2, depending on whether the signal and idler beams have parallel or orthogonal polarization. The SPDC conversion efficiency is typically on the order of 10(exp -9) to 10(exp -11), depending on the SPDC nonlinear material. The signal and idler intensities are extremely low, only single photon detection devices can register them. The quantum entanglement nature of SPDC has been demonstrated in EPR-Bohm experiments and Bell's inequality measurements. The following two experiments were recently performed in our laboratory, which are more closely related to the original 1935 EPR gedankenezperiment. The first experiment is a two-photon optical imaging type experiment, which has been named 'ghost image' by the physics community. The signal and idler beams of SPDC are sent in different directions, so that the detection of the signal and idler photons can be performed by two distant photon counting detectors. An aperture object (mask) is placed in front of the signal photon detector and illuminated by the signal beam through a

  14. Theory of deep ultraviolet generation at maximum coherence assisted by Stark-chirped two-photon resonance

    CERN Document Server

    Myslivets, S A; Kimberg, V V; George, T F; George, Thomas F.

    2003-01-01

    A scheme is analyzed for effcient generation of vacuum ultraviolet radiation through four-wave mixing processes assisted by the technique of Stark-chirped rapid adiabatic passage. These opportunities are associated with pulse excitation of laddertype short-wavelength two-photon atomic or molecular transitions so that relaxation processes can be neglected. In this three-laser technique, a delayed-pulse of strong oR-resonant infrared radiation sweeps the laser-induced Stark-shift of a two-photon transition in a such way that facilitates robust maximum two-photon coherence induced by the first ultraviolet laser. A judiciously delayed third pulse scatters at this coherence and generates short-wavelength radiation. A theoretical analysis of these problems based on the density matrix is performed. A numerical model is developed to carry out simulations of a typical experiment. The results illustrate a behavior of populations, coherence and generated radiation along the medium as well as opportunities of effcient ge...

  15. Higgs Decay into Two Photons at the Boundary of a Warped Extra Dimension

    CERN Document Server

    Hahn, Juliane; Malm, Raoul; Neubert, Matthias; Novotny, Kristiane; Schmell, Christoph

    2013-01-01

    A detailed, five-dimensional calculation of the Higgs decay process into two photons is performed in the minimal and custodially protected Randall-Sundrum (RS) model, where the Standard Model (SM) fields propagate in the bulk and the scalar sector is localized on or lives near the IR brane. It is explicitly shown that the $R_\\xi$ gauge invariance of the sum of diagrams involving bosonic fields in the SM also applies to the case of the discussed RS scenarios. For the first time, an exact expression for the $h\\rightarrow \\gamma\\gamma$ amplitude in terms of the five-dimensional fermion and $W$-boson propagators is derived, which includes the full dependence on the Higgs boson mass. The 5D $W$-boson propagators in both the minimal and the custodial RS model are exactly derived to all orders in $v^2/M_{\\rm{KK}}^2$ keeping the full momentum dependence. It is shown that, in contrast to the fermion case, the final results of the $W$-boson amplitudes are identical for the brane-localized and the narrow bulk-Higgs scen...

  16. Nuclear Jacobi and Poincaré transitions at high spins and temperatures: Account of dynamic effects and large-amplitude motion

    Science.gov (United States)

    Mazurek, K.; Dudek, J.; Maj, A.; Rouvel, D.

    2015-03-01

    We present a theoretical analysis of the competition between the so-called nuclear Jacobi and Poincaré shape transitions as a function of spin at high temperatures. The latter condition implies the method of choice, a realistic version of the nuclear liquid drop model, here the Lublin-Strasbourg drop model. We address specifically the fact that the Jacobi and Poincaré shape transitions are accompanied by the flattening of the total nuclear energy landscape as a function of the relevant deformation parameters, which enforces large-amplitude oscillation modes that need to be taken into account. For that purpose we introduce an approximate form of the collective Schrödinger equation whose solutions are used to calculate the most probable deformations associated with the nuclear Jacobi and Poincaré transitions. We discuss selected aspects of the new description focusing on the critical-spin values for both types of these transitions.

  17. Nuclear Jacobi and Poincar\\'e Transitions at High Spins and Temperatures: Account~of~Dynamic~Effects~and~Large-Amplitude Motion

    CERN Document Server

    Mazurek, K; Maj, A; Rouvel, D

    2013-01-01

    We present a theoretical analysis of the competition between so-called nuclear Jacobi and Poincar\\'e shape transitions in function of spin - at high temperatures. The latter condition implies the method of choice - a realistic version of the nuclear Liquid Drop Model (LDM), here: the Lublin-Strasbourg Drop (LSD) model. We address specifically the fact that the Jacobi and Poincar\\'e shape transitions are accompanied by the flattening of total nuclear energy landscape as function of the relevant deformation parameters what enforces large amplitude oscillation modes that need to be taken into account. For that purpose we introduce an approximate form of the collective Schr\\"odinger equation whose solutions are used to calculate the most probable deformations associated with both types of transitions and discuss the physical consequences in terms of the associated critical-spin values and transitions themselves.

  18. Atomic homodyne detection of weak atomic transitions.

    Science.gov (United States)

    Gunawardena, Mevan; Elliott, D S

    2007-01-26

    We have developed a two-color, two-pathway coherent control technique to detect and measure weak optical transitions in atoms by coherently beating the transition amplitude for the weak transition with that of a much stronger transition. We demonstrate the technique in atomic cesium, exciting the 6s(2)S(1/2) --> 8s(2)S(1/2) transition via a strong two-photon transition and a weak controllable Stark-induced transition. We discuss the enhancement in the signal-to-noise ratio for this measurement technique over that of direct detection of the weak transition rate, and project future refinements that may further improve its sensitivity and application to the measurement of other weak atomic interactions.

  19. Two-photon polymerization for fabrication of biomedical devices

    Science.gov (United States)

    Ovsianikov, Aleksandr; Doraiswamy, Anand; Narayan, R.; Chichkov, B. N.

    2007-01-01

    Two-photon polymerization (2PP) is a novel technology which allows the fabrication of complex three-dimensional (3D) microstructures and nanostructures. The number of applications of this technology is rapidly increasing; it includes the fabrication of 3D photonic crystals [1-4], medical devices, and tissue scaffolds [5-6]. In this contribution, we discuss current applications of 2PP for microstructuring of biomedical devices used in drug delivery. While in general this sector is still dominated by oral administration of drugs, precise dosing, safety, and convenience are being addressed by transdermal drug delivery systems. Currently, main limitations arise from low permeability of the skin. As a result, only few types of pharmacological substances can be delivered in this manner [7]. Application of microneedle arrays, whose function is to help overcome the barrier presented by the epidermis layer of the skin, provides a very promising solution. Using 2PP we have fabricated arrays of hollow microneedles with different geometries. The effect of microneedle geometry on skin penetration is examined. Our results indicate that microneedles created using 2PP technique are suitable for in vivo use, and for integration with the next generation of MEMS- and NEMS-based drug delivery devices.

  20. Review of two-photon exchange in electron scattering

    Energy Technology Data Exchange (ETDEWEB)

    J. Arrington, P. G. Blunden, W. Melnitchouk

    2011-10-01

    We review the role of two-photon exchange (TPE) in electron-hadron scattering, focusing in particular on hadronic frameworks suitable for describing the low and moderate Q^2 region relevant to most experimental studies. We discuss the effects of TPE on the extraction of nucleon form factors and their role in the resolution of the proton electric to magnetic form factor ratio puzzle. The implications of TPE on various other observables, including neutron form factors, electroproduction of resonances and pions, and nuclear form factors, are summarized. Measurements seeking to directly identify TPE effects, such as through the angular dependence of polarization measurements, nonlinear epsilon contributions to the cross sections, and via e+p to e-p cross section ratios, are also outlined. In the weak sector, we describe the role of TPE and gamma-Z interference in parity-violating electron scattering, and assess their impact on the extraction of the strange form factors of the nucleon and the weak charge of the proton.

  1. Two-Photon-Absorption Scheme for Optical Beam Tracking

    Science.gov (United States)

    Ortiz, Gerardo G.; Farr, William H.

    2011-01-01

    A new optical beam tracking approach for free-space optical communication links using two-photon absorption (TPA) in a high-bandgap detector material was demonstrated. This tracking scheme is part of the canonical architecture described in the preceding article. TPA is used to track a long-wavelength transmit laser while direct absorption on the same sensor simultaneously tracks a shorter-wavelength beacon. The TPA responsivity was measured for silicon using a PIN photodiode at a laser beacon wavelength of 1,550 nm. As expected, the responsivity shows a linear dependence with incident power level. The responsivity slope is 4.5 x 10(exp -7) A/W2. Also, optical beam spots from the 1,550-nm laser beacon were characterized on commercial charge coupled device (CCD) and complementary metal-oxide semiconductor (CMOS) imagers with as little as 13.7 microWatts of optical power (see figure). This new tracker technology offers an innovative solution to reduce system complexity, improve transmit/receive isolation, improve optical efficiency, improve signal-to-noise ratio (SNR), and reduce cost for free-space optical communications transceivers.

  2. Two-photon excited photoconversion of cyanine-based dyes

    Science.gov (United States)

    Kwok, Sheldon J. J.; Choi, Myunghwan; Bhayana, Brijesh; Zhang, Xueli; Ran, Chongzhao; Yun, Seok-Hyun

    2016-03-01

    The advent of phototransformable fluorescent proteins has led to significant advances in optical imaging, including the unambiguous tracking of cells over large spatiotemporal scales. However, these proteins typically require activating light in the UV-blue spectrum, which limits their in vivo applicability due to poor light penetration and associated phototoxicity on cells and tissue. We report that cyanine-based, organic dyes can be efficiently photoconverted by nonlinear excitation at the near infrared (NIR) window. Photoconversion likely involves singlet-oxygen mediated photochemical cleavage, yielding blue-shifted fluorescent products. Using SYTO62, a biocompatible and cell-permeable dye, we demonstrate photoconversion in a variety of cell lines, including depth-resolved labeling of cells in 3D culture. Two-photon photoconversion of cyanine-based dyes offer several advantages over existing photoconvertible proteins, including use of minimally toxic NIR light, labeling without need for genetic intervention, rapid kinetics, remote subsurface targeting, and long persistence of photoconverted signal. These findings are expected to be useful for applications involving rapid labeling of cells deep in tissue.

  3. Two-photon autofluorescence spectroscopy of oral mucosa tissue

    Science.gov (United States)

    Edward, Kert; Shilagard, Tuya; Qiu, Suimin; Vargas, Gracie

    2011-03-01

    The survival rate for individuals diagnosed with oral cancer is correlated with the stage of detection. Thus the development of novel techniques for the earliest possible detection of malignancies is of critical importance. Single photon (1P) autofluorescence spectroscopy has proven to be a powerful diagnostic tool in this regard, but 2P (two photon) spectroscopy remains essentially unexplored. In this investigation, a spectroscopic system was incorporated into a custom-built 2P laser scanning microscope. Oral cancer was induced in the buccal pouch of Syrian Golden hamsters by tri-weekly topical application of 9,10-dimethyl-1,2-benzanthracene (DMBA).Three separated sites where investigated in each hamster at four excitation wavelengths from 780 nm to 890 nm. A Total of 8 hamsters were investigated (4 normal and 4 DMBA treated). All investigated sites were imaged via 2p imaging, marked for biopsy, processed for histology and H&E staining, and graded by a pathologist. The in vivo emission spectrum for normal, mild/high grade dysplasia and squamous cell carcinoma is presented. It is shown that the hamsters with various stages of dysplasia are characterized by spectral differences as a function of depth and excitation wavelength, compared to normal hamsters.

  4. Time-resolved two-photon photoemission from metal surfaces

    CERN Document Server

    Weinelt, M

    2002-01-01

    The Rydberg-like series of image-potential states is a prototype system for loosely bound electrons at a metal surface. The electronic structure and the femtosecond dynamics of these states is studied by high-resolution energy-and time-resolved two-photon photoemission spectroscopy. The electron trapped in the image potential moves virtually freely laterally to the surface where it is subject to inelastic and quasielastic scattering processes which cause decay of population and phase relaxation. The influence of surface corrugation on these processes has been investigated for adsorbates on Cu(001) and stepped Cu(117) and Cu(119) surfaces which are vicinal to Cu(001). The dynamics depend on both the distance of the electron in front of the surface and the parallel momentum. For CO molecules on Cu(001) inelastic scattering into bulk states and adsorbate-induced resonances determine the decay rate. For small numbers of Cu adatoms on Cu(001) and the vicinal surfaces the decay rate of image-potential states is sig...

  5. Synergistic Two-Photon Absorption Enhancement in Photosynthetic Light Harvesting

    Science.gov (United States)

    Chen, Kuo-Mei; Chen, Yu-Wei; Gao, Ting-Fong

    2012-06-01

    The grand scale fixation of solar energies into chemical substances by photosynthetic reactions of light-harvesting organisms provides Earth's other life forms a thriving environment. Scientific explorations in the past decades have unraveled the fundamental photophysical and photochemical processes in photosynthesis. Higher plants, green algae, and light-harvesting bacteria utilize organized pigment-protein complexes to harvest solar power efficiently and the resultant electronic excitations are funneled into a reaction center, where the first charge separation process takes place. Here we show experimental evidences that green algae (Chlorella vulgaris) in vivo display a synergistic two-photon absorption enhancement in their photosynthetic light harvesting. Their absorption coefficients at various wavelengths display dramatic dependence on the photon flux. This newly found phenomenon is attributed to a coherence-electronic-energy-transfer-mediated (CEETRAM) photon absorption process of light-harvesting pigment-protein complexes of green algae. Under the ambient light level, algae and higher plants can utilize this quantum mechanical mechanism to create two entangled electronic excitations adjacently in their light-harvesting networks. Concerted multiple electron transfer reactions in the reaction centers and oxygen evolving complexes can be implemented efficiently by the coherent motion of two entangled excitons from antennae to the charge separation reaction sites. To fabricate nanostructured, synthetic light-harvesting apparatus, the paramount role of the CEETRAM photon absorption mechanism should be seriously considered in the strategic guidelines.

  6. Two-photon holographic optogenetics of neural circuits (Conference Presentation)

    Science.gov (United States)

    Yang, Weijian; Carrillo-Reid, Luis; Peterka, Darcy S.; Yuste, Rafael

    2016-03-01

    Optical manipulation of in vivo neural circuits with cellular resolution could be important for understanding cortical function. Despite recent progress, simultaneous optogenetic activation with cellular precision has either been limited to 2D planes, or a very small numbers of neurons over a limited volume. Here we demonstrate a novel paradigm for simultaneous 3D activation using a low repetition rate pulse-amplified fiber laser system and a spatial light modulator (SLM) to project 3D holographic excitation patterns on the cortex of mice in vivo for targeted volumetric 3D photoactivation. This method is compatible with two-photon imaging, and enables the simultaneous activation of multiple cells in 3D, using red-shifted opsins, such as C1V1 or ReaChR, while simultaneously imaging GFP-based sensors such as GCaMP6. This all-optical imaging and 3D manipulation approach achieves simultaneous reading and writing of cortical activity, and should be a powerful tool for the study of neuronal circuits.

  7. Effect of the coherent cancellation of the two-photon resonance on the generation of vacuum ultraviolet light by two-photon reasonantly enhanced four-wave mixing

    Energy Technology Data Exchange (ETDEWEB)

    Payne, M.G.; Garrett, W.R.; Judish, J.P.; Wunderlich, R.

    1988-11-01

    Many of the most impressive demonstrations of the efficient generation of vacuum ultraviolet (VUV) light have made use of two- photon resonantly enhanced four-wave mixing to generate light at ..omega../sub VUV/ = 2..omega../sub L1/ +- ..omega../sub L2/. The two-photon resonance state is coupled to the ground state both by two photons from the first laser, or by a photon from the second laser and one from the generated VUV beam. We show here that these two coherent pathways destructively interfere once the second laser is made sufficiently intense, thereby leading to an important limiting effect on the achievable conversion efficiency. 4 refs.

  8. Tuning Ag29 nanocluster light emission from red to blue with one and two-photon excitation

    Science.gov (United States)

    Russier-Antoine, Isabelle; Bertorelle, Franck; Hamouda, Ramzi; Rayane, Driss; Dugourd, Philippe; Sanader, Željka; Bonačić-Koutecký, Vlasta; Brevet, Pierre-François; Antoine, Rodolphe

    2016-01-01

    GM and the hyperpolarizability is 106 × 10-30 esu at the same excitation wavelength. The two-photon excited fluorescence spectrum appears strongly blue-shifted as compared to the one-photon excited spectrum, displaying a broad band between 400 and 700 nm. The density functional theory (DFT) provides insight into the structural and electronic properties of Ag29(DHLA)12 as well as into interplay between metallic subunit or core and ligands which is responsible for unique optical properties. Electronic supplementary information (ESI) available: CID spectrum of Ag29(DHLA)12, spectroscopic characterization of the synthesized Ag clusters, lifetime measurements of silver cluster, schematic diagram showing the excited state relaxation dynamics, HRS intensity versus wavelength for Ag29(DHLA)12, DFT optimized structures and TDDFT calculated one photon absorption spectra of Ag29(DHLA)12, Leading excitations for transition for prototype structures two-photon cross section for Ag29(DHLA)12 at different wavelengths and optimal setting for the ESI-MS. See DOI: 10.1039/c5nr08122j

  9. Peptide backbone orientation and dynamics in spider dragline silk and two-photon excitation in nuclear magnetic and quadrupole resonance

    Energy Technology Data Exchange (ETDEWEB)

    Eles, P.T

    2005-07-01

    In the first part of the dissertation, spider dragline silk is studied by solid state NMR techniques. The dependence of NMR frequency on molecular orientation is exploited using the DECODER experiment to determine the orientation of the protein backbone within the silk fibre. Practical experimental considerations require that the silk fibres be wound about a cylindrical axis perpendicular to the external magnetic field, complicating the reconstruction of the underlying orientation distribution and necessitating the development of numerical techniques for this purpose. A two-component model of silk incorporating static b-sheets and polyglycine II helices adequately fits the NMR data and suggests that the b-sheets are well aligned along the silk axis (20 FWHM) while the helices are poorly aligned (68 FWHM). The effects of fibre strain, draw rate and hydration on orientation are measured. Measurements of the time-scale for peptide backbone motion indicate that when wet, a strain-dependent fraction of the poorly aligned component becomes mobile. This suggests a mechanism for the supercontraction of silk involving latent entropic springs that undergo a local strain-dependent phase transition, driving supercontraction. In the second part of this dissertation a novel method is developed for exciting NMR and nuclear quadrupole resonance (NQR) by rf irradiation at multiple frequencies that sum to (or differ by) the resonance frequency. This is fundamentally different than traditional NMR experiments where irradiation is applied on-resonance. With excitation outside the detection bandwidth, two-photon excitation allows for detection of free induction signals during excitation, completely eliminating receiver dead-time. A theoretical approach to describing two-photon excitation is developed based on average Hamiltonian theory. An intuition for two-photon excitation is gained by analogy to the coherent absorption of multiple photons requiring conservation of total energy and

  10. Effect of Two-Photon Stark Shift on the Multi-Frequency Raman Spectra

    Directory of Open Access Journals (Sweden)

    Hao Yan

    2014-09-01

    Full Text Available High order Raman generation has received considerable attention as a possible method for generating ultrashort pulses. A large number of Raman orders can be generated when the Raman-active medium is pumped by two laser pulses that have a frequency separation equal to the Raman transition frequency. High order Raman generation has been studied in the different temporal regimes, namely: adiabatic, where the pump pulses are much longer than the coherence time of the transition; transient, where the pulse duration is comparable to the coherence time; and impulsive, where the bandwidth of the ultrashort pulse is wider than the transition frequency. To date, almost all of the work has been concerned with generating as broad a spectrum as possible, but we are interested in studying the spectra of the individual orders when pumped in the transient regime. We concentrate on looking at extra peaks that are generated when the Raman medium is pumped with linearly chirped pulses. The extra peaks are generated on the low frequency side of the Raman orders. We discuss how linear Raman scattering from two-photon dressed states can lead to the generation of these extra peaks.

  11. Distribution of quantum information between an atom and two photons

    Energy Technology Data Exchange (ETDEWEB)

    Weber, Bernhard

    2008-11-03

    The construction of networks consisting of optically interconnected processing units is a promising way to scale up quantum information processing systems. To store quantum information, single trapped atoms are among the most proven candidates. By placing them in high finesse optical resonators, a bidirectional information exchange between the atoms and photons becomes possible with, in principle, unit efficiency. Such an interface between stationary and ying qubits constitutes a possible node of a future quantum network. The results presented in this thesis demonstrate the prospects of a quantum interface consisting of a single atom trapped within the mode of a high-finesse optical cavity. In a two-step process, we distribute entanglement between the stored atom and two subsequently emitted single photons. The long atom trapping times achieved in the system together with the high photon collection efficiency of the cavity make the applied protocol in principle deterministic, allowing for the creation of an entangled state at the push of a button. Running the protocol on this quasi-stationary quantum interface, the internal state of the atom is entangled with the polarization state of a single emitted photon. The entanglement is generated by driving a vacuum-stimulated Raman adiabatic passage between states of the coupled atom-cavity system. In a second process, the atomic part of the entangled state is mapped onto a second emitted photon using a similar technique and resulting in a polarization-entangled two-photon state. To verify and characterize the photon-photon entanglement, we measured a violation of a Bell inequality and performed a full quantum state tomography. The results prove the prior atom-photon entanglement and demonstrate a quantum information transfer between the atom and the two emitted photons. This reflects the advantages of a high-finesse cavity as a quantum interface in future quantum networks. (orig.)

  12. Dynamical modeling of pulsed two-photon interference

    Science.gov (United States)

    Fischer, Kevin A.; Müller, Kai; Lagoudakis, Konstantinos G.; Vučković, Jelena

    2016-11-01

    Single-photon sources are at the heart of quantum-optical networks, with their uniquely quantum emission and phenomenon of two-photon interference allowing for the generation and transfer of nonclassical states. Although a few analytical methods have been briefly investigated for describing pulsed single-photon sources, these methods apply only to either perfectly ideal or at least extremely idealized sources. Here, we present the first complete picture of pulsed single-photon sources by elaborating how to numerically and fully characterize non-ideal single-photon sources operating in a pulsed regime. In order to achieve this result, we make the connection between quantum Monte-Carlo simulations, experimental characterizations, and an extended form of the quantum regression theorem. We elaborate on how an ideal pulsed single-photon source is connected to its photocount distribution and its measured degree of second- and first-order optical coherence. By doing so, we provide a description of the relationship between instantaneous source correlations and the typical experimental interferometers (Hanbury-Brown and Twiss, Hong-Ou-Mandel, and Mach-Zehnder) used to characterize such sources. Then, we use these techniques to explore several prototypical quantum systems and their non-ideal behaviors. As an example numerical result, we show that for the most popular single-photon source—a resonantly excited two-level system—its error probability is directly related to its excitation pulse length. We believe that the intuition gained from these representative systems and characters can be used to interpret future results with more complicated source Hamiltonians and behaviors. Finally, we have thoroughly documented our simulation methods with contributions to the Quantum Optics Toolbox in Python in order to make our work easily accessible to other scientists and engineers.

  13. Voltage-sensitive rhodol with enhanced two-photon brightness.

    Science.gov (United States)

    Kulkarni, Rishikesh U; Kramer, Daniel J; Pourmandi, Narges; Karbasi, Kaveh; Bateup, Helen S; Miller, Evan W

    2017-03-14

    We have designed, synthesized, and applied a rhodol-based chromophore to a molecular wire-based platform for voltage sensing to achieve fast, sensitive, and bright voltage sensing using two-photon (2P) illumination. Rhodol VoltageFluor-5 (RVF5) is a voltage-sensitive dye with improved 2P cross-section for use in thick tissue or brain samples. RVF5 features a dichlororhodol core with pyrrolidyl substitution at the nitrogen center. In mammalian cells under one-photon (1P) illumination, RVF5 demonstrates high voltage sensitivity (28% ΔF/F per 100 mV) and improved photostability relative to first-generation voltage sensors. This photostability enables multisite optical recordings from neurons lacking tuberous sclerosis complex 1, Tsc1, in a mouse model of genetic epilepsy. Using RVF5, we show that Tsc1 KO neurons exhibit increased activity relative to wild-type neurons and additionally show that the proportion of active neurons in the network increases with the loss of Tsc1. The high photostability and voltage sensitivity of RVF5 is recapitulated under 2P illumination. Finally, the ability to chemically tune the 2P absorption profile through the use of rhodol scaffolds affords the unique opportunity to image neuronal voltage changes in acutely prepared mouse brain slices using 2P illumination. Stimulation of the mouse hippocampus evoked spiking activity that was readily discerned with bath-applied RVF5, demonstrating the utility of RVF5 and molecular wire-based voltage sensors with 2P-optimized fluorophores for imaging voltage in intact brain tissue.

  14. Determining the Quark Charges by One and Two Photon Processes.

    Science.gov (United States)

    Janah, Arjun

    1982-05-01

    Testable predictions are presented, which may be used to decide between the gauge theories of integer and fractionally charged quarks (icq and fcq). Two distinctive features of icq are exploited, namely (a) presence of color non-singlet components in weak and electromagnetic currents and (b) possible liberation of color non-singlet states above a threshold energy. Consequences are sought in lepton-hadron interaction processes, taking into account the known "color-suppression" effect. Single photon/weak-boson processes such as (nu)N (--->) (nu)X distinguish between icq and fcq only above color-threshold. Experimental consequences of color-liberation in the above process are obtained. It is found that the gluon-parton contribution survives color-suppression to produce a significant rise in the structure functions when color-threshold is exceeded. Two-photon processes such as e('+)e('-) (--->) e('+)e('-) + 2 jets distinguish between the two theories even below color threshold. To obtain the icq predictions for this process, one must take into account (a) the (momentum -dependent) color suppression and (b) the added contribution from pair production of charged gluons. This is done, and it is observed that: (i) in icq, the ratio R('(gamma)(gamma)(2 jet)) is not simply a number given by the quark charges; it depends on the gluon mass, on kinematics and on the particular differential cross-section considered; (ii) the deviation of icq cross-sections from the fcq values depends crucially on whether one includes "untagged" events; if this is done, the deviation is large; the charged gluon contribution is mainly responsible for this deviation; the quark contribution is smaller than naively expected. Finally, comparison is made with experimental data on e('+)e('-) (--->) e('+)e('-) + 2 jets. Here, icq is found to be in better agreement than fcq, for a broad range of gluon masses. A suitably modified equivalent photon approximation is employed.

  15. Two-photon excitation photodynamic therapy with Photofrin

    Science.gov (United States)

    Karotki, Aliaksandr; Khurana, Mamta; Lepock, James R.; Wilson, Brian C.

    2005-09-01

    Photodynamic therapy (PDT) based on simultaneous two-photon (2-γ) excitation has a potential advantage of highly targeted treatment by means of nonlinear localized photosensitizer excitation. One of the possible applications of 2-γ PDT is a treatment of exodus age-related macular degeneration where highly targeted excitation of photosensitizer in neovasculature is vital for reducing collateral damage to healthy surrounding tissue. To investigate effect of 2-γ PDT Photofrin was used as an archetypal photosensitizer. First, 2-γ absorption properties of Photofrin in the 750 - 900 nm excitation wavelength range were investigated. It was shown that above 800 nm 2-γ interaction was dominant mode of excitation. The 2-γ cross section of Photofrin was rather small and varied between 5 and 10 GM (1 GM = 10-50 cm4s/photon) in this wavelength range. Next, endothelial cells treated with Photofrin were used to model initial effect of 2-γ PDT on neovasculature. Ultrashort laser pulses provided by mode-locked Ti:sapphire laser (pulse duration at the sample 300 fs, repetition rate 90 MHz, mean laser power 10 mW, excitation wavelength 850 nm) were used for the excitation of the photosensitizer. Before 2-γ excitation of the Photofrin cells formed a single continuous sheet at the bottom of the well. The tightly focused laser light was scanned repeatedly over the cell layer. After irradiation the cell layer of the control cells stayed intact while cells treated with photofrin became clearly disrupted. The light doses required were high (6300 Jcm(-2) for ~ 50% killing), but 2-γ cytotoxicity was unequivocally demonstrated.

  16. A Two- Photon Femtosecond Laser System for Three-Dimensional Microfabrication and Data Storage

    Institute of Scientific and Technical Information of China (English)

    蒋中伟; 周拥军; 袁大军; 黄文浩; 夏安东

    2003-01-01

    Utilizing the well-focused femtosecond laser with extreme high pulse intensity, we built a two-photon microfabrication and data storage system, which was introduced through several functional parts. Based on this homemade system, several three-dimensional microstructures were fabricated by two-photon polymerization, and three-dimensional data storage of six-layers was achieved by two-photon excitation with a photochromic material.

  17. Two-photon path-entangled states in multi-mode waveguides

    CERN Document Server

    Poem, Eilon; Silberberg, Yaron

    2012-01-01

    We experimentally show that two-photon path-entangled states can be coherently manipulated by multi-mode interference in multi-mode waveguides. By measuring the output two-photon spatial correlation function versus the phase of the input state, we show that multi-mode waveguides perform as nearly-ideal multi-port beam splitters at the quantum level, creating a large variety of entangled and separable multi-path two-photon states.

  18. Pressure broadening of atomic oxygen two-photon absorption laser induced fluorescence

    Science.gov (United States)

    Marinov, Daniil; Drag, Cyril; Blondel, Christophe; Guaitella, Olivier; Golda, Judith; Klarenaar, Bart; Engeln, Richard; Schulz-von der Gathen, Volker; Booth, Jean-Paul

    2016-12-01

    Atomic oxygen, considered to be a determining reactant in plasma applications at ambient pressure, is routinely detected by two-photon absorption laser induced fluorescence (TALIF). Here, pressure broadening of the (2p 4 3 P 2  →  3p 3 P J=0,1,2) two-photon transition in oxygen atoms was investigated using a high-resolution TALIF technique in normal and Doppler-free configurations. The pressure broadening coefficients determined were {γ{{\\text{O}2}}}   =  0.40  ±  0.08  cm-1/bar for oxygen molecules and {γ\\text{He}}   =  0.46  ±  0.03 cm-1/bar for helium atoms. These correspond to pressure broadening rate constants k\\text{PB}{{\\text{O}2}}   =  9 · 10-9 cm3 s-1 and k\\text{PB}\\text{He}   =  4 · 10-9 cm3 s-1, respectively. The well-known quenching rate constants of O(3p 3 P J ) by O2 and He are at least one order of magnitude smaller, which signifies that non-quenching collisions constitute the main line-broadening mechanism. In addition to providing new insights into collisional processes of oxygen atoms in electronically excited 3p 3 P J state, reported pressure broadening parameters are important for quantification of oxygen TALIF line profiles when both collisional and Doppler broadening mechanisms are important. Thus, the Doppler component (and hence the temperature of oxygen atoms) can be accurately determined from high resolution TALIF measurements in a broad range of conditions.

  19. Description of the states of two-photon interference in an optical gating Michelson interferometer

    Science.gov (United States)

    Pongophas, Ekkarat; Sriklin, Watthana; Sinsarp, Asawin; Suwanna, Sujin; Chunwachirasiri, Withoon; Singhsomroje, Wisit

    2016-01-01

    We investigate the interference of two photons in an optical gating Michelson interferometer. The phenomenon is studied using two different representations of photons: the space-time domain and a step-by-step two-photon state evolution. Both representations lead to identical results. The evolution analysis describes the result by the interference of four two-photon traveling states, whereas the space-time domain analysis reveals that the classical interference of the high-intensity light source is identical to two-photon interference in the quantum regime, except for a multiplicative factor of (n2), where n is the number of photons.

  20. Two-photon induced photoluminescence and singlet oxygen generation from aggregated gold nanoparticles.

    Science.gov (United States)

    Jiang, Cuifeng; Zhao, Tingting; Yuan, Peiyan; Gao, Nengyue; Pan, Yanlin; Guan, Zhenping; Zhou, Na; Xu, Qing-Hua

    2013-06-12

    Metal nanoparticles have potential applications as bioimaging and photosensitizing agents. Aggregation effects are generally believed to be adverse to their biomedical applications. Here we have studied the aggregation effects on two-photon induced photoluminescence and singlet oxygen generation of Au nanospheres and Au nanorods of two different aspect ratios. Aggregated Au nanospheres and short Au nanorods were found to display enhanced two-photon induced photoluminescence and singlet oxygen generation capabilities compared to the unaggregated ones. The two-photon photoluminescence of Au nanospheres and short Au nanorods were enhanced by up to 15.0- and 2.0-fold upon aggregation, and the corresponding two-photon induced singlet oxygen generation capabilities were enhanced by 8.3 and 1.8-fold, respectively. The two-photon induced photoluminescence and singlet oxygen generation of the aggregated long Au nanorods were found to be lower than the unaggregated ones. These results support that the change in their two-photon induced photoluminescence and singlet oxygen generation originate from aggregation modulated two-photon excitation efficiency. This finding is expected to foster more biomedical applications of metal nanoparticles as Au nanoparticles normally exist in an aggregated form in the biological environments. Considering their excellent biocompatibility, high inertness, ready conjugation, and easy preparation, Au nanoparticles are expected to find more applications in two-photon imaging and two-photon photodynamic therapy.

  1. Synthesis of two carbazole-based dyes and application of two-photon initiating polymerization

    Institute of Scientific and Technical Information of China (English)

    2009-01-01

    Two carbazole-based polymerization initiators possessing blue fluorescence emission have been synthesized via Wittig reaction in the solid phase at room temperature.Two-photon excited fluorescence(TPEF) spectra for them were investigated under 800 nm fs laser pulse and two-photon absorption cross sections were determined by the Z-scan technique.Then two-photon initiating polymerization(TPIP) microfabrication experiments were successfully carried out.Three-dimensional lattice and artificial defects were gained,indicating that they were viable candidates for the two-photon polymerization initiator in practical application of microfabrication.

  2. Time-reversed two-photon interferometry for phase super-resolution

    CERN Document Server

    Ogawa, Kazuhisa; Kobayashi, Hirokazu; Nakanishi, Toshihiro; Kitano, Masao

    2013-01-01

    We observed two-photon phase super-resolution in an unbalanced Michelson interferometer with classical Gaussian laser pulses. Our work is a time-reversed version of a two-photon interference experiment using an unbalanced Michelson interferometer. A measured interferogram exhibits two-photon phase super-resolution with a high visibility of 97.9% \\pm 0.4%. Its coherence length is about 22 times longer than that of the input laser pulses. It is a classical analogue to the large difference between the one- and two-photon coherence lengths of entangled photon pairs.

