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Sample records for two-photon electronic resonance

  1. Probing Electron-Phonon Interaction through Two-Photon Interference in Resonantly Driven Semiconductor Quantum Dots

    DEFF Research Database (Denmark)

    Reigue, Antoine; Iles-Smith, Jake; Lux, Fabian

    2017-01-01

    We investigate the temperature dependence of photon coherence properties through two-photon interference (TPI) measurements from a single quantum dot (QD) under resonant excitation. We show that the loss of indistinguishability is related only to the electron-phonon coupling and is not affected...

  2. Resonant two-photon annihilation of an electron-positron pair in a pulsed electromagnetic wave

    Science.gov (United States)

    Voroshilo, A. I.; Roshchupkin, S. P.; Nedoreshta, V. N.

    2016-09-01

    Two-photon annihilation of an electron-positron pair in the field of a plane low-intensity circularly polarized pulsed electromagnetic wave was studied. The conditions for resonance of the process which are related to an intermediate particle that falls within the mass shell are studied. In the resonant approximation the probability of the process was obtained. It is demonstrated that the resonant probability of two-photon annihilation of an electron-positron pair may be several orders of magnitude higher than the probability of this process in the absence of the external field. The obtained results may be experimentally verified by the laser facilities of the international megaprojects, for example, SLAC (National Accelerator Laboratory), FAIR (Facility for Antiproton and Ion Research), and XFEL (European X-Ray Free-Electron Laser).

  3. Probing Electron-Phonon Interaction through Two-Photon Interference in Resonantly Driven Semiconductor Quantum Dots

    Science.gov (United States)

    Reigue, Antoine; Iles-Smith, Jake; Lux, Fabian; Monniello, Léonard; Bernard, Mathieu; Margaillan, Florent; Lemaitre, Aristide; Martinez, Anthony; McCutcheon, Dara P. S.; Mørk, Jesper; Hostein, Richard; Voliotis, Valia

    2017-06-01

    We investigate the temperature dependence of photon coherence properties through two-photon interference (TPI) measurements from a single quantum dot (QD) under resonant excitation. We show that the loss of indistinguishability is related only to the electron-phonon coupling and is not affected by spectral diffusion. Through these measurements and a complementary microscopic theory, we identify two independent separate decoherence processes, both of which are associated with phonons. Below 10 K, we find that the relaxation of the vibrational lattice is the dominant contribution to the loss of TPI visibility. This process is non-Markovian in nature and corresponds to real phonon transitions resulting in a broad phonon sideband in the QD emission spectra. Above 10 K, virtual phonon transitions to higher lying excited states in the QD become the dominant dephasing mechanism, this leads to a broadening of the zero phonon line, and a corresponding rapid decay in the visibility. The microscopic theory we develop provides analytic expressions for the dephasing rates for both virtual phonon scattering and non-Markovian lattice relaxation.

  4. Selective Two-Photon Absorptive Resonance Femtosecond-Laser Electronic-Excitation Tagging (STARFLEET) Velocimetry in Flow and Combustion Diagnostics

    Science.gov (United States)

    Jiang, Naibo; Halls, Benjamin R.; Stauffer, Hans U.; Roy, Sukesh; Danehy, Paul M.; Gord, James R.

    2016-01-01

    Selective Two-Photon Absorptive Resonance Femtosecond-Laser Electronic-Excitation Tagging (STARFLEET), a non-seeded ultrafast-laser-based velocimetry technique, is demonstrated in reactive and non-reactive flows. STARFLEET is pumped via a two-photon resonance in N2 using 202.25-nm 100-fs light. STARFLEET greatly reduces the per-pulse energy required (30 µJ/pulse) to generate the signature FLEET emission compared to the conventional FLEET technique (1.1 mJ/pulse). This reduction in laser energy results in less energy deposited in the flow, which allows for reduced flow perturbations (reactive and non-reactive), increased thermometric accuracy, and less severe damage to materials. Velocity measurements conducted in a free jet of N2 and in a premixed flame show good agreement with theoretical velocities and further demonstrate the significantly less-intrusive nature of STARFLEET.

  5. Δ(1232) resonance contribution to two-photon exchange in electron-proton scattering revisited

    Energy Technology Data Exchange (ETDEWEB)

    Zhou, Hai-Qing [Southeast University, Department of Physics, NanJing (China); Yang, Shin Nan [National Taiwan University, Department of Physics and Center for Theoretical Sciences, Taipei (China)

    2015-08-15

    We revisit the question of the contributions of the two-photon exchange with Δ(1232) excitation to the electron-proton scattering in a hadronic model. Three improvements over the previous calculations are made, namely, correct vertex function for γN→Δ, realistic γNΔ form factors, and coupling constants. The discrepancy between the values of R≡μ{sub p} G{sub E}/G{sub M} extracted from Rosenbluth technique and polarization transfer method can be reasonably accounted for if the data of Andivahis et al. (Phys. Rev. D 50, 5491 (1994)) are analyzed. However, substantial discrepancy remains if the data of Qattan et al. (nucl-ex/0610006) are used. For the ratio R{sup ±} between e{sup ±} p scatterings, our predictions appear to be in satisfactory agreement with the preliminary data from VEPP-3. The agreement between our model predictions and the recent measurements on single spin asymmetry, transverse and longitudinal recoil proton polarizations ranges from good to poor. (orig.)

  6. Modulation of attosecond beating by resonant two-photon transition

    CERN Document Server

    Galán, Álvaro Jiménez; Martín, Fernando

    2015-01-01

    We present an analytical model that characterizes two-photon transitions in the presence of autoionising states. We applied this model to interpret resonant RABITT spectra, and show that, as a harmonic traverses a resonance, the phase of the sideband beating significantly varies with photon energy. This phase variation is generally very different from the $\\pi$ jump observed in previous works, in which the direct path contribution was negligible. We illustrate the possible phase profiles arising in resonant two-photon transitions with an intuitive geometrical representation.

  7. Modulation of attosecond beating in resonant two-photon ionization

    CERN Document Server

    Galán, Álvaro J; Martín, Fernando

    2014-01-01

    We present a theoretical study of the photoelectron attosecond beating at the basis of RABBIT (Reconstruction of Attosecond Beating By Interference of Two-photon transitions) in the presence of autoionizing states. We show that, as a harmonic traverses a resonance, its sidebands exhibit a peaked phase shift as well as a modulation of the beating frequency itself. Furthermore, the beating between two resonant paths persists even when the pump and the probe pulses do not overlap, thus providing a sensitive non-holographic interferometric means to reconstruct coherent metastable wave packets. We characterize these phenomena quantitatively with a general finite-pulse analytical model that accounts for the effect of both intermediate and final resonances on two-photon processes, at a negligible computational cost. The model predictions are in excellent agreement with those of accurate ab initio calculations for the helium atom in the region of the N=2 doubly excited states.

  8. Review of two-photon exchange in electron scattering

    Energy Technology Data Exchange (ETDEWEB)

    J. Arrington, P. G. Blunden, W. Melnitchouk

    2011-10-01

    We review the role of two-photon exchange (TPE) in electron-hadron scattering, focusing in particular on hadronic frameworks suitable for describing the low and moderate Q^2 region relevant to most experimental studies. We discuss the effects of TPE on the extraction of nucleon form factors and their role in the resolution of the proton electric to magnetic form factor ratio puzzle. The implications of TPE on various other observables, including neutron form factors, electroproduction of resonances and pions, and nuclear form factors, are summarized. Measurements seeking to directly identify TPE effects, such as through the angular dependence of polarization measurements, nonlinear epsilon contributions to the cross sections, and via e+p to e-p cross section ratios, are also outlined. In the weak sector, we describe the role of TPE and gamma-Z interference in parity-violating electron scattering, and assess their impact on the extraction of the strange form factors of the nucleon and the weak charge of the proton.

  9. Two photon exchange in elastic electron-nucleon scattering

    Energy Technology Data Exchange (ETDEWEB)

    Peter Blunden; Wolodymyr Melnitchouk; John Tjon

    2005-06-01

    A detailed study of two-photon exchange in unpolarized and polarized elastic electron-nucleon scattering is presented, taking particular account of nucleon finite size effects. Contributions from nucleon elastic intermediate states are found to have a strong angular dependence, which leads to a partial resolution of the discrepancy between the Rosenbluth and polarization transfer measurements of the proton electric to magnetic form factor ratio. The two-photon exchange contribution to the longitudinal polarization transfer ratio P{sub L} is small, whereas the contribution to the transverse polarization transfer ratio P{sub T} is enhanced at backward angles by several percent, increasing with Q{sup 2}. This gives rise to a several percent enhancement of the polarization transfer ratio P{sub T}/P{sub l} at large Q{sup 2} and backward angles. We compare the two-photon exchange effects with data on the ratio of e{sup +p} to e{sup -p} cross sections, which is predicted to be enhanced at backward angles. Finally, we evaluate the corrections to the form factors of the neutron, and estimate the elastic intermediate state contribution to the {sup 3}He form factors.

  10. Relativistic calculations of the non-resonant two-photon ionization of neutral atoms

    CERN Document Server

    Hofbrucker, Jiri; Fritzsche, Stephan

    2016-01-01

    The non-resonant two-photon one-electron ionization of neutral atoms is studied theoretically in the framework of relativistic second-order perturbation theory and independent particle approximation. In particular, the importance of relativistic and screening effects in the total two-photon ionization cross section is investigated. Detailed computations have been carried out for the K-shell ionization of neutral Ne, Ge, Xe, and U atoms. The relativistic effects significantly decrease the total cross section, for the case of U, for example, they reduce the total cross section by a factor of two. Moreover, we have found that the account for the screening effects of the remaining electrons leads to occurrence of an unexpected minimum in the total cross section at the total photon energies equal to the ionization threshold, for the case of Ne, for example, the cross section drops there by a factor of three.

  11. Two-photon resonant, stimulated processes in krypton and xenon

    Energy Technology Data Exchange (ETDEWEB)

    Miller, J.C.

    1988-11-01

    Both on-axis and conical emissions have been observed following two-photon pumping of the 5p states of krypton and the 6p', 7p, 8p, and 4f states of xenon. In the former case, coherent emissions from the 5p states to the 5s are observed, and in the latter case, many p..-->..s, d..-->..p, and f..-->..d cascade emissions are observed. By analogy to the well-studied alkali and alkaline earth examples, the emissions are discussed in terms of amplified spontaneous emission (ASE), stimulated hyper-Raman scattering, and parametric four-wave mixing. The physical processes responsible for the conical emission and for intensity anomalies in the xenon p..-->..s emissions are not understood at present. Interference effects due to coherent cancellation between competing excitation pathways may be occurring. 4 refs., 3 figs.

  12. Effect of the coherent cancellation of the two-photon resonance on the generation of vacuum ultraviolet light by two-photon reasonantly enhanced four-wave mixing

    Energy Technology Data Exchange (ETDEWEB)

    Payne, M.G.; Garrett, W.R.; Judish, J.P.; Wunderlich, R.

    1988-11-01

    Many of the most impressive demonstrations of the efficient generation of vacuum ultraviolet (VUV) light have made use of two- photon resonantly enhanced four-wave mixing to generate light at ..omega../sub VUV/ = 2..omega../sub L1/ +- ..omega../sub L2/. The two-photon resonance state is coupled to the ground state both by two photons from the first laser, or by a photon from the second laser and one from the generated VUV beam. We show here that these two coherent pathways destructively interfere once the second laser is made sufficiently intense, thereby leading to an important limiting effect on the achievable conversion efficiency. 4 refs.

  13. Confined optical-phonon-assisted cyclotron resonance in quantum wells via two-photon absorption process

    Science.gov (United States)

    Phuc, Huynh Vinh; Hien, Nguyen Dinh; Dinh, Le; Phong, Tran Cong

    2016-06-01

    The effect of confined phonons on the phonon-assisted cyclotron resonance (PACR) via both one and two photon absorption processes in a quantum well is theoretically studied. We consider cases when electrons are scattered by confined optical phonons described by the Fuchs-Kliewer slab, Ridley's guided, and Huang-Zhu models. The analytical expression of the magneto-optical absorption coefficient (MOAC) is obtained by relating it to the transition probability for the absorption of photons. It predicts resonant peaks caused by transitions between Landau levels and electric subband accompanied by confined phonons emission in the absorption spectrum. The MOAC and the full-width at half-maximum (FWHM) for the intra- and inter-subband transitions are given as functions of the magnetic field, temperature, and quantum well width. In narrow quantum wells, the phonon confinement becomes more important and should be taken into account in studying FWHM.

  14. Coherent control of non-resonant two-photon transition in molecular system

    Institute of Scientific and Technical Information of China (English)

    Zhang Hui; Zhang Shi-An; Wang Zu-Geng; Sun Zhen-Rong

    2010-01-01

    In this paper,we study theoretically and experimentally the coherent control of non-resonant two-photon transition in a molecular system (Perylene dissolved in chloroform solution) by shaping the femtosecond pulses with simple phase patterns (cosinusoidal and π phase step-function shape).The control efficiency of the two-photon transition probability is correlated with both the laser field and the molecular absorption bandwidth.Our results demonstrate that,the two-photon transition probability in a molecular system can be reduced but not completely eliminated by manipulating the laser field,and the control efficiency is minimal when the molecular absorption bandwidth is larger than twice the laser spectral bandwidth.

  15. Polarization properties of optical phase conjugation by two-photon resonant degenerate four-wave mixing

    Science.gov (United States)

    Kauranen, Martti; Gauthier, Daniel J.; Malcuit, Michelle S.; Boyd, Robert W.

    1989-08-01

    We develop a semiclassical theory of the polarization properties of phase conjugation by two-photon resonant degenerate four-wave mixing. The theory includes the effects of saturation by the pump waves. We solve the density-matrix equations of motion in steady state for a nonlinear medium consisting of stationary atoms with a ground and excited state connected by two-photon transitions. As an illustration of the general results, we consider an S0-->S0 two-photon transition, which is known to lead to perfect polarization conjugation in the limit of third-order theory. We show that the fidelity of the polarization-conjugation process is degraded for excessively large pump intensities. The degradation can occur both due to transfer of population to the excited state and due to nonresonant Stark shifts. Theoretical results are compared to those of a recent experiment [Malcuit, Gauthier, and Boyd, Opt. Lett. 13, 663 (1988)].

  16. Two-photon absorption measurements in graphene fragments: Role of electron-electron interactions

    Science.gov (United States)

    Sandhu, A.; Roberts, A.; Aryanpour, K.; Shukla, A.; Mazumdar, S.

    2012-02-01

    Many-body interactions in graphene are an active field of research. There is a clear evidence of strong electron correlation effects in other carbon based materials which have the same sp^2 hybridization as graphene. For example, in linear-polyenes, the electron-electron interactions are considered responsible for the occurrence of lowest two-photon state below the optical one-photon state. The electronic correlation in these linear systems is a strong function of the chain length. Thus, it is pertinent to question if the two-dimensional graphene fragments also exhibit strong correlation effects and how these effects scale with fragment size. Using a white light super-continuum source, we perform z-scan measurements to extract frequency-dependent two-photon absorption coefficients in symmetric molecular fragments of graphene, e.g. coronene and hexabenzocoronene. A comparison of one-photon and two-photon absorption coefficients is then used to uncover the extent of correlation effects. In the smallest fragment, coronene, our results indicate a strong signature of the Coulomb interactions. We will discuss how the importance of electron-electron interaction varies with system size and its implication for the correlation effects in graphene.

  17. The two-photon exchange contribution to elastic electron-nucleon scattering at large momentum transfer

    Energy Technology Data Exchange (ETDEWEB)

    Andrei V. Afanasev; Stanley J. Brodsky; Carl E. Carlson; Yu-Chun Chen; Marc Vanderhaeghen

    2005-01-01

    We estimate the two-photon exchange contribution to elastic electron-proton scattering at large momentum transfer by using a quark-parton representation of virtual Compton scattering. We thus can relate the two-photon exchange amplitude to the generalized parton distributions which also enter in other wide angle scattering processes. We find that the interference of one- and two-photon exchange contribution is able to substantially resolve the difference between electric form factor measurements from Rosenbluth and polarization transfer experiments.

  18. Two-photon finite-pulse model for resonant transitions in attosecond experiments

    CERN Document Server

    Galán, Álvaro Jiménez; Argenti, Luca

    2015-01-01

    We present an analytical model capable of describing two-photon ionization of atoms with attosecond pulses in the presence of intermediate and final isolated autoionizing states. The model is based on the finite-pulse formulation of second-order time-dependent perturbation theory. It approximates the intermediate and final states with Fano's theory for resonant continua, and it depends on a small set of atomic parameters that can either be obtained from separate \\emph{ab initio} calculations, or be extracted from few selected experiments. We use the model to compute the two-photon resonant photoelectron spectrum of helium below the N=2 threshold for the RABITT (Reconstruction of Attosecond Beating by Interference of Two-photon Transitions) pump-probe scheme, in which an XUV attosecond pulse train is used in association to a weak IR probe, obtaining results in quantitative agreement with those from accurate \\emph{ab initio} simulations. In particular, we show that: i) Use of finite pulses results in a homogene...

  19. Time-resolved two-photon photoemission at the Si(001)-surface. Hot electron dynamics and two-dimensional Fano resonance; Zeitaufgeloeste Zweiphotonen-Photoemission an der Si(001)-Oberflaeche. Dynamik heisser Elektronen und zweidimensionaler Fano-Effekt

    Energy Technology Data Exchange (ETDEWEB)

    Eickhoff, Christian

    2010-10-27

    By combining ultrafast laser excitation with energy-, angle- and time-resolved twophoton photoemission (2PPE), the electronic properties of bulk silicon and the Si(001) surface are investigated in this thesis. A custom-built laser- and UHV-systemequipped with a display type 2D-CCD-detector gives new insight into the relaxation dynamics of excited carriers on a femtosecond timescale. The bandgap between occupied valence bands and unoccupied conduction bands characteristically influences the dynamics of excited electrons in the bulk, as well as in surface states and resonances. For the electron-phonon interaction this leads to the formation of a bottleneck during the relaxation of hot electrons in the conduction band, which maintains the elevated electronic temperature for several picoseconds. During relaxation, excited electrons also scatter from the conduction band into the unoccupied dangling-bond surface state D{sub down}. Depending on the excitation density this surface recombination is dominated by electron-electron- or electron-phonon scattering. The relaxation of the carriers in the D{sub down}-band is again slowed down by the formation of a bottleneck in electron-phonon coupling. Furthermore, the new laser system has allowed detection of the Rydberg-like series of image-potential resonances on the Si(001)-surface. It is shown that the lifetime of these image-potential resonances in front of the semiconducting surface exhibits the same behavior as those in front of metallic surfaces. Moreover the electron-phonon coupling in the first image-potential resonance was investigated and compared to the D{sub down}-surface state. For the first time, Fano-type lineprofiles are demonstrated and analyzed in a 2PPEprocess on a surface. Tuning the photon energy of the pump-laser across the resonance between the occupied dangling-bond state D{sub up}, and the unoccupied image-potential resonance n=1, reveals a clear intensity variation that can be successfully described

  20. Two-photon photoemission investigation of electronic and dynamical properties of alkali atoms adsorbed on noble metal surfaces

    Science.gov (United States)

    Sametoglu, Vahit

    We present a systematic time-resolved two-photon photoemission study of the electronic and dynamical properties of Li through Cs adsorbed on Cu(111) and Ag(111) surfaces. A fundamental problem in surface science is how to describe the electronic structure of a chemisorption interface based on the intrinsic properties of the interacting materials. Because of their simple s-electron structure, elements of the alkali atom group comprise paradigmatic adsorbates in many theories of chemisorption, whereas the complementary experimental studies are sparse and incomplete. Through a combination of spectroscopic and femtosecond time-resolved surface measurements, we are able to probe systematically the binding energies, symmetries, and electron and nuclear relaxation dynamics of the initially unoccupied alkali atom resonances. As a prelude, we study the two-photon photoemission process occurring at the bare Ag(111) surface. We develop a quantitative model for two-photon photoemission process, where the nonresonant and k-dependent two-photon absorption between the lower and upper sp-bands is modeled by the optical Bloch equations, and the angle-dependent intensities are described by the Fresnel equations. Our two-photon photoemission spectra of Li through Cs chemisorbed Cu(111) and Ag(111) surfaces reveal two resonances with the m = 0 and m = +/-1 symmetry ('m' is the projection of the orbital angular momentum 'l' onto the surface plane). For the m = 0 resonance, which is derived from the hybridization of the ns and npz orbitals of alkali atoms, we find a binding energy of 1.84--1.99 eV below the vacuum level, which is independent of the alkali atom period, and tunes with coverage in a universal manner. At 0.3--0.7 eV higher energy, we discover and identify the m = +/-1 resonance by its characteristic angular intensity distribution, which derives from the antisymmetry of the npx and npy orbitals. We implement a quantitative model for the alkali atom chemisorption based on the

  1. A Study of Two-Prong Two-Photon Events at the Z0 Resonance

    Energy Technology Data Exchange (ETDEWEB)

    Kowalski, L.

    2004-08-09

    A study of electron-positron scattering leading to two electron-positron pairs via a two-photon interaction has been carried out at the Stanford Linear Accelerator Center (SLAC). The case where one pair is observed in the detector was investigated. These events were produced at the SLAC Linear Collider (SLC) operating in the center-of-mass energy range from 89.2 to 9.30 GeV. The data was collected using the Mark II detector. Two-photon interactions are described by the theory of quantum electrodynamics (QED). Such processes can be a significant background to new particle searches; consequently, and understanding of their production is imperative. A deviation from the event rate predicted by QED might indicate the existence of new particles. The event rate may also be useful as a luminosity monitor during data collection. The data sample from the Mark II is searched for events which have features indicative of two-photon events. For comparison with theory, the Berends, Daverveldt, and Keiss Monte Carlo event generator is used to simulate events according to QED theory. The data is compared to the theoretical predictions. Given the low event statistics from the SLC data run, the results are consistent with the QED theoretical prediction. However, due to the low statistics, this measurement cannot be used to indicate non-deviation from QED predictions.

  2. Resonance formation in the $\\pi^+\\pi^-\\pi^0$ final state in two-photon collisions

    CERN Document Server

    Acciarri, M; Aguilar-Benítez, M; Ahlen, S P; Alcaraz, J; Alemanni, G; Allaby, James V; Aloisio, A; Alverson, G; Alviggi, M G; Ambrosi, G; Anderhub, H; Andreev, V P; Angelescu, T; Anselmo, F; Arefev, A; Azemoon, T; Aziz, T; Bagnaia, P; Baksay, L; Ball, R C; Banerjee, S; Banerjee, Sw; Banicz, K; Barczyk, A; Barillère, R; Barone, L; Bartalini, P; Baschirotto, A; Basile, M; Battiston, R; Bay, A; Becattini, F; Becker, U; Behner, F; Berdugo, J; Berges, P; Bertucci, B; Betev, B L; Bhattacharya, S; Biasini, M; Biland, A; Bilei, G M; Blaising, J J; Blyth, S C; Bobbink, Gerjan J; Böck, R K; Böhm, A; Boldizsar, L; Borgia, B; Boucham, A; Bourilkov, D; Bourquin, Maurice; Boutigny, D; Braccini, S; Branson, J G; Brigljevic, V; Brock, I C; Buffini, A; Buijs, A; Burger, J D; Burger, W J; Busenitz, J K; Cai, X D; Campanelli, M; Capell, M; Cara Romeo, G; Carlino, G; Cartacci, A M; Casaus, J; Castellini, G; Cavallari, F; Cavallo, N; Cecchi, C; Cerrada-Canales, M; Cesaroni, F; Chamizo-Llatas, M; Chang, Y H; Chaturvedi, U K; Chekanov, S V; Chemarin, M; Chen, A; Chen, G; Chen, G M; Chen, H F; Chen, H S; Chen, M; Chiefari, G; Chien, C Y; Cifarelli, Luisa; Cindolo, F; Civinini, C; Clare, I; Clare, R; Cohn, H O; Coignet, G; Colijn, A P; Colino, N; Commichau, V; Costantini, S; Cotorobai, F; de la Cruz, B; Csilling, Akos; Dai, T S; D'Alessandro, R; De Asmundis, R; Degré, A; Deiters, K; Denes, P; De Notaristefani, F; DiBitonto, Daryl; Diemoz, M; Van Dierendonck, D N; Di Lodovico, F; Dionisi, C; Dittmar, Michael; Dominguez, A; Doria, A; Dorne, I; Dova, M T; Drago, E; Duchesneau, D; Duinker, P; Durán, I; Dutta, S; Easo, S; Efremenko, Yu V; El-Mamouni, H; Engler, A; Eppling, F J; Erné, F C; Ernenwein, J P; Extermann, Pierre; Fabre, M; Faccini, R; Falciano, S; Favara, A; Fay, J; Fedin, O; Felcini, Marta; Fenyi, B; Ferguson, T; Ferroni, F; Fesefeldt, H S; Fiandrini, E; Field, J H; Filthaut, Frank; Fisher, P H; Fisk, I; Forconi, G; Fredj, L; Freudenreich, Klaus; Furetta, C; Galaktionov, Yu; Ganguli, S N; García-Abia, P; Gau, S S; Gentile, S; Gerald, J; Gheordanescu, N; Giagu, S; Goldfarb, S; Goldstein, J; Gong, Z F; Gougas, Andreas; Gratta, Giorgio; Grünewald, M W; Gupta, V K; Gurtu, A; Gutay, L J; Hartmann, B; Hasan, A; Hatzifotiadou, D; Hebbeker, T; Hervé, A; Van Hoek, W C; Hofer, H; Hong, S J; Hoorani, H; Hou, S R; Hu, G; Innocente, Vincenzo; Janssen, H; Jenkes, K; Jin, B N; Jones, L W; de Jong, P; Josa-Mutuberria, I; Kasser, A; Khan, R A; Kamrad, D; Kamyshkov, Yu A; Kapustinsky, J S; Karyotakis, Yu; Kaur, M; Kienzle-Focacci, M N; Kim, D; Kim, D H; Kim, J K; Kim, S C; Kim, Y G; Kinnison, W W; Kirkby, A; Kirkby, D; Kirkby, Jasper; Kiss, D; Kittel, E W; Klimentov, A; König, A C; Kopp, A; Korolko, I; Koutsenko, V F; Krämer, R W; Krenz, W; Kunin, A; Ladrón de Guevara, P; Landi, G; Lapoint, C; Lassila-Perini, K M; Laurikainen, P; Lebeau, M; Lebedev, A; Lebrun, P; Lecomte, P; Lecoq, P; Le Coultre, P; Leggett, C; Le Goff, J M; Leiste, R; Leonardi, E; Levchenko, P M; Li Chuan; Lin, C H; Lin, W T; Linde, Frank L; Lista, L; Liu, Z A; Lohmann, W; Longo, E; Lu, W; Lü, Y S; Lübelsmeyer, K; Luci, C; Luckey, D; Luminari, L; Lustermann, W; Ma Wen Gan; Maity, M; Majumder, G; Malgeri, L; Malinin, A; Maña, C; Mangeol, D J J; Mangla, S; Marchesini, P A; Marin, A; Martin, J P; Marzano, F; Massaro, G G G; McNally, D; Mele, S; Merola, L; Meschini, M; Metzger, W J; Von der Mey, M; Mi, Y; Mihul, A; Van Mil, A J W; Mirabelli, G; Mnich, J; Molnár, P; Monteleoni, B; Moore, R; Morganti, S; Moulik, T; Mount, R; Müller, S; Muheim, F; Muijs, A J M; Nahn, S; Napolitano, M; Nessi-Tedaldi, F; Newman, H; Niessen, T; Nippe, A; Nisati, A; Nowak, H; Oh, Yu D; Opitz, H; Organtini, G; Ostonen, R; Palomares, C; Pandoulas, D; Paoletti, S; Paolucci, P; Park, H K; Park, I H; Pascale, G; Passaleva, G; Patricelli, S; Paul, T; Pauluzzi, M; Paus, C; Pauss, Felicitas; Peach, D; Pei, Y J; Pensotti, S; Perret-Gallix, D; Petersen, B; Petrak, S; Pevsner, A; Piccolo, D; Pieri, M; Pinto, J C; Piroué, P A; Pistolesi, E; Plyaskin, V; Pohl, M; Pozhidaev, V; Postema, H; Produit, N; Prokofev, D; Prokofiev, D O; Rahal-Callot, G; Raja, N; Rancoita, P G; Rattaggi, M; Raven, G; Razis, P A; Read, K; Ren, D; Rescigno, M; Reucroft, S; Van Rhee, T; Riemann, S; Riles, K; Robohm, A; Rodin, J; Roe, B P; Romero, L; Rosier-Lees, S; Rosselet, P; Van Rossum, W; Roth, S; Rubio, Juan Antonio; Ruschmeier, D; Rykaczewski, H; Salicio, J; Sánchez, E; Sanders, M P; Sarakinos, M E; Sarkar, S; Sassowsky, M; Sauvage, G; Schäfer, C; Shchegelskii, V; Schmidt-Kärst, S; Schmitz, D; Schmitz, P; Schneegans, M; Scholz, N; Schopper, Herwig Franz; Schotanus, D J; Schwenke, J; Schwering, G; Sciacca, C; Sciarrino, D; Servoli, L; Shevchenko, S; Shivarov, N; Shoutko, V; Shukla, J; Shumilov, E; Shvorob, A V; Siedenburg, T; Son, D; Sopczak, André; Soulimov, V; Smith, B; Spillantini, P; Steuer, M; Stickland, D P; Stone, H; Stoyanov, B; Strässner, A; Strauch, K; Sudhakar, K; Sultanov, G G; Sun, L Z; Susinno, G F; Suter, H; Swain, J D; Tang, X W; Tauscher, Ludwig; Taylor, L; Ting, Samuel C C; Ting, S M; Tonutti, M; Tonwar, S C; Tóth, J; Tully, C; Tuchscherer, H; Tung, K L; Uchida, Y; Ulbricht, J; Uwer, U; Valente, E; Van de Walle, R T; Vesztergombi, G; Vetlitskii, I; Viertel, Gert M; Vivargent, M; Völkert, R; Vogel, H; Vogt, H; Vorobev, I; Vorobyov, A A; Vorvolakos, A; Wadhwa, M; Wallraff, W; Wang, J C; Wang, X L; Wang, Z M; Weber, A; Wittgenstein, F; Wu, S X; Wynhoff, S; Xu, J; Xu, Z Z; Yang, B Z; Yang, C G; Yao, X Y; Ye, J B; Yeh, S C; You, J M; Zalite, A; Zalite, Yu; Zemp, P; Zeng, Y; Zhang, Z; Zhang, Z P; Zhou, B; Zhou, Y; Zhu, G Y; Zhu, R Y; Zichichi, Antonino; Ziegler, F

    1997-01-01

    A study of resonance formation is presented in the $\\pi^+\\pi^-\\pi^0$ final state in two-photon collisions at LEP. The $a_2(1320)$ radiative width is measured to be $\\Gamma_{\\gamma\\gamma}=0.98\\pm0.05\\pm0.09$ keV{}. The helicity 2 production is dominant. Exclusive $\\pi^+\\pi^-\\pi^0$ production has also been studied in the mass region above the $a_2$ in the $\\rho\\pi$ and $f_2\\pi$ channels. This region is dominated by a $\\rm J^P$=$2^+$ helicity 2 wave.

  3. Free electron laser induced two-photon photoconductivity in Hg1-xCdxTe

    Institute of Scientific and Technical Information of China (English)

    2001-01-01

    The Beijing free electron laser (BFEL) has been employed for the first time to study the nonlinear photoconductivity characteristics of the typical infrared photoelectronic material Hg1-xCdxTe. Taking advantage of the high photon flux density of BFEL, we have investigated the photoconductivity characteristics in Hg1-xCdxTe induced by two-photon absorption by means of the photoconductivity technique, observed the photoconductivity signals saturation, and studied the two-photon photoconductivity characteristics on different bias voltages across the sample.

  4. Resonant transfer of one- and two-photon excitations in quantum dot-bacteriorhodopsin complexes

    Science.gov (United States)

    Krivenkov, V. A.; Samokhvalov, P. S.; Bilan, R. S.; Chistyakov, A. A.; Nabiev, I. R.

    2017-01-01

    Light-sensitive protein bacteriorhodopsin (BR), which is capable of electrical response upon exposure to light, is a promising material for photovoltaics and optoelectronics. However, the rather narrow absorption spectrum of BR does not allow achieving efficient conversion of the light energy in the blue and infrared spectral regions. This paper summarizes the results of studies showing the possibility of extending the spectral region of the BR function by means of the Förster resonance energy transfer (FRET) from CdSe/ZnS quantum dots (QDs), which have a broad spectrum of one-photon absorption and a large twophoton absorption cross section (TPACS), to BR upon one- and two-photon excitation. In particular, it is shown that, on the basis of QDs and BR-containing purple membranes, it is possible to create electrostatically associated bio-nano hybrid systems in which FRET is implemented. In addition, the large TPACS of QDs, which is two orders of magnitude larger than those of BR and organic dyes, opens up a means for selective two-photon excitation of synthesized bio-nano hybrid complexes. On the basis of the results of this work, the spectral region in which BR converts the light energy into electrical energy can be extended from the UV to near-IR region, creating new opportunities for the use of this material in photovoltaics and optoelectronics.

  5. Resonance Two-Photon Ionization of Diarylethene in the Presence of Cyclodextrin

    Directory of Open Access Journals (Sweden)

    Michihiro Hara

    2013-01-01

    Full Text Available The transient absorption of the diarylethene 1,2-bis(2,4-dimethyl-5-phenyl-3-thienyl-3,3,4,4,5,5-hexafluoro-1-cyclopentene (DE was measured using 266 nm laser flash photolysis in the presence of various cyclodextrins (CDs in aqueous solvent. Ionization of DE occurred within the laser flash (5 ns to give the DE radical cation and water-solvated electron. The electron was generated by two-photon excitation through simultaneous irradiation with 266 nm laser light, and the ionization quantum yields of DE in the presence of α-CD, β-CD, m-β-CD, and γ-CD depended on the properties of the DE/CD complexes. These results suggest that useful two-photon ionization occurred for these complexes. The ionization quantum yield of DE was found to increase in aqueous solution after the addition of m-β-CD (50 mM, in which m-β-CD likely controlled the photochromic reactivity of DE.

  6. Efficient photoionization for barium ion trapping using a dipole-allowed resonant two-photon transition

    CERN Document Server

    Leschhorn, G; Schaetz, T

    2011-01-01

    Two efficient and isotope-selective resonant two-photon ionization techniques for loading barium ions into radio-frequency (RF)-traps are demonstrated. The scheme of using a strong dipole-allowed transition at \\lambda=553 nm as a first step towards ionization is compared to the established technique of using a weak intercombination line (\\lambda=413 nm). An increase of two orders of magnitude in the ionization efficiency is found favoring the transition at 553 nm. This technique can be implemented using commercial all-solid-state laser systems and is expected to be advantageous compared to other narrowband photoionization schemes of barium in cases where highest efficiency and isotope-selectivity are required.

  7. Resonant two-photon ionization spectroscopy of Al atoms and dimers solvated in helium nanodroplets

    Energy Technology Data Exchange (ETDEWEB)

    Krasnokutski, Serge A.; Huisken, Friedrich [Laboratory Astrophysics Group of the Max Planck Institute for Astronomy at the Friedrich Schiller University Jena, Institute of Solid State Physics, Helmholtzweg 3, D-07743 Jena (Germany)

    2015-02-28

    Resonant two-photon ionization (R2PI) spectroscopy has been applied to investigate the solvation of Al atoms in helium droplets. The R2PI spectra reveal vibrational progressions that can be attributed to Al–He{sub n} vibrations. It is found that small helium droplets have very little chance to pick up an aluminum atom after collision. However, the pick-up probability increases with the size of the helium droplets. The absorption band that is measured by monitoring the ions on the mass of the Al dimer is found to be very little shifted with respect to the Al monomer band (∼400 cm{sup −1}). However, using the same laser wavelength, we were unable to detect any Al{sub n} photoion with n larger than two.

  8. Resonant two-photon ionization spectroscopy of Al atoms and dimers solvated in helium nanodroplets.

    Science.gov (United States)

    Krasnokutski, Serge A; Huisken, Friedrich

    2015-02-28

    Resonant two-photon ionization (R2PI) spectroscopy has been applied to investigate the solvation of Al atoms in helium droplets. The R2PI spectra reveal vibrational progressions that can be attributed to Al-He(n) vibrations. It is found that small helium droplets have very little chance to pick up an aluminum atom after collision. However, the pick-up probability increases with the size of the helium droplets. The absorption band that is measured by monitoring the ions on the mass of the Al dimer is found to be very little shifted with respect to the Al monomer band (∼400 cm(-1)). However, using the same laser wavelength, we were unable to detect any Al(n) photoion with n larger than two.

  9. In vivo reactive neural plasticity investigation by means of correlative two photon: electron microscopy

    Science.gov (United States)

    Allegra Mascaro, A. L.; Cesare, P.; Sacconi, L.; Grasselli, G.; Mandolesi, G.; Maco, B.; Knott, G.; Huang, L.; De Paola, V.; Strata, P.; Pavone, F. S.

    2013-02-01

    In the adult nervous system, different populations of neurons correspond to different regenerative behavior. Although previous works showed that olivocerebellar fibers are capable of axonal regeneration in a suitable environment as a response to injury1, we have hitherto no details about the real dynamics of fiber regeneration. We set up a model of singularly axotomized climbing fibers (CF) to investigate their reparative properties in the adult central nervous system (CNS) in vivo. Time lapse two-photon imaging has been combined to laser nanosurgery2, 3 to define a temporal pattern of the degenerative event and to follow the structural rearrangement after injury. To characterize the damage and to elucidate the possible formation of new synaptic contacts on the sprouted branches of the lesioned CF, we combined two-photon in vivo imaging with block face scanning electron microscopy (FIB-SEM). Here we describe the approach followed to characterize the reactive plasticity after injury.

  10. Single & Two-photon Excited Fluorescence of Two New Compounds with 2-Benzothiazolyl as Electron Acceptor

    Institute of Scientific and Technical Information of China (English)

    2003-01-01

    Two new D-π-A type compounds, where electron-donor D is tertiary amino group, electron-acceptor A is 2-benzothiazolyl and π is two conjugated styryl units, have been synthesized.They are named as trans, trans-2-{4-[4-(N, N-diethylamino)styryl]styryl}-1, 3-benzothiazole and trans, trans-2-{4-[4-(N, N-diphenylamino)styryl]styryl}-1, 3-benzothiazole.Both compounds show strong two-photon excited fluorescence in yellow-orange region when excited by a femtosecond laser at 800 nm.

  11. Polarization control efficiency manipulation in resonance-mediated two-photon absorption by femtosecond spectral frequency modulation

    Science.gov (United States)

    Yao, Yunhua; Cheng, Wenjing; Zheng, Ye; Xu, Cheng; Liu, Pei; Jia, Tianqing; Qiu, Jianrong; Sun, Zhenrong; Zhang, Shian

    2017-04-01

    The femtosecond laser polarization modulation is considered as a very simple and efficient method to control the multi-photon absorption process. In this work, we theoretically and experimentally show that the polarization control efficiency in the resonance-mediated two-photon absorption can be artificially manipulated by modulating the femtosecond spectral frequency components. We theoretically demonstrate that the on- and near-resonant parts in the resonance-mediated two-photon absorption process depend on the different femtosecond spectral frequency components, and therefore their contributions in the whole excitation process can be controlled by properly designing the femtosecond spectral frequency components. The near-resonant two-photon absorption is correlated with the femtosecond laser polarization while the on-resonant two-photon absorption is independent of it, and thus the polarization control efficiency in the resonance-mediated two-photon absorption can be manipulated by the femtosecond spectral frequency modulation. We experimentally verify these theoretical results by performing the laser polarization control experiment in the Dy3+-doped glass sample under the modulated femtosecond spectral frequency components, and the experimental results show that the polarization control efficiency can be increased when the central spectral frequency components are cut off, while it is decreased when both the low and high spectral frequency components are cut off, which is in good agreement with the theoretical predictions. Our works can provide a feasible pathway to understand and control the resonance-mediated multi-photon absorption process under the femtosecond laser field excitation, and also may open a new opportunity to the related application areas.

  12. Electron correlation in two-photon double ionization of helium from attosecond to FEL pulses

    Energy Technology Data Exchange (ETDEWEB)

    Collins, Lee [Los Alamos National Laboratory

    2009-01-01

    We investigate the role of electron correlation in the two-photon double ionization of helium for ultrashort pulses in the extreme ultraviolet (XUV) regime with durations ranging from a hundred attoseconds to a few femtoseconds. We perform time-dependent ab initio calculations for pulses with mean frequencies in the so-called 'sequential' regime ({Dirac_h}{omega} > 54.4 eV). Electron correlation induced by the time correlation between emission events manifests itself in the angular distribution of the ejected electrons, which strongly depends on the energy sharing between them. We show that for ultrashort pulses two-photon double ionization probabilities scale non-uniformly with pulse duration depending on the energy sharing between the electrons. Most interestingly we find evidence for an interference between direct ('nonsequential') and indirect ('sequential') double photoionization with intermediate shake-up states, the strength of which is controlled by the pulse duration. This observation may provide a route towards measuring the pulse duration of x-ray free-electron laser (XFEL) pulses.

  13. Two-photon photoemission study of the coverage-dependent electronic structure of chemisorbed alkali atoms on a Ag(111) surface.

    Science.gov (United States)

    Wang, Lei-Ming; Sametoglu, Vahit; Winkelmann, Aimo; Zhao, Jin; Petek, Hrvoje

    2011-09-01

    We report a systematic investigation of the electronic structure of chemisorbed alkali atoms (Li-Cs) on a Ag(111) surface by two-photon photoemission spectroscopy. Angle-resolved two-photon photoemission spectra are obtained for 0-0.1 monolayer coverage of alkali atoms. The interfacial electronic structure as a function of periodic properties and the coverage of alkali atoms is observed and interpreted assuming ionic adsorbate/substrate interaction. The energy of the alkali atom σ-resonance at the limit of zero coverage is primarily determined by the image charge interaction, whereas at finite alkali atom coverages, it follows the formation of a dipolar surface field. The coverage- and angle-dependent two-photon photoemission spectra provide information on the photoinduced charge-transfer excitation of adsorbates on metal surfaces. This work complements the previous work on alkali/Cu(111) chemisorption [Phys. Rev. B 2008, 78, 085419].

  14. Spectral distribution of the 2 → 1 two-photon transition in atoms and few-electron ions

    Indian Academy of Sciences (India)

    Ajay Kumar; S Trotsenko; A V Volotka; D Banaś; H F Beyer; H Bräuning; S Fritzsche; A Gumberidze; S Hagmann; S Hess; C Kozhuharov; R Reuschl; U Spillmann; M Trassinelli; G Weber; Th Stöhlker

    2011-02-01

    The two-photon decay of the 2 state to the ground state in dressed atoms and oneor two-electron ions has been studied for several decades. Relativistic calculations have shown an -dependence of the spectral shape of this two-photon transition in one- or two-electron ions. We have measured the spectral distribution of the 121 0 → 12 1 0 two-photon transition in He-like tin at the ESR storage ring using a new approach for such experiments. In this method, relativistic collisions of initially Li-like projectiles with a gaseous target were used to populate exclusively the first excited state, 12, of He-like tin, which provided a clean two-photon spectrum. The measured two-photon spectral distribution was compared with fully relativistic calculations. The obtained results show very good agreement with the calculations for He-like tin

  15. In situ electrical and thermal monitoring of printed electronics by two-photon mapping.

    Science.gov (United States)

    Pastorelli, Francesco; Accanto, Nicolò; Jørgensen, Mikkel; van Hulst, Niek F; Krebs, Frederik C

    2017-06-19

    Printed electronics is emerging as a new, large scale and cost effective technology that will be disruptive in fields such as energy harvesting, consumer electronics and medical sensors. The performance of printed electronic devices relies principally on the carrier mobility and molecular packing of the polymer semiconductor material. Unfortunately, the analysis of such materials is generally performed with destructive techniques, which are hard to make compatible with in situ measurements, and pose a great obstacle for the mass production of printed electronics devices. A rapid, in situ, non-destructive and low-cost testing method is needed. In this study, we demonstrate that nonlinear optical microscopy is a promising technique to achieve this goal. Using ultrashort laser pulses we stimulate two-photon absorption in a roll coated polymer semiconductor and map the resulting two-photon induced photoluminescence and second harmonic response. We show that, in our experimental conditions, it is possible to relate the total amount of photoluminescence detected to important material properties such as the charge carrier density and the molecular packing of the printed polymer material, all with a spatial resolution of 400 nm. Importantly, this technique can be extended to the real time mapping of the polymer semiconductor film, even during the printing process, in which the high printing speed poses the need for equally high acquisition rates.

  16. Free electron laser induced two-photon photoconductivity in Hg1-xCdxTe

    Institute of Scientific and Technical Information of China (English)

    YUAN; Xianzhang

    2001-01-01

    [1]Nathan, V., Guenther, A. H., Mitra, S. S., Review of multiphoton absortion in crystalline solids, J. Opt. Soc. Am. B, 1985, 2: 294—316.[2]Gibson, A. F., Hatch, C. B., Maggs, P. N. D. et al., Two-photon absorption in indium antimonide and germanium, J. Phys., C, 1976, 9: 3259—3275.[3]Miller, A., Johnston, A., Dempsey, J. et al., Two-photon absorption in InSb and Hg1-xCdxTe, J. Phys. C, 1929, 12: 4839—4849.[4]Burghoorn, J., Anderegg, V. F., Klaassen, T. O. et al., Free electron laser induced two-photon absorption in Hg1-xCdxTe, Appl. Phys. Lett., 1992, 61(19): 2320—2322.[5]Hui, Z. X., Yang, Z. H., Free Electron Laser (in Chinese), Beijing: National Defense Industry Press, 1995, 7—8.[6]Matter, J. C., Smirt, A. L., Scully, M. O., Saturable transmission in mercury cadmium telluride, Appl. Phys. Lett., 1976, 28(9): 507—509.[7]Nurmikko, A. V., Nonlinear absorption at 10.6 μm in Hg1-xCdxTe, Optics Communications, 1976, 18(4): 522—524.[8]Catalano, I. M., Cingolani, A., Minafra, A., Multiphoton transitions in ionic crystals, Phys. Rev. B, 1972, 5(4): 1629—1632.[9]Blakemore, J. S., Semiconductor Statistics, Oxford: Pergamon, 1962, 221—222.[10]Shen, S. C., Optical Property of Semiconductor (in Chinese), Beijing: Science Press, 1992, 392—394.

  17. Observation of Rydberg Series in Sodium Vapour by Two-Photon Resonant Nondegenerate Four-Wave Mixing

    Institute of Scientific and Technical Information of China (English)

    王延帮; 姜谦; 李隆; 米辛; 俞祖和; 傅盘铭

    2001-01-01

    We apply two-photon resonant nondegenerate four-wave mixing with a resonant intermediate state for the obser- vation of Rydberg states in sodium vapour. The broadening and shift of the sodium 3S- 11D transition perturbed by argon are investigated. This technique can achieve Doppler-free resolution of narrow spectral structures of Rydberg levels if lasers with narrow bandwidths are employed.

  18. Non-Liouvillean ion injection via resonantly enhanced two-photon ionization

    Directory of Open Access Journals (Sweden)

    B. A. Knyazev

    2004-03-01

    Full Text Available The charge-exchange method is now one of the main techniques for ion injection into accelerators and storage rings. The disadvantages of conventional methods, based on the atom or ion stripping in a material target, are emittance growth, energy straggling, and production of ions in many charge states. Recently suggested stripping methods based on direct photoionization require employment of hard-UV lasers, which still do not exist and must obviously be very bulky and expensive. An alternative method, suggested for injection of proton beams, employs excitation of the atom to 3p intermediate state with subsequent Lorentz ionization in a magnetic field gradient. This technique applies rigid requirements to laser characteristic and is not free of growing of the beam divergence. In this paper a variant of the stripping technique based on the resonantly enhanced two-photon ionization (RETPI is considered. The technique allows ionization of singly charged ions of the elements from helium to bismuth. A variant of the technique can be used for proton injection. RETPI can be applied for both ion injection and stacking, as well as for diagnostics of ion beam characteristics on the orbit. Stripping efficiency can be about 100% for the singly charged ions having the singlet ground state and decreases for the other ions. Special methods for “cleaning” unwanted atomic states in such ions, that can provide high stripping efficiency, are discussed. Excimer lasers with very moderate parameters can be employed for implementation of this technique for almost all elements. Numerical examples show that for most of the singly charged ions and for hydrogen atom necessary laser-beam energy density is merely 0.5–8  J/cm^{2} for a 1 m interaction region, and is 10 times higher for several light ions.

  19. Non-Liouvillean ion injection via resonantly enhanced two-photon ionization

    Science.gov (United States)

    Knyazev, B. A.

    2004-03-01

    The charge-exchange method is now one of the main techniques for ion injection into accelerators and storage rings. The disadvantages of conventional methods, based on the atom or ion stripping in a material target, are emittance growth, energy straggling, and production of ions in many charge states. Recently suggested stripping methods based on direct photoionization require employment of hard-UV lasers, which still do not exist and must obviously be very bulky and expensive. An alternative method, suggested for injection of proton beams, employs excitation of the atom to 3p intermediate state with subsequent Lorentz ionization in a magnetic field gradient. This technique applies rigid requirements to laser characteristic and is not free of growing of the beam divergence. In this paper a variant of the stripping technique based on the resonantly enhanced two-photon ionization (RETPI) is considered. The technique allows ionization of singly charged ions of the elements from helium to bismuth. A variant of the technique can be used for proton injection. RETPI can be applied for both ion injection and stacking, as well as for diagnostics of ion beam characteristics on the orbit. Stripping efficiency can be about 100% for the singly charged ions having the singlet ground state and decreases for the other ions. Special methods for “cleaning” unwanted atomic states in such ions, that can provide high stripping efficiency, are discussed. Excimer lasers with very moderate parameters can be employed for implementation of this technique for almost all elements. Numerical examples show that for most of the singly charged ions and for hydrogen atom necessary laser-beam energy density is merely 0.5 8 J/cm2 for a 1m interaction region, and is 10times higher for several light ions.

  20. Two-photon exchange corrections in elastic electron-proton scattering

    CERN Document Server

    Tomalak, O

    2016-01-01

    We apply a subtracted dispersion relation (DR) formalism with the aim to improve predictions for the two-photon exchange (TPE) corrections to elastic electron-proton scattering observables at small momentum transfers. We study the formalism on the elastic TPE contribution in comparison with existing data for unpolarized cross sections. We extend the general formalism of TPE to elastic scattering with massive lepton and perform a numerical estimate of the muon-proton scattering at low momentum transfer in view of the upcoming muon-proton scattering experiment (MUSE). We study the influence of the double-virtual Compton scattering (VVCS) subtraction function on the unpolarized lepton-proton scattering cross-section. We show that the resulting TPE correction is negligible in the electron-proton scattering and smaller than planned uncertainties of the MUSE experiment for the subtraction functions evaluated in chiral perturbation theory.

  1. One-colour resonant two-photon ionization spectrum of the 1-fluoronaphthalene dimer and ab initio calculation

    Institute of Scientific and Technical Information of China (English)

    Liu Ye-Chao; Zhang Shu-Dong; Zhang Ming-Xia; Sun Miao; Kong Xiang-He

    2009-01-01

    The one-colour resonant two-photon ionization (R2PI) spectrum of the 1-fluoronaphthalene (1FN) dimer has been studied in the wavelength range of 304 to 322 nm by using a supersonic molecular beam and time-of-flight mass spectrometry. Compared with the original band 000 (at 313.8 nm) of the S1 ← S0 transition of the 1FN monomer,a red-shifted band was observed in the 1FN dimer spectrum at about 315 nm with a relatively large linewidth,nearly 2 nm. Based on the consideration of inductive effect and ab initio calculations,this red-shifted band is assigned to the first electronic excited transition of the 1FN dimer. A possible geometric structure of the 1FN dimer is also obtained with calculations that the two 1FN molecules are combined through two hydrogen bonds which are formed between the hydrogen atom of a molecule and the fluorine atom of a neighbouring molecule. A time-dependent calculation was also carried out and the results are consistent with the experimental data.

  2. Suppression and Enhancement in Parametric Two-Photon Resonant Nondegenerate Four-Wave Mixing via Quantum Interference

    Institute of Scientific and Technical Information of China (English)

    SUN Jiang; MI Xin; YU Zu-He; JIANG Qian; ZUO Zhan-Chun; WANG Yan-Bang; WU Ling-An; FU Pan-Ming

    2004-01-01

    @@ Quantum interference may lead to suppression and enhancement of the two-photon resonant nondegenerate fourwave mixing signal in a cascade four-level system. Such phenomena are demonstrated in Ba through inducing atomic coherence between the ground state 6s2 and the doubly excited autoionizing Rydberg state 6pnd. This method can be used as a new spectroscopic tool for measuring the transition dipole moment between two highly excited atomic states.

  3. Peptide backbone orientation and dynamics in spider dragline silk and two-photon excitation in nuclear magnetic and quadrupole resonance

    Energy Technology Data Exchange (ETDEWEB)

    Eles, P.T

    2005-07-01

    In the first part of the dissertation, spider dragline silk is studied by solid state NMR techniques. The dependence of NMR frequency on molecular orientation is exploited using the DECODER experiment to determine the orientation of the protein backbone within the silk fibre. Practical experimental considerations require that the silk fibres be wound about a cylindrical axis perpendicular to the external magnetic field, complicating the reconstruction of the underlying orientation distribution and necessitating the development of numerical techniques for this purpose. A two-component model of silk incorporating static b-sheets and polyglycine II helices adequately fits the NMR data and suggests that the b-sheets are well aligned along the silk axis (20 FWHM) while the helices are poorly aligned (68 FWHM). The effects of fibre strain, draw rate and hydration on orientation are measured. Measurements of the time-scale for peptide backbone motion indicate that when wet, a strain-dependent fraction of the poorly aligned component becomes mobile. This suggests a mechanism for the supercontraction of silk involving latent entropic springs that undergo a local strain-dependent phase transition, driving supercontraction. In the second part of this dissertation a novel method is developed for exciting NMR and nuclear quadrupole resonance (NQR) by rf irradiation at multiple frequencies that sum to (or differ by) the resonance frequency. This is fundamentally different than traditional NMR experiments where irradiation is applied on-resonance. With excitation outside the detection bandwidth, two-photon excitation allows for detection of free induction signals during excitation, completely eliminating receiver dead-time. A theoretical approach to describing two-photon excitation is developed based on average Hamiltonian theory. An intuition for two-photon excitation is gained by analogy to the coherent absorption of multiple photons requiring conservation of total energy and

  4. A study of Two Photon Decays of Charmonium Resonances Formed in Proton Anti-Proton Annihilations

    Energy Technology Data Exchange (ETDEWEB)

    Pedlar, Todd Kristofer [Northwestern Univ., Evanston, IL (United States)

    1999-06-01

    In this dissertation we describe the results of an investigation of the production of charmonium states (ηc, η'c, χ0 and χ2) in Fermilab experiment E835 via antiproton-proton annihilation and their detection via their decay into two photons.

  5. Two-photon approximation in the theory of the electron recombination in hydrogen

    OpenAIRE

    Solovyev, D.; Labzowsky, L.

    2010-01-01

    A rigorous QED theory of the multiphoton decay of excited states in hydrogen atom is presented. The "two-photon" approximation is formulated which is limited by the one-photon and two-photon transitions including cascades transitions with two-photon links. This may be helpful for the strict description of the recombination process in hydrogen atom and, in principle, for the history of the hydrogen recombination in the early Universe.

  6. Proton form factors and two-photon exchange in elastic electron-proton scattering

    Energy Technology Data Exchange (ETDEWEB)

    Nikolenko, D. M., E-mail: D.M.Nikolenko@inp.nsk.su [Russian Academy of Sciences, Budker Institute of Nuclear Physics, Siberian Branch (Russian Federation); Arrington, J. [Argonne National Laboratory (United States); Barkov, L. M. [Russian Academy of Sciences, Budker Institute of Nuclear Physics, Siberian Branch (Russian Federation); Vries, H. de [NIKHEF (Netherlands); Gauzshtein, V. V. [National Research Tomsk Polytechnic University, Physical-Technical Institute (Russian Federation); Golovin, R. A.; Gramolin, A. V.; Dmitriev, V. F.; Zhilich, V. N.; Zevakov, S. A.; Kaminsky, V. V.; Lazarenko, B. A.; Mishnev, S. I.; Muchnoi, N. Yu.; Neufeld, V. V.; Rachek, I. A.; Sadykov, R. Sh. [Russian Academy of Sciences, Budker Institute of Nuclear Physics, Siberian Branch (Russian Federation); Stibunov, V. N. [National Research Tomsk Polytechnic University, Physical-Technical Institute (Russian Federation); Toporkov, D. K. [Russian Academy of Sciences, Budker Institute of Nuclear Physics, Siberian Branch (Russian Federation); Holt, R. J. [Argonne National Laboratory (United States); and others

    2015-05-15

    Proton electromagnetic form factors are among the most important sources of information about the internal structure of the proton. Two different methods for measuring these form factors, the method proposed by Rosenbluth and the polarization-transfer method, yield contradictory results. It is assumed that this contradiction can be removed upon taking into account the hard part of the contribution of two-photon exchange to the cross section for elastic electron-proton scattering. This contribution can measured experimentally via a precision comparison of the cross sections for the elastic scattering of positrons and electrons on protons. Such a measurement, performed at the VEPP-3 storage ring in Novosibirsk at the beam energies of 1.6 and 1.0 GeV for positron (electron) scattering angles in the ranges of θ{sub e} = 15°–25° and 55°–75° in the first case and in the range of θ{sub e} = 65°–105° in the second case is described in the present article. Preliminary results of this experiment and their comparison with theoretical predictions are described.

  7. Resonantly-enhanced two-photon ionization and mass-analyzed threshold ionization (MATI) spectroscopy of 2-hydroxypyridine

    CERN Document Server

    Lee, D H; Choi, K W; Choi, Y S; Kim, S K

    2002-01-01

    Mass-analyzed threshold ionization (MATI) spectra of 2-hydroxypyridines existing as lactims (2-pyridionl) in a molecular beam are obtained via (1+1') two-photon process to give accurate ionization energies of 8.9344 +- 0.0005 and 8.9284 +- 0.0005 eV for 2-pyridinol (2Py-OH) and its deuterated analogue (2Py-OD), respectively. Resonantly-enhanced two-photon ionization spectra of these compounds are also presented to give vibrational structures of their S sub 1 states. Vibrational frequencies of 2Py-OH and 2Py-OD in ionic ground states are accurately determined from MATI spectra taken via various S sub 1 intermediate states, and associated vibrational modes are assigned with the aid of ab initio calculations.

  8. ARTICLES: A Surface Femtosecond Two-Photon Photoemission Spectrometer for Excited Electron Dynamics and Time-Dependent Photochemical Kinetics

    Science.gov (United States)

    Ren, Ze-feng; Zhou, Chuan-yao; Ma, Zhi-bo; Xiao, Chun-lei; Mao, Xin-chun; Dai, Dong-xu; LaRue, Jerry; Cooper, Russell; Wodtke, Alec M.; Yang, Xue-ming

    2010-06-01

    A surface femtosecond two-photon photoemission (2PPE) spectrometer devoted to the study of ultrafast excited electron dynamics and photochemical kinetics on metal and metal oxide surfaces has been constructed. Low energy photoelectrons are measured using a hemispherical electron energy analyzer with an imaging detector that allows us to detect the energy and the angular distributions of the photoelectrons simultaneously. A Mach-Zehnder interferometer was built for the time-resolved 2PPE (TR-2PPE) measurement to study ultrafast surface excited electron dynamics, which was demonstrated on the Cu(111) surface. A scheme for measuring time-dependent 2PPE (TD-2PPE) spectra has also been developed for studies of surface photochemistry. This technique has been applied to a preliminary study on the photochemical kinetics on ethanol/TiO2(110). We have also shown that the ultrafast dynamics of photoinduced surface excited resonances can be investigated in a reliable way by combining the TR-2PPE and TD-2PPE techniques.

  9. Test of theoretical models for ultrafast heterogeneous electron transfer with femtosecond two-photon photoemission data

    Indian Academy of Sciences (India)

    Lars Gundlach; Tobias Letzig; Frank Willig

    2009-09-01

    The energy distribution of electrons injected into acceptor states on the surface of TiO2 was measured with femtosecond two-photon photoemission. Shape and relative energetic position of these distribution curves with respect to the corresponding donor states, i.e. of perylene chromophores in the first excited singlet state attached via different bridge-anchor groups to the TiO2 surface, were compared with the predictions of different theoretical models for light-induced ultrafast heterogeneous electron transfer (HET). Gerischer’s early scenario for light-induced HET was considered and two recent explicit calculations, i.e. a fully quantum mechanical analytical model and a time-dependent density functional theory model based on molecular dynamics simulations for the vibrational modes were also considered. Based on the known vibrational structure in the photoionization spectrum of perylene in the gas phase and that measured in the linear absorption spectra of the perylene chromophores anchored on the TiO2 surface the energy distribution curves for the injected electrons were fitted assuming the excitation of the dominant 0.17 eV vibrational mode in the ionized perylene chromophore leading to a corresponding Franck-Condon dictated progression in the energy distribution curves. Each individual peak was fitted with a Voigt profile where the Lorentzian contribution was taken from the time-resolved HET data and the Gaussian contribution attributed to inhomogeneous broadening. The measured room temperature energy distribution curves for the injected electrons are explained with the fully quantum mechanical model for light-induced HET with the high energy, 0.17 eV, skeletal stretching mode excited in the ionized perylene chromophore. The corresponding energy distribution of the injected electrons is fully accommodated in acceptor states on the TiO2 surface fulfilling the wide band limit.

  10. Electron correlations and two-photon states in polycyclic aromatic hydrocarbon molecules: A peculiar role of geometry

    Energy Technology Data Exchange (ETDEWEB)

    Aryanpour, Karan [Department of Physics, University of Arizona, Tucson, Arizona 85721 (United States); Shukla, Alok [Department of Physics, Indian Institute of Technology, Powai, Mumbai 400076 (India); Mazumdar, Sumit [Department of Physics, University of Arizona, Tucson, Arizona 85721 (United States); College of Optical Sciences, University of Arizona, Tucson, Arizona 85721 (United States)

    2014-03-14

    We present numerical studies of one- and two-photon excited states ordering in a number of polycyclic aromatic hydrocarbon molecules: coronene, hexa-peri-hexabenzocoronene, and circumcoronene, all possessing D{sub 6h} point group symmetry versus ovalene with D{sub 2h} symmetry, within the Pariser-Parr-Pople model of interacting π-electrons. The calculated energies of the two-photon states as well as their relative two-photon absorption cross-sections within the interacting model are qualitatively different from single-particle descriptions. More remarkably, a peculiar role of molecular geometry is found. The consequence of electron correlations is far stronger for ovalene, where the lowest spin-singlet two-photon state is a quantum superposition of pairs of lowest spin triplet states, as in the linear polyenes. The same is not true for D{sub 6h} group hydrocarbons. Our work indicates significant covalent character, in valence bond language, of the ground state, the lowest spin triplet state and a few of the lowest two-photon states in D{sub 2h} ovalene but not in those with D{sub 6h} symmetry.

  11. Electron correlations and two-photon states in polycyclic aromatic hydrocarbon molecules: A peculiar role of geometry

    Science.gov (United States)

    Aryanpour, Karan; Shukla, Alok; Mazumdar, Sumit

    2014-03-01

    We present numerical studies of one- and two-photon excited states ordering in a number of polycyclic aromatic hydrocarbon molecules: coronene, hexa-peri-hexabenzocoronene, and circumcoronene, all possessing D6h point group symmetry versus ovalene with D2h symmetry, within the Pariser-Parr-Pople model of interacting π-electrons. The calculated energies of the two-photon states as well as their relative two-photon absorption cross-sections within the interacting model are qualitatively different from single-particle descriptions. More remarkably, a peculiar role of molecular geometry is found. The consequence of electron correlations is far stronger for ovalene, where the lowest spin-singlet two-photon state is a quantum superposition of pairs of lowest spin triplet states, as in the linear polyenes. The same is not true for D6h group hydrocarbons. Our work indicates significant covalent character, in valence bond language, of the ground state, the lowest spin triplet state and a few of the lowest two-photon states in D2h ovalene but not in those with D6h symmetry.

  12. Theory of deep ultraviolet generation at maximum coherence assisted by Stark-chirped two-photon resonance

    CERN Document Server

    Myslivets, S A; Kimberg, V V; George, T F; George, Thomas F.

    2003-01-01

    A scheme is analyzed for effcient generation of vacuum ultraviolet radiation through four-wave mixing processes assisted by the technique of Stark-chirped rapid adiabatic passage. These opportunities are associated with pulse excitation of laddertype short-wavelength two-photon atomic or molecular transitions so that relaxation processes can be neglected. In this three-laser technique, a delayed-pulse of strong oR-resonant infrared radiation sweeps the laser-induced Stark-shift of a two-photon transition in a such way that facilitates robust maximum two-photon coherence induced by the first ultraviolet laser. A judiciously delayed third pulse scatters at this coherence and generates short-wavelength radiation. A theoretical analysis of these problems based on the density matrix is performed. A numerical model is developed to carry out simulations of a typical experiment. The results illustrate a behavior of populations, coherence and generated radiation along the medium as well as opportunities of effcient ge...

  13. Investigation of some Rydberg states of ketene by two-photon resonance-enhanced multiphoton ionization spectroscopy

    Science.gov (United States)

    Wang, Shiliang; Shi, Yujun; Dénommée, Stéphane; Simard, Benoit; Lee, Yuan-Pern

    2003-10-01

    Rydberg states of CH2CO and CD2CO in the 54 000-72 000 cm-1 spectral range have been reinvestigated using two-photon resonance-enhanced multiphoton-ionization spectroscopy. Improved resolution and sensitivity has allowed for identifications of more Rydberg states than in previous work. Based on an analysis of rotational structures and quantum defects and a comparison with the results of theoretical calculations, transitions to the 3pz, 4py, 4pz, and 5py, three components of 4d, and two components of 4f Rydberg states with a ground-state ionic core (X˜ 2B1) are identified. Several transitions have been reassigned. Vibrational wave numbers indicate that the geometry of the [X˜ 2B1]3py(1A2) state is almost identical to that of the corresponding cation in its ground electronic state, with C2v symmetry, whereas that of the [X˜ 2B1]3px(1A1) state differs significantly from those of the neutral molecule and the cation in their ground states, consistent with previous quantum chemical calculations that indicated that the [X˜ 2B1]3px(1A1) state has Cs symmetry. The energy ordering of the three components of the 3p Rydberg states is found to be 3pxout-of-plane bending, CH2 or CD2 wagging) and b2 symmetries (e.g., C=C=O in-plane bending) are observed in several Rydberg states of CH2CO and CD2CO.

  14. Relaxation Process of Excitonic Molecules in CuCl under the Two-Photon Resonant Excitation. II. Transverse Relaxation

    Science.gov (United States)

    Itoh, Tadashi; Katohno, Takashi; Kirihara, Toshio; Ueta, Masayasu

    1984-02-01

    Under the off-resonant excitation at the slightly higher energy side of the giant two-photon absorption band (GTA) for the direct generation of excitonic molecules (EM) in CuCl, new narrow emission bands designated as XT and XL have been found in the energy region of the MT and ML broad bands, respectively. Their photon energies increase with the decrease of the pump photon energy from the higher-energy side of the resonance and finally, at the on-resonant excitation, their bands merge into MT0 and ML0 bands, respectively, previously reported by Mita et al. Based on the detailed studies on these bands, it is found that there exists a certain kind of transverse relaxation process which acts on the EM just after their generation by the GTA and brings about the X emission as a hot luminescence.

  15. Resonant metallic nanostructure for enhanced two-photon absorption in a thin GaAs p-i-n diode

    Energy Technology Data Exchange (ETDEWEB)

    Portier, Benjamin; Pardo, Fabrice; Péré-Laperne, Nicolas; Steveler, Emilie; Dupuis, Christophe; Bardou, Nathalie; Lemaître, Aristide; Pelouard, Jean-Luc, E-mail: jean-luc.pelouard@lpn.cnrs.fr [Laboratoire de Photonique et de Nanostructures (LPN-CNRS), Route de Nozay, 91460 Marcoussis (France); Vest, Benjamin; Jaeck, Julien; Rosencher, Emmanuel [ONERA The French Aerospace Lab, Chemin de la Hunière, F-91760 Palaiseau (France); Haïdar, Riad [ONERA The French Aerospace Lab, Chemin de la Hunière, F-91760 Palaiseau (France); École Polytechnique, Département de Physique, F-91128 Palaiseau (France)

    2014-07-07

    Degenerate two-photon absorption (TPA) is investigated in a 186 nm thick gallium arsenide (GaAs) p-i-n diode embedded in a resonant metallic nanostructure. The full device consists in the GaAs layer, a gold subwavelength grating on the illuminated side, and a gold mirror on the opposite side. For TM-polarized light, the structure exhibits a resonance close to 1.47 μm, with a confined electric field in the intrinsic region, far from the metallic interfaces. A 109 times increase in photocurrent compared to a non-resonant device is obtained experimentally, while numerical simulations suggest that both gain in TPA-photocurrent and angular dependence can be further improved. For optimized grating parameters, a maximum gain of 241 is demonstrated numerically and over incidence angle range of (−30°; +30°).

  16. Polarization Effects in Two-Photon Free-Free Transitions in Laser-Assisted Electron-Hydrogen Collisions

    CERN Document Server

    Cionga, Aurelia

    2013-01-01

    Two-photon free-free transitions in elastic laser-assisted electron-hydrogen collisions are studied in the domain of high scattering energies and low or moderate field intensities, in the third order of perturbation theory, taking into account all the involved Feynman diagrams. Based on the analytical expressions of the transition amplitudes, the differential cross sections for two-photon absorption/emission are computed at impact energy $E_i=100$ eV. The effect of field polarizations on the angular distribution and on the frequency dependence of the differential cross section is analyzed.

  17. Subtracted dispersion relation formalism for the two-photon exchange correction to elastic electron-proton scattering: Comparison with data

    Energy Technology Data Exchange (ETDEWEB)

    Tomalak, O. [Johannes Gutenberg Universitaet, Institut fuer Kernphysik, Mainz (Germany); Johannes Gutenberg-Universitaet, PRISMA Cluster of Excellence, Mainz (Germany); Taras Shevchenko National University of Kyiv, Department of Physics, Kyiv (Ukraine); Vanderhaeghen, M. [Johannes Gutenberg Universitaet, Institut fuer Kernphysik, Mainz (Germany); Johannes Gutenberg-Universitaet, PRISMA Cluster of Excellence, Mainz (Germany)

    2015-02-01

    We apply a subtracted dispersion relation formalism with the aim to improve predictions for the two-photon exchange corrections to elastic electron-proton scattering observables at finite momentum transfers. We study the formalism on the elastic contribution, and make a detailed comparison with existing data for unpolarized cross sections as well as polarization transfer observables. (orig.)

