Stable corrugated state of the two-dimensional electron gas
International Nuclear Information System (INIS)
Mendez-Moreno, R.M.; Moreno, M.; Ortiz, M.A.
1991-01-01
A corrugated and stable ground state is found for the two-dimensional electron gas in both the normal paramagnetic and the fully polarized phases. The self-consistent Hartree-Fock method is used with a modulated set of trial wave functions within the deformable jellium model. The results for high metallic densities reproduce the usual noncorrugated ferromagnetic electron-gas behavior. A transition to a paramagnetic corrugated state for values of r s ∼6.5 is predicted. At lower densities r s ∼30, a second transition to a corrugated ferromagnetic phase is suggested
Multifractal character of the electronic states in disordered two-dimensional systems
International Nuclear Information System (INIS)
Tit, N.; Schreiber, M.
1994-08-01
The nature of electronic states in disordered two-dimensional (2D) systems is investigated. To this aim, we present our calculations of both density of states and dc-conductivity for square lattices modelling the Anderson Hamiltonian with on-site energies randomly chosen from a box distribution of width W. For weak disorder (W), the eigenfunctions calculated by means of the Lanczos diagonalization algorithm display spatial fluctuations reflecting their (multi)fractal behaviour. For increasing disorder or energy the observed increase of the curdling of the wavefunction reflects its stronger localization. Our dc-conductivity results suggest a critical fractal dimension d * c =1.48±0.05 to discriminate between the exponentially and the power-law localized states. Consequences of the localization on transport properties are also discussed. (author). 30 refs, 10 figs, 1 tab
Surface electron states on the quasi-two-dimensional excess-electron compounds Ca2N and Y2C
Inoshita, Takeshi; Takemoto, Seiji; Tada, Tomofumi; Hosono, Hideo
2017-04-01
Compounds having excess electrons from the formal valence viewpoint (electrides) are a new class of materials, which often take low-dimensional structures. We studied the (001) surface electronic structures of quasi-two-dimensional electrides Ca2N and Y2C by density functional theory using a slab model. Both materials were found to have a clean surface state well separated in energy from the bulk states. Furthermore, this state virtually floats above the surface and may be considered to be a hallmark of two-dimensional electrides. For Ca2N , a tight-binding model in the Wannier representation was derived and analyzed, from which we concluded that the surface state, described by extra-surface s -like orbitals, is a Tamm state originating from an abrupt increase in potential energy at the surface.
Spin eigen-states of Dirac equation for quasi-two-dimensional electrons
Energy Technology Data Exchange (ETDEWEB)
Eremko, Alexander, E-mail: eremko@bitp.kiev.ua [Bogolyubov Institute for Theoretical Physics, Metrologichna Sttr., 14-b, Kyiv, 03680 (Ukraine); Brizhik, Larissa, E-mail: brizhik@bitp.kiev.ua [Bogolyubov Institute for Theoretical Physics, Metrologichna Sttr., 14-b, Kyiv, 03680 (Ukraine); Loktev, Vadim, E-mail: vloktev@bitp.kiev.ua [Bogolyubov Institute for Theoretical Physics, Metrologichna Sttr., 14-b, Kyiv, 03680 (Ukraine); National Technical University of Ukraine “KPI”, Peremohy av., 37, Kyiv, 03056 (Ukraine)
2015-10-15
Dirac equation for electrons in a potential created by quantum well is solved and the three sets of the eigen-functions are obtained. In each set the wavefunction is at the same time the eigen-function of one of the three spin operators, which do not commute with each other, but do commute with the Dirac Hamiltonian. This means that the eigen-functions of Dirac equation describe three independent spin eigen-states. The energy spectrum of electrons confined by the rectangular quantum well is calculated for each of these spin states at the values of energies relevant for solid state physics. It is shown that the standard Rashba spin splitting takes place in one of such states only. In another one, 2D electron subbands remain spin degenerate, and for the third one the spin splitting is anisotropic for different directions of 2D wave vector.
Energy Technology Data Exchange (ETDEWEB)
Forster, F.
2007-07-06
In this thesis investigations on two-dimensional electronic structures of (111)-noble metal surfaces and the influence of various adsorbates upon them is presented. It chiefly focuses on the surface-localized Shockley states of Cu, Ag and Au and their band dispersion (binding energy, band mass, and spin-orbit splitting) which turns out to be a sensitive probe for surface modifications induced by adsorption processes. Angular resolved photoelectron spectroscopy enables the observation of even subtle changes in the electronic band structure of these two dimensional systems. Different mechanisms taking place at surfaces and the substrate/adsorbate interfaces influence the Shockley state in a different manner and will be analyzed using suitable adsorbate model systems. The experimental results are matched with appropriate theoretical models like the phase accumulation model and the nearly-free electron model and - if possible - with ab initio calculations based on density functional theory. This allows for the integration of the results into a stringent overall picture. The influence of sub-monolayer adsorption of Na upon the surface state regarding the significant change in surface work function is determined. A systematic study of the physisorption of noble gases shows the effect of the repulsive adsorbate-substrate interaction upon the electrons of the surface state. A step-by-step coverage of the Cu and Au(111) surfaces by monolayers of Ag creates a gradual change in the surface potential and causes the surface state to become increasingly Ag-like. For N=7 ML thick and layer-by-layer growing Ag films on Au(111), new two-dimensional electronic structures can be observed, which are attributed to the quantum well states of the Ag adsorbate. The question whether they are localized within the Ag-layer or substantially within the substrate is resolved by the investigation of their energetic and spatial evolution with increasing Ag-film thicknesses N. For this, beside the
Control of two-dimensional electronic states at anatase Ti O2(001 ) surface by K adsorption
Yukawa, R.; Minohara, M.; Shiga, D.; Kitamura, M.; Mitsuhashi, T.; Kobayashi, M.; Horiba, K.; Kumigashira, H.
2018-04-01
The nature of the intriguing metallic electronic structures appearing at the surface of anatase titanium dioxide (a-Ti O2 ) remains to be elucidated, mainly owing to the difficulty of controlling the depth distribution of the oxygen vacancies generated by photoirradiation. In this study, K atoms were adsorbed onto the (001) surface of a-Ti O2 to dope electrons into the a-Ti O2 and to confine the electrons in the surface region. The success of the electron doping and its controllability were confirmed by performing in situ angle-resolved photoemission spectroscopy as well as core-level measurements. Clear subband structures were observed in the surface metallic states, indicating the creation of quasi-two-dimensional electron liquid (q2DEL) states in a controllable fashion. With increasing electron doping (K adsorption), the q2DEL states exhibited crossover from polaronic liquid states with multiple phonon-loss structures originating from the long-range Fröhlich interaction to "weakly correlated metallic" states. In the q2DEL states in the weakly correlated metallic region, a kink due to short-range electron-phonon coupling was clearly observed at about 80 ±10 meV . The characteristic energy is smaller than that previously observed for the metallic states of a-Ti O2 with three-dimensional nature (˜110 meV ) . These results suggest that the dominant electron-phonon coupling is modulated by anisotropic carrier screening in the q2DEL states.
Energy Technology Data Exchange (ETDEWEB)
Bykov, A. A.; Rodyakina, E. E.; Latyshev, A. V. [Rzhanov Institute of Semiconductor Physics, Novosibirsk 630090 (Russian Federation); Novosibirsk State University, Novosibirsk 630090 (Russian Federation); Strygin, I. S.; Goran, A. V.; Kalagin, A. K. [Rzhanov Institute of Semiconductor Physics, Novosibirsk 630090 (Russian Federation)
2016-01-04
In this study we fabricated lateral superlattices (LSLs) based on the selectively doped GaAs/AlAs heterostructures with a high-mobility two-dimensional (2D) electron gas. The LSLs were formed using the electron-beam lithography and lift-off techniques, which produced a set of metallic strips on top of a heterojunction. The amplitude of the 2D electron gas modulation in the LSL was controlled by the gate voltage applied to the metallic strips. The LSLs with two different periods (a = 200 nm and 500 nm) were used to investigate the influence of microwave radiation with the frequency of 110–150 GHz on the 2D electron transport at the temperature T = 1.6 K in the magnetic field B < 1 T. We have found that zero-resistance states (ZRSs) appear under the microwave radiation in the 2D systems with a unidirectional periodic modulation. These ZRSs are located at the minima of commensurability oscillations.
International Nuclear Information System (INIS)
Chai Zheng; Hu Mao-Jin; Wang Rui-Qiang; Hu Liang-Bin
2014-01-01
We study the theoretical effect of k-cubic (i.e. cubic-in-momentum) Dresselhaus spin—orbit coupling on the decay time of persistent spin helix states in semiconductor two-dimensional electron gases. We show that the decay time of persistent spin helix states may be suppressed substantially by k-cubic Dresselhaus spin—orbit coupling, and after taking the effect of k-cubic Dresselhaus spin—orbit interaction into account, the theoretical results obtained accord both qualitatively and quantitatively with other recent experimental results. (condensed matter: electronic structure, electrical, magnetic, and optical properties)
Two-dimensional vibrational-electronic spectroscopy
Courtney, Trevor L.; Fox, Zachary W.; Slenkamp, Karla M.; Khalil, Munira
2015-10-01
Two-dimensional vibrational-electronic (2D VE) spectroscopy is a femtosecond Fourier transform (FT) third-order nonlinear technique that creates a link between existing 2D FT spectroscopies in the vibrational and electronic regions of the spectrum. 2D VE spectroscopy enables a direct measurement of infrared (IR) and electronic dipole moment cross terms by utilizing mid-IR pump and optical probe fields that are resonant with vibrational and electronic transitions, respectively, in a sample of interest. We detail this newly developed 2D VE spectroscopy experiment and outline the information contained in a 2D VE spectrum. We then use this technique and its single-pump counterpart (1D VE) to probe the vibrational-electronic couplings between high frequency cyanide stretching vibrations (νCN) and either a ligand-to-metal charge transfer transition ([FeIII(CN)6]3- dissolved in formamide) or a metal-to-metal charge transfer (MMCT) transition ([(CN)5FeIICNRuIII(NH3)5]- dissolved in formamide). The 2D VE spectra of both molecules reveal peaks resulting from coupled high- and low-frequency vibrational modes to the charge transfer transition. The time-evolving amplitudes and positions of the peaks in the 2D VE spectra report on coherent and incoherent vibrational energy transfer dynamics among the coupled vibrational modes and the charge transfer transition. The selectivity of 2D VE spectroscopy to vibronic processes is evidenced from the selective coupling of specific νCN modes to the MMCT transition in the mixed valence complex. The lineshapes in 2D VE spectra report on the correlation of the frequency fluctuations between the coupled vibrational and electronic frequencies in the mixed valence complex which has a time scale of 1 ps. The details and results of this study confirm the versatility of 2D VE spectroscopy and its applicability to probe how vibrations modulate charge and energy transfer in a wide range of complex molecular, material, and biological systems.
Quantum wells physics and electronics of two-dimensional systems
Shik, A
1998-01-01
This invaluable book is devoted to the physics, technology and device applications of semiconductor structures with ultrathin layers where the electronic properties are governed by the quantum-mechanical laws. Such structures called quantum wells or structures with the two-dimensional electron gas, have become one of the most actively investigated objects in modern solid state physics. Electronic properties of quantum wells differ dramatically from those of bulk semiconductors, which allows one to observe new types of physical phenomena, such as the quantum Hall effect and many other so-far-un
Ultrafast Charge Transfer Visualized by Two-Dimensional Electronic Spectroscopy
Directory of Open Access Journals (Sweden)
Mančal T.
2013-03-01
Full Text Available Two-dimensional electronic spectroscopy (2D-ES is used to investigate ultrafast excited-state dynamics in a lutetium bisphthalocyanine dimer. Following optical excitation, a chain of electron and hole transfer steps gives rise to characteristic cross-peak dynamics in the electronic 2D spectra. The combination of density matrix propagation and quantum chemical calculations results in a molecular view of the charge transfer dynamics and highlights the role of the counter-ion in providing an energetic perturbation which promotes charge transfer across the complex.
Two-Dimensional Electron System in Electromagnetic Radiation Field
Lungu, Radu Paul; Manolescu, Andrei
We consider a two-dimensional electron gas in the presence of a monochromatic linear polarized electromagnetic field, within the Floquet formalism. The Floquet states have a simple relation with the energy eigenstates in the absence of the field. Therefore the single-particle and the two-particle Green functions of the many-body system with Coulomb interactions, in the radiation field, can be formally calculated by the standard diagrammatic techniques, as for the conservative system. We derive the elementary excitations of quasi-particle type, the plasma dispersion relation, and the ground state quasi-energy, and we relate them to the corresponding results for the conservative system.
Two-dimensional electron magnetohydrodynamic turbulence
Energy Technology Data Exchange (ETDEWEB)
Biskamp, D.; Schwarz, E.; Drake, J.F.
1995-11-01
A novel type of turbulence, which arises in 2D electron magnetohydrodynamics, is studied by numerical simulation. Energy dissipation rates are found to be independent of the dissipation coefficients. The energy spectrum E{sub k} follows the basic Kolmogorov-type predictions, k{sup -5/3} for kd{sub e} > 1 and k{sup -7/3} for kd{sub e} < 1 (d{sub e} = electron inertial length) and is hence independent of the linear wave properties. Results are compared with other 2D turbulent systems. (author).
Paul, Jagannath
Advent of ultrashort lasers made it possible to probe various scattering phenomena in materials that occur in a time scale on the order of few femtoseconds to several tens of picoseconds. Nonlinear optical spectroscopy techniques, such as pump-probe, transient four wave mixing (TFWM), etc., are very common to study the carrier dynamics in various material systems. In time domain, the transient FWM uses several ultrashort pulses separated by time delays to obtain the information of dephasing and population relaxation times, which are very important parameters that govern the carrier dynamics of materials. A recently developed multidimensional nonlinear optical spectroscopy is an enhanced version of TFWM which keeps track of two time delays simultaneously and correlate them in the frequency domain with the aid of Fourier transform in a two dimensional map. Using this technique, the nonlinear complex signal field is characterized both in amplitude and phase. Furthermore, this technique allows us to identify the coupling between resonances which are rather difficult to interpret from time domain measurements. This work focuses on the study of the coherent response of a two dimensional electron gas formed in a modulation doped GaAs/AlGaAs quantum well both at zero and at high magnetic fields. In modulation doped quantum wells, the excitons are formed as a result of the inter- actions of the charged holes with the electrons at the Fermi edge in the conduction band, leading to the formation of Mahan excitons, which is also referred to as Fermi edge singularity (FES). Polarization and temperature dependent rephasing 2DFT spectra in combination with TI-FWM measurements, provides insight into the dephasing mechanism of the heavy hole (HH) Mahan exciton. In addition to that strong quantum coherence between the HH and LH Mahan excitons is observed, which is rather surprising at this high doping concentration. The binding energy of Mahan excitons is expected to be greatly
Magnetoelectronic transport of the two-dimensional electron gas in ...
Indian Academy of Sciences (India)
Home; Journals; Pramana – Journal of Physics; Volume 72; Issue 2 ... CdSe quantum wells; 2D electron gas; magneto-electronic transport. Abstract. Hall mobility and magnetoresistance coefficient for the two-dimensional (2D) electron transport parallel to the heterojunction interfaces in a single quantum well of CdSe are ...
Two-dimensional optimization of free-electron-laser designs
Prosnitz, D.; Haas, R.A.
1982-05-04
Off-axis, two-dimensional designs for free electron lasers are described that maintain correspondence of a light beam with a synchronous electron at an optimal transverse radius r > 0 to achieve increased beam trapping efficiency and enhanced laser beam wavefront control so as to decrease optical beam diffraction and other deleterious effects.
Inter-layer Cooper pairing of two-dimensional electrons
International Nuclear Information System (INIS)
Inoue, Masahiro; Takemori, Tadashi; Yoshizaki, Ryozo; Sakudo, Tunetaro; Ohtaka, Kazuo
1987-01-01
The authors point out the possibility that the high transition temperatures of the recently discovered oxide superconductors are dominantly caused by the inter-layer Cooper pairing of two-dimensional electrons that are coupled through the exchange of three-dimensional phonons. (author)
Magnetoelectronic transport of the two-dimensional electron gas in ...
Indian Academy of Sciences (India)
Abstract. Hall mobility and magnetoresistance coefficient for the two-dimensional (2D) electron transport parallel to the heterojunction interfaces in a single quantum well of. CdSe are calculated with a numerical iterative technique in the framework of Fermi–Dirac statistics. Lattice scatterings due to polar-mode longitudinal ...
Noninteracting beams of ballistic two-dimensional electrons
International Nuclear Information System (INIS)
Spector, J.; Stormer, H.L.; Baldwin, K.W.; Pfeiffer, L.N.; West, K.W.
1991-01-01
We demonstrate that two beams of two-dimensional ballistic electrons in a GaAs-AlGaAs heterostructure can penetrate each other with negligible mutual interaction analogous to the penetration of two optical beams. This allows electrical signal channels to intersect in the same plane with negligible crosstalk between the channels
Engineering the Kondo state in two-dimensional semiconducting phosphorene
Babar, Rohit; Kabir, Mukul
2018-01-01
Correlated interaction between dilute localized impurity electrons and the itinerant host conduction electrons in metals gives rise to the conventional many-body Kondo effect below sufficiently low temperature. In sharp contrast to these conventional Kondo systems, we report an intrinsic, robust, and high-temperature Kondo state in two-dimensional semiconducting phosphorene. While absorbed at a thermodynamically stable lattice defect, Cr impurity triggers an electronic phase transition in phosphorene to provide conduction electrons, which strongly interact with the localized moment generated at the Cr site. These manifest into the intrinsic Kondo state, where the impurity moment is quenched in multiple stages and at temperatures in the 40-200 K range. Further, along with a much smaller extension of the Kondo cloud, the predicted Kondo state is shown to be robust under uniaxial strain and layer thickness, which greatly simplifies its future experimental realization. We predict the present study will open up new avenues in Kondo physics and trigger further theoretical and experimental studies.
Two-dimensional theory and simulation of free electron lasers
International Nuclear Information System (INIS)
Kwan, T.J.T.; Cary, J.R.
1981-01-01
Two-dimensional homogeneous theory of free-electron lasers with a wiggler magnetic field of constant wavelength is formulated. It has been found from the theory that waves propagating obliquely with respect to the electron beam are always unstable with appreciable growth rates; therefore, mode competition among the on-axis and off-axis modes is an important consideration in the design of the free-electron laser. Furthermore, electromagnetic waves with group velocities opposite to the direction of electron beam propagation are absolutely unstable if k/sub o/v/sub o/ > ω/sub pe/(1/γ/sup 3/2/ + 1/γ/sup 1/2/). Due to strong nonlinear saturation levels of the low-frequency absolute instability, the dynamics of the electron beam and the generation of the high-frequency electromagnetic radiation can be severely affected. Two-dimensional particle simulations show that the efficiency of generation of the on-axis high-frequency electromagnetic wave decreases significantly due to instability of the off-axis modes. In addition, complete disruption of the electron beam and laser oscillation due to the onset of the absolute instability have been observed in simulations
Stopping power of two-dimensional spin quantum electron gases
Zhang, Ya; Jiang, Wei; Yi, Lin
2015-04-01
Quantum effects can contribute significantly to the electronic stopping powers in the interactions between the fast moving beams and the degenerate electron gases. From the Pauli equation, the spin quantum hydrodynamic (SQHD) model is derived and used to calculate the stopping power and the induced electron density for protons moving above a two-dimensional (2D) electron gas with considering spin effect under an external in-plane magnetic field. In our calculation, the stopping power is not only modulated by the spin direction, but also varied with the strength of the spin effect. It is demonstrated that the spin effect can obviously enhance or reduce the stopping power of a 2D electron gas within a laboratory magnetic field condition (several tens of Tesla), thus a negative stopping power appears at some specific proton velocity, which implies the protons drain energy from the Pauli gas, showing another significant example of the low-dimensional physics.
Gaynor, James D.; Khalil, Munira
2017-09-01
Two-Dimensional Electronic-Vibrational (2D EV) spectroscopy and Two-Dimensional Vibrational-Electronic (2D VE) spectroscopy are new coherent four-wave mixing spectroscopies that utilize both electronically resonant and vibrationally resonant field-matter interactions to elucidate couplings between electronic and vibrational degrees of freedom. A system Hamiltonian is developed here to lay a foundation for interpreting the 2D EV and 2D VE signals that arise from a vibronically coupled molecular system in the condensed phase. A molecular system consisting of one anharmonic vibration and two electronic states is modeled. Equilibrium displacement of the vibrational coordinate and vibrational frequency shifts upon excitation to the first electronic excited state are included in our Hamiltonian through linear and quadratic vibronic coupling terms. We explicitly consider the nuclear dependence of the electronic transition dipole moment and demonstrate that these spectroscopies are sensitive to non-Condon effects. A series of simulations of 2D EV and 2D VE spectra obtained by varying parameters of the system, system-bath, and interaction Hamiltonians demonstrate that one of the following conditions must be met to observe signals: (1) non-zero linear and/or quadratic vibronic coupling in the electronic excited state, (2) vibrational-coordinate dependence of the electronic transition dipole moment, or (3) electronic-state-dependent vibrational dephasing dynamics. We explore how these vibronic interactions are manifested in the positions, amplitudes, and line shapes of the peaks in 2D EV and 2D VE spectroscopies.
Strongly anisotropic spin-orbit splitting in a two-dimensional electron gas
DEFF Research Database (Denmark)
Michiardi, Matteo; Bianchi, Marco; Dendzik, Maciej
2015-01-01
Near-surface two-dimensional electron gases on the topological insulator Bi$_2$Te$_2$Se are induced by electron doping and studied by angle-resolved photoemission spectroscopy. A pronounced spin-orbit splitting is observed for these states. The $k$-dependent splitting is strongly anisotropic...
Wan, Zhong; Kazakov, Aleksandr; Manfra, Michael J; Pfeiffer, Loren N; West, Ken W; Rokhinson, Leonid P
2015-06-11
Search for Majorana fermions renewed interest in semiconductor-superconductor interfaces, while a quest for higher-order non-Abelian excitations demands formation of superconducting contacts to materials with fractionalized excitations, such as a two-dimensional electron gas in a fractional quantum Hall regime. Here we report induced superconductivity in high-mobility two-dimensional electron gas in gallium arsenide heterostructures and development of highly transparent semiconductor-superconductor ohmic contacts. Supercurrent with characteristic temperature dependence of a ballistic junction has been observed across 0.6 μm, a regime previously achieved only in point contacts but essential to the formation of well separated non-Abelian states. High critical fields (>16 T) in NbN contacts enables investigation of an interplay between superconductivity and strongly correlated states in a two-dimensional electron gas at high magnetic fields.
Two-dimensional electronic spectroscopy with birefringent wedges
Energy Technology Data Exchange (ETDEWEB)
Réhault, Julien; Maiuri, Margherita; Oriana, Aurelio; Cerullo, Giulio [IFN-CNR, Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, 20133 Milano (Italy)
2014-12-15
We present a simple experimental setup for performing two-dimensional (2D) electronic spectroscopy in the partially collinear pump-probe geometry. The setup uses a sequence of birefringent wedges to create and delay a pair of phase-locked, collinear pump pulses, with extremely high phase stability and reproducibility. Continuous delay scanning is possible without any active stabilization or position tracking, and allows to record rapidly and easily 2D spectra. The setup works over a broad spectral range from the ultraviolet to the near-IR, it is compatible with few-optical-cycle pulses and can be easily reconfigured to two-colour operation. A simple method for scattering suppression is also introduced. As a proof of principle, we present degenerate and two-color 2D spectra of the light-harvesting complex 1 of purple bacteria.
Superconductivity in engineered two-dimensional electron gases
Chubukov, Andrey V.; Kivelson, Steven A.
2017-11-01
We consider Kohn-Luttinger mechanism for superconductivity in a two-dimensional electron gas confined to a narrow well between two grounded metallic planes with two occupied subbands with Fermi momenta kF L>kF S . On the basis of a perturbative analysis, we conclude that non-s -wave superconductivity emerges even when the bands are parabolic. We analyze the conditions that maximize Tc as a function of the distance to the metallic planes, the ratio kF L/kF S , and rs, which measures the strength of Coulomb correlations. The largest attraction is in p -wave and d -wave channels, of which p wave is typically the strongest. For rs=O (1 ) we estimate that the dimensionless coupling λ ≈10-1 , but it likely continues increasing for larger rs (where we lose theoretical control).
Two-dimensional electronic spectroscopy with birefringent wedges
Réhault, Julien; Maiuri, Margherita; Oriana, Aurelio; Cerullo, Giulio
2014-12-01
We present a simple experimental setup for performing two-dimensional (2D) electronic spectroscopy in the partially collinear pump-probe geometry. The setup uses a sequence of birefringent wedges to create and delay a pair of phase-locked, collinear pump pulses, with extremely high phase stability and reproducibility. Continuous delay scanning is possible without any active stabilization or position tracking, and allows to record rapidly and easily 2D spectra. The setup works over a broad spectral range from the ultraviolet to the near-IR, it is compatible with few-optical-cycle pulses and can be easily reconfigured to two-colour operation. A simple method for scattering suppression is also introduced. As a proof of principle, we present degenerate and two-color 2D spectra of the light-harvesting complex 1 of purple bacteria.
Numerical Studies of Collective Phenomena in Two-Dimensional Electron and Cold Atom Systems
Energy Technology Data Exchange (ETDEWEB)
Rezayi, Edward
2013-07-25
Numerical calculations were carried out to investigate a number of outstanding questions in both two-dimensional electron and cold atom systems. These projects aimed to increase our understanding of the properties of and prospects for non-Abelian states in quantum Hall matter.
Absolute negative conductivity in two-dimensional electron systems under microwave radiation
Ryzhii, Victor
2004-01-01
We overview mechanisms of absolute negative conductivity in two-dimensional electron systems in a magnetic field irradiated with microwaves and provide plausible explanations of the features observed in recent experiments related to the so-called zero-resistance (zero-conductance) states.
Two-dimensional materials based transparent flexible electronics
Yu, Lili; Ha, Sungjae; El-Damak, Dina; McVay, Elaine; Ling, Xi; Chandrakasan, Anantha; Kong, Jing; Palacios, Tomas
2015-03-01
Two-dimensional (2D) materials have generated great interest recently as a set of tools for electronics, as these materials can push electronics beyond traditional boundaries. These materials and their heterostructures offer excellent mechanical flexibility, optical transparency, and favorable transport properties for realizing electronic, sensing, and optical systems on arbitrary surfaces. These thin, lightweight, bendable, highly rugged and low-power devices may bring dramatic changes in information processing, communications and human-electronic interaction. In this report, for the first time, we demonstrate two complex transparent flexible systems based on molybdenum disulfide (MoS2) grown by chemical vapor method: a transparent active-matrix organic light-emitting diode (AMOLED) display and a MoS2 wireless link for sensor nodes. The 1/2 x 1/2 square inch, 4 x 5 pixels AMOLED structures are built on transparent substrates, containing MoS2 back plane circuit and OLEDs integrated on top of it. The back plane circuit turns on and off the individual pixel with two MoS2 transistors and a capacitor. The device is designed and fabricated based on SPICE simulation to achieve desired DC and transient performance. We have also demonstrated a MoS2 wireless self-powered sensor node. The system consists of as energy harvester, rectifier, sensor node and logic units. AC signals from the environment, such as near-field wireless power transfer, piezoelectric film and RF signal, are harvested, then rectified into DC signal by a MoS2 diode. CIQM, CICS, SRC.
Simulations of two-dimensional electronic correlation spectra
International Nuclear Information System (INIS)
Kim, Hack Jin; Jeon, Seung Joon
2001-01-01
Two-dimensional (2D) correlation method, which generates the synchronous and the asynchronous 2D spectrum by complex cross correlation of the Fourier transformed spectra, is an analysis method for the changes of the sample spectrum induced by various perturbations. In the present work, the 2D electronic correlation spectra have been simulated for the cases where the sample spectrum composed of two gaussian bands changes linearly. When only the band amplitudes of the sample spectrum change, the synchronous spectrum shows strong peaks at the band centers of the sample spectrum, but the asynchronous spectrum does not make peaks. When the sample spectrum shifts without changing intensity and width, the synchronous spectrum shows peaks around the initial and final positions of the band maximum and the asynchronous spectrum shows long peaks spanning the shifting range. The band width change produces the complex 2D correlation spectra. When the sample spectrum shifts with band broadening, the width change by 50 % of full width at half maximum (FWHM) does not give so large an effect on the correlation spectrum as the spectral shift by one half of FWHM of the sample spectrum
Anomalous magnetism for Dirac electrons in two dimensional Rashba systems
Vivas C., H.
2018-03-01
Spin-spin correlation function response in the low electronic density regime and externally applied electric field is evaluated for 2D metallic crystals under Rashba-type coupling, fixed number of particles and twofold energy band structure. Intrinsic Zeeman-like effect on electron spin polarization, density of states, Fermi surface topology and transverse magnetic susceptibility are analyzed in the zero temperature limit. A possible magnetic state for Dirac electrons depending on the zero field band gap magnitude under this conditions is found.
Tunable states of interlayer cations in two-dimensional materials
Energy Technology Data Exchange (ETDEWEB)
Sato, K.; Numata, K. [Department of Environmental Sciences, Tokyo Gakugei University, Koganei, Tokyo 184-8501 (Japan); Dai, W. [Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education), College of Chemistry, Nankai University, Tianjin 300071 (China); Hunger, M. [Institute of Chemical Technology, University of Stuttgart, 70550 Stuttgart (Germany)
2014-03-31
The local state of cations inside the Ångstrom-scale interlayer spaces is one of the controlling factors for designing sophisticated two-dimensional (2D) materials consisting of 2D nanosheets. In the present work, the molecular mechanism on how the interlayer cation states are induced by the local structures of the 2D nanosheets is highlighted. For this purpose, the local states of Na cations in inorganic 2D materials, in which the compositional fluctuations of a few percent are introduced in the tetrahedral and octahedral units of the 2D nanosheets, were systematically studied by means of {sup 23}Na magic-angle-spinning (MAS) nuclear magnetic resonance (NMR) and {sup 23}Na multiple-quantum MAS (MQMAS) NMR spectroscopy. In contrast with an uniform distribution of Na cations expected so far, various well-defined cation states sensitive to the local structures of the 2D nanosheets were identified. The tunability of the interlayer cation states along with the local structure of the 2D nanosheets, as the smallest structural unit of the 2D material, is discussed.
Electron correlations in two-dimensional small quantum dots
Sloggett, C.; Sushkov, O. P.
2005-06-01
We consider circular and elliptic quantum dots with parabolic external confinement, containing 0-22 electrons and with values of rs in the range 0perturbation theory. We demonstrate that in many cases correlations qualitatively change the spin structure of the ground state from that obtained under Hartree-Fock and spin-density-functional calculations. In some cases the correlation effects destroy Hund’s rule. We also demonstrate that the correlations destroy static spin-density waves observed in Hartree-Fock and spin-density-functional calculations.
Carrier transport in multi-terminal superconductor/two-dimensional electron gas Josephson junctions
Guzenko, V.A.; Schäpers, Th.; Müller, R.P.; Golubov, Alexandre Avraamovitch; Brinkman, Alexander; Crecelius, G.; Kaluza, A.; Lüth, H.
2001-01-01
The critical current in a superconductor/two-dimensional electron gas junction/superconductor junction is controlled by an injection current. In case of a carrier injection from one contact to the semiconductor through the two-dimensional electron gas region of the junction to an ohmic contact at
Center Line Slope Analysis in Two-Dimensional Electronic Spectroscopy
?anda, Franti?ek; Perl?k, V?clav; Lincoln, Craig N.; Hauer, J?rgen
2015-01-01
Center line slope (CLS) analysis in 2D infrared spectroscopy has been extensively used to extract frequency?frequency correlation functions of vibrational transitions. We apply this concept to 2D electronic spectroscopy, where CLS is a measure of electronic gap fluctuations. The two domains, infrared and electronic, possess differences: In the infrared, the frequency fluctuations are classical, often slow and Gaussian. In contrast, electronic spectra are subject to fast spectral diffusion and...
Temperature dependent transport of two dimensional electrons in the integral quantum Hall regime
International Nuclear Information System (INIS)
Wi, H.P.
1986-01-01
This thesis is concerned with the temperature dependent electronic transport properties of a two dimensional electron gas subject to background potential fluctuations and a perpendicular magnetic field. The author carried out an extensive temperature dependent study of the transport coefficients, in the region of an integral quantum plateau, in an In/sub x/Ga/sub 1-x/As/InP heterostructure for 4.2K 10 cm -2 meV -1 ) even at the middle between two Landau levels, which is unexpected from model calculations based on short ranged randomness. In addition, the different T dependent behavior of rho/sub xx/ between the states in the tails and those near the center of a Landau level, indicates the existence of different electron states in a Landau level. Additionally, the author reports T-dependent transport measurements in the transition region between two quantum plateaus in several different materials
Electron-phonon heat exchange in quasi-two-dimensional nanolayers
Anghel, Dragos-Victor; Cojocaru, Sergiu
2017-12-01
We study the heat power P transferred between electrons and phonons in thin metallic films deposited on free-standing dielectric membranes. The temperature range is typically below 1 K, such that the wavelengths of the excited phonon modes in the system is large enough so that the picture of a quasi-two-dimensional phonon gas is applicable. Moreover, due to the quantization of the components of the electron wavevectors perpendicular to the metal film's surface, the electrons spectrum forms also quasi two-dimensional sub-bands, as in a quantum well (QW). We describe in detail the contribution to the electron-phonon energy exchange of different electron scattering channels, as well as of different types of phonon modes. We find that heat flux oscillates strongly with thickness of the film d while having a much smoother variation with temperature (Te for the electrons temperature and Tph for the phonons temperature), so that one obtains a ridge-like landscape in the two coordinates, (d, Te) or (d, Tph), with crests and valleys aligned roughly parallel to the temperature axis. For the valley regions we find P ∝ Te3.5 - Tph3.5. From valley to crest, P increases by more than one order of magnitude and on the crests P cannot be represented by a simple power law. The strong dependence of P on d is indicative of the formation of the QW state and can be useful in controlling the heat transfer between electrons and crystal lattice in nano-electronic devices. Nevertheless, due to the small value of the Fermi wavelength in metals, the surface imperfections of the metallic films can reduce the magnitude of the oscillations of P vs. d, so this effect might be easier to observe experimentally in doped semiconductors.
Energy Technology Data Exchange (ETDEWEB)
Albert, Julian; Falge, Mirjam; Hildenbrand, Heiko; Engel, Volker [Universität Würzburg, Institut für Physikalische und Theoretische Chemie, Emil-Fischer-Str. 42, Campus Nord, Am Hubland, 97074 Würzburg (Germany); Gomez, Sandra; Sola, Ignacio R. [Departamento de Quimica Fisica, Universidad Complutense, 28040 Madrid (Spain)
2015-07-28
We theoretically investigate the photon-echo spectroscopy of coupled electron-nuclear quantum dynamics. Two situations are treated. In the first case, the Born-Oppenheimer (adiabatic) approximation holds. It is then possible to interpret the two-dimensional (2D) spectra in terms of vibrational motion taking place in different electronic states. In particular, pure vibrational coherences which are related to oscillations in the time-dependent third-order polarization can be identified. This concept fails in the second case, where strong non-adiabatic coupling leads to the breakdown of the Born-Oppenheimer-approximation. Then, the 2D-spectra reveal a complicated vibronic structure and vibrational coherences cannot be disentangled from the electronic motion.
Two Dimensional Steady State Eddy Current Analysis of a Spinning Conducting Cylinder
2017-03-09
UNCLASSIFIED UNCLASSIFIED AD-E403 855 Technical Report ARMET-TR-16045 TWO- DIMENSIONAL STEADY-STATE EDDY CURRENT ANALYSIS OF A...August 2014 4. TITLE AND SUBTITLE TWO- DIMENSIONAL STEADY-STATE EDDY CURRENT ANALYSIS OF A SPINNING CONDUCTING CYLINDER 5a. CONTRACT NUMBER 5b...analytical closed-form analysis performed by Michael P. Perry and Thomas B. Jones (ref. 4). Two- dimensional (2D) finite element steady state analyses
Energy spectrum of two-dimensional tight-binding electrons in a spatially varying magnetic field
International Nuclear Information System (INIS)
Oh, G.Y.; Lee, M.H.
1996-01-01
The electronic energy spectrum of a two-dimensional lattice in a spatially varying magnetic field is studied within the framework of the tight-binding model by using the scheme of the transfer matrix. It is found that, in comparison with the case of a uniform magnetic field, the energy spectrum exhibits more complicated behavior; band broadening (or gap closing) and band splitting (or gap opening) occur depending on characteristic parameters of the lattice. The origin of these phenomena lies in the existence of direct touching and indirect overlapping between neighboring subbands. Dependence of direct touching and indirect overlapping, and thus the electronic band structure together with the density of states, on characteristic parameters of the lattice is elucidated in detail. copyright 1996 The American Physical Society
International Nuclear Information System (INIS)
Moskalenko, S.A.; Podlesny, I.V.; Lelyakov, I.A.; Novikov, B.V.; Kiselyova, E.S.; Gherciu, L.
2011-01-01
The Rashba spin-orbit coupling (RSOC) in the case of two-dimensional (2D) electrons and holes in a strong perpendicular magnetic field was studied. The spinor-type wave functions are characterized by different numbers of Landau levels in different spin projections. For electrons they differ by 1 as was established earlier by Rashba, whereas for holes they differ by 3. Two lowest electron states and four lowest hole states of Landau quantization give rise to eight 2D magnetoexciton states. The exchange electron-hole interaction in the frame of these states is investigated.
Energy Technology Data Exchange (ETDEWEB)
Dahlberg, Peter D. [Graduate Program in the Biophysical Sciences, Institute for Biophysical Dynamics, and The James Franck Institute, The University of Chicago, Chicago, Illinois 60637 (United States); Norris, Graham J.; Wang, Cheng; Viswanathan, Subha; Singh, Ved P.; Engel, Gregory S., E-mail: gsengel@uchicago.edu [Department of Chemistry, Institute for Biophysical Dynamics, and The James Franck Institute, The University of Chicago, Chicago, Illinois 60637 (United States)
2015-09-14
Energy transfer through large disordered antenna networks in photosynthetic organisms can occur with a quantum efficiency of nearly 100%. This energy transfer is facilitated by the electronic structure of the photosynthetic antennae as well as interactions between electronic states and the surrounding environment. Coherences in time-domain spectroscopy provide a fine probe of how a system interacts with its surroundings. In two-dimensional electronic spectroscopy, coherences can appear on both the ground and excited state surfaces revealing detailed information regarding electronic structure, system-bath coupling, energy transfer, and energetic coupling in complex chemical systems. Numerous studies have revealed coherences in isolated photosynthetic pigment-protein complexes, but these coherences have not been observed in vivo due to the small amplitude of these signals and the intense scatter from whole cells. Here, we present data acquired using ultrafast video-acquisition gradient-assisted photon echo spectroscopy to observe quantum beating signals from coherences in vivo. Experiments were conducted on isolated light harvesting complex II (LH2) from Rhodobacter sphaeroides, whole cells of R. sphaeroides, and whole cells of R. sphaeroides grown in 30% deuterated media. A vibronic coherence was observed following laser excitation at ambient temperature between the B850 and the B850{sup ∗} states of LH2 in each of the 3 samples with a lifetime of ∼40-60 fs.
Henzl, Jörg; Morgenstern, Karina
2010-06-21
Supramolecular assemblies of 4-anilino-4'-nitroazobenzene are investigated on the Au(111) surface by low temperature scanning tunneling microscopy and spectroscopy with submolecular resolution. Adsorption at 250 K leads to three different structures that are formed via hydrogen bonds: a star structure and two types of line structures: a meandering and a zigzag line. The formation of these supramolecular assemblies is affected by the available space on the fcc domains of the reconstructed Au(111) substrate as well as by the two-dimensional chirality of the molecules on the surface. The star structure is enantiomerically pure, while both types of lines consist of a racemic mixture. Bonding between homochiral pairs differ from the one between heterochiral pairs in the position of the hydrogen bonds. Inside these supramolecular assemblies two configurations of the molecules are identified: An almost straight trans-configuration and a slightly bent cis*-configuration. The trans-configuration largely reflects the structure of this isomer in gas phase, while the cis*-configuration is two-dimensional on the surface in contrast to the three-dimensional gas phase cis-configuration. The reversible trans-cis* isomerization is induced by electron tunneling through the LUMO+1 state of the molecule, which is located at +2.9 V.
International Nuclear Information System (INIS)
Kamiya, Toshio; Ueda, Kazushige; Hiramatsu, Hidenori; Kamioka, Hayato; Ohta, Hiromichi; Hirano, Masahiro; Hosono, Hideo
2005-01-01
Electronic structures of layered oxychalcogenides LaCuOCh (Ch=S, Se, Te) were studied using relativistic ab initio band calculations to understand their optical and electronic properties. Step-like structures terminated with one or two sharp peaks were observed in low-temperature (10 K) optical absorption spectra. Third optical nonlinearity measurements supported that the sharp peaks came from split excitonic levels. The ab initio calculations reproduced well these characteristic structures in the spectra and proved that the step-like optical absorption structures originated from two-dimensional nature of the electronic structures associated with the layered crystal structure of LaCuOCh. The split energies of the excitonic levels were quantitatively explained by spin-orbit interaction in the chalcogen ions
Raichev, O. E.
2018-04-01
It is shown that the classical commensurability phenomena in weakly modulated two-dimensional electron systems is a manifestation of the intrinsic properties of the correlation functions describing a homogeneous electron gas in a magnetic field. The theory demonstrates the importance for consideration of nonlocal response and removes the gap between classical and quantum approaches to magnetotransport in such systems.
Spin-polarized transport in a two-dimensional electron gas with interdigital-ferromagnetic contacts
DEFF Research Database (Denmark)
Hu, C.-M.; Nitta, Junsaku; Jensen, Ane
2001-01-01
Ferromagnetic contacts on a high-mobility, two-dimensional electron gas (2DEG) in a narrow gap semiconductor with strong spin-orbit interaction are used to investigate spin-polarized electron transport. We demonstrate the use of magnetized contacts to preferentially inject and detect specific spi...
Electron transport in the two-dimensional channel material - zinc oxide nanoflake
Lai, Jian-Jhong; Jian, Dunliang; Lin, Yen-Fu; Ku, Ming-Ming; Jian, Wen-Bin
2018-03-01
ZnO nanoflakes of 3-5 μm in lateral size and 15-20 nm in thickness are synthesized. The nanoflakes are used to make back-gated transistor devices. Electron transport in the ZnO nanoflake channel between source and drain electrodes are investigated. In the beginning, we argue and determine that electrons are in a two-dimensional system. We then apply Mott's two-dimensional variable range hopping model to analyze temperature and electric field dependences of resistivity. The disorder parameter, localization length, hopping distance, and hopping energy of the electron system in ZnO nanoflakes are obtained and, additionally, their temperature behaviors and dependences on room-temperature resistivity are presented. On the other hand, the basic transfer characteristics of the channel material are carried out, as well, and the carrier concentration, the mobility, and the Fermi wavelength of two-dimensional ZnO nanoflakes are estimated.
Electronic properties of two-dimensional MoS2 and its nanoribbons: a theoretical study
Hsu, Cheng-Hsiang; Soleimanikahnoj, Sina; Karimi, Farhad; Knezevic, Irena
Recent advances in producing monolayer and bilayer molybdenum disulfide (MoS2) have generated considerable interest in its fundamental properties. Two-dimensional MoS2 has a variety of intriguing but unexplored electronic and optical properties that are dependent on the number of layers in the material. Here, we present calculations of the electronic properties of two-dimensional MoS2 and its nanoribbons based on a semi-empirical tight-binding model and ballistic quantum transport theory. Utilizing simulation results, we discuss the potential of two-dimensional MoS2 and its nanostructures for low-power electronic applications. UW-Madison Hilldale Undergraduate Research Fellowship.
International Nuclear Information System (INIS)
Mao Wei; She Wei-Bo; Zhang Chao; Zhang Jin-Cheng; Zhang Jin-Feng; Liu Hong-Xia; Yang Lin-An; Zhang Kai; Zhao Sheng-Lei; Chen Yong-He; Zheng Xue-Feng; Hao Yue; Yang Cui; Ma Xiao-Hua
2014-01-01
In this paper, we present a two-dimensional (2D) fully analytical model with consideration of polarization effect for the channel potential and electric field distributions of the gate field-plated high electron mobility transistor (FP-HEMT) on the basis of 2D Poisson's solution. The dependences of the channel potential and electric field distributions on drain bias, polarization charge density, FP structure parameters, AlGaN/GaN material parameters, etc. are investigated. A simple and convenient approach to designing high breakdown voltage FP-HEMTs is also proposed. The validity of this model is demonstrated by comparison with the numerical simulations with Silvaco—Atlas. The method in this paper can be extended to the development of other analytical models for different device structures, such as MIS-HEMTs, multiple-FP HETMs, slant-FP HEMTs, etc. (condensed matter: electronic structure, electrical, magnetic, and optical properties)
Magnetoresistance of a two-dimensional electron gas in a random magnetic field
DEFF Research Database (Denmark)
Smith, Anders; Taboryski, Rafael Jozef; Hansen, Luise Theil
1994-01-01
We report magnetoresistance measurements on a two-dimensional electron gas made from a high-mobility GaAs/AlxGa1-xAs heterostructure, where the externally applied magnetic field was expelled from regions of the semiconductor by means of superconducting lead grains randomly distributed on the surf......We report magnetoresistance measurements on a two-dimensional electron gas made from a high-mobility GaAs/AlxGa1-xAs heterostructure, where the externally applied magnetic field was expelled from regions of the semiconductor by means of superconducting lead grains randomly distributed...
Chern-Simons field theory of two-dimensional electrons in the lowest Landau level
International Nuclear Information System (INIS)
Zhang, L.
1996-01-01
We propose a fermion Chern-Simons field theory describing two-dimensional electrons in the lowest Landau level. This theory is constructed with a complete set of states, and the lowest-Landau-level constraint is enforced through a δ functional described by an auxiliary field λ. Unlike the field theory constructed directly with the states in the lowest Landau level, this theory allows one, utilizing the physical picture of open-quote open-quote composite fermion,close-quote close-quote to study the fractional quantum Hall states by mapping them onto certain integer quantum Hall states; but, unlike its application in the unconstrained theory, such a mapping is sensible only when interactions between electrons are present. An open-quote open-quote effective mass,close-quote close-quote which characterizes the scale of low energy excitations in the fractional quantum Hall systems, emerges naturally from our theory. We study a Gaussian effective theory and interpret physically the dressed stationary point equation for λ as an equation for the open-quote open-quote mass renormalization close-quote close-quote of composite fermions. copyright 1996 The American Physical Society
Direct Measurement of the Band Structure of a Buried Two-Dimensional Electron Gas
DEFF Research Database (Denmark)
Miwa, Jill; Hofmann, Philip; Simmons, Michelle Y.
2013-01-01
We directly measure the band structure of a buried two dimensional electron gas (2DEG) using angle resolved photoemission spectroscopy. The buried 2DEG forms 2 nm beneath the surface of p-type silicon, because of a dense delta-type layer of phosphorus n-type dopants which have been placed there...
Model of two-dimensional electron gas formation at ferroelectric interfaces
Energy Technology Data Exchange (ETDEWEB)
Aguado-Puente, P.; Bristowe, N. C.; Yin, B.; Shirasawa, R.; Ghosez, Philippe; Littlewood, P. B.; Artacho, Emilio
2015-07-01
The formation of a two-dimensional electron gas at oxide interfaces as a consequence of polar discontinuities has generated an enormous amount of activity due to the variety of interesting effects it gives rise to. Here, we study under what circumstances similar processes can also take place underneath ferroelectric thin films. We use a simple Landau model to demonstrate that in the absence of extrinsic screening mechanisms, a monodomain phase can be stabilized in ferroelectric films by means of an electronic reconstruction. Unlike in the LaAlO3/SrTiO3 heterostructure, the emergence with thickness of the free charge at the interface is discontinuous. This prediction is confirmed by performing first-principles simulations of free-standing slabs of PbTiO3. The model is also used to predict the response of the system to an applied electric field, demonstrating that the two-dimensional electron gas can be switched on and off discontinuously and in a nonvolatile fashion. Furthermore, the reversal of the polarization can be used to switch between a two-dimensional electron gas and a two-dimensional hole gas, which should, in principle, have very different transport properties. We discuss the possible formation of polarization domains and how such configuration competes with the spontaneous accumulation of free charge at the interfaces.
Magnetization of a two-dimensional electron gas with a spin-orbit interaction
International Nuclear Information System (INIS)
Hatano, Naomichi; Shirasaki, Ryoen; Nakamura, Hiroaki
2006-04-01
We argue that a two-dimensional electron gas with a spin-orbit interaction is magnetized when a voltage is applied with the Fermi level tuned to be in the energy gap. The magnetization is an indication of spin-carrying currents due to the spin-orbit interaction. (author)
Schapers, T; Nitta, J; Heersche, HB; Takayanagi, H
The spin dependent conductance of a ferromagnet/two-dimensional electron gas ferromagnet structure is theoretically examined in the ballistic transport regime. It is shown that the spin signal can be improved considerably by making use of the spin filtering effect of a barrier at the ferromagnet
High-mobility two-dimensional electron gases at oxide interfaces: Origins and opportunities
DEFF Research Database (Denmark)
Chen, Yunzhong; Pryds, Nini; Sun, Ji-Rong
2013-01-01
Our recent experimental work on metallic and insulating interfaces controlled by interfacial redox reactions in SrTiO3-based heterostructures is reviewed along with a more general background of two-dimensional electron gas (2DEG) at oxide interfaces. Due to the presence of oxygen vacancies at the...
Active ideal sedimentation: exact two-dimensional steady states.
Hermann, Sophie; Schmidt, Matthias
2018-02-28
We consider an ideal gas of active Brownian particles that undergo self-propelled motion and both translational and rotational diffusion under the influence of gravity. We solve analytically the corresponding Smoluchowski equation in two space dimensions for steady states. The resulting one-body density is given as a series, where each term is a product of an orientation-dependent Mathieu function and a height-dependent exponential. A lower hard wall is implemented as a no-flux boundary condition. Numerical evaluation of the suitably truncated analytical solution shows the formation of two different spatial regimes upon increasing Peclet number. These regimes differ in their mean particle orientation and in their variation of the orientation-averaged density with height.
General solution of the Dirac equation for quasi-two-dimensional electrons
Energy Technology Data Exchange (ETDEWEB)
Eremko, Alexander, E-mail: eremko@bitp.kiev.ua [Bogolyubov Institute for Theoretical Physics, Metrologichna Str., 14-b, Kyiv, 03680 (Ukraine); Brizhik, Larissa, E-mail: brizhik@bitp.kiev.ua [Bogolyubov Institute for Theoretical Physics, Metrologichna Str., 14-b, Kyiv, 03680 (Ukraine); Loktev, Vadim, E-mail: vloktev@bitp.kiev.ua [Bogolyubov Institute for Theoretical Physics, Metrologichna Str., 14-b, Kyiv, 03680 (Ukraine); National Technical University of Ukraine “KPI”, Peremohy av., 37, Kyiv, 03056 (Ukraine)
2016-06-15
The general solution of the Dirac equation for quasi-two-dimensional electrons confined in an asymmetric quantum well, is found. The energy spectrum of such a system is exactly calculated using special unitary operator and is shown to depend on the electron spin polarization. This solution contains free parameters, whose variation continuously transforms one known particular solution into another. As an example, two different cases are considered in detail: electron in a deep and in a strongly asymmetric shallow quantum well. The effective mass renormalized by relativistic corrections and Bychkov–Rashba coefficients are analytically obtained for both cases. It is demonstrated that the general solution transforms to the particular solutions, found previously (Eremko et al., 2015) with the use of spin invariants. The general solution allows to establish conditions at which a specific (accompanied or non-accompanied by Rashba splitting) spin state can be realized. These results can prompt the ways to control the spin degree of freedom via the synthesis of spintronic heterostructures with the required properties.
High-Resolution Two-Dimensional Optical Spectroscopy of Electron Spins
Directory of Open Access Journals (Sweden)
M. Salewski
2017-08-01
Full Text Available Multidimensional coherent optical spectroscopy is one of the most powerful tools for investigating complex quantum mechanical systems. While it was conceived decades ago in magnetic resonance spectroscopy using microwaves and radio waves, it has recently been extended into the visible and UV spectral range. However, resolving MHz energy splittings with ultrashort laser pulses still remains a challenge. Here, we analyze two-dimensional Fourier spectra for resonant optical excitation of resident electrons to localized trions or donor-bound excitons in semiconductor nanostructures subject to a transverse magnetic field. Particular attention is devoted to Raman coherence spectra, which allow one to accurately evaluate tiny splittings of the electron ground state and to determine the relaxation times in the electron spin ensemble. A stimulated steplike Raman process induced by a sequence of two laser pulses creates a coherent superposition of the ground-state doublet which can be retrieved only optically because of selective excitation of the same subensemble with a third pulse. This provides the unique opportunity to distinguish between different complexes that are closely spaced in energy in an ensemble. The related experimental demonstration is based on photon-echo measurements in an n-type CdTe/(Cd,MgTe quantum-well structure detected by a heterodyne technique. The difference in the sub-μeV range between the Zeeman splittings of donor-bound electrons and electrons localized at potential fluctuations can be resolved even though the homogeneous linewidth of the optical transitions is larger by 2 orders of magnitude.
Current-induced magnetoresistance oscillations in two-dimensional electron systems
Lei, X. L.
2006-01-01
Electric current-induced magnetoresistance oscillations recently discovered in two-dimensional electron systems are analyzed using a microscopic scheme for nonlinear magnetotransport direct controlled by the current. The magnetoresistance oscillations are shown to result from drift-motion assisted electron scatterings between Landau levels. The theoretical predictions not only reproduce all the main features observed in the experiments but also disclose other details of the phenomenon.
The static and dynamic screening of power loss of a two-dimensional electron gas
Bennett, C.; Balkan, N.; Tanatar, B.; Celik, H.; Cankurtaran, M.
1998-07-01
Experimental results concerning the well-width dependence of the acoustic-phonon-assisted energy relaxation of a two-dimensional electron gas in GaAs/Ga1 - xAlxAs quantum-well structures are compared with theoretical models that involve piezoelectric and deformation-potential scattering and the effects of static and dynamic screening of the electron-acoustic phonon interaction. It is shown that screening only slightly modifies the predictions of the approximate calculations.
Kinetics of two-dimensional electron plasma, interacting with fluctuating potential
International Nuclear Information System (INIS)
Boiko, I.I.; Sirenko, Y.M.
1990-01-01
In this paper, from the first principles, after the fashion of Klimontovich, the authors derive quantum kinetic equation for electron gas, inhomogeneous in z-direction and homogeneous in XY-plane. Special attention is given to the systems with quasi-two-dimensional electron gas (2 DEG), which are widely explored now. Both interaction between the particles of 2 DEG (in general, of several sorts), and interaction with an external system (phonons, impurities, after change carries etc.) are considered. General theory is used to obtain energy and momentum balance equations and relaxation frequencies for 2 DEG in the basis of plane waves. The case of crossed electric and magnetic fields is also treated. As an illustration the problems of 2 DEG scattering on semibounded three-dimensional electron gas and on two-dimensional hole gas are considered; transverse conductivity of nondegenerate 2 DEG, scattered by impurities in ultraquantum magnetic field, is calculated
Roslyak, O.; Gumbs, Godfrey; Mukamel, S.
2012-05-01
We study the localization of dressed Dirac electrons in a cylindrical quantum dot (QD) formed on monolayer and bilayer graphene by spatially different potential profiles. Short lived excitonic states which are too broad to be resolved in linear spectroscopy are revealed by cross peaks in the photon-echo nonlinear technique. Signatures of the dynamic gap in the two-dimensional spectra are discussed. The effect of the Coulomb induced exciton-exciton scattering and the formation of biexciton molecules are demonstrated.
Two-dimensional electron transport in AlGaN/GaN heterostructures
International Nuclear Information System (INIS)
Tan Renbing; Xu Wen; Zhou Yu; Zhang Xiaoyu; Qin Hua
2012-01-01
We present a theoretical study of electron transport properties of two-dimensional electron gas in AlGaN/GaN heterostructures. By assuming a drifted Fermi-Dirac distribution and taking into account all major scattering mechanisms, including polar optical and acoustic phonons, background impurities, dislocation and interface roughness, the momentum- and energy-balance equations derived from Boltzmann equation are solved self-consistently. The dependence of the electron drift velocity and electron temperature as a function of the applied electric field are obtained and discussed.
Two-dimensional electron transport in AlGaN/GaN heterostructures
Energy Technology Data Exchange (ETDEWEB)
Tan Renbing [Key Laboratory of Nanodevices and Applications, Suzhou Institute of Nano-tech and Nano-bionics, Chinese Academy of Sciences, Suzhou 215125 (China); Institute of Semiconductors, Chinese Academy of Sciences, Beijing 100083 (China); Graduate University of Chinese Academy of Sciences, Beijing 100049 (China); Xu Wen, E-mail: wenxu_issp@yahoo.cn [Key Laboratory of Materials Physics, Institute of Solid State Physics, Chinese Academy of Sciences, Hefei 230031 (China); Zhou Yu; Zhang Xiaoyu [Key Laboratory of Nanodevices and Applications, Suzhou Institute of Nano-tech and Nano-bionics, Chinese Academy of Sciences, Suzhou 215125 (China); Qin Hua, E-mail: hqin2007@sinano.ac.cn [Key Laboratory of Nanodevices and Applications, Suzhou Institute of Nano-tech and Nano-bionics, Chinese Academy of Sciences, Suzhou 215125 (China)
2012-11-01
We present a theoretical study of electron transport properties of two-dimensional electron gas in AlGaN/GaN heterostructures. By assuming a drifted Fermi-Dirac distribution and taking into account all major scattering mechanisms, including polar optical and acoustic phonons, background impurities, dislocation and interface roughness, the momentum- and energy-balance equations derived from Boltzmann equation are solved self-consistently. The dependence of the electron drift velocity and electron temperature as a function of the applied electric field are obtained and discussed.
Commensurability oscillations by snake-orbit magnetotransport in two-dimensional electron gases
Leuschner, A.; Schluck, J.; Cerchez, M.; Heinzel, T.; Pierz, K.; Schumacher, H. W.
2017-04-01
Commensurate magnetoresistance periodic oscillations generated by transversal electron snake orbits are found experimentally. A two-dimensional electron gas is exposed to a magnetic field that changes sign along the current longitudinal direction and is homogeneous in the transverse direction. The change in sign of the magnetic field directs the electron flow along the transversal direction, in snake orbits. This generates resistance oscillations with a predictable periodicity that is commensurate with the width of the electron gas. Numerical simulations are used to reveal the character of the oscillations.
Growth and electronic properties of two-dimensional systems on (110) oriented GaAs
Energy Technology Data Exchange (ETDEWEB)
Fischer, F.
