WorldWideScience

Sample records for stratospheric cloud surfaces

  1. Strong modification of stratospheric ozone forcing by cloud and sea-ice adjustments

    Directory of Open Access Journals (Sweden)

    Y. Xia

    2016-06-01

    Full Text Available We investigate the climatic impact of stratospheric ozone recovery (SOR, with a focus on the surface temperature change in atmosphere–slab ocean coupled climate simulations. We find that although SOR would cause significant surface warming (global mean: 0.2 K in a climate free of clouds and sea ice, it causes surface cooling (−0.06 K in the real climate. The results here are especially interesting in that the stratosphere-adjusted radiative forcing is positive in both cases. Radiation diagnosis shows that the surface cooling is mainly due to a strong radiative effect resulting from significant reduction of global high clouds and, to a lesser extent, from an increase in high-latitude sea ice. Our simulation experiments suggest that clouds and sea ice are sensitive to stratospheric ozone perturbation, which constitutes a significant radiative adjustment that influences the sign and magnitude of the global surface temperature change.

  2. Condensed Acids In Antartic Stratospheric Clouds

    Science.gov (United States)

    Pueschel, R. F.; Snetsinger, K. G.; Toon, O. B.; Ferry, G. V.; Starr, W. L.; Oberbeck, V. R.; Chan, K. R.; Goodman, J. K.; Livingston, J. M.; Verma, S.; hide

    1992-01-01

    Report dicusses nitrate, sulfate, and chloride contents of stratospheric aerosols during 1987 Airborne Antarctic Ozone Experiment. Emphasizes growth of HNO3*3H2O particles in polar stratospheric clouds. Important in testing theories concerning Antarctic "ozone hole".

  3. Detection of polar stratospheric clouds with ERS2/GOME data

    International Nuclear Information System (INIS)

    Meerkoetter, R.; Schumann, U.

    1994-01-01

    Based on radiative transfer calculations it is studied whether Polar Stratospheric Clouds (PSCs) can be detected by the new Global Ozone Monitoring Experiment (GOME) onboard the second European Research Satellite (ERS-2) planned to be launched in winter 1994/95. It is proposed to identify PSC covered areas by use of an indicator, the Normalized Radiance Difference (NRD), which relates the difference of two spectral radiances at 0.5 μm and 0.7 μm to one radiance measured in the center of the oxygen A-band at 0.76 μm. The presence of PSCs and under conditions of large solar zenith angles Θ>80 the NRD values are clearly below those derived under conditions of a cloud free stratosphere. In this case the method is successful for PSCs with optical depths greater than 0.03 at 0.55 μm. It is not affected by existing tropospheric clouds and by different tropospheric aerosol loadings or surface albedoes. For solar zenith angles Θ<80 PSCs located above a cloud free troposphere are detectable. PSC detection becomes difficult for Θ<80 when highly reflecting tropospheric clouds like dense cirrus or stratus clouds affect spectral radiances measured at the top of the atmosphere. (orig.)

  4. Laboratory investigation of nitrile ices of Titan's stratospheric clouds

    Science.gov (United States)

    Nna Mvondo, D.; Anderson, C. M.; McLain, J. L.; Samuelson, R. E.

    2017-09-01

    Titan's mid to lower stratosphere contains complex cloud systems of numerous organic ice particles comprised of both hydrocarbon and nitrile compounds. Most of these stratospheric ice clouds form as a result of vapor condensation formation processes. However, there are additional ice emission features such as dicyanoacetylene (C4N2) and the 220 cm-1 ice emission feature (the "Haystack") that are difficult to explain since there are no observed vapor emission features associated with these ices. In our laboratory, using a high-vacuum chamber coupled to a FTIR spectrometer, we are engaged in a dedicated investigation of Titan's stratospheric ices to interpret and constrain Cassini Composite InfraRed Spectrometer (CIRS) far-IR data. We will present laboratory transmittance spectra obtained for propionitrile (CH3CH2CN), cyanogen (C2N2) and hydrogen cyanide (HCN) ices, as well as various combinations of their mixtures, to better understand the cloud chemistry occurring in Titan's stratosphere.

  5. Solid-State Photochemistry as a Formation Mechanism for Titan's Stratospheric C4N2 Ice Clouds

    Science.gov (United States)

    Anderson, C. M.; Samuelson, R. E.; Yung, Y. L.; McLain, J. L.

    2016-01-01

    We propose that C4N2 ice clouds observed in Titan's springtime polar stratosphere arise due to solid-state photochemistry occurring within extant ice cloud particles of HCN-HC3N mixtures. This formation process resembles the halogen-induced ice particle surface chemistry that leads to condensed nitric acid trihydrate (NAT) particles and ozone depletion in Earth's polar stratosphere. As our analysis of the Cassini Composite Infrared Spectrometer 478 per centimeter ice emission feature demonstrates, this solid-state photochemistry mechanism eliminates the need for the relatively high C4N2 saturation vapor pressures required (even though they are not observed) when the ice is produced through the usual procedure of direct condensation from the vapor.

  6. Application of physical adsorption thermodynamics to heterogeneous chemistry on polar stratospheric clouds

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    Elliott, Scott; Turco, Richard P.; Toon, Owen B.; Hamill, Patrick

    1991-01-01

    Laboratory isotherms for the binding of several nonheterogeneously active atmospheric gases and for HCl to water ice are translated into adsorptive equilibrium constants and surface enthalpies. Extrapolation to polar conditions through the Clausius Clapeyron relation yields coverage estimates below the percent level for N2, Ar, CO2, and CO, suggesting that the crystal faces of type II stratospheric cloud particles may be regarded as clean with respect to these species. For HCl, and perhaps HF and HNO3, estimates rise to several percent, and the adsorbed layer may offer acid or proton sources alternate to the bulk solid for heterogeneous reactions with stratospheric nitrates. Measurements are lacking for many key atmospheric molecules on water ice, and almost entirely for nitric acid trihydrate as substrate. Adsorptive equilibria enter into gas to particle mass flux descriptions, and the binding energy determines rates for desorption of, and encounter between, potential surface reactants.

  7. Monstrous Ice Cloud System in Titan's Present South Polar Stratosphere

    Science.gov (United States)

    Anderson, Carrie; Samuelson, Robert; McLain, Jason; Achterberg, Richard; Flasar, F. Michael; Milam, Stefanie

    2015-11-01

    During southern autumn when sunlight was still available, Cassini's Imaging Science Subsystem discovered a cloud around 300 km near Titan's south pole (West, R. A. et al., AAS/DPS Abstracts, 45, #305.03, 2013); the cloud was later determined by Cassini's Visible and InfraRed Mapping Spectrometer to contain HCN ice (de Kok et al., Nature, 514, pp 65-67, 2014). This cloud has proven to be only the tip of an extensive ice cloud system contained in Titan's south polar stratosphere, as seen through the night-vision goggles of Cassini's Composite InfraRed Spectrometer (CIRS). As the sun sets and the gloom of southern winter approaches, evidence is beginning to accumulate from CIRS far-IR spectra that a massive system of nitrile ice clouds is developing in Titan's south polar stratosphere. Even during the depths of northern winter, nothing like the strength of this southern system was evident in corresponding north polar regions.From the long slant paths that are available from limb-viewing CIRS far-IR spectra, we have the first definitive detection of the ν6 band of cyanoacetylene (HC3N) ice in Titan’s south polar stratosphere. In addition, we also see a strong blend of nitrile ice lattice vibration features around 160 cm-1. From these data we are able to derive ice abundances. The most prominent (and still chemically unidentified) ice emission feature, the Haystack, (at 220 cm-1) is also observed. We establish the vertical distributions of the ice cloud systems associated with both the 160 cm-1 feature and the Haystack. The ultimate aim is to refine the physical and possibly the chemical relationships between the two. Transmittance thin film spectra of nitrile ice mixtures obtained in our Spectroscopy for Planetary ICes Environments (SPICE) laboratory are used to support these analyses.

  8. The Effect of Cirrus Clouds on Water Vapor Transport in the Upper Troposphere and Lower Stratosphere

    Science.gov (United States)

    Lei, L.; McCormick, M. P.; Anderson, J.

    2017-12-01

    Water vapor plays an important role in the Earth's radiation budget and stratospheric chemistry. It is widely accepted that a large percentage of water vapor entering the stratosphere travels through the tropical tropopause and is dehydrated by the cold tropopause temperature. The vertical transport of water vapor is also affected by the radiative effects of cirrus clouds in the tropical tropopause layer. This latter effect of cirrus clouds was investigated in this research. The work focuses on the tropical and mid-latitude region (50N-50S). Water vapor data from the Microwave Limb Sounder (MLS) and cirrus cloud data from the Cloud-Aerosol Lidar and Infrared pathfinder Satellite Observation (CALIPSO) instruments were used to investigate the relationship between the water vapor and the occurrence of cirrus cloud. A 10-degree in longitude by 10-degree in latitude resolution was chosen to bin the MLS and CALIPSO data. The result shows that the maximum water vapor in the upper troposphere (below 146 hPa) is matched very well with the highest frequency of cirrus cloud occurrences. Maximum water vapor in the lower stratosphere (100 hPa) is partly matched with the maximum cirrus cloud occurrence in the summer time. The National Oceanic and Atmospheric Administration Interpolated Outgoing Longwave Radiation data and NCEP-DOE Reanalysis 2 wind data were used also to investigate the relationship between the water vapor entering the stratosphere, deep convection, and wind. Results show that maximum water vapor at 100 hPa coincides with the northern hemisphere summer-time anticyclone. The effects from both single-layer cirrus clouds and cirrus clouds above the anvil top on the water vapor entering the stratosphere were also studied and will be presented.

  9. Measurements of size and composition of particles in polar stratospheric clouds from infrared solar absorption spectra

    International Nuclear Information System (INIS)

    Kinne, S.; Toon, O.B.; Toon, G.C.; Farmer, C.B.; Browell, E.V.; McCormick, M.P.

    1989-01-01

    The attenuation of solar radiation between 1.8- and 15-μm wavelength was measured with the airborne Jet Propulsion Laboratory Mark IV interferometer during the Airborne Antarctic Ozone Expedition in 1987. The measurements not only provide information about the abundance of stratospheric gases, but also about the optical depths of polar stratospheric clouds (PSCs) at wavelengths of negligible gas absorption. The spectral dependence of the PSC optical depth contains information about PSC particle size and particle composition. Thirty-three PSC cases were analyzed and categorized into two types. Type I clouds contain particles with radii of about 0.5 μm and nitric acid concentrations greater than 40%. Type II clouds contain particles composed of water ice with radii of 6 μm and larger. Cloud altitudes were determined from 1.064-μm backscattering observations of the airborne Langley DIAL lidar system. Based on the PSC geometrical thickness, both mass and particle density were estimated. Type I clouds typically had visible wavelength optical depths of about 0.008, mass densities of about 20 ppb, and about 2 particles/cm 3 . The observed type II clouds had optical depths of about 0.03, mass densities of about 400 ppb mass, and about 0.03 particles/cm 3 . The detected PSC type I clouds extended to altitudes of 21 km and were nearly in the ozone-depleted region of the polar stratosphere. The observed type II cases during September were predominantly found at altitudes below 15 km

  10. Persistence of Antarctic polar stratospheric clouds

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    Mccormick, M. Patrick; Trepte, C. R.

    1988-01-01

    The persistence of Polar Stratospheric Clouds (PSCs) observed by the Stratospheric Aerosol Measurement (SAM) 2 satellite sensor over a 9-year period is compared and contrasted. Histograms of the SAM 2 1.0 micron extinction ratio data (aerosol extinction normalized by the molecular extinction) at an altitude of 18 km in the Antarctic have been generated for three 10-day periods in the month of September. Statistics for eight different years (1979 to 1982 and 1984 to 1987) are shown in separate panels for each figure. Since the SAM 2 system is a solar occultation experiment, observations are limited to the edge of the polar night and no measurements are made deep within the vortex where temperatures could be colder. For this reason, use is made of the NMC global gridded fields and the known temperature-extinction relationship to infer additional information on the occurrence and areal coverage of PSCs. Calculations of the daily areal coverage of the 195 K isotherm will be presented for this same period of data. This contour level lies in the range of the predicted temperature for onset of the Type 1 particle enhancement mode at 50 mb (Poole and McCormick, 1988b) and should indicate approximately when formation of the binary HNO3-H2O particles begins.

  11. Heterogeneous Formation of Polar Stratospheric Clouds- Part 1: Nucleation of Nitric Acid Trihydrate (NAT)

    Science.gov (United States)

    Hoyle, C. R.; Engel, I.; Luo, B. P.; Pitts, M. C.; Poole, L. R.; Grooss, J.-U.; Peter, T.

    2013-01-01

    Satellite-based observations during the Arctic winter of 2009/2010 provide firm evidence that, in contrast to the current understanding, the nucleation of nitric acid trihydrate (NAT) in the polar stratosphere does not only occur on preexisting ice particles. In order to explain the NAT clouds observed over the Arctic in mid-December 2009, a heterogeneous nucleation mechanism is required, occurring via immersion freezing on the surface of solid particles, likely of meteoritic origin. For the first time, a detailed microphysical modelling of this NAT formation pathway has been carried out. Heterogeneous NAT formation was calculated along more than sixty thousand trajectories, ending at Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) observation points. Comparing the optical properties of the modelled NAT with these observations enabled a thorough validation of a newly developed NAT nucleation parameterisation, which has been built into the Zurich Optical and Microphysical box Model (ZOMM). The parameterisation is based on active site theory, is simple to implement in models and provides substantial advantages over previous approaches which involved a constant rate of NAT nucleation in a given volume of air. It is shown that the new method is capable of reproducing observed polar stratospheric clouds (PSCs) very well, despite the varied conditions experienced by air parcels travelling along the different trajectories. In a companion paper, ZOMM is applied to a later period of the winter, when ice PSCs are also present, and it is shown that the observed PSCs are also represented extremely well under these conditions.

  12. A closer look at Arctic ozone loss and polar stratospheric clouds

    Directory of Open Access Journals (Sweden)

    N. R. P. Harris

    2010-09-01

    Full Text Available The empirical relationship found between column-integrated Arctic ozone loss and the potential volume of polar stratospheric clouds inferred from meteorological analyses is recalculated in a self-consistent manner using the ERA Interim reanalyses. The relationship is found to hold at different altitudes as well as in the column. The use of a PSC formation threshold based on temperature dependent cold aerosol formation makes little difference to the original, empirical relationship. Analysis of the photochemistry leading to the ozone loss shows that activation is limited by the photolysis of nitric acid. This step produces nitrogen dioxide which is converted to chlorine nitrate which in turn reacts with hydrogen chloride on any polar stratospheric clouds to form active chlorine. The rate-limiting step is the photolysis of nitric acid: this occurs at the same rate every year and so the interannual variation in the ozone loss is caused by the extent and persistence of the polar stratospheric clouds. In early spring the ozone loss rate increases as the solar insolation increases the photolysis of the chlorine monoxide dimer in the near ultraviolet. However the length of the ozone loss period is determined by the photolysis of nitric acid which also occurs in the near ultraviolet. As a result of these compensating effects, the amount of the ozone loss is principally limited by the extent of original activation rather than its timing. In addition a number of factors, including the vertical changes in pressure and total inorganic chlorine as well as denitrification and renitrification, offset each other. As a result the extent of original activation is the most important factor influencing ozone loss. These results indicate that relatively simple parameterisations of Arctic ozone loss could be developed for use in coupled chemistry climate models.

  13. Detection and mapping of polar stratospheric clouds using limb scattering observations

    Directory of Open Access Journals (Sweden)

    C. von Savigny

    2005-01-01

    Full Text Available Satellite-based measurements of Visible/NIR limb-scattered solar radiation are well suited for the detection and mapping of polar stratospheric clouds (PSCs. This publication describes a method to detect PCSs from limb scattering observations with the Scanning Imaging Absorption spectroMeter for Atmospheric CartograpHY (SCIAMACHY on the European Space Agency's Envisat spacecraft. The method is based on a color-index approach and requires a priori knowledge of the stratospheric background aerosol loading in order to avoid false PSC identifications by stratospheric background aerosol. The method is applied to a sample data set including the 2003 PSC season in the Southern Hemisphere. The PSCs are correlated with coincident UKMO model temperature data, and with very few exceptions, the detected PSCs occur at temperatures below 195–198 K. Monthly averaged PSC descent rates are about 1.5 km/month for the −50° S to −75° S latitude range and assume a maximum between August and September with a value of about 2.5 km/month. The main cause of the PSC descent is the slow descent of the lower stratospheric temperature minimum.

  14. Cloud sensitivity studies for stratospheric and lower mesospheric ozone profile retrievals from measurements of limb-scattered solar radiation

    Directory of Open Access Journals (Sweden)

    T. Sonkaew

    2009-11-01

    Full Text Available Clouds in the atmosphere play an important role in reflection, absorption and transmission of solar radiation and thus affect trace gas retrievals. The main goal of this paper is to examine the sensitivity of stratospheric and lower mesospheric ozone retrievals from limb-scattered radiance measurements to clouds using the SCIATRAN radiative transfer model and retrieval package. The retrieval approach employed is optimal estimation, and the considered clouds are vertically and horizontally homogeneous. Assuming an aerosol-free atmosphere and Mie phase functions for cloud particles, we compute the relative error of ozone profile retrievals in a cloudy atmosphere if clouds are neglected in the retrieval. To access altitudes from the lower stratosphere up to the lower mesosphere, we combine the retrievals in the Chappuis and Hartley ozone absorption bands. We find significant cloud sensitivity of the limb ozone retrievals in the Chappuis bands at lower stratospheric altitudes. The relative error in the retrieved ozone concentrations gradually decreases with increasing altitude and becomes negligible above approximately 40 km. The parameters with the largest impact on the ozone retrievals are cloud optical thickness, ground albedo and solar zenith angle. Clouds with different geometrical thicknesses or different cloud altitudes have a similar impact on the ozone retrievals for a given cloud optical thickness value, if the clouds are outside the field of view of the instrument. The effective radius of water droplets has a small influence on the error, i.e., less than 0.5% at altitudes above the cloud top height. Furthermore, the impact of clouds on the ozone profile retrievals was found to have a rather small dependence on the solar azimuth angle (less than 1% for all possible azimuth angles. For the most frequent cloud types, the total error is below 6% above 15 km altitude, if clouds are completely neglected in the retrieval. Neglecting clouds in

  15. Radiative-dynamical and microphysical processes of thin cirrus clouds controlling humidity of air entering the stratosphere

    Science.gov (United States)

    Dinh, Tra; Fueglistaler, Stephan

    2016-04-01

    Thin cirrus clouds in the tropical tropopause layer (TTL) are of great interest due to their role in the control of water vapor and temperature in the TTL. Previous research on TTL cirrus clouds has focussed mainly on microphysical processes, specifically the ice nucleation mechanism and dehydration efficiency. Here, we use a cloud resolving model to analyse the sensitivity of TTL cirrus characteristics and impacts with respect to microphysical and radiative processes. A steady-state TTL cirrus cloud field is obtained in the model forced with dynamical conditions typical for the TTL (2-dimensional setup with a Kelvin-wave temperature perturbation). Our model results show that the dehydration efficiency (as given by the domain average relative humidity in the layer of cloud occurrence) is relatively insensitive to the ice nucleation mechanism, i.e. homogeneous versus heterogeneous nucleation. Rather, TTL cirrus affect the water vapor entering the stratosphere via an indirect effect associated with the cloud radiative heating and dynamics. Resolving the cloud radiative heating and the radiatively induced circulations approximately doubles the domain average ice mass. The cloud radiative heating is proportional to the domain average ice mass, and the observed increase in domain average ice mass induces a domain average temperature increase of a few Kelvin. The corresponding increase in water vapor entering the stratosphere is estimated to be about 30 to 40%.

  16. Laboratory studies of stratospheric aerosol chemistry

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    Molina, Mario J.

    1996-01-01

    In this report we summarize the results of the two sets of projects funded by the NASA grant NAG2-632, namely investigations of various thermodynamic and nucleation properties of the aqueous acid system which makes up stratospheric aerosols, and measurements of reaction probabilities directly on ice aerosols with sizes corresponding to those of polar stratospheric cloud particles. The results of these investigations are of importance for the assessment of the potential stratospheric effects of future fleets of supersonic aircraft. In particular, the results permit to better estimate the effects of increased amounts of water vapor and nitric acid (which forms from nitrogen oxides) on polar stratospheric clouds and on the chemistry induced by these clouds.

  17. A Climatology of Polar Stratospheric Cloud Types by MIPAS-Envisat

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    Spang, Reinhold; Hoffmann, Lars; Griessbach, Sabine; Orr, Andrew; Höpfner, Michael; Müller, Rolf

    2015-04-01

    For Chemistry Climate Models (CCM) it is still a challenging task to properly represent the evolution of the polar vortices over the entire winter season. The models usually do not include comprehensive microphysical modules to evolve the formation of different types of polar stratospheric clouds (PSC) over the winter. Consequently, predictions on the development and recovery of the future ozone hole have relatively large uncertainties. A climatological record of hemispheric measurement of PSC types could help to better validate and improve the PSC schemes in CCMs. The Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) instrument onboard the ESA Envisat satellite operated from July 2002 to April 2012. The infra-red limb emission measurements compile a unique dataset of day and night measurements of polar stratospheric clouds up to the poles. From the spectral measurements in the 4.15-14.6 microns range it is possible to select a number of atmospheric window regions and spectral signatures to classify PSC cloud types like nitric acid hydrates, sulfuric ternary solution droplets, and ice particles. The cloud detection sensitivity is similar to space borne lidars, but MIPAS adds complementary information due to its different measurement technique (limb instead of nadir) and wavelength region. Here we will describe a new classification method for PSCs based on the combination of multiple brightness temperature differences (BTD) and colour ratios. Probability density functions (PDF) of the MIPAS measurements in conjunction with a database of radiative transfer model calculations of realistic PSC particle size distributions enable the definition of regions attributed to specific or mixed types clouds. Applying a naive bias classifier for independent criteria to all defined classes in four 2D PDF distributions, it is possible to assign the most likely PSC type to any measured cloud spectrum. Statistical Monte Carlo test have been applied to quantify

  18. What Controls the Temperature of the Arctic Stratosphere during the Spring?

    Science.gov (United States)

    Newman, Paul A.; Nash, Eric R.; Rosenfield, Joan E.; Einaudi, Franco (Technical Monitor)

    2000-01-01

    Understanding the mechanisms that control the temperature of the polar lower stratosphere during spring is key to understanding ozone loss in the Arctic polar vortex. Spring ozone loss rates are directly tied to polar stratospheric temperatures by the formation of polar stratospheric clouds, and the conversion of chlorine species to reactive forms on these cloud particle surfaces. In this paper, we study those factors that control temperatures in the polar lower stratosphere. We use the National Centers for Environmental Prediction (NCEP)/NCAR reanalysis data covering the last two decades to investigate how planetary wave driving of the stratosphere is connected to polar temperatures. In particular, we show that planetary waves forced in the troposphere in mid- to late winter (January-February) are principally responsible for the mean polar temperature during the March period. These planetary waves are forced by both thermal and orographic processes in the troposphere, and propagate into the stratosphere in the mid and high latitudes. Strong mid-winter planetary wave forcing leads to a warmer Arctic lower stratosphere in early spring, while weak mid-winter forcing leads to cooler Arctic temperatures.

  19. A polar stratospheric cloud parameterization for the global modeling initiative three-dimensional model and its response to stratospheric aircraft

    International Nuclear Information System (INIS)

    Considine, D. B.; Douglass, A. R.; Connell, P. S.; Kinnison, D. E.; Rotman, D. A.

    2000-01-01

    We describe a new parameterization of polar stratospheric clouds (PSCs) which was written for and incorporated into the three-dimensional (3-D) chemistry and transport model (CTM) developed for NASA's Atmospheric Effects of Aviation Project (AEAP) by the Global Modeling Initiative (GMI). The parameterization was designed to respond to changes in NO y and H 2 O produced by high-speed civilian transport (HSCT) emissions. The parameterization predicts surface area densities (SADs) of both Type 1 and Type 2 PSCs for use in heterogeneous chemistry calculations. Type 1 PSCs are assumed to have a supercooled ternary sulfate (STS) composition, and Type 2 PSCs are treated as water ice with a coexisting nitric acid trihydrate (NAT) phase. Sedimentation is treated by assuming that the PSC particles obey lognormal size distributions, resulting in a realistic mass flux of condensed phase H 2 O and HNO 3 . We examine a simulation of the Southern Hemisphere high-latitude lower stratosphere winter and spring seasons driven by temperature and wind fields from a modified version of the National Center for Atmospheric Research (NCAR) Middle Atmosphere Community Climate Model Version 2 (MACCM2). Predicted PSC SADs and median radii for both Type 1 and Type 2 PSCs are consistent with observations. Gas phase HNO 3 and H 2 O concentrations in the high-latitude lower stratosphere qualitatively agree with Cryogenic Limb Array Etalon Spectrometer (CLAES) HNO 3 and Microwave Limb Sounder (MLS) H 2 O observations. The residual denitrification and dehydration of the model polar vortex after polar winter compares well with atmospheric trace molecule spectroscopy (ATMOS) observations taken during November 1994. When the NO x and H 2 O emissions of a standard 500-aircraft HSCT fleet with a NO x emission index of 5 are added, NO x and H 2 O concentrations in the Southern Hemisphere polar vortex before winter increase by up to 3%. This results in earlier onset of PSC formation, denitrification, and

  20. NASA Experiment on Tropospheric-Stratospheric Water Vapor Transport in the Intertropical Convergence Zone

    Science.gov (United States)

    Page, William A.

    1982-01-01

    The following six papers report preliminary results obtained from a field experiment designed to study the role of tropical cumulo-nimbus clouds in the transfer of water vapor from the troposphere to the stratosphere over the region of Panama. The measurements were made utilizing special NOAA enhanced IR satellite images, radiosonde-ozonesondes and a NASA U-2 aircraft carrying. nine experiments. The experiments were provided by a group of NASA, NOAA, industry, and university scientists. Measurements included atmospheric humidity, air and cloud top temperatures, atmospheric tracer constituents, cloud particle characteristics and cloud morphology. The aircraft made a total of eleven flights from August 30 through September 18, 1980, from Howard Air Force Base, Panama; the pilots obtained horizontal and vertical profiles in and near convectively active regions and flew around and over cumulo-nimbus towers and through the extended anvils in the stratosphere. Cumulo-nimbus clouds in the tropics appear to play an important role in upward water vapor transport and may represent the principal source influencing the stratospheric water vapor budget. The clouds provide strong vertical circulation in the troposphere, mixing surface air and its trace materials (water vapor, CFM's sulfur compounds, etc.) quickly up to the tropopause. It is usually assumed that large scale mean motions or eddy scale motions transport the trace materials through the tropopause and into the stratosphere where they are further dispersed and react with other stratospheric constituents. The important step between the troposphere and stratosphere for water vapor appears to depend upon the processes occurring at or near the tropopause at the tops of the cumulo-nimbus towers. Several processes have been sugested: (1) The highest towers penetrate the tropopause and carry water in the form of small ice particles directly into the stratosphere. (2) Water vapor from the tops of the cumulonimbus clouds is

  1. ATMOS Stratospheric Deuterated Water and Implications for Tropospheric-Stratospheric Transport

    Science.gov (United States)

    Moyer, Elisabeth J.; Irion, Fredrick W.; Yung, Yuk L.; Gunson, Michael R.

    1996-01-01

    Measurements of the isotopic composition of stratospheric water by the ATMOS instrument are used to infer the convective history of stratospheric air. The average water vapor entering the stratosphere is found to be highly depleted of deuterium, with delta-D(sub w) of -670 +/- 80 (67% deuterium loss). Model calculations predict, however, that under conditions of thermodynamic equilibrium, dehydration to stratospheric mixing ratios should produce stronger depletion to delta-D(sub w) of -800 to 900 (80-90% deuterium loss). Deuterium enrichment of water vapor in ascending parcels can occur only in conditions of rapid convection; enrichments persisting into the stratosphere require that those conditions continue to near-tropopause altitudes. We conclude that either the predominant source of water vapor to the uppermost troposphere is enriched convective water, most likely evaporated cloud ice, or troposphere-stratosphere transport occurs closely associated with tropical deep convection.

  2. Stratospheric effects on trends of mesospheric ice clouds (Invited)

    Science.gov (United States)

    Luebken, F.; Baumgarten, G.; Berger, U.

    2009-12-01

    Ice layers in the summer mesosphere at middle and polar latitudes appear as `noctilucent clouds' (NLC) and `polar mesosphere clouds'(PMC) when observed by optical methods from the ground or from satellites, respectively. A newly developed model of the atmosphere called LIMA (Leibniz Institute Middle Atmosphere Model) nicely reproduces the mean conditions of the summer mesopause region and is used to study the ice layer morphology (LIMA/ice). LIMA nudges to ECMWF data in the troposphere and lower stratosphere which influences the background conditions in the mesosphere and ice cloud morphology. Since ice layer formation is very sensitive to the thermal structure of the mesopause region the morphology of NLC and PMC is frequently discussed in terms of long term variations. Model runs of LIMA/ice are now available for 1961 until 2008. A strong correlation between temperatures and PMC altitudes is observed. Applied to historical measurements this gives negligible temperature trends at PMC altitudes (approximately 0.01-0.02 K/y). Trace gas concentrations are kept constant in LIMA except for water vapor which is modified by variable solar radiation. Still, long term trends in temperatures and ice layer parameters are observed, consistent with observations. We present results regarding inter-annual variability of upper mesosphere temperatures, water vapor, and ice clouds, and also long term variations. We compare our model results with satellite borne and lidar observations including some record high NLC parameters measured in the summer season of 2009. The latitudinal dependence of trends and ice layer parameters is discussed, including a NH/SH comparison. We will present an explanation of the trends in the background atmosphere and ice layer parameters.

  3. A new backscatter lidar for the whole-year study of temperatures and clouds in the polar stratosphere and mesosphere; Ein neues Rueckstreu-Lidar zur ganzjaehrigen Untersuchung von Temperaturen und Wolkenphaenomenen in der polaren Strato- und Mesosphaere

    Energy Technology Data Exchange (ETDEWEB)

    Mueller, K P

    2000-01-01

    Temperatures in the polar middle atmosphere can fall to extremely low values leading to cloud formation in otherwise cloud-free regions: in summer near the mesopause i.e. noctiluent clouds (NLC) and in winter in the lower stratosphere, i.e. polar stratospheric clouds (PSC). Both clouds are environmentally important, PSCs in the ozone problem and NLCs as early indicators of climate change. To investigate these clouds and to measure temperature profiles the atmospheric physics group set up a backscatter lidar on the Esrange in northern Sweden. Based on our experience with a lidar in Norway the mechanics and optics were redesigned to allow for simultaneous measurements of the depolarization of the backscattered light, three colour measurements and measurements in daylight. A numerical simulation of the daylight filter characteristics suggests that the presently used tuning method should be replaced. The first measurements with this new lidar design on the Esrange were obtained in January 1997. PSCs were observed on 19 days from January to March. Surprisingly, PSCs of type 2 were detected several times even when though synoptic stratospheric temperatures were too warm for such clouds to exist. Temperatures in the lee of the Scandinavian mountains had been lowered by internal waves sufficiently to generate PSC type 2 clouds. Among the previous PSC-observations in January 1995 when the lidar was located on the Norwegian island Andoeya was a singular PSC of type 2 on on January 14, 1995, which had a surface area density two orders of magnitudes higher than typically assumed in theoretical models describing ozone depletion. (orig.)

  4. Stratospheric Impact of Varying Sea Surface Temperatures

    Science.gov (United States)

    Newman, Paul A.; Nash, Eric R.; Nielsen, Jon E.; Waugh, Darryn; Pawson, Steven

    2004-01-01

    The Finite-Volume General Circulation Model (FVGCM) has been run in 50 year simulations with the: 1) 1949-1999 Hadley Centre sea surface temperatures (SST), and 2) a fixed annual cycle of SSTs. In this presentation we first show that the 1949-1999 FVGCM simulation produces a very credible stratosphere in comparison to an NCEP/NCAR reanalysis climatology. In particular, the northern hemisphere has numerous major and minor stratospheric warming, while the southern hemisphere has only a few over the 50-year simulation. During the northern hemisphere winter, temperatures are both warmer in the lower stratosphere and the polar vortex is weaker than is found in the mid-winter southern hemisphere. Mean temperature differences in the lower stratosphere are shown to be small (less than 2 K), and planetary wave forcing is found to be very consistent with the climatology. We then will show the differences between our varying SST simulation and the fixed SST simulation in both the dynamics and in two parameterized trace gases (ozone and methane). In general, differences are found to be small, with subtle changes in planetary wave forcing that lead to reduced temperatures in the SH and increased temperatures in the NH.

  5. Fast cloud parameter retrievals of MIPAS/Envisat

    Directory of Open Access Journals (Sweden)

    R. Spang

    2012-08-01

    Full Text Available The infrared limb spectra of the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS on board the Envisat satellite include detailed information on tropospheric clouds and polar stratospheric clouds (PSC. However, no consolidated cloud product is available for the scientific community. Here we describe a fast prototype processor for cloud parameter retrieval from MIPAS (MIPclouds. Retrieval of parameters such as cloud top height, temperature, and extinction are implemented, as well as retrieval of microphysical parameters, e.g. effective radius and the integrated quantities over the limb path (surface area density and volume density. MIPclouds classifies clouds as either liquid or ice cloud in the upper troposphere and polar stratospheric clouds types in the stratosphere based on statistical combinations of colour ratios and brightness temperature differences.

    Comparison of limb measurements of clouds with model results or cloud parameters from nadir looking instruments is often difficult due to different observation geometries. We therefore introduce a new concept, the limb-integrated surface area density path (ADP. By means of validation and radiative transfer calculations of realistic 2-D cloud fields as input for a blind test retrieval (BTR, we demonstrate that ADP is an extremely valuable parameter for future comparison with model data of ice water content, when applying limb integration (ray tracing through the model fields. In addition, ADP is used for a more objective definition of detection thresholds of the applied detection methods. Based on BTR, a detection threshold of ADP = 107 μm2 cm−2 and an ice water content of 10−5 g m−3 is estimated, depending on the horizontal and vertical extent of the cloud.

    Intensive validation of the cloud detection methods shows that the limb-sounding MIPAS instrument has a sensitivity in detecting stratospheric

  6. The Sensitivity of Arctic Ozone Loss to Polar Stratospheric Cloud Volume and Chlorine and Bromine Loading in a Chemistry and Transport Model

    Science.gov (United States)

    Douglass, A. R.; Stolarski, R. S.; Strahan, S. E.; Polansky, B. C.

    2006-01-01

    The sensitivity of Arctic ozone loss to polar stratospheric cloud volume (V(sub PSC)) and chlorine and bromine loading is explored using chemistry and transport models (CTMs). A simulation using multi-decadal output from a general circulation model (GCM) in the Goddard Space Flight Center (GSFC) CTM complements one recycling a single year s GCM output in the Global Modeling Initiative (GMI) CTM. Winter polar ozone loss in the GSFC CTM depends on equivalent effective stratospheric chlorine (EESC) and polar vortex characteristics (temperatures, descent, isolation, polar stratospheric cloud amount). Polar ozone loss in the GMI CTM depends only on changes in EESC as the dynamics repeat annually. The GSFC CTM simulation reproduces a linear relationship between ozone loss and Vpsc derived from observations for 1992 - 2003 which holds for EESC within approx.85% of its maximum (approx.1990 - 2020). The GMI simulation shows that ozone loss varies linearly with EESC for constant, high V(sub PSC).

  7. Ice condensation on sulfuric acid tetrahydrate: Implications for polar stratospheric ice clouds

    Directory of Open Access Journals (Sweden)

    T. J. Fortin

    2003-01-01

    Full Text Available The mechanism of ice nucleation to form Type 2 PSCs is important for controlling the ice particle size and hence the possible dehydration in the polar winter stratosphere. This paper probes heterogeneous ice nucleation on sulfuric acid tetrahydrate (SAT. Laboratory experiments were performed using a thin-film, high-vacuum apparatus in which the condensed phase is monitored via Fourier transform infrared spectroscopy and water pressure is monitored with the combination of an MKS baratron and an ionization gauge. Results show that SAT is an efficient ice nucleus with a critical ice saturation ratio of S*ice = 1.3 to 1.02 over the temperature range 169.8-194.5 K. This corresponds to a necessary supercooling of 0.1-1.3 K below the ice frost point. The laboratory data is used as input for a microphysical/photochemical model to probe the effect that this heterogeneous nucleation mechanism could have on Type 2 PSC formation and stratospheric dehydration. In the model simulations, even a very small number of SAT particles (e.g., 10-3 cm-3 result in ice nucleation on SAT as the dominant mechanism for Type 2 PSC formation. As a result, Type 2 PSC formation is more widespread, leading to larger-scale dehydration. The characteristics of the clouds are controlled by the assumed number of SAT particles present, demonstrating that a proper treatment of SAT is critical for correctly modeling Type 2 PSC formation and stratospheric dehydration.

  8. Relationship between cloud radiative forcing, cloud fraction and cloud albedo, and new surface-based approach for determining cloud albedo

    OpenAIRE

    Y. Liu; W. Wu; M. P. Jensen; T. Toto

    2011-01-01

    This paper focuses on three interconnected topics: (1) quantitative relationship between surface shortwave cloud radiative forcing, cloud fraction, and cloud albedo; (2) surfaced-based approach for measuring cloud albedo; (3) multiscale (diurnal, annual and inter-annual) variations and covariations of surface shortwave cloud radiative forcing, cloud fraction, and cloud albedo. An analytical expression is first derived to quantify the relationship between cloud radiative forcing, cloud fractio...

  9. A case study of formation and maintenance of a lower stratospheric cirrus cloud over the tropics

    Directory of Open Access Journals (Sweden)

    M. Sandhya

    2015-05-01

    Full Text Available A rare occurrence of stratospheric cirrus at 18.6 km height persisting for about 5 days during 3–7 March 2014 is inferred from the ground-based Mie lidar observations over Gadanki (13.5° N, 79.2° E and spaceborne observations. Due to the vertical transport by large updrafts on 3 March in the troposphere, triggered by a potential vorticity intrusion, the water vapour mixing ratio shows an increase around the height of 18.6 km. Relative humidity with respect to ice is ~ 150%, indicating that the cirrus cloud may be formed though homogeneous nucleation of sulfuric acid. The cirrus cloud persists due to the cold anomaly associated with the presence of a 4-day wave.

  10. Titan's Stratospheric Condensibles at High Northern Latitudes During Northern Winter

    Science.gov (United States)

    Anderson, Carrie; Samuelson, R.; Achterberg, R.

    2012-01-01

    The Infrared Interferometer Spectrometer (IRIS) instrument on board Voyager 1 caught the first glimpse of an unidentified particulate feature in Titan's stratosphere that spectrally peaks at 221 per centimeter. Until recently, this feature that we have termed 'the haystack,' has been seen persistently at high northern latitudes with the Composite Infrared Spectrometer (CIRS) instrument onboard Cassini, The strength of the haystack emission feature diminishes rapidly with season, becoming drastically reduced at high northern latitudes, as Titan transitions from northern winter into spring, In contrast to IRIS whose shortest wavenumber was 200 per centimeter, CIRS extends down to 10 per centimeter, thus revealing an entirely unexplored spectral region in which nitrile ices have numerous broad lattice vibration features, Unlike the haystack, which is only found at high northern latitudes during northern winter/early northern spring, this geometrically thin nitrile cloud pervades Titan's lower stratosphere, spectrally peaking at 160 per centimeter, and is almost global in extent spanning latitudes 85 N to 600 S, The inference of nitrile ices are consistent with the highly restricted altitude ranges over which these features are observed, and appear to be dominated by a mixture of HCN and HC3N, The narrow range in altitude over which the nitrile ices extend is unlike the haystack, whose vertical distribution is significantly broader, spanning roughly 70 kilometers in altitude in Titan's lower stratosphere, The nitrile clouds that CIRS observes are located in a dynamically stable region of Titan's atmosphere, whereas CH4 clouds, which ordinarily form in the troposphere, form in a more dynamically unstable region, where convective cloud systems tend to occur. In the unusual situation where Titan's tropopause cools significantly from the HASI 70.5K temperature minimum, CH4 should condense in Titan's lower stratosphere, just like the aforementioned nitrile clouds, although

  11. Simultaneous lidar observations of a polar stratospheric cloud on the east and west sides of the Scandinavian mountains and microphysical box model simulations

    Directory of Open Access Journals (Sweden)

    U. Blum

    2006-12-01

    Full Text Available The importance of polar stratospheric clouds (PSC for polar ozone depletion is well established. Lidar experiments are well suited to observe and classify polar stratospheric clouds. On 5 January 2005 a PSC was observed simultaneously on the east and west sides of the Scandinavian mountains by ground-based lidars. This cloud was composed of liquid particles with a mixture of solid particles in the upper part of the cloud. Multi-colour measurements revealed that the liquid particles had a mode radius of r≈300 nm, a distribution width of σ≈1.04 and an altitude dependent number density of N≈2–20 cm−3. Simulations with a microphysical box model show that the cloud had formed about 20 h before observation. High HNO3 concentrations in the PSC of 40–50 weight percent were simulated in the altitude regions where the liquid particles were observed, while this concentration was reduced to about 10 weight percent in that part of the cloud where a mixture between solid and liquid particles was observed by the lidar. The model simulations also revealed a very narrow particle size distribution with values similar to the lidar observations. Below and above the cloud almost no HNO3 uptake was simulated. Although the PSC shows distinct wave signatures, no gravity wave activity was observed in the temperature profiles measured by the lidars and meteorological analyses support this observation. The observed cloud must have formed in a wave field above Iceland about 20 h prior to the measurements and the cloud wave pattern was advected by the background wind to Scandinavia. In this wave field above Iceland temperatures potentially dropped below the ice formation temperature, so that ice clouds may have formed which can act as condensation nuclei for the nitric acid trihydrate (NAT particles observed at the cloud top above Esrange.

  12. Simulations of physics and chemistry of polar stratospheric clouds with a general circulation model

    Energy Technology Data Exchange (ETDEWEB)

    Buchholz, J.

    2005-04-20

    A polar stratospheric cloud submodel has been developed and incorporated in a general circulation model including atmospheric chemistry (ECHAM5/MESSy). The formation and sedimentation of polar stratospheric cloud (PSC) particles can thus be simulated as well as heterogeneous chemical reactions that take place on the PSC particles. For solid PSC particle sedimentation, the need for a tailor-made algorithm has been elucidated. A sedimentation scheme based on first order approximations of vertical mixing ratio profiles has been developed. It produces relatively little numerical diffusion and can deal well with divergent or convergent sedimentation velocity fields. For the determination of solid PSC particle sizes, an efficient algorithm has been adapted. It assumes a monodisperse radii distribution and thermodynamic equilibrium between the gas phase and the solid particle phase. This scheme, though relatively simple, is shown to produce particle number densities and radii within the observed range. The combined effects of the representations of sedimentation and solid PSC particles on vertical H{sub 2}O and HNO{sub 3} redistribution are investigated in a series of tests. The formation of solid PSC particles, especially of those consisting of nitric acid trihydrate, has been discussed extensively in recent years. Three particle formation schemes in accordance with the most widely used approaches have been identified and implemented. For the evaluation of PSC occurrence a new data set with unprecedented spatial and temporal coverage was available. A quantitative method for the comparison of simulation results and observations is developed and applied. It reveals that the relative PSC sighting frequency can be reproduced well with the PSC submodel whereas the detailed modelling of PSC events is beyond the scope of coarse global scale models. In addition to the development and evaluation of new PSC submodel components, parts of existing simulation programs have been

  13. Reaction of chlorine nitrate with hydrogen chloride and water at Antarctic stratospheric temperatures

    Science.gov (United States)

    Tolbert, Margaret A.; Rossi, Michel J.; Malhotra, Ripudaman; Golden, David M.

    1987-01-01

    Laboratory studies of heterogeneous reactions important for ozone depletion over Antarctica are reported. The reaction of chlorine nitrate (ClONO2) with H2O and HCl on surfacers that simulate polar stratospheric clouds are studied at temperatures relevant to the Antarctic stratosphere. The gaseous products of the resulting reactions, HOCl, Cl2O, and Cl2, could readily photolyze in the Antarctic spring to produce active chlorine for ozone depletion. Furthermore, the additional formation of condensed-phase HNO3 could serve as a sink for odd nitrogen species that would otherwise scavenge the active chlorine.

  14. Effects of stratospheric aerosol surface processes on the LLNL two-dimensional zonally averaged model

    International Nuclear Information System (INIS)

    Connell, P.S.; Kinnison, D.E.; Wuebbles, D.J.; Burley, J.D.; Johnston, H.S.

    1992-01-01

    We have investigated the effects of incorporating representations of heterogeneous chemical processes associated with stratospheric sulfuric acid aerosol into the LLNL two-dimensional, zonally averaged, model of the troposphere and stratosphere. Using distributions of aerosol surface area and volume density derived from SAGE 11 satellite observations, we were primarily interested in changes in partitioning within the Cl- and N- families in the lower stratosphere, compared to a model including only gas phase photochemical reactions

  15. Sudden Stratospheric Warming Compendium

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — Sudden Stratospheric Warming Compendium (SSWC) data set documents the stratospheric, tropospheric, and surface climate impacts of sudden stratospheric warmings. This...

  16. Simultaneous lidar observations of a polar stratospheric cloud on the east and west sides of the Scandinavian mountains and microphysical box model simulations

    Directory of Open Access Journals (Sweden)

    U. Blum

    2006-12-01

    Full Text Available The importance of polar stratospheric clouds (PSC for polar ozone depletion is well established. Lidar experiments are well suited to observe and classify polar stratospheric clouds. On 5 January 2005 a PSC was observed simultaneously on the east and west sides of the Scandinavian mountains by ground-based lidars. This cloud was composed of liquid particles with a mixture of solid particles in the upper part of the cloud. Multi-colour measurements revealed that the liquid particles had a mode radius of r≈300 nm, a distribution width of σ≈1.04 and an altitude dependent number density of N≈2–20 cm−3. Simulations with a microphysical box model show that the cloud had formed about 20 h before observation. High HNO3 concentrations in the PSC of 40–50 weight percent were simulated in the altitude regions where the liquid particles were observed, while this concentration was reduced to about 10 weight percent in that part of the cloud where a mixture between solid and liquid particles was observed by the lidar. The model simulations also revealed a very narrow particle size distribution with values similar to the lidar observations. Below and above the cloud almost no HNO3 uptake was simulated. Although the PSC shows distinct wave signatures, no gravity wave activity was observed in the temperature profiles measured by the lidars and meteorological analyses support this observation. The observed cloud must have formed in a wave field above Iceland about 20 h prior to the measurements and the cloud wave pattern was advected by the background wind to Scandinavia. In this wave field above Iceland temperatures potentially dropped below the ice formation temperature, so that ice clouds may have formed which can act as condensation nuclei for the nitric acid trihydrate (NAT particles observed at the cloud top above Esrange.

  17. Springtime high surface ozone events over the western United States: Quantifying the role of stratospheric intrusions

    Science.gov (United States)

    Fiore, A. M.; Lin, M.; Cooper, O. R.; Horowitz, L. W.; Naik, V.; Levy, H.; Langford, A. O.; Johnson, B. J.; Oltmans, S. J.; Senff, C. J.

    2011-12-01

    As the National Ambient Air Quality (NAAQS) standard for ozone (O_{3}) is lowered, it pushes closer to policy-relevant background levels (O_{3} concentrations that would exist in the absence of North American anthropogenic emissions), making attainment more difficult with local controls. We quantify the Asian and stratospheric components of this North American background, with a primary focus on the western United States. Prior work has identified this region as a hotspot for deep stratospheric intrusions in spring. We conduct global simulations at 200 km and 50 km horizontal resolution with the GFDL AM3 model, including a stratospheric O_{3} tracer and two sensitivity simulations with anthropogenic emissions from Asia and North America turned off. The model is evaluated with a suite of in situ and satellite measurements during the NOAA CalNex campaign (May-June 2010). The model reproduces the principle features in the observed surface to near tropopause distribution of O_{3} along the California coast, including its latitudinal variation and the development of regional high-O_{3} episodes. Four deep tropopause folds are diagnosed and we find that the remnants of these stratospheric intrusions are transported to the surface of Southern California and Western U.S. Rocky Mountains, contributing 10-30 ppbv positive anomalies relative to the simulated campaign mean stratospheric component in the model surface layer. We further examine the contribution of North American background, including its stratospheric and Asian components, to the entire distribution of observed MDA8 O_{3} at 12 high-elevation CASTNet sites in the Mountain West. We find that the stratospheric O_{3} tracer constitutes 50% of the North American background, and can enhance surface maximum daily 8-hour average (MDA8) O_{3} by 20 ppb when observed surface O_{3} is in the range of 60-80 ppbv. Our analysis highlights the potential for natural sources such as deep stratospheric intrusions to contribute

  18. Laboratory chemistry and stratospheric clouds

    Science.gov (United States)

    Molina, Mario J.

    1989-01-01

    Results are presented from laboratory experiments on the chemistry of ice particles to study the role of HCl and ClONO2 from CFCs in stratospheric ozone depletion over Antarctica. It is found that gaseous HCl is scavenged with high efficiency by the ice and the gas phase chlorine nitrate may react with the HCL-containing ice to produce Cl2. Also, consideration is given ot the behavior of solid nitric acid trihydrate and sulfuric acid aerosols.

  19. A condensed-mass advection based model for the simulation of liquid polar stratospheric clouds

    Directory of Open Access Journals (Sweden)

    D. Lowe

    2003-01-01

    Full Text Available We present a condensed-mass advection based model (MADVEC designed to simulate the condensation/evaporation of liquid polar stratospheric cloud (PSC particles. A (Eulerian-in-radius discretization scheme is used, making the model suitable for use in global or mesoscale chemistry and transport models (CTMs. The mass advection equations are solved using an adaption of the weighted average flux (WAF scheme. We validate the numerical scheme using an analytical solution for multicomponent aerosols. The physics of the model are tested using a test case designed by Meilinger et al. (1995. The results from this test corroborate the composition gradients across the size distribution under rapid cooling conditions that were reported in earlier studies.

  20. Polar stratospheric cloud evolution and chlorine activation measured by CALIPSO and MLS, and modeled by ATLAS

    Directory of Open Access Journals (Sweden)

    H. Nakajima

    2016-03-01

    Full Text Available We examined observations of polar stratospheric clouds (PSCs by CALIPSO, and of HCl and ClO by MLS along air mass trajectories, to investigate the dependence of the inferred PSC composition on the temperature history of the air parcels and the dependence of the level of chlorine activation on PSC composition. Several case studies based on individual trajectories from the Arctic winter 2009/2010 were conducted, with the trajectories chosen such that the first processing of the air mass by PSCs in this winter occurred on the trajectory. Transitions of PSC composition classes were observed to be highly dependent on the temperature history. In cases of a gradual temperature decrease, nitric acid trihydrate (NAT and super-cooled ternary solution (STS mixture clouds were observed. In cases of rapid temperature decrease, STS clouds were first observed, followed by NAT/STS mixture clouds. When temperatures dropped below the frost point, ice clouds formed and then transformed into NAT/STS mixture clouds when temperature increased above the frost point. The threshold temperature for rapid chlorine activation on PSCs is approximately 4 K below the NAT existence temperature, TNAT. Furthermore, simulations of the ATLAS chemistry and transport box model along the trajectories were used to corroborate the measurements and show good agreement with the observations. Rapid chlorine activation was observed when an air mass encountered PSCs. Usually, chlorine activation was limited by the amount of available ClONO2. Where ClONO2 was not the limiting factor, a large dependence on temperature was evident.

  1. Stratospheric changes caused by geoengineering applications: potential repercussions and uncertainties

    Science.gov (United States)

    Kenzelmann, P.; Weisenstein, D.; Peter, T.; Luo, B. P.; Rozanov, E.; Fueglistaler, S.; Thomason, L. W.

    2009-04-01

    Anthropogenic greenhouse gas emissions tend to warm the global climate, calling for significant rapid emission reductions. As potential support measures various ideas for geoengineering are currently being discussed. The assessment of the possible manifold and as yet substantially unexplored repercussions of implementing geoengineering ideas to ameliorate climate change poses enormous challenges not least in the realm of aerosol-cloud-climate interactions. Sulphur aerosols cool the Earth's surface by reflecting short wave radiation. By increasing the amount of sulphur aerosols in the stratosphere, for example by sulphur dioxide injections, part of the anthropogenic climate warming might be compensated due to enhanced albedo. However, we are only at the beginning of understanding possible side effects. One such effect that such aerosol might have is the warming of the tropical tropopause and consequently the increase of the amount of stratospheric water vapour. Using the 2D AER Aerosol Model we calculated the aerosol distributions for yearly injections of 1, 2, 5 and 10 Mt sulphur into the lower tropical stratosphere. The results serve as input for the 3D chemistry-climate model SOCOL, which allows calculating the aerosol effect on stratospheric temperatures and chemistry. In the injection region the continuously formed sulphuric acid condensates rapidly on sulphate aerosol, which eventually grow to such extent that they sediment down to the tropical tropopause region. The growth of the aerosol particles depends on non-linear processes: the more sulphur is emitted the faster the particles grow. As a consequence for the scenario with continuous sulphur injection of totally 10 Mt per year, only 6 Mt sulphur are in the stratosphere if equilibrium is reached. According to our model calculations this amount of sulphate aerosols leads to a net surface forcing of -3.4 W/m2, which is less then expected radiative forcing by doubling of carbon dioxide concentration. Hence

  2. Negative chlorine ion chemistry in the upper stratosphere and its application to an artificially created dense electron cloud

    Directory of Open Access Journals (Sweden)

    S. S. Prasad

    1995-03-01

    Full Text Available This paper discusses new potential reactions of chlorine-bearing anions (negative ions in the upper stratosphere. These reactions are then applied to the negative-ion chemistry following the injection of an electron cloud of very high density, of the order of 106-107 e- cm-3, in the 40-45-km region. The idea is to evaluate the recently proposed scheme to mitigate ozone depletion by converting the reactive chlorine atoms at these altitudes into Cl- ions which are unreactive towards ozone, i.e., electron scavenging of Cl. We find that the previously neglected photodetachment from Cl- is fast. For an overhead sun, this process may have a rate coefficient of 0.08 s-1 when multiple scattering is included. The rate could be even higher, depending on the ground albedo. Switching reaction between Cl-·H2O and HCl might lead to the formation of Cl-·HCl anion. Possible reactions of Cl-·H2O and Cl-·HCl with O atoms could produce ClO- and Cl-2. The production of ClO- in this manner is significant because Cl- having a high photodetachment rate constant would be regenerated in the very likely reactions of ClO- with O. When these possibilities are considered, then it is found that the chlorine anions may not be the major ions inside the electron cloud due to the rapid photodetachment from Cl-. Furthermore, in such a cloud, there may be the hazard that the Cl--Cl-·H2O-ClO--Cl- cycle amounts to catalytic destruction of two O atoms. Thus, the scheme could be risky if practised in the altitude region where atomic oxygen is an important constituent. Similar conclusions apply even if the ClO- species forms ClO-3 by three-body association with O2, instead of reacting with O. It must be emphasized that the present study is speculative at this time, because none of the relevant reactions have been investigated in the laboratory as yet. Nevertheless, it is very safe to say that the scheme of ozone preservation by electron scavenging of the upper stratospheric Cl is

  3. Effect of Recent Sea Surface Temperature Trends on the Arctic Stratospheric Vortex

    Science.gov (United States)

    Garfinkel, Chaim I.; Oman, Luke; Hurwitz, Margaret

    2015-01-01

    The springtime Arctic polar vortex has cooled significantly over the satellite era, with consequences for ozone concentrations in the springtime transition season. The causes of this cooling trend are deduced by using comprehensive chemistry-climate model experiments. Approximately half of the satellite era early springtime cooling trend in the Arctic lower stratosphere was caused by changing sea surface temperatures (SSTs). An ensemble of experiments forced only by changing SSTs is compared to an ensemble of experiments in which both the observed SSTs and chemically- and radiatively-active trace species are changing. By comparing the two ensembles, it is shown that warming of Indian Ocean, North Pacific, and North Atlantic SSTs, and cooling of the tropical Pacific, have strongly contributed to recent polar stratospheric cooling in late winter and early spring, and to a weak polar stratospheric warming in early winter. When concentrations of ozone-depleting substances and greenhouse gases are fixed, polar ozone concentrations show a small but robust decline due to changing SSTs. Ozone changes are magnified in the presence of changing gas concentrations. The stratospheric changes can be understood by examining the tropospheric height and heat flux anomalies generated by the anomalous SSTs. Finally, recent SST changes have contributed to a decrease in the frequency of late winter stratospheric sudden warmings.

  4. A Unified Satellite-Observation Polar Stratospheric Cloud (PSC) Database for Long-Term Climate-Change Studies

    Science.gov (United States)

    Fromm, Michael; Pitts, Michael; Alfred, Jerome

    2000-01-01

    This report summarizes the project team's activity and accomplishments during the period 12 February, 1999 - 12 February, 2000. The primary objective of this project was to create and test a generic algorithm for detecting polar stratospheric clouds (PSC), an algorithm that would permit creation of a unified, long term PSC database from a variety of solar occultation instruments that measure aerosol extinction near 1000 nm The second objective was to make a database of PSC observations and certain relevant related datasets. In this report we describe the algorithm, the data we are making available, and user access options. The remainder of this document provides the details of the algorithm and the database offering.

  5. Polar stratospheric cloud observations by MIPAS on ENVISAT: detection method, validation and analysis of the northern hemisphere winter 2002/2003

    Directory of Open Access Journals (Sweden)

    R. Spang

    2005-01-01

    Full Text Available The Michelson Interferometer for Passive Atmospheric Sounding (MIPAS on ENVISAT has made extensive measurements of polar stratospheric clouds (PSCs in the northern hemisphere winter 2002/2003. A PSC detection method based on a ratio of radiances (the cloud index has been implemented for MIPAS and is validated in this study with respect to ground-based lidar and space borne occultation measurements. A very good correspondence in PSC sighting and cloud altitude between MIPAS detections and those of other instruments is found for cloud index values of less than four. Comparisons with data from the Stratospheric Aerosol and Gas Experiment (SAGE III are used to further show that the sensitivity of the MIPAS detection method for this threshold value of cloud index is approximately equivalent to an extinction limit of 10-3km-1 at 1022nm, a wavelength used by solar occultation experiments. The MIPAS cloud index data are subsequently used to examine, for the first time with any technique, the evolution of PSCs throughout the Arctic polar vortex up to a latitude close to 90° north on a near-daily basis. We find that the winter of 2002/2003 is characterised by three phases of very different PSC activity. First, an unusual, extremely cold phase in the first three weeks of December resulted in high PSC occurrence rates. This was followed by a second phase of only moderate PSC activity from 5-13 January, separated from the first phase by a minor warming event. Finally there was a third phase from February to the end of March where only sporadic and mostly weak PSC events took place. The composition of PSCs during the winter period has also been examined, exploiting in particular an infra-red spectral signature which is probably characteristic of NAT. The MIPAS observations show the presence of these particles on a number of occasions in December but very rarely in January. The PSC type differentiation from MIPAS indicates that future comparisons of PSC

  6. What Controls the Arctic Lower Stratosphere Temperature?

    Science.gov (United States)

    Newman, Paul A.; Nash, Eric R.; Einaudi, Franco (Technical Monitor)

    2001-01-01

    The temperature of the Arctic lower stratosphere is critical for understanding polar ozone levels. As temperatures drop below about 195 K, polar stratospheric clouds form, which then convert HCl and ClONO2 into reactive forms that are catalysts for ozone loss reactions. Hence, the lower stratospheric temperature during the March period is a key parameter for understanding polar ozone losses. The temperature is basically understood to be a result of planetary waves which drive the polar temperature away from a cold "radiative equilibrium" state. This is demonstrated using NCEP/NCAR reanalysis calculations of the heat flux and the mean polar temperature. The temperature during the March period is fundamentally driven by the integrated impact of large scale waves moving from the troposphere to the stratosphere during the January through February period. We will further show that the recent cold years in the northern polar vortex are a result of this weakened wave driving of the stratosphere.

  7. New stratospheric UV/visible radiance measurements

    Directory of Open Access Journals (Sweden)

    F. J. Marceau

    1994-01-01

    Full Text Available A stratospheric balloon was launched on 12 October 1986 from the "CNES" base at Aire sur l'Adour (France to record twilight radiance in the stratosphere. The near-UV and visible radiances were continuously monitored by a photometer during sunrise. Some observations are presented for different viewing azimuthal planes and viewing elevation angles. They show the influence of aerosols layers and clouds which can be also seen on related photographs. The results as a whole may be used for testing some radiative models, especially for twilight conditions.

  8. Negative chlorine ion chemistry in the upper stratosphere and its application to an artificially created dense electron cloud

    Directory of Open Access Journals (Sweden)

    S. S. Prasad

    Full Text Available This paper discusses new potential reactions of chlorine-bearing anions (negative ions in the upper stratosphere. These reactions are then applied to the negative-ion chemistry following the injection of an electron cloud of very high density, of the order of 106-107 e- cm-3, in the 40-45-km region. The idea is to evaluate the recently proposed scheme to mitigate ozone depletion by converting the reactive chlorine atoms at these altitudes into Cl- ions which are unreactive towards ozone, i.e., electron scavenging of Cl. We find that the previously neglected photodetachment from Cl- is fast. For an overhead sun, this process may have a rate coefficient of 0.08 s-1 when multiple scattering is included. The rate could be even higher, depending on the ground albedo. Switching reaction between Cl-·H2O and HCl might lead to the formation of Cl-·HCl anion. Possible reactions of Cl-·H2O and Cl-·HCl with O atoms could produce ClO- and Cl-2. The production of ClO- in this manner is significant because Cl- having a high photodetachment rate constant would be regenerated in the very likely reactions of ClO- with O. When these possibilities are considered, then it is found that the chlorine anions may not be the major ions inside the electron cloud due to the rapid photodetachment from Cl-. Furthermore, in such a cloud, there may be the hazard that the Cl--Cl-·H2O-ClO--Cl- cycle amounts to catalytic destruction of two O atoms. Thus, the scheme could be risky if practised in the altitude region where atomic oxygen is an important constituent. Similar conclusions apply even if the ClO- species forms ClO-3 by three-body association with O2

  9. Comparison of cloud optical depth and cloud mask applying BRDF model-based background surface reflectance

    Science.gov (United States)

    Kim, H. W.; Yeom, J. M.; Woo, S. H.

    2017-12-01

    Over the thin cloud region, satellite can simultaneously detect the reflectance from thin clouds and land surface. Since the mixed reflectance is not the exact cloud information, the background surface reflectance should be eliminated to accurately distinguish thin cloud such as cirrus. In the previous research, Kim et al (2017) was developed the cloud masking algorithm using the Geostationary Ocean Color Imager (GOCI), which is one of significant instruments for Communication, Ocean, and Meteorology Satellite (COMS). Although GOCI has 8 spectral channels including visible and near infra-red spectral ranges, the cloud masking has quantitatively reasonable result when comparing with MODIS cloud mask (Collection 6 MYD35). Especially, we noticed that this cloud masking algorithm is more specialized in thin cloud detections through the validation with Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) data. Because this cloud masking method was concentrated on eliminating background surface effects from the top-of-atmosphere (TOA) reflectance. Applying the difference between TOA reflectance and the bi-directional reflectance distribution function (BRDF) model-based background surface reflectance, cloud areas both thick cloud and thin cloud can be discriminated without infra-red channels which were mostly used for detecting clouds. Moreover, when the cloud mask result was utilized as the input data when simulating BRDF model and the optimized BRDF model-based surface reflectance was used for the optimized cloud masking, the probability of detection (POD) has higher value than POD of the original cloud mask. In this study, we examine the correlation between cloud optical depth (COD) and its cloud mask result. Cloud optical depths mostly depend on the cloud thickness, the characteristic of contents, and the size of cloud contents. COD ranges from less than 0.1 for thin clouds to over 1000 for the huge cumulus due to scattering by droplets. With

  10. Radionuclide composition in the surface layer of particles in the troposphere and stratosphere falls

    International Nuclear Information System (INIS)

    Prokof'ev, O.N.