  18. Antiproton–to–electron mass ratio determined by two-photon laser spectroscopy of antiprotonic helium atoms

    Directory of Open Access Journals (Sweden)

    Sótér A.

    2014-03-01

    Full Text Available The ASACUSA collaboration of CERN has recently carried out two-photon laser spectroscopy of antiprotonic helium atoms. Three transition frequencies were determined with fractional precisions of 2.3–5 parts in 109. By comparing the results with three-body QED calculations, the antiproton-to-electron mass ratio was determined as 1836.1526736(23.

  19. Watching Electrons Transfer from Metals to Insulators using Two Photon Photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Johns, James E. [Univ. of California, Berkeley, CA (United States)

    2010-05-01

    Ultrafast angle-resolved two photon photoemission was used to study the dynamics and interfacial band structure of ultrathin films adsorbed onto Ag(111). Studies focused on the image potential state (IPS) in each system as a probe for measuring changes in electronic behavior in differing environments. The energetics and dynamics of the IPS at the toluene/Ag(111) interface are strongly dependent upon coverage. For a single monolayer, the first IPS is bound by 0.81 eV below the vacuum level and has a lifetime of 50 femtoseconds (fs). Further adsorption of toluene creates islands of toluene with an exposed wetting layer underneath. The IPS is then split into two peaks, one corresponding to the islands and one corresponding to the monolayer. The wetting layer IPS shows the same dynamics as the monolayer, while the lifetime of the islands increases exponentially with increasing thickness. Furthermore, the island IPS transitions from delocalized to localized within 500 fs, and electrons with larger parallel momenta decay much faster. Attempts were made using a stochastic model to extract the rates of localization and intraband cooling at differing momenta. In sexithiophene (6T) and dihexyl-sexithiophene (DH6T), the IPS was used as a probe to see if the nuclear motion of spectating side chains can interfere with molecular conduction. The energy and band mass of the IPS was measured for 6T and two geometries of DH6T on Ag(111). Electrons injected into the thicker coverages of DH6T grew exponentially heavier until they were completely localized by 230 fs, while those injected into 6T remained nearly free electron like. Based off of lifetime arguments and the density of defects, the most likely cause for the mass enhancement of the IPS in this system is small polaron formation caused by coupling of the electron to vibrations of the alkyl substituents. The energetic relaxation of the molecular adsorbate was also measured to be 20 meV/100 fs for the DH6T, and 0 meV/100 fs for

  20. Evidence for strong electron correlations in graphene molecular fragments: Theory and experiments on two-photon absorptions

    Science.gov (United States)

    Aryanpour, Karan; Roberts, Adam; Sandhu, Arvinder; Shukla, Alok; Mazumdar, Sumit

    2013-03-01

    Historically, the occurrence of the lowest two-photon state below the optical one-photon state in linear polyenes, polyacetylenes and polydiacetylenes provided the strongest evidence for strong electron correlations in these linear π-conjugated systems. We demonstrate similar behavior in several molecular fragments of graphene with D6 h symmetry, theoretically and experimentally. Theoretically, we have calculated one versus two-photon absorptions in coronene, two different hexabenzocoronenes and circumcoronene, within the Pariser-Parr-Pople π-electron Hamiltonian using high order configuration interaction. Experimentally, we have performed z-scan measurements using a white light super-continuum source on coronene and hexa-peri-hexabenzocoronene to determine frequency-dependent two-photon absorption coefficients, for comparison to the ground state absorptions. Excellent agreement between experiment and theory in our work gives strong evidence for significant electron correlations between the π-electrons in the graphene molecular fragments. We particularly benchmark high order electron-hole excitations in graphene fragments as a key element behind the agreement between theory and experiment in this work. We acknowledge NSF-CHE-1151475 grant as our funding source.

  1. Resonant generation of an electron–positron pair by two photons to excited Landau levels

    Energy Technology Data Exchange (ETDEWEB)

    Diachenko, M. M., E-mail: dyachenko.michail@mail.ru; Novak, O. P.; Kholodov, R. I. [National Academy of Sciences of Ukraine, Institute of Applied Physics (Ukraine)

    2015-11-15

    We consider the resonant generation of an electron–positron pair by two polarized photons to arbitrarily low Landau levels. The resonance occurs when the energy of one photon exceeds the one-photon generation threshold, and the energy of the other photon is multiple to the spacing between the levels. The cross section of the process is determined taking into account the spins of particles. The order of magnitude of the cross section is the highest when the magnetic moments of the particles are oriented along the magnetic field.

  2. Rabi oscillations of two-photon states in nonlinear optical resonators

    Science.gov (United States)

    Sherkunov, Y.; Whittaker, David M.; Fal'ko, Vladimir

    2016-02-01

    We demonstrate that four-wave mixing processes in high-quality nonlinear resonators can lead to Rabi-like oscillations in photon occupation numbers and second-order correlation functions, being a characteristic feature of the presence of entangled photon pairs in the optical signal. In the case of a system driven by a continuous coherent pump, the oscillations occur in the transient regime. We show that driving the system with pulsed coherent pumping would generate strongly antibunched photon states.

  3. Two-Photon Study on the Electronic Interactions between the First Excited Singlet States in Carotenoid-Tetrapyrrole Dyads

    Energy Technology Data Exchange (ETDEWEB)

    Liao, Pen-Nan [Technische Universitat Braunschweig (Germany); Pillai, Smitha [Arizona State Univ., Tempe, AZ (United States); Gust, Devens [Arizona State Univ., Tempe, AZ (United States); Moore, Thomas A. [Arizona State Univ., Tempe, AZ (United States); Moore, Ana L. [Arizona State Univ., Tempe, AZ (United States); Walla, Peter J. [Technische Universitat Braunschweig (Germany)

    2011-03-22

    Electronic interactions between the first excited states (S1) of carotenoids (Car) of different conjugation lengths (8-11 double bonds) and phthalocyanines (Pc) in different Car-Pc dyad molecules were investigated by two-photon spectroscopy and compared with Car S1-chlorophyll (Chl) interactions in photosynthetic light harvesting complexes (LHCs). The observation of Chl/Pc fluorescence after selective two-photon excitation of the Car S1 state allowed sensitive monitoring of the flow of energy between Car S1 and Pc or Chl. It is found that two-photon excitation excites to about 80% to 100% exclusively the carotenoid state Car S1 and that only a small fraction of direct tetrapyrrole two-photon excitation occurs. Amide-linked Car-Pc dyads in tetrahydrofuran demonstrate a molecular gear shift mechanism in that effective Car S1 → Pc energy transfer is observed in a dyad with 9 double bonds in the carotenoid, whereas in similar dyads with 11 double bonds in the carotenoid, the Pc fluorescence is strongly quenched by Pc → Car S1 energy transfer. In phenylamino-linked Car-Pc dyads in toluene extremely large electronic interactions between the Car S1 state and Pc were observed, particularly in the case of a dyad in which the carotenoid contained 10 double bonds. This observation together with previous findings in the same system provides strong evidence for excitonic Car S1-Pc Qy interactions. Very similar results were observed with photosynthetic LHC II complexes in the past, supporting an important role of such interactions in photosynthetic down-regulation.

  4. Quantum correlations in the two-photon decay of few-electron ions

    CERN Document Server

    Fratini, Filippo; Jahrsetz, Thorsten; Buchleitner, Andreas; Fritzsche, Stephan; Surzhykov, Andrey

    2010-01-01

    A theoretical study of the polarization entanglement of two photons emitted in the decay of metastable ionic states is performed within the framework of density matrix theory and second--order perturbative approach. Particular attention is paid to relativistic and non--dipole effects that become important for medium-- and high--$Z$ ions. To analyze these effects, the degree of entanglement is evaluated both in the dipole approximation and within the rigorous relativistic theory. Detailed calculations are performed for the two--photon $2s_{1/2}\\to 1s_{1/2}$ transition in hydrogen--like, as well as for the $1s_{1/2}\\, 2s_{1/2} \\; {}^1S_0 \\to 1s_{1/2}^2 \\; {}^1S_0$, $1s_{1/2} \\, 2s_{1/2} \\; {}^3S_1\\to 1s_{1/2}^2 \\; {}^1S_0$ and $1s_{1/2} \\, 2p_{1/2} \\; {}^3P_0\\to 1s_{1/2}^2 \\; {}^1S_0$ transitions in helium--like ions.

  5. Leptonic two-photon events measured with L3 at the Large Electron Positron Collider (LEP)

    CERN Document Server

    Dehmelt, Klaus

    2006-01-01

    Virtual photons can fluctuate into diverse final states and among other processes, such fluctuations can yield muon-pairs. The fluctuation is a statistical process and can be described in terms of structure functions for photons. Apart from supplying another test of QED, purely leptonic processes provide a calibration fro the hadronic processes. We report on a measurement of dimuon events with single-tagged two-photon events from the LEP experiment L3, at c.m.s. energies between 189 GeV and 206 GeV, with an integrated luminosity of $\\mathcal{L}$ = 600 pb$^{-1}$. An overview of the fundamental physical processes, the detector and the anaytical tools, used for measuring dimuon events, and a discussion of the structure of dimuon events will be presented.

  6. Two-Photon Exchange Effects in Elastic Electron-Proton Scattering

    Energy Technology Data Exchange (ETDEWEB)

    Johnson, Myriam James [Argonne National Lab. (ANL), Argonne, IL (United States)

    2013-08-01

    Two methods, Rosenbluth separation and polarization transfer, can be used to extract the proton form factor ratio μp GEp/GMp, but they do not yield the same results. It is thought that the disagreement is due to two photon exchange corrections to the differential cross sections. High precision proton Rosenbluth extractions were carried out at 102 kinematics points spanning 16 values of momentum transfer Q2, from 0.40 to 5.76 GeV2. Reduced cross sections were found to 1.1% or better for Q2 less than 3 GeV2 increasing to 4% at 5.76 GeV2 The form factor ratios were determined to 1:5-3% for Q2 < 1.5 GeV2, increasing to 9% by 3 GeV2 and rapidly above. Our data agrees with prior Rosenbluth, improving upon it the 1.0 - 2.0 GeV2 range to conclusively show a separation from polarization transfer where it had not been certain before. In addition, reduced cross sections at each Q2 were tested for nonlinearity in the angular variable. Such a departure from linearity would be a signature of two photon exchange effects, and prior data had not been sufficiently precise to show nonzero curvature. Our data begins to hint at negative curvature but does not yet show a significant departure from zero.

  7. The 2 1Ag state of isolated cis-trans-1,3,5,7-octatetraene: two-color resonance enhanced two-photon ionization studies

    NARCIS (Netherlands)

    B.E. Kohler; T. Shaler; W.J. Buma

    1992-01-01

    Vibrationally resolved 1 1Ag2 1Ag excitation spectra and decay times for cis,trans-1,3,5,7-octatetraene seeded in a supersonic He expansion have been measured by two-color resonance enhanced two-photon ionization spectroscopy. The excitation energy of the 1 1Ag2 1Ag 0-0 band (29 035 cm-1 ) is ~6500

  8. Two-photon exchange contribution in elastic electron-proton scattering, experiment at the VEPP-3 storage ring

    Directory of Open Access Journals (Sweden)

    Nikolenko D.M.

    2014-03-01

    Full Text Available We describe a precise measurement of the ratio of the (e+ p to (e− p elastic scattering cross sections. This comparison is sensitive to the effect of two-photon exchange contributions which may be the cause for inconsistent extractions of the proton form factors obtained using different methods. The experiment was performed at storage ring VEPP–3, Novosibirsk at energies of positron/electron beams of 1.0 and 1.6 GeV with electron/positron scattering angles θ = 65÷105° for the first case and 15÷25° and 55÷75° for the second case. Details of the experiment and the preliminary results are presented.

  9. Two-Photon Emission of a Hydrogenlike Atom with Photon Polarization and Electron Spin States Taken into Account

    Science.gov (United States)

    Skobelev, V. V.

    2017-02-01

    The process of two-photon emission ( Ze)* → ( Ze) + 2 γ of a hydrogenlike atom is considered with spin states of the electron and polarization of the photons taken into account, which had not been done before. A general expression for the probability of the process per unit time has been obtained for different polarization states of the photons with a formulation of hard and soft selection rules for the quantum numbers m and l. It is shown that by virtue of the established specifics of the properties of the two-photon emission process (absence of a Zeeman effect and dependence of the probability on the polarization states of the photons), it can in principle be identified against the background of single-photon emission ( Ze)* → ( Ze) + γ, despite the presence of additional small factors: 1) α = e 2/ ћc ≈ 1/137 of the perturbation theory in e, and 2) the square of the atomic expansion parameter ( Zα)2 in the expression for the probability.

  10. In situ electrical and thermal monitoring of printed electronics by two-photon mapping

    DEFF Research Database (Denmark)

    Pastorelli, Francesco; Accanto, Nicolo; Jørgensen, Mikkel

    2017-01-01

    Printed electronics is emerging as a new, large scale and cost effective technology that will be disruptive in fields such as energy harvesting, consumer electronics and medical sensors. The performance of printed electronic devices relies principally on the carrier mobility and molecular packing...... of the polymer semiconductor material. Unfortunately, the analysis of such materials is generally performed with destructive techniques, which are hard to make compatible with in situ measurements, and pose a great obstacle for the mass production of printed electronics devices. A rapid, in situ, non...... photoluminescence and second harmonic response. We show that, in our experimental conditions, it is possible to relate the total amount of photoluminescence detected to important material properties such as the charge carrier density and the molecular packing of the printed polymer material, all with a spatial...

  11. Direct observation of photocarrier electron dynamics in C60 films on graphite by time-resolved two-photon photoemission

    Science.gov (United States)

    Shibuta, Masahiro; Yamamoto, Kazuo; Ohta, Tsutomu; Nakaya, Masato; Eguchi, Toyoaki; Nakajima, Atsushi

    2016-10-01

    Time-resolved two-photon photoemission (TR-2PPE) spectroscopy is employed to probe the electronic states of a C60 fullerene film formed on highly oriented pyrolytic graphite (HOPG), acting as a model two-dimensional (2D) material for multi-layered graphene. Owing to the in-plane sp2-hybridized nature of the HOPG, the TR-2PPE spectra reveal the energetics and dynamics of photocarriers in the C60 film: after hot excitons are nascently formed in C60 via intramolecular excitation by a pump photon, they dissociate into photocarriers of free electrons and the corresponding holes, and the electrons are subsequently detected by a probe photon as photoelectrons. The decay rate of photocarriers from the C60 film into the HOPG is evaluated to be 1.31 × 1012 s‑1, suggesting a weak van der Waals interaction at the interface, where the photocarriers tentatively occupy the lowest unoccupied molecular orbital (LUMO) of C60. The photocarrier electron dynamics following the hot exciton dissociation in the organic thin films has not been realized for any metallic substrates exhibiting strong interactions with the overlayer. Furthermore, the thickness dependence of the electron lifetime in the LUMO reveals that the electron hopping rate in C60 layers is 3.3 ± 1.2 × 1013 s‑1.

  12. Stepwise Two-Photon-Induced Fast Photoswitching via Electron Transfer in Higher Excited States of Photochromic Imidazole Dimer.

    Science.gov (United States)

    Kobayashi, Yoichi; Katayama, Tetsuro; Yamane, Takuya; Setoura, Kenji; Ito, Syoji; Miyasaka, Hiroshi; Abe, Jiro

    2016-05-11

    Stepwise two-photon excitations have been attracting much interest because of their much lower power thresholds compared with simultaneous two-photon processes and because some stepwise two-photon processes can be initiated by a weak incoherent excitation light source. Here we apply stepwise two-photon optical processes to the photochromic bridged imidazole dimer, whose solution instantly changes color upon UV irradiation and quickly reverts to the initial color thermally at room temperature. We synthesized a zinc tetraphenylporphyrin (ZnTPP)-substituted bridged imidazole dimer, and wide ranges of time-resolved spectroscopic studies revealed that a ZnTPP-linked bridged imidazole dimer shows efficient visible stepwise two-photon-induced photochromic reactions upon excitation at the porphyrin moiety. The fast photoswitching property combined with stepwise two-photon processes is important not only for the potential for novel photochromic materials that are sensitive to the incident light intensity but also for fundamental photochemistry using higher excited states.

  13. Off-Resonant Two-Photon Absorption Cross-Section Enhancement of an Organic Chromophore on Gold Nanorods

    Science.gov (United States)

    Sivapalan, Sean T.; Vella, Jarrett H.; Yang, Timothy K.; Dalton, Matthew J.; Haley, Joy E.; Cooper, Thomas M.; Urbas, Augustine M.; Tan, Loon-Seng; Murphy, Catherine J.

    2013-01-01

    Surface-plasmon-initiated interference effects of polyelectrolyte-coated gold nanorods on the two-photon absorption of an organic chromophore were investigated. With polyelectrolyte bearing gold nanorods of 2,4,6 and 8 layers, the role of the plasmonic fields as function of distance on such effects was examined. An unusual distance dependence was found: enhancements in the two-photon cross-section were at a minimum at an intermediate distance, then rose again at a further distance. The observed values of enhancement were compared to theoretical predictions using finite element analysis and showed good agreementdue to constructive and destructive interference effects. PMID:23687561

  14. Exact steady-state of a Kerr resonator with one- and two-photon driving-dissipation: controllable Wigner-function multimodality and dissipative phase transitions

    CERN Document Server

    Bartolo, Nicola; Casteels, Wim; Ciuti, Cristiano

    2016-01-01

    We present exact results for the steady-state density matrix of a general class of driven-dissipative systems consisting of a nonlinear Kerr resonator in the presence of both coherent (one-photon) and parametric (two-photon) driving and dissipation. Thanks to the analytical solution, obtained via the complex P-representation formalism, we are able to explore any regime, including photon blockade, multi-photon resonant effects, and a mesoscopic regime with large photon density and quantum correlations. We show how the interplay between one- and two-photon driving provides a way to control the multi-modality of the Wigner function in regimes where the semiclassical theory exhibits multistability. We also study the emergence of dissipative phase transitions in the thermodynamic limit of large photon numbers.

  15. Difluorenyl carbo-Benzenes: Synthesis, Electronic Structure, and Two-Photon Absorption Properties of Hydrocarbon Quadrupolar Chromophores.

    Science.gov (United States)

    Baglai, Iaroslav; de Anda-Villa, Manuel; Barba-Barba, Rodrigo M; Poidevin, Corentin; Ramos-Ortíz, Gabriel; Maraval, Valérie; Lepetit, Christine; Saffon-Merceron, Nathalie; Maldonado, José-Luis; Chauvin, Remi

    2015-09-28

    The synthesis, crystal and electronic structures, and one- and two-photon absorption properties of two quadrupolar fluorenyl-substituted tetraphenyl carbo-benzenes are described. These all-hydrocarbon chromophores, differing in the nature of the linkers between the fluorenyl substituents and the carbo-benzene core (C-C bonds for 3 a, C-C=C-C expanders for 3 b), exhibit quasi-superimposable one-photon absorption (1PA) spectra but different two-photon absorption (2PA) cross-sections σ2PA. Z-scan measurements (under NIR femtosecond excitation) indeed showed that the C≡C expansion results in an approximately twofold increase in the σ2PA value, from 336 to 656 GM (1 GM = 10(-50) cm(4) s molecule(-1) photon(-1)) at λ = 800 nm. The first excited states of Au and Ag symmetry accounting for 1PA and 2PA, respectively, were calculated at the TDDFT level of theory and used for sum-over-state estimations of σ2PA(λi), in which λi = 2 hc/Ei, h is Planck's constant, c is the speed of light, and Ei is the energy of the 2PA-allowed transition. The calculated σ2PA values of 227 GM at 687 nm for 3 a and 349 GM at 708 nm for 3 b are in agreement with the Z-scan results.

  16. Two-photon physics

    Energy Technology Data Exchange (ETDEWEB)

    Bardeen, W.A.

    1981-10-01

    A new experimental frontier has recently been opened to the study of two photon processes. The first results of many aspects of these reactions are being presented at this conference. In contrast, the theoretical development of research ito two photon processes has a much longer history. This talk reviews the many different theoretical ideas which provide a detailed framework for our understanding of two photon processes.

  17. Electron paramagnetic resonance

    CERN Document Server

    Al'tshuler, S A

    2013-01-01

    Electron Paramagnetic Resonance is a comprehensive text on the field of electron paramagnetic resonance, covering both the theoretical background and the results of experiment. This book is composed of eight chapters that cover theoretical materials and experimental data on ionic crystals, since these are the materials that have been most extensively studied by the methods of paramagnetic resonance. The opening chapters provide an introduction to the basic principles of electron paramagnetic resonance and the methods of its measurement. The next chapters are devoted to the theory of spectra an

  18. Interferometric two-photon photoemission correlation technique and femtosecond wet-electron dynamics at the TiO2 (110) surface

    Institute of Scientific and Technical Information of China (English)

    Bin LI; Jin ZHAO; Min FENG; Ken ONDA

    2008-01-01

    The femtosecond time-resolved two-photon pho-toemission (TR-2PP) and the ultra high vacuum (UHV) sur-face science techniques are integrated to investigate the elec-tronic structures and the interracial electron transfer dynamics at the atomically ordered adsorbate overlayers on TiO,2single-crystalline surfaces. Our research into the CH,3OH/TiO,2sys-tem exhibits complex dynamics, providing abundant informa-tion with regard to electron transport and solvation processes in the interfacial solvent structures. These represent the fundamentally physical, photochemical, and photocatalytic reactions of protic chemicals covered with metal-oxides.

  19. Assessment of mode-mixing and Herzberg-Teller effects on two-photon absorption and resonance hyper-Raman spectra from a time-dependent approach.

    Science.gov (United States)

    Ma, HuiLi; Zhao, Yi; Liang, WanZhen

    2014-03-07

    A time-dependent approach is presented to simulate the two-photon absorption (TPA) and resonance hyper-Raman scattering (RHRS) spectra including Duschinsky rotation (mode-mixing) and Herzberg-Teller (HT) vibronic coupling effects. The computational obstacles for the excited-state geometries, vibrational frequencies, and nuclear derivatives of transition dipole moments, which enter the expressions of TPA and RHRS cross sections, are further overcome by the recently developed analytical excited-state energy derivative approaches in the framework of time-dependent density functional theory. The excited-state potential curvatures are evaluated at different levels of approximation to inspect the effects of frequency differences, mode-mixing and HT on TPA and RHRS spectra. Two types of molecules, one with high symmetry (formaldehyde, p-difluorobenzene, and benzotrifluoride) and the other with non-centrosymmetry (cis-hydroxybenzylidene-2,3-dimethylimidazolinone in the deprotonated anion state (HDBI(-))), are used as test systems. The calculated results reveal that it is crucial to adopt the exact excited-state potential curvatures in the calculations of TPA and RHRS spectra even for the high-symmetric molecules, and that the vertical gradient approximation leads to a large deviation. Furthermore, it is found that the HT contribution is evident in the TPA and RHRS spectra of HDBI(-) although its one- and two-photon transitions are strongly allowed, and its effect results in an obvious blueshift of the TPA maximum with respect to the one-photon absorption maximum. With the HT and solvent effects getting involved, the simulated blueshift of 1291 cm(-1) agrees well with the experimental measurement.

  20. Assessment of mode-mixing and Herzberg-Teller effects on two-photon absorption and resonance hyper-Raman spectra from a time-dependent approach

    Energy Technology Data Exchange (ETDEWEB)

    Ma, HuiLi [State Key Laboratory of Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and Institute of Fujian Provincial Theoretical and Computational Chemistry, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005 (China); Department of Chemical Physics, University of Science and Technology of China, Hefei 230026 (China); Zhao, Yi; Liang, WanZhen, E-mail: liangwz@xmu.edu.cn [State Key Laboratory of Physical Chemistry of Solid Surfaces, Collaborative Innovation Center of Chemistry for Energy Materials, and Institute of Fujian Provincial Theoretical and Computational Chemistry, College of Chemistry and Chemical Engineering, Xiamen University, Xiamen 361005 (China)

    2014-03-07

    A time-dependent approach is presented to simulate the two-photon absorption (TPA) and resonance hyper-Raman scattering (RHRS) spectra including Duschinsky rotation (mode-mixing) and Herzberg-Teller (HT) vibronic coupling effects. The computational obstacles for the excited-state geometries, vibrational frequencies, and nuclear derivatives of transition dipole moments, which enter the expressions of TPA and RHRS cross sections, are further overcome by the recently developed analytical excited-state energy derivative approaches in the framework of time-dependent density functional theory. The excited-state potential curvatures are evaluated at different levels of approximation to inspect the effects of frequency differences, mode-mixing and HT on TPA and RHRS spectra. Two types of molecules, one with high symmetry (formaldehyde, p-difluorobenzene, and benzotrifluoride) and the other with non-centrosymmetry (cis-hydroxybenzylidene-2,3-dimethylimidazolinone in the deprotonated anion state (HDBI{sup −})), are used as test systems. The calculated results reveal that it is crucial to adopt the exact excited-state potential curvatures in the calculations of TPA and RHRS spectra even for the high-symmetric molecules, and that the vertical gradient approximation leads to a large deviation. Furthermore, it is found that the HT contribution is evident in the TPA and RHRS spectra of HDBI{sup −} although its one- and two-photon transitions are strongly allowed, and its effect results in an obvious blueshift of the TPA maximum with respect to the one-photon absorption maximum. With the HT and solvent effects getting involved, the simulated blueshift of 1291 cm{sup −1} agrees well with the experimental measurement.

  1. Radiative electronic energy transfer-time studies of naphthalene-biacetyl system by one and two-photon excitation, and optical antenna mechanism.

    Science.gov (United States)

    Bayrakceken, Fuat

    2005-04-01

    In principle, the optical energy absorbed by a complex molecule raises that molecule to one of its excited states, and afterwards this excitation energy decays through the relaxation channels. Initially, electronically excited naphthalene emits photons and these emitted photons are absorbed by the acceptor molecule biacetyl, then excited biacetyl fluoresces. In this investigation radiative energy transfer-time is measured in cyclohexane by one and two-photon excitations. The UV-vis spectrum of biacetyl vapor at room temperature conditions was broad and structureless.

  2. Two-photon cryomicroscope

    Science.gov (United States)

    Breunig, H. G.; Köhler, C.; König, K.

    2012-03-01

    We report on a new two-photon cryomicroscope which consist of a compact laser-scanning microscope combined with a motorized heating and freezing stage. Samples can be cooled down to -196 °C (77 K) and heated up to 600 °C (873 K) with adjustable heating/freezing rates between 0.01 K / min and 150 K / min. Two-photon imaging is realized by near infrared femtosecond-laser pulse excitation. The abilities of the two-photon cryomicroscope are illustrated in several measurements: imaging of fluorescent microspheres inside a piece of ice illustrates the feasibility of deep-microscopic imaging inside frozen sample. The temperature-dependent structural integrity of collagen is monitored by detection of second harmonic generation signals from porcine cornea. The measurements reveal also the dependence of the collagendenaturation temperature on hydration state of the cornea collagen. Furthermore, the potential of the two-photon cryomicroscope for optimization of freezing and thawing procedures as well as to evaluate the viability of frozen cells and tissue is discussed.

  3. Adiabatic following in two-photon transition

    Energy Technology Data Exchange (ETDEWEB)

    Nayfeh, M.H.; Nayfeh, A.H.

    1977-01-01

    There has been much interest recently in coherent multiphoton transitions in many-level systems. The present work considers the effect of relaxation in the response of a three-level system to a smoothly varying, near-resonant, two-photon field. The relaxation-dependent contributions to the nonlinear refractive index are calculated. It is shown that the coherent interaction of two smoothly varying, near-resonant, two-photon pulses with a three-level system can be described by ''two-photon damped Bloch equations'' which are analogous to those for a one-photon transition in a two-level system except for the presence of a two-photon coupling and a frequency shift. 1 figure. (RWR)

  4. Sideband-Induced Two-Photon Transparency

    Institute of Scientific and Technical Information of China (English)

    CHENG Guang-Ling; HU Xiang-Ming

    2006-01-01

    @@ We show that it is possible to use a single sideband to induce two-photon transparency in a three-level cascade medium. The medium simultaneously absorbs two photons as a one-step process when the middle level is far off one-photon resonance. A resonant sideband coupling on the upper transition and the two-photon one-step process drive the medium into a trapped state, and the dominant component is the ground state. Thus almost all population is trapped in the ground state and the two-photon absorption is dramatically suppressed. We present a numerical calculation for arbitrary values of the atomic and field parameters and also provide an analytic description for the required conditions.

  5. Phase and ellipticity dependence of the photoelectron angular distribution in non-resonant two-photon ionization of atomic hydrogen. I

    Energy Technology Data Exchange (ETDEWEB)

    Faye, M; Wane, S T, E-mail: mamadou.faye@ucad.edu.sn [Departement de Physique, Faculte des Sciences et Techniques, Universite Cheikh Anta Diop, Boulevard Martin Luther King, (Corniche Ouest) BP 5005-Dakar Fann (Senegal)

    2011-03-14

    We study the ellipticity and the dependence on the phase lag (lead) (between the semimajor and the semiminor axes of the field components) of the photoelectron angular distribution (PAD) in the non-resonant two-photon ionization of atomic hydrogen. We establish exact analytical expressions for azimuthal PAD for 3s, 3p and 3d excited initial states, marked by the occurrence of an asymmetric term. This term gives rise to elliptic dichroism (ED), which can be obtained in two ways: either with the left (versus right) ellipticity, or with the phase lag (versus lead); for 3s and 3p initial states, it is shown that the quantum phase of continua is directly related to the phase lag, one-photon below-threshold ionization, and indirectly one photon above. Another important result is that the magnetic sublevels, m = 0, for 3p and m = {+-}1, for 3d, do not contribute to the azimuthal PAD. Our numerical results show, for 3s and 3d, and near-threshold ionization, that the PAD has maxima either along the semimajor or the semiminor axis, while for above-threshold ionization, they are always shifted from these axes. However, the maxima of the corresponding ED coincide with the PAD maxima, while for 3p, they are shifted from the PAD minima. A strong dependence of the ED sign is noted, regardless of the state or the process. However, strong ED signals are obtained for the 3s initial state and below-threshold ionization.

  6. Platinum Acetylide Two-Photon Chromophores (Preprint)

    Science.gov (United States)

    2007-04-01

    the higher energy range that lead to its photodegradation . Secondly, because there is a quadratic dependence of two-photon absorption (2PA) on the...to either an electron donating amino- fluorenyl or electron withdrawing benzothiazolyl-fluorene that are themselves known as two-photon absorbing dyes ...groups in place of phenyl groups have shown a doubling of the intrinsic cr2value at 740 nm.40,41In this paper we describe novel platinum dyes that

  7. Two-photon absorption and spectroscopy of the lowest two-photon transition in small donor-acceptor-substituted organic molecules

    Science.gov (United States)

    Beels, Marten T.; Biaggio, Ivan; Reekie, Tristan; Chiu, Melanie; Diederich, François

    2015-04-01

    We determine the dispersion of the third-order polarizability of small donor-acceptor substituted organic molecules using wavelength-dependent degenerate four-wave mixing experiments in solutions with varying concentrations. We find that donor-acceptor-substituted molecules that are characterized by extremely efficient off-resonant nonlinearities also have a correspondingly high two-photon absorption cross section. The width and shape of the first two-photon resonance for these noncentrosymmetric molecules follows what is expected from their longest wavelength absorption peak, and the observed two-photon absorption cross sections are record high when compared to the available literature data, the size of the molecule, and the fundamental limit for two-photon absorption to the lowest excited state, which is essentially determined by the number of conjugated electrons and the excited-state energies. The two-photon absorption of the smallest molecule, which only has 16 electrons in its conjugated system, is one order of magnitude larger than for the molecule called AF-50, a reference molecule for two-photon absorption [O.-K. Kim et al., Chem. Mater. 12, 284 (2000), 10.1021/cm990662r].

  8. Two-Photon Physics in Hadronic Processes

    Energy Technology Data Exchange (ETDEWEB)

    Carl Carlson; Marc Vanderhaeghen

    2007-11-01

    Two-photon exchange contributions to elastic electron-scattering are reviewed. The apparent discrepancy in the extraction of elastic nucleon form factors between unpolarized Rosenbluth and polarization transfer experiments is discussed, as well as the understanding of this puzzle in terms of two-photon exchange corrections. Calculations of such corrections both within partonic and hadronic frameworks are reviewed. In view of recent spin-dependent electron scattering data, the relation of the two-photon exchange process to the hyperfine splitting in hydrogen is critically examined. The imaginary part of the two-photon exchange amplitude as can be accessed from the beam normal spin asymmetry in elastic electron-nucleon scattering is reviewed. Further extensions and open issues in this field are outlined.

  9. Two-photon vibrational excitation of air by long-wave infrared laser pulses

    CERN Document Server

    Palastro, J P; Johnson, L A; Hafizi, B; Wahlstrand, J K; Milchberg, H M

    2016-01-01

    Ultrashort long-wave infrared (LWIR) laser pulses can resonantly excite vibrations in N2 and O2 through a two-photon transition. The absorptive, vibrational component of the ultrafast optical nonlinearity grows in time, starting smaller than, but quickly surpassing, the electronic, rotational, and vibrational refractive components. The growth of the vibrational component results in a novel mechanism of 3rd harmonic generation, providing an additional two-photon excitation channel, fundamental + 3rd harmonic. The original and emergent two-photon excitations drive the resonance exactly out of phase, causing spatial decay of the absorptive, vibrational nonlinearity. This nearly eliminates two-photon vibrational absorption. Here we present simulations and analytical calculations demonstrating how these processes modify the ultrafast optical nonlinearity in air. The results reveal nonlinear optical phenomena unique to the LWIR regime of ultrashort pulse propagation in atmosphere.

  10. A spectroscopic study of nicotine analogue 2-phenylpyrrolidine (PPD) using resonant two-photon ionization (R2PI), microwave, and 2D NMR techniques.

    Science.gov (United States)

    Martin, Danielle E; Robertson, Evan G; MacLellan, Jonathan G; Godfrey, Peter D; Thompson, Christopher D; Morrison, Richard J S

    2009-02-25

    Conformational preferences of the nicotine analogue 2-phenylpyrrolidine (PPD) have been studied in both gaseous and solution phases. Theoretical calculations at the MP2 and B3LYP levels point to 5-6 stable conformers which differ in three degrees of conformational freedom; torsion between the two rings, inversion at the pyrrolidine (PY) amine, and PY ring puckering, characterized using the Cremer-Pople definition for pseudorotation. Only one conformer has a trans arrangement between the amino hydrogen and the phenyl substituent. It is 6-8 kJ mol(-1) more stable than the cis conformers, has a perpendicular ring arrangement, and puckers at the nitrogen atom--similar to structures reported for nicotine. Resonant two-photon ionization (R2PI) data, including hole burn spectra, indicate only one conformer is present in the free jet expansion, and band contour analysis suggests assignment to the trans conformer. Confirmation was provided by microwave spectroscopy. Fifty-seven lines measured in the 48-72 GHz region were assigned to 206 b-type transitions and fitted to yield rotational constants within 2 MHz of MP2 values predicted for the trans conformer. The solution-phase conformers of PPD were studied using 1D and 2D (1)H NMR spectroscopy and solvent-based theoretical calculations. In marked contrast to the gas phase, NMR data reveals only cis conformers present in solution. Calculations confirm increased stability for these conformers when placed in simulated chloroform or water environments. Solvent molecules are believed to disrupt a crucial N...H(ortho) stabilizing interaction present within the trans conformer.

  11. Model-independent analysis of polarization effects in elastic electron-deuteron scattering in presence of two-photon exchange

    Energy Technology Data Exchange (ETDEWEB)

    Gakh, G.I.; Tomasi-Gustafsson, E

    2006-07-01

    The general spin structure of the matrix element, taking into account the 2-photon exchange contribution, for the elastic electron (positron) - deuteron scattering has been derived using general symmetry properties of the hadron electromagnetic interaction, such as P-, C- and T-invariances as well as lepton helicity conservation in QED at high energy. Taking into account also crossing symmetry, the amplitudes of e{sup {+-}}d scattering can be parametrized in terms of fifteen real functions. The expressions for the differential cross section and for all polarization observables are given in terms of these functions. We consider the case of an arbitrary polarized deuteron target and polarized electron beam (both longitudinal and transverse). The transverse polarization of the electron beam induces a single-spin asymmetry which is non-zero in presence of 2-photon exchange. It is shown that elastic deuteron electromagnetic form factors can still be extracted in presence of 2 photon exchange, from the measurements of the differential cross sections and of one polarization observable (for example, the tensor asymmetry) for electron and positron deuteron elastic scattering, in the same kinematical conditions. (authors)

  12. Benzothiazoles with tunable electron-withdrawing strength and reverse polarity: a route to triphenylamine-based chromophores with enhanced two-photon absorption.

    Science.gov (United States)

    Hrobárik, Peter; Hrobáriková, Veronika; Sigmundová, Ivica; Zahradník, Pavol; Fakis, Mihalis; Polyzos, Ioannis; Persephonis, Peter

    2011-11-01

    A series of dipolar and octupolar triphenylamine-derived dyes containing a benzothiazole positioned in the matched or mismatched fashion have been designed and synthesized via palladium-catalyzed Sonogashira cross-coupling reactions. Linear and nonlinear optical properties of the designed molecules were tuned by an additional electron-withdrawing group (EWG) and by changing the relative positions of the donor and acceptor substituents on the heterocyclic ring. This allowed us to examine the effect of positional isomerism and extend the structure-property relationships useful in the engineering of novel heteroaromatic-based systems with enhanced two-photon absorption (TPA). The TPA cross-sections (δ(TPA)) in the target compounds dramatically increased with the branching of the triphenylamine core and with the strength of the auxiliary acceptor. In addition, a change from the commonly used polarity in push-pull benzothiazoles to a reverse one has been revealed as a particularly useful strategy (regioisomeric control) for enhancing TPA cross-sections and shifting the absorption and emission maxima to longer wavelengths. The maximum TPA cross-sections of the star-shaped three-branched triphenylamines are ∼500-2300 GM in the near-infrared region (740-810 nm); thereby the molecular weight normalized δ(TPA)/MW values of the best performing dyes within the series (2.0-2.4 GM·g(-1)·mol) are comparable to those of the most efficient TPA chromophores reported to date. The large TPA cross-sections combined with high emission quantum yields and large Stokes shifts make these compounds excellent candidates for various TPA applications, including two-photon fluorescence microscopy.

  13. Two-photon physics at LEP2

    Energy Technology Data Exchange (ETDEWEB)

    Cartwright, Susan; Lehto, Mark [University of Sheffield Department of Physics, Sheffield S3 7RH (United Kingdom); Seymour, Michael H.; Close, Frank; Wright, Alison [Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire OX11 0QX (United Kingdom); Affholderbach, Klaus; Cowan, Glen [Universitaet Siegen, Fachbereich Physik, D-57068 Siegen (Germany); Finch, Alex [University of Lancaster, Lancaster LA1 4YB (United Kingdom); Lauber, Jan [University College London, Gower Street, London WC1E 6BT (United Kingdom)

    1998-02-01

    The working group on two-photon physics concentrated on three main subtopics: modelling the hadronic final state of deep inelastic scattering on a photon; unfolding the deep inelastic scattering data to obtain the photon structure function; and resonant production of exclusive final states, particularly of glueball candidates. In all three areas, new results were presented. (author)

  14. Resonant two-photon ionization of phenol in methylene chloride doped solid argon using 248 nm KrF laser and 254 nm Hg lamp radiation, a comparative study. The UV/VIS absorption spectrum of phenol radical cation

    Science.gov (United States)

    Kesper, Karl; Diehl, Frank; Simon, Jens Georg Günther; Specht, Harald; Schweig, Armin

    1991-06-01

    Resonant two-photon ionization (TPI) of phenol (PhOH) has been successfully achieved in methylene chloride (CH 2Cl 2) doped solid argon using a KrF laser and a Hg resonance lamp. The result constitutes the first-time TPI of a typically organic molecule in this medium using an excimer laser as well as the first-time spectroscopic identification of PhOH +•. A qualitative model is proposed which is consistent with both the unexpected photostability of PhOH +• and the incomplete running of the TPI process in the applied medium.

  15. Integrating two-photon microscopy and cryo-electron microscopy for studying the interaction of Cafeteria roenbergensis and CroV

    Science.gov (United States)

    Aghvami, Seyedmohammadali

    Cafeteria roenbergensis (Cro) is a marine zooplankton; its voracious appetite plays a significant role in regulating bacteria populations. The giant virus that lives within Cro, known as Cafeteria roenbergensis virus (CroV), has an important effect on the mortality of Cro populations. Although viral infections are extremely abundant in oceans, the complete procedure of the infection is still unknown. We study the infection process of Cro by CroV to find out whether the initial contact is through phagocytosis or CroV penetrating the host cell membrane directly. Cro is a moving at speed in the range of 10-100 um/s, therefore, there are many difficulties and challenges for traditional imaging techniques to study this viral-host interaction. We apply two-photon fluorescence microscopy to image this infection process. The image is taken at video rate (30 frame/s), which makes us able to catch the moment of interaction. We are able to image host and virus simultaneously where CroV is stained by SYBR gold dye and Cro is excited through NADH autofluorescence. For further structural biology study, we will obtain atomic level resolution information of infection. After catching the initial moment of infection, we will freeze the sample instantly and image it with cryo-electron microscope .

  16. Correlative two-photon and serial block face scanning electron microscopy in neuronal tissue using 3D near-infrared branding maps.

    Science.gov (United States)

    Lees, Robert M; Peddie, Christopher J; Collinson, Lucy M; Ashby, Michael C; Verkade, Paul

    2017-01-01

    Linking cellular structure and function has always been a key goal of microscopy, but obtaining high resolution spatial and temporal information from the same specimen is a fundamental challenge. Two-photon (2P) microscopy allows imaging deep inside intact tissue, bringing great insight into the structural and functional dynamics of cells in their physiological environment. At the nanoscale, the complex ultrastructure of a cell's environment in tissue can be reconstructed in three dimensions (3D) using serial block face scanning electron microscopy (SBF-SEM). This provides a snapshot of high resolution structural information pertaining to the shape, organization, and localization of multiple subcellular structures at the same time. The pairing of these two imaging modalities in the same specimen provides key information to relate cellular dynamics to the ultrastructural environment. Until recently, approaches to relocate a region of interest (ROI) in tissue from 2P microscopy for SBF-SEM have been inefficient or unreliable. However, near-infrared branding (NIRB) overcomes this by using the laser from a multiphoton microscope to create fiducial markers for accurate correlation of 2P and electron microscopy (EM) imaging volumes. The process is quick and can be user defined for each sample. Here, to increase the efficiency of ROI relocation, multiple NIRB marks are used in 3D to target ultramicrotomy. A workflow is described and discussed to obtain a data set for 3D correlated light and electron microscopy, using three different preparations of brain tissue as examples. Copyright © 2017 Elsevier Inc. All rights reserved.

  17. Two photon physics. Personal recollection

    CERN Document Server

    Ginzburg, Ilya F

    2015-01-01

    The term two--photon processes is used for the reactions in which some system of particles is produced in collision of two photons, either real or virtual. In the study of these processes our main goal was to suggest approach, allowing to extract from the data information on proper two--photon process separating it from mechanism which responsible for the production of photons. Here I present my view for history of two--photon physics. I don't try to give complete review, concentrating mainly on works of our team (which cover essential part of the topic) and some colleagues. My citation is strongly incomplete. I cite here only papers which were essential in our understanding of the problems. The choice of presented details is the result of my discussions with Gleb Kotkin and Valery Serbo. 1. Prehistory. 2. Two photon processes at e^+e^- colliders. 3. Photon colliders. 4. Notes on physical program.

  18. Two-photon physics

    Energy Technology Data Exchange (ETDEWEB)

    Mark Vanderhaeghen

    2005-10-22

    It is reviewed how Compton scattering sum rules relate low-energy nucleon structure quantities to the nucleon excitation spectrum. In particular, the GDH sum rule and recently proposed extensions of it will be discussed. These extensions are sometimes more calculationally robust, which may be an advantage when estimating the chiral extrapolations of lattice QCD results, such as for anomalous magnetic moments. Subsequently, new developments in our description of the nucleon excitation spectrum will be discussed, in particular a recently developed chiral effective field theory framework for the {Delta}(1232)-resonance region. Within this framework, we discuss results on N and {Delta} masses, the {gamma} N {Delta} transition and the {Delta} magnetic dipole moment.

  19. Electromagnetically induced absorption and transparency in an optical-rf two-photon coupling configuration

    Energy Technology Data Exchange (ETDEWEB)

    Fu Guangsheng [College of Physical Science and Technology, Hebei University, Baoding 071002 (China); Li Xiaoli [College of Physical Science and Technology, Hebei University, Baoding 071002 (China)], E-mail: xiaolixiaoli001@yahoo.com.cn; Zhuang Zhonghong; Zhang Lianshui; Yang Lijun; Li Xiaowei; Han Li [College of Physical Science and Technology, Hebei University, Baoding 071002 (China); Manson, Neil B.; Wei Changjiang [Laser Physics Center, Research School of Physical Sciences and Engineering, Australian Nation University, Canberra, ACT 0200 (Australia)

    2008-01-07

    We study electromagnetically induced absorption (EIA) and transparency (EIT) in an optical-rf two-photon coupling configuration. It is shown that the interference effect due to interacting dark resonances results in an EIA for a resonant two-photon coupling and this EIA is observed to evolve into an EIT when there is a detuning in the two-photon coupling.

  20. Two-photon microscopy for chemical neuroscience.

    Science.gov (United States)

    Ellis-Davies, Graham C R

    2011-04-20

    Microscopes using non-linear excitation of chromophores with pulsed near-IR light can generate highly localized foci of molecules in the electronic singlet state that are concentrated in volumes of less than one femtoliter. The three-dimensional confinement of excitation arises from the simultaneous absorption of two IR photons of approximately half the energy required for linear excitation. Two-photon microscopy is especially useful for two types of interrogation of neural processes. First, uncaging of signaling molecules such as glutamate, as stimulation is so refined it can be used to mimic normal unitary synaptic levels. In addition, uncaging allows complete control of the timing and position of stimulation, so the two-photon light beam provides the chemical neuroscientist with an "optical conductor's baton" which can command synaptic activity at will. A second powerful feature of two-photon microscopy is that when used for fluorescence imaging it enables the visualization of cellular structure and function in living animals at depths far beyond that possible with normal confocal microscopes. In this review I provide a survey of the many important applications of two-photon microscopy in these two fields of neuroscience, and suggest some areas for future technical development.

  1. Two-photon contributions to the elastic electron-nucleon scattering in the Skyrme model; Zwei-Photon-Beitraege zur elastischen Elektron-Nukleon-Streuung im Skyrme-Modell

    Energy Technology Data Exchange (ETDEWEB)

    Kuhn, Markus

    2008-09-23

    The electromagnetic form factors are crucial for our understanding of the inner structure of the proton. Recently it has become feasible to measure them by the use of polarisation transfer techniques in addition to the traditional Rosenbluth separation method. Thereby emerged an incompatibility of the results obtained by these two different experimental methods. It is commonly assumed that the discrepance is induced by higher order corrections to the cross section, especially through two-photon exchange processes. Unfortunately these processes cannot be calculated in a model independent manner because off-shell photon nucleon vertices arise. Effective chiral lagrangians contain already local two-photon couplings and therefore seem exceptionally well suited to study the anomaly contribution to the two-photon exchange. These couplings give two-photon exchange contributions that can be understood as the coupling of the nucleon to pions, decaying into two virtual photons. A particular contribution emerges from the chiral anomaly of QCD, that describes the two-photon decay of the neutral pion. The most important goal of this work is the calculation of the contribution arising from the anomaly to the elastic electron-proton scattering. The results are expected to be widely model independent since the anomaly directly reflects a QCD property. Based on the Skyrme model the protons are realized as soliton solutions in effective chiral theories. The next to leading order contribution to the cross section is given by the interference between the one- and two-photon exchange. The latter contains an ultraviolet divergence, which is renormalized by a local effective counterterm. This counterterm contributes to the width of the neutral pion decay which determines the finite part of the counterterm coefficient. The affect of the anomaly to the Rosenbluth separation of the electromagnetic form factors as well as the discrepance regarding the polarization measurements is extensively

  2. Two-Photon Collective Atomic Recoil Lasing

    Directory of Open Access Journals (Sweden)

    James A. McKelvie

    2015-11-01

    Full Text Available We present a theoretical study of the interaction between light and a cold gasof three-level, ladder configuration atoms close to two-photon resonance. In particular, weinvestigate the existence of collective atomic recoil lasing (CARL instabilities in differentregimes of internal atomic excitation and compare to previous studies of the CARL instabilityinvolving two-level atoms. In the case of two-level atoms, the CARL instability is quenchedat high pump rates with significant atomic excitation by saturation of the (one-photoncoherence, which produces the optical forces responsible for the instability and rapid heatingdue to high spontaneous emission rates. We show that in the two-photon CARL schemestudied here involving three-level atoms, CARL instabilities can survive at high pump rateswhen the atoms have significant excitation, due to the contributions to the optical forces frommultiple coherences and the reduction of spontaneous emission due to transitions betweenthe populated states being dipole forbidden. This two-photon CARL scheme may form thebasis of methods to increase the effective nonlinear optical response of cold atomic gases.

  3. Studies of the optical properties of solids. I. Two-photon electroabsorption. II. Electron-hole exchange coupling at L-II, L-III edges

    Energy Technology Data Exchange (ETDEWEB)

    Kolber, Michael Allen

    1978-01-01

    In Chapter I, it is shown that direct-gap covalent semiconductors, such as GaAs, should exhibit electric-field induced Franz-Keldysh-like structures in their two-photon absorption spectra. These structures are evaluated employing exciton theory; the resulting lineshapes are shown to be proportional to the lineshapes for one-photon ''forbidden'' transitions, a property which greatly facilitates computations of the two-photon absorption. In chapter two, exchange mixes the L/sub II/ and L/sub III/ soft x-ray absorption edges of metallic Na, Mg, and Al, affecting the detailed absorption lineshape and the L/sub II//L/sub III/ intensity ratio. The Onodera theory of this mixing is generalized and the requirements of particle conservation and causality lead to significant modifications of the theoretical absorption lineshape. It is shown that under certain conditions an exchange-free lineshape can be extracted from experimental data for comparison with non-asymptotic theories of x-ray edges.

  4. Higgs Decay to Two Photons

    OpenAIRE

    Marciano, William J.; Zhang, Cen; Willenbrock, Scott

    2011-01-01

    The amplitude for Higgs decay to two photons is calculated in renormalizable and unitary gauges using dimensional regularization at intermediate steps. The result is finite, gauge independent, and in agreement with previously published results. The large Higgs mass limit is examined using the Goldstone-boson equivalence theorem as a check on the use of dimensional regularization and to explain the absence of decoupling.

  5. Two-photon excited fluorescence from higher electronic states of chlorophylls in photosynthetic antenna complexes a new approach to detect strong excitonic chlorophyll a/b coupling

    CERN Document Server

    Leupold, D; Ehlert, J; Irrgang, K D; Renger, G; Lokstein, H

    2002-01-01

    Stepwise two-photon excitation of chlorophyll a and b in the higher plant main light-harvesting complex (LHC II) and the minor complex CP29 (as well as in organic solution) with 100-fs pulses in the Q/sub y/ region results in a weak blue fluorescence. The dependence of the spectral shape of the blue fluorescence on excitation wavelength offers a new approach to elucidate the long-standing problem of the origin of spectral "chlorophyll forms" in pigment-protein complexes, in particular the characterization of chlorophyll a/b-heterodimers. As a first result we present evidence for the existence of strong chlorophyll a/b-interactions (excitonically coupled transitions at 650 and 680 nm) in LHC II at ambient temperature. In comparison with LHC II, the experiments with CP29 provide further evidence that the lowest energy chlorophyll a transition (at ~680 nm) is not excitonically coupled to chlorophyll b. (22 refs).

  6. Pulse-shaping based two-photon FRET stoichiometry.

    Science.gov (United States)

    Flynn, Daniel C; Bhagwat, Amar R; Brenner, Meredith H; Núñez, Marcos F; Mork, Briana E; Cai, Dawen; Swanson, Joel A; Ogilvie, Jennifer P

    2015-02-09

    Förster Resonance Energy Transfer (FRET) based measurements that calculate the stoichiometry of intermolecular interactions in living cells have recently been demonstrated, where the technique utilizes selective one-photon excitation of donor and acceptor fluorophores to isolate the pure FRET signal. Here, we present work towards extending this FRET stoichiometry method to employ two-photon excitation using a pulse-shaping methodology. In pulse-shaping, frequency-dependent phases are applied to a broadband femtosecond laser pulse to tailor the two-photon excitation conditions to preferentially excite donor and acceptor fluorophores. We have also generalized the existing stoichiometry theory to account for additional cross-talk terms that are non-vanishing under two-photon excitation conditions. Using the generalized theory we demonstrate two-photon FRET stoichiometry in live COS-7 cells expressing fluorescent proteins mAmetrine as the donor and tdTomato as the acceptor.

  7. Adiabatic following in two-photon transition

    Energy Technology Data Exchange (ETDEWEB)

    Nayfeh, M.H.; Nayfeh, A.H.

    1977-03-01

    The coherent interaction of two smoothly varying, near-resonant, two-photon pulses with a three-level system can be described by ''two-photon damped Bloch equations'' which are analogous to those for a one-photon transition in a two-level system except for the presence of a two-photon coupling and a frequency shift. These equations are solved for the cases ..gamma../sub 1/, ..gamma../sub 2/ very-much-less-than ..cap omega.., ..gamma../sub 1/ = ..gamma../sub 2/, and ..gamma../sub 2/k/sup 2/epsilon/sup 4//..cap omega../sup 2/, ..gamma../sub 1/ very-much-less-than ..cap omega.., where ..gamma../sub 1/ and ..gamma../sub 2/ are the atomic energy and phase relaxation widths, respectively, and ..cap omega.. is the Rabi frequency. The leading contribution to the refractive index is intensity dependent, caused by the level shifts inherent in multiphoton processes; it includes a relaxation dependent part which is important at times shorter than ..gamma../sup -1//sub 1/. The second-order contributions depend on the square of the intensity and the time-integrated square of the intensity. The latter contribution, which is relaxation dependent, causes line asymmetry at the long-wavelength wing; it consists of a term proportional to ..gamma../sub 2/-..gamma../sub 1/ and only important at early times and a term proportional to 2..gamma../sub 2/-..gamma../sub 1/.

  8. Two-photon processes in highly charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Jahrsetz, Thorsten

    2015-03-05

    Two-photon processes are atomic processes in which an atom interacts simultaneously with two photons. Such processes describe a wide range of phenomena, such as two-photon decay and elastic or inelastic scattering of photons. In recent years two-photon processes involving highly charged heavy ions have become an active area of research. Such studies do not only consider the total transition or scattering rates but also their angular and polarization dependence. To support such examinations in this thesis I present a theoretical framework to describe these properties in all two-photon processes with bound initial and final states and involving heavy H-like or He-like ions. I demonstrate how this framework can be used in some detailed studies of different two-photon processes. Specifically a detailed analysis of two-photon decay of H-like and He-like ions in strong external electromagnetic fields shows the importance of considering the effect of such fields for the physics of such systems. Furthermore I studied the elastic Rayleigh as well as inelastic Raman scattering by heavy H-like ions. I found a number of previously unobserved phenomena in the angular and polarization dependence of the scattering cross-sections that do not only allow to study interesting details of the electronic structure of the ion but might also be useful for the measurement of weak physical effects in such systems.

  9. Two-Photon Flow Cytometry

    Science.gov (United States)

    Zhog, Cheng Frank; Ye, Jing Yong; Norris, Theodore B.; Myc, Andrzej; Cao, Zhengyl; Bielinska, Anna; Thomas, Thommey; Baker, James R., Jr.

    2004-01-01

    Flow cytometry is a powerful technique for obtaining quantitative information from fluorescence in cells. Quantitation is achieved by assuring a high degree of uniformity in the optical excitation and detection, generally by using a highly controlled flow such as is obtained via hydrodynamic focusing. In this work, we demonstrate a two-beam, two- channel detection and two-photon excitation flow cytometry (T(sup 3)FC) system that enables multi-dye analysis to be performed very simply, with greatly relaxed requirements on the fluid flow. Two-photon excitation using a femtosecond near-infrared (NIR) laser has the advantages that it enables simultaneous excitation of multiple dyes and achieves very high signal-to-noise ratio through simplified filtering and fluorescence background reduction. By matching the excitation volume to the size of a cell, single-cell detection is ensured. Labeling of cells by targeted nanoparticles with multiple fluorophores enables normalization of the fluorescence signal and thus ratiometric measurements under nonuniform excitation. Quantitative size measurements can also be done even under conditions of nonuniform flow via a two-beam layout. This innovative detection scheme not only considerably simplifies the fluid flow system and the excitation and collection optics, it opens the way to quantitative cytometry in simple and compact microfluidics systems, or in vivo. Real-time detection of fluorescent microbeads in the vasculature of mouse ear demonstrates the ability to do flow cytometry in vivo. The conditions required to perform quantitative in vivo cytometry on labeled cells will be presented.

  10. Time-resolved two-photon photoemission from metal surfaces

    CERN Document Server

    Weinelt, M

    2002-01-01

    The Rydberg-like series of image-potential states is a prototype system for loosely bound electrons at a metal surface. The electronic structure and the femtosecond dynamics of these states is studied by high-resolution energy-and time-resolved two-photon photoemission spectroscopy. The electron trapped in the image potential moves virtually freely laterally to the surface where it is subject to inelastic and quasielastic scattering processes which cause decay of population and phase relaxation. The influence of surface corrugation on these processes has been investigated for adsorbates on Cu(001) and stepped Cu(117) and Cu(119) surfaces which are vicinal to Cu(001). The dynamics depend on both the distance of the electron in front of the surface and the parallel momentum. For CO molecules on Cu(001) inelastic scattering into bulk states and adsorbate-induced resonances determine the decay rate. For small numbers of Cu adatoms on Cu(001) and the vicinal surfaces the decay rate of image-potential states is sig...

  11. Giant Two-photon Absorption in Circular Graphene Quantum Dots in Infrared Region

    Science.gov (United States)

    Feng, Xiaobo; Li, Zhisong; Li, Xin; Liu, Yingkai

    2016-01-01

    We investigate theoretically the two-photon absorption (TPA) for circular graphene quantum dots (GQDs) with the edge of armchair and zigzag on the basis of electronic energy states obtained by solving the Dirac-Weyl equation numerically under finite difference method. The expressions for TPA cross section are derived and the transition selection rules are obtained. Results reveal that the TPA is significantly greater in GQDs than conventional semiconductor QDs in infrared spectrum (2–6 um) with a resonant TPA cross section of up to 1011 GM. The TPA peaks are tuned by the GQDs’ size, edge and electron relaxation rate. PMID:27629800

  12. Giant Two-photon Absorption in Circular Graphene Quantum Dots in Infrared Region

    Science.gov (United States)

    Feng, Xiaobo; Li, Zhisong; Li, Xin; Liu, Yingkai

    2016-09-01

    We investigate theoretically the two-photon absorption (TPA) for circular graphene quantum dots (GQDs) with the edge of armchair and zigzag on the basis of electronic energy states obtained by solving the Dirac-Weyl equation numerically under finite difference method. The expressions for TPA cross section are derived and the transition selection rules are obtained. Results reveal that the TPA is significantly greater in GQDs than conventional semiconductor QDs in infrared spectrum (2-6 um) with a resonant TPA cross section of up to 1011 GM. The TPA peaks are tuned by the GQDs’ size, edge and electron relaxation rate.

  13. Two-Photon Photoemission Study of Competing Auger and Surface-Mediated Relaxation of Hot Electrons in CdSe Quantum Dot Solids

    NARCIS (Netherlands)

    Sippel, P.; Albrecht, W.; Mitoraj, D.; Eichberger, R.; Hannappel, T.; Vanmaekelbergh, D.A.M.

    2013-01-01

    Solids composed of colloidal quantum dots hold promise for third generation highly efficient thin-film photovoltaic cells. The presence of well-separated conduction electron states opens the possibility for an energy-selective collection of hot and equilibrated carriers, pushing the efficiency above

  14. Interaction of poxvirus intracellular mature virion proteins with the TPR domain of kinesin light chain in live infected cells revealed by two-photon-induced fluorescence resonance energy transfer fluorescence lifetime imaging microscopy.

    Science.gov (United States)

    Jeshtadi, Ananya; Burgos, Pierre; Stubbs, Christopher D; Parker, Anthony W; King, Linda A; Skinner, Michael A; Botchway, Stanley W

    2010-12-01

    Using two-photon-induced fluorescence lifetime imaging microscopy, we corroborate an interaction (previously demonstrated by yeast two-hybrid domain analysis) of full-length vaccinia virus (VACV; an orthopoxvirus) A36 protein with the cellular microtubule motor protein kinesin. Quenching of enhanced green fluorescent protein (EGFP), fused to the C terminus of VACV A36, by monomeric red fluorescent protein (mDsRed), fused to the tetratricopeptide repeat (TPR) domain of kinesin, was observed in live chicken embryo fibroblasts infected with either modified vaccinia virus Ankara (MVA) or wild-type fowlpox virus (FWPV; an avipoxvirus), and the excited-state fluorescence lifetime of EGFP was reduced from 2.5 ± 0.1 ns to 2.1 ± 0.1 ns due to resonance energy transfer to mDsRed. FWPV does not encode an equivalent of intracellular enveloped virion surface protein A36, yet it is likely that this virus too must interact with kinesin to facilitate intracellular virion transport. To investigate possible interactions between innate FWPV proteins and kinesin, recombinant FWPVs expressing EGFP fused to the N termini of FWPV structural proteins Fpv140, Fpv168, Fpv191, and Fpv198 (equivalent to VACV H3, A4, p4c, and A34, respectively) were generated. EGFP fusions of intracellular mature virion (IMV) surface protein Fpv140 and type II membrane protein Fpv198 were quenched by mDsRed-TPR in recombinant FWPV-infected cells, indicating that these virion proteins are found within 10 nm of mDsRed-TPR. In contrast, and as expected, EGFP fusions of the IMV core protein Fpv168 did not show any quenching. Interestingly, the p4c-like protein Fpv191, which demonstrates late association with preassembled IMV, also did not show any quenching.

  15. Spectroscopic Study of ThCl+ by Two-Photon Ionization

    Science.gov (United States)

    Bartlett, Joshua; VanGundy, Robert A.; Heaven, Michael; Peterson, Kirk

    2016-06-01

    Despite the irreplaceable role experimental data plays for evaluating the performance of computational predictions, diatomic actinide species have not received much spectroscopic attention. As an early actinide element, thorium-containing species are ideal candidates for these types of studies. The electronic structure is expected to be relatively simple compared to later actinides, and therefore allows straightforward assessment of calculations. Here, we have studied ThCl+ for the first time via resonant two-photon ionization of jet-cooled ThCl produced by laser ablation of the metal reacted with dilute Cl2. Laser-induced Fluorescence (LIF) spectra have been recorded for the neutral molecule from 16000 - 23500 cm-1 in search of a suitable intermediate state for subsequent two-photon ionization experiments. Monochromator dispersion of the fluorescence has recovered the ground state vibration and anharmonic constants of ThCl. Resonant Two-Photon Ionization (R2PI) within a time-of-flight mass spectrometer was used to confirm ThCl production, and Pulsed Field Ionization Zero Kinetic Energy photoelectron spectroscopy (PFI-ZEKE) has been performed to identify the ionization energy as well as several of the low-lying states of the ThCl+ molecule. These constants have been predicted at the CASPT2 and CCSD(T) levels of theory, and a discussion of the calculations' performance will be presented alongside the recorded spectra.

  16. Relativistic evaluation of the two-photon decay of the metastable ${1s}^{2} 2s 2p~^3\\mbox{P}_0$ state in berylliumlike ions with an active-electron model

    CERN Document Server

    Amaro, Pedro; Safari, Laleh; Machado, Jorge; Guerra, Mauro; Indelicato, Paul; Santos, José Paulo

    2015-01-01

    The two-photon ${1s}^{2} 2s 2p~^3\\mbox{P}_0 \\rightarrow {1s}^{2} {2s}^2$ $^1\\mbox{S}_0$ transition in berylliumlike ions is theoretically investigated within a full relativistic framework and a second-order perturbation theory. We focus our analysis on how electron correlation, as well as the negative-energy spectrum can affect the forbidden $E1M1$ decay rate. For this purpose we include the electronic correlation by an effective potential and within an active-electron model. Due to its experimental interest, evaluation of decay rates are performed for berylliumlike xenon and uranium. We find that the negative-energy contribution can be neglected in the present decay rate. On the other hand, if contributions of electronic correlation are not carefully taken into account, it may change the lifetime of the metastable state by 20\\%. By performing a full-relativistic $jj$-coupling calculation, we found discrepancies for the decay rate of an order of 2 compared to non-relativistic $LS$-coupling calculations, for t...

  17. Hybrid simulation of electron cyclotron resonance heating

    CERN Document Server

    Ropponen, T; Suominen, P; Koponen, T K; Kalvas, T; Koivisto, H

    2008-01-01

    Electron Cyclotron Resonance (ECR) heating is a fundamentally important aspect in understanding the physics of Electron Cyclotron Resonance Ion Sources (ECRIS). Absorption of the radio frequency (RF) microwave power by electron heating in the resonance zone depends on many parameters including frequency and electric field strength of the microwave, magnetic field structure and electron and ion density profiles. ECR absorption has been studied in the past by e.g. modelling electric field behaviour in the resonance zone and its near proximity. This paper introduces a new ECR heating code that implements damping of the microwave power in the vicinity of the resonance zone, utilizes electron density profiles and uses right hand circularly polarized (RHCP) electromagnetic waves to simulate electron heating in ECRIS plasma.

  18. Hybrid simulation of electron cyclotron resonance heating

    Energy Technology Data Exchange (ETDEWEB)

    Ropponen, T. [Department of Physics, University of Jyvaeskylae, P.O. Box 35, FI-40014 (Finland)], E-mail: tommi.ropponen@phys.jyu.fi; Tarvainen, O. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States); Suominen, P. [CERN Geneve 23, CH-1211 (Switzerland); Koponen, T.K. [Department of Physics, University of Jyvaeskylae, Nanoscience Center, P.O. Box 35, FI-40014 (Finland); Kalvas, T.; Koivisto, H. [Department of Physics, University of Jyvaeskylae, P.O. Box 35, FI-40014 (Finland)

    2008-03-11

    Electron Cyclotron Resonance (ECR) heating is a fundamentally important aspect in understanding the physics of Electron Cyclotron Resonance Ion Sources (ECRIS). Absorption of the radio frequency (RF) microwave power by electron heating in the resonance zone depends on many parameters including frequency and electric field strength of the microwave, magnetic field structure and electron and ion density profiles. ECR absorption has been studied in the past by e.g. modelling electric field behaviour in the resonance zone and its near proximity. This paper introduces a new ECR heating code that implements damping of the microwave power in the vicinity of the resonance zone, utilizes electron density profiles and uses right hand circularly polarized (RHCP) electromagnetic waves to simulate electron heating in ECRIS plasma.

  19. Theoretical foundations of electron spin resonance

    CERN Document Server

    Harriman, John E

    2013-01-01

    Theoretical Foundations of Electron Spin Resonance deals with the theoretical approach to electron paramagnetic resonance. The book discusses electron spin resonance in applications related to polyatomic, probably organic, free radicals in condensed phases. The book also focuses on essentially static phenomena, that is, the description and determination of stationary-state energy levels. The author reviews the Dirac theory of the electron in which a four-component wave function is responsible for the behavior of the electron. The author then connects this theory with the nonrelativistic wave f

  20. Holographic Two-Photon Induced Photopolymerization

    Data.gov (United States)

    Federal Laboratory Consortium — Holographic two-photon-induced photopolymerization (HTPIP) offers distinct advantages over conventional one-photon-induced photopolymerization and current techniques...

  1. Two-Photon Absorption of Metal-Assisted Chromophores.

    Science.gov (United States)

    Li, Xin; Rinkevicius, Zilvinas; Ågren, Hans

    2014-12-09

    Aiming to understand the effect of a metal surface on nonlinear optical properties and the combined effects of surface and solvent environments on such properties, we present a multiscale response theory study, integrated with dynamics of the two-photon absorption of 4-nitro-4'-amino-trans-stilbene physisorbed on noble metal surfaces, considering two such surfaces, Ag(111) and Au(111), and two solvents, cyclohexane and water, as cases for demonstration. A few conclusions of general character could be drawn: While the geometrical change of the chromophore induced by the environment was found to notably alter (diminish) the two-photon absorption cross section in the polar medium, the effects of the metal surface and solvent on the electronic structure of the chromophore surpasses the geometrical effects and leads to a considerably enhanced two-photon absorption cross section in the polar solvent. This enhancement of two-photon absorption arises essentially from the metal charge image induced enlargement of the difference between the dipole moment of the excited state and the ground state. The orientation-dependence of the two-photon absorption is found to connect with the lateral rotation of the chromophore, where the two-photon absorption reaches its maximum when the polarization of the incident light coincides with the long-axis of the chromophore. Our results demonstrate a distinct enhancement of the two-photon absorption by a metal surface and a polar medium and envisage the employment of metal-chromophore composite materials for future development of nonlinear optical materials with desirable properties.

  2. Three-dimensional microfabrication using two-photon polymerization

    Science.gov (United States)

    Cumpston, Brian H.; Ehrlich, Jeffrey E.; Kuebler, Stephen M.; Lipson, Matthew; Marder, Seth R.; McCord-Maughon, D.; Perry, Joseph W.; Roeckel, Harold; Rumi, Maria Cristina

    1998-09-01

    Photopolymerization initiated by the simultaneous absorption of two photons is unique in its ability to produce complex three-dimensional (3D) structures from a single, thick photopolymer film. Strong 3D confinement of the polymerization process is not possible in other polymer microfabrication techniques such as LIGA, rapid prototyping, and conventional photoresist technology. Two-photon polymerization also permits the fabrication of 3D structures and the definition of lithographic features on non-planar surfaces. We have developed a wide array of chromophores which hold great promise for 3D microfabrication, as well as other applications, such as two-photon fluorescence imaging and 3D optical data storage. These materials are based on a donor- (pi) -donor, donor-acceptor-donor, or acceptor-donor-acceptor structural motif. The magnitude of the two-photon absorption cross-section, (delta) , and the position of the two-photon absorption maximum, (lambda) (2)max, can be controlled by varying the length of the conjugated bridge and by varying the strength of the donor/acceptor groups. In this way, chromophores have been developed which exhibit strong two- photon absorption in the range of 500 - 975 nm, in some cases as high as 4400 X 10-50 cm4 s/photon-molecule. In the case of donor-(pi) -donor structures, quantum-chemical calculations show that the large absorption cross-sections arise from the symmetric re-distribution of charge from the donor end-groups to the conjugated bridge, resulting in an electronic excited-state which is more delocalized than the ground state. For many of these molecules, two-photon excitation populates a state which is sufficiently reducing that a charge transfer reaction can occur with acrylate monomers. The efficiency of these processes can be described using Marcus theory. Under suitable conditions, such reactions can induce radical polymerization of acrylate resins. Polymerization rates have been measured, and we show that these two-photon

  3. Coverage-dependent two-photon photoexcitation at the H2O/TiO2 interface

    Science.gov (United States)

    Payne, D. T.; Zhang, Y.; Pang, C. L.; Fielding, H. H.; Thornton, G.