2005-07-01
As the only non-polar plane the (110) surface has a unique role in GaAs. Together with Silicon as a dopant it is an important substrate orientation for the growth of n-type or p-type heterostructures. As a consequence, this thesis will concentrate on growth and research on that surface. In the course of this work we were able to realize two-dimensional electron systems with the highest mobilities reported so far on this orientation. Therefore, we review the necessary growth conditions and the accompanying molecular process. The two-dimensional electron systems allowed the study of a new, intriguing transport anisotropy not explained by current theory. Moreover, we were the first growing a two-dimensional hole gas on (110) GaAs with Si as dopant. For this purpose we invented a new growth modulation technique necessary to retrieve high mobility systems. In addition, we discovered and studied the metal-insulator transition in thin bulk p-type layers on (110) GaAs. Besides we investigated the activation process related to the conduction in the valence band and a parallelly conducting hopping band. The new two-dimensional hole gases revealed interesting physics. We studied the zero B-field spin splitting in these systems and compared it with the known theory. Furthermore, we investigated the anisotropy of the mobility. As opposed to the expectations we observed a strong persistent photoconductivity in our samples. Landau levels for two dimensional hole systems are non-linear and can show anticrossings. For the first time we were able to resolve anticrossings in a transport experiment and study the corresponding activation process. Finally, we compared these striking results with theoretical calculations. (orig.)
Polarizational stopping power of heavy-ion diclusters in two-dimensional electron liquids
International Nuclear Information System (INIS)
Ballester, D.; Fuentes, A. M.; Tkachenko, I. M.
2007-01-01
The in-plane polarizational stopping power of heavy-ion diclusters in a two-dimensional strongly coupled electron liquid is studied. Analytical expressions for the stopping power of both fast and slow projectiles are derived. To go beyond the random-phase approximation we make use of the inverse dielectric function obtained by means of the method of moments and some recent analytical expressions for the static local-field correction factor
Interaction-induced huge magnetoresistance in a high mobility two-dimensional electron gas
Energy Technology Data Exchange (ETDEWEB)
Bockhorn, L.; Haug, R. J. [Institut für Festkörperphysik, Leibniz Universität Hannover, D-30167 Hannover (Germany); Gornyi, I. V. [Institut für Nanotechnologie, Karlsruher Institut of Technology, D-76021 Karlsruhe (Germany); Schuh, D. [Institut für Experimentelle und Angewandte Physik, Universität Regensburg, D-93053 Regensburg (Germany); Wegscheider, W. [ETH Zürich (Switzerland)
2013-12-04
A strong negative magnetoresistance is observed in a high-mobility two-dimensional electron gas in a GaAs/Al{sub 0.3}Ga{sub 0.7}As quantum well. We discuss that the negative magnetoresistance consists of a small peak induced by a combination of two types of disorder and a huge magnetoresistance explained by the interaction correction to the conductivity for mixed disorder.
Curvature-tuned InAs-based shells containing two-dimensional electron gas
Energy Technology Data Exchange (ETDEWEB)
Mutilin, S V; Vorobyova, Ju S; Vorob' ev, A B; Putyato, M A; Prinz, V Ya, E-mail: s.mutilin@gmail.com [AV Rzhanov Institute of Semiconductor Physics, 630090, acad. Lavrentyev ave., 13, Novosibirsk (Russian Federation)
2011-09-14
Conducting InAs/AlSb/GaSb shells of curvature radius {approx}10 {mu}m are fabricated on GaSb (1 0 0) substrates. In the InAs quantum well, the shells are shown to contain a two-dimensional electron gas. Controlled tuning of the curvature of the formed shells in excess of three times is demonstrated. The sequence of fabrication steps for forming curvature-tuned InAs-based shells with quantum well is described.
Oliver, Thomas A A; Lewis, Nicholas H C; Fleming, Graham R
2014-07-15
Multidimensional nonlinear spectroscopy, in the electronic and vibrational regimes, has reached maturity. To date, no experimental technique has combined the advantages of 2D electronic spectroscopy and 2D infrared spectroscopy, monitoring the evolution of the electronic and nuclear degrees of freedom simultaneously. The interplay and coupling between the electronic state and vibrational manifold is fundamental to understanding ensuing nonradiative pathways, especially those that involve conical intersections. We have developed a new experimental technique that is capable of correlating the electronic and vibrational degrees of freedom: 2D electronic-vibrational spectroscopy (2D-EV). We apply this new technique to the study of the 4-(di-cyanomethylene)-2-methyl-6-p-(dimethylamino)styryl-4H-pyran (DCM) laser dye in deuterated dimethyl sulfoxide and its excited state relaxation pathways. From 2D-EV spectra, we elucidate a ballistic mechanism on the excited state potential energy surface whereby molecules are almost instantaneously projected uphill in energy toward a transition state between locally excited and charge-transfer states, as evidenced by a rapid blue shift on the electronic axis of our 2D-EV spectra. The change in minimum energy structure in this excited state nonradiative crossing is evident as the central frequency of a specific vibrational mode changes on a many-picoseconds timescale. The underlying electronic dynamics, which occur on the hundreds of femtoseconds timescale, drive the far slower ensuing nuclear motions on the excited state potential surface, and serve as a excellent illustration for the unprecedented detail that 2D-EV will afford to photochemical reaction dynamics.
Spin-charge conversion in disordered two-dimensional electron gases lacking inversion symmetry
Huang, Chunli; Milletarı, Mirco; Cazalilla, Miguel A.
2017-11-01
We study the spin-charge conversion mechanisms in a two-dimensional gas of electrons moving in a smooth disorder potential by accounting for both Rashba-type and Mott's skew scattering contributions. We find that the quantum interference effects between spin-flip and skew scattering give rise to anisotropic spin precession scattering (ASP), a direct spin-charge conversion mechanism that was discovered in an earlier study of graphene decorated with adatoms [Huang et al., Phys. Rev. B 94, 085414 (2016), 10.1103/PhysRevB.94.085414]. Our findings suggest that, together with other spin-charge conversion mechanisms such as the inverse galvanic effect, ASP is a fairly universal phenomenon that should be present in disordered two-dimensional systems lacking inversion symmetry.
Splitting rules for the electronic spectra of two-dimensional SML quasilattices
Chen, Fuming; Yang, Xiangbo; Xing, Da; Li, Feng
2004-12-01
In the framework of single-electronic tight-binding nearest-interaction transfer model, after establishing the method of constructing a class of two-dimensional SML quasilattices, we have studied the spectral properties of two-dimensional SML quasilattices by means of a decomposition-decimation method based the renormalization-group technique. It is found that the spectra have a variety of multifurcating structures, the total spectra are symmetrical, and every spectral line splits into odd sub-bands in the higher hierarchy. The analytic results show that under the first approximation, there exist only six kinds of clusters and the bare energy splits into thirteen subbands, and under the second approximation, several kinds of new spitting manners occur, e.g., 1:33, 1:19. The analytical results are confirmed by numerical simulations.
Directory of Open Access Journals (Sweden)
Mingxiao Ye
2017-06-01
Full Text Available Two-dimensional transition metal dichalcogenides (2D TMDCs offer several attractive features for use in next-generation electronic and optoelectronic devices. Device applications of TMDCs have gained much research interest, and significant advancement has been recorded. In this review, the overall research advancement in electronic and optoelectronic devices based on TMDCs are summarized and discussed. In particular, we focus on evaluating field effect transistors (FETs, photovoltaic cells, light-emitting diodes (LEDs, photodetectors, lasers, and integrated circuits (ICs using TMDCs.
Electron- and photon-induced plasmonic excitations in two-dimensional silver nanostructures
Energy Technology Data Exchange (ETDEWEB)
Hoang, C. V.; Rana, M. [International Center for Materials Nanoarchitectonics (MANA), National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044 (Japan); Nagao, T., E-mail: Nagao.Tadaaki@nims.go.jp [International Center for Materials Nanoarchitectonics (MANA), National Institute for Materials Science, 1-1 Namiki, Tsukuba 305-0044 (Japan); CREST, Japan Science and Technology Agency, 4-1-8 Honcho, Kawaguchi, Saitama 332-0012 (Japan)
2014-06-23
Plasmons are the quasi particles of collective oscillations of electrons and form the basis of plasmonics and optical metamaterials. We combined electron spectroscopy and optical spectroscopy techniques to study plasmons in atomically smooth Ag films and in epitaxial Ag nanodisks to map the momentum-energy dispersion curves of the two-dimensional (2D) sheet plasmon and the quasi-2D plasmons to clarify the essential differences between them. Our experimental results combined with the results of numerical electromagnetic simulations showed that the bulk-like nature of the silver plasmon starts in layers that are only two atoms thick.
Optical-phonon-induced frictional drag in coupled two-dimensional electron gases
DEFF Research Database (Denmark)
Hu, Ben Yu-Kuang
1998-01-01
The role of optical phonons in frictional drag between two adjacent but electrically isolated two-dimensional electron gases is investigated. Since the optical phonons in III-V materials have a considerably larger coupling to electrons than acoustic phonons (which are the dominant drag mechanism...... group velocity at the Brillouin zone center, and (ii) the typical momentum transfer for an optical-phonon-mediated scattering is relatively large. These considerations make optical-phonon-mediated drag difficult to see in single-subband GaAs systems, but it may be possible to see the effect in double...
Ramaswamy, Rahul
Two-dimensional electron gas (2DEG) in semiconductor heterostructures was identified as a promising medium for hot-electron bolometers (HEB) in the early 90s. Up until now all research based on 2DEG HEBs is done using high mobility AlGaAs/GaAs heterostructures. These systems have demonstrated very good performance, but only in the sub terahertz (THz) range. However, above ˜0.5 THz the performance of AlGaAs/GaAs detectors drastically deteriorates. It is currently understood, that detectors fabricated from standard AlGaAs/GaAs heterostructures do not allow for reasonable coupling to THz radiation while maintaining high conversion efficiency. In this work we have developed 2DEG HEBs based on disordered Gallium Nitride (GaN) semiconductor, that operate at frequencies beyond 1THz at room temperature. We observe strong free carrier absorption at THz frequencies in our disordered 2DEG film due to Drude absorption. We show the design and fabrication procedures of novel micro-bolometers having ultra-low heat capacities. In this work the mechanism of 2DEG response to THz radiation is clearly identified as bolometric effect through our direct detection measurements. With optimal doping and detector geometry, impedances of 10--100 O have been achieved, which allow integration of these devices with standard THz antennas. We also demonstrate performance of the antennas used in this work in effectively coupling THz radiation to the micro-bolometers through polarization dependence and far field measurements. Finally heterodyne mixing due to hot electrons in the 2DEG micro-bolometer has been performed at sub terahertz frequencies and a mixing bandwidth greater than 3GHz has been achieved. This indicates that the characteristic cooling time in our detectors is fast, less than 50ps. Due to the ultra-low heat capacity; these detectors can be used in a heterodyne system with a quantum cascade laser (QCL) as a local oscillator (LO) which typically provides output powers in the micro
Surface states of topological insulators: the Dirac fermion in curved two-dimensional spaces.
Lee, Dung-Hai
2009-11-06
The surface of a topological insulator is a closed two-dimensional manifold. The surface states are described by the Dirac Hamiltonian in curved two-dimensional spaces. For a slablike sample with a magnetic field perpendicular to its top and bottom surfaces, there are chiral states delocalized on the four side faces. These "chiral sheets" carry both charge and spin currents. In strong magnetic fields, the quantized charge Hall effect [sigma(xy) = (2n + 1)e2/h] will coexist with spin Hall effect.
Chimera states in two-dimensional networks of locally coupled oscillators
Kundu, Srilena; Majhi, Soumen; Bera, Bidesh K.; Ghosh, Dibakar; Lakshmanan, M.
2018-02-01
Chimera state is defined as a mixed type of collective state in which synchronized and desynchronized subpopulations of a network of coupled oscillators coexist and the appearance of such anomalous behavior has strong connection to diverse neuronal developments. Most of the previous studies on chimera states are not extensively done in two-dimensional ensembles of coupled oscillators by taking neuronal systems with nonlinear coupling function into account while such ensembles of oscillators are more realistic from a neurobiological point of view. In this paper, we report the emergence and existence of chimera states by considering locally coupled two-dimensional networks of identical oscillators where each node is interacting through nonlinear coupling function. This is in contrast with the existence of chimera states in two-dimensional nonlocally coupled oscillators with rectangular kernel in the coupling function. We find that the presence of nonlinearity in the coupling function plays a key role to produce chimera states in two-dimensional locally coupled oscillators. We analytically verify explicitly in the case of a network of coupled Stuart-Landau oscillators in two dimensions that the obtained results using Ott-Antonsen approach and our analytical finding very well matches with the numerical results. Next, we consider another type of important nonlinear coupling function which exists in neuronal systems, namely chemical synaptic function, through which the nearest-neighbor (locally coupled) neurons interact with each other. It is shown that such synaptic interacting function promotes the emergence of chimera states in two-dimensional lattices of locally coupled neuronal oscillators. In numerical simulations, we consider two paradigmatic neuronal oscillators, namely Hindmarsh-Rose neuron model and Rulkov map for each node which exhibit bursting dynamics. By associating various spatiotemporal behaviors and snapshots at particular times, we study the chimera
Directory of Open Access Journals (Sweden)
Armen N. Kocharian
2016-05-01
Full Text Available Rashba spin-orbit effects and electron correlations in the two-dimensional cylindrical lattices of square geometries are assessed using mesoscopic two-, three- and four-leg ladder structures. Here the electron transport properties are systematically calculated by including the spin-orbit coupling in tight binding and Hubbard models threaded by a magnetic flux. These results highlight important aspects of possible symmetry breaking mechanisms in square ladder geometries driven by the combined effect of a magnetic gauge field spin-orbit interaction and temperature. The observed persistent current, spin and charge polarizations in the presence of spin-orbit coupling are driven by separation of electron and hole charges and opposite spins in real-space. The modeled spin-flip processes on the pairing mechanism induced by the spin-orbit coupling in assembled nanostructures (as arrays of clusters engineered in various two-dimensional multi-leg structures provide an ideal playground for understanding spatial charge and spin density inhomogeneities leading to electron pairing and spontaneous phase separation instabilities in unconventional superconductors. Such studies also fall under the scope of current challenging problems in superconductivity and magnetism, topological insulators and spin dependent transport associated with numerous interfaces and heterostructures.
Inada, Yuki; Kamiya, Tomoki; Matsuoka, Shigeyasu; Kumada, Akiko; Ikeda, Hisatoshi; Hidaka, Kunihiko
2018-01-01
Two-dimensional electron density imaging over free burning SF6 arcs and SF6 gas-blast arcs was conducted at current zero using highly sensitive Shack-Hartmann type laser wavefront sensors in order to experimentally characterise electron density distributions for the success and failure of arc interruption in the thermal reignition phase. The experimental results under an interruption probability of 50% showed that free burning SF6 arcs with axially asymmetric electron density profiles were interrupted with a success rate of 88%. On the other hand, the current interruption of SF6 gas-blast arcs was reproducibly achieved under locally reduced electron densities and the interruption success rate was 100%.
Spin injection into a two-dimensional electron gas using inter-digital-ferromagnetic contacts
DEFF Research Database (Denmark)
Hu, C.M.; Nitta, J.; Jensen, Ane
2002-01-01
We present a model that describes the spin injection across a single interface with two electrodes. The spin-injection rate across a typical hybrid junction made of ferromagnet (FM) and a two-dimensional electron gas (2DEG) is found at the percentage level. We perforin spin-injection-detection ex......-injection-detection experiment on devices with two ferromagnetic contacts on a 2DEG confined in an InAs quantum well. A spin-injection rate of 4.5% is estimated from the measured magnetoresistance....
International Nuclear Information System (INIS)
Wang, C M; Lei, X L
2014-01-01
We study dc-current effects on the magnetoresistance oscillation in a two-dimensional electron gas with Rashba spin-orbit coupling, using the balance-equation approach to nonlinear magnetotransport. In the weak current limit the magnetoresistance exhibits periodical Shubnikov-de Haas oscillation with changing Rashba coupling strength for a fixed magnetic field. At finite dc bias, the period of the oscillation halves when the interbranch contribution to resistivity dominates. With further increasing current density, the oscillatory resistivity exhibits phase inversion, i.e., magnetoresistivity minima (maxima) invert to maxima (minima) at certain values of the dc bias, which is due to the current-induced magnetoresistance oscillation. (paper)
Determination of structure of oriented samples using two-dimensional solid state NMR techniques
International Nuclear Information System (INIS)
Jin Hong; Harbison, G.S.
1990-01-01
One dimensional and two-dimensional MAS techniques can give detailed information about the structure and dynamics of oriented systems. We describe the application of such techniques to the liquid-crystalline polymer poly(p-phenyleneterphtalimide) (PPTA), and thence deduce the solid-state structure of the material. (author). 9 refs.; 6 figs
Topological origin of edge states in two-dimensional inversion-symmetric insulators and semimetals
Miert, Guido van; Ortix, Carmine; de Morais Smith, C.
2017-01-01
Symmetries play an essential role in identifying and characterizing topological states of matter. Here, we classify topologically two-dimensional (2D) insulators and semimetals with vanishing spin-orbit coupling using time-reversal ($\\mathcal{T}$) and inversion ($\\mathcal{I}$) symmetry. This allows
Pseudo-time-reversal symmetry and topological edge states in two-dimensional acoustic crystals
Mei, Jun
2016-09-02
We propose a simple two-dimensional acoustic crystal to realize topologically protected edge states for acoustic waves. The acoustic crystal is composed of a triangular array of core-shell cylinders embedded in a water host. By utilizing the point group symmetry of two doubly degenerate eigenstates at the Î
Liquid structure and freezing of the two-dimensional classical electron fluid
International Nuclear Information System (INIS)
Ballone, P.; Pastore, G.; Rovere, M.; Tosi, M.P.
1984-11-01
Accurate theoretical results are reported for the pair correlation function of the classical two-dimensional electron liquid with r -1 interactions at strong coupling. The approach involves an evaluation of the bridge diagram corrections to the hypernetted-chain approximation, the role of low dimensionality being evident, relative to the case of the three-dimensional classical plasma, in an enhanced sensitivity to long range correlations. The liquid structure results are utilized in a density-wave theory of first-order freezing into the triangular lattice, the calculated coupling strength at freezing being in reasonable agreement with computer simulation results and with data on electron films on a liquid-He surface. The stability of the triangular electron lattice against deformation into a body-centered rectangular lattice is also discussed. (author)
Bonilla, L. L.; Carretero, M.; Segura, A.
2017-12-01
When quantized, traces of classically chaotic single-particle systems include eigenvalue statistics and scars in eigenfuntions. Since 2001, many theoretical and experimental works have argued that classically chaotic single-electron dynamics influences and controls collective electron transport. For transport in semiconductor superlattices under tilted magnetic and electric fields, these theories rely on a reduction to a one-dimensional self-consistent drift model. A two-dimensional theory based on self-consistent Boltzmann transport does not support that single-electron chaos influences collective transport. This theory agrees with existing experimental evidence of current self-oscillations, predicts spontaneous collective chaos via a period doubling scenario, and could be tested unambiguously by measuring the electric potential inside the superlattice under a tilted magnetic field.
Rajan, Arunkumar Chitteth; Rezapour, Mohammad Reza; Yun, Jeonghun; Cho, Yeonchoo; Cho, Woo Jong; Min, Seung Kyu; Lee, Geunsik; Kim, Kwang S
2014-02-25
Laser-driven molecular spectroscopy of low spatial resolution is widely used, while electronic current-driven molecular spectroscopy of atomic scale resolution has been limited because currents provide only minimal information. However, electron transmission of a graphene nanoribbon on which a molecule is adsorbed shows molecular fingerprints of Fano resonances, i.e., characteristic features of frontier orbitals and conformations of physisorbed molecules. Utilizing these resonance profiles, here we demonstrate two-dimensional molecular electronics spectroscopy (2D MES). The differential conductance with respect to bias and gate voltages not only distinguishes different types of nucleobases for DNA sequencing but also recognizes methylated nucleobases which could be related to cancerous cell growth. This 2D MES could open an exciting field to recognize single molecule signatures at atomic resolution. The advantages of the 2D MES over the one-dimensional (1D) current analysis can be comparable to those of 2D NMR over 1D NMR analysis.
Energy Technology Data Exchange (ETDEWEB)
Zhdanov, E. Yu., E-mail: zhdanov@isp.nsc.ru; Pogosov, A. G.; Budantsev, M. V.; Pokhabov, D. A.; Bakarov, A. K. [Siberian Branch of the Russian Academy of Sciences, Rzhanov Institute of Semiconductor Physics (Russian Federation)
2017-01-15
The magnetoresistance of suspended semiconductor nanostructures with a two-dimensional electron gas structured by periodic square antidot lattices is studied. It is shown that the ballistic regime of electron transport is retained after detaching the sample from the substrate. Direct comparative analysis of commensurability oscillations of magnetoresistance and their temperature dependences in samples before and after suspension is performed. It is found that the temperature dependences are almost identical for non-suspended and suspended samples, whereas significant differences are observed in the nonlinear regime, caused by direct current passage. Commensurability oscillations in the suspended samples are more stable with respect to exposure to direct current, which can be presumably explained by electron–electron interaction enhancement after detaching nanostructures from the high-permittivity substrate.
Zhou, Wenhan; Guo, Shiying; Liu, Xuhai; Cai, Bo; Song, Xiufeng; Zhu, Zhen; Zhang, Shengli
2018-01-01
We propose a family of hydrogenated- and halogenated-SbIV (SbIVX-2) materials that simultaneously have two-dimensional (2D) structures, high stability and appealing electronic properties. Based on first-principles total-energy and vibrational-spectra calculations, SbIVX-2 monolayers are found both thermally and dynamically stable. Varying IV and X elements can rationally tune the electronic properties of SbIVX-2 monolayers, effectively modulating the band gap from 0 to 3.42 eV. Regarding such superior stability and broad band-gap range, SbIVX-2 monolayers are expected to be synthesized in experiments and taken as promising candidates for low-dimensional electronic and optoelectronic devices, such as blue-to-ultraviolet light-emitting diodes (LED) and photodetectors.
Hernandez-Lamoneda, Ramón; Rosas, Victor Hugo Uc; Uruchurtu, Margarita I Bernal; Halberstadt, Nadine; Janda, Kenneth C
2008-01-10
All electron ab initio calculations for the interaction of H2O with Cl2 and Br2 are reported for the ground state and the lowest triplet and singlet Pi excited states as a function of both the X-X and O-X bond lengths (X = Cl or Br). For the ground state and lowest triplet state, the calculations are performed with the coupled cluster singles, doubles, and perturbative triple excitation level of correlation using an augmented triple-zeta basis set. For the 1Pi state the multireference average quadratic coupled cluster technique was employed. For several points on the potential, the calculations were repeated with the augmented quadruple-zeta basis set. The ground-state well depths were found to be 917 and 1,183 cm-1 for Cl2 and Br2, respectively, with the triple-zeta basis set, and they increased to 982 and 1,273 cm-1 for the quadruple-zeta basis set. At the geometry of the ground-state minimum, the lowest energy state corresponding to the unperturbed 1Pi states of the halogens increases in energy by 637 and 733 cm-1, respectively, relative to the ground-state dissociation limit of the H2O-X2 complex. Adding the attractive ground-state interaction energy to that of the repulsive excited state predicts a blue-shift, relative to that of the free halogen molecules, of approximately 1,600 cm-1 for H2O-Cl2 and approximately 2,000 cm-1 for H2O-Br2. These vertical blue-shifts for the dimers are greater than the shift of the band maximum upon solvation of either halogen in liquid water.
Terahertz Radiation Heterodyne Detector Using Two-Dimensional Electron Gas in a GaN Heterostructure
Karasik, Boris S.; Gill, John J.; Mehdi, Imran; Crawford, Timothy J.; Sergeev, Andrei V.; Mitin, Vladimir V.
2012-01-01
High-resolution submillimeter/terahertz spectroscopy is important for studying atmospheric and interstellar molecular gaseous species. It typically uses heterodyne receivers where an unknown (weak) signal is mixed with a strong signal from the local oscillator (LO) operating at a slightly different frequency. The non-linear mixer devices for this frequency range are unique and are not off-the-shelf commercial products. Three types of THz mixers are commonly used: Schottky diode, superconducting hot-electron bolometer (HEB), and superconductor-insulation-superconductor (SIS) junction. A HEB mixer based on the two-dimensional electron gas (2DEG) formed at the interface of two slightly dissimilar semiconductors was developed. This mixer can operate at temperatures between 100 and 300 K, and thus can be used with just passive radiative cooling available even on small spacecraft.
Two dimensional electron transport in disordered and ordered distributions of magnetic flux vortices
International Nuclear Information System (INIS)
Nielsen, M.; Hedegaard, P.
1994-04-01
We have considered the conductivity properties of a two dimensional electron gas (2DEG) in two different kinds of inhomogeneous magnetic fields, i.e. a disordered distribution of magnetic flux vortices, and a periodic array of magnetic flux vortices. The work falls in two parts. In the first part we show how the phase shifts for an electron scattering on an isolated vortex, can be calculated analytically, and related to the transport properties through the differential cross section. In the second part we present numerical results for the Hall conductivity of the 2DEG in a periodic array of flux vortices found by exact diagonalization. We find characteristic spikes in the Hall conductance, when it is plotted against the filling fraction. It is argued that the spikes can be interpreted in terms of ''topological charge'' piling up across local and global gaps in the energy spectrum. (au) (23 refs.)
Energy Technology Data Exchange (ETDEWEB)
Bizimana, Laurie A.; Brazard, Johanna; Carbery, William P.; Gellen, Tobias; Turner, Daniel B., E-mail: dturner@nyu.edu [Department of Chemistry, New York University, 100 Washington Square East, New York, New York 10003 (United States)
2015-10-28
Coherent multidimensional optical spectroscopy is an emerging technique for resolving structure and ultrafast dynamics of molecules, proteins, semiconductors, and other materials. A current challenge is the quality of kinetics that are examined as a function of waiting time. Inspired by noise-suppression methods of transient absorption, here we incorporate shot-by-shot acquisitions and balanced detection into coherent multidimensional optical spectroscopy. We demonstrate that implementing noise-suppression methods in two-dimensional electronic spectroscopy not only improves the quality of features in individual spectra but also increases the sensitivity to ultrafast time-dependent changes in the spectral features. Measurements on cresyl violet perchlorate are consistent with the vibronic pattern predicted by theoretical models of a highly displaced harmonic oscillator. The noise-suppression methods should benefit research into coherent electronic dynamics, and they can be adapted to multidimensional spectroscopies across the infrared and ultraviolet frequency ranges.
Bizimana, Laurie A; Brazard, Johanna; Carbery, William P; Gellen, Tobias; Turner, Daniel B
2015-10-28
Coherent multidimensional optical spectroscopy is an emerging technique for resolving structure and ultrafast dynamics of molecules, proteins, semiconductors, and other materials. A current challenge is the quality of kinetics that are examined as a function of waiting time. Inspired by noise-suppression methods of transient absorption, here we incorporate shot-by-shot acquisitions and balanced detection into coherent multidimensional optical spectroscopy. We demonstrate that implementing noise-suppression methods in two-dimensional electronic spectroscopy not only improves the quality of features in individual spectra but also increases the sensitivity to ultrafast time-dependent changes in the spectral features. Measurements on cresyl violet perchlorate are consistent with the vibronic pattern predicted by theoretical models of a highly displaced harmonic oscillator. The noise-suppression methods should benefit research into coherent electronic dynamics, and they can be adapted to multidimensional spectroscopies across the infrared and ultraviolet frequency ranges.
High-Current Gain Two-Dimensional MoS 2 -Base Hot-Electron Transistors
Torres, Carlos M.
2015-12-09
The vertical transport of nonequilibrium charge carriers through semiconductor heterostructures has led to milestones in electronics with the development of the hot-electron transistor. Recently, significant advances have been made with atomically sharp heterostructures implementing various two-dimensional materials. Although graphene-base hot-electron transistors show great promise for electronic switching at high frequencies, they are limited by their low current gain. Here we show that, by choosing MoS2 and HfO2 for the filter barrier interface and using a noncrystalline semiconductor such as ITO for the collector, we can achieve an unprecedentedly high-current gain (α ∼ 0.95) in our hot-electron transistors operating at room temperature. Furthermore, the current gain can be tuned over 2 orders of magnitude with the collector-base voltage albeit this feature currently presents a drawback in the transistor performance metrics such as poor output resistance and poor intrinsic voltage gain. We anticipate our transistors will pave the way toward the realization of novel flexible 2D material-based high-density, low-energy, and high-frequency hot-carrier electronic applications. © 2015 American Chemical Society.
Czech Academy of Sciences Publication Activity Database
Goncharuk, Natalya; Smrčka, Ludvík; Kučera, Jan
2004-01-01
Roč. 22, - (2004), s. 590-593 ISSN 1386-9477. [International Conference on Electronic Properties of Two-Dimensional Systems /15./. Nara, 14.07.2003-18.07.2003] R&D Projects: GA ČR GA202/01/0754 Institutional research plan: CEZ:AV0Z1010914 Keywords : single layer * double layer * two-dimensional electron system * cyclotron resonance Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 0.898, year: 2004
Energy Technology Data Exchange (ETDEWEB)
De Re, Eleonora; Schlau-Cohen, Gabriela S.; Leverenz, Ryan L.; Huxter, Vanessa M.; Oliver, Thomas A. A.; Mathies, Richard A.; Fleming, Graham R.
2014-05-22
Carotenoids play an essential role in photoprotection, interacting with other pigments to safely dissipate excess absorbed energy as heat. In cyanobacteria, the short time scale photoprotective mechanisms involve the photoactive orange carotenoid protein (OCP), which binds a single carbonyl carotenoid. Blue-green light induces the photoswitching of OCP from its ground state form (OCPO) to a metastable photoproduct (OCPR). OCPR can bind to the phycobilisome antenna and induce fluorescence quenching. The photoswitching is accompanied by structural and functional changes at the level of the protein and of the bound carotenoid. In this study, we use broadband two-dimensional electronic spectroscopy to look at the differences in excited state dynamics of the carotenoid in the two forms of OCP. Our results provide insight into the origin of the pronounced vibrational lineshape and oscillatory dynamics observed in linear absorption and 2D electronic spectroscopy of OCPO and the large inhomogeneous broadening in OCPR, with consequences for the chemical function of the two forms.
Gerhardts, Rolf R.
2015-11-01
Model calculations for commensurability oscillations of the low-field magnetoresistance of two-dimensional electron systems (2DES) in lateral superlattices, consisting of unit cells with an internal structure, are compared with recent experiments. The relevant harmonics of the effective modulation potential depend not only on the geometrical structure of the modulated unit cell, but also strongly on the nature of the modulation. While higher harmonics of an electrostatically generated surface modulation are exponentially damped at the position of the 2DES about 90 nm below the surface, no such damping appears for strain-induced modulation generated, e.g., by the deposition of stripes of calixarene resist on the surface before cooling down the sample.
Choi, Hyunwoo; Kim, Tae Geun; Shin, Changhwan
2017-06-01
A topological insulator (TI) is a new kind of material that exhibits unique electronic properties owing to its topological surface state (TSS). Previous studies focused on the transport properties of the TSS, since it can be used as the active channel layer in metal-oxide-semiconductor field-effect transistors (MOSFETs). However, a TI with a negative quantum capacitance (QC) effect can be used in the gate stack of MOSFETs, thereby facilitating the creation of ultra-low power electronics. Therefore, it is important to study the physics behind the QC in TIs in the absence of any external magnetic field, at room temperature. We fabricated a simple capacitor structure using a TI (TI-capacitor: Au-TI-SiO2-Si), which shows clear evidence of QC at room temperature. In the capacitance-voltage (C-V) measurement, the total capacitance of the TI-capacitor increases in the accumulation regime, since QC is the dominant capacitive component in the series capacitor model (i.e., CT-1 = CQ-1 + CSiO2-1). Based on the QC model of the two-dimensional electron systems, we quantitatively calculated the QC, and observed that the simulated C-V curve theoretically supports the conclusion that the QC of the TI-capacitor is originated from electron-electron interaction in the two-dimensional surface state of the TI.
Photon drag investigations of current relaxation processes in a two-dimensional electron gas
Graf, S; Kohler, K U; Bachtold, W
2000-01-01
We have investigated the photon drag current that is excited by an infrared laser beam in the plane of the two-dimensional electron gas of GaAs/Al/sub 0.35/Ga/sub 0.65/As multiple-quantum-well systems. An analysis of the spectral response, measured with the picosecond infrared pulses of the wavelength-tunable free electron laser source FELIX, is presented for different doping schemes and examined as a function of temperature and intensity. The influence of the subband- selective scattering by a delta doping is explored, which demonstrates that the photon drag spectral response allows the determination of the momentum relaxation time ratio, R= tau /sub 1// tau /sub 2/, of the electrons in the ground and excited subbands. The relaxation time ratio is found to be surprisingly constant over a large temperature range. The variation of the ratio with intensity can be attributed to heating of the electron gas, whose temperature exceeds 1000 K at saturation intensity. (41 refs).
A new series of two-dimensional silicon crystals with versatile electronic properties
Chae, Kisung; Kim, Duck Young; Son, Young-Woo
2018-04-01
Silicon (Si) is one of the most extensively studied materials owing to its significance to semiconductor science and technology. While efforts to find a new three-dimensional (3D) Si crystal with unusual properties have made some progress, its two-dimensional (2D) phases have not yet been explored as much. Here, based on a newly developed systematic ab initio materials searching strategy, we report a series of novel 2D Si crystals with unprecedented structural and electronic properties. The new structures exhibit perfectly planar outermost surface layers of a distorted hexagonal network with their thicknesses varying with the atomic arrangement inside. Dramatic changes in electronic properties ranging from semimetal to semiconducting with indirect energy gaps and even to one with direct energy gaps are realized by varying thickness as well as by surface oxidation. Our predicted 2D Si crystals with flat surfaces and tunable electronic properties will shed light on the development of silicon-based 2D electronics technology.
Energy Technology Data Exchange (ETDEWEB)
Choi, Hyunwoo, E-mail: chw0089@gmail.com [Department of Electrical and Computer Engineering, University of Seoul, Seoul 02504 (Korea, Republic of); Kim, Tae Geun, E-mail: tgkim1@korea.ac.kr [School of Electrical Engineering, Korea University, Seoul 02841 (Korea, Republic of); Shin, Changhwan, E-mail: cshin@uos.ac.kr [Department of Electrical and Computer Engineering, University of Seoul, Seoul 02504 (Korea, Republic of)
2017-06-15
Highlights: • The quantum capacitance in topological insulator (TI) at room temperature is directly revealed. • The physical origin of quantum capacitance, the two dimensional surface state of TI, is experimentally validated. • Theoretically calculated results of ideal quantum capacitance can well predict the experimental data. - Abstract: A topological insulator (TI) is a new kind of material that exhibits unique electronic properties owing to its topological surface state (TSS). Previous studies focused on the transport properties of the TSS, since it can be used as the active channel layer in metal-oxide-semiconductor field-effect transistors (MOSFETs). However, a TI with a negative quantum capacitance (QC) effect can be used in the gate stack of MOSFETs, thereby facilitating the creation of ultra-low power electronics. Therefore, it is important to study the physics behind the QC in TIs in the absence of any external magnetic field, at room temperature. We fabricated a simple capacitor structure using a TI (TI-capacitor: Au-TI-SiO{sub 2}-Si), which shows clear evidence of QC at room temperature. In the capacitance-voltage (C-V) measurement, the total capacitance of the TI-capacitor increases in the accumulation regime, since QC is the dominant capacitive component in the series capacitor model (i.e., C{sub T}{sup −1} = C{sub Q}{sup −1} + C{sub SiO2}{sup −1}). Based on the QC model of the two-dimensional electron systems, we quantitatively calculated the QC, and observed that the simulated C-V curve theoretically supports the conclusion that the QC of the TI-capacitor is originated from electron–electron interaction in the two-dimensional surface state of the TI.
DEFF Research Database (Denmark)
Dahl, Jens Peder; Schleich, W. P.
2009-01-01
For a closed quantum system the state operator must be a function of the Hamiltonian. When the state is degenerate, additional constants of the motion enter the play. But although it is the Weyl transform of the state operator, the Wigner function is not necessarily a function of the Weyl...... transforms of the constants of the motion. We derive conditions for which this is actually the case. The Wigner functions of the energy eigenstates of a two-dimensional isotropic harmonic oscillator serve as an important illustration....
Two-Dimensional Electronic-Vibrational Spectroscopy of Chlorophyll a and b
Energy Technology Data Exchange (ETDEWEB)
Lewis, Nicholas H. C. [Univ. of California, Berkeley, CA (United States). Dept. of Chemistry; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Molecular Biophysics and Integrated Bioimaging Div.; Kavli Energy Nanoscience Institute at Berkeley, CA (United States); Fleming, Graham R. [Univ. of California, Berkeley, CA (United States). Dept. of Chemistry; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Molecular Biophysics and Integrated Bioimaging Div.; Kavli Energy Nanoscience Institute at Berkeley, CA (United States)
2016-03-03
Presented are two-dimensional electronic-vibrational (2DEV) spectra of isolated chlorophyll a and b in deuterated ethanol. We excite the Q-band electronic transitions and measure the effects on the carbonyl and C=C double-bond stretch region of the infrared spectrum. With the aid of density functional theory calculations, we provide assignments for the major features of the spectrum. We show how the 2DEV spectra can be used to readily distinguish different solvation states of the chlorophyll, with features corresponding to the minority pentacoordinate magnesium (Mg) species being resolved along each dimension of the 2DEV spectra from the dominant hexacoordinate Mg species. These assignments represent a crucial first step toward the application of 2DEV spectroscopy to chlorophyll-containing pigment-protein complexes.
Khodel, V A
2001-01-01
Spectral functions of strongly correlated two-dimensional electron systems in solids are studied on the assumption that these systems undergo as phase transition, called fermion condensation, whose characteristic feature is flattening of the electron spectrum epsilon (p). Unlike the previous models in the present study, the decay of single-particle states is properly taken into account. Results of calculations are shown to be in qualitative agreement with ARPES data. The universal behavior of the ration Im EPSILON(p, epsilon, T)/T as a function of x = epsilon/T are found to be reproduced reasonably well. However, in the present model this behavior is destroyed in vicinities of the van Hove points where the fermion condensate resides
Yang, Ji-Hui; Zhang, Yueyu; Yin, Wan-Jian; Gong, X G; Yakobson, Boris I; Wei, Su-Huai
2016-02-10
Two-dimensional (2D) semiconductors can be very useful for novel electronic and optoelectronic applications because of their good material properties. However, all current 2D materials have shortcomings that limit their performance. As a result, new 2D materials are highly desirable. Using atomic transmutation and differential evolution global optimization methods, we identified two group IV-VI 2D materials, Pma2-SiS and silicene sulfide. Pma2-SiS is found to be both chemically, energetically, and thermally stable. Most importantly, Pma2-SiS has shown good electronic and optoelectronic properties, including direct bandgaps suitable for solar cells, good mobility for nanoelectronics, good flexibility of property tuning by layer control and applied strain, and good air stability as well. Therefore, Pma2-SiS is expected to be a promising 2D material in the field of 2D electronics and optoelectronics. The designing principles demonstrated in identifying these two tantalizing examples have great potential to accelerate the finding of new functional 2D materials.
High-mobility two-dimensional electron gases at oxide interfaces: Origin and opportunities
International Nuclear Information System (INIS)
Chen Yun-Zhong; Pryds Nini; Linderoth Søren; Sun Ji-Rong; Shen Bao-Gen
2013-01-01
Our recent experimental work on metallic and insulating interfaces controlled by interfacial redox reactions in SrTiO 3 -based heterostructures is reviewed along with a more general background of two-dimensional electron gas (2DEG) at oxide interfaces. Due to the presence of oxygen vacancies at the SrTiO 3 surface, metallic conduction can be created at room temperature in perovskite-type interfaces when the overlayer oxide ABO 3 has Al, Ti, Zr, or Hf elements at the B sites. Furthermore, relying on interface-stabilized oxygen vacancies, we have created a new type of 2DEG at the heterointerface between SrTiO 3 and a spinel γ-Al 2 O 3 epitaxial film with compatible oxygen ion sublattices. This 2DEG exhibits an electron mobility exceeding 100000 cm 2 V −1 s −1 , more than one order of magnitude higher than those of hitherto investigated perovskite-type interfaces. Our findings pave the way for the design of high-mobility all-oxide electronic devices and open a route toward the studies of mesoscopic physics with complex oxides. (topical review - magnetism, magnetic materials, and interdisciplinary research)
Dorozhkin, S. Â. I.; Kapustin, A. Â. A.; Dmitriev, I. Â. A.; Umansky, V.; von Klitzing, K.; Smet, J. H.
2017-10-01
We have studied the absorption of monochromatic microwave radiation in high-quality two-dimensional electron systems for the frequency span from 10 to 380 GHz using a bolometric method. For frequencies above 100 GHz the absorption exhibits an anomalous magnetic field dependence. Minima form at harmonics of the cyclotron resonance frequency. The results contrast previously reported data for other frequency ranges. Quasiclassical memory effects originating from the non-Markovian dynamics of electrons in a disorder potential containing short-range scatterers on top of a smooth potential background favorably account for the observed behavior.
Electron cryomicroscopy of two-dimensional crystals of the H+-ATPase from chloroplasts
Böttcher, Bettina; Gräber, Peter; Boekema, Egbert J.; Lücken, Uwe
1995-01-01
The H+-ATPase from spinach chloroplasts was isolated and purified. Two-dimensional crystals were obtained from the protein/lipid/detergent micelles by treatment with phospholipase and simultaneous removal of detergent and fatty acids by Biobeads. The resulting two-dimensionally ordered arrays were
Yang, Fan; Abe, Kazuhiro; Tani, Kazutoshi; Fujiyoshi, Yoshinori
2013-01-01
Received 7 June 2013; accepted 21 June 2013Abstract Electron crystallography is an important method for determining the structure of membrane proteins. In this paper, we show the impact of a carbon sandwich preparation on the preservation of crystalline sample quality, using characteristic examples of two-dimensional (2D) crystals from gastric H+,K+-ATPase and their analyzed images. Compared with the ordinary single carbon support film preparation, the carbon sandwich preparation dramatically enhanced the resolution of images from flat sheet 2D crystals. As water evaporation is restricted in the carbon-sandwiched specimen, the improvement could be due to the strong protective effect of the retained water against drastic changes in the environment surrounding the specimen, such as dehydration and increased salt concentrations. This protective effect by the carbon sandwich technique helped to maintain the inherent and therefore best crystal conditions for analysis. Together with its strong compensation effect for the image shift due to beam-induced specimen charging, the carbon sandwich technique is a powerful method for preserving crystals of membrane proteins with larger hydrophilic regions, such as H+,K+-ATPase, and thus constitutes an efficient and high-quality method for collecting data for the structural analysis of these types of membrane proteins by electron crystallography. PMID:23883606
Luo, Chen; Wang, Chaolun; Wu, Xing; Zhang, Jian; Chu, Junhao
2017-09-01
Two-dimensional (2D) ultra-thin materials beyond graphene with rich physical properties and unique layered structures are promising for applications in electronics, chemistry, energy, and bioscience, etc. The interaction mechanisms among the structures, chemical compositions and physical properties of 2D layered materials are critical for fundamental nanosciences and the practical fabrication of next-generation nanodevices. Transmission electron microscopy (TEM), with its high spatial resolution and versatile external fields, is undoubtedly a powerful tool for the static characterization and dynamic manipulation of nanomaterials and nanodevices at the atomic scale. The rapid development of thin-film and precision microelectromechanical systems (MEMS) techniques allows 2D layered materials and nanodevices to be probed and engineered inside TEM under external stimuli such as thermal, electrical, mechanical, liquid/gas environmental, optical, and magnetic fields at the nanoscale. Such advanced technologies leverage the traditional static TEM characterization into an in situ and interactive manipulation of 2D layered materials without sacrificing the resolution or the high vacuum chamber environment, facilitating exploration of the intrinsic structure-property relationship of 2D layered materials. In this Review, the dynamic properties tailored and observed by the most advanced and unprecedented in situ TEM technology are introduced. The challenges in spatial, time and energy resolution are discussed also. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Yang, Fan; Abe, Kazuhiro; Tani, Kazutoshi; Fujiyoshi, Yoshinori
2013-12-01
Electron crystallography is an important method for determining the structure of membrane proteins. In this paper, we show the impact of a carbon sandwich preparation on the preservation of crystalline sample quality, using characteristic examples of two-dimensional (2D) crystals from gastric H(+),K(+)-ATPase and their analyzed images. Compared with the ordinary single carbon support film preparation, the carbon sandwich preparation dramatically enhanced the resolution of images from flat sheet 2D crystals. As water evaporation is restricted in the carbon-sandwiched specimen, the improvement could be due to the strong protective effect of the retained water against drastic changes in the environment surrounding the specimen, such as dehydration and increased salt concentrations. This protective effect by the carbon sandwich technique helped to maintain the inherent and therefore best crystal conditions for analysis. Together with its strong compensation effect for the image shift due to beam-induced specimen charging, the carbon sandwich technique is a powerful method for preserving crystals of membrane proteins with larger hydrophilic regions, such as H(+),K(+)-ATPase, and thus constitutes an efficient and high-quality method for collecting data for the structural analysis of these types of membrane proteins by electron crystallography.
A compact system for two-dimensional readout of Gas Electron Multiplier detectors
International Nuclear Information System (INIS)
Mindur, B; Dąbrowski, W; Fiutowski, T; Wiącek, P; Zielińska, A
2013-01-01
There is a growing interest in the use of Gas Electron Multiplier (GEM) and other micro-pattern gas detectors (MPGD) for two-dimensional (2-D) position sensitive measurements of photons or charged particles. A Gas Electron Multiplier Readout Chip (GEMROC) is an Application Specific Integrated Circuit (ASIC) dedicated for 2-D strip readout of GEM detectors. The ASICs deliver the amplitudes and time coordinates of the signals recorded on two sets of orthogonal strips. Timing information is used for finding coincidences of signals on two spatial coordinates while amplitude information is used to find the center of gravity for the cluster of signals belonging to the same detection event. In this paper we present a Field Programmable Gate Array (FPGA) based compact readout system dedicated for these ASICs. The readout system consists of two synchronized FPGA-ADC boards connected to four front-end boards, each one equipped with two GEMROCs. Both FPGAs are connected to a DAQ PC using separate Gigabit Ethernet links. The DAQ PC is equipped with a dedicated C++ based software, which is responsible for configuration of the FPGAs and ASICs settings, storing all the incoming data as well as for on-line/off-line data processing and visualization. The performance of the system is illustrated by test bench measurements.
Shang, Jingzhi; Cong, Chunxiao; Shen, Xiaonan; Yang, Weihuang; Zou, Chenji; Peimyoo, Namphung; Cao, Bingchen; Eginligil, Mustafa; Lin, Wei; Huang, Wei; Yu, Ting
2017-12-01
Owing to unique electronic, excitonic, and valleytronic properties, atomically thin transition metal dichalcogenides are becoming a promising two-dimensional (2D) semiconductor system for diverse electronic and optoelectronic applications. In an ideal 2D semiconductor, efficient carrier transport is very difficult because of lacking free charge carriers. Doping is necessary for electrically driven device applications based on such 2D semiconductors, which requires investigation of electronic structure changes induced by dopants. Therefore probing correlations between localized electronic states and doping is important. Here, we address the electronic nature of broad bound exciton bands and their origins in exfoliated monolayer (1L) W S2 and Mo S2 through monitoring low-temperature photoluminescence and manipulating electrostatic doping. The dominant bound excitons in 1L W S2 vary from donor to acceptor bound excitons with the switching from n - to p -type doping. In 1L Mo S2 , two localized emission bands appear which are assigned to neutral and ionized donor bound excitons, respectively. The deep donor and acceptor states play critical roles in the observed bound exciton bands, indicating the presence of strongly localized excitons in such 2D semiconductors.
Doppler Velocimetry of Current Driven Spin Helices in a Two-Dimensional Electron Gas
Energy Technology Data Exchange (ETDEWEB)
Yang, Luyi [Univ. of California, Berkeley, CA (United States)
2013-05-17
Spins in semiconductors provide a pathway towards the development of spin-based electronics. The appeal of spin logic devices lies in the fact that the spin current is even under time reversal symmetry, yielding non-dissipative coupling to the electric field. To exploit the energy-saving potential of spin current it is essential to be able to control it. While recent demonstrations of electrical-gate control in spin-transistor configurations show great promise, operation at room temperature remains elusive. Further progress requires a deeper understanding of the propagation of spin polarization, particularly in the high mobility semiconductors used for devices. This dissertation presents the demonstration and application of a powerful new optical technique, Doppler spin velocimetry, for probing the motion of spin polarization at the level of 1 nm on a picosecond time scale. We discuss experiments in which this technique is used to measure the motion of spin helices in high mobility n-GaAs quantum wells as a function of temperature, in-plane electric field, and photoinduced spin polarization amplitude. We find that the spin helix velocity changes sign as a function of wave vector and is zero at the wave vector that yields the largest spin lifetime. This observation is quite striking, but can be explained by the random walk model that we have developed. We discover that coherent spin precession within a propagating spin density wave is lost at temperatures near 150 K. This finding is critical to understanding why room temperature operation of devices based on electrical gate control of spin current has so far remained elusive. We report that, at all temperatures, electron spin polarization co-propagates with the high-mobility electron sea, even when this requires an unusual form of separation of spin density from photoinjected electron density. Furthermore, although the spin packet co-propagates with the two-dimensional electron gas, spin diffusion is strongly
Numerical evidence for two types of localized states in a two-dimensional disordered lattice
International Nuclear Information System (INIS)
Tit, N.; Kumar, N.
1992-06-01
We report results of our numerical calculations, based on the equation of motion method, of dc-electrical conductivity and of density of states up to 40x40 two-dimensional square lattices modelling a right-binding Hamiltonian for a binary (AB) compound, disordered by randomly distributed B vacancies up to 10%. Our results indicate strongly localized states away from band centers separated from the relatively weakly localized states toward midband. This is in qualitative agreement with the idea of a ''mobility edge'' separating exponentially localized states from the power-law localized states as suggested by the two-parameter scaling theory of Kaevh in two dimensions. (author). 7 refs, 4 figs
Steady state bifurcations for phase field crystal equations with underlying two dimensional kernel
Directory of Open Access Journals (Sweden)
Appolinaire Abourou Ella
2015-10-01
Full Text Available This paper is concerned with the study of some properties of stationary solutions to phase field crystal equations bifurcating from a trivial solution. It is assumed that at this trivial solution, the kernel of the underlying linearized operator has dimension two. By means of the multiparameter method, we give a second order approximation of these bifurcating solutions and analyse their stability properties. The main result states that the stability of these solutions can be described by the variation of a certain angle in a two dimensional parameter space. The behaviour of the parameter curve is also investigated.
Crossover scaling in the two-dimensional three-state Potts model
Directory of Open Access Journals (Sweden)
T. Nagai
2013-06-01
Full Text Available We apply simulated tempering and magnetizing (STM Monte Carlo simulations to the two-dimensional three-state Potts model in an external magnetic field in order to investigate the crossover scaling behaviour in the temperature-field plane at the Potts critical point and towards the Ising universality class for negative magnetic fields. Our data set has been generated by STM simulations of several square lattices with sizes up to 160x160 spins, supplemented by conventional canonical simulations of larger lattices at selected simulation points. We present careful scaling and finite-size scaling analyses of the crossover behaviour with respect to temperature, magnetic field and lattice size.
Formulation and validation of a two-dimensional steady-state model of desiccant wheels
DEFF Research Database (Denmark)
Bellemo, Lorenzo; Elmegaard, Brian; Kærn, Martin R.
2015-01-01
systems. A steady-state two-dimensional model is formulated and implemented, aiming to obtain good accuracy and short computational times with the purpose of inclusion in complete system models. The model includes mass and energy balances and correlations for heat and mass transfer based on empirical...... relations from the scientific literature. Convective heat and mass transfer coefficients are computed locally accounting for the entrance length effects. Mass diffusion inside the desiccant material is neglected. Comparison with experimental data from the literature shows that the model reproduces...
Chen, Yunzhong; Trier, F.; Wijnands, Tom; Green, R.J.; Gauquelin, N.; Egoavil, R.; Christensen, D.V.; Koster, Gertjan; Huijben, Mark; Bovet, N.; Macke, S.; He, F.; Sutarto, R.; Andersen, N.H.; Sulpizio, J.A.; Honig, M.; Prawiroatmodjo, G.E.D.K.; Jespersen, T.S.; Linderoth, S.; Ilani, S.; Verbeeck, J.; van Tendeloo, G.; Rijnders, Augustinus J.H.M.; Sawatzky, G.A.; Pryds, N.
2015-01-01
Two-dimensional electron gases (2DEGs) formed at the interface of insulating complex oxides promise the development of all-oxide electronic devices. These 2DEGs involve many-body interactions that give rise to a variety of physical phenomena such as superconductivity, magnetism, tunable
Tunneling conductance of a two-dimensional electron gas with Dresselhaus spin-orbit coupling
International Nuclear Information System (INIS)
Srisongmuang, B.; Ka-oey, A.
2012-01-01
We theoretically studied the spin-dependent charge transport in a two-dimensional electron gas with Dresselhaus spin-orbit coupling (DSOC) and metal junctions. It is shown that the DSOC energy can be directly measured from the tunneling conductance spectrum. We found that spin polarization of the conductance in the propagation direction can be obtained by injecting from the DSOC system. We also considered the effect of the interfacial scattering barrier (both spin-flip and non-spin-flip scattering) on the overall conductance and the spin polarization of the conductance. It is found that the increase of spin-flip scattering can enhance the conductance under certain conditions. Moreover, both types of scattering can increase the spin polarization below the branches crossing of the energy band. - Highlights: → DSOC energy can be directly measured from tunneling conductance spectrum. → Spin polarization of conductance in the propagation direction can be obtained by injecting from DSOC system. → Both types of scattering can increase spin polarization.
Electrical detection of spin transport in Si two-dimensional electron gas systems
Chang, Li-Te; Fischer, Inga Anita; Tang, Jianshi; Wang, Chiu-Yen; Yu, Guoqiang; Fan, Yabin; Murata, Koichi; Nie, Tianxiao; Oehme, Michael; Schulze, Jörg; Wang, Kang L.
2016-09-01
Spin transport in a semiconductor-based two-dimensional electron gas (2DEG) system has been attractive in spintronics for more than ten years. The inherent advantages of high-mobility channel and enhanced spin-orbital interaction promise a long spin diffusion length and efficient spin manipulation, which are essential for the application of spintronics devices. However, the difficulty of making high-quality ferromagnetic (FM) contacts to the buried 2DEG channel in the heterostructure systems limits the potential developments in functional devices. In this paper, we experimentally demonstrate electrical detection of spin transport in a high-mobility 2DEG system using FM Mn-germanosilicide (Mn(Si0.7Ge0.3)x) end contacts, which is the first report of spin injection and detection in a 2DEG confined in a Si/SiGe modulation doped quantum well structure (MODQW). The extracted spin diffusion length and lifetime are l sf = 4.5 μm and {τ }{{s}}=16 {{ns}} at 1.9 K respectively. Our results provide a promising approach for spin injection into 2DEG system in the Si-based MODQW, which may lead to innovative spintronic applications such as spin-based transistor, logic, and memory devices.
Bottom-Up Two-Dimensional Electron-Capture Dissociation Mass Spectrometry of Calmodulin
Floris, Federico; van Agthoven, Maria A.; Chiron, Lionel; Wootton, Christopher A.; Lam, Pui Yiu Yuko; Barrow, Mark P.; Delsuc, Marc-André; O'Connor, Peter B.
2018-01-01
Two-dimensional mass spectrometry (2D MS) is a tandem mass spectrometry technique that allows data-independent fragmentation of all precursors in a mixture without previous isolation, through modulation of the ion cyclotron frequency in the ICR-cell prior to fragmentation. Its power as an analytical technique has been proven particularly for proteomics. Recently, a comparison study between 1D and 2D MS has been performed using infrared multiphoton dissociation (IRMPD) on calmodulin (CaM), highlighting the capabilities of the technique in both top-down (TDP) and bottom-up proteomics (BUP). The goal of this work is to expand this study on CaM using electron-capture dissociation (ECD) 2D MS as a single complementary BUP experiment in order to enhance the cleavage coverage of the protein under analysis. By adding the results of the BUP 2D ECD MS to the 2D IRMPD MS analysis of CaM, the total cleavage coverage increased from 40% to 68%. [Figure not available: see fulltext.
Mesoscopic Field-Effect-Induced Devices in Depleted Two-Dimensional Electron Systems
Bachsoliani, N.; Platonov, S.; Wieck, A. D.; Ludwig, S.
2017-12-01
Nanoelectronic devices embedded in the two-dimensional electron system (2DES) of a GaAs /(Al ,Ga )As heterostructure enable a large variety of applications ranging from fundamental research to high-speed transistors. Electrical circuits are thereby commonly defined by creating barriers for carriers by the selective depletion of a preexisting 2DES. We explore an alternative approach: we deplete the 2DES globally by applying a negative voltage to a global top gate and screen the electric field of the top gate only locally using nanoscale gates placed on the wafer surface between the plane of the 2DES and the top gate. Free carriers are located beneath the screen gates, and their properties can be controlled by means of geometry and applied voltages. This method promises considerable advantages for the definition of complex circuits by the electric-field effect, as it allows us to reduce the number of gates and simplify gate geometries. Examples are carrier systems with ring topology or large arrays of quantum dots. We present a first exploration of this method pursuing field effect, Hall effect, and Aharonov-Bohm measurements to study electrostatic, dynamic, and coherent properties.
Kozlov, I. V.; Kolesnichenko, Yu. A.
2017-07-01
We present a theoretical study of the spatial distribution of the local density of states (LDOS) and the local magnetization density (LMD) in the vicinity of a magnetic point-defect in a degenerate two-dimensional electron gas with a mixed Rashba-Dresselhaus spin-orbit coupling interaction (SOI). The dependence of the Friedel oscillations, which arise under these conditions, on the ratio of the SOI constants is investigated. We obtain asymptotic expressions for the oscillatory parts of the LDOS and the LMD, that are accurate for large distances from the defect. It is shown, that the Friedel oscillations are significantly anisotropic and contain several harmonics for certain ratios of the SOI constants. Period of the oscillations for directions along the symmetry axes of the Fermi contours are determined. Finally, we introduce a method for determining the values of the two SOI constants by measuring the period of the Friedel oscillations of the LDOS and the LMD for different harmonics.
Energy Technology Data Exchange (ETDEWEB)
Sang, Ling; Yang, Xuelin, E-mail: xlyang@pku.edu.cn; Cheng, Jianpeng; Guo, Lei; Hu, Anqi; Xiang, Yong; Yu, Tongjun; Xu, Fujun; Tang, Ning [State Key Laboratory of Artificial Microstructure and Mesoscopic Physics, School of Physics, Peking University, Beijing 100871 (China); Jia, Lifang; He, Zhi [Engineering Research Center for Semiconductor Integrated Technology, Institute of Semiconductors, Chinese Academy of Sciences, P. O. Box 912, Beijing 100083 (China); Wang, Maojun [Institute of Microelectronics, Peking University, Beijing 100871 (China); Wang, Xinqiang; Shen, Bo, E-mail: bshen@pku.edu.cn [State Key Laboratory of Artificial Microstructure and Mesoscopic Physics, School of Physics, Peking University, Beijing 100871 (China); Collaborative Innovation Center of Quantum Matter, Beijing 100871 (China); Ge, Weikun [Department of Physics, Tsinghua University, Beijing 100084 (China)
2015-08-03
High-temperature transport properties in high-mobility lattice-matched InAlN/GaN heterostructures have been investigated. An interesting hysteresis phenomenon of the two dimensional electron gas (2DEG) density is observed in the temperature-dependent Hall measurements. After high-temperature thermal cycles treatment, the reduction of the 2DEG density is observed, which is more serious in thinner InAlN barrier samples. This reduction can then be recovered by light illumination. We attribute these behaviors to the shallow trap states with energy level above the Fermi level in the GaN buffer layer. The electrons in the 2DEG are thermal-excited when temperature is increased and then trapped by these shallow trap states in the buffer layer, resulting in the reduction and hysteresis phenomenon of their density. Three trap states are observed in the GaN buffer layer and C{sub Ga} may be one of the candidates responsible for the observed behaviors. Our results provide an alternative approach to assess the quality of InAlN/GaN heterostructures for applications in high-temperature electronic devices.