  3. Synthesis of two carbazole-based dyes and application of two-photon initiating polymerization

    Institute of Scientific and Technical Information of China (English)

    HU RenTao; LU LiangFei; RUAN BanFeng; WANG Peng; ZHANG MingLiang; ZHOU HongPing; LI ShengLi; WU JieYing; TIAN YuPeng

    2009-01-01

    Two carbazole-based polymerization initiators possessing blue fluorescence emission have been synthesized via Wittig reaction in the solid phase at room temperature.Two-photon excited fluorescence (TPEF) spectra for them were investigated under 800 nm fs laser pulse and two-photon absorption cross sections were determined by the Z-scan technique.Then two-photon initiating polymerization (TPIP) microfabrication experiments were successfully carried out.Three-dimensional lattice and artificial defects were gained,indicating that they were viable candidates for the two-photon polymerization initiator in practical application of microfabrication.

  4. New formalism for two-photon quantum optics. I - Quadrature phases and squeezed states. II - Mathematical foundation and compact notation

    Science.gov (United States)

    Caves, C. M.; Schumaker, B. L.

    1985-01-01

    A new formalism for analyzing two-photon devices, such as parametric amplifiers and phase-conjugate mirrors, is proposed in part I, focusing on the properties and the significance of the quadrature-phase amplitudes and two-mode squeezed states. Time-stationary quasi-probability noise is also detailed for the case of Gaussian noise, and uncertainty principles for the quadrature-phase amplitudes are outlined, as well as some important properties of the two-mode states. Part II establishes a mathematical foundation for the formalism, with introduction of a vector notation for compact representation of two-mode properties. Fundamental unitary operators and special quantum states are also examined with an emphasis on the two-mode squeezed states. The results are applied to a previously studied degenerate limit (epsilon = 0).

  5. Fluorescence enhancement of asCP595 is due to consecutive absorbance of two photons

    Science.gov (United States)

    Savitsky, Alexander P.; Agranat, Michail B.; Lukyanov, Konstantin A.; Schuttrigkeit, Tanja; von Feilitzsch, Till; Kompa, Christian; Michel-Beyerle, Maria-Elisabeth

    2004-06-01

    Colored proteins are widely used as gene markers in biotechnology. Chromophores result from autocatalytic posttranslational reactions involving several amino acids. The protein asCP595 was isolated for the first time from the coral as a weakly fluorescent chromoprotein with a fluorescence maximum at 595 nm. Strong illumination in the blue wing of the low energy absorption band results in a superlinear increase of the fluorescence yield and shifts its fluorescence spectrum by about 10 nm to the red. Time resolved fluorescence measurements using excitation pulses with 10 ps duration revealed a multiexponential decay pattern with time constants in the range from 20 ps to 2.1 ns. The ratio of amplitudes related to the different time constants depends on the intensity of illumination favoring the ns component at high intensities. Transient absorption measurements using ultrashort excitation pulses (150 fs, 1 kHz repetition rate) did not reveal excited states with nanosecond lifetimes as observed in fluorescence upon excitation using 10 ps pulses. This observation leads to the notion that within 10 ps a second photon is absorbed by a state not yet populated within 150 fs. As a consequence we propose two different excited singlet states operative in asCP595, one with low fluorescence quantum yield peaking at 595 nm and one with high fluorescence quantum yield peaking at 605 nm which is populated via the consecutive absorption of two photons at high excitation intensities.

  6. Probing Electron-Phonon Interaction through Two-Photon Interference in Resonantly Driven Semiconductor Quantum Dots

    Science.gov (United States)

    Reigue, Antoine; Iles-Smith, Jake; Lux, Fabian; Monniello, Léonard; Bernard, Mathieu; Margaillan, Florent; Lemaitre, Aristide; Martinez, Anthony; McCutcheon, Dara P. S.; Mørk, Jesper; Hostein, Richard; Voliotis, Valia

    2017-06-01

    We investigate the temperature dependence of photon coherence properties through two-photon interference (TPI) measurements from a single quantum dot (QD) under resonant excitation. We show that the loss of indistinguishability is related only to the electron-phonon coupling and is not affected by spectral diffusion. Through these measurements and a complementary microscopic theory, we identify two independent separate decoherence processes, both of which are associated with phonons. Below 10 K, we find that the relaxation of the vibrational lattice is the dominant contribution to the loss of TPI visibility. This process is non-Markovian in nature and corresponds to real phonon transitions resulting in a broad phonon sideband in the QD emission spectra. Above 10 K, virtual phonon transitions to higher lying excited states in the QD become the dominant dephasing mechanism, this leads to a broadening of the zero phonon line, and a corresponding rapid decay in the visibility. The microscopic theory we develop provides analytic expressions for the dephasing rates for both virtual phonon scattering and non-Markovian lattice relaxation.

  7. Enhancement of Squeezing in Two-Photon Jaynes-Cummings Model with Atomic Measurement

    Institute of Scientific and Technical Information of China (English)

    YE Sai-Yun

    2006-01-01

    We investigate the squeezing properties of the cavity field in the degenerate two-photon Jaynes-Cummings model. Compared with the one-photon Jaynes-Cummings model, the squeezing is more pronounced in the case of two-photon Jaynes-Cummings model under certain conditions.

  8. Event-by-event simulation of nonclassical effects in two-photon interference experiments

    NARCIS (Netherlands)

    Michielsen, K.; Jin, F.; Delina, M.; Raedt, H. De

    2012-01-01

    A corpuscular simulation model for second-order intensity interference phenomena is discussed. It is shown that both the visibility V = 1/2 predicted for two-photon interference experiments with two independent sources and the visibility V = 1 predicted for two-photon interference experiments with a

  9. Integrated single- and two-photon light sheet microscopy using accelerating beams

    DEFF Research Database (Denmark)

    Piksarv, Peeter; Marti, Dominik; Le, Tuan

    2017-01-01

    We demonstrate the first light sheet microscope using propagation invariant, accelerating Airy beams that operates both in single- and two-photon modes. The use of the Airy beam permits us to develop an ultra compact, high resolution light sheet system without beam scanning. In two-photon mode, a...

  10. Two-photon fluorescence probes for imaging of mitochondria and lysosomes.

    Science.gov (United States)

    Yang, Wanggui; Chan, Pui Shan; Chan, Miu Shan; Li, King Fai; Lo, Pik Kwan; Mak, Nai Ki; Cheah, Kok Wai; Wong, Man Shing

    2013-04-28

    Novel biocompatible cyanines show not only a very large two-photon cross-section of up to 5130 GM at 910 nm in aqueous medium for high-contrast and -brightness two-photon fluorescence live cell imaging but also highly selective subcellular localization properties including localization of mitochondria and lysosomes.

  11. Effect of morphology and solvent on two-photon absorption of nano zinc oxide

    Energy Technology Data Exchange (ETDEWEB)

    Kavitha, M.K. [Department of Chemistry, Indian Institute of Space Science and Technology, Valiamala, Thiruvananthapuram 695547, Kerala (India); Haripadmam, P.C.; Gopinath, Pramod; Krishnan, Bindu [Department of Physics, Indian Institute of Space Science and Technology, Valiamala, Thiruvananthapuram 695547, Kerala (India); John, Honey, E-mail: honey@iist.ac.in [Department of Chemistry, Indian Institute of Space Science and Technology, Valiamala, Thiruvananthapuram 695547, Kerala (India)

    2013-05-15

    Highlights: ► ZnO nanospheres and triangular structures synthesis by novel precipitation technique. ► The effect of precursor concentration on the size and shape of nano ZnO. ► Open aperture Z-scan measurements of the ZnO nanoparticle dispersions. ► Nanospheres exhibit higher two photon absorption coefficient than triangular nanostructures. ► Nanospheres dispersed in water exhibit higher two photon absorption coefficient than its dispersion in 2-propanol. - Abstract: In this paper, we report the effect of morphology and solvent on the two-photon absorption of nano zinc oxide. Zinc oxide nanoparticles in two different morphologies like nanospheres and triangular nanostructures are synthesized by novel precipitation technique and their two-photon absorption coefficient is measured using open aperture Z-scan technique. Experimental results show that the zinc oxide nanospheres exhibit higher two-photon absorption coefficient than the zinc oxide triangular nanostructures. The zinc oxide nanospheres dispersed in water exhibit higher two-photon absorption coefficient than that of its dispersion in 2-propanol. The zinc oxide nanospheres dispersed in water shows a decrease in two-photon absorption coefficient with an increase in on-axis irradiance. The result confirms the dependence of shape and solvent on the two-photon absorption of nano zinc oxide.

  12. Production of e, $\\mu$ and $\\tau$ Pairs in Untagged Two-Photon Collisions at LEP

    CERN Document Server

    Acciarri, M; Aguilar-Benítez, M; Ahlen, S P; Alcaraz, J; Alemanni, G; Allaby, James V; Aloisio, A; Alverson, G; Alviggi, M G; Ambrosi, G; Anderhub, H; Andreev, V P; Angelescu, T; Anselmo, F; Arefev, A; Azemoon, T; Aziz, T; Bagnaia, P; Baksay, L; Ball, R C; Banerjee, S; Banerjee, Sw; Banicz, K; Barczyk, A; Barillère, R; Barone, L; Bartalini, P; Baschirotto, A; Basile, M; Battiston, R; Bay, A; Becattini, F; Becker, U; Behner, F; Berdugo, J; Berges, P; Bertucci, B; Betev, B L; Bhattacharya, S; Biasini, M; Biland, A; Bilei, G M; Blaising, J J; Blyth, S C; Bobbink, Gerjan J; Böck, R K; Böhm, A; Boldizsar, L; Borgia, B; Boucham, A; Bourilkov, D; Bourquin, Maurice; Boutigny, D; Braccini, S; Branson, J G; Brigljevic, V; Brock, I C; Buffini, A; Buijs, A; Burger, J D; Burger, W J; Busenitz, J K; Cai, X D; Campanelli, M; Capell, M; Cara Romeo, G; Carlino, G; Cartacci, A M; Casaus, J; Castellini, G; Cavallari, F; Cavallo, N; Cecchi, C; Cerrada-Canales, M; Cesaroni, F; Chamizo-Llatas, M; Chang, Y H; Chaturvedi, U K; Chekanov, S V; Chemarin, M; Chen, A; Chen, G; Chen, G M; Chen, H F; Chen, H S; Chen, M; Chiefari, G; Chien, C Y; Cifarelli, Luisa; Cindolo, F; Civinini, C; Clare, I; Clare, R; Cohn, H O; Coignet, G; Colijn, A P; Colino, N; Commichau, V; Costantini, S; Cotorobai, F; de la Cruz, B; Csilling, Akos; Dai, T S; D'Alessandro, R; De Asmundis, R; Degré, A; Deiters, K; Denes, P; De Notaristefani, F; DiBitonto, Daryl; Diemoz, M; Van Dierendonck, D N; Di Lodovico, F; Dionisi, C; Dittmar, Michael; Dominguez, A; Doria, A; Dorne, I; Dova, M T; Drago, E; Duchesneau, D; Duinker, P; Durán, I; Dutta, S; Easo, S; Efremenko, Yu V; El-Mamouni, H; Engler, A; Eppling, F J; Erné, F C; Ernenwein, J P; Extermann, Pierre; Fabre, M; Faccini, R; Falciano, S; Favara, A; Fay, J; Fedin, O; Felcini, Marta; Fenyi, B; Ferguson, T; Ferroni, F; Fesefeldt, H S; Fiandrini, E; Field, J H; Filthaut, Frank; Fisher, P H; Fisk, I; Forconi, G; Fredj, L; Freudenreich, Klaus; Furetta, C; Galaktionov, Yu; Ganguli, S N; García-Abia, P; Gau, S S; Gentile, S; Gerald, J; Gheordanescu, N; Giagu, S; Goldfarb, S; Goldstein, J; Gong, Z F; Gougas, Andreas; Gratta, Giorgio; Grünewald, M W; Gupta, V K; Gurtu, A; Gutay, L J; Hartmann, B; Hasan, A; Hatzifotiadou, D; Hebbeker, T; Hervé, A; Van Hoek, W C; Hofer, H; Hong, S J; Hoorani, H; Hou, S R; Hu, G; Innocente, Vincenzo; Janssen, H; Jenkes, K; Jin, B N; Jones, L W; de Jong, P; Josa-Mutuberria, I; Kasser, A; Khan, R A; Kamrad, D; Kamyshkov, Yu A; Kapustinsky, J S; Karyotakis, Yu; Kaur, M; Kienzle-Focacci, M N; Kim, D; Kim, D H; Kim, J K; Kim, S C; Kim, Y G; Kinnison, W W; Kirkby, A; Kirkby, D; Kirkby, Jasper; Kiss, D; Kittel, E W; Klimentov, A; König, A C; Kopp, A; Korolko, I; Koutsenko, V F; Krämer, R W; Krenz, W; Kunin, A; Ladrón de Guevara, P; Landi, G; Lapoint, C; Lassila-Perini, K M; Laurikainen, P; Lebeau, M; Lebedev, A; Lebrun, P; Lecomte, P; Lecoq, P; Le Coultre, P; Leggett, C; Le Goff, J M; Leiste, R; Leonardi, E; Levchenko, P M; Li Chuan; Lin, C H; Lin, W T; Linde, Frank L; Lista, L; Liu, Z A; Lohmann, W; Longo, E; Lu, W; Lü, Y S; Lübelsmeyer, K; Luci, C; Luckey, D; Luminari, L; Lustermann, W; Ma Wen Gan; Maity, M; Majumder, G; Malgeri, L; Malinin, A; Maña, C; Mangeol, D J J; Mangla, S; Marchesini, P A; Marin, A; Martin, J P; Marzano, F; Massaro, G G G; McNally, D; Mele, S; Merola, L; Meschini, M; Metzger, W J; Von der Mey, M; Mi, Y; Mihul, A; Van Mil, A J W; Mirabelli, G; Mnich, J; Molnár, P; Monteleoni, B; Moore, R; Morganti, S; Moulik, T; Mount, R; Müller, S; Muheim, F; Muijs, A J M; Nahn, S; Napolitano, M; Nessi-Tedaldi, F; Newman, H; Niessen, T; Nippe, A; Nisati, A; Nowak, H; Oh, Yu D; Opitz, H; Organtini, G; Ostonen, R; Palomares, C; Pandoulas, D; Paoletti, S; Paolucci, P; Park, H K; Park, I H; Pascale, G; Passaleva, G; Patricelli, S; Paul, T; Pauluzzi, M; Paus, C; Pauss, Felicitas; Peach, D; Pei, Y J; Pensotti, S; Perret-Gallix, D; Petersen, B; Petrak, S; Pevsner, A; Piccolo, D; Pieri, M; Pinto, J C; Piroué, P A; Pistolesi, E; Plyaskin, V; Pohl, M; Pozhidaev, V; Postema, H; Produit, N; Prokofev, D; Prokofiev, D O; Rahal-Callot, G; Raja, N; Rancoita, P G; Rattaggi, M; Raven, G; Razis, P A; Read, K; Ren, D; Rescigno, M; Reucroft, S; Van Rhee, T; Riemann, S; Riles, K; Rind, O; Robohm, A; Rodin, J; Roe, B P; Romero, L; Rosier-Lees, S; Rosselet, P; Van Rossum, W; Roth, S; Rubio, Juan Antonio; Ruschmeier, D; Rykaczewski, H; Salicio, J; Sánchez, E; Sanders, M P; Sarakinos, M E; Sarkar, S; Sassowsky, M; Sauvage, G; Schäfer, C; Shchegelskii, V; Schmidt-Kärst, S; Schmitz, D; Schmitz, P; Schneegans, M; Scholz, N; Schopper, Herwig Franz; Schotanus, D J; Schwenke, J; Schwering, G; Sciacca, C; Sciarrino, D; Servoli, L; Shevchenko, S; Shivarov, N; Shoutko, V; Shukla, J; Shumilov, E; Shvorob, A V; Siedenburg, T; Son, D; Sopczak, André; Soulimov, V; Smith, B; Spillantini, P; Steuer, M; Stickland, D P; Stone, H; Stoyanov, B; Strässner, A; Strauch, K; Sudhakar, K; Sultanov, G G; Sun, L Z; Susinno, G F; Suter, H; Swain, J D; Tang, X W; Tauscher, Ludwig; Taylor, L; Ting, Samuel C C; Ting, S M; Tonutti, M; Tonwar, S C; Tóth, J; Tully, C; Tuchscherer, H; Tung, K L; Uchida, Y; Ulbricht, J; Uwer, U; Valente, E; Van de Walle, R T; Vesztergombi, G; Vetlitskii, I; Viertel, Gert M; Vivargent, M; Völkert, R; Vogel, H; Vogt, H; Vorobev, I; Vorobyov, A A; Vorvolakos, A; Wadhwa, M; Wallraff, W; Wang, J C; Wang, X L; Wang, Z M; Weber, A; Wittgenstein, F; Wu, S X; Wynhoff, S; Xu, J; Xu, Z Z; Yang, B Z; Yang, C G; Yao, X Y; Ye, J B; Yeh, S C; You, J M; Zalite, A; Zalite, Yu; Zemp, P; Zeng, Y; Zhang, Z; Zhang, Z P; Zhou, B; Zhou, Y; Zhu, G Y; Zhu, R Y; Zichichi, Antonino; Ziegler, F

    1997-01-01

    The two-photon collision reaction e+e- --> e+e-l+l- has been studied at root(s) ~ 91 GeV using the L3 detector at LEP for l = e, muon , tau. We have analysed untagged configurations where the two photons are quasi-real. Good agreement is found between our measurements and the order alpha**4 QED expectation.

  13. Temporal dynamics of two-photon-pumped amplified spontaneous emission in slab organic crystals

    NARCIS (Netherlands)

    Fang, Hong-Hua; Chen, Qi-Dai; Ding, Ran; Yang, Jie; Ma, Yu-Guang; Wang, Hai-Yu; Gao, Bing-Rong; Feng, Jing; Sun, Hong-Bo; Fang, Honghua

    2010-01-01

    We have studied the ultrafast dynamics of two-photon-pumped amplified spontaneous emission (ASE) from a single crystal by the time-resolved fluorescence upconversion technique. With the increase of two-photon pump intensities, the emission decay time is dramatically shortened by 30 times (from 3 ns

  14. Two-Photon Interference with the Type Ⅱ Spontaneous Parametric Down-Conversion

    Institute of Scientific and Technical Information of China (English)

    江云坤; 史保森; 李剑; 段开敏; 范晓锋; 郭光灿

    2001-01-01

    The two-photon polarized entangled state is generated from the type Ⅱ spontaneous parametric down-conversion pumped by a femtosecond pulse. The two-photon interference is observed in the Hong-Ou-Mandel interferometer. The high visibility of the interference is restored with narrow band interference filters placed in front of the detectors.

  15. Description of states of two-photon interference in optical gating Michelson interferometer

    Science.gov (United States)

    Pongophas, Ekkarat; Sinsarp, Asawin; Suwanna, Sujin; Chunwachirasiri, Withoon; Singhsomroje, Wisit

    2015-07-01

    The interference of two photons in the optical gating Michelson interferometer is investigated. The phenomenon is studied using two different representations of photons: the space-time domain and a step-by-step two photon state evolution. Both representations lead to an equivalent description of the two-photon states which is the interference of four cases of two-photon traveling states, as implied by the evolution analysis. Additionally, the space-time domain analysis reveals that the classical interference of high-intensity light source is identical to the two-photon interference in the quantum regime except for a multiplicative factor of (n 2), where n is the number of photons.

  16. Imaging theory and resolution improvement of two-photon confocal microscopy

    Institute of Scientific and Technical Information of China (English)

    唐志列; 杨初平; 裴红津; 梁瑞生; 刘颂豪

    2002-01-01

    The nonlinear effect of two-photon excitation on the imaging property of two-photonconfocal microscopy has been analyzed by the two-photon fluorescence intensity transfer functionderived in this paper. The two-photon fluorescence intensity transfer function in a confocal micros-copy is given. Furthermore the three-dimensional point spread function (3D-PSF) and thethree-dimensional optical transfer function (3D-OTF) of two-photon confocal microscopy are de-rived based on the nonlinear effect of two-photon excitation. The imaging property of two-photonconfocal microscopy is discussed in detail based on 3D-OTF. Finally the spatial resolution limit oftwo-photon confocal microscopy is discussed according to the uncertainty principle.

  17. Computing transition rates for the 1-D stochastic Ginzburg--Landau--Allen--Cahn equation for finite-amplitude noise with a rare event algorithm

    CERN Document Server

    Rolland, J; Simonnet, E

    2015-01-01

    In this paper we compute and analyse the transition rates and duration of reactive trajectories of the stochastic 1-D Allen-Cahn equations for both the Freidlin-Wentzell regime (weak noise or temperature limit) and finite-amplitude white noise, as well as for small and large domain. We demonstrate that extremely rare reactive trajectories corresponding to direct transitions between two metastable states are efficiently computed using an algorithm called adaptive multilevel splitting. This algorithm is dedicated to the computation of rare events and is able to provide ensembles of reactive trajectories in a very efficient way. In the small noise limit, our numerical results are in agreement with large-deviation predictions such as instanton-like solutions, mean first passages and escape probabilities. We show that the duration of reactive trajectories follows a Gumbel distribution like for one degree of freedom systems. Moreover, the mean duration growths logarithmically with the inverse temperature. The prefa...

  18. Doppler-free two-photon spectroscopy on atomic hydrogen

    CERN Document Server

    Niering, M

    1999-01-01

    In the framework of the present thesis the internal structure of the hydrogen atom is studied by means of optical spectroscopic methods. The main interest is thereby devoted to the transition of the 1S ground-state into the metastable 2S-state.

  19. Effects of tidal amplitude on intertidal resource availability and dispersal pressure in prehistoric human coastal populations: the Mediterranean Atlantic transition

    Science.gov (United States)

    Fa, Darren Andrew

    2008-11-01

    In this paper I argue that there is a growing body of evidence supporting an increasingly central position of coastal environments in human evolution and dispersals, rather than as merely peripheral habitats. Eustatic fluctuations during glacial cycles have meant that most prehistoric coastlines are now underwater, and lack of evidence to date of a close relationship between people and the coast can be most plausibly ascribed to the limited studies so far on submerged sites. Coastal environments provide high diversity in food resources, consisting of multiple ecotones in close proximity, which reduces the need to forage widely. One of the richest and most easily exploited coastal resources by human populations living on the coast are molluscs from marine rocky intertidal communities, which recent evidence has highlighted as important as far back as the Middle Palaeolithic. However, the density of these resources is limited by a number of factors, and this varies geographically. One of the main large-scale factors limiting rocky intertidal mollusc densities is tidal amplitude, beyond which smaller-scale local factors such as exposure to wave action and shore aspect, further affect species distributions. The area around the Strait of Gibraltar is used as a case study of an area, which is affected by large variations in tidal amplitudes thus allowing for quantitative comparisons between taxonomically and climatically similar regions. Shorelines along the Mediterranean coast, with reduced tidal amplitudes, exhibit compressed zonations and harbour fewer macro-mollusc individuals, with the reverse being the case along the Atlantic coast, which has significantly larger tides. Data from Middle and Upper Palaeolithic sites along the Strait are used to establish harvested species and present-day data are used to model the potential distributions and associated variables such as calorific returns of key food species. An optimal foraging model is used to explore the effects of

  20. Two-photon excitation spectroscopy of Cr3+:K2NaScF6 elpasolite: II. Theoretical models

    Science.gov (United States)

    Bartram, R. H.; Wein, G. R.; Hamilton, D. S.

    2001-03-01

    Two-photon excitation (TPE) spectra of Cr3+:K2NaScF6, excited by a Raman-shifted, Nd:YAG-pumped tunable dye laser, exhibit several unexpected features. A weak TPE spectrum of the symmetry-forbidden 4A2g→ 4T2g transition is observed without a zero-phonon line. The symmetry-allowed TPE spectrum of the 4A2g→ 4T1ag transition has a multi-phonon side band with anomalously extended vibrational progressions, and an anomalously weak, split zero-phonon line with anomalous polarization anisotropy. These observations are explained, respectively, in terms of theoretical models involving phonon assistance, departures from the closure approximation that permit electron-lattice coupling in intermediate states and a low-temperature phase transition involving librational instability. Hypothetical line-shape simulations are compared with observed TPE spectra.

  1. Observability of the effects of curl-free magnetic vector potential on the macroscale and the nature of the ‘transition amplitude wave’

    Indian Academy of Sciences (India)

    Ram K Varma

    2010-04-01

    We discuss here the prediction, based on a formalism by the author, on the observable effects of a curl-free magnetic vector potential on the macroscale as against the microscale of the Aharonov–Bohm effect. A new quantum concept – the ‘transition amplitude wave’ – postulated in the formalism has already been shown to exhibit matter wave manifestations in the form of one-dimensional interference effects on the macroscale. It was predicted by the formalism that the same entity would lead to the detection of a curl-free magnetic vector potential on the macroscale. We describe here the manner of generation of this quantum entity in an inelastic scattering episode and work out an algorithm to observe this radically new phenomenon, the detection of a curl-free magnetic vector potential on the macroscale. We determine the various characteristic features of such an observation which can then be looked for experimentally so as to verify the predicted effect, establishing thereby the physical reality of the new quantum entity, and to fully validate the formalism predicting it. It is also shown that this ‘transition amplitude wave’ can be regarded as a novel kind of ‘quasiparticle’ excited in the charged particle trajectory as a consequence of the scattering episode.

  2. Collimated Blue and Infrared Beams Generated by Two-Photon Excitation in Rb Vapor

    CERN Document Server

    Sell, J F; DePaola, B D; Knize, R J

    2013-01-01

    Utilizing two-photon excitation in hot Rb vapor we demonstrate the generation of collimated optical fields at 420 nm and 1324 nm. Input laser beams at 780 nm and 776 nm enter a heated Rb vapor cell collinear and circularly polarized, driving Rb atoms to the $5D_{5/2}$ state. Under phase-matching conditions coherence among the $5S_{1/2}\\rightarrow 5P_{3/2}\\rightarrow 5D_{5/2} \\rightarrow 6P_{3/2}$ transitions produces a blue (420 nm) beam by four-wave mixing. We also observe a forward and backward propagating IR (1324 nm) beam, due to cascading decays through the $6S_{1/2}\\rightarrow 5P_{1/2}$ states. Power saturation of the generated beams is investigated by scaling the input powers to greater than 200 mW, resulting in a coherent blue beam of 9.1 mW power, almost an order of magnitude larger than previously achieved. We measure the dependences of both beams in relation to the Rb density, the frequency detuning between Rb ground state hyperfine levels, and the input laser intensities.

  3. Study of $\\pi^0$ pair production in single-tag two-photon collisions

    CERN Document Server

    Masuda, M; Watanabe, Y; Nakazawa, H; Abdesselam, A; Adachi, I; Aihara, H; Said, S Al; Asner, D M; Atmacan, H; Aulchenko, V; Aushev, T; Babu, V; Badhrees, I; Bakich, A M; Barberio, E; Behera, P; Bhuyan, B; Biswal, J; Bobrov, A; Bonvicini, G; Bozek, A; Bračko, M; Browder, T E; Červenkov, D; Chekelian, V; Chen, A; Cheon, B G; Chilikin, K; Chistov, R; Cho, K; Chobanova, V; Choi, S -K; Choi, Y; Cinabro, D; Dalseno, J; Danilov, M; Dash, N; Dingfelder, J; Doležal, Z; Drásal, Z; Dutta, D; Eidelman, S; Epifanov, D; Farhat, H; Fast, J E; Ferber, T; Fulsom, B G; Gaur, V; Gabyshev, N; Garmash, A; Gillard, R; Glattauer, R; Goh, Y M; Goldenzweig, P; Golob, B; Haba, J; Hayasaka, K; Hayashii, H; He, X H; Hou, W -S; Iijima, T; Inami, K; Ishikawa, A; Itoh, R; Iwasaki, Y; Jaegle, I; Joffe, D; Joo, K K; Julius, T; Kang, K H; Kato, E; Kawasaki, T; Kim, D Y; Kim, J B; Kim, J H; Kim, K T; Kim, M J; Kim, S H; Kim, Y J; Ko, B R; Korpar, S; Križan, P; Krokovny, P; Kumita, T; Kuzmin, A; Kwon, Y -J; Lange, J S; Lee, D H; Lee, I S; Li, C; Li, L; Li, Y; Libby, J; Liventsev, D; Lukin, P; Matvienko, D; Miyabayashi, K; Miyata, H; Mizuk, R; Mohanty, G B; Mohanty, S; Moll, A; Moon, H K; Mori, T; Mussa, R; Nakano, E; Nakao, M; Nanut, T; Natkaniec, Z; Nayak, M; Nisar, N K; Nishida, S; Ogawa, S; Pakhlov, P; Pakhlova, G; Pal, B; Park, C W; Park, H; Pedlar, T K; Pestotnik, R; Petrič, M; Piilonen, L E; Rauch, J; Ribežl, E; Ritter, M; Rostomyan, A; Sandilya, S; Santelj, L; Sanuki, T; Sato, Y; Savinov, V; Schneider, O; Schnell, G; Schwanda, C; Seino, Y; Senyo, K; Seon, O; Sevior, M E; Shebalin, V; Shen, C P; Shibata, T -A; Shiu, J -G; Shwartz, B; Simon, F; Sohn, Y -S; Sokolov, A; Solovieva, E; Starič, M; Sumihama, M; Sumiyoshi, T; Tamponi, U; Tanida, K; Teramoto, Y; Uglov, T; Unno, Y; Uno, S; Van Hulse, C; Vanhoefer, P; Varner, G; Vinokurova, A; Vorobyev, V; Vossen, A; Wagner, M N; Wang, C H; Wang, M -Z; Wang, P; Williams, K M; Won, E; Yamaoka, J; Yamashita, Y; Yashchenko, S; Ye, H; Yusa, Y; Zhang, C C; Zhang, Z P; Zhilich, V; Zhulanov, V; Zupanc, A

    2015-01-01

    We report a measurement of the differential cross section of $\\pi^0$ pair production in single-tag two-photon collisions, $\\gamma^* \\gamma \\to \\pi^0 \\pi^0$, in $e^+ e^-$ scattering. The cross section is measured for $Q^2$ up to 30 GeV$^2$, where $Q^2$ is the negative of the invariant mass squared of the tagged photon, in the kinematic range 0.5 GeV < W < 2.1 GeV and $|\\cos \\theta^*|$ < 1.0 for the total energy and pion scattering angle, respectively, in the $\\gamma^* \\gamma$ center-of-mass system. The results are based on a data sample of 759 fb$^{-1}$ collected with the Belle detector at the KEKB asymmetric-energy $e^+ e^-$ collider. The transition form factor of the $f_0(980)$ and that of the $f_2(1270)$ with the helicity-0, -1, and -2 components separately are measured for the first time and are compared with theoretical calculations.

  4. Plasma magnetic field diagnostic using two-photon Doppler-free LIF

    Science.gov (United States)

    Yoon, Young Dae; Bellan, Paul

    2015-11-01

    A detailed description of a new plasma B field diagnostic using Doppler-free two-photon laser-induced fluorescence is presented. The diagnostic is based on a method previously developed in the context of rubidium vapor experiments. Two counter-propagating 393nm diode laser beams are directed into an argon plasma to excite Ar-II ions from 3s2 3p4 4 s4P1 / 2 ⟶ 3s2 3p4 4 p4S3 / 2 ⟶ 3s2 3p4 4 d4P3 / 2 . These levels involve two similar (392.86 and 393.25nm) transition wavelengths, so the two counter-propagating beams effectively cancel out the Doppler effect. The excited ions then decay to the 3s2 3p4 4 p4P1 / 2 level, emitting a 324.98nm line which is to be detected by a photomultiplier tube. The Zeeman splitting -- normally unobservable because of the large Doppler broadening -- of the resultant fluorescence is then to be analyzed, yielding the magnetic field of the particular location. This method is expected to provide a 3-D localized, non-perturbing measurement of magnetic fields. An experimental implementation is currently in progress.

  5. Transition to kinetic turbulence at proton scales driven by large-amplitude Kinetic Alfv\\`en fluctuations

    CERN Document Server

    Valentini, F; Pezzi, O; Servidio, S; Malara, F; Pucci, F

    2016-01-01

    Space plasmas are dominated by the presence of large-amplitude waves, large-scale inhomogeneities, kinetic effects and turbulence. Beside the homogeneous turbulence, generation of small scale fluctuations can take place also in other realistic configurations, namely, when perturbations superpose to an inhomogeneous background magnetic field. When an Alfv\\'en wave propagates in a medium where the Alfv\\'en speed varies in a direction transverse to the mean field, it undergoes phase-mixing, which progressively bends wavefronts, generating small scales in the transverse direction. As soon as transverse scales get of the order of the proton inertial length $d_p$, kinetic Alfv\\'en waves (KAWs) are naturally generated. KAWs belong to the branch of Alfv\\'en waves and propagate nearly perpendicular to the ambient magnetic field, at scales close to $d_p$. Many numerical, observational and theoretical works have suggested that these fluctuations may play a determinant role in the development of the solar-wind turbulent ...

  6. Dispersion spreading of biphotons in optical fibres and two-photon interference

    CERN Document Server

    Brida, G; Genovèse, M; Gramegna, M; Krivitsky, L A

    2006-01-01

    We present the first observation of two-photon polarization interference structure in the second-order Glauber's correlation function of two-photon light generated via type-II spontaneous parametric down-conversion. In order to obtain this result, two-photon light is transmitted through an optical fibre and the coincidence distribution is analyzed by means of the START-STOP method. Beyond the experimental demonstration of an interesting effect in quantum optics, these results also have considerable relevance for quantum communications.

  7. Coalescence and Anti-Coalescence Interference of Two-Photon Wavepacket in a Beam Splitter

    Institute of Scientific and Technical Information of China (English)

    WANG Kai-Ge; YANG Guo-Jian

    2004-01-01

    @@ We study theoretically the interference of a two-photon wavepacket in a beam splitter. We find that the spectrum symmetry for the two-photon wavepacket dominates the perfect coalescence and anti-coalescence interference.The coalescence interference is unrelated to photon entanglement. Only the anti-coalescence interference has evidence of photon entanglement. We prove that the two-photon wavepacket with an anti-symmetric spectrum is transparent to pass the 50/50 beam splitter, showing perfect anti-coalescence interference.