    1977-01-01

    Radionuclide content in troposphere and stratosphere fall-outs as well as radionuclide washing-off from fall-out particle; are important to determine internal irradiation doses received by separate critical organs of human body. In surface-contaminated products (floury products of grain contaminated while in ears, vegetables, fruits, berries, noncovered or insufficiently covered products during fall-outs) radionuclides initially (in an initial state) are connected with fall-out particles. Radionuclides in biologically contaminated products (milk, meat etc.) are not connected with the particles and have the assimilable form. However, the degree of radionuclide transition from forage (grasses, hay etc.) surface-contaminated as a results of fall-outs into animal produce (milk, meat etc.) also depends on radionuclide washing-off from fall-out particles, which in the latter results from the formation nature and a kind of particles of the main substance. Radionuclide washing-off degree (and, consequently, biological availability) by glazed silicate particles is caused by radionuclide distribution between particle volume and surface in an appropriate sample. According to Israel Yu.A. method calculated were the shares of surface-bound atoms for all the particle totality in an explosion cloud for mass chains, which composition includes biologically important radionuclides. Particle solidification time is taken to equal 7 and 40s. Independent yields of chain radionuclides and its total yield are taken for 228 U fission under 14 MeV neutron effect. The calculation results are presented in the tables

  11. Stratospheric Aerosol Measurements

    Science.gov (United States)

    Pueschel, Rudolf, F.; Gore, Warren J. (Technical Monitor)

    1998-01-01

    Stratospheric aerosols affect the atmospheric energy balance by scattering and absorbing solar and terrestrial radiation. They also can alter stratospheric chemical cycles by catalyzing heterogeneous reactions which markedly perturb odd nitrogen, chlorine and ozone levels. Aerosol measurements by satellites began in NASA in 1975 with the Stratospheric Aerosol Measurement (SAM) program, to be followed by the Stratospheric Aerosol and Gas Experiment (SAGE) starting in 1979. Both programs employ the solar occultation, or Earth limb extinction, techniques. Major results of these activities include the discovery of polar stratospheric clouds (PSCs) in both hemispheres in winter, illustrations of the impacts of major (El Chichon 1982 and Pinatubo 1991) eruptions, and detection of a negative global trend in lower stratospheric/upper tropospheric aerosol extinction. This latter result can be considered a triumph of successful worldwide sulfur emission controls. The SAGE record will be continued and improved by SAGE III, currently scheduled for multiple launches beginning in 2000 as part of the Earth Observing System (EOS). The satellite program has been supplemented by in situ measurements aboard the ER-2 (20 km ceiling) since 1974, and from the DC-8 (13 km ceiling) aircraft beginning in 1989. Collection by wire impactors and subsequent electron microscopic and X-ray energy-dispersive analyses, and optical particle spectrometry have been the principle techniques. Major findings are: (1) The stratospheric background aerosol consists of dilute sulfuric acid droplets of around 0.1 micrometer modal diameter at concentration of tens to hundreds of monograms per cubic meter; (2) Soot from aircraft amounts to a fraction of one percent of the background total aerosol; (3) Volcanic eruptions perturb the sulfuric acid, but not the soot, aerosol abundance by several orders of magnitude; (4) PSCs contain nitric acid at temperatures below 195K, supporting chemical hypotheses

  12. Impact of chemical lateral boundary conditions in a regional air quality forecast model on surface ozone predictions during stratospheric intrusions

    Science.gov (United States)

    Pendlebury, Diane; Gravel, Sylvie; Moran, Michael D.; Lupu, Alexandru

    2018-02-01

    A regional air quality forecast model, GEM-MACH, is used to examine the conditions under which a limited-area air quality model can accurately forecast near-surface ozone concentrations during stratospheric intrusions. Periods in 2010 and 2014 with known stratospheric intrusions over North America were modelled using four different ozone lateral boundary conditions obtained from a seasonal climatology, a dynamically-interpolated monthly climatology, global air quality forecasts, and global air quality reanalyses. It is shown that the mean bias and correlation in surface ozone over the course of a season can be improved by using time-varying ozone lateral boundary conditions, particularly through the correct assignment of stratospheric vs. tropospheric ozone along the western lateral boundary (for North America). Part of the improvement in surface ozone forecasts results from improvements in the characterization of near-surface ozone along the lateral boundaries that then directly impact surface locations near the boundaries. However, there is an additional benefit from the correct characterization of the location of the tropopause along the western lateral boundary such that the model can correctly simulate stratospheric intrusions and their associated exchange of ozone from stratosphere to troposphere. Over a three-month period in spring 2010, the mean bias was seen to improve by as much as 5 ppbv and the correlation by 0.1 depending on location, and on the form of the chemical lateral boundary condition.

  13. Dispersion of the Volcanic Sulfate Cloud from the Mount Pinatubo Eruption

    Science.gov (United States)

    Aquila, Valentina; Oman, Luke D.; Stolarski, Richard S.; Colarco, Peter R.; Newman, Paul A.

    2012-01-01

    We simulate the transport of the volcanic cloud from the 1991 eruption of Mount Pinatubo with the GEOS-5 general circulation model. Our simulations are in good agreement with observational data. We tested the importance of initial condition corresponding to the specific meteorological situation at the time of the eruption by employing reanalysis from MERRA. We found no significant difference in the transport of the cloud. We show how the inclusion of the interaction between volcanic sulfate aerosol and radiation is essential for a reliable simulation of the transport of the volcanic cloud. The absorption of long wave radiation by the volcanic sulfate induces a rising of the volcanic cloud up to the middle stratosphere, combined with divergent motion from the latitude of the eruption to the tropics. Our simulations indicate that the cloud diffuses to the northern hemisphere through a lower stratospheric pathway, and to mid- and high latitudes of the southern hemisphere through a middle stratospheric pathway, centered at about 30 hPa. The direction of the middle stratospheric pathway depends on the season. We did not detect any significant change of the mixing between tropics and mid- and high latitudes in the southern hemisphere.

  14. Effect of remote clouds on surface UV irradiance

    Energy Technology Data Exchange (ETDEWEB)

    Deguenther, M.; Meerkoetter, R. [Deutsche Forschungsanstalt fuer Luft- und Raumfahrt e.V. (DLR), Wessling (Germany). Inst. fuer Physik der Atmosphaere

    2000-06-01

    Clouds affect local surface UV irradiance, even if the horizontal distance from the radiation observation site amounts to several kilometers. In order to investigate this effect, which we call remote clouds effect, a 3-dimensional radiative transfer model is applied. Assuming the atmosphere is subdivided into a quadratic based sector and its surrounding, we quantify the influence of changing cloud coverage within this surrounding from 0% to 100% on surface UV irradiance at the sector center. To work out this remote clouds influence as a function of sector base size, we made some calculations for different sizes between 10 km x 10 km and 100 km x 100 km. It appears that in the case of small sectors (base size {<=}20 km x 20 km) the remote clouds effect is highly variable: Depending on cloud structure, solar zenith angle and wavelength, the surface UV irradiance may be enhanced up to 15% as well as reduced by more than 50%. In contrast, for larger sectors it is always the case that enhancements become smaller by 5% if sector base size exceeds 60 km x 60 km. However, these values are upper estimates of the remote cloud effects and they are found only for special cloud structures. Since these structures might occur but cannot be regarded as typical, different satellite observed cloud formations (horizontal resolution about 1 km x 1 km) have also been investigated. For these more common cloud distributions we find remote cloud effects to be distinctly smaller than the corresponding upper estimates, e.g., for a sector with base size of 25 km x 25 km the surface UV irradiance error due to ignoring the actual remote clouds and replacing their influence with periodic horizontal boundary conditions is less than 3%, whereas the upper estimate of remote clouds effect would suggest an error close to 10%. (orig.)

  15. On the Climate Impacts of Upper Tropospheric and Lower Stratospheric Ozone

    Science.gov (United States)

    Xia, Yan; Huang, Yi; Hu, Yongyun

    2018-01-01

    The global warming simulations of the general circulation models (GCMs) are generally performed with different ozone prescriptions. We find that the differences in ozone distribution, especially in the upper tropospheric and lower stratospheric (UTLS) region, account for important model discrepancies shown in the ozone-only historical experiment of the Coupled Model Intercomparison Project Phase 5 (CMIP5). These discrepancies include global high cloud fraction, stratospheric temperature, and stratospheric water vapor. Through a set of experiments conducted by an atmospheric GCM with contrasting UTLS ozone prescriptions, we verify that UTLS ozone not only directly radiatively heats the UTLS region and cools the upper parts of the stratosphere but also strongly influences the high clouds due to its impact on relative humidity and static stability in the UTLS region and the stratospheric water vapor due to its impact on the tropical tropopause temperature. These consequences strongly affect the global mean effective radiative forcing of ozone, as noted in previous studies. Our findings suggest that special attention should be paid to the UTLS ozone when evaluating the climate effects of ozone depletion in the 20th century and recovery in the 21st century. UTLS ozone difference may also be important for understanding the intermodel discrepancy in the climate projections of the CMIP6 GCMs in which either prescribed or interactive ozone is used.

  16. International Workshop on Stratospheric Aerosols: Measurements, Properties, and Effects

    Science.gov (United States)

    Pueschel, Rudolf F. (Editor)

    1991-01-01

    Following a mandate by the International Aerosol Climatology Program under the auspices of International Association of Meteorology and Atmospheric Physics International Radiation Commission, 45 scientists from five nations convened to discuss relevant issues associated with the measurement, properties, and effects of stratospheric aerosols. A summary is presented of the discussions on formation and evolution, transport and fate, effects on climate, role in heterogeneous chemistry, and validation of lidar and satellite remote sensing of stratospheric aerosols. Measurements are recommended of the natural (background) and the volcanically enhanced aerosol (sulfuric acid and silica particles), the exhaust of shuttle, civil aviation and supersonic aircraft operations (alumina, soot, and ice particles), and polar stratospheric clouds (ice, condensed nitric and hydrochloric acids).

  17. Titan's Tropopause Temperatures from CIRS: Implications for Stratospheric Methane Cloud Formation

    Science.gov (United States)

    Anderson, C. M.; Samuelson, R. E.; Achterberg, R. K.; Barnes, J. W.; Flasar, F. M.

    2012-01-01

    Analysis of Cassini Composite Infrared Spectrometer (CIRS) far-IR spectra enable the construction of Titan's temperature profile in the altitude region containing the tropopause. Whereas the methane V4 band at 1306/cm (7.7 microns) is the primary opacity source for deducing thermal structure between 100 km and 500 km, N2-N2 collision-induced absorption between 70 and 140/cm (143 microns and 71 microns) is utilized to determine temperatures at Titan's tropopause. Additional opacity due to aerosol and nitrile ices must also be taken into account in this part of the far-IR spectral region. The spectral characteristics of these particulate opacities have been deduced from CIRS limb data at 58degS, 15degS, 15degN, and 85degN. Empirically, the spectral shapes of these opacities appear to be independent of both latitude and altitude below 300 km (Anderson and Samuelson, 2011, Icarus 212, 762-778), justifying the extension of these spectral properties to all latitudes. We find that Titan's tropopause temperature is cooler than the HAS! value of 70.5K by approx. 6K. This leads to the possibility that subsidence at high northern latitudes can cause methane condensation in the winter polar stratosphere. A search for methane clouds in this region is in progress.

  18. Surface reconstruction and deformation monitoring of stratospheric airship based on laser scanning technology

    Science.gov (United States)

    Guo, Kai; Xie, Yongjie; Ye, Hu; Zhang, Song; Li, Yunfei

    2018-04-01

    Due to the uncertainty of stratospheric airship's shape and the security problem caused by the uncertainty, surface reconstruction and surface deformation monitoring of airship was conducted based on laser scanning technology and a √3-subdivision scheme based on Shepard interpolation was developed. Then, comparison was conducted between our subdivision scheme and the original √3-subdivision scheme. The result shows our subdivision scheme could reduce the shrinkage of surface and the number of narrow triangles. In addition, our subdivision scheme could keep the sharp features. So, surface reconstruction and surface deformation monitoring of airship could be conducted precisely by our subdivision scheme.

  19. On particles in the Arctic stratosphere

    Directory of Open Access Journals (Sweden)

    T. S. Jørgensen

    2003-06-01

    Full Text Available Soon after the discovery of the Antarctic ozone hole it became clear that particles in the polar stratosphere had an infl uence on the destruction of the ozone layer. Two major types of particles, sulphate aerosols and Polar Stratospheric Clouds (PSCs, provide the surfaces where fast heterogeneous chemical reactions convert inactive halogen reservoir species into potentially ozone-destroying radicals. Lidar measurements have been used to classify the PSCs. Following the Mt. Pinatubo eruption in June 1991 it was found that the Arctic stratosphere was loaded with aerosols, and that aerosols observed with lidar and ozone observed with ozone sondes displayed a layered structure, and that the aerosol and ozone contents in the layers frequently appeared to be negatively correlated. The layered structure was probably due to modulation induced by the dynamics at the edge of the polar vortex. Lidar observations of the Mt. Pinatubo aerosols were in several cases accompanied by balloon-borne backscatter soundings, whereby backscatter measurements in three different wavelengths made it possible to obtain information about the particle sizes. An investigation of the infl uence of synoptic temperature histories on the physical properties of PSC particles has shown that most of the liquid type 1b particles were observed in the process of an ongoing, relatively fast, and continuous cooling from temperatures clearly above the nitric acid trihydrate condensation temperature (TNAT. On the other hand, it appeared that a relatively long period, with a duration of at least 1-2 days, at temperatures below TNAT provide the conditions which may lead to the production of solid type 1a PSCs.

  20. Reducing Surface Clutter in Cloud Profiling Radar Data

    Science.gov (United States)

    Tanelli, Simone; Pak, Kyung; Durden, Stephen; Im, Eastwood

    2008-01-01

    An algorithm has been devised to reduce ground clutter in the data products of the CloudSat Cloud Profiling Radar (CPR), which is a nadir-looking radar instrument, in orbit around the Earth, that measures power backscattered by clouds as a function of distance from the instrument. Ground clutter contaminates the CPR data in the lowest 1 km of the atmospheric profile, heretofore making it impossible to use CPR data to satisfy the scientific interest in studying clouds and light rainfall at low altitude. The algorithm is based partly on the fact that the CloudSat orbit is such that the geodetic altitude of the CPR varies continuously over a range of approximately 25 km. As the geodetic altitude changes, the radar timing parameters are changed at intervals defined by flight software in order to keep the troposphere inside a data-collection time window. However, within each interval, the surface of the Earth continuously "scans through" (that is, it moves across) a few range bins of the data time window. For each radar profile, only few samples [one for every range-bin increment ((Delta)r = 240 m)] of the surface-clutter signature are available around the range bin in which the peak of surface return is observed, but samples in consecutive radar profiles are offset slightly (by amounts much less than (Delta)r) with respect to each other according to the relative change in geodetic altitude. As a consequence, in a case in which the surface area under examination is homogenous (e.g., an ocean surface), a sequence of consecutive radar profiles of the surface in that area contains samples of the surface response with range resolution (Delta)p much finer than the range-bin increment ((Delta)p 10 dB and a reduction of the contaminated altitude over ocean from about 1 km to about 0.5 km (over the ocean). The algorithm has been embedded in CloudSat L1B processing as of Release 04 (July 2007), and the estimated flat surface clutter is removed in L2B-GEOPROF product from the

  1. Stratospheric dryness: model simulations and satellite observations

    Directory of Open Access Journals (Sweden)

    J. Lelieveld

    2007-01-01

    Full Text Available The mechanisms responsible for the extreme dryness of the stratosphere have been debated for decades. A key difficulty has been the lack of comprehensive models which are able to reproduce the observations. Here we examine results from the coupled lower-middle atmosphere chemistry general circulation model ECHAM5/MESSy1 together with satellite observations. Our model results match observed temperatures in the tropical lower stratosphere and realistically represent the seasonal and inter-annual variability of water vapor. The model reproduces the very low water vapor mixing ratios (below 2 ppmv periodically observed at the tropical tropopause near 100 hPa, as well as the characteristic tape recorder signal up to about 10 hPa, providing evidence that the dehydration mechanism is well-captured. Our results confirm that the entry of tropospheric air into the tropical stratosphere is forced by large-scale wave dynamics, whereas radiative cooling regionally decelerates upwelling and can even cause downwelling. Thin cirrus forms in the cold air above cumulonimbus clouds, and the associated sedimentation of ice particles between 100 and 200 hPa reduces water mass fluxes by nearly two orders of magnitude compared to air mass fluxes. Transport into the stratosphere is supported by regional net radiative heating, to a large extent in the outer tropics. During summer very deep monsoon convection over Southeast Asia, centered over Tibet, moistens the stratosphere.

  2. Long Term Stratospheric Aerosol Lidar Measurements in Kyushu

    Science.gov (United States)

    Fujiwara, Motowo

    1992-01-01

    Lidar soundings of the stratospheric aerosols have been made since 1972 at Fukuoka, Kyushu Island of Japan. Volcanic clouds from eruptions of La Soufriere, Sierra Negra, St. Helens, Uluwan, Alaid, unknown volcano, and El Chichon were detected one after another in only three years from 1979 to 1982. In july 1991 strong scattering layers which were originated from the serious eruptions of Pinatubo in June and were almost comparable to the El Chichon clouds were detected. Volcanic clouds from pinatubo and other volcanos mentioned are examined and carefully compared to each other and to the wind and temperature which was measured by Fukuoka Meteorological Observatory almost at the same time as the lidar observation was made.

  3. Letter to the Editor: A strange cloud in the Arctic summer stratosphere 1998 above Esrange (68°N, Sweden

    Directory of Open Access Journals (Sweden)

    J. Siebert

    2000-04-01

    Full Text Available When the University of Bonn lidar on the Esrange (68°N, 21°E, Sweden, was switched on in the evening of July 18, 1998, a geometrically and optically thin cloud layer was present near 14 km altitude or 400 K potential temperature, where it persisted for two hours. The tropopause altitude was 4 km below the cloud altitude. The cloud particles depolarized the lidar returns, thus must they have been aspherical and hence solid. Atmospheric temperatures near 230 K were approximately 40 K too high to support ice particles at stratospheric water vapour pressures of a few ppmv. The isentropic back trajectory on 400 K showed the air parcels to have stayed clear of active major rocket launch sites. The air parcels at 400 K had traveled from the Aleutians across Canada and the Atlantic Ocean arriving above central Europe and then turned northward to pass over above the lidar station. Parcels at levels at ±25 K from 400 K had come from the pole and joined the 400 K trajectory path above eastern Canada. Apparently the cloud existed in a filament of air with an origin different from those filaments both above and below. Possibly the 400 K level air parcels had carried soot particles from forest wild fires in northern Canada or volcanic ash from the eruption of the Korovin Volcano in the Aleutian Islands.Key words: Atmospheric composition and structure (aerosols and particles; biosphere-atmosphere interactions · Meteorology and atmospheric dynamics (middle atmospheric dynamics

  4. Letter to the Editor: A strange cloud in the Arctic summer stratosphere 1998 above Esrange (68°N, Sweden

    Directory of Open Access Journals (Sweden)

    K. H. Fricke

    Full Text Available When the University of Bonn lidar on the Esrange (68°N, 21°E, Sweden, was switched on in the evening of July 18, 1998, a geometrically and optically thin cloud layer was present near 14 km altitude or 400 K potential temperature, where it persisted for two hours. The tropopause altitude was 4 km below the cloud altitude. The cloud particles depolarized the lidar returns, thus must they have been aspherical and hence solid. Atmospheric temperatures near 230 K were approximately 40 K too high to support ice particles at stratospheric water vapour pressures of a few ppmv. The isentropic back trajectory on 400 K showed the air parcels to have stayed clear of active major rocket launch sites. The air parcels at 400 K had traveled from the Aleutians across Canada and the Atlantic Ocean arriving above central Europe and then turned northward to pass over above the lidar station. Parcels at levels at ±25 K from 400 K had come from the pole and joined the 400 K trajectory path above eastern Canada. Apparently the cloud existed in a filament of air with an origin different from those filaments both above and below. Possibly the 400 K level air parcels had carried soot particles from forest wild fires in northern Canada or volcanic ash from the eruption of the Korovin Volcano in the Aleutian Islands.Key words: Atmospheric composition and structure (aerosols and particles; biosphere-atmosphere interactions · Meteorology and atmospheric dynamics (middle atmospheric dynamics

  5. A transitioning Arctic surface energy budget: the impacts of solar zenith angle, surface albedo and cloud radiative forcing

    Energy Technology Data Exchange (ETDEWEB)

    Sedlar, Joseph; Tjernstroem, Michael; Leck, Caroline [Stockholm University, Department of Meteorology, Stockholm (Sweden); Mauritsen, Thorsten [Max-Planck-Institute for Meteorology, Hamburg (Germany); Shupe, Matthew D.; Persson, P.O.G. [University of Colorado, NOAA-ESRL-PSD, Boulder, CO (United States); Brooks, Ian M.; Birch, Cathryn E. [University of Leeds, School of Earth and Environment, Leeds (United Kingdom); Sirevaag, Anders [University of Bergen, Bjerknes Center for Climate Research, Bergen (Norway); Nicolaus, Marcel [Norwegian Polar Institute, Tromsoe (Norway); Alfred Wegener Institute for Polar and Marine Research, Bremerhaven (Germany)

    2011-10-15

    Snow surface and sea-ice energy budgets were measured near 87.5 N during the Arctic Summer Cloud Ocean Study (ASCOS), from August to early September 2008. Surface temperature indicated four distinct temperature regimes, characterized by varying cloud, thermodynamic and solar properties. An initial warm, melt-season regime was interrupted by a 3-day cold regime where temperatures dropped from near zero to -7 C. Subsequently mean energy budget residuals remained small and near zero for 1 week until once again temperatures dropped rapidly and the energy budget residuals became negative. Energy budget transitions were dominated by the net radiative fluxes, largely controlled by the cloudiness. Variable heat, moisture and cloud distributions were associated with changing air-masses. Surface cloud radiative forcing, the net radiative effect of clouds on the surface relative to clear skies, is estimated. Shortwave cloud forcing ranged between -50 W m{sup -2} and zero and varied significantly with surface albedo, solar zenith angle and cloud liquid water. Longwave cloud forcing was larger and generally ranged between 65 and 85 W m{sup -2}, except when the cloud fraction was tenuous or contained little liquid water; thus the net effect of the clouds was to warm the surface. Both cold periods occurred under tenuous, or altogether absent, low-level clouds containing little liquid water, effectively reducing the cloud greenhouse effect. Freeze-up progression was enhanced by a combination of increasing solar zenith angles and surface albedo, while inhibited by a large, positive surface cloud forcing until a new air-mass with considerably less cloudiness advected over the experiment area. (orig.)

  6. Impacts of stratospheric sulfate geoengineering on tropospheric ozone

    Directory of Open Access Journals (Sweden)

    L. Xia

    2017-10-01

    Full Text Available A range of solar radiation management (SRM techniques has been proposed to counter anthropogenic climate change. Here, we examine the potential effects of stratospheric sulfate aerosols and solar insolation reduction on tropospheric ozone and ozone at Earth's surface. Ozone is a key air pollutant, which can produce respiratory diseases and crop damage. Using a version of the Community Earth System Model from the National Center for Atmospheric Research that includes comprehensive tropospheric and stratospheric chemistry, we model both stratospheric sulfur injection and solar irradiance reduction schemes, with the aim of achieving equal levels of surface cooling relative to the Representative Concentration Pathway 6.0 scenario. This allows us to compare the impacts of sulfate aerosols and solar dimming on atmospheric ozone concentrations. Despite nearly identical global mean surface temperatures for the two SRM approaches, solar insolation reduction increases global average surface ozone concentrations, while sulfate injection decreases it. A fundamental difference between the two geoengineering schemes is the importance of heterogeneous reactions in the photochemical ozone balance with larger stratospheric sulfate abundance, resulting in increased ozone depletion in mid- and high latitudes. This reduces the net transport of stratospheric ozone into the troposphere and thus is a key driver of the overall decrease in surface ozone. At the same time, the change in stratospheric ozone alters the tropospheric photochemical environment due to enhanced ultraviolet radiation. A shared factor among both SRM scenarios is decreased chemical ozone loss due to reduced tropospheric humidity. Under insolation reduction, this is the dominant factor giving rise to the global surface ozone increase. Regionally, both surface ozone increases and decreases are found for both scenarios; that is, SRM would affect regions of the world differently in terms of air

  7. Impacts of stratospheric sulfate geoengineering on tropospheric ozone

    Science.gov (United States)

    Xia, Lili; Nowack, Peer J.; Tilmes, Simone; Robock, Alan

    2017-10-01

    A range of solar radiation management (SRM) techniques has been proposed to counter anthropogenic climate change. Here, we examine the potential effects of stratospheric sulfate aerosols and solar insolation reduction on tropospheric ozone and ozone at Earth's surface. Ozone is a key air pollutant, which can produce respiratory diseases and crop damage. Using a version of the Community Earth System Model from the National Center for Atmospheric Research that includes comprehensive tropospheric and stratospheric chemistry, we model both stratospheric sulfur injection and solar irradiance reduction schemes, with the aim of achieving equal levels of surface cooling relative to the Representative Concentration Pathway 6.0 scenario. This allows us to compare the impacts of sulfate aerosols and solar dimming on atmospheric ozone concentrations. Despite nearly identical global mean surface temperatures for the two SRM approaches, solar insolation reduction increases global average surface ozone concentrations, while sulfate injection decreases it. A fundamental difference between the two geoengineering schemes is the importance of heterogeneous reactions in the photochemical ozone balance with larger stratospheric sulfate abundance, resulting in increased ozone depletion in mid- and high latitudes. This reduces the net transport of stratospheric ozone into the troposphere and thus is a key driver of the overall decrease in surface ozone. At the same time, the change in stratospheric ozone alters the tropospheric photochemical environment due to enhanced ultraviolet radiation. A shared factor among both SRM scenarios is decreased chemical ozone loss due to reduced tropospheric humidity. Under insolation reduction, this is the dominant factor giving rise to the global surface ozone increase. Regionally, both surface ozone increases and decreases are found for both scenarios; that is, SRM would affect regions of the world differently in terms of air pollution. In conclusion

  8. Improvements of top-of-atmosphere and surface irradiance computations with CALIPSO-, CloudSat-, and MODIS-derived cloud and aerosol properties

    Science.gov (United States)

    Kato, Seiji; Rose, Fred G.; Sun-Mack, Sunny; Miller, Walter F.; Chen, Yan; Rutan, David A.; Stephens, Graeme L.; Loeb, Norman G.; Minnis, Patrick; Wielicki, Bruce A.; Winker, David M.; Charlock, Thomas P.; Stackhouse, Paul W., Jr.; Xu, Kuan-Man; Collins, William D.

    2011-10-01

    One year of instantaneous top-of-atmosphere (TOA) and surface shortwave and longwave irradiances are computed using cloud and aerosol properties derived from instruments on the A-Train Constellation: the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) on the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) satellite, the CloudSat Cloud Profiling Radar (CPR), and the Aqua Moderate Resolution Imaging Spectrometer (MODIS). When modeled irradiances are compared with those computed with cloud properties derived from MODIS radiances by a Clouds and the Earth's Radiant Energy System (CERES) cloud algorithm, the global and annual mean of modeled instantaneous TOA irradiances decreases by 12.5 W m-2 (5.0%) for reflected shortwave and 2.5 W m-2 (1.1%) for longwave irradiances. As a result, the global annual mean of instantaneous TOA irradiances agrees better with CERES-derived irradiances to within 0.5W m-2 (out of 237.8 W m-2) for reflected shortwave and 2.6W m-2 (out of 240.1 W m-2) for longwave irradiances. In addition, the global annual mean of instantaneous surface downward longwave irradiances increases by 3.6 W m-2 (1.0%) when CALIOP- and CPR-derived cloud properties are used. The global annual mean of instantaneous surface downward shortwave irradiances also increases by 8.6 W m-2 (1.6%), indicating that the net surface irradiance increases when CALIOP- and CPR-derived cloud properties are used. Increasing the surface downward longwave irradiance is caused by larger cloud fractions (the global annual mean by 0.11, 0.04 excluding clouds with optical thickness less than 0.3) and lower cloud base heights (the global annual mean by 1.6 km). The increase of the surface downward longwave irradiance in the Arctic exceeds 10 W m-2 (˜4%) in winter because CALIOP and CPR detect more clouds in comparison with the cloud detection by the CERES cloud algorithm during polar night. The global annual mean surface downward longwave irradiance of

  9. Refinement of the CALIOP cloud mask algorithm

    Science.gov (United States)

    Katagiri, Shuichiro; Sato, Kaori; Ohta, Kohei; Okamoto, Hajime

    2018-04-01

    A modified cloud mask algorithm was applied to the CALIOP data to have more ability to detect the clouds in the lower atmosphere. In this algorithm, we also adopt the fully attenuation discrimination and the remain noise estimation using the data obtained at an altitude of 40 km to avoid contamination of stratospheric aerosols. The new cloud mask shows an increase in the lower cloud fraction. Comparison of the results to the data observed with a PML ground observation was also made.

  10. Mechanism and Kinetics of the Formation and Transport of Aerosol Particles in the Lower Stratosphere

    Science.gov (United States)

    Aloyan, A. E.; Ermakov, A. N.; Arutyunyan, V. O.

    2018-03-01

    Field and laboratory observation data on aerosol particles in the lower stratosphere are considered. The microphysics of their formation, mechanisms of heterogeneous chemical reactions involving reservoir gases (e.g., HCl, ClONO2, etc.) and their kinetic characteristics are analyzed. A new model of global transport of gaseous and aerosol admixtures in the lower stratosphere is described. The preliminary results from a numerical simulation of the formation of sulfate particles of the Junge layer and particles of polar stratospheric clouds (PSCs, types Ia, Ib, and II) are presented, and their effect on the gas and aerosol composition is analyzed.

  11. Influence of Aerosol Heating on the Stratospheric Transport of the Mt. Pinatubo Eruption

    Science.gov (United States)

    Aquila, Valentina; Oman, Luke D.; Stolarski, Richard S.

    2011-01-01

    On June 15th, 1991 the eruption of Mt. Pinatubo (15.1 deg. N, 120.3 Deg. E) in the Philippines injected about 20 Tg of sulfur dioxide in the stratosphere, which was transformed into sulfuric acid aerosol. The large perturbation of the background aerosol caused an increase in temperature in the lower stratosphere of 2-3 K. Even though stratospheric winds climatological]y tend to hinder the air mixing between the two hemispheres, observations have shown that a large part of the SO2 emitted by Mt. Pinatubo have been transported from the Northern to the Southern Hemisphere. We simulate the eruption of Mt. Pinatubo with the Goddard Earth Observing System (GEOS) version 5 global climate model, coupled to the aerosol module GOCART and the stratospheric chemistry module StratChem, to investigate the influence of the eruption of Mt. Pinatubo on the stratospheric transport pattern. We perform two ensembles of simulations: the first ensemble consists of runs without coupling between aerosol and radiation. In these simulations the plume of aerosols is treated as a passive tracer and the atmosphere is unperturbed. In the second ensemble of simulations aerosols and radiation are coupled. We show that the set of runs with interactive aerosol produces a larger cross-equatorial transport of the Pinatubo cloud. In our simulations the local heating perturbation caused by the sudden injection of volcanic aerosol changes the pattern of the stratospheric winds causing more intrusion of air from the Northern into the Southern Hemisphere. Furthermore, we perform simulations changing the injection height of the cloud, and study the transport of the plume resulting from the different scenarios. Comparisons of model results with SAGE II and AVHRR satellite observations will be shown.

  12. A fiery birth of aluminosilica analogs of refractory dust in the upper stratosphere

    Science.gov (United States)

    Rietmeijer, F. J. M.; Ferrari, M.; Della Corte, V.; Rotundi, A.; Palumbo, P.; De Angelis, S.; Galluzzi, V.

    2017-11-01

    Following a successful dust collection flight in the upper stratosphere our DUSTER (Dust in the Upper Stratosphere Tracking Experiment and Retrieval) made a safe remote landing at its assigned location on Baffin Island during early June 2009. When the balloon payload that included DUSTER was retrieved it was found part of the payload had experienced a lithium-sparked fire while the payload was being dragged across the landing site. In this process the housing of DUSTER had developed a pin-sized hole that allowed smoke of the fire to enter the collector. Numerous smoke particles were found covering both the DUSTER collection and blank collector surfaces an indication that our experiment to collect upper stratospheric dust had failed! Both collector surfaces were covered by numerous carbon smoke and amorphous, aluminosilica nanoparticles. The compositions of vast majority of these aluminosilica nanoparticles, Al2O3 = 49 wt% and SiO2 = 51 wt%, was both surprising and unique because it was an exact match of the Deep Metastable Eutectic (DME) nanoparticles found in vapor phase condensation experiments. These vapor phase condensation experiments were conducted to explore the formation of extraterrestrial dust particles. We are not claiming an extraterrestrial origin for these particles from this DUSTER experiment. We submit that given the appropriate conditions of high temperature alumina and silica vapors and rapid quenching in a contained natural environment, DME aluminosilica nanoparticles will likely condense. This serendipitous result can be used to explore nanoparticle formation inside incandescent clouds associated with bolides and fireballs.

  13. Lower stratospheric observations from aircraft and satellite during the 2015/2016 El Nino

    Science.gov (United States)

    Rosenlof, K. H.; Avery, M. A.; Davis, S. M.; Gao, R. S.; Thornberry, T. D.

    2016-12-01

    Winter 2015/2016 experienced a strong El Nino that was heavily observed by aircraft, radiosonde and satellite platforms. During the National Oceanographic and Atmospheric Administration's (NOAA) Sensing Hazards with Operational Unmanned Technology (SHOUT)/El Nino Rapid Response (ENRR) flights of the NASA Global Hawk, in situ ozone measurements were made in the lower stratosphere over the Pacific. These will be contrasted with ozone measurements taken during La Nina and ENSO neutral conditions during past Global Hawk aircraft campaigns. Additionally, lower stratospheric water vapor and ozone measurements from the Microwave Limb Sounder satellite instrument and stratospheric ice measurements above the tropopause from the Cloud-Aerosol Aerosol Lidar with Orthogonal Polarization (CALIOP) will be presented. Our aircraft ozone measurements are higher for the El Nino flights than during other missions previously sampled, while zonally averaged lower stratospheric water vapor and central Pacific ice path above the tropopause reached record highs. Implications and possible reasons for these anomalous observations will be discussed. Winter 2015/2016 experienced a strong El Nino that was heavily observed by aircraft, radiosonde and satellite platforms. During the National Oceanographic and Atmospheric Administration's (NOAA) Sensing Hazards with Operational Unmanned Technology (SHOUT)/El Nino Rapid Response (ENRR) flights of the NASA Global Hawk, in situ ozone measurements were made in the upper troposphere and lower stratosphere (UTLS) over the Pacific. These will be contrasted with ozone measurements made during La Nina and ENSO neutral conditions during past Global Hawk aircraft campaigns. Additionally, UTLS water vapor and ozone measurements from the Microwave Limb Sounder (MLS) satellite instrument and stratospheric ice measurements above the tropopause from the Cloud-Aerosol Aerosol Lidar with Orthogonal Polarization (CALIOP) will be presented. Our aircraft ozone

  14. Variability of surface ozone with cloud coverage over Kolkata, India

    Indian Academy of Sciences (India)

    Critical analysis of experimental surface ozone data and cloud coverage is reported over Kolkata during the period January 2011 to December 2011. Significant relationship between these two parameters is observed. Analysis shows that the trend of surface ozone concentration and cloud coverage follow opposite ...

  15. PolyFit: Polygonal Surface Reconstruction from Point Clouds

    KAUST Repository

    Nan, Liangliang; Wonka, Peter

    2017-01-01

    We propose a novel framework for reconstructing lightweight polygonal surfaces from point clouds. Unlike traditional methods that focus on either extracting good geometric primitives or obtaining proper arrangements of primitives, the emphasis of this work lies in intersecting the primitives (planes only) and seeking for an appropriate combination of them to obtain a manifold polygonal surface model without boundary.,We show that reconstruction from point clouds can be cast as a binary labeling problem. Our method is based on a hypothesizing and selection strategy. We first generate a reasonably large set of face candidates by intersecting the extracted planar primitives. Then an optimal subset of the candidate faces is selected through optimization. Our optimization is based on a binary linear programming formulation under hard constraints that enforce the final polygonal surface model to be manifold and watertight. Experiments on point clouds from various sources demonstrate that our method can generate lightweight polygonal surface models of arbitrary piecewise planar objects. Besides, our method is capable of recovering sharp features and is robust to noise, outliers, and missing data.

  16. PolyFit: Polygonal Surface Reconstruction from Point Clouds

    KAUST Repository

    Nan, Liangliang

    2017-12-25

    We propose a novel framework for reconstructing lightweight polygonal surfaces from point clouds. Unlike traditional methods that focus on either extracting good geometric primitives or obtaining proper arrangements of primitives, the emphasis of this work lies in intersecting the primitives (planes only) and seeking for an appropriate combination of them to obtain a manifold polygonal surface model without boundary.,We show that reconstruction from point clouds can be cast as a binary labeling problem. Our method is based on a hypothesizing and selection strategy. We first generate a reasonably large set of face candidates by intersecting the extracted planar primitives. Then an optimal subset of the candidate faces is selected through optimization. Our optimization is based on a binary linear programming formulation under hard constraints that enforce the final polygonal surface model to be manifold and watertight. Experiments on point clouds from various sources demonstrate that our method can generate lightweight polygonal surface models of arbitrary piecewise planar objects. Besides, our method is capable of recovering sharp features and is robust to noise, outliers, and missing data.

  17. Extended observations of volcanic SO2 and sulfate aerosol in the stratosphere

    NARCIS (Netherlands)

    Carn, S.A.; Krotkov, N.A.; Yang, Kai; Hoff, R.M.; Prata, A.J.; Krueger, A.J.; Loughlin, S.C.; Levelt, P.F.

    2007-01-01

    Sulfate aerosol produced after injection of sulfur dioxide (SO2) into the stratosphere by volcanic eruptions can trigger climate change. We present new satellite data from the Ozone Monitoring Instrument (OMI) and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) missions

  18. A Climatology of Surface Cloud Radiative Effects at the ARM Tropical Western Pacific Sites

    Energy Technology Data Exchange (ETDEWEB)

    McFarlane, Sally A.; Long, Charles N.; Flaherty, Julia E.

    2013-04-01

    Cloud radiative effects on surface downwelling fluxes are investigated using long-term datasets from the three Atmospheric Radiation Measurement (ARM) sites in the Tropical Western Pacific (TWP) region. The Nauru and Darwin sites show significant variability in sky cover, downwelling radiative fluxes, and surface cloud radiative effect (CRE) due to El Niño and the Australian monsoon, respectively, while the Manus site shows little intra-seasonal or interannual variability. Cloud radar measurement of cloud base and top heights are used to define cloud types so that the effect of cloud type on the surface CRE can be examined. Clouds with low bases contribute 71-75% of the surface shortwave (SW) CRE and 66-74% of the surface longwave (LW) CRE at the three TWP sites, while clouds with mid-level bases contribute 8-9% of the SW CRE and 12-14% of the LW CRE, and clouds with high bases contribute 16-19% of the SW CRE and 15-21% of the LW CRE.

  19. Studying Stratospheric Temperature Variation with Cosmic Ray Measurements

    Science.gov (United States)

    Zhang, Xiaohang; He, Xiaochun

    2015-04-01

    The long term stratospheric cooling in recent decades is believed to be equally important as surface warming as evidence of influences of human activities on the climate system. Un- fortunatly, there are some discrepancies among different measurements of stratospheric tem- peratures, which could be partially caused by the limitations of the measurement techniques. It has been known for decades that cosmic ray muon flux is sensitive to stratospheric temperature change. Dorman proposed that this effect could be used to probe the tempera- ture variations in the stratophere. In this talk, a method for reconstructing stratospheric temperature will be discussed. We verify this method by comparing the stratospheric tem- perature measured by radiosonde with the ones derived from cosmic ray measurement at multiple locations around the globe.

  20. A robust real-time surface reconstruction method on point clouds captured from a 3D surface photogrammetry system

    Energy Technology Data Exchange (ETDEWEB)

    Liu, Wenyang [Department of Bioengineering, University of California, Los Angeles, Los Angeles, California 90095 (United States); Cheung, Yam [Department of Radiation Oncology, University of Texas Southwestern, Dallas, Texas 75390 (United States); Sawant, Amit [Department of Radiation Oncology, University of Texas Southwestern, Dallas, Texas, 75390 and Department of Radiation Oncology, University of Maryland, College Park, Maryland 20742 (United States); Ruan, Dan, E-mail: druan@mednet.ucla.edu [Department of Bioengineering, University of California, Los Angeles, Los Angeles, California 90095 and Department of Radiation Oncology, University of California, Los Angeles, Los Angeles, California 90095 (United States)

    2016-05-15

    Purpose: To develop a robust and real-time surface reconstruction method on point clouds captured from a 3D surface photogrammetry system. Methods: The authors have developed a robust and fast surface reconstruction method on point clouds acquired by the photogrammetry system, without explicitly solving the partial differential equation required by a typical variational approach. Taking advantage of the overcomplete nature of the acquired point clouds, their method solves and propagates a sparse linear relationship from the point cloud manifold to the surface manifold, assuming both manifolds share similar local geometry. With relatively consistent point cloud acquisitions, the authors propose a sparse regression (SR) model to directly approximate the target point cloud as a sparse linear combination from the training set, assuming that the point correspondences built by the iterative closest point (ICP) is reasonably accurate and have residual errors following a Gaussian distribution. To accommodate changing noise levels and/or presence of inconsistent occlusions during the acquisition, the authors further propose a modified sparse regression (MSR) model to model the potentially large and sparse error built by ICP with a Laplacian prior. The authors evaluated the proposed method on both clinical point clouds acquired under consistent acquisition conditions and on point clouds with inconsistent occlusions. The authors quantitatively evaluated the reconstruction performance with respect to root-mean-squared-error, by comparing its reconstruction results against that from the variational method. Results: On clinical point clouds, both the SR and MSR models have achieved sub-millimeter reconstruction accuracy and reduced the reconstruction time by two orders of magnitude to a subsecond reconstruction time. On point clouds with inconsistent occlusions, the MSR model has demonstrated its advantage in achieving consistent and robust performance despite the introduced

  1. A robust real-time surface reconstruction method on point clouds captured from a 3D surface photogrammetry system.

    Science.gov (United States)

    Liu, Wenyang; Cheung, Yam; Sawant, Amit; Ruan, Dan

    2016-05-01

    To develop a robust and real-time surface reconstruction method on point clouds captured from a 3D surface photogrammetry system. The authors have developed a robust and fast surface reconstruction method on point clouds acquired by the photogrammetry system, without explicitly solving the partial differential equation required by a typical variational approach. Taking advantage of the overcomplete nature of the acquired point clouds, their method solves and propagates a sparse linear relationship from the point cloud manifold to the surface manifold, assuming both manifolds share similar local geometry. With relatively consistent point cloud acquisitions, the authors propose a sparse regression (SR) model to directly approximate the target point cloud as a sparse linear combination from the training set, assuming that the point correspondences built by the iterative closest point (ICP) is reasonably accurate and have residual errors following a Gaussian distribution. To accommodate changing noise levels and/or presence of inconsistent occlusions during the acquisition, the authors further propose a modified sparse regression (MSR) model to model the potentially large and sparse error built by ICP with a Laplacian prior. The authors evaluated the proposed method on both clinical point clouds acquired under consistent acquisition conditions and on point clouds with inconsistent occlusions. The authors quantitatively evaluated the reconstruction performance with respect to root-mean-squared-error, by comparing its reconstruction results against that from the variational method. On clinical point clouds, both the SR and MSR models have achieved sub-millimeter reconstruction accuracy and reduced the reconstruction time by two orders of magnitude to a subsecond reconstruction time. On point clouds with inconsistent occlusions, the MSR model has demonstrated its advantage in achieving consistent and robust performance despite the introduced occlusions. The authors have

  2. A robust real-time surface reconstruction method on point clouds captured from a 3D surface photogrammetry system

    International Nuclear Information System (INIS)

    Liu, Wenyang; Cheung, Yam; Sawant, Amit; Ruan, Dan

    2016-01-01

    Purpose: To develop a robust and real-time surface reconstruction method on point clouds captured from a 3D surface photogrammetry system. Methods: The authors have developed a robust and fast surface reconstruction method on point clouds acquired by the photogrammetry system, without explicitly solving the partial differential equation required by a typical variational approach. Taking advantage of the overcomplete nature of the acquired point clouds, their method solves and propagates a sparse linear relationship from the point cloud manifold to the surface manifold, assuming both manifolds share similar local geometry. With relatively consistent point cloud acquisitions, the authors propose a sparse regression (SR) model to directly approximate the target point cloud as a sparse linear combination from the training set, assuming that the point correspondences built by the iterative closest point (ICP) is reasonably accurate and have residual errors following a Gaussian distribution. To accommodate changing noise levels and/or presence of inconsistent occlusions during the acquisition, the authors further propose a modified sparse regression (MSR) model to model the potentially large and sparse error built by ICP with a Laplacian prior. The authors evaluated the proposed method on both clinical point clouds acquired under consistent acquisition conditions and on point clouds with inconsistent occlusions. The authors quantitatively evaluated the reconstruction performance with respect to root-mean-squared-error, by comparing its reconstruction results against that from the variational method. Results: On clinical point clouds, both the SR and MSR models have achieved sub-millimeter reconstruction accuracy and reduced the reconstruction time by two orders of magnitude to a subsecond reconstruction time. On point clouds with inconsistent occlusions, the MSR model has demonstrated its advantage in achieving consistent and robust performance despite the introduced

  3. The Role of Overshooting Convection in Elevated Stratospheric Water Vapor over the Summertime Continental United States

    Science.gov (United States)

    Herman, R. L.; Ray, E. A.; Rosenlof, K. H.; Bedka, K. M.; Schwartz, M. J.; Read, W. G.; Troy, R. F.

    2016-12-01

    The NASA ER-2 aircraft sampled the UTLS region over North America during the NASA Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS) field mission. On four flights targeting convectively-influenced air parcels, in situ measurements of enhanced water vapor in the lower stratosphere over the summertime continental United States were made using the JPL Laser Hygrometer (JLH Mark2). Water vapor mixing ratios greater than 10 ppmv, twice the stratospheric background levels, were measured at pressure levels between 80 and 160 hPa. Through satellite observations and analysis, we make the connection between these in situ water measurements and overshooting cloud tops. The overshooting tops (OT) are identified from a SEAC4RS OT detection product based on satellite infrared window channel brightness temperature gradients. Back-trajectory analysis ties enhanced water to OT one to seven days prior to the intercept by the aircraft. The trajectory paths are dominated by the North American Monsoon (NAM) anticyclonic circulation. This connection suggests that ice is convectively transported to the overworld stratosphere in OT events and subsequently sublimated; such events may irreversibly enhance stratospheric water vapor in the summer over Mexico and the United States. Regional context is provided by water observations from the Aura Microwave Limb Sounder (MLS).

  4. Enhanced stratospheric water vapor over the summertime continental United States and the role of overshooting convection

    Science.gov (United States)

    Herman, Robert L.; Ray, Eric A.; Rosenlof, Karen H.; Bedka, Kristopher M.; Schwartz, Michael J.; Read, William G.; Troy, Robert F.; Chin, Keith; Christensen, Lance E.; Fu, Dejian; Stachnik, Robert A.; Bui, T. Paul; Dean-Day, Jonathan M.

    2017-05-01

    The NASA ER-2 aircraft sampled the lower stratosphere over North America during the field mission for the NASA Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS). This study reports observations of convectively influenced air parcels with enhanced water vapor in the overworld stratosphere over the summertime continental United States and investigates three case studies in detail. Water vapor mixing ratios greater than 10 ppmv, which is much higher than the background 4 to 6 ppmv of the overworld stratosphere, were measured by the JPL Laser Hygrometer (JLH Mark2) at altitudes between 16.0 and 17.5 km (potential temperatures of approximately 380 to 410 K). Overshooting cloud tops (OTs) are identified from a SEAC4RS OT detection product based on satellite infrared window channel brightness temperature gradients. Through trajectory analysis, we make the connection between these in situ water measurements and OT. Back trajectory analysis ties enhanced water to OT 1 to 7 days prior to the intercept by the aircraft. The trajectory paths are dominated by the North American monsoon (NAM) anticyclonic circulation. This connection suggests that ice is convectively transported to the overworld stratosphere in OT events and subsequently sublimated; such events may irreversibly enhance stratospheric water vapor in the summer over Mexico and the United States. A regional context is provided by water observations from the Aura Microwave Limb Sounder (MLS).

  5. Development of a climate record of tropospheric and stratospheric column ozone from satellite remote sensing: evidence of an early recovery of global stratospheric ozone

    Directory of Open Access Journals (Sweden)

    J. R. Ziemke

    2012-07-01

    Full Text Available Ozone data beginning October 2004 from the Aura Ozone Monitoring Instrument (OMI and Aura Microwave Limb Sounder (MLS are used to evaluate the accuracy of the Cloud Slicing technique in effort to develop long data records of tropospheric and stratospheric ozone and for studying their long-term changes. Using this technique, we have produced a 32-yr (1979–2010 long record of tropospheric and stratospheric column ozone from the combined Total Ozone Mapping Spectrometer (TOMS and OMI. Analyses of these time series suggest that the quasi-biennial oscillation (QBO is the dominant source of inter-annual variability of stratospheric ozone and is clearest in the Southern Hemisphere during the Aura time record with related inter-annual changes of 30–40 Dobson Units. Tropospheric ozone for the long record also indicates a QBO signal in the tropics with peak-to-peak changes varying from 2 to 7 DU. The most important result from our study is that global stratospheric ozone indicates signature of a recovery occurring with ozone abundance now approaching the levels of year 1980 and earlier. The negative trends in stratospheric ozone in both hemispheres during the first 15 yr of the record are now positive over the last 15 yr and with nearly equal magnitudes. This turnaround in stratospheric ozone loss is occurring about 20 yr earlier than predicted by many chemistry climate models. This suggests that the Montreal Protocol which was first signed in 1987 as an international agreement to reduce ozone destroying substances is working well and perhaps better than anticipated.

  6. A Climatology of Midlatitude Continental Clouds from the ARM SGP Site. Part II; Cloud Fraction and Surface Radiative Forcing

    Science.gov (United States)

    Xi, B.; Minnis, P.

    2006-01-01

    Data collected at the Department of Energy Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) Central Facility (SCF) are analyzed to determine the monthly and hourly variations of cloud fraction and radiative forcing between January 1997 and December 2002. Cloud fractions are estimated for total cloud cover and for single-layered low (0-3 km), middle (3-6 km), and high clouds (more than 6 km) using ARM SCG ground-based paired lidar-radar measurements. Shortwave (SW) and longwave (LW) fluxes are derived from up- and down-looking standard precision spectral pyranometers and precision infrared radiometer measurements with uncertainties of approximately 10 Wm(exp -2). The annual averages of total, and single-layered low, middle and high cloud fractions are 0.49, 0.11, 0.03, and 0.17, respectively. Both total and low cloud amounts peak during January and February and reach a minimum during July and August, high clouds occur more frequently than other types of clouds with a peak in summer. The average annual downwelling surface SW fluxes for total and low clouds (151 and 138 Wm(exp-2), respectively) are less than those under middle and high clouds (188 and 201 Wm(exp -2), respectively), but the downwelling LW fluxes (349 and 356 Wm(exp -2)) underneath total and low clouds are greater than those from middle and high clouds (337 and 333 Wm(exp -2)). Low clouds produce the largest LW warming (55 Wm(exp -2) and SW cooling (-91 Wm(exp -2)) effects with maximum and minimum absolute values in spring and summer, respectively. High clouds have the smallest LW warming (17 Wm(exp -2)) and SW cooling (-37 Wm(exp -2)) effects at the surface. All-sky SW CRF decreases and LW CRF increases with increasing cloud fraction with mean slopes of -0.984 and 0.616 Wm(exp -2)%(exp -1), respectively. Over the entire diurnal cycle, clouds deplete the amount of surface insolation more than they add to the downwelling LW flux. The calculated CRFs do not appear to be significantly

  7. The influence of surface roughness on cloud cavitation flow around hydrofoils

    Science.gov (United States)

    Hao, Jiafeng; Zhang, Mindi; Huang, Xu

    2018-02-01

    The aim of this study is to investigate experimentally the effect of surface roughness on cloud cavitation around Clark-Y hydrofoils. High-speed video and particle image velocimetry (PIV) were used to obtain cavitation patterns images (Prog. Aerosp. Sci. 37: 551-581, 2001), as well as velocity and vorticity fields. Results are presented for cloud cavitating conditions around a Clark-Y hydrofoil fixed at angle of attack of α =8{°} for moderate Reynolds number of Re=5.6 × 105. The results show that roughness had a great influence on the pattern, velocity and vorticity distribution of cloud cavitation. For cavitating flow around a smooth hydrofoil (A) and a rough hydrofoil (B), cloud cavitation occurred in the form of finger-like cavities and attached subulate cavities, respectively. The period of cloud cavitation around hydrofoil A was shorter than for hydrofoil B. Surface roughness had a great influence on the process of cloud cavitation. The development of cloud cavitation around hydrofoil A consisted of two stages: (1) Attached cavities developed along the surface to the trailing edge; (2) A reentrant jet developed, resulting in shedding and collapse of cluster bubbles or vortex structure. Meanwhile, its development for hydrofoil B included three stages: (1) Attached cavities developed along the surface to the trailing edge, with accumulation and rotation of bubbles at the trailing edge of the hydrofoil affecting the flow field; (2) Development of a reentrant jet resulted in the first shedding of cavities. Interaction and movement of flows from the pressure side and suction side brought liquid water from the pressure side to the suction side of the hydrofoil, finally forming a reentrant jet. The jet kept moving along the surface to the leading edge of the hydrofoil, resulting in large-scale shedding of cloud bubbles. Several vortices appeared and dissipated during the process; (3) Cavities grew and shed again.

  8. Examination of Regional Trends in Cloud Properties over Surface Sites Derived from MODIS and AVHRR using the CERES Cloud Algorithm

    Science.gov (United States)

    Smith, W. L., Jr.; Minnis, P.; Bedka, K. M.; Sun-Mack, S.; Chen, Y.; Doelling, D. R.; Kato, S.; Rutan, D. A.

    2017-12-01

    Recent studies analyzing long-term measurements of surface insolation at ground sites suggest that decadal-scale trends of increasing (brightening) and decreasing (dimming) downward solar flux have occurred at various times over the last century. Regional variations have been reported that range from near 0 Wm-2/decade to as large as 9 Wm-2/decade depending on the location and time period analyzed. The more significant trends have been attributed to changes in overhead clouds and aerosols, although quantifying their relative impacts using independent observations has been difficult, owing in part to a lack of consistent long-term measurements of cloud properties. This paper examines new satellite based records of cloud properties derived from MODIS (2000-present) and AVHRR (1981- present) data to infer cloud property trends over a number of surface radiation sites across the globe. The MODIS cloud algorithm was developed for the NASA Clouds and the Earth's Radiant Energy System (CERES) project to provide a consistent record of cloud properties to help improve broadband radiation measurements and to better understand cloud radiative effects. The CERES-MODIS cloud algorithm has been modified to analyze other satellites including the AVHRR on the NOAA satellites. Compared to MODIS, obtaining consistent cloud properties over a long period from AVHRR is a much more significant challenge owing to the number of different satellites, instrument calibration uncertainties, orbital drift and other factors. Nevertheless, both the MODIS and AVHRR cloud properties will be analyzed to determine trends, and their level of consistency and correspondence with surface radiation trends derived from the ground-based radiometer data. It is anticipated that this initial study will contribute to an improved understanding of surface solar radiation trends and their relationship to clouds.

  9. Quantifying Uncertainty in Satellite-Retrieved Land Surface Temperature from Cloud Detection Errors

    Directory of Open Access Journals (Sweden)

    Claire E. Bulgin

    2018-04-01

    Full Text Available Clouds remain one of the largest sources of uncertainty in remote sensing of surface temperature in the infrared, but this uncertainty has not generally been quantified. We present a new approach to do so, applied here to the Advanced Along-Track Scanning Radiometer (AATSR. We use an ensemble of cloud masks based on independent methodologies to investigate the magnitude of cloud detection uncertainties in area-average Land Surface Temperature (LST retrieval. We find that at a grid resolution of 625 km 2 (commensurate with a 0.25 ∘ grid size at the tropics, cloud detection uncertainties are positively correlated with cloud-cover fraction in the cell and are larger during the day than at night. Daytime cloud detection uncertainties range between 2.5 K for clear-sky fractions of 10–20% and 1.03 K for clear-sky fractions of 90–100%. Corresponding night-time uncertainties are 1.6 K and 0.38 K, respectively. Cloud detection uncertainty shows a weaker positive correlation with the number of biomes present within a grid cell, used as a measure of heterogeneity in the background against which the cloud detection must operate (e.g., surface temperature, emissivity and reflectance. Uncertainty due to cloud detection errors is strongly dependent on the dominant land cover classification. We find cloud detection uncertainties of a magnitude of 1.95 K over permanent snow and ice, 1.2 K over open forest, 0.9–1 K over bare soils and 0.09 K over mosaic cropland, for a standardised clear-sky fraction of 74.2%. As the uncertainties arising from cloud detection errors are of a significant magnitude for many surface types and spatially heterogeneous where land classification varies rapidly, LST data producers are encouraged to quantify cloud-related uncertainties in gridded products.

  10. LSAH: a fast and efficient local surface feature for point cloud registration

    Science.gov (United States)

    Lu, Rongrong; Zhu, Feng; Wu, Qingxiao; Kong, Yanzi

    2018-04-01

    Point cloud registration is a fundamental task in high level three dimensional applications. Noise, uneven point density and varying point cloud resolutions are the three main challenges for point cloud registration. In this paper, we design a robust and compact local surface descriptor called Local Surface Angles Histogram (LSAH) and propose an effectively coarse to fine algorithm for point cloud registration. The LSAH descriptor is formed by concatenating five normalized sub-histograms into one histogram. The five sub-histograms are created by accumulating a different type of angle from a local surface patch respectively. The experimental results show that our LSAH is more robust to uneven point density and point cloud resolutions than four state-of-the-art local descriptors in terms of feature matching. Moreover, we tested our LSAH based coarse to fine algorithm for point cloud registration. The experimental results demonstrate that our algorithm is robust and efficient as well.

  11. Projections of UV radiation changes in the 21st century: impact of ozone recovery and cloud effects

    Directory of Open Access Journals (Sweden)

    A. F. Bais

    2011-08-01

    Full Text Available Monthly averaged surface erythemal solar irradiance (UV-Ery for local noon from 1960 to 2100 has been derived using radiative transfer calculations and projections of ozone, temperature and cloud change from 14 chemistry climate models (CCM, as part of the CCMVal-2 activity of SPARC. Our calculations show the influence of ozone depletion and recovery on erythemal irradiance. In addition, we investigate UV-Ery changes caused by climate change due to increasing greenhouse gas concentrations. The latter include effects of both stratospheric ozone and cloud changes. The derived estimates provide a global picture of the likely changes in erythemal irradiance during the 21st century. Uncertainties arise from the assumed scenarios, different parameterizations – particularly of cloud effects on UV-Ery – and the spread in the CCM projections. The calculations suggest that relative to 1980, annually mean UV-Ery in the 2090s will be on average ~12 % lower at high latitudes in both hemispheres, ~3 % lower at mid latitudes, and marginally higher (~1 % in the tropics. The largest reduction (~16 % is projected for Antarctica in October. Cloud effects are responsible for 2–3 % of the reduction in UV-Ery at high latitudes, but they slightly moderate it at mid-latitudes (~1 %. The year of return of erythemal irradiance to values of certain milestones (1965 and 1980 depends largely on the return of column ozone to the corresponding levels and is associated with large uncertainties mainly due to the spread of the model projections. The inclusion of cloud effects in the calculations has only a small effect of the return years. At mid and high latitudes, changes in clouds and stratospheric ozone transport by global circulation changes due to greenhouse gases will sustain the erythemal irradiance at levels below those in 1965, despite the removal of ozone depleting substances. At northern high latitudes (60°–90°, the projected decreases in cloud

  12. Effects on stratospheric moistening by rates of change of aerosol optical depth and ozone due to solar activity in extra-tropics

    Science.gov (United States)

    Saha, U.; Maitra, A.

    2014-11-01

    The solar-induced changes in ozone and aerosol optical depth have relative effects on stratospheric moistening at upper troposphere/lower stratosphere region. Wavelet-based multi-scale principal component analysis technique has been applied to de-noise component of quasi-biennial oscillation and El Niño-Southern Oscillation from ozone and aerosol optical depth variations. Rate of change of aerosol optical depth sharply increases indicating a positive gradient whereas rate of change of ozone sharply decreases indicating a negative gradient with solar activity during the years 2004-2010. It is also observed that with increase of rate of change of aerosol optical depth, there is a sharp increase of stratospheric moistening caused by enhanced deep convection. On the contrary, with the increase of stratospheric moistening, there is a sharp decrease of rate of change of ozone resulting in a cross-over between the two parameters. An increase in aerosol optical depth may cause a significant increase in the gradient of vertical temperature profile, as well as formation of cloud condensation nuclei, clouds and hence rainfall. This may lead to formation of strong convective system in the atmosphere that is essential for vertical transfer of water vapour in the tropics percolating tropical tropopause layer and depleting stratospheric ozone in the extra-tropics.

  13. Chapter 3: Evaluating the impacts of carbonaceous aerosols on clouds and climate

    Energy Technology Data Exchange (ETDEWEB)

    Menon, Surabi; Del Genio, Anthony D.

    2007-09-03

    other models as well (cf. Jacobson, 2002) but the relative impacts on convective and stratiform processes were not separated. Other changes to atmospheric stability and thermodynamical quantities due to aerosol absorption are also known to be important in modifying cloud macro/micro properties. Linkages between convection and boreal biomass burning can also impact the upper troposphere and lower stratosphere, radiation and cloud microphysical properties via transport of tropospheric aerosols to the lower stratosphere during extreme convection (Fromm and Servranckx 2003). Relevant questions regarding the impact of biomass aerosols on convective cloud properties include the effects of vertical transport of aerosols, spatial and temporal distribution of rainfall, vertical shift in latent heat release, phase shift of precipitation, circulation and their impacts on radiation. Over land surfaces, a decrease in surface shortwave radiation ({approx} 3-6 W m{sup -2} per decade) has been observed between 1960 to 1990, whereas, increases of 0.4 K in land temperature during the same period that occurred have resulted in speculations that evaporation and precipitation should also have decreased (Wild et al. 2004). However, precipitation records for the same period over land do not indicate any significant trend (Beck et al. 2005). The changes in precipitation are thought to be related to increased moisture advection from the oceans (Wild et al. 2004), which may well have some contributions from aerosol-radiation-convection coupling that could modify circulation patterns and hence moisture advection in specific regions. Other important aspects of aerosol effects, besides the direct, semi-direct, microphysical and thermodynamical impacts include alteration of surface albedos, especially snow and ice covered surfaces, due to absorbing aerosols. These effects are uncertain (Jacobson, 2004) but may produce as much as 0.3 W m{sup -2} forcing in the Northern hemisphere that could

  14. Stratospheric aerosols

    International Nuclear Information System (INIS)

    Rosen, J.; Ivanov, V.A.