Pakmehr, Mehdi; McCombe, B. D.; Bruene, C.; Buhmann, H.; Molenkamp, L. W.
2015-10-01
HgTe quantum wells (QWs) have shown a number of interesting phenomena, recently the first two-dimensional topological insulating state. We have studied thermoelectric photovoltages of two-dimensional electrons in a 6.1 nm wide HgTe QW induced by cyclotron resonance absorption ( B = 2 to 5 T) of a THz laser beam. We have estimated thermopower coefficients by detailed analysis of the photovoltage signals developed across various contacts of a large Hall bar structure at a bath temperature of 1.6 K. The photovoltage signals are washed out at bath temperature of 18 K.
Energy Technology Data Exchange (ETDEWEB)
Ogilvie, Jennifer P. [Univ. of Michigan, Ann Arbor, MI (United States). Dept. of Physics
2016-11-22
Photosystem II (PSII) is the only known natural enzyme that uses solar energy to split water, making the elucidation of its design principles critical for our fundamental understanding of photosynthesis and for our ability to mimic PSII’s remarkable properties. This report discusses progress towards addressing key open questions about the PSII RC. It describes new spectroscopic methods that were developed to answer these questions, and summarizes the outcomes of applying these methods to study the PSII RC. Using 2D electronic spectroscopy and 2D electronic Stark spectroscopy, models for the PSII RC were tested and refined. Work is ongoing to use the collected data to elucidate the charge separation mechanism in the PSII RC. Coherent dynamics were also observed in the PSII RC for the first time. Through extensive characterization and modeling we have assigned these coherences as vibronic in nature, and believe that they reflect resonances between key vibrational pigment modes and electronic energy gaps that may facilitate charge separation. Work is ongoing to definitively test the functional relevance of electronic-vibrational resonances.
International Nuclear Information System (INIS)
Gallego, S; Munoz, M C; Huttel, Y; Avila, J; Asensio, M C
2003-01-01
The c(2 x 2)MnCu surface alloy on Cu(100) can be considered as a purely two-dimensional magnetic system where the Mn atoms exhibit a large corrugation closely related to their high spin moment. In this paper we investigate the influence of the atomic environment on the electronic and magnetic properties of the two-dimensional alloyed layer, extending our study to the less known multilayered system made of MnCu two-dimensional alloy layers embedded in a Cu crystal. The analysis is based on angle-resolved photoelectron spectroscopy measurements and calculations using the Green function matching method, which allows us to treat exactly the projection of the three-dimensional lattice on the c(2 x 2) plane. A complete study of the valence band is performed along the two-dimensional Brillouin zone in a wide energy range. We show that the presence of Mn results in an important redistribution of the spin-polarized electronic states of the neighbouring Cu atoms. This redistribution is not accompanied by a net charge transfer between different atoms, and also the spin moment of Cu remains small. Most of the new features induced by Mn in the surface alloy are also present in the multilayered system, evidencing that they are specific to the two-dimensional alloyed layer and not surface effects
Strain-modulated electronic and thermal transport properties of two-dimensional O-silica
Han, Yang; Qin, Guangzhao; Jungemann, Christoph; Hu, Ming
2016-07-01
Silica is one of the most abundant materials in the Earth’s crust and is a remarkably versatile and important engineering material in various modern science and technology. Recently, freestanding and well-ordered two-dimensional (2D) silica monolayers with octahedral (O-silica) building blocks were found to be theoretically stable by (Wang G et al 2015 J. Phys. Chem. C 119 15654-60). In this paper, by performing first-principles calculations, we systematically investigated the electronic and thermal transport properties of 2D O-silica and also studied how these properties can be tuned by simple mechanical stretching. Unstrained 2D O-silica is an insulator with an indirect band gap of 6.536 eV. The band gap decreases considerably with bilateral strain up to 29%, at which point a semiconductor-metal transition occurs. More importantly, the in-plane thermal conductivity of freestanding 2D O-silica is found to be unusually high, which is around 40 to 50 times higher than that of bulk α-quartz and more than two orders of magnitude higher than that of amorphous silica. The thermal conductivity of O-silica decreases by almost two orders of magnitude when the bilateral stretching strain reaches 10%. By analyzing the mode-dependent phonon properties and phonon-scattering channel, the phonon lifetime is found to be the dominant factor that leads to the dramatic decrease of the lattice thermal conductivity under strain. The very sensitive response of both band gap and phonon transport properties to the external mechanical strain will enable 2D O-silica to easily adapt to the different environment of realistic applications. Our study is expected to stimulate experimental exploration of further physical and chemical properties of 2D silica systems, and offers perspectives on modulating the electronic and thermal properties of related low-dimensional structures for applications such as thermoelectric, photovoltaic, and optoelectronic devices.
Spokoyny, Boris M.
Ultrafast spectroscopy offers an unprecedented view on the dynamic nature of chemical reactions. From charge transfer in semiconductors to folding and isomerization of proteins, these all important processes can now be monitored and in some instances even controlled on real, physical timescales. One of the biggest challenges of ultrafast science is the incredible energetic complexity of most systems. It is not uncommon to encounter macromolecules or materials with absorption spectra spanning significant portions of the visible spectrum. Monitoring a multitude of electronic and vibrational transitions, all dynamically interacting with each other on femtosecond timescales poses a truly daunting experimental task. The first part of this thesis deals with the development of a novel Two-Dimensional Electronic Spectroscopy (2DES) and its associated, advanced detection methodologies. Owing to its ultra-broadband implementation, this technique enables us to monitor femtosecond chemical dynamics that span the energetic landscape of the entire visible spectrum. In order to demonstrate the utility of our method, we apply it to two laser dye molecules, IR-144 and Cresyl Violet. Variation of photophysical properties on a microscopic scale in either man-made or naturally occurring systems can have profound implications on how we understand their macroscopic properties. Recently, inorganic hybrid perovskites have been tapped as the next generation solar energy harvesting materials. Their remarkable properties include low exciton binding energy, low exciton recombination rates and long carrier diffusion lengths. Nevertheless, considerable variability in device properties made with nearly identical preparation methods has puzzled the community. In the second part of this thesis we use non-linear pump probe microscopy to study the heterogeneous nature of femtosecond carrier dynamics in thin film perovskites. We show that the local morphology of the perovskite thin films has a
Entanglement properties of the two-dimensional SU(3) Affleck-Kennedy-Lieb-Tasaki state
Gauthé, Olivier; Poilblanc, Didier
2017-09-01
Two-dimensional (spin-2) Affleck-Kennedy-Lieb-Tasaki (AKLT) type valence bond solids on a square lattice are known to be symmetry-protected topological (SPT) gapped spin liquids [S. Takayoshi, P. Pujol, and A. Tanaka Phys. Rev. B 94, 235159 (2016), 10.1103/PhysRevB.94.235159]. Using the projected entangled pair state framework, we extend the construction of the AKLT state to the case of SU(3 ) , relevant for cold atom systems. The entanglement spectrum is shown to be described by an alternating SU(3 ) chain of "quarks" and "antiquarks", subject to exponentially decaying (with distance) Heisenberg interactions, in close similarity with its SU(2 ) analog. We discuss the SPT feature of the state.
Large Scale Parallel DNA Detection by Two-Dimensional Solid-State Multipore Systems.
Athreya, Nagendra Bala Murali; Sarathy, Aditya; Leburton, Jean-Pierre
2018-04-23
We describe a scalable device design of a dense array of multiple nanopores made from nanoscale semiconductor materials to detect and identify translocations of many biomolecules in a massively parallel detection scheme. We use molecular dynamics coupled to nanoscale device simulations to illustrate the ability of this device setup to uniquely identify DNA parallel translocations. We show that the transverse sheet currents along membranes are immune to the crosstalk effects arising from simultaneous translocations of biomolecules through multiple pores, due to their ability to sense only the local potential changes. We also show that electronic sensing across the nanopore membrane offers a higher detection resolution compared to ionic current blocking technique in a multipore setup, irrespective of the irregularities that occur while fabricating the nanopores in a two-dimensional membrane.
Baranov, Dmitry
This thesis describes new aspects of the synthesis and ultrafast spectroscopy of PbS nanocrystals. The first part of the thesis investigates two aspects of PbS nanocrystal synthesis: the identity and composition of oleylamine reagent and the nature of sulfur species in sulfur solutions in long-chain amines. Oleylamine, formally cis-9-octadecyl-1-amine, is a solvent, a reactant, and a ligand in the synthesis of high-quality PbS nanocrystals and other nanomaterials. It is shown that commercial oleylamine samples contain elaidylamine, trans-9-octadecen-1-amine. Sulfur solutions in long-chain amines (n-octylamine and oleylamine) are common precursors in metal sulfide nanomaterial synthesis. Resonance Raman experiments on sulfur-amine solutions established the presence of various polysulfide anions, which slowly equilibrate on the timescale of days, causing a change in reactivity of the sulfur precursor. This aging of sulfur-amine solutions is shown to be strongly correlated with irreproducibility in PbS nanocrystal syntheses. The second part of the thesis deals with non-linear optical experiments on sensitive samples, where vibrational stability, repetitive excitation, and sensitivity to air and moisture constitute a set of challenges often preventing an experiment without photoproduct contamination. As a solution to this problem, we designed, constructed and characterized a compact spinning sample cell suitable for liquid and thin film samples. The spinning sample cell, enclosed in a copper gasket sealed enclosure, enables complete sample exchange in optical experiments with up to 100 kHz repetition rates while maintaining an oxygen and water free environment at the 1 ppm level for over a month. The spinning sample cell was successfully used in a two-dimensional electronic spectroscopy experiment on PbS nanocrystals in solution, eliminating the buildup of the long-lived photoproducts and reducing trap emission in the spinning sample.
PEBBLE: a two-dimensional steady-state pebble bed reactor thermal hydraulics code
Energy Technology Data Exchange (ETDEWEB)
Vondy, D.R.
1981-09-01
This report documents the local implementation of the PEBBLE code to treat the two-dimensional steady-state pebble bed reactor thermal hydraulics problem. This code is implemented as a module of a computation system used for reactor core history calculations. Given power density data, the geometric description in (RZ), and basic heat removal conditions and thermal properties, the coolant properties, flow conditions, and temperature distributions in the pebble fuel elements are predicted. The calculation is oriented to the continuous fueling, steady state condition with consideration of the effect of the high energy neutron flux exposure and temperature history on the thermal conductivity. The coolant flow conditions are calculated for the same geometry as used in the neutronics calculation, power density and fluence data being used directly, and temperature results are made available for subsequent use.
Jun, Sunhong; Yang, Cheolhee; Kim, Tae Wu; Isaji, Megumi; Tamiaki, Hitoshi; Ihee, Hyotcherl; Kim, Jeongho
2015-07-21
Chlorosomes are the largest light harvesting complexes in nature and consist of many bacteriochlorophyll pigments forming self-assembled J-aggregates. In this work, we use two-dimensional electronic spectroscopy (2D-ES) to investigate ultrafast dynamics of excitation energy transfer (EET) in chlorosomes and their temperature dependence. From time evolution of the measured 2D electronic spectra of chlorosomes, we directly map out the distribution of the EET rate among the manifold of exciton states in a 2D energy space. In particular, it is found that the EET rate varies gradually depending on the energies of energy-donor and energy-acceptor states. In addition, from comparative 2D-ES measurements at 77 K and room temperature, we show that the EET rate exhibits subtle dependence on both the exciton energy and temperature, demonstrating the effect of thermal excitation on the EET rate. This observation suggests that active thermal excitation at room temperature prevents the excitation trapping at low-energy states and thus promotes efficient exciton diffusion in chlorosomes at ambient temperature.
Nenov, Artur; Mukamel, Shaul; Garavelli, Marco; Rivalta, Ivan
2015-08-11
First-principles simulations of two-dimensional electronic spectroscopy in the ultraviolet region (2DUV) require computationally demanding multiconfigurational approaches that can resolve doubly excited and charge transfer states, the spectroscopic fingerprints of coupled UV-active chromophores. Here, we propose an efficient approach to reduce the computational cost of accurate simulations of 2DUV spectra of benzene, phenol, and their dimer (i.e., the minimal models for studying electronic coupling of UV-chromophores in proteins). We first establish the multiconfigurational recipe with the highest accuracy by comparison with experimental data, providing reference gas-phase transition energies and dipole moments that can be used to construct exciton Hamiltonians involving high-lying excited states. We show that by reducing the active spaces and the number of configuration state functions within restricted active space schemes, the computational cost can be significantly decreased without loss of accuracy in predicting 2DUV spectra. The proposed recipe has been successfully tested on a realistic model proteic system in water. Accounting for line broadening due to thermal and solvent-induced fluctuations allows for direct comparison with experiments.
DEFF Research Database (Denmark)
Chen, Yunzhong; Trier, Felix; Kasama, Takeshi
2015-01-01
The discovery of two-dimensional electron gases (2DEGs) in SrTiO3-based heterostructures provides new opportunities for nanoelectronics. Herein, we create a new type of oxide 2DEG by the epitaxial-strain-induced polarization at an otherwise nonpolar perovskite-type interface of CaZrO3/SrTiO3. Rem...
Yin, Na; Dai, Ying; Wei, Wei; Huang, Baibiao
2018-04-01
A lot of efforts have been made towards the band gap opening in two-dimensional silicene, the silicon version of graphene. In the present work, the electronic structures of single atom doped (B, N, Al and P) and codoped (B/N and Al/P) silicene monolayers are systematically examined on the base of density functional electronic calculations. Our results demonstrate that single atom doping can realize electron or hole doping in the silicene; while codoping, due to the syergistic effects, results in finite band gap in silicene at the Dirac point without significantly degrading the electronic properties. In addition, the characteristic of band gap shows dependence on the doping concentration. Importantly, we predict a new two-dimensional Dirac structure, the graphene-like Si3C, which also shows linear band dispersion relation around the Fermi level. Our results demonstrates an important perspective to engineer the electronic and optical properties of silicene.
Two-dimensional effects in the problem of tearing modes control by electron cyclotron current drive
International Nuclear Information System (INIS)
Comisso, L.; Lazzaro, E.
2010-01-01
The design of means to counteract robustly the classical and neoclassical tearing modes in a tokamak by localized injection of an external control current requires an ever growing understanding of the physical process, beyond the Rutherford-type zero-dimensional models. Here a set of extended magnetohydrodynamic nonlinear equations for four continuum fields is used to investigate the two-dimensional effects in the response of the reconnecting modes to specific inputs of the localized external current. New information is gained on the space- and time-dependent effects of the external action on the two-dimensional structure of magnetic islands, which is very important to formulate applicable control strategies.
Directory of Open Access Journals (Sweden)
Kunal Pathak
2016-09-01
Full Text Available The calcium signaling plays a crucial role in expansion and contraction of cardiac myocytes. This calcium signaling is achieved by calcium diffusion, buffering mechanisms and influx in cardiac myocytes. The various calcium distribution patterns required for achieving calcium signaling in myocytes are still not well understood. In this paper an attempt has been made to develop a model of calcium distribution in myocytes incorporating diffusion of calcium, point source and excess buffer approximation. The model has been developed for a two dimensional unsteady state case. Appropriate boundary conditions and initial condition have been framed. The finite element method has been employed to obtain the solution. The numerical results have been used to study the effect of buffers and source amplitude on calcium distribution in myocytes.
Density of states of two-dimensional systems with long-range logarithmic interactions
Energy Technology Data Exchange (ETDEWEB)
Somoza, Andrés M.; Ortuño, Miguel; Baturina, Tatyana I.; Vinokur, Valerii M.
2015-08-03
We investigate a single-particle density of states (DOS) in strongly disordered two- dimensional high dielectric permittivity systems with logarithmic Coulomb interaction between particles. We derive self-consistent DOS at zero temperature and show that it is appreciably suppressed as compared to the DOS expected from the Efros-Shklovskii approach.We carry out zero- and finite-temperature Monte Carlo numerical studies of the DOS and find the perfect agreement between the numerical and analytical results at zero temperature, observing, in particular, a hardening of the Coulomb gap with the increasing electrostatic screening length. At finite temperatures, we reveal a striking scaling of the DOS as a function of energy normalized to the temperature of the system.
Shi, Zhiming
2016-07-12
Fluorination has been instrumental for tuning the properties of several two-dimensional (2D) materials, including graphene, h-BN, and MoS2. However, its potential application has not yet been explored in 2D silicon carbide (SiC), a promising material for nanoelectronic devices. We investigate the structural, electronic, and magnetic properties of fully and partially fluorinated 2D SiC sheets and nanoribbons by means of density functional theory combined with cluster expansion calculations. We find that fully fluorinated 2D SiC exhibits chair configurations and a nonmagnetic semiconducting behavior. Fluorination is shown to be an efficient approach for tuning the band gap. Four ground states of partially fluorinated SiC, SiCF2x with x = 0.0625, 0.25, 0.5, 0.75, are obtained by cluster expansion calculations. All of them exhibit nanoroad patterns, with the x = 0.5 structure identified as the most stable one. The x = 0.0625 structure is a nonmagnetic metal, while the other three are all ferromagnetic half-metals, whose properties are not affected by the edge states. We propose an effective approach for modulating the electronic and magnetic behavior of 2D SiC, paving the way to applications of SiC nanostructures in integrated multifunctional and spintronic nanodevices. © 2016 American Chemical Society.
Ang, Yee Sin; Ma, Zhongshui; Zhang, C
2014-01-21
The unusual tunneling effects of massless chiral fermions (mCF) and massive chiral fermions (MCF) in a single layer graphene and bilayer graphene represent some of the most bizarre quantum transport phenomena in condensed matter system. Here we show that in a two-dimensional semiconductor with Rashba spin-orbit coupling (R2DEG), the real-spin chiral-like tunneling of electrons at normal incidence simultaneously exhibits features of mCF and MCF. The parabolic branch of opposite spin in R2DEG crosses at a Dirac-like point and has a band turning point. These features generate transport properties not found in usual two-dimensional electron gas. Albeit its π Berry phase, electron backscattering is present in R2DEG. An electron mimics mCF if its energy is in the vicinity of the subband crossing point or it mimics MCF if its energy is near the subband minima.
Two-dimensional lattice model for the surface states of topological insulators
Zhou, Yan-Feng; Jiang, Hua; Xie, X. C.; Sun, Qing-Feng
2017-06-01
The surface states in three-dimensional (3D) topological insulators can be described by a two-dimensional (2D) continuous Dirac Hamiltonian. However, there exists the fermion doubling problem when putting the continuous 2D Dirac equation into a lattice model. In this paper, we introduce a Wilson term with a zero bare mass into the 2D lattice model to overcome the difficulty. By comparing with a 3D Hamiltonian, we show that the modified 2D lattice model can faithfully describe the low-energy electrical and transport properties of surface states of 3D topological insulators. So this 2D lattice model provides a simple and cheap way to numerically simulate the surface states of 3D topological-insulator nanostructures. Based on the 2D lattice model, we also establish the wormhole effect in a topological-insulator nanowire by a magnetic field along the wire and show the surface states being robust against disorder. The proposed 2D lattice model can be extensively applied to study the various properties and effects, such as the transport properties, Hall effect, universal conductance fluctuations, localization effect, etc. So, it paves a way to study the surface states of the 3D topological insulators.
Energy Technology Data Exchange (ETDEWEB)
Lewis, NHC; Gruenke, NL; Oliver, TAA; Ballottari, M; Bassi, R; Fleming, GR
2016-10-05
Light-harvesting complex II (LHCII) serves a central role in light harvesting for oxygenic photosynthesis and is arguably the most important photosynthetic antenna complex. In this article, we present two-dimensional electronic–vibrational (2DEV) spectra of LHCII isolated from spinach, demonstrating the possibility of using this technique to track the transfer of electronic excitation energy between specific pigments within the complex. We assign the spectral bands via comparison with the 2DEV spectra of the isolated chromophores, chlorophyll a and b, and present evidence that excitation energy between the pigments of the complex are observed in these spectra. Lastly, we analyze the essential components of the 2DEV spectra using singular value decomposition, which makes it possible to reveal the relaxation pathways within this complex.
International Nuclear Information System (INIS)
Prinz, A.
2002-03-01
For more than two decades it was the predominant view among the physical community that the every two-dimensional (2D) disordered electron system becomes insulating as the temperature approaches the absolute zero temperature (0 Kelvin or -273.15 o C). Two-dimensional means that the movement of the charge carriers is confined in one direction by a potential so that the carriers can move freely only perpendicular to the confinement. The most famous physical realization of a 2D system is the silicon metal-oxide-semiconductor field effect transistor (Si-MOSFET). It is one of the basic elements of most electronic devices in our daily life. The working principle is very simple. Charges are attracted to the semiconductor-oxide interface by an electric field applied between the metallic gate and the semiconductor, so that a 2D conductive channel is formed. The charge density can be adjusted by the voltage from zero up to 10 13 cm -2 . In 1994 Kravchenko and coworkers made a very important discovery. They studied high mobility Si-MOSFETs and found that for densities below a certain critical value, nc, the resistivity increases as the temperature is decreased below 2 K, whereas for densities above $n c $ the resistivity decreases unexpectedly. The transition from insulating to metallic behavior, known as metal-insulator transition (MIT), was obviously a contradiction to the commonly accepted theories which predict insulating behavior for any density. The insulating behavior is a consequence of the wave properties of electrons which leads to interference in disordered media and thus to enhanced backscattering. In the subsequent years, experimental studies were performed on a variety of 2D systems, which qualitatively showed a similar behavior. All the investigated samples had one thing in common. The interaction energy between the carriers was considerable higher than their mean kinetic energy due to their movement in the 2D plane. Since the electron-electron interaction was
Coupling effect of topological states and Chern insulators in two-dimensional triangular lattices
Zhang, Jiayong; Zhao, Bao; Xue, Yang; Zhou, Tong; Yang, Zhongqin
2018-03-01
We investigate topological states of two-dimensional (2D) triangular lattices with multiorbitals. Tight-binding model calculations of a 2D triangular lattice based on px and py orbitals exhibit very interesting doubly degenerate energy points at different positions (Γ and K /K' ) in momentum space, with quadratic non-Dirac and linear Dirac band dispersions, respectively. Counterintuitively, the system shows a global topologically trivial rather than nontrivial state with consideration of spin-orbit coupling due to the "destructive interference effect" between the topological states at the Γ and K /K' points. The topologically nontrivial state can emerge by introducing another set of triangular lattices to the system (bitriangular lattices) due to the breakdown of the interference effect. With first-principles calculations, we predict an intrinsic Chern insulating behavior (quantum anomalous Hall effect) in a family of the 2D triangular lattice metal-organic framework of Co(C21N3H15) (TPyB-Co) from this scheme. Our results provide a different path and theoretical guidance for the search for and design of new 2D topological quantum materials.
Sawada, A.; Koga, T.
2017-02-01
We have developed a method to calculate the weak localization and antilocalization corrections based on the real-space simulation, where we provide 147 885 predetermined return orbitals of quasi-two-dimensional electrons with up to 5000 scattering events that are repeatedly used. Our model subsumes that of Golub [L. E. Golub, Phys. Rev. B 71, 235310 (2005), 10.1103/PhysRevB.71.235310] when the Rashba spin-orbit interaction (SOI) is assumed. Our computation is very simple, fast, and versatile, where the numerical results, obtained all at once, cover wide ranges of the magnetic field under various one-electron interactions H' exactly. Thus, it has straightforward extensibility to incorporate interactions other than the Rashba SOI, such as the linear and cubic Dresselhaus SOIs, Zeeman effect, and even interactions relevant to the valley and pseudo spin degrees of freedom, which should provide a unique tool to study new classes of materials like emerging 2D materials. Using our computation, we also demonstrate the robustness of a persistent spin helix state against the cubic Dresselhaus SOI.
International Nuclear Information System (INIS)
Volkov, B.A.; Pankratov, O.A.
1986-01-01
Semiconductor inversion junction, presenting the contact of materials in which energy levels corresponding to band edges are mutually inverted. At that, the symmetry of wave function of conductivity band in one material coincides with the symmetry of valence band of the other and vice versa. Specificity of the inversion contact is determined by the presence of electron states independent of the transition band type, which are similar to soliton ones in one-dimensional systems. In the region of the junction the states are characterized by linear massless spectrum nondegenerate in spin. Energy spectrum of the inversion junction for semiconductors of the Pb 1-x Sn y Te x type is considered
Energy Technology Data Exchange (ETDEWEB)
Lewis, Nicholas H. C. [Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Dong, Hui [Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Oliver, Thomas A. A. [Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Fleming, Graham R. [Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
2015-09-28
Two dimensional electronic spectroscopy has proven to be a valuable experimental technique to reveal electronic excitation dynamics in photosynthetic pigment-protein complexes, nanoscale semiconductors, organic photovoltaic materials, and many other types of systems. It does not, however, provide direct information concerning the spatial structure and dynamics of excitons. 2D infrared spectroscopy has become a widely used tool for studying structural dynamics but is incapable of directly providing information concerning electronic excited states. 2D electronic-vibrational (2DEV) spectroscopy provides a link between these domains, directly connecting the electronic excitation with the vibrational structure of the system under study. In this work, we derive response functions for the 2DEV spectrum of a molecular dimer and propose a method by which 2DEV spectra could be used to directly measure the electronic site populations as a function of time following the initial electronic excitation. We present results from the response function simulations which show that our proposed approach is substantially valid. This method provides, to our knowledge, the first direct experimental method for measuring the electronic excited state dynamics in the spatial domain, on the molecular scale.
Energy Technology Data Exchange (ETDEWEB)
Lewis, Nicholas H. C.; Dong, Hui; Oliver, Thomas A. A.; Fleming, Graham R., E-mail: grfleming@lbl.gov [Department of Chemistry, University of California, Berkeley, California 94720 (United States); Physical Biosciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Kavli Energy Nanosciences Institute at Berkeley, Berkeley, California 94720 (United States)
2015-09-28
Two dimensional electronic spectroscopy has proved to be a valuable experimental technique to reveal electronic excitation dynamics in photosynthetic pigment-protein complexes, nanoscale semiconductors, organic photovoltaic materials, and many other types of systems. It does not, however, provide direct information concerning the spatial structure and dynamics of excitons. 2D infrared spectroscopy has become a widely used tool for studying structural dynamics but is incapable of directly providing information concerning electronic excited states. 2D electronic-vibrational (2DEV) spectroscopy provides a link between these domains, directly connecting the electronic excitation with the vibrational structure of the system under study. In this work, we derive response functions for the 2DEV spectrum of a molecular dimer and propose a method by which 2DEV spectra could be used to directly measure the electronic site populations as a function of time following the initial electronic excitation. We present results from the response function simulations which show that our proposed approach is substantially valid. This method provides, to our knowledge, the first direct experimental method for measuring the electronic excited state dynamics in the spatial domain, on the molecular scale.
Layer-dependent anisotropic electronic structure of freestanding quasi-two-dimensional Mo S 2
Hong, Jinhua
2016-02-29
The anisotropy of the electronic transition is a well-known characteristic of low-dimensional transition-metal dichalcogenides, but their layer-thickness dependence has not been properly investigated experimentally until now. Yet, it not only determines the optical properties of these low-dimensional materials, but also holds the key in revealing the underlying character of the electronic states involved. Here we used both angle-resolved electron energy-loss spectroscopy and spectral analysis of angle-integrated spectra to study the evolution of the anisotropic electronic transition involving the low-energy valence electrons in the freestanding MoS2 layers with different thicknesses. We are able to demonstrate that the well-known direct gap at 1.8 eV is only excited by the in-plane polarized field while the out-of-plane polarized optical gap is 2.4 ± 0.2 eV in monolayer MoS2. This contrasts with the much smaller anisotropic response found for the indirect gap in the few-layer MoS2 systems. In addition, we determined that the joint density of states associated with the indirect gap transition in the multilayer systems and the corresponding indirect transition in the monolayer case has a characteristic three-dimensional-like character. We attribute this to the soft-edge behavior of the confining potential and it is an important factor when considering the dynamical screening of the electric field at the relevant excitation energies. Our result provides a logical explanation for the large sensitivity of the indirect transition to thickness variation compared with that for the direct transition, in terms of quantum confinement effect.
Directory of Open Access Journals (Sweden)
Zhishuo Huang
2016-08-01
Full Text Available Neither of the two typical two-dimensional materials, graphene and single layer MoS 2 , are good enough for developing semiconductor logical devices. We calculated the electron mobility of 14 two-dimensional semiconductors with composition of MX 2 , where M (=Mo, W, Sn, Hf, Zr and Pt are transition metals, and Xs are S, Se and Te. We approximated the electron phonon scattering matrix by deformation potentials, within which long wave longitudinal acoustical and optical phonon scatterings were included. Piezoelectric scattering in the compounds without inversion symmetry is also taken into account. We found that out of the 14 compounds, WS 2 , PtS 2 and PtSe 2 are promising for logical devices regarding the possible high electron mobility and finite band gap. Especially, the phonon limited electron mobility in PtSe 2 reaches about 4000 cm 2 ·V - 1 ·s - 1 at room temperature, which is the highest among the compounds with an indirect bandgap of about 1.25 eV under the local density approximation. Our results can be the first guide for experiments to synthesize better two-dimensional materials for future semiconductor devices.
Directory of Open Access Journals (Sweden)
E. Kalesaki
2014-01-01
Full Text Available We study theoretically two-dimensional single-crystalline sheets of semiconductors that form a honeycomb lattice with a period below 10 nm. These systems could combine the usual semiconductor properties with Dirac bands. Using atomistic tight-binding calculations, we show that both the atomic lattice and the overall geometry influence the band structure, revealing materials with unusual electronic properties. In rocksalt Pb chalcogenides, the expected Dirac-type features are clouded by a complex band structure. However, in the case of zinc-blende Cd-chalcogenide semiconductors, the honeycomb nanogeometry leads to rich band structures, including, in the conduction band, Dirac cones at two distinct energies and nontrivial flat bands and, in the valence band, topological edge states. These edge states are present in several electronic gaps opened in the valence band by the spin-orbit coupling and the quantum confinement in the honeycomb geometry. The lowest Dirac conduction band has S-orbital character and is equivalent to the π-π^{⋆} band of graphene but with renormalized couplings. The conduction bands higher in energy have no counterpart in graphene; they combine a Dirac cone and flat bands because of their P-orbital character. We show that the width of the Dirac bands varies between tens and hundreds of meV. These systems emerge as remarkable platforms for studying complex electronic phases starting from conventional semiconductors. Recent advancements in colloidal chemistry indicate that these materials can be synthesized from semiconductor nanocrystals.
Energy Technology Data Exchange (ETDEWEB)
Tur, A.; Fruit, G.; Louarn, P. [Institut de Recherche en Astrophysique et Planétologie (IRAP), CNRS UMR5277/Université Paul Sabatier, Toulouse (France); Yanovsky, V. [Institute for Single Crystals, National Academy of Sciences of Ukraine, Kharkov 61001 (Ukraine)
2014-03-15
In the general context of understanding the possible destabilization of a current sheet with applications to magnetospheric substorms or solar flares, a kinetic model is proposed for studying the resonant interaction between electromagnetic fluctuations and trapped bouncing electrons in a 2D current sheet. Tur et al. [A. Tur et al., Phys. Plasmas 17, 102905 (2010)] and Fruit et al. [G. Fruit et al., Phys. Plasmas 20, 022113 (2013)] already used this model to investigate the possibilities of electrostatic instabilities. Here, the model is completed for full electromagnetic perturbations. Starting with a modified Harris sheet as equilibrium state, the linearized gyrokinetic Vlasov equation is solved for electromagnetic fluctuations with period of the order of the electron bounce period. The particle motion is restricted to its first Fourier component along the magnetic field and this allows the complete time integration of the non local perturbed distribution functions. The dispersion relation for electromagnetic modes is finally obtained through the quasineutrality condition and the Ampere's law for the current density. It is found that for mildly strechted current, undamped modes oscillate at typical electron bounce frequency with wavelength of the order of the plasma sheet half thickness. As the stretching of the plasma sheet becomes more intense, the frequency of these normal modes decreases and beyond a certain threshold in ε = B{sub z}/B{sub lobes}, the mode becomes explosive with typical growth rate of a few tens of seconds. The free energy contained in the bouncing motion of the electrons may trigger an electromagnetic instability able to disrupt the cross-tail current in a few seconds. This new instability–electromagnetic electron-bounce instability–may explain fast and global scale destabilization of current sheets as required to describe substorm phenomena.
DEFF Research Database (Denmark)
Kretschmer, Silvan; Komsa, Hannu-Pekka; Bøggild, Peter
2017-01-01
The polymorphism of two-dimensional (w2D) transition-metal dichalcogenides (TMDs) and different electronic properties of the polymorphs make TMDs particularly promising materials in the context of applications in electronics. Recently, local transformations from the semiconducting trigonal...... prismatic H phase to the metallic octahedral T phase in 2D MoS2 have been induced by electron irradiation [Nat. Nanotech. 2014, 9, 391], but the mechanism of the transformations remains elusive. Using density functional theory calculations, we study the energetics of the stable and metastable phases of 2D...
Quasi-steady-state analysis of two-dimensional random intermittent search processes
Bressloff, Paul C.
2011-06-01
We use perturbation methods to analyze a two-dimensional random intermittent search process, in which a searcher alternates between a diffusive search phase and a ballistic movement phase whose velocity direction is random. A hidden target is introduced within a rectangular domain with reflecting boundaries. If the searcher moves within range of the target and is in the search phase, it has a chance of detecting the target. A quasi-steady-state analysis is applied to the corresponding Chapman-Kolmogorov equation. This generates a reduced Fokker-Planck description of the search process involving a nonzero drift term and an anisotropic diffusion tensor. In the case of a uniform direction distribution, for which there is zero drift, and isotropic diffusion, we use the method of matched asymptotics to compute the mean first passage time (MFPT) to the target, under the assumption that the detection range of the target is much smaller than the size of the domain. We show that an optimal search strategy exists, consistent with previous studies of intermittent search in a radially symmetric domain that were based on a decoupling or moment closure approximation. We also show how the decoupling approximation can break down in the case of biased search processes. Finally, we analyze the MFPT in the case of anisotropic diffusion and find that anisotropy can be useful when the searcher starts from a fixed location. © 2011 American Physical Society.
Degenerate ground states and multiple bifurcations in a two-dimensional q-state quantum Potts model.
Dai, Yan-Wei; Cho, Sam Young; Batchelor, Murray T; Zhou, Huan-Qiang
2014-06-01
We numerically investigate the two-dimensional q-state quantum Potts model on the infinite square lattice by using the infinite projected entangled-pair state (iPEPS) algorithm. We show that the quantum fidelity, defined as an overlap measurement between an arbitrary reference state and the iPEPS ground state of the system, can detect q-fold degenerate ground states for the Z_{q} broken-symmetry phase. Accordingly, a multiple bifurcation of the quantum ground-state fidelity is shown to occur as the transverse magnetic field varies from the symmetry phase to the broken-symmetry phase, which means that a multiple-bifurcation point corresponds to a critical point. A (dis)continuous behavior of quantum fidelity at phase transition points characterizes a (dis)continuous phase transition. Similar to the characteristic behavior of the quantum fidelity, the magnetizations, as order parameters, obtained from the degenerate ground states exhibit multiple bifurcation at critical points. Each order parameter is also explicitly demonstrated to transform under the Z_{q} subgroup of the symmetry group of the Hamiltonian. We find that the q-state quantum Potts model on the square lattice undergoes a discontinuous (first-order) phase transition for q=3 and q=4 and a continuous phase transition for q=2 (the two-dimensional quantum transverse Ising model).
Two dimensional electron gas confined over a spherical surface: Magnetic moment
Energy Technology Data Exchange (ETDEWEB)
Hernando, A; Crespo, P [Instituto de Magnetismo Aplicado, UCM-CSIC-ADIF, Las Rozas. P. O. Box 155, Madrid 28230 (Spain) and Dpto. Fisica de Materiales, Universidad Complutense (Spain); Garcia, M A, E-mail: antonio.hernando@adif.es [Instituto de Ceramica y Vidrio, CSIC c/Kelsen, 5 Madrid 28049 (Spain)
2011-04-01
Magnetism of capped nanoparticles, NPs, of non-magnetic substances as Au and ZnO is briefly reviewed. The source of the magnetization is discussed on the light of recent X-ray magnetic circular dichroism experiments. As magnetic dichroism analysis has pointed out impurity atoms bonded to the surface act as donor or acceptor of electrons that occupy the surface states. It is proposed that mesoscopic collective orbital magnetic moments induced at the surface states can account for the experimental magnetism characteristic of these nanoparticles. The total magnetic moment of the surface originated at the unfilled Fermi level can reach values as large as 10{sup 2} or 10{sup 3} Bohr magnetons.
Energy Technology Data Exchange (ETDEWEB)
Quinn, John
2009-11-30
Work related to this project introduced the idea of an effective monopole strength Q* that acted as the effective angular momentum of the lowest shell of composite Fermions (CF). This allowed us to predict the angular momentum of the lowest band of energy states for any value of the applied magnetic field simply by determining N{sub QP} the number of quasielectrons (QE) or quasiholes (QH) in a partially filled CF shell and adding angular momenta of the N{sub QP} Fermions excitations. The approach reported treated the filled CF level as a vacuum state which could support QE and QH excitations. Numerical diagonalization of small systems allowed us to determine the angular momenta, the energy, and the pair interaction energies of these elementary excitations. The spectra of low energy states could then be evaluated in a Fermi liquid-like picture, treating the much smaller number of quasiparticles and their interactions instead of the larger system of N electrons with Coulomb interactions.
Phonon-driven electron scattering and magnetothermoelectric effect in two-dimensional tin selenide
Yang, Kaike; Ren, Ji-Chang; Qiu, Hongfei; Wang, Jian-Sheng
2018-02-01
The bulk tin selenide (SnSe) is the best thermoelectric material currently with the highest figure-of-merit due to strong phonon–phonon interactions. We investigate the effect of electron–phonon coupling (EPC) on the transport properties of a two-dimensional (2D) SnSe sheet. We demonstrate that EPC plays a key role in the scattering rate when the constant relaxation time approximation is deficient. The EPC strength is especially large in contrast to that of pristine graphene. The scattering rate depends sensitively on the system temperatures and the carrier densities when the Fermi energy approaches the band edge. We also investigate the magnetothermoelectric effect of the 2D SnSe. It is found that at low temperatures there is enormous magnetoelectrical resistivity and magnetothermal resistivity above 200%, suggesting possible potential applications in device design. Our results agree qualitatively well with the experimental data.
Hoffman, David Paul
Chemical reactions are defined by the change in the relative positions and bonding of nuclei in molecules. I have used femtosecond stimulated Raman spectroscopy (FSRS) to probe these transformations with structural specificity and high time precision revealing the mechanisms of two important classes of reactions; isomerization about an N=N bond and interfacial/intermolecular electron transfer. Isomerization about a double bond is one of the simplest, yet most important, photochemical reactions. In contrast to carbon double bonds, nitrogen double bonds can react via two possible mechanisms; rotation or inversion. To determine which pathway is predominant, I studied an azobenzene derivative using both FSRS and impulsive stimulated Raman spectroscopy (ISRS). The FSRS experiments demonstrated that the photochemical reaction occurs concomitantly with the 700 fs non-radiative decay of the excited state; because no major change in N=N stretching frequency was measured, I surmised that the reaction proceeds through an inversion pathway. My subsequent ISRS experiments confirmed this hypothesis; I observed a highly displaced, low frequency, inversion-like mode, indicating that initial movement out of the Franck-Condon region proceeds along an inversion coordinate. To probe which nuclear motions facilitate electron transfer and charge recombination, I used FSRS and the newly developed 2D-FSRS techniques to study two model systems, triphenylamine dyes bound to TiO2 nanoparticles and a molecular charge transfer (CT) dimer. In the dye-nanoparticle system I discovered that charge separation persists much longer (> 100 ps) than previously thought by using the juxtaposition of the FSRS and transient absorption data to separate the dynamics of the dye from that of the injected electron. Additionally, I discovered that dye constructs with an added vinyl group were susceptible to quenching via isomerization. The CT dimer offered an opportunity to study a system in which charge
Quasi-two-dimensional Fermi-liquid state in Sr2RhO4-δ
International Nuclear Information System (INIS)
Nagai, Ichiro; Shirakawa, Naoki; Umeyama, Norio; Ikeda, Shin-ichi
2010-01-01
Single crystals of layered perovskite Sr 2 RhO 4-δ (δ=0.0 and 0.1) are successfully grown by the floating-zone method. Stoichiometric single crystals (Sr 2 RhO 4.0 ) are obtained by O 2 -annealing the as-grown crystals (Sr 2 RhO 3.9 ). Sr 2 RhO 4.0 and Sr 2 RhO 3.9 show quasi-two-dimensional Fermi-liquid behavior at low temperatures, whereas there are large differences in the anisotropy of electrical resistivity ρ c (3 K)/ρ ab (3 K) and Wilson ratio R w between Sr 2 RhO 4.0 and Sr 2 RhO 3.9 : ρ c (3 K)/ρ ab (3 K)=2400 (19000) and R w =3.8 (6.4) for Sr 2 RhO 4.0 (Sr 2 RhO 3.9 ). The differences observed between the temperature dependence of the in-plane electrical resistivity (T 2 RhO 4.0 and Sr 2 RhO 3.9 are mainly derived from those between the density of states and band structure near the corresponding Fermi level. This indicates that the changes in these physical properties, which are accompanied by oxygen defects in the Sr 2 RhO 4-δ system, can be explained by the rigid band model. Moreover, these results suggest that t 2g band-filling can be controlled by adjusting the oxygen defect content δ in the Sr 2 RhO 4-δ system. Although many similarities are observed in this study between the physical properties of Sr 2 RhO 4.0 and Sr 2 RuO 4 . Sr 2 RhO 4.0 does not exhibit superconductivity down to 36 mK. (author)
Du, Xiang
As the sizes of individual components in electronic and optoelectronic devices approach nano scale, the performance of the devices is often determined by surface properties due to their large surface-to-volume ratio. Surface phenomena have become one of the cornerstones in nanoelectronic industry. For this reason, research on the surface functionalization has been tremendous amount of growth over the past decades, and promises to be an increasingly important field in the future. Surface functionalization, as an effective technique to modify the surface properties of a material through a physical or chemical approach, exhibits great potential to solve the problems and challenges, and modulate the performance of nanomaterials based functional devices. Surface functionalization drives the developments and applications of modern electronic and optoelectronic devices fabricated by nanomaterials. In this thesis, I demonstrate two surface functionalization approaches, namely, surface transfer doping and H2 annealing, to effectively solve the problems and significantly enhance the performance of 2D (single structure black phosphorus (BP) and heterostructure graphene/Si Schottky junction), and quasi-1D (molybdenum trioxide (MoO 3) nanobelt) nanomaterials based functional devices, respectively. In situ photoelectron spectroscopy (PES) measurements were also carried out to explore the interfacial charge transfer occurring at the interface between the nanostructures and doping layers, and the gap states in MoO 3 thin films, which provides the underlying mechanism to understand and support our device measurement results. In the first part of this thesis, I will discuss the first surface functionalization approach, namely, surface transfer doping, to effectively modulate the ambipolar characteristics of 2D few-layer BP flakes based FETs. The ambipolar characteristics of BP transistors were effectively modulated through in situ surface functionalization with cesium carbonate (Cs2
Czech Academy of Sciences Publication Activity Database
Tichý, V.; Kuběna, Aleš Antonín; Skála, L.
2012-01-01
Roč. 90, č. 6 (2012), s. 503-513 ISSN 0008-4204 Institutional support: RVO:67985556 Keywords : Schroninger equation * partial differential equation * analytic solution * anharmonic oscilator * double-well Subject RIV: BE - Theoretical Physics Impact factor: 0.902, year: 2012 http://library.utia.cas.cz/separaty/2012/E/kubena-analytic energies and wave functions of the two-dimensional schrodinger equation.pdf
Metallic ground state in an ion-gated two-dimensional superconductor
Saito, Yu; Kasahara, Yuichi; Ye, Jianting; Iwasa, Yoshihiro; Nojima, Tsutomu
2015-01-01
Recently emerging two-dimensional (2D) superconductors in atomically thin layers and at heterogeneous interfaces are attracting growing interest in condensed matter physics. Here, we report that an ion-gated zirconium nitride chloride surface, exhibiting a dome-shaped phase diagram with a maximum
Stationary states of the two-dimensional nonlinear Schrödinger model with disorder
DEFF Research Database (Denmark)
Gaididei, Yuri Borisovich; Hendriksen, D.; Christiansen, Peter Leth
1998-01-01
Solitonlike excitations in the presence of disorder in the two-dimensional cubic nonlinear Schrodinger equation are analyzed. The continuum as well as the discrete problem are analyzed. In the continuum model, otherwise unstable excitations are stabilized in the presence of disorder...
Heida, J.P.; Wees, B.J. van; Kuipers, J.J.; Klapwijk, T.M.; Borghs, G.
1998-01-01
We present experiments on the tuning of the spin-orbit interaction in a two-dimensional electron gas in an asymmetric InAs/AlSb quantum well using a gate. The observed dependence of the spin splitting energy on the electron density can be attributed solely to the change in the Fermi wave vector. The
Absolute and convective instabilities in two-dimensional free-electron lasers
International Nuclear Information System (INIS)
Kwan, T.J.T.; Cary, J.R.
1981-01-01
Computer simulations of the free-electron laser have been carried out using a two-and-one-half dimensional fully electromagnetic relativistic particle code. It has been found that waves propagating obliquely with respect to the electron beam are always unstable with appreciable growth rates and, therefore, mode competition is an important consideration in the design of free-electron lasers. Furthermore, electromagnetic waves with group velocities opposite to the direction of electron beam propagation can be absolutely unstable. It is shown that the absolutely unstable waves can completely disrupt the electron beam and any laser oscillaton; therefore, they are extremely detrimental to the operation of free electron lasers. However, it has been found that one can stabilize the absolute instability by taking particular precautions in the design of free-electron lasers
Magneto-transport studies on curved two-dimensional electron gases in InGaAs-microscrolls
International Nuclear Information System (INIS)
Schumacher, O.
2007-01-01
In this thesis magneto-resistance studies on evenly curved two-dimensional electron systems in cylindric geometry are presented and discussed. A principle first introduced by Prinz and co-workers in 1998 enables us to roll up thin semiconductor layer systems by taking advantage of internal elastic strain. The radius of such a semiconductor tube can be adjusted ranging from a few nanometers up to several micrometers. The tubes' shape and place on the substrate can be defined by lithographic methods which are presented in this work. Furthermore, we show rolled-up structures containing a two-dimensional electron system in the tube wall. With a special lithographic procedure we are able to structure, to contact and to roll up these 2D-electron-gases in Hall geometry. As a result, a cylindric two-dimensional electron system is produced, which experiences a modulation of the perpendicular magnetic field component. The radius of curvature of our structures is about 10 μm, the carrier mobility is optimized to values up to 125,000 cm 2 /Vs. In transport experiments on curved Hall bars containing two dimensional electron systems two Hall bar orientations, with respect to the curvature, may be distinguished. In this work both orientations, i.e. with a Hall bar along the tube curvature as well as a Hall bar along the tube axis, are presented and discussed. Measurements on Hall bars along the curvature show signatures in the longitudinal resistance, which can be understood with the help of the Landauer-Buettiker-formalism and the model of magnetic barriers. For Hall bars oriented along the tube axis the perpendicular magnetic field component averaged over the width of the bar defines the minimum position of the Shubnikov-de Haas-oscillations as well as the slope of the Hall resistance. Furthermore, measurements on so-called van the Pauw-lamellas are presented. In this geometry the magneto-resistance shows a slope which refers to highly mobile conditions at the zero crossing of
Lightcap, Ian V; Kosel, Thomas H; Kamat, Prashant V
2010-02-10
Using reduced graphene oxide (RGO) as a two-dimensional support, we have succeeded in selective anchoring of semiconductor and metal nanoparticles at separate sites. Photogenerated electrons from UV-irradiated TiO(2) are transported across RGO to reduce silver ions into silver nanoparticles at a location distinct from the TiO(2) anchored site. The ability of RGO to store and shuttle electrons, as visualized via a stepwise electron transfer process, demonstrates its capability to serve as a catalyst nanomat and transfer electrons on demand to adsorbed species. These findings pave the way for the development of next generation catalyst systems and can spur advancements in graphene-based composites for chemical and biological sensors.
Cai, Libing; Wang, Jianguo; Zhu, Xiangqin; Wang, Yue; Zhang, Dianhui
2015-01-01
Based on the secondary electron emission avalanche (SEEA) model, the SEEA discharge on the vacuum insulator surface is simulated by using a 2D PIC-MCC code developed by ourselves. The evolutions of the number of discharge electrons, insulator surface charge, current, and 2D particle distribution are obtained. The effects of the strength of the applied electric field, secondary electron yield coefficient, rise time of the pulse, length of the insulator on the discharge are investigated. The results show that the number of the SEEA electrons presents a quadratic dependence upon the applied field strength. The SEEA current, which is on the order of Ampere, is directly proportional to the field strength and secondary electron yield coefficient. Finally, the electron-stimulated outgassing is included in the simulation code, and a three-phase discharge curve is presented by the simulation, which agrees with the experimental data.
International Nuclear Information System (INIS)
Cai, Libing; Wang, Jianguo; Zhu, Xiangqin; Wang, Yue; Zhang, Dianhui
2015-01-01
Based on the secondary electron emission avalanche (SEEA) model, the SEEA discharge on the vacuum insulator surface is simulated by using a 2D PIC-MCC code developed by ourselves. The evolutions of the number of discharge electrons, insulator surface charge, current, and 2D particle distribution are obtained. The effects of the strength of the applied electric field, secondary electron yield coefficient, rise time of the pulse, length of the insulator on the discharge are investigated. The results show that the number of the SEEA electrons presents a quadratic dependence upon the applied field strength. The SEEA current, which is on the order of Ampere, is directly proportional to the field strength and secondary electron yield coefficient. Finally, the electron-stimulated outgassing is included in the simulation code, and a three-phase discharge curve is presented by the simulation, which agrees with the experimental data
International Nuclear Information System (INIS)
Lutgen, S.; Kaindl, R.A.; Woerner, M.; Elsaesser, T.; Hase, A.; Kuenzel, H.; Gulia, M.; Meglio, D.; Lugli, P.
1996-01-01
The dynamics of electrons in GaInAs/AlInAs quantum wells is studied after excitation from the n=1 to the n=2 conduction subband. Femtosecond pump-probe experiments demonstrate for the first time athermal distributions of n=1 electrons on a surprisingly long time scale of 2ps. Thermalization involves intersubband scattering of excited electrons via optical phonon emission with a time constant of 1ps and intrasubband Coulomb and phonon scattering. Ensemble Monte Carlo simulations show that the slow electron equilibration results from Pauli blocking and screening of carrier-carrier scattering. copyright 1996 The American Physical Society
Tunable bilayer two-dimensional electron gas in LaAlO3/SrTiO3 superlattices
International Nuclear Information System (INIS)
Ma, H. J. Harsan; Annadi, A.; Zeng, S. W.; Ariando; Huang, Z.; Lü, W. M.; Wong, L. M.; Wang, S. J.; Venkatesan, T.
2014-01-01
We report magnetotransport properties of double heterointerfaces in LaAlO 3 /SrTiO 3 /LaAlO 3 /SrTiO 3 (001) (LAO/STO/LAO/STO). A strong nonlinearity in the Hall resistivity is found when the temperature is below 80 K. This effect is attributed to multichannel conduction of interfacial charges generated in double heterostructures of LAO/STO where two-dimensional electron gas (2DEG) is produced. The multichannel conduction is confirmed by back gating modulation of Hall effect. Our result suggests the possibility to achieve coupled bilayer 2DEG layers in LAO/STO superlattices.
International Nuclear Information System (INIS)
den Hartog, S.G.; van Wees, B.J.; Klapwijk, T.M.; Nazarov, Y.V.; Borghs, G.
1997-01-01
We have investigated the superconducting-phase-modulated reduction in the resistance of a ballistic quantum point contact (QPC) connected via a disordered two-dimensional electron gas (2DEG) to superconductors. We show that this reduction is caused by coherent Andreev backscattering of holes through the QPC, which increases monotonically by reducing the bias voltage to zero. In contrast, the magnitude of the phase-dependent resistance of the disordered 2DEG displays a nonmonotonic reentrant behavior versus bias voltage. copyright 1997 The American Physical Society
Augulis, Ramūnas; Zigmantas, Donatas
2011-07-04
In many potential applications of two-dimensional (2D) electronic spectroscopy the excitation energies per pulse are strictly limited, while the samples are strongly scattering. We demonstrate a technique, based on double-modulation of incident laser beams with mechanical choppers, which can be implemented in almost any non-collinear four wave mixing scheme including 2D spectroscopy setup. The technique virtually eliminates artifacts or "ghost" signals in 2D spectra, which arise due to scattering and accumulation of long-lived species. To illustrate the advantages of the technique, we show a comparison of porphyrin J-aggregate 2D spectra obtained with different methods following by discussion.
Boudjada, Nazim; Wachtel, Gideon; Paramekanti, Arun
2018-02-01
Recent experiments have explored two-dimensional electron gases (2DEGs) at oxide (111) surfaces and interfaces, finding evidence for hexagonal symmetry breaking in SrTiO3 at low temperature. We discuss many-body instabilities of such (111) 2DEGs, incorporating multiorbital interactions in the t2 g manifold which can induce diverse magnetic and orbital orders. Such broken symmetries may partly account for the observed nematicity, cooperating or competing with phonon mechanisms. We present an effective field theory for the interplay of magnetism and nematic charge order, and discuss implications of the nematicity for transport and superconductivity in (111) 2DEGs.
Theoretical Studies of Two-Dimensional Effects in Free Electron Lasers.
1984-12-01
from the electrons is balanced by the energy losses at the mirrors. 871 TABLE Bl MATH SCIENCES FEL PARAMETERS ELECTRON BEAM EXPERIMENTAL SIMULATION...the EM pulse is: mc 2 AP = ,y, --- I(amps)e - 270 "IGW Yr ( Clil ) Let the power loss at the mirrors in the interval between interactions of the beam
Very large capacitance enhancement in a two-dimensional electron system.
Li, Lu; Richter, C; Paetel, S; Kopp, T; Mannhart, J; Ashoori, R C
2011-05-13
Increases in the gate capacitance of field-effect transistor structures allow the production of lower-power devices that are compatible with higher clock rates, driving the race for developing high-κ dielectrics. However, many-body effects in an electronic system can also enhance capacitance. Onto the electron system that forms at the LaAlO(3)/SrTiO(3) interface, we fabricated top-gate electrodes that can fully deplete the interface of all mobile electrons. Near depletion, we found a greater than 40% enhancement of the gate capacitance. Using an electric-field penetration measurement method, we show that this capacitance originates from a negative compressibility of the interface electron system. Capacitance enhancement exists at room temperature and arises at low electron densities, in which disorder is strong and the in-plane conductance is much smaller than the quantum conductance.
Two-dimensional delocalized states in organometallic bis-acetylide networks on Ag(111).
Yang, Zechao; Gebhardt, Julian; Schaub, Tobias A; Sander, Tim; Schönamsgruber, Jörg; Soni, Himadri; Görling, Andreas; Kivala, Milan; Maier, Sabine
2018-02-22
The electronic structure of surface-supported organometallic networks with Ag-bis-acetylide bonds that are intermediate products in the bottom-up synthesis of graphdiyne and graphdiyne-like networks were studied. Scanning tunneling microscopy (STM) and spectroscopy (STS) reveal a frontier, unoccupied electronic state that is delocalized along the entire organometallic network and proves the covalent nature of the Ag-bis-acetylide bonds. Density-functional theory (DFT) calculations corroborate the spatial distribution of the observed delocalized state and attribute it to band mixing of carbon and silver atoms combined with n-doping of the metal surface. The metal-bis-acetylide bonds are typical metal-organic bonds with mixed character containing covalent and strong ionic contributions. Moreover, the organometallic networks exhibit a characteristic graphene-like band structure with linear band dispersion at each K point.
National Research Council Canada - National Science Library
Holmes, Kenneth
2002-01-01
Gallium Nitride (GaN) High Electron Mobility Transistors (HEMT's) are microwave power devices that have the performance characteristics to improve the capabilities of current and future Navy radar and communication systems...
Zhang, You-Run; Zhang, Bo; Li, Zhao-Ji; Deng, Xiao-Chuan
2010-06-01
This paper studies two-dimensional analysis of the surface state effect on current gain for a 4H-SiC bipolar junction transistor (BJT). Simulation results indicate the mechanism of current gain degradation, which is surface Fermi level pinning leading to a strong downward bending of the energy bands to form the channel of surface electron recombination current. The experimental results are well-matched with the simulation, which is modeled by exponential distributions of the interface state density replacing the single interface state trap. Furthermore, the simulation reveals that the oxide quality of the base emitter junction interface is very important for 4H-SiC BJT performance.
Quantum spin-glass transition in the two-dimensional electron gas
Indian Academy of Sciences (India)
canting' enough to disrupt temporal memory of their orientation in the orthogonal plane. (The discussion of this present paper will restrict attention to the case where Hσ > 0. Experimentally, it is known that Hσ decreases as the density of electrons ...
Quantum spin-glass transition in the two-dimensional electron gas
Indian Academy of Sciences (India)
Home; Journals; Pramana – Journal of Physics; Volume 58; Issue 2 ... Spin glasses; quantum phase transition; ferromagnetism; electron gas. ... We argue that a quantum transition involving the destruction of the spin-glass order in an applied in-plane magnetic ﬁeld offers a natural explanation of some features of recent ...
Energy Technology Data Exchange (ETDEWEB)
Tizei, Luiz H. G., E-mail: luiz.galvao-tizei@u-psud.fr [Laboratoire de Physique des Solides, Université Paris-Sud, CNRS-UMR 8502, Orsay 91405 (France); Lin, Yung-Chang; Suenaga, Kazu, E-mail: suenaga-kazu@aist.go.jp [Nanotube Research Center, National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba 305-8565 (Japan); Lu, Ang-Yu; Li, Lain-Jong [Physical Science and Engineering Division, King Abdullah University of Science and Technology, Thuwal 23955-6900 (Saudi Arabia)
2016-04-18
We have explored the benefits of performing monochromated Electron Energy Loss Spectroscopy (EELS) in samples at cryogenic temperatures. As an example, we have observed the excitonic absorption peaks in single layer Transition Metal Dichalcogenides. These peaks appear separated by small energies due to spin orbit coupling. We have been able to distinguish the split for MoS{sub 2} below 300 K and for MoSe{sub 2} below 220 K. However, the distinction between peaks is only clear at 150 K. We have measured the change in absorption threshold between 150 K and 770 K for MoS{sub 2} and MoSe{sub 2}. We discuss the effect of carbon and ice contamination in EELS spectra. The increased spectral resolution available made possible with modern monochromators in electron microscopes will require the development of stable sample holders which reaches temperatures far below that of liquid nitrogen.
Two dimensional localization of electrons and positrons under high counting rate
International Nuclear Information System (INIS)
Barbosa, A.F.; Anjos, J.C.; Sanchez-Hernandez, A.; Pepe, I.M.; Barros, N.