    2016-10-01

    Excited electrons and holes are crucial for redox reactions on metal oxide surfaces. However, precise details of this charge transfer process are not known. We report two-photon photoemission (hν = 3.23 eV) measurements of rutile TiO2(110) as a function of exposure to water below room temperature. The two-photon resonance associated with bridging hydroxyls is enhanced following water exposure, reaching a maximum at a nominal coverage of one monolayer. Higher coverages attenuate the observed resonance. Ultraviolet photoemission spectroscopy (hν = 21.22 eV) of the initial, band gap states shows little change up to one monolayer water coverage. It is likely that the enhancement arises from dissociation within the adsorbed water monolayer, although other mechanisms cannot be excluded.

  4. Search for New Physics with Two Photons in the Final State with the ATLAS Detector

    CERN Document Server

    AUTHOR|(INSPIRE)INSPIRE-00441752

    This thesis reports on the search for new physics in the diphoton decay channel with the proton-proton collision data collected by ATLAS at a centre-of-mass energy of $\\sqrt{s}=8$~TeV in 2012 and $\\sqrt{s}=13$~TeV in 2015 and 2016. A feasibility study of the search for a pseudoscalar $A$ decaying to a $Z$ boson and a 125~GeV Higgs boson in the context of an extended Higgs sector, namedly the two-Higgs-doublet models, is presented. The search is performed with a final state of two jets and two photons using 20.3~${\\rm fb}^{-1}$ of data at $\\sqrt{s}=8$~TeV. The expected sensitivity is found to be competitive with the analysis with a final state of two electrons or muons and two $\\tau$ leptons, but less sensitive to the other searches with the Higgs decaying to a pair of $b$-quarks.%, due to the low branching ratios of the Higgs to two photons decay. Search for high mass resonances decaying to two photons at $\\sqrt{s}=13$~TeV is also presented. The analysed dataset corresponds to an integrated luminosity of $3.2...

  5. Fano interference in two-photon transport

    Science.gov (United States)

    Xu, Shanshan; Fan, Shanhui

    2016-10-01

    We present a general input-output formalism for the few-photon transport in multiple waveguide channels coupled to a local cavity. Using this formalism, we study the effect of Fano interference in two-photon quantum transport. We show that the physics of Fano interference can manifest as an asymmetric spectral line shape in the frequency dependence of the two-photon correlation function. The two-photon fluorescence spectrum, on the other hand, does not exhibit the physics of Fano interference.

  6. Simultaneous two-photon excitation of photodynamic therapy agents

    Energy Technology Data Exchange (ETDEWEB)

    Wachter, E.A.; Fisher, W.G. [Oak Ridge National Lab., TN (United States)]|[Photogen, Inc., Knoxville, TN (United States); Partridge, W.P. [Oak Ridge National Lab., TN (United States); Dees, H.C. [Photogen, Inc., Knoxville, TN (United States); Petersen, M.G. [Univ. of Tennessee, Knoxville, TN (United States). College of Veterinary Medicine

    1998-01-01

    The spectroscopic and photochemical properties of several photosensitive compounds are compared using conventional single-photon excitation (SPE) and simultaneous two-photon excitation (TPE). TPE is achieved using a mode-locked titanium:sapphire laser, the near infrared output of which allows direct promotion of non-resonant TPE. Excitation spectra and excited state properties of both type 1 and type 2 photodynamic therapy (PDT) agents are examined.

  7. Hyperfine selectivity using multiquantum electron-nuclear-electron triple resonance

    Science.gov (United States)

    Christidis, T. C.; Mchaourab, Hassane S.; Hyde, James S.

    1996-06-01

    Hyperfine selectivity is demonstrated in a continuous wave electron-nuclear double resonance (ENDOR) experiment. A multiquantum electron-electron double resonance (ELDOR) signal is monitored as a function of the nuclear radio frequency. The signs and relative intensities of the ENDOR lines permit separating the case where both ELDOR and ENDOR frequencies match hyperfine couplings from the cases where this condition is not satisfied.

  8. Electronic dipole resonance in smoky quartz

    NARCIS (Netherlands)

    Kerssen, J.; Volger, J.

    1967-01-01

    Microwave absorption in smoky quartz mono-crystal is ascribed to resonance transitions of trapped electrons between initially configurational degenerated states, which are Stark-splitted by a polarizing electric field.

  9. Quantum Effect in Mesoscopic Open Electron Resonator

    Institute of Scientific and Technical Information of China (English)

    YAN Zhan-Yuan; ZHANG Xiao-Hong; HAN Ying-Hui

    2008-01-01

    The open electron resonator is a mesoscopic device that has attracted considerable attention due to its remarkable behavior: conductance oscillations. In this paper, using an improved quantum theory to mesoscopic circuits developed recently by Li and Chen, the mesoscopic electron resonator is quantized based on the fundamental fact that the electric charge takes discrete value. With presentation transformation and unitary transformation, the Schrodinger equation becomes an standard Mathieu equation. Then, the detailed energy spectrum and wave functions in the system are obtained, which will be helpful to the observation of other characters of electron resonator. The average of currents and square of the current are calculated, the results show the existence of the current fluctuation, which causes the noise in the circuits, the influence of inductance to the noise is discussed. With the results achieved, the stability characters of mesoscopic electron resonator are studied firstly, these works would be benefit to the design and control of integrate circuit.

  10. Two-Photon-Pumped Perovskite Semiconductor Nanocrystal Lasers.

    Science.gov (United States)

    Xu, Yanqing; Chen, Qi; Zhang, Chunfeng; Wang, Rui; Wu, Hua; Zhang, Xiaoyu; Xing, Guichuan; Yu, William W; Wang, Xiaoyong; Zhang, Yu; Xiao, Min

    2016-03-23

    Two-photon-pumped lasers have been regarded as a promising strategy to achieve frequency up-conversion for situations where the condition of phase matching required by conventional approaches cannot be fulfilled. However, their practical applications have been hindered by the lack of materials holding both efficient two-photon absorption and ease of achieving population inversion. Here, we show that this challenge can be tackled by employing colloidal nanocrystals of perovskite semiconductors. We observe highly efficient two-photon absorption (with a cross section of 2.7 × 10(6) GM) in toluene solutions of CsPbBr3 nanocrystals that can excite large optical gain (>500 cm(-1)) in thin films. We have succeeded in demonstrating stable two-photon-pumped lasing at a remarkable low threshold by coupling CsPbBr3 nanocrystals with microtubule resonators. Our findings suggest perovskite nanocrystals can be used as excellent gain medium for high-performance frequency-up-conversion lasers toward practical applications.

  11. Correlations of two photons at hadron colliders

    OpenAIRE

    Kozlov, G. A.

    2011-01-01

    We study the Bose-Einstein correlations of two photons and their coherent properties that can provide the information about the space-time structure of the emitting source through the Higgs-boson decays into two photons. We argue that such an investigation could probe the Higgs-boson mass. The model is rather sensitive to the temperature of the environment and to the external distortion effect in medium.

  12. Pulsed electron-nuclear-electron triple resonance spectroscopy

    Science.gov (United States)

    Thomann, Hans; Bernardo, Marcelino

    1990-05-01

    A new experimental technique, pulsed electron-nuclear-electron triple resonance spectroscopy, is demonstrated. It is based on a modification of the pulse sequence for electron-nuclear double resonance (ENDOR) in which two EPR and one NMR transition are irradiated. The irradiation of one EPR transition is detected via a second EPR transition. The nuclear hyperfine coupling, which separates these EPR transition frequencies, is the irradiated NMR transition. The major advantages of triple resonance spectroscopy include the ability to resolve overlapping nuclear resonances in the ENDOR spectrum and a more direct quantitative assignment of nuclear hyperfine and quadrupole couplings. The triple resonance experiment is an alternative to the recently proposed method of employing rapid magnetic field jumps between microwave pulses for generating hyperfine selective ENDOR spectra.

  13. Electron cyclotron resonance heating on TEXTOR

    NARCIS (Netherlands)

    Westerhof, E.; Hoekzema, J. A.; Hogeweij, G. M. D.; Jaspers, R. J. E.; Schüller, F. C.; Barth, C. J.; Bongers, W. A.; Donne, A. J. H.; Dumortier, P.; van der Grift, A. F.; van Gorkom, J. C.; Kalupin, D.; Koslowski, H. R.; Kramer-Flecken, A.; Kruijt, O. G.; Cardozo, N. J. L.; Mantica, P.; van der Meiden, H. J.; Merkulov, A.; Messiaen, A.; Oosterbeek, J. W.; Oyevaar, T.; Poelman, A. J.; Polman, R. W.; Prins, P. R.; Scholten, J.; Sterk, A. B.; Tito, C. J.; Udintsev, V.S.; Unterberg, B.; Vervier, M.; van Wassenhove, G.

    2003-01-01

    The 110 GHz and the new 140 GHz gyrotron systems for electron cyclotron resonance heating (ECRH) and ECCD on TEXTOR are described and results of ECRH experiments with the 110 GHz system are reported. Central ECRH on Ohmic plasmas shows the presence of an internal electron transport barrier near q =

  14. Direct frequency comb two-photon laser cooling and trapping

    Science.gov (United States)

    Jayich, Andrew; Long, Xueping; Campbell, Wesley C.

    2016-05-01

    Generating and manipulating high energy photons for spectroscopy on electric dipole transitions of atoms and molecules with deeply bound valence electrons is difficult. Further, laser cooling of such species is even more challenging for lack of laser power. A possible solution is to drive two-photon transitions. This may alleviate the photon energy problem and open the door to cold, trapped samples of highly desirable species with tightly bound electrons. We perform a proof of principle experiment with rubidium by driving a two-photon transition with an optical frequency comb. We perform optical cooling and extend this technique to trapping, where we are able to make a magneto-optical trap in one dimension. This work is supported by the National Science Foundation CAREER program.

  15. Medical prototyping using two photon polymerization

    Directory of Open Access Journals (Sweden)

    Roger J Narayan

    2010-12-01

    Full Text Available Two photon polymerization involves nearly simultaneous absorption of ultrashort laser pulses for selective curing of photosensitive material. This process has recently been used to create small-scale medical devices out of several classes of photosensitive materials, such as acrylate-based polymers, organically-modified ceramic materials, zirconium sol-gels, and titanium-containing hybrid materials. In this review, the use of two photon polymerization for fabrication of several types of small-scale medical devices, including microneedles, artificial tissues, microfluidic devices, pumps, sensors, and valves, from computer models is described. Necessary steps in the development of two photon polymerization as a commercially viable medical device manufacturing method are also considered.

  16. Two Photon Couplings of Hybrid Mesons

    CERN Document Server

    Page, P R

    1996-01-01

    A new formalism is developed for the two photon production of hybrid mesons via intermediate hadronic decays. In an adiabatic and non--relativistic context with spin 1 pair creation we obtain the first absolute estimates of unmixed hybrid production strengths to be small (0.03 - 3 eV) in relation to experimental meson widths (0.1 - 5 keV). Within this context, two photon collisions therefore strongly discriminate between hybrid and conventional meson wave function components at BaBar, Cleo II, LEP2 and LHC, filtering out non--gluonic components. Decay widths of unmixed hybrids are tiny. The formalism also induces conventional meson two photon widths roughly in agreement with experiment.

  17. Study of charmonia in four-meson final states produced in two-photon collisions

    CERN Document Server

    Uehara, S; Aihara, H; Aulchenko, V; Aushev, T; Bakich, A M; Balagura, V; Barberio, E; Bay, A; Belous, K S; Bitenc, U; Bondar, A; Bozek, A; Bracko, M; Brodzicka, J; Browder, T E; Chang, P; Chao, Y; Chen, A; Chen, K F; Chen, W T; Cheon, B G; Cho, I S; Choi, Y; Choi, Y K; Dalseno, J; Dash, M; Drutskoy, A; Eidelman, S; Epifanov, D; Fratina, S; Gabyshev, N; Gokhroo, G; Golob, B; Ha, H; Haba, J; Hayasaka, K; Hayashii, H; Hazumi, M; Heffernan, D; Hokuue, T; Hoshi, Y; Hou, W S; Hyun, H J; Iijima, T; Ikado, K; Inami, K; Ishikawa, A; Itoh, R; Iwasaki, M; Iwasaki, Y; Kah, D H; Kaji, H; Kang, J H; Kawai, H; Kawasaki, T; Kichimi, H; Kim, H O; Kim, S K; Kim, Y J; Korpar, S; Krizan, P; Krokovny, P; Kumar, R; Kuo, C C; Kuzmin, A; Kwon, Y J; Lee, J S; Lee, M J; Lee, S E; Lesiak, T; Li, J; Limosani, A; Lin, S W; Liu, Y; Liventsev, D; Mandl, F; Matsumoto, T; Matyja, A; McOnie, S; Medvedeva, T; Miyake, H; Miyata, H; Miyazaki, Y; Mizuk, R; Nagasaka, Y; Nakano, E; Nakao, M; Nakazawa, H; Natkaniec, Z; Nishida, S; Nitoh, O; Ogawa, S; Ohshima, T; Okuno, S; Olsen, S L; Onuki, Y; Ozaki, H; Pakhlov, P; Pakhlova, G; Palka, H; Park, C W; Park, H; Peak, L S; Pestotnik, R; Piilonen, L E; Sahoo, H; Sakai, Y; Schneider, O; Seidl, R; Senyo, K; Sevior, M E; Shapkin, M; Shibuya, H; Shiu, J G; Shwartz, B; Singh, J B; Sokolov, A; Somov, A; Soni, N; Stanic, S; Staric, M; Stöck, H; Sumiyoshi, T; Takasaki, F; Tamai, K; Tanaka, M; Taylor, G N; Teramoto, Y; Tian, X C; Tikhomirov, I; Tsuboyama, T; Unno, Y; Uno, S; Urquijo, P; Usov, Yu; Varner, G; Vervink, K; Villa, S; Vinokurova, A; Wang, C H; Wang, P; Watanabe, Y; Won, E; Yabsley, B D; Yamaguchi, A; Yamashita, Y; Yuan, C Z; Zhang, C C; Zhang, Z P; Zhilich, V; Zupanc, A

    2008-01-01

    We report measurements of charmonia produced in two-photon collisions and decaying to four-meson final states, where the meson is either a charged pion or a charged kaon. The analysis is based on a 395fb^{-1} data sample accumulated with the Belle detector at the KEKB electron-positron collider. We observe signals for the three C-even charmonia eta_c(1S), chi_{c0}(1P) and chi_{c2}(1P) in the pi^+pi^-pi^+pi^-, K^+K^-pi^+pi^- and K^+K^-K^+K^- decay modes. No clear signals for eta_c(2S) production are found in these decay modes. We have also studied resonant structures in charmonium decays to two-body intermediate meson resonances. We report the products of the two-photon decay width and the branching fractions, Gamma_{gamma gamma}B, for each of the charmonium decay modes.

  18. A new approach to dual-color two-photon microscopy with fluorescent proteins

    Directory of Open Access Journals (Sweden)

    Rebane Aleks

    2010-02-01

    Full Text Available Abstract Background Two-photon dual-color imaging of tissues and cells labeled with fluorescent proteins (FPs is challenging because most two-photon microscopes only provide one laser excitation wavelength at a time. At present, methods for two-photon dual-color imaging are limited due to the requirement of large differences in Stokes shifts between the FPs used and their low two-photon absorption (2PA efficiency. Results Here we present a new method of dual-color two-photon microscopy that uses the simultaneous excitation of the lowest-energy electronic transition of a blue fluorescent protein and a higher-energy electronic transition of a red fluorescent protein. Conclusion Our method does not require large differences in Stokes shifts and can be extended to a variety of FP pairs with larger 2PA efficiency and more optimal imaging properties.

  19. Stability of the Electron Cyclotron Resonance

    Science.gov (United States)

    Asch, Joachim; Bourget, Olivier; Meresse, Cédric

    2015-12-01

    We consider the magnetic AC Stark effect for the quantum dynamics of a single particle in the plane under the influence of an oscillating homogeneous electric and a constant perpendicular magnetic field. We prove that the electron cyclotron resonance is insensitive to impurity potentials.

  20. Undergraduate Electron-Spin-Resonance Experiment.

    Science.gov (United States)

    Willis, James S.

    1980-01-01

    Describes the basic procedures for use of an electron-spin resonance spectrometer and potassium azide (KN3) in an experiment which extends from the phase of sample preparation (crystal growth, sample mounting, and orientation) through data taking to the stages of calculation and theoretical explanation. (Author/DS)

  1. Numerical methods in electron magnetic resonance

    Energy Technology Data Exchange (ETDEWEB)

    Soernes, A.R

    1998-07-01

    The focal point of the thesis is the development and use of numerical methods in the analysis, simulation and interpretation of Electron Magnetic Resonance experiments on free radicals in solids to uncover the structure, the dynamics and the environment of the system.

  2. Dicke Coherent Narrowing in Two-Photon and Raman Spectroscopy of Thin Vapour Cells

    CERN Document Server

    Dutier, G; Hamdi, I; Maurin, I; Saltiel, S; Bloch, D; Ducloy, M; Dutier, Gabriel; Todorov, Petko; Hamdi, Ismah\\`{e}ne; Maurin, Isabelle; Saltiel, Solomon; Bloch, Daniel; Ducloy, Martial

    2005-01-01

    The principle of coherent Dicke narrowing in a thin vapour cell, in which sub-Doppler spectral lineshapes are observed under a normal irradiation for a l/2 thickness, is generalized to two-photon spectroscopy. Only the sum of the two wave vectors must be normal to the cell, making the two-photon scheme highly versatile. A comparison is provided between the Dicke narrowing with copropagating fields, and the residual Doppler-broadening occurring with counterpropagating geometries. The experimental feasibility is discussed on the basis of a first observation of a two-photon resonance in a 300 nm-thick Cs cell. Extension to the Raman situation is finally considered.

  3. Two-photon excited ultraviolet photoluminescence of zinc oxide nanorods.

    Science.gov (United States)

    Zhu, Guangping; Xu, Chunxiang; Zhu, Jing; Lu, Changgui; Cui, Yiping; Sun, Xiaowei

    2008-11-01

    High density zinc oxide nanorods with uniform size were synthesized on (100) silicon substrate by vapor-phase transport method. The scanning electron microscopy images reveal that the nanorods have an average diameter of about 400 nm. The X-ray diffraction pattern demonstrates the wurtzite crystalline structure of the ZnO nanorods growing along [0001] direction. The single-photon excited photoluminescence presents a strong ultraviolet emission band at 394 nm and a weak visible emission band at 600 nm. When the ZnO nanorods were respectively pumped by various wavelength lasers from 520 nm to 700 nm, two-photon excited ultraviolet photoluminescence was observed. The dependence of the two-photon excited photoluminescence intensity on the excitation wavelength and power was investigated in detail.

  4. Two-photon interaction between trapped ions and cavity fields

    CERN Document Server

    Semião, F L

    2006-01-01

    In this paper, we generalize the ordinary two-photon Jaynes-Cummings model (TPJCM) by considering the atom (or ion) to be trapped in a simple harmonic well. A typical setup would be an optical cavity containing a single ion in a Paul trap. Due to the inclusion of atomic vibrational motion, the atom-field coupling becomes highly nonlinear what brings out quite different behaviors for the system dynamics when compared to the ordinary TPJCM. In particular, we derive an effective two-photon Hamiltonian with dependence on the number operator of the ion's center-of-mass motion. This dependence occurs both in the cavity induced Stark-shifs and in the ion-field coupling, and its role in the dynamics is illustrated by showing the time evolution of the probability of occupation of the electronic levels for simple initial preparations of the state of the system.

  5. Two-photon quantum interference in plasmonics: theory and applications.

    Science.gov (United States)

    Gupta, S Dutta; Agarwal, G S

    2014-01-15

    We report perfect two-photon quantum interference with near-unity visibility in a resonant tunneling plasmonic structure in folded Kretschmann geometry. This is despite absorption-induced loss of unitarity in plasmonic systems. The effect is traced to perfect destructive interference between the squares of amplitude reflection and transmission coefficients. We further highlight yet another remarkable potential of coincidence measurements as a probe with better resolution as compared to standard spectroscopic techniques. The finer features show up in both angle resolved and frequency resolved studies.

  6. Spectral Features of FM Spectroscopy of Two-Photon Interactions

    Institute of Scientific and Technical Information of China (English)

    夏慧荣; JohnL.Hall

    1994-01-01

    The spectral features of FM two-photon resonant interaction processes have been calculated for five different frequency modulation versions of counter-propagating incident fields. It is found that the proposed new modulation version (case b in the text) provides novel spectral features for a completely canceled absorption and a sharp dispersion shape at the fundamental beat note. Moreover, its absorption feature appears at the second harmonic of the RF modulation frequency generated by the joint modes via six interaction pathways without mutual phase shift. Such features persist even when the effects of the second-order sidebands of the incident fields are taken into account. Application potentials are emphasized.

  7. Two-photon photoassociative spectroscopy of ultracold 88-Sr

    CERN Document Server

    de Escobar, Y N Martinez; Pellegrini, P; Nagel, S B; Traverso, A; Yan, M; Côté, R; Killian, T C

    2008-01-01

    We present results from two-photon photoassociative spectroscopy of the least-bound vibrational level of the X$^1\\Sigma_g^+$ state of the $^{88}$Sr$_2$ dimer. Measurement of the binding energy allows us to determine the s-wave scattering length, $a_{88}=-1.4(6) a_0$. For the intermediate state, we use a bound level on the metastable $^1S_0$-$^3P_1$ potential, which provides large Franck-Condon transition factors and narrow one-photon photoassociative lines that are advantageous for observing quantum-optical effects such as Autler-Townes resonance splittings.

  8. Two-photon photoassociative spectroscopy of ultracold Sr88

    Science.gov (United States)

    Martinez de Escobar, Y. N.; Mickelson, P. G.; Pellegrini, P.; Nagel, S. B.; Traverso, A.; Yan, M.; Côté, R.; Killian, T. C.

    2008-12-01

    We present results from two-photon photoassociative spectroscopy of the least-bound vibrational level of the XΣg+1 state of the Sr288 dimer. Measurement of the binding energy allows us to determine the s -wave scattering length a88=-1.4(6)a0 . For the intermediate state, we use a bound level on the metastable S01-P13 potential, which provides large Franck-Condon transition factors and narrow one-photon photoassociative lines that are advantageous for observing quantum-optical effects such as Autler-Townes resonance splittings.

  9. Resonant electron capture by orotic acid molecules

    Science.gov (United States)

    Muftakhov, M. V.; Shchukin, P. V.; Khatymov, R. V.

    2017-09-01

    Resonant electron attachment by orotic acid molecules (6-COOH-uracil) are studied in the energy range of 0-14 eV via negative ion mass spectrometry. Molecular ions, whose lifetimes relative to electron autodetachment are found to be 300 μs are recorded in the region of thermal electron energies; they form in the valence state through a vibration-excited resonance mechanism. Unlike unsubstituted uracil, most dissociative processes occur in the low-energy region of <4 eV and are due to carboxylic anions. An absolute cross section of 2.4 × 10-17 cm2 is found for the most intense fragment ions [M-H]- at an output energy of 1.33 eV. The kinetics of decarboxylation is considered for these ions. This could be a model reaction for the last stage of uridine monophosphate biosynthesis.

  10. Ab initio study of the one- and two-photon circular dichroism of R-(+)-3-methyl-cyclopentanone

    Science.gov (United States)

    Rizzo, Antonio; Lin, Na; Ruud, Kenneth

    2008-04-01

    One- and two-photon circular dichroism spectra of R-(+)-3-methyl-cyclopentanone, a system that has been the subject of recent experimental studies of (2+1) resonance-enhanced multiphoton ionization circular dichroism, have been calculated with an origin-invariant density functional theory approximation in the region of the lowest electronic excited states, both for the gas phase and for a selection of solvents. A polarizable continuum model is used in the calculations performed on the solvated system. Two low-lying conformers are analyzed, and a comparison of the intensities and characteristic features is made with the corresponding two-photon absorption for each species, also for the Boltzmann-averaged spectra. The effect of the choice of geometry, basis set, and exchange-correlation functional is carefully analyzed. It is found that a density functional theory approach using the Coulomb attenuating method variant of Becke's three-parameter exchange and the Lee-Yang-Parr correlation functionals with correlation-consistent basis sets of double-zeta quality can reproduce the experimental electronic circular dichroism spectra very well. The features appearing in experiment are characterized in terms of molecular excitations, and the differences in the response of each state in the one- and two-photon processes are highlighted.

  11. Transparency induced by two photon interference in a beam splitter

    Institute of Scientific and Technical Information of China (English)

    Wang Kai-Ge; Yang Guo-Jian

    2004-01-01

    We propose a special two-photon state which is completely transparent in a 50/50 beam splitter. This effect is caused by the destructive two-photon interference and shows the signature of photon entanglement. We find that the symmetry of the two-photon spectrum plays the key role for the properties of two-photon interference.

  12. Electron paramagnetic resonance of transition ions

    CERN Document Server

    Abragam, A

    2012-01-01

    This book is a reissue of a classic Oxford text, and provides a comprehensive treatment of electron paramagnetic resonance of ions of the transition groups. The emphasis is on basic principles, with numerous references to publications containing further experimental results and more detailed developments of the theory. An introductory survey gives a general understanding, and a general survey presents such topics as the classical and quantum resonance equations, thespin-Hamiltonian, Endor, spin-spin and spin-lattice interactions, together with an outline of the known behaviour of ions of each

  13. Chromophore design for large two-photon absorption

    Science.gov (United States)

    Dudley, Christopher

    2014-11-01

    Conjugated oligothiophene chromophores are compared and studied for designing large linear and nonlinear absorption cross-sections. Optical properties of chromophores synthesized by the Naval Research Laboratory are modeled to construct a design factor of merit to predict and understand two-photon absorption (TPA) designs. Computer modeling to optimize parameters to produce photo active chromophores is conducted. Geometry, π-center (electron relay) and the electron donor or acceptor groups attached to the π-centers are considered for importance in TPA. This work could serve equally well as guide for quick back of the envelop research or industrial design verifications as well as an outline for introducing computation methods to students.

  14. The Nelson Model with Less Than Two Photons

    CERN Document Server

    Galtbayar, A; Yajima, K

    2002-01-01

    We study the spectral and scattering theory of the Nelson model for an atom interacting with a photon field in the subspace with less than two photons. For the free electron-photon system, the spectral property of the reduced Hamiltonian in the center of mass coordinates and the large time dynamics are determined. If the electron is under the influence of the nucleus via spatially decaying potentials, we locate the essential spectrum, prove the absence of singular continuous spectrum and the existence of the ground state, and construct wave operators giving the asymptotic dynamics.

  15. Theory of Two-Photon Absorptions in Graphene Fragments

    Science.gov (United States)

    Aryanpour, K.; Shukla, A.; Mazumdar, S.; Sandhu, A.; Roberts, A.

    2012-02-01

    Electron-electron correlations in graphene is currently an active field of research [1-3]. The carbon atoms in graphene have the same sp^2 hybridization as in strongly correlated π-conjugated polymer systems. The low energy behavior in graphene however appears to be reasonably described within the one-electron Dirac massless fermions model. Historically, the occurrence of the lowest two-photon state below the optical one-photon state provided the strongest proof for strong electron correlations in linear polyenes [4]. We systematically study the Coulomb interaction effects on the ground state and nonlinear absorptions in graphene fragments as a function of system size, beginning from the smallest stable fragment coronene. We report high order calculations of one- vs two-photon spin singlet and triplet states, in coronene, hexabenzocoronene and other molecular fragments that clearly indicate the strong role of electron-electron interactions. We will discuss the implications of our work on molecular systems for the thermodynamic limit of graphene. [4pt] [1] Siegel David A.; et al., PNAS, v108, 28, 11365-11369 (2011)[0pt] [2] Gr"onqvist J. H.; et al., arXiv: 1107.5653v1[0pt] [3] Uchoa B.; et al., arXiv: 1109.1577v1[0pt] [4] Ramasesha S.; et al., J. Chem. Phys. 80, 3278 (1984)

  16. Two-photon cooling of magnesium atoms

    DEFF Research Database (Denmark)

    Malossi, N.; Damkjær, S.; Hansen, P. L.

    2005-01-01

    A two-photon mechanism for cooling atoms below the Doppler temperature is analyzed. We consider the magnesium ladder system (3s2)S01¿(3s3p)P11 at 285.2nm followed by the (3s3p)P11¿(3s3d)D21 transition at 880.7nm . For the ladder system quantum coherence effects may become important. Combined...... with the basic two-level Doppler cooling process this allows for reduction of the atomic sample temperature by more than a factor of 10 over a broad frequency range. First experimental evidence for the two-photon cooling process is presented and compared to model calculations. Agreement between theory...... and experiment is excellent. In addition, by properly choosing the Rabi frequencies of the two optical transitions a velocity independent atomic dark state is observed....

  17. Two-photon production of charged pion and kaon pairs

    CERN Document Server

    Dominick, J; Sanghera, S; Shelkov, V; Skwarnicki, T; Stroynowski, R; Volobuev, I P; Wei, G; Zadorozhny, P; Artuso, M; Goldberg, M; He, D; Horwitz, N; Kennett, R; Mountain, R; Moneti, G C; Muheim, F; Mukhin, Y; Playfer, S; Rozen, Y; Stone, S; Thulasidas, M; Vasseur, G; Zhu, G; Bartelt, J; Csorna, S E; Egyed, Z; Jain, V; Kinoshita, K; Edwards, K W; Ogg, M; Britton, D I; Hyatt, E R F; MacFarlane, D B; Patel, P M; Akerib, D S; Barish, B C; Chadha, M; Chan, S; Cowen, D F; Eigen, G; Miller, J S; O'Grady, C; Urheim, J; Weinstein, A J; Acosta, D; Athanas, M; Masek, G E; Paar, H P; Sivertz, M; Gronberg, J B; Kutschke, R; Menary, S R; Morrison, R J; Nakanishi, S; Nelson, H N; Nelson, T K; Qiao, C; Richman, J D; Ryd, A; Tajima, H; Sperka, D; Witherell, M S; Procario, M; Balest, R; Cho, K; Daoudi, M; Ford, W T; Johnson, D R; Lingel, K; Lohner, M; Rankin, P; Smith, J G; Alexander, J P; Bebek, C; Berkelman, K; Bloom, K; Browder, T E; Cassel, David G; Cho, H A; Coffman, D M; Drell, P S; Ehrlich, R; Gaidarev, P B; Galik, R S; García-Sciveres, M; Geiser, B; Gittelman, B; Gray, S W; Hartill, D L; Heltsley, B K; Jones, C D; Jones, S L; Kandaswamy, J; Katayama, N; Kim, P C; Kreinick, D L; Ludwig, G S; Masui, J; Mevissen, J; Mistry, N B; Ng, C R; Nordberg, E; Patterson, J R; Peterson, D; Riley, D; Salman, S; Sapper, M; Würthwein, F; Avery, P; Freyberger, A P; Rodríguez, J; Stephens, R; Yang, S; Yelton, J; Cinabro, D; Henderson, S; Liu, T; Saulnier, M; Wilson, R; Yamamoto, H; Bergfeld, T; Eisenstein, B I; Gollin, G; Ong, B; Palmer, M; Selen, M; Thaler, J J; Sadoff, A J; Ammar, R; Ball, S; Baringer, P; Bean, A; Besson, D; Coppage, D; Copty, N K; Davis, R; Hancock, N; Kelly, M; Kwak, N; Lam, H; Kubota, Y; Lattery, M; Nelson, J K; Patton, S; Perticone, D; Poling, R A; Savinov, V; Schrenk, S; Wang, R; Alam, M S; Kim, I J; Nemati, B; O'Neill, J J; Severini, H; Sun, C R; Zoeller, M M; Crawford, G; Daubenmier, C M; Fulton, R; Fujino, D; Gan, K K; Honscheid, K; Kagan, H; Kass, R; Lee, J; Malchow, R L; Skovpen, Y; Sung, M; White, C; Butler, F; Fu, X; Kalbfleisch, G R; Ross, W R; Skubic, P L; Snow, J; Wang, P L; Wood, M; Brown, D N; Fast, J; McIlwain, R L; Miao, T; Miller, D H; Modesitt, M; Payne, D; Shibata, E I; Shipsey, I P J; Wang Pei Ning; Battle, M; Ernst, J; Kwon, Y; Roberts, S; Thorndike, E H; Wang, C H

    1994-01-01

    A measurement of the cross section for the combined two-photon production of charged pion and kaon pairs is performed using 1.2~\\rm fb^{-1} of data collected by the CLEO II detector at the Cornell Electron Storage Ring. The cross section is measured at invariant masses of the two-photon system between 1.5 and 5.0~GeV/c^2, and at scattering angles more than 53^\\circ away from the \\gamma\\gamma collision axis in the \\gamma\\gamma center-of-mass frame. The large background of leptonic events is suppressed by utilizing the CsI calorimeter in conjunction with the muon chamber system. The reported cross section is compared with leading order QCD models as well as previous experiments. In particular, although the functional dependence of the measured cross section disagrees with leading order QCD at small values of the two-photon invariant mass, the data show a transition to perturbative behavior at an invariant mass of approximately 2.5~GeV/c^2. hardcopies with figures can be obtained by writing to to: Pam Morehouse ...

  18. Magnetic two-photon scattering and two-photon emission - Cross sections and redistribution functions

    Science.gov (United States)

    Alexander, S. G.; Meszaros, P.

    1991-01-01

    The magnetic two-photon scattering cross section is discussed within the framework of QED, and the corresponding scattering redistribution function for this process and its inverse, as well as the scattering source function are calculated explicitly. In a similar way, the magnetic two-photon emission process which follows the radiative excitation of Landau levels above ground is calculated. The two-photon scattering and two-photon emission are of the same order as the single-photon magnetic scattering. All three of these processes, and in optically thick cases also their inverses, are included in radiative transport calculations modeling accreting pulsars and gamma-ray bursters. These processes play a prominent role in determining the relative strength of the first two cyclotron harmonics, and their effects extend also to the higher harmonics.

  19. Two-photon ionization of colliding atoms

    Energy Technology Data Exchange (ETDEWEB)

    Nayfeh, M.H.

    1977-09-01

    Semiclassical expressions of two-photon ionization of two colliding atoms are derived for a wide range of electromagnetic field intensity and detunings from the isolated atom line. The dependence of the ionization yield on the details of the interaction potential of the system is derived. This process promises an extremely sensitive method for studying line broadening on the far wing, especially when absorption or fluorescence becomes very weak.

  20. Two-photon cooling of magnesium atoms

    DEFF Research Database (Denmark)

    Malossi, N.; Damkjær, S.; Hansen, P. L.;

    2005-01-01

    A two-photon mechanism for cooling atoms below the Doppler temperature is analyzed. We consider the magnesium ladder system (3s2)S01¿(3s3p)P11 at 285.2nm followed by the (3s3p)P11¿(3s3d)D21 transition at 880.7nm . For the ladder system quantum coherence effects may become important. Combined...

  1. Two-photon super bunching of thermal light via multiple two-photon-path interference

    CERN Document Server

    Hong, Peilong; Zhang, Guoquan

    2012-01-01

    We propose a novel scheme to achieve two-photon super bunching of thermal light through multiple two-photon-path interference, in which two mutually first-order incoherent optical channels are introduced by inserting a modified Michelson interferometer into a traditional two-photon HBT interferometer, and the bunching peak-to-background ratio can reach 3 theoretically. Experimentally, the super bunching peak-to-background ratio was measured to be 2.4, much larger than the ratio 1.7 measured with the same thermal source in a traditional HBT interferometer. The peak-to-background ratio of two-photon super bunching of thermal light can be increased up to $2\\times1.5^n$ by inserting cascadingly $n$ pairs of mutually first-order incoherent optical channels into the traditional two-photon HBT interferometer. The two-photon super bunching of thermal light should be of great significance in improving the visibility of classical ghost imaging.

  2. Electron-electron double resonance (ELDOR) with a loop-gap resonator

    Science.gov (United States)

    Hyde, James S.; Yin, Jun-Jie; Froncisz, W.; Feix, Jimmy B.

    Electron-electron double-resonance (ELDOR) experiments on nitroxide-radical-spin-labeled liposomes have been performed using a loop-gap resonator. The signal-to-noise ratio expressed on a molarity basis is 20-fold over the best that has been achieved using a bimodal cavity. This improvement permits ELDOR experiments on spin-labeled plasma membranes of intact cells, as illustrated by a prototype experiment on red blood cells labeled with stearic acid spin label. Moreover, 20 times greater pumping energy density at the sample is achievable for a given incident pump power, permitting ELDOR experiments on less readily saturated systems. Pump and observing frequencies are introduced directly into the loop-gap resonator, which has a relatively low Q, and the pump electron paramagnetic resonance signal is isolated from the receiver using a high Q trap microwave filter.

  3. Modulation scheme for electron-electron double resonance spectroscopy

    Science.gov (United States)

    Mehlkopf, A. F.; Kuiper, F. G.; Smidt, J.; Tiggelman, T. A.

    1983-06-01

    A modulation scheme for electron-electron double resonance (ELDOR) spectrometers is presented. With this scheme an optimum stabilization signal for locking the pump microwave generator to the pumped electron paramagnetic resonance (EPR) line is generated. A separate pump power level and a separate magnetic field modulation amplitude are used for the purpose of locking. In general, such a modulation scheme introduces false ELDOR lines. These false lines disturb the real ELDOR signals, or introduce an ELDOR signal in the absence of any communication between the observed EPR line and the pumped EPR line. With the described modulation scheme the frequencies of the false ELDOR signals are limited to even multiples of the frequency of the wanted ELDOR signals. This makes a suppression of the false ELDOR lines easy.

  4. Search for New Physics with Two Photons in the Final State with the ATLAS Detector

    CERN Document Server

    AUTHOR|(INSPIRE)INSPIRE-00441752

    This thesis reports on the search for new physics in the diphoton decay channel with the proton-proton collision data collected by ATLAS at a centre-of-mass energy of $\\sqrt{s}=8$~TeV in 2012 and $\\sqrt{s}=13$~TeV in 2015 and 2016. A feasibility study of the search for a pseudoscalar $A$ decaying to a $Z$ boson and a 125~GeV Higgs boson in the context of an extended Higgs sector, namedly the two-Higgs-doublet models, is presented. The search is performed with a final state of two jets and two photons using 20.3~${\\rm fb}^{-1}$ of data at $\\sqrt{s}=8$~TeV. The expected sensitivity is found to be competitive with the analysis with a final state of two electrons or muons and two $\\tau$ leptons, but less sensitive to the other searches with the Higgs decaying to a pair of $b$-quarks. Search for high mass resonances decaying to two photons at $\\sqrt{s}=13$~TeV is also presented. The analysed dataset corresponds to an integrated luminosity of $3.2~{\\rm fb}^{-1}$ in 2015 and $12.2~{\\rm fb}^{-1}$ in 2016. Two searche...

  5. Electron-Spin Resonance in Boron Carbide

    Science.gov (United States)

    Wood, Charles; Venturini, Eugene L.; Azevedo, Larry J.; Emin, David

    1987-01-01

    Samples exhibit Curie-law behavior in temperature range of 2 to 100 K. Technical paper presents studies of electron-spin resonance of samples of hot pressed B9 C, B15 C2, B13 C2, and B4 C. Boron carbide ceramics are refractory solids with high melting temperatures, low thermal conductives, and extreme hardnesses. They show promise as semiconductors at high temperatures and have unusually large figures of merit for use in thermoelectric generators.

  6. Microwave Absorption in Electron Cyclotron Resonance Plasma

    Institute of Scientific and Technical Information of China (English)

    LIU Ming-Hai; HU Xi-Wei; WU Qin-Chong; YU Guo-Yang

    2000-01-01

    The microwave power absorption in electron cyclotron resonance plasma reactor was investigated with a twodimensional hybrid-code. Simulation results indicated that there are two typical power deposition profiles over the entire parameter region: (1) microwave power deposition peaks on the axis and decreases in radial direction,(2) microwave power deposition has its maximum at some radial position, i.e., a hollow distribution. The spatial distribution of electron temperature resembles always to the microwave power absorption profile. The dependence of plasma parameter on the gas pressure is discussed also.

  7. Plasmonic-enhanced two-photon fluorescence with single gold nanoshell

    Science.gov (United States)

    Zhang, TianYue; Lu, GuoWei; Shen, HongMing; Perriat, P.; Martini, M.; Tillement, O.; Gong, QiHuang

    2014-06-01

    Single gold nanoshell with mutilpolar plasmon resonances is proposed to enhance two-photon fluorescence efficiently. The single emitter single nanoshell configuration is studied systematically by employing the finite-difference time-domain method. The emitter located inside or outside the nanoshell at various positions leads to a significantly different enhancement effect. The fluorescent emitter placed outside the nanoshell can achieve large fluorescence intensity given that both the position and orientation of the emission dipole are optimally controlled. In contrast, for the case of the emitter placed inside the nanoshell, it can experience substantial two-photon fluorescence enhancement without strict requirements upon the position and dipole orientations. Metallic nanoshell encapsulating many fluorescent emitters should be a promising nanocomposite configuration for bright two-photon fluorescence label. The results provide a comprehensive understanding about the plasmonic-enhanced two-photon fluorescence behaviors, and the nanocomposite configuration has great potential for optical detecting, imaging and sensing in biological applications.

  8. Cyanines as new fluorescent probes for DNA detection and two-photon excited bioimaging.

    Science.gov (United States)

    Feng, Xin Jiang; Wu, Po Lam; Bolze, Frédéric; Leung, Heidi W C; Li, King Fai; Mak, Nai Ki; Kwong, Daniel W J; Nicoud, Jean-François; Cheah, Kok Wai; Wong, Man Shing

    2010-05-21

    A series of cyanine fluorophores based on fused aromatics as an electron donor for DNA sensing and two-photon bioimaging were synthesized, among which the carbazole-based biscyanine exhibits high sensitivity and efficiency as a fluorescent light-up probe for dsDNA, which shows selective binding toward the AT-rich regions. The synergetic effect of the bischromophoric skeleton gives a several-fold enhancement in a two-photon absorption cross-section as well as a 25- to 100-fold enhancement in two-photon excited fluorescence upon dsDNA binding.

  9. Denoising two-photon calcium imaging data.

    Science.gov (United States)

    Malik, Wasim Q; Schummers, James; Sur, Mriganka; Brown, Emery N

    2011-01-01

    Two-photon calcium imaging is now an important tool for in vivo imaging of biological systems. By enabling neuronal population imaging with subcellular resolution, this modality offers an approach for gaining a fundamental understanding of brain anatomy and physiology. Proper analysis of calcium imaging data requires denoising, that is separating the signal from complex physiological noise. To analyze two-photon brain imaging data, we present a signal plus colored noise model in which the signal is represented as harmonic regression and the correlated noise is represented as an order autoregressive process. We provide an efficient cyclic descent algorithm to compute approximate maximum likelihood parameter estimates by combing a weighted least-squares procedure with the Burg algorithm. We use Akaike information criterion to guide selection of the harmonic regression and the autoregressive model orders. Our flexible yet parsimonious modeling approach reliably separates stimulus-evoked fluorescence response from background activity and noise, assesses goodness of fit, and estimates confidence intervals and signal-to-noise ratio. This refined separation leads to appreciably enhanced image contrast for individual cells including clear delineation of subcellular details and network activity. The application of our approach to in vivo imaging data recorded in the ferret primary visual cortex demonstrates that our method yields substantially denoised signal estimates. We also provide a general Volterra series framework for deriving this and other signal plus correlated noise models for imaging. This approach to analyzing two-photon calcium imaging data may be readily adapted to other computational biology problems which apply correlated noise models.

  10. Beam induced electron cloud resonances in dipole magnetic fields

    Science.gov (United States)

    Calvey, J. R.; Hartung, W.; Makita, J.; Venturini, M.

    2016-07-01

    The buildup of low energy electrons in an accelerator, known as electron cloud, can be severely detrimental to machine performance. Under certain beam conditions, the beam can become resonant with the cloud dynamics, accelerating the buildup of electrons. This paper will examine two such effects: multipacting resonances, in which the cloud development time is resonant with the bunch spacing, and cyclotron resonances, in which the cyclotron period of electrons in a magnetic field is a multiple of bunch spacing. Both resonances have been studied directly in dipole fields using retarding field analyzers installed in the Cornell Electron Storage Ring. These measurements are supported by both analytical models and computer simulations.

  11. Two-photon ionization of atomic hydrogen with elliptically polarized light

    Science.gov (United States)

    Kassaee, A.; Rustgi, M. L.; Long, S. A. T.

    1988-01-01

    The theory of two-photon ionization of a hydrogenic state in the nonrelativistic dipole approximation is generalized for elliptically polarized light. An application to the metastable 2S state of atomic hydrogen is made. Significant differences in the angular distribution of the outgoing electrons are found depending upon the polarization of the photons. It is claimed that two-photon ionization employing elliptically polarized photons from lasers may provide an additional test for the theories of multiphoton ionization.

  12. Nonresonant two-photon transitions in length and velocity gauges

    Science.gov (United States)

    Jentschura, U. D.

    2016-08-01

    We reexamine the invariance of two-photon transition matrix elements and corresponding two-photon Rabi frequencies under the "gauge" transformation from the length to the velocity gauge. It is shown that gauge invariance, in the most general sense, only holds at exact resonance, for both one-color as well as two-color absorption. The arguments leading to this conclusion are supported by analytic calculations which express the matrix elements in terms of hypergeometric functions, and ramified by a "master identity" which is fulfilled by off-diagonal matrix elements of the Schrödinger propagator under the transformation from the velocity to the length gauge. The study of the gauge dependence of atomic processes highlights subtle connections between the concept of asymptotic states, the gauge transformation of the wave function, and infinitesimal damping parameters for perturbations and interaction Hamiltonians that switch off the terms in the infinite past and future [of the form exp(-ɛ |t |)] . We include a pertinent discussion.

  13. Simultaneous two-photon excitation of photodynamic therapy agents

    Science.gov (United States)

    Wachter, Eric A.; Partridge, W. P., Jr.; Fisher, Walter G.; Dees, Craig; Petersen, Mark G.

    1998-07-01

    The spectroscopic and photochemical properties of several photosensitive compounds are compared using conventional single-photon excitation (SPE) and simultaneous two-photon excitation (TPE). TPE is achieved using a mode-locked titanium:sapphire laser, the near infrared output of which allows direct promotion of non-resonant TPE. Excitation spectra and excited state properties of both type I and type II photodynamic therapy (PDT) agents are examined. In general, while SPE and TPE selection rules may be somewhat different, the excited state photochemical properties are equivalent for both modes of excitation. In vitro promotion of a two-photon photodynamic effect is demonstrated using bacterial and human breast cancer models. These results suggest that use of TPE may be beneficial for PDT, since the technique allows replacement of visible or ultraviolet excitation with non- damaging near infrared light. Further, a comparison of possible excitation sources for TPE indicates that the titanium:sapphire laser is exceptionally well suited for non- linear excitation of PDT agents in biological systems due to its extremely short pulse width and high repetition rate; these features combine to effect efficient PDT activation with minimal potential for non-specific biological damage.

  14. Electron Paramagnetic Resonance Study of Pr

    Energy Technology Data Exchange (ETDEWEB)

    Tezuka, Keitaro; Hinatsu, Yukio

    2001-01-01

    Electron paramagnetic resonance (EPR) spectra of tetravalent praseodymium ions doped in the cubic perovskite compound BaHfO{sub 3} have been measured at 4.2 K. A very large hyperfine interaction with the {sup 141}Pr nucleus was observed in the spectrum of Pr{sup 4+}/ BaHfO{sub 3}. The results were analyzed based on the weak field approximation, and the g value (|g|=0.619) and a hyperfine coupling constant (A=0.0589 cm{sup {minus}1}) were obtained. The measured g value is much smaller than |-10/7|, which indicates that the crystal field effect on the behavior of a 4f electron is large. These g and A values were compared with the EPR results for other f{sup 1} ions in an octahedral crystal field.

  15. Highly selective population of two excited states in nonresonant two-photon absorption

    Institute of Scientific and Technical Information of China (English)

    Zhang Hui; Zhang Shi-An; Sun Zhen-Rong

    2011-01-01

    A nonresonant two-photon absorption process can be manipulated by tailoring the ultra-short laser pulse.In this paper,we theoretically demonstrate a highly selective population of two excited states in the nonresonant two-photon absorption process by rationally designing a spectral phase distribution.Our results show that one excited state is maximally populated while the other state population is widely tunable from zero to the maximum value.We believe that the theoretical results may play an important role in the selective population of a more complex nonlinear process comprising nonresonant two-photon absorption,such as resonance-mediated(2+1)-three-photon absorption and (2+1)-resonant multiphoton ionization.

  16. Two-photon interference : spatial aspects of two-photon entanglement, diffraction, and scattering

    NARCIS (Netherlands)

    Peeters, Wouter Herman

    2010-01-01

    This dissertation contains scientific research within the realm of quantum optics, which is a branch of physics. An experimental and theoretical study is made of two-photon interference phenomena in various optical systems. Spatially entangled photon pairs are produced via the nonlinear optical proc

  17. Two-photon imaging of stem cells

    Science.gov (United States)

    Uchugonova, A.; Gorjup, E.; Riemann, I.; Sauer, D.; König, K.

    2008-02-01

    A variety of human and animal stem cells (rat and human adult pancreatic stem cells, salivary gland stem cells, dental pulpa stem cells) have been investigated by femtosecond laser 5D two-photon microscopy. Autofluorescence and second harmonic generation have been imaged with submicron spatial resolution, 270 ps temporal resolution, and 10 nm spectral resolution. In particular, NADH and flavoprotein fluorescence was detected in stem cells. Major emission peaks at 460nm and 530nm with typical mean fluorescence lifetimes of 1.8 ns and 2.0 ns, respectively, were measured using time-correlated single photon counting and spectral imaging. Differentiated stem cells produced the extracellular matrix protein collagen which was detected by SHG signals at 435 nm.

  18. Two-photon Interference with Non-identical Photons

    CERN Document Server

    Liu, Jianbin; Zheng, Huaibin; Chen, Hui; Li, Fu-Li; Xu, Zhuo

    2014-01-01

    The indistinguishability of non-identical photons is dependent on detection system in quantum physics. If two photons with different wavelengths are indistinguishable for a detection system, there can be two-photon interference when these two photons are incident to two input ports of a Hong-Ou-Mandel interferometer, respectively. The reason why two-photon interference phenomena are different for classical and nonclassical light is not due to interference, but due to the properties of light and detection system. These conclusions are helpful to understand the physics and applications of two-photon interference.

  19. Measurement of bottom quark production in two photon collisions

    CERN Document Server

    Saremi, Sepehr

    2001-01-01

    The cross section for bottom quark production in two-photon collisions, sigma( e+e- → e+e- bb¯X), is measured for the first time. The measurement is performed with the L3 detector at the Large Electron Positron (LEP) collider at the European Center for Nuclear and Particle Physics (CERN). The data corresponds to 410 pb-1 taken at center-of-mass energies from 189 GeV to 202 GeV. Hadrons containing a bottom quark are identified by detecting electrons or muons from their semi-leptonic decays. The measured cross section is in excess of the Next to Leading Order QCD prediction by a factor of three.

  20. Inclusive D*(+/-) production in two photon collisions at LEP

    CERN Document Server

    Prokofiev, Denis Olegovich

    2001-01-01

    In this thesis I present my results on the measurement of the open charm production in two-photon collision events done with the L3 detector at Large Electron Positron machine (LEP). The data sample was collected from 1997 through 2000 at center-of-mass energies ranging from 183 GeV to 209 GeV, corresponding to a total integrated luminosity of 683.4pb −1. The open charm production in two-photon collision events extrapolated to the full phase space is estimated to be: s&parl0;e+e-&rarrr;e +e-cc&d1;X&parr0;=9 23±69±109±222pb. The differential cross sections d s /dpT(D*±) and d s /d:η(D*±): are also measured as functions of transverse momentum pT(D*±) and the absolute value of pseudorapidity :η(D*±):, respectively. A fit to the data estimating the relative contributions of Direct and Resolved open charm production mechanisms is performed, giving (28.7 ± 5.6)% and (71.3 ± 8.8)%, respectively. Using those relative fractions, the Direct and Resolved process cross sections yield: s&p...

  1. Second harmonic generation and two-photon luminescence upconversion in glasses doped with ZnSe nanocrystalline quantum dots

    Energy Technology Data Exchange (ETDEWEB)

    Thantu, Napoleon [Idaho National Engineering and Environmental Laboratory, 2525 Fremont Avenue, Idaho Falls, ID 83415 (United States)]. E-mail: Napoleon.Thantu@ngc.com

    2005-01-01

    We report two-photon excited emission in borosilicate glasses doped with ZnSe nanocrystalline quantum dots. The emission, predominantly near the two-photon energy and detected in the direction of the excitation beam, is in the visible, and the fundamental excitation is the near-infrared output of a tunable femtosecond laser. Depending on the two-photon energy, time- and frequency-resolved measurements at room temperature reveal that the emission largely consists of second harmonic generation (SHG) and two-photon luminescence upconversion, and a much smaller luminescence from redshifted, low-lying trap states and other trap levels residing near the semiconductor band edge. We discuss the SHG origin in terms of bulk-like and surface contributions from the nanocrystals and the two-photon resonant enhancement near the excitonic absorption.

  2. Two-Dimensional Electron-Spin Resonance

    Science.gov (United States)

    Freed, Jack H.

    2000-03-01

    The extension of the concepts of 2D-NMR to ESR posed significant technological challenges, especially for liquids. ESR relaxation times are very short, as low as 10-15 ns. for T_2's. Spectral bandwidths are 100-250 MHz for nitroxide spin labels. Adequate coverage is obtained with 3-5 ns. π/2 (9-17 GHz) microwave pulses into a small low Q resonator. Dead-times are currently 25-30 ns. Additional requirements are rapid phase shifting for phase cycling, nsec. data acquisition, and fast repetition rates (10-100 kHz). 2D-ELDOR (electron-electron double resonance), which is a 3-pulse 2D-exchange experiment, takes about 30 minutes with just 0.5 nanomole spin-probe in solution (SNR 200). 2D-ELDOR is very useful in studies of molecular dynamics and local structure in complex fluids. For such media, the slow rotational dynamics requires a theory based upon the stochastic Liouville equation which enables quantitative interpretation of 2D-ELDOR experiments. In studies of spin-probes in a liquid crystal new insights could be obtained on the dynamic structure in different phases. One obtains, in addition to ordering and reorientation rates of the probes, details of the local dynamic cage: its orienting potential and (slow) relaxation rate. 2D-ELDOR overcomes the loss of resolution resulting from microscopically ordered but macroscopically disordered complex fluids. This is illustrated by studies of the dynamic structure of lipid membrane vesicles, and the effects of adding a peptide. The short dead times enable the observation of both the bulk lipids and the more immobilized lipids that coat (or are trapped) by the (aggregates of) peptides. Also, new developments of multi-quantum (2D) FT-ESR from nitroxide spin labels interacting by dipolar interactions show considerable promise in measuring distances of ca. 15-70A in macromolecules.

  3. Fluorenyl porphyrins for combined two-photon excited fluorescence and photosensitization

    Science.gov (United States)

    Mongin, Olivier; Hugues, Vincent; Blanchard-Desce, Mireille; Merhi, Areej; Drouet, Samuel; Yao, Dandan; Paul-Roth, Christine

    2015-04-01

    The two-photon absorption (2PA), the luminescence and the photosensitization properties of porphyrin-cored fluorenyl dendrimers and meso-substituted fluorenylporphyrin monomer, dimer and trimer are described. In comparison with model tetraphenylporphyrin, these compounds combine enhanced (non-resonant) 2PA cross-sections in the near infrared and enhanced fluorescence quantum yields, together with maintained singlet oxygen generation quantum yields. 'Semi-disconnection' between fluorenyl groups and porphyrins (i.e. direct meso substitution) proved to be more efficient than non-conjugated systems (based on efficient FRET between fluorenyl antennae and porphyrins). These results are of interest for combined two-photon imaging and photodynamic therapy.

  4. Sequential and coherent, optical and x-ray two-photon processes in atoms and molecules

    Science.gov (United States)

    Mills, Jeffrey Dean

    1997-09-01

    Vibronic and rovibronic implementations of conventional semiclassical theories, employing a phenomenological lineshape and descriptive of the absorption of a single photon by isolated chemical particles, are used to account for the absolute magnitude of the highly structured, broadband optical absorption, emission, radiation transfer, and refractive index of high- temperature (T ≈ 2000K), rare-gas-buffered, and locally equilibrated atomic and diatomic metal vapors (Li, Na, Al, and Li/Al). The polarized, resonant, inelastic scattering of x-rays (hν /approx 2.5 keV) from the K-edges of unoriented, chlorine- and sulfur- containing molecular gases (CH3Cl, H2S, and Cl2) is also modeled by means of the fully quantum- mechanical, time-independent Kramers-Heisenberg formalism applied in electronic and vibronic resolution. This accounts for the energy, polarization, and direction dependence of the anisotropic signal, concretely treats the demise of core-excited states by Auger-electron emission within the Feshbach-Fano theory of resonance- continuum mixing, and is in general valid for resonant, nonresonant, inelastic, and 'distinguishable' elastic scattering. Unusual, coherent interference phenomena within and between vibronic and electronic channels and related novel, otherwise-forbidden nondipole features expected to arise in molecules with equivalent atomic centers and recently observed in the chlorine molecule are explored along with their implications for common conceptions of 'localized, equivalent core-hole excited states.' Transition coherence, especially as manifested within the quantum-mechanical treatment of the spectral lineshape, is shown to provide the key to unifying the present single-step interpretation of two-photon x-ray scattering with that involving a pair of successive absorption and emission transitions generally regarded as two independent single-photon processes of the type described in the first portion of the work.

  5. Visualization of two-photon Rabi oscillations in evanescently coupled optical waveguides

    Energy Technology Data Exchange (ETDEWEB)

    Ornigotti, M; Valle, G Della; Fernandez, T Toney; Laporta, P; Longhi, S [Dipartimento di Fisica and Istituto di Fotonica e Nanotecnologie del CNR, Politecnico di Milano, Piazza L. da Vinci 32, I-20133 Milano (Italy); Coppa, A; Foglietti, V [Istituto di Fotonica e Nanotecnologie del CNR, sezione di Roma, Via Cineto Romano 42, 00156 Roma (Italy)], E-mail: longhi@fisi.polimi.it

    2008-04-28

    An optical analogue of two-photon Rabi oscillations, occurring in a three-level atomic or molecular system coherently driven by two detuned laser fields, is theoretically proposed and experimentally demonstrated using three evanescently coupled optical waveguides realized on an active glass substrate. The optical analogue stems from the formal analogy between spatial propagation of light waves in the three-waveguide structure and the coherent temporal evolution of populations in a three-level atomic medium driven by two laser fields under two-photon resonance. In our optical experiment, two-photon Rabi oscillations are thus visualized as a slow spatial oscillatory exchange of light power between the two outer waveguides of the structure with a small excitation of the central waveguide.

  6. Fokker-Planck Study of Tokamak Electron Cyclotron Resonance Heating

    Institute of Scientific and Technical Information of China (English)

    SHIBingren; LONGYongxing; DONGJiaqi; LIWenzhong; JIAOYiming; WANGAike

    2002-01-01

    In this study, we add a subroutine for describing the electron cyclotron resonant heating calculation to the Fokker-Planck code. By analyzing the wave-particle resonance condition in tokamak plasma and the fast motion of electrons along magnetic field lines, suitable quasi-linear diffusion coefficients are given.

  7. Electron paramagnetic resonance dosimetry using synthetic hydroxyapatite

    Energy Technology Data Exchange (ETDEWEB)

    Choi, Kwon; Kim, Hwi Young; Ye, Sung Joon [Seoul National University, Seoul (Korea, Republic of); Hirata, Hiroshi [Hokkaido University, Sapporo (Japan); Park, Jong Min [Seoul National University Hospital, Seoul (Korea, Republic of)

    2014-11-15

    The victims exposed doses under 3.5-4.0 Gy have chance to survive if treated urgently. To determine the priority of treatment among a large number of victims, the triage – distinguishing patients who need an urgent treatment from who may not be urgent – is necessary based on radiation biodosimetry. A current gold standard for radiation biodosimetry is the chromosomal assay using human lymphocytes. But this method requires too much time and skilled labors to cover the mass victims in radiation emergencies. Electron paramagnetic resonance (EPR) has been known for its capability of quantifying radicals in matters. EPR dosimetry is based on the measurement of stable radiation-induced radicals in tooth enamel. Hydroxyapatite (HAP) (Ca10(PO4)6(OH)2) contained in tooth enamel is a major probe for radiation dose reconstruction. This HAP dosimetry study was performed using a novel EPR spectrometer in Hokkaido University, Japan. The EPR dose-response curve was made using HAP samples. The blind test using 250 cGy samples showed the feasibility of EPR dosimetry for the triage purpose.

  8. Multifrequency pulsed electron paramagnetic resonance on metalloproteins.

    Science.gov (United States)

    Lyubenova, Sevdalina; Maly, Thorsten; Zwicker, Klaus; Brandt, Ulrich; Ludwig, Bernd; Prisner, Thomas

    2010-02-16

    Metalloproteins often contain metal centers that are paramagnetic in some functional state of the protein; hence electron paramagnetic resonance (EPR) spectroscopy can be a powerful tool for studying protein structure and function. Dipolar spectroscopy allows the determination of the dipole-dipole interactions between metal centers in protein complexes, revealing the structural arrangement of different paramagnetic centers at distances of up to 8 nm. Hyperfine spectroscopy can be used to measure the interaction between an unpaired electron spin and nuclear spins within a distance of 0.8 nm; it therefore permits the characterization of the local structure of the paramagnetic center's ligand sphere with very high precision. In this Account, we review our laboratory's recent applications of both dipolar and hyperfine pulsed EPR methods to metalloproteins. We used pulsed dipolar relaxation methods to investigate the complex of cytochrome c and cytochrome c oxidase, a noncovalent protein-protein complex involved in mitochondrial electron-transfer reactions. Hyperfine sublevel correlation spectroscopy (HYSCORE) was used to study the ligand sphere of iron-sulfur clusters in complex I of the mitochondrial respiratory chain and substrate binding to the molybdenum enzyme polysulfide reductase. These examples demonstrate the potential of the two techniques; however, they also highlight the difficulties of data interpretation when several paramagnetic species with overlapping spectra are present in the protein. In such cases, further approaches and data are very useful to enhance the information content. Relaxation filtered hyperfine spectroscopy (REFINE) can be used to separate the individual components of overlapping paramagnetic species on the basis of differences in their longitudinal relaxation rates; it is applicable to any kind of pulsed hyperfine or dipolar spectroscopy. Here, we show that the spectra of the iron-sulfur clusters in complex I can be separated by this

  9. Synergistic Two-Photon Absorption Enhancement in Photosynthetic Light Harvesting

    Science.gov (United States)

    Chen, Kuo-Mei; Chen, Yu-Wei; Gao, Ting-Fong

    2012-06-01

    The grand scale fixation of solar energies into chemical substances by photosynthetic reactions of light-harvesting organisms provides Earth's other life forms a thriving environment. Scientific explorations in the past decades have unraveled the fundamental photophysical and photochemical processes in photosynthesis. Higher plants, green algae, and light-harvesting bacteria utilize organized pigment-protein complexes to harvest solar power efficiently and the resultant electronic excitations are funneled into a reaction center, where the first charge separation process takes place. Here we show experimental evidences that green algae (Chlorella vulgaris) in vivo display a synergistic two-photon absorption enhancement in their photosynthetic light harvesting. Their absorption coefficients at various wavelengths display dramatic dependence on the photon flux. This newly found phenomenon is attributed to a coherence-electronic-energy-transfer-mediated (CEETRAM) photon absorption process of light-harvesting pigment-protein complexes of green algae. Under the ambient light level, algae and higher plants can utilize this quantum mechanical mechanism to create two entangled electronic excitations adjacently in their light-harvesting networks. Concerted multiple electron transfer reactions in the reaction centers and oxygen evolving complexes can be implemented efficiently by the coherent motion of two entangled excitons from antennae to the charge separation reaction sites. To fabricate nanostructured, synthetic light-harvesting apparatus, the paramount role of the CEETRAM photon absorption mechanism should be seriously considered in the strategic guidelines.

  10. Single-electron Spin Resonance in a Quadruple Quantum Dot

    Science.gov (United States)

    Otsuka, Tomohiro; Nakajima, Takashi; Delbecq, Matthieu R.; Amaha, Shinichi; Yoneda, Jun; Takeda, Kenta; Allison, Giles; Ito, Takumi; Sugawara, Retsu; Noiri, Akito; Ludwig, Arne; Wieck, Andreas D.; Tarucha, Seigo

    2016-08-01

    Electron spins in semiconductor quantum dots are good candidates of quantum bits for quantum information processing. Basic operations of the qubit have been realized in recent years: initialization, manipulation of single spins, two qubit entanglement operations, and readout. Now it becomes crucial to demonstrate scalability of this architecture by conducting spin operations on a scaled up system. Here, we demonstrate single-electron spin resonance in a quadruple quantum dot. A few-electron quadruple quantum dot is formed within a magnetic field gradient created by a micro-magnet. We oscillate the wave functions of the electrons in the quantum dots by applying microwave voltages and this induces electron spin resonance. The resonance energies of the four quantum dots are slightly different because of the stray field created by the micro-magnet and therefore frequency-resolved addressable control of each electron spin resonance is possible.

  11. Several Organic Salts with High Two-Photon Active

    Institute of Scientific and Technical Information of China (English)

    TIAN, Yu-Peng; JIANG, Min-Hua; WANG, He-Zhou; FANG, Qi

    2001-01-01

    Several organic salts with D-A molecular structure and different counterion have been prepared and experimentally investigated. The two-photon induced frequency-upconverted spectra and two-photon pumped lasing are measured for the organic salt solutions in various solvents. The results indicate that counterions have influence on their stability and lasing property.

  12. Two-photon absorption in arsenic sulfide glasses

    Science.gov (United States)

    Chunaev, D. S.; Snopatin, G. E.; Plotnichenko, V. G.; Karasik, A. Ya.

    2016-10-01

    The two-photon absorption coefficient of 1047-{\\text{nm}} light in {\\text{As}}35{\\text{S}}65 chalcogenide glass has been measured. CW probe radiation has been used to observe the linear absorption in glass induced by two-photon excitation. The induced absorption lifetime was found to be ∼ 2 {\\text{ms}}.

  13. The development of efficient two-photon singlet oxygen sensitizers

    DEFF Research Database (Denmark)

    Nielsen, Christian Benedikt

    The development of efficient two-photon singlet oxygen sensitizers is addressed focusing on organic synthesis. Photophysical measurements were carried out on new lipophilic molecules, where two-photon absorption cross sections and singlet oxygen quantumyields were measured. Design principles...... for making efficient two-photon singlet oxygen sensitizers were then constructed from these results. Charge-transfer in the excited state of the prepared molecules was shown to play a pivotal role in the generationof singlet oxygen. This was established through studies of substituent effects on both...... the singlet oxygen yield and the two-photon absorption cross section, where it was revealed that a careful balancing of the amount of charge transfer present in theexcited state of the sensitizer is necessary to obtain both a high singlet oxygen quantum yield and a high two-photon cross section. An increasing...

  14. Two-photon laser fabrication of three-dimensional silver microstructures with submicron scale linewidth

    Energy Technology Data Exchange (ETDEWEB)

    Tsutsumi, Naoto; Nagata, Kazuya; Sakai, Wataru [Kyoto Institute of Technology, Department of Macromolecular Science and Engineering, Graduate School of Science and Technology, Kyoto (Japan)

    2011-05-15

    We show three-dimensional silver microstructures with a submicron scale linewidth fabricated via two-photon photoreduction of silver ions in a poly(N-vinylpyrrolidone) (PVP) matrix. Femtosecond laser at 508 nm directly excites the carbonyl group of PVP via two-photon excitation to reduce silver ions. Lone pair electrons in PVP stabilized silver ions and lower molecular weight of PVP prevented silver clusters growing larger. The effect of molecular weight of PVP on linewidth of silver nanowire is investigated. (orig.)

  15. Two-photon exchange correction to $2S$-$2P$ splitting in muonic helium

    CERN Document Server

    Carlson, Carl E; Vanderhaeghen, Marc

    2016-01-01

    We calculate the two-photon exchange correction to the Lamb shift in muonic helium atoms within the dispersion relations framework. Part of the effort entailed making analytic fits to the electron-$^3$He quasielastic scattering data set, for purposes of doing the dispersion integrals. Our result is that the energy of the 2$S$ state is shifted downwards by two-photon exchange effects by 15.14(49) meV, in good accord with the result obtained from a potential model and effective field theory calculation.

  16. Enhancement of two-photon photoluminescence and SERS for low-coverage gold films

    DEFF Research Database (Denmark)

    Novikov, Sergey M.; Beermann, Jonas; Frydendahl, Christian

    2016-01-01

    Electromagnetic field enhancement (FE) effects occurring in thin gold films 3-12-nm are investigated with two-photon photoluminescence (TPL) and Raman scanning optical microscopies. The samples are characterized using scanning electron microscopy images and linear optical spectroscopy. TPL images...

  17. A triple resonance hyperfine sublevel correlation experiment for assignment of electron-nuclear double resonance lines

    Science.gov (United States)

    Potapov, Alexey; Epel, Boris; Goldfarb, Daniella

    2008-02-01

    A new, triple resonance, pulse electron paramagnetic resonance (EPR) sequence is described. It provides spin links between forbidden electron spin transitions (ΔMS=±1, ΔMI≠0) and allowed nuclear spin transitions (ΔMI=±1), thus, facilitating the assignment of nuclear frequencies to their respective electron spin manifolds and paramagnetic centers. It also yields the relative signs of the hyperfine couplings of the different nuclei. The technique is based on the combination of electron-nuclear double resonance (ENDOR) and electron-electron double resonance (ELDOR)-detected NMR experiments in a way similar to the TRIPLE experiment. The feasibility and the information content of the method are demonstrated first on a single crystal of Cu-doped L-histidine and then on a frozen solution of a Cu-histidine complex.