  8. Dispersion spreading of biphotons in optical fibers and two-photon interference.

    Science.gov (United States)

    Brida, G; Chekhova, M V; Genovese, M; Gramegna, M; Krivitsky, L A

    2006-04-14

    We present the first observation of two-photon polarization interference structure in the second-order Glauber correlation function of two-photon light generated via type-II spontaneous parametric down-conversion. In order to obtain this result, two-photon light is transmitted through an optical fiber and the coincidence distribution is analyzed by means of the start-stop method. Beyond the experimental demonstration of an interesting effect in quantum optics, these results also have considerable relevance for quantum communications.

  9. Search for a Higgs boson decaying into two photons in the CMS detector

    Indian Academy of Sciences (India)

    Roberta Volpe; on behalf of the CMS Collaboration

    2012-11-01

    A search for a Higgs boson decaying into two photons in collisions at the LHC at a centre-of-mass energy of 7 TeV is presented. The analysis is performed on a dataset corresponding to 1.66 fb-1 of data recorded in 2011 by the CMS experiment. Limits are set on the cross-section of a Standard Model Higgs boson decaying into two photons, and on the cross-section of a fermiophobic Higgs boson decaying into two photons.

  10. Two-photon absorption of [2.2]paracyclophane derivatives in solution: A theoretical investigation

    Science.gov (United States)

    Ferrighi, Lara; Frediani, Luca; Fossgaard, Eirik; Ruud, Kenneth

    2007-12-01

    The two-photon absorption of a class of [2.2]paracyclophane derivatives has been studied using quadratic response and density functional theories. For the molecules investigated, several effects influencing the two-photon absorption spectra have been investigated, such as side-chain elongation, hydrogen bonding, the use of ionic species, and solvent effects, the latter described by the polarizable continuum model. The calculations have been carried out using a recent parallel implementation of the polarizable continuum model in the DALTON code. Special attention is given to those aspects that could explain the large solvent effect on the two-photon absorption cross sections observed experimentally for this class of compounds.

  11. Cyanines as new fluorescent probes for DNA detection and two-photon excited bioimaging.

    Science.gov (United States)

    Feng, Xin Jiang; Wu, Po Lam; Bolze, Frédéric; Leung, Heidi W C; Li, King Fai; Mak, Nai Ki; Kwong, Daniel W J; Nicoud, Jean-François; Cheah, Kok Wai; Wong, Man Shing

    2010-05-21

    A series of cyanine fluorophores based on fused aromatics as an electron donor for DNA sensing and two-photon bioimaging were synthesized, among which the carbazole-based biscyanine exhibits high sensitivity and efficiency as a fluorescent light-up probe for dsDNA, which shows selective binding toward the AT-rich regions. The synergetic effect of the bischromophoric skeleton gives a several-fold enhancement in a two-photon absorption cross-section as well as a 25- to 100-fold enhancement in two-photon excited fluorescence upon dsDNA binding.

  12. Four-State Model for Three-Branch Molecule's Two-Photon Absorption Properties

    Institute of Scientific and Technical Information of China (English)

    SU Yan; WANG Pei-Ji; ZHAO Peng; RONG Zhen-Yu

    2006-01-01

    @@ We present a four-state model for calculating the two-photon absorption of multi-branched molecules by using the time-depended function method. The numerical results indicate that the two-photon absorption cross section has a strong enhancement for three-branch molecules compared to two-branch structures. The maximal two-photon-absorption cross section is 2.358 × 10-47 cm 4 s/photon. At the same time, the charge-transfer process for the charge-transfer states is visualized in order to explain mechanism about the maximal TPA cross section.

  13. Dicke Coherent Narrowing in Two-Photon and Raman Spectroscopy of Thin Vapour Cells

    CERN Document Server

    Dutier, G; Hamdi, I; Maurin, I; Saltiel, S; Bloch, D; Ducloy, M; Dutier, Gabriel; Todorov, Petko; Hamdi, Ismah\\`{e}ne; Maurin, Isabelle; Saltiel, Solomon; Bloch, Daniel; Ducloy, Martial

    2005-01-01

    The principle of coherent Dicke narrowing in a thin vapour cell, in which sub-Doppler spectral lineshapes are observed under a normal irradiation for a l/2 thickness, is generalized to two-photon spectroscopy. Only the sum of the two wave vectors must be normal to the cell, making the two-photon scheme highly versatile. A comparison is provided between the Dicke narrowing with copropagating fields, and the residual Doppler-broadening occurring with counterpropagating geometries. The experimental feasibility is discussed on the basis of a first observation of a two-photon resonance in a 300 nm-thick Cs cell. Extension to the Raman situation is finally considered.

  14. Lighting the Way to See Inside Two-Photon Absorption Materials: Structure-Property Relationship and Biological Imaging.

    Science.gov (United States)

    Zhang, Qiong; Tian, Xiaohe; Zhou, Hongping; Wu, Jieying; Tian, Yupeng

    2017-02-23

    ions, including transition metals and lanthanides, can serve as an important part of the structure to control the intramolecular charge-transfer process that drives the 2PA process. As templates, transition metal ions can assemble simple to more sophisticated ligands in a variety of multipolar arrangements resulting in interesting and tailorable electronic and optical properties, depending on the nature of the metal center and the energetics of the metal-ligand interactions, such as intraligand charge-transfer (ILCT) and metal-ligand charge-transfer (MLCT) processes. Lanthanide complexes are attractive for a number of reasons: (i) their visible emissions are quite long-lived; (ii) their absorption and emission can be tuned with the aid of appropriate photoactive ligands; (iii) the accessible energy-transfer path between the photo-active ligands and the lanthanide ion can facilitate efficient lanthanide-based 2PA properties. Thus, the above materials with excellent 2PA properties should be applied in two-photon applications, especially two-photon fluorescence microscopy (TPFM) and related emission-based applications. Furthermore, the progress of research into the use of those new 2PA materials with moderate 2PA cross section in the near-infrared region, good Materials 2017, 10, 223 2 of 37 biocompatibility, and enhanced two-photon excited fluorescence for two-photon bio-imaging is summarized. In addition, several possible future directions in this field are also discussed (146 references).

  15. Lighting the Way to See Inside Two-Photon Absorption Materials: Structure–Property Relationship and Biological Imaging

    Science.gov (United States)

    Zhang, Qiong; Tian, Xiaohe; Zhou, Hongping; Wu, Jieying; Tian, Yupeng

    2017-01-01

    ions, including transition metals and lanthanides, can serve as an important part of the structure to control the intramolecular charge-transfer process that drives the 2PA process. As templates, transition metal ions can assemble simple to more sophisticated ligands in a variety of multipolar arrangements resulting in interesting and tailorable electronic and optical properties, depending on the nature of the metal center and the energetics of the metal-ligand interactions, such as intraligand charge-transfer (ILCT) and metal-ligand charge-transfer (MLCT) processes. Lanthanide complexes are attractive for a number of reasons: (i) their visible emissions are quite long-lived; (ii) their absorption and emission can be tuned with the aid of appropriate photoactive ligands; (iii) the accessible energy-transfer path between the photo-active ligands and the lanthanide ion can facilitate efficient lanthanide-based 2PA properties. Thus, the above materials with excellent 2PA properties should be applied in two-photon applications, especially two-photon fluorescence microscopy (TPFM) and related emission-based applications. Furthermore, the progress of research into the use of those new 2PA materials with moderate 2PA cross section in the near-infrared region, good biocompatibility, and enhanced two-photon excited fluorescence for two-photon bio-imaging is summarized. In addition, several possible future directions in this field are also discussed (146 references). PMID:28772584

  16. Lighting the Way to See Inside Two-Photon Absorption Materials: Structure–Property Relationship and Biological Imaging

    Directory of Open Access Journals (Sweden)

    Qiong Zhang

    2017-02-01

    properties. The metal ions, including transition metals and lanthanides, can serve as an important part of the structure to control the intramolecular charge-transfer process that drives the 2PA process. As templates, transition metal ions can assemble simple to more sophisticated ligands in a variety of multipolar arrangements resulting in interesting and tailorable electronic and optical properties, depending on the nature of the metal center and the energetics of the metal-ligand interactions, such as intraligand charge-transfer (ILCT and metal-ligand charge-transfer (MLCT processes. Lanthanide complexes are attractive for a number of reasons: (i their visible emissions are quite long-lived; (ii their absorption and emission can be tuned with the aid of appropriate photoactive ligands; (iii the accessible energy-transfer path between the photo-active ligands and the lanthanide ion can facilitate efficient lanthanide-based 2PA properties. Thus, the above materials with excellent 2PA properties should be applied in two-photon applications, especially two-photon fluorescence microscopy (TPFM and related emission-based applications. Furthermore, the progress of research into the use of those new 2PA materials with moderate 2PA cross section in the near-infrared region, good Materials 2017, 10, 223 2 of 37 biocompatibility, and enhanced two-photon excited fluorescence for two-photon bio-imaging is summarized. In addition, several possible future directions in this field are also discussed (146 references.

  17. Local Two-Photon Couplings and the J=0 Fixed Pole in Real and Virtual Compton Scattering

    Energy Technology Data Exchange (ETDEWEB)

    Brodsky, Stanley J.; Llanes-Estrada, Felipe J.; Szczepaniak, Adam P.

    2008-12-05

    The local coupling of two photons to the fundamental quark currents of a hadron gives an energy-independent contribution to the Compton amplitude proportional to the charge squared of the struck quark, a contribution which has no analog in hadron scattering reactions. We show that this local contribution has a real phase and is universal, giving the same contribution for real or virtual Compton scattering for any photon virtuality and skewness at fixed momentum transfer squared t. The t-dependence of this J = 0 fixed Regge pole is parameterized by a yet unmeasured even charge-conjugation form factor of the target nucleon. The t = 0 limit gives an important constraint on the dependence of the nucleon mass on the quark mass through the Weisberger relation. We discuss how this 1=x form factor can be extracted from high energy deeply virtual Compton scattering and examine predictions given by models of the H generalized parton distribution.

  18. Plasmonic-enhanced two-photon fluorescence with single gold nanoshell

    Science.gov (United States)

    Zhang, TianYue; Lu, GuoWei; Shen, HongMing; Perriat, P.; Martini, M.; Tillement, O.; Gong, QiHuang

    2014-06-01

    Single gold nanoshell with mutilpolar plasmon resonances is proposed to enhance two-photon fluorescence efficiently. The single emitter single nanoshell configuration is studied systematically by employing the finite-difference time-domain method. The emitter located inside or outside the nanoshell at various positions leads to a significantly different enhancement effect. The fluorescent emitter placed outside the nanoshell can achieve large fluorescence intensity given that both the position and orientation of the emission dipole are optimally controlled. In contrast, for the case of the emitter placed inside the nanoshell, it can experience substantial two-photon fluorescence enhancement without strict requirements upon the position and dipole orientations. Metallic nanoshell encapsulating many fluorescent emitters should be a promising nanocomposite configuration for bright two-photon fluorescence label. The results provide a comprehensive understanding about the plasmonic-enhanced two-photon fluorescence behaviors, and the nanocomposite configuration has great potential for optical detecting, imaging and sensing in biological applications.

  19. LANTHANIDE ENHANCE LUMINESCENCE (LEL) WITH ONE AND TWO PHOTON EXCITATION OF QUANTUM DYES LANTHANIDE (III) - MACROCYCLES

    Science.gov (United States)

    Title: Lanthanide Enhance Luminescence (LEL) with one and two photon excitation of Quantum Dyes? Lanthanide(III)-Macrocycles Principal Author:Robert C. Leif, Newport InstrumentsSecondary Authors:Margie C. Becker, Phoenix Flow Systems Al Bromm, Virginia Commonw...

  20. A compact two photon light sheet microscope for applications in neuroscience

    DEFF Research Database (Denmark)

    Piksarv, Peeter; Marti, Dominik; Le, Tuan

    2016-01-01

    We present a compact setup for two photon light sheet microscopy. By using pulsed Airy beam illumination we demonstrate eight-fold increase of the FOV compared to Gaussian light sheet with the same axial resolution....

  1. Solving Two Kinds of JC Models Relating to Two-Photon Process by Supersymmetric Transformation

    Institute of Scientific and Technical Information of China (English)

    FAN Hong-Yi; Wei-Jun

    2004-01-01

    We propose two kinds of new Jaynes Cummings models relating to two-photon process by using the supersymmetric unitary transformation. The corresponding energy eigenvalues and eigenvectors are obtained.

  2. Two-photon absorption properties of a new series of 2CTσ chromophores

    Science.gov (United States)

    Zhou, Yu-fang; Meng, Fan-qing; Zhao, Xian; Xu, Dong; Jiang, Min-hu

    2000-10-01

    We have designed and synthesized a new series of two-photon ASPT-like charge transfer moieties linked by σ-bond spacers to N-position of pyridine cycle. Both theoretical and experimental results show there is no linear absorption in 600-1300 nm, so two-photon properties can be expected in this range. Two-photon absorption (TPA) cross-sections were calculated by using INDO/CI and SOS methods. The results show that those compounds possess large cross-sections as well as appropriate absorption wavelengths. Also the magnitude of the cross-section changes regularly with the number of the σ-bond spacers. These imply that they are good candidates for two-photon devices.

  3. LANTHANIDE ENHANCE LUMINESCENCE (LEL) WITH ONE AND TWO PHOTON EXCITATION OF QUANTUM DYES LANTHANIDE (III) - MACROCYCLES

    Science.gov (United States)

    Title: Lanthanide Enhance Luminescence (LEL) with one and two photon excitation of Quantum Dyes? Lanthanide(III)-Macrocycles Principal Author:Robert C. Leif, Newport InstrumentsSecondary Authors:Margie C. Becker, Phoenix Flow Systems Al Bromm, Virginia Commonw...

  4. Observation of Nondegenerate Two-Photon Gain in GaAs

    CERN Document Server

    Reichert, Matthew; Salamo, Greg; Hagan, David J; Van Stryland, Eric W

    2016-01-01

    Two-photon lasers require materials with large two-photon gain (2PG) coefficients and low linear and nonlinear losses. Our previous demonstration of large enhancement of two-photon absorption in semiconductors for very different photon energies translates directly into enhancement of 2PG. We experimentally demonstrate nondegenerate 2PG in optically excited bulk GaAs via femtosecond pump-probe measurements. 2PG is isolated from other pump induced effects through the difference between measurements performed with parallel and perpendicular polarizations of pump and probe. An enhancement in the 2PG coefficient of nearly two orders-of-magnitude is reported. The results point a possible way toward two-photon semiconductor lasers.

  5. Sequential and coherent, optical and x-ray two-photon processes in atoms and molecules

    Science.gov (United States)

    Mills, Jeffrey Dean

    1997-09-01

    Vibronic and rovibronic implementations of conventional semiclassical theories, employing a phenomenological lineshape and descriptive of the absorption of a single photon by isolated chemical particles, are used to account for the absolute magnitude of the highly structured, broadband optical absorption, emission, radiation transfer, and refractive index of high- temperature (T ≈ 2000K), rare-gas-buffered, and locally equilibrated atomic and diatomic metal vapors (Li, Na, Al, and Li/Al). The polarized, resonant, inelastic scattering of x-rays (hν /approx 2.5 keV) from the K-edges of unoriented, chlorine- and sulfur- containing molecular gases (CH3Cl, H2S, and Cl2) is also modeled by means of the fully quantum- mechanical, time-independent Kramers-Heisenberg formalism applied in electronic and vibronic resolution. This accounts for the energy, polarization, and direction dependence of the anisotropic signal, concretely treats the demise of core-excited states by Auger-electron emission within the Feshbach-Fano theory of resonance- continuum mixing, and is in general valid for resonant, nonresonant, inelastic, and 'distinguishable' elastic scattering. Unusual, coherent interference phenomena within and between vibronic and electronic channels and related novel, otherwise-forbidden nondipole features expected to arise in molecules with equivalent atomic centers and recently observed in the chlorine molecule are explored along with their implications for common conceptions of 'localized, equivalent core-hole excited states.' Transition coherence, especially as manifested within the quantum-mechanical treatment of the spectral lineshape, is shown to provide the key to unifying the present single-step interpretation of two-photon x-ray scattering with that involving a pair of successive absorption and emission transitions generally regarded as two independent single-photon processes of the type described in the first portion of the work.

  6. Induced structural defects in Ti-doped ZnO and its two-photon-excitation

    Science.gov (United States)

    Martínez Julca, Milton A.; Rivera, Ivonnemary; Santillan Mercado, Jaime; Sierra, Heidy; Perales-Pérez, Oscar

    2016-03-01

    ZnO is a well-known luminescent material that reacts with light to generate free radicals enabling its use in cancer treatment by Photodynamic Therapy (PDT). Unfortunately, up to know, the photo-excitation of ZnO-based materials' requires excitation with ultraviolet light, which limits their biomedical applications. In this regard, this work investigates the effect of Ti species incorporation into the lattice of ZnO nanoparticles (NPs) with the aim of improving the corresponding optical properties and enabling the two-photoexcitation with 690nm-light (near infrared light). A modified polyol-based route was used to synthesize pure and Ti-doped (9% at.) ZnO NPs. X-ray diffraction confirmed the formation of ZnO-wurtzite whereas Scanning Electron Microscopy confirmed the formation of monodispersed 100-nm NPs. Raman Spectroscopy measurements evidenced the presence of zinc interstitials (Zni) and oxygen vacancies (VO) in the host oxide strcuture. Asynthesized NPs were excited using the technique of two-photon fluorescence microscopy (TPFM). The photoluminescence (PL) spectra generated from the analysis of TPFM images revealed a high emission peak presence in the green region (555 nm) that was assigned to VO. Also, a weak but noticeable band at 420 nm was detected, which is attributed to electron transition from the shallow donor level of Zni to the valence band. These PL transitions will favor triplet states formation necessary to yield cytotoxic reactive oxygen species. Furthermore, the presence of the PL peaks confirmed the Ti-ZnO NPs capacity to be excited by 690-nm light, thus, opening new possibilities for this NPs to be used in lightinduced bio-medical applications.

  7. One- and two-photon spectroscopy of highly excited states of alkali-metal atoms on helium nanodroplets.

    Science.gov (United States)

    Pifrader, Alexandra; Allard, Olivier; Auböck, Gerald; Callegari, Carlo; Ernst, Wolfgang E; Huber, Robert; Ancilotto, Francesco

    2010-10-28

    Alkali-metal atoms captured on the surface of superfluid helium droplets are excited to high energies (≈3 eV) by means of pulsed lasers, and their laser-induced-fluorescence spectra are recorded. We report on the one-photon excitation of the (n+1)p←ns transition of K, Rb, and Cs (n=4, 5, and 6, respectively) and on the two-photon one-color excitation of the 5d←5s transition of Rb. Gated-photon-counting measurements are consistent with the relaxation rates of the bare atoms, hence consistent with the reasonable expectation that atoms quickly desorb from the droplet and droplet-induced relaxation need not be invoked.

  8. Fast two-photon neuronal imaging and control using a spatial light modulator and ruthenium compounds

    Science.gov (United States)

    Peterka, Darcy S.; Nikolenko, Volodymyr; Fino, Elodie; Araya, Roberto; Etchenique, Roberto; Yuste, Rafael

    2010-02-01

    We have developed a spatial light modulator (SLM) based microscope that uses diffraction to shape the incoming two-photon laser source to any arbitrary light pattern. This allows the simultaneous imaging or photostimulation of different regions of a sample with three-dimensional precision at high frame rates. Additionally, we have combined this microscope with a new class of two photon active neuromodulators with Ruthenium BiPyridine (RuBi) based cages that offer great flexibility for neuronal control.

  9. Influence of Two Photon Absorption on Soliton Self-Frequency Shift

    DEFF Research Database (Denmark)

    Steffensen, Henrik; Rottwitt, Karsten; Jepsen, Peter Uhd;

    2011-01-01

    The creation of mid-infrared supercontinua necessitates the use of soft-glass fibers. However, some materials, like chalcogenide, have a substantial two photon absorption. We introduce a model for soliton self-frequency shift that successfully includes this effect.......The creation of mid-infrared supercontinua necessitates the use of soft-glass fibers. However, some materials, like chalcogenide, have a substantial two photon absorption. We introduce a model for soliton self-frequency shift that successfully includes this effect....

  10. Two-photon ionization of atomic hydrogen with elliptically polarized light

    Science.gov (United States)

    Kassaee, A.; Rustgi, M. L.; Long, S. A. T.

    1988-01-01

    The theory of two-photon ionization of a hydrogenic state in the nonrelativistic dipole approximation is generalized for elliptically polarized light. An application to the metastable 2S state of atomic hydrogen is made. Significant differences in the angular distribution of the outgoing electrons are found depending upon the polarization of the photons. It is claimed that two-photon ionization employing elliptically polarized photons from lasers may provide an additional test for the theories of multiphoton ionization.

  11. Two-photon neuronal and astrocytic stimulation with azobenzene-based photoswitches.

    Science.gov (United States)

    Izquierdo-Serra, Mercè; Gascón-Moya, Marta; Hirtz, Jan J; Pittolo, Silvia; Poskanzer, Kira E; Ferrer, Èric; Alibés, Ramon; Busqué, Félix; Yuste, Rafael; Hernando, Jordi; Gorostiza, Pau

    2014-06-18

    Synthetic photochromic compounds can be designed to control a variety of proteins and their biochemical functions in living cells, but the high spatiotemporal precision and tissue penetration of two-photon stimulation have never been investigated in these molecules. Here we demonstrate two-photon excitation of azobenzene-based protein switches and versatile strategies to enhance their photochemical responses. This enables new applications to control the activation of neurons and astrocytes with cellular and subcellular resolution.

  12. Three-Dimensional Control of DNA Hybridization by Orthogonal Two-Color Two-Photon Uncaging.

    Science.gov (United States)

    Fichte, Manuela A H; Weyel, Xenia M M; Junek, Stephan; Schäfer, Florian; Herbivo, Cyril; Goeldner, Maurice; Specht, Alexandre; Wachtveitl, Josef; Heckel, Alexander

    2016-07-25

    We successfully introduced two-photon-sensitive photolabile groups ([7-(diethylamino)coumarin-4-yl]methyl and p-dialkylaminonitrobiphenyl) into DNA strands and demonstrated their suitability for three-dimensional photorelease. To visualize the uncaging, we used a fluorescence readout based on double-strand displacement in a hydrogel and in neurons. Orthogonal two-photon uncaging of the two cages is possible, thus enabling complex scenarios of three-dimensional control of hybridization with light.

  13. Two-photon cooperative emission in the presence of athermal electromagnetic field

    Energy Technology Data Exchange (ETDEWEB)

    Enaki, N.A.; Mihalache, D

    1997-05-15

    The possibility of cooperative spontaneous two-photon emission of an extended radiators system and the influence of the external thermal electromagnetic field on the spontaneous emission rate, in such a system, are investigated. It is concluded that, in an external electromagnetic field, the two-photon cooperative emission rate increases significantly. The importance of this effect on the emission of gamma rays from inverted long-lived isomers triggered by X-ray thermal fields, is emphasized.

  14. Engineering Two-Atom Thermal Entanglement via Two-Photon Process

    Institute of Scientific and Technical Information of China (English)

    GUO Yan-Qing; ZHOU Ling; SONG He-Shan; YI Xue-Xi

    2004-01-01

    We study that two atoms simultaneously interact with a single mode thermal field via different couplings and different spontaneous emission rates when two-photon process is involved. It is found that we indeed can employ the different couplings to produce the two-atom thermal entanglement in two-photon process. The different atomic spontaneous emission rates are also utilizable in generating thermal entanglement. We also investigate the effect of the can obtain a strong and steady entanglement.

  15. Two-Photon Exchange Corrections to Single Spin Asymmetry of Neutron and 3He

    Institute of Scientific and Technical Information of China (English)

    CHEN Dian-Yong; DONG Yu-Bing

    2011-01-01

    In a simple hadronic model, the two-photon exchange contributions to the single spin asymmetries for the nucleon and the 3He are estimated. The results show that the elastic contributions of two-photon exchange to the single spin asymmetries for the nucleon are rather small while those for the 3He are relatively large. Besides the strong angular dependence, the twophoton contributions to the single spin asymmetry for the 3He are very sensitive to the momentum transfer.

  16. Quantum dynamics of two-photon quantum Rabi model

    Science.gov (United States)

    Lü, Zhiguo; Zhao, Chunjian; Zheng, Hang

    2017-02-01

    We apply a simple analytical method based on a unitary transformation to calculate the ground state, its excitation spectrum and quantum dynamic evolution of physical quantities for the double-photon quantum Rabi Hamiltonian over the wide coupling-strength range. The concise analytical method possesses the same mathematical simplicity as the approach of the rotating wave approximation (RWA). By quantitative comparison with the numerically exact result obtained by matrix diagonalization, we confirm that our calculated results obtained by transformed rotating-wave method are not only accurate in the weak coupling regime but also correct in intermediate strong-coupling case. In the intermediate ultrastrong-coupling regime, the calculated values of the ground state and lower lying excited states are nearly the same as the exact ones. It turns out that our calculation for the energy spectrum is beyond the ordinary-RWA. Meanwhile, we demonstrate the signatures resulting from the counter-rotating wave terms by monitoring the population, the coherence, the squeezing of the photon under the ultra-strong conditions. In particular, we find that when the frequency of the photon is much larger than the transition frequency of the system, the lineshape of the time evolution becomes complicated with the increase of the coupling strength, which may be verified experimentally.

  17. Two-Photon and Second Harmonic Microscopy in Clinical and Translational Cancer Research

    Science.gov (United States)

    PERRY, SETH W.; BURKE, RYAN M.; BROWN, EDWARD B.

    2012-01-01

    Application of two-photon microscopy (TPM) to translational and clinical cancer research has burgeoned over the last several years, as several avenues of pre-clinical research have come to fruition. In this review, we focus on two forms of TPM—two-photon excitation fluorescence microscopy, and second harmonic generation microscopy—as they have been used for investigating cancer pathology in ex vivo and in vivo human tissue. We begin with discussion of two-photon theory and instrumentation particularly as applicable to cancer research, followed by an overview of some of the relevant cancer research literature in areas that include two-photon imaging of human tissue biopsies, human skin in vivo, and the rapidly developing technology of two-photon microendoscopy. We believe these and other evolving two-photon methodologies will continue to help translate cancer research from the bench to the bedside, and ultimately bring minimally invasive methods for cancer diagnosis and treatment to therapeutic reality. PMID:22258888

  18. Development of Two-Photon Pump Polarization Spectroscopy Probe Technique Tpp-Psp for Measurements of Atomic Hydrogen .

    Science.gov (United States)

    Satija, Aman; Lucht, Robert P.

    2015-06-01

    Atomic hydrogen (H) is a key radical in combustion and plasmas. Accurate knowledge of its concentration can be used to better understand transient phenomenon such as ignition and extinction in combustion environments. Laser induced polarization spectroscopy is a spatially resolved absorption technique which we have adapted for quantitative measurements of H atom. This adaptation is called two-photon pump, polarization spectroscopy probe technique (TPP-PSP) and it has been implemented using two different laser excitation schemes. The first scheme involves the two-photon excitation of 1S-2S transitions using a linearly polarized 243-nm beam. An anisotropy is created amongst Zeeman states in 2S-3P levels using a circularly polarized 656-nm pump beam. This anisotropy rotates the polarization of a weak, linearly polarized probe beam at 656 nm. As a result, the weak probe beam "leaks" past an analyzer in the detection channel and is measured using a PMT. This signal can be related to H atom density in the probe volume. The laser beams were created by optical parametric generation followed by multiple pulse dye amplification stages. This resulted in narrow linewidth beams which could be scanned in frequency domain and varied in energy. This allowed us to systematically investigate saturation and Stark effect in 2S-3P transitions with the goal of developing a quantitative H atom measurement technique. The second scheme involves the two-photon excitation of 1S-2S transitions using a linearly polarized 243-nm beam. An anisotropy is created amongst Zeeman states in 2S-4P transitions using a circularly polarized 486-nm pump beam. This anisotropy rotates the polarization of a weak, linearly polarized probe beam at 486 nm. As a result the weak probe beam "leaks" past an analyzer in the detection channel and is measured using a PMT. This signal can be related to H atom density in the probe volume. A dye laser was pumped by third harmonic of a Nd:YAG laser to create a laser beam

  19. Enhanced two-photon fluorescence imaging and therapy of cancer cells via Gold@bridged silsesquioxane nanoparticles.

    Science.gov (United States)

    Croissant, Jonas; Maynadier, Marie; Mongin, Olivier; Hugues, Vincent; Blanchard-Desce, Mireille; Chaix, Arnaud; Cattoën, Xavier; Wong Chi Man, Michel; Gallud, Audrey; Gary-Bobo, Magali; Garcia, Marcel; Raehm, Laurence; Durand, Jean-Olivier

    2015-01-21

    A two-photon photosensitizer with four triethoxysilyl groups is synthesized through the click reaction. This photosensitizer allows the design of bridged silsesquioxane (BS) nanoparticles through a sol-gel process; moreover, gold core BS shells or BS nanoparticles decorated with gold nanospheres are synthesized. An enhancement of the two-photon properties is noted with gold and the nanoparticles are efficient for two-photon imaging and two-photon photodynamic therapy of cancer cells.

  20. Two-photon absorption spectroscopy of stilbene and phenanthrene: Excited-state analysis and comparison with ethylene and toluene

    Science.gov (United States)

    de Wergifosse, Marc; Elles, Christopher G.; Krylov, Anna I.

    2017-05-01

    Two-photon absorption (2PA) spectra of several prototypical molecules (ethylene, toluene, trans- and cis-stilbene, and phenanthrene) are computed using the equation-of-motion coupled-cluster method with single and double substitutions. The states giving rise to the largest 2PA cross sections are analyzed in terms of their orbital character and symmetry-based selection rules. The brightest 2PA transitions correspond to Rydberg-like states from fully symmetric irreducible representations. Symmetry selection rules dictate that totally symmetric transitions typically have the largest 2PA cross sections for an orientationally averaged sample when there is no resonance enhancement via one-photon accessible intermediate states. Transition dipole arguments suggest that the strongest transitions also involve the most delocalized orbitals, including Rydberg states, for which the relative transition intensities can be rationalized in terms of atomic selection rules. Analysis of the 2PA transitions provides a foundation for predicting relative 2PA cross sections of conjugated molecules based on simple symmetry and molecular orbital arguments.

  1. Computing Transition Rates for the 1-D Stochastic Ginzburg-Landau-Allen-Cahn Equation for Finite-Amplitude Noise with a Rare Event Algorithm

    Science.gov (United States)

    Rolland, Joran; Bouchet, Freddy; Simonnet, Eric

    2016-01-01

    In this article we compute and analyse the transition rates and duration of reactive trajectories of the stochastic 1-D Allen-Cahn equations for both the Freidlin-Wentzell regime (weak noise or temperature limit) and finite-amplitude white noise, as well as for small and large domain. We demonstrate that extremely rare reactive trajectories corresponding to direct transitions between two metastable states are efficiently computed using an algorithm called adaptive multilevel splitting. This algorithm is dedicated to the computation of rare events and is able to provide ensembles of reactive trajectories in a very efficient way. In the small noise limit, our numerical results are in agreement with large-deviation predictions such as instanton-like solutions, mean first passages and escape probabilities. We show that the duration of reactive trajectories follows a Gumbel distribution like for one degree of freedom systems. Moreover, the mean duration growths logarithmically with the inverse temperature. The prefactor given by the potential curvature grows exponentially with size. The main novelty of our work is that we also perform an analysis of reactive trajectories for large noises and large domains. In this case, we show that the position of the reactive front is essentially a random walk. This time, the mean duration grows linearly with the inverse temperature and quadratically with the size. Using a phenomenological description of the system, we are able to calculate the transition rate, although the dynamics is described by neither Freidlin-Wentzell or Eyring-Kramers type of results. Numerical results confirm our analysis.

  2. Note: Derivation of two-photon circular dichroism - Addendum to "two-photon circular dichroism" [J. Chem. Phys. 62, 1006 (1975)

    OpenAIRE

    Friese, Daniel Henrik

    2015-01-01

    Published version, also available at http://dx.doi.org/10.1063/1.4930017 This addendum shows the detailed derivation of the fundamental equations for two-photon circular dichroism which are given in a very condensed form in the original publication [I. Tinoco, J. Chem. Phys. 62, 1006 (1975)]. In addition, some minor errors are corrected and some of the derivations in the original publication are commented.

  3. Two-photon excitation spectroscopy of Cr3+:K2NaScF6 elpasolite: I. Experimental aspects

    Science.gov (United States)

    Wein, G. R.; Hamilton, D. S.; Sliwczuk, U.; Rinzler, A. G.; Bartram, R. H.

    2001-03-01

    Two-photon excitation experiments were performed to improve understanding of electron-lattice coupling and its effects on intra-3d3 transitions. Cr3+ occupies a scandium octahedral site in K2NaScF6. The transitions studied were 4A2g→ 4T2g and 4A2g→ 4T1ag. Complete spectra were recorded at a temperature of 10 K with the polarization vector or crystallographic direction. The two bands exhibit different polarization anisotropies and phonon couplings. The electric-dipole-forbidden 4A2g→ 4T2g band appears to be built on an eg-mode false origin and contains Fano antiresonances. This broad transition band lacks a zero-phonon line or any other sharp structure. The 4A2g→ 4T1ag transition zero-phonon line is evident and shows a 163 cm-1 low-temperature phase-transition-induced splitting. It also contains an extended progression of 35 phonon peaks corresponding to a lattice mode with phonon energy 106 cm-1, and a second progression with phonon energy 310 cm-1. The very asymmetric phonon side band displays a polarization anisotropy that differs from that of the zero-phonon line. To facilitate analysis of the data, measurements of low-temperature 4T2g→ 4A2g emission spectra with one-photon excitation are also reported and interpreted in the present paper.