1997-12-01
The construction of two wire chambers for the experiment E831 at Fermilab is reported. Each chamber includes three wire planes - one anode and two orthogonal cathodes - in which the wires operate as independent proportional counters. One of the chambers is rotated with respect to the other, so that four position coordinates may be encoded for a charged particle crossing both chambers. Spatial resolution is determined by the wire pitch: 1 mm for cathodes, 2 mm for anodes. 320 electronic channels are involved in the detection system readout. Global counting rates in excess to 10 7 events per second have been measured, while the average electron-positron beam intensity may be as high as 3 x 10 7 events per second. (author)
Alekseev, P. S.; Dmitriev, A. P.; Gornyi, I. V.; Kachorovskii, V. Yu.; Narozhny, B. N.; Titov, M.
2018-02-01
Ultrapure conductors may exhibit hydrodynamic transport where the collective motion of charge carriers resembles the flow of a viscous fluid. In a confined geometry (e.g., in ultra-high-quality nanostructures), the electronic fluid assumes a Poiseuille-type flow. Applying an external magnetic field tends to diminish viscous effects leading to large negative magnetoresistance. In two-component systems near charge neutrality, the hydrodynamic flow of charge carriers is strongly affected by the mutual friction between the two constituents. At low fields, the magnetoresistance is negative, however, at high fields the interplay between electron-hole scattering, recombination, and viscosity results in a dramatic change of the flow profile: the magnetoresistance changes its sign and eventually becomes linear in very high fields. This nonmonotonic magnetoresistance can be used as a fingerprint to detect viscous flow in two-component conducting systems.
Tizei, Luiz H. G.
2016-04-21
We have explored the benefits of performing monochromated Electron Energy Loss Spectroscopy(EELS) in samples at cryogenic temperatures. As an example, we have observed the excitonic absorption peaks in single layer Transition Metal Dichalcogenides. These peaks appear separated by small energies due to spin orbit coupling. We have been able to distinguish the split for MoS2 below 300 K and for MoSe2 below 220 K. However, the distinction between peaks is only clear at 150 K. We have measured the change in absorption threshold between 150 K and 770 K for MoS2 and MoSe2. We discuss the effect of carbon and ice contamination in EELSspectra. The increased spectral resolution available made possible with modern monochromators in electron microscopes will require the development of stable sample holders which reaches temperatures far below that of liquid nitrogen.
International Nuclear Information System (INIS)
Chen Lijen; Lefebvre, Bertrand; Torbert, Roy B.; Daughton, William S.
2011-01-01
Based on two-dimensional fully kinetic simulations that resolve the electron diffusion layer in undriven collisionless magnetic reconnection with zero guide field, this paper reports the existence and evolution of an inversion layer of bipolar electric fields, its corresponding phase-space structure (an electron-hole layer), and the implication to collisionless dissipation. The inversion electric field layer is embedded in the layer of bipolar Hall electric field and extends throughout the entire length of the electron diffusion layer. The electron phase-space hole structure spontaneously arises during the explosive growth phase when there exist significant inflows into the reconnection layer, and electrons perform meandering orbits across the layer while being cyclotron-turned toward the outflow directions. The cyclotron turning of meandering electrons by the magnetic field normal to the reconnection layer is shown to be a primary factor limiting the current density in the region where the reconnection electric field is balanced by the gradient (along the current sheet normal) of the off-diagonal electron pressure-tensor.
Two-dimensional power-type electronic spectrographs with a symmetry plane
Krasnova, N. K.
2011-06-01
The electronic and optical characteristics of 2D electric fields with a complex potential of the type Ω = i( x + iy) n , where n is a real number, are investigated. Particle dynamics is studied in the symmetry plane and in its neighborhood for constructing an effective spectrograph of electron flows. It is shown that in the range of exponents 0 < n < 1, spatial focusing in the angles of incidence of conical bunches is effected in the system, which has second order in the symmetry plane and at least the first order across it. The line of images of a point source (focal line) is a straight line lying in the symmetry plane, the focusing order being independent of particle energy W. Thus, the spectrographic principle holds, and partial electron fluxes can be detected simultaneously by a position-sensitive detector in a wide range of energy variation. The electrode configuration of these systems is quite simple and can be used in practice for constructing spectrographs. The prospects of application of such spectrographs in energy analysis are considered.
Mokhtari, P.; Rezaei, G.; Zamani, A.
2017-06-01
In this paper, electronic structure of a two dimensional elliptic quantum dot under the influence of external electric and magnetic fields are studied in the presence of Rashba and Dresselhaus spin-orbit interactions. This investigation is done computationally and to do this, at first, the effective Hamiltonian of the system by considering the spin-orbit coupling is demonstrated in the presence of applied electric and magnetic fields and afterwards the Schrödinger equation is solved using the finite difference approach. Utilizing finite element method, eigenvalues and eigenstates of the system are calculated and the effect of the external fields, the size of the dot as well as the strength of Rashba spin-orbit interaction are studied. Our results indicate that, Spin-orbit interactions, external fields and the dot size have a great influence on the electronic structure of the system.
International Nuclear Information System (INIS)
Li Guowang; Cao Yu; Xing Huili Grace; Jena, Debdeep
2010-01-01
We report high-electron mobility nitride heterostructures with >70% Al composition AlGaN alloy barriers grown by molecular beam epitaxy. Direct growth of such AlGaN layers on GaN resulted in hexagonal trenches and a low mobility polarization-induced charge. By applying growth interruption at the heterojunction, the surface morphology improved dramatically and the room temperature two-dimensional electron gas (2DEG) mobility increased by an order of magnitude, exceeding 1300 cm 2 /V s. The 2DEG density was tunable at 0.4-3.7x10 13 /cm 2 by varying the total barrier thickness (t). Surface barrier heights of the heterostructures were extracted and exhibited dependence on t.
International Nuclear Information System (INIS)
Zhukov, Alexander V.; Bouffanais, Roland; Fedorov, E. G.; Belonenko, Mikhail B.
2014-01-01
Propagation of ultrashort laser pulses through various nano-objects has recently became an attractive topic for both theoretical and experimental studies due to its promising perspectives in a variety of problems of modern nanoelectronics. Here, we study the propagation of extremely short two-dimensional bipolar electromagnetic pulses in a heterogeneous array of semiconductor carbon nanotubes. Heterogeneity is defined as a region of enhanced electron density. The electromagnetic field in an array of nanotubes is described by Maxwell's equations, reduced to a multidimensional wave equation. Our numerical analysis shows the possibility of stable propagation of an electromagnetic pulse in a heterogeneous array of nanotubes. Furthermore, we establish that, depending on its speed of propagation, the pulse can pass through the area of increased electron concentration or be reflected therefrom.
Tarasov, Yu. V.
2005-03-01
The effect of an in-plane magnetic field upon open quasi-two-dimensional electron and hole systems is investigated in terms of the carrier ground-state spectrum. The magnetic field, classified as weak from the viewpoint of correlation between size parameters of classical electron motion and the gate potential spatial profile is shown to efficiently cutoff extended modes from the spectrum and to change singularly the mode density of states (MDOS). The reduction in the number of current-carrying modes, right up to zero in magnetic fields of moderate strength, can be viewed as the cause of magnetic-field-driven metal-to-insulator transition widely observed in two-dimensional systems. Both the mode number reduction and the MDOS singularity appear to be most pronounced in the mode states dephasing associated with their scattering by quenched-disorder potential. This sort of dephasing is proven to dominate the dephasing which involves solely the magnetic field whatever level of the disorder.
Mobility and bulk electron-phonon interaction in two-dimensional materials
DEFF Research Database (Denmark)
Gunst, Tue; Brandbyge, Mads; Markussen, Troels
2015-01-01
-of-plane modes. However, we find that graphene only has a slightly higher mobility compared to silicene. For MoS2 we obtain several orders of magnitude lower mobilities and in agreement with other recent theoretical results. The simulations illustrate the predictive capabilities of the newly implemented......We present calculations of the phonon-limited mobility in intrinsic n-type monolayer graphene, silicene and MoS2. The material properties, including the electron-phonon interaction, are calculated from first principles. Unlike graphene, the carriers in silicene show strong interaction with the out...
Directory of Open Access Journals (Sweden)
H. L. He
2016-05-01
Full Text Available We study theoretically the giant magnetoresistance (GMR effect of 2-dimensional electron system (2DES by the transfer matrix method. To produce the inhomogeneous magnetic field, two magnetic strips are pre-deposited on the surface of 2DES. In our work, we fix the magnetization M in one magnetic strip and adjust the tilting angle θ of magnetization in the other. The result shows that the electronic transmission and conductance vary significantly for different θ. The minimum conductance can be obtained at θ = π which corresponds to the magnetization anti-parallel alignment. The magnetoresistance ratio (MRR calculation also indicates we would get the maximum in that case. Furthermore, we consider the magnetization M dependence of MRR in this work. When M increases, MRR peaks get higher and broader and more numbers of peaks can be observed. These results offer an alternative to get a tunable GMR device which can be controlled by adjusting the magnetization M and the magnetized angle θ.
Directory of Open Access Journals (Sweden)
H. J. Harsan Ma
2015-08-01
Full Text Available The two-dimensional electron gas (2DEG formed at the perovskite oxides heterostructures is of great interest because of its potential applications in oxides electronics and nanoscale multifunctional devices. A canonical example is the 2DEG at the interface between a polar oxide LaAlO3 (LAO and non-polar SrTiO3 (STO. Here, the LAO polar oxide can be regarded as the modulating or doping layer and is expected to define the electronic properties of 2DEG at the LAO/STO interface. However, to practically implement the 2DEG in electronics and device design, desired properties such as tunable 2D carrier density are necessary. Here, we report the tuning of conductivity threshold, carrier density and electronic properties of 2DEG in LAO/STO heterostructures by insertion of a La0.5Sr0.5TiO3 (LSTO layer of varying thicknesses, and thus modulating the amount of polarization of the oxide over layers. Our experimental result shows an enhancement of carrier density up to a value of about five times higher than that observed at the LAO/STO interface. A complete thickness dependent metal-insulator phase diagram is obtained by varying the thickness of LAO and LSTO providing an estimate for the critical thickness needed for the metallic phase. The observations are discussed in terms of electronic reconstruction induced by polar oxides.
Directory of Open Access Journals (Sweden)
Shoubin Wang
2017-01-01
Full Text Available Addressing the problem of two-dimensional steady-state thermal boundary recognition, a hybrid algorithm of conjugate gradient method and social particle swarm optimization (CGM-SPSO algorithm is proposed. The global search ability of particle swarm optimization algorithm and local search ability of gradient algorithm are effectively combined, which overcomes the shortcoming that the conjugate gradient method tends to converge to the local solution and relies heavily on the initial approximation of the iterative process. The hybrid algorithm also avoids the problem that the particle swarm optimization algorithm requires a large number of iterative steps and a lot of time. The experimental results show that the proposed algorithm is feasible and effective in solving the problem of two-dimensional steady-state thermal boundary shape.
Two-dimensional and tubular structures of misfit compounds: Structural and electronic properties
Directory of Open Access Journals (Sweden)
Tommy Lorenz
2014-11-01
Full Text Available Misfit layer compounds are structures that consist of two sublattices differing in at least one of their lattice constants. The two different layers are stacked either an alternating or in a more complex series resulting in mono- or multi-layer misfit compounds. To date, planar and bent misfit structures, such as tubes, scrolls or nanoparticles, have been synthesized and interesting magnetic and physical properties have been observed as a result of their special structures. Based on these observations, we present an overview of such misfit systems and summarize and discuss their electronic structure as well as the interlayer bonding behaviour, which is not completely understood yet. Furthermore, a more detailed insight into the SnS–SnS2 system is given, which was the first tubular misfit compound that has been synthesized and extensively investigated.
A high density two-dimensional electron gas in an oxide heterostructure on Si (001)
Energy Technology Data Exchange (ETDEWEB)
Jin, E. N.; Kornblum, L.; Kumah, D. P.; Zou, K.; Walker, F. J. [Center for Research on Interface Structures and Phenomena and Department of Applied Physics, Yale University, New Haven, Connecticut 06511 (United States); Broadbridge, C. C. [Center for Research on Interface Structures and Phenomena and Department of Applied Physics, Yale University, New Haven, Connecticut 06511 (United States); Department of Physics, Southern Connecticut State University, 501 Crescent Street, New Haven, Connecticut 06515 (United States); Ngai, J. H. [Department of Physics, The University of Texas at Arlington, Arlington, Texas 76019 (United States); Ahn, C. H. [Center for Research on Interface Structures and Phenomena and Department of Applied Physics, Yale University, New Haven, Connecticut 06511 (United States); Department of Mechanical Engineering and Materials Science, Yale University, New Haven, Connecticut 06511 (United States)
2014-11-01
We present the growth and characterization of layered heterostructures comprised of LaTiO{sub 3} and SrTiO{sub 3} epitaxially grown on Si (001). Magnetotransport measurements show that the sheet carrier densities of the heterostructures scale with the number of LaTiO{sub 3}/SrTiO{sub 3} interfaces, consistent with the presence of an interfacial 2-dimensional electron gas (2DEG) at each interface. Sheet carrier densities of 8.9 × 10{sup 14} cm{sup −2} per interface are observed. Integration of such high density oxide 2DEGs on silicon provides a bridge between the exceptional properties and functionalities of oxide 2DEGs and microelectronic technologies.
Charging dynamics and strong localization of a two-dimensional electron cloud
International Nuclear Information System (INIS)
Dianoux, R; Smilde, H J H; Marchi, F; Buffet, N; Mur, P; Comin, F; Chevrier, J
2007-01-01
The dynamics of charge injection in silicon nanocrystals embedded in a silicon dioxide matrix is studied using electrostatic force microscopy. We show that the presence of silicon nanocrystals with a density of 10 11 cm -2 is essential for strong localization of charges, and results in exceptional charge retention properties compared to nanocrystal-free SiO 2 samples. In both systems, a logarithmic dependence of the diameter of the charged area on the injection time is experimentally observed on a timescale between 0.1 and 10 s (voltage≤10 V). A field-emission injection, limited by Coulomb blockade and a lateral charge spreading due to a repulsive radial electric field are used to model the sample charging. Once the tip is retracted, the electron cloud is strongly confined in the nanocrystals and remains static
Two-dimensional electron systems in functional oxides studied by photoemission spectroscopy
Rödel , Tobias
2016-01-01
Many transition metal oxides (TMOs) show complex physics, ranging from ferroelectricity to magnetism, high-Tc superconductivity and colossal magnetoresistance. The existence of a variety of ground states often occurs as different degrees of freedom (e.g. lattice, charge, spin, orbital) interact to form different competing phases which are quite similar in energy. The capability to epitaxially grow heterostructures of TMOs increased the complexity even more as new phenomena can emerge at the i...
Phosphorene oxide: stability and electronic properties of a novel two-dimensional material.
Wang, Gaoxue; Pandey, Ravindra; Karna, Shashi P
2015-01-14
Phosphorene, the monolayer form of (black) phosphorus, was recently exfoliated from its bulk counterpart. Phosphorene oxide, by analogy to graphene oxide, is expected to have novel chemical and electronic properties, and may provide an alternative route to the synthesis of phosphorene. In this research, the physical and chemical properties of phosphorene oxide including its formation by oxygen adsorption on the bare phosphorene was investigated. Analysis of the phonon dispersion curves finds stoichiometric and non-stoichiometric oxide configurations to be stable at ambient conditions, thus suggesting that the oxygen adsorption may not degrade the phosphorene. The nature of the band gap of the oxides depends on the degree of functionalization of phosphorene; an indirect gap is predicted for the non-stoichiometric configurations, whereas a direct gap is predicted for the stoichiometric oxide. Application of mechanical strain or an external electric field leads to tunability of the band gap of the phosphorene oxide. In contrast to the case of the bare phosphorene, dependence of the diode-like asymmetric current-voltage response on the degree of stoichiometry is predicted for the phosphorene oxide.
2012-01-01
unlike the GaAs/AlGaAs 2DES, the 3D n-GaAs epilayer, semiconducting Hg0.8Cd0.2Te, and some other systems. Further, we observe the transport data to follow...of τs represents the average lifetime of carriers in a quantum state. The Heisenberg uncertainty principal requires that ∆t∆E ∼ ~. Consequently, a...us consider the matrix form of eq. (2.27) in 3D , m τ eB 0 −eB m τ 0 0 0 m τ vx vy vz = −e E 0 0 . (2.28) 13
International Nuclear Information System (INIS)
Wang, C.M.; Pang, M.Q.; Liu, S.Y.; Lei, X.L.
2010-01-01
The current-induced spin polarization (CISP) is investigated in a combined Rashba-Dresselhaus spin-orbit-coupled two-dimensional electron gas, subjected to a homogeneous out-of-plane magnetization. It is found that, in addition to the usual collision-related in-plane parts of CISP, there are two impurity-density-free contributions, arising from intrinsic and disorder-mediated mechanisms. The intrinsic parts of spin polarization are related to the Berry curvature, analogous with the anomalous and spin Hall effects. For short-range collision, the disorder-mediated spin polarizations completely cancel the intrinsic ones and the total in-plane components of CISP equal those for systems without magnetization. However, for remote disorders, this cancellation does not occur and the total in-plane components of CISP strongly depend on the spin-orbit interaction coefficients and magnetization for both pure Rashba and combined Rashba-Dresselhaus models.
Ortiz, L.; Varona, S.; Viyuela, O.; Martin-Delgado, M. A.
2018-02-01
We study the localization and oscillation properties of the Majorana fermions that arise in a two-dimensional electron gas (2DEG) with spin-orbit coupling (SOC) and a Zeeman field coupled with a d -wave superconductor. Despite the angular dependence of the d -wave pairing, localization and oscillation properties are found to be similar to the ones seen in conventional s -wave superconductors. In addition, we study a microscopic lattice version of the previous system that can be characterized by a topological invariant. We derive its real space representation that involves nearest and next-to-nearest-neighbors pairing. Finally, we show that the emerging chiral Majorana fermions are indeed robust against static disorder. This analysis has potential applications to quantum simulations and experiments in high-Tc superconductors.
Equation of state for two-dimensional dusty plasma liquids and its applications
Feng, Yan
2017-10-01
Laboratory dusty plasma consists of free electrons, free ions, and micro-sized dust particles with thousands of negative elementary charges. Due to their extremely low charge-to-mass ratio, these dust particles are strongly coupled, arranging themselves like atoms in liquids or solids. Due to the shielding effects of electrons and ions, dust particles interact with each other through the Yukawa potential, so that simulations of Yukawa liquids or solids are used to study properties of dusty plasmas. In the past two decades, the properties of liquid 2D dusty plasmas have been widely studied from experiments to theories and simulations. However, from our literature search, we have not found a quantitative and comprehensive study of properties of 2D liquid dusty plasmas over a wide range of plasma conditions. Here, from molecular-dynamics simulations of Yukawa liquids, we have obtained a concise equation of state (EOS) for the 2D liquid dusty plasmas from empirical fitting, which contains three quantities of the internal pressure, the coupling parameter, and the screening parameter. From this EOS, different thermodynamical processes can be directly derived, such as isotherms, isobars and isochores. Also, various physical properties of 2D liquid dusty plasmas, like the bulk modulus of elasticity, can be analytically derived, so that the sound speeds can be obtained. Finally, an analytical expression of the specific heat for 2D liquid dusty plasmas has been achieved. Work supported by the National Natural Science Foundation of China under Grant No. 11505124, the 1000 Youth Talents Plan, and the startup funds from Soochow University.
Trends in data processing of comprehensive two-dimensional chromatography: state of the art.
Matos, João T V; Duarte, Regina M B O; Duarte, Armando C
2012-12-01
The operation of advanced chromatographic systems, namely comprehensive two-dimensional (2D) chromatography coupled to multidimensional detectors, allows achieving a great deal of data that need special care to be processed in order to characterize and quantify as much as possible the analytes under study. The aim of this review is to identify the main trends, research needs and gaps on the techniques for data processing of multidimensional data sets obtained from comprehensive 2D chromatography. The following topics have been identified as the most promising for new developments in the near future: data acquisition and handling, peak detection and quantification, measurement of overlapping of 2D peaks, and data analysis software for 2D chromatography. The rational supporting most of the data processing techniques is based on the generalization of one-dimensional (1D) chromatography although algorithms, such as the inverted watershed algorithm, use the 2D chromatographic data as such. However, for processing more complex N-way data there is a need for using more sophisticated techniques. Apart from using other concepts from 1D chromatography, which have not been tested for 2D chromatography, there is still room for new improvements and developments in algorithms and software for dealing with 2D comprehensive chromatographic data. Copyright © 2012 Elsevier B.V. All rights reserved.
Oh, J H; Lee, K-J; Lee, Hyun-Woo; Shin, M
2014-05-14
Starting with the indirect exchange model influenced by the Rashba and the Dresselhaus spin-orbit interactions, we derive the Dzyaloshinskii-Moriya interaction of localized spins. The strength of the Dzyaloshinskii-Moriya interaction is compared with that of the Heisenberg exchange term as a function of atomic distance. Using the calculated interaction strengths, we discuss the formation of various atomic ground states as a function of temperature and external magnetic field. By plotting the magnetic field-temperature phase diagram, we present approximate phase boundaries between the spiral, Skyrmion and ferromagnetic states of the two-dimensional weak ferromagnetic system.
International Nuclear Information System (INIS)
Oh, J H; Shin, M; Lee, K-J; Lee, Hyun-Woo
2014-01-01
Starting with the indirect exchange model influenced by the Rashba and the Dresselhaus spin–orbit interactions, we derive the Dzyaloshinskii–Moriya interaction of localized spins. The strength of the Dzyaloshinskii–Moriya interaction is compared with that of the Heisenberg exchange term as a function of atomic distance. Using the calculated interaction strengths, we discuss the formation of various atomic ground states as a function of temperature and external magnetic field. By plotting the magnetic field–temperature phase diagram, we present approximate phase boundaries between the spiral, Skyrmion and ferromagnetic states of the two-dimensional weak ferromagnetic system. (paper)
Nie, Y F; Di Sante, D; Chatterjee, S; King, P D C; Uchida, M; Ciuchi, S; Schlom, D G; Shen, K M
2015-08-28
We report the formation and observation of an electron liquid in Sr(2-x)La(x)TiO4, the quasi-two-dimensional counterpart of SrTiO3, through reactive molecular-beam epitaxy and in situ angle-resolved photoemission spectroscopy. The lowest lying states are found to be comprised of Ti 3d_{xy} orbitals, analogous to the LaAlO3/SrTiO3 interface and exhibit unusually broad features characterized by quantized energy levels and a reduced Luttinger volume. Using model calculations, we explain these characteristics through an interplay of disorder and electron-phonon coupling acting cooperatively at similar energy scales, which provides a possible mechanism for explaining the low free carrier concentrations observed at various oxide heterostructures such as the LaAlO3/SrTiO3 interface.
2015-08-16
Switchable Two-Dimensional Electron Gas at the Oxide Hetero-Interfaces by Using Electron Bean Inline Holography 5a. CONTRACT NUMBER FA2386-13-1-4136...directly imaged the charge carrier densities and spatial distributions at the (001) LaAlO3/SrTiO3 heterointerfaces by in-situ TEM holography . The new...Hetero-Interfaces by Using Electron Bean Inline Holography 5a. CONTRACT NUMBER FA2386-13-1-4136 5b. GRANT NUMBER 5c. PROGRAM ELEMENT NUMBER 61102F
International Nuclear Information System (INIS)
Hata, M.
2010-01-01
Complete text of publication follows. A cone-guided target is used in the Fast Ignition Realization Experiment project phase-I (FIREX-I) and optimization of its design is performed. However a laser profile is not optimized much, because the laser profile that is the best for core heating is not known well. To find that, it is useful to investigate characteristics of generated fast electrons in each condition of different laser profiles. In this research, effects of laser profiles on fast electron generation are investigated on somewhat simple conditions by two-dimensional Particle-In-Cell simulations. In these simulations, a target is made up of Au pre-plasma and Au plasma. The Au pre-plasma has the exponential profile in the x direction with the scale length L = 4.0 μm and the density from 0.10 n cr to 20 n cr . The Au plasma has the flat profile in the x direction with 10 μm width and 20 n cr . Plasma profiles are uniform in the y direction. The ionization degree and the mass number of plasmas are 40 and 197, where the ionization degree is determined by PINOCO simulations. PINOCO is a two-dimensional radiation hydrodynamics simulation code, which simulates formation of the high-density plasma during the compression phase in the fast ignition. A laser is assumed to propagate as plane wave from the negative x direction to the positive x direction. Laser profiles are supposed to be uniform in the y direction. Three different laser profiles, namely flat one with t flat = 100 fs, Gaussian one with t rise/fall = 47.0 fs and flat + Gaussian one with t rise/fall = 23.5 fs and t flat = 50 fs are used. The energy and the peak intensity are constant with E = 10 7 J/cm 2 and I L = 10 20 W/cm 2 in all cases of different laser profiles. We compare results in each condition of three different laser profiles and investigate effects of laser profiles on fast electron generation. Time-integrated energy spectra are similar in all cases of three different laser profiles. In the
Zhang, Qi; Gao, Weilu; Watson, John; Manfra, Michael; Kono, Junichiro
2015-03-01
Density-dependent Coulomb interactions can drive electron-hole (e - h) pairs in semiconductors through an excitonic Mott transition from an excitonic gas into an e - h plasma. Theoretical studies suggest that these interactions can be strongly modified by an external magnetic field, including the absence of inter-exciton interactions in the high magnetic field limit in two dimensions, due to an e - h charge symmetry, which results in ultrastable magneto-excitons. Here, we present a systematic experimental study of e - h pairs in photo-excited undoped GaAs quantum wells in magnetic fields with ultrafast terahertz spectroscopy. We simultaneously monitored the dynamics of the intraexcitonic 1 s-2 p transition (which splits into 1 s-2p+ and 1 s-2p- transitions in a magnetic field) and the cyclotron resonance of unbound electrons and holes up to 10 Tesla. We found that the 1 s-2p- absorption feature is robust at high magnetic fields even under high excitation fluences, indicating magnetically enhanced stability of excitons. We will discuss the Mott physics of magneto-excitons as a function of temperature, e - h pair density, optical pump delay time, as well as magnetic field, and also compare two-dimensional excitons in GaAs quantum wells with three-dimensional excitons in bulk GaAs.
Energy Technology Data Exchange (ETDEWEB)
Sharma, Munish, E-mail: munishsharmahpu@live.com, E-mail: pk-ahluwalia7@yahoo.com; Kumar, Ashok; Ahluwalia, P. K., E-mail: munishsharmahpu@live.com, E-mail: pk-ahluwalia7@yahoo.com [Department of Physics, Himachal Pradesh University, Shimla 171005 (India); Pandey, Ravindra [Department of Physics, Michigan Technological University, Houghton, Michigan 49931 (United States)
2014-08-14
Tunability of the electronic properties of two-dimensional bilayer hetero structures of transition-metal dichalcogenides (i.e., MX{sub 2}-M′X′{sub 2} with (M, M′ = Mo, W; X, X′ = S, Se) is investigated. Application of both strain and electric field is found to modify the band gap and carrier effective mass in the hybrid bilayers considered. The calculated results based on density functional theory suggest that the tensile strain considerably changes the band gap of semiconducting bilayers; it makes the band gap to be indirect, and later initiates the semiconductor-to-metal transition. Application of the external electric fields, on the other hand, shows asymmetric variation in the band gap leading to the closure of the gap at about 0.5–1.0 V/Å. Tuning of the band gap and carrier effective mass in such a controlled manner makes the hybrid bilayers of transition metal dichalcogenides to be promising candidates for application in electronic devices at nanoscale.
International Nuclear Information System (INIS)
Hrehor, M.
1979-01-01
The paper deals with an application of the finite element method to the heat transfer study in seven-pin models of LMFBR fuel subassembly. The developed code NCEL solves two-dimensional steady state heat conduction equation in the whole subassembly model cross-section and enebles to perform the analysis of thermal behaviour in both normal and accidental operational conditions as eccentricity of the central rod or full or partial (porous) blockage of some part of the cross-flow area. The heat removal is simulated by heat sinks in coolant under conditions of subchannels slug flow approximation
International Nuclear Information System (INIS)
Brasse, Matthias
2014-01-01
Torque magnetometry at low temperature is performed to investigate the magnetic properties of MnSi thin films, of a CrB 2 single crystal and of a two-dimensional electron system (2DESs) formed at the interface of MgZnO/ZnO. The magnetic anisotropy and phase diagram of MnSi as well as information on the electronic structure of CrB 2 are obtained. The MgZnO/ZnO 2DESs exhibits the de Haas-van Alphen effect and non-equilibrium currents which are analyzed in order to determine ground state properties and excited states, respectively.
Directory of Open Access Journals (Sweden)
Jun Takeda
2010-04-01
Full Text Available In this review, we demonstrate a real-time time-frequency two-dimensional (2D pump-probe imaging spectroscopy implemented on a single shot basis applicable to excited-state dynamics in solid-state organic and biological materials. Using this technique, we could successfully map ultrafast time-frequency 2D transient absorption signals of β-carotene in solid films with wide temporal and spectral ranges having very short accumulation time of 20 ms per unit frame. The results obtained indicate the high potential of this technique as a powerful and unique spectroscopic tool to observe ultrafast excited-state dynamics of organic and biological materials in solid-state, which undergo rapid photodegradation.
Choi, Tae-Hoon; Huh, Jae-Won; Woo, Jae-Hyeon; Kim, Jin-Hun; Jo, Young-Seo; Yoon, Tae-Hoon
2017-05-15
We report an electrically-switchable two-dimensional liquid crystal (LC) phase grating device for window display applications. The device consists of the top and bottom substrates with crossed interdigitated electrodes and vertically-aligned LCs sandwiched between the two substrates. The device, switchable between the transparent and translucent states by applying an electric field, can provide high haze by the strong diffraction effect thanks to a large spatial phase difference with little dependence on the azimuth angle. We found that the device has outstanding features, such as a low operating voltage, high transparency, and wide viewing angle characteristics in the transparent state and high haze in the translucent state. Moreover, we achieved submillisecond switching between transparent and translucent states by employing the overdrive scheme and a vertical trigger pulse.
International Nuclear Information System (INIS)
Charleston, B.D.; Beckman, F.H.; Franco, M.J.; Charleston, D.B.
1981-01-01
A versatile electronic-analogue image processing system has been developed for use in improving the quality of various types of images with emphasis on those encountered in experimental and diagnostic medicine. The operational principle utilizes spatial filtering which selectively controls the contrast of an image according to the spatial frequency content of relevant and non-relevant features of the image. Noise can be reduced or eliminated by selectively lowering the contrast of information in the high spatial frequency range. Edge sharpness can be enhanced by accentuating the upper midrange spatial frequencies. Both methods of spatial frequency control may be adjusted continuously in the same image to obtain maximum visibility of the features of interest. A precision video camera is used to view medical diagnostic images, either prints, transparencies or CRT displays. The output of the camera provides the analogue input signal for both the electronic processing system and the video display of the unprocessed image. The video signal input to the electronic processing system is processed by a two-dimensional spatial convolution operation. The system employs charged-coupled devices (CCDs), both tapped analogue delay lines (TADs) and serial analogue delay lines (SADs), to store information in the form of analogue potentials which are constantly being updated as new sampled analogue data arrive at the input. This information is convolved with a programmed bipolar radially symmetrical hexagonal function which may be controlled and varied at each radius by the operator in real-time by adjusting a set of front panel controls or by a programmed microprocessor control. Two TV monitors are used, one for processed image display and the other for constant reference to the original image. The working prototype has a full-screen display matrix size of 200 picture elements per horizontal line by 240 lines. The matrix can be expanded vertically and horizontally for the
Rizo, P. J.; Pugzlys, A.; Slachter, A.; Denega, S. Z.; Reuter, D.; Wieck, A. D.; van Loosdrecht, P. H. M.; van der Wal, C. H.
2010-01-01
The electron spin dynamics in a GaAs/AlGaAs heterojunction system containing a high-mobility two-dimensional electron gas (2DEG) have been studied in this paper by using pump-probe time-resolved Kerr rotation experiments. Owing to the complex layer structure of this material, the transient Kerr
Ab initio electronic transport study of two-dimensional silicon carbide-based p-n junctions
Zhou, Hanming; Lin, Xiao; Guo, Hongwei; Lin, Shisheng; Sun, Yiwei; Xu, Yang
2017-03-01
Two-dimensional silicon carbide (2d-SiC) is a viable material for next generation electronics due to its moderate, direct bandgap with huge potential. In particular, its potential for p-n junctions is yet to be explored. In this paper, three types of 2d-SiC-based p-n junctions with different doping configuration are modeled. The doping configurations refer to partially replacing carbon with boron or nitrogen atoms along the zigzag or armchair direction, respectively. By employing density functional theory, we calculate the transport properties of the SiC based p-n junctions and obtain negative differential resistance and high rectification ratio. We also find that the junction along the zigzag direction with lower doping density exhibits optimized rectification performance. Our study suggests that 2d-SiC is a promising candidate as a material platform for future nano-devices. Project supported by the National Science Foundation of China (Nos. 61474099, 61674127) and the ZJ-NSF (No. Z17F04003).
Kah, Cherno Baba; Yu, M.; Jayanthi, C. S.; Wu, S. Y.
2014-03-01
Our previous study on one-dimensional icosahedral B12 cluster (α-B12) based chain [Bulletin of APS Annual Meeting, p265 (2013)] and ring structures has prompted us to study the two-dimensional (2D) α-B12 based structures. Recently, we have carried out a systematic molecular dynamics study on the structural stabilities and electronic properties of the 2D α-B12 based structures using the SCED-LCAO method [PRB 74, 15540 (2006)]. We have considered several types of symmetry for these 2D structures such as δ3, δ4, δ6 (flat triangular), and α' types. We have found that the optimized structures are energetically in the order of δ6 < α' < δ3 < δ4 which is different from the energy order of α'< δ6 < δ4 < δ3 found in the 2D boron monolayer sheets [ACS Nano 6, 7443 (2012)]. A detailed discussion of this study will be presented. The first author acknowledges the McSweeny Fellowship for supporting his research in this work.
International Nuclear Information System (INIS)
Lungu, R. P.
2002-01-01
A fermion 2-dimensional interacting system that is coupled with an external classical field having a time periodic dependence is considered. In the absence of the external field, the single-particle Hamiltonian is quadratic and linear with respect to the canonical operators and the particles have static, scalar, two-body self-interactions; in addition, each particle interacts with an external classical field and the coupling functions with the canonical operators (both the momenta and the position coordinates) are time periodic. This model is a generalization of the two-dimensional electron gas in the presence of a monochromatic linear or circular polarized electromagnetic field. Using the Second Quantization version of the Floquet formalism, we obtain the solution of the eigenvalue problem for the Floquet Hamiltonian with the time-reducing transformation method. we construct an unitary transform that produces a transformed Floquet Hamiltonian that is not time dependent; then, the transformed eigenvalue equation can be resolved and this solution is closely related to the solution of the energy eigenvalue equation of the same system in the absence of the external field. This solution of the Floquet problem has the following important consequences: - Green functions and the correlation density functions of this system are related to the corresponding quantities of the conservative system, so it is possible to develop a diagrammatic method for the perturbed evaluation of these quantities in a similar manner to the conservative situation; - when the system is invariant with respect to space translations in the absence of the external field, the diagrammatic analysis can be performed using a space-time Fourier transform, and this property leads to great simplifications and close correspondences to the conservative theory; - it is possible to construct a result similar to the Pauli theorem, i.e. the quasi-energy eigenvalue of the interacting system (when the classical
DEFF Research Database (Denmark)
Rudner, Mark Spencer; Lindner, Netanel; Berg, Erez
2013-01-01
revealed phenomena that cannot be characterized by analogy to the topological classification framework for static systems. In particular, in driven systems in two dimensions (2D), robust chiral edge states can appear even though the Chern numbers of all the bulk Floquet bands are zero. Here, we elucidate...... the crucial distinctions between static and driven 2D systems, and construct a new topological invariant that yields the correct edge-state structure in the driven case. We provide formulations in both the time and frequency domains, which afford additional insight into the origins of the “anomalous” spectra...... that arise in driven systems. Possibilities for realizing these phenomena in solid-state and cold-atomic systems are discussed....
Two-dimensional systems from introduction to state of the art
Benzaouia, Abdellah; Tadeo, Fernando
2016-01-01
A solution permitting the stabilization of 2-dimensional (2-D) continuous-time saturated system under state feedback control is presented in this book. The problems of delay and saturation are treated at the same time. The authors obtain novel results on continuous 2-D systems using the unidirectional Lyapunov function. The control synthesis and the saturation and delay conditions are presented as linear matrix inequalities. Illustrative examples are worked through to show the effectiveness of the approach and many comparisons are made with existing results. The second half of the book moves on to consider robust stabilization and filtering of 2-D systems with particular consideration being given to 2-D fuzzy systems. Solutions for the filter-design problems are demonstrated by computer simulation. The text builds up to the development of state feedback control for 2-D Takagi–Sugeno systems with stochastic perturbation. Conservatism is reduced by using slack matrices and the coupling between the Lyapunov ma...
Quasi-two-dimensional quantum states of H2 in stage-2 Rb-intercalated graphite
International Nuclear Information System (INIS)
Smith, A.P.; Benedek, R.; Trouw, F.R.; Minkoff, M.; Yang, L.H.
1995-01-01
Inelastic-incoherent-neutron scattering can be a valuable nanostructural probe of H 2 -doped porous materials, provided the spectral peaks can be interpreted in terms of crystal-field-split hydrogen-molecule energy levels, which represent a signature of the local symmetry. Inelastic-neutron-scattering measurements as well as extensive theoretical analyses have been performed on stage-2 Rb-intercalated graphite (Rb-GIC), with physisorbed H 2 , HD, and D 2 , a layered porous system with abundant spectral peaks, to assess whether the crystal-field-state picture enables a quantitative understanding of the observed structure. Potential-energy surfaces for molecular rotational and translational motion, as well as the intermolecular interactions of hydrogen molecules in Rb-GIC, were calculated within local-density-functional theory (LDFT). Model potentials, parameterized using results of the LDFT calculations, were employed in schematic calculations of rotational and translational excited state spectra of a single physisorbed H 2 molecule in Rb-GIC. Results of the analysis are basically consistent with the assignment by Stead et al. of the lowest-lying peak at 1.4 meV to a rotational-tunneling transition of an isotropic hindered-rotor oriented normal to the planes, but indicate a small azimuthal anisotropy and a lower barrier than for the isotropic case. Based on the experimental isotope shifts and the theoretically predicted states, they conclude that spectral peaks at 11 and 22 meV are most likely related to center of mass excitations
User's manual for EVITS: a steady state fluids code for complex two-dimensional geometries
International Nuclear Information System (INIS)
Domanus, H.M.
1976-07-01
A 2-D computer code, EVITS, has been developed for estimating steady state, incompressible, isothermal flow fields in complex geometries. A vorticity-stream function formulation is used along with a model to resolve viscous effects at solid boundaries. Sufficient geometry and boundary type options are included within the code so that a large number of flow situations can be specified without modifying the program. All instructions to the code are via an input dataset. Detailed instructions for preparing the user oriented input, along with examples, are included in this users' manual
Energy Technology Data Exchange (ETDEWEB)
Department of Chemistry, The University of Chicago; Department of Biology, Department of Chemistry, Washington University; Fleming, Graham; Read, Elizabeth L.; Schlau-Cohen, Gabriela S.; Engel, Gregory S.; Wen, Jianzhong; Blankenship, Robert E.; Fleming, Graham R.
2008-05-26
Photosynthetic light-harvesting proceeds by the collection and highly efficient transfer of energy through a network of pigment-protein complexes. Inter-chromophore electronic couplings and interactions between pigments and the surrounding protein determine energy levels of excitonic states and dictate the mechanism of energy flow. The excitonic structure (orientation of excitonic transition dipoles) of pigment-protein complexes is generally deduced indirectly from x-ray crystallography in combination with predictions of transition energies and couplings in the chromophore site basis. Here, we demonstrate that coarse-grained excitonic structural information in the form of projection angles between transition dipole moments can be obtained from polarization-dependent two-dimensional electronic spectroscopy of an isotropic sample, particularly when the nonrephasing or free polarization decay signal rather than the photon echo signal is considered. The method provides an experimental link between atomic and electronic structure and accesses dynamical information with femtosecond time resolution. In an investigation of the Fenna-Matthews-Olson complex from green sulfur bacteria, energy transfer connecting two particular exciton states in the protein is isolated as being the primary contributor to a cross peak in the nonrephasing 2D spectrum at 400 fs under a specific sequence of polarized excitation pulses. The results suggest the possibility of designing experiments using combinations of tailored polarization sequencesto separate and monitor individual relaxation pathways.
International Nuclear Information System (INIS)
Jost, G.; Tran, T.M.; Appert, K.; Wuethrich, S.
1996-12-01
A two-dimensional PIC code aimed at the investigation of electron-cyclotron beam instabilities in gyrotrons and their effects on the beam quality is presented. The code is based on recently developed techniques for handling charge conservation and open boundaries and uses an electromagnetic field which is decomposed in its transverse magnetic (TM) and electric (TE) components. The code has been implemented on the massively parallel computer CRAY T3D, and on the CRAY Y-MP. (author) figs., tabs., refs
Two-dimensional solid-state NMR reveals two topologies of sarcolipin in oriented lipid bilayers.
Buffy, Jarrod J; Traaseth, Nathaniel J; Mascioni, Alessandro; Gor'kov, Peter L; Chekmenev, Eduard Y; Brey, William W; Veglia, Gianluigi
2006-09-12
Sarcolipin (SLN), a 31 amino acid integral membrane protein, regulates SERCA1a and SERCA2a, two isoforms of the sarco(endo)plasmic Ca-ATPase, by lowering their apparent Ca(2+) affinity and thereby enabling muscle relaxation. SLN is expressed in both fast-twitch and slow-twitch muscle fibers with significant expression levels also found in the cardiac muscle. SLN shares approximately 30% identity with the transmembrane domain of phospholamban (PLN), and recent solution NMR studies carried out in detergent micelles indicate that the two polypeptides bind to SERCA in a similar manner. Previous 1D solid-state NMR experiments on selectively (15)N-labeled sites showed that SLN crosses the lipid bilayer with an orientation nearly parallel to the bilayer normal. With a view toward the characterization of SLN structure and its interactions with both lipids and SERCA, herein we report our initial structural and topological assignments of SLN in mechanically oriented DOPC/DOPE lipid bilayers as mapped by 2D (15)N PISEMA experiments. The PISEMA spectra obtained on uniformly (15)N-labeled protein as well as (15)N-Leu, (15)N-Ile and (15)N-Val map the secondary structure of SLN and, simultaneously, reveal that SLN exists in two distinct topologies. Both the major and the minor populations assume an orientation with the helix axis tilted by approximately 23 degrees with respect to the lipid bilayer normal, but vary in the rotation angle about the helix axis by approximately 5 degrees . The existence of the multiple populations in model membranes may be a significant requirement for SLN interaction with SERCA.
AlGaAs/GaAs two-dimensional electron gas structures studied by photo reflectance spectroscopy
Energy Technology Data Exchange (ETDEWEB)
Guillen Cervantes, A; Rivera Alvarez, Z; Hernandez, F; Huerta, J. [Instituto Politecnico Nacional, Mexico, D.F. (Mexico); Mendez Garcia, V. H.; Lastras Martinez, A.; Zamora, L.; Saucedo, N. [Universidad Autonoma de San Luis Potosi, San Luis Potosi (Mexico); Melendez Lira, M; Lopez, M [Instituto Politecnico Nacional, Mexico, D.F. (Mexico)
2001-12-01
Al{sub x} Ga{sub 1}-x As/GaAs two-dimensional electron gas (2-DEG) heterostructures were fabricated by molecular beam epitaxy in three different laboratories. The samples were characterized by room temperature Photo reflectance (PR) spectroscopy and measurements at 77 K. Internal electric fields were detected by the presence of Franz-Keldysh (FK) oscillations in the PR spectra. >From a FK analysis we obtained the GaAs band-gap energy and the built-in electric field strength in each sample. On the other hand, in the energy region corresponding to Al{sub x} Ga{sub 1}-x As a broad PR signal was registered typical of a highly doped material. Using the third derivative theory we obtained the Al{sub x} Ga{sub 1}-x As band-gap energy, and from this value the Al concentration in the samples. Results showed that the sample with highest electron mobility exhibited the lowest internal electric field strength. [Spanish] Se fabricaron heteroestructuras del tipo Al{sub x} Ga{sub 1}-x As/GaAs con un gas de electrones en dos dimensiones por medio de epitaxia de haces moleculares en tres laboratorios diferentes. Las muestras se caracterizaron por fotorreflectancia (FR) a temperatura ambiente y por mediciones del efecto mayor a 77 K. Campos electricos internos se detectaron por la presencia de oscilaciones Franz-Leldysh (FK) en los espectros de FR. Del analisis de las oscilaciones FK obtuvimos la energia de la brecha prohibida del GaAs y la intensidad del campo electrico interno en cada muestra. Por otra parte, en la region de energia correspondiente al Al{sub x} Ga{sub 1}-x As observamos una senal de FR ancha, tipica de un material altamente impurificado. Usando la teoria de la tercera derivada, obtuvimos el valor de la brecha de energia del Al{sub x}Ga{sub 1}-xAs, y de este valor la concentracion de Al en las muestras. Los resultados mostraron que la estructura con el valor de movilidad electronica mas alto tiene la intensidad de campo electrico interno mas baja.
Oh, Ji Seop; Kang, Chang-Jong; Kim, Ye Ji; Sinn, Soobin; Han, Moonsup; Chang, Young Jun; Park, Byeong-Gyu; Kim, Sung Wng; Min, Byung Il; Kim, Hyeong-Do; Noh, Tae Won
2016-03-02
Angle-resolved photoemission spectroscopy (ARPES) study of a layered electride Ca2N was carried out to reveal its quasi-two-dimensional electronic structure. The band dispersions and the Fermi-surface map are consistent with the density functional theory results except for a chemical potential shift that may originate from the high reactivity of surface excess electrons. Thus, the existence of anionic excess electrons in the interlayer region of Ca2N is strongly supported by ARPES.
Korytar, P.; Parera, J.; Leonards, P.E.G.; Santos, F.J.; Boer, de J.; Brinkman, U.A.Th.
2005-01-01
Comprehensive two-dimensional gas chromatography with electron-capture negative ionization time-of-flight mass spectrometry (GC × GC¿ECNI-TOF-MS) is used to study the composition and characteristics of short-, medium- and long-chain polychlorinated n-alkane (PCA) mixtures. Distinct ordered
International Nuclear Information System (INIS)
Kondoh, Yoshiomi; Serizawa, Shunsuke; Nakano, Akihiro; Takahashi, Toshiki; Van Dam, James W.
2004-01-01
The final self-similar state of decaying two-dimensional (2D) turbulence in 2D incompressible viscous flow is analytically and numerically investigated for the case with periodic boundaries. It is proved by theoretical analysis and simulations that the sinh-Poisson state cω=-sinh(βψ) is not realized in the dynamical system of interest. It is shown by an eigenfunction spectrum analysis that a sufficient explanation for the self-organization to the decaying self-similar state is the faster energy decay of higher eigenmodes and the energy accumulation to the lowest eigenmode for given boundary conditions due to simultaneous normal and inverse cascading by nonlinear mode couplings. The theoretical prediction is demonstrated to be correct by simulations leading to the lowest eigenmode of {(1,0)+(0,1)} of the dissipative operator for the periodic boundaries. It is also clarified that an important process during nonlinear self-organization is an interchange between the dominant operators, which leads to the final decaying self-similar state
Nature of the Insulating Ground State of the Two-Dimensional Sn Atom Lattice on SiC(0001).
Yi, Seho; Lee, Hunpyo; Choi, Jin-Ho; Cho, Jun-Hyung
2016-07-28
Semiconductor surfaces with narrow surface bands provide unique playgrounds to search for Mott-insulating state. Recently, a combined experimental and theoretical study of the two-dimensional (2D) Sn atom lattice on a wide-gap SiC(0001) substrate proposed a Mott-type insulator driven by strong on-site Coulomb repulsion U within a single-band Hubbard model. However, our systematic density-functional theory (DFT) study with local, semilocal, and hybrid exchange-correlation functionals shows that the Sn dangling-bond state largely hybridizes with the substrate Si 3p and C 2p states to split into three surface bands due to the crystal field. Such a hybridization gives rise to the stabilization of the antiferromagnetic order via superexchange interactions. The band gap and the density of states predicted by the hybrid DFT calculation agree well with photoemission data. Our findings not only suggest that the Sn/SiC(0001) system can be represented as a Slater-type insulator driven by long-range magnetism, but also have an implication that taking into account long-range interactions beyond the on-site interaction would be of importance for properly describing the insulating nature of Sn/SiC(0001).
International Nuclear Information System (INIS)
Zaluzec, N.J.
1988-08-01
Parallel detection systems for spectroscopy have generally been based upon linear detector arrays. Replacing the linear arrays with two dimensional systems yields more complicated devices; however, there are corresponding benefits which can be realized for both x-ray and electron energy loss spectroscopy. The operational design of these systems, as well as preliminary results from the construction of such a device used for electron spectroscopy, are presented. 10 refs., 8 figs
Directory of Open Access Journals (Sweden)
Jun Liu
2015-04-01
Full Text Available With the continuing growth of highway construction and vehicle use expansion all over the world, highway vehicle traffic rule violation (TRV detection has become more and more important so as to avoid traffic accidents and injuries in intelligent transportation systems (ITS and vehicular ad hoc networks (VANETs. Since very few works have contributed to solve the TRV detection problem by moving vehicle measurements and surveillance devices, this paper develops a novel parallel ultrasonic sensor system that can be used to identify the TRV behavior of a host vehicle in real-time. Then a two-dimensional state method is proposed, utilizing the spacial state and time sequential states from the data of two parallel ultrasonic sensors to detect and count the highway vehicle violations. Finally, the theoretical TRV identification probability is analyzed, and actual experiments are conducted on different highway segments with various driving speeds, which indicates that the identification accuracy of the proposed method can reach about 90.97%.
Xiang-bo, Yang; You-yan, Liu
1995-07-01
After establishing the method of constructing a class of two-dimensional Fibonacci quasilattices, by means of a decomposition-decimation method based on the renormalization-group technique, we have studied the rules of energy spectrum splitting for the two-dimensional Fibonacci quasilattices in the framework of single-electron tight-binding on-site model. Analytic results show that there are only six kinds of clusters and the electronic energy band consists of nine subbands. For the higher hierarchy of the spectrum, instead of the on-site model, the transfer model should be used, the electronic energy spectra split as type F. The analytic results are confirmed by numerical simulations.
Energy Technology Data Exchange (ETDEWEB)
Dasgupta, Shivaji
2009-02-15
In this work two-dimensional electron systems (2DESs) based on AlAs/AlGaAs heterostructures doped with Si are investigated. The electrons are confined in AlAs quantum wells (QWs) sandwiched between AlGaAs buffers. Analytical calculations and simulations for AlAs QWs are presented in the first chapter. The results show a cross-over width, above which the wide (001)-oriented QWs show double valley occupancy and wide (110)-oriented QWs show single valley occupancy. We solve the Schroedinger equation analytically for anisotropic masses. The solution shows the orientation dependence of the elliptical cyclotron orbit due to the anisotropic mass. We also present an introduction to the Landau level crossings based on g{sup *}m{sup *} product. In the next chapter, we present experimental results for the double-valley (001)-oriented AlAs QWs. We present the different structures of the deep AlAs QWs along with the low temperature magnetotransport data for these QWs. Thereafter, we present the results on shallow AlAs QWs. We achieved a mobility of 4.2 x 10{sup 5} cm{sup 2}/Vs at 330 mK for the deep backside doped AlAs QW. For the shallow QWs, we achieved a mobility of2.3 x 10{sup 5} cm{sup 2}/Vs at 330 mK, for a density of 2.9 x 10{sup 11} cm{sup -2}. From the magneto-transport data, we see evidence of the double-valley occupation for the (001)-oriented AlAs wide QWs. In the next chapter, we present experimental results for the single-valley (110)-oriented AlAs QWs. We deduced the donor binding energy and the doping efficiency for this facet from a doping series of double-sided doped QWs. Thereafter, we designed different structures for the (110)-oriented AlAs QWs, which we present along with their respective low temperature magneto-transport data. We measured one of the double-sided doped AlAs QWs at very high magnetic fields and low temperatures, down to 60 mK. At the end of the chapter, we present a spike feature observed in the magneto-transport data of these QWs. This
Rapaport, R; Chen, Gang; Snoke, D; Simon, Steven H; Pfeiffer, Loren; West, Ken; Liu, Y; Denev, S
2004-03-19
We report on new experiments and theory that unambiguously resolve the recent puzzling observation of large diameter exciton emission halos around a laser excitation spot in two dimensional systems. We find a novel separation of plasmas of opposite charge with emission from the sharp circular boundary between these two regions. This charge separation allows for cooling of initially hot optically generated carriers as they dwell in the charge reservoirs for very long times.
Membrane-bound state of the colicin E1 channel domain as an extended two-dimensional helical array.
Zakharov, S D; Lindeberg, M; Griko, Y; Salamon, Z; Tollin, G; Prendergast, F G; Cramer, W A
1998-04-14
Atomic level structures have been determined for the soluble forms of several colicins and toxins, but the structural changes that occur after membrane binding have not been well characterized. Changes occurring in the transition from the soluble to membrane-bound state of the C-terminal 190-residue channel polypeptide of colicin E1 (P190) bound to anionic membranes are described. In the membrane-bound state, the alpha-helical content increases from 60-64% to 80-90%, with a concomitant increase in the average length of the helical segments from 12 to 16 or 17 residues, close to the length required to span the membrane bilayer in the open channel state. The average distance between helical segments is increased and interhelix interactions are weakened, as shown by a major loss of tertiary structure interactions, decreased efficiency of fluorescence resonance energy transfer from an energy donor on helix V of P190 to an acceptor on helix IX, and decreased resonance energy transfer at higher temperatures, not observed in soluble P190, implying freedom of motion of helical segments. Weaker interactions are also shown by a calorimetric thermal transition of low cooperativity, and the extended nature of the helical array is shown by a 3- to 4-fold increase in the average area subtended per molecule to 4,200 A2 on the membrane surface. The latter, with analysis of the heat capacity changes, implies the absence of a developed hydrophobic core in the membrane-bound P190. The membrane interfacial layer thus serves to promote formation of a highly helical extended two-dimensional flexible net. The properties of the membrane-bound state of the colicin channel domain (i.e., hydrophobic anchor, lengthened and loosely coupled alpha-helices, and close association with the membrane interfacial layer) are plausible structural features for the state that is a prerequisite for voltage gating, formation of transmembrane helices, and channel opening.
Yang, Xiangbo; Xing, Da
2002-04-01
On the basis of the substitution rules for a one-dimensional Fibonacci-class chain, we construct two-dimensional Fibonacci-class quasicrystals with one kind of atom and two bond lengths. In the framework of the single-electron tight-binding nearest-interaction transfer model, we study the splitting rules of the electronic energy spectra for two-dimensional Fibonacci-class quasicrystals by means of a decomposition-decimation method based on a renormalization-group technique, and we also calculate the electronic energy spectra numerically. It is found that there exist only three kinds of clusters-n×n, n×(n+1), and (n+1)×(n+1)-for all classes of two-dimensional quasilattices, and that the electronic energy bands split as Ym-n-l. The general formula of the number for energy levels is obtained. We discover that there is a kind of so-called Fibonacci-class-number set for the parameters used to describe the energy-level number, and we obtain the set formulas. The experienced formula are sought out. The analytical results are confirmed by numerical simulations.
One- and two-dimensional search of an equation of state using a newly released 2DRoptimize package
Jamal, M.; Reshak, A. H.
2018-05-01
A new package called 2DRoptimize has been released for performing two-dimensional searches of the equation of state (EOS) for rhombohedral, tetragonal, and hexagonal compounds. The package is compatible and available with the WIEN2k package. The 2DRoptimize package performs a convenient volume and c/a structure optimization. First, the package finds the best value for c/a and the associated energy for each volume. In the second step, it calculates the EoS. The package then finds the equation of the c/a ratio vs. volume to calculate the c/a ratio at the optimized volume. In the last stage, by using the optimized volume and c/a ratio, the 2DRoptimize package calculates a and c lattice constants for tetragonal and hexagonal compounds, as well as the a lattice constant with the α angle for rhombohedral compounds. We tested our new package based on several hexagonal, tetragonal, and rhombohedral structures, and the 2D search results for the EOS showed that this method is more accurate than 1D search. Our results agreed very well with the experimental data and they were better than previous theoretical calculations.
Directory of Open Access Journals (Sweden)
Daigo Ohki
2018-03-01
Full Text Available The optical conductivity in the charge order phase is calculated in the two-dimensional extended Hubbard model describing an organic Dirac electron system α -(BEDT-TTF 2 I 3 using the mean field theory and the Nakano-Kubo formula. Because the interband excitation is characteristic in a two-dimensional Dirac electron system, a peak structure is found above the charge order gap. It is shown that the peak structure originates from the Van Hove singularities of the conduction and valence bands, where those singularities are located at a saddle point between two Dirac cones in momentum space. The frequency of the peak structure exhibits drastic change in the vicinity of the charge order transition.
Dressed-state analysis of efficient two-dimensional atom localization in a four-level atomic system
International Nuclear Information System (INIS)
Wang, Zhiping; Yu, Benli
2014-01-01
We investigate two-dimensional atom localization via spontaneous emission in a four-level atomic system. It is found that the detection probability and precision of two-dimensional atom localization can be significantly improved due to the interference effect between the spontaneous decay channels and the dynamically induced quantum interference generated by the probe and composite fields. More importantly, a 100% probability of finding an atom within the sub-half-wavelength domain of the standing waves can be reached when the corresponding conditions are satisfied. As a result, our scheme may be helpful in laser cooling or atom nano-lithography via atom localization. (paper)
Waddell, R.K.
1982-01-01
A two-dimensional, steady-state model of ground-water flow beneath the Nevada Test Site and vicinity has been developed using inverse techniques. The area is underlain by clastic and carbonate rocks of Precambrian and Paleozoic age and by volcanic rocks and alluvium of Tertiary and Quaternary age that have been juxtaposed by normal and strike-slip faulting. Aquifers are composed of carbonate and volcanic rocks and alluvium. Characteristics of the flow system are determined by distribution of low-conductivity rocks (barriers); by recharge originating in the Spring Mountains, Pahranagat, Timpahute, and Sheep Ranges, and in Pahute Mesa; and by underflow beneath Pahute Mesa from Gold Flat and Kawich Valley. Discharge areas (Ash Meadows, Oasis Valley, Alkali Flat, and Furnace Creek Ranch) are upgradient from barriers. Sensitivities of simulated hydraulic heads and fluxes to variations in model parameters were calculated to guide field studies and to help estimate errors in predictions from transport modeling. Hydraulic heads and fluxes are very sensitive to variations in the greater magnitude recharge/discharge terms. Transmissivity at a location may not be the most important transmissivity for determining flux there. Transmissivities and geometries of large barriers that impede flow from Pahute Mesa have major effects on fluxes elsewhere; as their transmissivities are decreased, flux beneath western Jackass Flats and Yucca Mountains is increased as water is diverted around the barriers. Fortymile Canyon is underlain by highly transmissive rocks that cause potentiometric contours to vee upgradient; increasing their transmissivity increases flow through them, and decreases it beneath Yucca Mountain. (USGS)
Energy Technology Data Exchange (ETDEWEB)
Wadsworth, D.C.; Mudawar, I. (Purdue Univ., West Layfayette, IN (USA))
1990-11-01
Experiments were performed to investigate single-phase heat transfer froma smooth 12.7 {times} 12.7 mm{sup 2} simulated chip to a two-dimensional jet of dielectric Fluorinert FC-72 liquid issuing from a thin rectangular slot into a channel confined between the chip surface and nozzle plate. The effects of jet width, confined channel height, and impingement velocity have been examined. Channel height had a negligible effect ont eh theat transfer performance of the jet for the conditions of the present study. A correlation for the convective heat transfer coefficient is presented as a function of jet, width, heat length, flow velocity, and fluid properties. A self-contained multichip cooling module consisting of a 3 {times} 3 array of heat sources confirmed the uniformity and predictability of cooling for each of the nine chips, and proved the cooling module is well suited for packaging large arrays of high-power density chips.