  18. Quantum Stochastic Resonance in Electron Shelving

    CERN Document Server

    Huelga, S F

    2000-01-01

    Stochastic resonance shows that under some circumstances noise can enhance the response of a system to a periodic force. While this effect has been extensively investigated theoretically and demonstrated experimentally in classical systems, there is complete lack of experimental evidence within the purely quantum mechanical domain. Here we demonstrate that stochastic resonance can be exhibited in a single ion and would be experimentally observable using well mastered experimental techniques. We discuss the use of this scheme for the detection of the frequency difference of two lasers to demonstrate that stochastic resonance may have applications in precision measurements at the quantum limit.

  19. Synthesis of Two-Photon Materials and Two-Photon Liquid Crystals

    Science.gov (United States)

    Subramaniam, Girija

    2001-01-01

    The duration of the grant was interrupted by two major accidents that the PI met with-- an auto accident in Pasadena, CA during her second summer at JPL which took almost eight months for recovery and a second accident during Fall 2000 that left her in crutches for the entire semester. Further, the time released agreed by the University was not given in a timely fashion. The candidate has been given post-grant expire time off. In spite of all these problems, the PI synthesized a number of new two-photon materials and studied the structure-activity correlation to arrive at the best-optimized structure. The PI's design proved to be one of the best in the sense that these materials has a hitherto unreported two-photon absorption cross section. Many materials based on PI's design was later made by the NASA colleague. This is Phase 1. Phase II of this grant is to orate liquid crystalline nature into this potentially useful materials and is currently in progress. Recent observations of nano- and pico-second response time of homeotropically aligned liquid crystals suggest their inherent potentials to act as laser hardening materials, i.e., as protective devices against short laser pulses. The objective of the current project is to exploit this potential by the synthesis of liquid crystals with high optical nonlinearity and optimizing their performance. The PI is trying structural variations to bring in liquid crystalline nature without losing the high two-photon cross section. Both Phase I and Phase II led to many invited presentations and publications in reputed journals like 'Science' and 'Molecular Crystals'. The list of presentations and reprints are enclosed. Another important and satisfying outcome of this grant is the opportunity that this grant offered to the budding undergraduate scientists to get involved in a visible research of international importance. All the students had a chance to learn a lot during research, had the opportunity to present their work at

  20. Electron Cyclotron Resonance Heating of a High-Density Plasma

    DEFF Research Database (Denmark)

    Hansen, F. Ramskov

    1986-01-01

    Various schemes for electron cyclotron resonance heating of tokamak plasmas with the ratio of electron plasma frequency to electron cyclotron frequency, "»pe/^ce* larger than 1 on axis, are investigated. In particular, a mode conversion scheme is investigated using ordinary waves at the fundamental...

  1. Two-Photon or Higher-Order Absorbing Optical Materials for Generation of Reactive Species

    Science.gov (United States)

    Cumpston, Brian (Inventor); Lipson, Matthew (Inventor); Marder, Seth R. (Inventor); Perry, Joseph W. (Inventor)

    2013-01-01

    Disclosed are highly efficient multiphoton absorbing compounds and methods of their use. The compounds generally include a bridge of pi-conjugated bonds connecting electron donating groups or electron accepting groups. The bridge may be substituted with a variety of substituents as well. Solubility, lipophilicity, absorption maxima and other characteristics of the compounds may be tailored by changing the electron donating groups or electron accepting groups, the substituents attached to or the length of the pi-conjugated bridge. Numerous photophysical and photochemical methods are enabled by converting these compounds to electronically excited states upon simultaneous absorption of at least two photons of radiation. The compounds have large two-photon or higher-order absorptivities such that upon absorption, one or more Lewis acidic species, Lewis basic species, radical species or ionic species are formed.

  2. Two-photon interference of temporally separated photons

    Science.gov (United States)

    Kim, Heonoh; Lee, Sang Min; Moon, Han Seb

    2016-10-01

    We present experimental demonstrations of two-photon interference involving temporally separated photons within two types of interferometers: a Mach-Zehnder interferometer and a polarization-based Michelson interferometer. The two-photon states are probabilistically prepared in a symmetrically superposed state within the two interferometer arms by introducing a large time delay between two input photons; this state is composed of two temporally separated photons, which are in two different or the same spatial modes. We then observe two-photon interference fringes involving both the Hong-Ou-Mandel interference effect and the interference of path-entangled two-photon states simultaneously in a single interferometric setup. The observed two-photon interference fringes provide simultaneous observation of the interferometric properties of the single-photon and two-photon wavepackets. The observations can also facilitate a more comprehensive understanding of the origins of the interference phenomena arising from spatially bunched/anti-bunched two-photon states comprised of two temporally separated photons within the interferometer arms.

  3. Biological oxygen sensing via two-photon absorption by an Ir(III) complex using a femtosecond fiber laser

    Science.gov (United States)

    Moritomo, Hiroki; Fujii, Akinari; Suzuki, Yasutaka; Yoshihara, Toshitada; Tobita, Seiji; Kawamata, Jun

    2016-09-01

    Near-infrared two-photon absorption of the phosphorescent Ir(III) complex (2,4-pentanedionato-κO 2,κO 4)bis[2-(6-phenanthridinyl-κN)benzo[b]thien-3-yl-κC]iridium (BTPHSA) was characterized. It exhibited a 800-1200 nm two-photon absorption band, and thus could be electronically excited by 1030-nm femtosecond Ti:sapphire and Yb-doped fiber lasers. By using BTPHSA, oxygen concentrations in human embryonic kidney 293 (HEK293) cells were imaged. These results demonstrate two-photon oxygen sensing of live tissues via easily operable excitation sources.

  4. Two-photon spectroscopy of trapped HD$^+$ ions in the Lamb-Dicke regime

    CERN Document Server

    Tran, Vu Quang; Douillet, Albane; Koelemeij, Jeroen C J; Hilico, Laurent

    2013-01-01

    We study the feasibility of nearly-degenerate two-photon rovibrational spectroscopy in ensembles of trapped, sympathetically cooled hydrogen molecular ions using a resonance-enhanced multiphoton dissociation (REMPD) scheme. Taking advantage of quasi-coincidences in the rovibrational spectrum, the excitation lasers are tuned close to an intermediate level to resonantly enhance two-photon absorption. Realistic simulations of the REMPD signal are obtained using a four-level model that takes into account saturation effects, ion trajectories, laser frequency noise and redistribution of population by blackbody radiation. We show that the use of counterpropagating laser beams enables optical excitation in an effective Lamb-Dicke regime. Sub-Doppler lines having widths in the 100 Hz range can be observed with good signal-to-noise ratio for an optimal choice of laser detunings. Our results indicate the feasibility of molecular spectroscopy at the $10^{-14}$ accuracy level for improved tests of molecular QED, a new det...

  5. Two-photon gateway in one-atom cavity quantum electrodynamics.

    Science.gov (United States)

    Kubanek, A; Ourjoumtsev, A; Schuster, I; Koch, M; Pinkse, P W H; Murr, K; Rempe, G

    2008-11-14

    Single atoms absorb and emit light from a resonant laser beam photon by photon. We show that a single atom strongly coupled to an optical cavity can absorb and emit resonant photons in pairs. The effect is observed in a photon correlation experiment on the light transmitted through the cavity. We find that the atom-cavity system transforms a random stream of input photons into a correlated stream of output photons, thereby acting as a two-photon gateway. The phenomenon has its origin in the quantum anharmonicity of the energy structure of the atom-cavity system. Future applications could include the controlled interaction of two photons by means of one atom.

  6. Two-Photon Absorption in Conjugated Energetic Molecules.

    Science.gov (United States)

    Bjorgaard, Josiah A; Sifain, Andrew E; Nelson, Tammie; Myers, Thomas W; Veauthier, Jacqueline M; Chavez, David E; Scharff, R Jason; Tretiak, Sergei

    2016-07-07

    Time-dependent density functional theory (TD-DFT) was used to investigate the relationship between molecular structure and the one- and two-photon absorption (OPA and TPA, respectively) properties of novel and recently synthesized conjugated energetic molecules (CEMs). The molecular structures of CEMs can be strategically altered to influence the heat of formation and oxygen balance, two factors that can contribute to the sensitivity and strength of an explosive material. OPA and TPA are sensitive to changes in molecular structure as well, influencing the optical range of excitation. We found calculated vertical excitation energies to be in good agreement with experiment for most molecules. Peak TPA intensities were found to be significant and on the order of 10(2) GM. Natural transition orbitals for essential electronic states defining TPA peaks of relatively large intensity were used to examine the character of relevant transitions. Modification of molecular substituents, such as additional oxygen or other functional groups, produces significant changes in electronic structure, OPA, and TPA and improves oxygen balance. The results show that certain molecules are apt to undergo nonlinear absorption, opening the possibility for controlled, direct optical initiation of CEMs through photochemical pathways.

  7. Quantum homodyne tomography of a two-photon Fock state

    CERN Document Server

    Ourjoumtsev, A; Grangier, P; Ourjoumtsev, Alexei; Tualle-Brouri, Rosa; Grangier, Philippe

    2006-01-01

    We present a continuous-variable experimental analysis of a two-photon Fock state of free-propagating light. This state is obtained from a pulsed non-degenerate parametric amplifier, which produces two intensity-correlated twin beams. Counting two photons in one beam projects the other beam in the desired two-photon Fock state, which is analyzed by using a pulsed homodyne detection. The Wigner function of the measured state is clearly negative. We developed a detailed analytic model which allows a fast and efficient analysis of the experimental results.

  8. Quantum homodyne tomography of a two-photon Fock state.

    Science.gov (United States)

    Ourjoumtsev, Alexei; Tualle-Brouri, Rosa; Grangier, Philippe

    2006-06-02

    We present a continuous-variable experimental analysis of a two-photon Fock state of free-propagating light. This state is obtained from a pulsed nondegenerate parametric amplifier, which produces two intensity-correlated twin beams. Counting two photons in one beam projects the other beam in the desired two-photon Fock state, which is analyzed by using a pulsed homodyne detection. The Wigner function of the measured state is clearly negative. We developed a detailed analytic model which allows a fast and efficient analysis of the experimental results.

  9. Scattering of two photons from two distant qubits: exact solution

    Energy Technology Data Exchange (ETDEWEB)

    Laakso, Matti; Pletyukhov, Mikhail [Institute for Theory of Statistical Physics, RWTH Aachen, 52056 Aachen (Germany)

    2015-07-01

    We consider the inelastic scattering of two photons from two qubits separated by an arbitrary distance and coupled to a one-dimensional transmission line. We present an exact, analytical solution to the problem, and use it to explore a particular configuration of qubits which is transparent to single-photon scattering, thus highlighting non-Markovian effects of inelastic two-photon scattering: Strong two-photon interference and momentum dependent photon (anti)bunching. This latter effect can be seen as an inelastic generalization of the Hong-Ou-Mandel effect.

  10. Development and design of advanced two-photon microscope used in neuroscience

    Science.gov (United States)

    Doronin, M. S.; Popov, A. V.

    2016-08-01

    This work represents the real steps to development and design advanced two-photon microscope by efforts of laboratory staff. Self-developed microscopy system provides possibility to service it and modify the structure of microscope depending on highly specialized experimental design and scientific goals. We are presenting here module-based microscopy system which provides an opportunity to looking for new applications of this setup depending on laboratories needs using with galvo and resonant scanners.

  11. Tailored probes for atomic force microscopy fabricated by two-photon polymerization

    Science.gov (United States)

    Göring, Gerald; Dietrich, Philipp-Immanuel; Blaicher, Matthias; Sharma, Swati; Korvink, Jan G.; Schimmel, Thomas; Koos, Christian; Hölscher, Hendrik

    2016-08-01

    3D direct laser writing based on two-photon polymerization is considered as a tool to fabricate tailored probes for atomic force microscopy. Tips with radii of 25 nm and arbitrary shape are attached to conventionally shaped micro-machined cantilevers. Long-term scanning measurements reveal low wear rates and demonstrate the reliability of such tips. Furthermore, we show that the resonance spectrum of the probe can be tuned for multi-frequency applications by adding rebar structures to the cantilever.

  12. Electronically excited negative ion resonant states in chloroethylenes

    Energy Technology Data Exchange (ETDEWEB)

    Khvostenko, O.G., E-mail: khv@mail.ru; Lukin, V.G.; Tuimedov, G.M.; Khatymova, L.Z.; Kinzyabulatov, R.R.; Tseplin, E.E.

    2015-02-15

    Highlights: • Several novel dissociative negative ion channels were revealed in chloroethylenes. • The electronically excited resonant states were recorded in all chloroethylenes under study. • The states were assigned to the inter-shell types, but not to the core-excited Feshbach one. - Abstract: The negative ion mass spectra of the resonant electron capture by molecules of 1,1-dichloroethylene, 1,2-dichloroethylene-cis, 1,2-dichloroethylene-trans, trichloroethylene and tetrachloroethylene have been recorded in the 0–12 eV range of the captured electron energy using static magnetic sector mass spectrometer modified for operation in the resonant electron capture regime. As a result, several novel low-intensive dissociation channels were revealed in the compounds under study. Additionally, the negative ion resonant states were recorded at approximately 3–12 eV, mostly for the first time. These resonant states were assigned to the electronically excited resonances of the inter-shell type by comparing their energies with those of the parent neutral molecules triplet and singlet electronically excited states known from the energy-loss spectra obtained by previous studies.

  13. Electron waves and resonances in bounded plasmas

    CERN Document Server

    Vandenplas, Paul E

    1968-01-01

    General theoretical methods and experimental techniques ; the uniform plasma slab-condenser system ; the hollow cylindrical plasma ; scattering of a plane electromagnetic wave by a plasma column in steady magnetic fields (cold plasma approximation) ; hot non-uniform plasma column ; metallic and dielectric resonance probes, plasma-dielectric coated antenna, general considerations.

  14. NLO Electroweak Corrections to Higgs Decay to Two Photons

    OpenAIRE

    Actis, Stefano

    2009-01-01

    The recent calculation of the next-to-leading order electroweak corrections to the decay of the Standard Model Higgs boson to two photons in the framework of the complex-mass scheme is briefly summarized.

  15. Standard Model Higgs decay for two Photons in CMS

    CERN Multimedia

    Daniel Denegri

    2000-01-01

    Simulated two-photon mass distribution for SM Higgs and expected background in the CMS PbW04 crystal calorimeter for an integrated luminosity of 10 . 5 pb-1, with detailed simulation of calorimeter response.

  16. Two-photon pumped lead halide perovskite nanowire lasers

    CERN Document Server

    Gu, Zhiyuan; Sun, Wenzhao; Li, Jinakai; Liu, Shuai; Song, Qinghai; Xiao, Shumin

    2015-01-01

    Solution-processed lead halide perovskites have shown very bright future in both solar cells and microlasers. Very recently, the nonlinearity of perovskites started to attract considerable research attention. Second harmonic generation and two-photon absorption have been successfully demonstrated. However, the nonlinearity based perovskite devices such as micro- & nano- lasers are still absent. Here we demonstrate the two-photon pumped nanolasers from perovskite nanowires. The CH3NH3PbBr3 perovskite nanowires were synthesized with one-step solution self-assembly method and dispersed on glass substrate. Under the optical excitation at 800 nm, two-photon pumped lasing actions with periodic peaks have been successfully observed at around 546 nm. The obtained quality (Q) factors of two-photon pumped nanolasers are around 960, and the corresponding thresholds are about 674?J=cm2. Both the Q factors and thresholds are comparable to conventional whispering gallery modes in two-dimensional polygon microplates. Ou...

  17. Generating photon pairs from a silicon microring resonator using an electronic step recovery diode for pump pulse generation

    CERN Document Server

    Savanier, Marc

    2016-01-01

    Generation of photon pairs from compact, manufacturable and inexpensive silicon (Si) photonic devices at room temperature may help develop practical applications of quantum photonics. An important characteristic of photon-pair generation is the two-photon joint spectral intensity (JSI), which describes the frequency correlations of the photon pair. In particular, heralded single-photon generation requires uncorrelated photons, rather than the highly anti-correlated photons conventionally obtained under continuous-wave (CW) pumping. Recent attempts to achieve such a factorizable JSI have used short optical pulses from mode-locked lasers, which are much more expensive and bigger table-top or rack-sized instruments compared to the Si microchip pair generator, dominate the cost and inhibit the miniaturization of the source. Here, we generate photon pairs from a Si microring resonator by using an electronic step-recovery diode to drive an electro-optic modulator which carves the pump light from a CW optical diode ...

  18. Electron Spin Resonance at the Level of 1 04 Spins Using Low Impedance Superconducting Resonators

    Science.gov (United States)

    Eichler, C.; Sigillito, A. J.; Lyon, S. A.; Petta, J. R.

    2017-01-01

    We report on electron spin resonance measurements of phosphorus donors localized in a 200 μ m2 area below the inductive wire of a lumped element superconducting resonator. By combining quantum limited parametric amplification with a low impedance microwave resonator design, we are able to detect around 2 ×1 04 spins with a signal-to-noise ratio of 1 in a single shot. The 150 Hz coupling strength between the resonator field and individual spins is significantly larger than the 1-10 Hz coupling rates obtained with typical coplanar waveguide resonator designs. Because of the larger coupling rate, we find that spin relaxation is dominated by radiative decay into the resonator and dependent upon the spin-resonator detuning, as predicted by Purcell.

  19. Synthesis of a Series of Novel Organic Compounds with Two-photon Absorption and Two-photon pumped Lasing

    Institute of Scientific and Technical Information of China (English)

    2001-01-01

    A series of novel organic compounds named as CSPI, DPASPI, PSPI DEASPI and HEASPI respectively, with large two-photon absorption has been synthesized and their structures have been determined by 1HNMR and elemental analysis. The highest two-photon pumped (TPP) output /input efficiency is as high as 13.4% for PSPI in DMF with d0 = 0.03 mol/L and the effective two-photon absorption cross section is 8.8′10-48 cm4×s/photon for DPASPI in DMF with d0= 0.05mol/L.

  20. Two-photon photoemission from a copper cathode in an X -band photoinjector

    Science.gov (United States)

    Li, H.; Limborg-Deprey, C.; Adolphsen, C.; McCormick, D.; Dunning, M.; Jobe, K.; Raubenheimer, T.; Vrielink, A.; Vecchione, T.; Wang, F.; Weathersby, S.

    2016-02-01

    This paper presents two-photon photoemission from a copper cathode in an X -band photoinjector. We experimentally verified that the electron bunch charge from photoemission out of a copper cathode scales with laser intensity (I) square for 400 nm wavelength photons. We compare this two-photon photoemission process with the single photon process at 266 nm. Despite the high reflectivity (R ) of the copper surface for 400 nm photons (R =0.48 ) and higher thermal energy of photoelectrons (two-photon at 200 nm) compared to 266 nm photoelectrons, the quantum efficiency of the two-photon photoemission process (400 nm) exceeds the single-photon process (266 nm) when the incident laser intensity is above 300 GW /cm2 . At the same laser pulse energy (E ) and other experimental conditions, emitted charge scales inversely with the laser pulse duration. A thermal emittance of 2.7 mm-mrad per mm root mean square (rms) was measured on our cathode which exceeds by sixty percent larger compared to the theoretical predictions, but this discrepancy is similar to previous experimental thermal emittance on copper cathodes with 266 nm photons. The damage of the cathode surface of our first-generation X -band gun from both rf breakdowns and laser impacts mostly explains this result. Using a 400 nm laser can substantially simplify the photoinjector system, and make it an alternative solution for compact pulsed electron sources.

  1. Resonant enhancement of relativistic electron fluxes during geomagnetically active periods

    Directory of Open Access Journals (Sweden)

    I. Roth

    Full Text Available The strong increase in the flux of relativistic electrons during the recovery phase of magnetic storms and during other active periods is investigated with the help of Hamiltonian formalism and simulations of test electrons which interact with whistler waves. The intensity of the whistler waves is enhanced significantly due to injection of 10-100 keV electrons during the substorm. Electrons which drift in the gradient and curvature of the magnetic field generate the rising tones of VLF whistler chorus. The seed population of relativistic electrons which bounce along the inhomogeneous magnetic field, interacts resonantly with the whistler waves. Whistler wave propagating obliquely to the magnetic field can interact with energetic electrons through Landau, cyclotron, and higher harmonic resonant interactions when the Doppler-shifted wave frequency equals any (positive or negative integer multiple of the local relativistic gyrofrequency. Because the gyroradius of a relativistic electron may be the order of or greater than the perpendicular wavelength, numerous cyclotron, harmonics can contribute to the resonant interaction which breaks down the adiabatic invariant. A similar process diffuses the pitch angle leading to electron precipitation. The irreversible changes in the adiabatic invariant depend on the relative phase between the wave and the electron, and successive resonant interactions result in electrons undergoing a random walk in energy and pitch angle. This resonant process may contribute to the 10-100 fold increase of the relativistic electron flux in the outer radiation belt, and constitute an interesting relation between substorm-generated waves and enhancements in fluxes of relativistic electrons during geomagnetic storms and other active periods.

    Key words. Magnetospheric physics (energetic particles · trapped; plasma waves and instabilities; storms and substorms

  2. Mass distribution for the two-photon channel

    CERN Multimedia

    ATLAS, collaboration

    2012-01-01

    Mass distribution for the two-photon channel. The strongest evidence for this new particle comes from analysis of events containing two photons. The smooth dotted line traces the measured background from known processes. The solid line traces a statistical fit to the signal plus background. The new particle appears as the excess around 126.5 GeV. The full analysis concludes that the probability of such a peak is three chances in a million.

  3. Vibrationally dependent electron-electron interactions in resonant electron transport through single-molecule junctions

    Science.gov (United States)

    Erpenbeck, A.; Härtle, R.; Bockstedte, M.; Thoss, M.

    2016-03-01

    We investigate the role of electronic-vibrational coupling in resonant electron transport through single-molecule junctions, taking into account that the corresponding coupling strengths may depend on the charge and excitation state of the molecular bridge. Within an effective-model Hamiltonian approach for a molecule with multiple electronic states, this requires to extend the commonly used model and include vibrationally dependent electron-electron interaction. We use Born-Markov master equation methods and consider selected models to exemplify the effect of the additional interaction on the transport characteristics of a single-molecule junction. In particular, we show that it has a significant influence on local cooling and heating mechanisms, it may result in negative differential resistance, and it may cause pronounced asymmetries in the conductance map of a single-molecule junction.

  4. Resonant Production of Color Octet Electron at the Lhec

    CERN Document Server

    Sahin, M; Turkoz, S

    2010-01-01

    In composite models with colored preons leptogluons (l_(8)) has a same status with leptoquarks, excited leptons and quarks etc. We analyze resonant production of color octet electron (e_(8)) at QCD Explorer stage of the Large Hadron electron Collider (LHeC). It is shown that the e_(8) discovery at the LHeC will simultaneously determine the compositeness scale.

  5. Site directed spin labelling and pulsed dipolar electron paramagnetic resonance (double electron-electron resonance) of force activation in muscle

    Energy Technology Data Exchange (ETDEWEB)

    Fajer, Piotr G [Institute of Molecular Biophysics, Department of Biological Science, National High Magnetic Field Laboratory, Florida State University, Tallahassee, FL 32310 (United States)

    2005-05-11

    The recent development of site specific spin labelling and advances in pulsed electron paramagnetic resonance(EPR) have established spin labelling as a viable structural biology technique. Specific protein sites or whole domains can be selectively targeted for spin labelling by cysteine mutagenesis. The secondary structure of the proteins is determined from the trends in EPR signals of labels attached to consecutive residues. Solvent accessibility or label mobility display periodicities along the labelled polypeptide chain that are characteristic of {beta}-strands (periodicity of 2 residues) or {alpha}-helices (3.6 residues). Low-resolution 3D structure of proteins is determined from the distance restraints. Two spin labels placed within 60-70 A of each other create a local dipolar field experienced by the other spin labels. The strength of this field is related to the interspin distance, {proportional_to} r{sup -3}. The dipolar field can be measured by the broadening of the EPR lines for the short distances (8-20 A) or for the longer distances (17-70 A) by the pulsed EPR methods, double electron-electron resonance(DEER) and double quantum coherence (DQC). A brief review of the methodology and its applications to the multisubunit muscle protein troponin is presented below.

  6. Distribution of quantum information between an atom and two photons

    Energy Technology Data Exchange (ETDEWEB)

    Weber, Bernhard

    2008-11-03

    The construction of networks consisting of optically interconnected processing units is a promising way to scale up quantum information processing systems. To store quantum information, single trapped atoms are among the most proven candidates. By placing them in high finesse optical resonators, a bidirectional information exchange between the atoms and photons becomes possible with, in principle, unit efficiency. Such an interface between stationary and ying qubits constitutes a possible node of a future quantum network. The results presented in this thesis demonstrate the prospects of a quantum interface consisting of a single atom trapped within the mode of a high-finesse optical cavity. In a two-step process, we distribute entanglement between the stored atom and two subsequently emitted single photons. The long atom trapping times achieved in the system together with the high photon collection efficiency of the cavity make the applied protocol in principle deterministic, allowing for the creation of an entangled state at the push of a button. Running the protocol on this quasi-stationary quantum interface, the internal state of the atom is entangled with the polarization state of a single emitted photon. The entanglement is generated by driving a vacuum-stimulated Raman adiabatic passage between states of the coupled atom-cavity system. In a second process, the atomic part of the entangled state is mapped onto a second emitted photon using a similar technique and resulting in a polarization-entangled two-photon state. To verify and characterize the photon-photon entanglement, we measured a violation of a Bell inequality and performed a full quantum state tomography. The results prove the prior atom-photon entanglement and demonstrate a quantum information transfer between the atom and the two emitted photons. This reflects the advantages of a high-finesse cavity as a quantum interface in future quantum networks. (orig.)

  7. Dynamical modeling of pulsed two-photon interference

    Science.gov (United States)

    Fischer, Kevin A.; Müller, Kai; Lagoudakis, Konstantinos G.; Vučković, Jelena

    2016-11-01

    Single-photon sources are at the heart of quantum-optical networks, with their uniquely quantum emission and phenomenon of two-photon interference allowing for the generation and transfer of nonclassical states. Although a few analytical methods have been briefly investigated for describing pulsed single-photon sources, these methods apply only to either perfectly ideal or at least extremely idealized sources. Here, we present the first complete picture of pulsed single-photon sources by elaborating how to numerically and fully characterize non-ideal single-photon sources operating in a pulsed regime. In order to achieve this result, we make the connection between quantum Monte-Carlo simulations, experimental characterizations, and an extended form of the quantum regression theorem. We elaborate on how an ideal pulsed single-photon source is connected to its photocount distribution and its measured degree of second- and first-order optical coherence. By doing so, we provide a description of the relationship between instantaneous source correlations and the typical experimental interferometers (Hanbury-Brown and Twiss, Hong-Ou-Mandel, and Mach-Zehnder) used to characterize such sources. Then, we use these techniques to explore several prototypical quantum systems and their non-ideal behaviors. As an example numerical result, we show that for the most popular single-photon source—a resonantly excited two-level system—its error probability is directly related to its excitation pulse length. We believe that the intuition gained from these representative systems and characters can be used to interpret future results with more complicated source Hamiltonians and behaviors. Finally, we have thoroughly documented our simulation methods with contributions to the Quantum Optics Toolbox in Python in order to make our work easily accessible to other scientists and engineers.

  8. Two-Photon Exchange Corrections to Precise Measurements of Proton Electroweak Form Factors

    Science.gov (United States)

    Afanasev, Andrei

    2004-10-01

    Higher-order QED effects play an important role for extracting information on proton form factors from electron scattering data. For the electric form factor of the proton, a previously neglected two-photon-exchange correction reconciles an observed discrepancy between Rosenbluth and polarization techniques [1]. We use a similar approach based on General Parton Distributions to compute additional radiative corrections to parity-violating electron scattering. [1] Y.C. Chen, A. Afanasev, S.J. Brodsky, C.E. Carlson and M. Vanderhaeghen, ``Partonic calculation of the two-photon exchange contribution to elastic electron proton scattering at large momentum transfer,`` arXiv:hep-ph/0403058, to appear in Phys.Rev.Lett.

  9. Charmonium production in ultra-peripheral heavy ion collisions with two-photon processes

    Science.gov (United States)

    Yu, Gong-Ming; Yu, Yue-Chao; Li, Yun-De; Wang, Jian-Song

    2017-04-01

    We calculate the production of large-pT charmonium and narrow resonance state (exotic charmonium) in proton-proton, proton-nucleus, and nucleus-nucleus collisions with the semi-coherent two-photon interactions at Relativistic Heavy Ion Collider (RHIC), Large Hadron Collider (LHC), and Future Circular Collider (FCC) energies. Using the large quasi-real photon fluxes, we present the γγ → H differential cross section for charmonium and narrow resonance state production at large transverse momentum in ultra-peripheral heavy ion collisions. The numerical results demonstrate that the experimental study of ultra-peripheral collisions is feasible at RHIC, LHC, and FCC energies.

  10. Two-photon gateway in one-atom cavity quantum electrodynamics

    OpenAIRE

    2008-01-01

    Single atoms absorb and emit light from a resonant laser beam photon by photon. We show that a single atom strongly coupled to an optical cavity can absorb and emit resonant photons in pairs. The effect is observed in a photon correlation experiment on the light transmitted through the cavity. We find that the atom-cavity system transforms a random stream of input photons into a correlated stream of output photons, thereby acting as a two-photon gateway. The phenomenon has its origin in the q...

  11. Imaging marine virus CroV and its host Cafeteria roenbergensis with two-photon microscopy

    Science.gov (United States)

    Cao, Bin; Chakraborty, Sayan; Sun, Wenqing; Aghvami, Seyedmohammadali; Fischer, Matthias G.; Qian, Wei; Xiao, Chuan; Li, Chunqiang

    2014-02-01

    We use two-photon microscopy to monitor the infection process of marine zooplankton, Cafeteria roenbergensis (C.roenbergensis), by Cafeteria roenbergensis virus (CroV), a giant DNA virus named after its host. Here, we image C.roenbergensis in culture by two-photon excited NADH autofluorescence at video-rate (30 frame/s), and the movement of C.roenbergensis is recorded in live videos. Moreover, CroV is stained with DNA dye SYBR gold and recorded simultaneously with this two-photon microscope. We observed the initial infection moment with this method. The result demonstrates the potential use of two-photon microscopy to investigate the fast dynamic interaction between C.roenbergensis with virus CroV. After catching this initial moment, we will freeze the sample in liquid nitrogen for cryo-electron microscopy (EM) study to resolve the virus-host interaction at molecular level. The long-term goal is to study similar fast moving pathogen-host interaction process which could lead to important medical applications.

  12. Solvent effects on optical properties of a newly synthesized two-photon polymerization initiator: BPYPA

    Institute of Scientific and Technical Information of China (English)

    Guo Ya-Hui; Sun Yuan-Hong; Tao Li-Min; Zhao Ke; Wang Chuan-Kui

    2005-01-01

    Time-dependent hybrid density functional theory in combination with polarized continuum model is applied to study the solvent effects on the geometrical and electronic structures as well as one- and two-photon absorption processes,of a newly synthesized asymmetrical charge-transfer organic molecule bis-(4-bromo-phenyl)-[4-(2-pyridin-4-yl-vinyl)phenyl]-amine (BPYPA). There exist two charge-transfer states for the compound in visible region. The two-photon absorption cross section calculated by a three-state model and solvatochromic shift of the charge-transfer states are found to be solvent-dependent, where a nonmonotonic behaviour with respect to the polarity of the solvents is observed. The numerical results show that the organic molecule exhibits a rather large two-photon absorption cross section as compared with the compound 4-trans-[p-(N, N-Di-n-butylamino)-p-stilbenyl vinyl] pyridine (DBASVP) reported previously, and is predicted to be a good two-photon polymerization initiator. The hydrogen-bond effect is analysed. The computational results are in good agreement with the measurements.

  13. $\\chi_{c2}$ formation in two-photon collisions at LEP

    CERN Document Server

    Acciarri, M; Adriani, O; Aguilar-Benítez, M; Alcaraz, J; Alemanni, G; Allaby, James V; Aloisio, A; Alviggi, M G; Ambrosi, G; Anderhub, H; Andreev, V P; Angelescu, T; Anselmo, F; Arefev, A; Azemoon, T; Aziz, T; Bagnaia, P; Baksay, L; Balandras, A; Ball, R C; Banerjee, S; Banerjee, Sw; Banicz, K; Barczyk, A; Barillère, R; Barone, L; Bartalini, P; Basile, M; Battiston, R; Bay, A; Becattini, F; Becker, U; Behner, F; Berdugo, J; Berges, P; Bertucci, B; Betev, B L; Bhattacharya, S; Biasini, M; Biland, A; Blaising, J J; Blyth, S C; Bobbink, Gerjan J; Böck, R K; Böhm, A; Boldizsar, L; Borgia, B; Bourilkov, D; Bourquin, Maurice; Braccini, S; Branson, J G; Brigljevic, V; Brochu, F; Buffini, A; Buijs, A; Burger, J D; Burger, W J; Busenitz, J K; Button, A M; Cai, X D; Campanelli, M; Capell, M; Cara Romeo, G; Carlino, G; Cartacci, A M; Casaus, J; Castellini, G; Cavallari, F; Cavallo, N; Cecchi, C; Cerrada-Canales, M; Cesaroni, F; Chamizo-Llatas, M; Chang, Y H; Chaturvedi, U K; Chemarin, M; Chen, A; Chen, G; Chen, G M; Chen, H F; Chen, H S; Chéreau, X J; Chiefari, G; Cifarelli, Luisa; Cindolo, F; Civinini, C; Clare, I; Clare, R; Coignet, G; Colijn, A P; Colino, N; Costantini, S; Cotorobai, F; de la Cruz, B; Csilling, Akos; Dai, T S; van Dalen, J A; D'Alessandro, R; De Asmundis, R; Déglon, P L; Degré, A; Deiters, K; Della Volpe, D; Denes, P; De Notaristefani, F; De Salvo, A; Diemoz, M; Van Dierendonck, D N; Di Lodovico, F; Dionisi, C; Dittmar, Michael; Dominguez, A; Doria, A; Dova, M T; Duchesneau, D; Dufournaud, D; Duinker, P; Durán, I; El-Mamouni, H; Engler, A; Eppling, F J; Erné, F C; Extermann, Pierre; Fabre, M; Faccini, R; Falagán, M A; Falciano, S; Favara, A; Fay, J; Fedin, O; Felcini, Marta; Ferguson, T; Ferroni, F; Fesefeldt, H S; Fiandrini, E; Field, J H; Filthaut, Frank; Fisher, P H; Fisk, I; Forconi, G; Fredj, L; Freudenreich, Klaus; Furetta, C; Galaktionov, Yu; Ganguli, S N; García-Abia, P; Gataullin, M; Gau, S S; Gentile, S; Gheordanescu, N; Giagu, S; Goldfarb, S; Gong, Z F; Grünewald, M W; van Gulik, R; Gupta, V K; Gurtu, A; Gutay, L J; Haas, D; Hartmann, B; Hasan, A; Hatzifotiadou, D; Hebbeker, T; Hervé, A; Hidas, P; Hirschfelder, J; Hofer, H; Holzner, G; Hoorani, H; Hou, S R; Iashvili, I; Jin, B N; Jones, L W; de Jong, P; Josa-Mutuberria, I; Khan, R A; Kamrad, D; Kapustinsky, J S; Kaur, M; Kienzle-Focacci, M N; Kim, D; Kim, D H; Kim, J K; Kim, S C; Kinnison, W W; Kirkby, Jasper; Kiss, D; Kittel, E W; Klimentov, A; König, A C; Kopp, A; Korolko, I; Koutsenko, V F; Krämer, R W; Krenz, W; Kunin, A; Lacentre, P E; Ladrón de Guevara, P; Laktineh, I; Landi, G; Lapoint, C; Lassila-Perini, K M; Laurikainen, P; Lavorato, A; Lebeau, M; Lebedev, A; Lebrun, P; Lecomte, P; Lecoq, P; Le Coultre, P; Lee, H J; Le Goff, J M; Leiste, R; Leonardi, E; Levchenko, P M; Li Chuan; Lin, C H; Lin, W T; Linde, Frank L; Lista, L; Liu, Z A; Lohmann, W; Longo, E; Lü, Y S; Lübelsmeyer, K; Luci, C; Luckey, D; Luminari, L; Lustermann, W; Ma Wen Gan; Maity, M; Majumder, G; Malgeri, L; Malinin, A; Maña, C; Mangeol, D J J; Marchesini, P A; Marian, G; Martin, J P; Marzano, F; Massaro, G G G; Mazumdar, K; McNeil, R R; Mele, S; Merola, L; Meschini, M; Metzger, W J; Von der Mey, M; Migani, D; Mihul, A; Milcent, H; Mirabelli, G; Mnich, J; Molnár, P; Monteleoni, B; Moulik, T; Muanza, G S; Muheim, F; Muijs, A J M; Nahn, S; Napolitano, M; Nessi-Tedaldi, F; Newman, H; Niessen, T; Nippe, A; Nisati, A; Nowak, H; Oh, Yu D; Organtini, G; Ostonen, R; Palomares, C; Pandoulas, D; Paoletti, S; Paolucci, P; Park, H K; Park, I H; Pascale, G; Passaleva, G; Patricelli, S; Paul, T; Pauluzzi, M; Paus, C; Pauss, Felicitas; Peach, D; Pedace, M; Pei, Y J; Pensotti, S; Perret-Gallix, D; Petersen, B; Petrak, S; Piccolo, D; Pieri, M; Piroué, P A; Pistolesi, E; Plyaskin, V; Pohl, M; Pozhidaev, V; Postema, H; Pothier, J; Produit, N; Prokofev, D; Prokofiev, D O; Quartieri, J; Rahal-Callot, G; Raja, N; Rancoita, P G; Raven, G; Razis, P A; Ren, D; Rescigno, M; Reucroft, S; Van Rhee, T; Riemann, S; Riles, K; Robohm, A; Rodin, J; Roe, B P; Romero, L; Rosier-Lees, S; Roth, S; Rubio, Juan Antonio; Ruschmeier, D; Rykaczewski, H; Sakar, S; Salicio, J; Sánchez, E; Sanders, M P; Sarakinos, M E; Schäfer, C; Shchegelskii, V; Schmidt-Kärst, S; Schmitz, D; Scholz, N; Schopper, Herwig Franz; Schotanus, D J; Schwenke, J; Schwering, G; Sciacca, C; Sciarrino, D; Servoli, L; Shevchenko, S; Shivarov, N; Shoutko, V; Shukla, J; Shumilov, E; Shvorob, A V; Siedenburg, T; Son, D; Smith, B; Spillantini, P; Steuer, M; Stickland, D P; Stone, A; Stone, H; Stoyanov, B; Strässner, A; Sudhakar, K; Sultanov, G G; Sun, L Z; Suter, H; Swain, J D; Szillási, Z; Tang, X W; Tauscher, Ludwig; Taylor, L; Timmermans, C; Ting, Samuel C C; Ting, S M; Tonwar, S C; Tóth, J; Tully, C; Tung, K L; Uchida, Y; Ulbricht, J; Valente, E

    1999-01-01

    Two-photon formation of the charmonium resonance $\\chi_{{\\rm c}2}$ has been studied with the L3 detector at LEP. The $\\chi_{{\\rm c}2}$ is identified through its decay $\\chi_{{\\rm c}2} \\rightarrow \\gamma {\\rm J}$, with a subsequent decay ${\\rm J} \\rightarrow {\\mathrm{e^+ e^-}}$ or ${\\rm J} \\rightarrow {\\mathrm{\\mu^+ \\mu^-}}$. With an integrated luminosity of 140 pb$^{-1}$ at $\\sqrt{s} \\simeq$ 91~\\textrm{Ge\\kern -0.1em V} and 52 pb$^{-1}$ at $\\sqrt{s} \\simeq$ {Ge\\kern -0.1em V}, we measure the two-photon width of the $\\chi_{{\\rm c}2}$ to be \\begin{center} $\\Gamma_{\\gamma\\gamma}(\\chi_{{\\rm c}2})=1.02 \\pm 0.40 \\mbox{$\\;$(stat.)} \\pm 0.15 \\mbox{$\\;$(sys.)} \\pm 0.09(\\rm{BR.}) {\\mathrm{\\ ke\\kern -0.1em V}}$.

  14. Slow reflection and two-photon generation of microcavity exciton-polaritons

    CERN Document Server

    Steger, Mark; Snoke, David W; Pfeiffer, Loren; West, Ken

    2014-01-01

    We resonantly inject polaritons into a microcavity and track them in time and space as they feel a force due to the cavity gradient. This is an example of "slow reflection," as the polaritons, which can be viewed as renormalized photons, slow down to zero velocity and then move back in the opposite direction. These measurements accurately measure the lifetime of the polaritons in our samples, which is 180 $\\pm$ 10 ps, corresponding to a cavity leakage time of 135 ps and a cavity $Q$ of 320,000. Such long-lived polaritons propagate millimeters in these wedge-shaped microcavities. Additionally, we generate polaritons by two-photon excitation directly into the polariton states, allowing the possibility of modulation of the two-photon absorption by a polariton condensate.

  15. Two-photon interference from independent cavity-coupled emitters on-a-chip

    CERN Document Server

    Kim, Je-Hyung; Leavitt, Richard P; Waks, Edo

    2016-01-01

    Interactions between solid-state quantum emitters and cavities are important for a broad range of applications in quantum communication, linear optical quantum computing, nonlinear photonics, and photonic quantum simulation. These applications often require combining many devices on a single chip with identical emission wavelengths in order to generate two-photon interference, the primary mechanism for achieving effective photon-photon interactions. Such integration remains extremely challenging due to inhomogeneous broadening and fabrication errors that randomize the resonant frequencies of both the emitters and cavities. In this letter we demonstrate two-photon interference from independent cavity-coupled emitters on the same chip, providing a potential solution to this long-standing problem. We overcome spectral mismatch between different cavities due to fabrication errors by depositing and locally evaporating a thin layer of condensed nitrogen. We integrate optical heaters to tune individual dots within e...

  16. Generalized Kramers-Heisenberg expressions for stimulated Raman scattering and two-photon absorption

    Science.gov (United States)

    Roslyak, Oleksiy; Marx, Christoph A.; Mukamel, Shaul

    2010-01-01

    The frequency-domain pump-probe signal of a material system interacting with two quantum modes of the radiation field is recast in terms of products of scattering amplitudes (T matrix elements) rather than the third-order susceptibility Im χ(3). The resulting expression offers a more intuitive physical picture for the optical process compared with the semiclassical approach which treats the radiation field as classical. It can be derived and interpreted using closed-time-path-loop diagrams which represent the joint state of the matter and the field for each contribution to the signal. The signal has two components representing stimulated Raman scattering ω1 − ω2 and two-photon absorption ω1 + ω2 two-photon resonances. Both are expressed as nonequi-librium steady-state photon and matter fluxes, as is common in the description of dissipative processes in open quantum systems. PMID:20613889

  17. Additive controlled synthesis of gold nanorods (GNRs) for two-photon luminescence imaging of cancer cells

    Energy Technology Data Exchange (ETDEWEB)

    Zhu Jing; Roy, Indrajit; Hu Rui; Ding Hong; Zhao Lingling; He, Guang S; Prasad, Paras N [Institute for Lasers, Photonics and Biophotonics, University at Buffalo, State University of New York, Buffalo, NY 14260-4200 (United States); Yong, Ken-Tye [School of Electrical and Electronic Engineering, Nanyang Technological University, Singapore 639798 (Singapore); Swihart, Mark T [Department of Chemical and Biological Engineering, University at Buffalo, State University of New York, Buffalo, NY 14260-4200 (United States); Cui Yiping, E-mail: ktyong@ntu.edu.sg, E-mail: cyp@seu.edu.cn, E-mail: pnprasad@buffalo.edu [Advanced Photonics Center, School of Electronic Science and Engineering, Southeast University, Nanjing 210096 (China)

    2010-07-16

    Gold nanorods (GNRs) with a longitudinal surface plasmon resonance peak that is tunable from 600 to 1100 nm have been fabricated in a cetyl trimethylammoniumbromide (CTAB) micellar medium using hydrochloric acid and silver nitrate as additives to control their shape and size. By manipulating the concentrations of silver nitrate and hydrochloric acid, the aspect ratio of the GNRs was reliably and reproducibly tuned from 2.5 to 8. The GNRs were first coated with polyelectrolyte multilayers and then bioconjugated to transferrin (Tf) to target pancreatic cancer cells. Two-photon imaging excited from the bioconjugated GNRs demonstrated receptor-mediated uptake of the bioconjugates into Panc-1 cells, overexpressing the transferrin receptor (TfR). The bioconjugated GNR formulation exhibited very low toxicity, suggesting that it is biocompatible and potentially suitable for targeted two-photon bioimaging.

  18. Additive controlled synthesis of gold nanorods (GNRs) for two-photon luminescence imaging of cancer cells.

    Science.gov (United States)

    Zhu, Jing; Yong, Ken-Tye; Roy, Indrajit; Hu, Rui; Ding, Hong; Zhao, Lingling; Swihart, Mark T; He, Guang S; Cui, Yiping; Prasad, Paras N

    2010-07-16

    Gold nanorods (GNRs) with a longitudinal surface plasmon resonance peak that is tunable from 600 to 1100 nm have been fabricated in a cetyl trimethylammoniumbromide (CTAB) micellar medium using hydrochloric acid and silver nitrate as additives to control their shape and size. By manipulating the concentrations of silver nitrate and hydrochloric acid, the aspect ratio of the GNRs was reliably and reproducibly tuned from 2.5 to 8. The GNRs were first coated with polyelectrolyte multilayers and then bioconjugated to transferrin (Tf) to target pancreatic cancer cells. Two-photon imaging excited from the bioconjugated GNRs demonstrated receptor-mediated uptake of the bioconjugates into Panc-1 cells, overexpressing the transferrin receptor (TfR). The bioconjugated GNR formulation exhibited very low toxicity, suggesting that it is biocompatible and potentially suitable for targeted two-photon bioimaging.

  19. Electron Paramagnetic Resonance Imaging: 1. CW-EPR Imaging

    Indian Academy of Sciences (India)

    2016-07-01

    Twentieth century bore witness to remarkable scientists whohave advanced our understanding of the brain. Among them,EPR (Electron Paramagnetic Resonance) imaging is particularlyuseful in monitoring hypoxic zones in tumors which arehighly resistant to radiation and chemotherapeutic treatment.This first part of the article covers aspects of CW(continuous wave) imaging with details of FT (pulsed FourierTransform)-EPR imaging covered in Part 2, to be publishedin the next issue of Resonance.

  20. Two-photon flow cytometer with laser scanning Bessel beams

    Science.gov (United States)

    Wang, Yongdong; Ding, Yu; Ray, Supriyo; Paez, Aurelio; Xiao, Chuan; Li, Chunqiang

    2016-03-01

    Flow cytometry is an important technique in biomedical discovery for cell counting, cell sorting and biomarker detection. In vivo flow cytometers, based on one-photon or two-photon excited fluorescence, have been developed for more than a decade. One drawback of laser beam scanning two-photon flow cytometer is that the two-photon excitation volume is fairly small due to the short Rayleigh range of a focused Gaussian beam. Hence, the sampling volume is much smaller than one-photon flow cytometry, which makes it challenging to count or detect rare circulating cells in vivo. Bessel beams have narrow intensity profiles with an effective spot size (FWHM) as small as several wavelengths, making them comparable to Gaussian beams. More significantly, the theoretical depth of field (propagation distance without diffraction) can be infinite, making it an ideal solution as a light source for scanning beam flow cytometry. The trade-off of using Bessel beams rather than a Gaussian beam is the fact that Bessel beams have small concentric side rings that contribute to background noise. Two-photon excitation can reduce this noise, as the excitation efficiency is proportional to intensity squared. Therefore, we developed a two-photon flow cytometer using scanned Bessel beams to form a light sheet that intersects the micro fluidic channel.

  1. Confocal and Two-Photon Microscopy: Foundations, Applications and Advances

    Science.gov (United States)

    Diaspro, Alberto

    2001-11-01

    Confocal and Two-Photon Microscopy Foundations, Applications, and Advances Edited by Alberto Diaspro Confocal and two-photon fluorescence microscopy has provided researchers with unique possibilities of three-dimensional imaging of biological cells and tissues and of other structures such as semiconductor integrated circuits. Confocal and Two-Photon Microscopy: Foundations, Applications, and Advances provides clear, comprehensive coverage of basic foundations, modern applications, and groundbreaking new research developments made in this important area of microscopy. Opening with a foreword by G. J. Brakenhoff, this reference gathers the work of an international group of renowned experts in chapters that are logically divided into balanced sections covering theory, techniques, applications, and advances, featuring: In-depth discussion of applications for biology, medicine, physics, engineering, and chemistry, including industrial applications Guidance on new and emerging imaging technology, developmental trends, and fluorescent molecules Uniform organization and review-style presentation of chapters, with an introduction, historical overview, methodology, practical tips, applications, future directions, chapter summary, and bibliographical references Companion FTP site with full-color photographs The significant experience of pioneers, leaders, and emerging scientists in the field of confocal and two-photon excitation microscopy Confocal and Two-Photon Microscopy: Foundations, Applications, and Advances is invaluable to researchers in the biological sciences, tissue and cellular engineering, biophysics, bioengineering, physics of matter, and medicine, who use these techniques or are involved in developing new commercial instruments.

  2. Resonance effects of excitons and electrons. Basics and applications

    Energy Technology Data Exchange (ETDEWEB)

    Geru, Ion [Moldovan Academy of Sciences, Chisinau (Moldova, Republic of). Inst. of Chemistry; Suter, Dieter [Technische Univ. Dortmund (Germany). Fakultaet Physik

    2013-08-01

    Represents the first book on non-traditional resonance effects of excitons in semiconductors. Explains resonance phenomena of excitons and electrons in solids. Presents the Knight shift at the Bose-Einstein condensation of excitons. This book presents the various types of resonance effects on excitons, biexcitons and the local electronic centers (LEC) in solids, such as paramagnetic and paraelectric resonances on excitons, exciton acoustic resonance at intra- and interband transitions, radio-optical double resonance on excitons, hole-nuclear double resonance on localized biexcitons, ENDOR and acoustic ENDOR on LEC. The criteria for the generation of coherent photons, phonons and magnons by excitons are explained. The interactions of excitons and biexcitons with paramagnetic centers and nuclear spins, the indirect interaction between the PC through a field of excitons as well as the quasienergy spectrum of excitons and spin systems are discussed. It is proved that the interaction of paramagnetic centers with excitons increases the spin relaxation rate of paramagnetic centers in comparison with the case of their interaction with free carriers. The giant magneto-optical effects in semi-magnetic semiconductors are theoretically interpreted. In recent years, a new perspective has been added to these systems and their interactions: they can be used for storing and processing information in the form of quantum bits (qubits), the building blocks of quantum computers. The basics of this emerging technology are explained and examples of demonstration-type quantum computers based on localized spins in solids are discussed.

  3. Resonance fluorescence and electron spin in semiconductor quantum dots

    Energy Technology Data Exchange (ETDEWEB)

    Zhao, Yong

    2009-11-18

    The work presented in this dissertation contains the first observation of spin-resolved resonance fluorescence from a single quantum dot and its application of direct measurement of electron spin dynamics. The Mollow triplet and the Mollow quintuplet, which are the hallmarks of resonance fluorescence, are presented as the non-spin-resolved and spin-resolved resonance fluorescence spectrum, respectively. The negligible laser background contribution, the near pure radiative broadened spectrum and the anti-bunching photon statistics imply the sideband photons are background-free and near transform-limited single photons. This demonstration is a promising step towards the heralded single photon generation and electron spin readout. Instead of resolving spectrum, an alternative spin-readout scheme by counting resonance fluorescence photons under moderate laser power is demonstrated. The measurements of n-shot time-resolved resonance fluorescence readout are carried out to reveal electron spin dynamics of the measurement induced back action and the spin relaxation. Hyperfine interaction and heavy-light hole mixing are identified as the relevant mechanisms for the back action and phonon-assistant spin-orbit interaction dominates the spin relaxation. After a detailed discussion on charge-spin configurations in coupled quantum dots system, the single-shot readout on electron spin are proposed. (orig.)

  4. Electron cyclotron resonance heating and current drive

    Energy Technology Data Exchange (ETDEWEB)

    Fidone, I.; Castejon, F.

    1992-07-01

    A brief summary of the theory and experiments on electron- cyclotron heating and current drive is presented. The general relativistic formulation of wave propagation and linear absorption is considered in some detail. The O-mode and the X-mode for normal and oblique propagation are investigated and illustrated by several examples. The experimental verification of the theory in T-10 and D- III-D is briefly discussed. Quasilinear evolution of the momentum distribution and related applications as, for instance, non linear wave, damping and current drive, are also considered for special cases of wave frequencies, polarization and propagation. In the concluding section we present the general formulation of the wave damping and current drive in the absence of electron trapping for arbitrary values of the wave frequency. (Author) 13 refs.

  5. Rational Design of Fluorescent Phthalazinone Derivatives for One- and Two-Photon Imaging.

    Science.gov (United States)

    Yang, Lingfei; Zhu, Yuanjun; Shui, Mengyang; Zhou, Tongliang; Cai, Yuanbo; Wang, Wei; Xu, Fengrong; Niu, Yan; Wang, Chao; Zhang, Jun-Long; Xu, Ping; Yuan, Lan; Liang, Lei

    2016-08-22

    Phthalazinone derivatives were designed as optical probes for one- and two-photon fluorescence microscopy imaging. The design strategy involves stepwise extension and modification of pyridazinone by 1) expansion of pyridazinone to phthalazinone, a larger conjugated system, as the electron acceptor, 2) coupling of electron-donating aromatic groups such as N,N-diethylaminophenyl, thienyl, naphthyl, and quinolyl to the phthalazinone, and 3) anchoring of an alkyl chain to the phthalazinone with various terminal substituents such as triphenylphosphonio, morpholino, triethylammonio, N-methylimidazolio, pyrrolidino, and piperidino. Theoretical calculations were utilized to verify the initial design. The desired fluorescent probes were synthesized by two different routes in considerable yields. Twenty-two phthalazinone derivatives were synthesized and their photophysical properties were measured. Selected compounds were applied in cell imaging, and valuable information was obtained. Furthermore, the designed compounds showed excellent performance in two-photon microscopic imaging of mouse brain slices.

  6. Time-dependent R-matrix theory applied to two-photon double ionization of He

    Science.gov (United States)

    van der Hart, H. W.

    2014-05-01

    We introduce a time-dependent R-matrix theory generalized to describe double-ionization processes. The method is used to investigate two-photon double ionization of He by intense XUV laser radiation. We combine a detailed B-spline-based wave-function description in an extended inner region with a single-electron outer region containing channels representing both single ionization and double ionization. A comparison of wave-function densities for different box sizes demonstrates that the flow between the two regions is described with excellent accuracy. The obtained two-photon double-ionization cross sections are in excellent agreement with other cross sections available. Compared to calculations fully contained within a finite inner region, the present calculations can be propagated over the time it takes the slowest electron to reach the boundary.

  7. Time-dependent R-matrix theory applied to two-photon double ionization of He

    CERN Document Server

    van der Hart, H W

    2014-01-01

    We introduce a time-dependent R-matrix theory generalised to describe double ionization processes. The method is used to investigate two-photon double ionization of He by intense XUV laser radiation. We combine a detailed B-spline-based wavefunction description in a extended inner region with a single-electron outer region containing channels representing both single ionization and double ionization. A comparison of wavefunction densities for different box sizes demonstrates that the flow between the two regions is described with excellent accuracy. The obtained two-photon double ionization cross sections are in excellent agreement with other cross sections available. Compared to calculations fully contained within a finite inner region, the present calculations can be propagated over the time it takes the slowest electron to reach the boundary.

  8. Electron acceleration by Landau resonance with whistler mode wave packets

    Science.gov (United States)

    Gurnett, D. A.; Reinleitner, L. A.

    1983-01-01

    Recent observations of electrostatic waves associated with whistler mode chorus emissions provide evidence that electrons are being trapped by Landau resonance interactions with the chorus. In this paper, the trapping, acceleration and escape of electrons in Landau resonance with a whistler mode wave packet are discussed. It is shown that acceleration can occur by both inhomogeneous and dispersive effects. The maximum energy gained is controlled by the points where trapping and escape occur. Large energy changes are possible if the frequency of the wave packet or the magnetic field strength increase between the trapping and escape points. Various trapping and escape mechanisms are discussed.

  9. Electron spin resonance detected by a superconducting qubit

    CERN Document Server

    Kubo, Y; Grezes, C; Umeda, T; Isoya, J; Sumiya, H; Yamamoto, T; Abe, H; Onoda, S; Ohshima, T; Jacques, V; Dréau, A; Roch, J -F; Auffeves, A; Vion, D; Esteve, D; Bertet, P

    2012-01-01

    A new method for detecting the magnetic resonance of electronic spins at low temperature is demonstrated. It consists in measuring the signal emitted by the spins with a superconducting qubit that acts as a single-microwave-photon detector, resulting in an enhanced sensitivity. We implement this new type of electron-spin resonance spectroscopy using a hybrid quantum circuit in which a transmon qubit is coupled to a spin ensemble consisting of NV centers in diamond. With this setup we measure the NV center absorption spectrum at 30mK at an excitation level of \\thicksim15\\,\\mu_{B} out of an ensemble of 10^{11} spins.

  10. Nonlinear quantitative photoacoustic tomography with two-photon absorption

    CERN Document Server

    Ren, Kui

    2016-01-01

    Two-photon photoacoustic tomography (TP-PAT) is a non-invasive optical molecular imaging modality that aims at inferring two-photon absorption property of heterogeneous media from photoacoustic measurements. In this work, we analyze an inverse problem in quantitative TP-PAT where we intend to reconstruct optical coefficients in a semilinear elliptic PDE, the mathematical model for the propagation of near infra-red photons in tissue-like optical media with two-photon absorption, from the internal absorbed energy data. We derive uniqueness and stability results on the reconstructions of single and multiple optical coefficients, and present some numerical reconstruction results based on synthetic data to complement the theoretical analysis.

  11. Two-photon interference between disparate sources for quantum networking

    Science.gov (United States)

    McMillan, A. R.; Labonté, L.; Clark, A. S.; Bell, B.; Alibart, O.; Martin, A.; Wadsworth, W. J.; Tanzilli, S.; Rarity, J. G.

    2013-06-01

    Quantum networks involve entanglement sharing between multiple users. Ideally, any two users would be able to connect regardless of the type of photon source they employ, provided they fulfill the requirements for two-photon interference. From a theoretical perspective, photons coming from different origins can interfere with a perfect visibility, provided they are made indistinguishable in all degrees of freedom. Previous experimental demonstrations of such a scenario have been limited to photon wavelengths below 900 nm, unsuitable for long distance communication, and suffered from low interference visibility. We report two-photon interference using two disparate heralded single photon sources, which involve different nonlinear effects, operating in the telecom wavelength range. The measured visibility of the two-photon interference is 80 +/- 4%, which paves the way to hybrid universal quantum networks.

  12. Enhanced two-photon absorption using true thermal light

    CERN Document Server

    Jechow, Andreas; Kurzke, Henning; Heuer, Axel; Menzel, Ralf

    2013-01-01

    Two-photon excited fluorescence (TPEF) is a standard technique in modern microscopy but still affected by photo-damage of the probe. It was proposed that TPEF can be enhanced by using entangled photons, but has proven to be challenging. Recently it was shown that some features of entangled photons can be mimicked with thermal light, which finds application in ghost imaging, sub-wavelength lithography and metrology. Here, we utilize true thermal light from a super-luminescence diode to demonstrate enhanced TPEF compared to coherent light using two common fluorophores and luminescent quantum dots. We find that the two-photon absorption rate is directly proportional to the measured degree of second-order coherence, as predicted by theory. Our results show that photon bunching can be exploited in two-photon microscopy with the photon statistic providing a new degree of freedom.

  13. Field structure and electron life times in the MEFISTO electron cyclotron resonance ion source

    Energy Technology Data Exchange (ETDEWEB)

    Bodendorfer, M. [EPFL - Ecole Polytechnique Federale de Lausanne (Switzerland); University of Berne, Institute of Physics, Space Research and Planetary Sciences, Siedlerstrasse 5, 3012 Berne (Switzerland)], E-mail: michael.bodendorfer@space.unibe.ch; Altwegg, K. [University of Berne, Institute of Physics, Space Research and Planetary Sciences, Siedlerstrasse 5, 3012 Berne (Switzerland); Shea, H. [EPFL - Ecole Polytechnique Federale de Lausanne (Switzerland); Wurz, P. [University of Berne, Institute of Physics, Space Research and Planetary Sciences, Siedlerstrasse 5, 3012 Berne (Switzerland)

    2008-03-15

    The complex magnetic field of the permanent magnet electron cyclotron resonance (ECR) ion source MEFISTO located at the University of Berne has been numerically simulated. For the first time the magnetized volume qualified for electron cyclotron resonance at 2.45 GHz and 87.5 mT has been analyzed in highly detailed 3D simulations with unprecedented resolution. New results were obtained from the numerical simulation of 25,211 electron trajectories. The evident characteristic ion sputtering trident of hexapole confined ECR ion sources has been identified with the field and electron trajectory distribution. Furthermore, unexpected long electron trajectory lifetimes were found.

  14. Field structure and electron life times in the MEFISTO electron cyclotron resonance ion source

    Science.gov (United States)

    Bodendorfer, M.; Altwegg, K.; Shea, H.; Wurz, P.

    2008-03-01

    The complex magnetic field of the permanent magnet electron cyclotron resonance (ECR) ion source MEFISTO located at the University of Berne has been numerically simulated. For the first time the magnetized volume qualified for electron cyclotron resonance at 2.45 GHz and 87.5 mT has been analyzed in highly detailed 3D simulations with unprecedented resolution. New results were obtained from the numerical simulation of 25,211 electron trajectories. The evident characteristic ion sputtering trident of hexapole confined ECR ion sources has been identified with the field and electron trajectory distribution. Furthermore, unexpected long electron trajectory lifetimes were found.

  15. Field structure and electron life times in the MEFISTO Electron Cyclotron Resonance Ion Source

    CERN Document Server

    Bodendorfer, Michael; Shea, Herbert; Wurz, Peter

    2008-01-01

    The complex magnetic field of the permanent-magnet electron cyclotron resonance (ECR) ion source MEFISTO located at the University of Bern have been numerically simulated. For the first time the magnetized volume qualified for electron cyclotron resonance at 2.45 GHz and 87.5 mT has been analyzed in highly detailed 3D simulations with unprecedented resolution. New results were obtained from the numerical simulation of 25211 electron trajectories. The evident characteristic ion sputtering trident of hexapole confined ECR sources has been identified with the field and electron trajectory distribution. Furthermore, unexpected long electron trajectory lifetimes were found.

  16. Sensing for intracellular thiols by water-insoluble two-photon fluorescent probe incorporating nanogel

    Energy Technology Data Exchange (ETDEWEB)

    Guo, Xudong; Zhang, Xin; Wang, Shuangqing; Li, Shayu [Beijing National Laboratory for Molecular Sciences, Key laboratory of Photochemistry, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190 (China); Hu, Rui, E-mail: hurui@iccas.ac.cn [Beijing National Laboratory for Molecular Sciences, Key laboratory of Photochemistry, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190 (China); Li, Yi, E-mail: yili@mail.ipc.ac.cn [Key Laboratory of Photochemical Conversion and Optoelectronic Materials, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing 100190 (China); Yang, Guoqiang, E-mail: gqyang@iccas.ac.cn [Beijing National Laboratory for Molecular Sciences, Key laboratory of Photochemistry, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190 (China)

    2015-04-15

    Highlights: • A novel “turn-on” two-photon fluorescent probe based on a π-conjugated triarylboron luminogen was designed and synthesized. • Fast, selective and sensitive detection of biothiols in 100% aqueous solution by simply loaded on a nanogel. • Single-photon and two-photon fluorescent bioimaging of biothiols in NIH/3T3 fibroblasts. - Abstract: A novel “turn-on” two-photon fluorescent probe containing a π-conjugated triarylboron luminogen and a maleimide moiety DMDP-M based on the photo-induced electron transfer (PET) mechanism for biothiol detection was designed and synthesized. By simply loading the hydrophobic DMDP-M on a cross-linked Pluronic{sup ®} F127 nanogel (CL-F127), a probing system DMDP-M/CL-F127 was established, which shows quick response, high selectivity and sensitivity to cysteine (Cys), homocysteine (Hcy) and glutathione (GSH) in aqueous phase. The DMDP-M/CL-F127 system presented the fastest response to Cys with a rate constant of 0.56 min{sup −1}, and the detection limit to Cys was calculated to be as low as 0.18 μM. The DMDP-M/CL-F127 system has been successfully applied to the fluorescence imaging of biothiols in NIH/3T3 fibroblasts either with single-photon or two-photon excitation because of its high biocompatibility and cell-membrane permeability. The present work provides a general, simple and efficient strategy for the application of hydrophobic molecules to sensing biothiols in aqueous phase, and a novel sensing system for intracellular biothiols fitted for both single-photon and two-photon fluorescence imaging.

  17. Measuring Traces Of Oxygen By Resonant Electron Attachment

    Science.gov (United States)

    Man, Kin Fung; Boumsellek, Said; Chutjian, Ara

    1995-01-01

    Method of detecting trace amounts of oxygen based on dissociative attachment of electrons to oxygen molecules followed by measurement of resulting flux of negative oxygen ions in mass spectrometer. High sensitivity achieved in method by exploiting resonance in dissociative attachment of electrons to oxygen molecules: electron-attachment cross section rises to high peak at incident electron kinetic energy of 6.2 eV. Relative concentrations below 1 ppb detected. Devised to increase sensitivity of detection of oxygen in processing chambers in which oxygen regarded as contaminant; for example, chambers used in making semiconductor devices and in growing high-purity crystals.

  18. Two-photon interference with non-identical photons

    Science.gov (United States)

    Liu, Jianbin; Zhou, Yu; Zheng, Huaibin; Chen, Hui; Li, Fu-li; Xu, Zhuo

    2015-11-01

    Two-photon interference with non-identical photons is studied based on the superposition principle in Feynman's path integral theory. The second-order temporal interference pattern is observed by superposing laser and pseudothermal light beams with different spectra. The reason why there is two-photon interference for photons of different spectra is that non-identical photons can be indistinguishable for the detection system when Heisenberg's uncertainty principle is taken into account. These studies are helpful to understand the second-order interference of light in the language of photons.

  19. Two-Photon Total Annihilation of Molecular Positronium

    CERN Document Server

    Pérez-Ríos, Jesús; Greene, Chris H

    2014-01-01

    The rate for complete two-photon annihilation of molecular positronium Ps$_{2}$ is reported. This decay channel involves a four-body collision among the fermions forming Ps$_{2}$, and two photons of 1.022 MeV, each, as the final state. The quantum electrodynamics result for the rate of this process is found to be $\\Gamma_{Ps_{2} \\rightarrow \\gamma\\gamma}$ = 9.0 $\\times 10^{-12}$ s$^{-1}$. This decay channel completes the most comprehensive decay chart for Ps$_{2}$ up to date.

  20. Two-photon Compton process in pulsed intense laser fields

    CERN Document Server

    Seipt, D

    2012-01-01

    Based on strong-field QED in the Furry picture we use the Dirac-Volkov propagator to derive a compact expression for the differential emission probability of the two-photon Compton process in a pulsed intense laser field. The relation of real and virtual intermediate states is discussed, and the natural regularization of the on-shell contributions due to the finite laser pulse is highlighted. The inclusive two-photon spectrum is two orders of magnitude stronger than expected from a perturbative estimate.

  1. Precision two-photon spectroscopy of alkali elements

    Indian Academy of Sciences (India)

    P V Kiran Kumar; M V Suryanarayana

    2014-08-01

    In this paper, we have briefly reviewed the work on two-photon spectroscopy of alkali elements and its applications. The technique of Doppler-free two-photon spectroscopy is briefly summarized. A review of various techniques adopted for measuring absolute frequencies of the atomic transitions and precision measurements of isotope shifts and hyperfine structures (HFS) is presented. Some of the recent works on precision measurements of HFS constants of 6 ${}^2S_{1/2}$ level of ${}^{39}$K and ${}^{41}$K, 9 ${}^2S_{1/2}$ level and 7 ${}^2D_{3/2}$ level of 133Cs are also discussed.

  2. A fluorescent benzothiazole probe with efficient two-photon absorption

    Science.gov (United States)

    Echevarria, Lorenzo; Moreno, Iván; Camacho, José; Salazar, Mary Carmen; Hernández, Antonio

    2012-11-01

    In this work, we report the two-photon absorption of 2-[4-(dimethylamino)phenyl]-1,3-benzothiazole-6-carbonitrile (DBC) in DMSO solution pumping at 779 nm with a 10 ns pulse laser-Nd:YAG system. The obtained two-photon absorption cross-section in DBC (407 ± 18 GM) is considerably high. Because DBC is a novel compound and have high values of fluorescence quantum yield, this result is expected to have an impact in biomolecules detection, diagnosis and treatment of cancer. Similar structures have previously been reported to show remarkable antitumour effects.

  3. Electron paramagnetic resonance of material properties and processes

    Energy Technology Data Exchange (ETDEWEB)

    Brower, K. L.

    1980-01-01

    This paper demonstrates, primarily for the non-specialist and within the context of new and recent achievements, the diagnostic value of electron paramagnetic resonance (EPR) in the study of material properties and processes. I have selected three EPR studies which demonstrate the elegance and uniqueness of EPR in atomic defect studies and exemplify unusual achievements through the use of new techniques for material measurement and preparation. A brief introduction into the origin, interaction, and detection of unpaired electrons is included.

  4. Introduction to Spin Label Electron Paramagnetic Resonance Spectroscopy of Proteins

    Science.gov (United States)

    Melanson, Michelle; Sood, Abha; Torok, Fanni; Torok, Marianna

    2013-01-01

    An undergraduate laboratory exercise is described to demonstrate the biochemical applications of electron paramagnetic resonance (EPR) spectroscopy. The beta93 cysteine residue of hemoglobin is labeled by the covalent binding of 3-maleimido-proxyl (5-MSL) and 2,2,5,5-tetramethyl-1-oxyl-3-methyl methanethiosulfonate (MTSL), respectively. The excess…

  5. Electron beam imaging and spectroscopy of plasmonic nanoantenna resonances

    NARCIS (Netherlands)

    Vesseur, P.C.

    2011-01-01

    Nanoantennas are metal structures that provide strong optical coupling between a nanoscale volume and the far field. This coupling is mediated by surface plasmons, oscillations of the free electrons in the metal. Increasing the control over the resonant plasmonic field distribution opens up a wide r

  6. Introduction to Spin Label Electron Paramagnetic Resonance Spectroscopy of Proteins

    Science.gov (United States)

    Melanson, Michelle; Sood, Abha; Torok, Fanni; Torok, Marianna

    2013-01-01

    An undergraduate laboratory exercise is described to demonstrate the biochemical applications of electron paramagnetic resonance (EPR) spectroscopy. The beta93 cysteine residue of hemoglobin is labeled by the covalent binding of 3-maleimido-proxyl (5-MSL) and 2,2,5,5-tetramethyl-1-oxyl-3-methyl methanethiosulfonate (MTSL), respectively. The excess…

  7. Asymmetric Wave Transmission During Electron-Cyclotron Resonant Heating

    NARCIS (Netherlands)

    Peeters, A.G.; Smits, F. M. A.; Giruzzi, G.; Oomens, A. A. M.; Westerhof, E.