    1993-01-01

    Stratospheric aerosol measurements can provide both spatial and temporal data of sufficient resolution to be of use in climate models. Relatively recent results from a wide range of instrument techniques for measuring stratospheric aerosol parameters are described. Such techniques include impactor sampling, lidar system sensing, filter sampling, photoelectric particle counting, satellite extinction-sensing using the sun as a source, and optical depth probing, at sites mainly removed from tropospheric aerosol sources. Some of these techniques have also had correlative and intercomparison studies. The main methods for determining the vertical profiles of stratospheric aerosols are outlined: lidar extinction measurements from satellites; impactor measurements from balloons and aircraft; and photoelectric particle counter measurements from balloons, aircraft, and rockets. The conversion of the lidar backscatter to stratospheric aerosol mass loading is referred to. Absolute measurements of total solar extinction from satellite orbits can be used to extract the aerosol extinction, and several examples of vertical profiles of extinction obtained with the SAGE satellite are given. Stratospheric mass loading can be inferred from extinction using approximate linear relationships but under restrictive conditions. Impactor sampling is essentially the only method in which the physical nature of the stratospheric aerosol is observed visually. Vertical profiles of stratospheric aerosol number concentration using impactor data are presented. Typical profiles using a dual-size-range photoelectric dustsonde particle counter are given for volcanically disturbed and inactive periods. Some measurements of the global distribution of stratospheric aerosols are also presented. Volatility measurements are described, indicating that stratospheric aerosols are composed primarily of about 75% sulfuric acid and 25% water

  15. A continuous surface reconstruction method on point cloud captured from a 3D surface photogrammetry system

    Energy Technology Data Exchange (ETDEWEB)

    Liu, Wenyang [Department of Bioengineering, University of California, Los Angeles, California 90095 (United States); Cheung, Yam; Sabouri, Pouya; Arai, Tatsuya J.; Sawant, Amit [Department of Radiation Oncology, University of Texas Southwestern, Dallas, Texas 75390 (United States); Ruan, Dan, E-mail: druan@mednet.ucla.edu [Department of Bioengineering, University of California, Los Angeles, California 90095 and Department of Radiation Oncology, University of California, Los Angeles, California 90095 (United States)

    2015-11-15

    Purpose: To accurately and efficiently reconstruct a continuous surface from noisy point clouds captured by a surface photogrammetry system (VisionRT). Methods: The authors have developed a level-set based surface reconstruction method on point clouds captured by a surface photogrammetry system (VisionRT). The proposed method reconstructs an implicit and continuous representation of the underlying patient surface by optimizing a regularized fitting energy, offering extra robustness to noise and missing measurements. By contrast to explicit/discrete meshing-type schemes, their continuous representation is particularly advantageous for subsequent surface registration and motion tracking by eliminating the need for maintaining explicit point correspondences as in discrete models. The authors solve the proposed method with an efficient narrowband evolving scheme. The authors evaluated the proposed method on both phantom and human subject data with two sets of complementary experiments. In the first set of experiment, the authors generated a series of surfaces each with different black patches placed on one chest phantom. The resulting VisionRT measurements from the patched area had different degree of noise and missing levels, since VisionRT has difficulties in detecting dark surfaces. The authors applied the proposed method to point clouds acquired under these different configurations, and quantitatively evaluated reconstructed surfaces by comparing against a high-quality reference surface with respect to root mean squared error (RMSE). In the second set of experiment, the authors applied their method to 100 clinical point clouds acquired from one human subject. In the absence of ground-truth, the authors qualitatively validated reconstructed surfaces by comparing the local geometry, specifically mean curvature distributions, against that of the surface extracted from a high-quality CT obtained from the same patient. Results: On phantom point clouds, their method

  16. A continuous surface reconstruction method on point cloud captured from a 3D surface photogrammetry system.

    Science.gov (United States)

    Liu, Wenyang; Cheung, Yam; Sabouri, Pouya; Arai, Tatsuya J; Sawant, Amit; Ruan, Dan

    2015-11-01

    To accurately and efficiently reconstruct a continuous surface from noisy point clouds captured by a surface photogrammetry system (VisionRT). The authors have developed a level-set based surface reconstruction method on point clouds captured by a surface photogrammetry system (VisionRT). The proposed method reconstructs an implicit and continuous representation of the underlying patient surface by optimizing a regularized fitting energy, offering extra robustness to noise and missing measurements. By contrast to explicit/discrete meshing-type schemes, their continuous representation is particularly advantageous for subsequent surface registration and motion tracking by eliminating the need for maintaining explicit point correspondences as in discrete models. The authors solve the proposed method with an efficient narrowband evolving scheme. The authors evaluated the proposed method on both phantom and human subject data with two sets of complementary experiments. In the first set of experiment, the authors generated a series of surfaces each with different black patches placed on one chest phantom. The resulting VisionRT measurements from the patched area had different degree of noise and missing levels, since VisionRT has difficulties in detecting dark surfaces. The authors applied the proposed method to point clouds acquired under these different configurations, and quantitatively evaluated reconstructed surfaces by comparing against a high-quality reference surface with respect to root mean squared error (RMSE). In the second set of experiment, the authors applied their method to 100 clinical point clouds acquired from one human subject. In the absence of ground-truth, the authors qualitatively validated reconstructed surfaces by comparing the local geometry, specifically mean curvature distributions, against that of the surface extracted from a high-quality CT obtained from the same patient. On phantom point clouds, their method achieved submillimeter

  17. Observational constraints on Arctic boundary-layer clouds, surface moisture and sensible heat fluxes

    Science.gov (United States)

    Wu, D. L.; Boisvert, L.; Klaus, D.; Dethloff, K.; Ganeshan, M.

    2016-12-01

    The dry, cold environment and dynamic surface variations make the Arctic a unique but difficult region for observations, especially in the atmospheric boundary layer (ABL). Spaceborne platforms have been the key vantage point to capture basin-scale changes during the recent Arctic warming. Using the AIRS temperature, moisture and surface data, we found that the Arctic surface moisture flux (SMF) had increased by 7% during 2003-2013 (18 W/m2 equivalent in latent heat), mostly in spring and fall near the Arctic coastal seas where large sea ice reduction and sea surface temperature (SST) increase were observed. The increase in Arctic SMF correlated well with the increases in total atmospheric column water vapor and low-level clouds, when compared to CALIPSO cloud observations. It has been challenging for climate models to reliably determine Arctic cloud radiative forcing (CRF). Using the regional climate model HIRHAM5 and assuming a more efficient Bergeron-Findeisen process with generalized subgrid-scale variability for total water content, we were able to produce a cloud distribution that is more consistent with the CloudSat/CALIPSO observations. More importantly, the modified schemes decrease (increase) the cloud water (ice) content in mixed-phase clouds, which help to improve the modeled CRF and energy budget at the surface, because of the dominant role of the liquid water in CRF. Yet, the coupling between Arctic low clouds and the surface is complex and has strong impacts on ABL. Studying GPS/COSMIC radio occultation (RO) refractivity profiles in the Arctic coldest and driest months, we successfully derived ABL inversion height and surface-based inversion (SBI) frequency, and they were anti-correlated over the Arctic Ocean. For the late summer and early fall season, we further analyzed Japanese R/V Mirai ship measurements and found that the open-ocean surface sensible heat flux (SSHF) can explain 10 % of the ABL height variability, whereas mechanisms such as cloud

  18. Aerosol indirect effects on the nighttime Arctic Ocean surface from thin, predominantly liquid clouds

    Directory of Open Access Journals (Sweden)

    L. M. Zamora

    2017-06-01

    Full Text Available Aerosol indirect effects have potentially large impacts on the Arctic Ocean surface energy budget, but model estimates of regional-scale aerosol indirect effects are highly uncertain and poorly validated by observations. Here we demonstrate a new way to quantitatively estimate aerosol indirect effects on a regional scale from remote sensing observations. In this study, we focus on nighttime, optically thin, predominantly liquid clouds. The method is based on differences in cloud physical and microphysical characteristics in carefully selected clean, average, and aerosol-impacted conditions. The cloud subset of focus covers just ∼ 5 % of cloudy Arctic Ocean regions, warming the Arctic Ocean surface by ∼ 1–1.4 W m−2 regionally during polar night. However, within this cloud subset, aerosol and cloud conditions can be determined with high confidence using CALIPSO and CloudSat data and model output. This cloud subset is generally susceptible to aerosols, with a polar nighttime estimated maximum regionally integrated indirect cooling effect of ∼ −0.11 W m−2 at the Arctic sea ice surface (∼ 8 % of the clean background cloud effect, excluding cloud fraction changes. Aerosol presence is related to reduced precipitation, cloud thickness, and radar reflectivity, and in some cases, an increased likelihood of cloud presence in the liquid phase. These observations are inconsistent with a glaciation indirect effect and are consistent with either a deactivation effect or less-efficient secondary ice formation related to smaller liquid cloud droplets. However, this cloud subset shows large differences in surface and meteorological forcing in shallow and higher-altitude clouds and between sea ice and open-ocean regions. For example, optically thin, predominantly liquid clouds are much more likely to overlay another cloud over the open ocean, which may reduce aerosol indirect effects on the surface. Also, shallow clouds over

  19. CubeSat Constellation Cloud Winds(C3Winds) A New Wind Observing System to Study Mesoscale Cloud Dynamics and Processes

    Science.gov (United States)

    Wu, D. L.; Kelly, M.A.; Yee, J.-H.; Boldt, J.; Demajistre, R.; Reynolds, E. L.; Tripoli, G. J.; Oman, L. D.; Prive, N.; Heidinger, A. K.; hide

    2016-01-01

    The CubeSat Constellation Cloud Winds (C3Winds) is a NASA Earth Venture Instrument (EV-I) concept with the primary objective to better understand mesoscale dynamics and their structures in severe weather systems. With potential catastrophic damage and loss of life, strong extratropical and tropical cyclones (ETCs and TCs) have profound three-dimensional impacts on the atmospheric dynamic and thermodynamic structures, producing complex cloud precipitation patterns, strong low-level winds, extensive tropopause folds, and intense stratosphere-troposphere exchange. Employing a compact, stereo IR-visible imaging technique from two formation-flying CubeSats, C3Winds seeks to measure and map high-resolution (2 km) cloud motion vectors (CMVs) and cloud geometric height (CGH) accurately by tracking cloud features within 5-15 min. Complementary to lidar wind observations from space, the high-resolution wind fields from C3Winds will allow detailed investigations on strong low-level wind formation in an occluded ETC development, structural variations of TC inner-core rotation, and impacts of tropopause folding events on tropospheric ozone and air quality. Together with scatterometer ocean surface winds, C3Winds will provide a more comprehensive depiction of atmosphere-boundary-layer dynamics and interactive processes. Built upon mature imaging technologies and long history of stereoscopic remote sensing, C3Winds provides an innovative, cost-effective solution to global wind observations with potential of increased diurnal sampling via CubeSat constellation.

  20. Uncertainty Estimate of Surface Irradiances Computed with MODIS-, CALIPSO-, and CloudSat-Derived Cloud and Aerosol Properties

    Science.gov (United States)

    Kato, Seiji; Loeb, Norman G.; Rutan, David A.; Rose, Fred G.; Sun-Mack, Sunny; Miller, Walter F.; Chen, Yan

    2012-07-01

    Differences of modeled surface upward and downward longwave and shortwave irradiances are calculated using modeled irradiance computed with active sensor-derived and passive sensor-derived cloud and aerosol properties. The irradiance differences are calculated for various temporal and spatial scales, monthly gridded, monthly zonal, monthly global, and annual global. Using the irradiance differences, the uncertainty of surface irradiances is estimated. The uncertainty (1σ) of the annual global surface downward longwave and shortwave is, respectively, 7 W m-2 (out of 345 W m-2) and 4 W m-2 (out of 192 W m-2), after known bias errors are removed. Similarly, the uncertainty of the annual global surface upward longwave and shortwave is, respectively, 3 W m-2 (out of 398 W m-2) and 3 W m-2 (out of 23 W m-2). The uncertainty is for modeled irradiances computed using cloud properties derived from imagers on a sun-synchronous orbit that covers the globe every day (e.g., moderate-resolution imaging spectrometer) or modeled irradiances computed for nadir view only active sensors on a sun-synchronous orbit such as Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation and CloudSat. If we assume that longwave and shortwave uncertainties are independent of each other, but up- and downward components are correlated with each other, the uncertainty in global annual mean net surface irradiance is 12 W m-2. One-sigma uncertainty bounds of the satellite-based net surface irradiance are 106 W m-2 and 130 W m-2.

  1. One-dimensional numerical modeling of Blue Jet and its impact on stratospheric chemistry

    Science.gov (United States)

    Duruisseau, F.; Thiéblemont, R.; Huret, N.

    2011-12-01

    In the stratosphere the ozone layer is very sensitive to the NOx abundance. The ionisation of N2 and O2 molecules by TLE's (Transient Luminous Events) is a source of NOx which is currently not well quantified and could act as a loss of ozone. In this study a one dimensional explicit parameterization of a Blue-Jet propagation based on that proposed by Raizer et al. (2006 and 2007) has been developed. This parameterization considers Blue-Jet as a streamer initiated by a bidirectional leader discharge, emerging from the anvil and sustained by moderate cloud charge. The streamer growth varies with the electrical field induced by initial cloud charge and the initial altitude. This electrical parameterization and the chemical mechanisms associated with the discharge have been implemented into a detailed chemical model of stratospheric ozone including evolution of nitrogen, chlorine and bromine species. We will present several tests performed to validate the electrical code and evaluate the propagation velocity and the maximum altitude attains by the blue jet as a function of electrical parameters. The results obtained giving the spatiotemporal evolution of the electron density are then used to initiate the specific chemistry associated with the Blue Jet. Preliminary results on the impact of such discharge on the ozone content and the whole stratospheric system will be presented.

  2. Towards a Theory of Tropical/Midlatitude Mass Exchange from the Earth's Surface through the Stratosphere

    Science.gov (United States)

    Hartley, Dana

    1998-01-01

    The main findings of this research project have been the following: (1) there is a significant feedback from the stratosphere on tropospheric dynamics, and (2) a detailed analysis of the interaction between tropical and polar wave breaking in controlling stratospheric mixing. Two papers are were written and are included. The first paper is titled, "A New Perspective on the Dynamical Link Between the Stratosphere and Troposphere." Atmospheric processes of tropospheric origin can perturb the stratosphere, but direct feedback in the opposite direction is usually assumed to be negligible, despite the troposphere's sensitivity to changes in the release of wave activity into the stratosphere. Here, however, we present evidence that such a feedback exists and can be significant. We find that if the wintertime Arctic polar stratospheric vortex is distorted, either by waves propagating upward from the troposphere or by eastward-travelling stratospheric waves, then there is a concomitant redistribution of stratospheric potential vorticity that induces perturbations in key meteorological fields in the upper troposphere. The feedback is large despite the much greater mass of the troposphere: it can account for up to half of the geopotential height anomaly at the tropopause. Although the relative strength of the feedback is partly due to a cancellation between contributions to these anomalies from lower altitudes, our results imply that stratospheric dynamics and its feedback on the troposphere are more significant for climate modelling and data assimilation than was previously assumed. The second article is titled "Diagnosing the Polar Excitation of Subtropical Waves in the Stratosphere". The poleward migration of planetary scale tongues of subtropical air has often been associated with intense polar vortex disturbances in the stratosphere. This question of vortex influence is reexamined from a potential vorticity (PV) perspective. Anomalous geopotential height and wind fields

  3. A climatology of polar stratospheric cloud composition between 2002 and 2012 based on MIPAS/Envisat observations

    Science.gov (United States)

    Spang, Reinhold; Hoffmann, Lars; Müller, Rolf; Grooß, Jens-Uwe; Tritscher, Ines; Höpfner, Michael; Pitts, Michael; Orr, Andrew; Riese, Martin

    2018-04-01

    The Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) instrument aboard the European Space Agency (ESA) Envisat satellite operated from July 2002 to April 2012. The infrared limb emission measurements provide a unique dataset of day and night observations of polar stratospheric clouds (PSCs) up to both poles. A recent classification method for PSC types in infrared (IR) limb spectra using spectral measurements in different atmospheric window regions has been applied to the complete mission period of MIPAS. The method uses a simple probabilistic classifier based on Bayes' theorem with a strong independence assumption on a combination of a well-established two-colour ratio method and multiple 2-D probability density functions of brightness temperature differences. The Bayesian classifier distinguishes between solid particles of ice, nitric acid trihydrate (NAT), and liquid droplets of supercooled ternary solution (STS), as well as mixed types. A climatology of MIPAS PSC occurrence and specific PSC classes has been compiled. Comparisons with results from the classification scheme of the spaceborne lidar Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) on the Cloud-Aerosol-Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite show excellent correspondence in the spatial and temporal evolution for the area of PSC coverage (APSC) even for each PSC class. Probability density functions of the PSC temperature, retrieved for each class with respect to equilibrium temperature of ice and based on coincident temperatures from meteorological reanalyses, are in accordance with the microphysical knowledge of the formation processes with respect to temperature for all three PSC types.This paper represents unprecedented pole-covering day- and nighttime climatology of the PSC distributions and their composition of different particle types. The dataset allows analyses on the temporal and spatial development of the PSC formation process over

  4. A climatology of polar stratospheric cloud composition between 2002 and 2012 based on MIPAS/Envisat observations

    Directory of Open Access Journals (Sweden)

    R. Spang

    2018-04-01

    Full Text Available The Michelson Interferometer for Passive Atmospheric Sounding (MIPAS instrument aboard the European Space Agency (ESA Envisat satellite operated from July 2002 to April 2012. The infrared limb emission measurements provide a unique dataset of day and night observations of polar stratospheric clouds (PSCs up to both poles. A recent classification method for PSC types in infrared (IR limb spectra using spectral measurements in different atmospheric window regions has been applied to the complete mission period of MIPAS. The method uses a simple probabilistic classifier based on Bayes' theorem with a strong independence assumption on a combination of a well-established two-colour ratio method and multiple 2-D probability density functions of brightness temperature differences. The Bayesian classifier distinguishes between solid particles of ice, nitric acid trihydrate (NAT, and liquid droplets of supercooled ternary solution (STS, as well as mixed types. A climatology of MIPAS PSC occurrence and specific PSC classes has been compiled. Comparisons with results from the classification scheme of the spaceborne lidar Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP on the Cloud-Aerosol-Lidar and Infrared Pathfinder Satellite Observations (CALIPSO satellite show excellent correspondence in the spatial and temporal evolution for the area of PSC coverage (APSC even for each PSC class. Probability density functions of the PSC temperature, retrieved for each class with respect to equilibrium temperature of ice and based on coincident temperatures from meteorological reanalyses, are in accordance with the microphysical knowledge of the formation processes with respect to temperature for all three PSC types.This paper represents unprecedented pole-covering day- and nighttime climatology of the PSC distributions and their composition of different particle types. The dataset allows analyses on the temporal and spatial development of the PSC formation

  5. DETERMINING REFLECTANCE SPECTRA OF SURFACES AND CLOUDS ON EXOPLANETS

    Energy Technology Data Exchange (ETDEWEB)

    Cowan, Nicolas B.; Strait, Talia E., E-mail: n-cowan@northwestern.edu [Center for Interdisciplinary Exploration and Research in Astrophysics (CIERA), Northwestern University, 2131 Tech Dr., IL 60208 (United States)

    2013-03-01

    Planned missions will spatially resolve temperate terrestrial planets from their host star. Although reflected light from such a planet encodes information about its surface, it has not been shown how to establish surface characteristics of a planet without assuming known surfaces to begin with. We present a reanalysis of disk-integrated, time-resolved, multiband photometry of Earth obtained by the Deep Impact spacecraft as part of the EPOXI Mission of Opportunity. We extract reflectance spectra of clouds, ocean, and land without a priori knowledge of the numbers or colors of these surfaces. We show that the inverse problem of extracting surface spectra from such data is a novel and extreme instance of spectral unmixing, a well-studied problem in remote sensing. Principal component analysis is used to determine an appropriate number of model surfaces with which to interpret the data. Shrink-wrapping a simplex to the color excursions of the planet yields a conservative estimate of the planet's endmember spectra. The resulting surface maps are unphysical, however, requiring negative or larger-than-unity surface coverage at certain locations. Our ''rotational unmixing'' supersedes the endmember analysis by simultaneously solving for the surface spectra and their geographical distributions on the planet, under the assumption of diffuse reflection and known viewing geometry. We use a Markov Chain Monte Carlo to determine best-fit parameters and their uncertainties. The resulting albedo spectra are similar to clouds, ocean, and land seen through a Rayleigh-scattering atmosphere. This study suggests that future direct-imaging efforts could identify and map unknown surfaces and clouds on exoplanets.

  6. Stratospheric sulfate from the Gareloi eruption, 1980: Contribution to the ''ambient'' aerosol by a poorly documented volcanic eruption

    International Nuclear Information System (INIS)

    Sedlacek, W.A.; Mroz, E.J.; Heiken, G.

    1981-01-01

    While sampling stratospheric aerosols during July--August 1980 a plume of ''fresh'' volcanic debris was observed in the Northern hemisphere. The origin of this material seems to be a poorly documented explosive eruption of Gareloi valcano in the Aleutian Islands. The debris was sampled at an altitude of 19.2 km: almost twice the height of observed eruption clouds. Such remote, unobserved or poorly documented eruptions may be a source that helps maintain the ''ambient'' stratospheric aerosol background

  7. Mortality tradeoff between air quality and skin cancer from changes in stratospheric ozone

    Science.gov (United States)

    Eastham, Sebastian D.; Keith, David W.; Barrett, Steven R. H.

    2018-03-01

    Skin cancer mortality resulting from stratospheric ozone depletion has been widely studied. Similarly, there is a deep body of literature on surface ozone and its health impacts, with modeling and observational studies demonstrating that surface ozone concentrations can be increased when stratospheric air mixes to the Earth’s surface. We offer the first quantitative estimate of the trade-off between these two effects, comparing surface air quality benefits and UV-related harms from stratospheric ozone depletion. Applying an idealized ozone loss term in the stratosphere of a chemistry-transport model for modern-day conditions, we find that each Dobson unit of stratospheric ozone depletion results in a net decrease in the global annual mortality rate of ~40 premature deaths per billion population (d/bn/DU). The impacts are spatially heterogeneous in sign and magnitude, composed of a reduction in premature mortality rate due to ozone exposure of ~80 d/bn/DU concentrated in Southeast Asia, and an increase in skin cancer mortality rate of ~40 d/bn/DU, mostly in Western Europe. This is the first study to quantify air quality benefits of stratospheric ozone depletion, and the first to find that marginal decreases in stratospheric ozone around modern-day values could result in a net reduction in global mortality due to competing health impact pathways. This result, which is subject to significant methodological uncertainty, highlights the need to understand the health and environmental trade-offs involved in policy decisions regarding anthropogenic influences on ozone chemistry over the 21st century.

  8. Comparison of Monthly Mean Cloud Fraction and Cloud Optical depth Determined from Surface Cloud Radar, TOVS, AVHRR, and MODIS over Barrow, Alaska

    Science.gov (United States)

    Uttal, Taneil; Frisch, Shelby; Wang, Xuan-Ji; Key, Jeff; Schweiger, Axel; Sun-Mack, Sunny; Minnis, Patrick

    2005-01-01

    A one year comparison is made of mean monthly values of cloud fraction and cloud optical depth over Barrow, Alaska (71 deg 19.378 min North, 156 deg 36.934 min West) between 35 GHz radar-based retrievals, the TOVS Pathfinder Path-P product, the AVHRR APP-X product, and a MODIS based cloud retrieval product from the CERES-Team. The data sets represent largely disparate spatial and temporal scales, however, in this paper, the focus is to provide a preliminary analysis of how the mean monthly values derived from these different data sets compare, and determine how they can best be used separately, and in combination to provide reliable estimates of long-term trends of changing cloud properties. The radar and satellite data sets described here incorporate Arctic specific modifications that account for cloud detection challenges specific to the Arctic environment. The year 2000 was chosen for this initial comparison because the cloud radar data was particularly continuous and reliable that year, and all of the satellite retrievals of interest were also available for the year 2000. Cloud fraction was chosen as a comparison variable as accurate detection of cloud is the primary product that is necessary for any other cloud property retrievals. Cloud optical depth was additionally selected as it is likely the single cloud property that is most closely correlated to cloud influences on surface radiation budgets.

  9. Temporal Changes in the Observed Relationship between Cloud Cover and Surface Air Temperature.

    Science.gov (United States)

    Sun, Bomin; Groisman, Pavel Ya.; Bradley, Raymond S.; Keimig, Frank T.

    2000-12-01

    The relationship between cloud cover and near-surface air temperature and its decadal changes are examined using the hourly synoptic data for the past four to six decades from five regions of the Northern Hemisphere: Canada, the United States, the former Soviet Union, China, and tropical islands of the western Pacific. The authors define the normalized cloud cover-surface air temperature relationship, NOCET or dT/dCL, as a temperature anomaly with a unit (one-tenth) deviation of total cloud cover from its average value. Then mean monthly NOCET time series (night- and daytime, separately) are area-averaged and parameterized as functions of surface air humidity and snow cover. The day- and nighttime NOCET variations are strongly anticorrelated with changes in surface humidity. Furthermore, the daytime NOCET changes are positively correlated to changes in snow cover extent. The regionally averaged nighttime NOCET varies from 0.05 K tenth1 in the wet Tropics to 1.0 K tenth1 at midlatitudes in winter. The daytime regional NOCET ranges from 0.4 K tenth1 in the Tropics to 0.7 K tenth1 at midlatitudes in winter.The authors found a general strengthening of a daytime surface cooling during the post-World War II period associated with cloud cover over the United States and China, but a minor reduction of this cooling in higher latitudes. Furthermore, since the 1970s, a prominent increase in atmospheric humidity has significantly weakened the effectiveness of the surface warming (best seen at nighttime) associated with cloud cover.The authors apportion the spatiotemporal field of interactions between total cloud cover and surface air temperature into a bivariate relationship (described by two equations, one for daytime and one for nighttime) with surface air humidity and snow cover and two constant factors. These factors are invariant in space and time domains. It is speculated that they may represent empirical estimates of the overall cloud cover effect on the surface air

  10. Temperature thresholds for chlorine activation and ozone loss in the polar stratosphere

    Energy Technology Data Exchange (ETDEWEB)

    Drdla, K. [NASA Ames Research Center, Moffett Field, CA (United States); Mueller, R. [Forschungszentrum Juelich (DE). Inst. of Energy and Climate Research (IEK-7)

    2012-07-01

    Low stratospheric temperatures are known to be responsible for heterogeneous chlorine activation that leads to polar ozone depletion. Here, we discuss the temperature threshold below which substantial chlorine activation occurs. We suggest that the onset of chlorine activation is dominated by reactions on cold binary aerosol particles, without the formation of polar stratospheric clouds (PSCs), i.e. without any significant uptake of HNO{sub 3} from the gas phase. Using reaction rates on cold binary aerosol in a model of stratospheric chemistry, a chlorine activation threshold temperature, T{sub ACL}, is derived. At typical stratospheric conditions, T{sub ACL} is similar in value to T{sub NAT} (within 1-2 K), the highest temperature at which nitric acid trihydrate (NAT) can exist. T{sub NAT} is still in use to parameterise the threshold temperature for the onset of chlorine activation. However, perturbations can cause T{sub ACL} to differ from T{sub NAT}: T{sub ACL} is dependent upon H{sub 2} O and potential temperature, but unlike T{sub NAT} is not dependent upon HNO3. Furthermore, in contrast to T{sub NAT}, T{sub ACL} is dependent upon the stratospheric sulfate aerosol loading and thus provides a means to estimate the impact on polar ozone of strong volcanic eruptions and some geo-engineering options, which are discussed. A parameterisation of T{sub ACL} is provided here, allowing it to be calculated for low solar elevation (or high solar zenith angle) over a comprehensive range of stratospheric conditions. Considering T{sub ACL} as a proxy for chlorine activation cannot replace a detailed model calculation, and polar ozone loss is influenced by other factors apart from the initial chlorine activation. However, T{sub ACL} provides a more accurate description of the temperature conditions necessary for chlorine activation and ozone loss in the polar stratosphere than T{sub NAT}. (orig.)

  11. Evaluation of the Cloud Fields in the UK Met Office HadGEM3-UKCA Model Using the CCCM Satellite Data Product to Advance Our Understanding of the Influence of Clouds on Tropospheric Composition and Chemistry

    Science.gov (United States)

    Varma, Sunil; Voulgarakis, Apostolos; Liu, Hongyu; Crawford, James H.; White, James

    2016-01-01

    To determine the role of clouds in driving inter-annual and inter-seasonal variability of trace gases in the troposphere and lower stratosphere with a particular focus on the importance of cloud modification of photolysis. To evaluate the cloud fields and their vertical distribution in the HadGEM3 model utilizing CCCM, a unique 3-D cloud data product merged from multiple A-Train satellites (CERES, CloudSat, CALIPSO, and MODIS) developed at the NASA Langley Research Center.

  12. Effects of intense stratospheric ionisation events

    International Nuclear Information System (INIS)

    Reid, G.C.; McAfee, J.R.; Crutzen, P.J.

    1978-01-01

    High levels of ionising radiation in the Earth's stratosphere will lead to increased concentrations of nitrogen oxides and decreased concentrations of ozone. Changes in the surface environment will include an increased level, of biologically harmful UV radiation, caused by the ozone depletion, and a decreased level of visible solar radiation, due to the presence of major enhancements in the stratospheric concentration of nitrogen dioxide. These changes have been studied quantitatively, using the passage of the Solar System through a supernova remnant shell as an example. Some of the potential environmental changes are a substantial global cooling, abnormally dry conditions, a reduction in global photosynthesis and a large increase in the flux of atmospheric fixed nitrogen to the surface of the Earth. Such events might have been the cause of mass extinctions in the distant past. (Author)

  13. Stratospheric Platforms for Monitoring Purposes

    International Nuclear Information System (INIS)

    Konigorski, D.; Gratzel, U.; Obersteiner, M.; Schneidereit, M.

    2010-01-01

    Stratospheric platforms are emerging systems based on challenging technology. Goal is to create a platform, payload, and mission design which is able to complement satellite services on a local scale. Applications are close to traditional satellite business in telecommunication, navigation, science, and earth observation and include for example mobile telecommunications, navigation augmentation, atmospheric research, or border control. Stratospheric platforms could potentially support monitoring activities related to safeguards, e.g. by imagery of surfaces, operational conditions of nuclear facilities, and search for undeclared nuclear activities. Stratospheric platforms are intended to be flown in an altitude band between 16 and 30 km, above 16-20 km to take advantage of usually lower winds facilitating station keeping, below 30 km to limit the challenges to achieve a reasonable payload at acceptable platform sizes. Stratospheric platforms could substitute satellites which are expensive and lack upgrade capabilities for new equipment. Furthermore they have practically an unlimited time over an area of interest. It is intended to keep the platforms operational and maintenance free on a 24/7 basis with an average deployment time of 3 years. Geostationary satellites lack resolution. Potential customers like Armed Forces, National Agencies and commercial customers have indicated interest in the use of stratospheric platforms. Governmental entities are looking for cheaper alternatives to communications and surveillance satellites and stratospheric platforms could offer the following potential advantages: Lower operational cost than satellite or UAV (Unmanned Aerial Vehicles) constellation (fleet required); Faster deployment than satellite constellation; Repositioning capability and ability to loiter as required; Persistent long-term real-time services over a fairly large regional spot; Surge capability: Able to extend capability (either monitoring or communications

  14. On the cryogenic removal of NOy from the Antarctic polar stratosphere

    Directory of Open Access Journals (Sweden)

    S. Smyshlyaev

    2003-06-01

    Full Text Available We review current knowledge about the annual cycle of transport of nitrogen oxides to, and removal from, the polar stratosphere, with particular attention to Antarctica where the annual winter denitrifi cation process is both regular in occurrence and severe in effect. Evidence for a large downward fl ux of NOy from the mesosphere to the stratosphere, fi rst seen briefl y in the Limb Infrared Monitor of the Stratosphere (LIMS data from the Arctic winter of 1978-1979, has been found during the 1990s in both satellite and ground-based observations, though this still seems to be omitted from many atmospheric models. When incorporated in the Stony Brook- St. Petersburg two dimensional (2D transport and chemistry model, more realistic treatment of the NOy fl ux, along with sulfate transport from the mesosphere, sulfate aerosol formation where temperature is favorable, and the inclusion of a simple ion-cluster reaction, leads to good agreement with observed HNO3 formation in the mid-winter middle to upper stratosphere. To further emphasize the importance of large fl uxes of thermospheric and mesospheric NOy into the polar stratosphere, we have used observations, supplemented with model calculations, to defi ne new altitude dependent correlation curves between N2O and NOy. These are more suitable than those previously used in the literature to represent conditions within the Antarctic vortex region prior to and during denitrifi cation by Polar Stratospheric Cloud (PSC particles. Our NOy -N2O curves lead to a 40% increase in the average amount of NOy removed during the Antarctic winter with respect to estimates calculated using NOy-N2O curves from the Atmospheric Trace Molecule Spectroscopy (ATMOS/ATLAS-3 data set.

  15. Clouds, radiation, and the diurnal cycle of sea surface temperature in the tropical Western Pacific

    Energy Technology Data Exchange (ETDEWEB)

    Webster, P.J.; Clayson, C.A.; Curry, J.A. [Univ. of Colorado, Boulder, CO (United States)

    1996-04-01

    In the tropical Western Pacific (TWP) Ocean, the clouds and the cloud-radiation feedback can only be understood in the context of air/sea interactions and the ocean mixed layer. Considerable interest has been shown in attempting to explain why sea surface temperature (SST) rarely rises above 30{degrees}C, and gradients of the SST. For the most part, observational studies that address this issue have been conducted using monthly cloud and SST data, and the focus has been on intraseasonal and interannual time scales. For the unstable tropical atmosphere, using monthly averaged data misses a key feedback between clouds and SST that occurs on the cloud-SST coupling time scale, which was estimated to be 3-6 days for the unstable tropical atmosphere. This time scale is the time needed for a change in cloud properties, due to the change of ocean surface evaporation caused by SST variation, to feed back to the SST variation, to feed back to the SST through its effect on the surface heat flux. This paper addresses the relationship between clouds, surface radiation flux and SST of the TWP ocean over the diurnal cycle.

  16. Convectively Driven Tropopause-Level Cooling and Its Influences on Stratospheric Moisture

    Science.gov (United States)

    Kim, Joowan; Randel, William J.; Birner, Thomas

    2018-01-01

    Characteristics of the tropopause-level cooling associated with tropical deep convection are examined using CloudSat radar and Constellation Observing System for Meteorology, Ionosphere and Climate (COSMIC) GPS radio occultation measurements. Extreme deep convection is sampled based on the cloud top height (>17 km) from CloudSat, and colocated temperature profiles from COSMIC are composited around the deep convection. Response of moisture to the tropopause-level cooling is also examined in the upper troposphere and lower stratosphere using microwave limb sounder measurements. The composite temperature shows an anomalous warming in the troposphere and a significant cooling near the tropopause (at 16-19 km) when deep convection occurs over the western Pacific, particularly during periods with active Madden-Julian Oscillation (MJO). The composite of the tropopause cooling has a large horizontal scale ( 6,000 km in longitude) with minimum temperature anomaly of -2 K, and it lasts more than 2 weeks with support of mesoscale convective clusters embedded within the envelope of the MJO. The water vapor anomalies show strong correlation with the temperature anomalies (i.e., dry anomaly in the cold anomaly), showing that the convectively driven tropopause cooling actively dehydrate the lower stratosphere in the western Pacific region. The moisture is also affected by anomalous Matsuno-Gill-type circulation associated with the cold anomaly, in which dry air spreads over a wide range in the tropical tropopause layer (TTL). These results suggest that convectively driven tropopause cooling and associated transient circulation play an important role in the large-scale dehydration process in the TTL.

  17. Quantifying pollution transport from the Asian monsoon anticyclone into the lower stratosphere

    Directory of Open Access Journals (Sweden)

    F. Ploeger

    2017-06-01

    Full Text Available Pollution transport from the surface to the stratosphere within the Asian monsoon circulation may cause harmful effects on stratospheric chemistry and climate. Here, we investigate air mass transport from the monsoon anticyclone into the stratosphere using a Lagrangian chemistry transport model. We show how two main transport pathways from the anticyclone emerge: (i into the tropical stratosphere (tropical pipe, and (ii into the Northern Hemisphere (NH extratropical lower stratosphere. Maximum anticyclone air mass fractions reach around 5 % in the tropical pipe and 15 % in the extratropical lowermost stratosphere over the course of a year. The anticyclone air mass fraction correlates well with satellite hydrogen cyanide (HCN and carbon monoxide (CO observations, confirming that pollution is transported deep into the tropical stratosphere from the Asian monsoon anticyclone. Cross-tropopause transport occurs in a vertical chimney, but with the pollutants transported quasi-horizontally along isentropes above the tropopause into the tropics and NH.

  18. Cloud Tolerance of Remote-Sensing Technologies to Measure Land Surface Temperature

    Science.gov (United States)

    Holmes, Thomas R. H.; Hain, Christopher R.; Anderson, Martha C.; Crow, Wade T.

    2016-01-01

    Conventional methods to estimate land surface temperature (LST) from space rely on the thermal infrared(TIR) spectral window and is limited to cloud-free scenes. To also provide LST estimates during periods with clouds, a new method was developed to estimate LST based on passive microwave(MW) observations. The MW-LST product is informed by six polar-orbiting satellites to create a global record with up to eight observations per day for each 0.25resolution grid box. For days with sufficient observations, a continuous diurnal temperature cycle (DTC) was fitted. The main characteristics of the DTC were scaled to match those of a geostationary TIR-LST product. This paper tests the cloud tolerance of the MW-LST product. In particular, we demonstrate its stable performance with respect to flux tower observation sites (four in Europe and nine in the United States), over a range of cloudiness conditions up to heavily overcast skies. The results show that TIR based LST has slightly better performance than MW-LST for clear-sky observations but suffers an increasing negative bias as cloud cover increases. This negative bias is caused by incomplete masking of cloud-covered areas within the TIR scene that affects many applications of TIR-LST. In contrast, for MW-LST we find no direct impact of clouds on its accuracy and bias. MW-LST can therefore be used to improve TIR cloud screening. Moreover, the ability to provide LST estimates for cloud-covered surfaces can help expand current clear-sky-only satellite retrieval products to all-weather applications.

  19. DUSTER: collection of meteoric CaO and carbon smoke particles in the upper stratosphere .

    Science.gov (United States)

    Della Corte, V.; Rietmeijer, F. J. M.; Rotundi, A.; Ferrari, M.; Palumbo, P.

    Nanometer- to micrometer-size particles present in the upper stratosphere are a mixture of terrestrial and extra-terrestrial origins. They can be extraterrestrial particles condensed after meteor ablation. Meteoric dust in bolides is occasionally deposited into the lower stratosphere around 20 km altitude. Nanometer CaO and pure carbon smoke particles were collected at 38 km altitude in the upper stratosphere in the Arctic during June 2008 using DUSTER (Dust in the Upper Stratosphere Tracking Experiment and Retrieval), a balloon-borne instrument for the non-destructive collection of solid particles between 200 nm to 40 microns. We report the collection of micron sized CaCO_3 (calcite) grains. Their morphologies show evidence of melting and condensation after vaporization suggest at temperatures of approximately 3500 K. The formation environment of the collected grains was probably a dense dust cloud formed by the disintegration of a carbonaceous meteoroid during deceleration in the Earth� atmosphere. For the first time, DUSTER collected meteor ablation products that were presumably associated with the disintegration of a bolide crossing the Earth's atmosphere. The collected mostly CaO and pure carbon nanoparticles from the debris cloud of a fireball, included: 1) intact fragments; 2) quenched melted grains; and 3) vapor phase condensation products. The DUSTER project was funded by the Italian Space Agency (ASI), PRIN2008/MIUR (Ministero dell'Istruzione dell'Universitá e della Ricerca), PNRA 2013(Piano Nazionale Ricerca Antartide). CNES graciously provided this flight opportunity. We thank E. Zona and S. Inarta at the Laboratorio di Fisica Cosmica INAF, Osservatorio Astronomico di Capodimonte-Universitá di Napoli Parthenope. F.J.M.R. was supported by grant NNX07AI39G from the NASA Cosmochemistry Program. We thank three anonymous reviewers who assisted us in introducing our new instrument.

  20. High latitude stratospheric electrical measurements in fair and foul weather under various solar conditions

    International Nuclear Information System (INIS)

    Holzworth, R.H.

    1981-01-01

    Stratospheric electric field and conductivity measurements during a wide variety of weather and solar conditions are presented. These data are all from high latitude sites in the months of either April or August. The vector electric field is determined by orthogonal double probes connected through high impedance inputs to differential electrometers. The direct conductivity measurement involves determining the relaxation time constant of the medium after refloating a shorted pair of separated probes. Vertical electric field data from several balloon flights with average duration of 18 h at ceiling in fair weather are shown to be well modeled by a simple exponential altitude dependent equation. Examples of solar flare and magnetospheric effects on stratospheric electric fields are shown. Data collected over electrified clouds and thunderstorms are presented along with a discussion of the thunderstorm related electric currents. Lightning stroke signatures in the stratosphere during a large thunderstorm are identified in the electric field data. Current surges through the stratosphere due to DC currents as well as the sferic are calculated. In nearly 1000 h of balloon data no direct solar influence is identified in these data except during major flares. (author)

  1. SAGE II observations of a previously unreported stratospheric volcanic aerosol cloud in the northern polar summer of 1990

    Science.gov (United States)

    Yue, Glenn K.; Veiga, Robert E.; Wang, Pi-Huan

    1994-01-01

    Analysis of aerosol extinction profiles obtained by the spaceborne SAGE II sensor reveals that there was an anomalous increase of aerosol extinction below 18.5 km at latitudes poleward of 50 deg N from July 28 to September 9, 1990. This widespread increase of aerosol extinction in the lower stratosphere was apparently due to a remote high-latitude volcanic eruption that has not been reported to date. The increase in stratospheric optical depth in the northern polar region was about 50% in August and had diminished by October 1990. This eruption caused an increase in stratospheric aerosol mass of about 0.33 x 10(exp 5) tons, assuming the aerosol was composed of sulfuric acid and water.

  2. Cloud tolerance of remote sensing technologies to measure land surface temperature

    Science.gov (United States)

    Conventional means to estimate land surface temperature (LST) from space relies on the thermal infrared (TIR) spectral window and is limited to cloud-free scenes. To also provide LST estimates during periods with clouds, a new method was developed to estimate LST based on passive microwave (MW) obse...

  3. Lidar measurements of ozone and aerosol distributions during the 1992 airborne Arctic stratospheric expedition

    Science.gov (United States)

    Browell, Edward V.; Butler, Carolyn F.; Fenn, Marta A.; Grant, William B.; Ismail, Syed; Carter, Arlen F.

    1994-01-01

    The NASA Langley airborne differential absorption lidar system was operated from the NASA Ames DC-8 aircraft during the 1992 Airborne Arctic Stratospheric Expedition to investigate the distribution of stratospheric aerosols and ozone (O3) across the Arctic vortex from January to March 1992. Aerosols from the Mt. Pinatubo eruption were found outside and inside the Arctic vortex with distinctly different scattering characteristics and spatial distributions in the two regions. The aerosol and O3 distributions clearly identified the edge of the vortex and provided additional information on vortex dynamics and transport processes. Few polar stratospheric clouds were observed during the AASE-2; however, those that were found had enhanced scattering and depolarization over the background Pinatubo aerosols. The distribution of aerosols inside the vortex exhibited relatively minor changes during the AASE-2. Ozone depletion inside the vortex as limited to less than or equal to 20 percent in the altitude region from 15-20 km.

  4. Stratospheric ozone: History and concepts and interactions with climate

    Directory of Open Access Journals (Sweden)

    Bekki S.

    2009-02-01

    Full Text Available Although in relatively low concentration of a few molecules per million of e e air molecules, atmospheric ozone (trioxygen O3 is essential to sustaining life on the surface of the Earth. Indeed, by absorbing solar radiation between 240 and 320 nm, it shields living organisms including humans from the very harmful ultraviolet radiation UV-B. About 90% of the ozone resides in the stratosphere, a region that extends from the tropopause, whose altitude ranges from 7 km at the poles to 17 km in the tropics, to the stratopause located at about 50 km altitude. Stratospheric ozone is communally referred as the « ozone layer ». Unlike the atmosphere surrounding it, the stratosphere is vertically stratified and stable because the temperature increases with height within it. This particularity originates from heating produced by the absorption of UV radiation by stratospheric ozone. The present chapter describes the main mechanisms that govern the natural balance of ozone in the stratosphere, and its disruption under the influence of human activities.

  5. SGP Cloud and Land Surface Interaction Campaign (CLASIC): Measurement Platforms

    Energy Technology Data Exchange (ETDEWEB)

    MA Miller; R Avissar; LK Berg; SA Edgerton; ML Fischer; TJ Jackson; B. Kustas; PJ Lamb; G McFarquhar; Q Min; B Schmid; MS Torn; DD Tuner

    2007-06-01

    The Cloud and Land Surface Interaction Campaign (CLASIC) will be conducted from June 8 to June 30, 2007, at the U.S. Department of Energy’s Atmospheric Radiation Measurement (ARM) Climate Research Facility (ACRF) Southern Great Plains (SGP) site. Data will be collected using eight aircraft equipped with a variety of specialized sensors, four specially instrumented surface sites, and two prototype surface radar systems. The architecture of CLASIC includes a high-altitude surveillance aircraft and enhanced vertical thermodynamic and wind profile measurements that will characterize the synoptic scale structure of the clouds and the land surface within the ACRF SGP site. Mesoscale and microscale structures will be sampled with a variety of aircraft, surface, and radar observations. An overview of the measurement platforms that will be used during the CLASIC are described in this report. The coordination of measurements, especially as it relates to aircraft flight plans, will be discussed in the CLASIC Implementation Plan.

  6. Accuracy and precision of polar lower stratospheric temperatures from reanalyses evaluated from A-Train CALIOP and MLS, COSMIC GPS RO, and the equilibrium thermodynamics of supercooled ternary solutions and ice clouds

    Science.gov (United States)

    Lambert, Alyn; Santee, Michelle L.

    2018-02-01

    We investigate the accuracy and precision of polar lower stratospheric temperatures (100-10 hPa during 2008-2013) reported in several contemporary reanalysis datasets comprising two versions of the Modern-Era Retrospective analysis for Research and Applications (MERRA and MERRA-2), the Japanese 55-year Reanalysis (JRA-55), the European Centre for Medium-Range Weather Forecasts (ECMWF) interim reanalysis (ERA-I), and the National Oceanic and Atmospheric Administration (NOAA) National Centers for Environmental Prediction (NCEP) Climate Forecast System Reanalysis (NCEP-CFSR). We also include the Goddard Earth Observing System model version 5.9.1 near-real-time analysis (GEOS-5.9.1). Comparisons of these datasets are made with respect to retrieved temperatures from the Aura Microwave Limb Sounder (MLS), Constellation Observing System for Meteorology, Ionosphere and Climate (COSMIC) Global Positioning System (GPS) radio occultation (RO) temperatures, and independent absolute temperature references defined by the equilibrium thermodynamics of supercooled ternary solutions (STSs) and ice clouds. Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) observations of polar stratospheric clouds are used to determine the cloud particle types within the Aura MLS geometric field of view. The thermodynamic calculations for STS and the ice frost point use the colocated MLS gas-phase measurements of HNO3 and H2O. The estimated bias and precision for the STS temperature reference, over the 68 to 21 hPa pressure range, are 0.6-1.5 and 0.3-0.6 K, respectively; for the ice temperature reference, they are 0.4 and 0.3 K, respectively. These uncertainties are smaller than those estimated for the retrieved MLS temperatures and also comparable to GPS RO uncertainties (bias 0.7 K) in the same pressure range. We examine a case study of the time-varying temperature structure associated with layered ice clouds formed by orographic gravity waves forced by flow over the Palmer Peninsula and

  7. Upper Troposphere Lower Stratosphere structure during convective systems using GPS radio occultations

    DEFF Research Database (Denmark)

    Biondi, Riccardo

    The deep convective systems play a fundamental role in atmospheric circulation and climate. Thunderstorms and meso-scale convective systems produce fast vertical transport, redistributing water vapor and trace gases and influencing the thermal structure of the upper troposphere and lower...... stratosphere (UTLS) contributing to the troposphere-stratosphere transport and affecting the Earth global circulation and the climate changes. The Global Positioning System (GPS) Radio Occultation (RO) technique enables measurement of atmospheric density structure in any meteorological condition...... to the analysis of tropical storms for the future mission ACES will also be evaluated. Using data from the past and ongoing GPS RO missions we have defined an algorithm to detect the clouds top of the convective systems and their thermal structure. Other satellite and in-situ measurements co-located with GPS ROs...

  8. TH-AB-202-08: A Robust Real-Time Surface Reconstruction Method On Point Clouds Captured From a 3D Surface Photogrammetry System

    International Nuclear Information System (INIS)

    Liu, W; Sawant, A; Ruan, D

    2016-01-01

    Purpose: Surface photogrammetry (e.g. VisionRT, C-Rad) provides a noninvasive way to obtain high-frequency measurement for patient motion monitoring in radiotherapy. This work aims to develop a real-time surface reconstruction method on the acquired point clouds, whose acquisitions are subject to noise and missing measurements. In contrast to existing surface reconstruction methods that are usually computationally expensive, the proposed method reconstructs continuous surfaces with comparable accuracy in real-time. Methods: The key idea in our method is to solve and propagate a sparse linear relationship from the point cloud (measurement) manifold to the surface (reconstruction) manifold, taking advantage of the similarity in local geometric topology in both manifolds. With consistent point cloud acquisition, we propose a sparse regression (SR) model to directly approximate the target point cloud as a sparse linear combination from the training set, building the point correspondences by the iterative closest point (ICP) method. To accommodate changing noise levels and/or presence of inconsistent occlusions, we further propose a modified sparse regression (MSR) model to account for the large and sparse error built by ICP, with a Laplacian prior. We evaluated our method on both clinical acquired point clouds under consistent conditions and simulated point clouds with inconsistent occlusions. The reconstruction accuracy was evaluated w.r.t. root-mean-squared-error, by comparing the reconstructed surfaces against those from the variational reconstruction method. Results: On clinical point clouds, both the SR and MSR models achieved sub-millimeter accuracy, with mean reconstruction time reduced from 82.23 seconds to 0.52 seconds and 0.94 seconds, respectively. On simulated point cloud with inconsistent occlusions, the MSR model has demonstrated its advantage in achieving consistent performance despite the introduced occlusions. Conclusion: We have developed a real

  9. Dynamical response of the Arctic winter stratosphere to global warming

    Science.gov (United States)

    Karpechko, A.; Manzini, E.

    2017-12-01

    Climate models often simulate dynamical warming of the Arctic stratosphere as a response to global warming in association with a strengthening of the deep branch of the Brewer-Dobson circulation; however until now, no satisfactory mechanism for such a response has been suggested. Here we investigate the role of stationary planetary waves in the dynamical response of the Arctic winter stratosphere circulation to global warming by analysing simulations performed with atmosphere-only Coupled Model Intercomparison Project Phase 5 (CMIP5) models driven by prescribed sea surface temperatures (SSTs). We focus on December-February (DJF) because this is the period when the troposphere and stratosphere are strongly coupled. When forced by increased SSTs, all the models analysed here simulate Arctic stratosphere dynamical warming, mostly due to increased upward propagation of quasi-stationary wave number 1, as diagnosed by the meridional eddy heat flux. By analysing intermodel spread in the response we show that the stratospheric warming and increased wave flux to the stratosphere correlate with the strengthening of the zonal winds in subtropics and mid-latitudes near the tropopause- a robust response to global warming. These results support previous studies of future Arctic stratosphere changes and suggest a dynamical warming of the Arctic wintertime polar vortex as the most likely response to global warming.

  10. Jupiter's Multi-level Clouds

    Science.gov (United States)

    1997-01-01

    Clouds and hazes at various altitudes within the dynamic Jovian atmosphere are revealed by multi-color imaging taken by the Near-Infrared Mapping Spectrometer (NIMS) onboard the Galileo spacecraft. These images were taken during the second orbit (G2) on September 5, 1996 from an early-morning vantage point 2.1 million kilometers (1.3 million miles) above Jupiter. They show the planet's appearance as viewed at various near-infrared wavelengths, with distinct differences due primarily to variations in the altitudes and opacities of the cloud systems. The top left and right images, taken at 1.61 microns and 2.73 microns respectively, show relatively clear views of the deep atmosphere, with clouds down to a level about three times the atmospheric pressure at the Earth's surface.By contrast, the middle image in top row, taken at 2.17 microns, shows only the highest altitude clouds and hazes. This wavelength is severely affected by the absorption of light by hydrogen gas, the main constituent of Jupiter's atmosphere. Therefore, only the Great Red Spot, the highest equatorial clouds, a small feature at mid-northern latitudes, and thin, high photochemical polar hazes can be seen. In the lower left image, at 3.01 microns, deeper clouds can be seen dimly against gaseous ammonia and methane absorption. In the lower middle image, at 4.99 microns, the light observed is the planet's own indigenous heat from the deep, warm atmosphere.The false color image (lower right) succinctly shows various cloud and haze levels seen in the Jovian atmosphere. This image indicates the temperature and altitude at which the light being observed is produced. Thermally-rich red areas denote high temperatures from photons in the deep atmosphere leaking through minimal cloud cover; green denotes cool temperatures of the tropospheric clouds; blue denotes cold of the upper troposphere and lower stratosphere. The polar regions appear purplish, because small-particle hazes allow leakage and reflectivity

  11. Stratospheric impact on tropospheric ozone variability and trends: 1990–2009

    Directory of Open Access Journals (Sweden)

    P. G. Hess

    2013-01-01

    Full Text Available The influence of stratospheric ozone on the interannual variability and trends in tropospheric ozone is evaluated between 30 and 90° N from 1990–2009 using ozone measurements and a global chemical transport model, the Community Atmospheric Model with chemistry (CAM-chem. Long-term measurements from ozonesondes, at 150 and 500 hPa, and the Measurements of OZone and water vapour by in-service Airbus aircraft programme (MOZAIC, at 500 hPa, are analyzed over Japan, Canada, the Eastern US and Northern and Central Europe. The measurements generally emphasize northern latitudes, although the simulation suggests that measurements over the Canadian, Northern and Central European regions are representative of the large-scale interannual ozone variability from 30 to 90° N at 500 hPa. CAM-chem is run with input meteorology from the National Center for Environmental Prediction; a tagging methodology is used to identify the stratospheric contribution to tropospheric ozone concentrations. A variant of the synthetic ozone tracer (synoz is used to represent stratospheric ozone. Both the model and measurements indicate that on large spatial scales stratospheric interannual ozone variability drives significant tropospheric variability at 500 hPa and the surface. In particular, the simulation and the measurements suggest large stratospheric influence at the surface sites of Mace Head (Ireland and Jungfraujoch (Switzerland as well as many 500 hPa measurement locations. Both the measurements and simulation suggest the stratosphere has contributed to tropospheric ozone trends. In many locations between 30–90° N 500 hPa ozone significantly increased from 1990–2000, but has leveled off since (from 2000–2009. The simulated global ozone budget suggests global stratosphere-troposphere exchange increased in 1998–1999 in association with a global ozone anomaly. Discrepancies between the simulated and measured ozone budget include a large underestimation of

  12. Contrasting Effects of Central Pacific and Eastern Pacific El Nino on Stratospheric Water Vapor

    Science.gov (United States)

    Garfinkel, Chaim I.; Hurwitz, Margaret M.; Oman, Luke D.; Waugh, Darryn W.

    2013-01-01

    Targeted experiments with a comprehensive chemistry-climate model are used to demonstrate that seasonality and the location of the peak warming of sea surface temperatures dictate the response of stratospheric water vapor to El Nino. In spring, El Nino events in which sea surface temperature anomalies peak in the eastern Pacific lead to a warming at the tropopause above the warm pool region, and subsequently to more stratospheric water vapor (consistent with previous work). However, in fall and in early winter, and also during El Nino events in which the sea surface temperature anomaly is found mainly in the central Pacific, the response is qualitatively different: temperature changes in the warm pool region are nonuniform and less water vapor enters the stratosphere. The difference in water vapor in the lower stratosphere between the two variants of El Nino approaches 0.3 ppmv, while the difference between the winter and spring responses exceeds 0.5 ppmv.

  13. Inverse modeling of cloud-aerosol interactions -- Part 1: Detailed response surface analysis

    NARCIS (Netherlands)

    Partridge, D.G.; Vrugt, J.A.; Tunved, P.; Ekman, A.M.L.; Gorea, D.; Sooroshian, A.

    2011-01-01

    New methodologies are required to probe the sensitivity of parameters describing cloud droplet activation. This paper presents an inverse modeling-based method for exploring cloud-aerosol interactions via response surfaces. The objective function, containing the difference between the measured and

  14. "Analysis of the multi-layered cloud radiative effects at the surface using A-train data"

    Science.gov (United States)

    Viudez-Mora, A.; Smith, W. L., Jr.; Kato, S.

    2017-12-01

    Clouds cover about 74% of the planet and they are an important part of the climate system and strongly influence the surface energy budget. The cloud vertical distribution has important implications in the atmospheric heating and cooling rates. Based on observations by active sensors in the A-train satellite constellation, CALIPSO [Winker et. al, 2010] and CloudSat [Stephens et. al, 2002], more than 1/3 of all clouds are multi-layered. Detection and retrieval of multi-layer cloud physical properties are needed in understanding their effects on the surface radiation budget. This study examines the sensitivity of surface irradiances to cloud properties derived from satellite sensors. Surface irradiances were computed in two different ways, one using cloud properties solely from MODerate resolution Imaging Spectroradiometer (MODIS), and the other using MODIS data supplemented with CALIPSO and CloudSat (hereafter CLCS) cloud vertical structure information [Kato et. al, 2010]. Results reveal that incorporating more precise and realistic cloud properties from CLCS into radiative transfer calculations yields improved estimates of cloud radiative effects (CRE) at the surface (CREsfc). The calculations using only MODIS cloud properties, comparisons of the computed CREsfc for 2-layer (2L) overcast CERES footprints, CLCS reduces the SW CRE by 1.5±26.7 Wm-2, increases the LW CRE by 4.1±12.7 Wm-2, and increases the net CREsfc by 0.9±46.7 Wm-2. In a subsequent analysis, we classified up to 6 different combinations of multi-layered clouds depending on the cloud top height as: High-high (HH), high-middle (HM), high-low (HL), middle-middle (MM), middle-low (ML) and low-low (LL). The 3 most frequent 2L cloud systems were: HL (56.1%), HM (22.3%) and HH (12.1%). For these cases, the computed CREsfc estimated using CLCS data presented the most significant differences when compared using only MODIS data. For example, the differences for the SW and Net CRE in the case HH was 12.3±47

  15. Modification of cirrus clouds to reduce global warming

    International Nuclear Information System (INIS)

    Mitchell, David L; Finnegan, William

    2009-01-01

    Greenhouse gases and cirrus clouds regulate outgoing longwave radiation (OLR) and cirrus cloud coverage is predicted to be sensitive to the ice fall speed which depends on ice crystal size. The higher the cirrus, the greater their impact is on OLR. Thus by changing ice crystal size in the coldest cirrus, OLR and climate might be modified. Fortunately the coldest cirrus have the highest ice supersaturation due to the dominance of homogeneous freezing nucleation. Seeding such cirrus with very efficient heterogeneous ice nuclei should produce larger ice crystals due to vapor competition effects, thus increasing OLR and surface cooling. Preliminary estimates of this global net cloud forcing are more negative than -2.8 W m -2 and could neutralize the radiative forcing due to a CO 2 doubling (3.7 W m -2 ). A potential delivery mechanism for the seeding material is already in place: the airline industry. Since seeding aerosol residence times in the troposphere are relatively short, the climate might return to its normal state within months after stopping the geoengineering experiment. The main known drawback to this approach is that it would not stop ocean acidification. It does not have many of the drawbacks that stratospheric injection of sulfur species has.

  16. Modification of cirrus clouds to reduce global warming

    Energy Technology Data Exchange (ETDEWEB)

    Mitchell, David L; Finnegan, William, E-mail: david.mitchell@dri.ed [Desert Research Institute, Reno, NV 89512-1095 (United States)

    2009-10-15

    Greenhouse gases and cirrus clouds regulate outgoing longwave radiation (OLR) and cirrus cloud coverage is predicted to be sensitive to the ice fall speed which depends on ice crystal size. The higher the cirrus, the greater their impact is on OLR. Thus by changing ice crystal size in the coldest cirrus, OLR and climate might be modified. Fortunately the coldest cirrus have the highest ice supersaturation due to the dominance of homogeneous freezing nucleation. Seeding such cirrus with very efficient heterogeneous ice nuclei should produce larger ice crystals due to vapor competition effects, thus increasing OLR and surface cooling. Preliminary estimates of this global net cloud forcing are more negative than -2.8 W m{sup -2} and could neutralize the radiative forcing due to a CO{sub 2} doubling (3.7 W m{sup -2}). A potential delivery mechanism for the seeding material is already in place: the airline industry. Since seeding aerosol residence times in the troposphere are relatively short, the climate might return to its normal state within months after stopping the geoengineering experiment. The main known drawback to this approach is that it would not stop ocean acidification. It does not have many of the drawbacks that stratospheric injection of sulfur species has.

  17. Comparison of CERES-MODIS cloud microphysical properties with surface observations over Loess Plateau

    Science.gov (United States)

    Yan, Hongru; Huang, Jianping; Minnis, Patrick; Yi, Yuhong; Sun-Mack, Sunny; Wang, Tianhe; Nakajima, Takashi Y.

    2015-03-01

    To enhance the utility of satellite-derived cloud properties for studying the role of clouds in climate change and the hydrological cycle in semi-arid areas, it is necessary to know their uncertainties. This paper estimates the uncertainties of several cloud properties by comparing those derived over the China Loess Plateau from the MODerate-resolution Imaging Spectroradiometer (MODIS) on Terra and Aqua by the Clouds and Earth's Radiant Energy System (CERES) with surface observations at the Semi-Arid Climate and Environment Observatory of Lanzhou University (SACOL). The comparisons use data from January 2008 to June 2010 limited to single layer and overcast stratus conditions during daytime. Cloud optical depths (τ) and liquid water paths (LWP) from both Terra and Aqua generally track the variation of the surface counterparts with modest correlation, while cloud effective radius (re) is only weakly correlated with the surface retrievals. The mean differences between Terra and the SACOL retrievals are -4.7±12.9, 2.1±3.2 μm and 30.2±85.3 g m-2 for τ, re and LWP, respectively. The corresponding differences for Aqua are 2.1±8.4, 1.2±2.9 μm and 47.4±79.6 g m-2, respectively. Possible causes for biases of satellite retrievals are discussed through statistical analysis and case studies. Generally, the CERES-MODIS cloud properties have a bit larger biases over the Loess Plateau than those in previous studies over other locations.

  18. Stratospheric and solar cycle effects on long-term variability of mesospheric ice clouds

    Science.gov (United States)

    Lübken, F.-J.; Berger, U.; Baumgarten, G.

    2009-11-01

    Model results of mesospheric ice layers and background conditions at 69°N from 1961 to 2008 are analyzed. The model nudges to European Centre for Medium-Range Weather Forecasts data below ˜45 km. Greenhouse gas concentrations in the mesosphere are kept constant. At polar mesospheric cloud (PMC) altitudes (83 km) temperatures decrease until the mid 1990s by -0.08 K/yr resulting in trends of PMC brightness, occurrence rates, and, to a lesser extent, in PMC altitudes (-0.0166 km/yr). Ice layer trends are consistent with observations by ground-based and satellite instruments. Water vapor increases at PMC heights and decreases above due to increased freeze-drying caused by the temperature trend. Temperature trends in the mesosphere mainly come from shrinking of the stratosphere and from dynamical effects. A solar cycle modulation of H2O is observed in the model consistent with satellite observations. The effect on ice layers is reduced because of redistribution of H2O by freeze-drying. The accidental coincidence of low temperatures and solar cycle minimum in the mid 1990s leads to an overestimation of solar effects on ice layers. A strong correlation between temperatures and PMC altitudes is observed. Applied to historical measurements this gives negligible temperature trends at PMC altitudes (˜0.01-0.02 K/yr). Strong correlations between PMC parameters and background conditions deduced from the model confirm the standard scenario of PMC formation. The PMC sensitivity on temperatures, water vapor, and Ly-α is investigated. PMC heights show little variation with background parameters whereas brightness and occurrence rates show large variations. None of the background parameters can be ignored regarding its influence on ice layers.

  19. Latitudinal and interhemispheric variation of stratospheric effects on mesospheric ice layer trends

    Science.gov (United States)

    Lübken, F.-J.; Berger, U.