International Nuclear Information System (INIS)
Anon.
1991-01-01
This chapter addresses the extension of previous work in one-dimensional (linear) error theory to two-dimensional error analysis. The topics of the chapter include the definition of two-dimensional error, the probability ellipse, the probability circle, elliptical (circular) error evaluation, the application to position accuracy, and the use of control systems (points) in measurements
International Nuclear Information System (INIS)
Jin, Dong-Dong; Wang, Lian-shan; Yang, Shao-Yan; Li, Hui-jie; Zhang, Heng; Wang, Jian-xia; Xiang, Ruo-fei; Wei, Hong-yuan; Jiao, Chun-mei; Liu, Xiang-Lin; Zhu, Qin-Sheng; Wang, Zhan-Guo; Zhang, Liu-Wan
2014-01-01
In this paper, a theory is developed to study the anisotropic scattering effect of the inclined misfit dislocation on the two-dimensional electron gas in Al(In)GaN/GaN heterostructures. The inclined misfit dislocation, which differs from the well-known vertical threading dislocation, has a remarkable tilt angle from the vertical. The predicted electron mobility shows a remarkable anisotropy. It has a maximum mobility value along the direction perpendicular to the projection of the inclined dislocation line, and a minimum mobility value along the direction parallel to the projection. The degree of the anisotropic scattering effect will be even greater with the increase of the tilt angle
Quantum melting of a two-dimensional Wigner crystal
Dolgopolov, V. T.
2017-10-01
The paper reviews theoretical predictions about the behavior of two-dimensional low-density electron systems at nearly absolute zero temperatures, including the formation of an electron (Wigner) crystal, crystal melting at a critical electron density, and transitions between crystal modifications in more complex (for example, two-layer) systems. The paper presents experimental results obtained from real two-dimensional systems in which the nonconducting (solid) state of the electronic system with indications of collective localization is actually realized. Experimental methods for detecting a quantum liquid–solid phase interface are discussed.
Fullam, Jennifer; Boye, Carol; Standaert, Theodorus; Gaudiello, John; Tomlinson, Derek; Xiao, Hong; Fang, Wei; Zhang, Xu; Wang, Fei; Ma, Long; Zhao, Yan; Jau, Jack
2011-03-01
In this paper, we tested a novel methodology of measuring critical dimension (CD) uniformity, or CDU, with electron beam (e-beam) hotspot inspection and measurement systems developed by Hermes Microvision, Inc. (HMI). The systems were used to take images of two-dimensional (2D) array patterns and measure CDU values in a custom designated fashion. Because this methodology combined imaging of scanning micro scope (SEM) and CD value averaging over a large array pattern of optical CD, or OCD, it can measure CDU of 2D arrays with high accuracy, high repeatability and high throughput.
Suppression of the two-dimensional electron gas in LaGaO3/SrTiO3 by cation intermixing
Nazir, S.
2013-12-03
Cation intermixing at the n-type polar LaGaO 3 /SrTiO 3 (001) interface is investigated by first principles calculations. Ti"Ga, Sr"La, and SrTi"LaGa intermixing are studied in comparison to each other, with a focus on the interface stability. We demonstrate in which cases intermixing is energetically favorable as compared to a clean interface. A depopulation of the Ti 3d xy orbitals under cation intermixing is found, reflecting a complete suppression of the two-dimensional electron gas present at the clean interface.
Magnetic two-dimensional electron gas at the manganite-buffered LaAlO3/SrTiO3 interface
DEFF Research Database (Denmark)
R. Zhang, H.; Zhang, Y.; Zhang, H.
2017-01-01
Fabrication of highly mobile spin-polarized two-dimensional electron gas (2DEG) is crucially important for both fundamental and applied research. Usually, spin polarization appears below 10 K for the 2DEG of LaAlO3/SrTiO3 interface, stemming from the magnetic ordering of Ti3+ ions with the mediat......Fabrication of highly mobile spin-polarized two-dimensional electron gas (2DEG) is crucially important for both fundamental and applied research. Usually, spin polarization appears below 10 K for the 2DEG of LaAlO3/SrTiO3 interface, stemming from the magnetic ordering of Ti3+ ions...... with the mediation of itinerant electrons. Herein, we report a magnetic 2DEG at a La7/8Sr1/8MnO3-buffered LaAlO3/SrTiO3 interface, which simultaneously shows electrically tunable anomalous Hall effect and high conductivity. The spin-polarized temperature for the 2DEG is promoted to 30 K while the mobility remains...... high. The magnetism likely results from a gradient manganese interdiffusion into SrTiO3. The present work demonstrates the great potential of manganite-buffered LaAlO3/SrTiO3 interfaces for spintronic applications....
Energy Technology Data Exchange (ETDEWEB)
Kohda, M. [IBM Research–Zürich, Säumerstrasse 4, CH-8803 Rüschlikon (Switzerland); Department of Materials Science, Tohoku University, 980-8579 Sendai (Japan); Altmann, P.; Salis, G. [IBM Research–Zürich, Säumerstrasse 4, CH-8803 Rüschlikon (Switzerland); Schuh, D.; Ganichev, S. D. [Institute of Experimental and Applied Physics, University of Regensburg, D-93040 Regensburg (Germany); Wegscheider, W. [Solid State Physics Laboratory, ETH Zürich, CH-8093 Zürich (Switzerland)
2015-10-26
A method is presented that enables the measurement of spin-orbit coefficients in a diffusive two-dimensional electron gas without the need for processing the sample structure, applying electrical currents or resolving the spatial pattern of the spin mode. It is based on the dependence of the average electron velocity on the spatial distance between local excitation and detection of spin polarization, resulting in a variation of spin precession frequency that in an external magnetic field is linear in the spatial separation. By scanning the relative positions of the exciting and probing spots in a time-resolved Kerr rotation microscope, frequency gradients along the [100] and [010] crystal axes of GaAs/AlGaAs QWs are measured to obtain the Rashba and Dresselhaus spin-orbit coefficients, α and β. This simple method can be applied in a variety of materials with electron diffusion for evaluating spin-orbit coefficients.
DEFF Research Database (Denmark)
Chen, Yunzhong; Gan, Yulin; Christensen, Dennis Valbjørn
2017-01-01
Modulation-doped oxide two-dimensional electron gas formed at the LaMnO3 (LMO) buffered disorderd-LaAlO3/SrTiO3 (d-LAO/LMO/STO) heterointerface provides new opportunities for electronics as well as quantum physics. Herein, we studied the dependence of Sr-doping of La1-xSrxMnO3 (LSMO, x = 0, 1/8, ...... of LSMO during the deposition of disordered LAO or that the energy levels of Mn 3d electrons at the interface of LSMO/STO are hardly varied even when changing the LSMO composition from LMO to SrMnO3....
Energy Technology Data Exchange (ETDEWEB)
Lu, Mao-Wang; Huang, Xin-Hong; Zhang, Gui-Lin; Chen, Sai-Yan [College of Science, Guilin University of Technology, Guilin 541004 (China)
2012-11-15
We present a theoretical study on the spin-dependent Goos-Haenchen (GH) effect in a two-dimensional electron gas modulated by ferromagnetic and Schottky metal (SM) stripes. The GH shifts for spin electron beams across this device are calculated with the help of the stationary phase method. It is shown that the GH shift of spin-up beam is significantly different from that of spin-down beam, i.e., this device shows up a considerable spin polarization effect in GH shifts of electron beams. It also is shown that both magnitude and sign of spin polarization of GH shifts are closely related to the stripe width, the magnetic strength and the gated voltage under SM stripe. These interesting properties not only provide an effective method of spin injection for spintronics application, but also give rise to a tunable spin beam splitter. (Copyright copyright 2012 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)
International Nuclear Information System (INIS)
Kurzmann, A.; Beckel, A.; Lorke, A.; Geller, M.; Ludwig, A.; Wieck, A. D.
2015-01-01
We have investigated the influence of a layer of charged self-assembled quantum dots (QDs) on the mobility of a nearby two-dimensional electron gas (2DEG). Time-resolved transconductance spectroscopy was used to separate the two contributions of the change in mobility, which are: (i) The electrons in the QDs act as Coulomb scatterers for the electrons in the 2DEG. (ii) The screening ability and, hence, the mobility of the 2DEG decreases when the charge carrier density is reduced by the charged QDs, i.e., the mobility itself depends on the charge carrier concentration. Surprisingly, we find a negligible influence of the Coulomb scattering on the mobility for a 2DEG, separated by a 30 nm tunneling barrier to the layer of QDs. This means that the mobility change is completely caused by depletion, i.e., reduction of the charge carrier density in the 2DEG, which indirectly influences the mobility
The Two-Dimensional MnO2/Graphene Interface: Half-metallicity and Quantum Anomalous Hall State
Gan, Liyong
2015-10-07
We explore the electronic properties of the MnO2/graphene interface by first-principles calculations, showing that MnO2 becomes half-metallic. MnO2 in the MnO2/graphene/MnO2 system provides time-reversal and inversion symmetry breaking. Spin splitting by proximity occurs at the Dirac points and a topologically nontrivial band gap is opened, enabling a quantum anomalous Hall state. The half-metallicity, spin splitting, and size of the band gap depend on the interfacial interaction, which can be tuned by strain engineering.
International Nuclear Information System (INIS)
Zasimovich, I.N.; Klimenko, E.V.; Naumovets, A.G.
1988-01-01
The first observation of electron-induced disordering (EID) of the submonolayer film of heavier adsorbate-oxygen is reported. The investigation of energy dependence of the effective cross section of this process, which points to the fact that EID can be initiated by the electron transitions not only in adatoms, but in the substrate, is also presented. When irradiating by electrons, the sample surface cooled up to 77 K, intensity of diffraction reflects of the (2x2) and (6x2) structures decreases rather quickly, but the reflects of more dense (6x1) lattice do not practically attenuate. The conclusions are made that the knowledge of physical factors, determining the probability of radiation defect formation in an adfilm, gives the possibility either to avoid disordering, if it is undesirable, or to use it to control the surface properties
DEFF Research Database (Denmark)
Chen, Yunzhong; Bovet, N.; Kasama, Takeshi
2014-01-01
Well-controlled sub-unit-cell layer-bylayer epitaxial growth of spinel alumina is achieved at room temperature on a TiO2-terminated SrTiO3 single-crystalline substrate. By tailoring the interface redox reaction, 2D electron gases with mobilities exceeding 3000 cm 2 V−1 s−1 are achieved at this no...
International Nuclear Information System (INIS)
Weber, Christopher P.
2005-01-01
Spin diffusion in n-GaAs quantum wells, as measured by our optical transient-grating technique, is strongly suppressed relative to that of charge. Over a broad range of temperatures and dopings, the suppression of Ds relative to Dc agrees quantitatively with the prediction of ''spin Coulomb dra'' theory, which takes into account the exchange of spin in electron-electron collisions. Moreover, the spin-diffusion length, Ls, is a nearly constant 1 micrometer over the same range of T and n, despite Ds's varying by nearly two orders of magnitude. This constancy supports the D'yakonov-Perel'-Kachorovskii model of spin relaxation through interrupted precessional dephasing in the spin-orbit field
Energy Technology Data Exchange (ETDEWEB)
Weber, Christopher Phillip [Univ. of California, Berkeley, CA (United States)
2005-01-01
Spin diffusion in n-GaAs quantum wells, as measured by our optical transient-grating technique, is strongly suppressed relative to that of charge. Over a broad range of temperatures and dopings, the suppression of Ds relative to Dc agrees quantitatively with the prediction of ''spin Coulomb dra'' theory, which takes into account the exchange of spin in electron-electron collisions. Moreover, the spin-diffusion length, Ls, is a nearly constant 1 micrometer over the same range of T and n, despite Ds's varying by nearly two orders of magnitude. This constancy supports the D'yakonov-Perel'-Kachorovskii model of spin relaxation through interrupted precessional dephasing in the spin-orbit field.
Kunihashi, Yoji; Sanada, Haruki; Tanaka, Yusuke; Gotoh, Hideki; Onomitsu, Koji; Nakagawara, Keita; Kohda, Makoto; Nitta, Junsaku; Sogawa, Tetsuomi
2017-11-01
We investigated the effect of an in-plane electric field on drifting spins in a GaAs quantum well. Kerr rotation images of the drifting spins revealed that the spin precession wavelength increases with increasing drift velocity regardless of the transport direction. A model developed for drifting spins with a heated electron distribution suggests that the in-plane electric field enhances the effective magnetic field component originating from the cubic Dresselhaus spin-orbit interaction.
DEFF Research Database (Denmark)
Chen, Yunzhong; Trier, Felix; Wijnands, T.
2015-01-01
as applied research of complex oxides. Here, we inserted a single unit cell insulating layer of polar La1-xSrxMnO3 (x=0, 1/8, and 1/3) at the interface between disordered LaAlO3 and crystalline SrTiO3 created at room temperature. We find that the electron mobility of the interfacial 2DEG is enhanced by more...
Zharkikh, Y S; Tretyak, O V
2003-01-01
The electron scattering mechanisms in the dimensionally quantized channels of silicon MOS-structures are investigated. The conclusion of the Coulomb scattering mechanism prevailing is made from the ratio of transport and quantum lifetimes. The experimental transport mobility values are compared with the Born approximation calculations. It is shown that the agreement of the experimental and calculated mobility's values can be obtained by taking into account the interference effect of remote ion potentials.
On the coexistence of two-dimensional electron and hole gases in GaN-based heterostructures
International Nuclear Information System (INIS)
Granzner, R.; Mustafa, N.; Schwierz, F.; Racko, J.; Mikolasek, M.; Breza, J.
2011-01-01
In this work, the conditions for the coexistence of electron and hole gases in GaN/AlGaN/GaN heterostructures are investigated by means of both numerical Schroedinger- Poisson simulations and analytical models. Special emphasis is put on the effects of the layer design and the bias conditions. We focus on wurtzite Ga-face structures which are commonly used in GaN-based devices. The conditions for the coexistence of electron and hole gases in GaN/AlGaN/GaN heterostructures have been studied by means of numerical Schroedinger-Poisson simulations and analytical models. When a 2DHG is formed, it effectively shields the 2DEG from the gate field and the electron concentration saturates. The saturation value strongly depends on the AlGaN thickness but is independent of the cap layer thickness. Below a minimum AlGaN thickness it is impossible to form a 2DHG and a 2DEG simultaneously. (authors)
International Nuclear Information System (INIS)
Kormondy, Kristy J.; Posadas, Agham B.; Demkov, Alexander A.; Ngo, Thong Q.; Ekerdt, John G.; Lu, Sirong; Smith, David J.; McCartney, Martha R.; Goble, Nicholas; Gao, Xuan P. A.; Jordan-Sweet, Jean
2015-01-01
In this paper, we report on the highly conductive layer formed at the crystalline γ-alumina/SrTiO 3 interface, which is attributed to oxygen vacancies. We describe the structure of thin γ-alumina layers deposited by molecular beam epitaxy on SrTiO 3 (001) at growth temperatures in the range of 400–800 °C, as determined by reflection-high-energy electron diffraction, x-ray diffraction, and high-resolution electron microscopy. In situ x-ray photoelectron spectroscopy was used to confirm the presence of the oxygen-deficient layer. Electrical characterization indicates sheet carrier densities of ∼10 13 cm −2 at room temperature for the sample deposited at 700 °C, with a maximum electron Hall mobility of 3100 cm 2 V −1 s −1 at 3.2 K and room temperature mobility of 22 cm 2 V −1 s −1 . Annealing in oxygen is found to reduce the carrier density and turn a conductive sample into an insulator
International Nuclear Information System (INIS)
Rodriguez, B.D.A.; Vilhena, M.T.; Borges, V.; Hoff, G.
2008-01-01
In this paper we solve the Fokker-Planck (FP) equation, an alternative approach for the Boltzmann transport equation for charged particles in a rectangular domain. To construct the solution we begin applying the P N approximation in the angular variable and the Laplace Transform in the x-variable, thus obtaining a first order linear differential equation in y-variable, which the solution is straightforward. The angular flux of electrons and the parameters of the medium are used for the calculation of the energy deposited by the secondary electrons generated by Compton Effect. The remaining effects will not be taken into account. The results will be presented under absorbed energy form in several points of interested. We present numerical simulations and comparisons with results obtained by using Geant4 (version 8) program which applies the Monte Carlo's technique to low energy libraries for a two-dimensional problem assuming the screened Rutherford differential scattering cross-section
Laser-sub-cycle two-dimensional electron-momentum mapping using orthogonal two-color fields
Zhang, Li; Xie, Xinhua; Roither, Stefan; Kartashov, Daniil; Wang, YanLan; Wang, ChuanLiang; Schöffler, Markus; Shafir, Dror; Corkum, Paul B.; Baltuška, Andrius; Ivanov, Igor; Kheifets, Anatoli; Liu, XiaoJun; Staudte, André; Kitzler, Markus
2014-12-01
We study laser-sub-cycle control over electron trajectories concomitantly in space and time using orthogonally polarized two-color laser fields. We compare experimental photoelectron spectra of neon recorded by coincidence momentum imaging with photoelectron spectra obtained by semiclassical and numerical solutions of the time-dependent Schrödinger equation. We find that a resolution of a quarter optical cycle in the photoelectron trajectories can be achieved. It is shown that depending on their sub-cycle birth time the trajectories of photoelectrons are affected differently by the ion's Coulomb field.
DEFF Research Database (Denmark)
Chen, Yunzhong; Green, Robert J.; Sutarto, Ronny
2017-01-01
polarities and redox reactions from disordered overlayers grown at room temperature. Using resonant x-ray reflectometry experiments, we quantify redox reactions from oxide overlayers on STO as well as polarity induced electronic reconstruction at epitaxial LSMO/STO interfaces. The analysis reveals how...... these effects can be combined in a STO/LSMO/disordered film trilayer system to yield high mobility modulation doped 2DELs, where the buffer layer undergoes a partial transformation from perovskite to brownmillerite structure. This uncovered interplay between polar discontinuities and redox reactions via buffer...
Osherovich, V. A.; Fainberg, J.
2018-01-01
We consider simultaneous oscillations of electrons moving both along the axis of symmetry and also in the direction perpendicular to the axis. We derive a system of three nonlinear ordinary differential equations which describe self-similar oscillations of cold electrons in a constant proton density background (np = n0 = constant). These three equations represent an exact class of solutions. For weak nonlinear conditions, the frequency spectra of electric field oscillations exhibit split frequency behavior at the Langmuir frequency ωp0 and its harmonics, as well as presence of difference frequencies at low spectral values. For strong nonlinear conditions, the spectra contain peaks at frequencies with values ωp0(n +m √{2 }) , where n and m are integer numbers (positive and negative). We predict that both spectral types (weak and strong) should be observed in plasmas where axial symmetry may exist. To illustrate possible applications of our theory, we present a spectrum of electric field oscillations observed in situ in the solar wind by the WAVES experiment on the Wind spacecraft during the passage of a type III solar radio burst.
Energy Technology Data Exchange (ETDEWEB)
Griesbeck, Michael
2012-11-22
Since many years there has been great effort to explore the spin dynamics in low-dimensional electron systems embedded in GaAs/AlGaAs based heterostructures for the purpose of quantum computation and spintronics applications. Advances in technology allow for the design of high quality and well-defined two-dimensional electron systems (2DES), which are perfectly suited for the study of the underlying physics that govern the dynamics of the electron spin system. In this work, spin dynamics in high-mobility 2DES is studied by means of the all-optical time-resolved Kerr/Faraday rotation technique. In (001)-grown 2DES, a strong in-plane spin dephasing anisotropy is studied, resulting from the interference of comparable Rashba and Dresselhaus contributions to the spin-orbit field (SOF). The dependence of this anisotropy on parameters like the confinement length of the 2DES, the sample temperature, as well as the electron density is demonstrated. Furthermore, coherent spin dynamics of an ensemble of ballistically moving electrons is studied without and within an applied weak magnetic field perpendicular to the sample plane, which forces the electrons to move on cyclotron orbits. Finally, strongly anisotropic spin dynamics is investigated in symmetric (110)-grown 2DES, using the resonant spin amplification method. Here, extremely long out-of-plane spin dephasing times can be achieved, in consequence of the special symmetry of the Dresselhaus SOF.
Javadi, Mohammad; Alizadeh, Saba; Khosravi, Yusef; Abdi, Yaser
2016-11-04
The integration of fast electron transport and large effective surface area is critical to attaining higher gains in the nanostructured photovoltaic devices. Here, we report facilitated electron transport in the quasi-two-dimensional (Q2D) porous TiO 2 . Liquid electrolyte dye-sensitized solar cells were prepared by utilizing photoanodes based on the Q2D porous substructures. Due to electron confinement in a microscale porous medium, directional diffusion toward collecting electrode is induced into the electron transport. Our measurements based on the photocurrent and photovoltage time-of-flight transients show that at higher Fermi levels, the electron diffusion coefficient in the Q2D porous TiO 2 is about one order of magnitude higher when compared with the conventional layer of porous TiO 2 . The results show that microstructuring of the porous TiO 2 leads to an approximately threefold improvement in the electron diffusion length. Such a modification may considerably affects the electrical functionality of moderate or low performance dye-sensitized solar cells for which the internal gain or collection efficiency is typically low. © 2016 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.
Integrable two dimensional supersystems
International Nuclear Information System (INIS)
Tripathy, K.C.; Tripathy, L.K.
1988-08-01
The integrability of two dimensional time-dependent classical systems is examined in N=2 superspace using Dirac's second class constraints. The invariants involving quadratic powers in velocities for super harmonic oscillator and super Kepler potentials have been derived. (author). 5 refs
Wang, W.; Uhrberg, R. I. G.
2017-12-01
Low-energy electron diffraction (LEED), scanning tunneling microscopy (STM), and photoelectron spectroscopy have been used to study an ordered structure formed by Ge atoms deposited onto the Au(111) surface. Based on a careful analysis of STM images and LEED patterns, we propose a ( 5 0 8 -14 ) unit cell for the atomic structure of the Ge layer. Core-level data indicate that some Ge atoms diffuse into the Au(111) crystal during annealing after deposition at room temperature. This is further corroborated by angle-resolved photoelectron spectroscopy (ARPES) measured for different amounts of Ge remaining after sputtering and annealing. The results of the ARPES study clearly disprove an earlier assignment of a parabolic band, centered at normal emission, as a part of a Dirac cone of germanene.
International Nuclear Information System (INIS)
Wei, Tzu-Chieh; Raussendorf, Robert; Kwek, Leong Chuan
2011-01-01
Universal quantum computation can be achieved by simply performing single-qubit measurements on a highly entangled resource state, such as cluster states. Cai, Miyake, Duer, and Briegel recently constructed a ground state of a two-dimensional quantum magnet by combining multiple Affleck-Kennedy-Lieb-Tasaki quasichains of mixed spin-3/2 and spin-1/2 entities and by mapping pairs of neighboring spin-1/2 particles to individual spin-3/2 particles [Phys. Rev. A 82, 052309 (2010)]. They showed that this state enables universal quantum computation by single-spin measurements. Here, we give an alternative understanding of how this state gives rise to universal measurement-based quantum computation: by local operations, each quasichain can be converted to a one-dimensional cluster state and entangling gates between two neighboring logical qubits can be implemented by single-spin measurements. We further argue that a two-dimensional cluster state can be distilled from the Cai-Miyake-Duer-Briegel state.
Two dimensional image correlation processor
Yao, Shi-Kai
1992-06-01
Two dimensional images are converted into a very long 1-dimensional data stream by means of raster scan. It is shown that the 1-dimensional correlation function of such long data streams is equivalent to the raster scan converted data of 2-dimensional correlation function of images. Real time correlation of high resolution two-dimensional images has been demonstrated using commercially available components. The advantages of this approach includes programmable electronics reference images, easy interface to objects of interest using conventional image collection optics, real time operation with high resolution images using off-the shelf components, and usefulness in the form of either black and white or full colored images. Such system would be versatile enough for robotics vision, optical inspection, and other pattern recognition and identification applications.
DEFF Research Database (Denmark)
Petersen, Christian Leth; Hansen, Ole Per
1996-01-01
We have investigated the AC conductivity elements in the quantum Hall regime of two-dimensional electron gases coupled capacitively to electrodes with Corbino geometry. The samples are GaAlAs/GaAs single heterostructures, and the measurements are made at low frequencies, up to 20 kHz. The diagonal...... conductivity is derived from magnetocapacitance measurements. It increases with increasing frequency according to a power law at integer filling factors. The exponent of the power law depends on both temperature and filling factor. Ratios between Hall conductivities at different filling factors are obtained...... by inductive measurements of the circulating current. They are found to agree with quantization in multipla of e2/h at the integer filling factors. ©1996 American Institute of Physics....
Chou, Kuan-Yu; Hsu, Nai-Wen; Su, Yi-Hsin; Chou, Chung-Tao; Chiu, Po-Yuan; Chuang, Yen; Li, Jiun-Yun
2018-02-01
We investigate DC characteristics of a two-dimensional electron gas (2DEG) in an undoped Si/SiGe heterostructure and its temperature dependence. An insulated-gate field-effect transistor was fabricated, and transfer characteristics were measured at 4 K-300 K. At low temperatures (T tunneling from the buried channel to the surface channel. Finally, the drain current is saturated again at large gate biases due to parallel conduction of buried and surface channels. By increasing the temperature, an abrupt increase in threshold voltage is observed at T ˜ 45 K and it is speculated that negatively charged impurities at the Al2O3/Si interface are responsible for the threshold voltage shift. At T > 45 K, the current saturation and negative transconductance disappear and the device acts as a normal transistor.
Khouri, T; Zeitler, U; Reichl, C; Wegscheider, W; Hussey, N E; Wiedmann, S; Maan, J C
2016-12-16
We report a high-field magnetotransport study of an ultrahigh mobility (μ[over ¯]≈25×10^{6} cm^{2} V^{-1} s^{-1}) n-type GaAs quantum well. We observe a strikingly large linear magnetoresistance (LMR) up to 33 T with a magnitude of order 10^{5}% onto which quantum oscillations become superimposed in the quantum Hall regime at low temperature. LMR is very often invoked as evidence for exotic quasiparticles in new materials such as the topological semimetals, though its origin remains controversial. The observation of such a LMR in the "simplest system"-with a free electronlike band structure and a nearly defect-free environment-excludes most of the possible exotic explanations for the appearance of a LMR and rather points to density fluctuations as the primary origin of the phenomenon. Both, the featureless LMR at high T and the quantum oscillations at low T follow the empirical resistance rule which states that the longitudinal conductance is directly related to the derivative of the transversal (Hall) conductance multiplied by the magnetic field and a constant factor α that remains unchanged over the entire temperature range. Only at low temperatures, small deviations from this resistance rule are observed beyond ν=1 that likely originate from a different transport mechanism for the composite fermions.
International Nuclear Information System (INIS)
Umeda, Takayuki; Kidani, Yoshitaka; Matsukiyo, Shuichi; Yamazaki, Ryo
2014-01-01
Large-scale two-dimensional (2D) full particle-in-cell (PIC) simulations are carried out for studying the relationship between the dynamics of a perpendicular shock and microinstabilities generated at the shock foot. The structure and dynamics of collisionless shocks are generally determined by Alfven Mach number and plasma beta, while microinstabilities at the shock foot are controlled by the ratio of the upstream bulk velocity to the electron thermal velocity and the ratio of the plasma-to-cyclotron frequency. With a fixed Alfven Mach number and plasma beta, the ratio of the upstream bulk velocity to the electron thermal velocity is given as a function of the ion-to-electron mass ratio. The present 2D full PIC simulations with a relatively low Alfven Mach number (M A ∼ 6) show that the modified two-stream instability is dominant with higher ion-to-electron mass ratios. It is also confirmed that waves propagating downstream are more enhanced at the shock foot near the shock ramp as the mass ratio becomes higher. The result suggests that these waves play a role in the modification of the dynamics of collisionless shocks through the interaction with shock front ripples
Fujiwara, Kohei; Nishihara, Kazuki; Shiogai, Junichi; Tsukazaki, Atsushi
2017-05-01
Wide-bandgap oxides exhibiting high electron mobility hold promise for the development of useful electronic and optoelectronic devices as well as for basic research on two-dimensional electron transport phenomena. A perovskite-type tin oxide, BaSnO3, is currently one of such targets owing to distinctly high mobility at room temperature. The challenge to overcome towards the use of BaSnO3 thin films in applications is suppression of dislocation scattering, which is one of the dominant scattering origins for electron transport. Here, we show that the mobility of the BaSnO3 electric-double-layer transistor reaches 300 cm2 V-1 s-1 at 50 K. The improved mobility indicates that charged dislocation scattering is effectively screened by electrostatically doped high-density charge carriers. We also observed metallic conduction persisting down to 2 K, which is attributed to the transition to the degenerate semiconductor. The experimental verification of bulk-level mobility at the densely accumulated surface sheds more light on the importance of suppression of dislocation scattering by interface engineering in doped BaSnO3 thin films for transparent electrode applications.
Long, Jingming; Hróðmarsson, Helgi Rafn; Wang, Huasheng; Kvaran, Ágúst
2012-06-07
Mass spectra were recorded for one-colour resonance enhanced multiphoton ionization (REMPI) of H(i)Br (i = 79, 81) for the two-photon resonance excitation region 79,040-80,300 cm(-1) to obtain two-dimensional REMPI data. The data were analysed in terms of rotational line positions, intensities, and line-widths. Quantitative analysis of the data relevant to near-resonance interactions between the F(1)Δ(2)(v' = 1) and V(1)Σ(+)(v' = m + 7) states gives interaction strengths, fractional state mixing, and parameters relevant to dissociation of the F state. Qualitative analysis further reveals the nature of state interactions between ion-pair states and the E(1)Σ(+) (v' = 1) and H(1)Σ(+)(v' = 0) Rydberg states in terms of relative strengths and J' dependences. Large variety in line-widths, depending on electronic states and J' quantum numbers, is indicative of number of different predissociation channels. The relationship between line-widths, line-shifts, and signal intensities reveals dissociation mechanisms involving ion-pair to Rydberg state interactions prior to direct or indirect predissociations of Rydberg states. Quantum interference effects are found to be important. Moreover, observed bromine atom (2 + 1) REMPI signals support the importance of Rydberg state predissociation channels. A band system, not previously observed in REMPI, was observed and assigned to the k(3)Π(0)(v' = 0) ←← X transition with band origin 80,038 cm(-1) and rotational parameter B(v('))=7.238 cm(-1).
Energy Technology Data Exchange (ETDEWEB)
Al Lafi, Abdul G. [Department of Chemistry, Atomic Energy Commission, Damascus, P.O. Box 6091 (Syrian Arab Republic); Hay, James N., E-mail: cscientific9@aec.org.sy [The School of Metallurgy and Materials, College of Physical Sciences and Engineering, University of Birmingham, Edgbaston, Birmingham B15 2TT (United Kingdom)
2015-07-20
Highlights: • 2D-DSC mapping was applied to analyze the heat flow responses of hydrated crosslinked sPEEK. • Two types of loosely bond water were observed. • The first was bond to the sulfonic acid groups and increased with ion exchange capacity. • The second was attributed to the polar groups introduced by ions irradiation and increased with crosslinking degree. • DSC combined with 2D mapping provides a powerful tool for polymer structural determination. - Abstract: This paper reports the first application of two-dimensional differential scanning calorimetry correlation mapping, 2D-DSC-CM to analyze the heat flow responses of sulphonated poly(ether ether ketone), sPEEK, films having different ion exchange capacity and degrees of crosslinks. With the help of high resolution and high sensitivity of 2D-DSC-CM, it was possible to locate two types of loosely bound water within the structure of crosslinked sPEEK. The first was bound to the sulfonic acid groups and dependent on the ion exchange capacity of the sPEEK. The second was bound to other polar groups, either introduced by irradiation with ions and dependent on the crosslinking degree or present in the polymer such as the carbonyl groups or terminal units. The results suggest that the ability of the sulfonic acid groups in the crosslinked sPEEK membranes to adsorb water molecules is increased by crosslinking, probably due to the better close packing efficiency of the crosslinked samples. DSC combined with 2D correlation mapping provides a fast and powerful tool for polymer structural determination.
Freedsman, J. J.; Watanabe, A.; Urayama, Y.; Egawa, T.
2015-09-01
The authors report on Al2O3/Al0.85In0.15N/GaN Metal-Oxide-Semiconductor High-Electron-Mobility Transistor (MOS-HEMT) on Si fabricated by using atomic layer deposited Al2O3 as gate insulator and passivation layer. The MOS-HEMT with the gate length of 2 μm exhibits excellent direct-current (dc) characteristics with a drain current maximum of 1270 mA/mm at a gate bias of 3 V and an off-state breakdown voltage of 180 V for a gate-drain spacing of 4 μm. Also, the 1 μm-gate MOS-HEMT shows good radio-frequency (rf) response such as current gain and maximum oscillation cut-off frequencies of 10 and 34 GHz, respectively. The capacitance-voltage characteristics at 1 MHz revealed significant increase in two-dimensional electron gas (2DEG) density for the MOS-HEMT compared to conventional Schottky barrier HEMTs. Analyses using drain-source conductivity measurements showed improvements in 2DEG transport characteristics for the MOS-HEMT. The enhancements in dc and rf performances of the Al2O3/Al0.85In0.15N/GaN MOS-HEMT are attributed to the improvements in 2DEG characteristics.
International Nuclear Information System (INIS)
Freedsman, J. J.; Watanabe, A.; Urayama, Y.; Egawa, T.
2015-01-01
The authors report on Al 2 O 3 /Al 0.85 In 0.15 N/GaN Metal-Oxide-Semiconductor High-Electron-Mobility Transistor (MOS-HEMT) on Si fabricated by using atomic layer deposited Al 2 O 3 as gate insulator and passivation layer. The MOS-HEMT with the gate length of 2 μm exhibits excellent direct-current (dc) characteristics with a drain current maximum of 1270 mA/mm at a gate bias of 3 V and an off-state breakdown voltage of 180 V for a gate-drain spacing of 4 μm. Also, the 1 μm-gate MOS-HEMT shows good radio-frequency (rf) response such as current gain and maximum oscillation cut-off frequencies of 10 and 34 GHz, respectively. The capacitance-voltage characteristics at 1 MHz revealed significant increase in two-dimensional electron gas (2DEG) density for the MOS-HEMT compared to conventional Schottky barrier HEMTs. Analyses using drain-source conductivity measurements showed improvements in 2DEG transport characteristics for the MOS-HEMT. The enhancements in dc and rf performances of the Al 2 O 3 /Al 0.85 In 0.15 N/GaN MOS-HEMT are attributed to the improvements in 2DEG characteristics
Two-dimensional topological photonics
Khanikaev, Alexander B.; Shvets, Gennady
2017-12-01
Originating from the studies of two-dimensional condensed-matter states, the concept of topological order has recently been expanded to other fields of physics and engineering, particularly optics and photonics. Topological photonic structures have already overturned some of the traditional views on wave propagation and manipulation. The application of topological concepts to guided wave propagation has enabled novel photonic devices, such as reflection-free sharply bent waveguides, robust delay lines, spin-polarized switches and non-reciprocal devices. Discrete degrees of freedom, widely used in condensed-matter physics, such as spin and valley, are now entering the realm of photonics. In this Review, we summarize the latest advances in this highly dynamic field, with special emphasis on the experimental work on two-dimensional photonic topological structures.
Osserman, Robert
2011-01-01
The basic component of several-variable calculus, two-dimensional calculus is vital to mastery of the broader field. This extensive treatment of the subject offers the advantage of a thorough integration of linear algebra and materials, which aids readers in the development of geometric intuition. An introductory chapter presents background information on vectors in the plane, plane curves, and functions of two variables. Subsequent chapters address differentiation, transformations, and integration. Each chapter concludes with problem sets, and answers to selected exercises appear at the end o
Bian, Liang; Dong, Fa-qin; Song, Mian-xin; Dong, Hai-liang; Li, Wei-Min; Duan, Tao; Xu, Jin-bao; Zhang, Xiao-yan
2015-08-30
Understanding how plutonium (Pu) doping affects the crystalline zircon structure is very important for risk management. However, so far, there have been only a very limited number of reports of the quantitative simulation of the effects of the Pu charge and concentration on the phase transition. In this study, we used density functional theory (DFT), virtual crystal approximation (VCA), and two-dimensional correlation analysis (2D-CA) techniques to calculate the origins of the structural and electronic transitions of Zr1-cPucSiO4 over a wide range of Pu doping concentrations (c=0-10mol%). The calculations indicated that the low-angular-momentum Pu-fxy-shell electron excites an inner-shell O-2s(2) orbital to create an oxygen defect (VO-s) below c=2.8mol%. This oxygen defect then captures a low-angular-momentum Zr-5p(6)5s(2) electron to form an sp hybrid orbital, which exhibits a stable phase structure. When c>2.8mol%, each accumulated VO-p defect captures a high-angular-momentum Zr-4dz electron and two Si-pz electrons to create delocalized Si(4+)→Si(2+) charge disproportionation. Therefore, we suggest that the optimal amount of Pu cannot exceed 7.5mol% because of the formation of a mixture of ZrO8 polyhedral and SiO4 tetrahedral phases with the orientation (10-1). This study offers new perspective on the development of highly stable zircon-based solid solution materials. Copyright © 2015 Elsevier B.V. All rights reserved.
Prediction of a mobile two-dimensional electron gas at the LaSc O3 /BaSn O3 (001) interface
Paudel, Tula R.; Tsymbal, Evgeny Y.
2017-12-01
Two-dimensional electron gases (2DEG) at oxide interfaces, such as LaAl O3 /SrTi O3 (001), have aroused significant interest due to their high carrier density (˜1014c m-2 ) and strong lateral confinement (˜1 nm). However, these 2DEGs are normally hosted by the weakly dispersive and degenerate d bands (e.g., Ti -3 d bands), which are strongly coupled to the lattice, causing mobility of such 2DEGs to be relatively low at room temperature (˜1 c m2/Vs ). Here, we propose using oxide host materials with the conduction bands formed from s electrons to increase carrier mobility and soften its temperature dependence. Using first-principles density functional theory calculations, we investigate LaSc O3 /BaSn O3 (001) heterostructure and as a model system, where the conduction band hosts the s -like carriers. We find that the polar discontinuity at this interface leads to electronic reconstruction resulting in the formation of the 2DEG at this interface. The conduction electrons reside in the highly dispersive Sn -5 s bands, which have a large band width and a low effective mass. The predicted 2DEG is expected to be highly mobile even at room temperature due to the reduced electron-phonon scattering via the inter-band scattering channel. A qualitatively similar behavior is predicted for a doped BaSn O3 , where a monolayer of BaO is replaced with LaO. We anticipate that the quantum phenomena associated with these 2DEGs to be more pronounced owing to the high mobility of the carriers.
Sekihara, Takayuki; Masutomi, Ryuichi; Okamoto, Tohru
2013-08-02
Two-dimensional (2D) superconductivity was studied by magnetotransport measurements on single-atomic-layer Pb films on a cleaved GaAs(110) surface. The superconducting transition temperature shows only a weak dependence on the parallel magnetic field up to 14T, which is higher than the Pauli paramagnetic limit. Furthermore, the perpendicular-magnetic-field dependence of the sheet resistance is almost independent of the presence of the parallel field component. These results are explained in terms of an inhomogeneous superconducting state predicted for 2D metals with a large Rashba spin splitting.
International Nuclear Information System (INIS)
Wang, Erhui; Morita, Shigeru; Goto, Motoshi; Murakami, Izumi; Oishi, Tetsutarou; Dong, Chunfeng
2013-01-01
Two-dimensional distribution of impurity lines emitted from ergodic layer with stochastic magnetic field lines in Large Helical Device (LHD) has been observed using a space-resolved extreme ultraviolet (EUV) spectrometer. The two-dimensional electron temperature distribution in the ergodic layer is successfully measured using the line intensity ratio of Li-like NeVIII 2s-3p ( 2 S 1/2 - 2 P 3/2 : 88.09 Å, 2 S 1/2 - 2 P 1/2 : 88.13 Å) to 2p-3s ( 2 P 1/2 - 2 S 1/2 : 102.91 Å, 2 P 3/2 - 2 S 1/2 : 103.09 Å) transitions emitted from radial location near Last Closed Flux Surface (LCFS). The intensity ratio analyzed with ADAS code shows no dependence on the electron density below 10 14 cm -3 . The result indicates a little higher temperature, i.e., 220 eV, in the poloidal location at high-field side near helical coils called O-point compared to the temperature near X-point, i.e., 170 eV. The electron temperature profile is also measured at the edge boundary of ergodic layer using the line intensity ratio of Li-like CIV 2p-3d ( 2 P 1/2 - 2 D 3/2 : 384.03 Å, 2 P 3/2 - 2 D 5/2 : 384.18 Å) to 2p-3s ( 2 P 1/2 - 2 S 1/2 : 419.53 Å, 2 P 3/2 - 2 S 1/2 : 419.71 Å) transitions. The intensity ratios analyzed with CHIANTI, ADAS and T.Kawachi codes show a slightly higher temperature near O-point, i.e., 25 eV for CHIANTI, 21 eV for ADAS and 11 eV for T.Kawachi's codes, compared to the temperature at X-point, i.e., 15 - 21 eV for CHIANTI, 9 - 15 eV for ADAS and 6 - 9 eV for T.Kawachi codes. It suggests that the transport coefficient in the ergodic layer is varied with three-dimensional structure. (author)
Two-dimensional ferroelectrics
Energy Technology Data Exchange (ETDEWEB)
Blinov, L M; Fridkin, Vladimir M; Palto, Sergei P [A.V. Shubnikov Institute of Crystallography, Russian Academy of Sciences, Moscow, Russian Federaion (Russian Federation); Bune, A V; Dowben, P A; Ducharme, Stephen [Department of Physics and Astronomy, Behlen Laboratory of Physics, Center for Materials Research and Analysis, University of Nebraska-Linkoln, Linkoln, NE (United States)
2000-03-31
The investigation of the finite-size effect in ferroelectric crystals and films has been limited by the experimental conditions. The smallest demonstrated ferroelectric crystals had a diameter of {approx}200 A and the thinnest ferroelectric films were {approx}200 A thick, macroscopic sizes on an atomic scale. Langmuir-Blodgett deposition of films one monolayer at a time has produced high quality ferroelectric films as thin as 10 A, made from polyvinylidene fluoride and its copolymers. These ultrathin films permitted the ultimate investigation of finite-size effects on the atomic thickness scale. Langmuir-Blodgett films also revealed the fundamental two-dimensional character of ferroelectricity in these materials by demonstrating that there is no so-called critical thickness; films as thin as two monolayers (1 nm) are ferroelectric, with a transition temperature near that of the bulk material. The films exhibit all the main properties of ferroelectricity with a first-order ferroelectric-paraelectric phase transition: polarization hysteresis (switching); the jump in spontaneous polarization at the phase transition temperature; thermal hysteresis in the polarization; the increase in the transition temperature with applied field; double hysteresis above the phase transition temperature; and the existence of the ferroelectric critical point. The films also exhibit a new phase transition associated with the two-dimensional layers. (reviews of topical problems)
Scattering times in the two-dimensional electron gas of AlxGa1-xN/AlN/GaN heterostructures
International Nuclear Information System (INIS)
Han Xiuxun; Honda, Yoshio; Narita, Tetsuo; Yamaguchi, Masahito; Sawaki, Nobuhiko; Tanaka, Tooru; Guo Qixin; Nishio, Mitsushiro
2009-01-01
Low-field Hall and Shubnikov-de Haas (SdH) measurements were performed on two-dimensional electron gas of Al 0.24 Ga 0.76 N/GaN and Al 0.24 Ga 0.76 N/AlN/GaN heterostructures at a low temperature. A dramatic improvement in electron mobility is observed in Al 0.24 Ga 0.76 N/AlN/GaN heterostructures with 1 and 2 nm thick AlN interlayers. A further increase in the AlN thickness degrades the transport behaviour. Transport and quantum scattering times were derived from the corresponding Hall mobility and the oscillatory part of the SdH signal. The ratio of the transport scattering time and the quantum scattering time increases from 3.87 in the heterostructure without the AlN interlayer to 14.34 with the 1 nm AlN interlayer and to 12.45 with the 2 nm AlN interlayer. A modified scattering calculation due to charged dislocation with a finite length suggests that dislocation related long-range scattering event tends to dominate both transport and quantum scattering times when a thin AlN interlayer is introduced.
International Nuclear Information System (INIS)
Zhang Degang
2006-01-01
We study a two-dimensional electron system in the presence of both Rashba and Dresselhaus spin-orbit interactions in a perpendicular magnetic field. Defining two suitable boson operators and using the unitary transformations we are able to obtain the exact Landau levels in the range of all the parameters. When the strengths of the Rashba and Dresselhaus spin-orbit interactions are equal, a new analytical solution for the vanishing Zeeman energy is found, where the orbital and spin wavefunctions of the electron are separated. It is also shown that in this case the Zeeman and spin-orbit splittings are independent of the Landau level index n. Due to the Zeeman energy, new crossing between the eigenstates vertical bar n, k, s = 1, σ) and vertical bar n + 1, k, s' = -1, σ') is produced at a certain magnetic field for larger Rashba spin-orbit coupling. This degeneracy leads to a resonant spin Hall conductance if it happens at the Fermi level. (letter to the editor)
Energy Technology Data Exchange (ETDEWEB)
Zapf, Michael; Gabel, Judith; Scheiderer, Philipp; Dudy, Lenart; Sing, Michael; Claessen, Ralph [Physikalisches Institut and Roentgen Center for Complex Material Systems (RCCM), Universitaet Wuerzburg (Germany); Schlueter, Christoph; Lee, Tien-Lin [Diamond Light Source Ltd., Didcot (United Kingdom)
2016-07-01
Two-dimensional electron systems (2DESs) in oxide heterostructures based on SrTiO{sub 3} are considered to be a promising platform for future microelectronic technology. A variety of interesting properties such as ferromagnetism, resistive switching and superconductivity are linked to interfacial n-doping involving oxygen vacancies. The introduction of a high Z-cation with large spin-orbit coupling like Ta offers an exciting new parameter. We report on a new oxygen vacancy induced 2DES located at the interface of disordered LaAlO{sub 3} and crystalline KTaO{sub 3}, which exhibits remarkably high electron mobilities and charge carrier concentrations. The number of charge carriers can be readily manipulated by the film thickness and irradiation with intense X-rays. Our synchrotron-based hard X-ray photoemission experiments provide a direct probe of the Ta 5d charge carriers at the buried interface to obtain information on the charge carrier density, its depth distribution, and the band structure.
Singh, Rohit; Arif Khan, Md; Sharma, Pankaj; Than Htay, Myo; Kranti, Abhinav; Mukherjee, Shaibal
2018-04-01
This work reports on the formation of high-density (~1013-1014 cm-2) two-dimensional electron gas (2DEG) in ZnO-based heterostructures, grown by a dual ion beam sputtering system. We probe 2DEG in bilayer MgZnO/ZnO and capped ZnO/MgZnO/ZnO heterostructures utilizing MgZnO barrier layers with varying thickness and Mg content. The effect of the ZnO cap layer thickness on the ZnO/MgZnO/ZnO heterostructure is also studied. Hall measurements demonstrate that the addition of a 5 nm ZnO cap layer results in an enhancement of the 2DEG density by about 1.5 times compared to 1.11 × 1014 cm-2 for the uncapped bilayer heterostructure with the same 30 nm barrier thickness and 30 at.% Mg composition in the barrier layer. From the low-temperature Hall measurement, the sheet carrier concentration and mobility are both found to be independent of the temperature. The capacitance-voltage measurement suggests a carrier density of ~1020 cm-3, confined in 2DEG at the MgZnO/ZnO heterointerface. The results presented are significant for the optimization of 2DEG for the eventual realization of cost-effective and large-area MgZnO/ZnO-based high-electron-mobility transistors.
Kaul, Anupama B.
2013-05-01
Carbon-based nanomaterials such as graphene, a layered two-dimensional (2D) crystal, carbon nanotubes and carbon nanofibers have been explored extensively by researchers as well as the semiconductor industry as viable alternatives to silicon-based complimentary metal-oxide semiconductor transistors. Besides nanoscale transistors, the exceptional properties of carbon-based nanomaterials has stirred intense interest in considering these materials for applications ranging from interconnects, field-emission displays, photo-voltaics and nano-electro-mechanical-systems (NEMS). Recently, the emergence of other layered 2D crystals where the bonding between layers is held together by the weak van der Waals interaction, has opened up new avenues of research and exploration. Such material systems display a diverse array of properties ranging from insulating hexagonal-BN, metallic NbS2 to semiconducting MoS2. The ability to engineer the materials properties in these 2D layered materials provides promising prospects for their use in a wide variety of applications ranging from electronics, photonics, sensing, energy harvesting, flexible electronics and related applications over the coming years.
Energy Technology Data Exchange (ETDEWEB)
Bian, Liang, E-mail: bianliang@ms.xjb.ac.cn [Key Laboratory of Functional Materials and Devices for Special Environments, Chinese Academy of Sciences, Urumqi 830011, Xinjiang (China); Laboratory for Extreme Conditions Matter Properties, South West University of Science and Technology, Mianyang 621010, Sichuan (China); Dong, Fa-qin; Song, Mian-xin [Laboratory for Extreme Conditions Matter Properties, South West University of Science and Technology, Mianyang 621010, Sichuan (China); Dong, Hai-liang [Department of Geology and Environmental Earth Science, Miami University, Oxford, OH 45056 (United States); Li, Wei-Min [Key Laboratory of Functional Materials and Devices for Special Environments, Chinese Academy of Sciences, Urumqi 830011, Xinjiang (China); Duan, Tao; Xu, Jin-bao [Laboratory for Extreme Conditions Matter Properties, South West University of Science and Technology, Mianyang 621010, Sichuan (China); Zhang, Xiao-yan [Key Laboratory of Functional Materials and Devices for Special Environments, Chinese Academy of Sciences, Urumqi 830011, Xinjiang (China); Laboratory for Extreme Conditions Matter Properties, South West University of Science and Technology, Mianyang 621010, Sichuan (China)
2015-08-30
Highlights: • Effect of Pu f-shell electron on the electronic property of zircon is calculated via DFT and 2D-CA techniques. • Reasons of Pu f-shell electron influencing on electronic properties are systematically discussed. • Phase transitions are found at two point 2.8 mol% and 7.5 mol%. - Abstract: Understanding how plutonium (Pu) doping affects the crystalline zircon structure is very important for risk management. However, so far, there have been only a very limited number of reports of the quantitative simulation of the effects of the Pu charge and concentration on the phase transition. In this study, we used density functional theory (DFT), virtual crystal approximation (VCA), and two-dimensional correlation analysis (2D-CA) techniques to calculate the origins of the structural and electronic transitions of Zr{sub 1−c}Pu{sub c}SiO{sub 4} over a wide range of Pu doping concentrations (c = 0–10 mol%). The calculations indicated that the low-angular-momentum Pu-f{sub xy}-shell electron excites an inner-shell O-2s{sup 2} orbital to create an oxygen defect (V{sub O-s}) below c = 2.8 mol%. This oxygen defect then captures a low-angular-momentum Zr-5p{sup 6}5s{sup 2} electron to form an sp hybrid orbital, which exhibits a stable phase structure. When c > 2.8 mol%, each accumulated V{sub O-p} defect captures a high-angular-momentum Zr-4d{sub z} electron and two Si-p{sub z} electrons to create delocalized Si{sup 4+} → Si{sup 2+} charge disproportionation. Therefore, we suggest that the optimal amount of Pu cannot exceed 7.5 mol% because of the formation of a mixture of ZrO{sub 8} polyhedral and SiO{sub 4} tetrahedral phases with the orientation (10-1). This study offers new perspective on the development of highly stable zircon-based solid solution materials.
International Nuclear Information System (INIS)
Ngo, Thong Q.; McDaniel, Martin D.; Ekerdt, John G.; Goble, Nicholas J.; Gao, Xuan P. A.; Posadas, Agham; Kormondy, Kristy J.; Demkov, Alexander A.; Lu, Sirong; Jordan-Sweet, Jean; Smith, David J.
2015-01-01
We report the formation of a quasi-two-dimensional electron gas (2-DEG) at the interface of γ-Al 2 O 3 /TiO 2 -terminated SrTiO 3 (STO) grown by atomic layer deposition (ALD). The ALD growth of Al 2 O 3 on STO(001) single crystal substrates was performed at temperatures in the range of 200–345 °C. Trimethylaluminum and water were used as co-reactants. In situ reflection high energy electron diffraction, ex situ x-ray diffraction, and ex situ cross-sectional transmission electron microscopy were used to determine the crystallinity of the Al 2 O 3 films. As-deposited Al 2 O 3 films grown above 300 °C were crystalline with the γ-Al 2 O 3 phase. In situ x-ray photoelectron spectroscopy was used to characterize the Al 2 O 3 /STO interface, indicating that a Ti 3+ feature in the Ti 2p spectrum of STO was formed after 2–3 ALD cycles of Al 2 O 3 at 345 °C and even after the exposure to trimethylaluminum alone at 300 and 345 °C. The interface quasi-2-DEG is metallic and exhibits mobility values of ∼4 and 3000 cm 2 V −1 s −1 at room temperature and 15 K, respectively. The interfacial conductivity depended on the thickness of the Al 2 O 3 layer. The Ti 3+ signal originated from the near-interfacial region and vanished after annealing in an oxygen environment
Erpelding, Marion; Sinha, Santanu; Tallakstad, Ken Tore; Hansen, Alex; Flekkøy, Eirik Grude; Måløy, Knut Jørgen
2013-11-01
It is well known that the transient behavior during drainage or imbibition in multiphase flow in porous media strongly depends on the history and initial condition of the system. However, when the steady-state regime is reached and both drainage and imbibition take place at the pore level, the influence of the evolution history and initial preparation is an open question. Here, we present an extensive experimental and numerical work investigating the history dependence of simultaneous steady-state two-phase flow through porous media. Our experimental system consists of a Hele-Shaw cell filled with glass beads which we model numerically by a network of disordered pores transporting two immiscible fluids. From measurements of global pressure evolution, histograms of saturation, and cluster-size distributions, we find that when both phases are flowing through the porous medium, the steady state does not depend on the initial preparation of the system or on the way it has been reached.
Kumar, A.; Heise, H.; Blommers, M. J. J.; Krastel, P.; Schmitt, E.; Petersen, F.; Jeganathan, S.; Mandelkow, E. -M; Carlomagno, T.; Griesinger, C.; Baldus, M.
2010-01-01
Solid evidence: Induction of the polymerization of β-tubulin dimers into microtubules by epothilones, such as patupilone, by an as yet unknown mechanism leads to the apoptosis of cancer cells. Solid-state NMR spectroscopy of patupilone bound to microtubules has now enabled the identification of
Srisongmuang, B.; Pasanai, K.
2018-04-01
We theoretically studied the effect of interfacial scattering on the transport of charge and spin across the junction of a two-dimensional electron gas with Dresselhaus spin-orbit coupling and ferromagnetic material junction, via the conductance (G) and the spin-polarization of the conductance spectra (P) using the scattering method. At the interface, not only were the effects of spin-conserving (Z0) and spin-flip scattering (Zf) considered, but also the interfacial Rashba spin-orbit coupling scattering (ZRSOC) , which was caused by the asymmetry of the interface, was taken into account, and all of them were modeled by the delta potential. It was found that G was suppressed with increasing Z0 , as expected. Interestingly, a particular value of Zf can cause G and P to reach a maximum value. In particular, ZRSOC plays a crucial role to reduce G and P in the metallic limit, but its influence on the tunneling limit was quite weak. On the other hand, the effect of ZRSOC was diminished in the tunneling limit of the magnetic junction.
Li, Dandan; Du, Juan; Zhang, Qian; Xia, Congxin; Wei, Shuyi
2018-03-01
Through first-principles calculations we study the electronic structures and optical properties of two-dimensional (2D) Sn1-xTi(Zr)xS2 alloys. The results indicate that the band gap value of Sn1-xTi(Zr)xS2 alloys is decreased continuously when Ti(Zr) concentration is increased, which is very beneficial to optoelectronic devices applications. Moreover, the static dielectric constant is increased when the Ti(Zr) concentration is increased in the 2D Sn1-xTi(Zr)xS2 alloys. In addition, we also calculate the imaginary part 𝜀2(ω) dispersion of Sn1-xTi(Zr)xS2 alloys along the plane with different Ti(Zr) concentrations. The threshold energy values decrease with increasing Ti(Zr) concentrations in the Sn1-xTi(Zr)xS2 ternary alloys. Moreover, the calculations of formation energy also indicate that these 2D alloys can be fabricated under some experimental conditions. These results suggest that Ti(Zr) substituting Sn atom is an efficient way to tune the band gap and optical properties of 2D SnS2 nanosheets.
Energy Technology Data Exchange (ETDEWEB)
Gadiev, R. M., E-mail: gadiev.radik@gmail.com; Lachinov, A. N. [M. Akmullah Baskir State Pedagogical University (Russian Federation); Karamov, D. D. [Russian Academy of Sciences, Ufa Scientific Center (Russian Federation); Kiselev, D. A. [National University of Science and Technology MISiS (Russian Federation); Kornilov, V. M. [M. Akmullah Baskir State Pedagogical University (Russian Federation)
2016-07-15
The mechanism of formation of the two-dimensional conductivity along the interface between two polymer dielectrics is experimentally studied. The idea of “polar catastrophe,” which was successfully used earlier to explain the electronic properties of the interface between two perovskites LaAlO{sub 3}/SrTiO{sub 3}, is chosen as a base hypothesis. Piezoelectric response microscopy is used to reveal the presence of spontaneous polarization on the surface of a polymer film, and the remanent polarization is found to decrease with increasing film thickness. As in the case of perovskites, the polymer film thickness is found to strongly affect the electrical conductivity along the interface. Substantial differences between these phenomena are detected. The change in the electrical conductivity is shown to be caused by a significant increase in the charge carrier mobility when the film thickness decreases below a certain critical value. The relation between the change in the carrier mobility and the change in the spontaneous surface polarization of the polymer film when its thickness decreases is discussed.
Directory of Open Access Journals (Sweden)
Paulina Wiśniewska
2017-01-01
Full Text Available Whisky is one of the most popular alcoholic beverages. There are many types of whisky, for example, Scotch, Irish, and American whisky (called bourbon. The whisky market is highly diversified, and, because of this, it is important to have a method which would enable rapid quality evaluation and authentication of the type of whisky. The aim of this work was to compare 3 methods: an electronic nose based on the technology of ultrafast gas chromatography (Fast-GC, comprehensive two-dimensional gas chromatography (GC × GC, and sensory evaluation. The selected whisky brands included 6 blended whiskies from Scotland, 4 blended whiskies from Ireland, and 4 bourbons produced in the USA. For data analysis, peak heights of chromatograms were used. The panelists who took part in sensory evaluations included 4 women and 4 men. The obtained data were analyzed by 2 chemometric methods: partial least squares discriminant analysis (PLS-DA and discrimination function analysis (DFA. E-nose and GC × GC allowed for differentiation between whiskies by type. Sensory analysis did not allow for differentiation between whiskies by type, but it allowed giving consumer preferences.