    1995-01-01

    In low density plasmas in the RTP tokamak the single-pass absorption of O-mode waves at the fundamental electron cyclotron resonance is observed to be toroidally asymmetric. The absorption is highest for waves travelling in the direction opposite to the toroidal plasma current. Fokker-Planck

  8. Resonator design for a visible wavelength free-electron laser (*)

    Energy Technology Data Exchange (ETDEWEB)

    Bhowmik, A.; Lordi, N. (Rockwell International Corp., Canoga Park, CA (United States). Rocketdyne Div.); Ben-Zvi, I.; Gallardo, J. (Brookhaven National Lab., Upton, NY (United States))

    1990-01-01

    Design requirements for a visible wavelength free-electron laser being developed at the Accelerator Test Facility at Brookhaven National Laboratory are presented along with predictions of laser performance from 3-D numerical simulations. The design and construction of the optical resonator, its alignment and control systems are also described. 15 refs., 8 figs., 4 tabs.

  9. Phonon-Assisted Two-Photon Interference from Remote Quantum Emitters.

    Science.gov (United States)

    Reindl, Marcus; Jöns, Klaus D; Huber, Daniel; Schimpf, Christian; Huo, Yongheng; Zwiller, Val; Rastelli, Armando; Trotta, Rinaldo

    2017-07-12

    Photonic quantum technologies are on the verge of finding applications in everyday life with quantum cryptography and quantum simulators on the horizon. Extensive research has been carried out to identify suitable quantum emitters and single epitaxial quantum dots have emerged as near-optimal sources of bright, on-demand, highly indistinguishable single photons and entangled photon-pairs. In order to build up quantum networks, it is essential to interface remote quantum emitters. However, this is still an outstanding challenge, as the quantum states of dissimilar "artificial atoms" have to be prepared on-demand with high fidelity and the generated photons have to be made indistinguishable in all possible degrees of freedom. Here, we overcome this major obstacle and show an unprecedented two-photon interference (visibility of 51 ± 5%) from remote strain-tunable GaAs quantum dots emitting on-demand photon-pairs. We achieve this result by exploiting for the first time the full potential of a novel phonon-assisted two-photon excitation scheme, which allows for the generation of highly indistinguishable (visibility of 71 ± 9%) entangled photon-pairs (fidelity of 90 ± 2%), enables push-button biexciton state preparation (fidelity of 80 ± 2%) and outperforms conventional resonant two-photon excitation schemes in terms of robustness against environmental decoherence. Our results mark an important milestone for the practical realization of quantum repeaters and complex multiphoton entanglement experiments involving dissimilar artificial atoms.

  10. Internal conversions in Higgs decays to two photons

    OpenAIRE

    Firan, Ana; Stroynowski, Ryszard

    2007-01-01

    We evaluate the partial widths for internal conversions in the Higgs decays to two photons. For the Higgs masses of interest at LHC in the range of 100-150 GeV, the conversions to pairs of fermions represent significant fraction of Higgs decays.

  11. Two-photon absorbing porphyrins for oxygen microscopy (Conference Presentation)

    Science.gov (United States)

    Esipova, Tatiana V.; Vinogradov, Sergei A.

    2016-03-01

    The ability to quantify oxygen in vivo in 3D with high spatial and temporal resolution is invaluable for many areas of the biomedical science, including ophthalmology, neuroscience, cancer and stem biology. An optical method based on oxygen-dependent quenching of phosphorescence is being developed, that allows quantitative minimally invasive real-time imaging of partial pressure of oxygen (pO2) in tissue. In the past, dendritically protected phosphorescent oxygen probes with controllable quenching parameters and defined bio-distributions have been developed. More recently our probe strategy has extended to encompass two-photon excitable oxygen probes, which brought about first demonstrations of two-photon phosphorescence lifetime microscopy (2PLM) of oxygen in vivo, providing new valuable information for neuroscience and stem cell biology. However, current two-photon oxygen probes suffer from a number of limitations, such as low brightness and high cost of synthesis, which dramatically reduce imaging performance and limit usability of the method. Here we present an approach to new bright phosphorescent chromophores with internally enhanced two-photon absorption cross-sections, which pave a way to novel proves for 2PLM. In addition to substantial increase in performance, the new probes can be synthesized by much more efficient methods, thereby greatly reducing the cost of the synthesis and making the technique accessible to a broader range of researchers across different fields.

  12. Direct Writing of Photonic Structures by Two-Photon Polymerization

    Directory of Open Access Journals (Sweden)

    Li Yan

    2013-11-01

    Full Text Available Single-mode dielectric-loaded surface plasmon-polariton nanowaveguides with strong mode confinement at excitation wavelength of 830 nm and high-Q polymer whispering gallery mode microcavities with surface roughness less than 12 nm have been directly written by two-photon polymerization, which pave the way to fabricate 3D plasmonic photonic structures by direct laser writing.

  13. Morphology dependent two photon absorption in plasmonic structures and plasmonic-organic hybrids

    Science.gov (United States)

    Gambhir, Kaweri; Ray, Bhumika; Mehrotra, Ranjana; Sharma, Parag

    2017-05-01

    Two photon absorption coefficients of two distinct plasmonic structures, namely, gold nanoflowers (GNF) and gold nanopebbles (GNP) have been investigated and compared with conventional gold nanospheres (GNS). All three different nanoshapes were synthesized by changing the reaction solvent under the same experimental procedure. Further, hybrids of these plasmonic structures were prepared with an organic dye Eosin yellow (EY), to investigate the morphology effect of plasmonic structures on plasmonic-organic hybrids in terms of their linear extinction spectra and two photon absorption coefficients. The NLO investigations were conducted using 20 ps laser pulses of wavelength 532 nm as an excitation source in single beam Z-scan setup. UV/visible spectroscopy was employed for monitoring plasmon resonances and changes in linear extinction spectra. The experimental outcomes revealed two photon absorption coefficients of EY increased 120%, 32% and 39%, while 69%, 60% and 53% enhancement in the peaks of linear extinction maxima of EY has been observed, when hybridized with GNF, GNS and GNP, respectively. This boost in the optical coefficients may be attributed to dimerization of EY molecules on the surface of nanoparticles. Keeping the toxicity of EY in view, we propose that the two photon absorption coefficients of this dye and control thereof, by the addition of plasmonic structures would be helpful not only in understanding the interactions between plasmons and fluorophore, but also pave an efficient way, to reduce the operative concentration of this hazardous dye in a wide range of applications and thereby, mitigating the environmental degradation caused by its highly concentrated effluents.

  14. Electron Plasmas Cooled by Cyclotron-Cavity Resonance

    CERN Document Server

    Povilus, A P; Evans, L T; Evetts, N; Fajans, J; Hardy, W N; Hunter, E D; Martens, I; Robicheaux, F; Shanman, S; So, C; Wang, X; Wurtele, J S

    2016-01-01

    We observe that high-Q electromagnetic cavity resonances increase the cyclotron cooling rate of pure electron plasmas held in a Penning-Malmberg trap when the electron cyclotron frequency, controlled by tuning the magnetic field, matches the frequency of standing wave modes in the cavity. For certain modes and trapping configurations, this can increase the cooling rate by factors of ten or more. In this paper, we investigate the variation of the cooling rate and equilibrium plasma temperatures over a wide range of parameters, including the plasma density, plasma position, electron number, and magnetic field.

  15. Conjugated polymers with pyrrole as the conjugated bridge: synthesis, characterization, and two-photon absorption properties.

    Science.gov (United States)

    Li, Qianqian; Zhong, Cheng; Huang, Jing; Huang, Zhenli; Pei, Zhiguo; Liu, Jun; Qin, Jingui; Li, Zhen

    2011-07-14

    The synthesis, one- and two-photon absorption (2PA) and emission properties of two novel pyrrole-based conjugated polymers (P1 and P2) are reported. They emitted strong yellow-green and orange fluorescence with fluorescent quantum yields (Φ) of 46 and 33%, respectively. Their maximal 2PA cross sections (δ) measured by the two-photon-induced fluorescence method using femtosecond laser pulses in THF were 2392 and 1938 GM per repeating unit, respectively, indicating that the 2PA chromophores consisting of the triphenylamine with nonplanar structure as the donor and electron-rich pyrrole as the conjugated bridge could be the effective repeating units to enhance the δ values.

  16. A superradiant laser based on two-photon Raman transition of caesium atoms

    CERN Document Server

    Liu, Pengfei

    2013-01-01

    We propose a superradiant laser based on two-photon Raman transition of caesium-133 atoms which collectively emit photons on an ultra narrow transition into the mode of a low Q resonator known as optical bad-cavity regime. The spin-spin correlation which characterizes the collective effect is demonstrated. We theoretically predict that the optical radiation has an extremely narrow linewidth in the 98 (1) *10-2 mHz range, smaller than the transition itself due to collective effects, and a power level of 7 (1)*10-10 W is possible, which can provide a possible new way to realize an optical clock with a millihertz linewidth.

  17. Tunable two-photon correlation in a double-cavity optomechanical system

    Directory of Open Access Journals (Sweden)

    Zhi-Bo Feng

    2015-12-01

    Full Text Available Correlated photons are essential sources for quantum information processing. We propose a practical scheme to generate pairs of correlated photons in a controllable fashion from a double-cavity optomechanical system, where the variable optomechanical coupling strength makes it possible to tune the photon correlation at our will. The key operation is based on the repulsive or attractive interaction between the two photons intermediated by the mechanical resonator. The present protocol could provide a potential approach to coherent control of the photon correlation using the optomechanical cavity.

  18. Two-Photon Jaynes-Cummings Model Governed by Milburn Equation with Phase Damping

    Institute of Scientific and Technical Information of China (English)

    2006-01-01

    In this paper, we find an analytic solution of the master equation of a non-resonant two-photon JaynesCummings model (JCM) with phase damping with the help of the super-operator technique. We study the influence of phase damping on non-classical effects in the JCM, such as oscillations of the photon-number distribution, revivals of the atomic inversion, and sub-Possion photon statistics. It is demonstrated that the phase damping suppresses the revivals of the atomic inversion and non-classical effects of the cavity field in the JCM.

  19. Two Photon Exchange in Impact Parameter Space in the Relativistic Eikonal Approximation for Elastic e - N Scattering

    CERN Document Server

    Alhalholy, Tareq

    2016-01-01

    Using the relativistic Eikonal approximation, we study the one and two photon exchange amplitudes in elastic electron-nucleon scattering for the case of transversely polarized nucleons with unpolarized electrons beam. In our approach, we utilize the convolution theory of Fourier transforms and the transverse charge density in transverse momentum space to evaluate the one and two photon exchange Eikonal amplitudes. The results obtained for the $2\\gamma$ amplitude in impact parameter space are compared to the corresponding 4D case. We show that while the one and two photon cross sections are azimuthally symmetric, the interference term between them is azimuthally asymmetric, which is an indication of an azimuthal single spin asymmetry for proton and neutron which can be attributed to the fact that the nucleon charge density is transversely (azimuthally) distorted in the transverse plane for transversely polarized nucleons. In addition, the calculations of the interference term for proton and neutron show agreem...

  20. Coherent blue emission generated by Rb two-photon excitation using diode and femtosecond lasers

    Science.gov (United States)

    Lopez, Jesus P.; Moreno, Marco P.; de Miranda, Marcio H. G.; Vianna, Sandra S.

    2017-04-01

    The coherent blue light generated in rubidium vapor due to the combined action of an ultrashort pulse train and a continuous wave diode laser is investigated. Each step of the two-photon transition 5S-5P{}3/2-5D is excited by one of the lasers, and the induced coherence between the 5S and 6P{}3/2 states is responsible for generating the blue beam. Measurements of the excitation spectrum reveal the frequency comb structure and allow us to identify the resonant modes responsible for inducing the nonlinear process. Further, each resonant mode excites a different group of atoms, making the process selective in atomic velocity. The signal dependency on the atomic density is characterized by a sharp growth and a rapid saturation. We also show that for high intensity of the diode laser, the Stark shift at resonance causes the signal suppression observed at low atomic density.

  1. Quantum resonances in reflection of relativistic electrons and positrons

    Energy Technology Data Exchange (ETDEWEB)

    Eykhorn, Yu.L.; Korotchenko, K.B. [National Research Tomsk Polytechnic University, 30, Lenin Avenue, Tomsk 634050 (Russian Federation); Pivovarov, Yu.L. [National Research Tomsk Polytechnic University, 30, Lenin Avenue, Tomsk 634050 (Russian Federation); Tomsk State University, 36, Lenin Avenue, Tomsk 634050 (Russian Federation); Takabayashi, Y. [SAGA Light Source, 8-7 Yayoigaoka, Tosu, Saga 841-0005 (Japan)

    2015-07-15

    Calculations based on the use of realistic potential of the system of crystallographic planes confirm earlier results on existence of resonances in reflection of relativistic electrons and positrons by the crystal surface, if the crystallographic planes are parallel to the surface.The physical reason of predicted phenomena, similar to the band structure of transverse energy levels, is connected with the Bloch form of the wave functions of electrons (positrons) near the crystallographic planes, which appears both in the case of planar channeling of relativistic electrons (positrons) and in reflection by a crystal surface. Calculations show that positions of maxima in reflection of relativistic electrons and positrons by crystal surface specifically depend on the angle of incidence with respect to the crystal surface and relativistic factor of electrons/positrons. These maxima form the Darwin tables similar to that in ultra-cold neutron diffraction.

  2. Suppression of electron spin-echo envelope modulation peaks in double quantum coherence electron spin resonance.

    Science.gov (United States)

    Bonora, Marco; Becker, James; Saxena, Sunil

    2004-10-01

    We show the use of the observer blind spots effect for the elimination of electron spin-echo envelope modulation (ESEEM) peaks in double quantum coherence (DQC) electron spin resonance (ESR). The suppression of ESEEM facilitates the routine and unambiguous extraction of distances from DQC-ESR spectra. This is also the first demonstration of this challenging methodology on commercial instrumentation.

  3. Search for Anomalous Production of Events with Two Photons and Additional Energetic Objects at CDF

    Energy Technology Data Exchange (ETDEWEB)

    Aaltonen, T.; /Helsinki Inst. of Phys.; Adelman, J.; /Chicago U., EFI; Alvarez Gonzalez, B.; /Oviedo U. /Cantabria Inst. of Phys.; Amerio, S.; /Padua U. /INFN, Padua; Amidei, D.; /Michigan U.; Anastassov, A.; /Northwestern U.; Annovi, A.; /Frascati; Antos, J.; /Comenius U. /Kosice, IEF; Apollinari, G.; /Fermilab; Apresyan, A.; /Purdue U.; Arisawa, T.; /Waseda U. /Dubna, JINR

    2009-10-01

    The authors present results of a search for anomalous production of two photons together with an electron, muon, {tau} lepton, missing transverse energy, or jets using p{bar p} collision data from 1.1-2.0 fb{sup -1} of integrated luminosity collected by the Collider Detector at Fermilab (CDF). The event yields and kinematic distributions are examined for signs for new physics without favoring a specific model of new physics. The results are consistent with the standard model expectations. The search employs several new analysis techniques that significantly reduce instrumental backgrounds in channels with an electron and missing transverse energy.

  4. Observation of excess $\\lambda\\overline{\\lambda}$ production in two-photon processes at TRISTAN

    CERN Document Server

    Enomoto, R; Abe, T; Adachi, I; Adachi, K; Aoki, M; Awa, S; Emi, K; Fujii, H; Fujii, K; Fujii, T; Fujimoto, J; Fujita, K; Fujiwara, N; Hayashii, H; Howell, B; Iida, N; Itoh, R; Inoue, Y; Iwasaki, H; Iwasaki, M; Kaneyuki, K; Kajikawa, R; Kato, S; Kawabata, S; Kichimi, H; Kobayashi, M; Koltick, D S; Levine, I; Minami, S; Miyabayashi, K; Miyamoto, A; Muramatsu, K; Nagai, K; Nakabayashi, K; Nakano, E; Nitoh, O; Noguchi, S; Ochi, A; Ochiai, F; Ohishi, N; Ohnishi, Y; Ohshima, Y; Okuno, H; Okusawa, T; Shinohara, T; Sugiyama, A; Suzuki, S; Takahashi, K; Takahashi, T; Tanimori, T; Tauchi, T; Teramoto, Y; Toomi, N; Tsukamoto, T; Tsumura, O; Uno, S; Watanabe, T; Watanabe, Y; Yamaguchi, A; Yamamoto, A; Yamauchi, M; Enomoto, R

    1995-01-01

    We have carried out inclusive measurements of \\Lambda(\\overline{\\Lamb da}) production in two-photon processes at TRISTAN. The mean \\sqrt{s} was 58 GeV and the integrated luminosity was 265 pb^{-1}. Inclusive \\Lambda (\\overline{\\Lambda}) samples were obtained under such conditions as no-electron, anti-electron, and remnant-jet tags. The data were compared with theoretical calculations. The measured cross sections are two-times larger than the leading-order theoretical predictions, suggesting the necessity of next-to-leading-order Monte-Carlo generator.

  5. Two-photon Photo-emission of Ultrathin Film PTCDA Morphologies on Ag(111)

    Energy Technology Data Exchange (ETDEWEB)

    Yang, Aram; Yang, Aram; Shipman, Steven T.; Garrett-Roe, Sean; Johns, James; Strader, Matt; Szymanski, Paul; Muller, Eric; Harris, Charles B.

    2007-11-29

    Morphology- and layer-dependent electronic structure and dynamics at the PTCDA/Ag(111) interface have been studied with angle-resolved two-photon photoemission. In Stranski-Krastanov growth modes, the exposed wetting layer inhibited the evolution of the vacuum level and valence band to bulk values. For layer-by-layer growth, we observed the transition of electron structure from monolayer to bulk values within eight monolayers. Effective masses and lifetimes of the conduction band and the n=1 image potential state were measured to be larger for disordered layers. The effective mass was interpreted in the context of charge mobility measurements.

  6. Two-photon absorption of Zn(II) octupolar molecules.

    Science.gov (United States)

    Mazzucato, Simone; Fortunati, Ilaria; Scolaro, Sara; Zerbetto, Michele; Ferrante, Camilla; Signorini, Raffaella; Pedron, Danilo; Bozio, Renato; Locatelli, Danika; Righetto, Stefania; Roberto, Dominique; Ugo, Renato; Abbotto, Alessandro; Archetti, Graziano; Beverina, Luca; Ghezzi, Sergio

    2007-06-21

    In this work we present an investigation of the non-linear optical (NLO) properties of two octupolar chromophores: [Zn(4,4'-bis(dibutylaminostyryl)-[2,2']-bipyridine)(3)](2+) and [Zn(4,4'-bis((E)-2-(N-(TEG)pyrrol-2-yl)vinyl)-[2,2']-bipyridine)(3)](2+) with Zn(ii) as the coordination center, using two-photon emission technique (TPE) in fs-pulse temporal regime. Compared to the free ligands, our results do not show a net increase in the two-photon absorption (TPA) cross-section for the octupolar complexes, once normalized to the ligand unit. This is in partial disagreement with a previous theoretical study investigating the first molecule where a significant increase of the TPA cross-section was predicted (X. J. Liu, et al., J. Chem. Phys., 2004, 120, 11 493).

  7. Synthesizing arbitrary two-photon polarization mixed states

    CERN Document Server

    Wei, T C; Branning, D; Goldbart, P M; James, D F V; Jeffrey, E; Kwiat, P G; Mukhopadhyay, S; Peters, N A; Wei, Tzu-Chieh; Altepeter, Joseph B.; Branning, David; Goldbart, Paul M.; Jeffrey, Evan; Kwiat, Paul G.; Mukhopadhyay, Swagatam; Peters, Nicholas A.

    2005-01-01

    Two methods for creating arbitrary two-photon polarization pure states are introduced. Based on these, four schemes for creating two-photon polarization mixed states are proposed and analyzed. The first two schemes can synthesize completely arbitrary two-qubit mixed states, i.e., control all 15 free parameters: Scheme I requires several sets of crystals, while Scheme II requires only a single set, but relies on decohering the pump beam. Additionally, we describe two further schemes which are much easier to implement. Although the total capability of these is still being studied, we show that they can synthesize all two-qubit Werner states, maximally entangled mixed states, Collins-Gisin states, and arbitrary Bell-diagonal states.

  8. High-order dispersion effects in two-photon interference

    CERN Document Server

    Mazzotta, Z; Cipriani, D; Olivares, S; Paris, M G A

    2016-01-01

    Two-photon interference and Hong-Ou-Mandel (HOM) effect are relevant tools for quantum metrology and quantum information processing. In optical coherence tomography, HOM effect is exploited to achieve high-resolution measurements with the width of the HOM dip being the main parameter. On the other hand, applications like dense coding require high-visibility performances. Here we address high-order dispersion effects in two-photon interference and study, theoretically and experimentally, the dependence of the visibility and the width of the HOM dip on both the pump spectrum and the downconverted photon spectrum. In particular, a spatial light modulator is exploited to experimentally introduce and manipulate a custom phase function to simulate the high-order dispersion effects.

  9. Two-photon interference from two blinking quantum emitters

    Science.gov (United States)

    Jöns, Klaus D.; Stensson, Katarina; Reindl, Marcus; Swillo, Marcin; Huo, Yongheng; Zwiller, Val; Rastelli, Armando; Trotta, Rinaldo; Björk, Gunnar

    2017-08-01

    We investigate the effect of blinking on the two-photon interference measurement from two independent quantum emitters. We find that blinking significantly alters the statistics in the Hong-Ou-Mandel second-order intensity correlation function g(2 )(τ ) and the outcome of two-photon interference measurements performed with independent quantum emitters. We theoretically demonstrate that the presence of blinking can be experimentally recognized by a deviation from the gD(2 )(0 ) =0.5 value when distinguishable photons from two emitters impinge on a beam splitter. Our findings explain the significant differences between linear losses and blinking for correlation measurements between independent sources and are experimentally verified using a parametric down-conversion photon-pair source. We show that blinking imposes a mandatory cross-check measurement to correctly estimate the degree of indistinguishability of photons emitted by independent quantum emitters.

  10. Two-photon microscopy using fiber-based nanosecond excitation.

    Science.gov (United States)

    Karpf, Sebastian; Eibl, Matthias; Sauer, Benjamin; Reinholz, Fred; Hüttmann, Gereon; Huber, Robert

    2016-07-01

    Two-photon excitation fluorescence (TPEF) microscopy is a powerful technique for sensitive tissue imaging at depths of up to 1000 micrometers. However, due to the shallow penetration, for in vivo imaging of internal organs in patients beam delivery by an endoscope is crucial. Until today, this is hindered by linear and non-linear pulse broadening of the femtosecond pulses in the optical fibers of the endoscopes. Here we present an endoscope-ready, fiber-based TPEF microscope, using nanosecond pulses at low repetition rates instead of femtosecond pulses. These nanosecond pulses lack most of the problems connected with femtosecond pulses but are equally suited for TPEF imaging. We derive and demonstrate that at given cw-power the TPEF signal only depends on the duty cycle of the laser source. Due to the higher pulse energy at the same peak power we can also demonstrate single shot two-photon fluorescence lifetime measurements.

  11. Two-photon-induced cycloreversion reaction of chalcone photodimers

    Science.gov (United States)

    Träger, J.; Härtner, S.; Heinzer, J.; Kim, H.-C.; Hampp, N.

    2008-04-01

    The photocleavage reaction of chalcone photodimers has been studied using a two-photon process. For this purpose, a novel chalcone dimer has been synthesized as a low molecular weight model substance for polymer bound chalcones and its photochemistry triggered by two-photon-absorption (2PA) has been investigated using a pulsed frequency-doubled Nd:YAG-laser. The 2PA-induced cycloreversion reaction selectively leads to the cleavage of the chalcone photodimers resulting in the formation of monomeric chalcone molecules. Hence, as an application chalcones can be used as a photosensitive linker which can be cleaved beyond an UV-absorbing barrier. The 2PA cross section of the chalcone photodimer was determined to be of 1.1 × 10 -49 cm 4 s photon -1 (11 GM).

  12. Four-dimensional multi-site two-photon excitation

    CERN Document Server

    Daria, Vincent Ricardo; Bowman, Richard; Redman, Stephen; Bachor, Hans-A

    2009-01-01

    We report the first demonstration of dynamic and arbitrary multi-site two-photon excitation in three-dimensional (3D) space using the holographic projection method. Rapid temporal response (fourth dimension) is achieved through high-speed non-iterative and non-optimized calculation of the hologram using a video graphics accelerator board. We verify that the projected asymmetric spot configurations have sufficient spatiotemporal photon density for localized two-photon excitation. This system is a significant advance and ready for applications such as time-resolved 3D photolysis of complex biological cell and neuronal networks, 3D microscopy, non-linear micro-fabrication and volume holographic optical storage.

  13. Two-photon absorption in gapped bilayer graphene with a tunable chemical potential

    Science.gov (United States)

    Brinkley, M. K.; Abergel, D. S. L.; Clader, B. D.

    2016-09-01

    Despite the now vast body of two-dimensional materials under study, bilayer graphene remains unique in two ways: it hosts a simultaneously tunable band gap and electron density; and stems from simple fabrication methods. These two advantages underscore why bilayer graphene is critical as a material for optoelectronic applications. In the work that follows, we calculate the one- and two-photon absorption coefficients for degenerate interband absorption in a graphene bilayer hosting an asymmetry gap and adjustable chemical potential—all at finite temperature. Our analysis is comprehensive, characterizing one- and two-photon absorptive behavior over wide ranges of photon energy, gap, chemical potential, and thermal broadening. The two-photon absorption coefficient for bilayer graphene displays a rich structure as a function of photon energy and band gap due to the existence of multiple absorption pathways and the nontrivial dispersion of the low energy bands. This systematic work will prove integral to the design of bilayer-graphene-based nonlinear optical devices.

  14. Nonlinear processes upon two-photon interband picosecond excitation of PbWO4 crystal

    Science.gov (United States)

    Lukanin, V. I.; Karasik, A. Ya

    2016-09-01

    A new experimental method is proposed to study the dynamics of nonlinear processes occurring upon two-photon interband picosecond excitation of a lead tungstate crystal and upon its excitation by cw probe radiation in a temporal range from several nanoseconds to several seconds. The method is applied to the case of crystal excitation by a sequence of 25 high-power picosecond pulses with a wavelength of 523.5 nm and 633-nm cw probe radiation. Measuring the probe beam transmittance during crystal excitation, one can investigate the influence of two-photon interband absorption and the thermal nonlinearity of the refractive index on the dynamics of nonlinear processes in a wide range of times (from several nanoseconds to several seconds). The time resolution of the measuring system makes it possible to distinguish fast and slow nonlinear processes of electronic or thermal nature, including the generation of a thermal lens and thermal diffusion. An alternative method is proposed to study the dynamics of induced absorption transformation and, therefore, the dynamics of the development of nonlinear rocesses upon degenerate two-photon excitation of the crystal in the absence of external probe radiation.

  15. Enhanced two-photon emission in coupled metal nanoparticles induced by conjugated polymers.

    Science.gov (United States)

    Guan, Zhenping; Polavarapu, Lakshminarayana; Xu, Qing-Hua

    2010-12-01

    Interactions between noble metal (Ag and Au) nanoparticles and conjugated polymers as well as their one- and two-photon emission have been investigated. Ag and Au nanoparticles exhibited extraordinary quenching effects on the fluorescence of cationic poly(fluorinephenylene). The quenching efficiency by 37-nm Ag nanoparticles is ∼19 times more efficient than that by 13-nm Au nanoparticles, and 9-10 orders of magnitude more efficient than typical small molecule dye-quencher pairs. On the other hand, the cationic conjugated polymers induce the aggregate formation and plasmonic coupling of the metal nanoparticles, as evidenced by transmission electron microscopy images and appearance of a new longitudinal plasmon band in the near-infrared region. The two-photon emissions of Ag and Au nanoparticles were found to be significantly enhanced upon addition of conjugated polymers, by a factor of 51-times and 9-times compared to the isolated nanoparticles for Ag and Au, respectively. These studies could be further extended to the applications of two-photon imaging and sensing of the analytes that can induce formation of metal nanoparticle aggregates, which have many advantages over the conventional one-photon counterparts.

  16. Mechanism of spin diffusion in electron spin resonance spectra of trapped electrons in aqueous glasses. Electron--Electron double resonance studies. [. gamma. -rays

    Energy Technology Data Exchange (ETDEWEB)

    Lin, D.P.; Kevan, L.

    1977-05-19

    Electron--electron double resonance (ELDOR) has been used to test the validity of the noninteracting spin packet model for inhomogeneously broadened ESR lines. For trapped electrons in 10M NaOD/D/sub 2/O glassy ice the saturation of field-swept ELDOR spectra fits the above mentioned model in contrast to earlier work on trapped electrons in protiated matrices. In the protiated matrix spin diffusion produces significant interaction between the spin packets. The difference between the protiated and deuterated matrices suggests that nuclear relaxation is the mechanism for spin diffusion. The deuterated matrices show no structure in frequency-swept ELDOR spectra due to deuteron spin--flip transitions whereas structure due to proton spin--flips is seen in protiated matrices.

  17. Inversion of electron spin resonance signal in coals

    Science.gov (United States)

    Poklonski, N. A.; Vyrko, S. A.; Poklonskaya, O. N.; Lapchuk, N. M.; Munkhtsetseg, S.

    2013-07-01

    Samples of coal from the Donetsk basin (carbon content ~90 mass%) in both lump and powder forms were studied by continuous-wave electron spin resonance (ESR) at room temperature in air. Inversion of the ESR signal (being in phase with modulation of the constant magnetic field) with an increase of lump size along the magnetic component of the microwave field was observed in the cavity of the radiospectrometer.

  18. Study of metalloproteins using continuous wave electron paramagnetic resonance (EPR).

    Science.gov (United States)

    Gambarelli, Serge; Maurel, Vincent

    2014-01-01

    Electron paramagnetic resonance (EPR) is an invaluable tool when studying systems with paramagnetic centers. It is a sensitive spectroscopic method, which can be used with dilute samples in aqueous buffer solutions. Here, we describe the basic procedure for recording an X-band EPR spectrum of a metalloprotein sample at low temperature. We also discuss basic optimization techniques to provide spectra with a high signal to noise ratio and minimum distortion.

  19. Electron paramagnetic resonance of some {gamma}-irradiated drugs

    Energy Technology Data Exchange (ETDEWEB)

    Koeseoglu, R.; Koeseoglu, E.; Koeksal, F. E-mail: koksalf@ttnet.net.tr

    2003-01-01

    Some drugs, used mainly in treatment of some neurological diseases and hypertension were exposed to {gamma}-irradiation, and the samples were investigated by electron paramagnetic resonance (EPR). The observed spectra were interpreted in terms of some type of alkyl and amine radical fragments. The spectra were computer simulated and the g values of the radicals and the hyperfine structure constants of the free electron with nearby protons were determined. The species were found to be stable at room temperature for more than a year. The samples were found to display no EPR signal without irradiation.

  20. Two-photon imaging through a multimode fiber

    CERN Document Server

    Morales-Delgado, Edgar E; Moser, Christophe

    2015-01-01

    In this work we demonstrate 3D imaging using two-photon excitation through a 20 cm long multimode optical fiber (MMF) of 350 micrometers diameter. The imaging principle is similar to single photon fluorescence through a MMF, except that a focused femtosecond pulse is delivered and scanned over the sample. In our approach, focusing and scanning through the fiber is accomplished by digital phase conjugation using mode selection by time gating with an ultra-fast reference pulse. The excited two-photon emission is collected through the same fiber. We demonstrate depth sectioning by scanning the focused pulse in a 3D volume over a sample consisting of fluorescent beads suspended in a polymer. The achieved resolution is 1 micrometer laterally and 15 micrometers axially. Scanning is performed over an 80x80 micrometers field of view. To our knowledge, this is the first demonstration of high-resolution three-dimensional imaging using two-photon fluorescence through a multimode fiber.

  1. Recent two-photon physics results from ARGUS

    Science.gov (United States)

    Živko Representing Argus Collaboration, Tomi

    1995-07-01

    Two photon production of π+π+π0π-π-, K+K-π+π-, K+K-π+π0π-, π+π0π-, and π+π- has been studied using the ARGUS detector at the e+e- storage ring DORIS II at DESY. A partial wave analysis was performed on the five-pion and three-pion final states. In the reaction γγ→ωρ0 is showed that the partial-wave with spin and parity (JP,Jz)=(2+,±2) dominates. The cross section and angular distributions of the reaction γγ→φρ0→K+K-π+π- were measured for the first time. The production of the vector-meson pair φω is observed in the two-photon reaction γγ→K+K-π+π0π-. The two-photon width of the tensor meson a2(1320) was measured in the decay channel π+π0π-. An upper limit, significantly lower than indicated by previous experiments was set on the radiative width of the π2(1670) meson. An upper limit was set on the radiative width of the f0(975)in the decay channel π+π-.

  2. Two-Photon Absorption in Organometallic Bromide Perovskites

    KAUST Repository

    Walters, Grant

    2015-07-21

    Organometallic trihalide perovskites are solution processed semiconductors that have made great strides in third generation thin film light harvesting and light emitting optoelectronic devices. Recently it has been demonstrated that large, high purity single crystals of these perovskites can be synthesized from the solution phase. These crystals’ large dimensions, clean bandgap, and solid-state order, have provided us with a suitable medium to observe and quantify two-photon absorption in perovskites. When CH3NH3PbBr3 single crystals are pumped with intense 800 nm light, we observe band-to-band photoluminescence at 572 nm, indicative of two-photon absorption. We report the nonlinear absorption coefficient of CH3NH3PbBr3 perovskites to be 8.6 cm GW-1 at 800 nm, comparable to epitaxial single crystal semiconductors of similar bandgap. We have leveraged this nonlinear process to electrically autocorrelate a 100 fs pulsed laser using a two-photon perovskite photodetector. This work demonstrates the viability of organometallic trihalide perovskites as a convenient and low-cost nonlinear absorber for applications in ultrafast photonics.

  3. Exploring control parameters of two photon processes in solutions

    Indian Academy of Sciences (India)

    Debabrata Goswami; Amit Nag

    2012-01-01

    Two-photon microscopy depends extensively on the two-photon absorption cross-sections of biologically relevant chromophores. High repetition rate (HRR) lasers are essential in multiphoton microscopy for generating satisfactory signal to noise at low average powers. However, HRR lasers generate thermal distortions in samples even with the slightest single photon absorption. We use an optical chopper with HRR lasers to intermittently `blank’ irradiation and effectively minimize thermal effects to result in a femtosecond z-scan setup that precisely measures the two-photon absorption (TPA) cross-sections of chromophores. Though several experimental factors impact such TPA measurements, a systematic effort to modulate and influence TPA characteristics is yet to evolve. Here, we present the effect of several control parameters on the TPA process that are independent of chromophore characteristics for femtosecond laser pulse based measurements; and demonstrate how the femtosecond laser pulse repetition rate, chromophore environment and incident laser polarization can become effective control parameters for such nonlinear optical properties.

  4. Two-Photon Absorption in Organometallic Bromide Perovskites.

    Science.gov (United States)

    Walters, Grant; Sutherland, Brandon R; Hoogland, Sjoerd; Shi, Dong; Comin, Riccardo; Sellan, Daniel P; Bakr, Osman M; Sargent, Edward H

    2015-09-22

    Organometallic trihalide perovskites are solution-processed semiconductors that have made great strides in third-generation thin film light-harvesting and light-emitting optoelectronic devices. Recently, it has been demonstrated that large, high-purity single crystals of these perovskites can be synthesized from the solution phase. These crystals' large dimensions, clean bandgap, and solid-state order have provided us with a suitable medium to observe and quantify two-photon absorption in perovskites. When CH3NH3PbBr3 single crystals are pumped with intense 800 nm light, we observe band-to-band photoluminescence at 572 nm, indicative of two-photon absorption. We report the nonlinear absorption coefficient of CH3NH3PbBr3 perovskites to be 8.6 cm GW(-1) at 800 nm, comparable to epitaxial single-crystal semiconductors of similar bandgap. We have leveraged this nonlinear process to electrically autocorrelate a 100 fs pulsed laser using a two-photon perovskite photodetector. This work demonstrates the viability of organometallic trihalide perovskites as a convenient and low-cost nonlinear absorber for applications in ultrafast photonics.

  5. Investigation of Relativistic Electron Resonance with EMIC Waves

    Science.gov (United States)

    Woodger, L. A.; Millan, R. M.; Denton, R. E.

    2008-12-01

    Wave-particle interaction of relativistic electrons with EMIC waves has been proposed as an important loss mechanism for radiation belt electrons (e.g. Thorne and Andreoli, 1980). Lorentzen et al (2000) and Millan et al (2002) suggested this mechanism to be responsible for dusk side relativistic electron precipitation (REP) detected by balloon borne instrumentation. This study will use the linear electromagnetic dispersion code WHAMP to investigate the effects of density, magnetic field, anisotropy, and heavy ions on the minimum resonance energy for relativistic electrons with EMIC waves. Results will be compared with observations of REP during the MAXIS balloon campaign on Jan. 19, 2000 and the MINIS balloon campaign on Jan. 21, 2005.

  6. Theoretical studies on the one- and two-photon absorption properties of azulenylporphyrins and azulene-fused porphyrins

    Institute of Scientific and Technical Information of China (English)

    Li Wen-Chao; Feng Ji-Kang; Ren Ai-Min; Zhang Xiang-Biao; Sun Jia-Zhong

    2009-01-01

    The electronic structures, one-photon absorption (OPA) and two-photon absorption (TPA) properties of the azulenylporphyrins and azulene-fused porphyrins have been comparatively studied by using DFT/B3LYP/6-31G(d)and the ZINDO/SDCI method. With the number of azulenyl groups increasing, the OPA wavelengths of all molecules are red-shifted in 400-600 nm and the two-photon absorption cross section is gradually enlarged. The azulene-fused structures facilitate an expanding conjugated area and increasing TPA cross section. The origin of TPA properties of studied compounds is studied with a two-level model. In summary, the azulene-fused porphyrins exhibit strong two-photon absorption.

  7. (Un)determined finite regularization dependent quantum corrections: the Higgs decay into two photons and the two photon scattering examples

    CERN Document Server

    Cherchiglia, A L; Nemes, M C; Sampaio, Marcos

    2012-01-01

    We investigate the appearance of arbitrary, regularization dependent parameters introduced by divergent integrals in two a priori finite but superficially divergent amplitudes: the Higgs decay into two photons and the two photon scattering. We use a general parametrization of ultraviolet divergences which explicitates such ambiguities. Thus we separate in a consistent way using Implicit Regularization the divergent, finite and regularization dependent parts of the amplitudes which in turn are written as surface terms. We find that, although finite, these amplitudes are ambiguous before the imposition of physical conditions namely momentum routing invariance in the loops of Feynman diagrams. In the examples we study momentum routing invariance turns out to be equivalent to gauge invariance. We also discuss the results obtained by different regularizations and show how they can be reproduced within our framework allowing for a clear view on the origin of regularization ambiguities.

  8. In-situ electron paramagnetic resonance studies of paramagnetic point defects in superconducting microwave resonators

    Science.gov (United States)

    Zhang, Shengke; Kopas, Cameron; Wagner, Brian; Queen, Daniel; Newman, N.

    2016-09-01

    The physical nature and concentration of paramagnetic point defects in the dielectrics of superconducting planar microwave resonators have been determined using in-situ electron paramagnetic resonance spectroscopy. To perform this work, the quality factor of parallel plate and stripline resonators was measured as a function of the magnitude of a magnetic-field applied parallel to the electrode surfaces. YBa2Cu3O7-δ thin film electrodes proved to be a preferred choice over Nb and MgB2 because they are readily available and have a small surface resistance (Rs) up to high temperatures (˜77 K) and magnetic fields (i.e., dielectric, Co2+-doped Ba(Zn1/3Nb2/3)O3, are shown to have losses dominated by d-electron spin-excitations in exchange-coupled Co2+ point-defect clusters, even in the absence of an applied magnetic field. A significant enhanced microwave loss in stripline and parallel plate resonators is found to correlate with the presence of paramagnetic Mn2+ dopants in Ba(Zn1/3Ta2/3)O3 ceramics and dangling bond states in amorphous Si thin films, although the identification of the dominant loss mechanism(s) in these dielectrics requires further investigation.

  9. Measurement of two-photon exchange effect by comparing elastic $e^\\pm p$ cross sections

    CERN Document Server

    Rimal, D; Raue, B A; Weinstein, L B; Arrington, J; Brooks, W K; Ungaro, M; Adhikari, K P; Akbar, Z; Pereira, S Anefalos; Badui, R A; Ball, J; Baltzell, N A; Battaglieri, M; Batourine, V; Bedlinskiy, I; Bennett, R P; Biselli, A S; Boiarinov, S; Briscoe, W J; Bültmann, S; Carman, D S; Celentano, A; Chetry, T; Ciullo, G; Clark, L; Colaneri, L; Cole, P L; Compton, N; Contalbrigo, M; Cortes, O; Crede, V; D'Angelo, A; Dashyan, N; De Vita, R; Deur, A; Djalali, C; Dupre, R; Egiyan, H; Alaoui, A El; Fassi, L El; Eugenio, P; Fedotov, G; Fersch, R; Filippi, A; Fleming, J A; Forest, T A; Fradi, A; Gevorgyan, N; Ghandilyan, Y; Gilfoyle, G P; Giovanetti, K L; Girod, F X; Gleason, C; Gohn, W; Golovatch, E; Gothe, R W; Griffioen, K A; Guo, L; Hafidi, K; Hanretty, C; Harrison, N; Hattawy, M; Heddle, D; Hicks, K; Holtrop, M; Hughes, S M; Ilieva, Y; Ireland, D G; Ishkhanov, B S; Isupov, E L; Jenkins, D; Jiang, H; Joosten, S; Keller, D; Khetarpal, P; Khachatryan, G; Khandaker, M; Kim, W; Klein, A; Klein, F J; Kubarovsky, V; Kuhn, S E; Kuleshov, S V; Lanza, L; Lenisa, P; Livingston, K; Lu, H Y; MacGregor, I J D; Markov, N; McKinnon, B; Mestayer, M D; Mirazita, M; Mokeev, V; Movsisyan, A; Munevar, E; Camacho, C Munoz; Nadel-Turonski, P; Ni, A; Niccolai, S; Niculescu, G; Niculescu, I; Osipenko, M; Ostrovidov, A I; Paolone, M; Paremuzyan, R; Park, K; Pasyuk, E; Phelps, W; Pisano, S; Pogorelko, O; Price, J W; Prok, Y; Protopopescu, D; Puckett, A J R; Rizzo, A; Rosner, G; Rossi, P; Roy, P; Sabatié, F; Salgado, C; Schumacher, R A; Seder, E; Sharabian, Y G; Skorodumina, Iu; Smith, G D; Sokhan, D; Sparveris, N; Stankovic, Ivana; Stepanyan, S; Strauch, S; Sytnik, V; Taiuti, M; Torayev, B; Voskanyan, H; Voutier, E; Walford, N K; Watts, D P; Wei, X; Wood, M H; Zachariou, N; Zana, L; Zhang, J; Zhao, Z W; Zonta, I

    2016-01-01

    [Background] The electromagnetic form factors of the proton measured by unpolarized and polarized electron scattering experiments show a significant disagreement that grows with the squared four momentum transfer ($Q^{2}$). Calculations have shown that the two measurements can be largely reconciled by accounting for the contributions of two-photon exchange (TPE). TPE effects are not typically included in the standard set of radiative corrections since theoretical calculations of the TPE effects are highly model dependent, and, until recently, no direct evidence of significant TPE effects has been observed. [Purpose] We measured the ratio of positron-proton to electron-proton elastic-scattering cross sections in order to determine the TPE contribution to elastic electron-proton scattering and thereby resolve the proton electric form factor discrepancy. [Methods] We produced a mixed simultaneous electron-positron beam in Jefferson Lab's Hall B by passing the 5.6 GeV primary electron beam through a radiator to p...

  10. Reaching the quantum limit of sensitivity in electron spin resonance

    Science.gov (United States)

    Bienfait, A.; Pla, J. J.; Kubo, Y.; Stern, M.; Zhou, X.; Lo, C. C.; Weis, C. D.; Schenkel, T.; Thewalt, M. L. W.; Vion, D.; Esteve, D.; Julsgaard, B.; Mølmer, K.; Morton, J. J. L.; Bertet, P.

    2016-03-01

    The detection and characterization of paramagnetic species by electron spin resonance (ESR) spectroscopy is widely used throughout chemistry, biology and materials science, from in vivo imaging to distance measurements in spin-labelled proteins. ESR relies on the inductive detection of microwave signals emitted by the spins into a coupled microwave resonator during their Larmor precession. However, such signals can be very small, prohibiting the application of ESR at the nanoscale (for example, at the single-cell level or on individual nanoparticles). Here, using a Josephson parametric microwave amplifier combined with high-quality-factor superconducting microresonators cooled at millikelvin temperatures, we improve the state-of-the-art sensitivity of inductive ESR detection by nearly four orders of magnitude. We demonstrate the detection of 1,700 bismuth donor spins in silicon within a single Hahn echo with unit signal-to-noise ratio, reduced to 150 spins by averaging a single Carr-Purcell-Meiboom-Gill sequence. This unprecedented sensitivity reaches the limit set by quantum fluctuations of the electromagnetic field instead of thermal or technical noise, which constitutes a novel regime for magnetic resonance. The detection volume of our resonator is ˜0.02 nl, and our approach can be readily scaled down further to improve sensitivity, providing a new versatile toolbox for ESR at the nanoscale.

  11. Electron cyclotron resonance heating in a short cylindrical plasma system

    Indian Academy of Sciences (India)

    Vipin K Yadav; D Bora

    2004-09-01

    Electron cyclotron resonance (ECR) plasma is produced and studied in a small cylindrical system. Microwave power is delivered by a CW magnetron at 2.45 GHz in TE10 mode and launched radially to have extraordinary (X) wave in plasma. The axial magnetic field required for ECR in the system is such that the first two ECR surfaces ( = 875.0 G and = 437.5 G) reside in the system. ECR plasma is produced with hydrogen with typical plasma density e as 3.2 × 1010 cm-3 and plasma temperature e between 9 and 15 eV. Various cut-off and resonance positions are identified in the plasma system. ECR heating (ECRH) of the plasma is observed experimentally. This heating is because of the mode conversion of X-wave to electron Bernstein wave (EBW) at the upper hybrid resonance (UHR) layer. The power mode conversion efficiency is estimated to be 0.85 for this system. The experimental results are presented in this paper.

  12. Randomized benchmarking of quantum gates implemented by electron spin resonance

    Science.gov (United States)

    Park, Daniel K.; Feng, Guanru; Rahimi, Robabeh; Baugh, Jonathan; Laflamme, Raymond

    2016-06-01

    Spin systems controlled and probed by magnetic resonance have been valuable for testing the ideas of quantum control and quantum error correction. This paper introduces an X-band pulsed electron spin resonance spectrometer designed for high-fidelity coherent control of electron spins, including a loop-gap resonator for sub-millimeter sized samples with a control bandwidth ∼40 MHz. Universal control is achieved by a single-sideband upconversion technique with an I-Q modulator and a 1.2 GS/s arbitrary waveform generator. A single qubit randomized benchmarking protocol quantifies the average errors of Clifford gates implemented by simple Gaussian pulses, using a sample of gamma-irradiated quartz. Improvements in unitary gate fidelity are achieved through phase transient correction and hardware optimization. A preparation pulse sequence that selects spin packets in a narrowed distribution of static fields confirms that inhomogeneous dephasing (1 / T2∗) is the dominant source of gate error. The best average fidelity over the Clifford gates obtained here is 99.2 % , which serves as a benchmark to compare with other technologies.

  13. Electron energy-loss spectroscopy of branched gap plasmon resonators

    Science.gov (United States)

    Raza, Søren; Esfandyarpour, Majid; Koh, Ai Leen; Mortensen, N. Asger; Brongersma, Mark L.; Bozhevolnyi, Sergey I.

    2016-12-01

    The miniaturization of integrated optical circuits below the diffraction limit for high-speed manipulation of information is one of the cornerstones in plasmonics research. By coupling to surface plasmons supported on nanostructured metallic surfaces, light can be confined to the nanoscale, enabling the potential interface to electronic circuits. In particular, gap surface plasmons propagating in an air gap sandwiched between metal layers have shown extraordinary mode confinement with significant propagation length. In this work, we unveil the optical properties of gap surface plasmons in silver nanoslot structures with widths of only 25 nm. We fabricate linear, branched and cross-shaped nanoslot waveguide components, which all support resonances due to interference of counter-propagating gap plasmons. By exploiting the superior spatial resolution of a scanning transmission electron microscope combined with electron energy-loss spectroscopy, we experimentally show the propagation, bending and splitting of slot gap plasmons.

  14. Characteristics of surface sterilization using electron cyclotron resonance plasma

    Science.gov (United States)

    Yonesu, Akira; Hara, Kazufumi; Nishikawa, Tatsuya; Hayashi, Nobuya

    2016-07-01

    The characteristics of surface sterilization using electron cyclotron resonance (ECR) plasma were investigated. High-energy electrons and oxygen radicals were observed in the ECR zone using electric probe and optical emission spectroscopic methods. A biological indicator (BI), Geobacillus stearothermophilus, containing 1 × 106 spores was sterilized in 120 s by exposure to oxygen discharges while maintaining a temperature of approximately 55 °C at the BI installation position. Oxygen radicals and high-energy electrons were found to be the sterilizing species in the ECR region. It was demonstrated that the ECR plasma could be produced in narrow tubes with an inner diameter of 5 mm. Moreover, sterilization tests confirmed that the spores present inside the narrow tube were successfully inactivated by ECR plasma irradiation.

  15. The Electron Paramagnetic Resonance in the study of tissue specimens

    CERN Document Server

    Stefaniuk, Ireneusz; Skrȩt, Andrzej; Skrȩt-Magierło, Joanna; Góra, Tomasz; Szczerba, Piotr

    2014-01-01

    The Electron Paramagnetic Spectroscopy (EPR) is the most direct and powerful method for the detection and identification of free radicals and other species with unpaired electrons. Statistics disorders are a common gynaecological disorder occurring in women. The condition afflicts around 15% of women to the extent of impairing the quality of living. According to scientific reports as many as 50% of women experiencing problems related to genital statistics disorders. The aim of this work was to investigate tissue taken from women with genital statistics disorders using the Electron Paramagnetic Resonance method. The studies on the tissue of women is one of the first studies in this area. In this work we observed a close relationship between the observed EPR signal and the consumption of omega 3 acids.

  16. Resonance effects in electron-impact ionization of helium

    Science.gov (United States)

    Fang, Yanghua; Bartschat, Klaus

    2001-07-01

    We have extended our recent work on electron-impact ionization and ionization-excitation of helium (Fang Y and Bartschat K 2001 J. Phys. B: At. Mol. Opt. Phys. 34 L19) to investigate resonance structures in the ejected-electron-residual-ion interaction. The calculations were performed using a second-order perturbative model for a `fast' incident projectile together with a convergent R-matrix with pseudo-states close-coupling model for the initial bound state and the scattering of a `slow' ejected electron in the field of the ion. The agreement with previous calculations by Marchalant et al using a similar model is satisfactory and confirms the importance of the `two-step' mechanism in these processes. However, significant discrepancies remain with experimental data by Lower and Weigold and, to a lesser extent, by McDonald and Crowe.

  17. Studies of Beam Induced Electron Cloud Resonances in Dipole Magnetic Fields

    CERN Document Server

    Calvey, J R; Makita, J; Venturini, M

    2016-01-01

    The buildup of low energy electrons in an accelerator, known as electron cloud, can be severely detrimental to machine performance. Under certain beam conditions, the beam can become resonant with the cloud dynamics, accelerating the buildup of electrons. This paper will examine two such effects: multipacting resonances, in which the cloud development time is resonant with the bunch spacing, and cyclotron resonances, in which the cyclotron period of electrons in a magnetic field is a multiple of bunch spacing. Both resonances have been studied directly in dipole fields using retarding field analyzers installed in the Cornell Electron Storage Ring (CESR). These measurements are supported by both analytical models and computer simulations.

  18. Plasma production for electron acceleration by resonant plasma wave

    Science.gov (United States)

    Anania, M. P.; Biagioni, A.; Chiadroni, E.; Cianchi, A.; Croia, M.; Curcio, A.; Di Giovenale, D.; Di Pirro, G. P.; Filippi, F.; Ghigo, A.; Lollo, V.; Pella, S.; Pompili, R.; Romeo, S.; Ferrario, M.

    2016-09-01

    Plasma wakefield acceleration is the most promising acceleration technique known nowadays, able to provide very high accelerating fields (10-100 GV/m), enabling acceleration of electrons to GeV energy in few centimeter. However, the quality of the electron bunches accelerated with this technique is still not comparable with that of conventional accelerators (large energy spread, low repetition rate, and large emittance); radiofrequency-based accelerators, in fact, are limited in accelerating field (10-100 MV/m) requiring therefore hundred of meters of distances to reach the GeV energies, but can provide very bright electron bunches. To combine high brightness electron bunches from conventional accelerators and high accelerating fields reachable with plasmas could be a good compromise allowing to further accelerate high brightness electron bunches coming from LINAC while preserving electron beam quality. Following the idea of plasma wave resonant excitation driven by a train of short bunches, we have started to study the requirements in terms of plasma for SPARC_LAB (Ferrario et al., 2013 [1]). In particular here we focus on hydrogen plasma discharge, and in particular on the theoretical and numerical estimates of the ionization process which are very useful to design the discharge circuit and to evaluate the current needed to be supplied to the gas in order to have full ionization. Eventually, the current supplied to the gas simulated will be compared to that measured experimentally.

  19. Plasma production for electron acceleration by resonant plasma wave

    Energy Technology Data Exchange (ETDEWEB)

    Anania, M.P., E-mail: maria.pia.anania@lnf.infn.it [INFN - LNF, via Enrico Fermi, 40, 00044 Frascati (Italy); Biagioni, A.; Chiadroni, E. [INFN - LNF, via Enrico Fermi, 40, 00044 Frascati (Italy); Cianchi, A. [University of Rome Tor Vergata - INFN, via della Ricerca Scientifica, 1, 00133 Roma (Italy); INFN, Via della Ricerca Scientifica, 1, 00133 Roma (Italy); Croia, M.; Curcio, A. [INFN - LNF, via Enrico Fermi, 40, 00044 Frascati (Italy); University of Rome La Sapienza, Piazzale Aldo Moro, 2, 00185 Roma (Italy); Di Giovenale, D.; Di Pirro, G.P. [INFN - LNF, via Enrico Fermi, 40, 00044 Frascati (Italy); Filippi, F. [University of Rome La Sapienza, Piazzale Aldo Moro, 2, 00185 Roma (Italy); Ghigo, A.; Lollo, V.; Pella, S.; Pompili, R. [INFN - LNF, via Enrico Fermi, 40, 00044 Frascati (Italy); Romeo, S. [INFN - LNF, via Enrico Fermi, 40, 00044 Frascati (Italy); University of Rome La Sapienza, Piazzale Aldo Moro, 2, 00185 Roma (Italy); Ferrario, M. [INFN - LNF, via Enrico Fermi, 40, 00044 Frascati (Italy)

    2016-09-01

    Plasma wakefield acceleration is the most promising acceleration technique known nowadays, able to provide very high accelerating fields (10–100 GV/m), enabling acceleration of electrons to GeV energy in few centimeter. However, the quality of the electron bunches accelerated with this technique is still not comparable with that of conventional accelerators (large energy spread, low repetition rate, and large emittance); radiofrequency-based accelerators, in fact, are limited in accelerating field (10–100 MV/m) requiring therefore hundred of meters of distances to reach the GeV energies, but can provide very bright electron bunches. To combine high brightness electron bunches from conventional accelerators and high accelerating fields reachable with plasmas could be a good compromise allowing to further accelerate high brightness electron bunches coming from LINAC while preserving electron beam quality. Following the idea of plasma wave resonant excitation driven by a train of short bunches, we have started to study the requirements in terms of plasma for SPARC-LAB (Ferrario et al., 2013 [1]). In particular here we focus on hydrogen plasma discharge, and in particular on the theoretical and numerical estimates of the ionization process which are very useful to design the discharge circuit and to evaluate the current needed to be supplied to the gas in order to have full ionization. Eventually, the current supplied to the gas simulated will be compared to that measured experimentally.

  20. λ/26 silver nanodots fabricated by direct laser writing through highly sensitive two-photon photoreduction

    Energy Technology Data Exchange (ETDEWEB)

    Cao, Yaoyu; Gu, Min, E-mail: mgu@swin.edu.au [Centre for Micro-Photonics and CUDOS, Faculty of Engineering and Industrial Sciences, Swinburne University of Technology, P.O. Box 218, Hawthorn, Victoria 3122 (Australia)

    2013-11-18

    We demonstrated an approach to break the diffraction limit and realise deep-subwavelength two-photon direct laser writing by employing a highly sensitive photoreduction process. The photoreduction photosensitivity increased by at least 4 times while the wavelength of the fabrication laser beam was tuned from 800 nm to 580 nm. The increase of the photosensitivity resulted in improved resolution for the silver dot fabrication. By developing the photoreduction material with adding electron donors, the photosensitivity further increased and enabled the realisation of a single silver dot at 22 nm which is λ/26 for the wavelength of the fabrication laser beam.

  1. Two-photon imaging and analysis of neural network dynamics

    Science.gov (United States)

    Lütcke, Henry; Helmchen, Fritjof

    2011-08-01

    The glow of a starry night sky, the smell of a freshly brewed cup of coffee or the sound of ocean waves breaking on the beach are representations of the physical world that have been created by the dynamic interactions of thousands of neurons in our brains. How the brain mediates perceptions, creates thoughts, stores memories and initiates actions remains one of the most profound puzzles in biology, if not all of science. A key to a mechanistic understanding of how the nervous system works is the ability to measure and analyze the dynamics of neuronal networks in the living organism in the context of sensory stimulation and behavior. Dynamic brain properties have been fairly well characterized on the microscopic level of individual neurons and on the macroscopic level of whole brain areas largely with the help of various electrophysiological techniques. However, our understanding of the mesoscopic level comprising local populations of hundreds to thousands of neurons (so-called 'microcircuits') remains comparably poor. Predominantly, this has been due to the technical difficulties involved in recording from large networks of neurons with single-cell spatial resolution and near-millisecond temporal resolution in the brain of living animals. In recent years, two-photon microscopy has emerged as a technique which meets many of these requirements and thus has become the method of choice for the interrogation of local neural circuits. Here, we review the state-of-research in the field of two-photon imaging of neuronal populations, covering the topics of microscope technology, suitable fluorescent indicator dyes, staining techniques, and in particular analysis techniques for extracting relevant information from the fluorescence data. We expect that functional analysis of neural networks using two-photon imaging will help to decipher fundamental operational principles of neural microcircuits.

  2. Two-photon imaging and analysis of neural network dynamics

    Energy Technology Data Exchange (ETDEWEB)

    Luetcke, Henry; Helmchen, Fritjof [Brain Research Institute, University of Zurich, Winterthurerstrasse 190, CH-8057 Zurich (Switzerland)

    2011-08-15

    The glow of a starry night sky, the smell of a freshly brewed cup of coffee or the sound of ocean waves breaking on the beach are representations of the physical world that have been created by the dynamic interactions of thousands of neurons in our brains. How the brain mediates perceptions, creates thoughts, stores memories and initiates actions remains one of the most profound puzzles in biology, if not all of science. A key to a mechanistic understanding of how the nervous system works is the ability to measure and analyze the dynamics of neuronal networks in the living organism in the context of sensory stimulation and behavior. Dynamic brain properties have been fairly well characterized on the microscopic level of individual neurons and on the macroscopic level of whole brain areas largely with the help of various electrophysiological techniques. However, our understanding of the mesoscopic level comprising local populations of hundreds to thousands of neurons (so-called 'microcircuits') remains comparably poor. Predominantly, this has been due to the technical difficulties involved in recording from large networks of neurons with single-cell spatial resolution and near-millisecond temporal resolution in the brain of living animals. In recent years, two-photon microscopy has emerged as a technique which meets many of these requirements and thus has become the method of choice for the interrogation of local neural circuits. Here, we review the state-of-research in the field of two-photon imaging of neuronal populations, covering the topics of microscope technology, suitable fluorescent indicator dyes, staining techniques, and in particular analysis techniques for extracting relevant information from the fluorescence data. We expect that functional analysis of neural networks using two-photon imaging will help to decipher fundamental operational principles of neural microcircuits.

  3. New two-photon based nanoscopic modalities and optogenetics

    DEFF Research Database (Denmark)

    Glückstad, Jesper

    -matter interaction on these scales involves the combination of optimal light-sculpting [4] with the use of optimized shapes in micro-robotics structures [5]. Microfabrication processes such as two-photon photo-polymerization offer three-dimensional resolutions for creating custom-designed monolithic microstructures...... that can be equipped with optical trapping handles for convenient mechanical control using only optical forces [6]. These microstructures illustrated above can be effectively handled with simultaneous top- and side-view on our BioPhotonics Workstation to undertake six-degree-of-freedom optical actuation...

  4. Two-photon polymerization of immune cell scaffolds

    DEFF Research Database (Denmark)

    Olsen, Mark Holm

    and easy to use chip integrated migration platform. Free-form constructs with three-dimensional (3D) microporosity were fabricated by two-photon polymerization inside the closed microchannel of an injection molded commercially available polymer chip for analysis of directed cell migration. Acrylate...... also present a poly (ethylene glycol) diacrylate (PEGDA) based strategy to fabricate soft 3D hydrogel scaffolds. Our experiments with the hydrogel confirm we can control the mechanical properties and introduce biochemical cues on the surface that are recognized by fibroblast cells. Finally we present...

  5. Two-photon tomography using on-chip quantum walks

    CERN Document Server

    Titchener, James; Sukhorukov, Andrey

    2016-01-01

    We present a conceptual approach to quantum tomography based on first expanding a quantum state across extra degrees of freedom and then exploiting the introduced sparsity to perform reconstruction. We formulate its application to photonic circuits, and show that measured spatial photon correlations at the output of a specially tailored discrete-continuous quantum-walk can enable full reconstruction of any two-photon spatially entangled and mixed state at the input. This approach does not require any tunable elements, so is well suited for integration with on-chip superconducting photon detectors.

  6. Two Photon Decays of Charmonia from Lattice QCD

    Energy Technology Data Exchange (ETDEWEB)

    Jozef Dudek; Robert Edwards

    2006-07-12

    We make the first calculation in lattice QCD of two-photon decays of mesons. Working in the charmonium sector, using the LSZ reduction to relate a photon to a sum of hadronic vector eigenstates, we compute form-factors in both the space-like and time-like domains for the transitions {eta}{sub c} {yields} {gamma}*{gamma}* and {chi}{sub c0} {yields} {gamma}*{gamma}*. At the on-shell point we find approximate agreement with experimental world-average values.

  7. Quantum teleportation of one- and two-photon superposition states

    Institute of Scientific and Technical Information of China (English)

    李英; 张天才; 张俊香; 谢常德

    2003-01-01

    Quantum teleportation of one- and two-photon superposition states based on EPR entanglement of continuouswave two-mode squeezed state is discussed. The fidelities of teleportation are deduced for two different input quantum states. The dependence of the fidelity on the parameters of EPR entanglement and the gain of the classical channels are shown numerically. Comparing with the teleportation of Fock state and coherent state, it is pointed out that for given EPR entanglement and classical gain, the higher the nonclassicality of the input state, the lower the accessible fidelity of teleportation.

  8. Inclusive $D*^{+-}$ Production in Two-Photon Collisions at LEP

    CERN Document Server

    Achard, P; Aguilar-Benítez, M; Alcaraz, J; Alemanni, G; Allaby, James V; Aloisio, A; Alviggi, M G; Anderhub, H; Andreev, V P; Anselmo, F; Arefev, A; Azemoon, T; Aziz, T; Bagnaia, P; Bajo, A; Baksay, G; Baksay, L; Baldew, S V; Banerjee, S; Banerjee, Sw; Barczyk, A; Barillère, R; Bartalini, P; Basile, M; Batalova, N; Battiston, R; Bay, A; Becattini, F; Becker, U; Behner, F; Bellucci, L; Berbeco, R; Berdugo, J; Berges, P; Bertucci, B; Betev, B L; Biasini, M; Biglietti, M; Biland, A; Blaising, J J; Blyth, S C; Bobbink, Gerjan J; Böhm, A; Boldizsar, L; Borgia, B; Bottai, S; Bourilkov, D; Bourquin, Maurice; Braccini, S; Branson, J G; Brochu, F; Burger, J D; Burger, W J; Cai, X D; Capell, M; Cara Romeo, G; Carlino, G; Cartacci, A M; Casaus, J; Cavallari, F; Cavallo, N; Cecchi, C; Cerrada, M; Chamizo-Llatas, M; Chang, Y H; Chemarin, M; Chen, A; Chen, G; Chen, G M; Chen, H F; Chen, H S; Chiefari, G; Cifarelli, Luisa; Cindolo, F; Clare, I; Clare, R; Coignet, G; Colino, N; Costantini, S; de la Cruz, B; Cucciarelli, S; van Dalen, J A; De Asmundis, R; Déglon, P L; Debreczeni, J; Degré, A; Deiters, K; Della Volpe, D; Delmeire, E; Denes, P; De Notaristefani, F; De Salvo, A; Diemoz, M; Dierckxsens, M; Dionisi, C; Dittmar, Michael; Doria, A; Dova, M T; Duchesneau, D; Echenard, B; Eline, A; El-Mamouni, H; Engler, A; Eppling, F J; Ewers, A; Extermann, Pierre; Falagán, M A; Falciano, S; Favara, A; Fay, J; Fedin, O; Felcini, Marta; Ferguson, T; Fesefeldt, H S; Fiandrini, E; Field, J H; Filthaut, Frank; Fisher, P H; Fisher, W; Fisk, I; Forconi, G; Freudenreich, Klaus; Furetta, C; Galaktionov, Yu; Ganguli, S N; García-Abia, P; Gataullin, M; Gentile, S; Giagu, S; Gong, Z F; Grenier, G; Grimm, O; Grünewald, M W; Guida, M; van Gulik, R; Gupta, V K; Gurtu, A; Gutay, L J; Haas, D; Hakobyan, R S; Hatzifotiadou, D; Hebbeker, T; Hervé, A; Hirschfelder, J; Hofer, H; Hohlmann, M; Holzner, G; Hou, S R; Hu, Y; Jin, B N; Jones, L W; de Jong, P; Josa-Mutuberria, I; Käfer, D; Kaur, M; Kienzle-Focacci, M N; Kim, J K; Kirkby, Jasper; Kittel, E W; Klimentov, A; König, A C; Kopal, M; Koutsenko, V F; Kräber, M H; Krämer, R W; Krenz, W; Krüger, A; Kunin, A; Ladrón de Guevara, P; Laktineh, I; Landi, G; Lebeau, M; Lebedev, A; Lebrun, P; Lecomte, P; Lecoq, P; Le Coultre, P; Le Goff, J M; Leiste, R; Levtchenko, M; Levchenko, P M; Li, C; Likhoded, S A; Lin, C H; Lin, W T; Linde, Frank L; Lista, L; Liu, Z A; Lohmann, W; Longo, E; Lü, Y S; Lübelsmeyer, K; Luci, C; Luminari, L; Lustermann, W; Ma Wen Gan; Malgeri, L; Malinin, A; Maña, C; Mangeol, D J J; Mans, J; Martin, J P; Marzano, F; Mazumdar, K; McNeil, R R; Mele, S; Merola, L; Meschini, M; Metzger, W J; Mihul, A; Milcent, H; Mirabelli, G; Mnich, J; Mohanty, G B; Muanza, G S; Muijs, A J M; Musicar, B; Musy, M; Nagy, S; Natale, S; Napolitano, M; Nessi-Tedaldi, F; Newman, H; Niessen, T; Nisati, A; Nowak, H; Ofierzynski, R A; Organtini, G; Palomares, C; Pandoulas, D; Paolucci, P; Paramatti, R; Passaleva, G; Patricelli, S; Paul, T; Pauluzzi, M; Paus, C; Pauss, Felicitas; Pedace, M; Pensotti, S; Perret-Gallix, D; Petersen, B; Piccolo, D; Pierella, F; Pioppi, M; Piroué, P A; Pistolesi, E; Plyaskin, V; Pohl, M; Pozhidaev, V; Pothier, J; Prokofiev, D O; Prokofev, D; Quartieri, J; Rahal-Callot, G; Rahaman, M A; Raics, P; Raja, N; Ramelli, R; Rancoita, P G; Ranieri, R; Raspereza, A V; Razis, P A; Ren, D; Rescigno, M; Reucroft, S; Riemann, S; Riles, K; Roe, B P; Romero, L; Rosca, A; Rosier-Lees, S; Roth, S; Rosenbleck, C; Roux, B; Rubio, Juan Antonio; Ruggiero, G; Rykaczewski, H; Sakharov, A; Saremi, S; Sarkar, S; Salicio, J; Sánchez, E; Sanders, M P; Schäfer, C; Shchegelskii, V; Schmidt-Kärst, S; Schmitz, D; Schopper, Herwig Franz; Schotanus, D J; Schwering, G; Sciacca, C; Servoli, L; Shevchenko, S; Shivarov, N; Shoutko, V; Shumilov, E; Shvorob, A V; Siedenburg, T; Son, D; Spillantini, P; Steuer, M; Stickland, D P; Stoyanov, B; Strässner, A; Sudhakar, K; Sultanov, G G; Sun, L Z; Sushkov, S V; Suter, H; Swain, J D; Szillási, Z; Tang, X W; Tarjan, P; Tauscher, Ludwig; Taylor, L; Tellili, B; Teyssier, D; Timmermans, C; Ting, Samuel C C; Ting, S M; Tonwar, S C; Tóth, J; Tully, C; Tung, K L; Ulbricht, J; Valente, E; Van, R T; De Walle, M; Veszpremi, V; Vesztergombi, G; Vetlitskii, I; Vicinanza, D; Viertel, Gert M; Villa, S; Vivargent, M; Vlachos, S; Vodopyanov, I; Vogel, H; Vogt, H; Vorobev, I; Vorobyov, A A; Wadhwa, M; Wallraff, W; Wang, X L; Wang, Z M; Weber, M; Wienemann, P; Wilkens, H; Wynhoff, S; Xia, L; Xu, Z Z; Yamamoto, J; Yang, B Z; Yang, C G; Yang, H J; Yang, M; Yeh, S C; Zalite, A; Zalite, Yu; Zhang, Z P; Zhao, J; Zhu, G Y; Zhu, R Y; Zhuang, H L; Zichichi, A; Zilizi, G; Zimmermann, B; Zöller, M

    2002-01-01

    Inclusive D^{*+-} production in two-photon collisions is studied with the L3 detector at LEP, using 683 pb^{-1} of data collected at centre-of-mass energies from 183 to 208 GeV. Differential cross sections are determined as functions of the transverse momentum and pseudorapidity of the D^{*+-} mesons in the kinematic region 1 GeV e^+e^-D^{*+-}X)$ in this kinematical region is measured and the sigma(e^+e^- ---> e^+e^- cc{bar}X) cross section is derived. The measurements are compared with next-to-leading order perturbative QCD calculations.