  4. Measurement of degenerate two-photon absorption spectra of a series of developed two-photon initiators using a dispersive white light continuum Z-scan

    Science.gov (United States)

    Ajami, Aliasghar; Husinsky, Wolfgang; Tromayer, Maximilian; Gruber, Peter; Liska, Robert; Ovsianikov, Aleksandr

    2017-08-01

    To achieve efficient micro- and nanostructuring based on two-photon polymerization (2PP), the development and evaluation of specialized two-photon initiators (2PIs) are essential. Hence, a reliable method to determine the two-photon absorption (2PA) spectra of the synthesized 2PIs used for 2PP structuring is crucial. A technique by which absolute visible-to-near-infrared 2PA spectra of degenerate nature can be determined via performing a single dispersive white-light continuum (WLC) Z-scan has been realized. Using a dispersed white light beam containing 8 fs pulses at wavelengths ranging from 650 nm to 950 nm, the nonlinear transmittance as a function of the sample position can be measured for all spectral components by performing a single scan along the laser beam propagation direction. In this work, the 2PA spectrum of three different 2PIs was determined using this technique. 2PP structuring was also accomplished using the developed 2PIs at different wavelengths. Tuning the wavelength of the laser to match the peak of the 2PA spectra of the developed 2PIs resulted in lower intensity thresholds and facilitated higher structuring speeds. As an example, using M2CMK 2PI for 2PP, the scanning speed can be increased up to 5 folds when the laser wavelength is tuned to 760 nm (i.e., 2PA maximum) instead of the conventionally used 800 nm.

  5. Pseudopotential calculations and photothermal lensing measurements of two-photon absorption in solids

    Energy Technology Data Exchange (ETDEWEB)

    White, W.T. III

    1985-11-04

    We have studied two-photon absorption in solids theoretically and experimentally. We have shown that it is possible to use accurate band structure techniques to compute two-photon absorption spectra within 15% of measured values in a wide band-gap material, ZnS. The empirical pseudopotential technique that we used is significantly more accurate than previous models of two-photon absorption in zinc blende materials, including present tunneling theories (which are essentially parabolic-band results in disguise) and the nonparabolic-band formalism of Pidgeon et al. and Weiler. The agreement between our predictions and previous measurements allowed us to use ZnS as a reference material in order to validate a technique for measuring two-photon absorption that was previously untried in solids, pulsed dual-beam thermal lensing. With the validated technique, we examined nonlinear absorption in one other crystal (rutile) and in several glasses, including silicates, borosilicates, and one phosphate glass. Initially, we believed that the absorption edges of all the materials were comparable; however, subsequent evidence suggested that the effective band-gap energies of the glasses were above the energy of two photons in our measurement. Therefore, we attribute the nonlinear absorption that we observed in glasses to impurities or defects. The measured nonlinear absorption coefficients were of the order of a few cm/TW in the glasses and of the order of 10 cm/GW in the crystals, four orders of magnitude higher than in glasses. 292 refs.

  6. Near infrared two-photon excitation cross-sections of voltage-sensitive dyes.

    Science.gov (United States)

    Fisher, Jonathan A N; Salzberg, Brian M; Yodh, Arjun G

    2005-10-15

    Microscopy based on voltage-sensitive dyes has proven effective for revealing spatio-temporal patterns of neuronal activity in vivo and in vitro. Two-photon microscopy using voltage-sensitive dyes offers the possibility of wide-field visualization of membrane potential on sub-cellular length scales, hundreds of microns below the tissue surface. Very little information is available, however, about the utility of voltage-sensitive dyes for two-photon imaging purposes. Here we report on measurements of two-photon fluorescence excitation cross-sections for nine voltage-sensitive dyes in a solvent, octanol, intended to simulate the membrane environment. Ultrashort light pulses from a Ti:sapphire laser were used for excitation from 790 to 960 nm, and fluorescein dye was used as a calibration standard. Overall, dyes RH795, RH421, RH414, di-8-ANEPPS, and di-8-ANEPPDHQ had the largest two-photon excitation cross-sections ( approximately 15 x 10(-50)cm4 s photon(-1)) in this wavelength region and are therefore potentially useful for two-photon microscopy. Interestingly, di-8-ANEPPDHQ, a chimera constructed from the potentiometric dyes RH795 and di-8-ANEPPS, exhibited larger cross-sections than either of its constituents.

  7. Localized Polymerization Using Single Photon Photoinitiators in Two-photon process for Fabricating Subwavelength Structures

    CERN Document Server

    Ummethala, Govind; Chaudhary, Raghvendra P; Hawal, Suyog; Saxena, Sumit; Shukla, Shobha

    2016-01-01

    Localized polymerization in subwavelength volumes using two photon dyes has now become a well-established method for fabrication of subwavelength structures. Unfortunately, the two photon absorption dyes used in such process are not only expensive but also proprietary. LTPO-L is an inexpensive, easily available single photon photoinitiator and has been used extensively for single photon absorption of UV light for polymerization. These polymerization volumes however are not localized and extend to micron size resolution having limited applications. We have exploited high quantum yield of radicals of LTPO-Lfor absorption of two photons to achieve localized polymerization in subwavelength volumes, much below the diffraction limit. Critical concentration (10wt%) of LTPO-Lin acrylate (Sartomer) was found optimal to achieve subwavelength localized polymerization and has been demonstrated by fabricating 2D/3D complex nanostructures and functional devices such as variable polymeric gratings with nanoscaled subwavelen...

  8. In vivo two-photon calcium imaging in the visual system.

    Science.gov (United States)

    Ohki, Kenichi; Reid, R Clay

    2014-04-01

    Two-photon imaging of calcium-sensitive dyes in vivo has become a common tool used by neuroscientists, largely because of the development of bolus loading techniques, which can label every neuron in a local circuit with calcium-sensitive dye. Like multielectrode recordings, two-photon imaging paired with bolus loading provides a method for monitoring many neurons at once, but, in addition, it provides a means for determining the precise location of every neuron. Thus, it is an ideal method for studying the fine-scale functional architecture of the cortex and guiding the experimenter to individual neurons that can be targeted for further anatomical study. Two-photon calcium imaging enables study of the fine structure of functional maps in the visual cortex in cats and rodents. In mice, it can allow the characterization of specific cell types when paired with transgenic or retrograde labeling.

  9. Investigation of two-photon absorption induced excited state absorption in a fluorenyl-based chromophore.

    Science.gov (United States)

    Li, Changwei; Yang, Kun; Feng, Yan; Su, Xinyan; Yang, Junyi; Jin, Xiao; Shui, Min; Wang, Yuxiao; Zhang, Xueru; Song, Yinglin; Xu, Hongyao

    2009-12-03

    Two-photon absorption induced excited state absorption in the solution of a new fluorenyl-based chromophore is investigated by a time-resolved pump-probe technique using femtosecond pulses. With the help of an additional femtosecond open-aperture Z-scan technique, numerical simulations based on a three-energy level model are used to interpret the experimental results, and we determine the nonlinear optical parameters of this new chromophore uniquely. Large two-photon absorption cross section and excited state absorption cross section for singlet excited state are obtained, indicating a good candidate for optical limiting devices. Moreover, the influence of two-beam coupling induced energy transfer in neat N,N'-dimethylformamide solvent is also considered, although this effect is strongly restrained by the instantaneous two-photon absorption.

  10. Visualization of two-photon Rabi oscillations in evanescently coupled optical waveguides

    Energy Technology Data Exchange (ETDEWEB)

    Ornigotti, M; Valle, G Della; Fernandez, T Toney; Laporta, P; Longhi, S [Dipartimento di Fisica and Istituto di Fotonica e Nanotecnologie del CNR, Politecnico di Milano, Piazza L. da Vinci 32, I-20133 Milano (Italy); Coppa, A; Foglietti, V [Istituto di Fotonica e Nanotecnologie del CNR, sezione di Roma, Via Cineto Romano 42, 00156 Roma (Italy)], E-mail: longhi@fisi.polimi.it

    2008-04-28

    An optical analogue of two-photon Rabi oscillations, occurring in a three-level atomic or molecular system coherently driven by two detuned laser fields, is theoretically proposed and experimentally demonstrated using three evanescently coupled optical waveguides realized on an active glass substrate. The optical analogue stems from the formal analogy between spatial propagation of light waves in the three-waveguide structure and the coherent temporal evolution of populations in a three-level atomic medium driven by two laser fields under two-photon resonance. In our optical experiment, two-photon Rabi oscillations are thus visualized as a slow spatial oscillatory exchange of light power between the two outer waveguides of the structure with a small excitation of the central waveguide.

  11. Selective two-photon excitation of a vibronic state by correlated photons.

    Science.gov (United States)

    Oka, Hisaki

    2011-03-28

    We theoretically investigate the two-photon excitation of a molecular vibronic state by correlated photons with energy anticorrelation. A Morse oscillator having three sets of vibronic states is used, as an example, to evaluate the selectivity and efficiency of two-photon excitation. We show that a vibrational mode can be selectively excited with high efficiency by the correlated photons, without phase manipulation or pulse-shaping techniques. This can be achieved by controlling the quantum correlation so that the photon pair concurrently has two pulse widths, namely, a temporally narrow width and a spectrally narrow width. Though this concurrence is seemingly contradictory, we can create such a photon pair by tailoring the quantum correlation between two photons.

  12. Observation of single- and two-photon beating between independent Raman scattering

    CERN Document Server

    Chen, Li-Qing; Zhang, Guo-Wan; Ou, Z Y; Zhang, Weiping

    2010-01-01

    By using spontaneous Raman processes in the high gain regime, we produce two independent Raman Stokes fields from an atomic ensemble. Temporal beating is observed between the two directly generated Stokes fields in a single realization. The beat frequency is found to be a result of an AC Stark frequency shift effect. However, due to the spontaneous nature of the process, the phases of the two Stokes fields change from one realization to another so that the beat signal disappears after average over many realizations. On the other hand, the beat signal is recovered in a two-photon correlation measurement, showing a two-photon interference effect. The two-photon beat signal enables us to obtain dephasing information in the Raman process. The dephasing effect is found to depend on the temperature of the atomic medium.

  13. Enhanced-locality fiber-optic two-photon-fluorescence live-brain interrogation

    Energy Technology Data Exchange (ETDEWEB)

    Fedotov, I. V.; Doronina-Amitonova, L. V. [International Laser Center, Physics Department, M.V. Lomonosov Moscow State University, Moscow 119992 (Russian Federation); Russian Quantum Center, ul. Novaya 100, Skolkovo, Moscow Region 1430125 (Russian Federation); Kurchatov Institute National Research Center, Moscow (Russian Federation); Sidorov-Biryukov, D. A.; Fedotov, A. B. [International Laser Center, Physics Department, M.V. Lomonosov Moscow State University, Moscow 119992 (Russian Federation); Russian Quantum Center, ul. Novaya 100, Skolkovo, Moscow Region 1430125 (Russian Federation); Anokhin, K. V. [Kurchatov Institute National Research Center, Moscow (Russian Federation); P.K. Anokhin Institute of Normal Physiology, Russian Academy of Medical Sciences, Moscow (Russian Federation); Kilin, S. Ya. [B.I. Stepanov Institute of Physics, National Academy of Sciences of Belarus, Minsk (Belarus); Sakoda, K. [National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044 (Japan); Zheltikov, A. M. [International Laser Center, Physics Department, M.V. Lomonosov Moscow State University, Moscow 119992 (Russian Federation); Russian Quantum Center, ul. Novaya 100, Skolkovo, Moscow Region 1430125 (Russian Federation); Department of Physics and Astronomy, Texas A and M University, College Station, Texas 77843 (United States); Center of Photochemistry, Russian Academy of Sciences, ul. Novatorov 7a, Moscow 117421 (Russian Federation)

    2014-02-24

    Two-photon excitation is shown to substantially enhance the locality of fiber-based optical interrogation of strongly scattering biotissues. In our experiments, a high-numerical-aperture, large-core-are fiber probe is used to deliver the 200-fs output of a 100-MHz mode-locked ytterbium fiber laser to samples of live mouse brain, induce two-photon fluorescence of nitrogen–vacancy centers in diamond markers in brain sample. Fiber probes with a high numerical aperture and a large core area are shown to enable locality enhancement in fiber-laser–fiber-probe two-photon brain excitation and interrogation without sacrificing the efficiency of fluorescence response collection.

  14. Design, synthesis, and characterization of photoinitiators for two-photon polymerization

    Science.gov (United States)

    Whitby, Reece; MacMillan, Ryan; Janssens, Stefaan; Raymond, Sebastiampillai; Clarke, Dave; Kay, Andrew; Jin, Jianyong; Simpson, Cather M.

    2016-09-01

    A series of dipolar and quadrupolar two-photon absorption (2PA) photoinitiators (PIs) based around the well-known triphenylamine (TPA) core and tricyanofuran (TCF) acceptors have been prepared for use in two-photon polymerisation (TPP). The synthesised dipolar species are designated as 5 and 7, and the remaining quadrupolar species are 6, 8, 9 and 10. Large two-photon absorption cross-sections (δ2PA) ranging between 333 - 507 GM were measured at 780 nm using the z-scan technique. Fluorescence quantum yields (ΦF) were below 3% across the series when compared to Rhodamine 6G as a reference standard. Finally, TPP tests were conducted on PIs 7 and 8 to assess their ability to initiate the polymerisation of acrylate monomers using an 800 nm femtosecond Ti:Sapphire laser system.

  15. Two-photon calcium imaging in mice navigating a virtual reality environment.

    Science.gov (United States)

    Leinweber, Marcus; Zmarz, Pawel; Buchmann, Peter; Argast, Paul; Hübener, Mark; Bonhoeffer, Tobias; Keller, Georg B

    2014-02-20

    In recent years, two-photon imaging has become an invaluable tool in neuroscience, as it allows for chronic measurement of the activity of genetically identified cells during behavior(1-6). Here we describe methods to perform two-photon imaging in mouse cortex while the animal navigates a virtual reality environment. We focus on the aspects of the experimental procedures that are key to imaging in a behaving animal in a brightly lit virtual environment. The key problems that arise in this experimental setup that we here address are: minimizing brain motion related artifacts, minimizing light leak from the virtual reality projection system, and minimizing laser induced tissue damage. We also provide sample software to control the virtual reality environment and to do pupil tracking. With these procedures and resources it should be possible to convert a conventional two-photon microscope for use in behaving mice.

  16. Three-dimensional protein networks assembled by two-photon activation.

    Science.gov (United States)

    Gatterdam, Volker; Ramadass, Radhan; Stoess, Tatjana; Fichte, Manuela A H; Wachtveitl, Josef; Heckel, Alexander; Tampé, Robert

    2014-05-26

    Spatial and temporal control over chemical and biological processes plays a key role in life and material sciences. Here we synthesized a two-photon-activatable glutathione (GSH) to trigger the interaction with glutathione S-transferase (GST) by light at superior spatiotemporal resolution. The compound shows fast and well-confined photoconversion into the bioactive GSH, which is free to interact with GST-tagged proteins. The GSH/GST interaction can be phototriggered, changing its affinity over several orders of magnitude into the nanomolar range. Multiplexed three-dimensional (3D) protein networks are simultaneously generated in situ through two-photon fs-pulsed laser-scanning excitation. The two-photon activation facilitates the three-dimensional assembly of protein structures in real time at hitherto unseen resolution in time and space, thus opening up new applications far beyond the presented examples.

  17. Highly selective population of two excited states in nonresonant two-photon absorption

    Institute of Scientific and Technical Information of China (English)

    Zhang Hui; Zhang Shi-An; Sun Zhen-Rong

    2011-01-01

    A nonresonant two-photon absorption process can be manipulated by tailoring the ultra-short laser pulse.In this paper,we theoretically demonstrate a highly selective population of two excited states in the nonresonant two-photon absorption process by rationally designing a spectral phase distribution.Our results show that one excited state is maximally populated while the other state population is widely tunable from zero to the maximum value.We believe that the theoretical results may play an important role in the selective population of a more complex nonlinear process comprising nonresonant two-photon absorption,such as resonance-mediated(2+1)-three-photon absorption and (2+1)-resonant multiphoton ionization.

  18. Two-Photon Absorption Properties of Mn-Doped ZnS Quantum Dots

    Institute of Scientific and Technical Information of China (English)

    ZHENG Jia-Jin; ZHANG Gui-Lan; GUO Yang-Xue; WANG Xiao-Yan; CHEN Wen-Ju; ZHANG Xiao-Song; HUA Yu-Lin

    2006-01-01

    @@ We investigate the two-photon absorption and nonlinear refractive index properties of a quantum dot material based on ZnS nanocrystals doped with Mn isoelectronic impurities, using the Z-scan technique with 532nm picosecond laser pulses. The Mn-doped ZnS quantum dots have an average two-photon absorption cross section as high as 13600 Goeppert-Mayer units, which turn it into a very promising material for fluorescent label and imaging in biological samples. In addition, we also found that the two-photon absorption coeflicient initially increases and then decreases with increasing pulse irradiance, which demonstrates the presence of the higherorder nonlinearity under the strong excitation.

  19. Scanless functional imaging of hippocampal networks using patterned two-photon illumination through GRIN lenses

    KAUST Repository

    Moretti, Claudio

    2016-09-12

    Patterned illumination through the phase modulation of light is increasingly recognized as a powerful tool to investigate biological tissues in combination with two-photon excitation and light-sensitive molecules. However, to date two-photon patterned illumination has only been coupled to traditional microscope objectives, thus limiting the applicability of these methods to superficial biological structures. Here, we show that phase modulation can be used to efficiently project complex two-photon light patterns, including arrays of points and large shapes, in the focal plane of graded index (GRIN) lenses. Moreover, using this approach in combination with the genetically encoded calcium indicator GCaMP6, we validate our system performing scanless functional imaging in rodent hippocampal networks in vivo ~1.2 mm below the brain surface. Our results open the way to the application of patterned illumination approaches to deep regions of highly scattering biological tissues, such as the mammalian brain.

  20. Robust spatial-polarization hyperentanglement distribution of two-photon systems against collective noise

    Science.gov (United States)

    Gao, Cheng-Yan; Wang, Guan-Yu; Alzahrani, Faris; Hobiny, Aatef; Deng, Fu-Guo

    2017-03-01

    Hyperentanglement is a significant resource for high-capacity quantum communication. Here we present a robust spatial-polarization hyperentanglement distribution scheme for two-photon systems. The error on the polarization states of two-photon systems transmitted from two paths can be corrected resorting to the robust time-bin entanglement which suffers little from the channel noise. The spatial bit-flip error takes place with a very small probability and the spatial phase-flip error can be precluded by adjusting the path-length of spatial modes. Using this scheme, the two parties in quantum communication can share a maximally hyperentangled state of two-photon systems in a deterministic way, which will improve the efficiency of quantum communication largely.

  1. One- and two-photon scattering from generalized V-type atoms

    OpenAIRE

    Sánchez-Burillo, Eduardo; Martín-Moreno, Luis; Zueco, David; García-Ripoll, Juan José

    2016-01-01

    The one- and two-photon scattering matrix S is obtained analytically for a one-dimensional waveguide and a point-like scatterer with N excited levels (generalized V -type atom). We argue that the two-photon scattering matrix contains sufficient information to distinguish between different level structures which are equivalent for single-photon scattering, such as a V -atom with N = 2 excited levels and two two-level systems. In particular, we show that the scattering with the V -type atom exh...

  2. Insights into esophagus tissue architecture using two-photon confocal microscopy

    Science.gov (United States)

    Liu, Nenrong; Wang, Yue; Feng, Shangyuan; Chen, Rong

    2013-08-01

    In this paper, microstructures of human esophageal mucosa were evaluated using the two-photon laser scanning confocal microscopy (TPLSCM), based on two-photon excited fluorescence (TPEF) and second harmonic generation (SHG). The distribution of epithelial cells, muscle fibers of muscularis mucosae has been distinctly obtained. Furthermore, esophageal submucosa characteristics with cancer cells invading into were detected. The variation of collagen, elastin and cancer cells is very relevant to the pathology in esophagus, especially early esophageal cancer. Our experimental results indicate that the MPM technique has the much more advantages for label-free imaging, and has the potential application in vivo in the clinical diagnosis and monitoring of early esophageal cancer.

  3. Axial range of conjugate adaptive optics in two-photon microscopy

    CERN Document Server

    Paudel, Hari P; Mertz, Jerome; Bifano, Thomas

    2015-01-01

    We describe an adaptive optics technique for two-photon microscopy in which the deformable mirror used for aberration compensation is positioned in a plane conjugate to the plane of the aberration. We demonstrate in a proof-of-principle experiment that this technique yields a large field of view advantage in comparison to standard pupil-conjugate adaptive optics. Further, we show that the extended field of view in conjugate AO is maintained over a relatively large axial translation of the deformable mirror with respect to the conjugate plane. We conclude with a discussion of limitations and prospects for the conjugate AO technique in two-photon biological microscopy.

  4. Arduino Due based tool to facilitate in vivo two-photon excitation microscopy.

    Science.gov (United States)

    Artoni, Pietro; Landi, Silvia; Sato, Sebastian Sulis; Luin, Stefano; Ratto, Gian Michele

    2016-04-01

    Two-photon excitation spectroscopy is a powerful technique for the characterization of the optical properties of genetically encoded and synthetic fluorescent molecules. Excitation spectroscopy requires tuning the wavelength of the Ti:sapphire laser while carefully monitoring the delivered power. To assist laser tuning and the control of delivered power, we developed an Arduino Due based tool for the automatic acquisition of high quality spectra. This tool is portable, fast, affordable and precise. It allowed studying the impact of scattering and of blood absorption on two-photon excitation light. In this way, we determined the wavelength-dependent deformation of excitation spectra occurring in deep tissues in vivo.

  5. Two-photon luminescence microscopy of field enhancement at gold nanoparticles

    DEFF Research Database (Denmark)

    Beermann, Jonas; Bozhevolnyi, Sergey I.

    2005-01-01

    Using a reflection scanning optical microscope detecting two-photon luminescence (TPL) we have imaged square gold bumps positioned in a periodic array either on a smooth gold film or directly on a glass substrate. The second-harmonic (SH) and TPL response from these structures show both polarizat......Using a reflection scanning optical microscope detecting two-photon luminescence (TPL) we have imaged square gold bumps positioned in a periodic array either on a smooth gold film or directly on a glass substrate. The second-harmonic (SH) and TPL response from these structures show both...

  6. Two-photon laser fabrication of three-dimensional silver microstructures with submicron scale linewidth

    Energy Technology Data Exchange (ETDEWEB)

    Tsutsumi, Naoto; Nagata, Kazuya; Sakai, Wataru [Kyoto Institute of Technology, Department of Macromolecular Science and Engineering, Graduate School of Science and Technology, Kyoto (Japan)

    2011-05-15

    We show three-dimensional silver microstructures with a submicron scale linewidth fabricated via two-photon photoreduction of silver ions in a poly(N-vinylpyrrolidone) (PVP) matrix. Femtosecond laser at 508 nm directly excites the carbonyl group of PVP via two-photon excitation to reduce silver ions. Lone pair electrons in PVP stabilized silver ions and lower molecular weight of PVP prevented silver clusters growing larger. The effect of molecular weight of PVP on linewidth of silver nanowire is investigated. (orig.)

  7. Threshold Property of Photoresist Film for Two-photon Optical Memory

    Institute of Scientific and Technical Information of China (English)

    ZHANG Jiangying; MING Hai; LIANG Zhongcheng; WANG Pei; XIE Jianping; XIE Aifang; ZHANG Zebo

    2001-01-01

    Two-photon threshold property of photoresist films have been studied by changing exposure energy. When photoresist film is irradiated by Ti∶Sapphire laser with wavelength 770 nm, pulse width 130 fs, repetition rate 82 MHz, the damage and recording thresholds of the material are 9.15×105 J/cm2 and below 5.57×105 J/cm2, respectively. The principle experiments of two-photon optical memory are demonstrated in photoresist film. The patterns of optical bit data storage are realized at different input power density. The corresponding 3-D tomographies of these recorded spots are scanned under near-field optical microscope.

  8. Two-photon photoemission from metals induced by picosecond laser pulses

    Science.gov (United States)

    Bechtel, J. H.; Smith, W. L.; Bloembergen, N.

    1977-01-01

    We have measured the two-photon photoemission current density from tungsten, tantalum, and molybdenum when irradiated by 532-nm wavelength radiation. This wavelength was produced by the second-harmonic radiation of single picosecond laser pulses from a mode-locked neodymium-doped yttrium-aluminum-garnet laser. The results are interpreted in terms of both a simple temperature-independent two-photon photoemission effect and a generalization of the Fowler-DuBridge theory of photoemission. The laser polarization dependence of the emitted current is also reported.

  9. Two-photon quantum walks in an elliptical direct-write waveguide array

    CERN Document Server

    Owens, J O; Biggerstaff, D N; Goggin, M E; Fedrizzi, A; Linjordet, T; Ams, M; Marshall, G D; Twamley, J; Withford, M J; White, A G

    2011-01-01

    Integrated optics provides an ideal test bed for the emulation of quantum systems via continuous-time quantum walks. Here we study the evolution of two-photon states in an elliptic array of waveguides. We characterise the photonic chip via coherent-light tomography and use the results to predict distinct differences between temporally indistinguishable and distinguishable two-photon inputs which we then compare with experimental observations. Our work highlights the feasibility for emulation of coherent quantum phenomena in three-dimensional waveguide structures.

  10. Dynamics of Two-Photon Lasers with Λ Atomic Level Configuration

    Institute of Scientific and Technical Information of China (English)

    YANG Peng; QIAN Feng; HUANG Hong-Bin; XIE Xia; ZHANG Ya-Jun

    2006-01-01

    We derive the dimensionless dynamic equations of two-photon lasers with A atomic level configuration by using the quantum Langevin equation method with the considerations of atomic coherence and injected classical fields.Then we analyze the stability and the chaotic dynamics of the two-photon laser by calculating the bifurcation diagram and the maximum Lyapunov exponent (MLE). Our results show that the Lorenz strange attractors and one-focus strange attractors can exist in this system, and the chaos can be induced or inhibited by the injected classical fields via Hopfbifurcations or crises, while the atomic coherence induces chaos via crises, and inhibit chaos via Hopf bifurcation or crises.

  11. Two-photon exchange correction to $2S$-$2P$ splitting in muonic helium

    CERN Document Server

    Carlson, Carl E; Vanderhaeghen, Marc

    2016-01-01

    We calculate the two-photon exchange correction to the Lamb shift in muonic helium atoms within the dispersion relations framework. Part of the effort entailed making analytic fits to the electron-$^3$He quasielastic scattering data set, for purposes of doing the dispersion integrals. Our result is that the energy of the 2$S$ state is shifted downwards by two-photon exchange effects by 15.14(49) meV, in good accord with the result obtained from a potential model and effective field theory calculation.

  12. Nonsequential Two-Photon Double Ionization of Atoms: Identifying the Mechanism

    CERN Document Server

    F\\orre, Morten; Nepstad, Raymond

    2010-01-01

    We develop an approximate model for the process of direct (nonsequential) two-photon double ionization of atoms. Employing the model, we calculate (generalized) total cross sections as well as energy-resolved differential cross sections of helium for photon energies ranging from 39 to 54 eV. A comparison with results of \\textit{ab initio} calculations reveals that the agreement is at a quantitative level. We thus demonstrate that this complex ionization process is fully described by the simple model, providing insight into the underlying physical mechanism. Finally, we use the model to calculate generalized cross sections for the two-photon double ionization of neon in the nonsequential regime.

  13. Near IR two photon absorption of cyanines dyes: application to optical power limiting at telecommunication wavelengths

    Science.gov (United States)

    Bouit, Pierre-Antoine; Wetzel, Guillaume; Feneyrou, Patrick; Bretonnière, Yann; Kamada, Kenji; Maury, Olivier; Andraud, Chantal

    2008-02-01

    The design and synthesis of symmetrical and unsymmetrical heptamethine cyanines is reported. These chromophores present significant two-photon cross section in the 1400-1600 nm spectral range. In addition, they display optical power limiting (OPL) properties. OPL curves were interpreted on the basis of two-photon absorption (2PA) followed by excited state absorption (ESA). Finally, these molecules present several relevant properties (nonlinear absorption properties, two-step gram scale synthesis, high solubility, good thermal stability), which could lead to numerous practical applications in material science (solid state optical limiting, signal processing) or in biology (imaging).

  14. New insight in boron chemistry: Application in two-photon absorption

    Science.gov (United States)

    Bolze, F.; Hayek, A.; Sun, X. H.; Baldeck, P. L.; Bourgogne, C.; Nicoud, J.-F.

    2011-07-01

    Two groups of one-dimensional (1D) boron containing two-photon absorbing fluorophores have been prepared and characterized. One group includes boron atoms incorporated in the conjugated or pseudo conjugated central core and the other contain a boron cluster as an acceptor group at one end of the fluorophores. Two boron containing central cores (with two boron atoms) have been explored: the cyclodiborazane and the pyrazabole moieties. The chosen boron cluster, p-carborane, contains 10 boron atoms. All the prepared fluorophores present high two-photon absorption cross-sections. Some water-soluble as well as lipophylic dyes have been prepared and used in bio-imaging.

  15. Two-photon-excited fluorescence spectroscopy of atomic fluorine at 170 nm

    Science.gov (United States)

    Herring, G. C.; Dyer, Mark J.; Jusinski, Leonard E.; Bischel, William K.

    1988-01-01

    Two-photon-excited fluorescence spectroscopy of atomic fluorine is reported. A doubled dye laser at 286-nm is Raman shifted in H2 to 170 nm (sixth anti-Stokes order) to excite ground-state 2P(0)J fluorine atoms to the 2D(0)J level. The fluorine atoms are detected by one of two methods: observing the fluorescence decay to the 2PJ level or observing F(+) production through the absorption of an additional photon by the excited atoms. Relative two-photon absorption cross sections to and the radiative lifetimes of the 2D(0)J states are measured.

  16. Synthesis,structure and nonlinear optical properties of two novel two-photon absorption chromophores

    Institute of Scientific and Technical Information of China (English)

    2009-01-01

    Two triphenylamine-based derivatives that can be used as two-photon absorption chromophore,tris{4-[4-(3-trifluoromethyl-3-oxopanoyl)]phenyl}amine (1) and tris{4-[4-(3-phenyl-3-oxopanoyl)] phenyl} amine (2) were successfully synthesized and fully characterized by elemental analysis,IR,1H NMR and MS. The single crystal X-ray diffraction analysis showed that the molecules possess D-(π-A)3 structures. One-and two-photon absorption and fluorescence in various solvents were experimentally investigated. A data recording experiment proved the potential application of these chromophores.

  17. Fluorenyl porphyrins for combined two-photon excited fluorescence and photosensitization

    Science.gov (United States)

    Mongin, Olivier; Hugues, Vincent; Blanchard-Desce, Mireille; Merhi, Areej; Drouet, Samuel; Yao, Dandan; Paul-Roth, Christine

    2015-04-01

    The two-photon absorption (2PA), the luminescence and the photosensitization properties of porphyrin-cored fluorenyl dendrimers and meso-substituted fluorenylporphyrin monomer, dimer and trimer are described. In comparison with model tetraphenylporphyrin, these compounds combine enhanced (non-resonant) 2PA cross-sections in the near infrared and enhanced fluorescence quantum yields, together with maintained singlet oxygen generation quantum yields. 'Semi-disconnection' between fluorenyl groups and porphyrins (i.e. direct meso substitution) proved to be more efficient than non-conjugated systems (based on efficient FRET between fluorenyl antennae and porphyrins). These results are of interest for combined two-photon imaging and photodynamic therapy.

  18. Two-Photon Absorption-Induced Emission Properties of Dye HMASPS Doped Polymer

    Institute of Scientific and Technical Information of China (English)

    王东; 周广勇; 任燕; 杨胜军; 许心光; 邵宗书; 蒋民华

    2002-01-01

    The 0.01M two-photon absorption dye trans-4-[p-(N-hydroxyethyl-N-methylamino)styryl]-N-methyl-pyridinium p-toluene sulfonate (HMASPS) doped polymer has been prepared. When pumped by the picosecond pulse from the pulsed mode-locked Nd: YAG laser, the polymer emits more intense upconverted fluorescence and superradiance compared to the solution sample of the dye. The two-photon pumped lasing with oscillating pulses has also been obtained. Compared to the dye in its solution state, the emission spectra of the polymer are all blueshifted.The polymer has a long upconverted fluorescent lifetime of about 4.041 ± 0.04 ns.

  19. Free electron laser induced two-photon photoconductivity in Hg1-xCdxTe

    Institute of Scientific and Technical Information of China (English)

    2001-01-01

    The Beijing free electron laser (BFEL) has been employed for the first time to study the nonlinear photoconductivity characteristics of the typical infrared photoelectronic material Hg1-xCdxTe. Taking advantage of the high photon flux density of BFEL, we have investigated the photoconductivity characteristics in Hg1-xCdxTe induced by two-photon absorption by means of the photoconductivity technique, observed the photoconductivity signals saturation, and studied the two-photon photoconductivity characteristics on different bias voltages across the sample.

  20. Simultaneous two-photon imaging and photo-stimulation with structured light illumination.

    Science.gov (United States)

    Dal Maschio, Marco; Difato, Francesco; Beltramo, Riccardo; Blau, Axel; Benfenati, Fabio; Fellin, Tommaso

    2010-08-30

    Holographic microscopy is increasingly recognized as a promising tool for the study of the central nervous system. Here we present a "holographic module", a simple optical path that can be combined with commercial scanheads for simultaneous imaging and uncaging with structured two-photon light. The present microscope is coupled to two independently tunable lasers and has two principal configurations: holographic imaging combined with galvo-steered uncaging and holographic uncaging combined with conventional scanning imaging. We applied this flexible system for simultaneous two-photon imaging and photostimulation of neuronal cells with complex light patterns, opening new perspectives for the study of brain function in situ and in vivo.