    2011-02-01

    Latitudinal and interhemispheric differences of model results on trends in mesospheric ice layers and background conditions are analyzed. The model nudges to European Centre for Medium-Range Weather Forecasts data below ˜45 km. Greenhouse gas concentrations in the mesosphere are kept constant. Temperature trends in the mesosphere mainly come from shrinking of the stratosphere and from dynamical effects. Water vapor increases at noctilucent cloud (NLC) heights and decreases above due to increased freeze drying caused by temperature trends. There is no tendency for ice clouds in the Northern Hemisphere for extending farther southward with time. Trends of NLC albedo are similar to satellite measurements, but only if a time period longer than observations is considered. Ice cloud trends get smaller if albedo thresholds relevant to satellite instruments are applied, in particular at high polar latitudes. This implies that weak and moderate NLC is favored when background conditions improve for NLC formation, whereas strong NLC benefits less. Trends of ice cloud parameters are generally smaller in the Southern Hemisphere (SH) compared to the Northern Hemisphere (NH), consistent with observations. Trends in background conditions have counteracting effects on NLC: temperature trends would suggest stronger ice increase in the SH, and water vapor trends would suggest a weaker increase. Larger trends in NLC brightness or occurrence rates are not necessarily associated with larger (more negative) temperature trends. They can also be caused by larger trends of water vapor caused by larger freeze drying, which in turn can be caused by generally lower temperatures and/or more background water. Trends of NLC brightness and occurrence rates decrease with decreasing latitude in both hemispheres. The latitudinal variation of these trends is primarily determined by induced water vapor trends. Trends in NLC altitudes are generally small. Stratospheric temperature trends vary

  20. Influence of cloud fraction and snow cover to the variation of surface UV radiation at King Sejong station, Antarctica

    Science.gov (United States)

    Lee, Yun Gon; Koo, Ja-Ho; Kim, Jhoon

    2015-10-01

    This study investigated how cloud fraction and snow cover affect the variation of surface ultraviolet (UV) radiation by using surface Erythemal UV (EUV) and Near UV (NUV) observed at the King Sejong Station, Antarctica. First the Radiative Amplification Factor (RAF), the relative change of surface EUV according to the total-column ozone amount, is compared for different cloud fractions and solar zenith angles (SZAs). Generally, all cloudy conditions show that the increase of RAF as SZA becomes larger, showing the larger effects of vertical columnar ozone. For given SZA cases, the EUV transmission through mean cloud layer gradually decreases as cloud fraction increases, but sometimes the maximum of surface EUV appears under partly cloudy conditions. The high surface EUV transmittance under broken cloud conditions seems due to the re-radiation of scattered EUV by cloud particles. NUV transmission through mean cloud layer also decreases as cloud amount increases but the sensitivity to the cloud fraction is larger than EUV. Both EUV and NUV radiations at the surface are also enhanced by the snow cover, and their enhancement becomes higher as SZA increases implying the diurnal variation of surface albedo. This effect of snow cover seems large under the overcast sky because of the stronger interaction between snow surface and cloudy sky.

  1. The tropical Atlantic surface wind divergence belt and its effect on clouds

    OpenAIRE

    Y. Tubul; I. Koren; O. Altaratz

    2015-01-01

    A well-defined surface wind divergence (SWD) belt with distinct cloud properties forms over the equatorial Atlantic during the boreal summer months. This belt separates the deep convective clouds of the intertropical convergence zone (ITCZ) from the shallow marine stratocumulus cloud decks forming over the cold-water subtropical region of the southern Hadley cell. Using the QuikSCAT-SeaWinds and Aqua-MODIS instruments, we examined the large-scale spatiotemporal ...

  2. Sulfuric acid deposition from stratospheric geoengineering with sulfate aerosols

    KAUST Repository

    Kravitz, Ben

    2009-07-28

    We used a general circulation model of Earth\\'s climate to conduct geoengineering experiments involving stratospheric injection of sulfur dioxide and analyzed the resulting deposition of sulfate. When sulfur dioxide is injected into the tropical or Arctic stratosphere, the main additional surface deposition of sulfate occurs in midlatitude bands, because of strong cross-tropopause flux in the jet stream regions. We used critical load studies to determine the effects of this increase in sulfate deposition on terrestrial ecosystems by assuming the upper limit of hydration of all sulfate aerosols into sulfuric acid. For annual injection of 5 Tg of SO2 into the tropical stratosphere or 3 Tg of SO2 into the Arctic stratosphere, neither the maximum point value of sulfate deposition of approximately 1.5 mEq m−2 a−1 nor the largest additional deposition that would result from geoengineering of approximately 0.05 mEq m−2 a−1 is enough to negatively impact most ecosystems.

  3. Sulfuric acid deposition from stratospheric geoengineering with sulfate aerosols

    KAUST Repository

    Kravitz, Ben; Robock, Alan; Oman, Luke; Stenchikov, Georgiy L.; Marquardt, Allison B.

    2009-01-01

    We used a general circulation model of Earth's climate to conduct geoengineering experiments involving stratospheric injection of sulfur dioxide and analyzed the resulting deposition of sulfate. When sulfur dioxide is injected into the tropical or Arctic stratosphere, the main additional surface deposition of sulfate occurs in midlatitude bands, because of strong cross-tropopause flux in the jet stream regions. We used critical load studies to determine the effects of this increase in sulfate deposition on terrestrial ecosystems by assuming the upper limit of hydration of all sulfate aerosols into sulfuric acid. For annual injection of 5 Tg of SO2 into the tropical stratosphere or 3 Tg of SO2 into the Arctic stratosphere, neither the maximum point value of sulfate deposition of approximately 1.5 mEq m−2 a−1 nor the largest additional deposition that would result from geoengineering of approximately 0.05 mEq m−2 a−1 is enough to negatively impact most ecosystems.

  4. The tropical Atlantic surface wind divergence belt and its effect on clouds

    OpenAIRE

    Y. Tubul; I. Koren; O. Altaratz

    2015-01-01

    A well-defined surface wind divergence (SWD) belt with distinct cloud properties forms over the equatorial Atlantic during the boreal summer months. This belt separates the deep convective clouds of the Intertropical Convergence Zone (ITCZ) from the shallow marine stratocumulus cloud decks forming over the cold-water subtropical region of the southern branch of the Hadley cell in the Atlantic. Using the QuikSCAT-SeaWinds and Aqua-MODIS instruments, we examined the large-scal...

  5. Waves on the surface of the Orion molecular cloud.

    Science.gov (United States)

    Berné, Olivier; Marcelino, Núria; Cernicharo, José

    2010-08-19

    Massive stars influence their parental molecular cloud, and it has long been suspected that the development of hydrodynamical instabilities can compress or fragment the cloud. Identifying such instabilities has proved difficult. It has been suggested that elongated structures (such as the 'pillars of creation') and other shapes arise because of instabilities, but alternative explanations are available. One key signature of an instability is a wave-like structure in the gas, which has hitherto not been seen. Here we report the presence of 'waves' at the surface of the Orion molecular cloud near where massive stars are forming. The waves seem to be a Kelvin-Helmholtz instability that arises during the expansion of the nebula as gas heated and ionized by massive stars is blown over pre-existing molecular gas.

  6. Effects of stratospheric perturbations on the solar radiation budget

    International Nuclear Information System (INIS)

    Luther, F.M.

    1978-04-01

    The changes in solar absorption and in local heating rates due to perturbations to O 3 and NO 2 concentrations caused by stratospheric injection of NO/sub x/ and CFM pollutants are assessed. The changes in species concentration profiles are derived from theoretical calculations using a transport-kinetics model. Because of significant changes in our understanding of stratospheric chemistry during the past year, the assessment of the effect of stratospheric perturbations on the solar radiation budget differs from previous assessments. Previously, a reduction in O 3 due to an NO/sub x/ injection caused a net decrease in the gaseous solar absorption;now the same perturbation leads to a net increase. The implication of these changes on the surface temperature is also discussed

  7. STRATAQ: A three-dimensional Chemical Transport Model of the stratosphere

    Directory of Open Access Journals (Sweden)

    B. Grassi

    2002-06-01

    Full Text Available A three-dimensional (3-D Chemical Transport Model (CTM of the stratosphere has been developed and used for a test study of the evolution of chemical species in the arctic lower stratosphere during winter 1996/97. This particular winter has been chosen for testing the model’s capabilities for its remarkable dynamical situation (very cold and strong polar vortex along with the availability of sparse chlorine, HNO3 and O3 data, showing also very low O3 values in late March/April. Due to those unusual features, the winter 1996/97 can be considered an excellent example of the impact of both dynamics and heterogeneous reactions on the chemistry of the stratosphere. Model integration has been performed from January to March 1997 and the resulting long-lived and short-lived tracer fields compared with available measurements. The model includes a detailed gas phase chemical scheme and a parameterization of the heterogeneous reactions occurring on liquid aerosol and polar stratospheric cloud (PSC surfaces. The transport is calculated using a semi-lagrangian flux scheme, forced by meteorological analyses. In such form, the STRATAQ CTM model is suitable for short-term integrations to study transport and chemical evolution related to "real" meteorological situations. Model simulation during the chosen winter shows intense PSC formation, with noticeable local HNO3 capture by PSCs, and the activation of vortex air leading to chlorine production and subsequent O3 destruction. The resulting model fields show generally good agreement with satellite data (MLS and TOMS, although the available observations, due to their limited number and time/space sparse nature, are not enough to effectively constraint the model. In particular, the model seems to perform well in reproducing the rapid processing of air inside the polar vortex on PSC converting reservoir species in active chlorine. In addition, it satisfactorily reproduces the morphology of the continuous O3

  8. STRATAQ: A three-dimensional Chemical Transport Model of the stratosphere

    Directory of Open Access Journals (Sweden)

    B. Grassi

    Full Text Available A three-dimensional (3-D Chemical Transport Model (CTM of the stratosphere has been developed and used for a test study of the evolution of chemical species in the arctic lower stratosphere during winter 1996/97. This particular winter has been chosen for testing the model’s capabilities for its remarkable dynamical situation (very cold and strong polar vortex along with the availability of sparse chlorine, HNO3 and O3 data, showing also very low O3 values in late March/April. Due to those unusual features, the winter 1996/97 can be considered an excellent example of the impact of both dynamics and heterogeneous reactions on the chemistry of the stratosphere. Model integration has been performed from January to March 1997 and the resulting long-lived and short-lived tracer fields compared with available measurements. The model includes a detailed gas phase chemical scheme and a parameterization of the heterogeneous reactions occurring on liquid aerosol and polar stratospheric cloud (PSC surfaces. The transport is calculated using a semi-lagrangian flux scheme, forced by meteorological analyses. In such form, the STRATAQ CTM model is suitable for short-term integrations to study transport and chemical evolution related to "real" meteorological situations. Model simulation during the chosen winter shows intense PSC formation, with noticeable local HNO3 capture by PSCs, and the activation of vortex air leading to chlorine production and subsequent O3 destruction. The resulting model fields show generally good agreement with satellite data (MLS and TOMS, although the available observations, due to their limited number and time/space sparse nature, are not enough to effectively constraint the model. In particular, the model seems to perform well in reproducing the rapid processing of air inside the polar vortex on PSC converting reservoir species in active chlorine. In addition, it

  9. Climate change projections and stratosphere-troposphere interaction

    Energy Technology Data Exchange (ETDEWEB)

    Scaife, Adam A.; Fereday, David R.; Butchart, Neal; Hardiman, Steven C. [Met Office Hadley Centre, Exeter (United Kingdom); Spangehl, Thomas; Cubasch, Ulrich; Langematz, Ulrike [Freie Universitaet Berlin, Berlin (Germany); Akiyoshi, Hideharu [National Institute for Environmental Studies, Tsukuba (Japan); Bekki, Slimane [LATMOS-IPSL, UVSQ, UPMC, CNRS/INSU, Paris (France); Braesicke, Peter [University of Cambridge, Cambridge (United Kingdom); Chipperfield, Martyn P. [University of Leeds, School of Earth and Environment, Leeds (United Kingdom); Gettelman, Andrew [National Center for Atmospheric Research, Boulder, CO (United States); Michou, Martine [GAME/CNRM (Meteo France, CNRS), Toulouse (France); Rozanov, Eugene [PMOD/WRC and ETHZ, Davos (Switzerland); Shepherd, Theodore G. [University of Toronto, Toronto, ON (Canada)

    2012-05-15

    Climate change is expected to increase winter rainfall and flooding in many extratropical regions as evaporation and precipitation rates increase, storms become more intense and storm tracks move polewards. Here, we show how changes in stratospheric circulation could play a significant role in future climate change in the extratropics through an additional shift in the tropospheric circulation. This shift in the circulation alters climate change in regional winter rainfall by an amount large enough to significantly alter regional climate change projections. The changes are consistent with changes in stratospheric winds inducing a change in the baroclinic eddy growth rate across the depth of the troposphere. A change in mean wind structure and an equatorward shift of the tropospheric storm tracks relative to models with poor stratospheric resolution allows coupling with surface climate. Using the Atlantic storm track as an example, we show how this can double the predicted increase in extreme winter rainfall over Western and Central Europe compared to other current climate projections. (orig.)

  10. Influence of Ice Particle Surface Roughening on the Global Cloud Radiative Effect

    Science.gov (United States)

    Yi, Bingqi; Yang, Ping; Baum, Bryan A.; LEcuyer, Tristan; Oreopoulos, Lazaros; Mlawer, Eli J.; Heymsfield, Andrew J.; Liou, Kuo-Nan

    2013-01-01

    Ice clouds influence the climate system by changing the radiation budget and large-scale circulation. Therefore, climate models need to have an accurate representation of ice clouds and their radiative effects. In this paper, new broadband parameterizations for ice cloud bulk scattering properties are developed for severely roughened ice particles. The parameterizations are based on a general habit mixture that includes nine habits (droxtals, hollow/solid columns, plates, solid/hollow bullet rosettes, aggregate of solid columns, and small/large aggregates of plates). The scattering properties for these individual habits incorporate recent advances in light-scattering computations. The influence of ice particle surface roughness on the ice cloud radiative effect is determined through simulations with the Fu-Liou and the GCM version of the Rapid Radiative Transfer Model (RRTMG) codes and the National Center for Atmospheric Research Community Atmosphere Model (CAM, version 5.1). The differences in shortwave (SW) and longwave (LW) radiative effect at both the top of the atmosphere and the surface are determined for smooth and severely roughened ice particles. While the influence of particle roughening on the single-scattering properties is negligible in the LW, the results indicate that ice crystal roughness can change the SW forcing locally by more than 10 W m(exp -2) over a range of effective diameters. The global-averaged SW cloud radiative effect due to ice particle surface roughness is estimated to be roughly 1-2 W m(exp -2). The CAM results indicate that ice particle roughening can result in a large regional SW radiative effect and a small but nonnegligible increase in the global LW cloud radiative effect.

  11. Exposing Microorganisms in the Stratosphere for Planetary Protection

    Data.gov (United States)

    National Aeronautics and Space Administration — Earth’s stratosphere is similar to the surface of Mars: rarified air which is dry, cold, and irradiated. E-MIST is a balloon payload that has 4 independently...

  12. Tibetan Plateau glacier and hydrological change under stratospheric aerosol injection

    Science.gov (United States)

    Ji, D.

    2017-12-01

    As an important inland freshwater resource, mountain glaciers are highly related to human life, they provide water for many large rivers and play a very important role in regional water cycles. The response of mountain glaciers to future climate change is a topic of concern especially to the many people who rely on glacier-fed rivers for purposes such as irrigation. Geoengineering by stratospheric aerosol injection is a method of offsetting the global temperature rise from greenhouse gases. How the geoengineering by stratospheric aerosol injection affects the mass balance of mountain glaciers and adjacent river discharge is little understood. In this study, we use regional climate model WRF and catchment-based river model CaMa-Flood to study the impacts of stratospheric aerosol injection to Tibetan Plateau glacier mass balance and adjacent river discharge. To facilitate mountain glacier mass balance study, we improve the description of mountain glacier in the land surface scheme of WRF. The improvements include: (1) a fine mesh nested in WRF horizontal grid to match the highly non-uniform spatial distribution of the mountain glaciers, (2) revising the radiation flux at the glacier surface considering the surrounding terrain. We use the projections of five Earth system models for CMIP5 rcp45 and GeoMIP G4 scenarios to drive the WRF and CaMa-Flood models. The G4 scenario, which uses stratospheric aerosols to reduce the incoming shortwave while applying the rcp4.5 greenhouse gas forcing, starts stratospheric sulfate aerosol injection at a rate of 5 Tg per year over the period 2020-2069. The ensemble projections suggest relatively slower glacier mass loss rates and reduced river discharge at Tibetan Plateau and adjacent regions under geoengineering scenario by stratospheric aerosol injection.

  13. SUNYA Regional Climate Model Simulations of East Asia Summer Monsoon: Effects of Cloud Vertical Structure on the Surface Energy Balance

    Directory of Open Access Journals (Sweden)

    Wei Gong and Wei-Chyung Wang

    2007-01-01

    Full Text Available We used the State University of New York at Albany (SUNYA regional climate model to study the effect of cloud vertical distribution in affecting the surface energy balance of the East Asia summer monsoon (EASM. Simulations were conducted for the summers of 1988 and 1989, during which large contrast in the intra-seasonal cloud radiative forcing (CRF was observed at the top of the atmosphere. The model results indicate that both the high and low clouds are persistent throughout the summer months in both years. Because of large cloud water, low clouds significantly reduce the solar radiation flux reaching the surface, which nevertheless still dominate the surface energy balance, accounting for more than 50% of the surface heating. The low clouds also contribute significantly the downward longwave radiation to the surface with values strongly dependent on the cloud base temperature. The presence of low clouds effectively decreases the temperature and moisture gradients near surface, resulting in a substantial decrease in the sensible and latent heat fluxes from surface, which partially compensate the decrease of the net radiative cooling of the surface. For example, in the two days, May 8 and July 11 of 1988, the total cloud cover of 80% is simulated, but the respective low cloud cover (water was 63% (114 gm-2 and 22% (21 gm-2. As a result, the downward solar radiation is smaller by 161 Wm-2 in May 8. On the other hand, the cloud temperature was _ lower, yielding 56 Wm-2 smaller downward longwave radiation. The near surface temperature and gradient is more than _ smaller (and moisture gradient, leading to 21 and 81 Wm-2 smaller sensible heat and latent heat fluxes. It is also demonstrated that the model is capable to reproduce the intraseasonal variation of shortwave CRF, and catches the relationship between total cloud cover and SW CRF. The model results show the dominance of high cloud on the regional mean longwave CRF and low cloud on the intra

  14. A method for establishing a long duration, stratospheric platform for astronomical research

    Science.gov (United States)

    Fesen, Robert; Brown, Yorke

    2015-10-01

    During certain times of the year at middle and low latitudes, winds in the upper stratosphere move in nearly the opposite direction than the wind in the lower stratosphere. Here we present a method for maintaining a high-altitude balloon platform in near station-keeping mode that utilizes this stratospheric wind shear. The proposed method places a balloon-borne science platform high in the stratosphere connected by a lightweight, high-strength tether to a tug vehicle located in the lower or middle stratosphere. Using aerodynamic control surfaces, wind-induced aerodynamic forces on the tug can be manipulated to counter the wind drag acting on the higher altitude science vehicle, thus controlling the upper vehicle's geographic location. We describe the general framework of this station-keeping method, some important properties required for the upper stratospheric science payload and lower tug platforms, and compare this station-keeping approach with the capabilities of a high altitude airship and conventional tethered aerostat approaches. We conclude by discussing the advantages of such a platform for a variety of missions with emphasis on astrophysical research.

  15. Reliability Evaluation for the Surface to Air Missile Weapon Based on Cloud Model

    Directory of Open Access Journals (Sweden)

    Deng Jianjun

    2015-01-01

    Full Text Available The fuzziness and randomness is integrated by using digital characteristics, such as Expected value, Entropy and Hyper entropy. The cloud model adapted to reliability evaluation is put forward based on the concept of the surface to air missile weapon. The cloud scale of the qualitative evaluation is constructed, and the quantitative variable and the qualitative variable in the system reliability evaluation are corresponded. The practical calculation result shows that it is more effective to analyze the reliability of the surface to air missile weapon by this way. The practical calculation result also reflects the model expressed by cloud theory is more consistent with the human thinking style of uncertainty.

  16. Cosmogenic 35S as a Novel Detector of Stratospheric Air at the Earth's Surface: Key Findings from the Western United States and New Insights into the Seasonal Variations of Ozone and Sulfate in East Asia

    Science.gov (United States)

    Lin, M.; Thiemens, M. H.; Shaheen, R.; Biglari, S.; Crocker, D.; Zhang, Z.; Tao, J.; Su, L.; Fung, J. C. H.; Su, B.; Liu, L.

    2016-12-01

    The extent to which stratospheric intrusions on synoptic scales influence the tropospheric ozone (O3) levels remains poorly understood because quantitative detection of stratosphere air at the Earth's surface has been challenging. Cosmogenic 35S is invaluable in such quantification, but this has not yet been unambiguously demonstrated. As a global hot spot for stratospheric intrusions, the western United States (US) is a natural laboratory for testing the validity of this approach. Here, we present measurements of 35S in sulfate aerosols during a well-defined deep stratospheric intrusion event in the western US, which led to a regional O3 pollution event across southern California. The surprisingly high 35S activity in this episode is greater than any other natural radiogenic sulfate aerosols reported in the literature, providing the first and direct field-based evidence that 35S is a sensitive tracer for air mass of stratospheric origin and transported downward. Using this novel tracer, we quantify the seasonal variation for the strength of downward transport of stratospheric air to the planetary boundary layer in East Asia (EA) and what it may mean for surface O3 and sulfate levels. Our 35S measurements in sulfate aerosols collected from a background site (Mount Wuyi; 27.72°N, 117.68°E) during 2014-2015 show peaks in spring and autumn and the temporal variations of 35S were in tandem with surface O3 levels. These results imply that stratospheric O3 in aged stratospheric air masses may contribute to surface O3 levels in the study region in these two seasons. Along with radiogenic 35S analysis, measuring all seven stable isotopes (16O, 17O, 18O, 32S, 33S, 34S and 36S) in the same sulfate samples provides significantly deeper understanding of the atmospheric sulfur cycle in this region. Triple oxygen isotopes are being measured and preliminary results show that the relative importance of different formation pathways of secondary sulfate in EA is likely altitude

  17. Cloud effects on the SW radiation at the surface at a mid-latitude site in southwestern Europe

    Science.gov (United States)

    Salgueiro, Vanda; João Costa, Maria; Silva, Ana Maria; Lanconelli, Christian; Bortoli, Daniele

    2017-04-01

    This work presents a study of cloud radiative effects on shortwave (CRESW) radiation at the surface in Évora region (southwestern Europe) during 2015 and a case study is analyzed. CRESW (in Wm-2) is defined as the difference between the net shortwave irradiance (downward minus upward shortwave irradiance) in cloudy and clear sky conditions. This measure is usually used to translate changes in the SW radiation that reaches the surface due to changes in clouds (type and/or cover). The CRESW is obtained using measured SW irradiance recorded with a Kipp&Zonen CM 6B pyranometer (broadband 305 - 2800 nm) during the period from January to December 2015, and is related with the cloud liquid water path (LWP) and with cloud ice water path (IWP) showing the importance of the different type of clouds in attenuating the SW radiation at the surface. The cloud modification factor, also a measure of the cloud radiative effects (CMF; ratio between the measured SW irradiance under cloudy conditions and the estimated SW irradiance in clear-sky conditions) is related with the cloud optical thickness (COT; obtained from satellite data). This relation between CMF and COT is shown for different cloud fractions revealing an exponential decreasing of CMF as COT increases. Reductions in the SW radiation of the order of 80% (CMF = 0.2) as well enhancements in the SW radiation larger than 30% (CMF = 1.3) were found for small COT values and for different cloud fractions. A case study to analyse the enhancement events in a cloudy day was considered and the cloud properties, COT and LWP (from satellite and surface measurements), were related with the CRESW.

  18. Linking atmospheric synoptic transport, cloud phase, surface energy fluxes, and sea-ice growth: observations of midwinter SHEBA conditions

    Science.gov (United States)

    Persson, P. Ola G.; Shupe, Matthew D.; Perovich, Don; Solomon, Amy

    2017-08-01

    Observations from the Surface Heat Budget of the Arctic Ocean (SHEBA) project are used to describe a sequence of events linking midwinter long-range advection of atmospheric heat and moisture into the Arctic Basin, formation of supercooled liquid water clouds, enhancement of net surface energy fluxes through increased downwelling longwave radiation, and reduction in near-surface conductive heat flux loss due to a warming of the surface, thereby leading to a reduction in sea-ice bottom growth. The analyses provide details of two events during Jan. 1-12, 1998, one entering the Arctic through Fram Strait and the other from northeast Siberia; winter statistics extend the results. Both deep, precipitating frontal clouds and post-frontal stratocumulus clouds impact the surface radiation and energy budget. Cloud liquid water, occurring preferentially in stratocumulus clouds extending into the base of the inversion, provides the strongest impact on surface radiation and hence modulates the surface forcing, as found previously. The observations suggest a minimum water vapor threshold, likely case dependent, for producing liquid water clouds. Through responses to the radiative forcing and surface warming, this cloud liquid water also modulates the turbulent and conductive heat fluxes, and produces a thermal wave penetrating into the sea ice. About 20-33 % of the observed variations of bottom ice growth can be directly linked to variations in surface conductive heat flux, with retarded ice growth occurring several days after these moisture plumes reduce the surface conductive heat flux. This sequence of events modulate pack-ice wintertime environmental conditions and total ice growth, and has implications for the annual sea-ice evolution, especially for the current conditions of extensive thinner ice.

  19. STRATOSPHERIC TEMPERATURES AND WATER LOSS FROM MOIST GREENHOUSE ATMOSPHERES OF EARTH-LIKE PLANETS

    Energy Technology Data Exchange (ETDEWEB)

    Kasting, James F.; Kopparapu, Ravi K. [Department of Geosciences, The Pennsylvania State University, State College, PA 16801 (United States); Chen, Howard, E-mail: jfk4@psu.edu, E-mail: hwchen@bu.edu [Department of Astronomy, Boston University, 725 Commonwealth Ave., Boston, MA 02215 (United States)

    2015-11-01

    A radiative-convective climate model is used to calculate stratospheric temperatures and water vapor concentrations for ozone-free atmospheres warmer than that of modern Earth. Cold, dry stratospheres are predicted at low surface temperatures, in agreement with recent 3D calculations. However, at surface temperatures above 350 K, the stratosphere warms and water vapor becomes a major upper atmospheric constituent, allowing water to be lost by photodissociation and hydrogen escape. Hence, a moist greenhouse explanation for loss of water from Venus, or some exoplanet receiving a comparable amount of stellar radiation, remains a viable hypothesis. Temperatures in the upper parts of such atmospheres are well below those estimated for a gray atmosphere, and this factor should be taken into account when performing inverse climate calculations to determine habitable zone boundaries using 1D models.

  20. STRATOSPHERIC TEMPERATURES AND WATER LOSS FROM MOIST GREENHOUSE ATMOSPHERES OF EARTH-LIKE PLANETS

    International Nuclear Information System (INIS)

    Kasting, James F.; Kopparapu, Ravi K.; Chen, Howard

    2015-01-01

    A radiative-convective climate model is used to calculate stratospheric temperatures and water vapor concentrations for ozone-free atmospheres warmer than that of modern Earth. Cold, dry stratospheres are predicted at low surface temperatures, in agreement with recent 3D calculations. However, at surface temperatures above 350 K, the stratosphere warms and water vapor becomes a major upper atmospheric constituent, allowing water to be lost by photodissociation and hydrogen escape. Hence, a moist greenhouse explanation for loss of water from Venus, or some exoplanet receiving a comparable amount of stellar radiation, remains a viable hypothesis. Temperatures in the upper parts of such atmospheres are well below those estimated for a gray atmosphere, and this factor should be taken into account when performing inverse climate calculations to determine habitable zone boundaries using 1D models

  1. SURFACE FITTING FILTERING OF LIDAR POINT CLOUD WITH WAVEFORM INFORMATION

    Directory of Open Access Journals (Sweden)

    S. Xing

    2017-09-01

    Full Text Available Full-waveform LiDAR is an active technology of photogrammetry and remote sensing. It provides more detailed information about objects along the path of a laser pulse than discrete-return topographic LiDAR. The point cloud and waveform information with high quality can be obtained by waveform decomposition, which could make contributions to accurate filtering. The surface fitting filtering method with waveform information is proposed to present such advantage. Firstly, discrete point cloud and waveform parameters are resolved by global convergent Levenberg Marquardt decomposition. Secondly, the ground seed points are selected, of which the abnormal ones are detected by waveform parameters and robust estimation. Thirdly, the terrain surface is fitted and the height difference threshold is determined in consideration of window size and mean square error. Finally, the points are classified gradually with the rising of window size. The filtering process is finished until window size is larger than threshold. The waveform data in urban, farmland and mountain areas from “WATER (Watershed Allied Telemetry Experimental Research” are selected for experiments. Results prove that compared with traditional method, the accuracy of point cloud filtering is further improved and the proposed method has highly practical value.

  2. The Effects of Interactive Stratospheric Chemistry on Antarctic and Southern Ocean Climate Change in an AOGCM

    Science.gov (United States)

    Li, Feng; Newman, Paul; Pawson, Steven; Waugh, Darryn

    2014-01-01

    Stratospheric ozone depletion has played a dominant role in driving Antarctic climate change in the last decades. In order to capture the stratospheric ozone forcing, many coupled atmosphere-ocean general circulation models (AOGCMs) prescribe the Antarctic ozone hole using monthly and zonally averaged ozone field. However, the prescribed ozone hole has a high ozone bias and lacks zonal asymmetry. The impacts of these biases on model simulations, particularly on Southern Ocean and the Antarctic sea ice, are not well understood. The purpose of this study is to determine the effects of using interactive stratospheric chemistry instead of prescribed ozone on Antarctic and Southern Ocean climate change in an AOGCM. We compare two sets of ensemble simulations for the 1960-2010 period using different versions of the Goddard Earth Observing System 5 - AOGCM: one with interactive stratospheric chemistry, and the other with prescribed monthly and zonally averaged ozone and 6 other stratospheric radiative species calculated from the interactive chemistry simulations. Consistent with previous studies using prescribed sea surface temperatures and sea ice concentrations, the interactive chemistry runs simulate a deeper Antarctic ozone hole and consistently larger changes in surface pressure and winds than the prescribed ozone runs. The use of a coupled atmosphere-ocean model in this study enables us to determine the impact of these surface changes on Southern Ocean circulation and Antarctic sea ice. The larger surface wind trends in the interactive chemistry case lead to larger Southern Ocean circulation trends with stronger changes in northerly and westerly surface flow near the Antarctica continent and stronger upwelling near 60S. Using interactive chemistry also simulates a larger decrease of sea ice concentrations. Our results highlight the importance of using interactive chemistry in order to correctly capture the influences of stratospheric ozone depletion on climate

  3. Ozone mixing ratios inside tropical deep convective clouds from OMI satellite measurements

    Directory of Open Access Journals (Sweden)

    J. R. Ziemke

    2009-01-01

    Full Text Available We have developed a new technique for estimating ozone mixing ratio inside deep convective clouds. The technique uses the concept of an optical centroid cloud pressure that is indicative of the photon path inside clouds. Radiative transfer calculations based on realistic cloud vertical structure as provided by CloudSat radar data show that because deep convective clouds are optically thin near the top, photons can penetrate significantly inside the cloud. This photon penetration coupled with in-cloud scattering produces optical centroid pressures that are hundreds of hPa inside the cloud. We combine measured column ozone and the optical centroid cloud pressure derived using the effects of rotational-Raman scattering to estimate O3 mixing ratio in the upper regions of deep convective clouds. The data are obtained from the Ozone Monitoring Instrument (OMI onboard NASA's Aura satellite. Our results show that low O3 concentrations in these clouds are a common occurrence throughout much of the tropical Pacific. Ozonesonde measurements in the tropics following convective activity also show very low concentrations of O3 in the upper troposphere. These low amounts are attributed to vertical injection of ozone poor oceanic boundary layer air during convection into the upper troposphere followed by convective outflow. Over South America and Africa, O3 mixing ratios inside deep convective clouds often exceed 50 ppbv which are comparable to mean background (cloud-free amounts and are consistent with higher concentrations of injected boundary layer/lower tropospheric O3 relative to the remote Pacific. The Atlantic region in general also consists of higher amounts of O3 precursors due to both biomass burning and lightning. Assuming that O3 is well mixed (i.e., constant mixing ratio with height up to the tropopause, we can estimate the stratospheric column O3 over

  4. Visualizing Volcanic Clouds in the Atmosphere and Their Impact on Air Traffic.

    Science.gov (United States)

    Gunther, Tobias; Schulze, Maik; Friederici, Anke; Theisel, Holger

    2016-01-01

    Volcanic eruptions are not only hazardous in the direct vicinity of a volcano, but they also affect the climate and air travel for great distances. This article sheds light on the Grímsvötn, Puyehue-Cordón Caulle, and Nabro eruptions in 2011. The authors study the agreement of the complementary satellite data, reconstruct sulfate aerosol and volcanic ash clouds, visualize endangered flight routes, minimize occlusion in particle trajectory visualizations, and focus on the main pathways of Nabro's sulfate aerosol into the stratosphere. The results here were developed for the 2014 IEEE Scientific Visualization Contest, which centers around the fusion of multiple satellite data modalities to reconstruct and assess the movement of volcanic ash and sulfate aerosol emissions. Using data from three volcanic eruptions that occurred in the span of approximately three weeks, the authors study the agreement of the complementary satellite data, reconstruct sulfate aerosol and volcanic ash clouds, visualize endangered flight routes, minimize occlusion in particle trajectory visualizations, and focus on the main pathways of sulfate aerosol into the stratosphere. This video provides animations of the reconstructed ash clouds. https://youtu.be/D9DvJ5AvZAs.

  5. The Impact of Stratospheric Circulation Extremes on Minimum Arctic Sea Ice Extent

    Science.gov (United States)

    Smith, K. L.; Polvani, L. M.; Tremblay, B.

    2017-12-01

    The interannual variability of summertime Arctic sea ice extent (SIE) is anti-correlated with the leading mode of extratropical atmospheric variability in preceding winter, the Arctic Oscillation (AO). Given this relationship and the need for better seasonal predictions of Arctic SIE, we here examine the role of stratospheric circulation extremes and stratosphere-troposphere coupling in linking the AO and Arctic SIE variability. We show that extremes in the stratospheric circulation during the winter season, namely stratospheric sudden warming (SSW) and strong polar vortex (SPV) events, are associated with significant anomalies in sea ice concentration in the Bering Straight and the Sea of Okhotsk in winter, the Barents Sea in spring and along the Eurasian coastline in summer in both observations and a fully-coupled, stratosphere-resolving general circulation model. The accompanying figure shows the composite mean sea ice concentration anomalies from the Whole Atmosphere Community Climate Model (WACCM) for SSWs (N = 126, top row) and SPVs (N = 99, bottom row) for winter (a,d), spring (b,e) and summer (c,f). Consistent with previous work on the AO, we find that SSWs, which are followed by the negative phase of the AO at the surface, result in sea ice growth, whereas SPVs, which are followed by the positive phase of the AO at the surface, result in sea ice loss, although the dynamic and thermodynamic processes driving these sea ice anomalies in the three Arctic regions, noted above, are different. Our analysis suggests that the presence or absence of stratospheric circulation extremes in winter may play a non-trivial role in determining total September Arctic SIE when combined with other factors.

  6. Dust ablation on the giant planets: Consequences for stratospheric photochemistry

    Science.gov (United States)

    Moses, Julianne I.; Poppe, Andrew R.

    2017-11-01

    Ablation of interplanetary dust supplies oxygen to the upper atmospheres of Jupiter, Saturn, Uranus, and Neptune. Using recent dynamical model predictions for the dust influx rates to the giant planets (Poppe et al., 2016), we calculate the ablation profiles and investigate the subsequent coupled oxygen-hydrocarbon neutral photochemistry in the stratospheres of these planets. We find that dust grains from the Edgeworth-Kuiper Belt, Jupiter-family comets, and Oort-cloud comets supply an effective oxygen influx rate of 1.0-0.7+2.2 ×107 O atoms cm-2 s-1 to Jupiter, 7.4-5.1+16 ×104 cm-2 s-1 to Saturn, 8.9-6.1+19 ×104 cm-2 s-1 to Uranus, and 7.5-5.1+16 ×105 cm-2 s-1 to Neptune. The fate of the ablated oxygen depends in part on the molecular/atomic form of the initially delivered products, and on the altitude at which it was deposited. The dominant stratospheric products are CO, H2O, and CO2, which are relatively stable photochemically. Model-data comparisons suggest that interplanetary dust grains deliver an important component of the external oxygen to Jupiter and Uranus but fall far short of the amount needed to explain the CO abundance currently seen in the middle stratospheres of Saturn and Neptune. Our results are consistent with the theory that all of the giant planets have experienced large cometary impacts within the last few hundred years. Our results also suggest that the low background H2O abundance in Jupiter's stratosphere is indicative of effective conversion of meteoric oxygen to CO during or immediately after the ablation process - photochemistry alone cannot efficiently convert the H2O into CO on the giant planets.

  7. Retrieval of global upper tropospheric and stratospheric formaldehyde (H2CO distributions from high-resolution MIPAS-Envisat spectra

    Directory of Open Access Journals (Sweden)

    G. P. Stiller

    2008-02-01

    Full Text Available The Fourier transform spectrometer MIPAS (Michelson Interferometer for Passive Atmospheric Sounding on Envisat measures infrared emission of the Earth's atmosphere in a limb viewing mode. High spectral resolution measurements of MIPAS are sensitive to formaldehyde from the upper troposphere to the stratopause. Single profile retrievals of formaldehyde are dominated by a 60% noise error; however zonal mean values for 30 days of data during 8 September 2003 and 1 December 2003 reduces this error by a factor of 20 or more. The number of degrees of freedom for single profile retrieval ranges from 2 to 4.5 depending on latitude and number of cloud-free tangent altitudes. In the upper tropical troposphere zonal mean values of about 70 parts per trillion by volume (pptv were found, which have been attributed to biomass burning emissions. In the stratosphere, formaldehyde values are determined by photochemical reactions. In the upper tropical stratosphere, formaldehyde zonal mean maximum values can reach 130 pptv. Diurnal variations in this region can be up to 50 pptv. Comparisons with other satellite instruments show generally good agreement in the region of upper troposphere and lower stratosphere as well as in the upper stratosphere.

  8. Variability of surface ozone with cloud coverage over Kolkata, India

    Indian Academy of Sciences (India)

    influences the weather and climate of a place, thus acting as an ... earth by absorbing the most energetic part of the ... effect of cloud coverage on the surface ozone over. Kolkata. 2. ..... Burrows W R 1997 CART regression models for predicting.

  9. Ability of the CCSR-NIES atmospheric general circulation model in the stratosphere. Chapter 3

    International Nuclear Information System (INIS)

    Sugata, S.

    1997-01-01

    A quantitative evaluation of climate change such as global warming is impossible without a high-quality numerical model which describes the dynamics of the climate system and the circulation of energy and materials. The Center for Climate Research - National Institute for Environmental Studies (CCSR-NIES) atmospheric general circulation model (hereafter, GCM for a general circulation model) has been developed to obtain such a high-quality model. The emphasis of the development has been laid on the troposphere and the lower stratosphere below about 30 km altitude. This is natural because human beings live on the Earth's surface and the condition of the lower atmosphere directly affects human life. However, the stratosphere and the upper atmosphere beyond it have recently been the focus even in investigations of climate change, because they are relevant to many issues which relate closely to tropospheric climate change, such as the ozone hole, material exchange between the stratosphere and the troposphere, and physical interaction between the stratosphere and troposphere. This study extended the region of the CCSR-NIES GCM to the lower mesosphere (about 70 km from the surface). This is our first attempt to investigate this GCM's climatology in the upper atmosphere, although some studies for QBO in the middle and lower stratosphere had been done with the GCM

  10. Near-Real Time Satellite-Retrieved Cloud and Surface Properties for Weather and Aviation Safety Applications

    Science.gov (United States)

    Minnis, P.; Smith, W., Jr.; Bedka, K. M.; Nguyen, L.; Palikonda, R.; Hong, G.; Trepte, Q.; Chee, T.; Scarino, B. R.; Spangenberg, D.; Sun-Mack, S.; Fleeger, C.; Ayers, J. K.; Chang, F. L.; Heck, P. W.

    2014-12-01

    Cloud properties determined from satellite imager radiances provide a valuable source of information for nowcasting and weather forecasting. In recent years, it has been shown that assimilation of cloud top temperature, optical depth, and total water path can increase the accuracies of weather analyses and forecasts. Aircraft icing conditions can be accurately diagnosed in near-real time (NRT) retrievals of cloud effective particle size, phase, and water path, providing valuable data for pilots. NRT retrievals of surface skin temperature can also be assimilated in numerical weather prediction models to provide more accurate representations of solar heating and longwave cooling at the surface, where convective initiation. These and other applications are being exploited more frequently as the value of NRT cloud data become recognized. At NASA Langley, cloud properties and surface skin temperature are being retrieved in near-real time globally from both geostationary (GEO) and low-earth orbiting (LEO) satellite imagers for weather model assimilation and nowcasting for hazards such as aircraft icing. Cloud data from GEO satellites over North America are disseminated through NCEP, while those data and global LEO and GEO retrievals are disseminated from a Langley website. This paper presents an overview of the various available datasets, provides examples of their application, and discusses the use of the various datasets downstream. Future challenges and areas of improvement are also presented.

  11. Near-Real Time Satellite-Retrieved Cloud and Surface Properties for Weather and Aviation Safety Applications

    Science.gov (United States)

    Minnis, Patrick; Smith, William L., Jr.; Bedka, Kristopher M.; Nguyen, Louis; Palikonda, Rabindra; Hong, Gang; Trepte, Qing Z.; Chee, Thad; Scarino, Benjamin; Spangenberg, Douglas A.; hide

    2014-01-01

    Cloud properties determined from satellite imager radiances provide a valuable source of information for nowcasting and weather forecasting. In recent years, it has been shown that assimilation of cloud top temperature, optical depth, and total water path can increase the accuracies of weather analyses and forecasts. Aircraft icing conditions can be accurately diagnosed in near-­-real time (NRT) retrievals of cloud effective particle size, phase, and water path, providing valuable data for pilots. NRT retrievals of surface skin temperature can also be assimilated in numerical weather prediction models to provide more accurate representations of solar heating and longwave cooling at the surface, where convective initiation. These and other applications are being exploited more frequently as the value of NRT cloud data become recognized. At NASA Langley, cloud properties and surface skin temperature are being retrieved in near-­-real time globally from both geostationary (GEO) and low-­-earth orbiting (LEO) satellite imagers for weather model assimilation and nowcasting for hazards such as aircraft icing. Cloud data from GEO satellites over North America are disseminated through NCEP, while those data and global LEO and GEO retrievals are disseminated from a Langley website. This paper presents an overview of the various available datasets, provides examples of their application, and discusses the use of the various datasets downstream. Future challenges and areas of improvement are also presented.

  12. Probability Density Functions for the CALIPSO Lidar Version 4 Cloud-Aerosol Discrimination (CAD) Algorithm

    Science.gov (United States)

    Liu, Z.; Kar, J.; Zeng, S.; Tackett, J. L.; Vaughan, M.; Trepte, C. R.; Omar, A. H.; Hu, Y.; Winker, D. M.

    2017-12-01

    In the CALIPSO retrieval algorithm, detection layers in the lidar measurements is followed by their classification as a "cloud" or "aerosol" using 5-dimensional probability density functions (PDFs). The five dimensions are the mean attenuated backscatter at 532 nm, the layer integrated total attenuated color ratio, the mid-layer altitude, integrated volume depolarization ratio and latitude. The new version 4 (V4) level 2 (L2) data products, released in November 2016, are the first major revision to the L2 product suite since May 2010. Significant calibration changes in the V4 level 1 data necessitated substantial revisions to the V4 L2 CAD algorithm. Accordingly, a new set of PDFs was generated to derive the V4 L2 data products. The V4 CAD algorithm is now applied to layers detected in the stratosphere, where volcanic layers and occasional cloud and smoke layers are observed. Previously, these layers were designated as `stratospheric', and not further classified. The V4 CAD algorithm is also applied to all layers detected at single shot (333 m) resolution. In prior data releases, single shot detections were uniformly classified as clouds. The CAD PDFs used in the earlier releases were generated using a full year (2008) of CALIPSO measurements. Because the CAD algorithm was not applied to stratospheric features, the properties of these layers were not incorporated into the PDFs. When building the V4 PDFs, the 2008 data were augmented with additional data from June 2011, and all stratospheric features were included. The Nabro and Puyehue-Cordon volcanos erupted in June 2011, and volcanic aerosol layers were observed in the upper troposphere and lower stratosphere in both the northern and southern hemispheres. The June 2011 data thus provides the stratospheric aerosol properties needed for comprehensive PDF generation. In contrast to earlier versions of the PDFs, which were generated based solely on observed distributions, construction of the V4 PDFs considered the

  13. Impacts of Interactive Stratospheric Chemistry on Antarctic and Southern Ocean Climate Change in the Goddard Earth Observing System Version 5 (GEOS-5)

    Science.gov (United States)

    Li, Feng; Vikhliaev, Yury V.; Newman, Paul A.; Pawson, Steven; Perlwitz, Judith; Waugh, Darryn W.; Douglass, Anne R.

    2016-01-01

    Stratospheric ozone depletion plays a major role in driving climate change in the Southern Hemisphere. To date, many climate models prescribe the stratospheric ozone layer's evolution using monthly and zonally averaged ozone fields. However, the prescribed ozone underestimates Antarctic ozone depletion and lacks zonal asymmetries. In this study we investigate the impact of using interactive stratospheric chemistry instead of prescribed ozone on climate change simulations of the Antarctic and Southern Ocean. Two sets of 1960-2010 ensemble transient simulations are conducted with the coupled ocean version of the Goddard Earth Observing System Model, version 5: one with interactive stratospheric chemistry and the other with prescribed ozone derived from the same interactive simulations. The model's climatology is evaluated using observations and reanalysis. Comparison of the 1979-2010 climate trends between these two simulations reveals that interactive chemistry has important effects on climate change not only in the Antarctic stratosphere, troposphere, and surface, but also in the Southern Ocean and Antarctic sea ice. Interactive chemistry causes stronger Antarctic lower stratosphere cooling and circumpolar westerly acceleration during November-December-January. It enhances stratosphere-troposphere coupling and leads to significantly larger tropospheric and surface westerly changes. The significantly stronger surface wind stress trends cause larger increases of the Southern Ocean Meridional Overturning Circulation, leading to year-round stronger ocean warming near the surface and enhanced Antarctic sea ice decrease.

  14. The Influence of Stratospheric Sulphate Aerosol Deployment on the Surface Air Temperature and the Risk of an Abrupt Global Warming

    Directory of Open Access Journals (Sweden)

    Roland von Glasow

    2010-12-01

    Full Text Available We used the ‘Radiative-Convective Model of the Earth-atmosphere system’ (OGIM to investigate the cooling effects induced by sulphur injections into the stratosphere. The ensemble of numerical calculations was based on the A1B scenario from the IPCC Special Report on Emissions Scenarios (SRES. Several geoengineered scenarios were analysed, including the abrupt interruption of these injections in different scenarios and at different dates. We focused on the surface air temperature (SAT anomalies induced by stratospheric sulphate aerosol generated in order to compensate future warming. Results show that continuous deployment of sulphur into the stratosphere could induce a lasting decrease in SAT. Retaining a constant aerosol loading equivalent to 6 TgS would delay the expected global warming by 53 years. Keeping the SAT constant in a context of increasing greenhouse gases (GHGs means that the aerosol loading needs to be increased by 1.9% annually. This would offset the effect of increasing GHG under the A1B scenario. A major focus of this study was on the heating rates of SAT that would arise in different scenarios in case of an abrupt cessation of sulphur injections into the stratosphere. Our model results show that heating rates after geoengineering interruption would be 15–28 times higher than in a case without geoengineering, with likely important consequences for life on Earth. Larger initial sulphate loadings induced more intense warming rates when the geoengineering was stopped at the same time. This implies that, if sulphate loading was increased to maintain constant SAT in the light of increasing GHG concentrations, the later the geoengineering interruption was to occur, the higher the heating rates would be. Consequently, geoengineering techniques like this should only be regarded as last-resort measures and require intense further research should they ever become necessary.

  15. Effects of Greenhouse Gas Increase and Stratospheric Ozone Depletion on Stratospheric Mean Age of Air in 1960-2010

    Science.gov (United States)

    Li, F.; Newman, P. A.; Pawson, S.; Perlwitz, J.

    2017-12-01

    The strength of the stratospheric Brewer-Dobson circulation (BDC) in a changing climate has been extensively studied, but the relative importance of greenhouse gas (GHG) increases and stratospheric ozone depletion in driving the BDC changes remains uncertain. This study separates the impacts of GHG and stratospheric ozone forcings on stratospheric mean age of air in the 1960-2010 period using the Goddard Earth Observing System Model (GEOS) Chemistry-Climate Model (CCM). The experiment compares a set of controlled simulations using a coupled atmosphere-ocean version of the GEOS CCM, in which either GHGs, or stratospheric ozone, or both factors evolve over time. The model results show that GHGs and stratospheric ozone have about equal contributions to the simulated mean age decrease. It is also found that GHG increases account for about two thirds of the enhanced strength of the lower stratospheric residual circulation. The results show that ozone depletion causes an increase in the mean age of air in the Antarctic summer lower stratosphere through two processes: 1) a seasonal delay in the Antarctic polar vortex breakup, that inhibits young mid-latitude air from mixing with the older air inside the vortex; and 2) enhanced Antarctic downwelling, that brings older air from middle and upper stratosphere into the lower stratosphere.

  16. Modification of cirrus clouds to reduce global warming

    Science.gov (United States)

    Mitchell, D. L.

    2009-12-01

    Since both greenhouse gases and cirrus clouds strongly affect outgoing longwave radiation (OLR) with no affect or less affect on solar radiation, respectively, an attempt to delay global warming to buy time for emission reduction strategies to work might naturally target cirrus clouds. Cirrus having optical depths competition effects, thus increasing OLR and surface cooling. Preliminary estimates of this global net cloud forcing via GCM simulations are more negative than -2.8 W m-2 and could neutralize the radiative forcing due to a CO2 doubling (3.7 W m-2). This cirrus engineered net forcing is due to (1) reduced cirrus coverage and (2) reduced upper tropospheric water vapor, due to enhanced ice sedimentation. The implementation of this climate engineering could use the airline industry to disperse the seeding material. Commercial airliners typically fly at temperatures between -40 and -60 deg. C (where homogeneous freezing nucleation dominates). Weather modification research has developed ice nucleating substances that are extremely effective at these cold temperatures, are non-toxic and are relatively inexpensive. The seeding material could be released in both clear and cloudy conditions to build up a background concentration of efficient ice nuclei so that non-contrail cirrus will experience these nuclei and grow larger ice crystals. Flight corridors are denser in the high- and mid-latitudes where global warming is more severe. A risk with any geoengineering experiment is that it could affect climate in unforeseen ways, causing more harm than good. Since seeding aerosol residence times in the troposphere are 1-2 weeks, the climate might return back to its normal state within a few months after stopping the geoengineering. A drawback to this approach is that it would not stop ocean acidification. It may not have many of the draw-backs that stratospheric injection of sulfur species has, such as ozone destruction, decreased solar radiation possibly altering the

  17. A Stabilizing Feedback Between Cloud Radiative Effects and Greenland Surface Melt: Verification From Multi-year Automatic Weather Station Measurements

    Science.gov (United States)

    Zender, C. S.; Wang, W.; van As, D.

    2017-12-01

    Clouds have strong impacts on Greenland's surface melt through the interaction with the dry atmosphere and reflective surfaces. However, their effects are uncertain due to the lack of in situ observations. To better quantify cloud radiative effects (CRE) in Greenland, we analyze and interpret multi-year radiation measurements from 30 automatic weather stations encompassing a broad range of climatological and topographical conditions. During melt season, clouds warm surface over most of Greenland, meaning the longwave greenhouse effect outweighs the shortwave shading effect; on the other hand, the spatial variability of net (longwave and shortwave) CRE is dominated by shortwave CRE and in turn by surface albedo, which controls the potential absorption of solar radiation when clouds are absent. The net warming effect decreases with shortwave CRE from high to low altitudes and from north to south (Fig. 1). The spatial correlation between albedo and net CRE is strong (r=0.93, palbedo determines the net CRE seasonal trend, which decreases from May to July and increases afterwards. On an hourly timescale, we find two distinct radiative states in Greenland (Fig. 2). The clear state is characterized by clear-sky conditions or thin clouds, when albedo and solar zenith angle (SZA) weakly correlates with CRE. The cloudy state is characterized by opaque clouds, when the combination of albedo and SZA strongly correlates with CRE (r=0.85, palbedo and solar zenith angle, explains the majority of the CRE variation in spatial distribution, seasonal trend in the ablation zone, and in hourly variability in the cloudy radiative state. Clouds warm the brighter and colder surfaces of Greenland, enhance snow melt, and tend to lower the albedo. Clouds cool the darker and warmer surfaces, inhibiting snow melt, which increases albedo, and thus stabilizes surface melt. This stabilizing mechanism may also occur over sea ice, helping to forestall surface melt as the Arctic becomes dimmer.

  18. The Origins of Air Parcels Uplifted in a Two Dimensional Gravity Wave in the Tropical Upper Troposphere During the NASA Stratosphere Troposphere Exchange Project (STEP)

    Science.gov (United States)

    Selkirk, Henry B.; Pfister, Leonhard; Chan, K. Roland; Kritz, Mark; Kelly, Ken

    1989-01-01

    During January and February 1987, as part of the Stratosphere-Troposphere Exchange Project, the NASA ER-2 made 11 flights from Darwin, Australia to investigate dehydration mechanisms in the vicinity of the tropical tropopause. After the monsoon onset in the second week of January, steady easterly flow of 15-25 ms (exp -1) was established in the upper troposphere and lower stratosphere over northern Australia and adjacent seas. Penetrating into this regime were elements of the monsoon convection such as overshooting convective turrets and extensive anvils including cyclone cloud shields. In cases of the latter, the resulting flow obstructions tended to produce mesoscale gravity waves. In several instances the ER- 2 meteorological and trace constituent measurements provide a detailed description of the structure of these gravity waves. Among these was STEP Flight 6, 22-23 January. It is of particular interest to STEP because of the close proximity of ice-laden and dehydrated air on the same isentropic surfaces. Convective events inject large amounts of ice into the upper troposphere and lower stratosphere which may not be completely removed by local precipitation processes. In the present instance, a gravity wave for removed from the source region appears to induce relativity rapid upward motion in the ice-laden air and subsequent dessication. Potential mechanisms for such a localized removal process are under investigation.

  19. The Diversity of Cloud Responses to Twentieth Century Sea Surface Temperatures

    Science.gov (United States)

    Silvers, Levi G.; Paynter, David; Zhao, Ming

    2018-01-01

    Low-level clouds are shown to be the conduit between the observed sea surface temperatures (SST) and large decadal fluctuations of the top of the atmosphere radiative imbalance. The influence of low-level clouds on the climate feedback is shown for global mean time series as well as particular geographic regions. The changes of clouds are found to be important for a midcentury period of high sensitivity and a late century period of low sensitivity. These conclusions are drawn from analysis of amip-piForcing simulations using three atmospheric general circulation models (AM2.1, AM3, and AM4.0). All three models confirm the importance of the relationship between the global climate sensitivity and the eastern Pacific trends of SST and low-level clouds. However, this work argues that the variability of the climate feedback parameter is not driven by stratocumulus-dominated regions in the eastern ocean basins, but rather by the cloudy response in the rest of the tropics.

  20. Evidence for a continuous decline in lower stratospheric ozone offsetting ozone layer recovery

    Science.gov (United States)

    Ball, William T.; Alsing, Justin; Mortlock, Daniel J.; Staehelin, Johannes; Haigh, Joanna D.; Peter, Thomas; Tummon, Fiona; Stübi, Rene; Stenke, Andrea; Anderson, John; Bourassa, Adam; Davis, Sean M.; Degenstein, Doug; Frith, Stacey; Froidevaux, Lucien; Roth, Chris; Sofieva, Viktoria; Wang, Ray; Wild, Jeannette; Yu, Pengfei; Ziemke, Jerald R.; Rozanov, Eugene V.

    2018-02-01

    Ozone forms in the Earth's atmosphere from the photodissociation of molecular oxygen, primarily in the tropical stratosphere. It is then transported to the extratropics by the Brewer-Dobson circulation (BDC), forming a protective ozone layer around the globe. Human emissions of halogen-containing ozone-depleting substances (hODSs) led to a decline in stratospheric ozone until they were banned by the Montreal Protocol, and since 1998 ozone in the upper stratosphere is rising again, likely the recovery from halogen-induced losses. Total column measurements of ozone between the Earth's surface and the top of the atmosphere indicate that the ozone layer has stopped declining across the globe, but no clear increase has been observed at latitudes between 60° S and 60° N outside the polar regions (60-90°). Here we report evidence from multiple satellite measurements that ozone in the lower stratosphere between 60° S and 60° N has indeed continued to decline since 1998. We find that, even though upper stratospheric ozone is recovering, the continuing downward trend in the lower stratosphere prevails, resulting in a downward trend in stratospheric column ozone between 60° S and 60° N. We find that total column ozone between 60° S and 60° N appears not to have decreased only because of increases in tropospheric column ozone that compensate for the stratospheric decreases. The reasons for the continued reduction of lower stratospheric ozone are not clear; models do not reproduce these trends, and thus the causes now urgently need to be established.

  1. Evidence for a Continuous Decline in Lower Stratospheric Ozone Offsetting Ozone Layer Recovery

    Science.gov (United States)

    Ball, William T.; Alsing, Justin; Mortlock, Daniel J.; Staehelin, Johannes; Haigh, Joanna D.; Peter, Thomas; Tummon, Fiona; Stuebi, Rene; Stenke, Andrea; Anderson, John; hide

    2018-01-01

    Ozone forms in the Earth's atmosphere from the photodissociation of molecular oxygen, primarily in the tropical stratosphere. It is then transported to the extratropics by the Brewer-Dobson circulation (BDC), forming a protective "ozone layer" around the globe. Human emissions of halogen-containing ozone-depleting substances (hODSs) led to a decline in stratospheric ozone until they were banned by the Montreal Protocol, and since 1998 ozone in the upper stratosphere is rising again, likely the recovery from halogen-induced losses. Total column measurements of ozone between the Earth's surface and the top of the atmosphere indicate that the ozone layer has stopped declining across the globe, but no clear increase has been observed at latitudes between 60degS and 60degN outside the polar regions (60-90deg). Here we report evidence from multiple satellite measurements that ozone in the lower stratosphere between 60degS and 60degN has indeed continued to decline since 1998. We find that, even though upper stratospheric ozone is recovering, the continuing downward trend in the lower stratosphere prevails, resulting in a downward trend in stratospheric column ozone between 60degS and 60degN. We find that total column ozone between 60degS and 60degN appears not to have decreased only because of increases in tropospheric column ozone that compensate for the stratospheric decreases. The reasons for the continued reduction of lower stratospheric ozone are not clear; models do not reproduce these trends, and thus the causes now urgently need to be established.

  2. How stratospheric are deep stratospheric intrusions? LUAMI 2008

    Directory of Open Access Journals (Sweden)

    T. Trickl

    2016-07-01

    Full Text Available A large-scale comparison of water-vapour vertical-sounding instruments took place over central Europe on 17 October 2008, during a rather homogeneous deep stratospheric intrusion event (LUAMI, Lindenberg Upper-Air Methods Intercomparison. The measurements were carried out at four observational sites: Payerne (Switzerland, Bilthoven (the Netherlands, Lindenberg (north-eastern Germany, and the Zugspitze mountain (Garmisch-Partenkichen, German Alps, and by an airborne water-vapour lidar system creating a transect of humidity profiles between all four stations. A high data quality was verified that strongly underlines the scientific findings. The intrusion layer was very dry with a minimum mixing ratios of 0 to 35 ppm on its lower west side, but did not drop below 120 ppm on the higher-lying east side (Lindenberg. The dryness hardens the findings of a preceding study (“Part 1”, Trickl et al., 2014 that, e.g., 73 % of deep intrusions reaching the German Alps and travelling 6 days or less exhibit minimum mixing ratios of 50 ppm and less. These low values reflect values found in the lowermost stratosphere and indicate very slow mixing with tropospheric air during the downward transport to the lower troposphere. The peak ozone values were around 70 ppb, confirming the idea that intrusion layers depart from the lowermost edge of the stratosphere. The data suggest an increase of ozone from the lower to the higher edge of the intrusion layer. This behaviour is also confirmed by stratospheric aerosol caught in the layer. Both observations are in agreement with the idea that sections of the vertical distributions of these constituents in the source region were transferred to central Europe without major change. LAGRANTO trajectory calculations demonstrated a rather shallow outflow from the stratosphere just above the dynamical tropopause, for the first time confirming the conclusions in “Part 1” from the Zugspitze CO observations. The

  3. JUPITER AS AN EXOPLANET: UV TO NIR TRANSMISSION SPECTRUM REVEALS HAZES, A Na LAYER, AND POSSIBLY STRATOSPHERIC H{sub 2}O-ICE CLOUDS

    Energy Technology Data Exchange (ETDEWEB)

    Montañés-Rodríguez, Pilar; González-Merino, B.; Pallé, E. [Instituto de Astrofísica de Canarias, C/Vía Láctea s/n, E-38200 La Laguna (Spain); López-Puertas, Manuel [Departamento de Astrofísica, Universidad de La Laguna, Av., Astrofísico Francisco Sánchez, s/n, E-38206 La Laguna (Spain); García-Melendo, E., E-mail: pmr@iac.es [Instituto de Astrofísica de Andalucía (CSIC), Glorieta de la Astronomía s/n, E-18080 Granada (Spain)

    2015-03-01

    Currently, the analysis of transmission spectra is the most successful technique to probe the chemical composition of exoplanet atmospheres. However, the accuracy of these measurements is constrained by observational limitations and the diversity of possible atmospheric compositions. Here, we show the UV–VIS–IR transmission spectrum of Jupiter as if it were a transiting exoplanet, obtained by observing one of its satellites, Ganymede, while passing through Jupiter’s shadow, i.e., during a solar eclipse from Ganymede. The spectrum shows strong extinction due to the presence of clouds (aerosols) and haze in the atmosphere and strong absorption features from CH{sub 4}. More interestingly, the comparison with radiative transfer models reveals a spectral signature, which we attribute here to a Jupiter stratospheric layer of crystalline H{sub 2}O ice. The atomic transitions of Na are also present. These results are relevant for the modeling and interpretation of giant transiting exoplanets. They also open a new technique to explore the atmospheric composition of the upper layers of Jupiter’s atmosphere.

  4. 3D MODELING OF GJ1214b's ATMOSPHERE: FORMATION OF INHOMOGENEOUS HIGH CLOUDS AND OBSERVATIONAL IMPLICATIONS

    Energy Technology Data Exchange (ETDEWEB)

    Charnay, B.; Meadows, V.; Misra, A.; Arney, G. [Astronomy Department, University of Washington, Seattle, WA 98125 (United States); Leconte, J., E-mail: bcharnay@uw.edu [Canadian Institute for Theoretical Astrophysics, 60 St George Street, University of Toronto, Toronto, ON M5S 3H8 (Canada)

    2015-11-01

    The warm sub-Neptune GJ1214b has a featureless transit spectrum that may be due to the presence of high and thick clouds or haze. Here, we simulate the atmosphere of GJ1214b with a 3D General Circulation Model for cloudy hydrogen-dominated atmospheres, including cloud radiative effects. We show that the atmospheric circulation is strong enough to transport micrometric cloud particles to the upper atmosphere and generally leads to a minimum of cloud at the equator. By scattering stellar light, clouds increase the planetary albedo to 0.4–0.6 and cool the atmosphere below 1 mbar. However, the heating by ZnS clouds leads to the formation of a stratospheric thermal inversion above 10 mbar, with temperatures potentially high enough on the dayside to evaporate KCl clouds. We show that flat transit spectra consistent with Hubble Space Telescope observations are possible if cloud particle radii are around 0.5 μm, and that such clouds should be optically thin at wavelengths >3 μm. Using simulated cloudy atmospheres that fit the observed spectra we generate transit, emission, and reflection spectra and phase curves for GJ1214b. We show that a stratospheric thermal inversion would be readily accessible in near- and mid-infrared atmospheric spectral windows. We find that the amplitude of the thermal phase curves is strongly dependent on metallicity, but only slightly impacted by clouds. Our results suggest that primary and secondary eclipses and phase curves observed by the James Webb Space Telescope in the near- to mid-infrared should provide strong constraints on the nature of GJ1214b's atmosphere and clouds.