Guilhon, I.; Teles, L. K.; Marques, M.; Pela, R. R.; Bechstedt, F.
2015-08-01
The energetics and thermodynamic properties of two-dimensional binary graphene-like alloys made from graphene, silicene, or germanene are investigated by combining first-principles total energy calculations, and a statistical approach to account for disorder and composition effects. For the electronic properties the calculations are performed within the GGA-1/2 approach for an approximate quasiparticle bands. We derive lattice constants, first-neighbor distances, and buckling parameters as a function of composition x . The Si1 -xGex system is the only stable random alloy at usual growth temperatures. For Ge1 -xCx , we observe strong distortions of the lattice making the random configurations less favorable and leading to a pronounced tendency for phase separation. The situation for Si1 -xCx alloys is completely different. An ordered structure with composition x =0.5 is stable up to T ≈1000 K, while intermediate compositions are mainly realized by silicongraphene and graphene or silicene. The ordering and decomposition effects have a strong influence on the average fundamental energy gap versus composition. Whereas large gaps appear for Si1 -xCx systems they almost vanish for Ge1 -xSix and Ge1 -xCx . Moreover, the dependence of the Si1 -xCx energy gap on growth temperature is also obtained. The results can be very useful for chemical vapor deposition growth of these materials.
International Nuclear Information System (INIS)
Ramanayaka, A.N.; Ye, Tianyu; Liu, H.-C.; Wegscheider, W.; Mani, R.G.
2014-01-01
The influence of microwave excitation on the magnetotransport properties of the high mobility two-dimensional electron system (2DES) in the GaAs/AlGaAs heterostructure system is investigated by exploring (a) the dependence of the amplitude of the microwave-induced magnetoresistance-oscillations on the polarization direction of the linearly polarized microwaves and (b) the microwave reflection from the 2DES. The polarization study indicates that the amplitude of the magnetoresistance oscillations is remarkably responsive to the relative orientation between the linearly polarized microwaves and the current-axis in the specimen. At low microwave power, P, experiments indicate a strong sinusoidal variation in the diagonal resistance R xx vs. θ at the oscillatory extrema of the microwave-induced magnetoresistance oscillations. The reflection study indicates strong correlations between the microwave induced magnetoresistance oscillations and oscillatory features in the microwave reflection in a concurrent measurement of the magnetoresistance and the microwave magnetoreflection from the 2DES. The correlations are followed as a function of the microwave frequency and the microwave power, and the results are reported
Zeng, X. L.; Yu, J. L.; Cheng, S. Y.; Lai, Y. F.; Chen, Y. H.; Huang, W.
2017-05-01
The linear (LPGE) and circular photogalvanic effects (CPGE), induced by interband (532 nm) and intersubband (1064 nm) excitation, have been investigated in a temperature range from 77 to 300 K in GaAs/AlGaAs two-dimensional electron gas. The temperature dependences of the CPGE current induced by Rashba and Dresselhaus spin orbit coupling (SOC) under the interband and intersubband excitation are obtained, respectively. It is revealed that the CPGE and LPGE current induced by the intersubband excitation almost increases with increasing temperature, while that induced by interband excitation nearly decreases with increasing temperatures. These phenomena may be attributed to the different variation trends of photo-induced carrier density and SOC with increasing temperatures between interband and intersubband excitation. The evolutions of the ratio of the Rashba and Dresselhaus SOC (RD ratios) and the anisotropic ratio of linear photogalvanic tensors, corresponding to the interband and intersubband excitations, with temperatures are determined. The power dependence of CPGE and LPGE current induced by intersubband excitation is also investigated. It is found that for the power range from 0 to 275 mW, the CPGE current nearly increases linearly with increasing power, while the LPGE current shows a decreasing generation rate at higher power. This study also provides a method to manipulate the photogalvanic effects by temperatures and by using excitation light of different wavelengths.
Cramer, J. M.; Marshall, W. M.; Pal, S.; Santoro, R. J.
2003-01-01
Twin thruster tests have been conducted with the Penn State RBCC test article operating at sea- level static conditions. Significant differences were observed in the performance characteristics for two different thruster centerline spacings. Changing the thruster spacing from 2.50 to 1.75 in. reduced the entrained air velocity (-17%) and the thrust (-7%) for tests at a thruster chamber pressure of 200 psia and MR = 8. In addition, significant differences were seen in the static pressure profiles, the Raman spectroscopy profiles, and the acoustic power spectrum for these two configurations.
Energy Technology Data Exchange (ETDEWEB)
Curtis, Jeremy A. [Univ. of Alabama, Birmingham, AL (United States); Tokumoto, Takahisa [Univ. of Alabama, Birmingham, AL (United States); Cherian, Judy G. [Florida State Univ., Tallahassee, FL (United States). National High Magnetic Field Lab. (MagLab); Kuno, J. [Rice Univ., Houston, TX (United States); Reno, John L. [Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); McGill, Stephen A. [Florida State Univ., Tallahassee, FL (United States). National High Magnetic Field Lab. (MagLab); Karaiskaj, Denis [Univ. of South Florida, Tampa, FL (United States); Hilton, David J. [Univ. of Alabama, Birmingham, AL (United States)
2015-10-01
We have studied the cyclotron mobility of a Landau-quantized two-dimensional electron gas as a function of temperature (0.4 --100 K) at a fixed magnetic field (1.25 T) using terahertz time-domain spectroscopy in a sample with a low frequency mobility of μ_{dc} = 3.6 x 10^{6} cm^{2} V^{-1} s^{-1} and a carrier concentration of ns = 2 x 10_{6} cm^{-2}. The low temperature mobility in this sample results from both impurity scattering and acoustic deformation potential scattering, with μ$-1\\atop{CR}$ ≈ (2.1 x 10^{5} cm^{2} V^{-1} s^{-1})^{-1} + (3.8 x 10^{-8} V sK^{-1} cm^{-2} x T)^{-1} at low temperatures. Above 50 K, the cyclotron oscillations show a strong reduction in both the oscillation amplitude and lifetime that is dominated by the contribution due to polar optical phonons. These results suggest that electron dephasing times as long as ~ 300 ps are possible even at this high lling factor (v = 6:6) in higher mobility samples (> 10^{7} cm^{2} V^{-1} s^{-1}) that have lower impurity concentrations and where the cyclotron mobility at this carrier concentration would be limited by acoustic deformation potential scattering.
Maslar, J. E.; Dorsten, J. F.; Bohn, P. W.; Agarwala, S.; Adesida, I.; Caneau, C.; Bhat, R.
1993-10-01
Raman scattering by coupled longitudinal optic phonons and two-dimensional electron gas electrons in In0.53Ga0.47As-In0.52Al0.48As δ-doped heterostructures provides a powerful probe of electronic properties in these In-based structures. The two highest frequency modes, of the three coupled electron-phonon modes expected in this system, were observed, with the highest frequency mode being identified in InGaAs-based systems. The large dispersion of this mode makes it a particularly sensitive probe for changes in such properties as carrier concentration and subband energy. For structures with higher carrier concentrations coupling of the longitudinal optic phonon to multiple electron intersubband transitions is resolved. These measurements are particularly useful for heavily doped structures for which room-temperature Hall measurements cannot distinguish channel electrons from those in parallel conduction paths.
Djouder, M.; Kermoun, F.; Mitiche, M. D.; Lamrous, O.
2016-01-01
Dust particles observed in universe as well as in laboratory and technological plasma devices are still under investigation. At low temperature, these particles are strongly negatively charged and are able to form a 2D or 3D coulomb crystal. In this work, our aim was to check the ideal gas law validity for a 2D single-layer dust crystal recently reported in the literature. For this purpose, we have simulated, using the molecular dynamics method, its thermodynamic properties for different values of dust particles number and confinement parameters. The obtained results have allowed us to invalidate the ideal gas behaviour and to propose an effective equation of state which assumes a near zero dust temperature. Furthermore, the value of the calculated sound velocity was found to be in a good agreement with experimental data published elsewhere.
Energy Technology Data Exchange (ETDEWEB)
Djouder, M., E-mail: djouder-madjid@ummto.dz; Kermoun, F.; Mitiche, M. D.; Lamrous, O. [Laboratoire de Physique et Chimie Quantique, Université Mouloud Mammeri Tizi-Ouzou, BP 17 RP, 15000 Tizi-Ouzou (Algeria)
2016-01-15
Dust particles observed in universe as well as in laboratory and technological plasma devices are still under investigation. At low temperature, these particles are strongly negatively charged and are able to form a 2D or 3D coulomb crystal. In this work, our aim was to check the ideal gas law validity for a 2D single-layer dust crystal recently reported in the literature. For this purpose, we have simulated, using the molecular dynamics method, its thermodynamic properties for different values of dust particles number and confinement parameters. The obtained results have allowed us to invalidate the ideal gas behaviour and to propose an effective equation of state which assumes a near zero dust temperature. Furthermore, the value of the calculated sound velocity was found to be in a good agreement with experimental data published elsewhere.
Energy Technology Data Exchange (ETDEWEB)
Freedsman, J. J., E-mail: freedy54@gmail.com; Watanabe, A.; Urayama, Y. [Research Center for Nano-Devices and Advanced Materials, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466 8555 (Japan); Egawa, T., E-mail: egawa.takashi@nitech.ac.jp [Research Center for Nano-Devices and Advanced Materials, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466 8555 (Japan); Innovation Center for Multi-Business of Nitride Semiconductors, Nagoya Institute of Technology, Gokiso-cho, Showa-ku, Nagoya 466 8555 (Japan)
2015-09-07
The authors report on Al{sub 2}O{sub 3}/Al{sub 0.85}In{sub 0.15}N/GaN Metal-Oxide-Semiconductor High-Electron-Mobility Transistor (MOS-HEMT) on Si fabricated by using atomic layer deposited Al{sub 2}O{sub 3} as gate insulator and passivation layer. The MOS-HEMT with the gate length of 2 μm exhibits excellent direct-current (dc) characteristics with a drain current maximum of 1270 mA/mm at a gate bias of 3 V and an off-state breakdown voltage of 180 V for a gate-drain spacing of 4 μm. Also, the 1 μm-gate MOS-HEMT shows good radio-frequency (rf) response such as current gain and maximum oscillation cut-off frequencies of 10 and 34 GHz, respectively. The capacitance-voltage characteristics at 1 MHz revealed significant increase in two-dimensional electron gas (2DEG) density for the MOS-HEMT compared to conventional Schottky barrier HEMTs. Analyses using drain-source conductivity measurements showed improvements in 2DEG transport characteristics for the MOS-HEMT. The enhancements in dc and rf performances of the Al{sub 2}O{sub 3}/Al{sub 0.85}In{sub 0.15}N/GaN MOS-HEMT are attributed to the improvements in 2DEG characteristics.
Directory of Open Access Journals (Sweden)
Z. Q. Liu
2013-05-01
Full Text Available The relative importance of atomic defects and electron transfer in explaining conductivity at the crystalline LaAlO_{3}/SrTiO_{3} interface has been a topic of debate. Metallic interfaces with similar electronic properties produced by amorphous oxide overlayers on SrTiO_{3} [Y. Chen et al., Nano Lett. 11, 3774 (2011NALEFD1530-698410.1021/nl201821j; S. W. Lee et al., Nano Lett. 12, 4775 (2012NALEFD1530-698410.1021/nl302214x] have called in question the original polarization catastrophe model [N. Nakagawa et al., Nature Mater. 5, 204 (2006NMAACR1476-112210.1038/nmat1569]. We resolve the issue by a comprehensive comparison of (100-oriented SrTiO_{3} substrates with crystalline and amorphous overlayers of LaAlO_{3} of different thicknesses prepared under different oxygen pressures. For both types of overlayers, there is a critical thickness for the appearance of conductivity, but its value is always 4 unit cells (around 1.6 nm for the oxygen-annealed crystalline case, whereas in the amorphous case, the critical thickness could be varied in the range 0.5 to 6 nm according to the deposition conditions. Subsequent ion milling of the overlayer restores the insulating state for the oxygen-annealed crystalline heterostructures but not for the amorphous ones. Oxygen post-annealing removes the oxygen vacancies, and the interfaces become insulating in the amorphous case. However, the interfaces with a crystalline overlayer remain conducting with reduced carrier density. These results demonstrate that oxygen vacancies are the dominant source of mobile carriers when the LaAlO_{3} overlayer is amorphous, while both oxygen vacancies and polarization catastrophe contribute to the interface conductivity in unannealed crystalline LaAlO_{3}/SrTiO_{3} heterostructures, and the polarization catastrophe alone accounts for the conductivity in oxygen-annealed crystalline LaAlO_{3}/SrTiO_{3} heterostructures. Furthermore, we find that the crystallinity of the La
Topological states in a two-dimensional metal alloy in Si surface: BiAg/Si(111)-4 ×4 surface
Zhang, Xiaoming; Cui, Bin; Zhao, Mingwen; Liu, Feng
2018-02-01
A bridging topological state with a conventional semiconductor platform offers an attractive route towards future spintronics and quantum device applications. Here, based on first-principles and tight-binding calculations, we demonstrate the existence of topological states hosted by a two-dimensional (2D) metal alloy in a Si surface, the BiAg/Si(111)-4 ×4 surface, which has already been synthesized experimentally. It exhibits a topological insulating state with an energy gap of 71 meV (˜819 K ) above the Fermi level and a topological metallic state with quasiquantized conductance below the Fermi level. The underlying mechanism leading to the formation of such nontrivial states is revealed by analysis of the "charge-transfer" and "orbital-filtering" effect of the Si substrate. A minimal effective tight-binding model is employed to reveal the formation mechanism of the topological states. Our finding opens opportunities to detect topological states and measure its quantized conductance in a large family of 2D surface metal alloys, which have been or are to be grown on semiconductor substrates.
Gor'kov, L. P.
2015-06-01
To gain an insight into the origin of tunable two-dimensional (2D) electronic liquid at the interfaces of transition-metal oxides, we address properties of a conducting layer on the light-irradiated surfaces of SrTiO3; the energy spectrum of the latter is known and consists of the titanium dxz/dyz and dxy bands. Recently, Santander-Syro et al (2014 Nature Mater. 13 1085) revealed that the dxy bands actually comprise two chiral branches with the Kramers degeneracy at the zone center lifted in the absence of a magnetic moment. We suggest that interacting electrons on the irradiated SrTiO3 go over into a magnetic phase as the result of one of the instabilities of the 2D Fermi liquid with exchange interactions, and point out the concrete antiferromagnetic order parameter. Large energy scales of the order of Fermi energy ∼0.1 eV inherent in this mechanism warrant stability of the magnetic ground state against ever-present effects of disorder. Arguments are given that electrons at the irradiated SrTiO3 surface and at the LaAlO3/SrTiO3 interfaces undergo a kind of first-order transformation into one and the same phase of the 2D electronic Fermi liquid with reduced magnetic symmetry.
DEFF Research Database (Denmark)
Chen, Yunzhong; Bovet, N.; Trier, Felix
2013-01-01
of magnitude higher than those of hitherto-investigated perovskite-type interfaces are obtained. The spinel/perovskite twodimensional electron gas, where the two-dimensional conduction character is revealed by quantum magnetoresistance oscillations, is found to result from interface-stabilized oxygen vacancies...
Cui, Peng; Lin, Zhaojun; Fu, Chen; Liu, Yan; Lv, Yuanjie
2017-10-01
Taking into consideration the resistance variation in the free-contact area versus the gate bias, an applicable method to determine the electron mobility in AlGaN/GaN heterostructure field-effect transistors was presented. Based on the measured capacitance-voltage and current-voltage curves, the new method employed iteration calculation with different scattering mechanisms. Compared to the electron mobility calculated by the traditional method, the electron mobility calculated by the new method shows an apparent difference, especially for the device with a larger gate length. This difference originates from the device with a larger gate length that has a stronger polarization Coulomb field scattering. At last, the correctness and necessity of this method was demonstrated by the comparison between the experimental and calculated transconductance values.
Liu, Z. Q.; Li, C. J.; Lü, W. M.; Huang, X. H.; Huang, Z.; Zeng, S. W.; Qiu, X. P.; Huang, L. S.; Annadi, A.; Chen, J. S.; Coey, J. M. D.; Venkatesan, T.; Ariando
2013-01-01
The relative importance of atomic defects and electron transfer in explaining conductivity at the crystalline LaAlO_{3}/SrTiO_{3} interface has been a topic of debate. Metallic interfaces with similar electronic properties produced by amorphous oxide overlayers on SrTiO_{3} [Y. Chen et al., Nano Lett. 11, 3774 (2011)NALEFD1530-698410.1021/nl201821j; S. W. Lee et al., Nano Lett. 12, 4775 (2012)NALEFD1530-698410.1021/nl302214x] have called in question the original polarization catastrophe model...
International Nuclear Information System (INIS)
Lin, J.; Millis, A.J.
2011-01-01
We calculate the frequency-dependent longitudinal (σ xx ) and Hall (σ xy ) conductivities for two-dimensional metals with thermally disordered antiferromagnetism using a generalization of a theoretical model, involving a one-loop quasistatic fluctuation approximation, which was previously used to calculate the electron self-energy. The conductivities are calculated from the Kubo formula, with current vertex function treated in a conserving approximation satisfying the Ward identity. In order to obtain a finite dc limit, we introduce phenomenologically impurity scattering, characterized by a relaxation time τ. σ xx ((Omega)) satisfies the f-sum rule. For the infinitely peaked spin-correlation function, χ(q)∝(delta)(q-Q), we recover the expressions for the conductivities in the mean-field theory of the ordered state. When the spin-correlation length ζ is large but finite, both σ xx and σ xy show behaviors characteristic of the state with long-range order. The calculation runs into difficulty for (Omega) ∼ xx ((Omega)) and σ xy ((Omega)) are qualitatively consistent with data on electron-doped cuprates when (Omega) > 1/τ.
2014-11-17
mobilities can be obtained in the future by controlling the competing effects of interface strain and electron confinement. Ongoing work therefore... strain . This will necessitate the growth of a thin film of ZnO between the ZnO single crystal substrate and the ZnMgO thin film. 15...profile of Mg. .............................................................................................. 8 Figure 5: Longitudinal magnetoresistance
Gate-tunable polarized phase of two-dimensional electrons at the LaAlO3/SrTiO3 interface.
Joshua, Arjun; Ruhman, Jonathan; Pecker, Sharon; Altman, Ehud; Ilani, Shahal
2013-06-11
Controlling the coupling between localized spins and itinerant electrons can lead to exotic magnetic states. A novel system featuring local magnetic moments and extended 2D electrons is the interface between LaAlO3 and SrTiO3. The magnetism of the interface, however, was observed to be insensitive to the presence of these electrons and is believed to arise solely from extrinsic sources like oxygen vacancies and strain. Here we show the existence of unconventional electronic phases in the LaAlO3/SrTiO3 system pointing to an underlying tunable coupling between itinerant electrons and localized moments. Using anisotropic magnetoresistance and anomalous Hall effect measurements in a unique in-plane configuration, we identify two distinct phases in the space of carrier density and magnetic field. At high densities and fields, the electronic system is strongly polarized and shows a response, which is highly anisotropic along the crystalline directions. Surprisingly, below a density-dependent critical field, the polarization and anisotropy vanish whereas the resistivity sharply rises. The unprecedented vanishing of the easy axes below a critical field is in sharp contrast with other coupled magnetic systems and indicates strong coupling with the moments that depends on the symmetry of the itinerant electrons. The observed interplay between the two phases indicates the nature of magnetism at the LaAlO3/SrTiO3 interface as both having an intrinsic origin and being tunable.
Patil, Prasanna Dnyaneshwar
Investigations performed in order to understand the electronic and optoelectronic properties of field effect transistors based on few layers of 2D Copper Indium Selenide (CuIn7Se11) are reported. In general, field effect transistors (FETs), electric double layer field effect transistors (EDL-FETs), and photodetectors are crucial part of several electronics based applications such as tele-communication, bio-sensing, and opto-electronic industry. After the discovery of graphene, several 2D semiconductor materials like TMDs (MoS2, WS2, and MoSe2 etc.), group III-VI materials (InSe, GaSe, and SnS2 etc.) are being studied rigorously in order to develop them as components in next generation FETs. Traditionally, thin films of ternary system of Copper Indium Selenide have been extensively studied and used in optoelectronics industry as photoactive component in solar cells. Thus, it is expected that atomically thin 2D layered structure of Copper Indium Selenide can have optical properties that could potentially be more advantageous than its thin film counterpart and could find use for developing next generation nano devices with utility in opto/nano electronics. Field effect transistors were fabricated using few-layers of CuIn7Se11 flakes, which were mechanically exfoliated from bulk crystals grown using chemical vapor transport technique. Our FET transport characterization measurements indicate n-type behavior with electron field effect mobility microFE ≈ 36 cm2 V-1 s-1 at room temperature when Silicon dioxide (SiO2) is used as a back gate. We found that in such back gated field effect transistor an on/off ratio of 104 and a subthreshold swing ≈ 1 V/dec can be obtained. Our investigations further indicate that Electronic performance of these materials can be increased significantly when gated from top using an ionic liquid electrolyte [1-Butyl-3-methylimidazolium hexafluorophosphate (BMIM-PF6)]. We found that electron field effect mobility microFE can be increased from
Dirac cones in two-dimensional borane
Martinez-Canales, Miguel; Galeev, Timur R.; Boldyrev, Alexander I.; Pickard, Chris J.
2017-11-01
We introduce two-dimensional borane, a single-layered material of BH stoichiometry, with promising electronic properties. We show that, according to density functional theory calculations, two-dimensional borane is semimetallic, with two symmetry-related Dirac cones meeting right at the Fermi energy Ef. The curvature of the cones is lower than in graphene, thus closer to the ideal linear dispersion. Its structure, formed by a puckered trigonal boron network with hydrogen atoms connected to each boron atom, can be understood as distorted, hydrogenated borophene [Mannix et al., Science 350, 1513 (2015), 10.1126/science.aad1080]. Chemical bonding analysis reveals the boron layer in the network being bound by delocalized four-center two-electron σ bonds. Finally, we suggest high pressure could be a feasible route to synthesize two-dimensional borane.
Two-dimensional confinement of heavy fermions
International Nuclear Information System (INIS)
Shishido, Hiroaki; Shibauchi, Takasada; Matsuda, Yuji; Terashima, Takahito
2010-01-01
Metallic systems with the strongest electron correlations are realized in certain rare-earth and actinide compounds whose physics are dominated by f-electrons. These materials are known as heavy fermions, so called because the effective mass of the conduction electrons is enhanced via correlation effects up to as much as several hundreds times the free electron mass. To date the electronic structure of all heavy-fermion compounds is essentially three-dimensional. Here we report on the first realization of a two-dimensional heavy-fermion system, where the dimensionality is adjusted in a controllable fashion by fabricating heterostructures using molecular beam epitaxy. The two-dimensional heavy fermion system displays striking deviations from the standard Fermi liquid low-temperature electronic properties. (author)
Sakaki, Yukiya; Yamada, Tomoaki; Matsui, Chihiro; Yamaga, Yusuke; Takeuchi, Ken
2018-04-01
In order to improve performance of solid-state drives (SSDs), hybrid SSDs have been proposed. Hybrid SSDs consist of more than two types of NAND flash memories or NAND flash memories and storage-class memories (SCMs). However, the cost of hybrid SSDs adopting SCMs is more expensive than that of NAND flash only SSDs because of the high bit cost of SCMs. This paper proposes unique hybrid SSDs with two-dimensional (2D) horizontal multi-level cell (MLC)/three-dimensional (3D) vertical triple-level cell (TLC) NAND flash memories to achieve higher cost-performance. The 2D-MLC/3D-TLC hybrid SSD achieves up to 31% higher performance than the conventional 2D-MLC/2D-TLC hybrid SSD. The factors of different performance between the proposed hybrid SSD and the conventional hybrid SSD are analyzed by changing its block size, read/write/erase latencies, and write unit of 3D-TLC NAND flash memory, by means of a transaction-level modeling simulator.
Asymptotics for Two-dimensional Atoms
DEFF Research Database (Denmark)
Nam, Phan Thanh; Portmann, Fabian; Solovej, Jan Philip
2012-01-01
We prove that the ground state energy of an atom confined to two dimensions with an infinitely heavy nucleus of charge $Z>0$ and $N$ quantum electrons of charge -1 is $E(N,Z)=-{1/2}Z^2\\ln Z+(E^{\\TF}(\\lambda)+{1/2}c^{\\rm H})Z^2+o(Z^2)$ when $Z\\to \\infty$ and $N/Z\\to \\lambda$, where $E^{\\TF}(\\lambd......We prove that the ground state energy of an atom confined to two dimensions with an infinitely heavy nucleus of charge $Z>0$ and $N$ quantum electrons of charge -1 is $E(N,Z)=-{1/2}Z^2\\ln Z+(E^{\\TF}(\\lambda)+{1/2}c^{\\rm H})Z^2+o(Z^2)$ when $Z\\to \\infty$ and $N/Z\\to \\lambda$, where $E......^{\\TF}(\\lambda)$ is given by a Thomas-Fermi type variational problem and $c^{\\rm H}\\approx -2.2339$ is an explicit constant. We also show that the radius of a two-dimensional neutral atom is unbounded when $Z\\to \\infty$, which is contrary to the expected behavior of three-dimensional atoms....
International Nuclear Information System (INIS)
Kurowski, Ludovic; Bernard, Dorothee; Constant, Eugene; Decoster, Didier
2004-01-01
Hydrogen incorporation in n-type Si-doped GaAs epilayers is a well-known process which leads to the neutralization of the active Si impurities with the formation of SiH complexes. Recently, we have shown that SiH complex dissociation and, consequently, Si-dopant reactivation could occur when the epilayers are exposed to an electron beam. Two epilayers have been studied: the first is a 0.35 μm thick hydrogenated Si-doped GaAs epilayer and the second is Si planar-doped AlGaAs/GaAs/InGaAs heterostructures. Firstly, Hall effect measurements have been carried out on the epilayers exposed, after RF hydrogen plasma exposition, to increasing electron doses with different injection energies. For the 2D heterostructures, we have observed that the free carrier density N s does not vary significantly for weak electron densities. This reactivation presents a threshold value, contrary to the 0.35 μm epilayer in which N s varies quite linearly. It will be shown that such phenomena might be attributed to the filling of surface states as the dopants are progressively reactivated. Then, using a high spatial resolution electron beam lithography system, nanometric conductive patterns have been fabricated starting from hydrogenated epilayers. Electric measurements have been performed and the results obtained show that about 15 nm spatial resolution could be expected. In conclusion, taking into account this spatial resolution, the high spatial contrast of conductivity which could be expected due to the existence of an electron dose threshold, and the high mobility of the AlGaAs/GaAs/InGaAs heterostructure, the effects described in this paper could open a new way for the fabrication of III-V 1D or 2D mesoscopic structures for electronic or optoelectronic applications
Directory of Open Access Journals (Sweden)
Syed Mukulika Dinara
2015-04-01
Full Text Available Enhancement of two dimensional electron gas (2DEG concentrations at Al0.3Ga0.7N/GaN hetero interface after a-Si3N4 (SiN passivation has been investigated from non-destructive High Resolution X-ray Diffraction (HRXRD analysis, depletion depth and capacitance-voltage (C-V profile measurement. The crystalline quality and strained in-plane lattice parameters of Al0.3Ga0.7N and GaN were evaluated from double axis (002 symmetric (ω-2θ diffraction scan and double axis (105 asymmetric reciprocal space mapping (DA RSM which revealed that the tensile strain of the Al0.3Ga0.7N layer increased by 15.6% after SiN passivation. In accordance with the predictions from theoretical solution of Schrödinger-Poisson’s equations, both electrochemical capacitance voltage (ECV depletion depth profile and C-V characteristics analyses were performed which implied effective 9.5% increase in 2DEG carrier density after passivation. The enhancement of polarization charges results from increased tensile strain in the Al0.3Ga0.7N layer and also due to the decreased surface states at the interface of SiN/Al0.3Ga0.7N layer, effectively improving the carrier confinement at the interface.
Bera, A. K.; Yusuf, S. M.; Kumar, Amit; Ritter, C.
2017-03-01
The crystal structure, magnetic ground state, and the temperature-dependent microscopic spin-spin correlations of the frustrated honeycomb lattice antiferromagnet N a2C o2Te O6 have been investigated by powder neutron diffraction. A long-range antiferromagnetic (AFM) ordering has been found below TN˜24.8 K . The magnetic ground state, determined to be zigzag antiferromagnetic and characterized by a propagation vector k =(1 /2 0 0 ) , occurs due to the competing exchange interactions up to third-nearest neighbors within the honeycomb lattice. The exceptional existence of a limited magnetic correlation length along the c axis (perpendicular to the honeycomb layers in the a b planes) has been found even at 1.8 K, well below the TN˜24.8 K . The observed limited correlation along the c axis is explained by the disorder distribution of the Na ions within the intermediate layers between honeycomb planes. The reduced ordered moments mCo (1 )=2.77 (3 ) μB/C o2 + and mCo (2 )=2.45 (2 ) μB/C o2 + at 1.8 K reflect the persistence of spin fluctuations in the ordered state. Above TN˜24.8 K , the presence of short-range magnetic correlations, manifested by broad diffuse magnetic peaks in the diffraction patterns, has been found. Reverse Monte Carlo analysis of the experimental diffuse magnetic scattering data reveals that the spin correlations are mainly confined within the two-dimensional honeycomb layers (a b plane) with a correlation length of ˜12 Å at 25 K. The nature of the spin arrangements is found to be similar in both the short-range and long-range ordered magnetic states. This implies that the short-range correlation grows with decreasing temperature and leads to the zigzag AFM ordering at T ≤TN . The present study provides a comprehensive picture of the magnetic correlations over the temperature range above and below the TN and their relation to the crystal structure. The role of intermediate soft Na layers on the magnetic coupling between honeycomb planes is
Interaction of two-dimensional magnetoexcitons
Dumanov, E. V.; Podlesny, I. V.; Moskalenko, S. A.; Liberman, M. A.
2017-04-01
We study interaction of the two-dimensional magnetoexcitons with in-plane wave vector k→∥ = 0 , taking into account the influence of the excited Landau levels (ELLs) and of the external electric field perpendicular to the surface of the quantum well and parallel to the external magnetic field. It is shown that the account of the ELLs gives rise to the repulsion between the spinless magnetoexcitons with k→∥ = 0 in the Fock approximation, with the interaction constant g decreasing inverse proportional to the magnetic field strength B (g (0) ∼ 1 / B) . In the presence of the perpendicular electric field the Rashba spin-orbit coupling (RSOC), Zeeman splitting (ZS) and nonparabolicity of the heavy-hole dispersion law affect the Landau quantization of the electrons and holes. They move along the new cyclotron orbits, change their Coulomb interactions and cause the interaction between 2D magnetoexcitons with k→∥ = 0 . The changes of the Coulomb interactions caused by the electrons and by the holes moving with new cyclotron orbits are characterized by some coefficients, which in the absence of the electric field turn to be unity. The differences between these coefficients of the electron-hole pairs forming the magnetoexcitons determine their affinities to the interactions. The interactions between the homogeneous, semihomogeneous and heterogeneous magnetoexcitons forming the symmetric states with the same signs of their affinities are attractive whereas in the case of different sign affinities are repulsive. In the heterogeneous asymmetric states the interactions have opposite signs in comparison with the symmetric states. In all these cases the interaction constant g have the dependence g (0) 1 /√{ B} .
Quantum computation with two-dimensional graphene quantum dots
International Nuclear Information System (INIS)
Li Jie-Sen; Li Zhi-Bing; Yao Dao-Xin
2012-01-01
We study an array of graphene nano sheets that form a two-dimensional S = 1/2 Kagome spin lattice used for quantum computation. The edge states of the graphene nano sheets are used to form quantum dots to confine electrons and perform the computation. We propose two schemes of bang-bang control to combat decoherence and realize gate operations on this array of quantum dots. It is shown that both schemes contain a great amount of information for quantum computation. The corresponding gate operations are also proposed. (condensed matter: electronic structure, electrical, magnetic, and optical properties)
Analytical simulation of two dimensional advection dispersion ...
African Journals Online (AJOL)
The study was designed to investigate the analytical simulation of two dimensional advection dispersion equation of contaminant transport. The steady state flow condition of the contaminant transport where inorganic contaminants in aqueous waste solutions are disposed of at the land surface where it would migrate ...
Analytical Simulation of Two Dimensional Advection Dispersion ...
African Journals Online (AJOL)
ADOWIE PERE
ABSTRACT: The study was designed to investigate the analytical simulation of two dimensional advection dispersion equation of contaminant transport. The steady state flow condition of the contaminant transport where inorganic contaminants in aqueous waste solutions are disposed of at the land surface where it would ...
Two-dimensional topological photonic systems
Sun, Xiao-Chen; He, Cheng; Liu, Xiao-Ping; Lu, Ming-Hui; Zhu, Shi-Ning; Chen, Yan-Feng
2017-09-01
The topological phase of matter, originally proposed and first demonstrated in fermionic electronic systems, has drawn considerable research attention in the past decades due to its robust transport of edge states and its potential with respect to future quantum information, communication, and computation. Recently, searching for such a unique material phase in bosonic systems has become a hot research topic worldwide. So far, many bosonic topological models and methods for realizing them have been discovered in photonic systems, acoustic systems, mechanical systems, etc. These discoveries have certainly yielded vast opportunities in designing material phases and related properties in the topological domain. In this review, we first focus on some of the representative photonic topological models and employ the underlying Dirac model to analyze the edge states and geometric phase. On the basis of these models, three common types of two-dimensional topological photonic systems are discussed: 1) photonic quantum Hall effect with broken time-reversal symmetry; 2) photonic topological insulator and the associated pseudo-time-reversal symmetry-protected mechanism; 3) time/space periodically modulated photonic Floquet topological insulator. Finally, we provide a summary and extension of this emerging field, including a brief introduction to the Weyl point in three-dimensional systems.
Tuning spin transport across two-dimensional organometallic junctions
Liu, Shuanglong; Wang, Yun-Peng; Li, Xiangguo; Fry, James N.; Cheng, Hai-Ping
2018-01-01
We study via first-principles modeling and simulation two-dimensional spintronic junctions made of metal-organic frameworks consisting of two Mn-phthalocyanine ferromagnetic metal leads and semiconducting Ni-phthalocyanine channels of various lengths. These systems exhibit a large tunneling magnetoresistance ratio; the transmission functions of such junctions can be tuned using gate voltage by three orders of magnitude. We find that the origin of this drastic change lies in the orbital alignment and hybridization between the leads and the center electronic states. With physical insight into the observed on-off phenomenon, we predict a gate-controlled spin current switch based on two-dimensional crystallines and offer general guidelines for designing spin junctions using 2D materials.
Giant tunability of the two-dimensional electron gas at the interface of γ-Al_{2}O_{3}/SrTiO_{3}
DEFF Research Database (Denmark)
Niu, Wei; Zhang, Yu; Gan, Yulin
2017-01-01
a dielectric solid insulator, i.e. in the configuration of conventional field-effect transistors. To surpass this long-standing limit, we used ionic liquids as the dielectric layer for electrostatic gating of oxide interfaces in an electric double layer transistor (EDLT) configuration. Herein, we reported......Two-dimensional electron gases (2DEGs) formed at the interface between two oxide insulators provide a rich platform for the next generation of electronic devices. However, their high carrier density makes it rather challenging to control the interface properties under a low electric field through...
Lee, Eunsook; Kim, D. H.; Kim, Hyun Woo; Denlinger, J. D.; Kim, Heejung; Kim, Junwon; Kim, Kyoo; Min, B. I.; Min, B. H.; Kwon, Y. S.; Kang, J.-S.
2016-01-01
The electronic structure of a charge density wave (CDW) system PrTe3 and its modulated structure in the CDW phase have been investigated by employing ARPES, XAS, Pr 4 f RPES, and first-principles band structure calculation. Pr ions are found to be nearly trivalent, supporting the CDW instability in the metallic Te sheets through partial filling. Finite Pr 4 f spectral weight is observed near the Fermi level, suggesting the non-negligible Pr 4 f contribution to the CDW formation through the Pr 4 f -Te 5p hybridization. The two-fold symmetric features in the measured Fermi surface (FS) of PrTe3 are explained by the calculated FS for the assumed 7 × 1 CDW supercell formation in Te sheets. The shadow bands and the corresponding very weak FSs are observed, which originate from both the band folding due to the 3D interaction of Te sheets with neighboring Pr-Te layers and that due to the CDW-induced FS reconstruction. The straight vertical FSs are observed along kz, demonstrating the nearly 2D character for the near-EF states. The observed linear dichroism reveals the in-plane orbital character of the near-EF Te 5p states. PMID:27453329
Quasi-two-dimensional holography
International Nuclear Information System (INIS)
Kutzner, J.; Erhard, A.; Wuestenberg, H.; Zimpfer, J.
1980-01-01
The acoustical holography with numerical reconstruction by area scanning is memory- and time-intensive. With the experiences by the linear holography we tried to derive a scanning for the evaluating of the two-dimensional flaw-sizes. In most practical cases it is sufficient to determine the exact depth extension of a flaw, whereas the accuracy of the length extension is less critical. For this reason the applicability of the so-called quasi-two-dimensional holography is appropriate. The used sound field given by special probes is divergent in the inclined plane and light focussed in the perpendicular plane using cylindrical lenses. (orig.) [de
Two dimensional plasma simulation code
International Nuclear Information System (INIS)
Hazak, G.; Boneh, Y.; Goshen, Sh.; Oreg, J.
1977-03-01
An electrostatic two-dimensional particle code for plasma simulation is described. Boundary conditions which take into account the finiteness of the system are presented. An analytic solution for the case of crossed fields plasma acceleration is derived. This solution serves as a check on a computer test run
Photodetectors based on graphene, other two-dimensional materials and hybrid systems.
Koppens, F H L; Mueller, T; Avouris, Ph; Ferrari, A C; Vitiello, M S; Polini, M
2014-10-01
Graphene and other two-dimensional materials, such as transition metal dichalcogenides, have rapidly established themselves as intriguing building blocks for optoelectronic applications, with a strong focus on various photodetection platforms. The versatility of these material systems enables their application in areas including ultrafast and ultrasensitive detection of light in the ultraviolet, visible, infrared and terahertz frequency ranges. These detectors can be integrated with other photonic components based on the same material, as well as with silicon photonic and electronic technologies. Here, we provide an overview and evaluation of state-of-the-art photodetectors based on graphene, other two-dimensional materials, and hybrid systems based on the combination of different two-dimensional crystals or of two-dimensional crystals and other (nano)materials, such as plasmonic nanoparticles, semiconductors, quantum dots, or their integration with (silicon) waveguides.
Energy Technology Data Exchange (ETDEWEB)
Schumacher, O.
2007-07-20
In this thesis magneto-resistance studies on evenly curved two-dimensional electron systems in cylindric geometry are presented and discussed. A principle first introduced by Prinz and co-workers in 1998 enables us to roll up thin semiconductor layer systems by taking advantage of internal elastic strain. The radius of such a semiconductor tube can be adjusted ranging from a few nanometers up to several micrometers. The tubes' shape and place on the substrate can be defined by lithographic methods which are presented in this work. Furthermore, we show rolled-up structures containing a two-dimensional electron system in the tube wall. With a special lithographic procedure we are able to structure, to contact and to roll up these 2D-electron-gases in Hall geometry. As a result, a cylindric two-dimensional electron system is produced, which experiences a modulation of the perpendicular magnetic field component. The radius of curvature of our structures is about 10 {mu}m, the carrier mobility is optimized to values up to 125,000 cm{sup 2}/Vs. In transport experiments on curved Hall bars containing two dimensional electron systems two Hall bar orientations, with respect to the curvature, may be distinguished. In this work both orientations, i.e. with a Hall bar along the tube curvature as well as a Hall bar along the tube axis, are presented and discussed. Measurements on Hall bars along the curvature show signatures in the longitudinal resistance, which can be understood with the help of the Landauer-Buttiker-formalism and the model of magnetic barriers. For Hall bars oriented along the tube axis the perpendicular magnetic field component averaged over the width of the bar defines the minimum position of the Shubnikov-de Haas-oscillations as well as the slope of the Hall resistance. Furthermore, measurements on so-called van the Pauw-lamellas are presented. In this geometry the magneto-resistance shows a slope which refers to highly mobile conditions at the zero
Lowe, Ross H.; Karschner, Erin L.; Schwilke, Eugene W.; Barnes, Allan J.; Huestis, Marilyn A.
2007-01-01
A two-dimensional (2D) gas chromatography/electron impact-mass spectrometry (GC/EI-MS) method for simultaneous quantification of Δ9-tetrahydrocannabinol (THC), 11-hydroxy-Δ9-tetrahydrocannabinol (11-OH-THC), and 11-nor-Δ9-tetrahydrocannabinol-9-carboxylic acid (THCCOOH) in human plasma was developed and validated. The method employs 2D capillary GC and cryofocusing for enhanced resolution and sensitivity. THC, 11-OH-THC, and THCCOOH were extracted by precipitation with acetonitrile followed b...
Plasmonics with two-dimensional conductors
Yoon, Hosang; Yeung, Kitty Y. M.; Kim, Philip; Ham, Donhee
2014-01-01
A wealth of effort in photonics has been dedicated to the study and engineering of surface plasmonic waves in the skin of three-dimensional bulk metals, owing largely to their trait of subwavelength confinement. Plasmonic waves in two-dimensional conductors, such as semiconductor heterojunction and graphene, contrast the surface plasmonic waves on bulk metals, as the former emerge at gigahertz to terahertz and infrared frequencies well below the photonics regime and can exhibit far stronger subwavelength confinement. This review elucidates the machinery behind the unique behaviours of the two-dimensional plasmonic waves and discusses how they can be engineered to create ultra-subwavelength plasmonic circuits and metamaterials for infrared and gigahertz to terahertz integrated electronics. PMID:24567472
Optical Two Dimensional Fourier Transform Spectroscopy of Layered Metal Dichalcogenides
Dey, P.; Paul, J.; Stevens, C. E.; Kovalyuk, Z. D.; Kudrynskyi, Z. R.; Romero, A. H.; Cantarero, A.; Hilton, D. J.; Shan, J.; Karaiskaj, D.; Z. D. Kovalyuk; Z. R. Kudrynskyi Collaboration; A. H. Romero Collaboration; A. Cantarero Collaboration; D. J. Hilton Collaboration; J. Shan Collaboration
2015-03-01
Nonlinear two-dimensional Fourier transform (2DFT) measurements were used to study the mechanism of excitonic dephasing and probe the electronic structure of the excitonic ground state in layered metal dichalcogenides. Temperature-dependent 2DFT measurements were performed to probe exciton-phonon interactions. Excitation density dependent 2DFT measurements reveal exciton-exciton and exciton-carrier scattering, and the lower limit for the homogeneous linewidth of excitons on positively and negatively doped samples. U.S. Department of Energy, Office of Basic Energy Sciences, Division of Materials Sciences and Engineering under Award DE-SC0012635.
Vlasova, R M; Petrov, B V; Semkin, N D; Zhilyaeva, E I; Bogdanova, O A; Lyubovskaya, R N; Graja, A
2002-01-01
One studied the polarized spectra of reflection and spectra of optical transmission of theta-(BETS) sub 4 HgBr sub 4 (C sub 6 H sub 5 Cl) quasi-two-dimensional molecular conductor within 700-6500 cm sup - sup 1 range under 300-15 K temperatures and within 9000-40000 cm sup - sup 1 under 300 K for two principal directions within crystal plane parallel to conducting layers of BETS molecules. Under 300 K within IR region the spectra are characterized by the intensive essential peculiarities (1200-1400 cm sup - sup 1) caused by electron-oscillation coupling (EOC). At temperature drop within 180-80 K range one observes in the spectra a Lorentz term with omega sub t = 2900 cm sup - sup 1 and three extra bands within 800-1180 cm sup - sup 1 region caused by EOC. The derived results are indicative of unstable structural distortions along two principal directions in a crystal followed by formation of a charge density comparable wave
Directory of Open Access Journals (Sweden)
H. J. Harsan Ma
2015-06-01
Full Text Available We report emerging photoluminescence (PL of bilayer two-dimensional electron gases (2DEG in LaAlO3/SrTiO3 (LAO/STO systems. A strong blue PL emerges in bilayer-2DEGs in LAO/STO/LAO/STO which doesn’t show in LAO/STO. PL band in bilayer-2DEGs includes both nearly temperature independent Auger recombination and temperature dependent free electron trapping while it crossovers from Auger recombination to single carrier trapping in LAO/STO. The PL signal of free electron trapping appears at high temperatures and it is much stronger than Auger recombination in the conducting channel in bilayer 2DEGs. This observation shows that high mobility carriers dominate the carrier dynamics in bilayer-2DEGs in LAO/STO superlattices.
Two-dimensional critical phenomena
International Nuclear Information System (INIS)
Saleur, H.
1987-09-01
Two dimensional critical systems are studied using transformation to free fields and conformal invariance methods. The relations between the two approaches are also studied. The analytical results obtained generally depend on universality hypotheses or on renormalization group trajectories which are not established rigorously, so numerical verifications, mainly using the transfer matrix approach, are presented. The exact determination of critical exponents; the partition functions of critical models on toruses; and results as the critical point is approached are discussed [fr
Energy Technology Data Exchange (ETDEWEB)
Reinwald, Elisabeth
2009-06-25
In this thesis a two dimensional electron gas (2DEG) on a (110) cleavage plane of a GaAs/AlGaAs(001) heterostructure was produced by means of cleaved edge overgrowth (CEO) and modulated in two dimensions. The 2DEG was modulated in one direction by a superlattice of the subjacent GaAs/AlGaAs(001) heterostructure. A second modulation, perpendicular to the first was realized by local anodic oxidation (LAO) with an atomic force microscope (AFM). For the process of LAO an electric voltage is applied between the tip of the AFM and the surface of the GaAs. The natural water film on the surface acts as electrolyte so that the GaAs surface is locally oxidized underneath the AFM tip. This oxide leads to a band bending so that the 2DEG underneath the oxide is locally depleted. On these systems magnetotransport measurements revealed that it is actually possible to modulate 2DEGs on a sufficient large area by local anodic oxidation. On the cleaved surfaces the influence of the two dimensional modulation on the electron gas has been demonstrated. (orig.)
1983-01-01
Mobility in Inversion Layers toon Marcos H Degani and Oscar HIPl11ito 143 V 8 Shlkn soTwo-Dimenslonal Electrons Trapped n A liu Surface Critical...adsorbed on solid neon and electrons at the interface of phase- A HELIUM SURFACE separated He-e mixtures. Marcos If. Deliani and Oscar Hip6lito The...the d.c. value of Ic blk effect. It could also be cained by a dependence of the current wao another 3 lower. Increasing values of pas below the oe
Chen, M. J.; Ning, X. K.; Wang, Z. J.; Liu, P.; Wang, S. F.; Wang, J. L.; Fu, G. S.; Ma, S.; Liu, W.; Zhang, Z. D.
2018-01-01
The film thickness dependent transport properties of the LaNiO3 (LNO) layer epitaxially grown on LaAlO3/SrTiO3 (LAO) 2-dimensional electronic gas (2DEG) have been investigated. The ultrathin LNO films grown on the 2DEG have a sheet resistance below the values of h/e2 in all temperature ranges. The electron density is enhanced by more than one order of magnitude by capping LNO films. X-ray photoelectron spectroscopy shows that the interface undergoes unambiguous charge transfer and electronic reconstruction, leading to modulation doping of such atomically engineered complex oxide heterointerfaces. The polar-catastrophe of the 2DEG is directly linked to the electronic structure and transport properties of the LNO. The transport properties can be well modulated by the thickness of the LAO in the 2DEG, and the data can be well fitted with the polar-catastrophe scenario. These results suggest a general approach to tunable functional films in oxide heterostructures with the 2DEG.
Denega, S.Z.; Last, Thorsten; Liu, J.; Slachter, A.; Rizo, P.J.; Loosdrecht, P.H.M. van; Wees, B.J. van; Reuter, D.; Wieck, A.D.; Wal, C.H. van der
2010-01-01
We report a study of suppressed spin dephasing for quasi-one-dimensional electron ensembles in wires etched into a GaAs/AlGaAs heterojunction system. Time-resolved Kerr-rotation measurements show a suppression that is most pronounced for wires along the [110] crystal direction. This is the
Critical currents in ballistic two-dimensional InAs-based superconducting weak links
Heida, J.P.; Wees, B.J. van; Klapwijk, T.M.; Borghs, G.
1999-01-01
The critical supercurrent Ic carried by a short (0.3 to 0.8 µm) ballistic two-dimensional InAs-based electron gas between superconducting niobium electrodes is studied. In relating the maximum value to the resistance of the weak link in the normal state Rn a much lower value is found than
Energy Technology Data Exchange (ETDEWEB)
Link, A.
2004-12-01
The aim of this PhD thesis is to investigate the electronic properties of electron and hole gases in GaN/AlGaN heterostructures. Particularly, a deeper and broadened understanding of scattering mechanisms and transport properties is in the focus of this work. The main experimental techniques used for this purpose are the study of Shubnikov-de Haas (SdH) effect and Hall measurements at low temperatures. By means of these magnetotransport measurements, a series of GaN/AlGaN heterostructures with different Al content of the AlGaN barrier were investigated. Since the sheet carrier density of the 2DEG in these semiconductor structures is strongly dependent on the Al content (n{sub s}=2 x 10{sup 12}-10{sup 13} cm{sup -2}), the variation of transport parameters was determined as a function of sheet carrier concentration. First, from the temperature dependence of the SdH oscillations the effective transport mass was calculated. A Hall bar structure with an additional gate contact was used as an alternative to tune the carrier density of a 2DEG system independent of varying structural parametes such as Al content. Thus, the scattering mechanisms were investigated in the carrier density region between 3 x 10{sup 12} and 9.5 x 10{sup 12} cm{sup -2}. The transport properties of subband electrons were studied for a 2DEG system with two occupied subbands. (orig.)
Energy Technology Data Exchange (ETDEWEB)
Kormondy, Kristy J.; Posadas, Agham B.; Demkov, Alexander A., E-mail: demkov@physics.utexas.edu [Department of Physics, University of Texas at Austin, Austin, Texas 78712 (United States); Ngo, Thong Q.; Ekerdt, John G. [Department of Chemical Engineering, University of Texas at Austin, Austin, Texas 78712 (United States); Lu, Sirong; Smith, David J.; McCartney, Martha R. [Department of Physics, Arizona State University, Tempe, Arizona 85287 (United States); Goble, Nicholas; Gao, Xuan P. A. [Department of Physics, Case Western Reserve University, Cleveland, Ohio 44106 (United States); Jordan-Sweet, Jean [IBM T.J. Watson Research Center, Yorktown Heights, New York 10598 (United States)
2015-03-07
In this paper, we report on the highly conductive layer formed at the crystalline γ-alumina/SrTiO{sub 3} interface, which is attributed to oxygen vacancies. We describe the structure of thin γ-alumina layers deposited by molecular beam epitaxy on SrTiO{sub 3} (001) at growth temperatures in the range of 400–800 °C, as determined by reflection-high-energy electron diffraction, x-ray diffraction, and high-resolution electron microscopy. In situ x-ray photoelectron spectroscopy was used to confirm the presence of the oxygen-deficient layer. Electrical characterization indicates sheet carrier densities of ∼10{sup 13 }cm{sup −2} at room temperature for the sample deposited at 700 °C, with a maximum electron Hall mobility of 3100 cm{sup 2}V{sup −1}s{sup −1} at 3.2 K and room temperature mobility of 22 cm{sup 2}V{sup −1}s{sup −1}. Annealing in oxygen is found to reduce the carrier density and turn a conductive sample into an insulator.
Czech Academy of Sciences Publication Activity Database
Klimo, O.; Psikal, J.; Tikhonchuk, V.T.; Weber, Stefan A.
2014-01-01
Roč. 56, č. 5 (2014), 055010 ISSN 0741-3335 R&D Projects: GA MŠk ED1.1.00/02.0061; GA MŠk EE2.3.20.0279 Grant - others:ELI Beamlines(XE) CZ.1.05/1.1.00/02.0061; LaserZdroj (OP VK 3)(XE) CZ.1.07/2.3.00/20.0279 Institutional support: RVO:68378271 Keywords : laser plasma interaction * stimulated Raman scattering * hot electrons * particle-in-cell simulation Subject RIV: BL - Plasma and Gas Discharge Physics Impact factor: 2.186, year: 2014
Strain-engineered growth of two-dimensional materials.
Ahn, Geun Ho; Amani, Matin; Rasool, Haider; Lien, Der-Hsien; Mastandrea, James P; Ager Iii, Joel W; Dubey, Madan; Chrzan, Daryl C; Minor, Andrew M; Javey, Ali
2017-09-20
The application of strain to semiconductors allows for controlled modification of their band structure. This principle is employed for the manufacturing of devices ranging from high-performance transistors to solid-state lasers. Traditionally, strain is typically achieved via growth on lattice-mismatched substrates. For two-dimensional (2D) semiconductors, this is not feasible as they typically do not interact epitaxially with the substrate. Here, we demonstrate controlled strain engineering of 2D semiconductors during synthesis by utilizing the thermal coefficient of expansion mismatch between the substrate and semiconductor. Using WSe 2 as a model system, we demonstrate stable built-in strains ranging from 1% tensile to 0.2% compressive on substrates with different thermal coefficient of expansion. Consequently, we observe a dramatic modulation of the band structure, manifested by a strain-driven indirect-to-direct bandgap transition and brightening of the dark exciton in bilayer and monolayer WSe 2 , respectively. The growth method developed here should enable flexibility in design of more sophisticated devices based on 2D materials.Strain engineering is an essential tool for modifying local electronic properties in silicon-based electronics. Here, Ahn et al. demonstrate control of biaxial strain in two-dimensional materials based on the growth substrate, enabling more complex low-dimensional electronics.
Two-dimensional capillary origami
International Nuclear Information System (INIS)
Brubaker, N.D.; Lega, J.
2016-01-01
We describe a global approach to the problem of capillary origami that captures all unfolded equilibrium configurations in the two-dimensional setting where the drop is not required to fully wet the flexible plate. We provide bifurcation diagrams showing the level of encapsulation of each equilibrium configuration as a function of the volume of liquid that it contains, as well as plots representing the energy of each equilibrium branch. These diagrams indicate at what volume level the liquid drop ceases to be attached to the endpoints of the plate, which depends on the value of the contact angle. As in the case of pinned contact points, three different parameter regimes are identified, one of which predicts instantaneous encapsulation for small initial volumes of liquid. - Highlights: • Full solution set of the two-dimensional capillary origami problem. • Fluid does not necessarily wet the entire plate. • Global energy approach provides exact differential equations satisfied by minimizers. • Bifurcation diagrams highlight three different regimes. • Conditions for spontaneous encapsulation are identified.
Two-dimensional capillary origami
Energy Technology Data Exchange (ETDEWEB)
Brubaker, N.D., E-mail: nbrubaker@math.arizona.edu; Lega, J., E-mail: lega@math.arizona.edu
2016-01-08
We describe a global approach to the problem of capillary origami that captures all unfolded equilibrium configurations in the two-dimensional setting where the drop is not required to fully wet the flexible plate. We provide bifurcation diagrams showing the level of encapsulation of each equilibrium configuration as a function of the volume of liquid that it contains, as well as plots representing the energy of each equilibrium branch. These diagrams indicate at what volume level the liquid drop ceases to be attached to the endpoints of the plate, which depends on the value of the contact angle. As in the case of pinned contact points, three different parameter regimes are identified, one of which predicts instantaneous encapsulation for small initial volumes of liquid. - Highlights: • Full solution set of the two-dimensional capillary origami problem. • Fluid does not necessarily wet the entire plate. • Global energy approach provides exact differential equations satisfied by minimizers. • Bifurcation diagrams highlight three different regimes. • Conditions for spontaneous encapsulation are identified.
Energy Technology Data Exchange (ETDEWEB)
Bose, Sumanta; Fan, W. J., E-mail: ewjfan@ntu.edu.sg; Zhang, D. H. [School of Electrical and Electronic Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798 (Singapore); OPTIMUS, Centre for OptoElectronics and Biophotonics, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798 (Singapore); Song, Zhigang [School of Electrical and Electronic Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798 (Singapore); State Key Laboratory of Superlattices and Microstructures, Institute of Semiconductors, Chinese Academy of Sciences, P.O. Box 912, Beijing 100083 (China)
2016-04-14
The effect of lateral size and vertical thickness of CdSe and CdS nanoplatelets (NPLs) on their electronic structure and optical properties are investigated using an effective-mass envelope function theory based on the 8-band k ⋅ p model with valence force field considerations. Volumetrically larger NPLs have lower photon emission energy due to limited quantum confinement, but a greater transition matrix element (TME) due to larger electron-hole wavefunction overlap. The optical gain characteristics depend on several factors such as TME, Fermi factor, carrier density, NPL dimensions, material composition, and dephasing rate. There is a red shift in the peak position, more so with an increase in thickness than lateral size. For an increasing carrier density, the gain spectrum undergoes a slight blue shift due to band filling effect. For a fixed carrier density, the Fermi factor is higher for volumetrically larger NPLs and so is the difference between the quasi-Fermi level separation and the effective bandgap. The transparency injection carrier density (and thus input current density threshold) is dimension dependent and falls for volumetrically larger NPLs, as they can attain the requisite exciton count for transparency with a relatively lower density. Between CdSe and CdS, CdSe has lower emission energy due to smaller bandgap, but a higher TME due to lower effective mass. CdS, however, has a higher so hole contribution due to a lower spin-orbit splitting energy. Both CdSe and CdS NPLs are suitable candidates for short-wavelength LEDs and lasers in the visible spectrum, but CdSe is expected to exhibit better optical performance.
International Nuclear Information System (INIS)
Haas, Florian
2014-01-01
broad component dominated by non-resonant contributions. The simultaneous analysis in bins of the three-pion invariant mass and the squared four-momentum transfer t' allowed to study resonant and non-resonant contributions in more detail. Of special interest is the Deck effect, a non-resonant production mechanism, leading to the same final state and assumed to contribute to the partial waves that also contain the a 1 (1260) and the spin-exotic π 1 (1600). The hybrid nature of the two established states π(1800) and π 2 (1880) was investigated. In addition the π 1 (1880) was confirmed as a resonance separate from the π 1 (1670). For the first time a study of the t' dependence on the level of partial waves was undertaken. These findings will serve as input for future models of light-meson production. The same spin-parity analysis was applied to a smaller data set taken in 2009 with a lead target. The aim was to compare the result with the 2004 analysis and to learn more about the production by a direct comparison with the 2008 proton data set. In order to improve the tracking close to the high-intensity hadron beam, five GEM (Gas Electron Multiplier) detectors with pixelised readout were developed and constructed for the 2008 data-taking. Similar detectors with strip readout and inactive areas around the beam axis were already installed in COMPASS and proved their high-rate capability in combination with a small interaction length. These new detectors replaced parts of the inner tracking system and were the backbone of the Small Angle Tracker (SAT) system during the 2008/2009 hadron campaign.