  1. Search for a Higgs Boson Decaying into Two Photons at LEP

    CERN Document Server

    Achard, P; Aguilar-Benítez, M; Alcaraz, J; Alemanni, G; Allaby, James V; Aloisio, A; Alviggi, M G; Anderhub, H; Andreev, V P; Anselmo, F; Arefev, A; Azemoon, T; Aziz, T; Bagnaia, P; Bajo, A; Baksay, G; Baksay, L; Baldew, S V; Banerjee, S; Banerjee, Sw; Barczyk, A; Barillère, R; Bartalini, P; Basile, M; Batalova, N; Battiston, R; Bay, A; Becattini, F; Becker, U; Behner, F; Bellucci, L; Berbeco, R; Berdugo, J; Berges, P; Bertucci, B; Betev, B L; Biasini, M; Biglietti, M; Biland, A; Blaising, J J; Blyth, S C; Bobbink, Gerjan J; Böhm, A; Boldizsar, L; Borgia, B; Bottai, S; Bourilkov, D; Bourquin, Maurice; Braccini, S; Branson, J G; Brochu, F; Burger, J D; Burger, W J; Cai, X D; Capell, M; Cara Romeo, G; Carlino, G; Cartacci, A M; Casaus, J; Cavallari, F; Cavallo, N; Cecchi, C; Cerrada, M; Chamizo-Llatas, M; Chang, Y H; Chemarin, M; Chen, A; Chen, G; Chen, G M; Chen, H F; Chen, H S; Chiefari, G; Cifarelli, Luisa; Cindolo, F; Clare, I; Clare, R; Coignet, G; Colino, N; Costantini, S; de la Cruz, B; Cucciarelli, S; van Dalen, J A; De Asmundis, R; Déglon, P L; Debreczeni, J; Degré, A; Deiters, K; Della Volpe, D; Delmeire, E; Denes, P; De Notaristefani, F; De Salvo, A; Diemoz, M; Dierckxsens, M; Dionisi, C; Dittmar, Michael; Doria, A; Dova, M T; Duchesneau, D; Echenard, B; Eline, A; El-Mamouni, H; Engler, A; Eppling, F J; Ewers, A; Extermann, Pierre; Falagán, M A; Falciano, S; Favara, A; Fay, J; Fedin, O; Felcini, Marta; Ferguson, T; Fesefeldt, H S; Fiandrini, E; Field, J H; Filthaut, Frank; Fisher, P H; Fisher, W; Fisk, I; Forconi, G; Freudenreich, Klaus; Furetta, C; Galaktionov, Yu; Ganguli, S N; García-Abia, P; Gataullin, M; Gentile, S; Giagu, S; Gong, Z F; Grenier, G; Grimm, O; Grünewald, M W; Guida, M; van Gulik, R; Gupta, V K; Gurtu, A; Gutay, L J; Haas, D; Hakobyan, R S; Hatzifotiadou, D; Hebbeker, T; Hervé, A; Hirschfelder, J; Hofer, H; Hohlmann, M; Holzner, G; Hou, S R; Hu, Y; Jin, B N; Jones, L W; de Jong, P; Josa-Mutuberria, I; Käfer, D; Kaur, M; Kienzle-Focacci, M N; Kim, J K; Kirkby, Jasper; Kittel, E W; Klimentov, A; König, A C; Kopal, M; Koutsenko, V F; Kräber, M H; Krämer, R W; Krenz, W; Krüger, A; Kunin, A; Ladrón de Guevara, P; Laktineh, I; Landi, G; Lebeau, M; Lebedev, A; Lebrun, P; Lecomte, P; Lecoq, P; Le Coultre, P; Le Goff, J M; Leiste, R; Levtchenko, M; Levchenko, P M; Li, C; Likhoded, S A; Lin, C H; Lin, W T; Linde, Frank L; Lista, L; Liu, Z A; Lohmann, W; Longo, E; Lü, Y S; Lübelsmeyer, K; Luci, C; Luminari, L; Lustermann, W; Ma Wen Gan; Malgeri, L; Malinin, A; Maña, C; Mangeol, D J J; Mans, J; Martin, J P; Marzano, F; Mazumdar, K; McNeil, R R; Mele, S; Merola, L; Meschini, M; Metzger, W J; Mihul, A; Milcent, H; Mirabelli, G; Mnich, J; Mohanty, G B; Muanza, G S; Muijs, A J M; Musicar, B; Musy, M; Nagy, S; Natale, S; Napolitano, M; Nessi-Tedaldi, F; Newman, H; Niessen, T; Nisati, A; Nowak, H; Ofierzynski, R A; Organtini, G; Palomares, C; Pandoulas, D; Paolucci, P; Paramatti, R; Passaleva, G; Patricelli, S; Paul, T; Pauluzzi, M; Paus, C; Pauss, Felicitas; Pedace, M; Pensotti, S; Perret-Gallix, D; Petersen, B; Piccolo, D; Pierella, F; Pioppi, M; Piroué, P A; Pistolesi, E; Plyaskin, V; Pohl, M; Pozhidaev, V; Pothier, J; Prokofiev, D O; Prokofev, D; Quartieri, J; Rahal-Callot, G; Rahaman, M A; Raics, P; Raja, N; Ramelli, R; Rancoita, P G; Ranieri, R; Raspereza, A V; Razis, P A; Ren, D; Rescigno, M; Reucroft, S; Riemann, S; Riles, K; Roe, B P; Romero, L; Rosca, A; Rosier-Lees, S; Roth, S; Rosenbleck, C; Roux, B; Rubio, Juan Antonio; Ruggiero, G; Rykaczewski, H; Sakharov, A; Saremi, S; Sarkar, S; Salicio, J; Sánchez, E; Sanders, M P; Schäfer, C; Shchegelskii, V; Schmidt-Kärst, S; Schmitz, D; Schopper, Herwig Franz; Schotanus, D J; Schwering, G; Sciacca, C; Servoli, L; Shevchenko, S; Shivarov, N; Shoutko, V; Shumilov, E; Shvorob, A V; Siedenburg, T; Son, D; Spillantini, P; Steuer, M; Stickland, D P; Stoyanov, B; Strässner, A; Sudhakar, K; Sultanov, G G; Sun, L Z; Sushkov, S V; Suter, H; Swain, J D; Szillási, Z; Tang, X W; Tarjan, P; Tauscher, Ludwig; Taylor, L; Tellili, B; Teyssier, D; Timmermans, C; Ting, Samuel C C; Ting, S M; Tonwar, S C; Tóth, J; Tully, C; Tung, K L; Ulbricht, J; Valente, E; Van de Walle, R T; Veszpremi, V; Vesztergombi, G; Vetlitskii, I; Vicinanza, D; Viertel, Gert M; Villa, S; Vivargent, M; Vlachos, S; Vodopyanov, I; Vogel, H; Vogt, H; Vorobev, I; Vorobyov, A A; Wadhwa, M; Wallraff, W; Wang, X L; Wang, Z M; Weber, M; Wienemann, P; Wilkens, H; Wynhoff, S; Xia, L; Xu, Z Z; Yamamoto, J; Yang, B Z; Yang, C G; Yang, H J; Yang, M; Yeh, S C; Zalite, A; Zalite, Yu; Zhang, Z P; Zhao, J; Zhu, G Y; Zhu, R Y; Zhuang, H L; Zichichi, A; Zilizi, G; Zimmermann, B; Zöller, M

    2002-01-01

    A Higgs particle produced in association with a Z boson and decaying into two photons is searched for in the data collected by the L3 experiment at LEP. All possible decay modes of the Z boson are investigated. No signal is observed in 447.5 pb^-1 of data recorded at centre-of-mass energies up to 209 GeV. Limits on the branching fraction of the Higgs boson decay into two photons as a function of the Higgs mass are derived. A lower limit on the mass of a fermiophobic Higgs boson is set at 105.4 GeV at 95% confidence level.

  2. $B\\to \\rho$ transition form factors within the QCD light-cone sum rules and the $\\rho$-meson leading-twist distribution amplitude

    CERN Document Server

    Fu, Hai-Bing; Han, Hua-Yong; Ma, Yang

    2014-01-01

    The QCD light-cone sum rules (LCSR) provides an effective way for dealing with the heavy-to-light transition form factors (TFFs), whose non-perturbative dynamics are parameterized into the light-meson's light-cone distribution amplitudes (LCDAs) with various twist structures. By taking the chiral correlator as the starting point, we calculate the LCSRs for the $B\\to\\rho$ TFFs up to twist-4 accuracy. As for the TFFs at the large recoil region, we observe that the twist-2 transverse DA $\\phi_{2;\\rho}^\\bot$ provides the dominant contribution, while the contributions from the remaining twist-3 and twist-4 terms are $\\delta^2$-suppressed. Thus, our present improved LCSRs provides a good platform for testing the $\\phi_{2;\\rho}^\\bot$ behavior. For the purpose, we suggest a convenient WH-model for the $\\rho$-meson leading-twist wavefunction, in which the parameter $B_{2;\\rho}^\\bot\\sim a^\\bot_2$ dominantly controls its longitudinal distribution. Typically, its DA $\\phi_{2;\\rho}^\\bot$ is CZ-like as $B_{2;\\rho}^\\bot\\sim...

  3. Visualizing heterogeneity of photosynthetic properties of plant leaves with two-photon fluorescence lifetime imaging microscopy

    NARCIS (Netherlands)

    Iermak, Ievgeniia; Vink, Jochem; Bader, Arjen N.; Wientjes, Emilie; Amerongen, van Herbert

    2016-01-01

    Two-photon fluorescence lifetime imaging microscopy (FLIM) was used to analyse the distribution and properties of Photosystem I (PSI) and Photosystem II (PSII) in palisade and spongy chloroplasts of leaves from the C3 plant Arabidopsis thaliana and the C4 plant Miscanthus x giganteus. This was ac

  4. Enhancement of two-photon photoluminescence and SERS for low-coverage gold films

    DEFF Research Database (Denmark)

    Novikov, Sergey M.; Beermann, Jonas; Frydendahl, Christian

    2016-01-01

    Electromagnetic field enhancement (FE) effects occurring in thin gold films 3-12-nm are investigated with two-photon photoluminescence (TPL) and Raman scanning optical microscopies. The samples are characterized using scanning electron microscopy images and linear optical spectroscopy. TPL images...

  5. Imaging marine virus CroV and its host Cafeteria roenbergensis with two-photon microscopy

    Science.gov (United States)

    Cao, Bin; Chakraborty, Sayan; Sun, Wenqing; Aghvami, Seyedmohammadali; Fischer, Matthias G.; Qian, Wei; Xiao, Chuan; Li, Chunqiang

    2014-02-01

    We use two-photon microscopy to monitor the infection process of marine zooplankton, Cafeteria roenbergensis (C.roenbergensis), by Cafeteria roenbergensis virus (CroV), a giant DNA virus named after its host. Here, we image C.roenbergensis in culture by two-photon excited NADH autofluorescence at video-rate (30 frame/s), and the movement of C.roenbergensis is recorded in live videos. Moreover, CroV is stained with DNA dye SYBR gold and recorded simultaneously with this two-photon microscope. We observed the initial infection moment with this method. The result demonstrates the potential use of two-photon microscopy to investigate the fast dynamic interaction between C.roenbergensis with virus CroV. After catching this initial moment, we will freeze the sample in liquid nitrogen for cryo-electron microscopy (EM) study to resolve the virus-host interaction at molecular level. The long-term goal is to study similar fast moving pathogen-host interaction process which could lead to important medical applications.

  6. Gold Core Mesoporous Organosilica Shell Degradable Nanoparticles for Two-Photon Imaging and Gemcitabine Monophosphate Delivery

    KAUST Repository

    Rhamani, Saher

    2017-09-12

    The synthesis of gold core degradable mesoporous organosilica shell nanoparticles is described. The nanopaticles were very efficient for two-photon luminescence imaging of cancer cells and for in vitro gemcitabine monophosphate delivery, allowing promising theranostic applications in the nanomedicine field.

  7. Two-photon upconversion affected by intermolecule correlations near metallic nanostructures

    Science.gov (United States)

    Osaka, Yoshiki; Yokoshi, Nobuhiko; Ishihara, Hajime

    2016-04-01

    We investigate an efficient two-photon upconversion process in more than one molecule coupled to an optical antenna. In the previous paper [Y. Osaka et al., Phys. Rev. Lett. 112, 133601 (2014), 10.1103/PhysRevLett.112.133601], we considered the two-photon upconversion process in a single molecule within one-dimensional input-output theory and revealed that controlling the antenna-molecule coupling enables the efficient upconversion with radiative loss in the antenna suppressed. In this paper, aiming to propose a way to enhance the total probability of antenna-photon scattering, we extend the model to the case of multiple molecules. In general, the presence of more than one molecule decreases the upconversion probability because they equally share the energy of the two photons. However, it is shown that we can overcome the difficulty by controlling the intermolecule coupling. Our result implies that, without increasing the incident photon number (light power), we can enlarge the net probability of the two-photon upconversion.

  8. Higgs decay into two photons from a 3HDM with flavor symmetry

    Energy Technology Data Exchange (ETDEWEB)

    Aranda, Alfredo, E-mail: fefo@ucol.mx [Facultad de Ciencias, CUICBAS, Universidad de Colima, Colima (Mexico); Dual C-P Institute of High Energy Physics (Mexico); Bonilla, Cesar, E-mail: rasec.cmbd@gmail.com [Facultad de Ciencias Físico–Matemáticas, Benemérita Universidad Autónoma de Puebla (Mexico); Anda, Francisco de, E-mail: franciscojosedea@gmail.com [Departamento de Fisica, CUCEI, Universidad de Guadalajara (Mexico); Delgado, Antonio, E-mail: antonio.delgado@nd.edu [Department of Physics, University of Notre Dame, Notre Dame, IN 46556 (United States); Hernández-Sánchez, Jaime, E-mail: jaimeh@ece.buap.mx [Dual C-P Institute of High Energy Physics (Mexico); Facultad de Ciencias de la Electrónica, Benemérita Universidad Autónoma de Puebla, Apdo. Postal 542, 72570 Puebla, Puebla (Mexico)

    2013-08-09

    In this short Letter we show that the excess of events in the decay of Higgs to two photons reported by ATLAS and CMS can be easily accommodated in a flavor renormalizable three Higgs doublet model (3HDM). The model is consistent with all fermion masses, mixing angles, and flavor changing neutral current constraints.

  9. One-bit photon polarization in two-photon experiments. An information mechanics perspective

    Science.gov (United States)

    Kantor, Frederick W.

    1991-03-01

    Two-photon experiments of Aspect, Grangier, and Roger, directed toward testing Einstein, Podolsky, and Rosen's thought experiment, are seen in the context of Kantor's information mechanics as illustrating some consequences of the fact that the amount of information represented by the photon's polarization is one bit.

  10. Fabrication of 3D nano/microelectrodes via two-photon-polymerization

    DEFF Research Database (Denmark)

    Abaddi, Mohammed Al-; Sasso, Luigi; Dimaki, Maria

    2012-01-01

    The integration of two-photon polymerization technology with standard microfabrication techniques is imperative for the use of this tool in micro- and nanotechnology and especially for the future commercialization of the technology. In this work, we report a novel method for the fabrication of 3D...

  11. Solvent effects on optical properties of a newly synthesized two-photon polymerization initiator: BPYPA

    Institute of Scientific and Technical Information of China (English)

    Guo Ya-Hui; Sun Yuan-Hong; Tao Li-Min; Zhao Ke; Wang Chuan-Kui

    2005-01-01

    Time-dependent hybrid density functional theory in combination with polarized continuum model is applied to study the solvent effects on the geometrical and electronic structures as well as one- and two-photon absorption processes,of a newly synthesized asymmetrical charge-transfer organic molecule bis-(4-bromo-phenyl)-[4-(2-pyridin-4-yl-vinyl)phenyl]-amine (BPYPA). There exist two charge-transfer states for the compound in visible region. The two-photon absorption cross section calculated by a three-state model and solvatochromic shift of the charge-transfer states are found to be solvent-dependent, where a nonmonotonic behaviour with respect to the polarity of the solvents is observed. The numerical results show that the organic molecule exhibits a rather large two-photon absorption cross section as compared with the compound 4-trans-[p-(N, N-Di-n-butylamino)-p-stilbenyl vinyl] pyridine (DBASVP) reported previously, and is predicted to be a good two-photon polymerization initiator. The hydrogen-bond effect is analysed. The computational results are in good agreement with the measurements.

  12. Decay and coherence of two-photon excited yellow orthoexcitons in Cu2O

    NARCIS (Netherlands)

    Karpinska, Katarzyna; Mostovoy, M; van der Vegte, MA; Revcolevschi, A; van Loosdrecht, PHM

    2005-01-01

    Photoluminescence excitation spectroscopy has revealed a highly efficient two-photon excitation method to produce a cold, uniformly distributed high density excitonic gas in bulk cuprous oxide. A study of the time evolution of the density, temperature, and chemical potential of the exciton gas shows

  13. Polarization-resolved two-photon luminescence microscopy of V-groove arrays

    DEFF Research Database (Denmark)

    Beermann, J.; Novikov, S. M.; Holmgaard, T.

    2012-01-01

    Using two-photon luminescence (TPL) microscopy and local reflection spectroscopy we investigate electromagnetic field enhancement effects from a mu m-sized composition of 450-nm-deep V-grooves milled by focused ion beam in a thick gold film and assembled to feature, within the same structure...

  14. Mitigating thermal mechanical damage potential during two-photon dermal imaging.

    Science.gov (United States)

    Masters, Barry R; So, Peter T C; Buehler, Christof; Barry, Nicholas; Sutin, Jason D; Mantulin, William W; Gratton, Enrico

    2004-01-01

    Two-photon excitation fluorescence microscopy allows in vivo high-resolution imaging of human skin structure and biochemistry with a penetration depth over 100 microm. The major damage mechanism during two-photon skin imaging is associated with the formation of cavitation at the epidermal-dermal junction, which results in thermal mechanical damage of the tissue. In this report, we verify that this damage mechanism is of thermal origin and is associated with one-photon absorption of infrared excitation light by melanin granules present in the epidermal-dermal junction. The thermal mechanical damage threshold for selected Caucasian skin specimens from a skin bank as a function of laser pulse energy and repetition rate has been determined. The experimentally established thermal mechanical damage threshold is consistent with a simple heat diffusion model for skin under femtosecond pulse laser illumination. Minimizing thermal mechanical damage is vital for the potential use of two-photon imaging in noninvasive optical biopsy of human skin in vivo. We describe a technique to mitigate specimen thermal mechanical damage based on the use of a laser pulse picker that reduces the laser repetition rate by selecting a fraction of pulses from a laser pulse train. Since the laser pulse picker decreases laser average power while maintaining laser pulse peak power, thermal mechanical damage can be minimized while two-photon fluorescence excitation efficiency is maximized.

  15. Selective two-photon collagen crosslinking in situ measured by Brillouin microscopy (Conference Presentation)

    Science.gov (United States)

    Kwok, Sheldon J. J.; Kuznetsov, Ivan A.; Kim, Moonseok; Choi, Myunghwan; Scarcelli, Giuliano; Yun, Seok-Hyun

    2017-02-01

    Two-photon polymerization and crosslinking are commonly used methods for microfabrication of three-dimensional structures with applications spanning from photonic microdevices, drug delivery systems, to cellular scaffolds. However, the use of two-photon processes for precise, internal modification of biological tissues has not yet been reported. One of the major challenges has been a lack of appropriate tools to monitor and characterize crosslinked regions nondestructively. Here, we demonstrate spatially selective two-photon collagen crosslinking (2P-CXL) in intact tissue for the first time. Using riboflavin photosensitizer and femtosecond laser irradiation, we crosslinked a small volume of tissue within animal corneas. Collagen fiber orientations and photobleaching were characterized by second harmonic generation and two-photon fluorescence imaging, respectively. Using confocal Brillouin microscopy, we measured local changes in longitudinal mechanical moduli and visualized the cross-linked pattern without perturbing surrounding non-irradiated regions. 2P-CXL-induced tissue stiffening was comparable to that achieved with conventional one-photon CXL. Our results demonstrate the ability to selectively stiffen biological tissue in situ at high spatial resolution, with broad implications in ophthalmology, laser surgery, and tissue engineering.

  16. Dependence of the two-photon photoluminescence yield of gold nanostructures on the laser pulse duration

    DEFF Research Database (Denmark)

    Biagioni, P.; Celebrano, M.; Savoini, M.

    2009-01-01

    Two-photon photoluminescence (TPPL) from gold nanostructures is becoming one of the most relevant tools for plasmon-assisted biological imaging and photothermal therapy as well as for the investigation of plasmonic devices. Here we study the yield of TPPL as a function of the temporal width δ of ...

  17. Two-photon imaging and spectroscopy of fresh human colon biopsies

    Science.gov (United States)

    Cicchi, R.; Sturiale, A.; Nesi, G.; Tonelli, F.; Pavone, F. S.

    2012-03-01

    Two-photon fluorescence (TPEF) microscopy is a powerful tool to image human tissues up to 200 microns depth without any exogenously added probe. TPEF can take advantage of the autofluorescence of molecules intrinsically contained in a biological tissue, as such NADH, elastin, collagen, and flavins. Two-photon microscopy has been already successfully used to image several types of tissues, including skin, muscles, tendons, bladder. Nevertheless, its usefulness in imaging colon tissue has not been deeply investigated yet. In this work we have used combined two-photon excited fluorescence (TPEF), second harmonic generation microscopy (SHG), fluorescence lifetime imaging microscopy (FLIM), and multispectral two-photon emission detection (MTPE) to investigate different kinds of human ex-vivo fresh biopsies of colon. Morphological and spectroscopic analyses allowed to characterize both healthy mucosa, polyp, and colon samples in a good agreement with common routine histology. Even if further analysis, as well as a more significant statistics on a large number of samples would be helpful to discriminate between low, mild, and high grade cancer, our method is a promising tool to be used as diagnostic confirmation of histological results, as well as a diagnostic tool in a multiphoton endoscope or colonoscope to be used in in-vivo imaging applications.

  18. Observation of high-$p_{T}$ jets in two-photon interactions

    CERN Document Server

    Bartel, Wulfrin; Dittmann, P; Eichler, R; Felst, R; Haidt, Dieter; Krehbiel, H; Meier, K; Naroska, Beate; O'Neill, L H; Steffen, P; Wenninger, Horst; Zhang, Y; Elsen, E E; Helm, M; Petersen, A; Warming, P; Weber, G; Bethke, Siegfried; Drumm, H; Heintze, J; Heinzelmann, G; Hellenbrand, K H; Heuer, R D; Von Krogh, J; Lennert, P; Kawabata, S; Matsumura, H; Nozaki, T; Olsson, J; Rieseberg, H; Wagner, A; Bell, A; Foster, F; Hughes, G; Wriedt, H; Allison, J; Ball, A H; Bamford, G; Barlow, R; Bowdery, C K; Duerdoth, I P; Hassard, J F; King, B T; Loebinger, F K; MacBeth, A A; McCann, H; Mills, H E; Murphy, P G; Stephens, K; Clarke, D; Goddard, M C; Marshall, R; Pearce, G F; Kobayashi, T; Komamiya, S; Koshiba, M; Minowa, M; Nosaki, M; Orito, S; Sato, A; Suda, T; Takeda, H; Totsuka, Y; Watanabe, Y; Yamada, S; Yanagisawa, C

    1981-01-01

    Events with a characteristic two-jet topology have been observed in two-photon interactions. The production cross section is found to be higher than the point-like gamma gamma -qq cross section, which is approached only at transverse momenta larger than 3 GeV/c. (11 refs).

  19. Measurement Induced Enhancement of Squeezing in Nondegenerate Two-Photon Jaynes-Cummings Model

    Institute of Scientific and Technical Information of China (English)

    YE Sai-Yun

    2006-01-01

    Squeezing properties in the nondegenerate two-photon Jaynes-Cummings model are investigated. The effects of direct selective atomic measurement and the application of the classical field followed by atomic measurement are analyzed. Different values of the parameters of the classical field are taken into account. It is found that the field squeezing can be enhanced by measurement.

  20. Two-photon excited highly polarized and directional upconversion emission from slab organic crystals

    NARCIS (Netherlands)

    Fang, Hong-Hua; Chen, Qi-Dai; Yang, Jie; Xia, Hong; Ma, Yu-Guang; Wang, Hai-Yu; Sun, Hong-Bo; Fang, Honghua

    2010-01-01

    Effective upconversion emission from an organic crystal of cyano-substituted oligo (p-phenylenevinylene) (CNDPASDB) based on two-photon absorption is presented. Frequency upconverted cavityless lasing, or amplified spontaneous emission, from the crystal pumped by a femtosecond laser of 800 nm was ob

  1. Carbon quantum dot-NO photoreleaser nanohybrids for two-photon phototherapy of hypoxic tumors.

    Science.gov (United States)

    Fowley, Colin; McHale, Anthony P; McCaughan, Bridgeen; Fraix, Aurore; Sortino, Salvatore; Callan, John F

    2015-01-04

    We report a conjugate between carbon quantum dots and a NO photoreleaser able to photogenerate the anticancer NO radical via an energy transfer mechanism. This nanohybrid proved toxic to cancer cells in vitro and significantly reduced tumor volume in mice bearing human xenograft BxPC-3 pancreatic tumors upon two-photon excitation with the highly biocompatible 800 nm light.

  2. Probing Electron-Phonon Interaction through Two-Photon Interference in Resonantly Driven Semiconductor Quantum Dots

    DEFF Research Database (Denmark)

    Reigue, Antoine; Iles-Smith, Jake; Lux, Fabian

    2017-01-01

    We investigate the temperature dependence of photon coherence properties through two-photon interference (TPI) measurements from a single quantum dot (QD) under resonant excitation. We show that the loss of indistinguishability is related only to the electron-phonon coupling and is not affected...

  3. Sub-diffraction positioning of a two-photon excited and optically trapped quantum dot

    DEFF Research Database (Denmark)

    Jauffred, L.; Kyrsting, A.; Christensen, Eva Arnspang;

    2014-01-01

    Colloidal quantum dots are luminescent long-lived probes that can be two-photon excited and manipulated by a single laser beam. Therefore, quantum dots can be used for simultaneous single molecule visualization and force manipulation using an infra-red laser. Here, we show that even a single opti...

  4. [Intensity loss of two-photon excitation fluorescence microscopy images of mouse oocyte chromosomes].

    Science.gov (United States)

    Zhao, Feng-Ying; Wu, Hong-Xin; Chen, Die-Yan; Ma, Wan-Yun

    2014-07-01

    As an optical microscope with high resolution, two-photon excitation (TPE) fluorescence microscope is widely used in noninvasive 3D optical imaging of biological samples. Compared with confocal laser scanning microscope, TPE fluorescence microscope provides a deeper detecting depth. In spite of that, the image quality of sample always declines as the detecting depth increases when a noninvasive 3D optical imaging of thicker samples is performed. Mouse oocytes with a large diameter, which play an important role in clinical and biological fields, have obvious absorption and scattering effects. In the present paper, we performed compensation for two-photon fluorescence images of mouse oocyte chromosomes. Using volume as a parameter, the attenuation degree of these chromosomes was also studied. The result of our data suggested that there exists a severe axial intensity loss in two-photon microscopic images of mouse oocytes due to the absorption and scattering effects. It is necessary to make compensation for these images of mouse oocyte chromosomes obtained from two-photon microscopic system. It will be specially needed in studying the quantitative three-dimensional information of mouse oocytes.

  5. A two-photon activatable amino acid linker for the induction of fluorescence.

    Science.gov (United States)

    Friedrich, Felix; Klehs, Kathrin; Fichte, Manuela A H; Junek, Stephan; Heilemann, Mike; Heckel, Alexander

    2015-10-28

    A new one- and two-photon activatable fluorophore based on ATTO565 was developed using a photolabile linker that simultaneously acts as a quencher. It is especially interesting for protein and peptide applications because it can be incorporated by standard peptide chemistry. The application of the new fluorogenic construct in super-resolution microscopy of antibody conjugates is shown.

  6. Two-photon up-conversion affected by inter-molecule correlations near metallic nanostructure

    CERN Document Server

    Osaka, Yoshiki; Ishihara, Hajime

    2016-01-01

    We investigate an efficient two-photon up-conversion process in more than one molecule coupled to an optical antenna. In the previous work [Y. Osaka et al., PRL 112, 133601 (2014)], we considered the two-photon up-conversion process in a single molecule within one-dimensional input-output theory, and revealed that controlling the antenna-molecule coupling enables the efficient up-conversion with radiative loss in the antenna suppressed. In this work, aiming to propose a way to enhance the total probability of antenna-photon scattering, we extend the model to the case of multiple molecules. In general, the presence of more than one molecule decreases the up-conversion probability because they equally share the energy of the two photons. However, it is shown that we can overcome the difficulty by controlling the inter-molecule coupling. Our result implies that, without increasing the incident photon number (light power), we can enlarge the net probability of the two-photon up-conversion.

  7. Atomic Dipole Squeezing in the Correlated Two-Mode Two-Photon Jaynes-Cummings Model

    Science.gov (United States)

    Dong, Zhengchao; Zhao, Yonglin

    1996-01-01

    In this paper, we study the atomic dipole squeezing in the correlated two-mode two-photon JC model with the field initially in the correlated two-mode SU(1,1) coherent state. The effects of detuning, field intensity and number difference between the two field modes are investigated through numerical calculation.

  8. Engineering two-photon high-dimensional states through quantum interference

    CSIR Research Space (South Africa)

    Zhang, YI

    2016-02-01

    Full Text Available the storage and processing potential of quantum information systems. We demonstrate the controlled engineering of two-photon high-dimensional states entangled in their orbital angular momentum through Hong-Ou-Mandel interference. We prepare a large range...

  9. New cubic perovskites for one- and two-photon water splitting using the computational materials repository

    DEFF Research Database (Denmark)

    Castelli, Ivano Eligio; Landis, David; Thygesen, Kristian Sommer

    2012-01-01

    screening of around 19 000 oxides, oxynitrides, oxysulfides, oxyfluorides, and oxyfluoronitrides in the cubic perovskite structure with PEC applications in mind. We address three main applications: light absorbers for one- and two-photon water splitting and high-stability transparent shields to protect...

  10. A study of Two Photon Decays of Charmonium Resonances Formed in Proton Anti-Proton Annihilations

    Energy Technology Data Exchange (ETDEWEB)

    Pedlar, Todd Kristofer [Northwestern Univ., Evanston, IL (United States)

    1999-06-01

    In this dissertation we describe the results of an investigation of the production of charmonium states (ηc, η'c, χ0 and χ2) in Fermilab experiment E835 via antiproton-proton annihilation and their detection via their decay into two photons.

  11. Phosphorescent probes for two-photon microscopy of oxygen (Conference Presentation)

    Science.gov (United States)

    Vinogradov, Sergei A.; Esipova, Tatiana V.

    2016-03-01

    The ability to quantify oxygen in vivo in 3D with high spatial and temporal resolution is much needed in many areas of biological research. Our laboratory has been developing the phosphorescence quenching technique for biological oximetry - an optical method that possesses intrinsic microscopic capability. In the past we have developed dendritically protected oxygen probes for quantitative imaging of oxygen in tissue. More recently we expanded our design on special two-photon enhanced phosphorescent probes. These molecules brought about first demonstrations of the two-photon phosphorescence lifetime microscopy (2PLM) of oxygen in vivo, providing new information for neouroscience and stem cell biology. However, current two-photon oxygen probes suffer from a number of limitations, such as sub-optimal brightness and high cost of synthesis, which dramatically reduce imaging performance and limit usability of the method. In this paper we discuss principles of 2PLM and address the interplay between the probe chemistry, photophysics and spatial and temporal imaging resolution. We then present a new approach to brightly phosphorescent chromophores with internally enhanced two-photon absorption cross-sections, which pave a way to a new generation of 2PLM probes.

  12. Background-Free Optical Sampling System Using Si Avalanche Photodiode as Two-Photon Absorber

    Institute of Scientific and Technical Information of China (English)

    Kenji; Taira; Ryo; Ohta; Yasuyuki; Ozeki; Yutaka; Fukuchi; Kazuhiro; Katoh; Kazuro; Kikuchi

    2003-01-01

    The introduction of a double-chopping scheme eliminates the background level in the optical sampling system, where a Si avalanche photodiode acts as a two-photon absorber. We successfully demonstrate background-free optical sampling of 40-GHz and 160-GHz pulse trains.

  13. Simultaneous two-photon activation of type-I photodynamic therapy agents.

    Science.gov (United States)

    Fisher, W G; Partridge, W P; Dees, C; Wachter, E A

    1997-08-01

    The excitation and emission properties of several psoralen derivatives are compared using conventional single-photon excitation and simultaneous two-photon excitation (TPE). Two-photon excitation is effected using the output of a mode-locked titanium: sapphire laser, the near infrared output of which is used to promote nonresonant TPE directly. Specifically, the excitation spectra and excited-state properties of 8-methoxypsoralen and 4'-aminomethyl-4,5,8-trimethylpsoralen are shown to be equivalent using both modes of excitation. Further, in vitro feasibility of two-photon photodynamic therapy (PDT) is demonstrated using Salmonella typhimurium. Two-photon excitation may be beneficial in the practice of PDT because it would allow replacement of visible or UV excitation light with highly penetrating, nondamaging near infrared light and could provide a means for improving localization of therapy. Comparison of possible laser excitation sources for PDT reveals the titanium: sapphire laser to be exceptionally well suited for nonlinear excitation of PDT agents in biological systems due to its extremely short pulse width and high repetition rate that together provide efficient PDT activation and greatly reduced potential for biological damage.

  14. Rapid Prototyping of Chemical Microsensors Based on Molecularly Imprinted Polymers Synthesized by Two-Photon Stereolithography.

    Science.gov (United States)

    Gomez, Laura Piedad Chia; Spangenberg, Arnaud; Ton, Xuan-Anh; Fuchs, Yannick; Bokeloh, Frank; Malval, Jean-Pierre; Tse Sum Bui, Bernadette; Thuau, Damien; Ayela, Cédric; Haupt, Karsten; Soppera, Olivier

    2016-07-01

    Two-photon stereolithography is used for rapid prototyping of submicrometre molecularly imprinted polymer-based 3D structures. The structures are evaluated as chemical sensing elements and their specific recognition properties for target molecules are confirmed. The 3D design capability is exploited and highlighted through the fabrication of an all-organic molecularly imprinted polymeric microelectromechanical sensor.

  15. Superradiant dye solution laser with two-photon picosecond optical pumping

    Energy Technology Data Exchange (ETDEWEB)

    Prokhorenko, V.I.; Tikhonov, E.A.; Shpak, M.T.

    1981-01-01

    A superradiant (superfluorescent) dye solution laser with two-photon picosecond pumping was constructed for the first time. A preliminary study was made of the principal characteristics of the output radiation of this laser which performed up-conversion of the frequency of the pump radiation. The physical mechanisms governing the operation of lasers of this type were analyzed.

  16. Two-photon photoemission from a copper cathode in an X -band photoinjector

    Science.gov (United States)

    Li, H.; Limborg-Deprey, C.; Adolphsen, C.; McCormick, D.; Dunning, M.; Jobe, K.; Raubenheimer, T.; Vrielink, A.; Vecchione, T.; Wang, F.; Weathersby, S.