  5. Effects of ice crystal surface roughness and air bubble inclusions on cirrus cloud radiative properties from remote sensing perspective

    International Nuclear Information System (INIS)

    Tang, Guanglin; Panetta, R. Lee; Yang, Ping; Kattawar, George W.; Zhai, Peng-Wang

    2017-01-01

    We study the combined effects of surface roughness and inhomogeneity on the optical scattering properties of ice crystals and explore the consequent implications to remote sensing of cirrus cloud properties. Specifically, surface roughness and inhomogeneity are added to the Moderate Resolution Imaging Spectroradiometer (MODIS) collection 6 (MC6) cirrus cloud particle habit model. Light scattering properties of the new habit model are simulated using a modified version of the Improved Geometric Optics Method (IGOM). Both inhomogeneity and surface roughness affect the single scattering properties significantly. In visible bands, inhomogeneity and surface roughness both tend to smooth the phase function and eliminate halos and the backscattering peak. The asymmetry parameter varies with the degree of surface roughness following a U shape - decreases and then increases - with a minimum at around 0.15, whereas it decreases monotonically with the air bubble volume fraction. Air bubble inclusions significantly increase phase matrix element -P_1_2 for scattering angles between 20°–120°, whereas surface roughness has a much weaker effect, increasing -P_1_2 slightly from 60°–120°. Radiative transfer simulations and cirrus cloud property retrievals are conducted by including both the factors. In terms of surface roughness and air bubble volume fraction, retrievals of cirrus cloud optical thickness or the asymmetry parameter using solar bands show similar patterns of variation. Polarimetric simulations using the MC6 cirrus cloud particle habit model are shown to be more consistent with observations when both surface roughness and inhomogeneity are simultaneously considered. - Highlights: • Surface roughness and air bubble inclusions affect optical properties of ice crystals significantly. • Including both factors improves simulations of ice cloud.• Cirrus cloud particle habit model of the MODIS collection 6 achieves better self-consistency and consistency with

  6. Contrasting Cloud Composition Between Coupled and Decoupled Marine Boundary Layer Clouds

    Science.gov (United States)

    WANG, Z.; Mora, M.; Dadashazar, H.; MacDonald, A.; Crosbie, E.; Bates, K. H.; Coggon, M. M.; Craven, J. S.; Xian, P.; Campbell, J. R.; AzadiAghdam, M.; Woods, R. K.; Jonsson, H.; Flagan, R. C.; Seinfeld, J.; Sorooshian, A.

    2016-12-01

    Marine stratocumulus clouds often become decoupled from the vertical layer immediately above the ocean surface. This study contrasts cloud chemical composition between coupled and decoupled marine stratocumulus clouds. Cloud water and droplet residual particle composition were measured in clouds off the California coast during three airborne experiments in July-August of separate years (E-PEACE 2011, NiCE 2013, BOAS 2015). Decoupled clouds exhibited significantly lower overall mass concentrations in both cloud water and droplet residual particles, consistent with reduced cloud droplet number concentration and sub-cloud aerosol (Dp > 100 nm) number concentration, owing to detachment from surface sources. Non-refractory sub-micrometer aerosol measurements show that coupled clouds exhibit higher sulfate mass fractions in droplet residual particles, owing to more abundant precursor emissions from the ocean and ships. Consequently, decoupled clouds exhibited higher mass fractions of organics, nitrate, and ammonium in droplet residual particles, owing to effects of long-range transport from more distant sources. Total cloud water mass concentration in coupled clouds was dominated by sodium and chloride, and their mass fractions and concentrations exceeded those in decoupled clouds. Conversely, with the exception of sea salt constituents (e.g., Cl, Na, Mg, K), cloud water mass fractions of all species examined were higher in decoupled clouds relative to coupled clouds. These results suggest that an important variable is the extent to which clouds are coupled to the surface layer when interpreting microphysical data relevant to clouds and aerosol particles.

  7. High cloud variations with surface temperature from 2002 to 2015: Contributions to atmospheric radiative cooling rate and precipitation changes

    Science.gov (United States)

    Liu, Run; Liou, Kuo-Nan; Su, Hui; Gu, Yu; Zhao, Bin; Jiang, Jonathan H.; Liu, Shaw Chen

    2017-05-01

    The global mean precipitation is largely constrained by atmospheric radiative cooling rates (Qr), which are sensitive to changes in high cloud fraction. We investigate variations of high cloud fraction with surface temperature (Ts) from July 2002 to June 2015 and compute their radiative effects on Qr using the Fu-Liou-Gu plane-parallel radiation model. We find that the tropical mean (30°S-30°N) high cloud fraction decreases with increasing Ts at a rate of about -1.0 ± 0.34% K-1 from 2002 to 2015, which leads to an enhanced atmospheric cooling around 0.86 W m-2 K-1. On the other hand, the northern midlatitudes (30°N-60°N) high cloud fraction increases with surface warming at a rate of 1.85 ± 0.65% K-1 and the near-global mean (60°S-60°N) high cloud fraction shows a statistically insignificant decreasing trend with increasing Ts over the analysis period. Dividing high clouds into cirrus, cirrostratus, and deep convective clouds, we find that cirrus cloud fraction increases with surface warming at a rate of 0.32 ± 0.11% K-1 (0.01 ± 0.17% K-1) for the near-global mean (tropical mean), while cirrostratus and deep convective clouds decrease with surface warming at a rate of -0.02 ± 0.18% K-1 and -0.33 ± 0.18% K-1 for the near-global mean and -0.64 ± 0.23% K-1 and -0.37 ± 0.13% K-1 for the tropical mean, respectively. High cloud fraction response to feedback to Ts accounts for approximately 1.9 ± 0.7% and 16.0 ± 6.1% of the increase in precipitation per unit surface warming over the period of 2002-2015 for the near-global mean and the tropical mean, respectively.

  8. Stratospheric cooling and polar ozone loss due to H2 emissions of a global hydrogen economy

    Science.gov (United States)

    Feck, T.; Grooß, J.-U.; Riese, M.; Vogel, B.

    2009-04-01

    "Green" hydrogen is seen as a major element of the future energy supply to reduce greenhouse gas emissions substantially. However, due to the possible interactions of hydrogen (H2) with other atmospheric constituents there is a need to analyse the implications of additional atmospheric H2 that could result from hydrogen leakage of a global hydrogen infrastructure. Emissions of molecular H2 can occur along the whole hydrogen process chain which increase the tropospheric H2 burden. Across the tropical tropopause H2 reaches the stratosphere where it is oxidised and forms water vapour (H2O). This causes increased IR-emissions into space and hence a cooling of the stratosphere. Both effects, the increase of stratospheric H2O and the cooling, enhances the potential of chlorine activation on liquid sulfate aerosol and polar stratospheric clouds (PSCs), which increase polar ozone destruction. Hence a global hydrogen economy could provoke polar ozone loss and could lead to a substantial delay of the current projected recovery of the stratospheric ozone layer. Our investigations show that even if 90% of the current global fossil primary energy input could be replaced by hydrogen and approximately 9.5% of the product gas would leak to the atmosphere, the ozone loss would be increased between 15 to 26 Dobson Units (DU) if the stratospheric CFC loading would retain unchanged. A consistency check of the used approximation methods with the Chemical Lagrangian Model of the Stratosphere (CLaMS) shows that this additional ozone loss can probably be treated as an upper limit. Towards more realistic future H2 leakage rate assumptions (< 3%) the additional ozone loss would be rather small (? 10 DU). However, in all cases the full damage would only occur if stratospheric CFC-levels would retain unchanged. Due to the CFC-prohibition as a result of the Montreal Protocol the forecasts suggest a decline of the stratospheric CFC loading about 50% until 2050. In this case our calculations

  9. A multilinear regression methodology to analyze the effect of atmospheric and surface forcing on Arctic clouds

    Science.gov (United States)

    Boeke, R.; Taylor, P. C.; Li, Y.

    2017-12-01

    Arctic cloud amount as simulated in CMIP5 models displays large intermodel spread- models disagree on the processes important for cloud formation as well as the radiative impact of clouds. The radiative response to cloud forcing can be better assessed when the drivers of Arctic cloud formation are known. Arctic cloud amount (CA) is a function of both atmospheric and surface conditions, and it is crucial to separate the influences of unique processes to understand why the models are different. This study uses a multilinear regression methodology to determine cloud changes using 3 variables as predictors: lower tropospheric stability (LTS), 500-hPa vertical velocity (ω500), and sea ice concentration (SIC). These three explanatory variables were chosen because their effects on clouds can be attributed to unique climate processes: LTS is a thermodynamic indicator of the relationship between clouds and atmospheric stability, SIC determines the interaction between clouds and the surface, and ω500 is a metric for dynamical change. Vertical, seasonal profiles of necessary variables are obtained from the Coupled Model Intercomparison Project 5 (CMIP5) historical simulation, an ocean-atmosphere couple model forced with the best-estimate natural and anthropogenic radiative forcing from 1850-2005, and statistical significance tests are used to confirm the regression equation. A unique heuristic model will be constructed for each climate model and for observations, and models will be tested by their ability to capture the observed cloud amount and behavior. Lastly, the intermodel spread in Arctic cloud amount will be attributed to individual processes, ranking the relative contributions of each factor to shed light on emergent constraints in the Arctic cloud radiative effect.

  10. The maintenance of elevated active chlorine levels in the Antarctic lower stratosphere through HCl null cycles

    Science.gov (United States)

    Müller, Rolf; Grooß, Jens-Uwe; Mannan Zafar, Abdul; Robrecht, Sabine; Lehmann, Ralph

    2018-03-01

    The Antarctic ozone hole arises from ozone destruction driven by elevated levels of ozone destroying (active) chlorine in Antarctic spring. These elevated levels of active chlorine have to be formed first and then maintained throughout the period of ozone destruction. It is a matter of debate how this maintenance of active chlorine is brought about in Antarctic spring, when the rate of formation of HCl (considered to be the main chlorine deactivation mechanism in Antarctica) is extremely high. Here we show that in the heart of the ozone hole (16-18 km or 85-55 hPa, in the core of the vortex), high levels of active chlorine are maintained by effective chemical cycles (referred to as HCl null cycles hereafter). In these cycles, the formation of HCl is balanced by immediate reactivation, i.e. by immediate reformation of active chlorine. Under these conditions, polar stratospheric clouds sequester HNO3 and thereby cause NO2 concentrations to be low. These HCl null cycles allow active chlorine levels to be maintained in the Antarctic lower stratosphere and thus rapid ozone destruction to occur. For the observed almost complete activation of stratospheric chlorine in the lower stratosphere, the heterogeneous reaction HCl + HOCl is essential; the production of HOCl occurs via HO2 + ClO, with the HO2 resulting from CH2O photolysis. These results are important for assessing the impact of changes of the future stratospheric composition on the recovery of the ozone hole. Our simulations indicate that, in the lower stratosphere, future increased methane concentrations will not lead to enhanced chlorine deactivation (through the reaction CH4 + Cl → HCl + CH3) and that extreme ozone destruction to levels below ≈ 0.1 ppm will occur until mid-century.

  11. Clouds in ECMWF's 30 KM Resolution Global Atmospheric Forecast Model (TL639)

    Science.gov (United States)

    Cahalan, R. F.; Morcrette, J. J.

    1999-01-01

    Global models of the general circulation of the atmosphere resolve a wide range of length scales, and in particular cloud structures extend from planetary scales to the smallest scales resolvable, now down to 30 km in state-of-the-art models. Even the highest resolution models do not resolve small-scale cloud phenomena seen, for example, in Landsat and other high-resolution satellite images of clouds. Unresolved small-scale disturbances often grow into larger ones through non-linear processes that transfer energy upscale. Understanding upscale cascades is of crucial importance in predicting current weather, and in parameterizing cloud-radiative processes that control long term climate. Several movie animations provide examples of the temporal and spatial variation of cloud fields produced in 4-day runs of the forecast model at the European Centre for Medium-Range Weather Forecasts (ECMWF) in Reading, England, at particular times and locations of simultaneous measurement field campaigns. model resolution is approximately 30 km horizontally (triangular truncation TL639) with 31 vertical levels from surface to stratosphere. Timestep of the model is about 10 minutes, but animation frames are 3 hours apart, at timesteps when the radiation is computed. The animations were prepared from an archive of several 4-day runs at the highest available model resolution, and archived at ECMWF. Cloud, wind and temperature fields in an approximately 1000 km X 1000 km box were retrieved from the archive, then approximately 60 Mb Vis5d files were prepared with the help of Graeme Kelly of ECMWF, and were compressed into MPEG files each less than 3 Mb. We discuss the interaction of clouds and radiation in the model, and compare the variability of cloud liquid as a function of scale to that seen in cloud observations made in intensive field campaigns. Comparison of high-resolution global runs to cloud-resolving models, and to lower resolution climate models is leading to better

  12. The Diversity of Cloud Responses to Twentieth-Century Sea Surface Temperatures

    Science.gov (United States)

    Silvers, L. G.; Paynter, D.; Zhao, M.

    2017-12-01

    Clouds play a crucial role in determining the magnitude of the global temperature response to forcing. Previous work has shown strong connections between cloud feedbacks and climate change, and between these feedbacks and changing patterns of surface temperature. We show that strong variability of the climate feedback parameter is present in three GFDL atmospheric general circulation models (AM2.1, AM3, AM4) over the twentieth century. This variability is highly correlated with the global mean cloud radiative effect (CRE) and low-cloud cover (LCC) anomalies. The decadal variability is characterized by a period of high climate sensitivity (1925-1955) and a period of low climate sensitivity (1975-2005). Observed trends of surface temperature also show distinct differences over these two periods. Although it is the SST that drives the atmospheric response, the estimated inversion strength (EIS) is necessary to reproduce the changing LCC field. During both periods, trends of EIS are shown to closely mirror trends of LCC over much of the globe, not only in the typical stratocumulus regions. Trends of the shortwave CRE (SWCRE), LCC, and the EIS are analyzed in particular geographic regions. All of these regions show a consistent relationship between LCC, SWCRE, and EIS, as well as significant differences between the two time periods. This study uses a 15 member ensemble of amip-piForcing simulations from 1870 -2005. These experiments are driven by observed SST patterns and hold greenhouse gases and other atmospheric forcing agents fixed at constant pre-industrial levels. This allows for a clean analysis of how clouds respond to changing patterns of SST and the resulting influence on the climate feedback parameter. The cloudy response of the atmosphere to changing SST patterns is critical in driving the variability of the climate feedback parameter during periods of both high and low climate sensitivity.

  13. Sensitivity of surface radiation budget to clouds over the Asian ...

    Indian Academy of Sciences (India)

    National Climate Centre, India Meteorological Department, Pune 400 005. ... down on the earth surface–atmosphere system also as an imbalance between surface netcloud ... the clouds produce more cooling effect in short-wave band than the warming effect in long-wave .... In the present study, we use the analysis method.

  14. A case study of gravity waves in noctilucent clouds

    Directory of Open Access Journals (Sweden)

    P. Dalin

    2004-06-01

    Full Text Available We present a case study of a noctilucent cloud (NLC display appearing on 10-11 August 2000 over Northern Sweden. Clear wave structures were visible in the clouds and time-lapse photography was used to derive the parameters characterising the gravity waves which could account for the observed NLC modulation. Using two nearby atmospheric radars, the Esrange MST Radar data and Andoya MF radar, we have identified gravity waves propagating upward from the upper stratosphere to NLC altitudes. The wave parameters derived from the radar measurements support the suggestion that gravity waves are responsible for the observed complex wave dynamics in the NLC.

  15. Northern Winter Climate Change: Assessment of Uncertainty in CMIP5 Projections Related to Stratosphere-Troposphere Coupling

    Science.gov (United States)

    Manzini, E.; Karpechko, A.Yu.; Anstey, J.; Shindell, Drew Todd; Baldwin, M.P.; Black, R.X.; Cagnazzo, C.; Calvo, N.; Charlton-Perez, A.; Christiansen, B.; hide

    2014-01-01

    Future changes in the stratospheric circulation could have an important impact on northern winter tropospheric climate change, given that sea level pressure (SLP) responds not only to tropospheric circulation variations but also to vertically coherent variations in troposphere-stratosphere circulation. Here we assess northern winter stratospheric change and its potential to influence surface climate change in the Coupled Model Intercomparison Project-Phase 5 (CMIP5) multimodel ensemble. In the stratosphere at high latitudes, an easterly change in zonally averaged zonal wind is found for the majority of the CMIP5 models, under the Representative Concentration Pathway 8.5 scenario. Comparable results are also found in the 1% CO2 increase per year projections, indicating that the stratospheric easterly change is common feature in future climate projections. This stratospheric wind change, however, shows a significant spread among the models. By using linear regression, we quantify the impact of tropical upper troposphere warming, polar amplification, and the stratospheric wind change on SLP. We find that the intermodel spread in stratospheric wind change contributes substantially to the intermodel spread in Arctic SLP change. The role of the stratosphere in determining part of the spread in SLP change is supported by the fact that the SLP change lags the stratospheric zonally averaged wind change. Taken together, these findings provide further support for the importance of simulating the coupling between the stratosphere and the troposphere, to narrow the uncertainty in the future projection of tropospheric circulation changes.

  16. Stratospheric ozone changes under solar geoengineering: implications for UV exposure and air quality

    Science.gov (United States)

    Nowack, Peer Johannes; Abraham, Nathan Luke; Braesicke, Peter; Pyle, John Adrian

    2016-03-01

    Various forms of geoengineering have been proposed to counter anthropogenic climate change. Methods which aim to modify the Earth's energy balance by reducing insolation are often subsumed under the term solar radiation management (SRM). Here, we present results of a standard SRM modelling experiment in which the incoming solar irradiance is reduced to offset the global mean warming induced by a quadrupling of atmospheric carbon dioxide. For the first time in an atmosphere-ocean coupled climate model, we include atmospheric composition feedbacks for this experiment. While the SRM scheme considered here could offset greenhouse gas induced global mean surface warming, it leads to important changes in atmospheric composition. We find large stratospheric ozone increases that induce significant reductions in surface UV-B irradiance, which would have implications for vitamin D production. In addition, the higher stratospheric ozone levels lead to decreased ozone photolysis in the troposphere. In combination with lower atmospheric specific humidity under SRM, this results in overall surface ozone concentration increases in the idealized G1 experiment. Both UV-B and surface ozone changes are important for human health. We therefore highlight that both stratospheric and tropospheric ozone changes must be considered in the assessment of any SRM scheme, due to their important roles in regulating UV exposure and air quality.

  17. A global space-based stratospheric aerosol climatology: 1979-2016

    Science.gov (United States)

    Thomason, Larry W.; Ernest, Nicholas; Millán, Luis; Rieger, Landon; Bourassa, Adam; Vernier, Jean-Paul; Manney, Gloria; Luo, Beiping; Arfeuille, Florian; Peter, Thomas

    2018-03-01

    We describe the construction of a continuous 38-year record of stratospheric aerosol optical properties. The Global Space-based Stratospheric Aerosol Climatology, or GloSSAC, provided the input data to the construction of the Climate Model Intercomparison Project stratospheric aerosol forcing data set (1979-2014) and we have extended it through 2016 following an identical process. GloSSAC focuses on the Stratospheric Aerosol and Gas Experiment (SAGE) series of instruments through mid-2005, and on the Optical Spectrograph and InfraRed Imager System (OSIRIS) and the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) data thereafter. We also use data from other space instruments and from ground-based, air, and balloon borne instruments to fill in key gaps in the data set. The end result is a global and gap-free data set focused on aerosol extinction coefficient at 525 and 1020 nm and other parameters on an "as available" basis. For the primary data sets, we developed a new method for filling the post-Pinatubo eruption data gap for 1991-1993 based on data from the Cryogenic Limb Array Etalon Spectrometer. In addition, we developed a new method for populating wintertime high latitudes during the SAGE period employing a latitude-equivalent latitude conversion process that greatly improves the depiction of aerosol at high latitudes compared to earlier similar efforts. We report data in the troposphere only when and where it is available. This is primarily during the SAGE II period except for the most enhanced part of the Pinatubo period. It is likely that the upper troposphere during Pinatubo was greatly enhanced over non-volcanic periods and that domain remains substantially under-characterized. We note that aerosol levels during the OSIRIS/CALIPSO period in the lower stratosphere at mid- and high latitudes is routinely higher than what we observed during the SAGE II period. While this period had nearly continuous low-level volcanic activity, it

  18. Solar wind: A possible factor driving the interannual sea surface temperature tripolar mode over North Atlantic

    Science.gov (United States)

    Xiao, Ziniu; Li, Delin

    2016-06-01

    The effect of solar wind (SW) on the North Atlantic sea surface temperature (SST) in boreal winter is examined through an analysis of observational data during 1964-2013. The North Atlantic SSTs show a pronounced meridional tripolar pattern in response to solar wind speed (SWS) variations. This pattern is broadly similar to the leading empirical orthogonal function (EOF) mode of interannual variations in the wintertime SSTs over North Atlantic. The time series of this leading EOF mode of SST shows a significant interannual period, which is the same as that of wintertime SWS. This response also appears as a compact north-south seesaw of sea level pressure and a vertical tripolar structure of zonal wind, which simultaneously resembles the North Atlantic Oscillation (NAO) in the overlying atmosphere. As compared with the typical low SWS winters, during the typical high SWS winters, the stratospheric polar night jet (PNJ) is evidently enhanced and extends from the stratosphere to the troposphere, even down to the North Atlantic Ocean surface. Notably, the North Atlantic Ocean is an exclusive region in which the SW signal spreads downward from the stratosphere to the troposphere. Thus, it seems that the SW is a possible factor for this North Atlantic SST tripolar mode. The dynamical process of stratosphere-troposphere coupling, together with the global atmospheric electric circuit-cloud microphysical process, probably accounts for the particular downward propagation of the SW signal.

  19. Outcrop-scale fracture trace identification using surface roughness derived from a high-density point cloud

    Science.gov (United States)

    Okyay, U.; Glennie, C. L.; Khan, S.

    2017-12-01

    Owing to the advent of terrestrial laser scanners (TLS), high-density point cloud data has become increasingly available to the geoscience research community. Research groups have started producing their own point clouds for various applications, gradually shifting their emphasis from obtaining the data towards extracting more and meaningful information from the point clouds. Extracting fracture properties from three-dimensional data in a (semi-)automated manner has been an active area of research in geosciences. Several studies have developed various processing algorithms for extracting only planar surfaces. In comparison, (semi-)automated identification of fracture traces at the outcrop scale, which could be used for mapping fracture distribution have not been investigated frequently. Understanding the spatial distribution and configuration of natural fractures is of particular importance, as they directly influence fluid-flow through the host rock. Surface roughness, typically defined as the deviation of a natural surface from a reference datum, has become an important metric in geoscience research, especially with the increasing density and accuracy of point clouds. In the study presented herein, a surface roughness model was employed to identify fracture traces and their distribution on an ophiolite outcrop in Oman. Surface roughness calculations were performed using orthogonal distance regression over various grid intervals. The results demonstrated that surface roughness could identify outcrop-scale fracture traces from which fracture distribution and density maps can be generated. However, considering outcrop conditions and properties and the purpose of the application, the definition of an adequate grid interval for surface roughness model and selection of threshold values for distribution maps are not straightforward and require user intervention and interpretation.

  20. Near-Surface Meteorology During the Arctic Summer Cloud Ocean Study (ASCOS): Evaluation of Reanalyses and Global Climate Models.

    Science.gov (United States)

    De Boer, G.; Shupe, M.D.; Caldwell, P.M.; Bauer, Susanne E.; Persson, O.; Boyle, J.S.; Kelley, M.; Klein, S.A.; Tjernstrom, M.

    2014-01-01

    Atmospheric measurements from the Arctic Summer Cloud Ocean Study (ASCOS) are used to evaluate the performance of three atmospheric reanalyses (European Centre for Medium Range Weather Forecasting (ECMWF)- Interim reanalysis, National Center for Environmental Prediction (NCEP)-National Center for Atmospheric Research (NCAR) reanalysis, and NCEP-DOE (Department of Energy) reanalysis) and two global climate models (CAM5 (Community Atmosphere Model 5) and NASA GISS (Goddard Institute for Space Studies) ModelE2) in simulation of the high Arctic environment. Quantities analyzed include near surface meteorological variables such as temperature, pressure, humidity and winds, surface-based estimates of cloud and precipitation properties, the surface energy budget, and lower atmospheric temperature structure. In general, the models perform well in simulating large-scale dynamical quantities such as pressure and winds. Near-surface temperature and lower atmospheric stability, along with surface energy budget terms, are not as well represented due largely to errors in simulation of cloud occurrence, phase and altitude. Additionally, a development version of CAM5, which features improved handling of cloud macro physics, has demonstrated to improve simulation of cloud properties and liquid water amount. The ASCOS period additionally provides an excellent example of the benefits gained by evaluating individual budget terms, rather than simply evaluating the net end product, with large compensating errors between individual surface energy budget terms that result in the best net energy budget.

  1. Trends in Upper-Level Cloud Cover and Surface Divergence Over the Tropical Indo-Pacific Ocean Between 1952 And 1997

    Science.gov (United States)

    Norris, Joel R.

    2005-01-01

    This study investigated the spatial pattern of linear trends in surface-observed upper-level (combined mid-level and High-level) cloud cover, precipitation, and surface divergence over the tropical Indo-Pacific Ocean during 1952-1957. Cloud values were obtained from the Extended Edited Cloud Report Archive (EECRA), precipitation values were obtained from the Hulme/Climate Research Unit Data Set, and surface divergence was alternatively calculated from wind reported Comprehensive Ocean-Atmosphere Data Set and from Smith and Reynolds Extended Reconstructed sea level pressure data.

  2. [Cii] emission from L1630 in the Orion B molecular cloud.

    Science.gov (United States)

    Pabst, C H M; Goicoechea, J R; Teyssier, D; Berné, O; Ochsendorf, B B; Wolfire, M G; Higgins, R D; Riquelme, D; Risacher, C; Pety, J; Le Petit, F; Roueff, E; Bron, E; Tielens, A G G M

    2017-10-01

    L1630 in the Orion B molecular cloud, which includes the iconic Horsehead Nebula, illuminated by the star system σ Ori, is an example of a photodissociation region (PDR). In PDRs, stellar radiation impinges on the surface of dense material, often a molecular cloud, thereby inducing a complex network of chemical reactions and physical processes. Observations toward L1630 allow us to study the interplay between stellar radiation and a molecular cloud under relatively benign conditions, that is, intermediate densities and an intermediate UV radiation field. Contrary to the well-studied Orion Molecular Cloud 1 (OMC1), which hosts much harsher conditions, L1630 has little star formation. Our goal is to relate the [Cii] fine-structure line emission to the physical conditions predominant in L1630 and compare it to studies of OMC1. The [Cii] 158 μ m line emission of L1630 around the Horsehead Nebula, an area of 12' × 17', was observed using the upgraded German Receiver for Astronomy at Terahertz Frequencies (upGREAT) onboard the Stratospheric Observatory for Infrared Astronomy (SOFIA). Of the [Cii] emission from the mapped area 95%, 13 L ⊙ , originates from the molecular cloud; the adjacent Hii region contributes only 5%, that is, 1 L ⊙ . From comparison with other data (CO(1-0)-line emission, far-infrared (FIR) continuum studies, emission from polycyclic aromatic hydrocarbons (PAHs)), we infer a gas density of the molecular cloud of n H ∼ 3 · 10 3 cm -3 , with surface layers, including the Horsehead Nebula, having a density of up to n H ∼ 4 · 10 4 cm -3 . The temperature of the surface gas is T ∼ 100 K. The average [Cii] cooling efficiency within the molecular cloud is 1.3 · 10 -2 . The fraction of the mass of the molecular cloud within the studied area that is traced by [Cii] is only 8%. Our PDR models are able to reproduce the FIR-[Cii] correlations and also the CO(1-0)-[Cii] correlations. Finally, we compare our results on the heating efficiency of the

  3. Numerical simulation of convective generated gravity waves in the stratosphere and MLT regions.

    Science.gov (United States)

    Heale, C. J.; Snively, J. B.

    2017-12-01

    Convection is an important source of gravity wave generation, especially in the summer tropics and midlatitudes, and coherent wave fields above convection are now routinely measured in the stratosphere and mesosphere [e.g. Hoffmann et al., JGR, 118, 2013; Gong et al., JGR, 120, 2015; Perwitasari et al., GRL, 42, 22, 2016]. Numerical studies have been performed to investigate the generation mechanisms, source spectra, and their effects on the middle and upper atmosphere [e.g. Fovell et al., AMS, 49,16, 1992; Alexander and Holton, Atmos. Chem. Phys., 4 2004; Vincent et al., JGR, 1118, 2013], however there is still considerable work needed to fully describe these parameters. GCMs currently lack the resolution to explicitly simulate convection generation and rely on simplified parameterizations while full cloud resolving models are computationally expensive and often only extend into the stratosphere. More recent studies have improved the realism of these simulations by using radar derived precipitation rates to drive latent heating in models that simulate convection [Grimsdell et al., AMS, 67, 2010; Stephan and Alexander., J. Adv. Model. Earth. Syst, 7, 2015], however they too only consider wave propagation in the troposphere and stratosphere. We use a 2D nonlinear, fully compressible model [Snively and Pasko., JGR, 113, 2008] to excite convectively generated waves, based on NEXRAD radar data, using the Stephan and Alexander [2015] algorithms. We study the propagation, and spectral evolution of the generated waves up into the MLT region. Ambient atmosphere parameters are derived from observations and MERRA-2 reanalysis data, and stratospheric (AIRS) and mesospheric (Lidar, OH airglow) observations enable comparisons with simulation results.

  4. Causes and impacts of changes in the stratospheric meridional circulation in a chemistry-climate model

    Energy Technology Data Exchange (ETDEWEB)

    Garny, Hella

    2011-05-13

    The stratospheric meridional circulation is projected to be subject to changes due to enhanced greenhouse-gas concentrations in the atmosphere. This study aims to diagnose and explain long-term changes in the stratospheric meridional circulation using the chemistry-climate model E39CA. The diagnosed strengthening of the circulation is found to be driven by increases in tropical sea surface temperatures which lead to a strengthening and upward shift of the subtropical jets. This enables enhanced vertical propagation of large scale waves into the lower stratosphere, and therefore stronger local wave forcing of the meridional circulation in the tropical lower stratosphere. The impact of changes in transport on the ozone layer is analysed using a newly developed method that allows the separation of the effects of transport and chemistry changes on ozone. It is found that future changes of mean stratospheric ozone concentrations are largely determined by changes in chemistry, while changes in transport of ozone play a minor role. (orig.)

  5. Quantifying Diurnal Cloud Radiative Effects by Cloud Type in the Tropical Western Pacific

    Energy Technology Data Exchange (ETDEWEB)

    Burleyson, Casey D.; Long, Charles N.; Comstock, Jennifer M.

    2015-06-01

    Cloud radiative effects are examined using long-term datasets collected at the three Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Climate Research Facilities in the tropical western Pacific. We quantify the surface radiation budget, cloud populations, and cloud radiative effects by partitioning the data by cloud type, time of day, and as a function of large scale modes of variability such as El Niño Southern Oscillation (ENSO) phase and wet/dry seasons at Darwin. The novel facet of our analysis is that we break aggregate cloud radiative effects down by cloud type across the diurnal cycle. The Nauru cloud populations and subsequently the surface radiation budget are strongly impacted by ENSO variability whereas the cloud populations over Manus only shift slightly in response to changes in ENSO phase. The Darwin site exhibits large seasonal monsoon related variations. We show that while deeper convective clouds have a strong conditional influence on the radiation reaching the surface, their limited frequency reduces their aggregate radiative impact. The largest source of shortwave cloud radiative effects at all three sites comes from low clouds. We use the observations to demonstrate that potential model biases in the amplitude of the diurnal cycle and mean cloud frequency would lead to larger errors in the surface energy budget compared to biases in the timing of the diurnal cycle of cloud frequency. Our results provide solid benchmarks to evaluate model simulations of cloud radiative effects in the tropics.

  6. Composite Materials With Uncured Epoxy Matrix Exposed in Stratosphere During NASA Stratospheric Balloon Flight

    Science.gov (United States)

    Kondyurin, Alexey; Kondyurina, Irina; Bilek, Marcela; de Groh, Kim K.

    2013-01-01

    A cassette of uncured composite materials with epoxy resin matrixes was exposed in the stratosphere (40 km altitude) over three days. Temperature variations of -76 to 32.5C and pressure up to 2.1 torr were recorded during flight. An analysis of the chemical structure of the composites showed, that the polymer matrix exposed in the stratosphere becomes crosslinked, while the ground control materials react by way of polymerization reaction of epoxy groups. The space irradiations are considered to be responsible for crosslinking of the uncured polymers exposed in the stratosphere. The composites were cured on Earth after landing. Analysis of the cured composites showed that the polymer matrix remains active under stratospheric conditions. The results can be used for predicting curing processes of polymer composites in a free space environment during an orbital space flight.

  7. Tropical troposphere to stratosphere transport of carbon monoxide and long-lived trace species in the Chemical Lagrangian Model of the Stratosphere (CLaMS

    Directory of Open Access Journals (Sweden)

    R. Pommrich

    2014-12-01

    Full Text Available Variations in the mixing ratio of trace gases of tropospheric origin entering the stratosphere in the tropics are of interest for assessing both troposphere to stratosphere transport fluxes in the tropics and the impact of these transport fluxes on the composition of the tropical lower stratosphere. Anomaly patterns of carbon monoxide (CO and long-lived tracers in the lower tropical stratosphere allow conclusions about the rate and the variability of tropical upwelling to be drawn. Here, we present a simplified chemistry scheme for the Chemical Lagrangian Model of the Stratosphere (CLaMS for the simulation, at comparatively low numerical cost, of CO, ozone, and long-lived trace substances (CH4, N2O, CCl3F (CFC-11, CCl2F2 (CFC-12, and CO2 in the lower tropical stratosphere. For the long-lived trace substances, the boundary conditions at the surface are prescribed based on ground-based measurements in the lowest model level. The boundary condition for CO in the lower troposphere (below about 4 km is deduced from MOPITT measurements. Due to the lack of a specific representation of mixing and convective uplift in the troposphere in this model version, enhanced CO values, in particular those resulting from convective outflow are underestimated. However, in the tropical tropopause layer and the lower tropical stratosphere, there is relatively good agreement of simulated CO with in situ measurements (with the exception of the TROCCINOX campaign, where CO in the simulation is biased low ≈10–15 ppbv. Further, the model results (and therefore also the ERA-Interim winds, on which the transport in the model is based are of sufficient quality to describe large scale anomaly patterns of CO in the lower stratosphere. In particular, the zonally averaged tropical CO anomaly patterns (the so called "tape recorder" patterns simulated by this model version of CLaMS are in good agreement with observations, although the simulations show a too rapid upwelling

  8. Impacts of Stratospheric Sulfate Geoengineering on PM2.5

    Science.gov (United States)

    Robock, A.; Xia, L.; Tilmes, S.; Mills, M. J.; Richter, J.; Kravitz, B.; MacMartin, D.

    2017-12-01

    Particulate matter (PM) includes sulfate, nitrate, organic carbon, elemental carbon, soil dust, and sea salt. The first four components are mostly present near the ground as fine particulate matter with a diameter less than 2.5 µm (PM2.5), and these are of the most concern for human health. PM is efficiently scavenged by precipitation, which is its main atmospheric sink. Here we examine the impact of stratospheric climate engineering on this important pollutant and health risk, taking advantage of two sets of climate model simulations conducted at the National Center for Atmospheric Research. We use the full tropospheric and stratospheric chemistry version of the Community Earth System Model - Community Atmospheric Model 4 (CESM CAM4-chem) with a horizontal resolution of 0.9° x 1.25° lat-lon to simulate a stratospheric sulfate injection climate intervention of 8 Tg SO2 yr-1 combined with an RCP6.0 global warming forcing, the G4 Specified Stratospheric Aerosol (G4SSA) scenario. We also analyze the output from a 20-member ensemble of Community Earth System Model, version 1 with the Whole Atmosphere Community Climate Model as its atmospheric component (CESM1(WACCM)) simulations, also at 0.9° x 1.25° lat-lon resolution, with sulfur dioxide injection at 15°N, 15°S, 30°N, and 30°S varying in time to balance RCP8.5 forcing. While the CESM CAM4-chem model has full tropospheric and stratospheric chemistry, CESM1(WACCM) has an internally generated quasi-biennial oscillation and a comprehensive tropospheric and stratospheric sulfate aerosol treatment, but only stratospheric chemistry. For G4SSA, there are a global temperature reduction of 0.8 K and global averaged precipitation decrease of 3% relative to RCP6.0. The global averaged surface PM2.5 reduces about 1% compared with RCP6.0, mainly over Eurasian and East Asian regions in Northern Hemisphere winter. The PM2.5 concentration change is a combination of effects from tropospheric chemistry and precipitation

  9. Stratospheric ozone changes under solar geoengineering: implications for UV exposure and air quality

    Directory of Open Access Journals (Sweden)

    P. J. Nowack

    2016-03-01

    Full Text Available Various forms of geoengineering have been proposed to counter anthropogenic climate change. Methods which aim to modify the Earth's energy balance by reducing insolation are often subsumed under the term solar radiation management (SRM. Here, we present results of a standard SRM modelling experiment in which the incoming solar irradiance is reduced to offset the global mean warming induced by a quadrupling of atmospheric carbon dioxide. For the first time in an atmosphere–ocean coupled climate model, we include atmospheric composition feedbacks for this experiment. While the SRM scheme considered here could offset greenhouse gas induced global mean surface warming, it leads to important changes in atmospheric composition. We find large stratospheric ozone increases that induce significant reductions in surface UV-B irradiance, which would have implications for vitamin D production. In addition, the higher stratospheric ozone levels lead to decreased ozone photolysis in the troposphere. In combination with lower atmospheric specific humidity under SRM, this results in overall surface ozone concentration increases in the idealized G1 experiment. Both UV-B and surface ozone changes are important for human health. We therefore highlight that both stratospheric and tropospheric ozone changes must be considered in the assessment of any SRM scheme, due to their important roles in regulating UV exposure and air quality.

  10. Complex chemical composition of colored surface films formed from reactions of propanal in sulfuric acid at upper troposphere/lower stratosphere aerosol acidities.

    Science.gov (United States)

    Van Wyngarden, A L; Pérez-Montaño, S; Bui, J V H; Li, E S W; Nelson, T E; Ha, K T; Leong, L; Iraci, L T

    Particles in the upper troposphere and lower stratosphere (UT/LS) consist mostly of concentrated sulfuric acid (40-80 wt %) in water. However, airborne measurements have shown that these particles also contain a significant fraction of organic compounds of unknown chemical composition. Acid-catalyzed reactions of carbonyl species are believed to be responsible for significant transfer of gas phase organic species into tropospheric aerosols and are potentially more important at the high acidities characteristic of UT/LS particles. In this study, experiments combining sulfuric acid (H 2 SO 4 ) with propanal and with mixtures of propanal with glyoxal and/or methylglyoxal at acidities typical of UT/LS aerosols produced highly colored surface films (and solutions) that may have implications for aerosol properties. In order to identify the chemical processes responsible for the formation of the surface films, attenuated total reflectance-Fourier transform infrared (ATR-FTIR) and 1 H nuclear magnetic resonance (NMR) spectroscopies were used to analyze the chemical composition of the films. Films formed from propanal were a complex mixture of aldol condensation products, acetals and propanal itself. The major aldol condensation products were the dimer (2-methyl-2-pentenal) and 1,3,5-trimethylbenzene that was formed by cyclization of the linear aldol condensation trimer. Additionally, the strong visible absorption of the films indicates that higher-order aldol condensation products must also be present as minor species. The major acetal species were 2,4,6-triethyl-1,3,5-trioxane and longer-chain linear polyacetals which are likely to separate from the aqueous phase. Films formed on mixtures of propanal with glyoxal and/or methylglyoxal also showed evidence of products of cross-reactions. Since cross-reactions would be more likely than self-reactions under atmospheric conditions, similar reactions of aldehydes like propanal with common aerosol organic species like glyoxal

  11. Lidar investigations on the optical and dynamical properties of cirrus clouds in the upper troposphere and lower stratosphere regions at a tropical station, Gadanki, India (13.5°N, 79.2°E)

    Science.gov (United States)

    Krishnakumar, Vasudevannair; Satyanarayana, Malladi; Radhakrishnan, Soman R.; Dhaman, Reji K.; Jayeshlal, Glory Selvan; Motty, Gopinathan Nair S.; Pillai, Vellara P. Mahadevan; Raghunath, Karnam; Ratnam, Madineni Venkat; Rao, Duggirala Ramakrishna; Sudhakar, Pindlodi

    2014-01-01

    High altitude cirrus clouds are composed mainly of ice crystals with a variety of sizes and shapes. They have a large influence on Earth's energy balance and global climate. Recent studies indicate that the formation, dissipation, life time, optical, and micro-physical properties are influenced by the dynamical conditions of the surrounding atmosphere like background aerosol, turbulence, etc. In this work, an attempt has been made to quantify some of these characteristics by using lidar and mesosphere-stratosphere-troposphere (MST) radar. Mie lidar and 53 MHz MST radar measurements made over 41 nights during the period 2009 to 2010 from the tropical station, Gadanki, India (13.5°N, 79.2°E). The optical and microphysical properties along with the structure and dynamics of the cirrus are presented as observed under different atmospheric conditions. The study reveals the manifestation of different forms of cirrus with a preferred altitude of formation in the 13 to 14 km altitude. There are considerable differences in the properties obtained among 2009 and 2010 showing significant anomalous behavior in 2010. The clouds observed during 2010 show relatively high asymmetry and large multiple scattering effects. The anomalies found during 2010 may be attributed to the turbulence noticed in the surrounding atmosphere. The results show a clear correlation between the crystal morphology in the clouds and the dynamical conditions of the prevailing atmosphere during the observational period.

  12. An energy balance model exploration of the impacts of interactions between surface albedo, cloud cover and water vapor on polar amplification

    Science.gov (United States)

    Södergren, A. Helena; McDonald, Adrian J.; Bodeker, Gregory E.

    2017-11-01

    We examine the effects of non-linear interactions between surface albedo, water vapor and cloud cover (referred to as climate variables) on amplified warming of the polar regions, using a new energy balance model. Our simulations show that the sum of the contributions to surface temperature changes due to any variable considered in isolation is smaller than the temperature changes from coupled feedback simulations. This non-linearity is strongest when all three climate variables are allowed to interact. Surface albedo appears to be the strongest driver of this non-linear behavior, followed by water vapor and clouds. This is because increases in longwave radiation absorbed by the surface, related to increases in water vapor and clouds, and increases in surface absorbed shortwave radiation caused by a decrease in surface albedo, amplify each other. Furthermore, our results corroborate previous findings that while increases in cloud cover and water vapor, along with the greenhouse effect itself, warm the polar regions, water vapor also significantly warms equatorial regions, which reduces polar amplification. Changes in surface albedo drive large changes in absorption of incoming shortwave radiation, thereby enhancing surface warming. Unlike high latitudes, surface albedo change at low latitudes are more constrained. Interactions between surface albedo, water vapor and clouds drive larger increases in temperatures in the polar regions compared to low latitudes. This is in spite of the fact that, due to a forcing, cloud cover increases at high latitudes and decreases in low latitudes, and that water vapor significantly enhances warming at low latitudes.

  13. The Diurnal Cycle of the Boundary Layer, Convection, Clouds, and Surface Radiation in a Coastal Monsoon Environment (Darwin Australia)

    Energy Technology Data Exchange (ETDEWEB)

    May, Peter T.; Long, Charles N.; Protat, Alain

    2012-08-01

    The diurnal variation of convection and associated cloud and radiative properties remains a significant issue in global NWP and climate models. This study analyzes observed diurnal variability of convection in a coastal monsoonal environment examining the interaction of convective rain clouds, their associated cloud properties, and the impact on the surface radiation and corresponding boundary layer structure during periods where convection is suppressed or active on the large scale. The analysis uses data from the Tropical Warm Pool International Cloud Experiment (TWP-ICE) as well as routine measurements from the Australian Bureau of Meteorology and the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) program. Both active monsoonal and large-scale suppressed (buildup and break) conditions are examined and demonstrate that the diurnal variation of rainfall is much larger during the break periods and the spatial distribution of rainfall is very different between the monsoon and break regimes. During the active monsoon the total net radiative input to the surface is decreased by more than 3 times the amount than during the break regime - this total radiative cloud forcing is found to be dominated by the shortwave (SW) cloud effects because of the much larger optical thicknesses and persistence of long-lasting anvils and cirrus cloud decks associated with the monsoon regime. These differences in monsoon versus break surface radiative energy contribute to low-level air temperature differences in the boundary layer over the land surfaces.

  14. A 10-Year Climatology of Cloud Cover and Vertical Distribution Derived from Both Surface and GOES Observations Over the DOE ARM SGP Site

    Science.gov (United States)

    Xi, Baike; Dong, Xiquan; Minnis, P.; Khaiyer, M.

    2010-01-01

    Analysis of a decade of ARM radar-lidar and GOES observations at the SGP site reveal that 0.5 and 4-hr averages of the surface cloud fraction correspond closely to 0.5deg and 2.5deg averages of GOES cloudiness, respectively. The long-term averaged surface and GOES cloud fractions agree to within 0.5%. Cloud frequency increases and cloud amount decreases as the temporal and spatial averaging scales increase. Clouds occurred most often during winter and spring. Single-layered clouds account for 61.5% of the total cloud frequency. There are distinct bimodal vertical distributions of clouds with a lower peak around 1 km and an upper one that varies from 7.5 to 10.8 km between winter and summer, respectively. The frequency of occurrence for nighttime GOES high-cloud tops agree well with the surface observations, but are underestimated during the day.

  15. A global space-based stratospheric aerosol climatology: 1979–2016

    Directory of Open Access Journals (Sweden)

    L. W. Thomason

    2018-03-01

    Full Text Available We describe the construction of a continuous 38-year record of stratospheric aerosol optical properties. The Global Space-based Stratospheric Aerosol Climatology, or GloSSAC, provided the input data to the construction of the Climate Model Intercomparison Project stratospheric aerosol forcing data set (1979–2014 and we have extended it through 2016 following an identical process. GloSSAC focuses on the Stratospheric Aerosol and Gas Experiment (SAGE series of instruments through mid-2005, and on the Optical Spectrograph and InfraRed Imager System (OSIRIS and the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO data thereafter. We also use data from other space instruments and from ground-based, air, and balloon borne instruments to fill in key gaps in the data set. The end result is a global and gap-free data set focused on aerosol extinction coefficient at 525 and 1020 nm and other parameters on an "as available" basis. For the primary data sets, we developed a new method for filling the post-Pinatubo eruption data gap for 1991–1993 based on data from the Cryogenic Limb Array Etalon Spectrometer. In addition, we developed a new method for populating wintertime high latitudes during the SAGE period employing a latitude-equivalent latitude conversion process that greatly improves the depiction of aerosol at high latitudes compared to earlier similar efforts. We report data in the troposphere only when and where it is available. This is primarily during the SAGE II period except for the most enhanced part of the Pinatubo period. It is likely that the upper troposphere during Pinatubo was greatly enhanced over non-volcanic periods and that domain remains substantially under-characterized. We note that aerosol levels during the OSIRIS/CALIPSO period in the lower stratosphere at mid- and high latitudes is routinely higher than what we observed during the SAGE II period. While this period had nearly continuous low

  16. Effects of sea surface temperature, cloud radiative and microphysical processes, and diurnal variations on rainfall in equilibrium cloud-resolving model simulations

    International Nuclear Information System (INIS)

    Jiang Zhe; Li Xiao-Fan; Zhou Yu-Shu; Gao Shou-Ting

    2012-01-01

    The effects of sea surface temperature (SST), cloud radiative and microphysical processes, and diurnal variations on rainfall statistics are documented with grid data from the two-dimensional equilibrium cloud-resolving model simulations. For a rain rate of higher than 3 mm·h −1 , water vapor convergence prevails. The rainfall amount decreases with the decrease of SST from 29 °C to 27 °C, the inclusion of diurnal variation of SST, or the exclusion of microphysical effects of ice clouds and radiative effects of water clouds, which are primarily associated with the decreases in water vapor convergence. However, the amount of rainfall increases with the increase of SST from 29 °C to 31 °C, the exclusion of diurnal variation of solar zenith angle, and the exclusion of the radiative effects of ice clouds, which are primarily related to increases in water vapor convergence. For a rain rate of less than 3 mm·h −1 , water vapor divergence prevails. Unlike rainfall statistics for rain rates of higher than 3 mm·h −1 , the decrease of SST from 29 °C to 27 °C and the exclusion of radiative effects of water clouds in the presence of radiative effects of ice clouds increase the rainfall amount, which corresponds to the suppression in water vapor divergence. The exclusion of microphysical effects of ice clouds decreases the amount of rainfall, which corresponds to the enhancement in water vapor divergence. The amount of rainfall is less sensitive to the increase of SST from 29 °C to 31 °C and to the radiative effects of water clouds in the absence of the radiative effects of ice clouds. (electromagnetism, optics, acoustics, heat transfer, classical mechanics, and fluid dynamics)

  17. Airborne hyperspectral observations of surface and cloud directional reflectivity using a commercial digital camera

    Directory of Open Access Journals (Sweden)

    A. Ehrlich

    2012-04-01

    Full Text Available Spectral radiance measurements by a digital single-lens reflex camera were used to derive the directional reflectivity of clouds and different surfaces in the Arctic. The camera has been calibrated radiometrically and spectrally to provide accurate radiance measurements with high angular resolution. A comparison with spectral radiance measurements with the Spectral Modular Airborne Radiation measurement sysTem (SMART-Albedometer showed an agreement within the uncertainties of both instruments (6% for both. The directional reflectivity in terms of the hemispherical directional reflectance factor (HDRF was obtained for sea ice, ice-free ocean and clouds. The sea ice, with an albedo of ρ = 0.96 (at 530 nm wavelength, showed an almost isotropic HDRF, while sun glint was observed for the ocean HDRF (ρ = 0.12. For the cloud observations with ρ = 0.62, the cloudbow – a backscatter feature typically for scattering by liquid water droplets – was covered by the camera. For measurements above heterogeneous stratocumulus clouds, the required number of images to obtain a mean HDRF that clearly exhibits the cloudbow has been estimated at about 50 images (10 min flight time. A representation of the HDRF as a function of the scattering angle only reduces the image number to about 10 (2 min flight time.

    The measured cloud and ocean HDRF have been compared to radiative transfer simulations. The ocean HDRF simulated with the observed surface wind speed of 9 m s−1 agreed best with the measurements. For the cloud HDRF, the best agreement was obtained by a broad and weak cloudbow simulated with a cloud droplet effective radius of Reff = 4 μm. This value agrees with the particle sizes derived from in situ measurements and retrieved from the spectral radiance of the SMART-Albedometer.

  18. El Chichon and 'mystery cloud' aerosols between 30 and 55 km Global observations from the SME visible spectrometer

    Science.gov (United States)

    Clancy, R. T.

    1986-01-01

    Visible limb radiances measured by the Solar Mesosphere Explorer (SME) are used to obtain volume scattering ratios for aerosol loading in the 30-55 km altitude range of the stratosphere. Global maps of these ratios are presented for the period January 1982 to August 1984. Significant aerosol scattering from the 'mystery cloud' and El Chichon aerosol layers are found above 30 km. A timescale of approximately 2 months between the appearance of the aerosol at 30.5 km and at 37.5 km is consistent with vertical transport of aerosol or vapor by eddy diffusion above 30 km. An anticorrelation exists between aerosol scattering and stratospheric temperatures. Periods of lower stratospheric temperatures may account for the formation of aerosol between 40 and 55 km altitude.

  19. Cloud Masking and Surface Temperature Distribution in the Polar Regions Using AVHRR and other Satellite Data

    Science.gov (United States)

    Comiso, Joey C.

    1995-01-01

    Surface temperature is one of the key variables associated with weather and climate. Accurate measurements of surface air temperatures are routinely made in meteorological stations around the world. Also, satellite data have been used to produce synoptic global temperature distributions. However, not much attention has been paid on temperature distributions in the polar regions. In the polar regions, the number of stations is very sparse. Because of adverse weather conditions and general inaccessibility, surface field measurements are also limited. Furthermore, accurate retrievals from satellite data in the region have been difficult to make because of persistent cloudiness and ambiguities in the discrimination of clouds from snow or ice. Surface temperature observations are required in the polar regions for air-sea-ice interaction studies, especially in the calculation of heat, salinity, and humidity fluxes. They are also useful in identifying areas of melt or meltponding within the sea ice pack and the ice sheets and in the calculation of emissivities of these surfaces. Moreover, the polar regions are unique in that they are the sites of temperature extremes, the location of which is difficult to identify without a global monitoring system. Furthermore, the regions may provide an early signal to a potential climate change because such signal is expected to be amplified in the region due to feedback effects. In cloud free areas, the thermal channels from infrared systems provide surface temperatures at relatively good accuracies. Previous capabilities include the use of the Temperature Humidity Infrared Radiometer (THIR) onboard the Nimbus-7 satellite which was launched in 1978. Current capabilities include the use of the Advance Very High Resolution Radiometer (AVHRR) aboard NOAA satellites. Together, these two systems cover a span of 16 years of thermal infrared data. Techniques for retrieving surface temperatures with these sensors in the polar regions have

  20. MIPAS detection of cloud and aerosol particle occurrence in the UTLS with comparison to HIRDLS and CALIOP

    Directory of Open Access Journals (Sweden)

    H. Sembhi

    2012-10-01

    Full Text Available Satellite infrared emission instruments require efficient systems that can separate and flag observations which are affected by clouds and aerosols. This paper investigates the identification of cloud and aerosols from infrared, limb sounding spectra that were recorded by the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS, a high spectral resolution Fourier transform spectrometer on the European Space Agency's (ESA ENVISAT (Now inoperative since April 2012 due to loss of contact. Specifically, the performance of an existing cloud and aerosol particle detection method is simulated with a radiative transfer model in order to establish, for the first time, confident detection limits for particle presence in the atmosphere from MIPAS data. The newly established thresholds improve confidence in the ability to detect particle injection events, plume transport in the upper troposphere and lower stratosphere (UTLS and better characterise cloud distributions utilising MIPAS spectra. The method also provides a fast front-end detection system for the MIPClouds processor; a processor designed for the retrieval of macro- and microphysical cloud properties from the MIPAS data.

    It is shown that across much of the stratosphere, the threshold for the standard cloud index in band A is 5.0 although threshold values of over 6.0 occur in restricted regimes. Polar regions show a surprising degree of uncertainty at altitudes above 20 km, potentially due to changing stratospheric trace gas concentrations in polar vortex conditions and poor signal-to-noise due to cold atmospheric temperatures. The optimised thresholds of this study can be used for much of the time, but time/composition-dependent thresholds are recommended for MIPAS data for the strongly perturbed polar stratosphere. In the UT, a threshold of 5.0 applies at 12 km and above but decreases rapidly at lower altitudes. The new thresholds are shown to allow much more sensitive

  1. The major stratospheric final warming in 2016: dispersal of vortex air and termination of Arctic chemical ozone loss

    Directory of Open Access Journals (Sweden)

    G. L. Manney

    2016-12-01

    Full Text Available The 2015/16 Northern Hemisphere winter stratosphere appeared to have the greatest potential yet seen for record Arctic ozone loss. Temperatures in the Arctic lower stratosphere were at record lows from December 2015 through early February 2016, with an unprecedented period of temperatures below ice polar stratospheric cloud thresholds. Trace gas measurements from the Aura Microwave Limb Sounder (MLS show that exceptional denitrification and dehydration, as well as extensive chlorine activation, occurred throughout the polar vortex. Ozone decreases in 2015/16 began earlier and proceeded more rapidly than those in 2010/11, a winter that saw unprecedented Arctic ozone loss. However, on 5–6 March 2016 a major final sudden stratospheric warming ("major final warming", MFW began. By mid-March, the mid-stratospheric vortex split after being displaced far off the pole. The resulting offspring vortices decayed rapidly preceding the full breakdown of the vortex by early April. In the lower stratosphere, the period of temperatures low enough for chlorine activation ended nearly a month earlier than that in 2011 because of the MFW. Ozone loss rates were thus kept in check because there was less sunlight during the cold period. Although the winter mean volume of air in which chemical ozone loss could occur was as large as that in 2010/11, observed ozone values did not drop to the persistently low values reached in 2011.We use MLS trace gas measurements, as well as mixing and polar vortex diagnostics based on meteorological fields, to show how the timing and intensity of the MFW and its impact on transport and mixing halted chemical ozone loss. Our detailed characterization of the polar vortex breakdown includes investigations of individual offspring vortices and the origins and fate of air within them. Comparisons of mixing diagnostics with lower-stratospheric N2O and middle-stratospheric CO from MLS (long-lived tracers show rapid vortex erosion and

  2. Stratospheric Temperature Trends Observed by TIMED/SABER

    Science.gov (United States)

    Xian, T.; Tan, R.

    2017-12-01

    Trends in the stratospheric temperature are studied based on the temperature profile observation from the Sounding of the Atmosphere using Broadband Emission Radiometry (SABER). The spatially trends are evaluated in different time scales ranging from decadal to monthly resolved. The results indicate a signature of BDC acceleration. There are strong warming trends (up to 9 K/decade) in the middle to upper stratosphere in the high latitude spring, summer, and autumn seasons, accompanied by strong cooling trends in the lower stratosphere. Besides, strong warming trends occurs through the whole stratosphere over the Southern Hemisphere, which confirms Antarctic ozone layer healing since 2000. In addition, the results demonstrate a significant warming trends in the middle of tropical stratosphere, which becomes strongest during June-July-August.

  3. Solid-State Chemistry as a Formation Mechanism for C 4N 2 Ice and Possibly the Haystack (220 cm -1 ice emission feature) in Titan's Stratosphere as Observed by Cassini CIRS

    Science.gov (United States)

    Anderson, Carrie; Samuelson, Robert E.; McLain, Jason L.; Nna Mvondo, Delphine; Romani, Paul; Flasar, F. Michael

    2016-10-01

    A profusion of organic ices containing hydrocarbons, nitriles, and combinations of their mixtures comprise Titan's complex stratospheric cloud systems, and are typically formed via vapor condensation. These ice particles are then distributed throughout the mid-to-lower stratosphere, with an increased abundance near the winter poles (see Anderson et al., 2016). The cold temperatures and the associated strong circumpolar winds that isolate polar air act in much the same way as on Earth, giving rise to compositional anomalies and stratospheric clouds that provide heterogeneous chemistry sites.Titan's C4N2 ice emission feature at 478 cm-1 and "the Haystack," a strong unidentified stratospheric ice emission feature centered at 220 cm-1, share a common characteristic. Even though both are distinctive ice emission features evident in Cassini Composite InfraRed (CIRS) far-IR spectra, no associated vapor emission features can be found in Titan's atmosphere. Without a vapor phase, solid-state chemistry provides an alternate mechanism beside vapor condensation for producing these observed stratospheric ices.Anderson et al., (2016) postulated that C4N2 ice formed in Titan's stratosphere via the solid-state photochemical reaction HCN + HC3N → C4N2 + H2 can occur within extant HCN-HC3N composite ice particles. Such a reaction, and potentially similar reactions that may produce the Haystack ice, are specific examples of solid-state chemistry in solar system atmospheres. This is in addition to the reaction HCl + ClONO2 → HNO3 + Cl2, which is known to produce HNO3 coatings on terrestrial water ice particles, a byproduct of the catalytic chlorine chemistry that produces ozone holes in Earth's polar stratosphere (see for example, Molina et al., 1987 Soloman, 1999).A combination of radiative transfer modeling of CIRS far-IR spectra, coupled with optical constants derived from thin film transmittance spectra of organic ice mixtures obtained in our Spectroscopy for Planetary ICes

  4. Progress in Understanding Land-Surface-Atmosphere Coupling from LBA Research

    Directory of Open Access Journals (Sweden)

    Alan K Betts

    2010-06-01

    Full Text Available LBA research has deepened our understanding of the role of soil water storage, clouds and aerosols in land-atmosphere coupling. We show how the reformulation of cloud forcing in terms of an effective cloud albedo per unit area of surface gives a useful measure of the role of clouds in the surface energy budget over the Amazon. We show that the diurnal temperature range has a quasi-linear relation to the daily mean longwave cooling; and to effective cloud albedo because of the tight coupling between the near-surface climate, the boundary layer and the cloud field. The coupling of surface and atmospheric processes is critical to the seasonal cycle: deep forest rooting systems make water available throughout the year, whereas in the dry season the shortwave cloud forcing is reduced by regional scale subsidence, so that more light is available for photosynthesis. At sites with an annual precipitation above 1900 mm and a dry season length less than 4 months, evaporation rates increased in the dry season, coincident with increased radiation. In contrast, ecosystems with precipitation less than 1700 mm and a longer dry season showed clear evidence of reduced evaporation in the dry season coming from water stress. In all these sites, the seasonal variation of the effective cloud albedo is a major factor in determining the surface available energy. Dry season fires add substantial aerosol to the atmosphere. Aerosol scattering and absorption both reduce the total downward surface radiative flux, but increase the diffuse/direct flux ratio, which increases photosynthetic efficiency. Convective plumes produced by fires enhance the vertical transport of aerosols over the Amazon, and effectively inject smoke aerosol and gases directly into the middle troposphere with substantial impacts on mid- tropospheric dispersion. In the rainy season in Rondônia, convection in low-level westerly flows with low aerosol content resembles oceanic convection with

  5. A Lightweight Surface Reconstruction Method for Online 3D Scanning Point Cloud Data Oriented toward 3D Printing

    Directory of Open Access Journals (Sweden)

    Buyun Sheng

    2018-01-01

    Full Text Available The existing surface reconstruction algorithms currently reconstruct large amounts of mesh data. Consequently, many of these algorithms cannot meet the efficiency requirements of real-time data transmission in a web environment. This paper proposes a lightweight surface reconstruction method for online 3D scanned point cloud data oriented toward 3D printing. The proposed online lightweight surface reconstruction algorithm is composed of a point cloud update algorithm (PCU, a rapid iterative closest point algorithm (RICP, and an improved Poisson surface reconstruction algorithm (IPSR. The generated lightweight point cloud data are pretreated using an updating and rapid registration method. The Poisson surface reconstruction is also accomplished by a pretreatment to recompute the point cloud normal vectors; this approach is based on a least squares method, and the postprocessing of the PDE patch generation was based on biharmonic-like fourth-order PDEs, which effectively reduces the amount of reconstructed mesh data and improves the efficiency of the algorithm. This method was verified using an online personalized customization system that was developed with WebGL and oriented toward 3D printing. The experimental results indicate that this method can generate a lightweight 3D scanning mesh rapidly and efficiently in a web environment.

  6. Shortwave surface radiation network for observing small-scale cloud inhomogeneity fields

    Science.gov (United States)

    Lakshmi Madhavan, Bomidi; Kalisch, John; Macke, Andreas

    2016-03-01

    As part of the High Definition Clouds and Precipitation for advancing Climate Prediction Observational Prototype Experiment (HOPE), a high-density network of 99 silicon photodiode pyranometers was set up around Jülich (10 km × 12 km area) from April to July 2013 to capture the small-scale variability of cloud-induced radiation fields at the surface. In this paper, we provide the details of this unique setup of the pyranometer network, data processing, quality control, and uncertainty assessment under variable conditions. Some exemplary days with clear, broken cloudy, and overcast skies were explored to assess the spatiotemporal observations from the network along with other collocated radiation and sky imager measurements available during the HOPE period.

  7. Variability of cirrus clouds in a convective outflow during the Hibiscus campaign

    Science.gov (United States)

    Fierli, F.; di Donfrancesco, G.; Cairo, F.; Marécal, V.; Zampieri, M.; Orlandi, E.; Durry, G.

    2008-08-01

    Light-weight microlidar and water vapour measurements were taken on-board a stratospheric balloon during the HIBISCUS 2004 campaign, held in Bauru, Brazil (49° W, 22° S). Cirrus clouds were observed throughout the flight between 12 and 15 km height with a high mesoscale variability in optical and microphysical properties. It was found that the cirrus clouds were composed of different layers characterized by marked differences in height, thickness and optical properties. Simultaneous water vapour observations show that the different layers are characterized by different values of the saturation with respect to ice. A mesoscale simulation and a trajectory analysis clearly revealed that the clouds had formed in the outflow of a large and persistent convective region and that the observed variability of the optical properties and of the cloud structure is likely linked to the different residence times of the convectively-processed air in the upper troposphere.

  8. An assessment of thin cloud detection by applying bidirectional reflectance distribution function model-based background surface reflectance using Geostationary Ocean Color Imager (GOCI): A case study for South Korea

    Science.gov (United States)

    Kim, Hye-Won; Yeom, Jong-Min; Shin, Daegeun; Choi, Sungwon; Han, Kyung-Soo; Roujean, Jean-Louis

    2017-08-01

    In this study, a new assessment of thin cloud detection with the application of bidirectional reflectance distribution function (BRDF) model-based background surface reflectance was undertaken by interpreting surface spectra characterized using the Geostationary Ocean Color Imager (GOCI) over a land surface area. Unlike cloud detection over the ocean, the detection of cloud over land surfaces is difficult due to the complicated surface scattering characteristics, which vary among land surface types. Furthermore, in the case of thin clouds, in which the surface and cloud radiation are mixed, it is difficult to detect the clouds in both land and atmospheric fields. Therefore, to interpret background surface reflectance, especially underneath cloud, the semiempirical BRDF model was used to simulate surface reflectance by reflecting solar angle-dependent geostationary sensor geometry. For quantitative validation, Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) data were used to make a comparison with the proposed cloud masking result. As a result, the new cloud masking scheme resulted in a high probability of detection (POD = 0.82) compared with the Moderate Resolution Imaging Spectroradiometer (MODIS) (POD = 0.808) for all cloud cases. In particular, the agreement between the CALIPSO cloud product and new GOCI cloud mask was over 94% when detecting thin cloud (e.g., altostratus and cirrus) from January 2014 to June 2015. This result is relatively high in comparison with the result from the MODIS Collection 6 cloud mask product (MYD35).