  9. Sound waves and resonances in electron-hole plasma

    Science.gov (United States)

    Lucas, Andrew

    2016-06-01

    Inspired by the recent experimental signatures of relativistic hydrodynamics in graphene, we investigate theoretically the behavior of hydrodynamic sound modes in such quasirelativistic fluids near charge neutrality, within linear response. Locally driving an electron fluid at a resonant frequency to such a sound mode can lead to large increases in the electrical response at the edges of the sample, a signature, which cannot be explained using diffusive models of transport. We discuss the robustness of this signal to various effects, including electron-acoustic phonon coupling, disorder, and long-range Coulomb interactions. These long-range interactions convert the sound mode into a collective plasmonic mode at low frequencies unless the fluid is charge neutral. At the smallest frequencies, the response in a disordered fluid is quantitatively what is predicted by a "momentum relaxation time" approximation. However, this approximation fails at higher frequencies (which can be parametrically small), where the classical localization of sound waves cannot be neglected. Experimental observation of such resonances is a clear signature of relativistic hydrodynamics, and provides an upper bound on the viscosity of the electron-hole plasma.

  10. Confinement of pyridinium hemicyanine dye within an anionic metal-organic framework for two-photon-pumped lasing

    Science.gov (United States)

    Yu, Jiancan; Cui, Yuanjing; Xu, Hui; Yang, Yu; Wang, Zhiyu; Chen, Banglin; Qian, Guodong

    2013-10-01

    Two-photon-pumped dye lasers are very important because of their applications in wavelength up-conversion, optical data storage, biological imaging and photodynamic therapy. Such lasers are very difficult to realize in the solid state because of the aggregation-caused quenching. Here we demonstrate a new two-photon-pumped micro-laser by encapsulating the cationic pyridinium hemicyanine dye into an anionic metal-organic framework (MOF). The resultant MOF⊃dye composite exhibits significant two-photon fluorescence because of the large absorption cross-section and the encapsulation-enhanced luminescent efficiency of the dye. Furthermore, the well-faceted MOF crystal serves as a natural Fabry-Perot resonance cavity, leading to lasing around 640 nm when pumped with a 1064-nm pulse laser. This strategy not only combines the crystalline benefit of MOFs and luminescent behaviour of organic dyes but also creates a new synergistic two-photon-pumped lasing functionality, opening a new avenue for the future creation of solid-state photonic materials and devices.

  11. Visualization of Distance Distribution from Pulsed Double Electron-Electron Resonance Data

    Energy Technology Data Exchange (ETDEWEB)

    Bowman, Michael K.; Maryasov, Alexander G.; Kim, Nak-Kyoon; DeRose, Victoria J.

    2004-01-01

    Double electron-electron resonance (DEER), also known as pulsed electron-electron double resonance (PELDOR), is a time-domain electron paramagnetic resonance method that can measure the weak dipole-dipole interactions between unpaired electrons. DEER has been applied to discrete pairs of free radicals in biological macromolecules and to clusters containing small numbers of free radicals in polymers and irradiated materials. The goal of such work is to determine the distance or distribution of distances between radicals, which is an underdetermined problem. That is, the spectrum of dipolar interactions can be readily calculated for any distribution of free radicals, but there are many, quite different distributions of radicals that could produce the same experimental dipolar spectrum. This paper describes two methods that are useful for approximating the distance distributions for the large subset of cases in which the mutual orientations of the free radicals are uncorrelated and the width of the distribution is more than a few percent of its mean. The first method relies on a coordinate transformation and is parameter free, while the second is based on iterative least-squares with Tikhonov regularization. Both methods are useful in DEER studies of spin labeled biomolecules containing more than two labels.

  12. Hard Two-Photon Contribution to Elastic Lepton-Proton Scattering Determined by the OLYMPUS Experiment

    Science.gov (United States)

    Henderson, B. S.; Ice, L. D.; Khaneft, D.; O'Connor, C.; Russell, R.; Schmidt, A.; Bernauer, J. C.; Kohl, M.; Akopov, N.; Alarcon, R.; Ates, O.; Avetisyan, A.; Beck, R.; Belostotski, S.; Bessuille, J.; Brinker, F.; Calarco, J. R.; Carassiti, V.; Cisbani, E.; Ciullo, G.; Contalbrigo, M.; de Leo, R.; Diefenbach, J.; Donnelly, T. W.; Dow, K.; Elbakian, G.; Eversheim, P. D.; Frullani, S.; Funke, Ch.; Gavrilov, G.; Gläser, B.; Görrissen, N.; Hasell, D. K.; Hauschildt, J.; Hoffmeister, Ph.; Holler, Y.; Ihloff, E.; Izotov, A.; Kaiser, R.; Karyan, G.; Kelsey, J.; Kiselev, A.; Klassen, P.; Krivshich, A.; Lehmann, I.; Lenisa, P.; Lenz, D.; Lumsden, S.; Ma, Y.; Maas, F.; Marukyan, H.; Miklukho, O.; Milner, R. G.; Movsisyan, A.; Murray, M.; Naryshkin, Y.; Perez Benito, R.; Perrino, R.; Redwine, R. P.; Rodríguez Piñeiro, D.; Rosner, G.; Schneekloth, U.; Seitz, B.; Statera, M.; Thiel, A.; Vardanyan, H.; Veretennikov, D.; Vidal, C.; Winnebeck, A.; Yeganov, V.; Olympus Collaboration

    2017-03-01

    The OLYMPUS Collaboration reports on a precision measurement of the positron-proton to electron-proton elastic cross section ratio, R2 γ , a direct measure of the contribution of hard two-photon exchange to the elastic cross section. In the OLYMPUS measurement, 2.01 GeV electron and positron beams were directed through a hydrogen gas target internal to the DORIS storage ring at DESY. A toroidal magnetic spectrometer instrumented with drift chambers and time-of-flight scintillators detected elastically scattered leptons in coincidence with recoiling protons over a scattering angle range of ≈20 ° to 80°. The relative luminosity between the two beam species was monitored using tracking telescopes of interleaved gas electron multiplier and multiwire proportional chamber detectors at 12°, as well as symmetric Møller or Bhabha calorimeters at 1.29°. A total integrated luminosity of 4.5 fb-1 was collected. In the extraction of R2 γ, radiative effects were taken into account using a Monte Carlo generator to simulate the convolutions of internal bremsstrahlung with experiment-specific conditions such as detector acceptance and reconstruction efficiency. The resulting values of R2 γ, presented here for a wide range of virtual photon polarization 0.456 <ɛ <0.978 , are smaller than some hadronic two-photon exchange calculations predict, but are in reasonable agreement with a subtracted dispersion model and a phenomenological fit to the form factor data.

  13. Handbook of multifrequency electron paramagnetic resonance data and techniques

    CERN Document Server

    Misra, Sushil K

    2014-01-01

    This handbook is aimed to deliver an up-to-date account of some of the recently developed experimental and theoretical methods in EPR, as well as a complete up-to-date listing of the experimentally determined values of multifrequency transition-ion spin Hamiltonian parameters by Sushil Misra, reported in the past 20 years, extending such a listing published by him in the Handbook on Electron Spin Resonance, volume 2. This extensive data tabulation makes up roughly 60% of the book`s content. It is complemented by the first full compilation of hyperfine splittings and g-factors for aminoxyl (nit

  14. Potential applications of an electron cyclotron resonance multicusp plasma source

    Energy Technology Data Exchange (ETDEWEB)

    Tsai, C.C.; Berry, L.A.; Gorbatkin, S.M.; Haselton, H.H.; Roberto, J.B.; Stirling, W.L. (Oak Ridge National Laboratory, Oak Ridge, TN (USA))

    1990-05-01

    An electron cyclotron resonance (ECR) multicusp plasmatron has been developed by feeding a multicusp bucket arc chamber with a compact ECR plasma source. This novel source produces large (about 25 cm diam), uniform (to within {plus minus}10%), dense ({gt}10{sup 11} cm{sup {minus}3}) plasmas of argon, helium, hydrogen, and oxygen. It has been operated to produce an oxygen plasma for etching 12.7 cm (5 in.) positive photoresist-coated silicon wafers with uniformity within {plus minus}8%. Results and potential applications of this new ECR plasma source for plasma processing of thin films are discussed.

  15. Electronically Tunable Fully Integrated Fractional-Order Resonator

    KAUST Repository

    Tsirimokou, Georgia

    2017-03-20

    A fully integrated implementation of a parallel fractional-order resonator which employs together a fractional order capacitor and a fractional-order inductor is proposed in this paper. The design utilizes current-controlled Operational Transconductance Amplifiers as building blocks, designed and fabricated in AMS 0:35m CMOS process, and based on a second-order approximation of a fractional-order differentiator/ integrator magnitude optimized in the range 10Hz–700Hz. An attractive benefit of the proposed scheme is its electronic tuning capability.

  16. Resonance electronic Raman scattering in rare earth crystals

    Energy Technology Data Exchange (ETDEWEB)

    Williams, G.M.

    1988-11-10

    The intensities of Raman scattering transitions between electronic energy levels of trivalent rare earth ions doped into transparent crystals were measured and compared to theory. A particle emphasis was placed on the examination of the effect of intermediate state resonances on the Raman scattering intensities. Two specific systems were studied: Ce/sup 3 +/(4f/sup 1/) in single crystals of LuPO/sub 4/ and Er/sup 3 +/(4f/sup 11/) in single crystals of ErPO/sub 4/. 134 refs., 92 figs., 33 tabs.

  17. Electron Paramagnetic Resonance Imaging and Spectroscopy of Polydopamine Radicals.

    Science.gov (United States)

    Mrówczyński, Radosław; Coy, L Emerson; Scheibe, Błażej; Czechowski, Tomasz; Augustyniak-Jabłokow, Maria; Jurga, Stefan; Tadyszak, Krzysztof

    2015-08-13

    A thorough investigation of biomimetic polydopamine (PDA) by Electron Paramagnetic Resonance (EPR) is shown. In addition, temperature dependent spectroscopic EPR data are presented in the range 3.8-300 K. Small discrepancies in magnetic susceptibility behavior are observed between previously reported melanin samples. These variations were attributed to thermally acitivated processes. More importantly, EPR spatial-spatial 2D imaging of polydopamine radicals on a phantom is presented for the first time. In consequence, a new possible application of polydopamine as EPR imagining marker is addressed.

  18. Two-Photon Holographic Stimulation of ReaChR

    Science.gov (United States)

    Chaigneau, Emmanuelle; Ronzitti, Emiliano; Gajowa, Marta A.; Soler-Llavina, Gilberto J.; Tanese, Dimitrii; Brureau, Anthony Y. B.; Papagiakoumou, Eirini; Zeng, Hongkui; Emiliani, Valentina

    2016-01-01

    Optogenetics provides a unique approach to remotely manipulate brain activity with light. Reaching the degree of spatiotemporal control necessary to dissect the role of individual cells in neuronal networks, some of which reside deep in the brain, requires joint progress in opsin engineering and light sculpting methods. Here we investigate for the first time two-photon stimulation of the red-shifted opsin ReaChR. We use two-photon (2P) holographic illumination to control the activation of individually chosen neurons expressing ReaChR in acute brain slices. We demonstrated reliable action potential generation in ReaChR-expressing neurons and studied holographic 2P-evoked spiking performances depending on illumination power and pulse width using an amplified laser and a standard femtosecond Ti:Sapphire oscillator laser. These findings provide detailed knowledge of ReaChR's behavior under 2P illumination paving the way for achieving in depth remote control of multiple cells with high spatiotemporal resolution deep within scattering tissue. PMID:27803649

  19. High-order dispersion effects in two-photon interference

    Science.gov (United States)

    Mazzotta, Zeudi; Cialdi, Simone; Cipriani, Daniele; Olivares, Stefano; Paris, Matteo G. A.

    2016-12-01

    Two-photon interference and Hong-Ou-Mandel (HOM) effect are relevant tools for quantum metrology and quantum information processing. In optical coherence tomography, the HOM effect is exploited to achieve high-resolution measurements with the width of the HOM dip being the main parameter. On the other hand, applications like dense coding require high-visibility performance. Here we address high-order dispersion effects in two-photon interference and study, theoretically and experimentally, the dependence of the visibility and the width of the HOM dip on both the pump spectrum and the downconverted photon spectrum. In particular, a spatial light modulator is exploited to experimentally introduce and manipulate a custom phase function to simulate the high-order dispersion effects. Overall, we show that it is possible to effectively introduce high-order dispersion effects on the propagation of photons and also to compensate for such effect. Our results clarify the role of the different dispersion phenomena and pave the way for optimization procedures in quantum technological applications involving PDC photons and optical fibers.

  20. Relativistic (Z alpha)^2-Corrections and Leading Quantum Electrodynamic Corrections to the Two-Photon Decay Rate of Ionic States

    CERN Document Server

    Wundt, B J; 10.1103/PhysRevA.80.022505

    2009-01-01

    We calculate the relativistic corrections of relative order (Z alpha)^2$ to the two-photon decay rate of higher excited S and D states in ionic atomic systems, and we also evaluate the leading radiative corrections of relative order alpha (Z alpha)^2 ln[(Z alpha)^(-2)]. We thus complete the theory of the two-photon decay rates up to relative order alpha^3 ln(alpha). An approach inspired by nonrelativistic quantum electrodynamics is used. We find that the corrections of relative order (Z alpha)^2 to the two-photon decay are given by the zitterbewegung, the spin-orbit coupling and by relativistic corrections to the electron mass, and by quadrupole interactions. We show that all corrections are separately gauge-invariant with respect to a "hybrid" transformation from velocity to length gauge, where the gauge transformation of the wave function is neglected. The corrections are evaluated for the two-photon decay from 2S, 3S, 3D, and 4S states in one-electron (hydrogenlike) systems, with 1S and 2S final states.

  1. A [111]-Cut Si Hemisphere Two-Photon Response Photodetector

    Institute of Scientific and Technical Information of China (English)

    LIU Xiu-Huan; CHEN Zhan-Guo; JIA Gang; WANG Hai-Yan; GAO Yan-Jun; LI Yi1

    2011-01-01

    Properties of two-photon response in a [lll]-cut nearly-intrinsic Si hemisphere photodetector are studied. The measured photocurrent of the photodetector responding to the 1.32μm continuous wave laser shows a quadratic dependence on the coupled optical power and is saturated with the bias voitage. Also, the photocurrent is independent of polarization. Such properties are in good agreement with the theory of two-photon absorption. The isotropic photocurrent generated from the [lll]-cut Si hemisphere is compared to the anisotropic one induced in the [110]-cut Si sample and the ratio of Xxxxx /Xxxyy for silicon performing at 1.32μm is calculated to be 2.4 via the fitted function of the anisotropic photocurrent from the [110]-cut sample.%Properties of two-photon response in a [111]-cut nearly-intrinsic Si hemisphere photodetector are studied.The measured photocurrent of the photodetector responding to the 1.32 μm continuous wave laser shows a quadratic dependence on the coupled optical power and is saturated with the bias voltage.Also,the photocurrent is independent of polarization.Such properties are in good agreement with the theory of two-photon absorption.The isotropic photocurrent generated from the [111]-cut Si hemisphere is compared to the anisotropic one induced in the [110]-cut Si sample and the ratio of Xxxxx /Xxxyy for silicon performing at 1.32μm is calculated to be 2.4via the fitted function of the anisotropic photocurrent from the [110]-cut sample.Silicon materials have a variety of applications in microelectronics and silicon optoelectronics and are still attractive to relevant researchers.Commercial Si photodetectors are largely designed based on singlephoton absorption (SPA).However,nonlinear characteristics have been exhibited in silicon devices.Specifically,two-photon absorption (TPA) has attracted much attention in such devices of Si p-n and p-i-n photodiodes,Si waveguides and Si avalanche diodes,etc.for the autocorrelation measurements of

  2. Relativistic surfatron process for Landau resonant electrons in radiation belts

    CERN Document Server

    Osmane, A

    2014-01-01

    Recent theoretical studies of the nonlinear wave-particle interactions for relativistic particles have shown that Landau resonant orbits could be efficiently accelerated along the mean background magnetic field for propagation angles $\\theta$ in close proximity to a critical propagation $\\theta_\\textrm{c}$ associated with a Hopf--Hopf bifurcation condition. In this report, we extend previous studies to reach greater modeling capacities for the study of electrons in radiation belts by including longitudinal wave effects and inhomogeneous magnetic fields. We find that even though both effects can limit the surfatron acceleration of electrons in radiation belts, gains in energy of the order of 100 keV, taking place on the order of ten milliseconds, are sufficiently strong for the mechanism to be relevant to radiation belt dynamics.

  3. Resonance enhanced electron impact excitation of Cu-like gadolinium

    Science.gov (United States)

    Li, Shuang; Si, Ran; Zhang, Chun yu; Guo, Xue Ling; Chen, Zhan Bin; Wang, Kai; Chen, Chong Yang; Yan, Jun

    2017-06-01

    Employing the independent processes and isolated resonances approximation using distorted-waves (IPIRDW), we perform a large calculation and a detail investigation on resonance enhanced electron impact excitation (EIE) among the 27 singly excited levels from n ≤ 6 configurations of Cu-like gadolinium (Gd, Z = 64). We take into account the RE contributions from both the relevant Zn-like doubly excited series [Ne]3 l 18 n' l' n'' l'' with n' = 4-7, and the series [Ne]3 l 174 l4 l' n'' l''. Results show that the RE contributions are significant and enhance effective collision strengths ( Υ) of certain excitations by even up to an order of magnitude at low temperature (105.8 K), and still important at relative high temperature (106.8 K), where the fraction abundance of Gd XXXVI is expected at peak. We expect present resonance enhanced EIE results among the 27 levels, which is the first results with the RE contributions from n = 3 → 4 core excitation for Cu-like isoelectronic sequence, are more accurate due to our consideration of RE contributions for this ion for the first time.

  4. A superheterodyne spectrometer for electronic paramagnetic. Resonance; Spectrometre superheterodyne de resonance paramagnetique electronique

    Energy Technology Data Exchange (ETDEWEB)

    Laffon, J.L. [Commissariat a l' Energie Atomique, Grenoble (France). Centre d' Etudes Nucleaires

    1963-12-15

    After a few generalities about electron paramagnetic resonance, a consideration of different experimental techniques authorises the choice of a particular type of apparatus. An EPR superheterodyne spectrometer built in the laboratory and having a novel circuit is described in detail. With this apparatus, many experimental results have been obtained and some of these are described as example. (author) [French] Apres quelques generalites sur le phenomene de resonance paramagnetique electronique, une synthese des differentes techniques experimentales, permet de fixer le choix d'un type d'appareillage. Un spectrometre de RPE superheterodyne realise en laboratoire et comportant un circuit original est expose dans le detail. Cet appareil a permis de nombreux resultats experimentaux dont quelques-uns sont decrits a titre d'exemple. (auteur)

  5. A simple approach for measuring FRET in fluorescent biosensors using two-photon microscopy.

    Science.gov (United States)

    Day, Richard N; Tao, Wen; Dunn, Kenneth W

    2016-11-01

    Genetically encoded fluorescent protein (FP)-based biosensor probes are useful tools for monitoring cellular events in living cells and tissues. Because these probes were developed for one-photon excitation approaches, their broad two-photon excitation (2PE) and poorly understood photobleaching characteristics have made their implementation in studies using two-photon laser-scanning microscopy (TPLSM) challenging. Here we describe a protocol that simplifies the use of Förster resonance energy transfer (FRET)-based biosensors in TPLSM. First, the TPLSM system is evaluated and optimized using FRET standards expressed in living cells, which enables the determination of spectral bleed-through (SBT) and the confirmation of FRET measurements from the known standards. Next, we describe how to apply the approach experimentally using a modified version of the A kinase activity reporter (AKAR) protein kinase A (PKA) biosensor as an example-first in cells in culture and then in hepatocytes in the liver of living mice. The microscopic imaging can be accomplished in a day in laboratories that routinely use TPLSM.

  6. Polarization-entangled twin photons from two-photon quantum-dot emission

    Science.gov (United States)

    Heinze, Dirk; Zrenner, Artur; Schumacher, Stefan

    2017-06-01

    Semiconductor quantum dots are promising sources for polarization-entangled photons. As an alternative to the usual cascaded biexciton-exciton emission, direct two-photon emission from the biexciton can be used. With a high-quality optical resonator tuned to half the biexciton energy, a large proportion of the photons can be steered into the two-photon emission channel. In this case the degree of polarization entanglement is inherently insensitive to the exciton fine-structure splitting. In the present work we analyze the biexciton emission with particular emphasis on the influence of coupling of the quantum-dot cavity system to its environment. Especially for a high-quality cavity, the coupling to the surrounding semiconductor material can open up additional phonon-assisted decay channels. Our analysis demonstrates that with the cavity tuned to half the biexciton energy, the potentially detrimental influence of the phonons on the polarization entanglement is strongly suppressed—high degrees of entanglement can still be achieved. We further discuss spectral properties and statistics of the emitted twin photons.

  7. Measurement of Ultra-Short Single-Photon Pulse Duration with Two-Photon Interference

    Institute of Scientific and Technical Information of China (English)

    LV Fan; SUN Fang-Wen; ZOU Chang-Ling; HAN Zheng-Fu; GUO Guang-Can

    2011-01-01

    We proposed a protocol of measuring the duration of ultra-short single-photon pulse with two-photon interference.The pulse duration can be obtained from the width of the visibility of two-photon Hong-Ou-Mandel interference or the indistinguishability of the two photons. Moreover, the shape of a single-photon pulse can be measured with ultra-short single-photon pulses through the two-photon interference.%@@ We proposed a protocol of measuring the duration of ultra-short single-photon pulse with two-photon interference.The pulse duration can be obtained from the width of the visibility of two-photon Hong-Ou-Mandel interference or the indistinguishability of the two photons.Moreover, the shape of a single-photon pulse can be measured with ultra-short single-photon pulses through the two-photon interference.

  8. A microwave resonator for limiting depth sensitivity for electron paramagnetic resonance spectroscopy of surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Sidabras, Jason W.; Varanasi, Shiv K.; Hyde, James S. [Department of Biophysics, Medical College of Wisconsin, Milwaukee, Wisconsin 53211 (United States); Mett, Richard R. [Department of Biophysics, Medical College of Wisconsin, Milwaukee, Wisconsin 53211 (United States); Department of Physics and Chemistry, Milwaukee School of Engineering, Milwaukee, Wisconsin 53202 (United States); Swarts, Steven G. [Department of Radiation Oncology, University of Florida, Gainesville, Florida, 32610 (United States); Swartz, Harold M. [Department of Radiology, Geisel Medical School at Dartmouth, Hanover, New Hampshire 03755 (United States)

    2014-10-15

    A microwave Surface Resonator Array (SRA) structure is described for use in Electron Paramagnetic Resonance (EPR) spectroscopy. The SRA has a series of anti-parallel transmission line modes that provides a region of sensitivity equal to the cross-sectional area times its depth sensitivity, which is approximately half the distance between the transmission line centers. It is shown that the quarter-wave twin-lead transmission line can be a useful element for design of microwave resonators at frequencies as high as 10 GHz. The SRA geometry is presented as a novel resonator for use in surface spectroscopy where the region of interest is either surrounded by lossy material, or the spectroscopist wishes to minimize signal from surrounding materials. One such application is in vivo spectroscopy of human finger-nails at X-band (9.5 GHz) to measure ionizing radiation dosages. In order to reduce losses associated with tissues beneath the nail that yield no EPR signal, the SRA structure is designed to limit depth sensitivity to the thickness of the fingernail. Another application, due to the resonator geometry and limited depth penetration, is surface spectroscopy in coating or material science. To test this application, a spectrum of 1.44 μM of Mg{sup 2+} doped polystyrene 1.1 mm thick on an aluminum surface is obtained. Modeling, design, and simulations were performed using Wolfram Mathematica (Champaign, IL; v. 9.0) and Ansys High Frequency Structure Simulator (HFSS; Canonsburg, PA; v. 15.0). A micro-strip coupling circuit is designed to suppress unwanted modes and provide a balanced impedance transformation to a 50 Ω coaxial input. Agreement between simulated and experimental results is shown.

  9. A microwave resonator for limiting depth sensitivity for electron paramagnetic resonance spectroscopy of surfaces

    Science.gov (United States)

    Sidabras, Jason W.; Varanasi, Shiv K.; Mett, Richard R.; Swarts, Steven G.; Swartz, Harold M.; Hyde, James S.

    2014-10-01

    A microwave Surface Resonator Array (SRA) structure is described for use in Electron Paramagnetic Resonance (EPR) spectroscopy. The SRA has a series of anti-parallel transmission line modes that provides a region of sensitivity equal to the cross-sectional area times its depth sensitivity, which is approximately half the distance between the transmission line centers. It is shown that the quarter-wave twin-lead transmission line can be a useful element for design of microwave resonators at frequencies as high as 10 GHz. The SRA geometry is presented as a novel resonator for use in surface spectroscopy where the region of interest is either surrounded by lossy material, or the spectroscopist wishes to minimize signal from surrounding materials. One such application is in vivo spectroscopy of human finger-nails at X-band (9.5 GHz) to measure ionizing radiation dosages. In order to reduce losses associated with tissues beneath the nail that yield no EPR signal, the SRA structure is designed to limit depth sensitivity to the thickness of the fingernail. Another application, due to the resonator geometry and limited depth penetration, is surface spectroscopy in coating or material science. To test this application, a spectrum of 1.44 μM of Mg2+ doped polystyrene 1.1 mm thick on an aluminum surface is obtained. Modeling, design, and simulations were performed using Wolfram Mathematica (Champaign, IL; v. 9.0) and Ansys High Frequency Structure Simulator (HFSS; Canonsburg, PA; v. 15.0). A micro-strip coupling circuit is designed to suppress unwanted modes and provide a balanced impedance transformation to a 50 Ω coaxial input. Agreement between simulated and experimental results is shown.

  10. A microwave resonator for limiting depth sensitivity for electron paramagnetic resonance spectroscopy of surfaces.

    Science.gov (United States)

    Sidabras, Jason W; Varanasi, Shiv K; Mett, Richard R; Swarts, Steven G; Swartz, Harold M; Hyde, James S

    2014-10-01

    A microwave Surface Resonator Array (SRA) structure is described for use in Electron Paramagnetic Resonance (EPR) spectroscopy. The SRA has a series of anti-parallel transmission line modes that provides a region of sensitivity equal to the cross-sectional area times its depth sensitivity, which is approximately half the distance between the transmission line centers. It is shown that the quarter-wave twin-lead transmission line can be a useful element for design of microwave resonators at frequencies as high as 10 GHz. The SRA geometry is presented as a novel resonator for use in surface spectroscopy where the region of interest is either surrounded by lossy material, or the spectroscopist wishes to minimize signal from surrounding materials. One such application is in vivo spectroscopy of human finger-nails at X-band (9.5 GHz) to measure ionizing radiation dosages. In order to reduce losses associated with tissues beneath the nail that yield no EPR signal, the SRA structure is designed to limit depth sensitivity to the thickness of the fingernail. Another application, due to the resonator geometry and limited depth penetration, is surface spectroscopy in coating or material science. To test this application, a spectrum of 1.44 μM of Mg(2+) doped polystyrene 1.1 mm thick on an aluminum surface is obtained. Modeling, design, and simulations were performed using Wolfram Mathematica (Champaign, IL; v. 9.0) and Ansys High Frequency Structure Simulator (HFSS; Canonsburg, PA; v. 15.0). A micro-strip coupling circuit is designed to suppress unwanted modes and provide a balanced impedance transformation to a 50 Ω coaxial input. Agreement between simulated and experimental results is shown.

  11. Two-photon or higher-order absorbing optical materials and methods of use

    Science.gov (United States)

    Marder, Seth (Inventor); Perry, Joseph (Inventor)

    2012-01-01

    Compositions capable of simultaneous two-photon absorption and higher order absorptivities are provided. Compounds having a donor-pi-donor or acceptor-pi-acceptor structure are of particular interest, where the donor is an electron donating group, acceptor is an electron accepting group, and pi is a pi bridge linking the donor and/or acceptor groups. The pi bridge may additionally be substituted with electron donating or withdrawing groups to alter the absorptive wavelength of the structure. Also disclosed are methods of generating an excited state of such compounds through optical stimulation with light using simultaneous absorption of photons of energies individually insufficient to achieve an excited state of the compound, but capable of doing so upon simultaneous absorption of two or more such photons. Applications employing such methods are also provided, including controlled polymerization achieved through focusing of the light source(s) used.

  12. Electron spin resonance and electron nuclear double resonance of photogenerated polarons in polyfluorene and its fullerene composite

    Science.gov (United States)

    Marumoto, K.; Kato, M.; Kondo, H.; Kuroda, S.; Greenham, N. C.; Friend, R. H.; Shimoi, Y.; Abe, S.

    2009-06-01

    Electron spin resonance (ESR) and electron-nuclear double resonance (ENDOR) of photogenerated polarons in poly(9,9-dioctylfluorene) (PFO) and its composite with fullerene (C60) using variable photoexcitation energy up to 4.1 eV are reported. For PFO, a light-induced ESR (LESR) signal (g=2.003) is observed below 60 K, and its transient response and excitation spectrum indicate that the observed spins are photogenerated polarons on PFO. For the PFO-C60 composite, two LESR signals of photogenerated positive polarons on PFO (g1=2.003) and radical anions on C60 (g2=1.999) , respectively, are observed below 120 K, which are caused by photoinduced electron transfer from PFO to C60 . A remarkable enhancement of the LESR signals in the excitation spectrum at ˜2.8eV is observed compared with the case of pure PFO. The bimolecular-recombination kinetics of photogenerated charge carriers in the composite are confirmed by the dependence of the LESR on excitation-light intensity and by the decay dynamics. Light-induced ENDOR (LENDOR) signals are clearly observed for excitation around 2.8 eV owing to the highly efficient photoinduced electron transfer in the composite. Broad LENDOR shifts directly reflect the spin-density distribution of the polarons in PFO. We have determined its maximum shift using LENDOR-induced ESR, and have evaluated the maximum spin density on the carbon site coupled to the proton as 0.032. This value is consistent with the theoretical result obtained by Pariser-Parr-Pople (PPP) model, where the spatial extent of the polarons is calculated as ˜3 monomer units of PFO. The calculated LESR spectra of PFO based on the PPP model are consistent with the experimental spectra, which confirm the above spatial extension of the polaron in PFO.

  13. 540--900 nm photodissociation of 300 K NCNO: One- and two-photon processes

    Energy Technology Data Exchange (ETDEWEB)

    Nadler, I.; Pfab, J.; Reisler, H.; Wittig, C.

    1984-07-15

    The laser photodissociation of 300 K NCNO throughout the region 540--900 nm is reported, and both 1- and 2-photon processes are discussed. By monitoring CN fragments produced via the 1-photon process, we show that with photolysis wavelengths >592 nm, dissociation occurs predominantly by exciting NCNO ''hot bands.'' At shorter photolysis wavelengths, dissociation from the ground vibrational state of NCNO is observed as well, but the contributions from hot bands are still manifest in high CN rotational levels which are energetically inaccessible from the ground state (D/sub 0/ = 48.8 kcal mol/sup -1/). Energy distributions in the CN fragments were determined for excess energies up to 1800 cm/sup -1/, and are in agreement with phase space theory calculations and a vibrational predissociation mechanism. In addition, throughout the region 620--900 nm, stepwise two-photon photodissociation proceeds using the A /sup 1/A'' state as a gateway, and results in rotationally and vibrationally ''hot'' CN fragments. The hot CN fragment yield vs photolysis wavelength shows peaks which correspond exactly to peaks in the NCNO absorption spectrum, allowing us to obtain high resolution spectra of the A /sup 1/A''reverse arrow X /sup 1/A' absorption system. The one- and two-photon processes are in competition, and the latter disappears at wavelengths where one-photon photodissociation of NCNO via its ground vibrational level sets in. The nature of the electronic states involved in the one- and two-photon processes is also discussed.

  14. Clinical multiphoton tomography and clinical two-photon microendoscopy

    Science.gov (United States)

    König, Karsten; Bückle, Rainer; Weinigel, Martin; Elsner, Peter; Kaatz, Martin

    2009-02-01

    We report on applications of high-resolution clinical multiphoton tomography based on the femtosecond laser system DermaInspectTM with its flexible mirror arm in Australia, Asia, and Europe. Applications include early detection of melanoma, in situ tracing of pharmacological and cosmetical compounds including ZnO nanoparticles in the epidermis and upper dermis, the determination of the skin aging index SAAID as well as the study of the effects of anti-aging products. In addition, first clinical studies with novel rigid high-NA two-photon 1.6 mm GRIN microendoscopes have been conducted to study the effect of wound healing in chronic wounds (ulcus ulcera) as well as to perform intrabody imaging with subcellular resolution in small animals.

  15. Two-Photon Micromaser with Initial Atomic Coherence

    Institute of Scientific and Technical Information of China (English)

    SUN Wei-Hui; DU Si-De; CHEN Xiao-Shuang

    2005-01-01

    @@ We investigate the quantum dynamics ora two-photon micromaser pumped by atoms injected in the superpositionstate of the upper and intermediate levels. We simulate a master equation governing the system by the MonteCarlo wavefunction approach and analyse the steady-state behaviour as a function of the atomic transit time.The atomic coherence can effectively enhance the intensity and sub-Poissonian of the cavity field as comparedwith the atomic mixture. It is also discovered that the phase of the cavity field can be shifted by adjusting thedetuning between the atom and field. This result shows that it is possible to manipulate the phase of the cavityfield by detuning, due to atomic coherence.

  16. Whole brain imaging with Serial Two-Photon Tomography

    Directory of Open Access Journals (Sweden)

    Stephen P Amato

    2016-03-01

    Full Text Available Imaging entire mouse brains at submicron resolution has historically been a challenging undertaking and largely confined to the province of dedicated atlasing initiatives. The has limited systematic investigations into important areas of neuroscience, such as neural circuits, brain mapping and neurodegeneration. In this paper, we describe in detail Serial Two-Photon (STP tomography, a robust, reliable method for imaging entire brains with histological detail. We provide examples of how the basic methodology can be extended to other imaging modalities, such as optical coherence tomography, in order to provide unique contrast mechanisms. Furthermore we provide a survey of the research that STP tomography has enabled in the field of neuroscience, provide examples of how this technology enables quantitative whole brain studies, and discuss the current limitations of STP tomography-based approaches

  17. Two-photon assisted clock comparison to picosecond precision

    CERN Document Server

    Zhang, Shi-Wei; Yao, Yin-Ping; Wan, Ren-Gang; Zhang, Tong-Yi

    2015-01-01

    We have experimentally demonstrated a clock comparison scheme utilizing time-correlated photon pairs generated from the spontaneous parametric down conversion process of a laser pumped beta-barium borate crystal. The coincidence of two-photon events are analyzed by the cross correlation of the two time stamp sequences. Combining the coarse and fine part of the time differences at different resolutions, a 64 ps precision for clock synchronization has been realized. We also investigate the effects of hardware devices used in the system on the precision of clock comparison. The results indicate that the detector's time jitter and the background noise will degrade the system performance. With this method, comparison and synchronization of two remote clocks could be implemented with a precision at the level of a few tens of picoseconds.

  18. High contrast two-photon imaging of fingermarks

    Science.gov (United States)

    Stoltzfus, Caleb R.; Rebane, Aleksander

    2016-04-01

    Optically-acquired fingermarks are widely used as evidence across law enforcement agencies as well as in the courts of law. A common technique for visualizing latent fingermarks on nonporous surfaces consists of cyanoacrylate fuming of the fingerprint material, followed by impregnation with a fluorescent dye, which under ultra violet (UV) illumination makes the fingermarks visible and thus accessible for digital recording. However, there exist critical circumstances, when the image quality is compromised due to high background scattering, high auto-fluorescence of the substrate material, or other detrimental photo-physical and photo-chemical effects such as light-induced damage to the sample. Here we present a novel near-infrared (NIR), two-photon induced fluorescence imaging modality, which significantly enhances the quality of the fingermark images, especially when obtained from highly reflective and/or scattering surfaces, while at the same time reducing photo-damage to sensitive forensic samples.

  19. Anomalous two-photon spectral features in warm rubidium vapor

    Science.gov (United States)

    Perrella, C.; Light, P. S.; Milburn, T. J.; Kielpinski, D.; Stace, T. M.; Luiten, A. N.

    2016-09-01

    We report observation of anomalous fluorescence spectral features in the environs of a two-photon transition in a rubidium vapor when excited with two different wavelength lasers that are both counterpropagating through the vapor. These features are characterized by an unusual trade-off between the detunings of the driving fields. Three different hypothetical processes are presented to explain the observed spectra: a simultaneous three-atom and four-photon collision, a four-photon excitation involving a light field produced via amplified spontaneous emission, and population pumping perturbing the expected steady-state spectra. Numerical modeling of each hypothetical process is presented, supporting the population pumping process as the most plausible mechanism.

  20. Two-photon transition form factor of c ¯ quarkonia

    Science.gov (United States)

    Chen, Jing; Ding, Minghui; Chang, Lei; Liu, Yu-xin

    2017-01-01

    The two-photon transition of c ¯c quarkonia are studied within a covariant approach based on the consistent truncation scheme of the quantum chromodynamics Dyson-Schwinger equation for the quark propagator and the Bethe-Salpeter equation for the mesons. We find the decay widths of ηc→γ γ and χc 0 ,2→γ γ in good agreement with experimental data. The obtained transition form factor of ηc→γ γ* for a wide range of spacelike photon-momentum-transfer squared is also in agreement with the experimental findings of the BABAR experiment. As a by-product, the decay widths of ηb,χb 0 ,2→γ γ and the transition form factor of ηb,χc 0 ,b 0→γ γ* are predicted, which await experimental testing.

  1. Nuclear two-photon decay in 0 +→0 + transitions

    Science.gov (United States)

    Kramp, J.; Habs, D.; Kroth, R.; Music, M.; Schirmer, J.; Schwalm, D.; Broude, C.

    1987-11-01

    The two-photon decay of the first excited 0 + state of 16O has been measured using the Heidelberg-Darmstadt crystal ball. A branching ratio of {Γ γγ}/{Γ tot} = (6.6±0.5) · 10 -4 was obtained. As in the cases of 40Ca and 90Zr previously reported by us, the 2γ decay of 16O proceeds via double E1 and M1 transitions of similar strength; the evidence is the observed interference term in the 2γ angular correlation. The ratio of the matrix elements {α E1 }/{χ} for 16O was restricted to the two inverse values (-6.2±1.5) or (-0.16±0.04). An interpretation of 2γ matrix elements observed for 16O, 40Ca and 90Zr in terms of the electric polarizabilities and magnetic susceptibility is given leading to a qualitative understanding of this decay mode.

  2. Nanoshells for in vivo imaging using two-photon excitation microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Gao Liang; Nammalvar, Vengadesan [Department of Bioengineering, Rice University, Houston, TX 77005 (United States); Vadakkan, Tegy J, E-mail: lg3@rice.edu, E-mail: venkyn@rice.edu [Department of Molecular Physiology and Biophysics, Baylor College of Medicine, Houston, TX 77030 (United States)

    2011-09-07

    Gold nanoshells have been intensively investigated and applied to various biomedical fields because of their flexible optical tunability and biological compatibility. They hold great potential to serve as luminescent contrast agents excitable with near-infrared (NIR) lasers. In this paper, we describe the development of nanoshells with a peak of plasmon resonance at 800 nm and their subsequent use for in vivo blood vessel imaging using two-photon excitation microscopy at an excitation wavelength of 750 nm. We were able to image single nanoshell particles in blood vessels and generate optical contrast for blood vessel structure using luminescent signals. These results confirm the feasibility of engineering nanoshells with controlled optical properties for single-particle-based in vivo imaging.

  3. Nanoshells for in vivo imaging using two-photon excitation microscopy.

    Science.gov (United States)

    Gao, Liang; Vadakkan, Tegy J; Nammalvar, Vengadesan

    2011-09-07

    Gold nanoshells have been intensively investigated and applied to various biomedical fields because of their flexible optical tunability and biological compatibility. They hold great potential to serve as luminescent contrast agents excitable with near-infrared (NIR) lasers. In this paper, we describe the development of nanoshells with a peak of plasmon resonance at 800 nm and their subsequent use for in vivo blood vessel imaging using two-photon excitation microscopy at an excitation wavelength of 750 nm. We were able to image single nanoshell particles in blood vessels and generate optical contrast for blood vessel structure using luminescent signals. These results confirm the feasibility of engineering nanoshells with controlled optical properties for single-particle-based in vivo imaging.

  4. Electric field allowed molecular transitions for one and two photon excitation microscopy.

    Science.gov (United States)

    Mondal, Partha Pratim; Diaspro, Alberto

    2008-07-01

    We propose an excitation technique for observing single and two photon excitation in those molecules for which such transitions are forbidden by the selection rules. This is possible by the application of an external electric field that perturbs the molecular orbitals, thereby resulting in a significant shift of energy levels. Such a shift of energy levels may bring those levels in resonance with the radiation field which is normally forbidden by selection rules. Further, parity of the these states may significantly improve the emission process. The external electric field results in the mixing of excited (short lifetime) and metastable states (long lifetime), thus reducing the lifetime of metastable (or near metastable) states. This may provide an effective channel for allowing transition from the metastable states. An application of electric field may result in the excitation of poorly excitable biomolecules. This excitation technique may find applications in single- and multi-photon fluorescence microscopy, bioimaging and optical devices.

  5. Theoretical analysis on two-photon absorption spectroscopy in a confined four-level atomic system

    Institute of Scientific and Technical Information of China (English)

    Yuanyuan Li; Jintao Bai; Li Li; Yanpeng Zhang; Xun Hou

    2009-01-01

    We investigate theoretically two-photon absorption spectroscopy modified by a control field in a confined Y-type four-level system. Dicke-narrowing effect occurs both in two-photon absorption lines and the dips of transparency against two-photon absorption due to enhanced contribution of slow atoms. We also find that the suppression and the enhancement of two-photon absorption can be modified by changing the strength of the control field and the detuning of three laser fields. This control of two-photon absorption may have some applications in information processing and optical devices.

  6. Two-photon STED spectral determination for a new V-shaped organic fluorescent probe with efficient two-photon absorption.

    Science.gov (United States)

    Belfield, Kevin D; Bondar, Mykhailo V; Morales, Alma R; Padilha, Lazaro A; Przhonska, Olga V; Wang, Xuhua

    2011-10-24

    Two-photon stimulated emission depletion (STED) cross sections were determined over a broad spectral range for a novel two-photon absorbing organic molecule, representing the first such report. The synthesis, comprehensive linear photophysical, two-photon absorption (2PA), and stimulated emission properties of a new fluorene-based compound, (E)-2-{3-[2-(7-(diphenylamino)-9,9-diethyl-9H-fluoren-2-yl)vinyl]-5-methyl-4-oxocyclohexa-2,5-dienylidene} malononitrile (1), are presented. Linear spectral parameters, including excitation anisotropy and fluorescence lifetimes, were obtained over a broad range of organic solvents at room temperature. The degenerate two-photon absorption (2PA) spectrum of 1 was determined with a combination of the direct open-aperture Z-scan and relative two-photon-induced fluorescence methods using 1 kHz femtosecond excitation. The maximum value of the 2PA cross section ~1700 GM was observed in the main, long wavelength, one-photon absorption band. One- and two-photon stimulated emission spectra of 1 were obtained over a broad spectral range using a femtosecond pump-probe technique, resulting in relatively high two-photon stimulated emission depletion cross sections (~1200 GM). A potential application of 1 in bioimaging was demonstrated through one- and two-photon fluorescence microscopy images of HCT 116 cells incubated with micelle-encapsulated dye.

  7. Experimental observation of electron bounce resonance through electron energy distribution measurement in a finite size inductively coupled plasma

    Energy Technology Data Exchange (ETDEWEB)

    Gu, Seuli [Department of Nanoscale Semiconductor Engineering, Hanyang University, 222 Wangsimni-ro, Seongdong-gu, Seoul 04763 (Korea, Republic of); Kang, Hyun-Ju; Kim, Yu-Sin; Chang, Yoon-Min; Chung, Chin-Wook, E-mail: joykang@hanyang.ac.kr [Department of Electrical Engineering, Hanyang University, 222 Wangsimni-ro, Seongdong-gu, Seoul 04763 (Korea, Republic of); Kwon, Deuk-Chul [Plasma Technology Research Center, National Fusion Research Institute, 169-148 Gwahak-ro, Yuseong-gu, Daejeon 34133 (Korea, Republic of)

    2016-06-15

    The electron bounce resonance was experimentally investigated in a low pressure planar inductively coupled plasma. The electron energy probability functions (EEPFs) were measured at different chamber heights and the energy diffusion coefficients were calculated by the kinetic model. It is found that the EEPFs begin to flatten at the first electron bounce resonance condition, and the plateau shifts to a higher electron energy as the chamber height increases. The plateau which indicates strong electron heating corresponds not only to the electron bounce resonance condition but also to the peaks of the first component of the energy diffusion coefficients. As a result, the plateau formation in the EEPFs is mainly due to the electron bounce resonance in a finite inductive discharge.

  8. Electron-positron pair production by an electron in a magnetic field in the resonant case

    CERN Document Server

    Novak, O P

    2012-01-01

    Resonant e+e- pair production by an electron in a magnetic field near the process threshold has been analytically studied. Using the Nikishov's theorem an estimation of the number of events has been made in the magnetic field equivalent to laser wave in the SLAC experiment [D.Burke et.al. Phys. Rev. Lett.79, 1626 (1997)]. The obtained estimation is in reasonable agreement with the experimental data.

  9. Electron cyclotron resonance breakdown studies in a linear plasma system

    Indian Academy of Sciences (India)

    Vipin K Yadav; K Sathyanarayana; D Bora

    2008-03-01

    Electron cyclotron resonance (ECR) plasma breakdown is studied in a small linear cylindrical system with four different gases - hydrogen, helium, argon and nitrogen. Microwave power in the experimental system is delivered by a magnetron at 2.45 ± 0.02 GHz in TE10 mode and launched radially to have extra-ordinary (X) wave in plasma. The axial magnetic field required for ECR in the system is such that the fundamental ECR surface ( = 875.0 G) resides at the geometrical centre of the plasma system. ECR breakdown parameters such as plasma delay time and plasma decay time from plasma density measurements are carried out at the centre using a Langmuir probe. The operating parameters such as working gas pressure (1 × 10-5 -1 × 10-2 mbar) and input microwave power (160{800 W) are varied and the corresponding effect on the breakdown parameters is studied. The experimental results obtained are presented in this paper.

  10. Multicusp type Electron Cyclotron Resonance ion source for plasma processing

    Energy Technology Data Exchange (ETDEWEB)

    Amemiya, Hiroshi; Shigueoka, Yoshyuki (Institute of Physical and Chemical Research, Wako, Saitama (Japan)); Ishii, Shigeyuki

    1991-02-01

    A multi-cusp type ECR (electron cyclotron resonance) ion source is built with use of SmCo magnets and 2.45 GHz-TE{sub 11} circular mode microwave. The ion source is operated at pressures from 10{sup -4} to 10{sup -3} Torr with the input microwave power from 100 to 400 W. In hydrogen, the current density of H{sup +} is higher than those of H{sub 2}{sup +} and H{sub 3}{sup +}. The dependence of the fraction of each ion species on the power and pressure is measured and explained by rate equations. The source is operated also in other gases. Mass spectra in He, N{sub 2}, O{sub 2}, Ar and CH{sub 4} are shown together with the pressure and power dependences. Multicharged state of up to 3 has been obtained. (author).

  11. Numerical model of electron cyclotron resonance ion source

    Directory of Open Access Journals (Sweden)

    V. Mironov

    2015-12-01

    Full Text Available Important features of the electron cyclotron resonance ion source (ECRIS operation are accurately reproduced with a numerical code. The code uses the particle-in-cell technique to model the dynamics of ions in ECRIS plasma. It is shown that a gas dynamical ion confinement mechanism is sufficient to provide the ion production rates in ECRIS close to the experimentally observed values. Extracted ion currents are calculated and compared to the experiment for a few sources. Changes in the simulated extracted ion currents are obtained with varying the gas flow into the source chamber and the microwave power. Empirical scaling laws for ECRIS design are studied and the underlying physical effects are discussed.

  12. Thermal History of Archaeological Objects, Studied by Electron Spin Resonance

    Science.gov (United States)

    Bartoll, Jens; Tani, Atsushi

    Electron spin resonance (ESR) spectroscopy is a sensitive tool for distinguishing between "burned" and "unburned" states of archaeological objects. Prehistoric heating conditions, such as the temperature, atmosphere, time of exposure to heat, and when the heating took place, can be studied by this method with some success. ESR "reporters," such as (a) radiation defects, (b) pyrolytic defects, and (c) transition metal ions, can even reflect changes induced at relatively low temperatures (e.g., in the range of 200° C for objects containing organic compounds). Several ESR heating markers are so stable that samples dating back to the ages when fire first began to be used can be analyzed today. An overview is presented of the literature concerning objects, such as stone, soil, pottery, and plant and animal products.

  13. Electron spin resonance from semiconductor-metal separated SWCNTs

    Energy Technology Data Exchange (ETDEWEB)

    Havlicek, M.; Jantsch, W. [Institut fuer Halbleiter- und Festkoerperphysik, Johannes Kepler Universitaet, 4040 Linz (Austria); Ruemmeli, M.; Schoenfelder, R. [Leibniz Institute fuer Festkoerperphysik und Werkstoffforschung, Dresden (Germany); Yanagi, K. [Department of Physics, Tokyo Metropolitan University, Hachioji, Tokyo (Japan); Miyata, Y. [Department of Chemistry, Nagoya University, Nagoya, Aichi (Japan); Kataura, H. [Nanotechnology Research Institute, AIST, 1-1-1 Higashi, Tsukuba 305-8562 (Japan); Simon, F.; Peterlik, H.; Kuzmany, H. [Fakultaet fuer Physik, Universitaet Wien, Strudlhofgasse 4, 1090 Wien (Austria)

    2010-12-15

    Electron spin resonance in the X band is reported for fully metal-semiconductor separated SWCNTs. For the experiments samples were immersed in ethanol or wrapped into a teflon foil. The response from the metallic tubes exhibits a strong asymmetry in the line shape whereas the asymmetry for the semiconducting (SC) tubes is comparatively small. In both cases the line widths are unusual small, of the order of 4 G. Particular attention is paid to SC nanotubes which exhibit a much stronger signal as compared to the metallic tubes. The signal intensity is nearly Curie like with a small enhancement beyond 1/T in the low temperature range. The 1/T behavior renders the ESR response unobservable at 300 K. The finite value for the asymmetry parameter in the SC tubes is assumed to originate from charges picked up during exposure to air or to ethanol. (Copyright copyright 2010 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  14. Egyptian limestone for gamma dosimetry: an electron paramagnetic resonance study

    Science.gov (United States)

    Salama, E.

    2014-04-01

    The electron paramagnetic resonance (EPR) properties of limestone from a certain Egyptian site were investigated in order to propose an efficient and low-cost gamma dosimeter. Radiation-induced free radicals were of one type which was produced in the limestone samples at g=2.0066 after exposure to gamma radiation (60Co). EPR spectrum was recorded and analyzed. The microwave power saturation curve and the effect of changing modulation amplitude on peak-to- peak signal height were investigated. The response of limestone to different radiation doses (0.5-20 kGy) was studied. Except for the decrease in signal intensities during the first five hours following irradiation, over the period of two months fair stabilities of signal intensities were noticed. From the current results, it is possible to conclude that natural limestone may be a suitable material for radiation dosimetry in the range of irradiation processing.

  15. Electron Spin Resonance Measurement with Microinductor on Chip

    Directory of Open Access Journals (Sweden)

    Akio Kitagawa

    2011-01-01

    Full Text Available The detection of radicals on a chip is demonstrated. The proposed method is based on electron spin resonance (ESR spectroscopy and the measurement of high-frequency impedance of the microinductor fabricated on the chip. The measurement was by using a frequency sweep of approximately 100 MHz. The ESR spectra of di(phenyl-(2,4,6-trinitrophenyliminoazanium (DPPH dropped on the microinductor which is fabricated with CMOS 350-nm technology were observed at room temperature. The volume of the DPPH ethanol solution was 2 μL, and the number of spins on the micro-inductor was estimated at about 1014. The sensitivity is not higher than that of the standard ESR spectrometers. However, the result indicates the feasibility of a near field radical sensor in which the microinductor as a probe head and ESR signal processing circuit are integrated.

  16. Electron magnetic resonance investigation of chromium diffusion in yttria powders

    Energy Technology Data Exchange (ETDEWEB)

    Biasi, R.S. de, E-mail: rsbiasi@ime.eb.b [Secao de Engenharia Mecanica e de Materiais, Instituto Militar de Engenharia, Pr. General Tiburcio, 80, 22290-270 Rio de Janeiro, RJ (Brazil); Grillo, M.L.N., E-mail: mluciag@uerj.b [Instituto de Fisica, Universidade do Estado do Rio de Janeiro, 20550-013 Rio de Janeiro, RJ (Brazil)

    2010-03-01

    The electron magnetic resonance (EMR) technique was used to investigate the diffusion of chromium in yttria (Y{sub 2}O{sub 3}) powders. The EMR absorption intensity was measured for several annealing times and three different temperatures of isothermal annealing: 1273, 1323 and 1373 K. The activation temperature for diffusion, calculated from the experimental data using a theoretical model based on the Fick equation, was found to be E{sub A}=342+-5 kJ mol{sup -1}. This value is larger than the activation energy for the diffusion of chromium in rutile (TiO{sub 2}), periclase (MgO) and cobalt monoxide (CoO) and smaller than the activation energy for the diffusion of chromium in chrysoberyl (BeAl{sub 2}O{sub 4}).

  17. Pulsed electron-electron double resonance (PELDOR) as EPR spectroscopy in nanometre range

    Energy Technology Data Exchange (ETDEWEB)

    Tsvetkov, Yu D; Milov, A D; Maryasov, A G [Institute of Chemical Kinetics and Combustion, Siberian Branch of the Russian Academy of Sciences, Novosibirsk (Russian Federation)

    2008-06-30

    The results of development of pulsed electron-electron double resonance (PELDOR) method and its applications in structural studies are generalised and described systematically. The foundations of the theory of the method are outlined, some methodological features and applications are considered, in particular, determination of the distances between spin labels in the nanometre range for iminoxyl biradicals, spin-labelled biomacromolecules, radical ion pairs and peptide-membrane complexes. The attention is focussed on radical systems that form upon self-assembly of nanosized complexes (in particular, peptide complexes), spatial effects, and radical pairs in photolysis and photosynthesis. The position of PELDOR among other structural EPR techniques is analysed.

  18. Electron spin coherence and electron nuclear double resonance of Bi donors in natural Si.

    Science.gov (United States)

    George, Richard E; Witzel, Wayne; Riemann, H; Abrosimov, N V; Nötzel, N; Thewalt, Mike L W; Morton, John J L

    2010-08-06

    Donors in silicon hold considerable promise for emerging quantum technologies, due to their uniquely long electron spin coherence times. Bismuth donors in silicon differ from more widely studied group V donors, such as phosphorous, in several significant respects: They have the strongest binding energy (70.98 meV), a large nuclear spin (I=9/2), and a strong hyperfine coupling constant (A=1475.4  MHz). These larger energy scales allow us to perform a detailed test of theoretical models describing the spectral diffusion mechanism that is known to govern the electron spin decoherence of P donors in natural silicon. We report the electron-nuclear double resonance spectra of the Bi donor, across the range 200 MHz to 1.4 GHz, and confirm that coherence transfer is possible between electron and nuclear spin degrees of freedom at these higher frequencies.

  19. Measurement of the two-photon exchange contribution in elastic ep scattering at VEPP-3

    Energy Technology Data Exchange (ETDEWEB)

    Gramolin, A.V. [Budker Institute of Nuclear Physics of SB RAS, Novosibirsk (Russian Federation); Arrington, J. [Argonne National Laboratory, Argonne (United States); Barkov, L.M. [Budker Institute of Nuclear Physics of SB RAS, Novosibirsk (Russian Federation); Dmitriev, V.F. [Budker Institute of Nuclear Physics of SB RAS, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation); Gauzshtein, V.V. [Nuclear Physics Institute of Tomsk Polytechnic University, Tomsk (Russian Federation); Golovin, R.A. [Budker Institute of Nuclear Physics of SB RAS, Novosibirsk (Russian Federation); Holt, R.J. [Argonne National Laboratory, Argonne (United States); Kaminsky, V.V.; Lazarenko, B.A.; Mishnev, S.I. [Budker Institute of Nuclear Physics of SB RAS, Novosibirsk (Russian Federation); Muchnoi, N.Yu. [Budker Institute of Nuclear Physics of SB RAS, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation); Neufeld, V.V.; Nikolenko, D.M.; Rachek, I.A.; Sadykov, R.Sh. [Budker Institute of Nuclear Physics of SB RAS, Novosibirsk (Russian Federation); Shestakov, Yu.V. [Budker Institute of Nuclear Physics of SB RAS, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation); Stibunov, V.N. [Nuclear Physics Institute of Tomsk Polytechnic University, Tomsk (Russian Federation); Toporkov, D.K. [Budker Institute of Nuclear Physics of SB RAS, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation); Vries, H. de [NIKHEF, Amsterdam (Netherlands); Zevakov, S.A. [Budker Institute of Nuclear Physics of SB RAS, Novosibirsk (Russian Federation); and others

    2012-04-15

    We report on the status of the Novosibirsk experiment on a precision measurement of the ratio R of the elastic e{sup +}p and e{sup -}p scattering cross sections. Such measurements determine the two-photon exchange effect in elastic electron-proton scattering. The experiment is conducted at the VEPP-3 storage ring using a hydrogen internal gas target. The ratio R is measured with a beam energy of 1.6 GeV (electron/positron scattering angles are {theta}=55 Division-Sign 75 Degree-Sign and {theta}=15 Division-Sign 25 Degree-Sign ) and 1 GeV ({theta}=65 Division-Sign 105 Degree-Sign ). We briefly describe the experimental method, paying special attention to the radiative corrections. Some preliminary results are presented.

  20. Measurement of the two-photon exchange contribution in elastic $ep$ scattering at VEPP-3

    CERN Document Server

    Gramolin, A V; Barkov, L M; Dmitriev, V F; Gauzshtein, V V; Golovin, R A; Holt, R J; Kaminsky, V V; Lazarenko, B A; Mishnev, S I; Muchnoi, N Yu; Neufeld, V V; Nikolenko, D M; Rachek, I A; Sadykov, R Sh; Shestakov, Yu V; Stibunov, V N; Toporkov, D K; de Vries, H; Zevakov, S A; Zhilich, V N

    2011-01-01

    We report on the status of the Novosibirsk experiment on a precision measurement of the ratio $R$ of the elastic $e^+ p$ and $e^- p$ scattering cross sections. Such measurements determine the two-photon exchange effect in elastic electron-proton scattering. The experiment is conducted at the VEPP-3 storage ring using a hydrogen internal gas target. The ratio $R$ is measured with a beam energy of 1.6 GeV (electron/positron scattering angles are $\\theta = 55 \\div 75^{\\circ}$ and $\\theta = 15 \\div 25^{\\circ}$) and 1 GeV ($\\theta = 65 \\div 105^{\\circ}$). We briefly describe the experimental method, paying special attention to the radiative corrections. Some preliminary results are presented.

  1. PHOTOCHROMISM AND LUMINESCENCE OF DOPANT CHROMOPHORES THROUGH TWO-PHOTON IONIZATION IN POLYMER FILMS

    Institute of Scientific and Technical Information of China (English)

    Masahide Yamamoto; Hideo Ohkita; Shinzaburo Ito

    2001-01-01

    Two-photon ionization and recombination processes of an aromatic chromophore doped in polymer films were studied and the features of these processes were discussed in relation to photofunctional polymers. An aromatic molecule having low ionization potential, e.g., N,N,N',N'-tetramethyl-p-phenylene diamine doped in poly(methyl methacrylate)(PMMA) film was easily photoionized by intense laser light excitation, giving a colored radical cation (photochromism) and a trapped electron in PMMA matrix. As a reversed process, the radical cation recombined with the trapped electron, showing discoloration and emitting luminescence, either isothermal luminescence (ITL), or thermoluminescence (TL). In this report,ITL and TL through the charge recombination process were studied and the luminescence was suggested as a mean of the read-out of photorecording.

  2. Study of Two-Photon Transistions in CLEO III Upsilon(3S) Data

    CERN Document Server

    Cinabro, D; McGee, S; Bornheim, A; Lipeles, E; Pappas, S P; Shapiro, A; Sun, W M; Weinstein, A J; Mahapatra, R; Briere, R A; Chen, G P; Ferguson, T; Tatishvili, G T; Vogel, H; Adam, N E; Alexander, J P; Berkelman, K; Boisvert, V; Cassel, David G; Drell, P S; Duboscq, J E; Ecklund, K M; Ehrlich, R; Galik, R S; Gibbons, L; Gittelman, B; Gray, S W; Hartill, D L; Heltsley, B K; Hsu, L; Jones, C D; Kandaswamy, J; Kreinick, D L; Magerkurth, A; Mahlke-Krüger, H; Meyer, T O; Mistry, N B; Nordberg, E; Patterson, J R; Peterson, D; Pivarski, J; Riley, D; Sadoff, A J; Schwarthoff, H; Shepherd, M R; Thayer, J G; Urner, D; Viehhauser, G; Warburton, A; Weinberger, M; Athar, S B; Avery, P; Breva-Newell, L; Potlia, V; Stöck, H; Yelton, J; Brandenburg, G; Kim, D Y J; Wilson, R; Benslama, K; Eisenstein, B I; Ernst, J; Gollin, G D; Hans, R M; Karliner, I; Lowrey, N; Plager, C; Sedlack, C; Selen, M; Thaler, J J; Williams, J; Edwards, K W; Ammar, R; Besson, D; Zhao, X; Anderson, S; Frolov, V V; Kubota, Y; Lee, S J; Li, S Z; Poling, R A; Smith, A; Stepaniak, C J; Urheim, J; Metreveli, Z V; Seth, K K; Tomaradze, A G; Zweber, P; Ahmed, S; Alam, M S; Jian, L; Saleem, M; Wappler, F; Eckhart, E; Gan, K K; Gwon, C; Hart, T; Honscheid, K; Hufnagel, D; Kagan, H; Kass, R; Pedlar, T K; Thayer, J B; Von Törne, E; Wilksen, T; Zoeller, M M; Muramatsu, H; Richichi, S J; Severini, H; Skubic, P L; Dytman, S A; Müller, J A; Nam, S; Savinov, V; Chen, S; Hinson, J W; Lee, J; Miller, D H; Pavlunin, V; Shibata, E I; Shipsey, I P J; Cronin-Hennessy, D; Lyon, A L; Park, C S; Park, W; Thorndike, E H; Coan, T E; Gao, Y S; Liu, F; Maravin, Y; Stroynowski, R; Artuso, M; Boulahouache, C; Bukin, K; Dambasuren, E; Khroustalev, K; Mountain, R; Nandakumar, R; Skwarnicki, T; Stone, S; Wang, J C; Mahmood, A H; Csorna, S E; Danko, I

    2002-01-01

    We have studied two-photon transitions from Upsilon(3S) decays recorded by the CLEO-III detector in exclusive events with two photons and either two electrons or two muons. We obtain precision measurements of the chi_b(2P_J) masses for J=2 and J=1. The transition rates for all three spin states of the 2P triplet are measured with improved precision which leads to a better determination of their hadronic width ratios. We also observe rare transitions via the chi_b(1P) states. The measured rates for these transitions allow a determination of , the E1 matrix element, which is more sensitive to the structure of the bb states than the matrix element which dominates the radiative decays of the Upsilon(3S) state. We also present first upper limits on the branching ratios for Upsilon(3S)-> pi0 Upsilon(2S) Upsilon(3S) -> pi0 Upsilon(1S) and a new limit for the branching ratio for Upsilon(3S) -> eta Upsilon(1S).

  3. Correction-free remotely scanned two-photon in vivo mouse retinal imaging

    Institute of Scientific and Technical Information of China (English)

    Adi Schejter Bar-Noam; Nairouz Farah; Shy Shoham

    2016-01-01

    Non-invasive fluorescence retinal imaging in small animals is an important requirement for an array of translational vision applications.The in vivotwo-photon imaging of the mouse retina may enable the long-term investigation of the structure and function of healthy and diseased retinal tissue.However,to date,this has only been possible using relatively complex adaptive-optics systems.Here,the optical modeling of the murine eye and of the imaging system is used to achieve correction-free two-photon microscopy through the pupil of a mouse eye to yield high-quality,optically sectioned fundus images.By remotely scanning the focus using an electronically tunable lens,high-resolution three-dimensional fluorescein angiograms and cellular-scale images are acquired,thus introducing a correction-free baseline performance level for two-photon in vivo retinal imaging.Moreover,the system enables functional calcium imaging of repeated retinal responses to light stimulation using the genetically encoded indicator,GCaMP6s.These results and the simplicity of the new add-on optics are an important step toward several structural,functional,and multimodal imaging applications that will benefit from the tight optical sectioning and the use of near-infrared light.

  4. One- and two-photon absorption properties of two metalloporphyrin complexes

    Institute of Scientific and Technical Information of China (English)

    Sun Yuan-Hong; Wang Chuan-Kui

    2011-01-01

    The linear and nonlinear optical properties of two metalloporphyrin complexes formed by the complementary coordination of central zinc or magnesium ions to the ligand 5,10,15-tri-(p-tolyl)-20-phenylethynylporphyrin are theoretically investigated by using the analytic response theory at the density functional theory level.The results indicate that the studied complexes present more symmetric geometry structures than the ligand.The charge-transfer states of the two complexes in the lower energy region are all almost degenerate but those of the ligand are well separated.The ratio of the two-photon absorption cross sections of the ligand,zinc-porphyrin and magnesium-porphyrin complexes is 1.0:1.5:1.8,demonstrating that the two-photon absorption capability can be greatly increased when the ligand is coordinated with a metal ion.Moreover,several physical micro-mechanisms including electron transitions and intramolecular charge-transfer processes are discussed to explore the differences in optical property between the ligand and two complexes.

  5. Molecular engineering of nanoscale quadrupolar chromophores for two-photon absorption

    Science.gov (United States)

    Porres, Laurent; Mongin, Olivier; Blanchard-Desce, Mireille H.; Ventelon, Lionel; Barzoukas, Marguerite; Moreaux, Laurent; Pons, Thomas; Mertz, Jerome

    2003-02-01

    Our aim has been the design of optimized NLO-phores with very high two-photon absorption (TPA) cross-sections (s2) in the red-NIR region, while maintaining high linear transparency and high fluorescence quantum yield. Our molecular engineering strategy is based on the push-push or pull-pull functionalization of semi-rigid nanoscale conjugated systems. The central building blocks were selected as rigid units that may assist quadrupolar intramolecular charge transfer by acting either as a (weak) donor or acceptor core. Quadrupolar molecules derived either from a phenyl unit, a rigidified biphenyl moiety or a fused bithiophene unit have been considered. Conjugated oligomers made of phenylene-vinylene and/or phenylene-ethynylene units were selected as connecting spacers between the core and the electroactive end groups to ensure effective electronic conjugation while maintaining suitable transparency/fluorescence. The TPA cross-sections were determined by investigating the two-photon-excited fluorescence properties using a Ti:sapphire laser delivering fs pulses. Both the nature of the end groups and of the core moiety play an important role in determining the TPA spectra. In addition, by adjusting the length and nature of the conjugated extensor, both amplification and spectral tuning of TPA cross-sections can be achieved. As a result, push-push fluorophores which demonstrate giant TPA cross-sections (up to 3000 GM) in the visible red, high fluorescence quantum yields and good transparency in the visible range have been obtained.

  6. Charge Transport in Two-Photon Semiconducting Structures for Solar Fuels.

    Science.gov (United States)

    Liu, Guohua; Du, Kang; Haussener, Sophia; Wang, Kaiying

    2016-10-20

    Semiconducting heterostructures are emerging as promising light absorbers and offer effective electron-hole separation to drive solar chemistry. This technology relies on semiconductor composites or photoelectrodes that work in the presence of a redox mediator and that create cascade junctions to promote surface catalytic reactions. Rational tuning of their structures and compositions is crucial to fully exploit their functionality. In this review, we describe the possibilities of applying the two-photon concept to the field of solar fuels. A wide range of strategies including the indirect combination of two semiconductors by a redox couple, direct coupling of two semiconductors, multicomponent structures with a conductive mediator, related photoelectrodes, as well as two-photon cells are discussed for light energy harvesting and charge transport. Examples of charge extraction models from the literature are summarized to understand the mechanism of interfacial carrier dynamics and to rationalize experimental observations. We focus on a working principle of the constituent components and linking the photosynthetic activity with the proposed models. This work gives a new perspective on artificial photosynthesis by taking simultaneous advantages of photon absorption and charge transfer, outlining an encouraging roadmap towards solar fuels.

  7. Bounce resonance scattering of radiation belt electrons by H+ band EMIC waves

    Science.gov (United States)

    Cao, Xing; Ni, Binbin; Summers, Danny; Bortnik, Jacob; Tao, Xin; Shprits, Yuri Y.; Lou, Yuequn; Gu, Xudong; Fu, Song; Shi, Run; Xiang, Zheng; Wang, Qi

    2017-02-01

    We perform a detailed analysis of bounce-resonant pitch angle scattering of radiation belt electrons due to electromagnetic ion cyclotron (EMIC) waves. It is found that EMIC waves can resonate with near-equatorially mirroring electrons over a wide range of L shells and energies. H+ band EMIC waves efficiently scatter radiation belt electrons of energy >100 keV from near 90° pitch angles to lower pitch angles where the cyclotron resonance mechanism can take over to further diffuse electrons into the loss cone. Bounce-resonant electron pitch angle scattering rates show a strong dependence on L shell, wave normal angle distribution, and wave spectral properties. We find distinct quantitative differences between EMIC wave-induced bounce-resonant and cyclotron-resonant diffusion coefficients. Cyclotron-resonant electron scattering by EMIC waves has been well studied and found to be a potentially crucial electron scattering mechanism. The new investigation here demonstrates that bounce-resonant electron scattering may also be very important. We conclude that bounce resonance scattering by EMIC waves should be incorporated into future modeling efforts of radiation belt electron dynamics.