Babizhetskyy, Volodymyr; Zheng, Chong; Mattausch, Hansjürgen; Simon, Arndt
2007-12-01
The ternary rare earth boride carbides R2B4C (R=Tb, Dy, Ho, Er) have been synthesized by reacting the elements at temperatures between 1800 and 2000K. The crystal structure of Dy2B4C has been determined from single-crystal X-ray diffraction data. It crystallizes in a new structure type in the orthorhombic space group Immm (a=3.2772(6) Å, b=6.567(2) Å, c=7.542(1) Å, Z=2, R1=0.035 (wR2=0.10) for 224 reflections with Io>2σ(Io)). Boron atoms form infinite chains of fused B6 rings in [100] joined with carbon atoms into planar, two-dimensional networks which alternate with planar sheets of rare earth metal atoms. The electronic structure of Dy2B4C was also analyzed using the tight-binding extended Hückel method.
Binding energy of two-dimensional biexcitons
DEFF Research Database (Denmark)
Singh, Jai; Birkedal, Dan; Vadim, Lyssenko
1996-01-01
Using a model structure for a two-dimensional (2D) biexciton confined in a quantum well, it is shown that the form of the Hamiltonian of the 2D biexciton reduces into that of an exciton. The binding energies and Bohr radii of a 2D biexciton in its various internal energy states are derived...... analytically using the fractional dimension approach. The ratio of the binding energy of a 2D biexciton to that of a 2D exciton is found to be 0.228, which agrees very well with the recent experimental value. The results of our approach are compared with those of earlier theories....
Stability analysis of two-dimensional digital recursive filters
Alexander, W. E.; Pruess, S. A.
1980-01-01
A new approach to the stability problem for the two-dimensional digital recursive filter is presented. The bivariate difference equation representation of the two-dimensional recursive digital filter is converted to a multiinput-multioutput (MIMO) system similar to the state-space representation of the one-dimensional digital recursive filter. In this paper, a pseudo-state representation is used and three coefficient matrices are obtained. A general theorem for stability of two-dimensional digital recursive filters is derived and a very useful theorem is presented which expresses sufficient requirements for instability in terms of the spectral radii of these matrices.
Proteome research : two-dimensional gel electrophoresis and identification methods
National Research Council Canada - National Science Library
Rabilloud, Thierry, 1961
2000-01-01
"Two-dimensional electrophoresis is the central methodology in proteome research, and the state of the art is described in detail in this text, together with extensive coverage of the detection methods available...
Directory of Open Access Journals (Sweden)
Mousumi Garai
2015-09-01
Full Text Available The homologous series of phenyl and pyridyl substituted bis(acrylamidoalkanes have been synthesized with the aim of systematic analysis of their crystal structures and their solid-state [2 + 2] reactivities. The changes in the crystal structures with respect to a small change in the molecular structure, that is by varying alkyl spacers between acrylamides and/or by varying the end groups (phenyl, 2-pyridyl, 3-pyridyl, 4-pyridyl on the C-terminal of the amide, were analyzed in terms of hydrogen-bonding interference (N—H...Npy versus N—H...O=C and network geometries. In this series, a greater tendency towards the formation of N—H...O hydrogen bonds (β-sheets and two-dimensional networks over N—H...N hydrogen bonds was observed. Among all the structures seven structures were found to have the required alignments of double bonds for the [2 + 2] reaction such that the formations of single dimer, double dimer and polymer are facilitated. However, only four structures were found to exhibit such a solid-state [2 + 2] reaction to form a single dimer and polymers. The two-dimensional hydrogen-bonding layer via N—H...O hydrogen bonds was found to promote solid-state [2 + 2] photo-polymerization in a single-crystal-to-single-crystal manner. Such two-dimensional layers were encountered only when the spacer between acryl amide moieties is butyl. Only four out of the 16 derivatives were found to form hydrates, two each from 2-pyridyl and 4-pyridyl derivatives. The water molecules in these structures govern the hydrogen-bonding networks by the formation of an octameric water cluster and one-dimensional zigzag water chains. The trends in the melting points and densities were also analyzed.
Wiśniewska, Paulina; Śliwińska, Magdalena; Dymerski, Tomasz; Wardencki, Waldemar; Namieśnik, Jacek
2017-03-01
Vodka is a spirit-based beverage made from ethyl alcohol of agricultural origin. At present, increasingly more vodka brands have labels that specify the botanical origin of the product. Until now, the techniques for distinguishing between vodkas of different botanical origin have been costly, time-consuming and insufficient for making a distinction between vodka produced from similar raw materials. Therefore, it is of utmost importance to find a fast and relatively inexpensive technique for conducting such tests. In the present study, we employed comprehensive two-dimensional gas chromatography (GC×GC) and an electronic nose based on the technology of ultra-fast GC with chemometric methods such as partial least square discriminant analysis, discriminant function analysis and soft independent modeling of class analogy. Both techniques allow a distinction between the vodkas produced from different raw materials. In the case of GC×GC, the differences between vodkas were more noticeable than in the analysis by electronic nose; however, the electronic nose allowed the significantly faster analysis of vodkas. © 2016 Society of Chemical Industry. © 2016 Society of Chemical Industry.
Two-dimensional Quantum Gravity
Rolf, Juri
1998-10-01
This Ph.D. thesis pursues two goals: The study of the geometrical structure of two-dimensional quantum gravity and in particular its fractal nature. To address these questions we review the continuum formalism of quantum gravity with special focus on the scaling properties of the theory. We discuss several concepts of fractal dimensions which characterize the extrinsic and intrinsic geometry of quantum gravity. This work is partly based on work done in collaboration with Jan Ambjørn, Dimitrij Boulatov, Jakob L. Nielsen and Yoshiyuki Watabiki (1997). The other goal is the discussion of the discretization of quantum gravity and to address the so called quantum failure of Regge calculus. We review dynamical triangulations and show that it agrees with the continuum theory in two dimensions. Then we discuss Regge calculus and prove that a continuum limit cannot be taken in a sensible way and that it does not reproduce continuum results. This work is partly based on work done in collaboration with Jan Ambjørn, Jakob L. Nielsen and George Savvidy (1997).
Topological Valley Transport in Two-dimensional Honeycomb Photonic Crystals.
Yang, Yuting; Jiang, Hua; Hang, Zhi Hong
2018-01-25
Two-dimensional photonic crystals, in analogy to AB/BA stacking bilayer graphene in electronic system, are studied. Inequivalent valleys in the momentum space for photons can be manipulated by simply engineering diameters of cylinders in a honeycomb lattice. The inequivalent valleys in photonic crystal are selectively excited by a designed optical chiral source and bulk valley polarizations are visualized. Unidirectional valley interface states are proved to exist on a domain wall connecting two photonic crystals with different valley Chern numbers. With the similar optical vortex index, interface states can couple with bulk valley polarizations and thus valley filter and valley coupler can be designed. Our simple dielectric PC scheme can help to exploit the valley degree of freedom for future optical devices.
Lowe, Ross H.; Karschner, Erin L.; Schwilke, Eugene W.; Barnes, Allan J.; Huestis, Marilyn A.
2009-01-01
A two-dimensional (2D) gas chromatography/electron impact-mass spectrometry (GC/EI-MS) method for simultaneous quantification of Δ9-tetrahydrocannabinol (THC), 11-hydroxy-Δ9-tetrahydrocannabinol (11-OH-THC), and 11-nor-Δ9-tetrahydrocannabinol-9-carboxylic acid (THCCOOH) in human plasma was developed and validated. The method employs 2D capillary GC and cryofocusing for enhanced resolution and sensitivity. THC, 11-OH-THC, and THCCOOH were extracted by precipitation with acetonitrile followed by solid-phase extraction. GC separation of trimethylsilyl derivatives of analytes was accomplished with two capillary columns in series coupled via a pneumatic Deans switch system. Detection and quantification were accomplished with a bench-top single quadrupole mass spectrometer operated in electron impact-selected ion monitoring mode. Limits of quantification (LOQ) were 0.125, 0.25 and 0.125 ng/mL for THC, 11-OH-THC, and THCCOOH, respectively. Accuracy ranged from 86.0 to 113.0% for all analytes. Intra- and inter-assay precision, as percent relative standard deviation, was less than 14.1% for THC, 11-OH-THC, and THCCOOH. The method was successfully applied to quantification of THC and its 11-OH-THC and THCCOOH metabolites in plasma specimens following controlled administration of THC. PMID:17640656
Lowe, Ross H; Karschner, Erin L; Schwilke, Eugene W; Barnes, Allan J; Huestis, Marilyn A
2007-09-07
A two-dimensional (2D) gas chromatography/electron impact-mass spectrometry (GC/EI-MS) method for simultaneous quantification of Delta(9)-tetrahydrocannabinol (THC), 11-hydroxy-Delta(9)-tetrahydrocannabinol (11-OH-THC), and 11-nor-Delta(9)-tetrahydrocannabinol-9-carboxylic acid (THCCOOH) in human plasma was developed and validated. The method employs 2D capillary GC and cryofocusing for enhanced resolution and sensitivity. THC, 11-OH-THC, and THCCOOH were extracted by precipitation with acetonitrile followed by solid-phase extraction. GC separation of trimethylsilyl derivatives of analytes was accomplished with two capillary columns in series coupled via a pneumatic Deans switch system. Detection and quantification were accomplished with a bench-top single quadrupole mass spectrometer operated in electron impact-selected ion monitoring mode. Limits of quantification (LOQ) were 0.125, 0.25 and 0.125 ng/mL for THC, 11-OH-THC, and THCCOOH, respectively. Accuracy ranged from 86.0 to 113.0% for all analytes. Intra- and inter-assay precision, as percent relative standard deviation, was less than 14.1% for THC, 11-OH-THC, and THCCOOH. The method was successfully applied to quantification of THC and its 11-OH-THC and THCCOOH metabolites in plasma specimens following controlled administration of THC.
Two-Dimensional Materials for Sensing: Graphene and Beyond
Directory of Open Access Journals (Sweden)
Seba Sara Varghese
2015-09-01
Full Text Available Two-dimensional materials have attracted great scientific attention due to their unusual and fascinating properties for use in electronics, spintronics, photovoltaics, medicine, composites, etc. Graphene, transition metal dichalcogenides such as MoS2, phosphorene, etc., which belong to the family of two-dimensional materials, have shown great promise for gas sensing applications due to their high surface-to-volume ratio, low noise and sensitivity of electronic properties to the changes in the surroundings. Two-dimensional nanostructured semiconducting metal oxide based gas sensors have also been recognized as successful gas detection devices. This review aims to provide the latest advancements in the field of gas sensors based on various two-dimensional materials with the main focus on sensor performance metrics such as sensitivity, specificity, detection limit, response time, and reversibility. Both experimental and theoretical studies on the gas sensing properties of graphene and other two-dimensional materials beyond graphene are also discussed. The article concludes with the current challenges and future prospects for two-dimensional materials in gas sensor applications.
Two-dimensional heterostructures for energy storage
Energy Technology Data Exchange (ETDEWEB)
Gogotsi, Yury G. [Drexel Univ., Philadelphia, PA (United States); Pomerantseva, Ekaterina [Drexel Univ., Philadelphia, PA (United States)
2017-06-12
Two-dimensional (2D) materials provide slit-shaped ion diffusion channels that enable fast movement of lithium and other ions. However, electronic conductivity, the number of intercalation sites, and stability during extended cycling are also crucial for building high-performance energy storage devices. While individual 2D materials, such as graphene, show some of the required properties, none of them can offer all properties needed to maximize energy density, power density, and cycle life. Here we argue that stacking different 2D materials into heterostructured architectures opens an opportunity to construct electrodes that would combine the advantages of the individual building blocks while eliminating the associated shortcomings. We discuss characteristics of common 2D materials and provide examples of 2D heterostructured electrodes that showed new phenomena leading to superior electrochemical performance. As a result, we also consider electrode fabrication approaches and finally outline future steps to create 2D heterostructured electrodes that could greatly expand current energy storage technologies.
Two-dimensional electroacoustic waves in silicene
Zhukov, Alexander V.; Bouffanais, Roland; Konobeeva, Natalia N.; Belonenko, Mikhail B.
2018-01-01
In this letter, we investigate the propagation of two-dimensional electromagnetic waves in a piezoelectric medium built upon silicene. Ultrashort optical pulses of Gaussian form are considered to probe this medium. On the basis of Maxwell's equations supplemented with the wave equation for the medium's displacement vector, we obtain the effective governing equation for the vector potential associated with the electromagnetic field, as well as the component of the displacement vector. The dependence of the pulse shape on the bandgap in silicene and the piezoelectric coefficient of the medium was analyzed, thereby revealing a nontrivial triadic interplay between the characteristics of the pulse dynamics, the electronic properties of silicene, and the electrically induced mechanical vibrations of the medium. In particular, we uncovered the possibility for an amplification of the pulse amplitude through the tuning of the piezoelectric coefficient. This property could potentially offer promising prospects for the development of amplification devices for the optoelectronics industry.
Ward identities in two-dimensional gravity
International Nuclear Information System (INIS)
Polchinski, J.
1991-01-01
We study the decoupling of null states in two-dimensional gravity, using methods of critical string theory. We identify a family of null states which fail to decouple due to curvature and boundary terms. This gives relations involving amplitudes at different genus. At genus zero, these determine certain operator product coefficients. At genus one, they determine the partition function. At higher genus, we obtain a relation similar in form to the Painleve equation, but due to an incomplete understanding of a certain ghost/curvature term we do not have a closed relation for the partition function. Our results appear to correspond to the L 0 and L 1 equations in the topological and matrix model approaches. (orig.)
Two dimensional compass model with Heisenberg interactions
Pires, A. S. T.
2018-04-01
We consider a two dimensional compass model with a next and a next near Heisenberg term. The interactions are of two types: frustrated near neighbor compass interactions of amplitudes Jx and Jy, and next and next near neighbor Heisenberg interactions with exchanges J1 and J2 respectively. The Heisenberg interactions are isotropic in spin space, but the compass interactions depend on the bond direction. The ground state of the pure compass model is degenerated with a complex phase diagram. This degeneracy is removed by the Heisenberg terms leading to the arising of a magnetically ordered phase with a preferred direction. We calculate the phase diagrams at zero temperature for the case where, for J2 = 0, we have an antiferromagnetic ground state. We show that varying the value of J2, a magnetically disordered phase can be reached for small values of the compass interactions. We also calculate the critical temperature for a specified value of parameters.
Structures of two-dimensional three-body systems
International Nuclear Information System (INIS)
Ruan, W.Y.; Liu, Y.Y.; Bao, C.G.
1996-01-01
Features of the structure of L = 0 states of a two-dimensional three-body model system have been investigated. Three types of permutation symmetry of the spatial part, namely symmetric, antisymmetric, and mixed, have been considered. A comparison has been made between the two-dimensional system and the corresponding three-dimensional one. The effect of symmetry on microscopic structures is emphasized. (author)
Spin precession in inversion-asymmetric two-dimensional systems
International Nuclear Information System (INIS)
Liu, M.-H.; Chang, C.-R.
2006-01-01
We present a theoretical method to calculate the expectation value of spin in an inversion-asymmetric two-dimensional (2D) system with respect to an arbitrarily spin-polarized electron state, injected via an ideal point contact. The 2D system is confined in a [0 0 1]-grown quantum well, where both the Rashba and the Dresselhaus spin-orbit couplings are taken into account. The obtained analytical results allow more concrete description of the spatial behaviors of the spin precession caused individually by the Rashba and the Dresselhaus terms. Applying the calculation on the Datta-Das spin-FET, whose original design considers only the Rashba effect inside the channel, we investigate the possible influence due to the Dresselhaus spin-orbit coupling. Concluded solution is the choice of ±[1±10], in particular [1 1 0], as the channel direction
Photostrictive Two-Dimensional Materials in the Monochalcogenide Family
Haleoot, Raad; Paillard, Charles; Kaloni, Thaneshwor P.; Mehboudi, Mehrshad; Xu, Bin; Bellaiche, L.; Barraza-Lopez, Salvador
2017-06-01
Photostriction is predicted for group-IV monochalcogenide monolayers, two-dimensional ferroelectrics with rectangular unit cells (the lattice vector a1 is larger than a2) and an intrinsic dipole moment parallel to a1. Photostriction is found to be related to the structural change induced by a screened electric polarization (i.e., a converse piezoelectric effect) in photoexcited electronic states with either px or py (in-plane) orbital symmetry that leads to a compression of a1 and a comparatively smaller increase of a2 for a reduced unit cell area. The structural change documented here is 10 times larger than that observed in BiFeO3 , making monochalcogenide monolayers an ultimate platform for this effect. This structural modification should be observable under experimentally feasible densities of photexcited carriers on samples that have been grown already, having a potential usefulness for light-induced, remote mechano-optoelectronic applications.
Patched Green's function techniques for two-dimensional systems
DEFF Research Database (Denmark)
Settnes, Mikkel; Power, Stephen; Lin, Jun
2015-01-01
We present a numerically efficient technique to evaluate the Green's function for extended two-dimensional systems without relying on periodic boundary conditions. Different regions of interest, or “patches,” are connected using self-energy terms which encode the information of the extended parts...... of the system. The calculation scheme uses a combination of analytic expressions for the Green's function of infinite pristine systems and an adaptive recursive Green's function technique for the patches. The method allows for an efficient calculation of both local electronic and transport properties, as well...... as the inclusion of multiple probes in arbitrary geometries embedded in extended samples. We apply the patched Green's function method to evaluate the local densities of states and transmission properties of graphene systems with two kinds of deviations from the pristine structure: bubbles and perforations...
International Nuclear Information System (INIS)
Wu, T.; Cowan, C.L.; Lauer, A.; Schwiegk, H.J.
1982-03-01
The ASTERIX modular code package was developed at KFA Laboratory-Juelich for the steady state and xenon transient analysis of a pebble bed high temperature reactor. The code package was implemented on the Stanford Linear Accelerator Center Computer in August, 1980, and a user's manual for the current version of the code, identified as ASTERIX-2, was prepared as a cooperative effort by KFA Laboratory and GE-ARSD. The material in the manual includes the requirements for accessing the program, a description of the major subroutines, a listing of the input options, and a listing of the input data for a sample problem. The material is provided in sufficient detail for the user to carry out a wide range of analysis from steady state operations to the xenon induced power transients in which the local xenon, temperature, buckling and control feedback effects have been incorporated in the problem solution. (orig.)
Energy Technology Data Exchange (ETDEWEB)
Ngo, Thong Q.; McDaniel, Martin D.; Ekerdt, John G., E-mail: ekerdt@che.utexas.edu [Department of Chemical Engineering, University of Texas at Austin, Austin, Texas 78712 (United States); Goble, Nicholas J.; Gao, Xuan P. A. [Department of Physics, Case Western Reserve University, Cleveland, Ohio 44106 (United States); Posadas, Agham; Kormondy, Kristy J.; Demkov, Alexander A. [Department of Physics, University of Texas at Austin, Austin, Texas 78712 (United States); Lu, Sirong [School of Engineering for Matter, Transport and Engineering, Arizona State University, Tempe, Arizona 85287 (United States); Jordan-Sweet, Jean [IBM T.J. Watson Research Center, Yorktown Heights, New York 10598 (United States); Smith, David J. [Department of Physics, Arizona State University, Tempe, Arizona 85287 (United States)
2015-09-21
We report the formation of a quasi-two-dimensional electron gas (2-DEG) at the interface of γ-Al{sub 2}O{sub 3}/TiO{sub 2}-terminated SrTiO{sub 3} (STO) grown by atomic layer deposition (ALD). The ALD growth of Al{sub 2}O{sub 3} on STO(001) single crystal substrates was performed at temperatures in the range of 200–345 °C. Trimethylaluminum and water were used as co-reactants. In situ reflection high energy electron diffraction, ex situ x-ray diffraction, and ex situ cross-sectional transmission electron microscopy were used to determine the crystallinity of the Al{sub 2}O{sub 3} films. As-deposited Al{sub 2}O{sub 3} films grown above 300 °C were crystalline with the γ-Al{sub 2}O{sub 3} phase. In situ x-ray photoelectron spectroscopy was used to characterize the Al{sub 2}O{sub 3}/STO interface, indicating that a Ti{sup 3+} feature in the Ti 2p spectrum of STO was formed after 2–3 ALD cycles of Al{sub 2}O{sub 3} at 345 °C and even after the exposure to trimethylaluminum alone at 300 and 345 °C. The interface quasi-2-DEG is metallic and exhibits mobility values of ∼4 and 3000 cm{sup 2} V{sup −1} s{sup −1} at room temperature and 15 K, respectively. The interfacial conductivity depended on the thickness of the Al{sub 2}O{sub 3} layer. The Ti{sup 3+} signal originated from the near-interfacial region and vanished after annealing in an oxygen environment.
Haas, Florian
2014-02-19
The dynamics of strong interaction in the regime of low energies, i.e. large distances, is still not understood. Given its simplicity the non-relativistic simple quark model (SQM) describes successfully the observed hadronic spectra. QCD-inspired models, however, predict hadronic states where the gluonic content contributes to the hadron quantum numbers. These so-called hybrids cannot be explained within the SQM. A solid experimental proof of the existence of such systems would be the observation of spin-exotic states, with spin-parity quantum numbers, not allowed in the SQM. The study of mesons, the simplest hadrons, permits to gain insight into the realm of strong interaction where hadrons are the relevant degrees of freedom. The most promising spin-exotic meson candidate is the $\\pi_1(1600)$, which was claimed in several experiments and in particular in data taken during a previous hadron campaign of the COMPASS experiment. The hadron spectroscopy program of the COMPASS experiment at CER...
Basu, A.; Middya, T. R.; Bhattacharya, D. P.
2017-09-01
The field-effect mobility characteristics of a non-degenerate ensemble of a two dimensional electron gas for interaction with acoustic mode lattice vibrations in the Si-SiO2 MOS structure at the high surface electric fields are calculated here for the low and high temperature cases. The calculation takes due account of some features which are usually neglected. These include the effects of (i) the transverse component of the phonon wave vector, (ii) the realistic model of the infinite triangular potential well along the transverse direction, while applying the momentum conservation approximation, and (iii) the full form of the phonon distribution function at low temperatures. The results seem to be interesting in that they are significantly different from what follows from other theories that neglect the effects of the above features. Moreover, the agreement between the results which are obtained here with the experimental data seems to be significantly better. The scope for further refinement of the present theory has been discussed.
Nonlinear excitations in two-dimensional molecular structures with impurities
DEFF Research Database (Denmark)
Gaididei, Yuri Borisovich; Rasmussen, Kim; Christiansen, Peter Leth
1995-01-01
We study the nonlinear dynamics of electronic excitations interacting with acoustic phonons in two-dimensional molecular structures with impurities. We show that the problem is reduced to the nonlinear Schrodinger equation with a varying coefficient. The latter represents the influence of the imp......We study the nonlinear dynamics of electronic excitations interacting with acoustic phonons in two-dimensional molecular structures with impurities. We show that the problem is reduced to the nonlinear Schrodinger equation with a varying coefficient. The latter represents the influence...... excitations. Analytical results are in good agreement with numerical simulations of the nonlinear Schrodinger equation....
Radiation effects on two-dimensional materials
Energy Technology Data Exchange (ETDEWEB)
Walker, R.C. II; Robinson, J.A. [Department of Materials Science, Penn State, University Park, PA (United States); Center for Two-Dimensional Layered Materials, Penn State, University Park, PA (United States); Shi, T. [Department of Mechanical and Nuclear Engineering, Penn State, University Park, PA (United States); Department of Nuclear Engineering and Radiological Sciences, University of Michigan, Ann Arbor, MI (United States); Silva, E.C. [GlobalFoundries, Malta, NY (United States); Jovanovic, I. [Department of Nuclear Engineering and Radiological Sciences, University of Michigan, Ann Arbor, MI (United States)
2016-12-15
The effects of electromagnetic and particle irradiation on two-dimensional materials (2DMs) are discussed in this review. Radiation creates defects that impact the structure and electronic performance of materials. Determining the impact of these defects is important for developing 2DM-based devices for use in high-radiation environments, such as space or nuclear reactors. As such, most experimental studies have been focused on determining total ionizing dose damage to 2DMs and devices. Total dose experiments using X-rays, gamma rays, electrons, protons, and heavy ions are summarized in this review. We briefly discuss the possibility of investigating single event effects in 2DMs based on initial ion beam irradiation experiments and the development of 2DM-based integrated circuits. Additionally, beneficial uses of irradiation such as ion implantation to dope materials or electron-beam and helium-beam etching to shape materials have begun to be used on 2DMs and are reviewed as well. For non-ionizing radiation, such as low-energy photons, we review the literature on 2DM-based photo-detection from terahertz to UV. The majority of photo-detecting devices operate in the visible and UV range, and for this reason they are the focus of this review. However, we review the progress in developing 2DMs for detecting infrared and terahertz radiation. (copyright 2016 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)
International Nuclear Information System (INIS)
Katayama, Shinya; Suzumura, Yoshikazu; Kobayashi, Akito
2008-01-01
The organic conductor α-(BEDT-TTF) 2 I 3 exhibits the zero-gap state (ZGS) described by the massless Dirac fermions, and is in contrast to that of the single layer graphite, i.e. graphene since the former is robust against the site potential compared with the latter. However, the ZGS of the organic conductor is not fully clarified due to the complexity of several kinds of transfer energies arising from four kinds of donor molecules in a unit cell. In the present paper, we analyze the details of the ZGS by focusing on the role of the anion potential, which acts differently on respective site of donor molecules. We show that the anion potential with a small magnitude does not destroy the ZGS but has an effect of varying the location of the contact point between the conduction and valence bands as found in the case of pressure. Such a behavior can be understood by the tilted Weyl equation with a perturbation for the potential. Further, the ZGS is discussed by examining the relation between the anion potential and the charge disproportionation.
Bates, J. W.; Velikovich, A. L.; Gardner, J. H.; Mostovych, A. N.; Schmitt, A. J.
2002-11-01
We investigate the behavior of small perturbations to a planar shock wave in two dimensions. The undisturbed state is a steady planar shock propagating through a material with constant upstream and downstream values of pressure, density, and velocity. First order perturbations are introduced in the position of the shock and in the hydrodynamic quantities behind it. The objective is to explicitly determine the temporal evolution of the system for any initially specified disturbance. The earliest analysis of this problem is likely due to Roberts (Los Alamos Scientific Laboratory Report No. LA-299, 1945) who reduced the linearized system of perturbed fluid equations to an integral expression, the evaluation of which yields the time-dependent amplitude of each Fourier component of the initial disturbance. One shortcoming of Roberts' approach, though, is that the presence of entropy-vortex waves behind the shock front is overlooked, and moreover, results are specialized to the case of an ideal gas. Here, we generalize Roberts' calculation and derive explicit expressions governing the temporal evolution of a rippled shock in a material with an arbitrary EOS. Popular EOS models for materials relevant for inertial confinement fusion (ICF) studies are considered as examples. It is shown that in general, two branches of the solution exist. In one case, perturbations to the shock front decay at late time as "t to the minus three-halves power;" in the other branch, the behavior is more critically damped. The methodology developed herein provides a means of directly checking the accuracy of the D'yakov-Kontorovich instability criterion derived from a linearized normal-mode analysis.
Topology optimization of two-dimensional waveguides
DEFF Research Database (Denmark)
Jensen, Jakob Søndergaard; Sigmund, Ole
2003-01-01
In this work we use the method of topology optimization to design two-dimensional waveguides with low transmission loss.......In this work we use the method of topology optimization to design two-dimensional waveguides with low transmission loss....
Two-dimensional atomic crystals beyond graphene
Kaul, Anupama B.
2014-06-01
Carbon-based nanostructures have been the center of intense research and development for more than two decades now. Of these materials, graphene, a two-dimensional (2D) layered material system, has had a significant impact on science and technology over the past decade after monolayers of this material were experimentally isolated in 2004. The recent emergence of other classes of 2D graphene-like layered materials has added yet more exciting dimensions for research in exploring the diverse properties and applications arising from these 2D material systems. For example, hexagonal-BN, a layered material closest in structure to graphene, is an insulator, while NbSe2, a transition metal di-chalcogenide, is metallic and monolayers of other transition metal di-chalcogenides such as MoS2 are direct band-gap semiconductors. The rich spectrum of properties that 2D layered material systems offer can potentially be engineered ondemand, and creates exciting prospects for using such materials in applications ranging from electronics, sensing, photonics, energy harvesting and flexible electronics over the coming years.
Equivalency of two-dimensional algebras
International Nuclear Information System (INIS)
Santos, Gildemar Carneiro dos; Pomponet Filho, Balbino Jose S.
2011-01-01
Full text: Let us consider a vector z = xi + yj over the field of real numbers, whose basis (i,j) satisfy a given algebra. Any property of this algebra will be reflected in any function of z, so we can state that the knowledge of the properties of an algebra leads to more general conclusions than the knowledge of the properties of a function. However structural properties of an algebra do not change when this algebra suffers a linear transformation, though the structural constants defining this algebra do change. We say that two algebras are equivalent to each other whenever they are related by a linear transformation. In this case, we have found that some relations between the structural constants are sufficient to recognize whether or not an algebra is equivalent to another. In spite that the basis transform linearly, the structural constants change like a third order tensor, but some combinations of these tensors result in a linear transformation, allowing to write the entries of the transformation matrix as function of the structural constants. Eventually, a systematic way to find the transformation matrix between these equivalent algebras is obtained. In this sense, we have performed the thorough classification of associative commutative two-dimensional algebras, and find that even non-division algebra may be helpful in solving non-linear dynamic systems. The Mandelbrot set was used to have a pictorial view of each algebra, since equivalent algebras result in the same pattern. Presently we have succeeded in classifying some non-associative two-dimensional algebras, a task more difficult than for associative one. (author)
Electron-electron bound states in parity-preserving QED3
International Nuclear Information System (INIS)
Belich, H.; Helayel-Neto, J.A.; Centro Brasileiro de Pesquisas Fisicas; Cima, O.M. del; Ferreira Junior, M.M.; Maranhao Univ., Sao Luis, MA
2002-04-01
By considering the Higgs mechanism in the framework of a parity-preserving Planar Quantum Electrodynamics, one shows that an attractive electron-electron interaction may dominate. The e - e - interaction potential emerges as the non-relativistic limit of the Moeller scattering amplitude and it results attractive with a suitable choice of parameters. Numerically values of the e - e - binding energy are obtained by solving the two-dimensional Schroedinger equation. The existence of bound states is a strong indicative that this model may be adopted to address the pairing mechanism of high-T c superconductivity. (author)
Electron-electron bound states in parity-preserving QED{sub 3}
Energy Technology Data Exchange (ETDEWEB)
Belich, H.; Helayel-Neto, J.A. [Universidade Catolica do Petropolis, RJ (Brazil). Grupo de Fisica Teorica]|[Centro Brasileiro de Pesquisas Fisicas (CBPF), Rio de Janeiro, RJ (Brazil). Coordenacao de Teoria de Campos e Particulas; Cima, O.M. del [Universidade Catolica do Petropolis, RJ (Brazil). Grupo de Fisica Teorica; Ferreira Junior, M.M. [Centro Brasileiro de Pesquisas Fisicas (CBPF), Rio de Janeiro, RJ (Brazil). Coordenacao de Teoria de Campos e Particulas]|[Maranhao Univ., Sao Luis, MA (Brazil). Dept. de Fisica
2002-04-01
By considering the Higgs mechanism in the framework of a parity-preserving Planar Quantum Electrodynamics, one shows that an attractive electron-electron interaction may dominate. The e{sup -}e{sup -} interaction potential emerges as the non-relativistic limit of the Moeller scattering amplitude and it results attractive with a suitable choice of parameters. Numerically values of the e{sup -}e{sup -} binding energy are obtained by solving the two-dimensional Schroedinger equation. The existence of bound states is a strong indicative that this model may be adopted to address the pairing mechanism of high-T{sub c} superconductivity. (author)
Electron-electron bound states in parity-preserving QED sub 3
Belich, H; Helayel-Neto, J A; Monteiro del Cima, O
2002-01-01
By considering the Higgs mechanism in the framework of a parity-preserving Planar Quantum Electrodynamics, one shows that an attractive electron-electron interaction may dominate. The e sup - e sup - interaction potential emerges as the non-relativistic limit of the Moeller scattering amplitude and it results attractive with a suitable choice of parameters. Numerically values of the e sup - e sup - binding energy are obtained by solving the two-dimensional Schroedinger equation. The existence of bound states is a strong indicative that this model may be adopted to address the pairing mechanism of high-T sub c superconductivity.
Solitary wave solutions of two-dimensional nonlinear Kadomtsev ...
Indian Academy of Sciences (India)
Aly R Seadawy
2017-09-13
Sep 13, 2017 ... We considered the two-dimensional DASWs in colli- sionless, unmagnetized cold plasma consisting of dust fluid, ions and electrons. The dynamics of DASWs is governed by the normalized fluid equations of nonlin- ear continuity (1), nonlinear motion of system (2) and. (3) and linear Poisson equation (4) as.
Two-Dimensional Light Diffraction from an EPROM Chip
Ekkens, Tom
2018-01-01
In introductory physics classes, a laser pointer and a compact disc are all the items required to illustrate diffraction of light in a single dimension. If a two-dimensional diffraction pattern is desired, double axis diffraction grating material is available or a CCD sensor can be extracted from an unused electronics device. This article presents…
Wen, Yongli; Li, Huan; Xiao, Jian; Wang, Chang; Shen, Qirong; Ran, Wei; He, Xinhua; Zhou, Quansuo; Yu, Guanghui
2014-09-01
Understanding the organomineral associations in soils is of great importance. Using two-dimensional correlation spectroscopy (2DCOS) and high resolution-transmission electron microscopy (HRTEM) techniques, this study compared the binding characteristics of organic ligands to Al(III) in dissolved organic matter (DOM) from soils under short-term (3-years) and long-term (22-years) fertilizations. Three fertilization treatments were examined: (i) no fertilization (Control), (ii) chemical nitrogen, phosphorus and potassium (NPK), and (iii) NPK plus swine manure (NPKM). Soil spectra detected by the 2DCOS Fourier transform infrared (FTIR) spectroscopy showed that fertilization modified the binding characteristics of organic ligands to Al(III) in soil DOM at both short- and long- term location sites. The CH deformations in aliphatic groups played an important role in binding to Al(III) but with minor differences among the Control, NPK and NPKM at the short-term site. While at the long-term site both C-O stretching of polysaccharides or polysaccharide-like substances and aliphatic O-H were bound to Al(III) under the Control, whereas only aliphatic O-H, and only polysaccharides and silicates, were bound to Al(III) under NPK and NPKM, respectively. Images from HRTEM demonstrated that crystalline nanominerals, composed of Fe and O, were predominant in soil DOM under NPK, while amorphous nanominerals, predominant in Al, Si, and O, were dominant in soil DOM under Control and NPKM. In conclusion, fertilization strategies, especially under long-term, could affect the binding of organic ligands to Al(III) in soil DOM, which resulted in alterations in the turnover, reactivity, and bioavailability of soil organic matter. Our results demonstrated that the FTIR-2DCOS combined with HRTEM techniques could enhance our understanding in the binding characteristics of DOM to Al(III) and the resulted nanominerals in soils. Copyright © 2014 Elsevier Ltd. All rights reserved.
Wang, Yun-Peng; Li, Xiang-Guo; Liu, Shuang-Long; Fry, James N.; Cheng, Hai-Ping
2018-03-01
We investigate theoretically magnetism and magnetic phase transitions induced by electrostatic gating of two-dimensional square metal-organic framework compounds. We find that electrostatic gating can induce phase transitions between homogeneous ferromagnetic and various spin-textured antiferromagnetic states. Electronic structure and Wannier function analysis can reveal hybridizations between transition-metal d orbitals and conjugated π orbitals in the organic framework. Mn-containing compounds exhibit a strong d -π hybridization that leads to partially occupied spin-minority bands, in contrast to compounds containing transition-metal ions other than Mn, for which electronic structure around the Fermi energy is only slightly spin split due to weak d -π hybridization and the magnetic interaction is of the Ruderman-Kittel-Kasuya-Yosida type. We use a ferromagnetic Kondo lattice model to understand the phase transition in Mn-containing compounds in terms of carrier density and illuminate the complexity and the potential to control two-dimensional magnetization.
Electronic states of myricetin
DEFF Research Database (Denmark)
Vojta, Danijela; Karlsen, Eva; Spanget-Larsen, Jens
2017-01-01
Myricetin (3,3',4',5,5',7'-hexahydroxyflavone) was investigated by linear dichroism spectroscopy on molecular samples partially aligned in stretched poly(vinyl alcohol) (PVA). At least five electronic transitions in the range 40000 – 20000 cm–1 were characterized with respect to their wavenumbers......, relative intensities, and transition moment directions. The observed bands were assigned to electronic transitions predicted with TD-B3LYP/6-31+G(d,p)....
Hettiarachchi, Gayan Prasad; Moriasa, Fumiya; Nishida, Yoshihumi; Nakano, Takehito; Muhid, Mohd Nazlan Mohd; Hamdan, Halimaton
2017-10-01
The evolution of the electronic properties of guest Na and Rb atoms in a disordered deformable lattice is investigated for a series of guest-atom densities n . The quasi-two-dimensional host M7.8 -δAl7.8Si8.2O32.0 (M =Na, Rb), known as zeolite P, is used. The Na system is a stubborn bipolaronic insulator to the maximum n of 1.03. In contrast, the Rb system exhibits a crossover from a bipolaronic insulator to a conducting phase analogous to a disordered metal at n = 0.89. A critical region undergoing polaronic melting appears in the vicinity of the crossover on the insulating side, evidenced by a reduction in the small bipolaron absorption band and a drop in the activation energy. Transition to the conducting phase coincides with the appearance of a midinfrared band and an increase in the charge-carrier decay length, suggesting the polaronic and extended nature of the carriers. These findings constitute rare examples of electron-lattice coupling opening (or closing) a mobility gap and scaling the continuity (or discontinuity) of a conducting transition in the face of disorder.
Two-dimensional spin diffusion in multiterminal lateral spin valves
Saha, D.; Basu, D.; Holub, M.; Bhattacharya, P.
2008-01-01
The effects of two-dimensional spin diffusion on spin extraction in lateral semiconductor spin valves have been investigated experimentally and theoretically. A ferromagnetic collector terminal of variable size is placed between the ferromagnetic electron spin injector and detector of a conventional lateral spin valve for spin extraction. It is observed that transverse spin diffusion beneath the collector terminal plays an important role along with the conventional longitudinal spin diffusion in describing the overall transport of spin carriers. Two-dimensional spin diffusion reduces the perturbation of the channel electrochemical potentials and improves spin extraction.
Two-dimensional transition metal dichalcogenides: interface and defect engineering.
Hu, Zehua; Wu, Zhangting; Han, Cheng; He, Jun; Ni, Zhenhua; Chen, Wei
2018-03-06
Two-dimensional (2D) transition metal dichalcogenides (TMDCs) have been considered as promising candidates for next generation nanoelectronics. Because of their atomically-thin structure and high surface to volume ratio, the interfaces involved in TMDC-based devices play a predominant role in determining the device performance, such as charge injection/collection at the metal/TMDC interface, and charge carrier trapping at the dielectric/TMDC interface. On the other hand, the crystalline structures of TMDCs are enriched by a variety of intrinsic defects, including vacancies, adatoms, grain boundaries, and substitutional impurities. Customized design and engineering of the interfaces and defects provides an effective way to modulate the properties of TMDCs and finally enhance the device performance. Herein, we summarize and highlight recent advances and state-of-the-art investigations on the interface and defect engineering of TMDCs and their corresponding applications in electronic and optoelectronic devices. Various interface engineering approaches for TMDCs are overviewed, including surface charge transfer doping, TMDC/metal contact engineering, and TMDC/dielectric interface engineering. Subsequently, different types of structural defects in TMDCs are introduced. Defect engineering strategies utilized to modulate the optical and electronic properties of TMDCs, as well as the developed high-performance and functional devices are summarized. Finally, we highlight the challenges and opportunities for interface and defect engineering in TMDC materials for electronics and optoelectronics.
Gate-induced superconductivity in two-dimensional atomic crystals
Saito, Yu; Nojima, Tsutomu; Iwasa, Yoshihiro
2016-09-01
Two-dimensional (2D) crystals are attracting growing interest in condensed matter physics, since these systems exhibit not only rich electronic and photonic properties but also exotic electronic phase transitions including superconductivity and charge density wave. Moreover, owing to the recent development of transfer methods after exfoliation and electric-double-layer transistors, superconducting 2D atomic crystals, the thicknesses of which are below 1-2 nm, have been successfully obtained. Here, we present a topical review on the recent discoveries of 2D crystalline superconductors by ionic-liquid gating and a series of their novel properties. In particular, we highlight two topics; quantum metallic states (or possible metallic ground states) and superconductivity robust against in-plane magnetic fields. These phenomena can be discussed with the effects of weakened disorder and/or broken spacial inversion symmetry leading to valley-dependent spin-momentum locking (spin-valley locking). These examples suggest the superconducting 2D crystals are new platforms for investigating the intrinsic quantum phases as well as exotic nature in 2D superconductors.
Traditional Semiconductors in the Two-Dimensional Limit
Lucking, Michael C.; Xie, Weiyu; Choe, Duk-Hyun; West, Damien; Lu, Toh-Ming; Zhang, S. B.
2018-02-01
Interest in two-dimensional materials has exploded in recent years. Not only are they studied due to their novel electronic properties, such as the emergent Dirac fermion in graphene, but also as a new paradigm in which stacking layers of distinct two-dimensional materials may enable different functionality or devices. Here, through first-principles theory, we reveal a large new class of two-dimensional materials which are derived from traditional III-V, II-VI, and I-VII semiconductors. It is found that in the ultrathin limit the great majority of traditional binary semiconductors studied (a series of 28 semiconductors) are not only kinetically stable in a two-dimensional double layer honeycomb structure, but more energetically stable than the truncated wurtzite or zinc-blende structures associated with three dimensional bulk. These findings both greatly increase the landscape of two-dimensional materials and also demonstrate that in the double layer honeycomb form, even ordinary semiconductors, such as GaAs, can exhibit exotic topological properties.
Photodetectors based on two dimensional materials
Zheng, Lou; Zhongzhu, Liang; Guozhen, Shen
2016-09-01
Two-dimensional (2D) materials with unique properties have received a great deal of attention in recent years. This family of materials has rapidly established themselves as intriguing building blocks for versatile nanoelectronic devices that offer promising potential for use in next generation optoelectronics, such as photodetectors. Furthermore, their optoelectronic performance can be adjusted by varying the number of layers. They have demonstrated excellent light absorption, enabling ultrafast and ultrasensitive detection of light in photodetectors, especially in their single-layer structure. Moreover, due to their atomic thickness, outstanding mechanical flexibility, and large breaking strength, these materials have been of great interest for use in flexible devices and strain engineering. Toward that end, several kinds of photodetectors based on 2D materials have been reported. Here, we present a review of the state-of-the-art in photodetectors based on graphene and other 2D materials, such as the graphene, transition metal dichalcogenides, and so on. Project supported by the National Natural Science Foundation of China (Nos. 61377033, 61574132, 61504136) and the State Key Laboratory of Applied Optics, Changchun Institute of Optics, Fine Mechanics and Physics, Chinese Academy of Sciences.
Development of Two-Dimensional NMR
Indian Academy of Sciences (India)
Home; Journals; Resonance – Journal of Science Education; Volume 20; Issue 11. Development of Two-Dimensional NMR: Strucure Determination of Biomolecules in Solution. Anil Kumar. General Article Volume 20 Issue 11 November 2015 pp 995-1002 ...
Conoscopic holography: two-dimensional numerical reconstructions.
Mugnier, L M; Sirat, G Y; Charlot, D
1993-01-01
Conoscopic holography is an incoherent light holographic technique based on the properties of crystal optics. We present experimental results of the numerical reconstruction of a two-dimensional object from its conoscopic hologram.
The one-particle scenario for the metal-insulator transition in two-dimensional systems at T = 0
Tarasov, Y V
2003-01-01
The conductance of bounded disordered electron systems is calculated by reducing the original dynamic problem of arbitrary dimensionality to a set of strictly one-dimensional problems for one-particle mode propagators. The metallic ground state of a two-dimensional conductor, which is considered as a limiting case of three-dimensional quantum waveguide, is shown to result from its multi-modeness. As the waveguide thickness is reduced, e.g., by applying a 'pressing' potential, the electron system undergoes a set of continuous phase transitions related to discrete variations of the number of extended modes. The closing of the last current carrying mode is regarded as a phase transition of the electron system from metallic to dielectric state. The obtained results agree qualitatively with the observed 'anomalies' of resistivity of different two-dimensional electron and hole systems.
Spilling of electronic states in Pb quantum wells
Jałochowski, M.; Palotás, K.; Krawiec, M.
2016-01-01
Energy-dependent apparent step heights of two-dimensional ultrathin Pb islands grown on the Si(111)6 ×6 -Au surface have been investigated by a combination of scanning tunneling microscopy, first-principles density-functional theory, and the particle-in-a-box model calculations. The apparent step height shows the thickness- and energy-dependent oscillatory behaviors, which are directly related to the spilling of electron states into the vacuum exhibiting a quantum size effect. This has been unambiguously proven by extensive first-principles scanning tunneling microscopy and spectroscopy simulations. An electronic contribution to the apparent step height is directly determined. At certain energies it reaches values as high as a half of the atomic contribution. The applicability of the particle-in-a-box model to the spilling of electron states is also discussed.
Energy Technology Data Exchange (ETDEWEB)
Eickhoff, Christian
2010-10-27
By combining ultrafast laser excitation with energy-, angle- and time-resolved twophoton photoemission (2PPE), the electronic properties of bulk silicon and the Si(001) surface are investigated in this thesis. A custom-built laser- and UHV-systemequipped with a display type 2D-CCD-detector gives new insight into the relaxation dynamics of excited carriers on a femtosecond timescale. The bandgap between occupied valence bands and unoccupied conduction bands characteristically influences the dynamics of excited electrons in the bulk, as well as in surface states and resonances. For the electron-phonon interaction this leads to the formation of a bottleneck during the relaxation of hot electrons in the conduction band, which maintains the elevated electronic temperature for several picoseconds. During relaxation, excited electrons also scatter from the conduction band into the unoccupied dangling-bond surface state D{sub down}. Depending on the excitation density this surface recombination is dominated by electron-electron- or electron-phonon scattering. The relaxation of the carriers in the D{sub down}-band is again slowed down by the formation of a bottleneck in electron-phonon coupling. Furthermore, the new laser system has allowed detection of the Rydberg-like series of image-potential resonances on the Si(001)-surface. It is shown that the lifetime of these image-potential resonances in front of the semiconducting surface exhibits the same behavior as those in front of metallic surfaces. Moreover the electron-phonon coupling in the first image-potential resonance was investigated and compared to the D{sub down}-surface state. For the first time, Fano-type lineprofiles are demonstrated and analyzed in a 2PPEprocess on a surface. Tuning the photon energy of the pump-laser across the resonance between the occupied dangling-bond state D{sub up}, and the unoccupied image-potential resonance n=1, reveals a clear intensity variation that can be successfully described
Two-Dimensional Superfluidity of Exciton Polaritons Requires Strong Anisotropy
Directory of Open Access Journals (Sweden)
Ehud Altman
2015-02-01
Full Text Available Fluids of exciton polaritons, excitations of two-dimensional quantum wells in optical cavities, show collective phenomena akin to Bose condensation. However, a fundamental difference from standard condensates stems from the finite lifetime of these excitations, which necessitates continuous driving to maintain a steady state. A basic question is whether a two-dimensional condensate with long-range algebraic correlations can exist under these nonequilibrium conditions. Here, we show that such driven two-dimensional Bose systems cannot exhibit algebraic superfluid order except in low-symmetry, strongly anisotropic systems. Our result implies, in particular, that recent apparent evidence for Bose condensation of exciton polaritons must be an intermediate-scale crossover phenomenon, while the true long-distance correlations fall off exponentially. We obtain these results through a mapping of the long-wavelength condensate dynamics onto the anisotropic Kardar-Parisi-Zhang equation.
Control Operator for the Two-Dimensional Energized Wave Equation
Directory of Open Access Journals (Sweden)
Sunday Augustus REJU
2006-07-01
Full Text Available This paper studies the analytical model for the construction of the two-dimensional Energized wave equation. The control operator is given in term of space and time t independent variables. The integral quadratic objective cost functional is subject to the constraint of two-dimensional Energized diffusion, Heat and a source. The operator that shall be obtained extends the Conjugate Gradient method (ECGM as developed by Hestenes et al (1952, [1]. The new operator enables the computation of the penalty cost, optimal controls and state trajectories of the two-dimensional energized wave equation when apply to the Conjugate Gradient methods in (Waziri & Reju, LEJPT & LJS, Issues 9, 2006, [2-4] to appear in this series.
Two-dimensional effects in nonlinear Kronig-Penney models
DEFF Research Database (Denmark)
Gaididei, Yuri Borisovich; Christiansen, Peter Leth; Rasmussen, Kim
1997-01-01
An analysis of two-dimensional (2D) effects in the nonlinear Kronig-Penney model is presented. We establish an effective one-dimensional description of the 2D effects, resulting in a set of pseudodifferential equations. The stationary states of the 2D system and their stability is studied...
Prediction of two-dimensional diluted magnetic semiconductors: Doped monolayer MoS2 systems
Cheng, Yingchun
2013-03-05
Using first-principles calculations, we propose a two-dimensional diluted magnetic semiconductor: monolayer MoS2 doped by transition metals. Doping of transition metal atoms from the IIIB to VIB groups results in nonmagnetic states, since the number of valence electrons is smaller or equal to that of Mo. Doping of atoms from the VIIB to IIB groups becomes energetically less and less favorable. Magnetism is observed for Mn, Fe, Co, Zn, Cd, and Hg doping, while for the other dopants from these groups it is suppressed by Jahn-Teller distortions. Analysis of the binding energies and magnetic properties indicates that (Mo,X)S2 (X=Mn, Fe, Co, and Zn) are promising systems to explore two-dimensional diluted magnetic semiconductors.
TWO-DIMENSIONAL TOPOLOGY OF COSMOLOGICAL REIONIZATION
International Nuclear Information System (INIS)
Wang, Yougang; Xu, Yidong; Chen, Xuelei; Park, Changbom; Kim, Juhan
2015-01-01
We study the two-dimensional topology of the 21-cm differential brightness temperature for two hydrodynamic radiative transfer simulations and two semi-numerical models. In each model, we calculate the two-dimensional genus curve for the early, middle, and late epochs of reionization. It is found that the genus curve depends strongly on the ionized fraction of hydrogen in each model. The genus curves are significantly different for different reionization scenarios even when the ionized faction is the same. We find that the two-dimensional topology analysis method is a useful tool to constrain the reionization models. Our method can be applied to the future observations such as those of the Square Kilometre Array
Huang, Jian; Pfeiffer, L. N.; West, K. W.
2012-02-01
It is well-known that the insulating behavior in the two-dimensional metal-to-insulator transition demonstrates a finite temperature conduction via hopping. Recently, however, some very strongly interacting higher purity two-dimensional electron systems at temperatures T->0 demonstrate certain nonactivated insulating behaviors that are absent in more disordered systems. Through measuring in dark the T-dependence of the conductivity of ultra-high quality 2D holes with charge densities down to 7x10^8 cm-2, an approximate power-law behavior is identified. Moreover, for the lowest charge densities, the exponent exhibits a linearly decreasing density-dependence which suggests an interaction-driven nature. Such an electron state is fragile to even a slight increase of disorder which causes a crossover from nonactivated to activated conduction. The non-activated conduction may well be an universal interaction-driven signature of an electron state of strongly correlated (semiquantum) liquid.
Two-dimensional x-ray diffraction
He, Bob B
2009-01-01
Written by one of the pioneers of 2D X-Ray Diffraction, this useful guide covers the fundamentals, experimental methods and applications of two-dimensional x-ray diffraction, including geometry convention, x-ray source and optics, two-dimensional detectors, diffraction data interpretation, and configurations for various applications, such as phase identification, texture, stress, microstructure analysis, crystallinity, thin film analysis and combinatorial screening. Experimental examples in materials research, pharmaceuticals, and forensics are also given. This presents a key resource to resea
Directional detection of dark matter with two-dimensional targets
Directory of Open Access Journals (Sweden)
Yonit Hochberg
2017-09-01
Full Text Available We propose two-dimensional materials as targets for direct detection of dark matter. Using graphene as an example, we focus on the case where dark matter scattering deposits sufficient energy on a valence-band electron to eject it from the target. We show that the sensitivity of graphene to dark matter of MeV to GeV mass can be comparable, for similar exposure and background levels, to that of semiconductor targets such as silicon and germanium. Moreover, a two-dimensional target is an excellent directional detector, as the ejected electron retains information about the angular dependence of the incident dark matter particle. This proposal can be implemented by the PTOLEMY experiment, presenting for the first time an opportunity for directional detection of sub-GeV dark matter.
Directional detection of dark matter with two-dimensional targets
Hochberg, Yonit; Kahn, Yonatan; Lisanti, Mariangela; Tully, Christopher G.; Zurek, Kathryn M.
2017-09-01
We propose two-dimensional materials as targets for direct detection of dark matter. Using graphene as an example, we focus on the case where dark matter scattering deposits sufficient energy on a valence-band electron to eject it from the target. We show that the sensitivity of graphene to dark matter of MeV to GeV mass can be comparable, for similar exposure and background levels, to that of semiconductor targets such as silicon and germanium. Moreover, a two-dimensional target is an excellent directional detector, as the ejected electron retains information about the angular dependence of the incident dark matter particle. This proposal can be implemented by the PTOLEMY experiment, presenting for the first time an opportunity for directional detection of sub-GeV dark matter.
Atomic-like high-harmonic generation from two-dimensional materials.
Tancogne-Dejean, Nicolas; Rubio, Angel
2018-02-01
The generation of high-order harmonics from atomic and molecular gases enables the production of high-energy photons and ultrashort isolated pulses. Obtaining efficiently similar photon energy from solid-state systems could lead, for instance, to more compact extreme ultraviolet and soft x-ray sources. We demonstrate from ab initio simulations that it is possible to generate high-order harmonics from free-standing monolayer materials, with an energy cutoff similar to that of atomic and molecular gases. In the limit in which electrons are driven by the pump laser perpendicularly to the monolayer, they behave qualitatively the same as the electrons responsible for high-harmonic generation (HHG) in atoms, where their trajectories are described by the widely used semiclassical model, and exhibit real-space trajectories similar to those of the atomic case. Despite the similarities, the first and last steps of the well-established three-step model for atomic HHG are remarkably different in the two-dimensional materials from gases. Moreover, we show that the electron-electron interaction plays an important role in harmonic generation from monolayer materials because of strong local-field effects, which modify how the material is ionized. The recombination of the accelerated electron wave packet is also found to be modified because of the infinite extension of the material in the monolayer plane, thus leading to a more favorable wavelength scaling of the harmonic yield than in atomic HHG. Our results establish a novel and efficient way of generating high-order harmonics based on a solid-state device, with an energy cutoff and a more favorable wavelength scaling of the harmonic yield similar to those of atomic and molecular gases. Two-dimensional materials offer a unique platform where both bulk and atomic HHG can be investigated, depending on the angle of incidence. Devices based on two-dimensional materials can extend the limit of existing sources.
Negative differential Rashba effect in two-dimensional hole systems
Habib, B.; Tutuc, E.; Melinte, S.; Shayegan, M.; Wasserman, D.; Lyon, S. A.; Winkler, R.
2004-01-01
We demonstrate experimentally and theoretically that two-dimensional (2D) heavy hole systems in single heterostructures exhibit a \\emph{decrease} in spin-orbit interaction-induced spin splitting with an increase in perpendicular electric field. Using front and back gates, we measure the spin splitting as a function of applied electric field while keeping the density constant. Our results are in contrast to the more familiar case of 2D electrons where spin splitting increases with electric field.
Acoustic dispersion in a two-dimensional dipole system
International Nuclear Information System (INIS)
Golden, Kenneth I.; Kalman, Gabor J.; Donko, Zoltan; Hartmann, Peter
2008-01-01
We calculate the full density response function and from it the long-wavelength acoustic dispersion for a two-dimensional system of strongly coupled point dipoles interacting through a 1/r 3 potential at arbitrary degeneracy. Such a system has no random-phase-approximation (RPA) limit and the calculation has to include correlations from the outset. We follow the quasilocalized charge (QLC) approach, accompanied by molecular-dynamics (MD) simulations. Similarly to what has been recently reported for the closely spaced classical electron-hole bilayer [G. J. Kalman et al., Phys. Rev. Lett. 98, 236801 (2007)] and in marked contrast to the RPA, we report a long-wavelength acoustic phase velocity that is wholly maintained by particle correlations and varies linearly with the dipole moment p. The oscillation frequency, calculated both in an extended QLC approximation and in the Singwi-Tosi-Land-Sjolander approximation [Phys. Rev. 176, 589 (1968)], is invariant in form over the entire classical to quantum domains all the way down to zero temperature. Based on our classical MD-generated pair distribution function data and on ground-state energy data generated by recent quantum Monte Carlo simulations on a bosonic dipole system [G. E. Astrakharchik et al., Phys. Rev. Lett. 98, 060405 (2007)], there is a good agreement between the QLC approximation kinetic sound speeds and the standard thermodynamic sound speeds in both the classical and quantum domains
Dipolar vortices in two-dimensional flows
DEFF Research Database (Denmark)
Juul Rasmussen, J.; Hesthaven, J.S.; Lynov, Jens-Peter
1996-01-01
The dynamics of dipolar vortex solutions to the two-dimensional Euler equations is studied. A new type of nonlinear dipole is found and its dynamics in a slightly viscous system is compared with the dynamics of the Lamb dipole. The evolution of dipolar structures from an initial turbulent patch...
Two-dimensional position sensitive neutron detector
Indian Academy of Sciences (India)
A two-dimensional position sensitive neutron detector has been developed. The detector is a 3He + Kr filled multiwire proportional counter with charge division position readout and has a sensitive area of 345 mm × 345 mm, pixel size 5 mm × 5 mm, active depth 25 mm and is designed for efficiency of 70% for 4 Å neutrons.
Stability of two-dimensional vorticity filaments
International Nuclear Information System (INIS)
Elhmaidi, D.; Provenzale, A.; Lili, T.; Babiano, A.
2004-01-01
We discuss the results of a numerical study on the stability of two-dimensional vorticity filaments around a circular vortex. We illustrate how the stability of the filaments depends on the balance between the strain associated with the far field of the vortex and the local vorticity of the filament, and we discuss an empirical criterion for filament stability
Two-dimensional membranes in motion
Davidovikj, D.
2018-01-01
This thesis revolves around nanomechanical membranes made of suspended two - dimensional materials. Chapters 1-3 give an introduction to the field of 2D-based nanomechanical devices together with an overview of the underlying physics and the measurementtools used in subsequent chapters. The research
Piezoelectricity in Two-Dimensional Materials
Wu, Tao
2015-02-25
Powering up 2D materials: Recent experimental studies confirmed the existence of piezoelectricity - the conversion of mechanical stress into electricity - in two-dimensional single-layer MoS2 nanosheets. The results represent a milestone towards embedding low-dimensional materials into future disruptive technologies. © 2015 Wiley-VCH Verlag GmbH & Co. KGaA.
Sums of two-dimensional spectral triples
DEFF Research Database (Denmark)
Christensen, Erik; Ivan, Cristina
2007-01-01
We study countable sums of two dimensional modules for the continuous complex functions on a compact metric space and show that it is possible to construct a spectral triple which gives the original metric back. This spectral triple will be finitely summable for any positive parameter. We also co...
A novel two dimensional particle velocity sensor
Pjetri, O.; Wiegerink, Remco J.; Lammerink, Theodorus S.J.; Krijnen, Gijsbertus J.M.