  9. On the aliasing of the solar cycle in the lower stratospheric tropical temperature

    Science.gov (United States)

    Kuchar, Ales; Ball, William T.; Rozanov, Eugene V.; Stenke, Andrea; Revell, Laura; Miksovsky, Jiri; Pisoft, Petr; Peter, Thomas

    2017-09-01

    The double-peaked response of the tropical stratospheric temperature profile to the 11 year solar cycle (SC) has been well documented. However, there are concerns about the origin of the lower peak due to potential aliasing with volcanic eruptions or the El Niño-Southern Oscillation (ENSO) detected using multiple linear regression analysis. We confirm the aliasing using the results of the chemistry-climate model (CCM) SOCOLv3 obtained in the framework of the International Global Atmospheric Chemisty/Stratosphere-troposphere Processes And their Role in Climate Chemistry-Climate Model Initiative phase 1. We further show that even without major volcanic eruptions included in transient simulations, the lower stratospheric response exhibits a residual peak when historical sea surface temperatures (SSTs)/sea ice coverage (SIC) are used. Only the use of climatological SSTs/SICs in addition to background stratospheric aerosols removes volcanic and ENSO signals and results in an almost complete disappearance of the modeled solar signal in the lower stratospheric temperature. We demonstrate that the choice of temporal subperiod considered for the regression analysis has a large impact on the estimated profile signal in the lower stratosphere: at least 45 consecutive years are needed to avoid the large aliasing effect of SC maxima with volcanic eruptions in 1982 and 1991 in historical simulations, reanalyses, and observations. The application of volcanic forcing compiled for phase 6 of the Coupled Model Intercomparison Project (CMIP6) in the CCM SOCOLv3 reduces the warming overestimation in the tropical lower stratosphere and the volcanic aliasing of the temperature response to the SC, although it does not eliminate it completely.

  10. Deep convective clouds at the tropopause

    Directory of Open Access Journals (Sweden)

    H. H. Aumann

    2011-02-01

    Full Text Available Data from the Atmospheric Infrared Sounder (AIRS on the EOS Aqua spacecraft each day show tens of thousands of Cold Clouds (CC in the tropical oceans with 10 μm window channel brightness temperatures colder than 225 K. These clouds represent a mix of cold anvil clouds and Deep Convective Clouds (DCC. This mix can be separated by computing the difference between two channels, a window channel and a channel with strong CO2 absorption: for some cold clouds this difference is negative, i.e. the spectra for some cold clouds are inverted. We refer to cold clouds with spectra which are more than 2 K inverted as DCCi2. Associated with DCCi2 is a very high rain rate and a local upward displacement of the tropopause, a cold "bulge", which can be seen directly in the brightness temperatures of AIRS and Advanced Microwave Sounding Unit (AMSU temperature sounding channels in the lower stratosphere. The very high rain rate and the local distortion of the tropopause indicate that DCCi2 objects are associated with severe storms. Significant long-term trends in the statistical properties of DCCi2 could be interesting indicators of climate change. While the analysis of the nature and physical conditions related to DCCi2 requires hyperspectral infrared and microwave data, the identification of DCCi2 requires only one good window channel and one strong CO2 sounding channel. This suggests that improved identification of severe storms with future advanced geostationary satellites could be accomplished with the addition of one or two narrow band channels.

  11. Long-term evolution of upper stratospheric ozone at selected stations of the Network for the Detection of Stratospheric Change (NDSC)

    NARCIS (Netherlands)

    Steinbrecht, W; Claude, H; Schönenborn, F; McDermid, I S; Leblanc, T; Godin, S; Song, T; Swart, D P J; Meijer, Y J; Bodeker, G E; Connor, B J; Kämpfer, N; Hocke, K; Calisesi, Y; Schneider, N; Noë, J de la; Parrish, A D; Boyd, I S; Brühl, C; Steil, B; Giorgetta, M A; Manzini, E; Thomason, L W; Zawodny, J M; McCormick, M P; Russell, J M; Bhartia, P K; Stolarski, R S; Hollandsworth-Frith, S M

    2006-01-01

    The long-term evolution of upper stratospheric ozone has been recorded by lidars and microwave radiometers within the ground-based Network for the Detection of Stratospheric Change (NDSC), and by the space-borne Solar Backscatter Ultra-Violet instruments (SBUV), Stratospheric Aerosol and Gas

  12. Quantifying and Modelling the Effect of Cloud Shadows on the Surface Irradiance at Tropical and Midlatitude Forests

    Science.gov (United States)

    Kivalov, Sergey N.; Fitzjarrald, David R.

    2018-02-01

    Cloud shadows lead to alternating light and dark periods at the surface, with the most abrupt changes occurring in the presence of low-level forced cumulus clouds. We examine multiyear irradiance time series observed at a research tower in a midlatitude mixed deciduous forest (Harvard Forest, Massachusetts, USA: 42.53{°}N, 72.17{°}W) and one made at a similar tower in a tropical rain forest (Tapajós National Forest, Pará, Brazil: 2.86{°}S, 54.96{°}W). We link the durations of these periods statistically to conventional meteorological reports of sky type and cloud height at the two forests and present a method to synthesize the surface irradiance time series from sky-type information. Four classes of events describing distinct sequential irradiance changes at the transition from cloud shadow and direct sunlight are identified: sharp-to-sharp, slow-to-slow, sharp-to-slow, and slow-to-sharp. Lognormal and the Weibull statistical distributions distinguish among cloudy-sky types. Observers' qualitative reports of `scattered' and `broken' clouds are quantitatively distinguished by a threshold value of the ratio of mean clear to cloudy period durations. Generated synthetic time series based on these statistics adequately simulate the temporal "radiative forcing" linked to sky type. Our results offer a quantitative way to connect the conventional meteorological sky type to the time series of irradiance experienced at the surface.

  13. The global atmospheric electric circuit and its effects on cloud microphysics

    International Nuclear Information System (INIS)

    Tinsley, B A

    2008-01-01

    This review is an overview of progress in understanding the theory and observation of the global atmospheric electric circuit, with the focus on its dc aspects, and its short and long term variability. The effects of the downward ionosphere-earth current density, J z , on cloud microphysics, with its variability as an explanation for small observed changes in weather and climate, will also be reviewed. The global circuit shows responses to external as well as internal forcing. External forcing arises from changes in the distribution of conductivity due to changes in the cosmic ray flux and other energetic space particle fluxes, and at high magnetic latitudes from solar wind electric fields. Internal forcing arises from changes in the generators and changes in volcanic and anthropogenic aerosols in the troposphere and stratosphere. All these result in spatial and temporal variation in J z . Variations in J z affect the production of space charge in layer clouds, with the charges being transferred to droplets and aerosol particles. New observations and new analyses are consistent with non-negligible effects of the charges on the microphysics of such clouds. Observed effects are small, but of high statistical significance for cloud cover and precipitation changes, with resulting atmospheric temperature, pressure and dynamics changes. These effects are detectable on the day-to-day timescale for repeated J z changes of order 10%, and are thus second order electrical effects. The implicit first order effects have not, as yet, been incorporated into basic cloud and aerosol physics. Long term (multidecadal through millennial) global circuit changes, due to solar activity modulating the galactic cosmic ray flux, are an order of magnitude greater at high latitudes and in the stratosphere, as can be inferred from geological cosmogenic isotope records. Proxies for climate change in the same stratified depositories show strong correlations of climate with the inferred global

  14. The global atmospheric electric circuit and its effects on cloud microphysics

    Energy Technology Data Exchange (ETDEWEB)

    Tinsley, B A [Physics Department and Center for Space Sciences, WT15, University of Texas at Dallas, 800 W Campbell Road, Richardson, TX, 75080-3021 (United States)], E-mail: Tinsley@UTDallas.edu

    2008-06-15

    This review is an overview of progress in understanding the theory and observation of the global atmospheric electric circuit, with the focus on its dc aspects, and its short and long term variability. The effects of the downward ionosphere-earth current density, J{sub z}, on cloud microphysics, with its variability as an explanation for small observed changes in weather and climate, will also be reviewed. The global circuit shows responses to external as well as internal forcing. External forcing arises from changes in the distribution of conductivity due to changes in the cosmic ray flux and other energetic space particle fluxes, and at high magnetic latitudes from solar wind electric fields. Internal forcing arises from changes in the generators and changes in volcanic and anthropogenic aerosols in the troposphere and stratosphere. All these result in spatial and temporal variation in J{sub z}. Variations in J{sub z} affect the production of space charge in layer clouds, with the charges being transferred to droplets and aerosol particles. New observations and new analyses are consistent with non-negligible effects of the charges on the microphysics of such clouds. Observed effects are small, but of high statistical significance for cloud cover and precipitation changes, with resulting atmospheric temperature, pressure and dynamics changes. These effects are detectable on the day-to-day timescale for repeated J{sub z} changes of order 10%, and are thus second order electrical effects. The implicit first order effects have not, as yet, been incorporated into basic cloud and aerosol physics. Long term (multidecadal through millennial) global circuit changes, due to solar activity modulating the galactic cosmic ray flux, are an order of magnitude greater at high latitudes and in the stratosphere, as can be inferred from geological cosmogenic isotope records. Proxies for climate change in the same stratified depositories show strong correlations of climate with the

  15. A-train CALIOP and MLS observations of early winter Antarctic polar stratospheric clouds and nitric acid in 2008

    Directory of Open Access Journals (Sweden)

    A. Lambert

    2012-03-01

    Full Text Available A-train Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP and Microwave Limb Sounder (MLS observations are used to investigate the development of polar stratospheric clouds (PSCs and the gas-phase nitric acid distribution in the early 2008 Antarctic winter. Observational evidence of gravity-wave activity is provided by Atmospheric Infrared Sounder (AIRS radiances and infrared spectroscopic detection of nitric acid trihydrate (NAT in PSCs is obtained from the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS. Goddard Earth Observing System Data Assimilation System (GEOS-5 DAS analyses are used to derive Lagrangian trajectories and to determine temperature-time histories of air parcels. We use CALIOP backscatter and depolarization measurements to classify PSCs and the MLS measurements to determine the corresponding gas-phase HNO3 as a function of temperature. For liquid PSCs the uptake of HNO3 follows the theoretical equilibrium curve for supercooled ternary solutions (STS, but at temperatures about 1 K lower as determined from GEOS-5. In the presence of solid phase PSCs, above the ice frost-point, the HNO3 depletion occurs over a wider range of temperatures (+2 to −7 K distributed about the NAT equilibrium curve. Rapid gas-phase HNO3 depletion is first seen by MLS from from 23–25 May 2008, consisting of a decrease in the volume mixing ratio from 14 ppbv (parts per billion by volume to 7 ppbv on the 46–32 hPa (hectopascal pressure levels and accompanied by a 2–3 ppbv increase by renitrification at the 68 hPa pressure level. The observed region of depleted HNO3 is substantially smaller than the region bounded by the NAT existence temperature threshold. Temperature-time histories of air parcels demonstrate that the depletion is more clearly correlated with prior exposure to temperatures a few kelvin above the frost-point. From the combined data we infer the presence

  16. Retrieval of macrophysical cloud parameters from MIPAS: algorithm description

    Directory of Open Access Journals (Sweden)

    J. Hurley

    2011-04-01

    Full Text Available The Michelson Interferometer for Passive Atmospheric Sounding (MIPAS onboard ENVISAT has the potential to be particularly useful for studying high, thin clouds, which have been difficult to observe in the past. This paper details the development, implementation and testing of an optimal-estimation-type retrieval for three macrophysical cloud parameters (cloud top height, cloud top temperature and cloud extinction coefficient from infrared spectra measured by MIPAS. A preliminary estimation of a parameterisation of the optical and geometrical filling of the measurement field-of-view by cloud is employed as the first step of the retrieval process to improve the choice of a priori for the macrophysical parameters themselves.

    Preliminary application to single-scattering simulations indicates that the retrieval error stemming from uncertainties introduced by noise and by a priori variances in the retrieval process itself is small – although it should be noted that these retrieval errors do not include the significant errors stemming from the assumption of homogeneity and the non-scattering nature of the forward model. Such errors are preliminarily and qualitatively assessed here, and are likely to be the dominant error sources. The retrieval converges for 99% of input cases, although sometimes fails to converge for vetically-thin (<1 km clouds. The retrieval algorithm is applied to MIPAS data; the results of which are qualitatively compared with CALIPSO cloud top heights and PARASOL cloud opacities. From comparison with CALIPSO cloud products, it must be noted that the cloud detection method used in this algorithm appears to potentially misdetect stratospheric aerosol layers as cloud.

    This algorithm has been adopted by the European Space Agency's "MIPclouds" project.

  17. Thin Cloud Detection Method by Linear Combination Model of Cloud Image

    Science.gov (United States)

    Liu, L.; Li, J.; Wang, Y.; Xiao, Y.; Zhang, W.; Zhang, S.

    2018-04-01

    The existing cloud detection methods in photogrammetry often extract the image features from remote sensing images directly, and then use them to classify images into cloud or other things. But when the cloud is thin and small, these methods will be inaccurate. In this paper, a linear combination model of cloud images is proposed, by using this model, the underlying surface information of remote sensing images can be removed. So the cloud detection result can become more accurate. Firstly, the automatic cloud detection program in this paper uses the linear combination model to split the cloud information and surface information in the transparent cloud images, then uses different image features to recognize the cloud parts. In consideration of the computational efficiency, AdaBoost Classifier was introduced to combine the different features to establish a cloud classifier. AdaBoost Classifier can select the most effective features from many normal features, so the calculation time is largely reduced. Finally, we selected a cloud detection method based on tree structure and a multiple feature detection method using SVM classifier to compare with the proposed method, the experimental data shows that the proposed cloud detection program in this paper has high accuracy and fast calculation speed.

  18. Modeling of Solar Radiation Management: A Comparison of Simulations Using Reduced Solar Constant and Stratospheric Sulphate Aerosols

    Science.gov (United States)

    Bala, G.; Kalidindi, S.; Modak, A.; Caldeira, K.

    2014-12-01

    Several climate modelling studies in the past have used reduction in solar constant to simulate the climatic effects of Solar Radiation Management (SRM) geoengineering. This is most likely valid only for space-based mirrors/reflectors but not for SRM methods that rely on stratospheric aerosols. In this study, we use a climate model to evaluate the differences in climate response to SRM by uniform solar constant reduction and stratospheric aerosols. The experiments are designed such that global mean warming from a doubling of atmospheric CO2 concentration (2xCO2) is nearly cancelled in each case. In such a scenario, the residual climate effects are similar when important surface and tropospheric climate variables such as temperature and precipitation are considered. However, there are significant differences in stratospheric temperature response and diffuse and direct radiation reaching the surface. A difference of 1K in the global mean stratospheric (61-9.8 hPa) temperature is simulated between the two SRM methods, with warming in the aerosol scheme and a slight cooling for sunshades. While the global mean surface diffuse radiation increases by ~23% and direct radiation decreases by about 9% in the case of aerosol SRM method, both direct and diffuse radiation decrease by similar fractional amounts (~1.0%) when solar constant is reduced. When CO2 fertilization effects from elevated CO2 concentration levels are removed, the contribution from shaded leaves to gross primary productivity (GPP) increases by 1.8 % in aerosol SRM because of increased diffuse light. However, this increase is almost offset by a 15.2% decline in sunlit contribution due to reduced direct light. Overall both the SRM simulations show similar decrease in GPP (~ 8%) and NPP (~3%) relative to 2xCO2, indicating the negligible effect of the fractional changes in direct/diffuse radiation on the overall plant productivity. Based on our modelling study, we conclude that the climate states produced by a

  19. Chlorine in the stratosphere

    OpenAIRE

    VON CLARMANN, T.

    2013-01-01

    This paper reviews the various aspects of chlorine compounds in the stratosphere, both their roles as reactants and as tracers of dynamical processes. In the stratosphere, reactive chlorine is released from chlorofluorocarbons and other chlorine-containing organic source gases. To a large extent reactive chlorine is then sequestered in reservoir species ClONO2 and HCl. Re-activation of chlorine happens predominantly in polar winter vortices by heterogeneous reaction in combination with sunlig...

  20. On the role of atmosphere-ocean interactions in the expected long-term changes of the Earth's ozone layer caused by greenhouse gases

    Science.gov (United States)

    Zadorozhny, Alexander; Dyominov, Igor

    It is well known that anthropogenic emissions of greenhouse gases into the atmosphere produce a global warming of the troposphere and a global cooling of the stratosphere. The expected stratospheric cooling essentially influences the ozone layer via increased polar stratospheric cloud formation and via temperature dependences of the gas phase reaction rates. One more mechanism of how greenhouse gases influences the ozone layer is enhanced water evaporation from the oceans into the atmosphere because of increasing temperatures of the ocean surface due to greenhouse effect. The subject of this paper is a study of the influence of anthropogenic pollution of the atmosphere by the greenhouse gases CO2, CH4, N2O and ozone-depleting chlorine and bromine compounds on the expected long-term changes of the ozone layer with taking into account an increase of water vapour content in the atmosphere due to greenhouse effect. The study based on 2-D zonally averaged interactive dynamical radiative-photochemical model of the troposphere and stratosphere. The model allows to self-consistently calculating diabatic circulation, temperature, gaseous composition of the troposphere and stratosphere at latitudes from the South to North Poles, as well as distribution of sulphate aerosol particles and polar stratospheric clouds of two types. It was supposed in the model that an increase of the ocean surface temperature caused by greenhouse effect is similar to calculated increase of atmospheric surface temperature. Evaporation rate from the ocean surface was computed in dependence of latitude. The model time-dependent runs were made for the period from 1975 to 2100 using two IPCC scenarios depicting maximum and average expected increases of greenhouse gases in the atmosphere. The model calculations show that anthropogenic increasing of water vapour abundance in the atmosphere due to heating of the ocean surface caused by greenhouse effect gives a sensible contribution to the expected ozone

  1. A warming tropical central Pacific dries the lower stratosphere

    Science.gov (United States)

    Ding, Qinghua; Fu, Qiang

    2018-04-01

    The amount of water vapor in the tropical lower stratosphere (TLS), which has an important influence on the radiative energy budget of the climate system, is modulated by the temperature variability of the tropical tropopause layer (TTL). The TTL temperature variability is caused by a complex combination of the stratospheric quasi-biennial oscillation (QBO), tropospheric convective processes in the tropics, and the Brewer-Dobson circulation (BDC) driven by mid-latitude and subtropical atmospheric waves. In 2000, the TLS water vapor amount exhibited a stepwise transition to a dry phase, apparently caused by a change in the BDC. In this study, we present observational and modeling evidence that the epochal change of water vapor between the periods of 1992-2000 and 2001-2005 was also partly caused by a concurrent sea surface temperature (SST) warming in the tropical central Pacific. This SST warming cools the TTL above by enhancing the equatorial wave-induced upward motion near the tropopause, which consequently reduces the amount of water vapor entering the stratosphere. The QBO affects the TLS water vapor primarily on inter-annual timescales, whereas a classical El Niño southern oscillation (ENSO) event has small effect on tropical mean TLS water vapor because its responses are longitudinally out of phase. This study suggests that the tropical central Pacific SST is another driver of TLS water vapor variability on inter-decadal timescales and the tropical SST changes could contribute to about 30% of the step-wise drop of the lower stratospheric water vapor from 1992-2000 to 2001-2005.

  2. Stratospheric role in interdecadal changes of El Niño impacts over Europe

    Science.gov (United States)

    Ayarzagüena, B.; López-Parages, J.; Iza, M.; Calvo, N.; Rodríguez-Fonseca, B.

    2018-04-01

    The European precipitation response to El Niño (EN) has been found to present interdecadal changes, with alternated periods of important or negligible EN impact in late winter. These periods are associated with opposite phases of multi-decadal sea surface temperature (SST) variability, which modifies the tropospheric background and EN teleconnections. In addition, other studies have shown how SST anomalies in the equatorial Pacific, and in particular, the location of the largest anomalous SST, modulate the stratospheric response to EN. Nevertheless, the role of the stratosphere on the stationarity of EN response has not been investigated in detail so far. Using reanalysis data, we present a comprehensive study of EN teleconnections to Europe including the role of the ocean background and the stratosphere in the stationarity of the signal. The results reveal multidecadal variability in the location of EN-related SST anomalies that determines different teleconnections. In periods with relevant precipitation signal over Europe, the EN SST pattern resembles Eastern Pacific EN and the stratospheric pathway plays a key role in transmitting the signal to Europe in February, together with two tropospheric wavetrains that transmit the signal in February and April. Conversely, the stratospheric pathway is not detected in periods with a weak EN impact on European precipitation, corresponding to EN-related SST anomalies primarily located over the central Pacific. SST mean state and its associated atmospheric background control the location of EN-related SST anomalies in different periods and modulate the establishment of the aforementioned stratospheric pathway of EN teleconnection to Europe too.

  3. The propagation of orographic gravity waves into the stratosphere. Linear theory, idealized and realistic numerical simulation; Die Ausbreitung orographisch angeregter Schwerewellen in die Stratosphaere. Lineare Theorie, idealisierte und realitaetsnahe numerische Simulation

    Energy Technology Data Exchange (ETDEWEB)

    Leutbecher, M. [DLR Deutsches Zentrum fuer Luft- und Raumfahrt e.V., Wessling (Germany). Inst. fuer Physik der Atmosphaere

    1998-07-01

    Flow over mountains in the stably stratified atmosphere excites gravity waves. The three-dimensional propagation of these waves into the stratosphere is studied using linear theority as well as idealized and realistic numerical simulations. Stagnation, momentum fluxes and temperature anomalies are analyzed for idealized types of flow. Isolated mountains with elliptical contours are considered. The unperturbed atmosphere has constant wind speed and constant static stability or two layers (troposphere/stratosphere) of constant stability each. Real flow over orography is investigated where gravity waves in the stratosphere have been observed. Characteristics of the gravity wave event over the southern tip of Greenland on 6 January 1992 were recorded on a flight of the ER-2 at an altitude of 20 km. In the second case polar stratospheric clouds (PSC) were observed by an airborne Lidar over Northern Scandinavia on 9 January 1997. The PSC were induced by temperature anomalies in orographic gravity waves. (orig.)

  4. Effects of Greenhouse Gas Increase and Stratospheric Ozone Depletion on Stratospheric Mean Age of Air in 1960-2010

    Science.gov (United States)

    Li, Feng; Newman, Paul; Pawson, Steven; Perlwitz, Judith

    2018-01-01

    The relative impacts of greenhouse gas (GHG) increase and stratospheric ozone depletion on stratospheric mean age of air in the 1960-2010 period are quantified using the Goddard Earth Observing System Chemistry-�Climate Model. The experiment compares controlled simulations using a coupled atmosphere-�ocean version of the Goddard Earth Observing System Chemistry-�Climate Model, in which either GHGs or ozone depleting substances, or both factors evolve over time. The model results show that GHGs and ozone-depleting substances have about equal contributions to the simulated mean age decrease, but GHG increases account for about two thirds of the enhanced strength of the lower stratospheric residual circulation. It is also found that both the acceleration of the diabatic circulation and the decrease of the mean age difference between downwelling and upwelling regions are mainly caused by GHG forcing. The results show that ozone depletion causes an increase in the mean age of air in the Antarctic summer lower stratosphere through two processes: (1) a seasonal delay in the Antarctic polar vortex breakup that inhibits young midlatitude air from mixing with the older air inside the vortex, and (2) enhanced Antarctic downwelling that brings older air from middle and upper stratosphere into the lower stratosphere.

  5. A review of optical measurements at the aerosol and cloud chamber AIDA

    International Nuclear Information System (INIS)

    Wagner, Robert; Linke, Claudia; Naumann, Karl-Heinz; Schnaiter, Martin; Vragel, Marlen; Gangl, Martin; Horvath, Helmuth

    2009-01-01

    This paper provides a survey of recent studies on the optical properties of aerosol and cloud particles that have been conducted at the AIDA facility of Forschungszentrum Karlsruhe (Aerosol Interactions and Dynamics in the Atmosphere). Reflecting the broad accessible temperature range of the AIDA chamber which extends from ambient temperature down to 183 K, the investigations feature a broad diversity of research topics, such as the wavelength-dependence of the specific absorption cross sections of soot and mineral dust aerosols at room temperature, depolarization and infrared extinction measurements of ice crystal clouds generated at temperatures below 235 K, and the optical properties of polar stratospheric cloud constituents whose formation was studied in chamber experiments at temperatures well below 200 K. After reviewing the AIDA research activity of the past decade and introducing the optical instrumentation of the AIDA facility, this paper presents illustrative examples of ongoing and already published work on optical measurements of soot aerosols, mineral dust particles, and ice crystal clouds.

  6. Summary of photochemical and radiative data used in the LLNL one-dimensional transport-kinetics model of the troposphere and stratosphere: 1982

    International Nuclear Information System (INIS)

    Connell, P.S.; Wuebbles, D.J.

    1983-01-01

    This report summarizes the contents and sources of the photochemical and radiative segment of the LLNL one-dimensional transport-kinetics model of the troposphere and stratosphere. Data include the solar flux incident at the top of the atmosphere, absorption spectra for O 2 , O 3 and NO 2 , and effective absorption coefficients for about 40 photolytic processes as functions of wavelength and, in a few cases, temperature and pressure. The current data set represents understanding of atmospheric photochemical processes as of late 1982 and relies largely on NASA Evaluation Number 5 of Chemical Kinetics and Photochemical Data for Use in Stratospheric Modeling, JPL Publication 82-57 (DeMore et al., 1982). Implementation in the model, including the treatment of multiple scattering and cloud cover, is discussed in Wuebbles (1981)

  7. Stratospheric HTO perturbations 1980-1983

    Science.gov (United States)

    Mason, A. S.

    1985-02-01

    Three perturbations of the stratospheric tritiated water burden have occurred. An atmospheric nuclear detonation in 1980 injected about 2.1 MCi. The massive eruptions of the volcano El Chichon may have contributed to a doubling of the removal rate in 1982. An unusually large wintertime exchange with the upper stratosphere may have occurred between 1982 and 1983.

  8. Stratospheric H2O

    International Nuclear Information System (INIS)

    Ellsaesser, H.W.

    1979-01-01

    Documentation of the extreme aridity (approx. 3% relative humidity) of the lower stratosphere and the rapid decrease of mixing ratio with height just above the polar tropopause (20-fold in the 1st km) was begun by Dobson et al., (1946) in 1943. They recognized that this extreme and persistent aridity must be dynamically maintained else it would have been wiped out by turbulent diffusion. This led Brewer (1949) to hypothesize a stratospheric circulation in which all air enters through the tropical tropopause where it is freeze dried to a mass mixing ratio of 2 to 3 ppM. This dry air then spreads poleward and descends through the polar tropopauses overpowering upward transport of water vapor by diffusion which would otherwise be permitted by the much warmer temperatures of the polar tropopauses. Questions can indeed be raised as to the absolute magnitudes of stratospheric mixing ratios, the effective temperature of the tropical tropopause cold trap, the reality of winter pole freeze-dry sinks and the representativeness of the available observations suggesting an H 2 O mixing ratio maximum just above the tropical tropopause and a constant mixing ratio from the tropopause to 30 to 35 km. However, no model that better fits all of the available data is available, than does the Brewer (1949) hypothesis coupled with a lower stratosphere winter pole, freeze-dry sink, at least over Antarctica

  9. Low level of stratospheric ozone near the Jharia coal field in India

    Indian Academy of Sciences (India)

    on the possible impact of coal fires on the stratospheric ozone concentration has been reported so far. ... dry soil and a local rise in the surface tempera- ture. Smoke plumes ..... of the impact on the air environment due to opencast coal mining–.

  10. Quantitative evaluation for small surface damage based on iterative difference and triangulation of 3D point cloud

    Science.gov (United States)

    Zhang, Yuyan; Guo, Quanli; Wang, Zhenchun; Yang, Degong

    2018-03-01

    This paper proposes a non-contact, non-destructive evaluation method for the surface damage of high-speed sliding electrical contact rails. The proposed method establishes a model of damage identification and calculation. A laser scanning system is built to obtain the 3D point cloud data of the rail surface. In order to extract the damage region of the rail surface, the 3D point cloud data are processed using iterative difference, nearest neighbours search and a data registration algorithm. The curvature of the point cloud data in the damage region is mapped to RGB color information, which can directly reflect the change trend of the curvature of the point cloud data in the damage region. The extracted damage region is divided into three prism elements by a method of triangulation. The volume and mass of a single element are calculated by the method of geometric segmentation. Finally, the total volume and mass of the damage region are obtained by the principle of superposition. The proposed method is applied to several typical injuries and the results are discussed. The experimental results show that the algorithm can identify damage shapes and calculate damage mass with milligram precision, which are useful for evaluating the damage in a further research stage.

  11. Arctic cloud-climate feedbacks: On relationships between Arctic clouds, sea ice, and lower tropospheric stability

    Science.gov (United States)

    Taylor, P. C.; Boeke, R.; Hegyi, B.

    2017-12-01

    Arctic low clouds strongly affect the Arctic surface energy budget. Through this impact Arctic low clouds influence other important aspects of the Arctic climate system, namely surface and atmospheric temperature, sea ice extent and thickness, and atmospheric circulation. Arctic clouds are in turn influenced by these Arctic climate system elements creating the potential for Arctic cloud-climate feedbacks. To further our understanding of the potential for Arctic cloud-climate feedbacks, we quantify the influence of atmospheric state on the surface cloud radiative effect (CRE). In addition, we quantify the covariability between surface CRE and sea ice concentration (SIC). This paper builds on previous research using instantaneous, active remote sensing satellite footprint data from the NASA A-Train. First, the results indicate significant differences in the surface CRE when stratified by atmospheric state. Second, a statistically insignificant covariability is found between CRE and SIC for most atmospheric conditions. Third, we find a statistically significant increase in the average surface longwave CRE at lower SIC values in fall. Specifically, a +3-5 W m-2 larger longwave CRE is found over footprints with 0% versus 100% SIC. Because systematic changes on the order of 1 W m-2 are sufficient to explain the observed long-term reductions in sea ice extent, our results indicate a potentially significant amplifying sea ice-cloud feedback that could delay the fall freeze-up and influence the variability in sea ice extent and volume, under certain meteorological conditions. Our results also suggest that a small change in the frequency of occurrence of atmosphere states may yield a larger Arctic cloud feedback than any cloud response to sea ice.

  12. Climate impact of idealized winter polar mesospheric and stratospheric ozone losses as caused by energetic particle precipitation

    Science.gov (United States)

    Meraner, Katharina; Schmidt, Hauke

    2018-01-01

    Energetic particles enter the polar atmosphere and enhance the production of nitrogen oxides and hydrogen oxides in the winter stratosphere and mesosphere. Both components are powerful ozone destroyers. Recently, it has been inferred from observations that the direct effect of energetic particle precipitation (EPP) causes significant long-term mesospheric ozone variability. Satellites observe a decrease in mesospheric ozone up to 34 % between EPP maximum and EPP minimum. Stratospheric ozone decreases due to the indirect effect of EPP by about 10-15 % observed by satellite instruments. Here, we analyze the climate impact of winter boreal idealized polar mesospheric and polar stratospheric ozone losses as caused by EPP in the coupled Max Planck Institute Earth System Model (MPI-ESM). Using radiative transfer modeling, we find that the radiative forcing of mesospheric ozone loss during polar night is small. Hence, climate effects of mesospheric ozone loss due to energetic particles seem unlikely. Stratospheric ozone loss due to energetic particles warms the winter polar stratosphere and subsequently weakens the polar vortex. However, those changes are small, and few statistically significant changes in surface climate are found.

  13. Millimeter wave spectroscopic measurements of stratospheric and mesospheric constituents over the Italian Alps: stratospheric ozone

    Directory of Open Access Journals (Sweden)

    V. Romaniello

    2007-06-01

    Full Text Available Measurements of rotational lines emitted by middle atmospheric trace gases have been carried out from the Alpine station of Testa Grigia (45.9°N, 7.7°E, elev. 3500 m by means of a Ground-Based Millimeter-wave Spectrometer (GBMS. Observations of species such as O3, HNO3, CO, N2O, HCN, and HDO took place during 4 winter periods, from February 2004 to March 2007, for a total of 116 days of measurements grouped in about 18 field campaigns. By studying the pressure-broadened shape of emission lines the vertical distribution of the observed constituents is retrieved within an altitude range of ?17-75 km, constrained by the 600 MHz pass band and the 65 kHz spectral resolution of the back-end spectrometer. This work discusses the behavior of stratospheric O3 during the entire period of operation at Testa Grigia. Mid-latitude O3 columnar content as estimated using GBMS measurements can vary by large amounts over a period of very few days, with the largest variations observed in December 2005, February 2006, and March 2006, confirming that the northern winter of 2005-2006 was characterized by a particularly intense planetary wave activity. The largest rapid variation from maximum to minimum O3 column values over Testa Grigia took place in December 2006 and reached a relative value of 72% with respect to the average column content for that period. During most GBMS observation times much of the variability is concentrated in the column below 20 km, with tropospheric weather systems and advection of tropical tropospheric air into the lower stratosphere over Testa Grigia having a large impact on the observed variations in column contents. Nonetheless, a wide variability is also found in middle stratospheric GBMS O3 measurements, as expected for mid-latitude ozone. We find that O3 mixing ratios at ?32 km are very well correlated with the solar illumination experienced by air masses over the previous ?15 days, showing that already at 32 km

  14. Simulation of stratospheric water vapor trends: impact on stratospheric ozone chemistry

    Directory of Open Access Journals (Sweden)

    A. Stenke

    2005-01-01

    Full Text Available A transient model simulation of the 40-year time period 1960 to 1999 with the coupled climate-chemistry model (CCM ECHAM4.L39(DLR/CHEM shows a stratospheric water vapor increase over the last two decades of 0.7 ppmv and, additionally, a short-term increase after major volcanic eruptions. Furthermore, a long-term decrease in global total ozone as well as a short-term ozone decline in the tropics after volcanic eruptions are modeled. In order to understand the resulting effects of the water vapor changes on lower stratospheric ozone chemistry, different perturbation simulations were performed with the CCM ECHAM4.L39(DLR/CHEM feeding the water vapor perturbations only to the chemistry part. Two different long-term perturbations of lower stratospheric water vapor, +1 ppmv and +5 ppmv, and a short-term perturbation of +2 ppmv with an e-folding time of two months were applied. An additional stratospheric water vapor amount of 1 ppmv results in a 5–10% OH increase in the tropical lower stratosphere between 100 and 30 hPa. As a direct consequence of the OH increase the ozone destruction by the HOx cycle becomes 6.4% more effective. Coupling processes between the HOx-family and the NOx/ClOx-family also affect the ozone destruction by other catalytic reaction cycles. The NOx cycle becomes 1.6% less effective, whereas the effectiveness of the ClOx cycle is again slightly enhanced. A long-term water vapor increase does not only affect gas-phase chemistry, but also heterogeneous ozone chemistry in polar regions. The model results indicate an enhanced heterogeneous ozone depletion during antarctic spring due to a longer PSC existence period. In contrast, PSC formation in the northern hemisphere polar vortex and therefore heterogeneous ozone depletion during arctic spring are not affected by the water vapor increase, because of the less PSC activity. Finally, this study shows that 10% of the global total ozone decline in the transient model run

  15. The Role of Gravity Waves in the Formation and Organization of Clouds during TWPICE

    Energy Technology Data Exchange (ETDEWEB)

    Reeder, Michael J. [Monash University; Lane, Todd P. [University of Melbourne; Hankinson, Mai Chi Nguyen [Monash University

    2013-09-27

    All convective clouds emit gravity waves. While it is certain that convectively-generated waves play important parts in determining the climate, their precise roles remain uncertain and their effects are not (generally) represented in climate models. The work described here focuses mostly on observations and modeling of convectively-generated gravity waves, using the intensive observations from the DoE-sponsored Tropical Warm Pool International Cloud Experiment (TWP-ICE), which took place in Darwin, from 17 January to 13 February 2006. Among other things, the research has implications the part played by convectively-generated gravity waves in the formation of cirrus, in the initiation and organization of further convection, and in the subgrid-scale momentum transport and associated large-scale stresses imposed on the troposphere and stratosphere. The analysis shows two groups of inertia-gravity waves are detected: group L in the middle stratosphere during the suppressed monsoon period, and group S in the lower stratosphere during the monsoon break period. Waves belonging to group L propagate to the south-east with a mean intrinsic period of 35 h, and have vertical and horizontal wavelengths of about 5-6 km and 3000-6000 km, respectively. Ray tracing calculations indicate that these waves originate from a deep convective region near Indonesia. Waves belonging to group S propagate to the south-south-east with an intrinsic period, vertical wavelength and horizontal wavelength of about 45 h, 2 km and 2000-4000 km, respectively. These waves are shown to be associated with shallow convection in the oceanic area within about 1000 km of Darwin. The intrinsic periods of high-frequency waves are estimated to be between 20-40 minutes. The high-frequency wave activity in the stratosphere, defined by mass-weighted variance of the vertical motion of the sonde, has a maximum following the afternoon local convection indicating that these waves are generated by local convection

  16. Laboratory Investigations of Stratospheric Halogen Chemistry

    Science.gov (United States)

    Wine, Paul H.; Nicovich, J. Michael; Stickel, Robert E.; Hynes, Anthony J.

    1997-01-01

    A final report for the NASA-supported project on laboratory investigations of stratospheric halogen chemistry is presented. In recent years, this project has focused on three areas of research: (1) kinetic, mechanistic, and thermochemical studies of reactions which produce weakly bound chemical species of atmospheric interest; (2) development of flash photolysis schemes for studying radical-radical reactions of stratospheric interest; and (3) photochemistry studies of interest for understanding stratospheric chemistry. The first section of this paper contains a discussion of work which has not yet been published. All subsequent chapters contain reprints of published papers that acknowledge support from this grant.

  17. Corona-producing ice clouds: A case study of a cold mid-latitude cirrus layer

    International Nuclear Information System (INIS)

    Sassen, K.; Mace, G.G.; Hallett, J.; Poellot, M.R.

    1998-01-01

    A high (14.0-km), cold (-71.0thinsp degree C) cirrus cloud was studied by ground-based polarization lidar and millimeter radar and aircraft probes on the night of 19 April 1994 from the Cloud and Radiation Testbed site in northern Oklahoma. A rare cirrus cloud lunar corona was generated by this 1 - 2-km-deep cloud, thus providing an opportunity to measure the composition in situ, which had previously been assumed only on the basis of lidar depolarization data and simple diffraction theory for spheres. In this case, corona ring analysis indicated an effective particle diameter of ∼22 μm. A variety of in situ data corroborates the approximate ice-particle size derived from the passive retrieval method, especially near the cloud top, where impacted cloud samples show simple solid crystals. The homogeneous freezing of sulfuric acid droplets of stratospheric origin is assumed to be the dominant ice-particle nucleation mode acting in corona-producing cirrus clouds. It is speculated that this process results in a previously unrecognized mode of acid-contaminated ice-particle growth and that such small-particle cold cirrus clouds are potentially a radiatively distinct type of cloud. copyright 1998 Optical Society of America

  18. Satellite-observed cold-ring-shaped features atop deep convective clouds

    Czech Academy of Sciences Publication Activity Database

    Setvák, M.; Lindsey, D. T.; Novák, P.; Wang, P. K.; Radová, Michaela; Kerkmann, J.; Grasso, L.; Su, S.-H.; Rabin, R. M.; Šťástka, J.; Charvát, Z.

    2010-01-01

    Roč. 97, 1-2 (2010), s. 80-96 ISSN 0169-8095 R&D Projects: GA ČR GA205/07/0905; GA MŠk ME09033 Institutional research plan: CEZ:AV0Z30420517 Keywords : convective storm * storm top * cloud top height * cold-ring shape * cold-U shape * enhanced-V feature * overshooting top * lower stratosphere * Meteosat second generation Subject RIV: DG - Athmosphere Sciences, Meteorology Impact factor: 1.597, year: 2010 http://www.sciencedirect.com/science/article/pii/S016980951000058X

  19. Prolonged effect of the stratospheric pathway in linking Barents-Kara Sea sea ice variability to the midlatitude circulation in a simplified model

    Science.gov (United States)

    Zhang, Pengfei; Wu, Yutian; Smith, Karen L.

    2018-01-01

    To better understand the dynamical mechanism that accounts for the observed lead-lag correlation between the early winter Barents-Kara Sea (BKS) sea ice variability and the later winter midlatitude circulation response, a series of experiments are conducted using a simplified atmospheric general circulation model with a prescribed idealized near-surface heating over the BKS. A prolonged effect is found in the idealized experiments following the near-surface heating and can be explicitly attributed to the stratospheric pathway and the long time scale in the stratosphere. The analysis of the Eliassen-Palm flux shows that, as a result of the imposed heating and linear constructive interference, anomalous upward propagating planetary-scale waves are excited and weaken the stratospheric polar vortex. This stratospheric response persists for approximately 1-2 months accompanied by downward migration to the troposphere and the surface. This downward migration largely amplifies and extends the low-level jet deceleration in the midlatitudes and cold air advection over central Asia. The idealized model experiments also suggest that the BKS region is the most effective in affecting the midlatitude circulation than other regions over the Arctic.

  20. The effect of clouds on photolysis rates and ozone formation in the unpolluted troposphere

    Science.gov (United States)

    Thompson, A. M.

    1984-01-01

    The photochemistry of the lower atmosphere is sensitive to short- and long-term meteorological effects; accurate modeling therefore requires photolysis rates for trace gases which reflect this variability. As an example, the influence of clouds on the production of tropospheric ozone has been investigated, using a modification of Luther's two-stream radiation scheme to calculate cloud-perturbed photolysis rates in a one-dimensional photochemical transport model. In the unpolluted troposphere, where stratospheric inputs of odd nitrogen appear to represent the photochemical source of O3, strong cloud reflectance increases the concentration of NO in the upper troposphere, leading to greatly enhanced rates of ozone formation. Although the rate of these processes is too slow to verify by observation, the calculation is useful in distinguishing some features of the chemistry of regions of differing mean cloudiness.

  1. Towards constraining the stratosphere-troposphere exchange of radiocarbon: strategies of stratospheric 14CO2 measurements using AirCore

    Science.gov (United States)

    Chen, Huilin; Paul, Dipayan; Meijer, Harro; Miller, John; Kivi, Rigel; Krol, Maarten

    2016-04-01

    Radiocarbon (14C) plays an important role in the carbon cycle studies to understand both natural and anthropogenic carbon fluxes, but also in atmospheric chemistry to constrain hydroxyl radical (OH) concentrations in the atmosphere. Apart from the enormous 14C emissions from nuclear bomb testing in the 1950s and 1960s, radiocarbon is primarily produced in the stratosphere due to the cosmogenic production. To this end, better understanding the stratospheric radiocarbon source is very useful to advance the use of radiocarbon for these applications. However, stratospheric 14C observations have been very limited so that there are large uncertainties on the magnitude and the location of the 14C production as well as the transport of radiocarbon from the stratosphere to the troposphere. Recently we have successfully made stratospheric 14C measurements using AirCore samples from Sodankylä, Northern Finland. AirCore is an innovative atmospheric sampling system, which passively collects atmospheric air samples into a long piece of coiled stainless steel tubing during the descent of a balloon flight. Due to the relatively low cost of the consumables, there is a potential to make such AirCore profiling in other parts of the world on a regular basis. In this study, we simulate the 14C in the atmosphere and assess the stratosphere-troposphere exchange of radiocarbon using the TM5 model. The Sodankylä radiocarbon measurements will be used to verify the performance of the model at high latitude. Besides this, we will also evaluate the influence of different cosmogenic 14C production scenarios and the uncertainties in the OH field on the seasonal cycles of radiocarbon and on the stratosphere-troposphere exchange, and based on the results design a strategy to set up a 14C measurement program using AirCore.

  2. Possible effect of extreme solar energetic particle event of 20 January 2005 on polar stratospheric aerosols: direct observational evidence

    Directory of Open Access Journals (Sweden)

    I. A. Mironova

    2012-01-01

    Full Text Available Energetic cosmic rays are the main source of ionization of the low-middle atmosphere, leading to associated changes in atmospheric properties. Via the hypothetical influence of ionization on aerosol growth and facilitated formation of clouds, this may be an important indirect link relating solar variability to climate. This effect is highly debated, however, since the proposed theoretical mechanisms still remain illusive and qualitative, and observational evidence is inconclusive and controversial. Therefore, important questions regarding the existence and magnitude of the effect, and particularly the fraction of aerosol particles that can form and grow, are still open. Here we present empirical evidence of the possible effect caused by cosmic rays upon polar stratospheric aerosols, based on a case study of an extreme solar energetic particle (SEP event of 20 January 2005. Using aerosol data obtained over polar regions from different satellites with optical instruments that were operating during January 2005, such as the Stratospheric Aerosol and Gas Experiment III (SAGE III, and Optical Spectrograph and Infrared Imaging System (OSIRIS, we found a significant simultaneous change in aerosol properties in both the Southern and Northern Polar regions in temporal association with the SEP event. We speculate that ionization of the atmosphere, which was abnormally high in the lower stratosphere during the extreme SEP event, might have led to formation of new particles and/or growth of preexisting ultrafine particles in the polar stratospheric region. However, a detailed interpretation of the effect is left for subsequent studies. This is the first time high vertical resolution measurements have been used to discuss possible production of stratospheric aerosols under the influence of cosmic ray induced ionization. The observed effect is marginally detectable for the analyzed severe SEP event and can be undetectable for the majority of weak

  3. Possible effect of extreme solar energetic particle event of 20 January 2005 on polar stratospheric aerosols: direct observational evidence

    Science.gov (United States)

    Mironova, I. A.; Usoskin, I. G.; Kovaltsov, G. A.; Petelina, S. V.

    2012-01-01

    Energetic cosmic rays are the main source of ionization of the low-middle atmosphere, leading to associated changes in atmospheric properties. Via the hypothetical influence of ionization on aerosol growth and facilitated formation of clouds, this may be an important indirect link relating solar variability to climate. This effect is highly debated, however, since the proposed theoretical mechanisms still remain illusive and qualitative, and observational evidence is inconclusive and controversial. Therefore, important questions regarding the existence and magnitude of the effect, and particularly the fraction of aerosol particles that can form and grow, are still open. Here we present empirical evidence of the possible effect caused by cosmic rays upon polar stratospheric aerosols, based on a case study of an extreme solar energetic particle (SEP) event of 20 January 2005. Using aerosol data obtained over polar regions from different satellites with optical instruments that were operating during January 2005, such as the Stratospheric Aerosol and Gas Experiment III (SAGE III), and Optical Spectrograph and Infrared Imaging System (OSIRIS), we found a significant simultaneous change in aerosol properties in both the Southern and Northern Polar regions in temporal association with the SEP event. We speculate that ionization of the atmosphere, which was abnormally high in the lower stratosphere during the extreme SEP event, might have led to formation of new particles and/or growth of preexisting ultrafine particles in the polar stratospheric region. However, a detailed interpretation of the effect is left for subsequent studies. This is the first time high vertical resolution measurements have been used to discuss possible production of stratospheric aerosols under the influence of cosmic ray induced ionization. The observed effect is marginally detectable for the analyzed severe SEP event and can be undetectable for the majority of weak-moderate events. The present

  4. Transport of Ice into the Stratosphere and the Humidification of the Stratosphere over the 21st Century

    Science.gov (United States)

    Dessler, A. E.; Ye, H.; Wang, T.; Schoeberl, M. R.; Oman, L. D.; Douglass, A. R.; Butler, A. H.; Rosenlof, K. H.; Davis, S. M.; Portmann, R. W.

    2016-01-01

    Climate models predict that tropical lower-stratospheric humidity will increase as the climate warms. We examine this trend in two state-of-the-art chemistry-climate models. Under high greenhouse gas emissions scenarios, the stratospheric entry value of water vapor increases by approx. 1 part per million by volume (ppmv) over this century in both models. We show with trajectory runs driven by model meteorological fields that the warming tropical tropopause layer (TTL) explains 50-80% of this increase. The remainder is a consequence of trends in evaporation of ice convectively lofted into the TTL and lower stratosphere. Our results further show that, within the models we examined, ice lofting is primarily important on long time scales - on interannual time scales, TTL temperature variations explain most of the variations in lower stratospheric humidity. Assessing the ability of models to realistically represent ice-lofting processes should be a high priority in the modeling community.

  5. Study on the cloud detection of GOCI by using the simulated surface reflectance from BRDF-model for the land application and meteorological utilization

    Science.gov (United States)

    Kim, Hye-Won; Yeom, Jong-Min; Woo, Sun-Hee; Chae, Tae-Byeong

    2016-04-01

    COMS (Communication, Ocean, and Meteorological Satellite) was launched at French Guiana Kourou space center on 27 June 2010. Geostationary Ocean Color Imager (GOCI), which is the first ocean color geostationary satellite in the world for observing the ocean phenomena, is able to obtain the scientific data per an hour from 00UTC to 07UTC. Moreover, the spectral channels of GOCI would enable not only monitoring for the ocean, but for extracting the information of the land surface over the Korean Peninsula, Japan, and Eastern China. Since it is extremely important to utilize GOCI data accurately for the land application, cloud pixels over the surface have to be removed. Unfortunately, infra-red (IR) channels that can easily detect the water vapor with the cloud top temperature, are not included in the GOCI sensor. In this paper, the advanced cloud masking algorithm will be proposed with visible and near-IR (NIR) bands that are within GOCI bands. The main obstacle of cloud masking with GOCI is how to handle the high variable surface reflectance, which is mainly depending on the solar zenith angle. In this study, we use semi-empirical BRDF model to simulate the surface reflectance by using 16 day composite cloudy free image. When estimating the simulated surface reflectance, same geometry for GOCI observation was applied. The simulated surface reflectance is used to discriminate cloud areas especially for the thin cloud and shows more reasonable result than original threshold methods.

  6. The 2009–2010 Arctic stratospheric winter – general evolution, mountain waves and predictability of an operational weather forecast model

    Directory of Open Access Journals (Sweden)

    A. Dörnbrack

    2012-04-01

    Full Text Available The relatively warm 2009–2010 Arctic winter was an exceptional one as the North Atlantic Oscillation index attained persistent extreme negative values. Here, selected aspects of the Arctic stratosphere during this winter inspired by the analysis of the international field experiment RECONCILE are presented. First of all, and as a kind of reference, the evolution of the polar vortex in its different phases is documented. Special emphasis is put on explaining the formation of the exceptionally cold vortex in mid winter after a sequence of stratospheric disturbances which were caused by upward propagating planetary waves. A major sudden stratospheric warming (SSW occurring near the end of January 2010 concluded the anomalous cold vortex period. Wave ice polar stratospheric clouds were frequently observed by spaceborne remote-sensing instruments over the Arctic during the cold period in January 2010. Here, one such case observed over Greenland is analysed in more detail and an attempt is made to correlate flow information of an operational numerical weather prediction model to the magnitude of the mountain-wave induced temperature fluctuations. Finally, it is shown that the forecasts of the ECMWF ensemble prediction system for the onset of the major SSW were very skilful and the ensemble spread was very small. However, the ensemble spread increased dramatically after the major SSW, displaying the strong non-linearity and internal variability involved in the SSW event.

  7. First Simulations of Designing Stratospheric Sulfate Aerosol Geoengineering to Meet Multiple Simultaneous Climate Objectives: DESIGNING STRATOSPHERIC GEOENGINEERING

    Energy Technology Data Exchange (ETDEWEB)

    Kravitz, Ben [Atmospheric Sciences and Global Change Division, Pacific Northwest National Laboratory, Richland WA USA; MacMartin, Douglas G. [Mechanical and Aerospace Engineering, Cornell University, Ithaca NY USA; Department of Computing and Mathematical Sciences, California Institute of Technology, Pasadena CA USA; Mills, Michael J. [Atmospheric Chemistry, Observations, and Modeling Laboratory, National Center for Atmospheric Research, Boulder CO USA; Richter, Jadwiga H. [Climate and Global Dynamics Laboratory, National Center for Atmospheric Research, Boulder CO USA; Tilmes, Simone [Atmospheric Chemistry, Observations, and Modeling Laboratory, National Center for Atmospheric Research, Boulder CO USA; Climate and Global Dynamics Laboratory, National Center for Atmospheric Research, Boulder CO USA; Lamarque, Jean-Francois [Atmospheric Chemistry, Observations, and Modeling Laboratory, National Center for Atmospheric Research, Boulder CO USA; Tribbia, Joseph J. [Climate and Global Dynamics Laboratory, National Center for Atmospheric Research, Boulder CO USA; Vitt, Francis [Atmospheric Chemistry, Observations, and Modeling Laboratory, National Center for Atmospheric Research, Boulder CO USA

    2017-12-07

    We describe the first simulations of stratospheric sulfate aerosol geoengineering using multiple injection locations to meet multiple simultaneous surface temperature objectives. Simulations were performed using CESM1(WACCM), a coupled atmosphere-ocean general circulation model with fully interactive stratospheric chemistry, dynamics (including an internally generated quasi-biennial oscillation), and a sophisticated treatment of sulfate aerosol formation, microphysical growth, and deposition. The objectives are defined as maintaining three temperature features at their 2020 levels against a background of the RCP8.5 scenario over the period 2020-2099. These objectives are met using a feedback mechanism in which the rate of sulfur dioxide injection at each of the four locations is adjusted independently every year of simulation. Even in the presence of uncertainties, nonlinearities, and variability, the objectives are met, predominantly by SO2 injection at 30°N and 30°S. By the last year of simulation, the feedback algorithm calls for a total injection rate of 51 Tg SO2 per year. The injections are not in the tropics, which results in a greater degree of linearity of the surface climate response with injection amount than has been found in many previous studies using injection at the equator. Because the objectives are defined in terms of annual mean temperature, the required geeongineering results in "overcooling" during summer and "undercooling" during winter. The hydrological cycle is also suppressed as compared to the reference values corresponding to the year 2020. The demonstration we describe in this study is an important step toward understanding what geoengineering can do and what it cannot do.

  8. Comment on "Tropospheric temperature response to stratospheric ozone recovery in the 21st century" by Hu et al. (2011

    Directory of Open Access Journals (Sweden)

    C. McLandress

    2012-03-01

    Full Text Available In a recent paper Hu et al. (2011 suggest that the recovery of stratospheric ozone during the first half of this century will significantly enhance free tropospheric and surface warming caused by the anthropogenic increase of greenhouse gases, with the effects being most pronounced in Northern Hemisphere middle and high latitudes. These surprising results are based on a multi-model analysis of CMIP3 model simulations with and without prescribed stratospheric ozone recovery. Hu et al. suggest that in order to properly quantify the tropospheric and surface temperature response to stratospheric ozone recovery, it is necessary to run coupled atmosphere-ocean climate models with stratospheric ozone chemistry. The results of such an experiment are presented here, using a state-of-the-art chemistry-climate model coupled to a three-dimensional ocean model. In contrast to Hu et al., we find a much smaller Northern Hemisphere tropospheric temperature response to ozone recovery, which is of opposite sign. We suggest that their result is an artifact of the incomplete removal of the large effect of greenhouse gas warming between the two different sets of models.

  9. Development of methods for inferring cloud thickness and cloud-base height from satellite radiance data

    Science.gov (United States)

    Smith, William L., Jr.; Minnis, Patrick; Alvarez, Joseph M.; Uttal, Taneil; Intrieri, Janet M.; Ackerman, Thomas P.; Clothiaux, Eugene

    1993-01-01

    Cloud-top height is a major factor determining the outgoing longwave flux at the top of the atmosphere. The downwelling radiation from the cloud strongly affects the cooling rate within the atmosphere and the longwave radiation incident at the surface. Thus, determination of cloud-base temperature is important for proper calculation of fluxes below the cloud. Cloud-base altitude is also an important factor in aircraft operations. Cloud-top height or temperature can be derived in a straightforward manner using satellite-based infrared data. Cloud-base temperature, however, is not observable from the satellite, but is related to the height, phase, and optical depth of the cloud in addition to other variables. This study uses surface and satellite data taken during the First ISCCP Regional Experiment (FIRE) Phase-2 Intensive Field Observation (IFO) period (13 Nov. - 7 Dec. 1991, to improve techniques for deriving cloud-base height from conventional satellite data.

  10. Clouds across the Arctic: A spatial perspective uniting surface observations of downwelling infrared radiation, reanalyses and education

    Science.gov (United States)

    Cox, Christopher J.

    The polar regions serve an important role in the Earth's energy balance by acting as a heat sink for the global climate system. In the Arctic, a complex distribution of continental and oceanic features support large spatial variability in environmental parameters important for climate. Additionally, feedbacks that are unique to the cryosphere cause the region to be very sensitive to climate perturbations. Environmental changes are being observed, including increasing temperatures, reductions in sea ice extent and thickness, melting permafrost, changing atmospheric circulation patterns and changing cloud properties, which may be signaling a shift in climate. Despite these changes, the Arctic remains an understudied region, including with respect to the atmosphere and clouds. A better understanding of cloud properties and their geographical variability is needed to better understand observed changes and to forecast the future state of the system, to support adaptation and mitigation strategies, and understand how Arctic change impacts other regions of the globe. Surface-based observations of the atmosphere are critical measurements in this effort because they are high quality and have high temporal resolution, but there are few atmospheric observatories in the Arctic and the period of record is short. Reanalyses combine assimilated observations with models to fill in spatial and temporal data gaps, and also provide additional model-derived parameters. Reanalyses are spatially comprehensive, but are limited by large uncertainties and biases, in particular with respect to derived parameters. Infrared radiation is a large component of the surface energy budget. Infrared emission from clouds is closely tied to cloud properties, so measurements of the infrared spectrum can be used to retrieve information about clouds and can also be used to investigate the influence clouds have on the surface radiation balance. In this dissertation, spectral infrared radiances and other

  11. Inverse modelling estimates of N2O surface emissions and stratospheric losses using a global dataset

    Science.gov (United States)

    Thompson, R. L.; Bousquet, P.; Chevallier, F.; Dlugokencky, E. J.; Vermeulen, A. T.; Aalto, T.; Haszpra, L.; Meinhardt, F.; O'Doherty, S.; Moncrieff, J. B.; Popa, M.; Steinbacher, M.; Jordan, A.; Schuck, T. J.; Brenninkmeijer, C. A.; Wofsy, S. C.; Kort, E. A.

    2010-12-01

    Nitrous oxide (N2O) levels have been steadily increasing in the atmosphere over the past few decades at a rate of approximately 0.3% per year. This trend is of major concern as N2O is both a long-lived Greenhouse Gas (GHG) and an Ozone Depleting Substance (ODS), as it is a precursor of NO and NO2, which catalytically destroy ozone in the stratosphere. Recently, N2O emissions have been recognised as the most important ODS emissions and are now of greater importance than emissions of CFC's. The growth in atmospheric N2O is predominantly due to the enhancement of surface emissions by human activities. Most notably, the intensification and proliferation of agriculture since the mid-19th century, which has been accompanied by the increased input of reactive nitrogen to soils and has resulted in significant perturbations to the natural N-cycle and emissions of N2O. There exist two approaches for estimating N2O emissions, the so-called 'bottom-up' and 'top-down' approaches. Top-down approaches, based on the inversion of atmospheric measurements, require an estimate of the loss of N2O via photolysis and oxidation in the stratosphere. Uncertainties in the loss magnitude contribute uncertainties of 15 to 20% to the global annual surface emissions, complicating direct comparisons between bottom-up and top-down estimates. In this study, we present a novel inversion framework for the simultaneous optimization of N2O surface emissions and the magnitude of the loss, which avoids errors in the emissions due to incorrect assumptions about the lifetime of N2O. We use a Bayesian inversion with a variational formulation (based on 4D-Var) in order to handle very large datasets. N2O fluxes are retrieved at 4-weekly resolution over a global domain with a spatial resolution of 3.75° x 2.5° longitude by latitude. The efficacy of the simultaneous optimization of emissions and losses is tested using a global synthetic dataset, which mimics the available atmospheric data. Lastly, using real

  12. Climatology and energy budget of the northern hemisphere middle stratosphere during 1972

    Energy Technology Data Exchange (ETDEWEB)

    Tahnk, W R [Air Force Geophysics Lab., Bedforo, MA; Newell, R E

    1975-01-01

    The 10-2 mb (approx. 30 to 40 km) layer of the atmosphere in winter receives energy from two different sources: mechanical energy is carried up from the troposphere and lower stratosphere while energy is generated in situ by the gradients of radiative heating and cooling. We show here from data for 1972 that the latter primarily governs the energy budget of the middle stratosphere in early winter while the former becomes of comparable size, and often dominates, in the middle and late winter. Radiative energy sources for the summer hemisphere are very small, as there is considerable compensation between solar heating through ozone absorption and infrared cooling by carbon dioxide and ozone. Standing and travelling waves are quite clear-cut at 5 and 2 mb in winter, as much of the chaos of lower regions is filtered out in the lower stratosphere; the standing waves at 2 mb may reflect surface properties more effectively than flow patterns at lower levels. A westward-travelling wave, with a period of about a month, was evident in early 1972.

  13. Co-ordinated ozone and UV project COZUV

    International Nuclear Information System (INIS)

    Braathen, Geir

    1999-01-01

    The project encompasses all the major Norwegian research groups in the field of stratospheric ozone and UV research. the duration is from the 1st January 1999 to the 31st December 2000. The tasks carried out will include investigations of the ozone layer over the North Polar and middle latitudes, 3-D chemical modelling, diagnosis of chemical ozone loss, investigations of transport mechanisms between the polar vortex and middle latitudes, study of the coupling between ozone change and climate change in the stratosphere and upper troposphere, scenario calculations in order to investigate the consequences of temperature change in the stratosphere, development of methods to measure global, direct and radiance distribution of UV, to improve UV dose calculations, investigate the influence of clouds on the surface UV radiation and to use existing surface UV radiation measurements together with existing radiation models to investigate the connection between UV radiation and ozone, clouds and surface albedo. The results will be published in various publications, progress reports, by participation in international conferences, through information to the environmental authorities and through information on the Internet

  14. EVALUATION MODEL FOR PAVEMENT SURFACE DISTRESS ON 3D POINT CLOUDS FROM MOBILE MAPPING SYSTEM

    Directory of Open Access Journals (Sweden)

    K. Aoki

    2012-07-01

    Full Text Available This paper proposes a methodology to evaluate the pavement surface distress for maintenance planning of road pavement using 3D point clouds from Mobile Mapping System (MMS. The issue on maintenance planning of road pavement requires scheduled rehabilitation activities for damaged pavement sections to keep high level of services. The importance of this performance-based infrastructure asset management on actual inspection data is globally recognized. Inspection methodology of road pavement surface, a semi-automatic measurement system utilizing inspection vehicles for measuring surface deterioration indexes, such as cracking, rutting and IRI, have already been introduced and capable of continuously archiving the pavement performance data. However, any scheduled inspection using automatic measurement vehicle needs much cost according to the instruments’ specification or inspection interval. Therefore, implementation of road maintenance work, especially for the local government, is difficult considering costeffectiveness. Based on this background, in this research, the methodologies for a simplified evaluation for pavement surface and assessment of damaged pavement section are proposed using 3D point clouds data to build urban 3D modelling. The simplified evaluation results of road surface were able to provide useful information for road administrator to find out the pavement section for a detailed examination and for an immediate repair work. In particular, the regularity of enumeration of 3D point clouds was evaluated using Chow-test and F-test model by extracting the section where the structural change of a coordinate value was remarkably achieved. Finally, the validity of the current methodology was investigated by conducting a case study dealing with the actual inspection data of the local roads.

  15. Radiative effect differences between multi-layered and single-layer clouds derived from CERES, CALIPSO, and CloudSat data

    International Nuclear Information System (INIS)

    Li Jiming; Yi Yuhong; Minnis, Patrick; Huang Jianping; Yan Hongru; Ma Yuejie; Wang Wencai; Kirk Ayers, J.