  8. Photo-redox activated drug delivery systems operating under two photon excitation in the near-IR.

    Science.gov (United States)

    Guardado-Alvarez, Tania M; Devi, Lekshmi Sudha; Vabre, Jean-Marie; Pecorelli, Travis A; Schwartz, Benjamin J; Durand, Jean-Olivier; Mongin, Olivier; Blanchard-Desce, Mireille; Zink, Jeffrey I

    2014-05-07

    We report the design and synthesis of a nano-container consisting of mesoporous silica nanoparticles with the pore openings covered by "snap-top" caps that are opened by near-IR light. A photo transducer molecule that is a reducing agent in an excited electronic state is covalently attached to the system. Near IR two-photon excitation causes inter-molecular electron transfer that reduces a disulfide bond holding the cap in place, thus allowing the cargo molecules to escape. We describe the operation of the "snap-top" release mechanism by both one- and two-photon activation. This system presents a proof of concept of a near-IR photoredox-induced nanoparticle delivery system that may lead to a new type of photodynamic drug release therapy.

  9. Excited-state kinetics of the carotenoid S//1 state in LHC II and two-photon excitation spectra of lutein and beta-carotene in solution Efficient Car S//1 yields Chl electronic energy transfer via hot S//1 states?

    CERN Document Server

    Walla, P J; Linden, Patricia A; Ohta, Kaoru

    2002-01-01

    The excited-state dynamics of the carotenoids (Car) in light- harvesting complex II (LHC II) of Chlamydomonas reinhardtii were studied by transient absorption measurements. The decay of the Car S //1 population ranges from similar to 200 fs to over 7 ps, depending on the excitation and detection wavelengths. In contrast, a 200 fs Car S//1 yields Chlorophyll (Chl) energy transfer component was the dominant time constant for our earlier two-photon fluorescence up- conversion measurements (Walla, P.J. ; et al. J. Phys. Chem. B 2000, 104, 4799-4806). We also present the two-photon excitation (TPE) spectra of lutein and beta-carotene in solution and compare them with the TPE spectrum of LHC II. The TPE-spectrum of LHC II has an onset much further to the blue and a width that is narrower than expected from comparison to the S//1 fluorescence of lutein and beta-carotene in solution. Different environments may affect the shape of the S//1 spectrum significantly. To explain the blue shift of the TPE spectrum and the d...

  10. Two-Photon Ghost Image and Interference-Diffraction

    Science.gov (United States)

    Shih, Y. H.; Sergienko, A. V.; Pittman, T. B.; Strekalov, D. V.; Klyshko, D. N.

    1996-01-01

    One of the most surprising consequences of quantum mechanics is entanglement of two or more distance particles. The two-particle entangled state was mathematically formulated by Schrodinger. Based on this unusual quantum behavior, EPR defined their 'physical reality' and then asked the question: 'Can Quantum-Mechanical Description of Physical Reality Be Considered Complete?' One may not appreciate EPR's criterion of physical reality and insist that 'no elementary quantum phenomenon is a phenomenon until it is a recorded phenomenon'. Optical spontaneous parametric down conversion (SPDC) is the most effective mechanism to generate an EPR type entangled two-photon state. In SPDC, an optical beam, called the pump, is incident on a birefringent crystal. The pump is intense enough so that nonlinear effects lead to the conversion of pump photons into pairs of photons, historically called signal and idler. Technically, the SPDC is said to be type-1 or type-2, depending on whether the signal and idler beams have parallel or orthogonal polarization. The SPDC conversion efficiency is typically on the order of 10(exp -9) to 10(exp -11), depending on the SPDC nonlinear material. The signal and idler intensities are extremely low, only single photon detection devices can register them. The quantum entanglement nature of SPDC has been demonstrated in EPR-Bohm experiments and Bell's inequality measurements. The following two experiments were recently performed in our laboratory, which are more closely related to the original 1935 EPR gedankenezperiment. The first experiment is a two-photon optical imaging type experiment, which has been named 'ghost image' by the physics community. The signal and idler beams of SPDC are sent in different directions, so that the detection of the signal and idler photons can be performed by two distant photon counting detectors. An aperture object (mask) is placed in front of the signal photon detector and illuminated by the signal beam through a

  11. Magneto-Photoluminescence Based on Two-Photon Excitation in Lanthanide-Doped Up-Conversion Crystal Particles.

    Science.gov (United States)

    Xu, Hengxing; Qin, Wei; Li, Mingxing; Wu, Ting; Hu, Bin

    2017-04-01

    Experimental studies on magneto-photoluminescence based on two-photon excitation in up-conversion Y2 O2 S:Er, Yb crystal particles are reported. It is found that the up-conversion photoluminescence generated by two-photon excitation exhibits magnetic field effects at room temperature, leading to a two-photon excitation-induced magneto-photoluminescence, when the two-photon excitation exceeds the critical intensity. By considering the spin selection rule in electronic transitions, it is proposed that spin-antiparallel and spin-parallel transition dipoles with spin mixing are accountable for the observed magneto-photoluminescence. Specifically, the two-photon excitation generates spin-antiparallel electric dipoles between (4) S3/2 -(4) I15/2 in Er(3+) ions. The antiparallel spins are conserved by exchange interaction within dipoles. When the photoexcitation exceeds the critical intensity, the Coulomb screening can decrease the exchange interaction. Consequently, the spin-orbital coupling can partially convert the antiparallel dipoles into parallel dipoles, generating a spin mixing. Eventually, the populations between antiparallel and parallel dipoles reach an equilibrium established by the competition between exchange interaction and spin-orbital coupling. Applying a magnetic field can break the equilibrium by disturbing spin mixing through introducing spin precessions, changing the spin populations on antiparallel and parallel dipoles and leading to the magneto-photoluminescence. Therefore, spin-dependent transition dipoles present a convenient mechanism to realize magneto-photoluminescence in multiphoton up-conversion crystal particles. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  12. Fast, High Fidelity Quantum Dot Spin Initialization without a Strong Magnetic Field by Two-Photon Processes

    CERN Document Server

    Majumdar, Arka; Faraon, Andrei; Vuckovic, Jelena

    2009-01-01

    We describe a proposal for fast electron spin initialization in a negatively charged quantum dot coupled to a microcavity without the need for a strong magnetic field. We employ two-photon excitation to access trion states that are spin forbidden by one-photon excitation. Our simulation shows a maximum initialization speed of 1.3 GHz and maximum fidelity of 99.7% with realistic system parameters.

  13. Solvent and branching effect on the two-photon absorption properties of push-pull triphenylamine derivatives

    OpenAIRE

    Cvejn, Daniel; Michail, E.; Seintis, M.; Klikar, M.; Pytela, Oldřich; Mikysek, Tomáš; Almonasy, Numan; Ludwig, Miroslav; Giannetas, V.; Fakis, M.; Bureš, Filip

    2016-01-01

    The photophysical and two-photon absorption (2PA) properties of two tri-podal molecules and of their quadrupolar and dipolar counterparts are reported for a series of solvents with varying polarity. The molecules possess a tri-phenylamine electron donating group and mono-cyano acceptors while olefinic and acetylenic π-linkers have been used. Branching led to an increase of the molar extinction coefficient and to a slight bathochromic shift of the absorption spectra while the fluorescence quan...

  14. ATLAS 10 GHz electron cyclotron resonance ion source upgrade project

    Energy Technology Data Exchange (ETDEWEB)

    Moehs, D. P. [Argonne National Laboratory, Physics Division, Argonne, Illinois 60439 (United States); Vondrasek, R. [Argonne National Laboratory, Physics Division, Argonne, Illinois 60439 (United States); Pardo, R. C. [Argonne National Laboratory, Physics Division, Argonne, Illinois 60439 (United States); Xie, D. [Berkeley Ion Equipment Inc., Santa Clara, California 95054 (United States)

    2000-02-01

    A major upgrade of the first ATLAS 10 GHz electron cyclotron resonance (ECR) ion source, which began operations in 1987, is in the planning and procurement phase. The new design will convert the old two-stage source into a single-stage source with an electron donor disk and high gradient magnetic field that preserves radial access for solid material feeds and pumping of the plasma chamber. The new magnetic-field profile allows for the possibility of a second ECR zone at a frequency of 14 GHz. An open hexapole configuration, using a high-energy-product Nd-Fe-B magnet material, having an inner diameter of 8.8 cm and pole gaps of 2.4 cm, has been adopted. Models indicate that the field strengths at the chamber wall, 4 cm in radius, will be 9.3 kG along the magnet poles and 5.6 kG along the pole gaps. The individual magnet bars will be housed in austenitic stainless steel, allowing the magnet housing within the aluminum plasma chamber to be used as a water channel for direct cooling of the magnets. Eight solenoid coils from the existing ECR will be enclosed in an iron yoke to produce the axial mirror. Based on a current of 500 A, the final model predicts a minimum B field of 3 kG with injection and extraction mirror ratios of 4.4 and 2.9, respectively. (c) 2000 American Institute of Physics.

  15. Tetrachloridocuprates(II—Synthesis and Electron Paramagnetic Resonance (EPR Spectroscopy

    Directory of Open Access Journals (Sweden)

    Peter Strauch

    2012-02-01

    Full Text Available Ionic liquids (ILs on the basis of metal containing anions and/or cations are of interest for a variety of technical applications e.g., synthesis of particles, magnetic or thermochromic materials. We present the synthesis and the results of electron paramagnetic resonance (EPR spectroscopic analyses of a series of some new potential ionic liquids based on tetrachloridocuprates(II, [CuCl4]2−, with different sterically demanding cations: hexadecyltrimethylammonium 1, tetradecyltrimethylammonium 2, tetrabutylammonium 3 and benzyltriethylammonium 4. The cations in the new compounds were used to achieve a reasonable separation of the paramagnetic Cu(II ions for EPR spectroscopy. The EPR hyperfine structure was not resolved. This is due to the exchange broadening, resulting from still incomplete separation of the paramagnetic Cu(II centers. Nevertheless, the principal values of the electron Zeemann tensor (g║ and g┴ of the complexes could be determined. Even though the solid substances show slightly different colors, the UV/Vis spectra are nearly identical, indicating structural changes of the tetrachloridocuprate moieties between solid state and solution. The complexes have a promising potential e.g., as high temperature ionic liquids, as precursors for the formation of copper chloride particles or as catalytic paramagnetic ionic liquids.

  16. ATLAS 10 GHz electron cyclotron resonance ion source upgrade project

    CERN Document Server

    Moehs, D P; Pardo, R C; Xie, D

    2000-01-01

    A major upgrade of the first ATLAS 10 GHz electron cyclotron resonance (ECR) ion source, which began operations in 1987, is in the planning and procurement phase. The new design will convert the old two-stage source into a single-stage source with an electron donor disk and high gradient magnetic field that preserves radial access for solid material feeds and pumping of the plasma chamber. The new magnetic-field profile allows for the possibility of a second ECR zone at a frequency of 14 GHz. An open hexapole configuration, using a high-energy-product Nd-Fe-B magnet material, having an inner diameter of 8.8 cm and pole gaps of 2.4 cm, has been adopted. Models indicate that the field strengths at the chamber wall, 4 cm in radius, will be 9.3 kG along the magnet poles and 5.6 kG along the pole gaps. The individual magnet bars will be housed in austenitic stainless steel, allowing the magnet housing within the aluminum plasma chamber to be used as a water channel for direct cooling of the magnets. Eight solenoid...

  17. Tunable structures comprising two photonic crystal slabs--optical study in view of multi-analyte enhanced detection.

    Science.gov (United States)

    Shi, Lina; Pottier, Pierre; Skorobogatiy, Maksim; Peter, Yves-Alain

    2009-06-22

    Using finite-difference time-domain method, we characterize the normal-incidence transmission properties of a two slab photonic crystal device in a view of its applications in fluorescence enhancement and multi-analyte detection. Individual slabs consist of a square or a triangular lattice of air holes embedded into a silicon nitride slab. The geometrical parameters are chosen so that the individual slabs operate in a guided resonance regime where strong reflectivity under the normal incidence angle is observed in a broad spectral range. When placed in the close proximity of each other, the two photonic crystal slab system exhibits a narrow Fabry-Perot type transmission peak corresponding to the excitation of a resonant mode in the cavity formed by the two slabs. We then study the effects of the size of the air gap between the two photonic crystal slabs on the spectral position and bandwidth of a resonance transmission peak. Finally, we investigate the electromagnetic energy distributions at the wavelength of a transmission resonance in the double slab photonic crystals. As a final result we demonstrate that this structure can provide electric field enhancement at the slab surface, which can be used for fluorescence enhancement.

  18. Electron paramagnetic resonance: a powerful tool to support magnetic resonance imaging research.

    Science.gov (United States)

    Danhier, Pierre; Gallez, Bernard

    2015-01-01

    The purpose of this paper is to describe some of the areas where electron paramagnetic resonance (EPR) has provided unique information to MRI developments. The field of application mainly encompasses the EPR characterization of MRI paramagnetic contrast agents (gadolinium and manganese chelates, nitroxides) and superparamagnetic agents (iron oxide particles). The combined use of MRI and EPR has also been used to qualify or disqualify sources of contrast in MRI. Illustrative examples are presented with attempts to qualify oxygen sensitive contrast (i.e. T1 - and T2 *-based methods), redox status or melanin content in tissues. Other areas are likely to benefit from the combined EPR/MRI approach, namely cell tracking studies. Finally, the combination of EPR and MRI studies on the same models provides invaluable data regarding tissue oxygenation, hemodynamics and energetics. Our description will be illustrative rather than exhaustive to give to the readers a flavour of 'what EPR can do for MRI'.

  19. Tuning Ag29 nanocluster light emission from red to blue with one and two-photon excitation

    Science.gov (United States)

    Russier-Antoine, Isabelle; Bertorelle, Franck; Hamouda, Ramzi; Rayane, Driss; Dugourd, Philippe; Sanader, Željka; Bonačić-Koutecký, Vlasta; Brevet, Pierre-François; Antoine, Rodolphe

    2016-01-01

    We demonstrate that the tuning of the light emission from red to blue in dihydrolipoic acid (DHLA) capped Ag29 nanoclusters can be trigged with one and two photon excitations. The cluster stoichiometry was determined with mass spectrometry and found to be Ag29(DHLA)12. In a detailed optical investigation, we show that these silver nanoclusters exhibit a strong red photoluminescence visible to the naked eye and characterized by a quantum yield of nearly ~2% upon one-photon excitation. In the nonlinear optical (NLO) study of the properties of the clusters, the two-photon excited fluorescence spectra were recorded and their first hyperpolarizability obtained. The two-photon absorption cross-section at ~800 nm for Ag29(DHLA)12 is higher than 104 GM and the hyperpolarizability is 106 × 10-30 esu at the same excitation wavelength. The two-photon excited fluorescence spectrum appears strongly blue-shifted as compared to the one-photon excited spectrum, displaying a broad band between 400 and 700 nm. The density functional theory (DFT) provides insight into the structural and electronic properties of Ag29(DHLA)12 as well as into interplay between metallic subunit or core and ligands which is responsible for unique optical properties.We demonstrate that the tuning of the light emission from red to blue in dihydrolipoic acid (DHLA) capped Ag29 nanoclusters can be trigged with one and two photon excitations. The cluster stoichiometry was determined with mass spectrometry and found to be Ag29(DHLA)12. In a detailed optical investigation, we show that these silver nanoclusters exhibit a strong red photoluminescence visible to the naked eye and characterized by a quantum yield of nearly ~2% upon one-photon excitation. In the nonlinear optical (NLO) study of the properties of the clusters, the two-photon excited fluorescence spectra were recorded and their first hyperpolarizability obtained. The two-photon absorption cross-section at ~800 nm for Ag29(DHLA)12 is higher than 104

  20. Spin labeling and Double Electron-Electron Resonance (DEER) to Deconstruct Conformational Ensembles of HIV Protease

    Science.gov (United States)

    Casey, Thomas M.; Fanucci, Gail E.

    2016-01-01

    An understanding of macromolecular conformational equilibrium in biological systems is oftentimes essential to understand function, dysfunction, and disease. For the past few years, our lab has been utilizing site-directed spin labeling (SDSL), coupled with electron paramagnetic resonance (EPR) spectroscopy, to characterize the conformational ensemble and ligand-induced conformational shifts of HIV-1 protease (HIV-1PR). The biomedical importance of characterizing the fractional occupancy of states within the conformational ensemble critically impacts our hypothesis of a conformational selection mechanism of drug-resistance evolution in HIV-1PR. The purpose of the following chapter is to give a timeline perspective of our SDSL EPR approach to characterizing conformational sampling of HIV-1PR. We provide detailed instructions for the procedure utilized in analyzing distance profiles for HIV-1PR obtained from pulsed electron–electron double resonance (PELDOR). Specifically, we employ a version of PELDOR known as double electron–electron resonance (DEER). Data are processed with the software package “DeerAnalysis” (http://www.epr.ethz.ch/software), which implements Tikhonov regularization (TKR), to generate a distance profile from electron spin-echo amplitude modulations. We assign meaning to resultant distance profiles based upon a conformational sampling model, which is described herein. The TKR distance profiles are reconstructed with a linear combination of Gaussian functions, which is then statistically analyzed. In general, DEER has proven powerful for observing structural ensembles in proteins and, more recently, nucleic acids. Our goal is to present our advances in order to aid readers in similar applications. PMID:26477251

  1. Two-photon polymerization for fabrication of biomedical devices

    Science.gov (United States)

    Ovsianikov, Aleksandr; Doraiswamy, Anand; Narayan, R.; Chichkov, B. N.

    2007-01-01

    Two-photon polymerization (2PP) is a novel technology which allows the fabrication of complex three-dimensional (3D) microstructures and nanostructures. The number of applications of this technology is rapidly increasing; it includes the fabrication of 3D photonic crystals [1-4], medical devices, and tissue scaffolds [5-6]. In this contribution, we discuss current applications of 2PP for microstructuring of biomedical devices used in drug delivery. While in general this sector is still dominated by oral administration of drugs, precise dosing, safety, and convenience are being addressed by transdermal drug delivery systems. Currently, main limitations arise from low permeability of the skin. As a result, only few types of pharmacological substances can be delivered in this manner [7]. Application of microneedle arrays, whose function is to help overcome the barrier presented by the epidermis layer of the skin, provides a very promising solution. Using 2PP we have fabricated arrays of hollow microneedles with different geometries. The effect of microneedle geometry on skin penetration is examined. Our results indicate that microneedles created using 2PP technique are suitable for in vivo use, and for integration with the next generation of MEMS- and NEMS-based drug delivery devices.

  2. Higgs decay into two photons in a warped extra dimension

    Energy Technology Data Exchange (ETDEWEB)

    Hahn, Juliane; Hoerner, Clara; Malm, Raoul; Novotny, Kristiane; Schmell, Christoph [Johannes Gutenberg University, PRISMA Cluster of Excellence and Mainz Institute for Theoretical Physics, Mainz (Germany); Neubert, Matthias [Johannes Gutenberg University, PRISMA Cluster of Excellence and Mainz Institute for Theoretical Physics, Mainz (Germany); Cornell University, Department of Physics, LEPP, Ithaca, NY (United States)

    2014-05-15

    A detailed five-dimensional calculation of the Higgs-boson decay into two photons is performed in both the minimal and the custodially protected Randall-Sundrum (RS) model, where the Standard Model (SM) fields propagate in the bulk and the scalar sector lives on or near the IR brane. It is explicitly shown that the R{sub ξ} gauge invariance of the sum of diagrams involving bosonic fields in the SM also applies to the case of these RS scenarios. An exact expression for the h → γγ amplitude in terms of the five-dimensional (5D) gauge-boson and fermion propagators is presented, which includes the full dependence on the Higgs-boson mass. Closed expressions for the 5D W-boson propagators in theminimal and the custodial RS model are derived, which are valid to all orders in v{sup 2}/M{sup 2}{sub KK}. In contrast to the fermion case, the result for the bosonic contributions to the h → γγ amplitude is insensitive to the details of the localization of the Higgs profile on or near the IR brane. The various RS predictions for the rate of the pp → h → γγ process are compared with the latest LHC data, and exclusion regions for the RS model parameters are derived. (orig.)

  3. Two-Photon-Absorption Scheme for Optical Beam Tracking

    Science.gov (United States)

    Ortiz, Gerardo G.; Farr, William H.

    2011-01-01

    A new optical beam tracking approach for free-space optical communication links using two-photon absorption (TPA) in a high-bandgap detector material was demonstrated. This tracking scheme is part of the canonical architecture described in the preceding article. TPA is used to track a long-wavelength transmit laser while direct absorption on the same sensor simultaneously tracks a shorter-wavelength beacon. The TPA responsivity was measured for silicon using a PIN photodiode at a laser beacon wavelength of 1,550 nm. As expected, the responsivity shows a linear dependence with incident power level. The responsivity slope is 4.5 x 10(exp -7) A/W2. Also, optical beam spots from the 1,550-nm laser beacon were characterized on commercial charge coupled device (CCD) and complementary metal-oxide semiconductor (CMOS) imagers with as little as 13.7 microWatts of optical power (see figure). This new tracker technology offers an innovative solution to reduce system complexity, improve transmit/receive isolation, improve optical efficiency, improve signal-to-noise ratio (SNR), and reduce cost for free-space optical communications transceivers.

  4. Two-photon excited photoconversion of cyanine-based dyes

    Science.gov (United States)

    Kwok, Sheldon J. J.; Choi, Myunghwan; Bhayana, Brijesh; Zhang, Xueli; Ran, Chongzhao; Yun, Seok-Hyun

    2016-03-01

    The advent of phototransformable fluorescent proteins has led to significant advances in optical imaging, including the unambiguous tracking of cells over large spatiotemporal scales. However, these proteins typically require activating light in the UV-blue spectrum, which limits their in vivo applicability due to poor light penetration and associated phototoxicity on cells and tissue. We report that cyanine-based, organic dyes can be efficiently photoconverted by nonlinear excitation at the near infrared (NIR) window. Photoconversion likely involves singlet-oxygen mediated photochemical cleavage, yielding blue-shifted fluorescent products. Using SYTO62, a biocompatible and cell-permeable dye, we demonstrate photoconversion in a variety of cell lines, including depth-resolved labeling of cells in 3D culture. Two-photon photoconversion of cyanine-based dyes offer several advantages over existing photoconvertible proteins, including use of minimally toxic NIR light, labeling without need for genetic intervention, rapid kinetics, remote subsurface targeting, and long persistence of photoconverted signal. These findings are expected to be useful for applications involving rapid labeling of cells deep in tissue.

  5. Two-Photon-Exchange Effects and $\\Delta(1232)$ Deformation

    CERN Document Server

    Zhou, Hai-Qing

    2016-01-01

    The two-photon-exchange (TPE) contribution in $ep\\rightarrow ep\\pi ^0$ with $W=M_{\\Delta}$ and small $Q^2$ is calculated and its corrections to the ratios of electromagnetic transition form factors $R_{EM} = E_{1+}^{(3/2)}/M_{1+}^{(3/2)} $ and $R_{SM} = S_{1+}^{(3/2)}/M_{1+}^{(3/2)}$, are analysed. A simple hadronic model is used to estimate the TPE amplitude. Two phenomenological models, MAID2007 and SAID, are used to approximate the full $ep\\rightarrow ep\\pi ^0$ cross sections which contain both the TPE and the one-photon-exchange (OPE) contributions. The genuine the OPE amplitude is then extracted from an integral equation by iteration. We find that the TPE contribution is not sensitive to whether MAID or SAID is used as input in the region with $Q^2<2$ GeV$^2$. It gives small correction to $R_{EM}$ while for $R_{SM}$, the correction is about -10\\% at small $\\epsilon$ and about $1\\%$ at large $\\epsilon$ for $Q^2\\approx2.5$ GeV$^2$. The large correction from TPE at small $\\epsilon$ must be included in th...

  6. Two-photon autofluorescence spectroscopy of oral mucosa tissue

    Science.gov (United States)

    Edward, Kert; Shilagard, Tuya; Qiu, Suimin; Vargas, Gracie

    2011-03-01

    The survival rate for individuals diagnosed with oral cancer is correlated with the stage of detection. Thus the development of novel techniques for the earliest possible detection of malignancies is of critical importance. Single photon (1P) autofluorescence spectroscopy has proven to be a powerful diagnostic tool in this regard, but 2P (two photon) spectroscopy remains essentially unexplored. In this investigation, a spectroscopic system was incorporated into a custom-built 2P laser scanning microscope. Oral cancer was induced in the buccal pouch of Syrian Golden hamsters by tri-weekly topical application of 9,10-dimethyl-1,2-benzanthracene (DMBA).Three separated sites where investigated in each hamster at four excitation wavelengths from 780 nm to 890 nm. A Total of 8 hamsters were investigated (4 normal and 4 DMBA treated). All investigated sites were imaged via 2p imaging, marked for biopsy, processed for histology and H&E staining, and graded by a pathologist. The in vivo emission spectrum for normal, mild/high grade dysplasia and squamous cell carcinoma is presented. It is shown that the hamsters with various stages of dysplasia are characterized by spectral differences as a function of depth and excitation wavelength, compared to normal hamsters.

  7. Two-photon holographic optogenetics of neural circuits (Conference Presentation)

    Science.gov (United States)

    Yang, Weijian; Carrillo-Reid, Luis; Peterka, Darcy S.; Yuste, Rafael

    2016-03-01

    Optical manipulation of in vivo neural circuits with cellular resolution could be important for understanding cortical function. Despite recent progress, simultaneous optogenetic activation with cellular precision has either been limited to 2D planes, or a very small numbers of neurons over a limited volume. Here we demonstrate a novel paradigm for simultaneous 3D activation using a low repetition rate pulse-amplified fiber laser system and a spatial light modulator (SLM) to project 3D holographic excitation patterns on the cortex of mice in vivo for targeted volumetric 3D photoactivation. This method is compatible with two-photon imaging, and enables the simultaneous activation of multiple cells in 3D, using red-shifted opsins, such as C1V1 or ReaChR, while simultaneously imaging GFP-based sensors such as GCaMP6. This all-optical imaging and 3D manipulation approach achieves simultaneous reading and writing of cortical activity, and should be a powerful tool for the study of neuronal circuits.

  8. Two-resonance probe for measuring electron density in low-pressure plasmas

    Science.gov (United States)

    Kim, D. W.; You, S. J.; Kim, S. J.; Kim, J. H.; Oh, W. Y.

    2017-04-01

    A technique for measuring double-checked electron density using two types of microwave resonance is presented. Simultaneous measurement of the resonances (plasma and quarter-wavelength resonator resonances), which were used for the cutoff probe (CP) and hairpin probe (HP), was achieved by the proposed microwave resonance probe. The developed two-resonance probe (TRP) consists of parallel separated coaxial cables exposing the radiation and detection tips. The structure resembles that of the CP, except the gapped coaxial cables operate not only as a microwave feeder for the CP but also as a U- shaped quarter-wavelength resonator for the HP. By virtue of this structure, the microwave resonances that have typically been used for measuring the electron density for the CP and HP were clearly identified on the microwave transmission spectrum of the TRP. The two types of resonances were measured experimentally under various power and pressure conditions for the plasma. A three-dimensional full-wave simulation model for the TRP is also presented and used to investigate and reproduce the resonances. The electron densities inferred from the resonances were compared and showed good agreement. Quantitative differences between the densities were attributed to the effects of the sheath width and spatial density gradient on the resonances. This accessible technique of using the TRP to obtain double-checked electron densities may be useful for comparative study and provides complementary uses for the CP and HP.

  9. The controlled excitation of forbidden transitions in the two-photon spectrum of strontium by using collisions and electric fields

    Science.gov (United States)

    Philip, G.; Connerade, J.-P.

    2007-11-01

    We present experimental results involving controlled configuration mixing in two-photon spectroscopy of highly-excited states by exploiting a weak external electric field and collisions. The method has allowed new extensions to high members of the two-photon forbidden J = 3 odd-parity 5snf 1F 3 and the J = 0, even-parity 5sns 1S 0 Rydberg series of neutral strontium to be observed. We achieve resonant two-photon transverse excitation of a high density atomic jet by using a narrow bandwidth tunable dye laser in a heat pipe setup with sensitive ionization detection. Experimental term values are extended for the 5sns 1S 0 series up to n = 46. By suitable exploitation of the composition and pressure of the buffer gases in conjunction with the electric field strength in the excitation region and the exciting laser beam intensity we have also extended observations up to n = 44 for the 5snf 1F 3 series and up to n = 46 for the 5snp 1P 1 series. Our results demonstrate a novel and remarkably simple experimental method to access high Rydberg states to which transitions are forbidden from the ground state by parity and other selection rules.

  10. Resonant Acceleration of Magnetospheric Electrons Driven by the R-X Mode

    Institute of Scientific and Technical Information of China (English)

    XIAO Fu-Liang; ZHENG Hui-Nan; WANG Shui

    2005-01-01

    @@ An extended relativistic model is developed to evaluate the superluminous R-X-mode resonance especially the second-order and third-order resonances with electrons in the Earth's magnetosphere. The potential for stochastic electron acceleration driven by the R-X mode is determined by the dispersive properties of the R-X mode and specifically the resonant harmonic N. In contrast to the limited acceleration at the first harmonic (N = 1)resonance, for the higher harmonic (N > 1) resonances, the R-X mode is capable of accelerating electrons from ~10keV to ~ MeV energies, over a wide range of wave normal angles, in spatial regions extending from the auroral cavity to the latitude (>30°) outer radiation belt. This indicates that higher-order resonance is essentially important for the electron acceleration for the oblique wave propagation.

  11. Carbon nanodots featuring efficient FRET for two-photon photodynamic cancer therapy with a low fs laser power density.

    Science.gov (United States)

    Wang, Jing; Zhang, Zehui; Zha, Shuai; Zhu, Yinyan; Wu, Peiyi; Ehrenberg, Benjamin; Chen, Ji-Yao

    2014-11-01

    The 5,10,15,20-tetrakis(1-methyl 4-pyridinio) porphyrins (TMPyP), a photosensitizer used for photodynamic therapy of cancers (PDT), were linked to carbon dots (CDots) to form the conjugates of CDot-TMPyP by the electrostatic force. The 415 nm emission band of CDots was well overlapped with the absorption band of TMPyP, so that the Cdots in conjugates can work as donor to transfer the energy to TMPyP moiety by fluorescence resonance energy transfer (FRET) with an FRET efficiency of 45%, determined by the fluorescence lifetime change between the free CDots and conjugated CDots. The two-photon absorption cross section (TPACS) of TMPyP is as low as 110 GM and the TMPyP thus be not suitable for two-photon PDT. Whereas the CDots have high TPACS, and their TPACS are excitation wavelength dependent with the maximum value of 15000 GM at 700 nm. Therefore, the conjugates of CDot-TMPyP were explored for two-photon excitation (TPE) PDT. The two-photon image of CDot-TMPyP in Hela cells was clearly seen under the excitation of a 700 nm femto-second (fs) laser. The singlet oxygen production of CDot-TMPyP was also much higher than that of TMPyP alone under TPE of a 700 nm fs laser. The in vitro PDT killing was further achieved with CDot-TMPyP by TPE of the 700 nm fs laser. Particularly herein the low power density of fs laser from unfocused laser beam was successfully used to carry out the TPE PDT, because of the high TPACS of CDots. These results demonstrate that the CDot-TMPyP conjugates are promising for TPE PDT and needed to investigate further. Copyright © 2014 Elsevier Ltd. All rights reserved.

  12. A line-of-sight electron cyclotron emission receiver for electron cyclotron resonance heating feedback control of tearing modes

    DEFF Research Database (Denmark)

    Oosterbeek, J.W.; Bürger, A.; Westerhof, E.;

    2008-01-01

    An electron cyclotron emission (ECE) receiver inside the electron cyclotron resonance heating (ECRH) transmission line has been brought into operation. The ECE is extracted by placing a quartz plate acting as a Fabry-Perot interferometer under an angle inside the electron cyclotron wave (ECW) beam...

  13. Electron spin resonance in Eu-based iron pnictides

    Science.gov (United States)

    Krug von Nidda, H.-A.; Kraus, S.; Schaile, S.; Dengler, E.; Pascher, N.; Hemmida, M.; Eom, M. J.; Kim, J. S.; Jeevan, H. S.; Gegenwart, P.; Deisenhofer, J.; Loidl, A.

    2012-09-01

    The phase diagrams of EuFe2-xCoxAs2 (0≤x≤0.4) and EuFe2As2-yPy (0≤y≤0.43) are investigated by Eu2+ electron spin resonance (ESR) in single crystals. From the temperature dependence of the linewidth ΔH(T) of the exchange narrowed ESR line, the spin-density wave (SDW) (TTSDW) are clearly distinguished. At T>TSDW the isotropic linear increase of the linewidth is driven by the Korringa relaxation which measures the conduction-electron density of states at the Fermi level. For Trate from 8 Oe/K at x=y=0 down to 3 Oe/K at the onset of superconductivity. For x>0.2 and y>0.3 it remains nearly constant. Comparative ESR measurements on single crystals of the Eu diluted SDW compound Eu0.2Sr0.8Fe2As2 and superconducting (SC) Eu0.22Sr0.78Fe1.72Co0.28As2 corroborate the leading influence of the ligand field on the Eu2+ spin relaxation in the SDW regime as well as the Korringa relaxation in the normal metallic regime. A coherence peak is not detected in the latter compound below Tc=21 K, which is in agreement with the expected complex anisotropic SC gap structure. In contrast, indications for phase coexistence and BCS-type superconductivity are found in EuFe2As1.57P0.43.

  14. Voltage-sensitive rhodol with enhanced two-photon brightness.

    Science.gov (United States)

    Kulkarni, Rishikesh U; Kramer, Daniel J; Pourmandi, Narges; Karbasi, Kaveh; Bateup, Helen S; Miller, Evan W

    2017-03-14

    We have designed, synthesized, and applied a rhodol-based chromophore to a molecular wire-based platform for voltage sensing to achieve fast, sensitive, and bright voltage sensing using two-photon (2P) illumination. Rhodol VoltageFluor-5 (RVF5) is a voltage-sensitive dye with improved 2P cross-section for use in thick tissue or brain samples. RVF5 features a dichlororhodol core with pyrrolidyl substitution at the nitrogen center. In mammalian cells under one-photon (1P) illumination, RVF5 demonstrates high voltage sensitivity (28% ΔF/F per 100 mV) and improved photostability relative to first-generation voltage sensors. This photostability enables multisite optical recordings from neurons lacking tuberous sclerosis complex 1, Tsc1, in a mouse model of genetic epilepsy. Using RVF5, we show that Tsc1 KO neurons exhibit increased activity relative to wild-type neurons and additionally show that the proportion of active neurons in the network increases with the loss of Tsc1. The high photostability and voltage sensitivity of RVF5 is recapitulated under 2P illumination. Finally, the ability to chemically tune the 2P absorption profile through the use of rhodol scaffolds affords the unique opportunity to image neuronal voltage changes in acutely prepared mouse brain slices using 2P illumination. Stimulation of the mouse hippocampus evoked spiking activity that was readily discerned with bath-applied RVF5, demonstrating the utility of RVF5 and molecular wire-based voltage sensors with 2P-optimized fluorophores for imaging voltage in intact brain tissue.

  15. Determining the Quark Charges by One and Two Photon Processes.

    Science.gov (United States)

    Janah, Arjun

    1982-05-01

    Testable predictions are presented, which may be used to decide between the gauge theories of integer and fractionally charged quarks (icq and fcq). Two distinctive features of icq are exploited, namely (a) presence of color non-singlet components in weak and electromagnetic currents and (b) possible liberation of color non-singlet states above a threshold energy. Consequences are sought in lepton-hadron interaction processes, taking into account the known "color-suppression" effect. Single photon/weak-boson processes such as (nu)N (--->) (nu)X distinguish between icq and fcq only above color-threshold. Experimental consequences of color-liberation in the above process are obtained. It is found that the gluon-parton contribution survives color-suppression to produce a significant rise in the structure functions when color-threshold is exceeded. Two-photon processes such as e('+)e('-) (--->) e('+)e('-) + 2 jets distinguish between the two theories even below color threshold. To obtain the icq predictions for this process, one must take into account (a) the (momentum -dependent) color suppression and (b) the added contribution from pair production of charged gluons. This is done, and it is observed that: (i) in icq, the ratio R('(gamma)(gamma)(2 jet)) is not simply a number given by the quark charges; it depends on the gluon mass, on kinematics and on the particular differential cross-section considered; (ii) the deviation of icq cross-sections from the fcq values depends crucially on whether one includes "untagged" events; if this is done, the deviation is large; the charged gluon contribution is mainly responsible for this deviation; the quark contribution is smaller than naively expected. Finally, comparison is made with experimental data on e('+)e('-) (--->) e('+)e('-) + 2 jets. Here, icq is found to be in better agreement than fcq, for a broad range of gluon masses. A suitably modified equivalent photon approximation is employed.

  16. Two-photon excitation photodynamic therapy with Photofrin

    Science.gov (United States)

    Karotki, Aliaksandr; Khurana, Mamta; Lepock, James R.; Wilson, Brian C.

    2005-09-01

    Photodynamic therapy (PDT) based on simultaneous two-photon (2-γ) excitation has a potential advantage of highly targeted treatment by means of nonlinear localized photosensitizer excitation. One of the possible applications of 2-γ PDT is a treatment of exodus age-related macular degeneration where highly targeted excitation of photosensitizer in neovasculature is vital for reducing collateral damage to healthy surrounding tissue. To investigate effect of 2-γ PDT Photofrin was used as an archetypal photosensitizer. First, 2-γ absorption properties of Photofrin in the 750 - 900 nm excitation wavelength range were investigated. It was shown that above 800 nm 2-γ interaction was dominant mode of excitation. The 2-γ cross section of Photofrin was rather small and varied between 5 and 10 GM (1 GM = 10-50 cm4s/photon) in this wavelength range. Next, endothelial cells treated with Photofrin were used to model initial effect of 2-γ PDT on neovasculature. Ultrashort laser pulses provided by mode-locked Ti:sapphire laser (pulse duration at the sample 300 fs, repetition rate 90 MHz, mean laser power 10 mW, excitation wavelength 850 nm) were used for the excitation of the photosensitizer. Before 2-γ excitation of the Photofrin cells formed a single continuous sheet at the bottom of the well. The tightly focused laser light was scanned repeatedly over the cell layer. After irradiation the cell layer of the control cells stayed intact while cells treated with photofrin became clearly disrupted. The light doses required were high (6300 Jcm(-2) for ~ 50% killing), but 2-γ cytotoxicity was unequivocally demonstrated.

  17. A Two- Photon Femtosecond Laser System for Three-Dimensional Microfabrication and Data Storage

    Institute of Scientific and Technical Information of China (English)

    蒋中伟; 周拥军; 袁大军; 黄文浩; 夏安东

    2003-01-01

    Utilizing the well-focused femtosecond laser with extreme high pulse intensity, we built a two-photon microfabrication and data storage system, which was introduced through several functional parts. Based on this homemade system, several three-dimensional microstructures were fabricated by two-photon polymerization, and three-dimensional data storage of six-layers was achieved by two-photon excitation with a photochromic material.

  18. Two-photon path-entangled states in multi-mode waveguides

    CERN Document Server

    Poem, Eilon; Silberberg, Yaron

    2012-01-01

    We experimentally show that two-photon path-entangled states can be coherently manipulated by multi-mode interference in multi-mode waveguides. By measuring the output two-photon spatial correlation function versus the phase of the input state, we show that multi-mode waveguides perform as nearly-ideal multi-port beam splitters at the quantum level, creating a large variety of entangled and separable multi-path two-photon states.

  19. Measurements of the Mass, Total Width and Two-Photon Partial Width of the $\\eta_{c}$ Meson

    CERN Document Server

    Brandenburg, G; Gao, Y S; Kim, D Y J; Wilson, R; Browder, T E; Li, Y; Rodríguez, J L; Yamamoto, H; Bergfeld, T; Eisenstein, B I; Ernst, J; Gladding, G E; Gollin, G D; Hans, R M; Johnson, E; Karliner, I; Marsh, M A; Palmer, M; Plager, C; Sedlack, C; Selen, M; Thaler, J J; Williams, J; Edwards, K W; Janicek, R; Patel, P M; Sadoff, A J; Ammar, R; Bean, A; Besson, D; Davis, R; Kwak, N; Zhao, X; Anderson, S; Frolov, V V; Kubota, Y; Lee, S J; Mahapatra, R; O'Neill, J J; Poling, R A; Riehle, T; Smith, A; Stepaniak, C J; Urheim, J; Ahmed, S; Alam, M S; Athar, S B; Jian, L; Ling, L; Saleem, M; Timm, S; Wappler, F; Anastassov, A; Duboscq, J E; Eckhart, E; Gan, K K; Gwon, C; Hart, T; Honscheid, K; Hufnagel, D; Kagan, H; Kass, R; Pedlar, T K; Schwarthoff, H; Thayer, J B; Von Törne, E; Zoeller, M M; Richichi, S J; Severini, H; Skubic, P L; Undrus, A; Chen, S; Fast, J; Hinson, J W; Lee, J; Miller, D H; Shibata, E I; Shipsey, I P J; Pavlunin, V; Cronin-Hennessy, D; Lyon, A L; Thorndike, E H; Jessop, C P; Marsiske, H; Perl, Martin Lewis; Savinov, V; Ugolini, D W; Zhou, X; Coan, T E; Fadeev, V; Maravin, Y; Narsky, I; Stroynowski, R; Ye, J; Wlodek, T; Artuso, M; Ayad, R; Boulahouache, C; Bukin, K; Dambasuren, E; Karamov, S; Majumder, G; Moneti, G C; Mountain, R; Schuh, S; Skwarnicki, T; Stone, S; Viehhauser, G; Wang, J C; Wolf, A; Wu, J; Kopp, S E; Mahmood, A H; Csorna, S E; Danko, I; McLean, K W; Marka, S; Xu, Z; Godang, R; Kinoshita, K; Lai, I C; Schrenk, S; Bonvicini, G; Cinabro, D; McGee, S; Perera, L P; Zhou, G J; Lipeles, E; Pappas, S P; Schmidtler, M; Shapiro, A; Sun, W M; Weinstein, A J; Würthwein, F; Jaffe, D E; Masek, G E; Paar, H P; Potter, E M; Prell, S; Sharma, V; Asner, D M; Eppich, A; Hill, T S; Morrison, R J; Briere, R A; Ferguson, T; Vogel, H; Behrens, B H; Ford, W T; Gritsan, A; Roy, J D; Smith, J G; Alexander, J P; Baker, R; Bebek, C; Berger, B E; Berkelman, K; Blanc, F; Boisvert, V; Cassel, David G; Dickson, M; Drell, P S; Ecklund, K M; Ehrlich, R; Foland, A D; Gaidarev, P B; Galik, R S; Gibbons, L K; Gittelman, B; Gray, S W; Hartill, D L; Heltsley, B K; Hopman, P I; Jones, C D; Kreinick, D L; Lohner, M; Magerkurth, A; Meyer, T O; Mistry, N B; Nordberg, E; Patterson, J R; Peterson, D; Riley, D; Thayer, J G; Thies, P G; Urner, D; Valant-Spaight, B L; Warburton, A; Avery, P; Prescott, C; Rubiera, A I; Yelton, J; Zheng, J

    2000-01-01

    Using 13.4 $fb^{-1}$ of data collected with the CLEO detector at the Cornell Electron Storage Ring, we have observed 300 events for the two-photon production of ground-state pseudo-scalar charmonium in the decay $\\eta_c$ -> $K_S K^{\\mp} \\pi^{\\pm}$. We have measured the $\\eta_c$ mass to be (2980.4 +- 2.3 (stat) +- 0.6 (sys)) MeV and its full width as (27.0 +- 5.8 (stat) +- 1.4 (sys)) MeV. We have determined the two-photon partial width of the $\\eta_c$ meson to be (7.6 +- 0.8 (stat) +- 0.4 (sys) +- 2.3 (br)) keV, with the last uncertainty associated with the decay branching fraction.

  20. Imaging of Fluoride Ion in Living Cells and Tissues with a Two-Photon Ratiometric Fluorescence Probe

    Directory of Open Access Journals (Sweden)

    Xinyue Zhu

    2015-01-01

    Full Text Available A reaction-based two-photon (TP ratiometric fluorescence probe Z2 has been developed and successfully applied to detect and image fluoride ion in living cells and tissues. The Z2 probe was designed designed to utilize an ICT mechanism between n-butylnaphthalimide as a fluorophore and tert-butyldiphenylsilane (TBDPS as a response group. Upon addition of fluoride ion, the Si-O bond in the Z2 would be cleaved, and then a stronger electron-donating group was released. The fluorescent changes at 450 and 540 nm, respectively, made it possible to achieve ratiometric fluorescence detection. The results indicated that the Z2 could ratiometrically detect and image fluoride ion in living cells and tissues in a depth of 250 μm by two-photon microscopy (TPM.

  1. Reconstruction of images from radiofrequency electron paramagnetic resonance spectra.

    Science.gov (United States)

    Smith, C M; Stevens, A D

    1994-12-01

    This paper discusses methods for obtaining image reconstructions from electron paramagnetic resonance (EPR) spectra which constitute object projections. An automatic baselining technique is described which treats each spectrum consistently; rotating the non-horizontal baselines which are caused by stray magnetic effects onto the horizontal axis. The convolved backprojection method is described for both two- and three-dimensional reconstruction and the effect of cut-off frequency on the reconstruction is illustrated. A slower, indirect, iterative method, which does a non-linear fit to the projection data, is shown to give a far smoother reconstructed image when the method of maximum entropy is used to determine the value of the final residual sum of squares. Although this requires more computing time than the convolved backprojection method, it is more flexible and overcomes the problem of numerical instability encountered in deconvolution. Images from phantom samples in vitro are discussed. The spectral data for these have been accumulated quickly and have a low signal-to-noise ratio. The results show that as few as 16 spectra can still be processed to give an image. Artifacts in the image due to a small number of projections using the convolved backprojection reconstruction method can be removed by applying a threshold, i.e. only plotting contours higher than a given value. These artifacts are not present in an image which has been reconstructed by the maximum entropy technique. At present these techniques are being applied directly to in vivo studies.

  2. A new electron paramagnetic resonance method to identify irradiated soybean.

    Science.gov (United States)

    Sanyal, Bhaskar; Sharma, Arun

    2009-10-01

    Low-dose gamma irradiation causes minimal changes in food matrix making identification of radiation-processed foods a challenging task. In the present study, soybean samples were irradiated with commercially permitted gamma radiation dose in the 0.25 to 1.0 kGy range for insect disinfestations of food. Immediately after irradiation electron paramagnetic resonance (EPR) spectrum of the skin part of soybean showed a triplet signal (g = 2.0046, hyperfine coupling constant hfcc = 3.0 mT) superimposed on naturally present singlet. These signals were characterized as cellulose and phenoxyl radicals using EPR spectrum simulation technique. Kernel part of the samples exhibited a short-lived, radiation-induced singlet of carbon-centered radical superimposed on naturally present sextet signal of Mn2+. A detailed study on relaxation and thermal behavior of induced radicals in skin part was carried out using EPR spectroscopy. These findings revealed that progressive saturation and thermal characteristics of the induced radicals may be the most suitable parameters to distinguish soybean subjected to radiation dose as low as 0.25 kGy from thermally treated and nonirradiated samples, even after a prolonged period of storage.

  3. Identification of irradiated cashew nut by electron paramagnetic resonance spectroscopy.

    Science.gov (United States)

    Sanyal, Bhaskar; Sajilata, M G; Chatterjee, Suchandra; Singhal, Rekha S; Variyar, Prasad S; Kamat, M Y; Sharma, Arun

    2008-10-01

    Cashew nut samples were irradiated at gamma-radiation doses of 0.25, 0.5, 0.75, and 1 kGy, the permissible dose range for insect disinfestation of food commodities. A weak and short-lived triplet (g = 2.004 and hfcc = 30 G) along with an anisotropic signal (g perpendicular = 2.0069 and g parallel = 2.000) were produced immediately after irradiation. These signals were assigned to that of cellulose and CO 2 (-) radicals. However, the irradiated samples showed a dose-dependent increase of the central line (g = 2.0045 +/- 0.0002). The nature of the free radicals formed during conventional processing such as thermal treatment was investigated and showed an increase in intensity of the central line (g = 2.0045) similar to that of irradiation. Characteristics of the free radicals were studied by their relaxation and thermal behaviors. The present work explores the possibility to identify irradiated cashew nuts from nonirradiated ones by the thermal behaviors of the radicals beyond the period, when the characteristic electron paramagnetic resonance spectral lines of the cellulose free radicals have essentially disappeared. In addition, this study for the first time reports that relaxation behavior of the radicals could be a useful tool to distinguish between roasted and irradiated cashew nuts.

  4. Two dimensional electron spin resonance: Structure and dynamics of biomolecules

    Science.gov (United States)

    Saxena, Sunil; Freed, Jack H.

    1998-03-01

    The potential of two dimensional (2D) electron spin resonance (ESR) for measuring the structural properties and slow dynamics of labeled biomolecules will be presented. Specifically, it will be shown how the recently developed method of double quantum (DQ) 2D ESR (S. Saxena and J. H. Freed, J. Chem. Phys. 107), 1317, (1997) can be used to measure large interelectron distances in bilabeled peptides. The need for DQ ESR spectroscopy, as well as the challenges and advantages of this method will be discussed. The elucidation of the slow reorientational dynamics of this peptide (S. Saxena and J. H. Freed, J. Phys. Chem. A, 101) 7998 (1997) in a glassy medium using COSY and 2D ELDOR ESR spectroscopy will be demonstrated. The contributions to the homogeneous relaxation time, T_2, from the overall and/or internal rotations of the nitroxide can be distinguished from the COSY spectrum. The growth of spectral diffusion cross-peaks^2 with mixing time in the 2D ELDOR spectra can be used to directly determine a correlation time from the experiment which can be related to the rotational correlation time.

  5. Uniform spinning sampling gradient electron paramagnetic resonance imaging.

    Science.gov (United States)

    Johnson, David H; Ahmad, Rizwan; Liu, Yangping; Chen, Zhiyu; Samouilov, Alexandre; Zweier, Jay L

    2014-02-01

    To improve the quality and speed of electron paramagnetic resonance imaging (EPRI) acquisition by combining a uniform sampling distribution with spinning gradient acquisition. A uniform sampling distribution was derived for spinning gradient EPRI acquisition (uniform spinning sampling, USS) and compared to the existing (equilinear spinning sampling, ESS) acquisition strategy. Novel corrections were introduced to reduce artifacts in experimental data. Simulations demonstrated that USS puts an equal number of projections near each axis whereas ESS puts excessive projections at one axis, wasting acquisition time. Artifact corrections added to the magnetic gradient waveforms reduced noise and correlation between projections. USS images had higher SNR (85.9 ± 0.8 vs. 56.2 ± 0.8) and lower mean-squared error than ESS images. The quality of the USS images did not vary with the magnetic gradient orientation, in contrast to ESS images. The quality of rat heart images was improved using USS compared to that with ESS or traditional fast-scan acquisitions. A novel EPRI acquisition which combines spinning gradient acquisition with a uniform sampling distribution was developed. This USS spinning gradient acquisition offers superior SNR and reduced artifacts compared to prior methods enabling potential improvements in speed and quality of EPR imaging in biological applications. Copyright © 2013 Wiley Periodicals, Inc.

  6. Electron paramagnetic resonance in Cu-doped ZnO

    Science.gov (United States)

    Buchheit, R.; Acosta-Humánez, F.; Almanza, O.

    2016-04-01

    In this work, ZnO and Cu-doped ZnO nanoparticles (Zn1-xCuxO, x = 3%), with a calcination temperature of 500∘C were synthesized using the sol-gel method. The particles were analyzed using atomic absorption spectroscopy (AAS), X-ray diffraction (XRD) and electron paramagnetic resonance (EPR) at X-band, measurement in a temperature range from 90 K to room temperature. AAS confirmed a good correspondence between the experimental doping concentration and the theoretical value. XRD reveals the presence of ZnO phase in hexagonal wurtzite structure and a nanoparticle size for the samples synthesized. EPR spectroscopy shows the presence of point defects in both samples with g-values of g = 1.959 for shallow donors and g = 2.004 for ionized vacancies. It is important when these materials are required have been used as catalysts, as suggested that it is not necessary prepare them at higher temperature. A simulation of the Cu EPR signal using an anisotropic spin Hamiltonian was performed and showed good coincidence with the experimental spectra. It was shown that Cu2+ ions enter interstitial octahedral sites of orthorhombic symmetry in the wurtzite crystal structure. Temperature dependence of the EPR linewidth and signal intensity shows a paramagnetic behavior of the sample in the measurement range. A Néel temperature TN = 78 ± 19 K was determined.

  7. Mechanical detection of electron spin resonance beyond 1 THz

    Energy Technology Data Exchange (ETDEWEB)

    Takahashi, Hideyuki [Organization of Advanced Science and Technology, Kobe University, 1-1, Rokkodai, Nada, Kobe 657-8501 (Japan); Ohmichi, Eiji [Graduate School of Science, Kobe University, 1-1 Rokkodai-cho, Nada, Kobe 657-8501 (Japan); Ohta, Hitoshi [Molecular Photoscience Research Center, Kobe University, 1-1 Rokkodai-cho, Nada, Kobe 657-8501 (Japan)

    2015-11-02

    We report the cantilever detection of electron spin resonance (ESR) in the terahertz (THz) region. This technique mechanically detects ESR as a change in magnetic torque that acts on the cantilever. The ESR absorption of a tiny single crystal of Co Tutton salt, Co(NH{sub 4}){sub 2}(SO{sub 4}){sub 2}⋅6H{sub 2}O, was observed in frequencies of up to 1.1 THz using a backward travelling wave oscillator as a THz-wave source. This is the highest frequency of mechanical detection of ESR till date. The spectral resolution was evaluated with the ratio of the peak separation to the sum of the half-width at half maximum of two absorption peaks. The highest resolution value of 8.59 ± 0.53 was achieved at 685 GHz, while 2.47 ± 0.01 at 80 GHz. This technique will not only broaden the scope of ESR spectroscopy application but also lead to high-spectral-resolution ESR imaging.

  8. Electron magnetic resonance of gadolinium-doped calcium fluoride

    Energy Technology Data Exchange (ETDEWEB)

    Biasi, R.S. de, E-mail: rsbiasi@ime.eb.br [Secao de Engenharia Mecanica e de Materiais, Instituto Militar de Engenharia, 22290-270 Rio de Janeiro, RJ (Brazil); Grillo, M.L.N., E-mail: mluciag@uerj.br [Instituto de Fisica, Universidade do Estado do Rio de Janeiro, 20550-013 Rio de Janeiro, RJ (Brazil)

    2012-06-15

    Electron magnetic resonance (EMR) spectra of gadolinium-doped calcium fluoride have been studied at room temperature for Gd concentrations between 0.01 and 2.00 mol%. Gd{sup 3+} ions in sites with two different symmetries were observed. One of the sites, with cubic symmetry, is unstable at room temperature and decays with a time constant of 2.2 day{sup -1}. The other site, with tetragonal symmetry, is stable and is attributed to Gd{sup 3+} ions in substitutional sites next to a charge-compensating F{sup -} interstitial ion. The linewidth and intensity of the EMR spectrum with tetragonal symmetry increase with increasing Gd concentration. A theoretical calculation based on the concentration dependence of the EMR linewidth yields an effective range of the exchange interaction between Gd{sup 3+} ions in CaF{sub 2} of 0.774 nm, of the same order as that of Gd{sup 3+} ions in other cubic ionic compounds.

  9. Broadband Two-Photon Absorption Characteristics of Highly Photostable Fluorenyl-Dicyanoethylenylated [60]Fullerene Dyads

    Directory of Open Access Journals (Sweden)

    Seaho Jeon

    2016-05-01

    Full Text Available We synthesized four C60-(light-harvesting antenna dyads C60 (>CPAF-Cn (n = 4, 9, 12, or 18 1-Cn for the investigation of their broadband nonlinear absorption effect. Since we have previously demonstrated their high function as two-photon absorption (2PA materials at 1000 nm, a different 2PA wavelength of 780 nm was applied in the study. The combined data taken at two different wavelength ranges substantiated the broadband characteristics of 1-Cn. We proposed that the observed broadband absorptions may be attributed by a partial π-conjugation between the C60 > cage and CPAF-Cn moieties, via endinitrile tautomeric resonance, giving a resonance state with enhanced molecular conjugation. This transient state could increase its 2PA and excited-state absorption at 800 nm. In addition, a trend of concentration-dependent 2PA cross-section (σ2 and excited-state absorption magnitude was detected showing a higher σ value at a lower concentration that was correlated to increasing molecular separation with less aggregation for dyads C60(>CPAF-C18 and C60(>CPAF-C9, as better 2PA and excited-state absorbers.

  10. Two-photon Photoemission of Organic Semiconductor Molecules on Ag(111)

    Energy Technology Data Exchange (ETDEWEB)

    Yang, Aram [Univ. of California, Berkeley, CA (United States)

    2008-05-01

    Angle- and time-resolved two-photon photoemission (2PPE) was used to study systems of organic semiconductors on Ag(111). The 2PPE studies focused on electronic behavior specific to interfaces and ultrathin films. Electron time dynamics and band dispersions were characterized for ultrathin films of a prototypical n-type planar aromatic hydrocarbon, PTCDA, and representatives from a family of p-type oligothiophenes.In PTCDA, electronic behavior was correlated with film morphology and growth modes. Within a fewmonolayers of the interface, image potential states and a LUMO+1 state were detected. The degree to which the LUMO+1 state exhibited a band mass less than a free electron mass depended on the crystallinity of the layer. Similarly, image potential states were measured to have free electron-like effective masses on ordered surfaces, and the effective masses increased with disorder within the thin film. Electron lifetimes were correlated with film growth modes, such that the lifetimes of electrons excited into systems created by layer-by-layer, amorphous film growth increased by orders of magnitude by only a few monolayers from the surface. Conversely, the decay dynamics of electrons in Stranski-Krastanov systems were limited by interaction with the exposed wetting layer, which limited the barrier to decay back into the metal.Oligothiophenes including monothiophene, quaterthiophene, and sexithiophene were deposited on Ag(111), and their electronic energy levels and effective masses were studied as a function of oligothiophene length. The energy gap between HOMO and LUMO decreased with increasing chain length, but effective mass was found to depend on domains from high- or low-temperature growth conditions rather than chain length. In addition, the geometry of the molecule on the surface, e.g., tilted or planar, substantially affected the electronic structure.

  11. Description of the states of two-photon interference in an optical gating Michelson interferometer

    Science.gov (United States)

    Pongophas, Ekkarat; Sriklin, Watthana; Sinsarp, Asawin; Suwanna, Sujin; Chunwachirasiri, Withoon; Singhsomroje, Wisit

    2016-01-01

    We investigate the interference of two photons in an optical gating Michelson interferometer. The phenomenon is studied using two different representations of photons: the space-time domain and a step-by-step two-photon state evolution. Both representations lead to identical results. The evolution analysis describes the result by the interference of four two-photon traveling states, whereas the space-time domain analysis reveals that the classical interference of the high-intensity light source is identical to two-photon interference in the quantum regime, except for a multiplicative factor of (n2), where n is the number of photons.

  12. Two-photon induced photoluminescence and singlet oxygen generation from aggregated gold nanoparticles.

    Science.gov (United States)

    Jiang, Cuifeng; Zhao, Tingting; Yuan, Peiyan; Gao, Nengyue; Pan, Yanlin; Guan, Zhenping; Zhou, Na; Xu, Qing-Hua

    2013-06-12

    Metal nanoparticles have potential applications as bioimaging and photosensitizing agents. Aggregation effects are generally believed to be adverse to their biomedical applications. Here we have studied the aggregation effects on two-photon induced photoluminescence and singlet oxygen generation of Au nanospheres and Au nanorods of two different aspect ratios. Aggregated Au nanospheres and short Au nanorods were found to display enhanced two-photon induced photoluminescence and singlet oxygen generation capabilities compared to the unaggregated ones. The two-photon photoluminescence of Au nanospheres and short Au nanorods were enhanced by up to 15.0- and 2.0-fold upon aggregation, and the corresponding two-photon induced singlet oxygen generation capabilities were enhanced by 8.3 and 1.8-fold, respectively. The two-photon induced photoluminescence and singlet oxygen generation of the aggregated long Au nanorods were found to be lower than the unaggregated ones. These results support that the change in their two-photon induced photoluminescence and singlet oxygen generation originate from aggregation modulated two-photon excitation efficiency. This finding is expected to foster more biomedical applications of metal nanoparticles as Au nanoparticles normally exist in an aggregated form in the biological environments. Considering their excellent biocompatibility, high inertness, ready conjugation, and easy preparation, Au nanoparticles are expected to find more applications in two-photon imaging and two-photon photodynamic therapy.

  13. Synthesis of two carbazole-based dyes and application of two-photon initiating polymerization

    Institute of Scientific and Technical Information of China (English)

    2009-01-01

    Two carbazole-based polymerization initiators possessing blue fluorescence emission have been synthesized via Wittig reaction in the solid phase at room temperature.Two-photon excited fluorescence(TPEF) spectra for them were investigated under 800 nm fs laser pulse and two-photon absorption cross sections were determined by the Z-scan technique.Then two-photon initiating polymerization(TPIP) microfabrication experiments were successfully carried out.Three-dimensional lattice and artificial defects were gained,indicating that they were viable candidates for the two-photon polymerization initiator in practical application of microfabrication.

  14. Time-reversed two-photon interferometry for phase super-resolution

    CERN Document Server

    Ogawa, Kazuhisa; Kobayashi, Hirokazu; Nakanishi, Toshihiro; Kitano, Masao

    2013-01-01

    We observed two-photon phase super-resolution in an unbalanced Michelson interferometer with classical Gaussian laser pulses. Our work is a time-reversed version of a two-photon interference experiment using an unbalanced Michelson interferometer. A measured interferogram exhibits two-photon phase super-resolution with a high visibility of 97.9% \\pm 0.4%. Its coherence length is about 22 times longer than that of the input laser pulses. It is a classical analogue to the large difference between the one- and two-photon coherence lengths of entangled photon pairs.

  15. Synthesis of two carbazole-based dyes and application of two-photon initiating polymerization

    Institute of Scientific and Technical Information of China (English)

    HU RenTao; LU LiangFei; RUAN BanFeng; WANG Peng; ZHANG MingLiang; ZHOU HongPing; LI ShengLi; WU JieYing; TIAN YuPeng

    2009-01-01

    Two carbazole-based polymerization initiators possessing blue fluorescence emission have been synthesized via Wittig reaction in the solid phase at room temperature.Two-photon excited fluorescence (TPEF) spectra for them were investigated under 800 nm fs laser pulse and two-photon absorption cross sections were determined by the Z-scan technique.Then two-photon initiating polymerization (TPIP) microfabrication experiments were successfully carried out.Three-dimensional lattice and artificial defects were gained,indicating that they were viable candidates for the two-photon polymerization initiator in practical application of microfabrication.

  16. Experimental constraints on non-linearities induced by two-photon effects in elastic and inelastic Rosenbluth separations

    Energy Technology Data Exchange (ETDEWEB)

    Vladas Tvaskis; John Arrington; Michael Christy; Rolf Ent; Cynthia Keppel; Yongguang Liang; Grahame Vittorini

    2006-01-26

    The effects of two-photon exchange corrections, suggested to explain the difference between measurements of the proton elastic electromagnetic form factors using the polarization transfer and Rosenbluth techniques, have been studied in elastic and inelastic scattering data. Such corrections could introduce epsilon-dependent non-linearities in inelastic Rosenbluth separations, where epsilon is the virtual photon polarization parameter. It is concluded that such non-linear effects are consistent with zero for elastic, resonance, and deep-inelastic scattering for all Q{sup 2} and W{sup 2} values measured.

  17. Phase- and Polarization-Controlled Two-Photon Rabi Oscillation of the Biexciton State in a Semiconductor Quantum Dot

    Directory of Open Access Journals (Sweden)

    Erlin Sun

    2014-01-01

    Full Text Available Under a degenerate two-photon resonant excitation, the Rabi oscillation of the four-level biexciton system in a semiconductor quantum dot is theoretically investigated. The influence of the laser phases on the state manipulation is modeled and numerically calculated. Due to the interference between different excitation paths, the laser phase plays an important role and can be utilized as an alternate control knob to coherently manipulate the biexciton state. The phase control can be facilely implemented by changing the light polarization via a quarter-wave plate.

  18. Electron spin resonance and transient photocurrent measurements on microcrystalline silicon

    Energy Technology Data Exchange (ETDEWEB)

    Dylla, T.

    2004-09-01

    The electronic properties of microcrystalline silicon ({mu}c-Si:H) films have been studied using electron spin resonance (ESR), transient photocurrent time-of-flight (TOF) techniques, and electrical conductivity measurements. Structural properties were determined by Raman spectroscopy. A wide range of structure compositions, from highly crystalline films with no discernable amorphous content, to predominantly amorphous films with no crystalline phase contributions, was investigated. Models and possible explanations concerning the nature and energetic distribution of electronic defects as a function of film composition are discussed. It is shown that the spin density N{sub S} in {mu}c-Si:H films is linked strongly to the structure composition of the material. Both reversible and irreversible changes in the ESR signal and dark conductivity due to atmospheric effects are found in {mu}c-Si:H. The porous structure of highly crystalline material facilitates in-diffusion of atmospheric gases, which strongly affects the character and/or density of surface states. Two contributing processes have been identified, namely adsorption and oxidation. Both processes lead to an increase of N{sub S}. Measurements on n-type {mu}c-Si:H films were used as a probe of the density of gap states, confirming that the spin density NS is related to the density of defects. The results confirm that for a wide range of structural compositions, the doping induced Fermi level shift in {mu}c-Si:H is governed by compensation of defect states, for doping concentrations up to the dangling bond spin density. At higher concentrations a doping efficiency close to unity was found, confirming that in {mu}c-Si:H the measured spin densities represent the majority of gap states (N{sub S}=N{sub DB}). By applying the TOF technique to study pin solar cells based on {mu}c-Si:H, conclusive hole drift mobility data were obtained. Despite the predominant crystallinity of these samples, the temperature-dependence of

  19. Prospects for advanced electron cyclotron resonance and electron beam ion source charge breeding methods for EURISOL

    Energy Technology Data Exchange (ETDEWEB)

    Delahaye, P.; Jardin, P.; Maunoury, L.; Traykov, E.; Varenne, F. [GANIL, CEA/DSM-CNRS/IN2P3, Bd. Becquerel, BP 55027, 14076 Caen Cedex 05 (France); Galata, A.; Porcellato, A. M.; Prete, G. F. [INFN-Laboratori Nazionali di Legnaro, Viale dell' Universita 2, 35020 Legnaro, Padova (Italy); Angot, J.; Lamy, T.; Sortais, P.; Thuillier, T. [LPSC Grenoble, 53, rue des Martyrs, 38026 Grenoble Cedex (France); Ban, G. [LPC Caen, 6 bd Marechal Juin, 14050 Caen Cedex (France); Celona, L.; Lunney, D. [INFN-Laboratori Nazionali del Sud, via S.Sofia 62, 95125 Catania (Italy); Choinski, J.; Gmaj, P.; Jakubowski, A.; Steckiewicz, O. [Heavy Ion Laboratory, University of Warsaw, ul. Pasteura 5a, 02 093 Warsaw (Poland); Kalvas, T. [Department of Physics, University of Jyvaeskylae, PB 35 (YFL) 40351 Jyvaeskylae (Finland); and others

    2012-02-15

    As the most ambitious concept of isotope separation on line (ISOL) facility, EURISOL aims at producing unprecedented intensities of post-accelerated radioactive isotopes. Charge breeding, which transforms the charge state of radioactive beams from 1+ to an n+ charge state prior to post-acceleration, is a key technology which has to overcome the following challenges: high charge states for high energies, efficiency, rapidity and purity. On the roadmap to EURISOL, a dedicated R and D is being undertaken to push forward the frontiers of the present state-of-the-art techniques which use either electron cyclotron resonance or electron beam ion sources. We describe here the guidelines of this R and D.

  20. Multifunctional superparamagnetic nanoshells: combining two-photon luminescence imaging, surface-enhanced Raman scattering and magnetic separation

    Science.gov (United States)

    Jin, Xiulong; Li, Haiyan; Wang, Shanshan; Kong, Ni; Xu, Hong; Fu, Qihua; Gu, Hongchen; Ye, Jian

    2014-11-01

    constructed a novel type of core-shell superparamagnetic nanoshell (Fe3O4@SiO2@Au), composed of a Fe3O4 cluster core, a thin Au shell and a SiO2 layer in between. The obtained multifunctional nanoparticles combine the magnetic properties and plasmonic optical properties effectively, which were well investigated by a number of experimental characterization methods and theoretical simulations. We have demonstrated that Fe3O4@SiO2@Au nanoparticles can be utilized for two-photon luminescence (TPL) imaging, near-infrared surface-enhanced Raman scattering (NIR SERS) and cell collection by magnetic separation. The TPL intensity could be further greatly enhanced through the plasmon coupling effect in the self-assembled nanoparticle chains, which were triggered by an external magnetic field. In addition, Fe3O4@SiO2@Au nanoparticles may have great potential applications such as enhanced magnetic resonance imaging (MRI) and photo-thermotherapy. Successful combination of multifunctions including magnetic response, biosensing and bioimaging in single nanoparticles allows further manipulation, real-time tracking, and intracellular molecule analysis of live cells at a single-cell level. Electronic supplementary information (ESI) available. See DOI: 10.1039/c4nr04111a

  1. Plasmon-exciton coupling at Ag nanocluster decorated TiO2(110) surface studied by time-resolved two-photon photoemission spectroscopy

    Science.gov (United States)

    Tan, Shijing; Argondizzo, Adam; Petek, Hrvoje

    We study the spectroscopy and electron dynamics at Ag nanocluster decorated TiO2(110) surface upon photoexcitation of plasmonic modes by two-photon photoemission spectroscopy (2PP). Depositing Ag onto a reduced rutile TiO2(110) surface at room temperature forms pancake-like Ag particles with an average diameter of 4 nm and height of 1.5 nm. Measurements of the 2PP yield from Ag/TiO2 surface with tunable femtosecond laser excitation show enhancement at plasmonic resonances. Exciting with s-polarization (S -->) the plasmonic resonance enhancement has a single peak at 3.1 eV, whereas with p-polarization (P -->) there is an additional more intense resonance at 3.8 eV. We attribute the 3.1 and 3.8 eV peaks to the in-plane and the surface-normal plasmon modes respectively. Crystal azimuth orientation dependent excitation with (S -->) shows an anisotropy in the 2PP spectra for the 3.1 eV in-plane plasmon mode when the laser electric field is aligned in the [001] vs. [ 1 1 0 ] directions. The existence of two plasmon modes and the in-plane plasmon anisotropy imply that the plasmon modes are perturbed by coherent coupling with excitons in the rutile TiO2 substrate. We speculate that plasmon-exciton resonant energy transfer could play an important role in the plasmonically enhanced photocatalysis at the Ag/TiO2 surface.