    2016-02-01

    This paper presents two-photon photoemission from a copper cathode in an X -band photoinjector. We experimentally verified that the electron bunch charge from photoemission out of a copper cathode scales with laser intensity (I) square for 400 nm wavelength photons. We compare this two-photon photoemission process with the single photon process at 266 nm. Despite the high reflectivity (R ) of the copper surface for 400 nm photons (R =0.48 ) and higher thermal energy of photoelectrons (two-photon at 200 nm) compared to 266 nm photoelectrons, the quantum efficiency of the two-photon photoemission process (400 nm) exceeds the single-photon process (266 nm) when the incident laser intensity is above 300 GW /cm2 . At the same laser pulse energy (E ) and other experimental conditions, emitted charge scales inversely with the laser pulse duration. A thermal emittance of 2.7 mm-mrad per mm root mean square (rms) was measured on our cathode which exceeds by sixty percent larger compared to the theoretical predictions, but this discrepancy is similar to previous experimental thermal emittance on copper cathodes with 266 nm photons. The damage of the cathode surface of our first-generation X -band gun from both rf breakdowns and laser impacts mostly explains this result. Using a 400 nm laser can substantially simplify the photoinjector system, and make it an alternative solution for compact pulsed electron sources.

  17. Applying two-photon excitation fluorescence lifetime imaging microscopy to study photosynthesis in plant leaves

    NARCIS (Netherlands)

    Broess, K.; Borst, J.W.; Amerongen, van H.

    2009-01-01

    This study investigates to which extent two-photon excitation (TPE) fluorescence lifetime imaging microscopy can be applied to study picosecond fluorescence kinetics of individual chloroplasts in leaves. Using femtosecond 860 nm excitation pulses, fluorescence lifetimes can be measured in leaves of

  18. A scheme to realize time-bin entanglement between two photons that never interacted

    Institute of Scientific and Technical Information of China (English)

    2008-01-01

    We propose a scheme of entangling two photons from two separated sources.Our proposal which is inspired by the time-bin entanglement developed recently,provides a novel alternative for revealing contradiction between quantum nonlocality and local realism based on two independent single photon sources.

  19. Stepwise Two-Photon-Induced Fast Photoswitching via Electron Transfer in Higher Excited States of Photochromic Imidazole Dimer.

    Science.gov (United States)

    Kobayashi, Yoichi; Katayama, Tetsuro; Yamane, Takuya; Setoura, Kenji; Ito, Syoji; Miyasaka, Hiroshi; Abe, Jiro

    2016-05-11

    Stepwise two-photon excitations have been attracting much interest because of their much lower power thresholds compared with simultaneous two-photon processes and because some stepwise two-photon processes can be initiated by a weak incoherent excitation light source. Here we apply stepwise two-photon optical processes to the photochromic bridged imidazole dimer, whose solution instantly changes color upon UV irradiation and quickly reverts to the initial color thermally at room temperature. We synthesized a zinc tetraphenylporphyrin (ZnTPP)-substituted bridged imidazole dimer, and wide ranges of time-resolved spectroscopic studies revealed that a ZnTPP-linked bridged imidazole dimer shows efficient visible stepwise two-photon-induced photochromic reactions upon excitation at the porphyrin moiety. The fast photoswitching property combined with stepwise two-photon processes is important not only for the potential for novel photochromic materials that are sensitive to the incident light intensity but also for fundamental photochemistry using higher excited states.

  20. Sensing for intracellular thiols by water-insoluble two-photon fluorescent probe incorporating nanogel

    Energy Technology Data Exchange (ETDEWEB)

    Guo, Xudong; Zhang, Xin; Wang, Shuangqing; Li, Shayu [Beijing National Laboratory for Molecular Sciences, Key laboratory of Photochemistry, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190 (China); Hu, Rui, E-mail: hurui@iccas.ac.cn [Beijing National Laboratory for Molecular Sciences, Key laboratory of Photochemistry, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190 (China); Li, Yi, E-mail: yili@mail.ipc.ac.cn [Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190 (China); Yang, Guoqiang, E-mail: gqyang@iccas.ac.cn [Beijing National Laboratory for Molecular Sciences, Key laboratory of Photochemistry, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190 (China)

    2015-04-15

    Highlights: • A novel “turn-on” two-photon fluorescent probe based on a π-conjugated triarylboron luminogen was designed and synthesized. • Fast, selective and sensitive detection of biothiols in 100% aqueous solution by simply loaded on a nanogel. • Single-photon and two-photon fluorescent bioimaging of biothiols in NIH/3T3 fibroblasts. - Abstract: A novel “turn-on” two-photon fluorescent probe containing a π-conjugated triarylboron luminogen and a maleimide moiety DMDP-M based on the photo-induced electron transfer (PET) mechanism for biothiol detection was designed and synthesized. By simply loading the hydrophobic DMDP-M on a cross-linked Pluronic{sup ®} F127 nanogel (CL-F127), a probing system DMDP-M/CL-F127 was established, which shows quick response, high selectivity and sensitivity to cysteine (Cys), homocysteine (Hcy) and glutathione (GSH) in aqueous phase. The DMDP-M/CL-F127 system presented the fastest response to Cys with a rate constant of 0.56 min{sup −1}, and the detection limit to Cys was calculated to be as low as 0.18 μM. The DMDP-M/CL-F127 system has been successfully applied to the fluorescence imaging of biothiols in NIH/3T3 fibroblasts either with single-photon or two-photon excitation because of its high biocompatibility and cell-membrane permeability. The present work provides a general, simple and efficient strategy for the application of hydrophobic molecules to sensing biothiols in aqueous phase, and a novel sensing system for intracellular biothiols fitted for both single-photon and two-photon fluorescence imaging.

  1. Difluorenyl carbo-Benzenes: Synthesis, Electronic Structure, and Two-Photon Absorption Properties of Hydrocarbon Quadrupolar Chromophores.

    Science.gov (United States)

    Baglai, Iaroslav; de Anda-Villa, Manuel; Barba-Barba, Rodrigo M; Poidevin, Corentin; Ramos-Ortíz, Gabriel; Maraval, Valérie; Lepetit, Christine; Saffon-Merceron, Nathalie; Maldonado, José-Luis; Chauvin, Remi

    2015-09-28

    The synthesis, crystal and electronic structures, and one- and two-photon absorption properties of two quadrupolar fluorenyl-substituted tetraphenyl carbo-benzenes are described. These all-hydrocarbon chromophores, differing in the nature of the linkers between the fluorenyl substituents and the carbo-benzene core (C-C bonds for 3 a, C-C=C-C expanders for 3 b), exhibit quasi-superimposable one-photon absorption (1PA) spectra but different two-photon absorption (2PA) cross-sections σ2PA. Z-scan measurements (under NIR femtosecond excitation) indeed showed that the C≡C expansion results in an approximately twofold increase in the σ2PA value, from 336 to 656 GM (1 GM = 10(-50) cm(4) s molecule(-1) photon(-1)) at λ = 800 nm. The first excited states of Au and Ag symmetry accounting for 1PA and 2PA, respectively, were calculated at the TDDFT level of theory and used for sum-over-state estimations of σ2PA(λi), in which λi = 2 hc/Ei, h is Planck's constant, c is the speed of light, and Ei is the energy of the 2PA-allowed transition. The calculated σ2PA values of 227 GM at 687 nm for 3 a and 349 GM at 708 nm for 3 b are in agreement with the Z-scan results.

  2. The Correlated Two-Photon Transport in a One-Dimensional Waveguide Coupling to a Hybrid Atom-Optomechanical System

    Science.gov (United States)

    Liu, Jingyi; Zhang, Wenzhao; Li, Xun; Yan, Weibin; Zhou, Ling

    2016-10-01

    We investigate the two-photon transport properties inside one-dimensional waveguide side coupled to an atom-optomechanical system, aiming to control the two-photon transport by using the nonlinearity. By generalizing the scheme of Phys. Rev. A 90, 033832, we show that Kerr nonlinearity induced by the four-level atoms is remarkable and can make the photons antibunching, while the nonlinear interaction of optomechanical coupling participates in both the single photon and the two photon processes so that it can make the two photons exhibiting bunching and antibunching.

  3. Effects of torsional disorder and position isomerism on two-photon absorption properties of polar chromophore dimers

    Science.gov (United States)

    Jia, Hai-Hong; Zhao, Ke; Wu, Xiang-Lian

    2014-09-01

    Two-photon absorption properties of a push-pull molecule and its covalent dimers have been studied by density functional response theory in combination with polarizable continuum model. A set of constrained geometries with different torsional angles are optimized and used to calculate two-photon absorption spectra. It is found that the torsional disorder could possibly produce the experimental two-photon absorption additive behavior. We have also designed a series of covalent dimers and investigated the effects of position isomerism. Our results suggest that the cooperative two-photon absorption enhancement can be achieved when the subunits are substituted in closer proximity and have larger interchromophore angle.

  4. A spirobifluorene-based two-photon fluorescence probe for mercury ions and its applications in living cells

    Energy Technology Data Exchange (ETDEWEB)

    Xiao, Haibo, E-mail: xiaohb@shnu.edu.cn; Zhang, Yanzhen; Zhang, Wu; Li, Shaozhi; Tan, Jingjing; Han, Zhongying

    2017-05-01

    A novel spirobifluorene derivative SPF-TMS, which containing dithioacetal groups and triphenylamine units, was synthesized. The probing behaviors toward various metal ions were investigated via UV/Vis absorption spectra as well as one-photon fluorescence changes. The results indicated that SPF-TMS exhibits high sensitivity and selectivity for mercury ions. The detection limit was at least 8.6 × 10{sup −8}M, which is excellent comparing with other optical sensors for Hg{sup 2+}. When measured by two-photon excited fluorescence technique in THF at 800 nm, the two-photon cross-section of SPF-TMS is 272 GM. Especially, upon reaction with mercury species, SPF-TMS yielded another two-photon dye SPF-DA. Both SPF-TMS and SPF-DA emit strong two-photon induced fluorescence and can be applied in cell imaging by two-photon microscopy. - Highlights: • We report a spirobifluorene-based molecule as two-photon fluorescent probe with large two-photon cross-section. • The molecule has exclusive selectivity and sensitivity for mercury species. • The molecule has large two-photon emission changes before and after addition of Hg{sup 2+}. • Both the probe and the mercury ion-promoted reaction product can be applied in cell imaging by two-photon microscopy.

  5. Calculation of parity violating effects in the 6/sup 2/P/sub 1/2/-7/sup 2/P/sub 1/2/ forbidden M1 transition in thallium. [E1 amplitude, circular dichroism, parity violation, hyperfine structure

    Energy Technology Data Exchange (ETDEWEB)

    Neuffer, D.B.

    1977-05-01

    Calculations are presented of the E1 amplitude expected in forbidden M1 transitions of Tl and Cs if parity is violated in the neutral weak e-N interaction, as proposed in a number of gauge models, including that of Weinberg and Salam. Valence electron wave functions are generated as numerical solutions to the Dirac equation in a modified Tietz central potential. These wave functions are used to calculate allowed E1 transition rates, hfs splittings, and Stark E1 transition ampitudes. These results are compared with experiment and the agreement is generally good. The relativistic Tl 6/sup 2/P/sub 1/2/-7/sup 2/P/sub 1/2/ M1 transition amplitude M is also calculated, and corrections due to interconfiguration interaction, Breit interaction, and hfs mixing are included. The parity violating E1 amplitude E/sub PV/ is calculated and a value for the circular dichroism in the Weinberg model delta = -2.6 x 10/sup -3/ is obtained. Parity violating effects in other Tl transitions are discussed. Contributions to the M1 amplitude for the forbidden Cs 6/sup 2/S/sub 1/2/-7/sup 2/S/sub 1/2/ and 6/sup 2/S/sub 1/2/-8/sup 2/S/sub 1/2/ transitions and to the Cs 6/sup 2/S/sub 1/2/ g-factor anomaly from relativistic effects, Breit interaction, interconfiguration interaction, and hfs mixing are calculated, and it is found that this current theoretical description is not entirely adequate. The parity violating E1 amplitude E/sub PV/ for the 6S/sub 1/2/-7/sup 2/S/sub 1/2/ and 6S/sub 1/2/-8/sup 2/S/sub 1/2/ transitions is evaluated. With a measured value M/sub expt/ and the Weinberg value Q/sub W/ = -99, a circular dichroism delta = 1.64 x 10/sup -4/ for the 6/sup 2/S/sub 1/2/-7/sup 2/S/sub 1/2/ transition is found.

  6. One-colour resonant two-photon ionization spectrum of the 1-fluoronaphthalene dimer and ab initio calculation

    Institute of Scientific and Technical Information of China (English)

    Liu Ye-Chao; Zhang Shu-Dong; Zhang Ming-Xia; Sun Miao; Kong Xiang-He

    2009-01-01

    The one-colour resonant two-photon ionization (R2PI) spectrum of the 1-fluoronaphthalene (1FN) dimer has been studied in the wavelength range of 304 to 322 nm by using a supersonic molecular beam and time-of-flight mass spectrometry. Compared with the original band 000 (at 313.8 nm) of the S1 ← S0 transition of the 1FN monomer,a red-shifted band was observed in the 1FN dimer spectrum at about 315 nm with a relatively large linewidth,nearly 2 nm. Based on the consideration of inductive effect and ab initio calculations,this red-shifted band is assigned to the first electronic excited transition of the 1FN dimer. A possible geometric structure of the 1FN dimer is also obtained with calculations that the two 1FN molecules are combined through two hydrogen bonds which are formed between the hydrogen atom of a molecule and the fluorine atom of a neighbouring molecule. A time-dependent calculation was also carried out and the results are consistent with the experimental data.

  7. $\\chi_{c2}$ formation in two-photon collisions at LEP

    CERN Document Server

    Acciarri, M; Adriani, O; Aguilar-Benítez, M; Alcaraz, J; Alemanni, G; Allaby, James V; Aloisio, A; Alviggi, M G; Ambrosi, G; Anderhub, H; Andreev, V P; Angelescu, T; Anselmo, F; Arefev, A; Azemoon, T; Aziz, T; Bagnaia, P; Baksay, L; Balandras, A; Ball, R C; Banerjee, S; Banerjee, Sw; Banicz, K; Barczyk, A; Barillère, R; Barone, L; Bartalini, P; Basile, M; Battiston, R; Bay, A; Becattini, F; Becker, U; Behner, F; Berdugo, J; Berges, P; Bertucci, B; Betev, B L; Bhattacharya, S; Biasini, M; Biland, A; Blaising, J J; Blyth, S C; Bobbink, Gerjan J; Böck, R K; Böhm, A; Boldizsar, L; Borgia, B; Bourilkov, D; Bourquin, Maurice; Braccini, S; Branson, J G; Brigljevic, V; Brochu, F; Buffini, A; Buijs, A; Burger, J D; Burger, W J; Busenitz, J K; Button, A M; Cai, X D; Campanelli, M; Capell, M; Cara Romeo, G; Carlino, G; Cartacci, A M; Casaus, J; Castellini, G; Cavallari, F; Cavallo, N; Cecchi, C; Cerrada-Canales, M; Cesaroni, F; Chamizo-Llatas, M; Chang, Y H; Chaturvedi, U K; Chemarin, M; Chen, A; Chen, G; Chen, G M; Chen, H F; Chen, H S; Chéreau, X J; Chiefari, G; Cifarelli, Luisa; Cindolo, F; Civinini, C; Clare, I; Clare, R; Coignet, G; Colijn, A P; Colino, N; Costantini, S; Cotorobai, F; de la Cruz, B; Csilling, Akos; Dai, T S; van Dalen, J A; D'Alessandro, R; De Asmundis, R; Déglon, P L; Degré, A; Deiters, K; Della Volpe, D; Denes, P; De Notaristefani, F; De Salvo, A; Diemoz, M; Van Dierendonck, D N; Di Lodovico, F; Dionisi, C; Dittmar, Michael; Dominguez, A; Doria, A; Dova, M T; Duchesneau, D; Dufournaud, D; Duinker, P; Durán, I; El-Mamouni, H; Engler, A; Eppling, F J; Erné, F C; Extermann, Pierre; Fabre, M; Faccini, R; Falagán, M A; Falciano, S; Favara, A; Fay, J; Fedin, O; Felcini, Marta; Ferguson, T; Ferroni, F; Fesefeldt, H S; Fiandrini, E; Field, J H; Filthaut, Frank; Fisher, P H; Fisk, I; Forconi, G; Fredj, L; Freudenreich, Klaus; Furetta, C; Galaktionov, Yu; Ganguli, S N; García-Abia, P; Gataullin, M; Gau, S S; Gentile, S; Gheordanescu, N; Giagu, S; Goldfarb, S; Gong, Z F; Grünewald, M W; van Gulik, R; Gupta, V K; Gurtu, A; Gutay, L J; Haas, D; Hartmann, B; Hasan, A; Hatzifotiadou, D; Hebbeker, T; Hervé, A; Hidas, P; Hirschfelder, J; Hofer, H; Holzner, G; Hoorani, H; Hou, S R; Iashvili, I; Jin, B N; Jones, L W; de Jong, P; Josa-Mutuberria, I; Khan, R A; Kamrad, D; Kapustinsky, J S; Kaur, M; Kienzle-Focacci, M N; Kim, D; Kim, D H; Kim, J K; Kim, S C; Kinnison, W W; Kirkby, Jasper; Kiss, D; Kittel, E W; Klimentov, A; König, A C; Kopp, A; Korolko, I; Koutsenko, V F; Krämer, R W; Krenz, W; Kunin, A; Lacentre, P E; Ladrón de Guevara, P; Laktineh, I; Landi, G; Lapoint, C; Lassila-Perini, K M; Laurikainen, P; Lavorato, A; Lebeau, M; Lebedev, A; Lebrun, P; Lecomte, P; Lecoq, P; Le Coultre, P; Lee, H J; Le Goff, J M; Leiste, R; Leonardi, E; Levchenko, P M; Li Chuan; Lin, C H; Lin, W T; Linde, Frank L; Lista, L; Liu, Z A; Lohmann, W; Longo, E; Lü, Y S; Lübelsmeyer, K; Luci, C; Luckey, D; Luminari, L; Lustermann, W; Ma Wen Gan; Maity, M; Majumder, G; Malgeri, L; Malinin, A; Maña, C; Mangeol, D J J; Marchesini, P A; Marian, G; Martin, J P; Marzano, F; Massaro, G G G; Mazumdar, K; McNeil, R R; Mele, S; Merola, L; Meschini, M; Metzger, W J; Von der Mey, M; Migani, D; Mihul, A; Milcent, H; Mirabelli, G; Mnich, J; Molnár, P; Monteleoni, B; Moulik, T; Muanza, G S; Muheim, F; Muijs, A J M; Nahn, S; Napolitano, M; Nessi-Tedaldi, F; Newman, H; Niessen, T; Nippe, A; Nisati, A; Nowak, H; Oh, Yu D; Organtini, G; Ostonen, R; Palomares, C; Pandoulas, D; Paoletti, S; Paolucci, P; Park, H K; Park, I H; Pascale, G; Passaleva, G; Patricelli, S; Paul, T; Pauluzzi, M; Paus, C; Pauss, Felicitas; Peach, D; Pedace, M; Pei, Y J; Pensotti, S; Perret-Gallix, D; Petersen, B; Petrak, S; Piccolo, D; Pieri, M; Piroué, P A; Pistolesi, E; Plyaskin, V; Pohl, M; Pozhidaev, V; Postema, H; Pothier, J; Produit, N; Prokofev, D; Prokofiev, D O; Quartieri, J; Rahal-Callot, G; Raja, N; Rancoita, P G; Raven, G; Razis, P A; Ren, D; Rescigno, M; Reucroft, S; Van Rhee, T; Riemann, S; Riles, K; Robohm, A; Rodin, J; Roe, B P; Romero, L; Rosier-Lees, S; Roth, S; Rubio, Juan Antonio; Ruschmeier, D; Rykaczewski, H; Sakar, S; Salicio, J; Sánchez, E; Sanders, M P; Sarakinos, M E; Schäfer, C; Shchegelskii, V; Schmidt-Kärst, S; Schmitz, D; Scholz, N; Schopper, Herwig Franz; Schotanus, D J; Schwenke, J; Schwering, G; Sciacca, C; Sciarrino, D; Servoli, L; Shevchenko, S; Shivarov, N; Shoutko, V; Shukla, J; Shumilov, E; Shvorob, A V; Siedenburg, T; Son, D; Smith, B; Spillantini, P; Steuer, M; Stickland, D P; Stone, A; Stone, H; Stoyanov, B; Strässner, A; Sudhakar, K; Sultanov, G G; Sun, L Z; Suter, H; Swain, J D; Szillási, Z; Tang, X W; Tauscher, Ludwig; Taylor, L; Timmermans, C; Ting, Samuel C C; Ting, S M; Tonwar, S C; Tóth, J; Tully, C; Tung, K L; Uchida, Y; Ulbricht, J; Valente, E

    1999-01-01

    Two-photon formation of the charmonium resonance $\\chi_{{\\rm c}2}$ has been studied with the L3 detector at LEP. The $\\chi_{{\\rm c}2}$ is identified through its decay $\\chi_{{\\rm c}2} \\rightarrow \\gamma {\\rm J}$, with a subsequent decay ${\\rm J} \\rightarrow {\\mathrm{e^+ e^-}}$ or ${\\rm J} \\rightarrow {\\mathrm{\\mu^+ \\mu^-}}$. With an integrated luminosity of 140 pb$^{-1}$ at $\\sqrt{s} \\simeq$ 91~\\textrm{Ge\\kern -0.1em V} and 52 pb$^{-1}$ at $\\sqrt{s} \\simeq$ {Ge\\kern -0.1em V}, we measure the two-photon width of the $\\chi_{{\\rm c}2}$ to be \\begin{center} $\\Gamma_{\\gamma\\gamma}(\\chi_{{\\rm c}2})=1.02 \\pm 0.40 \\mbox{$\\;$(stat.)} \\pm 0.15 \\mbox{$\\;$(sys.)} \\pm 0.09(\\rm{BR.}) {\\mathrm{\\ ke\\kern -0.1em V}}$.

  8. Relativistic calculations of the non-resonant two-photon ionization of neutral atoms

    CERN Document Server

    Hofbrucker, Jiri; Fritzsche, Stephan

    2016-01-01

    The non-resonant two-photon one-electron ionization of neutral atoms is studied theoretically in the framework of relativistic second-order perturbation theory and independent particle approximation. In particular, the importance of relativistic and screening effects in the total two-photon ionization cross section is investigated. Detailed computations have been carried out for the K-shell ionization of neutral Ne, Ge, Xe, and U atoms. The relativistic effects significantly decrease the total cross section, for the case of U, for example, they reduce the total cross section by a factor of two. Moreover, we have found that the account for the screening effects of the remaining electrons leads to occurrence of an unexpected minimum in the total cross section at the total photon energies equal to the ionization threshold, for the case of Ne, for example, the cross section drops there by a factor of three.

  9. In Vivo Monitoring of Multiple Circulating Cell Populations Using Two-photon Flow Cytometry.

    Science.gov (United States)

    Tkaczyk, Eric R; Zhong, Cheng Frank; Ye, Jing Yong; Myc, Andrzej; Thomas, Thommey; Cao, Zhengyi; Duran-Struuck, Raimon; Luker, Kathryn E; Luker, Gary D; Norris, Theodore B; Baker, James R

    2008-02-15

    To detect and quantify multiple distinct populations of cells circulating simultaneously in the blood of living animals, we developed a novel optical system for two-channel, two-photon flow cytometry in vivo. We used this system to investigate the circulation dynamics in live animals of breast cancer cells with low (MCF-7) and high (MDA-MB-435) metastatic potential, showing for the first time that two different populations of circulating cells can be quantified simultaneously in the vasculature of a single live mouse. We also non-invasively monitored a population of labeled, circulating red blood cells for more than two weeks, demonstrating that this technique can also quantify the dynamics of abundant cells in the vascular system for prolonged periods of time. These data are the first in vivo application of multichannel flow cytometry utilizing two-photon excitation, which will greatly enhance our capability to study circulating cells in cancer and other disease processes.

  10. Evaluation of human sclera after femtosecond laser ablation using two photon and confocal microscopy

    Science.gov (United States)

    Sun, Hui; Kurtz, Ronald; Juhasz, Tibor

    2012-08-01

    Glaucoma is the second-leading cause of blindness worldwide and is often associated with elevated intraocular pressure (IOP). Partial thickness intrascleral channels can be created with a femtosecond laser operating at a wavelength of 1700 nm. Such channels have the potential to increase outflow facility and reduce elevated IOP. Analysis of the dimensions and location of these channels is important in understanding their effects. We describe the application of two-photon microscopy and confocal microscopy for noninvasive imaging of the femtosecond laser created partial-thickness scleral channels in human cadaver eyes. High-resolution images, hundreds of microns deep in the sclera, were obtained to allow determination of the shape and dimension of such channels. This demonstrates that concept of integrating femtosecond laser surgery, and two-photon and confocal imaging has the future potential for image-guided high-precision surgery in transparent and translucent tissue.

  11. Adaptive optics for in vivo two-photon calcium imaging of neuronal networks

    Science.gov (United States)

    Meimon, Serge; Conan, Jean-Marc; Mugnier, Laurent M.; Michau, Vincent; Cossart, Rosa; Malvache, Arnaud

    2014-03-01

    The landscape of biomedical research in neuroscience has changed dramatically in recent years as a result of spectacular progress in dynamic microscopy. However, the optical accessibility of deep brain structures or deeper regions of the surgically exposed hippocampus (a few 100 microns typically) remains limited, due to volumic aberrations created by the sample inhomogeneities. Adaptive optics can correct for these aberrations. Our goal is to realize a novel adaptive optics module dedicated to in vivo two-photon calcium imaging of the hippocampus. The key issue in adaptive optics is the ability to perform an accurate and reliable wavefront sensing. In two- photon microscopy indirect methods are required. Two families of approaches have been proposed so far, the modal sensorless technique and a method based on pupil segmentation. We present here a formal comparison of these approaches, in particular as a function of the amount of aberrations.

  12. Resonant two-photon annihilation of an electron-positron pair in a pulsed electromagnetic wave

    Science.gov (United States)

    Voroshilo, A. I.; Roshchupkin, S. P.; Nedoreshta, V. N.

    2016-09-01

    Two-photon annihilation of an electron-positron pair in the field of a plane low-intensity circularly polarized pulsed electromagnetic wave was studied. The conditions for resonance of the process which are related to an intermediate particle that falls within the mass shell are studied. In the resonant approximation the probability of the process was obtained. It is demonstrated that the resonant probability of two-photon annihilation of an electron-positron pair may be several orders of magnitude higher than the probability of this process in the absence of the external field. The obtained results may be experimentally verified by the laser facilities of the international megaprojects, for example, SLAC (National Accelerator Laboratory), FAIR (Facility for Antiproton and Ion Research), and XFEL (European X-Ray Free-Electron Laser).

  13. Two-Photon or Higher-Order Absorbing Optical Materials for Generation of Reactive Species

    Science.gov (United States)

    Cumpston, Brian (Inventor); Lipson, Matthew (Inventor); Marder, Seth R. (Inventor); Perry, Joseph W. (Inventor)

    2013-01-01

    Disclosed are highly efficient multiphoton absorbing compounds and methods of their use. The compounds generally include a bridge of pi-conjugated bonds connecting electron donating groups or electron accepting groups. The bridge may be substituted with a variety of substituents as well. Solubility, lipophilicity, absorption maxima and other characteristics of the compounds may be tailored by changing the electron donating groups or electron accepting groups, the substituents attached to or the length of the pi-conjugated bridge. Numerous photophysical and photochemical methods are enabled by converting these compounds to electronically excited states upon simultaneous absorption of at least two photons of radiation. The compounds have large two-photon or higher-order absorptivities such that upon absorption, one or more Lewis acidic species, Lewis basic species, radical species or ionic species are formed.

  14. Two-photon spectroscopy of trapped HD$^+$ ions in the Lamb-Dicke regime

    CERN Document Server

    Tran, Vu Quang; Douillet, Albane; Koelemeij, Jeroen C J; Hilico, Laurent

    2013-01-01

    We study the feasibility of nearly-degenerate two-photon rovibrational spectroscopy in ensembles of trapped, sympathetically cooled hydrogen molecular ions using a resonance-enhanced multiphoton dissociation (REMPD) scheme. Taking advantage of quasi-coincidences in the rovibrational spectrum, the excitation lasers are tuned close to an intermediate level to resonantly enhance two-photon absorption. Realistic simulations of the REMPD signal are obtained using a four-level model that takes into account saturation effects, ion trajectories, laser frequency noise and redistribution of population by blackbody radiation. We show that the use of counterpropagating laser beams enables optical excitation in an effective Lamb-Dicke regime. Sub-Doppler lines having widths in the 100 Hz range can be observed with good signal-to-noise ratio for an optimal choice of laser detunings. Our results indicate the feasibility of molecular spectroscopy at the $10^{-14}$ accuracy level for improved tests of molecular QED, a new det...

  15. Two-photon excited fluorescence microendoscopic imaging using a GRIN lens

    Science.gov (United States)

    Yan, Wei; Peng, Xiao; Lin, Danying; Wang, Qi; Gao, Jian; Zhou, Jie; Ye, Tong; Qu, Junle; Niu, Hanben

    2015-03-01

    With the rapid development of life sciences, there is an increasing demand for intravital fluorescence imaging of small animals. However, large dimensions and limited working distances of objective lenses in traditional fluorescence microscopes have limited the imaging applications mostly to superficial tissues. To overcome this disadvantage, researchers have developed the graded-index (GRIN) probes with small diameters for imaging internal organs of small animals in a minimally invasive fashion. Here, we present the development of a fluorescence endoscopic imaging system based on a GRIN lens using two-photon excitation. Experimental results showed that this system could perform dynamic fluorescence microendoscopic imaging and monitor the blood flow in anesthetized living mice using two-photon excitation.

  16. Slow reflection and two-photon generation of microcavity exciton-polaritons

    CERN Document Server

    Steger, Mark; Snoke, David W; Pfeiffer, Loren; West, Ken

    2014-01-01

    We resonantly inject polaritons into a microcavity and track them in time and space as they feel a force due to the cavity gradient. This is an example of "slow reflection," as the polaritons, which can be viewed as renormalized photons, slow down to zero velocity and then move back in the opposite direction. These measurements accurately measure the lifetime of the polaritons in our samples, which is 180 $\\pm$ 10 ps, corresponding to a cavity leakage time of 135 ps and a cavity $Q$ of 320,000. Such long-lived polaritons propagate millimeters in these wedge-shaped microcavities. Additionally, we generate polaritons by two-photon excitation directly into the polariton states, allowing the possibility of modulation of the two-photon absorption by a polariton condensate.

  17. Two-photon interference from independent cavity-coupled emitters on-a-chip

    CERN Document Server

    Kim, Je-Hyung; Leavitt, Richard P; Waks, Edo

    2016-01-01

    Interactions between solid-state quantum emitters and cavities are important for a broad range of applications in quantum communication, linear optical quantum computing, nonlinear photonics, and photonic quantum simulation. These applications often require combining many devices on a single chip with identical emission wavelengths in order to generate two-photon interference, the primary mechanism for achieving effective photon-photon interactions. Such integration remains extremely challenging due to inhomogeneous broadening and fabrication errors that randomize the resonant frequencies of both the emitters and cavities. In this letter we demonstrate two-photon interference from independent cavity-coupled emitters on the same chip, providing a potential solution to this long-standing problem. We overcome spectral mismatch between different cavities due to fabrication errors by depositing and locally evaporating a thin layer of condensed nitrogen. We integrate optical heaters to tune individual dots within e...

  18. Functional screening of intracardiac cell transplants using two-photon fluorescence microscopy.

    Science.gov (United States)

    Tao, Wen; Soonpaa, Mark H; Field, Loren J; Chen, Peng-Sheng; Firulli, Anthony B; Shou, Weinian; Rubart, Michael

    2012-08-01

    Although the adult mammalian myocardium exhibits a limited ability to undergo regenerative growth, its intrinsic renewal rate is insufficient to compensate for myocyte loss during cardiac disease. Transplantation of donor cardiomyocytes or cardiomyogenic stem cells is considered a promising strategy for reconstitution of cardiac mass, provided the engrafted cells functionally integrate with host myocardium and actively contribute to its contractile force. The authors previously developed a two-photon fluorescence microscopy-based assay that allows in situ screening of donor cell function after intracardiac delivery of the cells. This report reviews the techniques of two-photon fluorescence microscopy and summarizes its application for quantifying the extent to which a variety of donor cell types stably and functionally couple with the recipient myocardium.

  19. Diagnostics of MCF plasmas using Lyman-{alpha} fluorescence excited by one or two photons

    Energy Technology Data Exchange (ETDEWEB)

    Voslamber, D

    1998-11-01

    Laser-induced Lyman-{alpha} fluorescence of the hydrogen isotopes is investigated with regard to diagnostic applications in magnetically confined fusion plasmas. A formal analysis is presented for two excitation schemes: one-photon and Doppler-free two-photon excitation. The analysis includes estimates of the expected experimental errors arising from the photon noise and from the sensitivity of the observed fluorescence signals to variations of the plasma and laser parameters. Both excitation schemes are suitable primarily for application in the plasma edge, but even in the plasma bulk of large machines they can still be applied in combination with a diagnostic neutral beam. The two-photon excitation scheme is particularly attractive because it involves absorption spectra that are resolved within the Doppler width. This implies a large diagnostic potential and in particular offers a way to measure the deuterium-tritium fuel mix in fusion reactors. (author) 37 refs.

  20. Two-Photon Photodynamic Therapy by Water-Soluble Self-Assembled Conjugated Porphyrins

    Directory of Open Access Journals (Sweden)

    Kazuya Ogawa

    2013-01-01

    Full Text Available Studies on two-photon absorption (2PA photodynamic therapy (PDT by using three water-soluble porphyrin self-assemblies consisting of ethynylene-linked conjugated bis (imidazolylporphyrin are reviewed. 2PA cross-section values in water were obtained by an open aperture Z-scan measurement, and values were extremely large compared with those of monomeric porphyrins such as hematoporphyrin. These compounds were found to generate singlet oxygen efficiently upon one- as well as two-photon absorption as demonstrated by the time-resolved luminescence measurement at the characteristic band of singlet oxygen at 1270 nm and by using its scavenger. Photocytotoxicities for HeLa cancer cells were examined and found to be as high as those of hematoporphyrin, demonstrating that these compounds are potential candidates for 2PA-photodynamic therapy agents.