    2011-01-01

    Clouds alter general circulation through modification of the radiative heating profile within the atmosphere. Their effects are complex and depend on height, vertical structure, and phase. The instantaneous cloud radiative effect (CRE) induced by multi-layered (ML) and single-layer (SL) clouds is estimated by analyzing data collected by the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO), CloudSat, and Clouds and Earth's Radiation Energy Budget System (CERES) missions from March 2007 through February 2008. The CRE differences between ML and SL clouds at the top of the atmosphere (TOA) and at the surface were also examined. The zonal mean shortwave (SW) CRE differences between the ML and SL clouds at the TOA and surface were positive at most latitudes, peaking at 120 W m -2 in the tropics and dropping to -30 W m -2 at higher latitudes. This indicated that the ML clouds usually reflected less sunlight at the TOA and transmitted more to the surface than the SL clouds, due to their higher cloud top heights. The zonal mean longwave (LW) CRE differences between ML and SL clouds at the TOA and surface were relatively small, ranging from -30 to 30 W m -2 . This showed that the ML clouds only increased the amount of thermal radiation at the TOA relative to the SL clouds in the tropics, decreasing it elsewhere. In other words, ML clouds tended to cool the atmosphere in the tropics and warm it elsewhere when compared to SL clouds. The zonal mean net CRE differences were positive at most latitudes and dominated by the SW CRE differences.

  16. Climate impact of idealized winter polar mesospheric and stratospheric ozone losses as caused by energetic particle precipitation

    Directory of Open Access Journals (Sweden)

    K. Meraner

    2018-01-01

    Full Text Available Energetic particles enter the polar atmosphere and enhance the production of nitrogen oxides and hydrogen oxides in the winter stratosphere and mesosphere. Both components are powerful ozone destroyers. Recently, it has been inferred from observations that the direct effect of energetic particle precipitation (EPP causes significant long-term mesospheric ozone variability. Satellites observe a decrease in mesospheric ozone up to 34 % between EPP maximum and EPP minimum. Stratospheric ozone decreases due to the indirect effect of EPP by about 10–15 % observed by satellite instruments. Here, we analyze the climate impact of winter boreal idealized polar mesospheric and polar stratospheric ozone losses as caused by EPP in the coupled Max Planck Institute Earth System Model (MPI-ESM. Using radiative transfer modeling, we find that the radiative forcing of mesospheric ozone loss during polar night is small. Hence, climate effects of mesospheric ozone loss due to energetic particles seem unlikely. Stratospheric ozone loss due to energetic particles warms the winter polar stratosphere and subsequently weakens the polar vortex. However, those changes are small, and few statistically significant changes in surface climate are found.

  17. Aerosol-Induced Changes of Convective Cloud Anvils Produce Strong Climate Warming

    Science.gov (United States)

    Koren, I.; Remer, L. A.; Altaratz, O.; Martins, J. V.; Davidi, A.

    2010-01-01

    The effect of aerosol on clouds poses one of the largest uncertainties in estimating the anthropogenic contribution to climate change. Small human-induced perturbations to cloud characteristics via aerosol pathways can create a change in the top-of-atmosphere radiative forcing of hundreds of Wm(exp-2) . Here we focus on links between aerosol and deep convective clouds of the Atlantic and Pacific Intertropical Convergence Zones, noting that the aerosol environment in each region is entirely different. The tops of these vertically developed clouds consisting of mostly ice can reach high levels of the atmosphere, overshooting the lower stratosphere and reaching altitudes greater than 16 km. We show a link between aerosol, clouds and the free atmosphere wind profile that can change the magnitude and sign of the overall climate radiative forcing. We find that increased aerosol loading is associated with taller cloud towers and anvils. The taller clouds reach levels of enhanced wind speeds that act to spread and thin the anvi1 clouds, increasing areal coverage and decreasing cloud optical depth. The radiative effect of this transition is to create a positive radiative forcing (warming) at top-of-atmosphere. Furthermore we introduce the cloud optical depth (r), cloud height (Z) forcing space and show that underestimation of radiative forcing is likely to occur in cases of non homogenous clouds. Specifically, the mean radiative forcing of towers and anvils in the same scene can be several times greater than simply calculating the forcing from the mean cloud optical depth in the scene. Limitations of the method are discussed, alternative sources of aerosol loading are tested and meteorological variance is restricted, but the trend of taller clouds; increased and thinner anvils associated with increased aerosol loading remains robust through all the different tests and perturbations.

  18. Aerosol-induced changes of convective cloud anvils produce strong climate warming

    Directory of Open Access Journals (Sweden)

    I. Koren

    2010-05-01

    Full Text Available The effect of aerosol on clouds poses one of the largest uncertainties in estimating the anthropogenic contribution to climate change. Small human-induced perturbations to cloud characteristics via aerosol pathways can create a change in the top-of-atmosphere radiative forcing of hundreds of Wm−2. Here we focus on links between aerosol and deep convective clouds of the Atlantic and Pacific Intertropical Convergence Zones, noting that the aerosol environment in each region is entirely different. The tops of these vertically developed clouds consisting of mostly ice can reach high levels of the atmosphere, overshooting the lower stratosphere and reaching altitudes greater than 16 km. We show a link between aerosol, clouds and the free atmosphere wind profile that can change the magnitude and sign of the overall climate radiative forcing.

    We find that increased aerosol loading is associated with taller cloud towers and anvils. The taller clouds reach levels of enhanced wind speeds that act to spread and thin the anvil clouds, increasing areal coverage and decreasing cloud optical depth. The radiative effect of this transition is to create a positive radiative forcing (warming at top-of-atmosphere.

    Furthermore we introduce the cloud optical depth (τ, cloud height (Z forcing space and show that underestimation of radiative forcing is likely to occur in cases of non homogenous clouds. Specifically, the mean radiative forcing of towers and anvils in the same scene can be several times greater than simply calculating the forcing from the mean cloud optical depth in the scene.

    Limitations of the method are discussed, alternative sources of aerosol loading are tested and meteorological variance is restricted, but the trend of taller clouds, increased and thinner anvils associated with increased aerosol loading remains robust through all the different tests and perturbations.

  19. Uncertainties of Large-Scale Forcing Caused by Surface Turbulence Flux Measurements and the Impacts on Cloud Simulations at the ARM SGP Site

    Science.gov (United States)

    Tang, S.; Xie, S.; Tang, Q.; Zhang, Y.

    2017-12-01

    Two types of instruments, the eddy correlation flux measurement system (ECOR) and the energy balance Bowen ratio system (EBBR), are used at the Atmospheric Radiation Measurement (ARM) program Southern Great Plains (SGP) site to measure surface latent and sensible fluxes. ECOR and EBBR typically sample different land surface types, and the domain-mean surface fluxes derived from ECOR and EBBR are not always consistent. The uncertainties of the surface fluxes will have impacts on the derived large-scale forcing data and further affect the simulations of single-column models (SCM), cloud-resolving models (CRM) and large-eddy simulation models (LES), especially for the shallow-cumulus clouds which are mainly driven by surface forcing. This study aims to quantify the uncertainties of the large-scale forcing caused by surface turbulence flux measurements and investigate the impacts on cloud simulations using long-term observations from the ARM SGP site.

  20. Triton - Stratospheric molecules and organic sediments

    Science.gov (United States)

    Thompson, W. Reid; Singh, Sushil K.; Khare, B. N.; Sagan, Carl

    1989-01-01

    Continuous-flow plasma discharge techniques show production rates of hydrocarbons and nitriles in N2 + CH4 atmospheres appropriate to the stratosphere of Titan, and indicate that a simple eddy diffusion model together with the observed electron flux quantitatively matches the Voyager IRIS observations for all the hydrocarbons, except for the simplest ones. Charged particle chemistry is very important in Triton's stratosphere. In the more CH4-rich case of Titan, many hydrocarbons and nitriles are produced in high yield. If N2 is present, the CH4 fraction is low, but hydrocarbons and nitriles are produced in fair yield, abundances of HCN and C2H2 in Triton's stratosphere exceed 10 to the 19th molecules/sq cm per sec, and NCCN, C3H4, and other species are predicted to be present. These molecules may be detected by IRIS if the stratosphere is as warm as expected. Both organic haze and condensed gases will provide a substantial UV and visible opacity in Triton's atmosphere.

  1. Combined retrieval of Arctic liquid water cloud and surface snow properties using airborne spectral solar remote sensing

    Science.gov (United States)

    Ehrlich, André; Bierwirth, Eike; Istomina, Larysa; Wendisch, Manfred

    2017-09-01

    The passive solar remote sensing of cloud properties over highly reflecting ground is challenging, mostly due to the low contrast between the cloud reflectivity and that of the underlying surfaces (sea ice and snow). Uncertainties in the retrieved cloud optical thickness τ and cloud droplet effective radius reff, C may arise from uncertainties in the assumed spectral surface albedo, which is mainly determined by the generally unknown effective snow grain size reff, S. Therefore, in a first step the effects of the assumed snow grain size are systematically quantified for the conventional bispectral retrieval technique of τ and reff, C for liquid water clouds. In general, the impact of uncertainties of reff, S is largest for small snow grain sizes. While the uncertainties of retrieved τ are independent of the cloud optical thickness and solar zenith angle, the bias of retrieved reff, C increases for optically thin clouds and high Sun. The largest deviations between the retrieved and true original values are found with 83 % for τ and 62 % for reff, C. In the second part of the paper a retrieval method is presented that simultaneously derives all three parameters (τ, reff, C, reff, S) and therefore accounts for changes in the snow grain size. Ratios of spectral cloud reflectivity measurements at the three wavelengths λ1 = 1040 nm (sensitive to reff, S), λ2 = 1650 nm (sensitive to τ), and λ3 = 2100 nm (sensitive to reff, C) are combined in a trispectral retrieval algorithm. In a feasibility study, spectral cloud reflectivity measurements collected by the Spectral Modular Airborne Radiation measurement sysTem (SMART) during the research campaign Vertical Distribution of Ice in Arctic Mixed-Phase Clouds (VERDI, April/May 2012) were used to test the retrieval procedure. Two cases of observations above the Canadian Beaufort Sea, one with dense snow-covered sea ice and another with a distinct snow-covered sea ice edge are analysed. The retrieved values of τ, reff

  2. Low cloud precipitation climatology in the southeastern Pacific marine stratocumulus region using CloudSat

    International Nuclear Information System (INIS)

    Rapp, Anita D; Lebsock, Matthew; L’Ecuyer, Tristan

    2013-01-01

    A climatology of low cloud surface precipitation occurrence and intensity from the new CloudSat 2C-RAIN-PROFILE algorithm is presented from June 2006 through December 2010 for the southeastern Pacific region of marine stratocumulus. Results show that over 70% of low cloud precipitation falls as drizzle. Application of an empirical evaporation model suggests that 50–80% of the precipitation evaporates before it reaches the surface. Segregation of the CloudSat ascending and descending overpasses shows that the majority of precipitation occurs at night. Examination of the seasonal cycle shows that the precipitation is most frequent during the austral winter and spring; however there is considerable regional variability. Conditional rain rates increase from east to west with a maximum occurring in the region influenced by the South Pacific Convergence Zone. Area average rain rates are highest in the region where precipitation rates are moderate, but most frequent. The area average surface rain rate for low cloud precipitation for this region is ∼0.22 mm d −1 , in good agreement with in situ estimates, and is greatly improved over earlier CloudSat precipitation products. These results provide a much-needed quantification of surface precipitation in a region that is currently underestimated in existing satellite-based precipitation climatologies. (letter)

  3. How does Interactive Chemistry Influence the Representation of Stratosphere-Troposphere Coupling in a Climate Model?

    Science.gov (United States)

    Haase, S.; Matthes, K. B.

    2017-12-01

    Changes in stratospheric ozone can trigger tropospheric circulation changes. In the Southern hemisphere (SH), the observed shift of the Southern Annular Mode was attributed to the observed trend in lower stratospheric ozone. In the Northern Hemisphere (NH), a recent study showed that extremely low stratospheric ozone conditions during spring produce robust anomalies in the troposphere (zonal wind, temperature and precipitation). This could only be reproduced in a coupled chemistry climate model indicating that chemical-dynamical feedbacks are also important on the NH. To further investigate the importance of interactive chemistry for surface climate, we conducted a set of experiments using NCAR's Community Earth System Model (CESM1) with the Whole Atmosphere Community Climate Model (WACCM) as the atmosphere component. WACCM contains a fully interactive stratospheric chemistry module in its standard configuration. It also allows for an alternative configuration, referred to as SC-WACCM, in which the chemistry (O3, NO, O, O2, CO2 and chemical and shortwave heating rates) is specified as a 2D field in the radiation code. A comparison of the interactive vs. the specified chemistry version enables us to evaluate the relative importance of interactive chemistry by systematically inhibiting the feedbacks between chemistry and dynamics. To diminish the effect of temporal interpolation when prescribing ozone, we use daily resolved zonal mean ozone fields for the specified chemistry run. Here, we investigate the differences in stratosphere-troposphere coupling between the interactive and specified chemistry simulations for the mainly chemically driven SH as well as for the mainly dynamically driven NH. We will especially consider years that are characterized by extremely low stratospheric ozone on the one hand and by large dynamical disturbances, i.e. Sudden Stratospheric Warmings, on the other hand.

  4. 30-year lidar observations of the stratospheric aerosol layer state over Tomsk (Western Siberia, Russia)

    Science.gov (United States)

    Zuev, Vladimir V.; Burlakov, Vladimir D.; Nevzorov, Aleksei V.; Pravdin, Vladimir L.; Savelieva, Ekaterina S.; Gerasimov, Vladislav V.

    2017-02-01

    There are only four lidar stations in the world which have almost continuously performed observations of the stratospheric aerosol layer (SAL) state over the last 30 years. The longest time series of the SAL lidar measurements have been accumulated at the Mauna Loa Observatory (Hawaii) since 1973, the NASA Langley Research Center (Hampton, Virginia) since 1974, and Garmisch-Partenkirchen (Germany) since 1976. The fourth lidar station we present started to perform routine observations of the SAL parameters in Tomsk (56.48° N, 85.05° E, Western Siberia, Russia) in 1986. In this paper, we mainly focus on and discuss the stratospheric background period from 2000 to 2005 and the causes of the SAL perturbations over Tomsk in the 2006-2015 period. During the last decade, volcanic aerosol plumes from tropical Mt. Manam, Soufrière Hills, Rabaul, Merapi, Nabro, and Kelut and extratropical (northern) Mt. Okmok, Kasatochi, Redoubt, Sarychev Peak, Eyjafjallajökull, and Grímsvötn were detected in the stratosphere over Tomsk. When it was possible, we used the NOAA HYSPLIT trajectory model to assign aerosol layers observed over Tomsk to the corresponding volcanic eruptions. The trajectory analysis highlighted some surprising results. For example, in the cases of the Okmok, Kasatochi, and Eyjafjallajökull eruptions, the HYSPLIT air mass backward trajectories, started from altitudes of aerosol layers detected over Tomsk with a lidar, passed over these volcanoes on their eruption days at altitudes higher than the maximum plume altitudes given by the Smithsonian Institution Global Volcanism Program. An explanation of these facts is suggested. The role of both tropical and northern volcanic eruptions in volcanogenic aerosol loading of the midlatitude stratosphere is also discussed. In addition to volcanoes, we considered other possible causes of the SAL perturbations over Tomsk, i.e., the polar stratospheric cloud (PSC) events and smoke plumes from strong forest fires. At least

  5. A Statistical Review of CALIOP Version 3 and Version 4 Cloud Aerosol Discrimination

    Science.gov (United States)

    Zeng, S.

    2016-12-01

    The Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) on board the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) mission has now delivered a 10-year record of high-resolution profiles of backscatter at 532 nm and 1064 nm and linear depolarization at 532 nm. These long-term active sensor measurements at global scale have led to significant advances in our understanding of the vertical distribution of clouds and aerosols in the atmosphere. In the fall of 2016, the CALIPSO science team is scheduled to release a new version of their cloud and aerosol data products. The new cloud and aerosol discrimination products are derived using updated probability density functions that account for numerous improvements to the CALIOP calibration and the use of the GMAO MERRA-2 meteorological data. Moreover, the CAD algorithm is now applied to all layers detected, thus greatly improving the identification of such features as overshooting convective clouds, stratospheric aerosol layers, and high intensity dust storms. Post-processing modules are added to the standard CAD algorithm to ensure proper identification of (for example) the tenuous edges of cirrus clouds and water clouds lying beneath optically dense smoke layers. This work presents statistical comparisons between the CALIOP version 3 and version 4 data sets. Areas of improvement are highlighted, sources of continuing uncertainty are discussed and a list of best practices for data users is provided.

  6. Influence of stratospheric aerosol on albedo

    Energy Technology Data Exchange (ETDEWEB)

    Gormatyuk, Yu K; Kaufman, Yu G; Kolomeev, M P

    1985-06-01

    The influence of stratospheric aerosol (SA) on the transfer of solar radiation in the atmosphere is the principal factor determining the effect of SA on climate. The change in the radiation balance under the influence of SA is computed most precisely in radiative-convective models. However, the complex method used in these models cannot be used for other types of climate models. The objective of the study was to obtain a quantitative evaluation of the influence of SA on albedo without the use of simplifying assumptions. In the approximation of single scattering an expression is derived for change in albedo under the influence of stratospheric aerosol taking into account the dependence of albedo of the atmosphere-earth's surface system on solar zenith distance. The authors give the results of computations of the response of mean annual albedo to sulfuric acid aerosol for 10/sup 0/ latitude zones in the Northern Hemisphere. Specifically, computations of the optical characteristics of aerosol were made using the Mie theory for 10 spectral intervals taking in the range of wavelengths of solar radiation from 0.29 to 4.0 ..mu.. m. The refractive index of aerosol was stipulated in accordance with Palmer and Williams. The angular dependence of albedo for cloudless and cloudy atmospheres given by Harshvardhan was used. The values of undisturbed albedo were assumed to be identical for all wavelengths due to lack of climatological data on the spectral dependence of albedo of the atmosphere-earth's surface system. The angular distribution of the intensity of solar radiation for each of the latitude zones was computed by the method described by I.M. Alekseyev, et al.

  7. Role of Stratospheric Water Vapor in Global Warming from GCM Simulations Constrained by MLS Observation

    Science.gov (United States)

    Wang, Y.; Stek, P. C.; Su, H.; Jiang, J. H.; Livesey, N. J.; Santee, M. L.

    2014-12-01

    Over the past century, global average surface temperature has warmed by about 0.16°C/decade, largely due to anthropogenic increases in well-mixed greenhouse gases. However, the trend in global surface temperatures has been nearly flat since 2000, raising a question regarding the exploration of the drivers of climate change. Water vapor is a strong greenhouse gas in the atmosphere. Previous studies suggested that the sudden decrease of stratospheric water vapor (SWV) around 2000 may have contributed to the stall of global warming. Since 2004, the SWV observed by Microwave Limb Sounder (MLS) on Aura satellite has shown a slow recovery. The role of recent SWV variations in global warming has not been quantified. We employ a coupled atmosphere-ocean climate model, the NCAR CESM, to address this issue. It is found that the CESM underestimates the stratospheric water vapor by about 1 ppmv due to limited representations of the stratospheric dynamic and chemical processes important for water vapor variabilities. By nudging the modeled SWV to the MLS observation, we find that increasing SWV by 1 ppmv produces a robust surface warming about 0.2°C in global-mean when the model reaches equilibrium. Conversely, the sudden drop of SWV from 2000 to 2004 would cause a surface cooling about -0.08°C in global-mean. On the other hand, imposing the observed linear trend of SWV based on the 10-year observation of MLS in the CESM yields a rather slow surface warming, about 0.04°C/decade. Our model experiments suggest that SWV contributes positively to the global surface temperature variation, although it may not be the dominant factor that drives the recent global warming hiatus. Additional sensitivity experiments show that the impact of SWV on surface climate is mostly governed by the SWV amount at 100 hPa in the tropics. Furthermore, the atmospheric model simulations driven by observed sea surface temperature (SST) show that the inter-annual variation of SWV follows that of SST

  8. Comparison of stratospheric temperature profiles from a ground-based microwave radiometer with lidar, radiosonde and satellite data

    Science.gov (United States)

    Navas-Guzmán, Francisco; Kämpfer, Niklaus; Haefele, Alexander; Keckhut, Philippe; Hauchecorne, Alain

    2015-04-01

    The importance of the knowledge of the temperature structure in the atmosphere has been widely recognized. Temperature is a key parameter for dynamical, chemical and radiative processes in the atmosphere. The cooling of the stratosphere is an indicator for climate change as it provides evidence of natural and anthropogenic climate forcing just like surface warming ( [1] and references therein). However, our understanding of the observed stratospheric temperature trend and our ability to test simulations of the stratospheric response to emissions of greenhouse gases and ozone depleting substances remains limited. Stratospheric long-term datasets are sparse and obtained trends differ from one another [1]. Therefore it is important that in the future such datasets are generated. Different techniques allow to measure stratospheric temperature profiles as radiosonde, lidar or satellite. The main advantage of microwave radiometers against these other instruments is a high temporal resolution with a reasonable good spatial resolution. Moreover, the measurement at a fixed location allows to observe local atmospheric dynamics over a long time period, which is crucial for climate research. TEMPERA (TEMPERature RAdiometer) is a newly developed ground-based microwave radiometer designed, built and operated at the University of Bern. The instrument and the retrieval of temperature profiles has been described in detail in [2]. TEMPERA is measuring a pressure broadened oxygen line at 53.1 GHz in order to determine stratospheric temperature profiles. The retrieved profiles of TEMPERA cover an altitude range of approximately 20 to 45 km with a vertical resolution in the order of 15 km. The lower limit is given by the instrumental baseline and the bandwidth of the measured spectrum. The upper limit is given by the fact that above 50 km the oxygen lines are splitted by the Zeeman effect in the terrestrial magnetic field. In this study we present a comparison of stratospheric

  9. Hierarchical Threshold Adaptive for Point Cloud Filter Algorithm of Moving Surface Fitting

    Directory of Open Access Journals (Sweden)

    ZHU Xiaoxiao

    2018-02-01

    Full Text Available In order to improve the accuracy,efficiency and adaptability of point cloud filtering algorithm,a hierarchical threshold adaptive for point cloud filter algorithm of moving surface fitting was proposed.Firstly,the noisy points are removed by using a statistic histogram method.Secondly,the grid index is established by grid segmentation,and the surface equation is set up through the lowest point among the neighborhood grids.The real height and fit are calculated.The difference between the elevation and the threshold can be determined.Finally,in order to improve the filtering accuracy,hierarchical filtering is used to change the grid size and automatically set the neighborhood size and threshold until the filtering result reaches the accuracy requirement.The test data provided by the International Photogrammetry and Remote Sensing Society (ISPRS is used to verify the algorithm.The first and second error and the total error are 7.33%,10.64% and 6.34% respectively.The algorithm is compared with the eight classical filtering algorithms published by ISPRS.The experiment results show that the method has well-adapted and it has high accurate filtering result.

  10. Trajectory tracking control for underactuated stratospheric airship

    Science.gov (United States)

    Zheng, Zewei; Huo, Wei; Wu, Zhe

    2012-10-01

    Stratospheric airship is a new kind of aerospace system which has attracted worldwide developing interests for its broad application prospects. Based on the trajectory linearization control (TLC) theory, a novel trajectory tracking control method for an underactuated stratospheric airship is presented in this paper. Firstly, the TLC theory is described sketchily, and the dynamic model of the stratospheric airship is introduced with kinematics and dynamics equations. Then, the trajectory tracking control strategy is deduced in detail. The designed control system possesses a cascaded structure which consists of desired attitude calculation, position control loop and attitude control loop. Two sub-loops are designed for the position and attitude control loops, respectively, including the kinematics control loop and dynamics control loop. Stability analysis shows that the controlled closed-loop system is exponentially stable. Finally, simulation results for the stratospheric airship to track typical trajectories are illustrated to verify effectiveness of the proposed approach.

  11. Kinetic model framework for aerosol and cloud surface chemistry and gas-particle interactions - Part 1: General equations, parameters, and terminology

    Science.gov (United States)

    Pöschl, U.; Rudich, Y.; Ammann, M.

    2007-12-01

    Aerosols and clouds play central roles in atmospheric chemistry and physics, climate, air pollution, and public health. The mechanistic understanding and predictability of aerosol and cloud properties, interactions, transformations, and effects are, however, still very limited. This is due not only to the limited availability of measurement data, but also to the limited applicability and compatibility of model formalisms used for the analysis, interpretation, and description of heterogeneous and multiphase processes. To support the investigation and elucidation of atmospheric aerosol and cloud surface chemistry and gas-particle interactions, we present a comprehensive kinetic model framework with consistent and unambiguous terminology and universally applicable rate equations and parameters. It enables a detailed description of mass transport and chemical reactions at the gas-particle interface, and it allows linking aerosol and cloud surface processes with gas phase and particle bulk processes in systems with multiple chemical components and competing physicochemical processes. The key elements and essential aspects of the presented framework are: a simple and descriptive double-layer surface model (sorption layer and quasi-static layer); straightforward flux-based mass balance and rate equations; clear separation of mass transport and chemical reactions; well-defined and consistent rate parameters (uptake and accommodation coefficients, reaction and transport rate coefficients); clear distinction between gas phase, gas-surface, and surface-bulk transport (gas phase diffusion, surface and bulk accommodation); clear distinction between gas-surface, surface layer, and surface-bulk reactions (Langmuir-Hinshelwood and Eley-Rideal mechanisms); mechanistic description of concentration and time dependences (transient and steady-state conditions); flexible addition of unlimited numbers of chemical species and physicochemical processes; optional aggregation or resolution

  12. Stratospheric Aerosol and Gas Experiment (SAGE) IV Pathfinder

    Data.gov (United States)

    National Aeronautics and Space Administration — The Clean Air Act mandates NASA to monitor stratospheric ozone, and stratospheric aerosol measurements are vital to our understanding of climate.  Maintaining...

  13. Improved SAGE II cloud/aerosol categorization and observations of the Asian tropopause aerosol layer: 1989–2005

    Directory of Open Access Journals (Sweden)

    L. W. Thomason

    2013-05-01

    Full Text Available We describe the challenges associated with the interpretation of extinction coefficient measurements by the Stratospheric Aerosol and Gas Experiment (SAGE II in the presence of clouds. In particular, we have found that tropospheric aerosol analyses are highly dependent on a robust method for identifying when clouds affect the measured extinction coefficient. Herein, we describe an improved cloud identification method that appears to capture cloud/aerosol events more effectively than early methods. In addition, we summarize additional challenges to observing the Asian Tropopause Aerosol Layer (ATAL using SAGE II observations. Using this new approach, we perform analyses of the upper troposphere, focusing on periods in which the UTLS (upper troposphere/lower stratosphere is relatively free of volcanic material (1989–1990 and after 1996. Of particular interest is the Asian monsoon anticyclone where CALIPSO (Cloud-Aerosol Lidar Pathfinder Satellite Observations has observed an aerosol enhancement. This enhancement, called the ATAL, has a similar morphology to observed enhancements in long-lived trace gas species like CO. Since the CALIPSO record begins in 2006, the question of how long this aerosol feature has been present requires a new look at the long-lived SAGE II data sets despite significant hurdles to its use in the subtropical upper troposphere. We find that there is no evidence of ATAL in the SAGE II data prior to 1998. After 1998, it is clear that aerosol in the upper troposphere in the ATAL region is substantially enhanced relative to the period before that time. In addition, the data generally supports the presence of the ATAL beginning in 1999 and continuing through the end of the mission, though some years (e.g., 2003 are complicated by the presence of episodic enhancements most likely of volcanic origin.

  14. The effects of the Indo-Pacific warm pool on the stratosphere

    Science.gov (United States)

    Zhou, Xin; Li, Jianping; Xie, Fei; Ding, Ruiqiang; Li, Yanjie; Zhao, Sen; Zhang, Jiankai; Li, Yang

    2017-03-01

    Sea surface temperature (SST) in the Indo-Pacific warm pool (IPWP) plays a key role in influencing East Asian climate, and even affects global-scale climate change. This study defines IPWP Niño and IPWP Niña events to represent the warm and cold phases of IPWP SST anomalies, respectively, and investigates the effects of these events on stratospheric circulation and temperature. Results from simulations forced by observed SST anomalies during IPWP Niño and Niña events show that the tropical lower stratosphere tends to cool during IPWP Niño events and warm during IPWP Niña events. The responses of the northern and southern polar vortices to IPWP Niño events are fairly symmetric, as both vortices are significantly warmed and weakened. However, the responses of the two polar vortices to IPWP Niña events are of opposite sign: the northern polar vortex is warmed and weakened, but the southern polar vortex is cooled and strengthened. These features are further confirmed by composite analysis using reanalysis data. A possible dynamical mechanism connecting IPWP SST to the stratosphere is suggested, in which IPWP Niño and Niña events excite teleconnections, one similar to the Pacific-North America pattern in the Northern Hemisphere and a Rossby wave train in the Southern Hemisphere, which project onto the climatological wave in the mid-high latitudes, intensifying the upward propagation of planetary waves into the stratosphere and, in turn, affecting the polar vortex.

  15. Isopleths of surface air concentration and surface air kerma rate due to a radioactive cloud released from a stack (3)

    International Nuclear Information System (INIS)

    Tachibana, Haruo; Kikuchi, Masamitsu; Sekita, Tsutomu; Yamaguchi, Takenori

    2004-06-01

    This report is a revised edition of 'Isopleths of Surface Air Concentration and Surface Air Absorbed Dose Rate due to a Radioactive Cloud Released from a Stack(II) '(JAERI-M 90-206) and based on the revised Nuclear Safety Guidelines reflected the ICRP1990 Recommendation. Characteristics of this report are the use of Air Karma Rate (Gy/h) instead of Air Absorbed Dose Rate (Gy/h), and the record of isopleths of surface air concentration and surface air karma rate on CD-ROM. These recorded data on CD-ROM can be printed out on paper and/or pasted on digital map by personal computer. (author)

  16. Size-specific composition of aerosols in the El Chichon volcanic cloud

    Science.gov (United States)

    Woods, D. C.; Chuan, R. L.

    1983-01-01

    A NASA U-2 research aircraft flew sampling missions in April, May, July, November, and December 1982 aimed at obtaining in situ data in the stratospheric cloud produced from the March-April 1982 El Chichon eruptions. Post flight analyses provided information on the aerosol composition and morphology. The particles ranged in size from smaller than 0.05 m to larger than 20 m diameter and were quite complex in composition. In the April, May, and July samples the aerosol mass was dominated by magmatic and lithic particles larger than about 3 m. The submicron particles consisted largely of sulfuric acid. Halite particles, believed to be related to a salt dome beneath El Chichon, were collected in the stratosphere in April and May. On the July 23 flight, copper-zinc oxide particles were collected. In July, November, and December, in addition to the volcanic ash and acid particles, carbon-rich particles smaller than about 0.1 m aerodynamic diameter were abundant.

  17. Combined retrieval of Arctic liquid water cloud and surface snow properties using airborne spectral solar remote sensing

    Directory of Open Access Journals (Sweden)

    A. Ehrlich

    2017-09-01

    Full Text Available The passive solar remote sensing of cloud properties over highly reflecting ground is challenging, mostly due to the low contrast between the cloud reflectivity and that of the underlying surfaces (sea ice and snow. Uncertainties in the retrieved cloud optical thickness τ and cloud droplet effective radius reff, C may arise from uncertainties in the assumed spectral surface albedo, which is mainly determined by the generally unknown effective snow grain size reff, S. Therefore, in a first step the effects of the assumed snow grain size are systematically quantified for the conventional bispectral retrieval technique of τ and reff, C for liquid water clouds. In general, the impact of uncertainties of reff, S is largest for small snow grain sizes. While the uncertainties of retrieved τ are independent of the cloud optical thickness and solar zenith angle, the bias of retrieved reff, C increases for optically thin clouds and high Sun. The largest deviations between the retrieved and true original values are found with 83 % for τ and 62 % for reff, C.In the second part of the paper a retrieval method is presented that simultaneously derives all three parameters (τ, reff, C, reff, S and therefore accounts for changes in the snow grain size. Ratios of spectral cloud reflectivity measurements at the three wavelengths λ1 = 1040 nm (sensitive to reff, S, λ2 = 1650 nm (sensitive to τ, and λ3 = 2100 nm (sensitive to reff, C are combined in a trispectral retrieval algorithm. In a feasibility study, spectral cloud reflectivity measurements collected by the Spectral Modular Airborne Radiation measurement sysTem (SMART during the research campaign Vertical Distribution of Ice in Arctic Mixed-Phase Clouds (VERDI, April/May 2012 were used to test the retrieval procedure. Two cases of observations above the Canadian Beaufort Sea, one with dense snow-covered sea ice and another with a distinct snow-covered sea ice

  18. Different Stratospheric Polar Vortex States linked to Cold-Spells in North America and Northern Eurasia

    Science.gov (United States)

    Kretschmer, M.; Cohen, J. L.; Runge, J.; Coumou, D.

    2017-12-01

    The stratospheric polar vortex in boreal winter can influence the tropospheric circulation and thereby surface weather in the mid-latitudes. Weak states of the vortex, e.g. associated with Sudden Stratospheric Warmings (SSWs), often precede a negative phase of the North Atlantic Oscillation (NAO), and thus increase the risk of mid-latitude cold-spells especially over Eurasia. Here we show using cluster analysis that next to the well-documented relationship between a zonally symmetric disturbed vortex and a negative NAO, there exists a zonally asymmetric pattern linked to a negative Western Pacific Oscillation (WPO) and cold-spells in the northeastern US, like for example observed in February 2014. The latter is more synoptic in time-scale but occurs more frequently than SSWs. A causal effect network (CEN) approach gives insights into the underlying physical pathways and time-lags showing that high-pressure around Greenland leads to vertical wave activity over eastern Siberia leading to downward propagating waves over Alaska and high pressure over the North Pacific. Moreover, composites propose that a rather strong mid-stratospheric vortex seems to be favorable for this zonally asymmetric and reflective mechanism. Overall, the mutual relationship between stratospheric circulation and high-latitude blocking in both the Pacific and Atlantic Oceans is complex and involves mechanisms operating at different time-scales. Our results suggest that the stratospheric influence on winter circulation should not exclusively be analyzed in terms of a downward propagating Northern Annular Mode (NAM) signal and SSWs. In particular when studying the stratospheric impacts on North American temperature it is crucial to also consider the more transient and zonally asymmetric events which might help to improve seasonal winter predictions for this region.

  19. Evaluation of cloud fraction and its radiative effect simulated by IPCC AR4 global models against ARM surface observations

    Directory of Open Access Journals (Sweden)

    Y. Qian

    2012-02-01

    Full Text Available Cloud Fraction (CF is the dominant modulator of radiative fluxes. In this study, we evaluate CF simulated in the IPCC AR4 GCMs against ARM long-term ground-based measurements, with a focus on the vertical structure, total amount of cloud and its effect on cloud shortwave transmissivity. Comparisons are performed for three climate regimes as represented by the Department of Energy Atmospheric Radiation Measurement (ARM sites: Southern Great Plains (SGP, Manus, Papua New Guinea and North Slope of Alaska (NSA. Our intercomparisons of three independent measurements of CF or sky-cover reveal that the relative differences are usually less than 10% (5% for multi-year monthly (annual mean values, while daily differences are quite significant. The total sky imager (TSI produces smaller total cloud fraction (TCF compared to a radar/lidar dataset for highly cloudy days (CF > 0.8, but produces a larger TCF value than the radar/lidar for less cloudy conditions (CF < 0.3. The compensating errors in lower and higher CF days result in small biases of TCF between the vertically pointing radar/lidar dataset and the hemispheric TSI measurements as multi-year data is averaged. The unique radar/lidar CF measurements enable us to evaluate seasonal variation of cloud vertical structures in the GCMs.

    Both inter-model deviation and model bias against observation are investigated in this study. Another unique aspect of this study is that we use simultaneous measurements of CF and surface radiative fluxes to diagnose potential discrepancies among the GCMs in representing other cloud optical properties than TCF. The results show that the model-observation and inter-model deviations have similar magnitudes for the TCF and the normalized cloud effect, and these deviations are larger than those in surface downward solar radiation and cloud transmissivity. This implies that other dimensions of cloud in addition to cloud amount, such as cloud optical thickness and

  20. A Model of the Effect of Ozone Depletion on Lower-Stratospheric Structure

    Science.gov (United States)

    Olsen, Mark A.; Stolarski, Richard S.; Gupta, Mohan L.; Nielsen, J. Eric; Pawson, Steven

    2005-01-01

    We have run two twenty-year integrations of a global circulation model using 1978-1980 and 1998-2000 monthly mean ozone climatologies. The ozone climatology is used solely in the radiation scheme of the model. Several key differences between the model runs will be presented. The temperature and potential vorticity (PV) structure of the lower stratosphere, particularly in the Southern Hemisphere, is significantly changed using the 1998-2000 ozone climatology. In the Southern Hemisphere summer, the lapse rate and PV-defined polar tropopauses are both at altitudes on the order of several hundred meters greater than the 1978-1980 climatological run. The 380 K potential temperature surf= is likewise at a greater altitude. The mass of the extratropical lowermost stratosphere (between the tropopause and 380 K surface) remains unchanged. The altitude differences are not observed in the Northern Hemisphere. The different ozone fields do not produce a significant change in the annual extratropical stratosphere-troposphere exchange of mass although slight variations in the spatial distribution of the exchange exist. We are also investigating a delay in the breakup of the Southern Hemisphere polar vortex due to the differing ozone climatologies.

  1. Monitoring cirrus cloud and tropopause height over Hanoi using a compact lidar system

    International Nuclear Information System (INIS)

    Bui Van Hai; Dinh Van Trung; Nguyen Xuan Tuan; Dao Duy Thang; Nguyen Thanh Binh

    2012-01-01

    Cirrus clouds in the upper troposphere and the lower stratosphere have attracted great attention due to their important role and impact on the atmospheric radioactive balance. Because cirrus clouds are located high in the atmosphere, their study requires a high resolution remote sensing technique not only for detection but also for the characterization of their properties. The lidar technique with its inherent high sensitivity and resolution has become an indispensable tool for studying and improving our understanding of cirrus cloud. Using lidar technique we can simultaneously measure the cloud height, thickness and follow its temporal evolution. In this paper we describe the development of a compact and highly sensitive lidar system with the aim to remotely monitor for the first time the cirrus clouds over Hanoi (2101:42 N, 10551:12 W). From the lidar data collected during the year 2011. We derive the mean cloud height, location of cloud top, the cloud mean thickness and their temporal evolution. We then compare the location of the cloud top with the position of the tropopause determined the radiosonde data and found good that the distance between cloud top and tropopause remains fairly stable, indicating that generally the top of cirrus clouds is the good tracer of the tropopause. We found that the cirrus clouds are generally located at height between 11.2 to 15 km with average height of 13.4 km. Their thickness is between 0.3 and 3.8 km with average value of 1.7 km. We also compare the properties of cirrus cloud with that observed at other locations around the world based on lidar technique. (author)

  2. Daily cycle of the surface energy balance in Antarctica and the influence of clouds

    NARCIS (Netherlands)

    van den Broeke, M.R.|info:eu-repo/dai/nl/073765643; Reijmer, C.H.|info:eu-repo/dai/nl/229345956; van As, D.; Boot, W.

    2006-01-01

    We present the summertime daily cycle of the Antarctic surface energy balance (SEB) and its sensitivity to cloud cover. We use data of automatic weather stations (AWS) located in four major Antarctic climate zones: the coastal ice shelf, the coastal and interior katabatic wind zone and the interior

  3. Stratospheric BrONO2 observed by MIPAS

    Directory of Open Access Journals (Sweden)

    H. Fischer

    2009-03-01

    Full Text Available The first measurements of stratospheric bromine nitrate (BrONO2 are reported. Bromine nitrate has been clearly identified in atmospheric infrared emission spectra recorded with the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS aboard the European Envisat satellite, and stratospheric concentration profiles have been determined for different conditions (day and night, different latitudes. The BrONO2 concentrations show strong day/night variations, with much lower concentrations during the day. Maximum volume mixing ratios observed during night are 20 to 25 pptv. The observed concentration profiles are in agreement with estimations from photochemical models and show that the current understanding of stratospheric bromine chemistry is generally correct.

  4. Efficient transport of tropospheric aerosol into the stratosphere via the Asian summer monsoon anticyclone

    Science.gov (United States)

    Yu, Pengfei; Rosenlof, Karen H.; Liu, Shang; Telg, Hagen; Thornberry, Troy D.; Rollins, Andrew W.; Portmann, Robert W.; Bai, Zhixuan; Ray, Eric A.; Duan, Yunjun; Pan, Laura L.; Toon, Owen B.; Bian, Jianchun; Gao, Ru-Shan

    2017-07-01

    An enhanced aerosol layer near the tropopause over Asia during the June-September period of the Asian summer monsoon (ASM) was recently identified using satellite observations. Its sources and climate impact are presently not well-characterized. To improve understanding of this phenomenon, we made in situ aerosol measurements during summer 2015 from Kunming, China, then followed with a modeling study to assess the global significance. The in situ measurements revealed a robust enhancement in aerosol concentration that extended up to 2 km above the tropopause. A climate model simulation demonstrates that the abundant anthropogenic aerosol precursor emissions from Asia coupled with rapid vertical transport associated with monsoon convection leads to significant particle formation in the upper troposphere within the ASM anticyclone. These particles subsequently spread throughout the entire Northern Hemispheric (NH) lower stratosphere and contribute significantly (˜15%) to the NH stratospheric column aerosol surface area on an annual basis. This contribution is comparable to that from the sum of small volcanic eruptions in the period between 2000 and 2015. Although the ASM contribution is smaller than that from tropical upwelling (˜35%), we find that this region is about three times as efficient per unit area and time in populating the NH stratosphere with aerosol. With a substantial amount of organic and sulfur emissions in Asia, the ASM anticyclone serves as an efficient smokestack venting aerosols to the upper troposphere and lower stratosphere. As economic growth continues in Asia, the relative importance of Asian emissions to stratospheric aerosol is likely to increase.

  5. Cloud and surface textural features in polar regions

    Science.gov (United States)

    Welch, Ronald M.; Kuo, Kwo-Sen; Sengupta, Sailes K.

    1990-01-01

    The study examines the textural signatures of clouds, ice-covered mountains, solid and broken sea ice and floes, and open water. The textural features are computed from sum and difference histogram and gray-level difference vector statistics defined at various pixel displacement distances derived from Landsat multispectral scanner data. Polar cloudiness, snow-covered mountainous regions, solid sea ice, glaciers, and open water have distinguishable texture features. This suggests that textural measures can be successfully applied to the detection of clouds over snow-covered mountains, an ability of considerable importance for the modeling of snow-melt runoff. However, broken stratocumulus cloud decks and thin cirrus over broken sea ice remain difficult to distinguish texturally. It is concluded that even with high spatial resolution imagery, it may not be possible to distinguish broken stratocumulus and thin clouds from sea ice in the marginal ice zone using the visible channel textural features alone.

  6. A boundary-layer cloud study using Southern Great Plains Cloud and radiation testbed (CART) data

    Energy Technology Data Exchange (ETDEWEB)

    Albrecht, B.; Mace, G.; Dong, X.; Syrett, W. [Pennsylvania State Univ., University Park, PA (United States)] [and others

    1996-04-01

    Boundary layer clouds-stratus and fairweather cumulus - are closely coupled involves the radiative impact of the clouds on the surface energy budget and the strong dependence of cloud formation and maintenance on the turbulent fluxes of heat and moisture in the boundary layer. The continuous data collection at the Southern Great Plains (SGP) Cloud and Radiation Testbed (CART) site provides a unique opportunity to study components of the coupling processes associated with boundary layer clouds and to provide descriptions of cloud and boundary layer structure that can be used to test parameterizations used in climate models. But before the CART data can be used for process studies and parameterization testing, it is necessary to evaluate and validate data and to develop techniques for effectively combining the data to provide meaningful descriptions of cloud and boundary layer characteristics. In this study we use measurements made during an intensive observing period we consider a case where low-level stratus were observed at the site for about 18 hours. This case is being used to examine the temporal evolution of cloud base, cloud top, cloud liquid water content, surface radiative fluxes, and boundary layer structure. A method for inferring cloud microphysics from these parameters is currently being evaluated.

  7. Clouds and snowmelt on the north slope of Alaska

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, T.; Stamnes, K.; Bowling, S.A. [Univ. of Alaska, Fairbanks, AK (United States)

    1996-04-01

    Clouds have a large effect on the radiation field. Consequently, possible changes in cloud properties may have a very substantial impact on climate. Of all natural surfaces, seasonal snow cover has the highest surface albedo, which is one of the most important components of the climatic system. Interactions between clouds and seasonal snow cover are expected to have a significant effect on climate and its change at high latitudes. The purpose of this paper is to investigate the sensitivity of the surface cloud-radiative forcing during the period of snowmelt at high latitudes. The primary variables investigated are cloud liquid path (LWP) and droplet equivalent radius (r{sub e}). We will also examine the sensitivity of the surface radiative fluxes to cloud base height and cloud base temperature.

  8. A risk-based framework for assessing the effectiveness of stratospheric aerosol geoengineering.

    Directory of Open Access Journals (Sweden)

    Angus J Ferraro

    Full Text Available Geoengineering by stratospheric aerosol injection has been proposed as a policy response to warming from human emissions of greenhouse gases, but it may produce unequal regional impacts. We present a simple, intuitive risk-based framework for classifying these impacts according to whether geoengineering increases or decreases the risk of substantial climate change, with further classification by the level of existing risk from climate change from increasing carbon dioxide concentrations. This framework is applied to two climate model simulations of geoengineering counterbalancing the surface warming produced by a quadrupling of carbon dioxide concentrations, with one using a layer of sulphate aerosol in the lower stratosphere, and the other a reduction in total solar irradiance. The solar dimming model simulation shows less regional inequality of impacts compared with the aerosol geoengineering simulation. In the solar dimming simulation, 10% of the Earth's surface area, containing 10% of its population and 11% of its gross domestic product, experiences greater risk of substantial precipitation changes under geoengineering than under enhanced carbon dioxide concentrations. In the aerosol geoengineering simulation the increased risk of substantial precipitation change is experienced by 42% of Earth's surface area, containing 36% of its population and 60% of its gross domestic product.

  9. A Risk-Based Framework for Assessing the Effectiveness of Stratospheric Aerosol Geoengineering

    Science.gov (United States)

    Ferraro, Angus J.; Charlton-Perez, Andrew J.; Highwood, Eleanor J.

    2014-01-01

    Geoengineering by stratospheric aerosol injection has been proposed as a policy response to warming from human emissions of greenhouse gases, but it may produce unequal regional impacts. We present a simple, intuitive risk-based framework for classifying these impacts according to whether geoengineering increases or decreases the risk of substantial climate change, with further classification by the level of existing risk from climate change from increasing carbon dioxide concentrations. This framework is applied to two climate model simulations of geoengineering counterbalancing the surface warming produced by a quadrupling of carbon dioxide concentrations, with one using a layer of sulphate aerosol in the lower stratosphere, and the other a reduction in total solar irradiance. The solar dimming model simulation shows less regional inequality of impacts compared with the aerosol geoengineering simulation. In the solar dimming simulation, 10% of the Earth's surface area, containing 10% of its population and 11% of its gross domestic product, experiences greater risk of substantial precipitation changes under geoengineering than under enhanced carbon dioxide concentrations. In the aerosol geoengineering simulation the increased risk of substantial precipitation change is experienced by 42% of Earth's surface area, containing 36% of its population and 60% of its gross domestic product. PMID:24533155

  10. CERN: Antiprotons probe the nuclear stratosphere

    Energy Technology Data Exchange (ETDEWEB)

    Anon.

    1995-06-15

    The outer periphery of heavy stable nuclei is notoriously difficult to study experimentally. While the well understood electromagnetic interaction between electrons (or muons) and protons has given the nuclear charge (or proton) distribution with high precision for almost all stable nuclei, neutron distribution studies are much less precise. This is especially true for large nuclear distances, where the nuclear density is small. A few previous experiments probing the nuclear ''stratosphere'' suggested that far from the centre of the nucleus (of the order of 2 nuclear radii) this stratosphere may be composed predominantly of neutrons. At the end of the sixties the term ''neutron halo'' was introduced to describe this phenomenon, but experimental evidence was scarce or even controversial, and remained so for almost a quarter of a century. Recently, the Warsaw/Munich/Berlin collaboration working within the PS203 experiment at CERN's LEAR low energy antiproton ring, proposed a new method to study the nuclear periphery using stopped antiprotons. The halo now looks firmer. A 200 MeV/c beam of antiprotons was slowed down by interactions with atomic electrons. When antiproton kinetic energy drops well below 1 keV, the particles are captured in the outermost orbits of ''exotic atoms'', where the antiprotons take the place of the usual orbital electrons. With the lower orbits in this antiprotonic atom empty, the antiproton drops toward the nuclear surface, first emitting Auger electrons and later predominantly antiprotonic X-rays. Due to the strong interaction between antiprotons and nucleons, the antiproton succumbs to annihilation with a nucleon in the rarified nuclear stratosphere, far above the innermost Bohr orbit of the atom. The annihilation probability in heavy nuclei is maximal where the nuclear density is about 3% of its central value and extends to densities many orders of magnitude smaller. Antiproton annihilation on a proton or on a neutron at the nuclear

  11. Intercomparison of model simulations of mixed-phase clouds observed during the ARM Mixed-Phase Arctic Cloud Experiment. Part II: Multi-layered cloud

    Energy Technology Data Exchange (ETDEWEB)

    Morrison, H; McCoy, R B; Klein, S A; Xie, S; Luo, Y; Avramov, A; Chen, M; Cole, J; Falk, M; Foster, M; Genio, A D; Harrington, J; Hoose, C; Khairoutdinov, M; Larson, V; Liu, X; McFarquhar, G; Poellot, M; Shipway, B; Shupe, M; Sud, Y; Turner, D; Veron, D; Walker, G; Wang, Z; Wolf, A; Xu, K; Yang, F; Zhang, G

    2008-02-27

    Results are presented from an intercomparison of single-column and cloud-resolving model simulations of a deep, multi-layered, mixed-phase cloud system observed during the ARM Mixed-Phase Arctic Cloud Experiment. This cloud system was associated with strong surface turbulent sensible and latent heat fluxes as cold air flowed over the open Arctic Ocean, combined with a low pressure system that supplied moisture at mid-level. The simulations, performed by 13 single-column and 4 cloud-resolving models, generally overestimate the liquid water path and strongly underestimate the ice water path, although there is a large spread among the models. This finding is in contrast with results for the single-layer, low-level mixed-phase stratocumulus case in Part I of this study, as well as previous studies of shallow mixed-phase Arctic clouds, that showed an underprediction of liquid water path. The overestimate of liquid water path and underestimate of ice water path occur primarily when deeper mixed-phase clouds extending into the mid-troposphere were observed. These results suggest important differences in the ability of models to simulate Arctic mixed-phase clouds that are deep and multi-layered versus shallow and single-layered. In general, models with a more sophisticated, two-moment treatment of the cloud microphysics produce a somewhat smaller liquid water path that is closer to observations. The cloud-resolving models tend to produce a larger cloud fraction than the single-column models. The liquid water path and especially the cloud fraction have a large impact on the cloud radiative forcing at the surface, which is dominated by the longwave flux for this case.

  12. Improving Estimates of Cloud Radiative Forcing over Greenland

    Science.gov (United States)

    Wang, W.; Zender, C. S.

    2014-12-01

    Multiple driving mechanisms conspire to increase melt extent and extreme melt events frequency in the Arctic: changing heat transport, shortwave radiation (SW), and longwave radiation (LW). Cloud Radiative Forcing (CRF) of Greenland's surface is amplified by a dry atmosphere and by albedo feedback, making its contribution to surface melt even more variable in time and space. Unfortunately accurate cloud observations and thus CRF estimates are hindered by Greenland's remoteness, harsh conditions, and low contrast between surface and cloud reflectance. In this study, cloud observations from satellites and reanalyses are ingested into and evaluated within a column radiative transfer model. An improved CRF dataset is obtained by correcting systematic discrepancies derived from sensitivity experiments. First, we compare the surface radiation budgets from the Column Radiation Model (CRM) driven by different cloud datasets, with surface observations from Greenland Climate Network (GC-Net). In clear skies, CRM-estimated surface radiation driven by water vapor profiles from both AIRS and MODIS during May-Sept 2010-2012 are similar, stable, and reliable. For example, although AIRS water vapor path exceeds MODIS by 1.4 kg/m2 on a daily average, the overall absolute difference in downwelling SW is CRM estimates are within 20 W/m2 range of GC-Net downwelling SW. After calibrating CRM in clear skies, the remaining differences between CRM and observed surface radiation are primarily attributable to differences in cloud observations. We estimate CRF using cloud products from MODIS and from MERRA. The SW radiative forcing of thin clouds is mainly controlled by cloud water path (CWP). As CWP increases from near 0 to 200 g/m2, the net surface SW drops from over 100 W/m2 to 30 W/m2 almost linearly, beyond which it becomes relatively insensitive to CWP. The LW is dominated by cloud height. For clouds at all altitudes, the lower the clouds, the greater the LW forcing. By applying

  13. Forecast, observation and modelling of a deep stratospheric intrusion event over Europe

    Directory of Open Access Journals (Sweden)

    P. Zanis

    2003-01-01

    Full Text Available A wide range of measurements was carried out in central and southeastern Europe within the framework of the EU project STACCATO (Influence of Stratosphere-Troposphere Exchange in a Changing Climate on Atmospheric Transport and Oxidation Capacity with the principle goal to create a comprehensive data set on stratospheric air intrusions into the troposphere along a rather frequently observed pathway over central Europe from the North Sea to the Mediterranean Sea. The measurements were based on predictions by suitable quasi-operational trajectory calculations using ECMWF forecast data. A predicted deep Stratosphere to Troposphere Transport (STT event, encountered during the STACCATO period on 20-21 June 2001, was followed by the measurements network almost from its inception. Observations provide evidence that the intrusion affected large parts of central and southeastern Europe. Especially, the ozone lidar observations on 20-21 June 2001 at Garmisch-Partenkirchen, Germany captured the evolution of two marked tongues of high ozone with the first one descending to nearly 2 km, thus providing an excellent data set for model intercomparisons and validation. In addition, for the first time to our knowledge concurrent surface measurements of the cosmogenic radionuclides 10Be and 7Be and their ratio 10Be/7Be are presented together as stratospheric tracers in a case study of a stratospheric intrusion. The ozone tracer columns calculated with the FLEXPART model were found to be in good agreement with water vapour satellite images, capturing the evolution of the observed dry streamers of stratospheric origin. Furthermore, the time-height cross section of ozone tracer simulated with FLEXPART over Garmisch-Partenkirchen captures many details of the evolution of the two observed high-ozone filaments measured with the IFU lidar, thus demonstrating the considerable progress in model simulations. Finally, the modelled ozone (operationally available since October

  14. A stochastic model with a low-frequency amplification feedback for the stratospheric northern annular mode

    Science.gov (United States)

    Yu, Yueyue; Cai, Ming; Ren, Rongcai

    2017-08-01

    We consider three indices to measure the polar stratospheric mass and stratospheric meridional mass circulation variability: anomalies of (1) total mass in the polar stratospheric cap (60-90°N, above the isentropic surface 400 K, PSM), (2) total adiabatic mass transport across 60°N into the polar stratosphere cap (AMT), (3) and total diabetic mass transport across 400 K from the polar stratosphere into the troposphere below (DMT). It is confirmed that the negative stratospheric Northern Annular Mode (NAM) and PSM indices have a nearly indistinguishable temporal evolution and a similar red-noise-like spectrum with a de-correlation timescale of 4 weeks. This enables us to examine the low-frequency nature of the NAM in the framework of mass circulation, namely, d/{dt}{PSM}={AMT} - {DMT} . The DMT index tends to be positively correlated with the PSM with a red-noise-like spectrum, representing slow radiative cooling processes giving rise to a de-correlation timescale of 3-4 weeks. The AMT is nearly perfectly correlated with the day-to-day tendency of PSM, reflecting a robust quasi 90° out-of-phase relation between the AMT and PSM at all frequency bands. Variations of vertically westward tilting of planetary waves contribute mainly to the high-frequency portion of AMT. It is the wave amplitude's slow vacillation that plays the leading role in the quasi 90° out-of-phase relation between the AMT and PSM. Based on this, we put forward a linear stochastic model with a low-frequency amplification feedback from low-frequency amplitude vacillations of planetary waves to explain the amplified low-frequency response of PSM/NAM to a stochastic forcing from the westward tilting variability.

  15. THERMAL AND CHEMICAL STRUCTURE VARIATIONS IN TITAN'S STRATOSPHERE DURING THE CASSINI MISSION

    Energy Technology Data Exchange (ETDEWEB)

    Bampasidis, Georgios; Coustenis, A.; Vinatier, S. [Laboratoire d' Etudes Spatiales et d' Instrumentation en Astrophysique (LESIA), Observatoire de Paris, CNRS, UPMC Univ. Paris 06, Univ. Paris-Diderot, 5, place Jules Janssen, F-92195 Meudon Cedex (France); Achterberg, R. K. [Department of Astronomy, University of Maryland, College Park, MD 20742 (United States); Lavvas, P. [GSMA, Universite Reims Champagne-Ardenne, F-51687 Reims Cedex 2 (France); Nixon, C. A.; Jennings, D. E.; Flasar, F. M.; Carlson, R. C.; Romani, P. N.; Guandique, E. A. [Goddard Space Flight Center, Greenbelt, MD 20771 (United States); Teanby, N. A. [School of Earth Sciences, University of Bristol, Bristol BS8 1RJ (United Kingdom); Moussas, X.; Preka-Papadema, P.; Stamogiorgos, S., E-mail: gbabasid@phys.uoa.gr [Faculty of Physics, National and Kapodistrian University of Athens, Panepistimioupolis, GR 15783 Zographos, Athens (Greece)

    2012-12-01

    We have developed a line-by-line Atmospheric Radiative Transfer for Titan code that includes the most recent laboratory spectroscopic data and haze descriptions relative to Titan's stratosphere. We use this code to model Cassini Composite Infrared Spectrometer data taken during the numerous Titan flybys from 2006 to 2012 at surface-intercepting geometry in the 600-1500 cm{sup -1} range for latitudes from 50 Degree-Sign S to 50 Degree-Sign N. We report variations in temperature and chemical composition in the stratosphere during the Cassini mission, before and after the Northern Spring Equinox (NSE). We find indication for a weakening of the temperature gradient with warming of the stratosphere and cooling of the lower mesosphere. In addition, we infer precise concentrations for the trace gases and their main isotopologues and find that the chemical composition in Titan's stratosphere varies significantly with latitude during the 6 years investigated here, with increased mixing ratios toward the northern latitudes. In particular, we monitor and quantify the amplitude of a maximum enhancement of several gases observed at northern latitudes up to 50 Degree-Sign N around mid-2009, at the time of the NSE. We find that this rise is followed by a rapid decrease in chemical inventory in 2010 probably due to a weakening north polar vortex with reduced lateral mixing across the vortex boundary.

  16. A daytime climatological distribution of high opaque ice cloud classes over the Indian summer monsoon region observed from 25-year AVHRR data

    Directory of Open Access Journals (Sweden)

    A. Devasthale

    2009-06-01

    Full Text Available A daytime climatological spatio-temporal distribution of high opaque ice cloud (HOIC classes over the Indian subcontinent (0–40° N, 60° E–100° E is presented using 25-year data from the Advanced Very High Resolution Radiometers (AVHRRs for the summer monsoon months. The HOICs are important for regional radiative balance, precipitation and troposphere-stratosphere exchange. In this study, HOICs are sub-divided into three classes based on their cloud top brightness temperatures (BT. Class I represents very deep convection (BT<220 K. Class II represents deep convection (220 K<=BT<233 K and Class III background convection (233 K<=BT<253 K. Apart from presenting finest spatial resolution (0.1×0.1 degrees and long-term climatology of such cloud classes from AVHRRs to date, this study for the first time illustrates on (1 how these three cloud classes are climatologically distributed during monsoon months, and (2 how their distribution changes during active and break monsoon conditions. It is also investigated that how many deep convective clouds reach the tropopause layer during individual monsoon months. It is seen that Class I and Class II clouds dominate the Indian subcontinent during monsoon. The movement of monsoon over continent is very well reflected in these cloud classes. During monsoon breaks strong suppression of convective activity is observed over the Arabian Sea and the western coast of India. On the other hand, the presence of such convective activity is crucial for active monsoon conditions and all-India rainfall. It is found that a significant fraction of HOICs (3–5% reach the tropopause layer over the Bay of Bengal during June and over the north and northeast India during July and August. Many cases are observed when clouds penetrate the tropopause layer and reach the lower stratosphere. Such cases mostly occur during June compared to the other months.

  17. Evaluation of Passive Multilayer Cloud Detection Using Preliminary CloudSat and CALIPSO Cloud Profiles

    Science.gov (United States)

    Minnis, P.; Sun-Mack, S.; Chang, F.; Huang, J.; Nguyen, L.; Ayers, J. K.; Spangenberg, D. A.; Yi, Y.; Trepte, C. R.

    2006-12-01

    During the last few years, several algorithms have been developed to detect and retrieve multilayered clouds using passive satellite data. Assessing these techniques has been difficult due to the need for active sensors such as cloud radars and lidars that can "see" through different layers of clouds. Such sensors have been available only at a few surface sites and on aircraft during field programs. With the launch of the CALIPSO and CloudSat satellites on April 28, 2006, it is now possible to observe multilayered systems all over the globe using collocated cloud radar and lidar data. As part of the A- Train, these new active sensors are also matched in time ad space with passive measurements from the Aqua Moderate Resolution Imaging Spectroradiometer (MODIS) and Advanced Microwave Scanning Radiometer - EOS (AMSR-E). The Clouds and the Earth's Radiant Energy System (CERES) has been developing and testing algorithms to detect ice-over-water overlapping cloud systems and to retrieve the cloud liquid path (LWP) and ice water path (IWP) for those systems. One technique uses a combination of the CERES cloud retrieval algorithm applied to MODIS data and a microwave retrieval method applied to AMSR-E data. The combination of a CO2-slicing cloud retireval technique with the CERES algorithms applied to MODIS data (Chang et al., 2005) is used to detect and analyze such overlapped systems that contain thin ice clouds. A third technique uses brightness temperature differences and the CERES algorithms to detect similar overlapped methods. This paper uses preliminary CloudSat and CALIPSO data to begin a global scale assessment of these different methods. The long-term goals are to assess and refine the algorithms to aid the development of an optimal combination of the techniques to better monitor ice 9and liquid water clouds in overlapped conditions.

  18. Aerosol-associated changes in tropical stratospheric ozone following the eruption of Mount Pinatubo

    Science.gov (United States)

    Grant, William B.; Browell, Edward V.; Fishman, Jack; Brackett, Vincent G.; Veiga, Robert E.; Nganga, Dominique; Minga, A.; Cros, Bernard; Butler, Carolyn F.; Fenn, Marta A.

    1994-01-01

    The large amount of sulfuric acid aerosol formed in the stratosphere by conversion of sulfur dioxide emitted by the eruption of Mount Pinatubo (15.14 deg N, 120.35 deg E) in the Philippines around June 15, 1991, has had a pronounced effect on lower stratospheric ozone in the tropics. Measurements of stratospheric ozone in the tropics using electrochemical concentration cell (ECC) sondes before and after the eruption and the airborne UV differential absorption lidar (DIAL) system after the eruption are compared with Stratospheric Aerosol and Gas Experiment II (SAGE II) measurements from several years before the eruption and ECC sonde measurements from the year prior to the eruption to determine the resulting changes. Ozone decreases of up to 33 % compared with SAGE II climatological values were found to be directly correlated with altitude regions of enhanced aerosol loading in the 16- to 28-km range. A maximum partial-column decrease of 29 +/- Dobson units (DU) was found over the 16- to 28-km range in September 1991 along with small increases (to 5.9 +/- 2 DU) from 28 to 31.5 km. A large decrease of ozone was also found at 4 deg to 8 deg S from May to August 1992, with a maximum decrease of 33 +/- 7 DU found above Brazzaville in July. Aerosol data form the visible channel of the advanced very high resolution radiometer (AVHRR) and the visible wavelength of the UV DIAL system were used to examine the relationship between aerosol (surface area) densities and ozone changes. The tropical stratospheric ozone changes we observed in 1991 and 1992 are likely be explained by a combination of dynamical (vertical transport) perturbations, radiative perturbations on ozone photochemistry, and heterogeneous chemistry.

  19. Is there any chlorine monoxide in the stratosphere?

    Science.gov (United States)

    Mumma, M. J.; Rogers, J. D.; Kostiuk, T.; Deming, D.; Hillman, J. J.; Zipoy, D.