  2. Temperature and density evolution during decay in a 2.45 GHz hydrogen electron cyclotron resonance plasma: Off-resonant and resonant cases

    Energy Technology Data Exchange (ETDEWEB)

    Cortázar, O. D. [ESS Bilbao, Edificio Cosimet, Landabarri 2, 48940-Leioa, Vizcaya (Spain); Universidad de Castilla-La Mancha, ETSII, C.J. Cela s/n, 13170 Ciudad Real (Spain); Megía-Macías, A.; Vizcaíno-de-Julián, A. [ESS Bilbao, Edificio Cosimet, Landabarri 2, 48940-Leioa, Vizcaya (Spain)

    2013-09-15

    Time resolved electron temperature and density measurements during the decay stage in a hydrogen electron cyclotron resonance (ECR) plasma are presented for a resonance and off-resonance magnetic field configurations. The measurements are conducted on a ECR plasma generator excited at 2.45 GHz denominated test-bench for ion-sources plasma studies at ESS Bilbao. The plasma parameters evolution is studied by Langmuir probe diagnostic with synchronized sample technique developed for repetitive pulsed plasmas with a temporal resolution of 200 ns in typical decay processes of about 40 μs. An afterglow transient is clearly observed in the reflected microwave power signal from the plasma. Simultaneously, the electron temperature evolution shows rebounding peaks that may be related to the interplay between density drop and microwave coupling with deep impact on the Electron Energy Distribution Function. The correlation of such structures with the plasma absorbed power and the coupling quality is also reported.

  3. Strong-field QED processes in short laser pulses. One- and two-photon Compton scattering

    Energy Technology Data Exchange (ETDEWEB)

    Seipt, Daniel

    2012-12-20

    The purpose of this thesis is to advance the understanding of strong-field QED processes in short laser pulses. The processes of non-linear one-photon and two-photon Compton scattering are studied, that is the scattering of photons in the interaction of relativistic electrons with ultra-short high-intensity laser pulses. These investigations are done in view of the present and next generation of ultra-high intensity optical lasers which are supposed to achieve unprecedented intensities of the order of 10{sup 24} W/cm{sup 2} and beyond, with pulse lengths in the order of some femtoseconds. The ultra-high laser intensity requires a non-perturbative description of the interaction of charged particles with the laser field to allow for multi-photon interactions, which is beyond the usual perturbative expansion of QED organized in powers of the fine structure constant. This is achieved in strong-field QED by employing the Furry picture and non-perturbative solutions of the Dirac equation in the presence of a background laser field as initial and final state wave functions, as well as the laser dressed Dirac-Volkov propagator. The primary objective is a realistic description of scattering processes with regard to the finite laser pulse duration beyond the common approximation of infinite plane waves, which is made necessary by the ultra-short pulse length of modern high-intensity lasers. Non-linear finite size effects are identified, which are a result of the interplay between the ultra-high intensity and the ultra-short pulse length. In particular, the frequency spectra and azimuthal photon emission spectra are studied emphasizing the differences between pulsed and infinite laser fields. The proper description of the finite temporal duration of the laser pulse leads to a regularization of unphysical infinities (due to the infinite plane-wave description) of the laser-dressed Dirac-Volkov propagator and in the second-order strong-field process of two-photon Compton

  4. Exp erimental study of the effects of two-photon detuning on slow light and light memory%双光子失谐对慢光和光存储影响的实验研究∗

    Institute of Scientific and Technical Information of China (English)

    闫研; 李淑静; 田龙; 王海

    2016-01-01

    Electromagnetically induced transparency (EIT) effect is an effective means to store light field into the atom ensemble. The extra noise introduced in the stored procedure can be suppressed greatly under the condition of large one-photon detuning and proper two-photon detuning. In this paper, we experimentally investigate the slow light and light storage in 87Rb vapor by using EIT effect, and study the effects of the two-photon detuning on light pulse delay and light memory at 650 MHz one-photon red detuning. In order to avoid some unwanted effects under the high optical depth condition, such as four-wave mixing, etc., the temperature of the atomic cell is controlled at 65 degrees Celsius. The experimental results show that the delay and the retrieval signals are significant in a two-photon detuning range from 0 to 0.5 MHz. The pulse delay decreases with the increase of two-photon detuning. The delay is 0.36 µs at two-photon resonance, and it is 0.07 µs at 1 MHz two-photon detuning. We simulate the delayed light pulse by using a three-levelΛ-type EIT model. The shapes of the measured slow light are in agreement with the theoretical results. The retrieval signals are observed at different two-photon detunings. The shapes of the retrieval pulses change with the two-photon detuning. The shape variations of the retrieval pulses cannot be explained by the three-level EIT theoretical model. By considering the atomic Zeeman sublevels interacting with the left-circular and right-circular polarized components of probe and coupling fields, multiple Λ-type EIT systems will be formed. The interference between the retrieval signals from multiple EIT subsystems causes the shape distortions of retrieval pulses. The retrieval efficiency is measured as a function of two-photon detuning. The retrieval efficiency oscillates, and multiple peaks appear with the increase of two-photon detuning. The first peak appears at two-photon resonance, and the second peak appears at 0.48 MHz

  5. On Cu(II) Cu(II) distance measurements using pulsed electron electron double resonance

    Science.gov (United States)

    Yang, Zhongyu; Becker, James; Saxena, Sunil

    2007-10-01

    The effects of orientational selectivity on the 4-pulse electron electron double resonance (PELDOR) ESR spectra of coupled Cu(II)-Cu(II) spins are presented. The data were collected at four magnetic fields on a poly-proline peptide containing two Cu(II) centers. The Cu(II)-PELDOR spectra of this peptide do not change appreciably with magnetic field at X-band. The data were analyzed by adapting the theory of Maryasov, Tsvetkov, and Raap [A.G. Maryasov, Y.D. Tsvetkov, J. Raap, Weakly coupled radical pairs in solids:ELDOR in ESE structure studies, Appl. Magn. Reson. 14 (1998) 101-113]. Simulations indicate that orientational effects are important for Cu(II)-PELDOR. Based on simulations, the field-independence of the PELDOR data for this peptide is likely due to two effects. First, for this peptide, the Cu(II) g-tensor(s) are in a very specific orientation with respect to the interspin vector. Second, the flexibility of the peptide washes out the orientation effects. These effects reduce the suitability of the poly-proline based peptide as a good model system to experimentally probe orientational effects in such experiments. An average Cu(II)-Cu(II) distance of 2.1-2.2 nm was determined, which is consistent with earlier double quantum coherence ESR results.

  6. Ejected-electron spectroscopy of autoionizing resonances of helium excited by fast-electron impact

    Science.gov (United States)

    Zhang, Zhe; Shan, Xu; Wang, Enliang; Chen, Xiangjun

    2012-06-01

    The autoionizing resonances (2s2)1S, (2p2)1D, and (2s2p)1P of helium have been investigated employing ejected-electron spectroscopy by fast-electron impact at incident energies of 250-2000 eV and ejected angles of 26°-116°. Shore parameters of the line shapes for these three resonances have been obtained in such high incident energy regime except at 250 eV. Distinct discrepancies between the present results at 250 eV and those of McDonald and Crowe at 200 eV [D. G. McDonald and A. Crowe, J. Phys. BJPAMA40953-407510.1088/0953-4075/25/9/018 25, 2129 (1992); D. G. McDonald and A. Crowe, J. Phys. BJPAMA40953-407510.1088/0953-4075/25/20/024 25, 4313 (1992)] and Sise at 250 eV [O. Sise, M. Dogan, I. Okur, and A. Crowe, Phys. Rev. APLRAAN1050-294710.1103/PhysRevA.84.022705 84, 022705 (2011)], especially for 1D and 1P states, are also observed.

  7. The Strength of Chaos: Accurate Simulation of Resonant Electron Scattering by Many-Electron Ions and Atoms in the Presence of Quantum Chaos

    Science.gov (United States)

    2017-01-20

    AFRL-AFOSR-JP-TR-2017-0012 The Strength of Chaos: accurate simulation of resonant electron scattering by many-electron ions and atoms in the presence...SUBTITLE The Strength of Chaos: accurate simulation of resonant electron scattering by many- electron ions and atoms in the presence of quantum chaos...Strength of Chaos: accurate simulation of resonant electron scattering by many-electron ions and atoms in the presence of quantum chaos” Date 13

  8. Direct detection of resonant electron pitch angle scattering by whistler waves in a laboratory plasma.

    Science.gov (United States)

    Van Compernolle, B; Bortnik, J; Pribyl, P; Gekelman, W; Nakamoto, M; Tao, X; Thorne, R M

    2014-04-11

    Resonant interactions between energetic electrons and whistler mode waves are an essential ingredient in the space environment, and in particular in controlling the dynamic variability of Earth's natural radiation belts, which is a topic of extreme interest at the moment. Although the theory describing resonant wave-particle interaction has been present for several decades, it has not been hitherto tested in a controlled laboratory setting. In the present Letter we report on the first laboratory experiment to directly detect resonant pitch angle scattering of energetic (∼keV) electrons due to whistler mode waves. We show that the whistler mode wave deflects energetic electrons at precisely the predicted resonant energy, and that varying both the maximum beam energy, and the wave frequency, alters the energetic electron beam very close to the resonant energy.

  9. Variable Coupling Scheme for High Frequency Electron Spin Resonance Resonators Using Asymmetric Meshes.

    Science.gov (United States)

    Tipikin, D S; Earle, K A; Freed, J H

    2010-01-01

    The sensitivity of a high frequency electron spin resonance (ESR) spectrometer depends strongly on the structure used to couple the incident millimeter wave to the sample that generates the ESR signal. Subsequent coupling of the ESR signal to the detection arm of the spectrometer is also a crucial consideration for achieving high spectrometer sensitivity. In previous work, we found that a means for continuously varying the coupling was necessary for attaining high sensitivity reliably and reproducibly. We report here on a novel asymmetric mesh structure that achieves continuously variable coupling by rotating the mesh in its own plane about the millimeter wave transmission line optical axis. We quantify the performance of this device with nitroxide spin-label spectra in both a lossy aqueous solution and a low loss solid state system. These two systems have very different coupling requirements and are representative of the range of coupling achievable with this technique. Lossy systems in particular are a demanding test of the achievable sensitivity and allow us to assess the suitability of this approach for applying high frequency ESR to the study of biological systems at physiological conditions, for example. The variable coupling technique reported on here allows us to readily achieve a factor of ca. 7 improvement in signal to noise at 170 GHz and a factor of ca. 5 at 95 GHz over what has previously been reported for lossy samples.

  10. Statistical reconstruction algorithms for continuous wave electron spin resonance imaging

    Science.gov (United States)

    Kissos, Imry; Levit, Michael; Feuer, Arie; Blank, Aharon

    2013-06-01

    Electron spin resonance imaging (ESRI) is an important branch of ESR that deals with heterogeneous samples ranging from semiconductor materials to small live animals and even humans. ESRI can produce either spatial images (providing information about the spatially dependent radical concentration) or spectral-spatial images, where an extra dimension is added to describe the absorption spectrum of the sample (which can also be spatially dependent). The mapping of oxygen in biological samples, often referred to as oximetry, is a prime example of an ESRI application. ESRI suffers frequently from a low signal-to-noise ratio (SNR), which results in long acquisition times and poor image quality. A broader use of ESRI is hampered by this slow acquisition, which can also be an obstacle for many biological applications where conditions may change relatively quickly over time. The objective of this work is to develop an image reconstruction scheme for continuous wave (CW) ESRI that would make it possible to reduce the data acquisition time without degrading the reconstruction quality. This is achieved by adapting the so-called "statistical reconstruction" method, recently developed for other medical imaging modalities, to the specific case of CW ESRI. Our new algorithm accounts for unique ESRI aspects such as field modulation, spectral-spatial imaging, and possible limitation on the gradient magnitude (the so-called "limited angle" problem). The reconstruction method shows improved SNR and contrast recovery vs. commonly used back-projection-based methods, for a variety of simulated synthetic samples as well as in actual CW ESRI experiments.

  11. Pressure broadening of atomic oxygen two-photon absorption laser induced fluorescence

    Science.gov (United States)

    Marinov, Daniil; Drag, Cyril; Blondel, Christophe; Guaitella, Olivier; Golda, Judith; Klarenaar, Bart; Engeln, Richard; Schulz-von der Gathen, Volker; Booth, Jean-Paul

    2016-12-01

    Atomic oxygen, considered to be a determining reactant in plasma applications at ambient pressure, is routinely detected by two-photon absorption laser induced fluorescence (TALIF). Here, pressure broadening of the (2p 4 3 P 2  →  3p 3 P J=0,1,2) two-photon transition in oxygen atoms was investigated using a high-resolution TALIF technique in normal and Doppler-free configurations. The pressure broadening coefficients determined were {γ{{\\text{O}2}}}   =  0.40  ±  0.08  cm-1/bar for oxygen molecules and {γ\\text{He}}   =  0.46  ±  0.03 cm-1/bar for helium atoms. These correspond to pressure broadening rate constants k\\text{PB}{{\\text{O}2}}   =  9 · 10-9 cm3 s-1 and k\\text{PB}\\text{He}   =  4 · 10-9 cm3 s-1, respectively. The well-known quenching rate constants of O(3p 3 P J ) by O2 and He are at least one order of magnitude smaller, which signifies that non-quenching collisions constitute the main line-broadening mechanism. In addition to providing new insights into collisional processes of oxygen atoms in electronically excited 3p 3 P J state, reported pressure broadening parameters are important for quantification of oxygen TALIF line profiles when both collisional and Doppler broadening mechanisms are important. Thus, the Doppler component (and hence the temperature of oxygen atoms) can be accurately determined from high resolution TALIF measurements in a broad range of conditions.

  12. Electron Transport Through a Quantum Wire with a Side-Coupled Quantum Dot:Fano Resonance

    Institute of Scientific and Technical Information of China (English)

    熊永建; 贺舟波

    2004-01-01

    The Fano resonance of a quantum wire (QW) with a side-coupled quantum dot (QD) is investigated. The QD has multilevel and is in the Coulomb blockade regime. We show that there are two aspects in contribution to asymmetric Fano dip line shape of conductance: (1) the quantum interference between the resonant level and non-resonant levels, (2) the asymmetric electron occupation of levels in the two sides of a resonant level in the QD. The smearing of the asymmetry of the dip structure with the increasing temperature is partially attributed to fluctuation of electron state in the QD.

  13. Temperature-dependent excitonic photoluminescence Excited by Two-Photon Absorption in Perovskite CsPbBr3 Quantum Dots

    CERN Document Server

    Wei, Ke; Xu, Zhongjie; Shen, Chao; Cheng, Xiangai; Jiang, Tian

    2016-01-01

    Recently lead halide nanocrystals (quantum dots) have been reported with potential for photovoltaic and optoelectronic applications due to their excellent luminescent properties. Herein excitonic photoluminescence (PL) excited by two-photon absorption in perovskite CsPbBr3 quantum dots (QDs) have been studied across a broad temperature range from 80K to 380K. Two-photon absorption has been investigated with absorption coefficient up to 0.085 cm/GW at room temperature. Moreover, the photoluminescence excited by two-photon absorption shows a linear blue-shift (0.25meV/K) below temperature of ~220K and turned steady with fluctuation below 1nm (4.4meV) for higher temperature up to 380K. These phenomena are distinctly different from general red-shift of semiconductor and can be explained by the competition between lattice expansion and electron-phonon couplling.Our results reveal the strong nonlinear absorption and temperature-independent chromaticity in a large temperature range from 220K to 380K in the CsPbX3 QD...

  14. Electrically Detected Magnetic Resonance of Neutral Donors Interacting with a Two-Dimensional Electron Gas

    Energy Technology Data Exchange (ETDEWEB)

    Lo, C. C.; Lang, V.; George, R. E.; Morton, J. J. L.; Tyryshkin, A. M.; Lyon, A.; Bokor, J.; Schenkel, T.

    2011-04-20

    We have measured the electrically detected magnetic resonance of donor-doped silicon field-effect transistors in resonant X- (9.7 GHz) and W-band (94 GHz) microwave cavities. The two-dimensional electron gas (2DEG) resonance signal increases by two orders of magnitude from X- to W-band, while the donor resonance signals are enhanced by over one order of magnitude. Bolometric effects and spin-dependent scattering are inconsistent with the observations. We propose that polarization transfer from the donor to the 2DEG is the main mechanism giving rise to the spin resonance signals.

  15. Enhancement of Squeezing in Two-Photon Jaynes-Cummings Model with Atomic Measurement

    Institute of Scientific and Technical Information of China (English)

    YE Sai-Yun

    2006-01-01

    We investigate the squeezing properties of the cavity field in the degenerate two-photon Jaynes-Cummings model. Compared with the one-photon Jaynes-Cummings model, the squeezing is more pronounced in the case of two-photon Jaynes-Cummings model under certain conditions.

  16. Event-by-event simulation of nonclassical effects in two-photon interference experiments

    NARCIS (Netherlands)

    Michielsen, K.; Jin, F.; Delina, M.; Raedt, H. De

    2012-01-01

    A corpuscular simulation model for second-order intensity interference phenomena is discussed. It is shown that both the visibility V = 1/2 predicted for two-photon interference experiments with two independent sources and the visibility V = 1 predicted for two-photon interference experiments with a

  17. Integrated single- and two-photon light sheet microscopy using accelerating beams

    DEFF Research Database (Denmark)

    Piksarv, Peeter; Marti, Dominik; Le, Tuan

    2017-01-01

    We demonstrate the first light sheet microscope using propagation invariant, accelerating Airy beams that operates both in single- and two-photon modes. The use of the Airy beam permits us to develop an ultra compact, high resolution light sheet system without beam scanning. In two-photon mode, a...

  18. Two-photon fluorescence probes for imaging of mitochondria and lysosomes.

    Science.gov (United States)

    Yang, Wanggui; Chan, Pui Shan; Chan, Miu Shan; Li, King Fai; Lo, Pik Kwan; Mak, Nai Ki; Cheah, Kok Wai; Wong, Man Shing

    2013-04-28

    Novel biocompatible cyanines show not only a very large two-photon cross-section of up to 5130 GM at 910 nm in aqueous medium for high-contrast and -brightness two-photon fluorescence live cell imaging but also highly selective subcellular localization properties including localization of mitochondria and lysosomes.

  19. Effect of morphology and solvent on two-photon absorption of nano zinc oxide

    Energy Technology Data Exchange (ETDEWEB)

    Kavitha, M.K. [Department of Chemistry, Indian Institute of Space Science and Technology, Valiamala, Thiruvananthapuram 695547, Kerala (India); Haripadmam, P.C.; Gopinath, Pramod; Krishnan, Bindu [Department of Physics, Indian Institute of Space Science and Technology, Valiamala, Thiruvananthapuram 695547, Kerala (India); John, Honey, E-mail: honey@iist.ac.in [Department of Chemistry, Indian Institute of Space Science and Technology, Valiamala, Thiruvananthapuram 695547, Kerala (India)

    2013-05-15

    Highlights: ► ZnO nanospheres and triangular structures synthesis by novel precipitation technique. ► The effect of precursor concentration on the size and shape of nano ZnO. ► Open aperture Z-scan measurements of the ZnO nanoparticle dispersions. ► Nanospheres exhibit higher two photon absorption coefficient than triangular nanostructures. ► Nanospheres dispersed in water exhibit higher two photon absorption coefficient than its dispersion in 2-propanol. - Abstract: In this paper, we report the effect of morphology and solvent on the two-photon absorption of nano zinc oxide. Zinc oxide nanoparticles in two different morphologies like nanospheres and triangular nanostructures are synthesized by novel precipitation technique and their two-photon absorption coefficient is measured using open aperture Z-scan technique. Experimental results show that the zinc oxide nanospheres exhibit higher two-photon absorption coefficient than the zinc oxide triangular nanostructures. The zinc oxide nanospheres dispersed in water exhibit higher two-photon absorption coefficient than that of its dispersion in 2-propanol. The zinc oxide nanospheres dispersed in water shows a decrease in two-photon absorption coefficient with an increase in on-axis irradiance. The result confirms the dependence of shape and solvent on the two-photon absorption of nano zinc oxide.

  20. Production of e, $\\mu$ and $\\tau$ Pairs in Untagged Two-Photon Collisions at LEP

    CERN Document Server

    Acciarri, M; Aguilar-Benítez, M; Ahlen, S P; Alcaraz, J; Alemanni, G; Allaby, James V; Aloisio, A; Alverson, G; Alviggi, M G; Ambrosi, G; Anderhub, H; Andreev, V P; Angelescu, T; Anselmo, F; Arefev, A; Azemoon, T; Aziz, T; Bagnaia, P; Baksay, L; Ball, R C; Banerjee, S; Banerjee, Sw; Banicz, K; Barczyk, A; Barillère, R; Barone, L; Bartalini, P; Baschirotto, A; Basile, M; Battiston, R; Bay, A; Becattini, F; Becker, U; Behner, F; Berdugo, J; Berges, P; Bertucci, B; Betev, B L; Bhattacharya, S; Biasini, M; Biland, A; Bilei, G M; Blaising, J J; Blyth, S C; Bobbink, Gerjan J; Böck, R K; Böhm, A; Boldizsar, L; Borgia, B; Boucham, A; Bourilkov, D; Bourquin, Maurice; Boutigny, D; Braccini, S; Branson, J G; Brigljevic, V; Brock, I C; Buffini, A; Buijs, A; Burger, J D; Burger, W J; Busenitz, J K; Cai, X D; Campanelli, M; Capell, M; Cara Romeo, G; Carlino, G; Cartacci, A M; Casaus, J; Castellini, G; Cavallari, F; Cavallo, N; Cecchi, C; Cerrada-Canales, M; Cesaroni, F; Chamizo-Llatas, M; Chang, Y H; Chaturvedi, U K; Chekanov, S V; Chemarin, M; Chen, A; Chen, G; Chen, G M; Chen, H F; Chen, H S; Chen, M; Chiefari, G; Chien, C Y; Cifarelli, Luisa; Cindolo, F; Civinini, C; Clare, I; Clare, R; Cohn, H O; Coignet, G; Colijn, A P; Colino, N; Commichau, V; Costantini, S; Cotorobai, F; de la Cruz, B; Csilling, Akos; Dai, T S; D'Alessandro, R; De Asmundis, R; Degré, A; Deiters, K; Denes, P; De Notaristefani, F; DiBitonto, Daryl; Diemoz, M; Van Dierendonck, D N; Di Lodovico, F; Dionisi, C; Dittmar, Michael; Dominguez, A; Doria, A; Dorne, I; Dova, M T; Drago, E; Duchesneau, D; Duinker, P; Durán, I; Dutta, S; Easo, S; Efremenko, Yu V; El-Mamouni, H; Engler, A; Eppling, F J; Erné, F C; Ernenwein, J P; Extermann, Pierre; Fabre, M; Faccini, R; Falciano, S; Favara, A; Fay, J; Fedin, O; Felcini, Marta; Fenyi, B; Ferguson, T; Ferroni, F; Fesefeldt, H S; Fiandrini, E; Field, J H; Filthaut, Frank; Fisher, P H; Fisk, I; Forconi, G; Fredj, L; Freudenreich, Klaus; Furetta, C; Galaktionov, Yu; Ganguli, S N; García-Abia, P; Gau, S S; Gentile, S; Gerald, J; Gheordanescu, N; Giagu, S; Goldfarb, S; Goldstein, J; Gong, Z F; Gougas, Andreas; Gratta, Giorgio; Grünewald, M W; Gupta, V K; Gurtu, A; Gutay, L J; Hartmann, B; Hasan, A; Hatzifotiadou, D; Hebbeker, T; Hervé, A; Van Hoek, W C; Hofer, H; Hong, S J; Hoorani, H; Hou, S R; Hu, G; Innocente, Vincenzo; Janssen, H; Jenkes, K; Jin, B N; Jones, L W; de Jong, P; Josa-Mutuberria, I; Kasser, A; Khan, R A; Kamrad, D; Kamyshkov, Yu A; Kapustinsky, J S; Karyotakis, Yu; Kaur, M; Kienzle-Focacci, M N; Kim, D; Kim, D H; Kim, J K; Kim, S C; Kim, Y G; Kinnison, W W; Kirkby, A; Kirkby, D; Kirkby, Jasper; Kiss, D; Kittel, E W; Klimentov, A; König, A C; Kopp, A; Korolko, I; Koutsenko, V F; Krämer, R W; Krenz, W; Kunin, A; Ladrón de Guevara, P; Landi, G; Lapoint, C; Lassila-Perini, K M; Laurikainen, P; Lebeau, M; Lebedev, A; Lebrun, P; Lecomte, P; Lecoq, P; Le Coultre, P; Leggett, C; Le Goff, J M; Leiste, R; Leonardi, E; Levchenko, P M; Li Chuan; Lin, C H; Lin, W T; Linde, Frank L; Lista, L; Liu, Z A; Lohmann, W; Longo, E; Lu, W; Lü, Y S; Lübelsmeyer, K; Luci, C; Luckey, D; Luminari, L; Lustermann, W; Ma Wen Gan; Maity, M; Majumder, G; Malgeri, L; Malinin, A; Maña, C; Mangeol, D J J; Mangla, S; Marchesini, P A; Marin, A; Martin, J P; Marzano, F; Massaro, G G G; McNally, D; Mele, S; Merola, L; Meschini, M; Metzger, W J; Von der Mey, M; Mi, Y; Mihul, A; Van Mil, A J W; Mirabelli, G; Mnich, J; Molnár, P; Monteleoni, B; Moore, R; Morganti, S; Moulik, T; Mount, R; Müller, S; Muheim, F; Muijs, A J M; Nahn, S; Napolitano, M; Nessi-Tedaldi, F; Newman, H; Niessen, T; Nippe, A; Nisati, A; Nowak, H; Oh, Yu D; Opitz, H; Organtini, G; Ostonen, R; Palomares, C; Pandoulas, D; Paoletti, S; Paolucci, P; Park, H K; Park, I H; Pascale, G; Passaleva, G; Patricelli, S; Paul, T; Pauluzzi, M; Paus, C; Pauss, Felicitas; Peach, D; Pei, Y J; Pensotti, S; Perret-Gallix, D; Petersen, B; Petrak, S; Pevsner, A; Piccolo, D; Pieri, M; Pinto, J C; Piroué, P A; Pistolesi, E; Plyaskin, V; Pohl, M; Pozhidaev, V; Postema, H; Produit, N; Prokofev, D; Prokofiev, D O; Rahal-Callot, G; Raja, N; Rancoita, P G; Rattaggi, M; Raven, G; Razis, P A; Read, K; Ren, D; Rescigno, M; Reucroft, S; Van Rhee, T; Riemann, S; Riles, K; Rind, O; Robohm, A; Rodin, J; Roe, B P; Romero, L; Rosier-Lees, S; Rosselet, P; Van Rossum, W; Roth, S; Rubio, Juan Antonio; Ruschmeier, D; Rykaczewski, H; Salicio, J; Sánchez, E; Sanders, M P; Sarakinos, M E; Sarkar, S; Sassowsky, M; Sauvage, G; Schäfer, C; Shchegelskii, V; Schmidt-Kärst, S; Schmitz, D; Schmitz, P; Schneegans, M; Scholz, N; Schopper, Herwig Franz; Schotanus, D J; Schwenke, J; Schwering, G; Sciacca, C; Sciarrino, D; Servoli, L; Shevchenko, S; Shivarov, N; Shoutko, V; Shukla, J; Shumilov, E; Shvorob, A V; Siedenburg, T; Son, D; Sopczak, André; Soulimov, V; Smith, B; Spillantini, P; Steuer, M; Stickland, D P; Stone, H; Stoyanov, B; Strässner, A; Strauch, K; Sudhakar, K; Sultanov, G G; Sun, L Z; Susinno, G F; Suter, H; Swain, J D; Tang, X W; Tauscher, Ludwig; Taylor, L; Ting, Samuel C C; Ting, S M; Tonutti, M; Tonwar, S C; Tóth, J; Tully, C; Tuchscherer, H; Tung, K L; Uchida, Y; Ulbricht, J; Uwer, U; Valente, E; Van de Walle, R T; Vesztergombi, G; Vetlitskii, I; Viertel, Gert M; Vivargent, M; Völkert, R; Vogel, H; Vogt, H; Vorobev, I; Vorobyov, A A; Vorvolakos, A; Wadhwa, M; Wallraff, W; Wang, J C; Wang, X L; Wang, Z M; Weber, A; Wittgenstein, F; Wu, S X; Wynhoff, S; Xu, J; Xu, Z Z; Yang, B Z; Yang, C G; Yao, X Y; Ye, J B; Yeh, S C; You, J M; Zalite, A; Zalite, Yu; Zemp, P; Zeng, Y; Zhang, Z; Zhang, Z P; Zhou, B; Zhou, Y; Zhu, G Y; Zhu, R Y; Zichichi, Antonino; Ziegler, F

    1997-01-01

    The two-photon collision reaction e+e- --> e+e-l+l- has been studied at root(s) ~ 91 GeV using the L3 detector at LEP for l = e, muon , tau. We have analysed untagged configurations where the two photons are quasi-real. Good agreement is found between our measurements and the order alpha**4 QED expectation.

  1. Temporal dynamics of two-photon-pumped amplified spontaneous emission in slab organic crystals

    NARCIS (Netherlands)

    Fang, Hong-Hua; Chen, Qi-Dai; Ding, Ran; Yang, Jie; Ma, Yu-Guang; Wang, Hai-Yu; Gao, Bing-Rong; Feng, Jing; Sun, Hong-Bo; Fang, Honghua

    2010-01-01

    We have studied the ultrafast dynamics of two-photon-pumped amplified spontaneous emission (ASE) from a single crystal by the time-resolved fluorescence upconversion technique. With the increase of two-photon pump intensities, the emission decay time is dramatically shortened by 30 times (from 3 ns

  2. Two-Photon Interference with the Type Ⅱ Spontaneous Parametric Down-Conversion

    Institute of Scientific and Technical Information of China (English)

    江云坤; 史保森; 李剑; 段开敏; 范晓锋; 郭光灿

    2001-01-01

    The two-photon polarized entangled state is generated from the type Ⅱ spontaneous parametric down-conversion pumped by a femtosecond pulse. The two-photon interference is observed in the Hong-Ou-Mandel interferometer. The high visibility of the interference is restored with narrow band interference filters placed in front of the detectors.

  3. Progressive and resonant wave helices application to electron paramagnetic resonance; Helices a ondes progressives et resonnantes application a la resonance paramagnetique electronique

    Energy Technology Data Exchange (ETDEWEB)

    Volino, F. [Commissariat a l' Energie Atomique, Grenoble (France). Centre d' Etudes Nucleaires

    1969-07-01

    We show that helices can be used as resonant systems. Their properties are theoretically and experimentally studied. We describe resonant helices for electron paramagnetic resonance in X-band and develop a comparison between their sensitivity and the sensitivity of a normal resonant cavity. For cylindrical samples less than 3 mm diameter, the helix is more sensitive and can produce more intense microwave magnetic fields. (author) [French] Il est montre que les helices peuvent etre utilisees comme systeme resonnant. Leurs proprietes sont discutees theoriquement et experimentalement. Des helices resonnantes en bande X pour la resonance paramagnetique electronique sont decrites et leur sensibilite est comparee a celle des cavites resonnantes. Pour des echantillons cylindriques de moins de 3 mm de diametre, l'helice est plus sensible et peut produire des champs magnetiques hyper fins plus intenses. (auteur)

  4. New design strategy for the two-photon active material based on push-pull substituted bisanthene molecule.

    Science.gov (United States)

    Chattopadhyaya, Mausumi; Alam, Md Mehboob; Chakrabarti, Swapan

    2011-03-31

    In the present work, we have critically examined the origin of strong two-photon transition probability of a donor-acceptor substituted bisanthene molecule that imitates a small piece of edge passivated (4, 4) graphene nanoribbon. In our calculations, we have considered -OMe, and -NH(2) as donors and -NO(2) as an acceptor. The one- and two-photon absorption parameters are evaluated using state-of-the-art linear and quadratic response theory, respectively, and all these calculations are carried out within the framework of time dependent density functional theory. To give a proper judgment on our findings, we have used the long-range corrected CAMB3LYP functional for all of the time dependent calculations. The present investigation reveals that the bisanthene molecule with three pairs of donor/acceptor moiety has a lower two-photon transition probability than that of a suitably designed bisanthene with only a single pair of donor/acceptor moiety. This in silico observation is consistent for all of the donor/acceptor moieties chosen in the present work. A comprehensive analysis at the two state model level of theory clearly offers us a verdict that by placing the donor/acceptor moiety in a suitable position of bisanthene, we can create a significant asymmetry in the electron density in the first excited state, which eventually leads to a significant difference in the ground and excited state dipole moment and is attributed to the higher two-photon transition probability of a particular bisanthene with a single pair of donor/acceptor moiety than bisanthene with three pairs of donor/acceptor.

  5. Description of states of two-photon interference in optical gating Michelson interferometer

    Science.gov (United States)

    Pongophas, Ekkarat; Sinsarp, Asawin; Suwanna, Sujin; Chunwachirasiri, Withoon; Singhsomroje, Wisit

    2015-07-01

    The interference of two photons in the optical gating Michelson interferometer is investigated. The phenomenon is studied using two different representations of photons: the space-time domain and a step-by-step two photon state evolution. Both representations lead to an equivalent description of the two-photon states which is the interference of four cases of two-photon traveling states, as implied by the evolution analysis. Additionally, the space-time domain analysis reveals that the classical interference of high-intensity light source is identical to the two-photon interference in the quantum regime except for a multiplicative factor of (n 2), where n is the number of photons.

  6. Imaging theory and resolution improvement of two-photon confocal microscopy

    Institute of Scientific and Technical Information of China (English)

    唐志列; 杨初平; 裴红津; 梁瑞生; 刘颂豪

    2002-01-01

    The nonlinear effect of two-photon excitation on the imaging property of two-photonconfocal microscopy has been analyzed by the two-photon fluorescence intensity transfer functionderived in this paper. The two-photon fluorescence intensity transfer function in a confocal micros-copy is given. Furthermore the three-dimensional point spread function (3D-PSF) and thethree-dimensional optical transfer function (3D-OTF) of two-photon confocal microscopy are de-rived based on the nonlinear effect of two-photon excitation. The imaging property of two-photonconfocal microscopy is discussed in detail based on 3D-OTF. Finally the spatial resolution limit oftwo-photon confocal microscopy is discussed according to the uncertainty principle.

  7. Atomic and molecular complex resonances from real eigenvalues using standard (hermitian) electronic structure calculations

    CERN Document Server

    Landau, Arie; Kaprálová-Žďánská, Petra Ruth; Moiseyev, Nimrod

    2015-01-01

    Complex eigenvalues, resonances, play an important role in large variety of fields in physics and chemistry. For example, in cold molecular collision experiments and electron scattering experiments, autoionizing and pre-dissociative metastable resonances are generated. However, the computation of complex resonance eigenvalues is difficult, since it requires severe modifications of standard electronic structure codes and methods. Here we show how resonance eigenvalues, positions and widths, can be calculated using the standard, widely used, electronic-structure packages. Our method enables the calculations of the complex resonance eigenvalues by using analytical continuation procedures (such as Pad\\'{e}). The key point in our approach is the existence of narrow analytical passages from the real axis to the complex energy plane. In fact, the existence of these analytical passages relies on using finite basis sets. These passages become narrower as the basis set becomes more complete, whereas in the exact limit,...

  8. Two-photon microscopy measurement of CMRO2 using periarteriolar PO2 gradients(Conference Presentation)

    Science.gov (United States)

    Sakadžić, Sava; Yaseen, Mohammad A.; Jaswal, Rajeshwer S.; Roussakis, Emmanuel; Dale, Anders M.; Buxton, Richard B.; Vinogradov, Sergei A.; Boas, David A.; Devor, Anna

    2017-02-01

    The cerebral metabolic rate of oxygen (CMRO2) is an essential parameter for evaluating brain function and pathophysiology. Measurements of CMRO2 with high spatio-temporal resolution are critically important for understanding how the brain copes with metabolic and blood perfusion changes associated with various clinical conditions, such as stroke, periinfarct depolarizations, and various microvasculopathies (e.g., Alzheimer's disease, chronic hypertension). CMRO2 measurements are also important for understanding the physiological underpinnings of functional Magnetic Resonance Imaging signals. However, the currently available approaches for quantifying CMRO2 rely on complex multimodal imaging and mathematical modeling. Here, we introduce a novel method that allows estimation of CMRO2 based on a single measurement modality - two-photon phosphorescence lifetime microscopy (2PLM) imaging of the partial pressure of oxygen (PO2) in cortical tissue. CMRO2 is estimated by fitting the changes of tissue PO2 around cortical penetrating arterioles with the Krogh cylinder model of oxygen diffusion. We measured the baseline CMRO2 in anesthetized rats, and modulated tissue PO2 levels by manipulating the depth of anesthesia. This method has a spatial resolution of approximately 200 μm and it may provide CMRO2 measurements in individual cortical layers or within confined cortical regions such as in ischemic penumbra and the foci of functional activation.

  9. Search for two Higgs bosons in final states containing two photons and two bottom quarks

    Energy Technology Data Exchange (ETDEWEB)

    Khachatryan, Vardan; et al.

    2016-03-22

    A search is presented for the production of two Higgs bosons in final states containing two photons and two bottom quarks. Both resonant and nonresonant hypotheses are investigated. The analyzed data correspond to an integrated luminosity of 19.7 inverse femtobarns of proton-proton collisions at sqrt(s) = 8 TeV collected with the CMS detector. Good agreement is observed between data and predictions of the standard model (SM). Upper limits are set at 95% confidence level on the production cross section of new particles and compared to the prediction for the existence of a warped extra dimension. When the decay to two Higgs bosons is kinematically allowed, assuming a mass scale LambdaR = 1 TeV for the model, the data exclude a radion scalar at masses below 980 GeV. The first Kaluza-Klein excitation mode of the graviton in Randall-Sundrum models is excluded for masses between 325 and 450 GeV. Limits set on nonresonant production constrain the parameter space for anomalous Higgs boson couplings.

  10. Enhancement of Two-photon Absorption in Quantum Wells for Extremely Nondegenerate Photon Pairs

    CERN Document Server

    Pattanaik, Himansu S; Khurgin, Jacob B; Hagan, David J; Van Stryland, Eric W

    2015-01-01

    We recently demonstrated orders of magnitude enhancement of two-photon absorption (2PA) in direct gap semiconductors due to intermediate state resonance enhancement for photons of very different energies. It can be expected that further enhancement of nondegenerate 2PA will be observed in quantum wells (QWs) since the intraband matrix elements do not vanish near the band center as they do in the bulk, and the density of states in QWs is larger near the band edge. Here we present a perturbation-theory based theoretical description of nondegenerate 2PA in semiconductor QWs, where both frequency and polarization of two incident waves can vary independently. Analytical expressions for all possible permutations of frequencies and polarizations have been obtained, and the results are compared with degenerate 2PA in quantum wells along with degenerate and nondegenerate 2PA in bulk semiconductors. We show that using QWs in place of bulk semiconductors with both beams in the TM-polarized mode leads to an additional or...

  11. Electron Spin Resonance and Related Phenomena in Low-Dimensional Structures

    CERN Document Server

    Fanciulli, Marco

    2009-01-01

    Deals with the discussion of the development of spin resonance in low dimensional structures, such as two-dimensional electron systems, quantum wires, and quantum dots. This title discusses opportunities for spin resonance techniques, with emphasis on fundamental physics, nanoelectronics, spintronics, and quantum information processing

  12. Nuclear Tuning and Detuning of the Electron Spin Resonance in a Quantum Dot: Theoretical Consideration

    NARCIS (Netherlands)

    Danon, J.; Nazarov, Y.V.

    2008-01-01

    We study nuclear spin dynamics in a quantum dot close to the conditions of electron spin resonance. We show that at a small frequency mismatch, the nuclear field detunes the resonance. Remarkably, at larger frequency mismatch, its effect is opposite: The nuclear system is bistable, and in one of the

  13. Electron Spin Resonance of Tetrahedral Transition Metal Oxyanions (MO4n-) in Solids.

    Science.gov (United States)

    Greenblatt, M.

    1980-01-01

    Outlines general principles in observing sharp electron spin resonance (ESR) lines in the solid state by incorporating the transition metal ion of interest into an isostructural diamagnetic host material in small concentration. Examples of some recent studies are described. (CS)

  14. Multifractal scaling of electronic transmission resonances in perfect and imperfect Fibonacci δ-function potentials

    Science.gov (United States)

    Thakur, PrabhatK.; Biswas, Parthapratim

    We present here a detailed multifractal scaling study for the electronic transmission resonances with the system size for an infinitely large one-dimensional perfect and imperfect quasiperiodic system represented by a sequence of δ-function potentials. The electronic transmission resonances in the energy minibands manifest more and more fragmented nature of the transmittance with the change of system size. We claim that when a small perturbation is randomly present at a few number of sites or layers, the nature of electronic states will change and this can be understood by studying the electronic transmittance with the change of system size. We report the different critical states manifested in the size variation of the transmittance corresponding to the resonant energies for both perfect and imperfect cases through multifractal scaling study for few of these resonances.

  15. Resonance-like structure for soliton characteristics in an electron beam-plasma system

    Energy Technology Data Exchange (ETDEWEB)

    Gell, Y.; Nakach, R.

    1978-08-01

    The characteristics of ion acoustic solitons in an electron beam-plasma system are considered. The dependence of the amplitude of the soliton on the density of the beam electrons is found to exhibit a pronounced resonance-like structure. A numerical analysis of the analytic expressions for the soliton characteristics (amplitude and width) is performed for different values of the relevant parameters of the system. The existence and origin of the resonance structure is discussed.

  16. Two-photon absorption and two-photon circular dichroism of L-tryptophan in the near to far UV region

    Science.gov (United States)

    Vesga, Yuly; Hernandez, Florencio E.

    2017-09-01

    Herein we report on the first measurements of the two-photon absorption (TPA) spectrum of L-tryptophan in DMSO solution in the near to far UV region and the two-photon circular dichroism (TPCD) signal corresponding to a transition at 200 nm. We demonstrate the application of the Double L-scan technique in the near to far UV region to perform polarization dependent TPA measurements of chiral molecules. TPCD measurements below 400 nm reveal that chiral molecules in solution, such as tryptophan/DMSO, can undergo photochemical reactions in front of prolonged exposure to UV radiation.

  17. Hard Two-Photon Contribution to Elastic Lepton-Proton Scattering: Determined by the OLYMPUS Experiment

    CERN Document Server

    Henderson, B S; Khaneft, D; O'Connor, C; Russell, R; Schmidt, A; Bernauer, J C; Kohl, M; Akopov, N; Alarcon, R; Ates, O; Avetisyan, A; Beck, R; Belostotski, S; Bessuille, J; Brinker, F; Calarco, J R; Carassiti, V; Cisbani, E; Ciullo, G; Contalbrigo, M; De Leo, R; Diefenbach, J; Donnelly, T W; Dow, K; Elbakian, G; Eversheim, P D; Frullani, S; Funke, Ch; Gavrilov, G; Gläser, B; Görrissen, N; Hasell, D K; Hauschildt, J; Hoffmeister, Ph; Holler, Y; Ihloff, E; Izotov, A; Kaiser, R; Karyan, G; Kelsey, J; Kiselev, A; Klassen, P; Krivshich, A; Lehmann, I; Lenisa, P; Lenz, D; Lumsden, S; Ma, Y; Maas, F; Marukyan, H; Miklukho, O; Milner, R G; Movsisyan, A; Murray, M; Naryshkin, Y; Benito, R Perez; Perrino, R; Redwine, R P; neiro, D Rodríguez Pi\\; Rosner, G; Schneekloth, U; Seitz, B; Statera, M; Thiel, A; Vardanyan, H; Veretennikov, D; Vidal, C; Winnebeck, A; Yeganov, V

    2016-01-01

    The OLYMPUS collaboration reports on a precision measurement of the positron-proton to electron-proton elastic cross section ratio $R_{2\\gamma}$, a direct measure of the contribution of hard two-photon exchange to the elastic cross section. In the OLYMPUS measurement, 2.01 GeV electron and positron beams were directed through a hydrogen gas target internal to the DORIS storage ring at DESY. A toroidal magnetic spectrometer instrumented with drift chambers and time-of-flight scintillators detected elastically scattered leptons in coincidence with recoiling protons over a scattering angle range of $\\approx 20^\\circ$ to $80^\\circ$. The relative luminosity between the two beam species was monitored using tracking telescopes of interleaved GEM and MWPC detectors at $12^\\circ$, as well as symmetric M{\\o}ller/Bhabha calorimeters at $1.29^\\circ$. A total integrated luminosity of 4.5 fb$^{-1}$ was collected. In the extraction of $R_{2\\gamma}$, radiative effects were taken into account using a Monte Carlo generator to ...

  18. Pi resonance of chemisorbed alkali atoms on noble metals.

    Science.gov (United States)

    Borisov, A G; Sametoglu, V; Winkelmann, A; Kubo, A; Pontius, N; Zhao, J; Silkin, V M; Gauyacq, J P; Chulkov, E V; Echenique, P M; Petek, H

    2008-12-31

    We have performed a joint experimental and theoretical study of the unoccupied electronic structure of alkali adsorbates on the (111) surfaces of Cu and Ag. Combining angle- and time-resolved two-photon photoemission spectroscopy with wave packet propagation calculations we show that, along with the well known sigma resonance oriented along the surface normal, there exist long-lived alkali-localized resonances oriented parallel to the surface (pi symmetry). These new resonances are stabilized by the projected band gap of the substrate and emerge primarily from the mixing of the p and d Rydberg orbitals of the free alkali atom modified by the interaction with the surface.

  19. Resonant and non-resonant internal kink modes excited by the energetic electrons on HL-2A tokamak

    Science.gov (United States)

    Yu, L. M.; Chen, W.; Jiang, M.; Shi, Z. B.; Ji, X. Q.; Ding, X. T.; Li, Y. G.; Ma, R. R.; Shi, P. W.; Song, S. D.; Yuan, B. S.; Zhou, Y.; Ma, R.; Song, X. M.; Dong, J. Q.; Xu, M.; Liu, Y.; Yan, L. W.; Yang, Q. W.; Xu, Y. H.; Duan, X. R.; HL-2A Team

    2017-03-01

    Strong resonant and non-resonant internal kink modes (abbreviated as RKs and NRKs, respectively), which are also called resonant and non-resonant fishbones, are observed on HL-2A tokamak with high-power ECRH  +  ECCD‑ (or ECRH) and ECRH  +  ECCD+, respectively. (‘Resonant’ derives from the existence of q  =  1 surface (the resonant surface), and ‘non-resonant’ originates from the absence of q  =  1 surface ({{q}\\text{min}}>1 ). ECCD+ and ECCD‑ mean the driving direction of energetic electrons is the same and opposite to plasma current, respectively.) RK has features of periodic strong bursting amplitude and rapid chirping-down frequency, but NRK usually has the saturated amplitude, slow changed or constant frequency and long-lasting time. The NRK excited by energetic electrons is found for the first time. The reversed q-profiles are formed, and q min decreases during plasma current ramp-up. The value of q min is slightly smaller and a bit bigger than unity for RK and NRK conditions, respectively. The internal kink mode (IKM) structures of RKs and NRKs are confirmed by the ECEI system. Although there are different current drive directions of ECCD for excitation of RK and NRK, they all propagate in electron diamagnetic directions in poloidal. The radial mode structures, frequency and growth rate for IKMs are obtained by solving the dispersion relationship. The NRK is stable when q min is larger than a certain value, and with the decreasing q min the frequency drops, but the growth rate almost keeps constant when {{q}\\text{min}}>1 . This result is in agreement with experimental observation. Studying IKMs excited by energetic electrons can provide important experimental experiences for ITER, because the NRKs may be excited by high-power non-inductive drive of ECCD or ECRH in the operation of hybrid scenarios.

  20. Integrated Analysis of Piezoelectric Resonators as Components of Electronic Systems

    Science.gov (United States)

    2015-09-07

    10.1016/S0894-9166(13)60012-9 Huijing He, Jinxi Liu, Jiashi Yang. Thickness-shear and thickness- twist vibrations of an AT-Cut quartz mesa resonator...2013 09/11/2013 09/11/2013 09/11/2013 09/11/2013 09/16/2013 Received Paper Haifeng Zhang, John A. Kosinski, Yuan Xie, and Joseph A. Turner. Drive -Level...Turner,, John A. Kosinski.. Drive level dependence of doubly rotated langasite resonators with different configurations, 2011 International Frequency

  1. Isotopically-selective two-photon ionization of 12C- and 13C-benzene and hexadeuterobenzene in a time-of-flight mass spectrometer

    Science.gov (United States)

    de La Cruz, A.; Ortiz, M.; Cabrera, J. A.; Campos, J.

    1994-04-01

    In this work the 610 band spectra for 12C6H6, 12C6D6, 13C12C5H6 and 13C12C5D6 isotopically-substituted benzenes are reported. Spectra of deuterated species are given for the first time. These molecular spectra can be employed to test the technical performances of REMPI-TOFMS systems. The experimental method was laser-induced two-photon ionization of molecules cooled in a He supersonic beam followed by time-of-flight mass spectrometry. A splitting of the 610 band appears when a 13C atom is present in the benzene-ring, favoring the isotope selectivity. In the present experiment a complete mass discrimination has been accomplished by using appropriate electronic circuits. A proportional counter has been used to obtain the corresponding spectra of the molecules at 300 K. The device is very useful to tune the laser wavelength to resonance in this kind of mass spectrometry experiment.

  2. Dispersion spreading of biphotons in optical fibres and two-photon interference

    CERN Document Server

    Brida, G; Genovèse, M; Gramegna, M; Krivitsky, L A

    2006-01-01

    We present the first observation of two-photon polarization interference structure in the second-order Glauber's correlation function of two-photon light generated via type-II spontaneous parametric down-conversion. In order to obtain this result, two-photon light is transmitted through an optical fibre and the coincidence distribution is analyzed by means of the START-STOP method. Beyond the experimental demonstration of an interesting effect in quantum optics, these results also have considerable relevance for quantum communications.

  3. Coalescence and Anti-Coalescence Interference of Two-Photon Wavepacket in a Beam Splitter

    Institute of Scientific and Technical Information of China (English)

    WANG Kai-Ge; YANG Guo-Jian

    2004-01-01

    @@ We study theoretically the interference of a two-photon wavepacket in a beam splitter. We find that the spectrum symmetry for the two-photon wavepacket dominates the perfect coalescence and anti-coalescence interference.The coalescence interference is unrelated to photon entanglement. Only the anti-coalescence interference has evidence of photon entanglement. We prove that the two-photon wavepacket with an anti-symmetric spectrum is transparent to pass the 50/50 beam splitter, showing perfect anti-coalescence interference.

  4. Dispersion spreading of biphotons in optical fibers and two-photon interference.

    Science.gov (United States)

    Brida, G; Chekhova, M V; Genovese, M; Gramegna, M; Krivitsky, L A

    2006-04-14

    We present the first observation of two-photon polarization interference structure in the second-order Glauber correlation function of two-photon light generated via type-II spontaneous parametric down-conversion. In order to obtain this result, two-photon light is transmitted through an optical fiber and the coincidence distribution is analyzed by means of the start-stop method. Beyond the experimental demonstration of an interesting effect in quantum optics, these results also have considerable relevance for quantum communications.

  5. Search for a Higgs boson decaying into two photons in the CMS detector

    Indian Academy of Sciences (India)

    Roberta Volpe; on behalf of the CMS Collaboration

    2012-11-01

    A search for a Higgs boson decaying into two photons in collisions at the LHC at a centre-of-mass energy of 7 TeV is presented. The analysis is performed on a dataset corresponding to 1.66 fb-1 of data recorded in 2011 by the CMS experiment. Limits are set on the cross-section of a Standard Model Higgs boson decaying into two photons, and on the cross-section of a fermiophobic Higgs boson decaying into two photons.

  6. Two-photon absorption of [2.2]paracyclophane derivatives in solution: A theoretical investigation

    Science.gov (United States)

    Ferrighi, Lara; Frediani, Luca; Fossgaard, Eirik; Ruud, Kenneth

    2007-12-01

    The two-photon absorption of a class of [2.2]paracyclophane derivatives has been studied using quadratic response and density functional theories. For the molecules investigated, several effects influencing the two-photon absorption spectra have been investigated, such as side-chain elongation, hydrogen bonding, the use of ionic species, and solvent effects, the latter described by the polarizable continuum model. The calculations have been carried out using a recent parallel implementation of the polarizable continuum model in the DALTON code. Special attention is given to those aspects that could explain the large solvent effect on the two-photon absorption cross sections observed experimentally for this class of compounds.

  7. Four-State Model for Three-Branch Molecule's Two-Photon Absorption Properties

    Institute of Scientific and Technical Information of China (English)

    SU Yan; WANG Pei-Ji; ZHAO Peng; RONG Zhen-Yu

    2006-01-01

    @@ We present a four-state model for calculating the two-photon absorption of multi-branched molecules by using the time-depended function method. The numerical results indicate that the two-photon absorption cross section has a strong enhancement for three-branch molecules compared to two-branch structures. The maximal two-photon-absorption cross section is 2.358 × 10-47 cm 4 s/photon. At the same time, the charge-transfer process for the charge-transfer states is visualized in order to explain mechanism about the maximal TPA cross section.

  8. Electron paramagnetic resonance study on n-type electron-irradiated 3C-SiC

    Energy Technology Data Exchange (ETDEWEB)

    Carlsson, P; Rabia, K; Son, N T; Janzen, E [Department of Physics, Chemistry and Biology, Linkoeping University, SE-581 83 Linkoeping (Sweden); Ohshima, T; Morishita, N; Itoh, H [Japan Atomic Energy Research Institute, Takasaki 370-1292 (Japan); Isoya, J [University of Tsukuba, Tsukuba 305-8550 (Japan)], E-mail: paca@ifm.liu.se

    2008-03-15

    Electron Paramagnetic Resonance (EPR) was used to study defects in n-type 3C-SiC films irradiated by 3-MeV electrons at room temperature with a dose of 2x10{sup 18} cm{sup -2}. After electron irradiation, two new EPR spectra with an effective spin S = 1, labeled L5 and L6, were observed. The L5 center has C{sub 3v} symmetry with g = 2.004 and a fine-structure parameter D = 436.5x10{sup -4} cm{sup -1}. The L5 spectrum was only detected under light illumination and it could not be detected after annealing at {approx}550{sup 0}C. The principal z-axis of the D tensor is parallel to the <111>-directions, indicating the location of spins along the Si-C bonds. Judging from the symmetry and the fact that the signal was detected under illumination in n-type material, the L5 center may be related to the divacancy in the neutral charge state. The L6 center has a C{sub 2v}-symmetry with an isotropic g-value of g = 2.003 and the fine structure parameters D = 547.7x10{sup -4} cm{sup -1} and E = 56.2x10{sup -4} cm{sup -1}. The L6 center disappeared after annealing at a rather low temperature ({approx}200 deg. C), which is substantially lower than the known annealing temperatures for vacancy-related defects in 3C-SiC. This highly mobile defect may be related to carbon interstitials.

  9. Electron Cloud Density Measurements in Accelerator Beam-pipe Using Resonant Microwave Excitation

    CERN Document Server

    Sikora, John P

    2013-01-01

    An accelerator beam can generate low energy electrons in the beam-pipe, generally called electron cloud, that can produce instabilities in a positively charged beam. One method of measuring the electron cloud density is by coupling microwaves into and out of the beam-pipe and observing the response of the microwaves to the presence of the electron cloud. This paper describes a technique in which the beam-pipe is resonantly excited with microwaves and the electron cloud density calculated from the change that it produces in the resonant frequency of the beam-pipe. The resonant technique has the advantage that measurements can be localized to sections of beam-pipe that are a meter or less in length, as well as greatly improving the signal to noise ratio.

  10. Effect of the third π ∗ resonance on the angular distributions for electron-pyrimidine scattering

    Science.gov (United States)

    Mašín, Zdeněk; Gorfinkiel, Jimena D.

    2016-07-01

    We present a detailed analysis of the effect of the well known third π∗ resonance on the angular behaviour of the elastic cross section in electron scattering from pyrimidine. This resonance, occurring approximately at 4.7 eV, is of mixed shape and core-excited character. Experimental and theoretical results show the presence of a peak/dip behaviour in this energy range, that is absent for other resonances. Our investigations show that the cause of the peak/dip is an interference of background p-wave to p-wave scattering amplitudes with the amplitudes for resonant scattering. The equivalent resonance in pyrazine shows the same behaviour and the effect is therefore likely to appear in other benzene-like molecules. Contribution to the Topical Issue "Advances in Positron and Electron Scattering", edited by Paulo Limao-Vieira, Gustavo Garcia, E. Krishnakumar, James Sullivan, Hajime Tanuma and Zoran Petrovic.

  11. A Theranostic Agent Combining a Two-Photon-Absorbing Photosensitizer for Photodynamic Therapy and a Gadolinium(III) Complex for MRI Detection.

    Science.gov (United States)

    Schmitt, Julie; Heitz, Valérie; Sour, Angélique; Bolze, Frédéric; Kessler, Pascal; Flamigni, Lucia; Ventura, Barbara; Bonnet, Célia S; Tóth, Éva

    2016-02-18

    The convergent synthesis and characterization of a potential theranostic agent, [DPP-ZnP-GdDOTA](-), which combines a diketopyrrolopyrrole-porphyrin component DPP-ZnP as a two-photon photosensitizer for photodynamic therapy (PDT) with a gadolinium(III) DOTA complex as a magnetic resonance imaging probe, is presented. [DPP-ZnP-GdDOTA](-) has a remarkably high longitudinal water proton relaxivity (19.94 mm(-1)  s(-1) at 20 MHz and 25 °C) for a monohydrated molecular system of this size. The Nuclear Magnetic Relaxation Dispersion (NMRD) profile is characteristic of slow rotation, related to the extended and rigid aromatic units integrated in the molecule and to self-aggregation occurring in aqueous solution. The two-photon properties were examined and large two-photon absorption cross-sections around 1000 GM were determined between 910 and 940 nm in DCM with 1 % pyridine and in DMSO. Furthermore, the new conjugate was able to generate singlet oxygen, with quantum yield of 0.42 and 0.68 in DCM with 1 % pyridine and DMSO, respectively. Cellular studies were also performed. The [DPP-ZnP-GdDOTA](-) conjugate demonstrated low dark toxicity and was able to induce high one-photon and moderate two-photon phototoxicity on cancer cells.

  12. Lighting the Way to See Inside Two-Photon Absorption Materials: Structure-Property Relationship and Biological Imaging.

    Science.gov (United States)

    Zhang, Qiong; Tian, Xiaohe; Zhou, Hongping; Wu, Jieying; Tian, Yupeng

    2017-02-23

    The application of two-photon absorption (2PA) materials is a classical research field and has recently attracted increasing interest. It has generated a demand for new dyes with high 2PA cross-sections. In this short review, we briefly cover the structure-2PA property relationships of organic fluorophores, organic-inorganic nanohybrids and metal complexes explored by our group. (1) The two-photon absorption cross-section (δ) of organic fluorophores increases with the extent of charge transfer, which is important to optimize the core, donor-acceptor pair, and conjugation-bridge to obtain a large δ value. Among the various cores, triphenylamine appears to be an efficient core. Lengthening of the conjugation with styryl groups in the D-π-D quadrupoles and D-π-A dipoles increased δ over a long wavelength range than when vinylene groups were used. Large values of δ were observed for extended conjugation length and moderate donor-acceptors in the near-IR wavelengths. The δ value of the three-arm octupole is larger than that of the individual arm, if the core has electron accepting groups that allow significant electronic coupling between the arms; (2) Optical functional organic/inorganic hybrid materials usually show high thermal stability and excellent optical activity; therefore the design of functional organic molecules to build functional organic-inorganic hybrids and optimize the 2PA properties are significant. Advances have been made in the design of organic-inorganic nanohybrid materials of different sizes and shapes for 2PA property, which provide useful examples to illustrate the new features of the 2PA response in comparison to the more thoroughly investigated donor-acceptor based organic compounds and inorganic components; (3) Metal complexes are of particular interest for the design of new materials with large 2PA ability. They offer a wide range of metals with different ligands, which can give rise to tunable electronic and 2PA properties. The metal

  13. Lighting the Way to See Inside Two-Photon Absorption Materials: Structure–Property Relationship and Biological Imaging

    Science.gov (United States)

    Zhang, Qiong; Tian, Xiaohe; Zhou, Hongping; Wu, Jieying; Tian, Yupeng

    2017-01-01

    The application of two-photon absorption (2PA) materials is a classical research field and has recently attracted increasing interest. It has generated a demand for new dyes with high 2PA cross-sections. In this short review, we briefly cover the structure-2PA property relationships of organic fluorophores, organic-inorganic nanohybrids and metal complexes explored by our group. (1) The two-photon absorption cross-section (δ) of organic fluorophores increases with the extent of charge transfer, which is important to optimize the core, donor-acceptor pair, and conjugation-bridge to obtain a large δ value. Among the various cores, triphenylamine appears to be an efficient core. Lengthening of the conjugation with styryl groups in the D-π-D quadrupoles and D-π-A dipoles increased δ over a long wavelength range than when vinylene groups were used. Large values of δ were observed for extended conjugation length and moderate donor-acceptors in the near-IR wavelengths. The δ value of the three-arm octupole is larger than that of the individual arm, if the core has electron accepting groups that allow significant electronic coupling between the arms; (2) Optical functional organic/inorganic hybrid materials usually show high thermal stability and excellent optical activity; therefore the design of functional organic molecules to build functional organic-inorganic hybrids and optimize the 2PA properties are significant. Advances have been made in the design of organic-inorganic nanohybrid materials of different sizes and shapes for 2PA property, which provide useful examples to illustrate the new features of the 2PA response in comparison to the more thoroughly investigated donor-acceptor based organic compounds and inorganic components; (3) Metal complexes are of particular interest for the design of new materials with large 2PA ability. They offer a wide range of metals with different ligands, which can give rise to tunable electronic and 2PA properties. The metal

  14. Lighting the Way to See Inside Two-Photon Absorption Materials: Structure–Property Relationship and Biological Imaging

    Directory of Open Access Journals (Sweden)

    Qiong Zhang

    2017-02-01

    Full Text Available The application of two-photon absorption (2PA materials is a classical research field and has recently attracted increasing interest. It has generated a demand for new dyes with high 2PA cross-sections. In this short review, we briefly cover the structure-2PA property relationships of organic fluorophores, organic-inorganic nanohybrids and metal complexes explored by our group. (1 The two-photon absorption cross-section (δ of organic fluorophores increases with the extent of charge transfer, which is important to optimize the core, donor-acceptor pair, and conjugation-bridge to obtain a large δ value. Among the various cores, triphenylamine appears to be an efficient core. Lengthening of the conjugation with styryl groups in the D-π-D quadrupoles and D-π-A dipoles increased δ over a long wavelength range than when vinylene groups were used. Large values of δ were observed for extended conjugation length and moderate donor-acceptors in the near-IR wavelengths. The δ value of the three-arm octupole is larger than that of the individual arm, if the core has electron accepting groups that allow significant electronic coupling between the arms; (2 Optical functional organic/inorganic hybrid materials usually show high thermal stability and excellent optical activity; therefore the design of functional organic molecules to build functional organic-inorganic hybrids and optimize the 2PA properties are significant. Advances have been made in the design of organic-inorganic nanohybrid materials of different sizes and shapes for 2PA property, which provide useful examples to illustrate the new features of the 2PA response in comparison to the more thoroughly investigated donor-acceptor based organic compounds and inorganic components; (3 Metal complexes are of particular interest for the design of new materials with large 2PA ability. They offer a wide range of metals with different ligands, which can give rise to tunable electronic and 2PA

  15. Simultaneous control of emission localization and two-photon absorption efficiency in dissymmetrical chromophores

    Energy Technology Data Exchange (ETDEWEB)

    Tretiak, Sergei [Los Alamos National Laboratory

    2009-01-01

    The aim of the present work is to demonstrate that combined spectral tuning of fluorescence and two-photon absorption (TPA) properties of multipolar chromophores can be achieved by introduction of slight electronic chemical dissymmetry. In that perspective, two novel series of structurally related chromophores have been designed and studied: a first series based on rod-like quadrupolar chromophores bearing different electron-donating (D) end groups and a second series based on three-branched octupolar chromophores built from a trigonal donating moiety and bearing various acceptor (A) peripheral groups. The influence of the electronic dissymmetry is investigated by combined experimental and theoretical studies of the linear and nonlinear optical properties of dissymmetric chromophores compared to their symmetrical counterparts. In both types of systems (i.e. quadrupoles and octupoles) experiments and theory reveal that excitation is essentially delocalized and that excitation involves synchronized charge redistribution between the different D and A moieties within the multipolar structure (i.e. concerted intramolecular charge transfer). In contrast, the emission stems only from a particular dipolar subunit bearing the strongest D or A moieties due to fast excitation localization after excitation prior to emission. Hence control of emission characteristics (polarization and emission spectrum) in addition to localization can be achieved by controlled introduction of electronic dissymmetry (i.e. replacement of one of the D or A end-groups by a slightly stronger D{prime} or A{prime} units). Interestingly dissymmetrical functionalization of both quadrupolar and octupolar compounds does not lead to significant loss in TPA responses and can even be beneficial due to the spectral broadening and peak position tuning that it allows. This study thus reveals an original molecular engineering route strategy allowing major TPA enhancement in multipolar structures due to concerted

  16. Electron- and neutrino-nucleus scattering from the quasielastic to the resonance region

    CERN Document Server

    Leitner, T; Alvarez-Ruso, L; Mosel, U

    2008-01-01

    We present a model for electron- and neutrino-scattering off nucleons and nuclei focussing on the quasielastic and resonance region. The lepton-nucleon reaction is described within a relativistic formalism that includes, besides quasielastic scattering, the excitation of 13 N* and Delta resonances and a non-resonant single-pion background. Recent electron-scattering data is used for the state-of-the-art parametrizations of the vector form factors; the axial couplings are determined via PCAC and, in the case of the Delta resonance, the axial form factor is refitted using neutrino-scattering data. Scattering off nuclei is treated within the GiBUU framework that takes into account various nuclear effects: the local density approximation for the nuclear ground state, mean-field potentials and in-medium spectral functions. Results for inclusive scattering off Oxygen are presented and, in the case of electron-induced reactions, compared to experimental data and other models.

  17. A bistriphenylamine-substituted spirobifluorene derivative exhibiting excellent nonlinearity/transparency/thermal stability trade-off and strong two-photon induced blue fluorescence

    Energy Technology Data Exchange (ETDEWEB)

    Yin, Hongyao [Department of Chemistry, Shanghai Normal University, Shanghai 200234 (China); Xiao, Haibo, E-mail: xiaohb@shnu.edu.cn [Department of Chemistry, Shanghai Normal University, Shanghai 200234 (China); Ding, Lei [Department of Chemistry, Shanghai Normal University, Shanghai 200234 (China); Zhang, Chun; Ren, Aiming [State Key Laboratory of Theoretical and Computational Chemistry, Institute of Theoretical Chemistry, Jilin University, Changchun 130023 (China); Li, Bo [Key Laboratory of Polar Materials and Devices, Ministry of Education, East China Normal University, Shanghai 200241 (China)

    2015-02-01

    A spirobifluorene-bridged donor/donor chromophore, 2,7-bis-(4-(N,N-diphenylamino)phen-1-yl)-9,9′-spirobifluorene (SPF-TP), was found to combine excellent transparency in the near UV–visible region (λ{sub cut-off} ≤ 420 nm), large two-photon absorption cross-section (4.5 × 10{sup 3}GM) and high thermal stability (T{sub d} = 501 °C). In comparison to the reported two-photon absorption molecules, SPF-TP represents the best thermal stability so far described in the literature. The main electronic factors explaining the high two-photon absorption activities of SPF-TP were analyzed by theoretical calculations. Cyclic voltammograms were employed to explore the causes of the excellent transparency of SPF-TP. It was found that the spiroconjugation effect is responsible for the excellent nonlinearity/transparency/thermal stability trade-off in SPF-TP. In addition, SPF-TP is also a good two-photon induced blue fluorescent material with high fluorescence quantum yield (Φ = 0.90, in THF). - Highlights: • We report a molecule exhibiting excellent transparency. • The two-photon absorption cross-section is as large as 4.5 × 10{sup 3}GM. • The molecule exhibits excellent thermal stability. • The molecule is a good two-photon induced blue fluorescent material. • The spiroconjugation effect explains the excellent properties.

  18. Electron beam asymmetry measurements from exclusive pi0 electroproduction in the Delta(1232) resonance region

    Energy Technology Data Exchange (ETDEWEB)

    K. Joo

    2003-05-01

    The polarized longitudinal-transverse structure function sigma_LT'in the p(e,e'p)pi^0 reaction has been measured for the first time in the Delta(1232) resonance region for invariant mass W = 1.1 - 1.3 GeV and at four-momentum transfer Q^2 = 0.40 and 0.65 GeV^2. Data were taken at the Thomas Jefferson National Accelerator Facility with the CEBAF Large Acceptance Spectrometer (CLAS) using longitudinally polarized electrons at an energy of 1.515 GeV. This newly measured sigma_LT' provides new and unique information on the interference between resonant and non-resonant amplitudes in the Delta(1232) resonance region. The comparison to recent phenomenological calculations shows sensitivity to the description of non-resonant amplitudes and higher resonances.

  19. Electron beam asymmetry measurements from exclusive pi0 electroproduction in the Delta(1232) resonance region

    Energy Technology Data Exchange (ETDEWEB)

    K. Joo

    2003-05-01

    The polarized longitudinal-transverse structure function sigma_LT'in the p(e,e'p)pi^0 reaction has been measured for the first time in the Delta(1232) resonance region for invariant mass W = 1.1 - 1.3 GeV and at four-momentum transfer Q^2 = 0.40 and 0.65 GeV^2. Data were taken at the Thomas Jefferson National Accelerator Facility with the CEBAF Large Acceptance Spectrometer (CLAS) using longitudinally polarized electrons at an energy of 1.515 GeV. This newly measured sigma_LT' provides new and unique information on the interference between resonant and non-resonant amplitudes in the Delta(1232) resonance region. The comparison to recent phenomenological calculations shows sensitivity to the description of non-resonant amplitudes and higher resonances.

  20. A dual-mode microwave resonator for double electron-electron spin resonance spectroscopy at W-band microwave frequencies

    Science.gov (United States)

    Tkach, Igor; Sicoli, Giuseppe; Höbartner, Claudia; Bennati, Marina

    2011-04-01

    We present a dual-mode resonator operating at/near 94 GHz (W-band) microwave frequencies and supporting two microwave modes with the same field polarization at the sample position. Numerical analysis shows that the frequencies of both modes as well as their frequency separation can be tuned in a broad range up to GHz. The resonator was constructed to perform pulsed ELDOR experiments with a variable separation of "pump" and "detection" frequencies up to Δ ν = 350 MHz. To examine its performance, test ESE/PELDOR experiments were performed on a representative biradical system.