  1. Determination of Kerr and two-photon absorption coefficients of indandione derivatives

    Science.gov (United States)

    Bundulis, Arturs; Mihailovs, Igors; Nitiss, Edgars; Busenbergs, Janis; Rutkis, Martins

    2017-05-01

    We studied nonlinear optical properties of two different aminobenziliden-1,3-indandione derivatives - DDMABI and DMABI-OH by employing the Z-scan method. Through this we described how different donor and acceptor groups influence third-order nonlinear optical properties such as Kerr effect and two-photon absorption. During experimental measurements we used 1064 nm Nd:YAG laser with 30 ps pulse duration and 10 Hz repetition rate. From acquired values of Kerr and two-photon absorption coefficients we calculated values for real and imaginary parts of third-order susceptibility, as well as second-order hyperpolarizability. Quantum chemical calculations were carried out for secondorder hyperpolarizability to study how well calculations correlate with experimental values. Acquired data for DDMABI and DMABI-OH were compared with data for other ABI derivatives studied previously.

  2. Mitochondrial Dynamics Tracking with Two-Photon Phosphorescent Terpyridyl Iridium(III) Complexes

    Science.gov (United States)

    Huang, Huaiyi; Zhang, Pingyu; Qiu, Kangqiang; Huang, Juanjuan; Chen, Yu; Ji, Liangnian; Chao, Hui

    2016-02-01

    Mitochondrial dynamics, including fission and fusion, control the morphology and function of mitochondria, and disruption of mitochondrial dynamics leads to Parkinson’s disease, Alzheimer’s disease, metabolic diseases, and cancers. Currently, many types of commercial mitochondria probes are available, but high excitation energy and low photo-stability render them unsuitable for tracking mitochondrial dynamics in living cells. Therefore, mitochondrial targeting agents that exhibit superior anti-photo-bleaching ability, deep tissue penetration and intrinsically high three-dimensional resolutions are urgently needed. Two-photon-excited compounds that use low-energy near-infrared excitation lasers have emerged as non-invasive tools for cell imaging. In this work, terpyridyl cyclometalated Ir(III) complexes (Ir1-Ir3) are demonstrated as one- and two-photon phosphorescent probes for real-time imaging and tracking of mitochondrial morphology changes in living cells.

  3. In vitro imaging of thyroid tissues using two-photon excited fluorescence and second harmonic generation.

    Science.gov (United States)

    Huang, Zufang; Li, Zuanfang; Chen, Rong; Lin, Juqiang; Li, Yongzeng; Li, Chao

    2010-08-01

    To evaluate the feasibility of two-photon excited fluorescence (TPEF) and second harmonic generation (SHG) imaging to discriminate the normal, nodular goiter and papillary cancerous thyroid tissue. In total, 45 fresh thyroid specimens (normal, 15; nodular goiter, 12; and papillary cancerous, 18) from 31 subjects were directly imaged by the TPEF and SHG combination method. The microstructure of follicle and collagen structure in thyroid tissue were clearly identified, morphologic changes between normal, nodular goiter, and papillary cancerous thyroid tissue were well characterized by using two-photon excitation fluorescence. SHG imaging of the collagen matrix also revealed the differences between normal and abnormal. Our preliminary study suggests that the TPEF and SHG combination method might be a useful tool in revealing pathologic changes in thyroid tissue.

  4. Two-photon polymerization of an epoxy-acrylate resin material system

    Energy Technology Data Exchange (ETDEWEB)

    Winfield, R.J., E-mail: richard.winfield@tyndall.ie [Tyndall National Institute, Lee Maltings, Prospect Row, Cork (Ireland); O' Brien, S. [Tyndall National Institute, Lee Maltings, Prospect Row, Cork (Ireland)

    2011-04-01

    Improved material systems are of great interest in the development of two-photon polymerization techniques for the fabrication of three dimensional micro- and nano-structures. The properties of the photosensitive resin are important in the realisation of structures with submicron dimensions. In this study investigation of a custom organic resin, cross-linked by a two-photon induced process, using a femtosecond Ti:sapphire laser, is described. A structural, optical and mechanical analysis of the optimised material is presented. The influence of both material system and laser processing parameters on achievable micro-structure and size is presented as are representative structures. Parameters include: laser power, photo-initiator concentration and material composition.

  5. Efficient simultaneous dense coding and teleportation with two-photon four-qubit cluster states

    Science.gov (United States)

    Zhang, Cai; Situ, Haozhen; Li, Qin; He, Guang Ping

    2016-08-01

    We firstly propose a simultaneous dense coding protocol with two-photon four-qubit cluster states in which two receivers can simultaneously get their respective classical information sent by a sender. Because each photon has two degrees of freedom, the protocol will achieve a high transmittance. The security of the simultaneous dense coding protocol has also been analyzed. Secondly, we investigate how to simultaneously teleport two different quantum states with polarization and path degree of freedom using cluster states to two receivers, respectively, and discuss its security. The preparation and transmission of two-photon four-qubit cluster states is less difficult than that of four-photon entangled states, and it has been experimentally generated with nearly perfect fidelity and high generation rate. Thus, our protocols are feasible with current quantum techniques.

  6. Self-Energy Correction to the Two-Photon Decay Width in Hydrogenlike Atoms

    CERN Document Server

    Jentschura, U D

    2004-01-01

    We investigate the gauge invariance of the leading logarithmic radiative correction to the two-photon decay width in hydrogenlike atoms. It is shown that an effective treatment of the correction using a Lamb-shift "potential" leads to equivalent results in both the length as well as the velocity gauges provided all relevant correction terms are taken into account. Specifically, the relevant radiative corrections are related to the energies that enter into the propagator denominators, to the Hamiltonian, to the wave functions, and to the energy conservation condition that holds between the two photons; the form of all of these effects is different in the two gauges, but the final result is shown to be gauge invariant, as it should be. Although the actual calculation only involves integrations over nonrelativistic hydrogenic Green functions, the derivation of the leading logarithmic correction can be regarded as slightly more complex than that of other typical logarithmic terms. The dominant radiative correctio...

  7. Programmable two-photon quantum interference in $10^3$ channels in opaque scattering media

    CERN Document Server

    Wolterink, Tom A W; Ctistis, Georgios; Vos, Willem L; Boller, Klaus -J; Pinkse, Pepijn W H

    2015-01-01

    We investigate two-photon quantum interference in an opaque scattering medium that intrinsically supports $10^6$ transmission channels. By adaptive spatial phase-modulation of the incident wavefronts, the photons are directed at targeted speckle spots or output channels. From $10^3$ experimentally available coupled channels, we select two channels and enhance their transmission, to realize the equivalent of a fully programmable $2\\times2$ beam splitter. By sending pairs of single photons from a parametric down-conversion source through the opaque scattering medium, we observe two-photon quantum interference. The programmed beam splitter need not fulfill energy conservation over the two selected output channels and hence could be non-unitary. Consequently, we have the freedom to tune the quantum interference from bunching (Hong-Ou-Mandel-like) to antibunching. Our results establish opaque scattering media as a platform for high-dimensional quantum interference that is notably relevant for boson sampling and ph...

  8. Programmable two-photon quantum interference in 103 channels in opaque scattering media

    Science.gov (United States)

    Wolterink, Tom A. W.; Uppu, Ravitej; Ctistis, Georgios; Vos, Willem L.; Boller, Klaus-J.; Pinkse, Pepijn W. H.

    2016-05-01

    We investigate two-photon quantum interference in an opaque scattering medium that intrinsically supports a large number of transmission channels. By adaptive spatial phase modulation of the incident wave fronts, the photons are directed at targeted speckle spots or output channels. From 103 experimentally available coupled channels, we select two channels and enhance their transmission to realize the equivalent of a fully programmable 2 ×2 beam splitter. By sending pairs of single photons from a parametric down-conversion source through the opaque scattering medium, we observe two-photon quantum interference. The programed beam splitter need not fulfill energy conservation over the two selected output channels and hence could be nonunitary. Consequently, we have the freedom to tune the quantum interference from bunching (Hong-Ou-Mandel-like) to antibunching. Our results establish opaque scattering media as a platform for high-dimensional quantum interference that is notably relevant for boson sampling and physical-key-based authentication.

  9. Dependence of the two-photon photoluminescence yield of gold nanostructures on the laser pulse duration

    Science.gov (United States)

    Biagioni, P.; Celebrano, M.; Savoini, M.; Grancini, G.; Brida, D.; Mátéfi-Tempfli, S.; Mátéfi-Tempfli, M.; Duò, L.; Hecht, B.; Cerullo, G.; Finazzi, M.

    2009-07-01

    Two-photon photoluminescence (TPPL) from gold nanostructures is becoming one of the most relevant tools for plasmon-assisted biological imaging and photothermal therapy as well as for the investigation of plasmonic devices. Here we study the yield of TPPL as a function of the temporal width δ of the excitation laser pulses for a fixed average power. In the δ>1ps regime, the TPPL yield decreases as δ is increased, while for shorter pulse widths it becomes independent of δ and, consequently, of the laser-pulse peak power. This peculiar dynamics is understood and modeled by considering that two-photon absorption in Au is a two-step process governed by the lifetime of the metastable state populated by the first photon absorption.

  10. Wide-field two-photon microscopy: features and advantages for biomedical applications

    Science.gov (United States)

    Wachsmann-Hogiu, S.; Hwang, J. Y.; Lindsley, E.; Farkas, D. L.

    2007-02-01

    We describe a simple fluorescence microscope based on wide-field two-photon excitation. While still taking advantage of some inherent properties of non-linear (two-photon) microscopy, such as increased penetration depth through tissue and reduced phototoxicity, this approach provides video frame rate imaging, can be easily coupled to fluorescence spectral and lifetime detection modules, and makes efficient use of the high average power currently available from ultrashort pulsed lasers. For a standard histopathology specimen, we were able to identify different structures based on spectral and fluorescence lifetime detection and analysis. We examined the use of 200fs and 2ps pulses from Spectra Physics MaiTai and Tsunami lasers, respectively, with average power ranging from 50mW to 500mW.

  11. Two-photon gateway in one-atom cavity quantum electrodynamics.

    Science.gov (United States)

    Kubanek, A; Ourjoumtsev, A; Schuster, I; Koch, M; Pinkse, P W H; Murr, K; Rempe, G

    2008-11-14

    Single atoms absorb and emit light from a resonant laser beam photon by photon. We show that a single atom strongly coupled to an optical cavity can absorb and emit resonant photons in pairs. The effect is observed in a photon correlation experiment on the light transmitted through the cavity. We find that the atom-cavity system transforms a random stream of input photons into a correlated stream of output photons, thereby acting as a two-photon gateway. The phenomenon has its origin in the quantum anharmonicity of the energy structure of the atom-cavity system. Future applications could include the controlled interaction of two photons by means of one atom.

  12. Enhanced two-photon excited fluorescence from imaging agents using true thermal light

    Science.gov (United States)

    Jechow, Andreas; Seefeldt, Michael; Kurzke, Henning; Heuer, Axel; Menzel, Ralf

    2013-12-01

    Two-photon excited fluorescence (TPEF) is a standard technique in modern microscopy, but is still affected by photodamage to the probe. It has been proposed that TPEF can be enhanced using entangled photons, but this has proven challenging. Recently, it was shown that some features of entangled photons can be mimicked with thermal light, which finds application in ghost imaging, subwavelength lithography and metrology. Here, we use true thermal light from a superluminescent diode to demonstrate TPEF that is enhanced compared to coherent light, using two common fluorophores and luminescent quantum dots, which suit applications in imaging and microscopy. We find that the TPEF rate is directly proportional to the measured degree of second-order coherence, as predicted by theory. Our results show that photon bunching in thermal light can be exploited in two-photon microscopy, with the photon statistic providing a new degree of freedom.

  13. 3D fabrication of all-polymer conductive microstructures by two photon polymerization.

    Science.gov (United States)

    Kurselis, Kestutis; Kiyan, Roman; Bagratashvili, Victor N; Popov, Vladimir K; Chichkov, Boris N

    2013-12-16

    A technique to fabricate electrically conductive all-polymer 3D microstructures is reported. Superior conductivity, high spatial resolution and three-dimensionality are achieved by successive application of two-photon polymerization and in situ oxidative polymerization to a bi-component formulation, containing a photosensitive host matrix and an intrinsically conductive polymer precursor. By using polyethylene glycol diacrylate (PEG-DA) and 3,4-ethylenedioxythiophene (EDOT), the conductivity of 0.04 S/cm is reached, which is the highest value for the two-photon polymerized all-polymer microstructures to date. The measured electrical conductivity dependency on the EDOT concentration indicates percolation phenomenon and a three-dimensional nature of the conductive pathways. Tunable conductivity, biocompatibility, and environmental stability are the characteristics offered by PEG-DA/EDOT blends which can be employed in biomedicine, MEMS, microfluidics, and sensorics.

  14. Additive controlled synthesis of gold nanorods (GNRs) for two-photon luminescence imaging of cancer cells

    Energy Technology Data Exchange (ETDEWEB)

    Zhu Jing; Roy, Indrajit; Hu Rui; Ding Hong; Zhao Lingling; He, Guang S; Prasad, Paras N [Institute for Lasers, Photonics and Biophotonics, University at Buffalo, State University of New York, Buffalo, NY 14260-4200 (United States); Yong, Ken-Tye [School of Electrical and Electronic Engineering, Nanyang Technological University, Singapore 639798 (Singapore); Swihart, Mark T [Department of Chemical and Biological Engineering, University at Buffalo, State University of New York, Buffalo, NY 14260-4200 (United States); Cui Yiping, E-mail: ktyong@ntu.edu.sg, E-mail: cyp@seu.edu.cn, E-mail: pnprasad@buffalo.edu [Advanced Photonics Center, School of Electronic Science and Engineering, Southeast University, Nanjing 210096 (China)

    2010-07-16

    Gold nanorods (GNRs) with a longitudinal surface plasmon resonance peak that is tunable from 600 to 1100 nm have been fabricated in a cetyl trimethylammoniumbromide (CTAB) micellar medium using hydrochloric acid and silver nitrate as additives to control their shape and size. By manipulating the concentrations of silver nitrate and hydrochloric acid, the aspect ratio of the GNRs was reliably and reproducibly tuned from 2.5 to 8. The GNRs were first coated with polyelectrolyte multilayers and then bioconjugated to transferrin (Tf) to target pancreatic cancer cells. Two-photon imaging excited from the bioconjugated GNRs demonstrated receptor-mediated uptake of the bioconjugates into Panc-1 cells, overexpressing the transferrin receptor (TfR). The bioconjugated GNR formulation exhibited very low toxicity, suggesting that it is biocompatible and potentially suitable for targeted two-photon bioimaging.

  15. Conjugated polymers with pyrrole as the conjugated bridge: synthesis, characterization, and two-photon absorption properties.

    Science.gov (United States)

    Li, Qianqian; Zhong, Cheng; Huang, Jing; Huang, Zhenli; Pei, Zhiguo; Liu, Jun; Qin, Jingui; Li, Zhen

    2011-07-14

    The synthesis, one- and two-photon absorption (2PA) and emission properties of two novel pyrrole-based conjugated polymers (P1 and P2) are reported. They emitted strong yellow-green and orange fluorescence with fluorescent quantum yields (Φ) of 46 and 33%, respectively. Their maximal 2PA cross sections (δ) measured by the two-photon-induced fluorescence method using femtosecond laser pulses in THF were 2392 and 1938 GM per repeating unit, respectively, indicating that the 2PA chromophores consisting of the triphenylamine with nonplanar structure as the donor and electron-rich pyrrole as the conjugated bridge could be the effective repeating units to enhance the δ values.

  16. Two-Photon Exchange Corrections to Precise Measurements of Proton Electroweak Form Factors

    Science.gov (United States)

    Afanasev, Andrei

    2004-10-01

    Higher-order QED effects play an important role for extracting information on proton form factors from electron scattering data. For the electric form factor of the proton, a previously neglected two-photon-exchange correction reconciles an observed discrepancy between Rosenbluth and polarization techniques [1]. We use a similar approach based on General Parton Distributions to compute additional radiative corrections to parity-violating electron scattering. [1] Y.C. Chen, A. Afanasev, S.J. Brodsky, C.E. Carlson and M. Vanderhaeghen, ``Partonic calculation of the two-photon exchange contribution to elastic electron proton scattering at large momentum transfer,`` arXiv:hep-ph/0403058, to appear in Phys.Rev.Lett.

  17. Rational Design of Fluorescent Phthalazinone Derivatives for One- and Two-Photon Imaging.

    Science.gov (United States)

    Yang, Lingfei; Zhu, Yuanjun; Shui, Mengyang; Zhou, Tongliang; Cai, Yuanbo; Wang, Wei; Xu, Fengrong; Niu, Yan; Wang, Chao; Zhang, Jun-Long; Xu, Ping; Yuan, Lan; Liang, Lei

    2016-08-22

    Phthalazinone derivatives were designed as optical probes for one- and two-photon fluorescence microscopy imaging. The design strategy involves stepwise extension and modification of pyridazinone by 1) expansion of pyridazinone to phthalazinone, a larger conjugated system, as the electron acceptor, 2) coupling of electron-donating aromatic groups such as N,N-diethylaminophenyl, thienyl, naphthyl, and quinolyl to the phthalazinone, and 3) anchoring of an alkyl chain to the phthalazinone with various terminal substituents such as triphenylphosphonio, morpholino, triethylammonio, N-methylimidazolio, pyrrolidino, and piperidino. Theoretical calculations were utilized to verify the initial design. The desired fluorescent probes were synthesized by two different routes in considerable yields. Twenty-two phthalazinone derivatives were synthesized and their photophysical properties were measured. Selected compounds were applied in cell imaging, and valuable information was obtained. Furthermore, the designed compounds showed excellent performance in two-photon microscopic imaging of mouse brain slices.

  18. Additive controlled synthesis of gold nanorods (GNRs) for two-photon luminescence imaging of cancer cells.

    Science.gov (United States)

    Zhu, Jing; Yong, Ken-Tye; Roy, Indrajit; Hu, Rui; Ding, Hong; Zhao, Lingling; Swihart, Mark T; He, Guang S; Cui, Yiping; Prasad, Paras N

    2010-07-16

    Gold nanorods (GNRs) with a longitudinal surface plasmon resonance peak that is tunable from 600 to 1100 nm have been fabricated in a cetyl trimethylammoniumbromide (CTAB) micellar medium using hydrochloric acid and silver nitrate as additives to control their shape and size. By manipulating the concentrations of silver nitrate and hydrochloric acid, the aspect ratio of the GNRs was reliably and reproducibly tuned from 2.5 to 8. The GNRs were first coated with polyelectrolyte multilayers and then bioconjugated to transferrin (Tf) to target pancreatic cancer cells. Two-photon imaging excited from the bioconjugated GNRs demonstrated receptor-mediated uptake of the bioconjugates into Panc-1 cells, overexpressing the transferrin receptor (TfR). The bioconjugated GNR formulation exhibited very low toxicity, suggesting that it is biocompatible and potentially suitable for targeted two-photon bioimaging.

  19. Time-dependent R-matrix theory applied to two-photon double ionization of He

    Science.gov (United States)

    van der Hart, H. W.

    2014-05-01

    We introduce a time-dependent R-matrix theory generalized to describe double-ionization processes. The method is used to investigate two-photon double ionization of He by intense XUV laser radiation. We combine a detailed B-spline-based wave-function description in an extended inner region with a single-electron outer region containing channels representing both single ionization and double ionization. A comparison of wave-function densities for different box sizes demonstrates that the flow between the two regions is described with excellent accuracy. The obtained two-photon double-ionization cross sections are in excellent agreement with other cross sections available. Compared to calculations fully contained within a finite inner region, the present calculations can be propagated over the time it takes the slowest electron to reach the boundary.

  20. Time-dependent R-matrix theory applied to two-photon double ionization of He

    CERN Document Server

    van der Hart, H W

    2014-01-01

    We introduce a time-dependent R-matrix theory generalised to describe double ionization processes. The method is used to investigate two-photon double ionization of He by intense XUV laser radiation. We combine a detailed B-spline-based wavefunction description in a extended inner region with a single-electron outer region containing channels representing both single ionization and double ionization. A comparison of wavefunction densities for different box sizes demonstrates that the flow between the two regions is described with excellent accuracy. The obtained two-photon double ionization cross sections are in excellent agreement with other cross sections available. Compared to calculations fully contained within a finite inner region, the present calculations can be propagated over the time it takes the slowest electron to reach the boundary.

  1. In vivo reactive neural plasticity investigation by means of correlative two photon: electron microscopy

    Science.gov (United States)

    Allegra Mascaro, A. L.; Cesare, P.; Sacconi, L.; Grasselli, G.; Mandolesi, G.; Maco, B.; Knott, G.; Huang, L.; De Paola, V.; Strata, P.; Pavone, F. S.

    2013-02-01

    In the adult nervous system, different populations of neurons correspond to different regenerative behavior. Although previous works showed that olivocerebellar fibers are capable of axonal regeneration in a suitable environment as a response to injury1, we have hitherto no details about the real dynamics of fiber regeneration. We set up a model of singularly axotomized climbing fibers (CF) to investigate their reparative properties in the adult central nervous system (CNS) in vivo. Time lapse two-photon imaging has been combined to laser nanosurgery2, 3 to define a temporal pattern of the degenerative event and to follow the structural rearrangement after injury. To characterize the damage and to elucidate the possible formation of new synaptic contacts on the sprouted branches of the lesioned CF, we combined two-photon in vivo imaging with block face scanning electron microscopy (FIB-SEM). Here we describe the approach followed to characterize the reactive plasticity after injury.

  2. Aggregation induced enhanced emission of conjugated dendrimers with a large intrinsic two-photon absorption cross-section

    NARCIS (Netherlands)

    Xu, Bin; Zhang, Jibo; Fang, Honghua; Ma, Suqian; Chen, Qidai; Sun, Hongbo; Im, Chan; Tian, Wenjing

    2014-01-01

    Organic nonlinear optical materials combining high luminescence quantum yields and large two-photon absorption cross-sections are attractive for both fundamental research and practical applications, such as up-converted lasers and two-photon fluorescence microscopy. Herein, we reported a series of

  3. Fs-transient absorption and fluorescence upconversion after two- photon excitation of carotenoids in solution and in LHC II

    CERN Document Server

    Wall, P J; Fleming, G R

    2000-01-01

    With time resolved two-photon techniques we determined the lifetime and two-photon spectrum of the forbidden S/sub 1/ state of beta - carotene (9+or-0.2 ps), lutein (15+or-0.5 ps) and the energy transferring carotenoids in LHC II (250+or-50 fs). (7 refs).

  4. Polarization and spectral characteristics of the two-photon luminescence from colloidal gold nanoparticles excited by tunable laser radiation

    Energy Technology Data Exchange (ETDEWEB)

    Yashunin, D. A., E-mail: yashuninda@yandex.ru; Korytin, A. I.; Stepanov, A. N. [Russian Academy of Sciences, Institute of Applied Physics (Russian Federation)

    2015-12-15

    We have experimentally studied two-photon luminescence from a colloidal solution of spherical gold nanoparticles by tuning the wavelength of the exciting radiation. The measured polarization and spectral characteristics of the two-photon luminescence signal show that the observed nonlinear optical response is determined by the dimers present in the solution with a concentration of a few percent of total nanoparticle number.

  5. Measurement of ηc production in untagged two-photon collisions at LEP

    Science.gov (United States)

    Adriani, O.; Aguilar-Benitez, M.; Ahlen, S.; Alcaraz, J.; Aloisio, A.; Alverson, G.; Alviggi, M. G.; Ambrosi, G.; An, Q.; Anderhub, H.; Anderson, A. L.; Andreev, V. P.; Angelescu, T.; Antonov, L.; Antreasyan, D.; Arce, P.; Arefiev, A.; Atamanchuk, A.; Azemoon, T.; Aziz, T.; Baba, P. V. K. S.; Bagnaia, P.; Bakken, J. A.; Ball, R. C.; Banerjee, S.; Bao, J.; Barillère, R.; Barone, L.; Baschirotto, A.; Battiston, R.; Bay, A.; Becattini, F.; Bechtluft, J.; Becker, R.; Becker, U.; Behner, F.; Behrens, J.; Bencze, Gy. L.; Berdugo, J.; Berges, P.; Bertucci, B.; Betev, B. L.; Biasini, M.; Biland, A.; Bilei, G. M.; Bizzarri, R.; Blaising, J. J.; Bobbink, G. J.; Bock, R.; Böhm, A.; Borgia, B.; Bosetti, M.; Bourilkov, D.; Bourquin, M.; Boutigny, D.; Bouwens, B.; Brambilla, E.; Branson, J. G.; Brock, I. C.; Brooks, M.; Bujak, A.; Burger, J. D.; Burger, W. J.; Busenitz, J.; Buytenhuijs, A.; Cai, X. D.; Capell, M.; Caria, M.; Carlino, G.; Cartacci, A. M.; Castello, R.; Cerrada, M.; Cesaroni, F.; Chang, Y. H.; Chaturvedi, U. K.; Chemarin, M.; Chen, A.; Chen, C.; Chen, G.; Chen, G. M.; Chen, H. F.; Chen, H. S.; Chen, M.; Chen, W. Y.; Chiefari, G.; Chien, C. Y.; Choi, M. T.; Chung, S.; Civinini, C.; Clare, I.; Clare, R.; Coan, T. E.; Cohn, H. O.; Coignet, G.; Colino, N.; Contin, A.; Costantini, S.; Cotorobai, F.; Cui, X. T.; Cui, X. Y.; Dai, T. S.; D'Alessandro, R.; de Asmundis, R.; Degré, A.; Deiters, K.; Dénes, E.; Denes, P.; DeNotaristefani, F.; Dhina, M.; DiBitonto, D.; Diemoz, M.; Dimitrov, H. R.; Dionisi, C.; Dittmar, M.; Djambazov, L.; Dova, M. T.; Drago, E.; Duchesneau, D.; Duinker, P.; Duran, I.; Easo, S.; El Mamouni, H.; Engler, A.; Eppling, F. J.; Erné, F. C.; Extermann, P.; Fabbretti, R.; Fabre, M.; Falciano, S.; Fan, S. J.; Fackler, O.; Fay, J.; Felcini, M.; Ferguson, T.; Fernandez, D.; Fernandez, G.; Ferroni, F.; Fesefeldt, H.; Fiandrini, E.; Field, J. H.; Filthaut, F.; Fisher, P. H.; Forconi, G.; Fredj, L.; Freudenreich, K.; Friebel, W.; Fukushima, M.; Gailloud, M.; Galaktionov, Yu.; Gallo, E.; Ganguli, S. N.; Garcia-Abia, P.; Gele, D.; Gentile, S.; Gheordanescu, N.; Giagu, S.; Goldfarb, S.; Gong, Z. F.; Gonzalez, E.; Gougas, A.; Goujon, D.; Gratta, G.; Gruenewald, M.; Gu, C.; Guanziroli, M.; Guo, J. K.; Gupta, V. K.; Gurtu, A.; Gustafson, H. R.; Gutay, L. J.; Hangarter, K.; Hartmann, B.; Hasan, A.; Hauschildt, D.; He, C. F.; He, J. T.; Hebbeker, T.; Hebert, M.; Hervé, A.; Hilgers, K.; Hofer, H.; Hoorani, H.; Hu, G.; Hu, G. Q.; Ille, B.; Ilyas, M. M.; Innocente, V.; Janssen, H.; Jezequel, S.; Jin, B. N.; Jones, L. W.; Josa-Mutuberria, I.; Kasser, A.; Khan, R. A.; Kamyshkov, Yu.; Kapinos, P.; Kapustinsky, J. S.; Karyotakis, Y.; Kaur, M.; Khokhar, S.; Kienzle-Focacci, M. N.; Kim, J. K.; Kim, S. C.; Kim, Y. G.; Kinnison, W. W.; Kirkby, A.; Kirkby, D.; Kirsch, S.; Kittel, W.; Klimentov, A.; Klöckner, R.; König, A. C.; Koffeman, E.; Kornadt, O.; Koutsenko, V.; Koulbardis, A.; Kraemer, R. W.; Kramer, T.; Krastev, V. R.; Krenz, W.; Krivshich, A.; Kuijten, H.; Kumar, K. S.; Kunin, A.; Landi, G.; Lanske, D.; Lanzano, S.; Lebedev, A.; Lebrun, P.; Lecomte, P.; Lecoq, P.; Le Coultre, P.; Lee, D. M.; Lee, J. S.; Lee, K. Y.; Leedom, I.; Leggett, C.; Le Goff, J. M.; Leiste, R.; Lenti, M.; Leonardi, E.; Li, C.; Li, H. T.; Li, P. J.; Liao, J. Y.; Lin, W. T.; Lin, Z. Y.; Linde, F. L.; Lindemann, B.; Lista, L.; Liu, Y.; Lohmann, W.; Longo, E.; Lu, Y. S.; Lubbers, J. M.; Lübelsmeyer, K.; Luci, C.; Luckey, D.; Ludovici, L.; Luminari, L.; Lustermann, W.; Ma, J. M.; Ma, W. G.; MacDermott, M.; Malik, R.; Malinin, A.; Maña, C.; Maolinbay, M.; Marchesini, P.; Marion, F.; Marin, A.; Martin, J. P.; Martinez-Laso, L.; Marzano, F.; Massaro, G. G. G.; Mazumdar, K.; McBride, P.; McMahon, T.; McNally, D.; Merk, M.; Merola, L.; Meschini, M.; Metzger, W. J.; Mi, Y.; Mihul, A.; Mills, G. B.; Mir, Y.; Mirabelli, G.; Mnich, J.; Möller, M.; Morand, R.; Morganti, S.; Moulai, N. E.; Mount, R.; Müller, S.; Nadtochy, A.; Nagy, E.; Napolitano, M.; Nessi-Tedaldi, F.; Newman, H.; Neyer, C.; Niaz, M. A.; Nippe, A.; Nowak, H.; Organtini, G.; Pandoulas, D.; Paoletti, S.; Paolucci, P.; Pascale, G.; Passaleva, G.; Patricelli, S.; Paul, T.; Pauluzzi, M.; Paus, C.; Pauss, F.; Pei, Y. J.; Pensotti, S.; Perret-Gallix, D.; Perrier, J.; Pevsner, A.; Piccolo, D.; Pieri, M.; Piroué, P. A.; Plasil, F.; Plyaskin, V.; Pohl, M.; Pojidaev, V.; Postema, H.; Qi, Z. D.; Qian, J. M.; Qureshi, K. N.; Raghavan, R.; Rahal-Callot, G.; Rancoita, P. G.; Rattaggi, M.; Raven, G.; Razis, P.; Read, K.; Ren, D.; Ren, Z.; Rescigno, M.; Reucroft, S.; Ricker, A.; Riemann, S.; Riemers, B. C.; Riles, K.; Rind, O.; Rizvi, H. A.; Ro, S.; Rodriguez, F. J.; Roe, B. P.; Röhner, M.; Romero, L.; Rosier-Lees, S.; Rosmalen, R.; Rosselet, Ph.; van Rossum, W.; Roth, S.; Rubbia, A.; Rubio, J. A.; Rykaczewski, H.; Sachwitz, M.; Salicio, J.; Salicio, J. M.; Sanders, G. S.; Santocchia, A.; Sarakinos, M. S.; Sartorelli, G.; Sassowsky, M.; Sauvage, G.; Schegelsky, V.; Schmitz, D.; Schmitz, P.; Schneegans, M.; Schopper, H.; Schotanus, D. J.; Shotkin, S.; Schreiber, H. J.; Shukla, J.; Schulte, R.; Schulte, S.; Schultze, K.; Schwenke, J.; Schwering, G.; Sciacca, C.; Scott, I.; Sehgal, R.; Seiler, P. G.; Sens, J. C.; Servoli, L.; Sheer, I.; Shen, D. Z.; Shevchenko, S.; Shi, X. R.; Shumilov, E.; Shoutko, V.; Son, D.; Sopczak, A.; Soulimov, V.; Spartiotis, C.; Spickermann, T.; Spillantini, P.; Starosta, R.; Steuer, M.; Stickland, D. P.; Sticozzi, F.; Stone, H.; Strauch, K.; Stringfellow, B. C.; Sudhakar, K.; Sultanov, G.; Sun, L. Z.; Susinno, G. F.; Suter, H.; Swain, J. D.; Syed, A. A.; Tang, X. W.; Taylor, L.; Terzi, G.; Ting, Samuel C. C.; Ting, S. M.; Tonutti, M.; Tonwar, S. C.; Tóth, J.; Tsaregorodtsev, A.; Tsipolitis, G.; Tully, C.; Tung, K. L.; Ulbricht, J.; Urbán, L.; Uwer, U.; Valente, E.; Van de Walle, R. T.; Vetlitsky, I.; Viertel, G.; Vikas, P.; Vikas, U.; Vivargent, M.; Vogel, H.; Vogt, H.; Vorobiev, I.; Vorobyov, A. A.; Vuilleumier, L.; Wadhwa, M.; Wallraff, W.; Wang, C.; Wang, C. R.; Wang, X. L.; Wang, Y. F.; Wang, Z. M.; Warner, C.; Weber, A.; Weber, J.; Weill, R.; Wenaus, T. J.; Wenninger, J.; White, M.; Willmott, C.; Wittgenstein, F.; Wright, D.; Wu, S. X.; Wynhoff, S.; Wysłouch, B.; Xie, Y. Y.; Xu, J. G.; Xu, Z. Z.; Xue, Z. L.; Yan, D. S.; Yang, B. Z.; Yang, C. G.; Yang, G.; Ye, C. H.; Ye, J. B.; Ye, Q.; Yeh, S. C.; Yin, Z. W.; You, J. M.; Yunus, N.; Yzerman, M.; Zaccardelli, C.; Zaitsev, N.; Zemp, P.; Zeng, M.; Zeng, Y.; Zahang, D. H.; Zhang, Z. P.; Zhou, B.; Zhou, G. J.; Zhou, J. F.; Zhu, R. Y.; Zichichi, A.; van der Zwaan, B. C. C.; L3 Collaboration

    1993-12-01

    A study of twelve distinct decay channels of the ηc has been performed with the L3 detector at LEP, for an integrated luminosity of 30 pb -1. Summing all channels, 28 candidate events have been identified, with an estimated background of 11 events. The two-photon radiative width is evaluated to be Γγγ( ηc) = 8.0 ± 2.3 ± 2.4 keV.

  6. Two-photon absorption in mesoionic compounds pumped at the visible and at the infrared

    CERN Document Server

    Rakov, N; Da Rocha, G B; Simas, A M; Athayde-Filho, P A F; Miller, J

    2000-01-01

    Intensity dependent transmission and laser-induced fluorescence were observed in liquid solutions of mesoionic compounds (MIC) pumped with nanosecond lasers operating at 1064, 604, and 570 nm. The results indicate that two-photon absorption (TPA) is the dominant mechanism which causes the observed behavior. The TPA cross-sections measured have values from 0.33*10/sup -20/ cm/sup 4//GW to 0.43*10/sup -18/ cm /sup 4//GW. (20 refs).