2013-01-01
In this paper we present a two wire, two-dimensional particle velocity sensor. The miniature sensor of size 1.0x2.5x0.525 mm, consisting of only two crossed wires, shows excellent directional sensitivity in both directions, thus requiring no directivity calibration, and is relatively easy to
Two-dimensional microstrip detector for neutrons
Energy Technology Data Exchange (ETDEWEB)
Oed, A. [Institut Max von Laue - Paul Langevin (ILL), 38 - Grenoble (France)
1997-04-01
Because of their robust design, gas microstrip detectors, which were developed at ILL, can be assembled relatively quickly, provided the prefabricated components are available. At the beginning of 1996, orders were received for the construction of three two-dimensional neutron detectors. These detectors have been completed. The detectors are outlined below. (author). 2 refs.
Introduction to solid state electronics
Wang, FFY
1989-01-01
This textbook is specifically tailored for undergraduate engineering courses offered in the junior year, providing a thorough understanding of solid state electronics without relying on the prerequisites of quantum mechanics. In contrast to most solid state electronics texts currently available, with their generalized treatments of the same topics, this is the first text to focus exclusively and in meaningful detail on introductory material. The original text has already been in use for 10 years. In this new edition, additional problems have been added at the end of most chapters. These proble
Two-dimensional silica opens new perspectives
Büchner, Christin; Heyde, Markus
2017-12-01
In recent years, silica films have emerged as a novel class of two-dimensional (2D) materials. Several groups succeeded in epitaxial growth of ultrathin SiO2 layers using different growth methods and various substrates. The structures consist of tetrahedral [SiO4] building blocks in two mirror symmetrical planes, connected via oxygen bridges. This arrangement is called a silica bilayer as it is the thinnest 2D arrangement with the stoichiometry SiO2 known today. With all bonds saturated within the nano-sheet, the interaction with the substrate is based on van der Waals forces. Complex ring networks are observed, including hexagonal honeycomb lattices, point defects and domain boundaries, as well as amorphous domains. The network structures are highly tuneable through variation of the substrate, deposition parameters, cooling procedure, introducing dopants or intercalating small species. The amorphous networks and structural defects were resolved with atomic resolution microscopy and modeled with density functional theory and molecular dynamics. Such data contribute to our understanding of the formation and characteristic motifs of glassy systems. Growth studies and doping with other chemical elements reveal ways to tune ring sizes and defects as well as chemical reactivities. The pristine films have been utilized as molecular sieves and for confining molecules in nanocatalysis. Post growth hydroxylation can be used to tweak the reactivity as well. The electronic properties of silica bilayers are favourable for using silica as insulators in 2D material stacks. Due to the fully saturated atomic structure, the bilayer interacts weakly with the substrate and can be described as quasi-freestanding. Recently, a mm-scale film transfer under structure retention has been demonstrated. The chemical and mechanical stability of silica bilayers is very promising for technological applications in 2D heterostacks. Due to the impact of this bilayer system for glass science
De Sanctis, Adolfo; Mehew, Jake D.; Alkhalifa, Saad; Tate, Callum P.; White, Ashley; Woodgate, Adam R.; Craciun, Monica F.; Russo, Saverio
2018-02-01
Two-dimensional materials offer a novel platform for the development of future quantum technologies. However, the electrical characterisation of topological insulating states, non-local resistance, and bandgap tuning in atomically thin materials can be strongly affected by spurious signals arising from the measuring electronics. Common-mode voltages, dielectric leakage in the coaxial cables, and the limited input impedance of alternate-current amplifiers can mask the true nature of such high-impedance states. Here, we present an optical isolator circuit which grants access to such states by electrically decoupling the current-injection from the voltage-sensing circuitry. We benchmark our apparatus against two state-of-the-art measurements: the non-local resistance of a graphene Hall bar and the transfer characteristic of a WS2 field-effect transistor. Our system allows the quick characterisation of novel insulating states in two-dimensional materials with potential applications in future quantum technologies.
The electrostatic ion-cyclotron instability-a two-dimensional potential relaxation instability
DEFF Research Database (Denmark)
Popa, G.; Schrittwieser, R.; Juul Rasmussen, Jens
1985-01-01
An experimental investigation shows that the electrostatic ion-cyclotron instability, driven by an electron current to a positively biased collector, is accompanied by strong coherent two-dimensional fluctuations of the plasma potential in front of the collector. These results suggest that this i...... that this instability evolves like a two-dimensional potential relaxation instability....
Directory of Open Access Journals (Sweden)
D. A. Fetisov
2015-01-01
Full Text Available The controllability conditions are well known if we speak about linear stationary systems: a linear stationary system is controllable if and only if the dimension of the state vector is equal to the rank of the controllability matrix. The concept of the controllability matrix is extended to affine systems, but relations between affine systems controllability and properties of this matrix are more complicated. Various controllability conditions are set for affine systems, but they deal as usual either with systems of some special form or with controllability in some small neighborhood of the concerned point. An affine system is known to be controllable if the system is equivalent to a system of a canonical form, which is defined and regular in the whole space of states. In this case, the system is said to be feedback linearizable in the space of states. However there are examples, which illustrate that a system can be controllable even if it is not feedback linearizable in any open subset in the space of states. In this article we deal with such systems.Affine systems with two-dimensional control are considered. The system in question is assumed to be equivalent to a system of a quasicanonical form with two-dimensional zero dynamics which is defined and regular in the whole space of states. Therefore the controllability of the original system is equivalent to the controllability of the received system of a quasicanonical form. In this article the sufficient condition for an available solution of the terminal problem is proven for systems of a quasicanonical form with two-dimensional control and two-dimensional zero dynamics. The condition is valid in the case of an arbitrary time interval and arbitrary initial and finite states of the system. Therefore the controllability condition is set for systems of a quasicanonical form with two-dimensional control and two-dimensional zero dynamics. An example is given which illustrates how the proved
Observation of hidden Fermi surface nesting in a two dimensional conductor
International Nuclear Information System (INIS)
Breuer, K.; Stagerescu, C.; Smith, K.E.; Greenblatt, M.; Ramanujachary, K.
1996-01-01
We report the first direct measurement of hidden Fermi surface nesting in a two dimensional conductor. The system studied was Na 0.9 Mo 6 O 17 , and the measured Fermi surface consists of electron and hole pockets that can be combined to form sets of pseudo-one-dimensional Fermi surfaces, exhibiting the nesting necessary to drive a Peierls transition to a charge density wave state. The observed nesting vector is shown to be in excellent agreement with theory. copyright 1996 The American Physical Society
Highly luminescent two dimensional excitons in atomically thin CdSe nanosheets
Energy Technology Data Exchange (ETDEWEB)
Halder, O.; Pradhani, A.; Rath, S., E-mail: srath@iitbbs.ac.in [School of Basic Sciences, Indian Institute of Technology Bhubaneswar, Toshali Bhawan, Satyanagar, Bhubaneswar 751 007 (India); Sahoo, P. K. [Department of Physics, National Institute of Science Education and Research, Sachivalaya marg, Bhubaneswar 751 005 (India); Satpati, B. [Saha Institute of Nuclear Physics, 1/AF Bidhannagar, Kolkata 700 064 (India)
2014-05-05
Atomically thin Cadmium Selenide (CdSe) nanosheets have been synthesized using a surfactant mediated growth technique. The transmission electron microscopy studies confirm the presence of single layered nanosheets with thickness 1.31 nm and their stacking structures which are complemented by the small angle x-ray scattering measurements. The strongly bound and polarized character of two dimensional excitonic states with enhanced oscillator strength yielding distinct narrow blue luminescence has been observed from the CdSe nanosheets using room temperature based optical studies.
A method for controlling the synthesis of stable twisted two-dimensional conjugated molecules
Li, Yongjun; Jia, Zhiyu; Xiao, Shengqiang; Liu, Huibiao; Li, Yuliang
2016-01-01
Thermodynamic stabilization (π-electron delocalization through effective conjugation) and kinetic stabilization (blocking the most-reactive sites) are important considerations when designing stable polycyclic aromatic hydrocarbons displaying tunable optoelectronic properties. Here, we demonstrate an efficient method for preparing a series of stable two-dimensional (2D) twisted dibenzoterrylene-acenes. We investigated their electronic structures and geometries in the ground state through various experiments assisted by calculations using density functional theory. We find that the length of the acene has a clear effect on the photophysical, electrochemical, and magnetic properties. These molecules exhibit tunable ground-state structures, in which a stable open-shell quintet tetraradical can be transferred to triplet diradicals. Such compounds are promising candidates for use in nonlinear optics, field effect transistors and organic spintronics; furthermore, they may enable broader applications of 2D small organic molecules in high-performance electronic and optical devices. PMID:27181692
The stability of a two-dimensional rising bubble
International Nuclear Information System (INIS)
Nie, Q.; Tanveer, S.
1995-01-01
The stability of an inviscid two-dimensional bubble subject to two-dimensional disturbances is considered and the bubbles are found to be linearly stable for all Weber numbers, for which a steady solution is known. Certain aspects of the nonlinear initial value problem are also studied. An initial condition that consists of a superposition of a suitable symmetric eigenmode (of the linear stability operator) on a steady state is found to result in pinching of the bubble neck as it tends to oscillate about the steady state. An estimate of the threshold amplitude of such a disturbance needed to cause breakup of a large aspect ratio bubble is obtained. The presence of gravity appears to inhibit this pinching process
Two-dimensional silicon: the advent of silicene
Grazianetti, Carlo; Cinquanta, Eugenio; Molle, Alessandro
2016-03-01
Silicene is sometimes thought of as the Si alter ego of graphene. However, experimental evidence indicates that silicene is substantially different from graphene in terms of its stability, atomic structure, electronic properties, and device process issues. Some of these aspects hamper the feasibility of silicene for practical application, but at the same time they may offer routes to engineer or functionalize silicene as a complementary material to graphene if a good control of the material can be achieved. As such, the research on silicene runs along the cutting edge between unsurmountable limitation and pioneering opportunities. In the present review, we examine the issues that are representative of this dual edge and try to make a preliminary balance of the state-of-the-art features of this material. Each relevant topic will be explored in a dedicated section. We start with the introduction of ‘experimental’ silicene in the so-called ’flatland’ from the point of view of technology drivers and of its conceptual precursor, freestanding silicene. We then explore the following: specific aspects of the silicene on substrates; the tendency of silicene to have multiple structural forms (what we call the polymorphic nature of silicene) the role of the strong hybridization with the substrate in the electronic band structure of silicene; the Raman spectrum of silicene, and silicene processing and integration into a transistor. Finally we conclude by proposing an investigation into silicene’s emerging contemporaries in the realm of elementary two-dimensional materials. Mindful of ongoing discussions and current issues, we try to go to the heart of the problems by treating each topic objectively and scientifically and we then provide our personal views in the discussion.
Two-dimensional self-consistent microwave argon plasma simulations with experimental verification
International Nuclear Information System (INIS)
Li, Y.; Gordon, M.H.; Roe, L.A.; Hassouni, K.; Grotjohn, T.
2003-01-01
Optical emission spectroscopy (OES), absorption measurements, and thermal energy rate analysis were used in tandem with numerical models to characterize microwave argon plasmas. A WAVEMAT (model MPDR-3135) microwave diamond deposition system was used to generate argon plasmas at 5 Torr. Three excited state number densities (4p, 5p, and 5d) were obtained from the OES measurements, and a fourth excited state number density (4s) was obtained from the absorption measurements. Further, power absorbed in the substrate was monitored. A self-consistent two-dimensional argon model coupled with an electromagnetic field model and a 25-level two-dimensional (2D)-collisional-radiative model (CRM) was developed and validated with the experimental measurements. The 2D model provides the gas and electron temperature distributions, and the electron, ion, and 4s state number densities, which are then iteratively fed into the electromagnetic and CRM models. Both the numerically predicted thermal energy rates and excited state densities agreed, within the experimental and numerical uncertainties, with the experimental results
Two-dimensional sensitivity calculation code: SENSETWO
International Nuclear Information System (INIS)
Yamauchi, Michinori; Nakayama, Mitsuo; Minami, Kazuyoshi; Seki, Yasushi; Iida, Hiromasa.
1979-05-01
A SENSETWO code for the calculation of cross section sensitivities with a two-dimensional model has been developed, on the basis of first order perturbation theory. It uses forward neutron and/or gamma-ray fluxes and adjoint fluxes obtained by two-dimensional discrete ordinates code TWOTRAN-II. The data and informations of cross sections, geometry, nuclide density, response functions, etc. are transmitted to SENSETWO by the dump magnetic tape made in TWOTRAN calculations. The required input for SENSETWO calculations is thus very simple. The SENSETWO yields as printed output the cross section sensitivities for each coarse mesh zone and for each energy group, as well as the plotted output of sensitivity profiles specified by the input. A special feature of the code is that it also calculates the reaction rate with the response function used as the adjoint source in TWOTRAN adjoint calculation and the calculated forward flux from the TWOTRAN forward calculation. (author)
Two-dimensional ranking of Wikipedia articles
Zhirov, A. O.; Zhirov, O. V.; Shepelyansky, D. L.
2010-10-01
The Library of Babel, described by Jorge Luis Borges, stores an enormous amount of information. The Library exists ab aeterno. Wikipedia, a free online encyclopaedia, becomes a modern analogue of such a Library. Information retrieval and ranking of Wikipedia articles become the challenge of modern society. While PageRank highlights very well known nodes with many ingoing links, CheiRank highlights very communicative nodes with many outgoing links. In this way the ranking becomes two-dimensional. Using CheiRank and PageRank we analyze the properties of two-dimensional ranking of all Wikipedia English articles and show that it gives their reliable classification with rich and nontrivial features. Detailed studies are done for countries, universities, personalities, physicists, chess players, Dow-Jones companies and other categories.
Toward two-dimensional search engines
International Nuclear Information System (INIS)
Ermann, L; Shepelyansky, D L; Chepelianskii, A D
2012-01-01
We study the statistical properties of various directed networks using ranking of their nodes based on the dominant vectors of the Google matrix known as PageRank and CheiRank. On average PageRank orders nodes proportionally to a number of ingoing links, while CheiRank orders nodes proportionally to a number of outgoing links. In this way, the ranking of nodes becomes two dimensional which paves the way for the development of two-dimensional search engines of a new type. Statistical properties of information flow on the PageRank–CheiRank plane are analyzed for networks of British, French and Italian universities, Wikipedia, Linux Kernel, gene regulation and other networks. A special emphasis is done for British universities networks using the large database publicly available in the UK. Methods of spam links control are also analyzed. (paper)
Two-dimensional Kagome photonic bandgap waveguide
DEFF Research Database (Denmark)
Nielsen, Jens Bo; Søndergaard, Thomas; Libori, Stig E. Barkou
2000-01-01
The transverse-magnetic photonic-bandgap-guidance properties are investigated for a planar two-dimensional (2-D) Kagome waveguide configuration using a full-vectorial plane-wave-expansion method. Single-moded well-localized low-index guided modes are found. The localization of the optical modes...... is investigated with respect to the width of the 2-D Kagome waveguide, and the number of modes existing for specific frequencies and waveguide widths is mapped out....
Superintegrability on the two dimensional hyperboloid
International Nuclear Information System (INIS)
Akopyan, E.; Pogosyan, G.S.; Kalnins, E.G.; Miller, W. Jr
1998-01-01
This work is devoted to the investigation of the quantum mechanical systems on the two dimensional hyperboloid which admit separation of variables in at least two coordinate systems. Here we consider two potentials introduced in a paper of C.P.Boyer, E.G.Kalnins and P.Winternitz, which haven't been studied yet. An example of an interbasis expansion is given and the structure of the quadratic algebra generated by the integrals of motion is carried out
Energy Technology Data Exchange (ETDEWEB)
Sukhanov, Aleksei A.
2017-05-15
We study the energy spectra of bound states in quantum dots (QDs) formed by an electrostatic potential in two-dimensional topological insulator (TI) and their transformation with changes in QD depth and radius. It is found that, unlike a trivial insulator, the energy difference between the levels of the ground state and first excited state can decrease with decreasing the radius and increasing the depth of the QD so that these levels intersect under some critical condition. The crossing of the levels results in unusual features of optical properties caused by intraceneter electron transitions. In particular, it leads to significant changes of light absorption due to electron transitions between such levels and to the transient electroluminescence induced by electrical tuning of QD and TI parameters. In the case of magnetic TIs, the polarization direction of the absorbed or emitted circularly polarized light is changed due to the level crossing.
ν =2 /3 fractional quantum Hall state in an AlAs quantum well probed by electron spin resonance
Shchepetilnikov, A. V.; Frolov, D. D.; Nefyodov, Yu. A.; Kukushkin, I. V.; Tiemann, L.; Reichl, C.; Dietsche, W.; Wegscheider, W.
2017-10-01
The electron spin resonance (ESR) of two-dimensional electrons confined in a high-quality, 16-nm AlAs quantum well was investigated near the filling factor ν =2 /3 of the fractional quantum Hall effect (FQHE). The spin resonance was robust in the vicinity of the fractional filling ν =2 /3 , indicating that the ν =2 /3 state is at least partially spin polarized. The formation of the 2 /3 FQHE state did not result in any modifications of the ESR linewidth and, hence, of the electron spin relaxation rate. Yet the nuclear spin-lattice relaxation rate extracted from the time decay of the ESR Overhauser shift demonstrated a strong nonmonotonic dependence on the electron filling factor with a minimum near ν =2 /3 . This observation suggests the enhancement of the energy gap in the spin excitation spectrum of two-dimensional electrons at the ν =2 /3 state.
Quantum oscillations in quasi-two-dimensional conductors
Galbova, O
2002-01-01
The electronic absorption of sound waves in quasi-two-dimensional conductors in strong magnetic fields, is investigated theoretically. A longitudinal acoustic wave, propagating along the normal n-> to the layer of quasi-two-dimensional conductor (k-> = left brace 0,0,k right brace; u-> = left brace 0,0,u right brace) in magnetic field (B-> = left brace 0, 0, B right brace), is considered. The quasiclassical approach for this geometry is of no interest, due to the absence of interaction between electromagnetic and acoustic waves. The problem is of interest in strong magnetic field when quantization of the charge carriers energy levels takes place. The quantum oscillations in the sound absorption coefficient, as a function of the magnetic field, are theoretically observed. The experimental study of the quantum oscillations in quasi-two-dimensional conductors makes it possible to solve the inverse problem of determining from experimental data the extrema closed sections of the Fermi surface by a plane p sub z = ...
Observations of two-dimensional monolayer zinc oxide
Energy Technology Data Exchange (ETDEWEB)
Sahoo, Trilochan, E-mail: trilochansahoo@gmail.com [Department of Physics and Nanotechnology, SRM University, Kattankulathur, 603203 Tamilnadu (India); Nayak, Sanjeev K. [Institute of Physics, Martin Luther University Halle-Wittenberg, Von Seckendorff Platz 1, 06120 Halle (Germany); Chelliah, Pandian [Department of Physics and Nanotechnology, SRM University, Kattankulathur, 603203 Tamilnadu (India); Rath, Manasa K.; Parida, Bhaskar [Division of Advanced Materials Engineering, Chonbuk National University, Jeonju 561756 (Korea, Republic of)
2016-03-15
Highlights: • Synthesis of planer ZnO nanostructure. • Observation of multilayered and monolayer ZnO. • DFT calculation of (10-10), (11-20) and (0 0 0 1) planes of ZnO. • Stability of non-polar (10-10) and (11-20) planes of ZnO. - Abstract: This letter reports the observations of planar two-dimensional ZnO synthesized using the hydrothermal growth technique. High-resolution transmission electron microscopy revealed the formation of a two-dimensional honeycomb lattice and aggregated structures of layered ZnO. The nonpolar (10-10) and (11-20) planes were present in the X-ray diffraction patterns, but the characteristic (0 0 0 1) peak of bulk ZnO was absent. The study found that nonpolar freestanding ZnO structures composed of a single or few layers may be more stable and may have a higher probability of formation than their polar counterparts. The stability of the nonpolar two-dimensional hexagonal ZnO slabs is supported by density functional theory studies.
Transient two-dimensional fuel-concentration measurement technique
Konishi, Tadashi; Naka, Syuji; Ito, Akihiko; Saito, Kozo
1997-11-01
We propose a nonintrusive experimental technique, the transient fuel-concentration measurement technique (TFMT), that is capable of being used to measure two-dimensional profiles of transient fuel concentrations over an open liquid fuel surface. The TFMT is based on single-wavelength holographic interferometry; its response time is less than 1 s and spatial resolution is 0.1 mol. % /0.1 mm. It was applied to measure both methanol vapor and n-propanol vapor concentrations. To assess the accuracy of the technique, our results were compared with steady-state methanol and n-propanol fuel-vapor concentrations measured by other researchers with a microsampling technique combined with gas chromatography. We found the TFMT to be accurate for on-line monitoring of two-dimensional profiles of fuel-vapor concentrations.
Recombination in one- and two-dimensional fitness landscapes.
Avetisyan, Zh; Saakian, David B
2010-05-01
We consider many-site mutation-recombination models of molecular evolution, where fitness is a function of a Hamming distance from one (one-dimensional case) or two (two-dimensional case) sequences. For the one-dimensional case, we calculate the population distribution dynamics for a model with zero fitness and an arbitrary symmetric initial distribution and find an error threshold transition point in the single-peak fitness model for a given initial symmetric distribution. We calculate the recombination period in the case of a single-peak fitness function, when the original population is located at one sequence, at some Hamming distance from the peak configuration. Steady-state fitness is calculated with finite genome length corrections. We derive analytical equations for the two-dimensional mutation-recombination model.
Chemical modulation of electronic structure at the excited state
Li, F.; Song, C.; Gu, Y. D.; Saleem, M. S.; Pan, F.
2017-12-01
Spin-polarized electronic structures are the cornerstone of spintronics, and have thus attracted a significant amount of interest; in particular, researchers are looking into how to modulate the electronic structure to enable multifunctional spintronics applications, especially in half-metallic systems. However, the control of the spin polarization has only been predicted in limited two-dimensional systems with spin-polarized Dirac structures and is difficult to achieve experimentally. Here, we report the modulation of the electronic structure in the light-induced excited state in a typical half-metal, L a1 /2S r1 /2Mn O3 -δ . According to the spin-transport measurements, there appears a light-induced increase in magnetoresistance due to the enhanced spin scattering, which is closely associated with the excited spin polarization. Strikingly, the light-induced variation can be enhanced via alcohol processing and reduced by oxygen annealing. X-ray photoelectron spectroscopy measurements show that in the chemical process, a redox reaction occurs with a change in the valence of Mn. Furthermore, first-principles calculations reveal that the change in the valence of Mn alters the electronic structure and consequently modulates the spin polarization in the excited state. Our findings thus report a chemically tunable electronic structure, demonstrating interesting physics and the potential for multifunctional applications and ultrafast spintronics.
Gyroscope with two-dimensional optomechanical mirror
Davuluri, Sankar; Li, Kai; Li, Yong
2017-11-01
We propose an application of two-dimensional optomechanical oscillator as a gyroscope by detecting the Coriolis force which is modulated at the natural frequency of the optomechanical oscillator. Dependence of gyroscope's sensitivity on shot noise, back-action noise, thermal noise, and input laser power is studied. At optimal input laser power, the gyroscope's sensitivity can be improved by increasing the mass or by decreasing the temperature and decay rate of the mechanical oscillator. When the mechanical oscillator's thermal occupation number, n th, is zero, sensitivity improves with decrease in frequency of the mechanical oscillator. For {n}{{th}}\\gg 1, the sensitivity is independent of the mechanical oscillator's frequency.
Versatile two-dimensional transition metal dichalcogenides
DEFF Research Database (Denmark)
Canulescu, Stela; Affannoukoué, Kévin; Döbeli, Max
Two-dimensional transition metal dichalcogenides (2D-TMDCs), such as MoS2, have emerged as a new class of semiconducting materials with distinct optical and electrical properties. The availability of 2D-TMDCs with distinct band gaps allows for unlimited combinations of TMDC monolayers (MLs...... vacancies. We have found that the absorption spectra of the MoS2 films exhibit distinct excitonic peaks at ~1.8 and ~2 eV when grown in the presence of a sulfur evaporation beam as compared to those deposited in vacuum. The structure of the PLD-grown MoS2 films will be further discussed based Raman...
Energy Technology Data Exchange (ETDEWEB)
Cahoon, James Francis [Univ. of California, Berkeley, CA (United States)
2008-12-01
One and two dimensional time-resolved vibrational spectroscopy has been used to investigate the elementary reactions of several prototypical organometallic complexes in room temperature solution. The electron transfer and ligand substitution reactions of photogenerated 17-electron organometallic radicals CpW(CO)_{3} and CpFe(CO)_{2} have been examined with one dimensional spectroscopy on the picosecond through microsecond time-scales, revealing the importance of caging effects and odd-electron intermediates in these reactions. Similarly, an investigation of the photophysics of the simple Fischer carbene complex Cr(CO)_{5}[CMe(OMe)] showed that this class of molecule undergoes an unusual molecular rearrangement on the picosecond time-scale, briefly forming a metal-ketene complex. Although time-resolved spectroscopy has long been used for these types of photoinitiated reactions, the advent of two dimensional vibrational spectroscopy (2D-IR) opens the possibility to examine the ultrafast dynamics of molecules under thermal equilibrium conditions. Using this method, the picosecond fluxional rearrangements of the model metal carbonyl Fe(CO)_{5} have been examined, revealing the mechanism, time-scale, and transition state of the fluxional reaction. The success of this experiment demonstrates that 2D-IR is a powerful technique to examine the thermally-driven, ultrafast rearrangements of organometallic molecules in solution.
Moore, Christine; Rana, Sumandeep; Coulter, Cynthia; Feyerherm, Fred; Prest, Harry
2006-04-01
The proposed federal regulations for the detection in hair of 11-nor-Delta(9)-tetrahydrocannabinol-9-carboxylic acid (THC-COOH), a metabolite of marijuana, require a confirmatory detection level of 0.05 pg/mg. At present, the only way to achieve this on a routine basis has been with the use gas chromatography with tandem mass spectrometry (GC-MS-MS) technology. Tandem MS is an expensive approach and dissuades laboratories from attempting to enter the hair-testing market. A procedure for the determination of THC-COOH in hair using two-dimensional gas chromatography (GC x GC) coupled to mass spectrometry (GC-GC-MS) is described for the first time. The method makes use of several small improvements in the extraction, GC, and MS procedures to allow the required sensitivity to be achieved. The results of this approach demonstrate detection of THC-COOH in hair at a concentration level of 0.05 pg/mg with both a target quantitation ion and a unique confirming qualifier ion, using a single-quadrupole mass selective detector. These two ions and the enhanced separation of the GC-GC provide a high degree of confidence in the determinations. The method has been successfully applied to the detection of THC-COOH in hair specimens from known marijuana users, and it reaches the levels currently proposed in the Federal Register.
Parallel comprehensive two-dimensional gas chromatography.
Yan, DanDan; Tedone, Laura; Koutoulis, Anthony; Whittock, Simon P; Shellie, Robert A
2017-11-17
We introduce an information rich analytical approach called parallel comprehensive two-dimensional gas chromatography (2GC×2GC). This parallel chromatography approach splits injected samples into two independent two-dimensional column ensembles and provides two GC×GC separations by using contra-directional thermal modulation. The first-dimension ( 1 D) and second-dimension ( 2 D) columns are connected using planar three-port microchannel devices, which are supplied with supplementary flow via two pressure controller modules. Precise carrier gas flow control at the junction of the 1 D and 2 D columns permits independent control of flow conditions in each separation column. The 2GC×2GC approach provides two entirely independent GC×GC separations for each injection. Analysis of hop (Humulus lupulus L.) essential oils is used to demonstrate the capability of the approach. The analytical performance of each GC×GC separation in the 2GC×2GC experiment is comparable to individual GC×GC separation with matching column configurations. The peak capacity of 2GC×2GC is about 2 times than that of single GC×GC system. The dual 2D chromatograms produced by this single detector system provide complementary separations and additional identification information by harnessing different selectivity provided by the four separation columns. Copyright © 2017 Elsevier B.V. All rights reserved.
Flow transitions in two-dimensional foams.
Gilbreth, Christopher; Sullivan, Scott; Dennin, Michael
2006-11-01
For sufficiently slow rates of strain, flowing foam can exhibit inhomogeneous flows. The nature of these flows is an area of active study in both two-dimensional model foams and three dimensional foam. Recent work in three-dimensional foam has identified three distinct regimes of flow [S. Rodts, J. C. Baudez, and P. Coussot, Europhys. Lett. 69, 636 (2005)]. Two of these regimes are identified with continuum behavior (full flow and shear banding), and the third regime is identified as a discrete regime exhibiting extreme localization. In this paper, the discrete regime is studied in more detail using a model two-dimensional foam: a bubble raft. We characterize the behavior of the bubble raft subjected to a constant rate of strain as a function of time, system size, and applied rate of strain. We observe localized flow that is consistent with the coexistence of a power-law fluid with rigid-body rotation. As a function of applied rate of strain, there is a transition from a continuum description of the flow to discrete flow when the thickness of the flow region is approximately ten bubbles. This occurs at an applied rotation rate of approximately 0.07 s-1.
Energy Technology Data Exchange (ETDEWEB)
Dinara, Syed Mukulika, E-mail: smdinara.iit@gmail.com; Jana, Sanjay Kr.; Ghosh, Saptarsi; Mukhopadhyay, Partha; Kumar, Rahul [Advanced Technology Development Centre, Indian Institute of Technology, Kharagpur, India 721302 (India); Chakraborty, Apurba; Biswas, Dhrubes [Dept. of Electronics and Electrical Communication Engineering, Indian Institute of Technology, Kharagpur, India 721 302 (India); Bhattacharya, Sekhar [SSN Research Center, Tamilnadu, India 603110 (India)
2015-04-15
Enhancement of two dimensional electron gas (2DEG) concentrations at Al{sub 0.3}Ga{sub 0.7}N/GaN hetero interface after a-Si{sub 3}N{sub 4} (SiN) passivation has been investigated from non-destructive High Resolution X-ray Diffraction (HRXRD) analysis, depletion depth and capacitance-voltage (C-V) profile measurement. The crystalline quality and strained in-plane lattice parameters of Al{sub 0.3}Ga{sub 0.7}N and GaN were evaluated from double axis (002) symmetric (ω-2θ) diffraction scan and double axis (105) asymmetric reciprocal space mapping (DA RSM) which revealed that the tensile strain of the Al{sub 0.3}Ga{sub 0.7}N layer increased by 15.6% after SiN passivation. In accordance with the predictions from theoretical solution of Schrödinger-Poisson’s equations, both electrochemical capacitance voltage (ECV) depletion depth profile and C-V characteristics analyses were performed which implied effective 9.5% increase in 2DEG carrier density after passivation. The enhancement of polarization charges results from increased tensile strain in the Al{sub 0.3}Ga{sub 0.7}N layer and also due to the decreased surface states at the interface of SiN/Al{sub 0.3}Ga{sub 0.7}N layer, effectively improving the carrier confinement at the interface.
International Nuclear Information System (INIS)
Taneichi, T.; Kobayashi, T.
2007-01-01
Discussion on wavelength dependent 'anharmonic' effects in a pump-probe signal for a system of wavepacket on one- and two-dimensional harmonic potentials was given. The Fourier power spectrum of the signal, calculated for a model composed of a three-state electronic system coupled to a set of displaced harmonic oscillators, depends on the pulse duration. Condition under which the wavepacket motion in the harmonic potential substantially deviates from that of the classical point mass is derived. The Fourier power spectrum has enhanced components with frequencies of harmonics even in a system composed of ideally harmonic potentials. Utility of the Fourier analysis of the spectrum for clarification of the squeezed molecular vibrational state is discussed. Calculated oscillatory behavior in phase of a pump-probe signal, as a function of probe frequency, was discussed in terms of a two-dimensional effect on a pump-probe signal
Quantum tunneling of electron snake states in an inhomogeneous magnetic field.
Hoodbhoy, Pervez
2018-05-10
In a two dimensional free electron gas subjected to a perpendicular spatially varying magnetic field, the classical paths of electrons are snake-like trajectories that weave along the line where the field crosses zero. But quantum mechanically this system is described by a symmetric double well potential which, for low excitations, leads to very different electron behavior. We compute the spectrum, as well as the wavefunctions, for states of definite parity in the limit of nearly degenerate states, i.e. for electrons sufficiently far from the B z = 0 line. Transitions between the states are shown to give rise to a tunneling current. If the well is made asymmetrical by a time-dependent parity breaking perturbation then Rabi-like oscillations between parity states occur. Resonances can be excited and used to stimulate the transfer of electrons from one side of the potential barrier to the other through quantum tunneling.
Splitting rules for spectra of two-dimensional Fibonacci quasilattices
Yang, Xiangbo; Liu, Youyan
1997-10-01
In the framework of the single-electron tight-binding on-site model, after establishing the method of constructing a class of two-dimensional Fibonacci quasilattices, we have studied the rules of energy spectra splitting for these quasilattices by means of a decomposition-decimation method based on the renormalization-group technique. Under the first approximation, the analytic results show that there exist only six kinds of clusters and the electronic energy bands split as type Y and consist of nine subbands. Instead of the on-site model, the transfer model should be used for the higher hierarchy of the spectra, the electronic energy spectra split as type F. The analytic results are confirmed by numerical simulations.
Two dimensional NMR studies of polysaccharides
International Nuclear Information System (INIS)
Byrd, R.A.; Egan, W.; Summers, M.F.
1987-01-01
Polysaccharides are very important components in the immune response system. Capsular polysaccharides and lipopolysaccharides occupy cell surface sites of bacteria, play key roles in recognition and some have been used to develop vaccines. Consequently, the ability to determine chemical structures of these systems is vital to an understanding of their immunogenic action. The authors have been utilizing recently developed two-dimensional homonuclear and heteronuclear correlation spectroscopy for unambiguous assignment and structure determination of a number of polysaccharides. In particular, the 1 H-detected heteronuclear correlation experiments are essential to the rapid and sensitive determination of these structures. Linkage sites are determined by independent polarization transfer experiments and multiple quantum correlation experiments. These methods permit the complete structure determination on very small amounts of the polysaccharides. They present the results of a number of structural determinations and discuss the limits of these experiments in terms of their applications to polysaccharides
Two-dimensional fourier transform spectrometer
DeFlores, Lauren; Tokmakoff, Andrei
2013-09-03
The present invention relates to a system and methods for acquiring two-dimensional Fourier transform (2D FT) spectra. Overlap of a collinear pulse pair and probe induce a molecular response which is collected by spectral dispersion of the signal modulated probe beam. Simultaneous collection of the molecular response, pulse timing and characteristics permit real time phasing and rapid acquisition of spectra. Full spectra are acquired as a function of pulse pair timings and numerically transformed to achieve the full frequency-frequency spectrum. This method demonstrates the ability to acquire information on molecular dynamics, couplings and structure in a simple apparatus. Multi-dimensional methods can be used for diagnostic and analytical measurements in the biological, biomedical, and chemical fields.
Two-dimensional materials for ultrafast lasers
International Nuclear Information System (INIS)
Wang Fengqiu
2017-01-01
As the fundamental optical properties and novel photophysics of graphene and related two-dimensional (2D) crystals are being extensively investigated and revealed, a range of potential applications in optical and optoelectronic devices have been proposed and demonstrated. Of the many possibilities, the use of 2D materials as broadband, cost-effective and versatile ultrafast optical switches (or saturable absorbers) for short-pulsed lasers constitutes a rapidly developing field with not only a good number of publications, but also a promising prospect for commercial exploitation. This review primarily focuses on the recent development of pulsed lasers based on several representative 2D materials. The comparative advantages of these materials are discussed, and challenges to practical exploitation, which represent good future directions of research, are laid out. (paper)
Two dimensional generalizations of the Newcomb equation
International Nuclear Information System (INIS)
Dewar, R.L.; Pletzer, A.
1989-11-01
The Bineau reduction to scalar form of the equation governing ideal, zero frequency linearized displacements from a hydromagnetic equilibrium possessing a continuous symmetry is performed in 'universal coordinates', applicable to both the toroidal and helical cases. The resulting generalized Newcomb equation (GNE) has in general a more complicated form than the corresponding one dimensional equation obtained by Newcomb in the case of circular cylindrical symmetry, but in this cylindrical case , the equation can be transformed to that of Newcomb. In the two dimensional case there is a transformation which leaves the form of the GNE invariant and simplifies the Frobenius expansion about a rational surface, especially in the limit of zero pressure gradient. The Frobenius expansions about a mode rational surface is developed and the connection with Hamiltonian transformation theory is shown. 17 refs
Strategies for Interpreting Two Dimensional Microwave Spectra
Martin-Drumel, Marie-Aline; Crabtree, Kyle N.; Buchanan, Zachary
2017-06-01
Microwave spectroscopy can uniquely identify molecules because their rotational energy levels are sensitive to the three principal moments of inertia. However, a priori predictions of a molecule's structure have traditionally been required to enable efficient assignment of the rotational spectrum. Recently, automated microwave double resonance spectroscopy (AMDOR) has been employed to rapidly generate two dimensional spectra based on transitions that share a common rotational level, which may enable automated extraction of rotational constants without any prior estimates of molecular structure. Algorithms used to date for AMDOR have relied on making several initial assumptions about the nature of a subset of the linked transitions, followed by testing possible assignments by "brute force." In this talk, we will discuss new strategies for interpreting AMDOR spectra, using eugenol as a test case, as well as prospects for library-free, automated identification of the molecules in a volatile mixture.
Modified black holes in two dimensional gravity
International Nuclear Information System (INIS)
Mohammedi, N.
1991-11-01
The SL(2,R)/U(1) gauged WZWN model is modified by a topological term and the accompanying change in the geometry of the two dimensional target space is determined. The possibility of this additional term arises from a symmetry in the general formalism of gauging an isometry subgroup of a non-linear sigma model with an antisymmetric tensor. It is shown, in particular, that the space-time exhibits some general singularities for which the recently found black hole is just a special case. From a conformal field theory point of view and for special values of the unitary representation of SL(2,R), this topological term can be interpreted as a small perturbation by a (1,1) conformal operator of the gauged WZWN action. (author). 26 refs
Thermal properties of two-dimensional materials
International Nuclear Information System (INIS)
Zhang Gang; Zhang Yong-Wei
2017-01-01
Two-dimensional (2D) materials, such as graphene, phosphorene, and transition metal dichalcogenides (e.g., MoS 2 and WS 2 ), have attracted a great deal of attention recently due to their extraordinary structural, mechanical, and physical properties. In particular, 2D materials have shown great potential for thermal management and thermoelectric energy generation. In this article, we review the recent advances in the study of thermal properties of 2D materials. We first review some important aspects in thermal conductivity of graphene and discuss the possibility to enhance the ultra-high thermal conductivity of graphene. Next, we discuss thermal conductivity of MoS 2 and the new strategy for thermal management of MoS 2 device. Subsequently, we discuss the anisotropic thermal properties of phosphorene. Finally, we review the application of 2D materials in thermal devices, including thermal rectifier and thermal modulator. (topical reviews)
The Penalty Cost Functional for the Two-Dimensional
Directory of Open Access Journals (Sweden)
Victor Onomza WAZIRI
2006-07-01
Full Text Available This paper constructs the penalty cost functional for optimizing the two-dimensional control operator of the energized wave equation. In some multiplier methods such as the Lagrange multipliers and Pontrygean maximum principle, the cost of merging the constraint equation to the integral quadratic objective functional to obtain an unconstraint equation is normally guessed or obtained from the first partial derivatives of the unconstrained equation. The Extended Conjugate Gradient Method (ECGM necessitates that the penalty cost be sequentially obtained algebraically. The ECGM problem contains a functional which is completely given in terms of state and time spatial dependent variables.
Confinement and dynamical regulation in two-dimensional convective turbulence
DEFF Research Database (Denmark)
Bian, N.H.; Garcia, O.E.
2003-01-01
In this work the nature of confinement improvement implied by the self-consistent generation of mean flows in two-dimensional convective turbulence is studied. The confinement variations are linked to two distinct regulation mechanisms which are also shown to be at the origin of low......-frequency bursting in the fluctuation level and the convective heat flux integral, both resulting in a state of large-scale intermittency. The first one involves the control of convective transport by sheared mean flows. This regulation relies on the conservative transfer of kinetic energy from tilted fluctuations...
Persistence of Precursor Waves in Two-dimensional Relativistic Shocks
Energy Technology Data Exchange (ETDEWEB)
Iwamoto, Masanori; Amano, Takanobu; Hoshino, Masahiro [Department of Earth and Planetary Science, University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033 (Japan); Matsumoto, Yosuke, E-mail: iwamoto@eps.s.u-tokyo.ac.jp [Department of Physics, Chiba University, 1-33 Yayoi, Inage-ku, Chiba 263-8522 (Japan)
2017-05-01
We investigated the efficiency of coherent upstream large-amplitude electromagnetic wave emission via synchrotron maser instability in relativistic magnetized shocks using two-dimensional particle-in-cell simulations. We considered a purely perpendicular shock in an electron–positron plasma. The coherent wave emission efficiency was measured as a function of the magnetization parameter σ , which is defined as the ratio of the Poynting flux to the kinetic energy flux. The wave amplitude was systematically smaller than that observed in one-dimensional simulations. However, it continued to persist, even at a considerably low magnetization rate, where the Weibel instability dominated the shock transition. The emitted electromagnetic waves were sufficiently strong to disturb the upstream medium, and transverse filamentary density structures of substantial amplitude were produced. Based on this result, we discuss the possibility of the wakefield acceleration model to produce nonthermal electrons in a relativistic magnetized ion–electron shock.
Coulomb interaction and phonons in doped semiconducting and metallic two-dimensional materials
Schönhoff, Gunnar
2017-01-01
Two-dimensional (2D) materials present a rapidly developing field of research with sometimes highly unusual and uniquely two-dimensional physics. Starting with graphene, many recent studies have investigated 2D materials, with results for properties encompassing such different topics as Dirac electrons, charge ordering, and superconductivity. To get closer to a predictive theory of the phases of 2D materials, this thesis systematically tackles the previously unclear problem of the Coulomb int...
Nematic Equilibria on a Two-Dimensional Annulus
Lewis, A. H.
2017-01-16
We study planar nematic equilibria on a two-dimensional annulus with strong and weak tangent anchoring, in the Oseen–Frank theoretical framework. We analyze a radially invariant defect-free state and compute analytic stability criteria for this state in terms of the elastic anisotropy, annular aspect ratio, and anchoring strength. In the strong anchoring case, we define and characterize a new spiral-like equilibrium which emerges as the defect-free state loses stability. In the weak anchoring case, we compute stability diagrams that quantify the response of the defect-free state to radial and azimuthal perturbations. We study sector equilibria on sectors of an annulus, including the effects of weak anchoring and elastic anisotropy, giving novel insights into the correlation between preferred numbers of boundary defects and the geometry. We numerically demonstrate that these sector configurations can approximate experimentally observed equilibria with boundary defects.
Seismic isolation of two dimensional periodic foundations
Energy Technology Data Exchange (ETDEWEB)
Yan, Y.; Mo, Y. L., E-mail: yilungmo@central.uh.edu [University of Houston, Houston, Texas 77004 (United States); Laskar, A. [Indian Institute of Technology Bombay, Powai, Mumbai (India); Cheng, Z.; Shi, Z. [Beijing Jiaotong University, Beijing (China); Menq, F. [University of Texas, Austin, Texas 78712 (United States); Tang, Y. [Argonne National Laboratory, Argonne, Illinois 60439 (United States)
2014-07-28
Phononic crystal is now used to control acoustic waves. When the crystal goes to a larger scale, it is called periodic structure. The band gaps of the periodic structure can be reduced to range from 0.5 Hz to 50 Hz. Therefore, the periodic structure has potential applications in seismic wave reflection. In civil engineering, the periodic structure can be served as the foundation of upper structure. This type of foundation consisting of periodic structure is called periodic foundation. When the frequency of seismic waves falls into the band gaps of the periodic foundation, the seismic wave can be blocked. Field experiments of a scaled two dimensional (2D) periodic foundation with an upper structure were conducted to verify the band gap effects. Test results showed the 2D periodic foundation can effectively reduce the response of the upper structure for excitations with frequencies within the frequency band gaps. When the experimental and the finite element analysis results are compared, they agree well with each other, indicating that 2D periodic foundation is a feasible way of reducing seismic vibrations.
Comparative Two-Dimensional Fluorescence Gel Electrophoresis.
Ackermann, Doreen; König, Simone
2018-01-01
Two-dimensional comparative fluorescence gel electrophoresis (CoFGE) uses an internal standard to increase the reproducibility of coordinate assignment for protein spots visualized on 2D polyacrylamide gels. This is particularly important for samples, which need to be compared without the availability of replicates and thus cannot be studied using differential gel electrophoresis (DIGE). CoFGE corrects for gel-to-gel variability by co-running with the sample proteome a standardized marker grid of 80-100 nodes, which is formed by a set of purified proteins. Differentiation of reference and analyte is possible by the use of two fluorescent dyes. Variations in the y-dimension (molecular weight) are corrected by the marker grid. For the optional control of the x-dimension (pI), azo dyes can be used. Experiments are possible in both vertical and horizontal (h) electrophoresis devices, but hCoFGE is much easier to perform. For data analysis, commercial software capable of warping can be adapted.
Stress distribution in two-dimensional silos
Blanco-Rodríguez, Rodolfo; Pérez-Ángel, Gabriel
2018-01-01
Simulations of a polydispersed two-dimensional silo were performed using molecular dynamics, with different numbers of grains reaching up to 64 000, verifying numerically the model derived by Janssen and also the main assumption that the walls carry part of the weight due to the static friction between grains with themselves and those with the silo's walls. We vary the friction coefficient, the radii dispersity, the silo width, and the size of grains. We find that the Janssen's model becomes less relevant as the the silo width increases since the behavior of the stresses becomes more hydrostatic. Likewise, we get the normal and tangential stress distribution on the walls evidencing the existence of points of maximum stress. We also obtained the stress matrix with which we observe zones of concentration of load, located always at a height around two thirds of the granular columns. Finally, we observe that the size of the grains affects the distribution of stresses, increasing the weight on the bottom and reducing the normal stress on the walls, as the grains are made smaller (for the same total mass of the granulate), giving again a more hydrostatic and therefore less Janssen-type behavior for the weight of the column.
Two-dimensional bipolar junction transistors
Gharekhanlou, Behnaz; Khorasani, Sina; Sarvari, Reza
2014-03-01
Recent development in fabrication technology of planar two-dimensional (2D) materials has introduced the possibility of numerous novel applications. Our recent analysis has revealed that by definition of p-n junctions through appropriate patterned doping of 2D semiconductors, ideal exponential I-V characteristics may be expected. However, the theory of 2D junctions turns out to be very different to that of standard bulk junctions. Based on this theory of 2D diodes, we construct for the first time a model to describe 2D bipolar junction transistors (2D-BJTs). We derive the small-signal equivalent model, and estimate the performance of a 2D-BJT device based on graphone as the example material. A current gain of about 138 and maximum threshold frequency of 77 GHz, together with a power-delay product of only 4 fJ per 1 μm lateral width is expected at an operating voltage of 5 V. In addition, we derive the necessary formulae and a new approximate solution for the continuity equation in the 2D configuration, which have been verified against numerical solutions.
Highly mobile charge-transfer excitons in two-dimensional WS2/tetracene heterostructures
Zhu, Tong; Yuan, Long; Zhao, Yan; Zhou, Mingwei; Wan, Yan; Mei, Jianguo; Huang, Libai
2018-01-01
Charge-transfer (CT) excitons at heterointerfaces play a critical role in light to electricity conversion using organic and nanostructured materials. However, how CT excitons migrate at these interfaces is poorly understood. We investigate the formation and transport of CT excitons in two-dimensional WS2/tetracene van der Waals heterostructures. Electron and hole transfer occurs on the time scale of a few picoseconds, and emission of interlayer CT excitons with a binding energy of ~0.3 eV has been observed. Transport of the CT excitons is directly measured by transient absorption microscopy, revealing coexistence of delocalized and localized states. Trapping-detrapping dynamics between the delocalized and localized states leads to stretched-exponential photoluminescence decay with an average lifetime of ~2 ns. The delocalized CT excitons are remarkably mobile with a diffusion constant of ~1 cm2 s−1. These highly mobile CT excitons could have important implications in achieving efficient charge separation. PMID:29340303
A microprocessor based on a two-dimensional semiconductor
Wachter, Stefan; Polyushkin, Dmitry K.; Bethge, Ole; Mueller, Thomas
2017-04-01
The advent of microcomputers in the 1970s has dramatically changed our society. Since then, microprocessors have been made almost exclusively from silicon, but the ever-increasing demand for higher integration density and speed, lower power consumption and better integrability with everyday goods has prompted the search for alternatives. Germanium and III-V compound semiconductors are being considered promising candidates for future high-performance processor generations and chips based on thin-film plastic technology or carbon nanotubes could allow for embedding electronic intelligence into arbitrary objects for the Internet-of-Things. Here, we present a 1-bit implementation of a microprocessor using a two-dimensional semiconductor--molybdenum disulfide. The device can execute user-defined programs stored in an external memory, perform logical operations and communicate with its periphery. Our 1-bit design is readily scalable to multi-bit data. The device consists of 115 transistors and constitutes the most complex circuitry so far made from a two-dimensional material.
Growth and characterization of two-dimensional nanostructures
International Nuclear Information System (INIS)
Herrera Sancho, Oscar Andrey
2008-01-01
Two dimensional nanostructures of palladium, nickel, silver and gadolinium were grown by means of physical evaporation in atmospheres of high vacuum and ultra high vacuum. The qualitative characterization, in situ, of the nanostructures was carried out with techniques of surface analysis: Auger electron spectroscopy and X-ray photoelectron spectroscopy (XPS). The model for the quantification of contaminants in the nanostructures, was proposed by Seah and Shirley, and was made using the spectra XPS measured in situ in the atmospheres of vacuum. For the two-dimensional nanostructures of gadolinium of thicknesses 8 Å, 16 Å, 24 Å, 32 Å, 36 Å, 44 Å, 50 Å, 61 Å, 77 Å, 81 Å, 92 Å and 101 Å, were obtained optical spectra of transmission measured in situ. An band of absorption centered at approximately 2,40 eV is obtained by an increase in the dynamic conductivity from the optical constants, i.e. refractive index and extinction coefficient, of the nanostructure of gadolinium. In addition, the optical constants for the gadolinium nanostructures have presented a maximum of 80 Å of thickness and then it was continued a decreasing tendency toward the values that were reported in the literature for bulk of gadolinium. (author) [es
Thermal expansion of two-dimensional itinerant nearly ferromagnetic metal
International Nuclear Information System (INIS)
Konno, R; Hatayama, N; Takahashi, Y; Nakano, H
2009-01-01
Thermal expansion of two-dimensional itinerant nearly ferromagnetic metal is investigated according to the recent theoretical development of magneto-volume effect for the three-dimensional weak ferromagnets. We particularly focus on the T 2 -linear thermal expansion of magnetic origin at low temperatures, so far disregarded by conventional theories. As the effect of thermal spin fluctuations we have found that the T-linear thermal expansion coefficient shows strong enhancement by assuming the double Lorentzian form of the non-interacting dynamical susceptibility justified in the small wave-number and low frequency region. It grows faster in proportional to y -1/2 as we approach the magnetic instability point than two-dimensional nearly antiferromagnetic metals with ln(1/y s ) dependence, where y and y s are the inverses of the reduced uniform and staggered magnetic susceptibilities, respectively. Our result is consistent with the Grueneisen's relation between the thermal expansion coefficient and the specific heat at low temperatures. In 2-dimensional electron gas we find that the thermal expansion coefficient is divergent with a finite y when the higher order term of non-interacting dynamical susceptibility is taken into account.
Two-dimensional nuclear magnetic resonance of quadrupolar systems
Energy Technology Data Exchange (ETDEWEB)
Wang, Shuanhu [Univ. of California, Berkeley, CA (United States)
1997-09-01
This dissertation describes two-dimensional nuclear magnetic resonance theory and experiments which have been developed to study quadruples in the solid state. The technique of multiple-quantum magic-angle spinning (MQMAS) is extensively reviewed and expanded upon in this thesis. Specifically, MQMAS is first compared with another technique, dynamic-angle spinning (DAS). The similarity between the two techniques allows us to extend much of the DAS work to the MQMAS case. Application of MQMAS to a series of aluminum containing materials is then presented. The superior resolution enhancement through MQMAS is exploited to detect the five- and six-coordinated aluminum in many aluminosilicate glasses. Combining the MQMAS method with other experiments, such as HETCOR, greatly expands the possibility of the use of MQMAS to study a large range of problems and is demonstrated in Chapter 5. Finally, the technique switching-angle spinning (SAS) is applied to quadrupolar nuclei to fully characterize a quadrupolar spin system in which all of the 8 NMR parameters are accurately determined. This dissertation is meant to demonstrate that with the combination of two-dimensional NMR concepts and new advanced spinning technologies, a series of multiple-dimensional NMR techniques can be designed to allow a detailed study of quadrupolar nuclei in the solid state.
Statistical mechanics of two-dimensional and geophysical flows
International Nuclear Information System (INIS)
Bouchet, Freddy; Venaille, Antoine
2012-01-01
The theoretical study of the self-organization of two-dimensional and geophysical turbulent flows is addressed based on statistical mechanics methods. This review is a self-contained presentation of classical and recent works on this subject; from the statistical mechanics basis of the theory up to applications to Jupiter’s troposphere and ocean vortices and jets. Emphasize has been placed on examples with available analytical treatment in order to favor better understanding of the physics and dynamics. After a brief presentation of the 2D Euler and quasi-geostrophic equations, the specificity of two-dimensional and geophysical turbulence is emphasized. The equilibrium microcanonical measure is built from the Liouville theorem. Important statistical mechanics concepts (large deviations and mean field approach) and thermodynamic concepts (ensemble inequivalence and negative heat capacity) are briefly explained and described. On this theoretical basis, we predict the output of the long time evolution of complex turbulent flows as statistical equilibria. This is applied to make quantitative models of two-dimensional turbulence, the Great Red Spot and other Jovian vortices, ocean jets like the Gulf-Stream, and ocean vortices. A detailed comparison between these statistical equilibria and real flow observations is provided. We also present recent results for non-equilibrium situations, for the studies of either the relaxation towards equilibrium or non-equilibrium steady states. In this last case, forces and dissipation are in a statistical balance; fluxes of conserved quantity characterize the system and microcanonical or other equilibrium measures no longer describe the system.
Energy Technology Data Exchange (ETDEWEB)
Lyubovskii, R. B.; Pesotskii, S. I., E-mail: pesot@icp.ac.ru; Zhilyaeva, E. I.; Lyubovskaya, R. N. [Russian Academy of Sciences, Institute of Problems of Chemical Physics (Russian Federation)
2016-01-15
The behavior of the interlayer resistance and the magnetoresistance in the organic quasi-twodimensional bilayer metal θ-(BETS){sub 4}HgBr{sub 4}(C{sub 6}H{sub 5}Cl) is studied at normal pressure and a hydrostatic pressure of 10 kbar. The interlayer transport under atmospheric pressure is found to occur in an incoherent mode. The applied pressure does not change the electronic structure of the conducting layers and causes a transition to a weakly coherent mode at low temperatures.
Asano, Takanori; Takaishi, Riichiro; Oda, Minoru; Sakuma, Kiwamu; Saitoh, Masumi; Tanaka, Hiroki
2018-04-01
We visualize the grain structures for individual nanosized thin film transistors (TFTs), which are electrically characterized, with an improved data processing technique for the dark-field image reconstruction of nanobeam electron diffraction maps. Our individual crystal analysis gives the one-to-one correspondence of TFTs with different grain boundary structures, such as random and coherent boundaries, to the characteristic degradations of ON-current and threshold voltage. Furthermore, the local crystalline uniformity inside a single grain is detected as the difference in diffraction intensity distribution.
Dynamics of two-dimensional bubbles
Piedra, Saúl; Ramos, Eduardo; Herrera, J. Ramón
2015-06-01
The dynamics of two-dimensional bubbles ascending under the influence of buoyant forces is numerically studied with a one-fluid model coupled with the front-tracking technique. The bubble dynamics are described by recording the position, shape, and orientation of the bubbles as functions of time. The qualitative properties of the bubbles and their terminal velocities are described in terms of the Eötvos (ratio of buoyancy to surface tension) and Archimedes numbers (ratio of buoyancy to viscous forces). The terminal Reynolds number result from the balance of buoyancy and drag forces and, consequently, is not an externally fixed parameter. In the cases that yield small Reynolds numbers, the bubbles follow straight paths and the wake is steady. A more interesting behavior is found at high Reynolds numbers where the bubbles follow an approximately periodic zigzag trajectory and an unstable wake with properties similar to the Von Karman vortex street is formed. The dynamical features of the motion of single bubbles are compared to experimental observations of air bubbles ascending in a water-filled Hele-Shaw cell. Although the comparison is not strictly valid in the sense that the effect of the lateral walls is not incorporated in the model, most of the dynamical properties observed are in good qualitative agreement with the numerical calculations. Hele-Shaw cells with different gaps have been used to determine the degree of approximation of the numerical calculation. It is found that for the relation between the terminal Reynolds number and the Archimedes number, the numerical calculations are closer to the observations of bubble dynamics in Hele-Shaw cells of larger gaps.
Suspension and simple optical characterization of two-dimensional membranes
Northeast, David B.; Knobel, Robert G.
2018-03-01
We report on a method for suspending two-dimensional crystal materials in an electronic circuit using an only photoresists and solvents. Graphene and NbSe2 are suspended tens of nanometers above metal electrodes with clamping diameters of several microns. The optical cavity formed from the membrane/air/metal structures enables a quick method to measure the number of layers and the gap separation using comparisons between the expected colour and optical microscope images. This characterization technique can be used with just an illuminated microscope with a digital camera which makes it adaptable to environments where other means of characterization are not possible, such as inside nitrogen glove boxes used in handling oxygen-sensitive materials.
The first principle calculation of two-dimensional Dirac materials
Lu, Jin
2017-12-01
As the size of integrated device becoming increasingly small, from the last century, semiconductor industry is facing the enormous challenge to break the Moore’s law. The development of calculation, communication and automatic control have emergent expectation of new materials at the aspect of semiconductor industrial technology and science. In spite of silicon device, searching the alternative material with outstanding electronic properties has always been a research point. As the discovery of graphene, the research of two-dimensional Dirac material starts to express new vitality. This essay studied the development calculation of 2D material’s mobility and introduce some detailed information of some approximation method of the first principle calculation.
Two-dimensional spectrophotometry of planetary nebulae by CCD imaging
International Nuclear Information System (INIS)
Jacoby, G.H.; Africano, J.L.; Quigley, R.J.; Western Washington Univ., Bellingham, WA)
1987-01-01
The spatial distribution of the electron temperature and density and the ionic abundances of O(+), O(2+), N(+), and S(+) have been derived from CCD images of the planetary nebulae NGC 40 and NGC 6826 taken in the important emission lines of forbidden O II, forbidden O III, H-beta, forbidden N II, and forbidden S II. The steps required in the derivation of the absolute fluxes, line, ratios, and ionic abundances are outlined and then discussed in greater detail. The results show that the CCD imaging technique for two-dimensional spectrophotometry can effectively compete with classical spectrophotometry, providing the added benefits of complete spatial coverage at seeing-disk spatial resolution. The multiplexing in the spatial dimension, however, results in a loss of spectral information, since only one emission line is observed at any one time. 37 references