  7. Two-Photon-Exchange Correction to Elastic ep Scattering in the Forward Angle Limit

    Institute of Scientific and Technical Information of China (English)

    ZHOU Hai-Qing

    2009-01-01

    The two-photon-exchange (TPE) correction to elastic ep ecattering in the forward angle region is discussed based on a simple hadronic model.It is found that the correction is exactly zero in the forward angle limit.This analytical result gives a good explanation of the previous numerical results and shows the clear power behavior of the TPE correction to elastic ep scattering in the forward angle region.

  8. Multiscale vision model for event detection and reconstruction in two-photon imaging data

    DEFF Research Database (Denmark)

    Brazhe, Alexey; Mathiesen, Claus; Lind, Barbara;

    2014-01-01

    on a modified multiscale vision model, an object detection framework based on the thresholding of wavelet coefficients and hierarchical trees of significant coefficients followed by nonlinear iterative partial object reconstruction, for the analysis of two-photon calcium imaging data. The framework is discussed...... of the multiscale vision model is similar in the denoising, but provides a better segmenation of the image into meaningful objects, whereas other methods need to be combined with dedicated thresholding and segmentation utilities....

  9. Development and design of advanced two-photon microscope used in neuroscience

    Science.gov (United States)

    Doronin, M. S.; Popov, A. V.

    2016-08-01

    This work represents the real steps to development and design advanced two-photon microscope by efforts of laboratory staff. Self-developed microscopy system provides possibility to service it and modify the structure of microscope depending on highly specialized experimental design and scientific goals. We are presenting here module-based microscopy system which provides an opportunity to looking for new applications of this setup depending on laboratories needs using with galvo and resonant scanners.

  10. Morphology dependent two photon absorption in plasmonic structures and plasmonic-organic hybrids

    Science.gov (United States)

    Gambhir, Kaweri; Ray, Bhumika; Mehrotra, Ranjana; Sharma, Parag

    2017-05-01

    Two photon absorption coefficients of two distinct plasmonic structures, namely, gold nanoflowers (GNF) and gold nanopebbles (GNP) have been investigated and compared with conventional gold nanospheres (GNS). All three different nanoshapes were synthesized by changing the reaction solvent under the same experimental procedure. Further, hybrids of these plasmonic structures were prepared with an organic dye Eosin yellow (EY), to investigate the morphology effect of plasmonic structures on plasmonic-organic hybrids in terms of their linear extinction spectra and two photon absorption coefficients. The NLO investigations were conducted using 20 ps laser pulses of wavelength 532 nm as an excitation source in single beam Z-scan setup. UV/visible spectroscopy was employed for monitoring plasmon resonances and changes in linear extinction spectra. The experimental outcomes revealed two photon absorption coefficients of EY increased 120%, 32% and 39%, while 69%, 60% and 53% enhancement in the peaks of linear extinction maxima of EY has been observed, when hybridized with GNF, GNS and GNP, respectively. This boost in the optical coefficients may be attributed to dimerization of EY molecules on the surface of nanoparticles. Keeping the toxicity of EY in view, we propose that the two photon absorption coefficients of this dye and control thereof, by the addition of plasmonic structures would be helpful not only in understanding the interactions between plasmons and fluorophore, but also pave an efficient way, to reduce the operative concentration of this hazardous dye in a wide range of applications and thereby, mitigating the environmental degradation caused by its highly concentrated effluents.

  11. Acute two-photon imaging of the neurovascular unit in the cortex of active mice

    Science.gov (United States)

    Tran, Cam Ha T.; Gordon, Grant R.

    2015-01-01

    In vivo two-photon scanning fluorescence imaging is a powerful technique to observe physiological processes from the millimeter to the micron scale in the intact animal. In neuroscience research, a common approach is to install an acute cranial window and head bar to explore neocortical function under anesthesia before inflammation peaks from the surgery. However, there are few detailed acute protocols for head-restrained and fully awake animal imaging of the neurovascular unit during activity. This is because acutely performed awake experiments are typically untenable when the animal is naïve to the imaging apparatus. Here we detail a method that achieves acute, deep-tissue two-photon imaging of neocortical astrocytes and microvasculature in behaving mice. A week prior to experimentation, implantation of the head bar alone allows mice to train for head-immobilization on an easy-to-learn air-supported ball treadmill. Following just two brief familiarization sessions to the treadmill on separate days, an acute cranial window can subsequently be installed for immediate imaging. We demonstrate how running and whisking data can be captured simultaneously with two-photon fluorescence signals with acceptable movement artifacts during active motion. We also show possible applications of this technique by (1) monitoring dynamic changes to microvascular diameter and red blood cells in response to vibrissa sensory stimulation, (2) examining responses of the cerebral microcirculation to the systemic delivery of pharmacological agents using a tail artery cannula during awake imaging, and (3) measuring Ca2+ signals from synthetic and genetically encoded Ca2+ indicators in astrocytes. This method will facilitate acute two-photon fluorescence imaging in awake, active mice and help link cellular events within the neurovascular unit to behavior. PMID:25698926

  12. Acute two-photon imaging of the neurovascular unit in the cortex of active mice

    Directory of Open Access Journals (Sweden)

    Cam Ha Thai Tran

    2015-02-01

    Full Text Available In vivo two-photon scanning fluorescence imaging is a powerful technique to observe physiological processes from the millimeter to the micron scale in the intact animal. In neuroscience research, a common approach is to install an acute cranial window and head bar to explore neocortical function under anesthesia before inflammation peaks from the surgery. However, there are few detailed acute protocols for head-restrained and fully awake animal imaging of the neurovascular unit during activity. This is because acutely performed awake experiments are typically untenable when the animal is naïve to the imaging apparatus. Here we detail a protocol that achieves acute, deep-tissue two-photon imaging of neocortical astrocytes and microvasculature in behaving mice. A week prior to experimentation, implantation of the head bar alone allows mice to train for head-immobilization on an easy-to-learn air-supported ball treadmill. Following just two brief familiarization sessions to the treadmill on separate days, an acute cranial window can subsequently be installed for immediate imaging. We demonstrate how running and whisking data can be captured simultaneously with two-photon fluorescence signals with acceptable movement artifacts during active motion. We also show possible applications of this technique by 1 monitoring dynamic changes to microvascular diameter and red blood cells movements in response to vibrissa sensory stimulation, 2 examining responses of the cerebral microcirculation to the systemic delivery of pharmacological agents using a tail artery cannula during awake imaging, and 3 measuring Ca2+ signals from synthetic and genetically encoded Ca2+ indicators in astrocytes. This method will facilitate acute two-photon fluorescence imaging in awake, active mice and help link cellular events within the neurovascular unit to behaviour.

  13. Tailored probes for atomic force microscopy fabricated by two-photon polymerization

    Science.gov (United States)

    Göring, Gerald; Dietrich, Philipp-Immanuel; Blaicher, Matthias; Sharma, Swati; Korvink, Jan G.; Schimmel, Thomas; Koos, Christian; Hölscher, Hendrik

    2016-08-01

    3D direct laser writing based on two-photon polymerization is considered as a tool to fabricate tailored probes for atomic force microscopy. Tips with radii of 25 nm and arbitrary shape are attached to conventionally shaped micro-machined cantilevers. Long-term scanning measurements reveal low wear rates and demonstrate the reliability of such tips. Furthermore, we show that the resonance spectrum of the probe can be tuned for multi-frequency applications by adding rebar structures to the cantilever.

  14. Intravital two-photon imaging: a versatile tool for dissecting the immune system.

    Science.gov (United States)

    Ishii, Taeko; Ishii, Masaru

    2011-03-01

    During the past decade, multi-photon or 'two-photon' excitation microscopy has launched a new era in the field of biological imaging. The near-infrared excitation laser for two-photon microscopy can penetrate thicker specimens, enabling the visualisation of living cell behaviour deep within tissues and organs without thin sectioning. The minimised photobleaching and toxicity enables the visualisation of live and intact specimens for extended periods. In this brief review, recent findings in intravital two-photon imaging for the physiology and pathology of the immune system are discussed. The immune system configures highly dynamic networks, where many cell types actively travel throughout the body and interact with each other in specific areas. Hence, real-time intravital imaging may be a powerful tool for dissecting the mechanisms of this dynamic system. The most unique characteristic of the immune system is its highly dynamic nature. A variety of cell types, such as lymphocytes, macrophages and dendritic cells (DCs), are continuously circulating throughout the body, migrating through the peripheral tissues and interacting with each other in their respective niches. Conventional methodologies in immunology, such as flow cytometry, cell or tissue culture, biochemistry and histology, have brought tremendous achievement within this field, although the dynamics of immune cells in an entire animal remain less clear. Technological progress of fluorescence microscopy has enabled us to visualise the intact biological phenomenon that has been uninvestigated. Among the advancements, the recent emergence and prevalence of two-photon, excitation-based, laser microscopy has revolutionised the research field, such that the dynamic behaviour of cells deep inside living organs can be visualised and analysed.

  15. Quantum Teleportation of One-Photon and Two-Photon Superposition States

    Institute of Scientific and Technical Information of China (English)

    2002-01-01

    @@ One-photon and two-photon superposition states are the fundamental quantum states, which have shown interesting features, such as squeezing and anti-bunching. In this paper we discuss the quantum teleportation of such quantum states with the continuous-wave EPR states. Fidelity as a function of EPR correlation is obtained. We also compared the results with Fock state and coherent state teleportation.

  16. Angular distributions in two-colour two-photon ionization of He

    CERN Document Server

    Rey, H F

    2014-01-01

    We present R-Matrix with time dependence (RMT) calculations for the photoionization of helium irradiated by an EUV laser pulse and an overlapping IR pulse with an emphasis on the anisotropy parameters of the sidebands generated by the dressing laser field. We investigate how these parameters depend on the amount of atomic structure included in the theoretical model for two-photon ionization. To verify the accuracy of the RMT approach, our theoretical results are compared with experiment.

  17. Angular distributions in two-colour two-photon ionization of He

    Science.gov (United States)

    Rey, H. F.; van der Hart, H. W.

    2014-11-01

    We present R-Matrix with time dependence (RMT) calculations for the photoionization of helium irradiated by an EUV laser pulse and an overlapping IR pulse with an emphasis on the anisotropy parameters of the sidebands generated by the dressing laser field. We investigate how these parameters depend on the amount of atomic structure included in the theoretical model for two-photon ionization. To verify the accuracy of the RMT approach, our theoretical results are compared with the experiment.

  18. Experimental Entanglement and Nonlocality of a Two-Photon Six-Qubit Cluster State

    CERN Document Server

    Ceccarelli, Raino; De Martini, Francesco; Mataloni, Paolo; Cabello, Adan

    2009-01-01

    We create a six-qubit linear cluster state by transforming a two-photon hyper-entangled state in which three qubits are encoded in each particle, one in the polarization and two in linear momentum degrees of freedom. For this state, we demonstrate genuine six-qubit entanglement, robustness of entanglement against the loss of qubits, and higher violation of Bell inequalities than in previous experiments.

  19. Two-photon absorption coefficient dichroism in Ⅱ-Ⅵ semiconductor crystals

    Institute of Scientific and Technical Information of China (English)

    Ma Guo-Hong; Ma Hong-Liang; Tang Sing-Hai

    2007-01-01

    Considering two beams propagate in semiconductor crystal, this paper discusses the polarization dependence of pump beam-induced intensity attenuation of probe beam due to two-photon absorption (TPA). Numerical calculation and experimental measurement demonstrate that TPA coefficient is polarization dependent. For homogeneous materials,probe beam attenuation arises from the imaginary part of diagonal and off-diagonal components of third-order nonlinear susceptibilities.

  20. Functionalized 3D Architected Materials via Thiol-Michael Addition and Two-Photon Lithography.

    Science.gov (United States)

    Yee, Daryl W; Schulz, Michael D; Grubbs, Robert H; Greer, Julia R

    2017-04-01

    Fabrication of functionalized 3D architected materials is achieved by a facile method using functionalized acrylates synthesized via thiol-Michael addition, which are then polymerized using two-photon lithography. A wide variety of functional groups can be attached, from Boc-protected amines to fluoroalkanes. Modification of surface wetting properties and conjugation with fluorescent tags are demonstrated to highlight the potential applications of this technique. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  1. Polarization-resolved two-photon luminescence microscopy of V-groove arrays

    DEFF Research Database (Denmark)

    Beermann, J.; Novikov, S. M.; Holmgaard, T.;

    2012-01-01

    Using two-photon luminescence (TPL) microscopy and local reflection spectroscopy we investigate electromagnetic field enhancement effects from a mu m-sized composition of 450-nm-deep V-grooves milled by focused ion beam in a thick gold film and assembled to feature, within the same structure...... obtained to evaluation of local field enhancements using TPL microscopy, especially when investigating extended structures exhibiting different radiation channels, are discussed. (C)2011 Optical Society of America...

  2. Two-photon annihilation into octet meson pairs. Symmetry relations in the handbag approach

    Energy Technology Data Exchange (ETDEWEB)

    Diehl, M. [Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Kroll, P. [Wuppertal Univ. (Gesamthochschule) (Germany). Fachbereich Physik; Regensburg Univ. (Germany). Institut fuer Theoretische Physik

    2009-11-15

    We explore the implications of SU(3) flavor symmetry in the soft handbag mechanism for two-photon annihilation into pairs of pseudoscalar octet mesons. In this approach we obtain a good description of the experimental results for all measured channels at high energy, with two complex form factors adjusted to the data. We also predict the cross section for {gamma}{gamma}{yields}{eta}{eta}. (orig.)

  3. Enhanced weak-signal sensitivity in two-photon microscopy by adaptive illumination.

    Science.gov (United States)

    Chu, Kengyeh K; Lim, Daryl; Mertz, Jerome

    2007-10-01

    We describe a technique to enhance both the weak-signal relative sensitivity and the dynamic range of a laser scanning optical microscope. The technique is based on maintaining a fixed detection power by fast feedback control of the illumination power, thereby transferring high measurement resolution to weak signals while virtually eliminating the possibility of image saturation. We analyze and demonstrate the benefits of adaptive illumination in two-photon fluorescence microscopy.

  4. Adiabatic rapid passage two-photon excitation of a Rydberg atom

    CERN Document Server

    Kuznetsova, Elena; Malinovskaya, Svetlana A

    2015-01-01

    We considered the two-photon adiabatic rapid passage excitation of a single atom from the ground to a Rydberg state. Three schemes were analyzed: both pump and Stokes fields chirped and pulsed, only the pump field is chirped, and only the pump field is pulsed and chirped while the Stokes field is continuous wave (CW). In all three cases high transfer efficiencies $>99\\%$ were achieved for the experimentally realizable Rabi frequencies and the pulse durations of the fields.

  5. Photon Emission and Reabsorption Processes in CH3NH3PbBr3 Single Crystals Revealed by Time-Resolved Two-Photon-Excitation Photoluminescence Microscopy

    Science.gov (United States)

    Yamada, Takumi; Yamada, Yasuhiro; Nakaike, Yumi; Wakamiya, Atsushi; Kanemitsu, Yoshihiko

    2017-01-01

    The dynamical processes of radiative recombination of photocarriers and reabsorption of emitted photons in CH3NH3PbBr3 single crystals are studied using time-resolved two-photon-excitation photoluminescence (PL) microscopy. We find that the PL spectrum and its decay dynamics depend on the excitation-depth profile. As the excitation depth increases, the PL spectrum becomes asymmetric, the peak energy redshifts, and the PL decay time becomes longer. These observations can be well explained by a simple model including photon recycling (photon emission and reabsorption) in thick samples with strong band-to-band transitions and high radiative recombination efficiencies.

  6. Diagnosis of basal cell carcinoma by two photon excited fluorescence combined with lifetime imaging

    Science.gov (United States)

    Fan, Shunping; Peng, Xiao; Liu, Lixin; Liu, Shaoxiong; Lu, Yuan; Qu, Junle

    2014-02-01

    Basal cell carcinoma (BCC) is the most common type of human skin cancer. The traditional diagnostic procedure of BCC is histological examination with haematoxylin and eosin staining of the tissue biopsy. In order to reduce complexity of the diagnosis procedure, a number of noninvasive optical methods have been applied in skin examination, for example, multiphoton tomography (MPT) and fluorescence lifetime imaging microscopy (FLIM). In this study, we explored two-photon optical tomography of human skin specimens using two-photon excited autofluorescence imaging and FLIM. There are a number of naturally endogenous fluorophores in skin sample, such as keratin, melanin, collagen, elastin, flavin and porphyrin. Confocal microscopy was used to obtain structures of the sample. Properties of epidermic and cancer cells were characterized by fluorescence emission spectra, as well as fluorescence lifetime imaging. Our results show that two-photon autofluorescence lifetime imaging can provide accurate optical biopsies with subcellular resolution and is potentially a quantitative optical diagnostic method in skin cancer diagnosis.

  7. Two-photon absorption in gapped bilayer graphene with a tunable chemical potential

    Science.gov (United States)

    Brinkley, M. K.; Abergel, D. S. L.; Clader, B. D.

    2016-09-01

    Despite the now vast body of two-dimensional materials under study, bilayer graphene remains unique in two ways: it hosts a simultaneously tunable band gap and electron density; and stems from simple fabrication methods. These two advantages underscore why bilayer graphene is critical as a material for optoelectronic applications. In the work that follows, we calculate the one- and two-photon absorption coefficients for degenerate interband absorption in a graphene bilayer hosting an asymmetry gap and adjustable chemical potential—all at finite temperature. Our analysis is comprehensive, characterizing one- and two-photon absorptive behavior over wide ranges of photon energy, gap, chemical potential, and thermal broadening. The two-photon absorption coefficient for bilayer graphene displays a rich structure as a function of photon energy and band gap due to the existence of multiple absorption pathways and the nontrivial dispersion of the low energy bands. This systematic work will prove integral to the design of bilayer-graphene-based nonlinear optical devices.

  8. Two-photon light-sheet nanoscopy by fluorescence fluctuation correlation analysis

    Science.gov (United States)

    Chen, Xuanze; Zong, Weijian; Li, Rongqin; Zeng, Zhiping; Zhao, Jia; Xi, Peng; Chen, Liangyi; Sun, Yujie

    2016-05-01

    Advances in light-sheet microscopy have enabled the fast three-dimensional (3D) imaging of live cells and bulk specimens with low photodamage and phototoxicity. Combining light-sheet illumination with super-resolution imaging is expected to resolve subcellular structures. Actually, such kind of super-resolution light-sheet microscopy was recently demonstrated using a single-molecule localization algorithm. However, the imaging depth and temporal resolution of this method are limited owing to the requirements of precise single molecule localization and reconstruction. In this work, we present two-photon super-resolution light-sheet imaging via stochastic optical fluctuation imaging (2PLS-SOFI), which acquires high spatiotemporal resolution and excellent optical sectioning ability. 2PLS-SOFI is based on non-linear excitation of fluctuation/blinking probes using our recently developed fast two-photon three-axis digital scanned light-sheet microscope (2P3A-DSLM), which enables both deep penetration and thin sheet of light. Overall, 2PLS-SOFI demonstrates up to 3-fold spatial resolution enhancement compared with conventional two-photon light-sheet (2PLS) microscopy and about 40-fold temporal resolution enhancement compared with individual molecule localization-selective plane illumination microscopy (IML-SPIM). Therefore, 2PLS-SOFI is promising for 3D long-term, deep-tissue imaging with high spatiotemporal resolution.

  9. New developments in two-photon analysis of human skin in vivo

    Science.gov (United States)

    Riemann, I.; Schwarz, M.; Stracke, F.; Ehlers, A.; Dimitrow, E.; Kaatz, M.; König, K.; Le Harzic, R.

    2009-02-01

    Two-photon imaging of human skin using ultra short laser pulses can be used to obtain information about the state of cells and tissues by means of their natural autofluorescence. Using this method, it is possible to determine whether the normal cell pattern is disturbed or the autofluorescence is influenced by internal or external stimuli. Two-photon fluorescence lifetime imaging (FLIM) can further enhance this providing information about physiological processes, fluorophores (like NAD(P)H, collagen, keratin, elastin, flavins, melanin,...) and external applied probes inside cells and tissue parts. For example the part of the cells metabolism and energy level can be determined by analyzing the NADH regarding its free / bound state and its oxidized / reduced state. The combination of two-photon imaging with FLIM may lead to a better understanding and diagnosis of skin reactions and disorders. We also present some results of in vivo simultaneous collagen and elastin measurements in skin dermis. Changes of dermal collagen and elastin content are characteristic for skin aging as well as for pathological skin conditions.

  10. Two-photon fluorescent sensor for K+ imaging in live cells (Conference Presentation)

    Science.gov (United States)

    Sui, Binglin; Yue, Xiling; Kim, Bosung; Belfield, Kevin D.

    2016-03-01

    It is difficult to overstate the physiological importance of potassium for life as its indispensable roles in a variety of biological processes are widely known. As a result, efficient methods for determining physiological levels of potassium are of paramount importance. Despite this, relatively few K+ fluorescence sensors have been reported, with only one being commercially available. A new two-photon excited fluorescent K+ sensor is reported. The sensor is comprised of three moieties, a highly selective K+ chelator as the K+ recognition unit, a boron-dipyrromethene (BODIPY) derivative modified with phenylethynyl groups as the fluorophore, and two polyethylene glycol chains to afford water solubility. The sensor displays very high selectivity (physiological metal cations. Upon binding K+, the sensor switches from non-fluorescent to highly fluorescent, emitting red to near-IR (NIR) fluorescence. The sensor exhibited a good two-photon absorption cross section, 500 GM at 940 nm. Moreover, it is not sensitive to pH in the physiological pH range. Time-dependent cell imaging studies via both one- and two-photon fluorescence microscopy demonstrate that the sensor is suitable for dynamic K+ sensing in living cells.

  11. Cell flow analysis with a two-photon fluorescence fiber probe

    Science.gov (United States)

    Chang, Yu-Chung; Ye, Jing Yong; Thomas, Thommey P.; Baker, James R., Jr.; Norris, Theodore B.

    2010-11-01

    We report the use of a sensitive double-clad fiber (DCF) probe for in situ cell flow velocity measurements and cell analysis by means of two-photon excited fluorescence correlation spectroscopy (FCS). We have demonstrated the feasibility to use this fiber probe for in vivo two-photon flow cytometry previously. However, because of the viscosity of blood and the non-uniform flow nature in vivo, it is problematic to use the detected cell numbers to estimate the sampled blood volume. To precisely calibrate the sampled blood volume, it is necessary to conduct real time flow velocity measurement. We propose to use FCS technique to measure the flow velocity. The ability to measure the flow velocities of labeled cells in whole blood has been demonstrated. Our two-photon fluorescence fiber probe has the ability to monitor multiple fluorescent biomarkers simultaneously. We demonstrate that we can distinguish differently labeled cells by their distinct features on the correlation curves. The ability to conduct in situ cell flow analysis using the fiber probe may be useful in disease diagnosis or further comprehension of the circulation system.

  12. Nonlinear processes upon two-photon interband picosecond excitation of PbWO4 crystal

    Science.gov (United States)

    Lukanin, V. I.; Karasik, A. Ya

    2016-09-01

    A new experimental method is proposed to study the dynamics of nonlinear processes occurring upon two-photon interband picosecond excitation of a lead tungstate crystal and upon its excitation by cw probe radiation in a temporal range from several nanoseconds to several seconds. The method is applied to the case of crystal excitation by a sequence of 25 high-power picosecond pulses with a wavelength of 523.5 nm and 633-nm cw probe radiation. Measuring the probe beam transmittance during crystal excitation, one can investigate the influence of two-photon interband absorption and the thermal nonlinearity of the refractive index on the dynamics of nonlinear processes in a wide range of times (from several nanoseconds to several seconds). The time resolution of the measuring system makes it possible to distinguish fast and slow nonlinear processes of electronic or thermal nature, including the generation of a thermal lens and thermal diffusion. An alternative method is proposed to study the dynamics of induced absorption transformation and, therefore, the dynamics of the development of nonlinear rocesses upon degenerate two-photon excitation of the crystal in the absence of external probe radiation.

  13. Hyperentanglement purification for two-photon six-qubit quantum systems

    Science.gov (United States)

    Wang, Guan-Yu; Liu, Qian; Deng, Fu-Guo

    2016-09-01

    Recently, two-photon six-qubit hyperentangled states were produced in experiment and they can improve the channel capacity of quantum communication largely. Here we present a scheme for the hyperentanglement purification of nonlocal two-photon systems in three degrees of freedom (DOFs), including the polarization, the first-longitudinal-momentum, and the second-longitudinal-momentum DOFs. Our hyperentanglement purification protocol (hyper-EPP) is constructed with two steps resorting to parity-check quantum nondemolition measurement on the three DOFs and swap gates, respectively. With these two steps, the bit-flip errors in the three DOFs can be corrected efficiently. Also, we show that using swap gates is a universal method for hyper-EPP in the polarization DOF and multiple-longitudinal-momentum DOFs. The implementation of our hyper-EPP is assisted by nitrogen-vacancy centers in optical microcavities, which could be achieved with current techniques. It is useful for long-distance high-capacity quantum communication with two-photon six-qubit hyperentanglement.

  14. Spectroscopic Study of ThCl+ by Two-Photon Ionization

    Science.gov (United States)

    Bartlett, Joshua; VanGundy, Robert A.; Heaven, Michael; Peterson, Kirk

    2016-06-01

    Despite the irreplaceable role experimental data plays for evaluating the performance of computational predictions, diatomic actinide species have not received much spectroscopic attention. As an early actinide element, thorium-containing species are ideal candidates for these types of studies. The electronic structure is expected to be relatively simple compared to later actinides, and therefore allows straightforward assessment of calculations. Here, we have studied ThCl+ for the first time via resonant two-photon ionization of jet-cooled ThCl produced by laser ablation of the metal reacted with dilute Cl2. Laser-induced Fluorescence (LIF) spectra have been recorded for the neutral molecule from 16000 - 23500 cm-1 in search of a suitable intermediate state for subsequent two-photon ionization experiments. Monochromator dispersion of the fluorescence has recovered the ground state vibration and anharmonic constants of ThCl. Resonant Two-Photon Ionization (R2PI) within a time-of-flight mass spectrometer was used to confirm ThCl production, and Pulsed Field Ionization Zero Kinetic Energy photoelectron spectroscopy (PFI-ZEKE) has been performed to identify the ionization energy as well as several of the low-lying states of the ThCl+ molecule. These constants have been predicted at the CASPT2 and CCSD(T) levels of theory, and a discussion of the calculations' performance will be presented alongside the recorded spectra.

  15. Two-photon absorption measurements in graphene fragments: Role of electron-electron interactions

    Science.gov (United States)

    Sandhu, A.; Roberts, A.; Aryanpour, K.; Shukla, A.; Mazumdar, S.

    2012-02-01

    Many-body interactions in graphene are an active field of research. There is a clear evidence of strong electron correlation effects in other carbon based materials which have the same sp^2 hybridization as graphene. For example, in linear-polyenes, the electron-electron interactions are considered responsible for the occurrence of lowest two-photon state below the optical one-photon state. The electronic correlation in these linear systems is a strong function of the chain length. Thus, it is pertinent to question if the two-dimensional graphene fragments also exhibit strong correlation effects and how these effects scale with fragment size. Using a white light super-continuum source, we perform z-scan measurements to extract frequency-dependent two-photon absorption coefficients in symmetric molecular fragments of graphene, e.g. coronene and hexabenzocoronene. A comparison of one-photon and two-photon absorption coefficients is then used to uncover the extent of correlation effects. In the smallest fragment, coronene, our results indicate a strong signature of the Coulomb interactions. We will discuss how the importance of electron-electron interaction varies with system size and its implication for the correlation effects in graphene.

  16. Enhanced two-photon emission in coupled metal nanoparticles induced by conjugated polymers.

    Science.gov (United States)

    Guan, Zhenping; Polavarapu, Lakshminarayana; Xu, Qing-Hua

    2010-12-01

    Interactions between noble metal (Ag and Au) nanoparticles and conjugated polymers as well as their one- and two-photon emission have been investigated. Ag and Au nanoparticles exhibited extraordinary quenching effects on the fluorescence of cationic poly(fluorinephenylene). The quenching efficiency by 37-nm Ag nanoparticles is ∼19 times more efficient than that by 13-nm Au nanoparticles, and 9-10 orders of magnitude more efficient than typical small molecule dye-quencher pairs. On the other hand, the cationic conjugated polymers induce the aggregate formation and plasmonic coupling of the metal nanoparticles, as evidenced by transmission electron microscopy images and appearance of a new longitudinal plasmon band in the near-infrared region. The two-photon emissions of Ag and Au nanoparticles were found to be significantly enhanced upon addition of conjugated polymers, by a factor of 51-times and 9-times compared to the isolated nanoparticles for Ag and Au, respectively. These studies could be further extended to the applications of two-photon imaging and sensing of the analytes that can induce formation of metal nanoparticle aggregates, which have many advantages over the conventional one-photon counterparts.

  17. A Study of Two-Prong Two-Photon Events at the Z0 Resonance

    Energy Technology Data Exchange (ETDEWEB)

    Kowalski, L.

    2004-08-09

    A study of electron-positron scattering leading to two electron-positron pairs via a two-photon interaction has been carried out at the Stanford Linear Accelerator Center (SLAC). The case where one pair is observed in the detector was investigated. These events were produced at the SLAC Linear Collider (SLC) operating in the center-of-mass energy range from 89.2 to 9.30 GeV. The data was collected using the Mark II detector. Two-photon interactions are described by the theory of quantum electrodynamics (QED). Such processes can be a significant background to new particle searches; consequently, and understanding of their production is imperative. A deviation from the event rate predicted by QED might indicate the existence of new particles. The event rate may also be useful as a luminosity monitor during data collection. The data sample from the Mark II is searched for events which have features indicative of two-photon events. For comparison with theory, the Berends, Daverveldt, and Keiss Monte Carlo event generator is used to simulate events according to QED theory. The data is compared to the theoretical predictions. Given the low event statistics from the SLC data run, the results are consistent with the QED theoretical prediction. However, due to the low statistics, this measurement cannot be used to indicate non-deviation from QED predictions.

  18. Phonon-Assisted Two-Photon Interference from Remote Quantum Emitters.

    Science.gov (United States)

    Reindl, Marcus; Jöns, Klaus D; Huber, Daniel; Schimpf, Christian; Huo, Yongheng; Zwiller, Val; Rastelli, Armando; Trotta, Rinaldo

    2017-07-12

    Photonic quantum technologies are on the verge of finding applications in everyday life with quantum cryptography and quantum simulators on the horizon. Extensive research has been carried out to identify suitable quantum emitters and single epitaxial quantum dots have emerged as near-optimal sources of bright, on-demand, highly indistinguishable single photons and entangled photon-pairs. In order to build up quantum networks, it is essential to interface remote quantum emitters. However, this is still an outstanding challenge, as the quantum states of dissimilar "artificial atoms" have to be prepared on-demand with high fidelity and the generated photons have to be made indistinguishable in all possible degrees of freedom. Here, we overcome this major obstacle and show an unprecedented two-photon interference (visibility of 51 ± 5%) from remote strain-tunable GaAs quantum dots emitting on-demand photon-pairs. We achieve this result by exploiting for the first time the full potential of a novel phonon-assisted two-photon excitation scheme, which allows for the generation of highly indistinguishable (visibility of 71 ± 9%) entangled photon-pairs (fidelity of 90 ± 2%), enables push-button biexciton state preparation (fidelity of 80 ± 2%) and outperforms conventional resonant two-photon excitation schemes in terms of robustness against environmental decoherence. Our results mark an important milestone for the practical realization of quantum repeaters and complex multiphoton entanglement experiments involving dissimilar artificial atoms.

  19. [Two-photon excitation fluorescence of 5-ALA induced PpIX in DHL cells].

    Science.gov (United States)

    Huang, Zu-Fang; Chen, Rong; Li, Yong-Zeng; Chen, Guan-Nan; Chen, Xian-Ling; Feng, Shang-Yuan; Jia, Pei-Min

    2008-11-01

    Two-photon fluorescence microscopy is a novel imaging technique, which is primarily sensitive to a specimen's response coming from an in-focus plane, thus has low photo-bleaching and photo-damage to biological samples. 5-ALA induced production of PpIX in DHL cells was excited by 820 nm femtosecond laser; two-photon excitation fluorescence of single cell was obtained in Lambda mode of laser scanning confocal microscope. The specific fluorescence intensity of PpIX which accumulated in DHL cells was measured at 2, 4 and 10 mmol x L(-1) concentration of 5-ALA with different incubation time, which reflected the kinetics of 5-ALA accumulated in DHL cells. Accumulation of PpIX in DHL cells was a dynamic change process. Biphasic alterations of PpIX accumulation were noted: PpIX content enhanced with the increasing time and reached the maximal value around 3 h, however PpIX content decreased in the subsequent incubation time. Results indicate that two-photon fluorescence based on laser scanning microscope can be a useful technology for studying the kinetics of 5-ALA induced PpIX production in DHL cells and other leukemia cells.

  20. Search for New Physics with Two Photons in the Final State with the ATLAS Detector

    CERN Document Server

    AUTHOR|(INSPIRE)INSPIRE-00441752

    This thesis reports on the search for new physics in the diphoton decay channel with the proton-proton collision data collected by ATLAS at a centre-of-mass energy of $\\sqrt{s}=8$~TeV in 2012 and $\\sqrt{s}=13$~TeV in 2015 and 2016. A feasibility study of the search for a pseudoscalar $A$ decaying to a $Z$ boson and a 125~GeV Higgs boson in the context of an extended Higgs sector, namedly the two-Higgs-doublet models, is presented. The search is performed with a final state of two jets and two photons using 20.3~${\\rm fb}^{-1}$ of data at $\\sqrt{s}=8$~TeV. The expected sensitivity is found to be competitive with the analysis with a final state of two electrons or muons and two $\\tau$ leptons, but less sensitive to the other searches with the Higgs decaying to a pair of $b$-quarks.%, due to the low branching ratios of the Higgs to two photons decay. Search for high mass resonances decaying to two photons at $\\sqrt{s}=13$~TeV is also presented. The analysed dataset corresponds to an integrated luminosity of $3.2...