    1983-01-01

    A ground-based search for stratospheric 35-ClO was carried out using an infrared heterodyne spectrometer in the solar absorption mode. Lines due to stratospheric HNO3 and tropospheric OCS were detected at about 0.2 percent absorptance levels, but the expected 0.1 percent lines of ClO in this same region were not seen. We find that stratospheric ClO is at least a factor of seven less abundant than is indicated by in situ measurements, and we set an upper limit of 2.3 x 10 to the 13th molecules/sq cm at the 95 percent confidence level for the integrated vertical column density of ClO. Our results imply that the release of chlorofluorocarbons may be significantly less important for the destruction of stratospheric ozone (O3) than is currently thought. Previously announced in STAR as N83-27518

  20. Ocean Heat Uptake Slows 21st Century Surface Warming Driven by Extratropical Cloud Feedbacks

    Science.gov (United States)

    Frey, W.; Maroon, E.; Pendergrass, A. G.; Kay, J. E.

    2017-12-01

    Equilibrium climate sensitivity (ECS), the warming in response to instantaneously doubled CO2, has long been used to compare climate models. In many models, ECS is well correlated with warming produced by transient forcing experiments. Modifications to cloud phase at high latitudes in a state-of-the-art climate model, the Community Earth System Model (CESM), produce a large increase in ECS (1.5 K) via extratropical cloud feedbacks. However, only a small surface warming increase occurs in a realistic 21st century simulation including a full-depth dynamic ocean and the "business as usual" RCP8.5 emissions scenario. In fact, the increase in surface warming is only barely above the internal variability-generated range in the CESM Large Ensemble. The small change in 21st century warming is attributed to subpolar ocean heat uptake in both hemispheres. In the Southern Ocean, the mean-state circulation takes up heat while in the North Atlantic a slowdown in circulation acts as a feedback to slow surface warming. These results show the importance of subpolar ocean heat uptake in controlling the pace of warming and demonstrate that ECS cannot be used to reliably infer transient warming when it is driven by extratropical feedbacks.

  1. Early Evaluation of the VIIRS Calibration, Cloud Mask and Surface Reflectance Earth Data Records

    Science.gov (United States)

    Vermote, Eric; Justice, Chris; Csiszar, Ivan

    2014-01-01

    Surface reflectance is one of the key products fromVIIRS and as withMODIS, is used in developing several higherorder land products. The VIIRS Surface Reflectance (SR) Intermediate Product (IP) is based on the heritageMODIS Collection 5 product (Vermote, El Saleous, & Justice, 2002). The quality and character of surface reflectance depend on the accuracy of the VIIRS Cloud Mask (VCM), the aerosol algorithms and the adequate calibration of the sensor. The focus of this paper is the early evaluation of the VIIRS SR product in the context of the maturity of the operational processing system, the Interface Data Processing System (IDPS). After a brief introduction, the paper presents the calibration performance and the role of the surface reflectance in calibration monitoring. The analysis of the performance of the cloud mask with a focus on vegetation monitoring (no snow conditions) shows typical problems over bright surfaces and high elevation sites. Also discussed is the performance of the aerosol input used in the atmospheric correction and in particular the artifacts generated by the use of the Navy Aerosol Analysis and Prediction System. Early quantitative results of the performance of the SR product over the AERONET sites showthatwith the fewadjustments recommended, the accuracy iswithin the threshold specifications. The analysis of the adequacy of the SR product (Land PEATE adjusted version) in applications of societal benefits is then presented. We conclude with a set of recommendations to ensure consistency and continuity of the JPSS mission with the MODIS Land Climate Data Record.

  2. Observation of near-infrared surface brightness of the large Magellanic cloud

    International Nuclear Information System (INIS)

    Hayakawa, Satio; Koizumi, Yutaka; Matsumoto, Toshio; Murakami, Hiroshi; Uyama, Kiichiro.

    1981-01-01

    The near-infrared surface brightness of the large Magellanic cloud was observed by an infrared telescope carried by a balloon. The balloon flight was made at Australian Balloon Launching Station. The brightness distribution of 2.4 Mu m radiation was obtained. A part of Bar was bright, and the expansion of the contour at the east end of Bar corresponded to the 30 Dor region. Many near-infrared sources distribute in this region. Discussions on the color and brightness of the center of Bar and the 30 Dor region are presented. (Kato, T.)

  3. Sources and sinks of stratospheric water vapor

    International Nuclear Information System (INIS)

    Ellsaesser, H.W.

    1979-11-01

    A tutorial review of the understanding of stratospheric H 2 O and the processes controlling it is presented. Paradoxes posed by currently available observational data are cited and suggestions made as to how they might be resolved. Such resolution appears to require: that the bulk of our current data provides unrepresentative and misleading vertical and latitudinal H 2 O gradients immediately downstream from the tropical tropopause; and, that there exists within the troposphere a mechanism different from or in addition to the tropical tropopause cold trap for drying air to the mixing ratios found in the lower stratosphere. Satisfaction of these requirements will reconcile much heretofore puzzling observational data and will obviate the necessity for a stratospheric sink for H 2 O

  4. Stratospheric ozone, ultraviolet radiation and climate change

    International Nuclear Information System (INIS)

    Boucher, O.

    2008-01-01

    It is well known that an overexposure to ultraviolet radiation is associated with a number of health risks such as an increased risk of cataracts and skin cancers. At a time when climate change is often blamed for all our environmental problems, what is the latest news about the stratospheric ozone layer and other factors controlling ultraviolet radiation at the surface of the Earth? Will the expected changes in the chemical composition of the atmosphere and changes in our climate increase or decrease the risk for skin cancer? This article investigates the role of the various factors influencing ultraviolet radiation and presents the latest knowledge on the subject. (author)

  5. Connection of stratospheric QBO with global atmospheric general circulation and tropical SST. Part I: methodology and composite life cycle

    Energy Technology Data Exchange (ETDEWEB)

    Huang, Bohua; Kinter, James L. [George Mason University, Department of Atmospheric, Oceanic, and Earth Sciences, College of Science, Fairfax, VA (United States); Center for Ocean-Land-Atmosphere Studies, Calverton, MD (United States); Hu, Zeng-Zhen [Center for Ocean-Land-Atmosphere Studies, Calverton, MD (United States); Climate Prediction Center (suite 605), NCEP/NWS/NOAA, Camp Springs, MD (United States); Wu, Zhaohua [Florida State University, Department of Earth, Ocean, and Atmospheric Science, and Center for Ocean-Atmospheric Prediction Studies, Tallahassee, FL (United States); Kumar, Arun [Climate Prediction Center (suite 605), NCEP/NWS/NOAA, Camp Springs, MD (United States)

    2012-01-15

    The stratospheric quasi-biennial oscillation (QBO) and its association with the interannual variability in the stratosphere and troposphere, as well as in tropical sea surface temperature anomalies (SSTA), are examined in the context of a QBO life cycle. The analysis is based on the ERA40 and NCEP/NCAR reanalyses, radiosonde observations at Singapore, and other observation-based datasets. Both reanalyses reproduce the QBO life cycle and its associated variability in the stratosphere reasonably well, except that some long-term changes are detected only in the NCEP/NCAR reanalysis. In order to separate QBO from variability on other time scales and to eliminate the long-term changes, a scale separation technique [Ensemble Empirical Mode Decomposition (EEMD)] is applied to the raw data. The QBO component of zonal wind anomalies at 30 hPa, extracted using the EEMD method, is defined as a QBO index. Using this index, the QBO life cycle composites of stratosphere and troposphere variables, as well as SSTA, are constructed and examined. The composite features in the stratosphere are generally consistent with previous investigations. The correlations between the QBO and tropical Pacific SSTA depend on the phase in a QBO life cycle. On average, cold (warm) SSTA peaks about half a year after the maximum westerlies (easterlies) at 30 hPa. The connection of the QBO with the troposphere seems to be associated with the differences of temperature anomalies between the stratosphere and troposphere. While the anomalies in the stratosphere propagate downward systematically, some anomalies in the troposphere develop and expand vertically. Therefore, it is possible that the temperature difference between the troposphere and stratosphere may alter the atmospheric stability and tropical deep convection, which modulates the Walker circulation and SSTA in the equatorial Pacific Ocean. (orig.)

  6. Connection of stratospheric QBO with global atmospheric general circulation and tropical SST. Part I: methodology and composite life cycle

    Science.gov (United States)

    Huang, Bohua; Hu, Zeng-Zhen; Kinter, James L.; Wu, Zhaohua; Kumar, Arun

    2012-01-01

    The stratospheric quasi-biennial oscillation (QBO) and its association with the interannual variability in the stratosphere and troposphere, as well as in tropical sea surface temperature anomalies (SSTA), are examined in the context of a QBO life cycle. The analysis is based on the ERA40 and NCEP/NCAR reanalyses, radiosonde observations at Singapore, and other observation-based datasets. Both reanalyses reproduce the QBO life cycle and its associated variability in the stratosphere reasonably well, except that some long-term changes are detected only in the NCEP/NCAR reanalysis. In order to separate QBO from variability on other time scales and to eliminate the long-term changes, a scale separation technique [Ensemble Empirical Mode Decomposition (EEMD)] is applied to the raw data. The QBO component of zonal wind anomalies at 30 hPa, extracted using the EEMD method, is defined as a QBO index. Using this index, the QBO life cycle composites of stratosphere and troposphere variables, as well as SSTA, are constructed and examined. The composite features in the stratosphere are generally consistent with previous investigations. The correlations between the QBO and tropical Pacific SSTA depend on the phase in a QBO life cycle. On average, cold (warm) SSTA peaks about half a year after the maximum westerlies (easterlies) at 30 hPa. The connection of the QBO with the troposphere seems to be associated with the differences of temperature anomalies between the stratosphere and troposphere. While the anomalies in the stratosphere propagate downward systematically, some anomalies in the troposphere develop and expand vertically. Therefore, it is possible that the temperature difference between the troposphere and stratosphere may alter the atmospheric stability and tropical deep convection, which modulates the Walker circulation and SSTA in the equatorial Pacific Ocean.

  7. Atmospheric diffusion of large clouds

    Energy Technology Data Exchange (ETDEWEB)

    Crawford, T. V. [Univ. of California, Lawrence Radiation Lab., Livermore, California (United States)

    1967-07-01

    Clouds of pollutants travel within a coordinate system that is fixed to the earth's surface, and they diffuse and grow within a coordinate system fixed to the cloud's center. This paper discusses an approach to predicting the cloud's properties, within the latter coordinate system, on space scales of a few hundred meters to a few hundred kilometers and for time periods of a few days. A numerical cloud diffusion model is presented which starts with a cloud placed arbitrarily within the troposphere. Similarity theories of atmospheric turbulence are used to predict the horizontal diffusivity as a function of initial cloud size, turbulent atmospheric dissipation, and time. Vertical diffusivity is input as a function of time and height. Therefore, diurnal variations of turbulent diffusion in the boundary layer and effects of temperature inversions, etc. can be modeled. Nondiffusive cloud depletion mechanisms, such as dry deposition, washout, and radioactive decay, are also a part of this numerical model. An effluent cloud, produced by a reactor run at the Nuclear Rocket Development Station, Nevada, is discussed in this paper. Measurements on this cloud, for a period of two days, are compared to calculations with the above numerical cloud diffusion model. In general, there is agreement. within a factor of two, for airborne concentrations, cloud horizontal area, surface air concentrations, and dry deposition as airborne concentration decreased by seven orders of magnitude during the two-day period. (author)

  8. An Atmospheric Tape Recorder: The Imprint of Tropical Tropopause Temperatures on Stratospheric Water Vapor

    Science.gov (United States)

    Mote, Philip W.; Rosenlof, Karen H.; McIntyre, Michael E.; Carr, Ewan S.; Gille, John C.; Holton, James R.; Kinnersley, Jonathan S.; Pumphrey, Hugh C.; Russell, James M., III; Waters, Joe W.

    1996-01-01

    We describe observations of tropical stratospheric water vapor q that show clear evidence of large-scale upward advection of the signal from annual fluctuations in the effective 'entry mixing ratio' q(sub E) of air entering the tropical stratosphere. In other words, air is 'marked,' on emergence above the highest cloud tops, like a signal recorded on an upward moving magnetic tape. We define q(sub E) as the mean water vapor mixing ratio, at the tropical tropopause, of air that will subsequently rise and enter the stratospheric 'overworld' at about 400 K. The observations show a systematic phase lag, increasing with altitude, between the annual cycle in q(sub E) and the annual cycle in q at higher altitudes. The observed phase lag agrees with the phase lag calculated assuming advection by the transformed Eulerian-mean vertical velocity of a q(sub E) crudely estimated from 100-hPa temperatures, which we use as a convenient proxy for tropopause temperatures. The phase agreement confirms the overall robustness of the calculation and strongly supports the tape recorder hypothesis. Establishing a quantitative link between q(sub E) and observed tropopause temperatures, however, proves difficult because the process of marking the tape depends subtly on both small- and large-scale processes. The tape speed, or large-scale upward advection speed, has a substantial annual variation and a smaller variation due to the quasi-biennial oscillation, which delays or accelerates the arrival of the signal by a month or two in the middle stratosphere. As the tape moves upward, the signal is attenuated with an e-folding time of about 7 to 9 months between 100 and 50 hPa and about 15 to 18 months between 50 and 20 hPa, constraining possible orders of magnitude both of vertical diffusion K(sub z) and of rates of mixing in from the extratropics. For instance, if there were no mixing in, then K(sub z) would be in the range 0.03-0.09 m(exp 2)/s; this is an upper bound on K(sub z).

  9. Cirrus cloud mimic surfaces in the laboratory: organic acids, bases and NOx heterogeneous reactions

    Science.gov (United States)

    Sodeau, J.; Oriordan, B.

    2003-04-01

    CIRRUS CLOUD MIMIC SURFACES IN THE LABORATORY:ORGANIC ACIDS, BASES AND NOX HETEROGENEOUS REACTIONS. B. ORiordan, J. Sodeau Department of Chemistry and Environment Research Institute, University College Cork, Ireland j.sodeau@ucc.ie /Fax: +353-21-4902680 There are a variety of biogenic and anthropogenic sources for the simple carboxylic acids to be found in the troposphere giving rise to levels as high as 45 ppb in certain urban areas. In this regard it is of note that ants of genus Formica produce some 10Tg of formic acid each year; some ten times that produced by industry. The expected sinks are those generally associated with tropospheric chemistry: the major routes studied, to date, being wet and dry deposition. No studies have been carried out hitherto on the role of water-ice surfaces in the atmospheric chemistry of carboxylic acids and the purpose of this paper is to indicate their potential function in the heterogeneous release of atmospheric species such as HONO. The deposition of formic acid on a water-ice surface was studied using FT-RAIR spectroscopy over a range of temperatures between 100 and 165K. In all cases ionization to the formate (and oxonium) ions was observed. The results were confirmed by TPD (Temperature Programmed Desorption) measurements, which indicated that two distinct surface species adsorb to the ice. Potential reactions between the formic acid/formate ion surface and nitrogen dioxide were subsequently investigated by FT-RAIRS. Co-deposition experiments showed that N2O3 and the NO+ ion (associated with water) were formed as products. A mechanism is proposed to explain these results, which involves direct reaction between the organic acid and nitrogen dioxide. Similar experiments involving acetic acid also indicate ionization on a water-ice surface. The results are put into the context of atmospheric chemistry potentially occuring on cirrus cloud surfaces.

  10. Radiative effects of clouds and cryosphere in the Antarctic

    Directory of Open Access Journals (Sweden)

    Takashi Yamanouchi

    1997-03-01

    Full Text Available Examination of the effects of clouds, ice sheet and sea ice on the radiation budget in the Antarctic using Earth Radiation Budget Experiment (ERBE data were reported. The continental ice sheet affects not only the albedo, but also the surface temperature because of elevation, and hence the OLR. Sea ice, which is a critical climate feedback factor, appears to have less impact on radiation than do clouds. However, these surfaces lie underneath clouds, and it was found that the independent effect of sea ice is as large as that of clouds, and clouds are masking the radiative effect of sea ice by more than half. The radiation budget at the top of the atmosphere from satellite observation and that at the surface from the surface radiation measurements at Syowa and South Pole Stations were compared. Cloud radiative forcing at both stations for the surface, atmosphere and top of the atmosphere was derived.

  11. Investigation of the question of a danger to the population by fallout from the stratospheric depot

    International Nuclear Information System (INIS)

    Reiter, R.; Kanter, H.J.; Sladkovic, R.; Poetzl, K.

    1975-01-01

    The self-developed evaluation programme modified for the present tasks - a programme to set up continuous isentropical trajectory analyses and to investigate the tropopause fine structure for the determination of the climatology of the intrusion of stratospheric (contaminated) air into the troposphere and its transport to a point of the earth's surface in the temperate latitudes, is fully efficient. It does not merely determine trivial cases with direct sinking from the lower stratoshere to the measuring station (pure adiabatic case), but cases of non-adiabatic mixture processes can also be described by using several trajectories corresponding with one another. The method of cross-section and longitudinal section analyses gives the data necessary for the description of the intrusion of stratospheric air through the tropopause with sufficient accuracy. Based on the knowledge obtained sofar, a scheme to predict stratospheric intrusions has been set up and experimentally applied. The very first results are already promising. (orig.) [de

  12. A distribution law for relative humidity in the upper troposphere and lower stratosphere derived from three years of MOZAIC measurements

    Directory of Open Access Journals (Sweden)

    K. Gierens

    1999-09-01

    Full Text Available Data from three years of MOZAIC measurements made it possible to determine a distribution law for the relative humidity in the upper troposphere and lower stratosphere. Data amounting to 13.5% of the total were obtained in regions with ice supersaturation. Troposphere and stratosphere are distinguished by an ozone concentration of 130 ppbv as threshold. The probability of measuring a certain amount of ice supersaturation in the troposphere decreases exponentially with the degree of ice supersaturation. The probability of measuring a certain relative humidity in the stratosphere (both with respect to water and ice decreases exponentially with the relative humidity. A stochastic model that naturally leads to the exponential distribution is provided. Mean supersaturation in the troposphere is about 15%, whereas ice nucleation requires 30% supersaturation on the average. This explains the frequency of regions in which aircraft induce persistent contrails but which are otherwise free of clouds. Ice supersaturated regions are 3-4 K colder and contain more than 50% more vapour than other regions in the upper troposphere. The stratospheric air masses sampled are dry, as expected, having mean relative humidity over water of 12% and over ice of 23%, respectively. However, 2% of the stratospheric data indicate ice supersaturation. As the MOZAIC measurements have been obtained on commercial flights mainly between Europe and North America, the data do not provide a complete global picture, but the exponential character of the distribution laws found is probably valid globally. Since water vapour is the most important greenhouse gas and since it might enhance the anthropogenic greenhouse effects via positive feedback mechanisms, it is important to represent its distribution correctly in climate models. The discovery of the distribution law of the relative humidity makes possible simple tests to show whether the hydrological cycle in climate models is

  13. The response of clouds and aerosols to cosmic ray decreases

    DEFF Research Database (Denmark)

    Svensmark, J.; Enghoff, Martin Andreas Bødker; Shaviv, N. J.

    2016-01-01

    A method is developed to rank Forbush Decreases (FDs) in the galactic cosmic ray radiation according to their expected impact on the ionization of the lower atmosphere. Then a Monte Carlo bootstrap based statistical test is formulated to estimate the significance of the apparent response in physi......A method is developed to rank Forbush Decreases (FDs) in the galactic cosmic ray radiation according to their expected impact on the ionization of the lower atmosphere. Then a Monte Carlo bootstrap based statistical test is formulated to estimate the significance of the apparent response...... in physical and micro-physical cloud parameters to FDs. The test is subsequently applied to one ground based and three satellite based datasets. Responses (> 95%) to FDs are found in the following parameters of the analyzed datasets. AERONET: Ångström exponent (cloud condensation nuclei changes), SSM...... with the strength of the FDs, and the signs and magnitudes of the responses agree with model based expectations. The effect is mainly seen in liquid clouds. An impact through changes in UV driven photo chemistry is shown to be negligible and an impact via UV absorption in the stratosphere is found to have no effect...

  14. Stratospheric concentrations of N2O in July 1975

    International Nuclear Information System (INIS)

    Krey, P.W.; Lagomarsino, R.J.; Schonberg, M.

    1977-01-01

    The first measurement of the hemispheric distribution of N 2 O concentrations in the lower stratosphere of the Northern Hemisphere is reported for July 1975. This distribution is similar to those of CCl 3 F and SF 6 , although N 2 O is more stable in the stratosphere than either of the other trace gases. The inventory of N 2 O in the stratosphere of the Northern Hemisphere in July 1975 against which future observations can be compared is 136 Tg

  15. Persistent gravity wave coupling from the stratosphere to the MLT versus secondary wave generation in Antarctica

    Science.gov (United States)

    Zhao, J.; Geraghty, I.; Chu, X.; Vadas, S.; Becker, E.; Harvey, V. L.; Jones, R. M.; Chen, C.; Lu, X.

    2017-12-01

    After Antarctic persistent gravity waves (GWs) in the Mesosphere and Lower Thermosphere (MLT) were discovered from lidar observations [Chen et al., 2013, 2016], secondary wave generation theory was proposed to explain the source. Here we perform a source investigation of such persistent GWs through analyzing both stratospheric and MLT GWs at McMurdo using temperature measurements (30 - 50 km, year 2011 - 2015) obtained by Fe Boltzmann lidar. In the stratosphere, GW vertical wavelengths (λ) and periods exhibit seasonal cycles with winter maxima and summer minima, which linearly correlated with mean zonal wind velocities. GWs dissipate more in winter than in summer due to larger wave amplitudes. The potential energy density (Ep) are anti-correlated with wind rotation angles but positively correlated with surface and stratospheric winds. Critical level filtering, in-situ generation of GWs, and wave saturation changes play roles in Ep seasonal variations (winter maxima and summer minima). The large increase of Ep from summer to winter possibly results from the decrease in critical level filtering. The gradual variations of Ep from Mar to Oct are likely related both to the increased λ towards winter, allowing larger wave amplitudes before saturation, and to in-situ GW generation via geostrophic adjustment, secondary GW generation. Large Ep occur when McMurdo is inside the jet stream core 5-24º poleward from vortex edge. In winter MLT, the persistent GWs cause larger temperature perturbations (± 30 K, compared to ± 10 K in the stratosphere) with longer λ (23.5 km) and larger vertical phase speeds (1.8 m/s). More waves (95.4%) show downward phase progression compared to the stratospheric GWs (70.4%). Since the inferred horizontal wavelength of stratospheric GWs (350 - 450 km) are much shorter than those of the persistent GWs in the MLT (1000 - 2000 km), the dominant stratospheric GWs are not the direct source of the MLT persistent GWs. Secondary wave generation

  16. The Temperature of the Arctic and Antarctic Lower Stratosphere

    Science.gov (United States)

    Newman, Paul A.; Nash, Eric R.; Bhartia, P. K. (Technical Monitor)

    2002-01-01

    The temperature of the polar lower stratosphere during spring is the key factor in changing the magnitude of ozone loss in the polar vortices. In this talk, we will review the results of Newman et al. [2000] that quantitatively demonstrate that the polar lower stratospheric temperature is primarily controlled by planetary-scale waves. In particular, the tropospheric eddy heat flux in middle to late winter (January--February) is highly correlated with the mean polar stratospheric temperature during March. Strong midwinter planetary wave forcing leads to a warmer spring Arctic lower stratosphere in early spring, while weak midwinter forcing leads to cooler spring Arctic temperatures. In addition, this planetary wave driving also has a strong impact on the strength of the polar vortex. These results from the Northern Hemisphere will be contrasted with the Southern Hemisphere.

  17. Satellite-Surface Perspectives of Air Quality and Aerosol-Cloud Effects on the Environment: An Overview of 7-SEAS BASELInE

    Science.gov (United States)

    Tsay, Si-Chee; Maring, Hal B.; Lin, Neng-Huei; Buntoung, Sumaman; Chantara, Somporn; Chuang, Hsiao-Chi; Gabriel, Philip M.; Goodloe, Colby S.; Holben, Brent N.; Hsiao, Ta-Chih; hide

    2016-01-01

    The objectives of 7-SEASBASELInE (Seven SouthEast Asian Studies Biomass-burning Aerosols and Stratocumulus Environment: Lifecycles and Interactions Experiment) campaigns in spring 2013-2015 were to synergize measurements from uniquely distributed ground-based networks (e.g., AERONET (AErosol RObotic NETwork)), MPLNET ( NASA Micro-Pulse Lidar Network)) and sophisticated platforms (e.g.,SMARTLabs (Surface-based Mobile Atmospheric Research and Testbed Laboratories), regional contributing instruments), along with satellite observations retrievals and regional atmospheric transport chemical models to establish a critically needed database, and to advance our understanding of biomass-burning aerosols and trace gases in Southeast Asia (SEA). We present a satellite-surface perspective of 7-SEASBASELInE and highlight scientific findings concerning: (1) regional meteorology of moisture fields conducive to the production and maintenance of low-level stratiform clouds over land; (2) atmospheric composition in a biomass-burning environment, particularly tracers-markers to serve as important indicators for assessing the state and evolution of atmospheric constituents; (3) applications of remote sensing to air quality and impact on radiative energetics, examining the effect of diurnal variability of boundary-layer height on aerosol loading; (4) aerosol hygroscopicity and ground-based cloud radar measurements in aerosol-cloud processes by advanced cloud ensemble models; and (5) implications of air quality, in terms of toxicity of nanoparticles and trace gases, to human health. This volume is the third 7-SEAS special issue (after Atmospheric Research, vol. 122, 2013; and Atmospheric Environment, vol. 78, 2013) and includes 27 papers published, with emphasis on air quality and aerosol-cloud effects on the environment. BASELInE observations of stratiform clouds over SEA are unique, such clouds are embedded in a heavy aerosol-laden environment and feature characteristically greater

  18. Stratospheric experiments on curing of composite materials

    Science.gov (United States)

    Chudinov, Viacheslav; Kondyurin, Alexey; Svistkov, Alexander L.; Efremov, Denis; Demin, Anton; Terpugov, Viktor; Rusakov, Sergey

    2016-07-01

    Future space exploration requires a large light-weight structure for habitats, greenhouses, space bases, space factories and other constructions. A new approach enabling large-size constructions in space relies on the use of the technology of polymerization of fiber-filled composites with a curable polymer matrix applied in the free space environment on Erath orbit. In orbit, the material is exposed to high vacuum, dramatic temperature changes, plasma of free space due to cosmic rays, sun irradiation and atomic oxygen (in low Earth orbit), micrometeorite fluence, electric charging and microgravitation. The development of appropriate polymer matrix composites requires an understanding of the chemical processes of polymer matrix curing under the specific free space conditions to be encountered. The goal of the stratospheric flight experiment is an investigation of the effect of the stratospheric conditions on the uncured polymer matrix of the composite material. The unique combination of low residual pressure, high intensity UV radiation including short-wave UV component, cosmic rays and other aspects associated with solar irradiation strongly influences the chemical processes in polymeric materials. We have done the stratospheric flight experiments with uncured composites (prepreg). A balloon with payload equipped with heater, temperature/pressure/irradiation sensors, microprocessor, carrying the samples of uncured prepreg has been launched to stratosphere of 25-30 km altitude. After the flight, the samples have been tested with FTIR, gel-fraction, tensile test and DMA. The effect of cosmic radiation has been observed. The composite was successfully cured during the stratospheric flight. The study was supported by RFBR grants 12-08-00970 and 14-08-96011.

  19. Cirrus cloud-temperature interactions in the tropical tropopause layer: a case study

    Directory of Open Access Journals (Sweden)

    J. R. Taylor

    2011-10-01

    Full Text Available Thin cirrus clouds in the Tropical Tropopause Layer (TTL have important ramifications for radiative transfer, stratospheric humidity, and vertical transport. A horizontally extensive and vertically thin cirrus cloud in the TTL was detected by the Cloud Aerosol LIDAR and Infrared Pathfinder Satellite Observations (CALIPSO on 27–29 January 2009 in the Tropical Eastern Pacific region, distant from any regions of deep convection. These observations indicate that the cloud is close to 3000 km in length along the CALIPSO orbit track. Measurements over this three day period indicate that the cloud event extended over a region from approximately 15° S to 10° N and 90° W to 150° W and may be one of the most extensive cirrus events ever observed. Coincident temperature observations from the Constellation of Observing Satellites for Meteorology, Ionosphere, and Climate (COSMIC suggest that the cloud formed in-situ as a result of a cold anomaly arising from a midlatitude intrusion. The event appears to last for up to 2 days and the temperature observations do not show any indication of the expected infrared heating. It is hypothesized that the cloud could be maintained by either nucleation of numerous small ice crystals that don't sediment or by multiple localized ice nucleation events driven by temperature variability at scales smaller than the overall cloud field, producing small ice-crystal sizes which have sufficiently long residence times (≈53 h to maintain the cloud. It is possible that the residence times are augmented by vertical motion which could also act to offset the expected infrared heating. Further observations of similar events will be required in order to conclusively explain this curious cloud.

  20. Spectral Dependence of MODIS Cloud Droplet Effective Radius Retrievals for Marine Boundary Layer Clouds

    Science.gov (United States)

    Zhang, Zhibo; Platnick, Steven E.; Ackerman, Andrew S.; Cho, Hyoun-Myoung

    2014-01-01

    Low-level warm marine boundary layer (MBL) clouds cover large regions of Earth's surface. They have a significant role in Earth's radiative energy balance and hydrological cycle. Despite the fundamental role of low-level warm water clouds in climate, our understanding of these clouds is still limited. In particular, connections between their properties (e.g. cloud fraction, cloud water path, and cloud droplet size) and environmental factors such as aerosol loading and meteorological conditions continue to be uncertain or unknown. Modeling these clouds in climate models remains a challenging problem. As a result, the influence of aerosols on these clouds in the past and future, and the potential impacts of these clouds on global warming remain open questions leading to substantial uncertainty in climate projections. To improve our understanding of these clouds, we need continuous observations of cloud properties on both a global scale and over a long enough timescale for climate studies. At present, satellite-based remote sensing is the only means of providing such observations.

  1. Nonlinear response of tropical lower-stratospheric temperature and water vapor to ENSO

    Directory of Open Access Journals (Sweden)

    C. I. Garfinkel

    2018-04-01

    Full Text Available A series of simulations using the NASA Goddard Earth Observing System Chemistry–Climate Model are analyzed in order to aid in the interpretation of observed interannual and sub-decadal variability in the tropical lower stratosphere over the past 35 years. The impact of El Niño–Southern Oscillation on temperature and water vapor in this region is nonlinear in boreal spring. While moderate El Niño events lead to cooling in this region, strong El Niño events lead to warming, even as the response of the large-scale Brewer–Dobson circulation appears to scale nearly linearly with El Niño. This nonlinearity is shown to arise from the response in the Indo-West Pacific to El Niño: strong El Niño events lead to tropospheric warming extending into the tropical tropopause layer and up to the cold point in this region, where it allows for more water vapor to enter the stratosphere. The net effect is that both strong La Niña and strong El Niño events lead to enhanced entry water vapor and stratospheric moistening in boreal spring and early summer. These results lead to the following interpretation of the contribution of sea surface temperatures to the decline in water vapor in the early 2000s: the very strong El Niño event in 1997/1998, followed by more than 2 consecutive years of La Niña, led to enhanced lower-stratospheric water vapor. As this period ended in early 2001, entry water vapor concentrations declined. This effect accounts for approximately one-quarter of the observed drop.

  2. Nonlinear response of tropical lower-stratospheric temperature and water vapor to ENSO

    Science.gov (United States)

    Garfinkel, Chaim I.; Gordon, Amit; Oman, Luke D.; Li, Feng; Davis, Sean; Pawson, Steven

    2018-04-01

    A series of simulations using the NASA Goddard Earth Observing System Chemistry-Climate Model are analyzed in order to aid in the interpretation of observed interannual and sub-decadal variability in the tropical lower stratosphere over the past 35 years. The impact of El Niño-Southern Oscillation on temperature and water vapor in this region is nonlinear in boreal spring. While moderate El Niño events lead to cooling in this region, strong El Niño events lead to warming, even as the response of the large-scale Brewer-Dobson circulation appears to scale nearly linearly with El Niño. This nonlinearity is shown to arise from the response in the Indo-West Pacific to El Niño: strong El Niño events lead to tropospheric warming extending into the tropical tropopause layer and up to the cold point in this region, where it allows for more water vapor to enter the stratosphere. The net effect is that both strong La Niña and strong El Niño events lead to enhanced entry water vapor and stratospheric moistening in boreal spring and early summer. These results lead to the following interpretation of the contribution of sea surface temperatures to the decline in water vapor in the early 2000s: the very strong El Niño event in 1997/1998, followed by more than 2 consecutive years of La Niña, led to enhanced lower-stratospheric water vapor. As this period ended in early 2001, entry water vapor concentrations declined. This effect accounts for approximately one-quarter of the observed drop.

  3. New capability for ozone dial profiling measurements in the troposphere and lower stratosphere from aircraft

    Science.gov (United States)

    Hair, Johnathan; Hostetler, Chris; Cook, Anthony; Harper, David; Notari, Anthony; Fenn, Marta; Newchurch, Mike; Wang, Lihua; Kuang, Shi; Knepp, Travis; Burton, Sharon; Ferrare, Richard; Butler, Carolyn; Collins, Jim; Nehrir, Amin

    2018-04-01

    Recently, we successfully demonstrated a new compact and robust ozone DIAL lidar for smaller aircraft such as the NASA B200 and the ER-2 high-altitude aircraft. This is the first NASA airborne lidar to incorporate advanced solid-state lasers to produce the required power at the required ultraviolet wavelengths, and is compact and robust enough to operate nearly autonomously on the high-altitude ER-2 aircraft. This technology development resulted in the first new NASA airborne ozone DIAL instrument in more than 15 years. The combined ozone, aerosol, and clouds measurements provide valuable information on the chemistry, radiation, and dynamics of the atmosphere. In particular, from the ER-2 it offers a unique capability to study the upper troposphere and lower stratosphere.

  4. New capability for ozone dial profiling measurements in the troposphere and lower stratosphere from aircraft

    Directory of Open Access Journals (Sweden)

    Hair Johnathan

    2018-01-01

    Full Text Available Recently, we successfully demonstrated a new compact and robust ozone DIAL lidar for smaller aircraft such as the NASA B200 and the ER-2 high-altitude aircraft. This is the first NASA airborne lidar to incorporate advanced solid-state lasers to produce the required power at the required ultraviolet wavelengths, and is compact and robust enough to operate nearly autonomously on the high-altitude ER-2 aircraft. This technology development resulted in the first new NASA airborne ozone DIAL instrument in more than 15 years. The combined ozone, aerosol, and clouds measurements provide valuable information on the chemistry, radiation, and dynamics of the atmosphere. In particular, from the ER-2 it offers a unique capability to study the upper troposphere and lower stratosphere.

  5. Sulphur-rich volcanic eruptions and stratospheric aerosols

    Science.gov (United States)

    Rampino, M. R.; Self, S.

    1984-01-01

    Data from direct measurements of stratospheric optical depth, Greenland ice-core acidity, and volcanological studies are compared, and it is shown that relatively small but sulfur-rich volcanic eruptions can have atmospheric effects equal to or even greater than much larger sulfur-poor eruptions. These small eruptions are probably the most frequent cause of increased stratospheric aerosols. The possible sources of the excess sulfur released in these eruptions are discussed.

  6. Influence of an Internally-Generated QBO on Modeled Stratospheric Dynamics and Ozone

    Science.gov (United States)

    Hurwitz, M. M.; Newman, P. A.; Song, I. S.

    2011-01-01

    A GEOS V2 CCM simulation with an internally generated quasi-biennial oscillation (QBO) signal is compared to an otherwise identical simulation without a QBO. In a present-day climate, inclusion of the modeled QBO makes a significant difference to stratospheric dynamics and ozone throughout the year. The QBO enhances variability in the tropics, as expected, but also in the polar stratosphere in some seasons. The modeled QBO also affects the mean stratospheric climate. Because tropical zonal winds in the baseline simulation are generally easterly, there is a relative increase in zonal wind magnitudes in tropical lower and middle stratosphere in the QBO simulation. Extra-tropical differences between the QBO and 'no QBO' simulations thus reflect a bias toward the westerly phase of the QBO: a relative strengthening and poleward shifting the polar stratospheric jets, and a reduction in Arctic lower stratospheric ozone.

  7. Effect of chemical structure on the cloud point of some new non-ionic surfactants based on bisphenol in relation to their surface active properties

    Directory of Open Access Journals (Sweden)

    A.M. Al-Sabagh

    2011-06-01

    Full Text Available A series of non-ionic surfactants were prepared from bisphenol derived from acetone (A, acetophenone (AC and cyclohexanone (CH. The prepared bisphenols were ethoxylated at different degrees of ethylene oxide (27, 35, 43. The ethoxylated bisphenols were non-esterified by fatty acids; decanoic, lauric, myristic, palmitic, stearic, oleic, linoloic and linolinic. Some surface active properties for these surfactants were measured and calculated such as, surface tension [γ], critical micelle concentration [CMC], minimum area per molecule [Amin], surface excess [Cmax], free energy of micellization and adsorption [ΔGmic] and [ΔGads]. At a certain temperature, the cloud point was measured for these surfactants. From the obtained data it was found that; the cloud point is very sensitive to the increase of the alkyl chain length, content of ethylene oxide and degree of unsaturation. The core of bisphenol affected the cloud point sharply and they are ranked regarding bisphenol structure as BA > BCH > BAC. By inspection of the surface active properties of these surfactants, a good relation was obtained with their cloud points. The data were discussed on the light of their chemical structures.

  8. Insight into Chemistry on Cloud/Aerosol Water Surfaces.

    Science.gov (United States)

    Zhong, Jie; Kumar, Manoj; Francisco, Joseph S; Zeng, Xiao Cheng

    2018-05-15

    Cloud/aerosol water surfaces exert significant influence over atmospheric chemical processes. Atmospheric processes at the water surface are observed to follow mechanisms that are quite different from those in the gas phase. This Account summarizes our recent findings of new reaction pathways on the water surface. We have studied these surface reactions using Born-Oppenheimer molecular dynamics simulations. These studies provide useful information on the reaction time scale, the underlying mechanism of surface reactions, and the dynamic behavior of the product formed on the aqueous surface. According to these studies, the aerosol water surfaces confine the atmospheric species into a specific orientation depending on the hydrophilicity of atmospheric species or the hydrogen-bonding interactions between atmospheric species and interfacial water. As a result, atmospheric species are activated toward a particular reaction on the aerosol water surface. For example, the simplest Criegee intermediate (CH 2 OO) exhibits high reactivity toward the interfacial water and hydrogen sulfide, with the reaction times being a few picoseconds, 2-3 orders of magnitude faster than that in the gas phase. The presence of interfacial water molecules induces proton-transfer-based stepwise pathways for these reactions, which are not possible in the gas phase. The strong hydrophobicity of methyl substituents in larger Criegee intermediates (>C1), such as CH 3 CHOO and (CH 3 ) 2 COO, blocks the formation of the necessary prereaction complexes for the Criegee-water reaction to occur at the water droplet surface, which lowers their proton-transfer ability and hampers the reaction. The aerosol water surface provides a solvent medium for acids (e.g., HNO 3 and HCOOH) to participate in reactions via mechanisms that are different from those in the gas and bulk aqueous phases. For example, the anti-CH 3 CHOO-HNO 3 reaction in the gas phase follows a direct reaction between anti-CH 3 CHOO and HNO 3

  9. Benefits, risks, and costs of stratospheric geoengineering

    KAUST Repository

    Robock, Alan

    2009-10-02

    Injecting sulfate aerosol precursors into the stratosphere has been suggested as a means of geoengineering to cool the planet and reduce global warming. The decision to implement such a scheme would require a comparison of its benefits, dangers, and costs to those of other responses to global warming, including doing nothing. Here we evaluate those factors for stratospheric geoengineering with sulfate aerosols. Using existing U.S. military fighter and tanker planes, the annual costs of injecting aerosol precursors into the lower stratosphere would be several billion dollars. Using artillery or balloons to loft the gas would be much more expensive. We do not have enough information to evaluate more exotic techniques, such as pumping the gas up through a hose attached to a tower or balloon system. Anthropogenic stratospheric aerosol injection would cool the planet, stop the melting of sea ice and land-based glaciers, slow sea level rise, and increase the terrestrial carbon sink, but produce regional drought, ozone depletion, less sunlight for solar power, and make skies less blue. Furthermore it would hamper Earth-based optical astronomy, do nothing to stop ocean acidification, and present many ethical and moral issues. Further work is needed to quantify many of these factors to allow informed decision-making.

  10. Stratospheric controlled perturbation experiment (SCoPEx): overview, status, and results from related laboratory experiments

    Science.gov (United States)

    Keith, D.; Dykema, J. A.; Keutsch, F. N.

    2017-12-01

    Stratospheric Controlled Perturbation Experiment (SCoPEx), is a scientific experiment to advance understanding of stratospheric aerosols. It aims to make quantitative measurements of aerosol microphysics and atmospheric chemistry to improve large-scale models used to assess the risks and benefits of solar geoengineering. A perturbative experiment requires: (a) means to create a well-mixed, small perturbed volume, and (b) observation of time evolution of chemistry and aerosols in the volume. SCoPEx will used a propelled balloon gondola containing all instruments and drive system. The propeller wake forms a well-mixed volume (roughly 1 km long and 100 meters in diameter) that serves as an experimental `beaker' into which aerosols (e.g., budget, etc; (d) results from CFD simulation of propeller wake and simulation of chemistry and aerosol microphysics; and finally (e) proposed concept of operations and schedule. We will also provide an overview of the plans for governance including management of health safety and environmental risks, transparency, public engagement, and larger questions about governance of solar geoengineering experiments. Finally, we will briefly present results of laboratory experiments of the interaction of chemical such as ClONO2 and HCl on particle surfaces relevant for stratospheric solar geoengineering.

  11. An Integrated Cloud-Aerosol-Radiation Product Using CERES, MODIS, CALIPSO and CloudSat Data

    Science.gov (United States)

    Sun-Mack, S.; Gibson, S.; Chen, Y.; Wielicki, B.; Minnis, P.

    2006-12-01

    The goal of this paper is to provide the first integrated data set of global vertical profiles of aerosols, clouds, and radiation using the combined NASA A-Train data from Aqua CERES and MODIS, CALIPSO, and CloudSat. All of these instruments are flying in formation as part of the Aqua Train, or A-Train. This paper will present the preliminary results of merging aerosol and cloud data from the CALIPSO active lidar, cloud data from CloudSat, integrated column aerosol and cloud data from the MODIS CERES analyses, and surface and top-of-atmosphere broadband radiation fluxes from CERES. These new data will provide unprecedented ability to test and improve global cloud and aerosol models, to investigate aerosol direct and indirect radiative forcing, and to validate the accuracy of global aerosol, cloud, and radiation data sets especially in polar regions and for multi-layered cloud conditions.

  12. Automatic extraction of discontinuity orientation from rock mass surface 3D point cloud

    Science.gov (United States)

    Chen, Jianqin; Zhu, Hehua; Li, Xiaojun

    2016-10-01

    This paper presents a new method for extracting discontinuity orientation automatically from rock mass surface 3D point cloud. The proposed method consists of four steps: (1) automatic grouping of discontinuity sets using an improved K-means clustering method, (2) discontinuity segmentation and optimization, (3) discontinuity plane fitting using Random Sample Consensus (RANSAC) method, and (4) coordinate transformation of discontinuity plane. The method is first validated by the point cloud of a small piece of a rock slope acquired by photogrammetry. The extracted discontinuity orientations are compared with measured ones in the field. Then it is applied to a publicly available LiDAR data of a road cut rock slope at Rockbench repository. The extracted discontinuity orientations are compared with the method proposed by Riquelme et al. (2014). The results show that the presented method is reliable and of high accuracy, and can meet the engineering needs.

  13. Mass-velocity and size-velocity distributions of ejecta cloud from shock-loaded tin surface using atomistic simulations

    Energy Technology Data Exchange (ETDEWEB)

    Durand, O.; Soulard, L. [CEA, DAM, DIF, F-91297 Arpajon (France)

    2015-04-28

    The mass (volume and areal densities) versus velocity as well as the size versus velocity distributions of a shock-induced cloud of particles are investigated using large scale molecular dynamics simulations. A generic three-dimensional tin crystal with a sinusoidal free surface roughness (single wavelength) is set in contact with vacuum and shock-loaded so that it melts directly on shock. At the reflection of the shock wave onto the perturbations of the free surface, two-dimensional sheets/jets of liquid metal are ejected. The simulations show that the distributions may be described by an analytical model based on the propagation of a fragmentation zone, from the tip of the sheets to the free surface, in which the kinetic energy of the atoms decreases as this zone comes closer to the free surface on late times. As this kinetic energy drives (i) the (self-similar) expansion of the zone once it has broken away from the sheet and (ii) the average size of the particles which result from fragmentation in the zone, the ejected mass and the average size of the particles progressively increase in the cloud as fragmentation occurs closer to the free surface. Though relative to nanometric scales, our model may help in the analysis of experimental profiles.

  14. CERN: Antiprotons probe the nuclear stratosphere

    International Nuclear Information System (INIS)

    Anon.

    1995-01-01

    The outer periphery of heavy stable nuclei is notoriously difficult to study experimentally. While the well understood electromagnetic interaction between electrons (or muons) and protons has given the nuclear charge (or proton) distribution with high precision for almost all stable nuclei, neutron distribution studies are much less precise. This is especially true for large nuclear distances, where the nuclear density is small. A few previous experiments probing the nuclear ''stratosphere'' suggested that far from the centre of the nucleus (of the order of 2 nuclear radii) this stratosphere may be composed predominantly of neutrons. At the end of the sixties the term ''neutron halo'' was introduced to describe this phenomenon, but experimental evidence was scarce or even controversial, and remained so for almost a quarter of a century. Recently, the Warsaw/Munich/Berlin collaboration working within the PS203 experiment at CERN's LEAR low energy antiproton ring, proposed a new method to study the nuclear periphery using stopped antiprotons. The halo now looks firmer. A 200 MeV/c beam of antiprotons was slowed down by interactions with atomic electrons. When antiproton kinetic energy drops well below 1 keV, the particles are captured in the outermost orbits of ''exotic atoms'', where the antiprotons take the place of the usual orbital electrons. With the lower orbits in this antiprotonic atom empty, the antiproton drops toward the nuclear surface, first emitting Auger electrons and later predominantly antiprotonic X-rays. Due to the strong interaction between antiprotons and nucleons, the antiproton succumbs to annihilation with a nucleon in the rarified nuclear stratosphere, far above the innermost Bohr orbit of the atom. The annihilation probability in heavy nuclei is maximal where the nuclear density is about 3% of its central value and extends to densities many orders of magnitude smaller

  15. Stable Water Isotopologues in the Stratosphere Retrieved from Odin/SMR Measurements

    Directory of Open Access Journals (Sweden)

    Tongmei Wang

    2018-01-01

    Full Text Available Stable Water Isotopologues (SWIs are important diagnostic tracers for understanding processes in the atmosphere and the global hydrological cycle. Using eight years (2002–2009 of retrievals from Odin/SMR (Sub-Millimetre Radiometer, the global climatological features of three SWIs, H216O, HDO and H218O, the isotopic composition δD and δ18O in the stratosphere are analysed for the first time. Spatially, SWIs are found to increase with altitude due to stratospheric methane oxidation. In the tropics, highly depleted SWIs in the lower stratosphere indicate the effect of dehydration when the air comes through the cold tropopause, while, at higher latitudes, more enriched SWIs in the upper stratosphere during summer are produced and transported to the other hemisphere via the Brewer–Dobson circulation. Furthermore, we found that more H216O is produced over summer Northern Hemisphere and more HDO is produced over summer Southern Hemisphere. Temporally, a tape recorder in H216O is observed in the lower tropical stratosphere, in addition to a pronounced downward propagating seasonal signal in SWIs from the upper to the lower stratosphere over the polar regions. These observed features in SWIs are further compared to SWI-enabled model outputs. This helped to identify possible causes of model deficiencies in reproducing main stratospheric features. For instance, choosing a better advection scheme and including methane oxidation process in a specific model immediately capture the main features of stratospheric water vapor. The representation of other features, such as the observed inter-hemispheric difference of isotopic component, is also discussed.

  16. An Estimation of the Climatic Effects of Stratospheric Ozone Losses during the 1980s. Appendix K

    Science.gov (United States)

    MacKay, Robert M.; Ko, Malcolm K. W.; Shia, Run-Lie; Yang, Yajaing; Zhou, Shuntai; Molnar, Gyula

    1997-01-01

    In order to study the potential climatic effects of the ozone hole more directly and to assess the validity of previous lower resolution model results, the latest high spatial resolution version of the Atmospheric and Environmental Research, Inc., seasonal radiative dynamical climate model is used to simulate the climatic effects of ozone changes relative to the other greenhouse gases. The steady-state climatic effect of a sustained decrease in lower stratospheric ozone, similar in magnitude to the observed 1979-90 decrease, is estimated by comparing three steady-state climate simulations: 1) 1979 greenhouse gas concentrations and 1979 ozone, II) 1990 greenhouse gas concentrations with 1979 ozone, and III) 1990 greenhouse gas concentrations with 1990 ozone. The simulated increase in surface air temperature resulting from nonozone greenhouse gases is 0.272 K. When changes in lower stratospheric ozone are included, the greenhouse warming is 0.165 K, which is approximately 39% lower than when ozone is fixed at the 1979 concentrations. Ozone perturbations at high latitudes result in a cooling of the surface-troposphere system that is greater (by a factor of 2.8) than that estimated from the change in radiative forcing resulting from ozone depiction and the model's 2 x CO, climate sensitivity. The results suggest that changes in meridional heat transport from low to high latitudes combined with the decrease in the infrared opacity of the lower stratosphere are very important in determining the steady-state response to high latitude ozone losses. The 39% compensation in greenhouse warming resulting from lower stratospheric ozone losses is also larger than the 28% compensation simulated previously by the lower resolution model. The higher resolution model is able to resolve the high latitude features of the assumed ozone perturbation, which are important in determining the overall climate sensitivity to these perturbations.

  17. Chemistry and Microphysics of Lower Stratospheric Aerosols Determined by Satellite Remote Sensing

    Science.gov (United States)

    Zasetsky, A. Y.; Khalizov, A.; Sloan, J.

    2003-12-01

    Observations of broadband Infrared satellites such as ILAS-II (Ministry of the Environment, Japan, launched 14 December 2002) and SciSat-1 (Canadian Space Agency, launched 12 August 2003) can provide details of the chemical composition and particle size of atmospheric aerosols by direct inversion without recourse to models. During the past decade, we have developed mathematical methods to achieve this inversion by working with FTIR observations of model atmospheric aerosols in cryogenic flowtubes. More recently, we have converted these to operational algorithms for use in the above missions. In this presentation, we will briefly outline these procedures and illustrate their capabilities using laboratory data. These laboratory results show that the chemical compositions, phases and sizes of ensembles of particles can be obtained simultaneously using these procedures. We will also report chemical and microphysical properties of lower stratospheric clouds and aerosols derived by applying these procedures to observations from space.

  18. Variability of Irreversible Poleward Transport in the Lower Stratosphere

    Science.gov (United States)

    Olsen, Mark; Douglass, Anne; Newman, Paul; Nash, Eric; Witte, Jacquelyn; Ziemke, Jerry

    2011-01-01

    The ascent and descent of the Brewer-Dobson circulation plays a large role in determining the distributions of many constituents in the extratropical lower stratosphere. However, relatively fast, quasi-horizontal transport out of the tropics and polar regions also significantly contribute to determining these distributions. The tropical tape recorder signal assures that there must be outflow from the tropics into the extratropical lower stratosphere. The phase of the quasi-biennial oscillation (QBO) and state of the polar vortex are known to modulate the transport from the tropical and polar regions, respectively. In this study we examine multiple years of ozone distributions in the extratropical lower stratosphere observed by the Aura Microwave Limb Sounder (MLS) and the Aura High Resolution Dynamic Limb Sounder (HIRDLS). The distributions are compared with analyses of irreversible, meridional isentropic transport. We show that there is considerable year-to-year seasonal variability in the amount of irreversible transport from the tropics, which is related to both the phase of the QBO and the state of the polar vortex. The reversibility of the transport is consistent with the number of observed breaking waves. The variability of the atmospheric index of refraction in the lower stratosphere is shown to be significantly correlated with the wave breaking and amount of irreversible transport. Finally, we will show that the seasonal extratropical stratosphere to troposphere transport of ozone can be substantially modulated by the amount of irreversible meridional transport in the lower stratosphere and we investigate how observable these differences are in data of tropospheric ozone.

  19. Impact of high speed civil transports on stratospheric ozone. A 2-D model investigation

    Energy Technology Data Exchange (ETDEWEB)

    Kinnison, D E; Connell, P S [Lawrence Livermore National Lab., CA (United States)

    1998-12-31

    This study investigates the effect on stratospheric ozone from a fleet of proposed High Speed Civil Transports (HSCTs). The new LLNL 2-D operator-split chemical-radiative-transport model of the troposphere and stratosphere is used for this HSCT investigation. This model is integrated in a diurnal manner, using an implicit numerical solver. Therefore, rate coefficients are not modified by any sort of diurnal average factor. This model also does not make any assumptions on lumping of chemical species into families. Comparisons to previous model-derived HSCT assessment of ozone change are made, both to the previous LLNL 2-D model and to other models from the international assessment modeling community. The sensitivity to the NO{sub x} emission index and sulfate surface area density is also explored. (author) 7 refs.

  20. Impact of high speed civil transports on stratospheric ozone. A 2-D model investigation

    Energy Technology Data Exchange (ETDEWEB)

    Kinnison, D.E.; Connell, P.S. [Lawrence Livermore National Lab., CA (United States)

    1997-12-31

    This study investigates the effect on stratospheric ozone from a fleet of proposed High Speed Civil Transports (HSCTs). The new LLNL 2-D operator-split chemical-radiative-transport model of the troposphere and stratosphere is used for this HSCT investigation. This model is integrated in a diurnal manner, using an implicit numerical solver. Therefore, rate coefficients are not modified by any sort of diurnal average factor. This model also does not make any assumptions on lumping of chemical species into families. Comparisons to previous model-derived HSCT assessment of ozone change are made, both to the previous LLNL 2-D model and to other models from the international assessment modeling community. The sensitivity to the NO{sub x} emission index and sulfate surface area density is also explored. (author) 7 refs.

  1. The Limb Infrared Monitor of the Stratosphere (LIMS) experiment

    Science.gov (United States)

    Russell, J. M.; Gille, J. C.

    1978-01-01

    The Limb Infrared Monitor of the Stratosphere is used to obtain vertical profiles and maps of temperature and the concentration of ozone, water vapor, nitrogen dioxide, and nitric acid for the region of the stratosphere bounded by the upper troposphere and the lower mesosphere.

  2. Impact of lower stratospheric ozone on seasonal prediction systems

    Directory of Open Access Journals (Sweden)

    Kelebogile Mathole

    2014-03-01

    Full Text Available We conducted a comparison of trends in lower stratospheric temperatures and summer zonal wind fields based on 27 years of reanalysis data and output from hindcast simulations using a coupled ocean-atmospheric general circulation model (OAGCM. Lower stratospheric ozone in the OAGCM was relaxed to the observed climatology and increasing greenhouse gas concentrations were neglected. In the reanalysis, lower stratospheric ozone fields were better represented than in the OAGCM. The spring lower stratospheric/ upper tropospheric cooling in the polar cap observed in the reanalysis, which is caused by a direct ozone depletion in the past two decades and is in agreement with previous studies, did not appear in the OAGCM. The corresponding summer tropospheric response also differed between data sets. In the reanalysis, a statistically significant poleward trend of the summer jet position was found, whereas no such trend was found in the OAGCM. Furthermore, the jet position in the reanalysis exhibited larger interannual variability than that in the OAGCM. We conclude that these differences are caused by the absence of long-term lower stratospheric ozone changes in the OAGCM. Improper representation or non-inclusion of such ozone variability in a prediction model could adversely affect the accuracy of the predictability of summer rainfall forecasts over South Africa.

  3. Tiny Ultraviolet Polarimeter for Earth Stratosphere from Space Investigation

    Science.gov (United States)

    Nevodovskyi, P. V.; Morozhenko, O. V.; Vidmachenko, A. P.; Ivakhiv, O.; Geraimchuk, M.; Zbrutskyi, O.

    2015-09-01

    One of the reasons for climate change (i.e., stratospheric ozone concentrations) is connected with the variations in optical thickness of aerosols in the upper sphere of the atmosphere (at altitudes over 30 km). Therefore, aerosol and gas components of the atmosphere are crucial in the study of the ultraviolet (UV) radiation passing upon the Earth. Moreover, a scrupulous study of aerosol components of the Earth atmosphere at an altitude of 30 km (i.e., stratospheric aerosol), such as the size of particles, the real part of refractive index, optical thickness and its horizontal structure, concentration of ozone or the upper border of the stratospheric ozone layer is an important task in the research of the Earth climate change. At present, the Main Astronomical Observatory of the National Academy of Sciences (NAS) of Ukraine, the National Technical University of Ukraine "KPI"and the Lviv Polytechnic National University are engaged in the development of methodologies for the study of stratospheric aerosol by means of ultraviolet polarimeter using a microsatellite. So fare, there has been created a sample of a tiny ultraviolet polarimeter (UVP) which is considered to be a basic model for carrying out space experiments regarding the impact of the changes in stratospheric aerosols on both global and local climate.

  4. An Investigation of Multi-Satellite Stratospheric Measurements on Tropospheric Weather Predictions over Continental United States

    Science.gov (United States)

    Shao, Min

    The troposphere and stratosphere are the two closest atmospheric layers to the Earth's surface. These two layers are separated by the so-called tropopause. On one hand, these two layers are largely distinguished, on the other hand, lots of evidences proved that connections are also existed between these two layers via various dynamical and chemical feedbacks. Both tropospheric and stratospheric waves can propagate through the tropopause and affect the down streams, despite the fact that this propagation of waves is relatively weaker than the internal interactions in both atmospheric layers. Major improvements have been made in numerical weather predictions (NWP) via data assimilation (DA) in the past 30 years. From optimal interpolation to variational methods and Kalman Filter, great improvements are also made in the development of DA technology. The availability of assimilating satellite radiance observation and the increasing amount of satellite measurements enabled the generation of better atmospheric initials for both global and regional NWP systems. The selection of DA schemes is critical for regional NWP systems. The performance of three major data assimilation (3D-Var, Hybrid, and EnKF) schemes on regional weather forecasts over the continental United States during winter and summer is investigated. Convergence rate in the variational methods can be slightly accelerated especially in summer by the inclusion of ensembles. When the regional model lid is set at 50-mb, larger improvements (10˜20%) in the initials are obtained over the tropopause and lower troposphere. Better forecast skills (˜10%) are obtained in all three DA schemes in summer. Among these three DA schemes, slightly better (˜1%) forecast skills are obtained in Hybrid configuration than 3D-Var. Overall better forecast skills are obtained in summer via EnKF scheme. An extra 22% skill in predicting summer surface pressure but 10% less skills in winter are given by EnKF when compared to 3D

  5. Delivery of halogenated very short-lived substances from the west Indian Ocean to the stratosphere during the Asian summer monsoon

    Directory of Open Access Journals (Sweden)

    A. Fiehn

    2017-06-01

    Full Text Available Halogenated very short-lived substances (VSLSs are naturally produced in the ocean and emitted to the atmosphere. When transported to the stratosphere, these compounds can have a significant influence on the ozone layer and climate. During a research cruise on RV Sonne in the subtropical and tropical west Indian Ocean in July and August 2014, we measured the VSLSs, methyl iodide (CH3I and for the first time bromoform (CHBr3 and dibromomethane (CH2Br2, in surface seawater and the marine atmosphere to derive their emission strengths. Using the Lagrangian particle dispersion model FLEXPART with ERA-Interim meteorological fields, we calculated the direct contribution of observed VSLS emissions to the stratospheric halogen burden during the Asian summer monsoon. Furthermore, we compare the in situ calculations with the interannual variability of transport from a larger area of the west Indian Ocean surface to the stratosphere for July 2000–2015. We found that the west Indian Ocean is a strong source for CHBr3 (910 pmol m−2 h−1, very strong source for CH2Br2 (930 pmol m−2 h−1, and an average source for CH3I (460 pmol m−2 h−1. The atmospheric transport from the tropical west Indian Ocean surface to the stratosphere experiences two main pathways. On very short timescales, especially relevant for the shortest-lived compound CH3I (3.5 days lifetime, convection above the Indian Ocean lifts oceanic air masses and VSLSs towards the tropopause. On a longer timescale, the Asian summer monsoon circulation transports oceanic VSLSs towards India and the Bay of Bengal, where they are lifted with the monsoon convection and reach stratospheric levels in the southeastern part of the Asian monsoon anticyclone. This transport pathway is more important for the longer-lived brominated compounds (17 and 150 days lifetime for CHBr3 and CH2Br2. The entrainment of CHBr3 and CH3I from the west Indian Ocean to the stratosphere during the

  6. The global warming potential of methane reassessed with combined stratosphere and troposphere chemistry

    Science.gov (United States)

    Holmes, C. D.; Archibald, A. T.; Eastham, S. D.; Søvde, O. A.

    2017-12-01

    Methane is a direct and indirect greenhouse gas. The direct greenhouse effect comes from the radiation absorbed and emitted by methane itself. The indirect greenhouse effect comes from radiatively active gases that are produced during methane oxidation: principally O3, H2O, and CO2. Methane also suppresses tropospheric OH, which indirectly affects numerous greenhouses gases and aerosols. Traditionally, the methane global warming potential (GWP) has included the indirect effects on tropospheric O3 and OH and stratospheric H2O, with these effects estimated independently from unrelated tropospheric and stratospheric chemistry models and observations. Using this approach the CH4 is about 28 over 100 yr (without carbon cycle feedbacks, IPCC, 2013). Here we present a comprehensive analysis of the CH4 GWP in several 3-D global atmospheric models capable of simulating both tropospheric and stratospheric chemistry (GEOS-Chem, Oslo CTM3, UKCA). This enables us to include, for the first time, the indirect effects of CH4 on stratospheric O3 and stratosphere-troposphere coupling. We diagnose the GWP from paired simulations with and without a 5% perturbation to tropospheric CH4 concentrations. Including stratospheric chemistry nearly doubles the O3 contribution to CH4 GWP because of O3 production in the lower stratosphere and because CH4 inhibits Cl-catalyzed O3 loss in the upper stratosphere. In addition, stratosphere-troposphere coupling strengthens the chemical feedback on its own lifetime. In the stratosphere, this feedback operates by a CH4 perturbation thickening the stratospheric O3 layer, which impedes UV-driven OH production in the troposphere and prolongs the CH4 lifetime. We also quantify the impact of CH4-derived H2O on the stratospheric HOx cycles but these effects are small. Combining all of the above, these models suggest that the 100-yr GWP of CH4 is over 33.5, a 20% increase over the latest IPCC assessment.

  7. SAGE measurements of the stratospheric aerosol dispersion and loading from the Soufriere Volcano

    Science.gov (United States)

    Mccormick, M. P.; Kent, G. S.; Yue, G. K.; Cunnold, D. M.

    1981-01-01

    Explosions of the Soufriere volcano on the Caribbean Island of St. Vincent reduced two major stratospheric plumes which the stratospheric aerosol and gas experiment (SAGE) satellite tracked to West Africa and the North Atlantic Ocean. The total mass of the stratospheric ejecta measured is less than 0.5% of the global stratospheric aerosol burden. No significant temperature or climate perturbation is expected. It is found that the movement and dispersion of the plumes agree with those deduced from high altitude meteorological data and dispersion theory. The stratospheric aerosol dispersion and loading from the Soufrier volcano was measured.

  8. Sedimentation Efficiency of Condensation Clouds in Substellar Atmospheres

    Science.gov (United States)

    Gao, Peter; Marley, Mark S.; Ackerman, Andrew S.

    2018-03-01

    Condensation clouds in substellar atmospheres have been widely inferred from spectra and photometric variability. Up until now, their horizontally averaged vertical distribution and mean particle size have been largely characterized using models, one of which is the eddy diffusion–sedimentation model from Ackerman and Marley that relies on a sedimentation efficiency parameter, f sed, to determine the vertical extent of clouds in the atmosphere. However, the physical processes controlling the vertical structure of clouds in substellar atmospheres are not well understood. In this work, we derive trends in f sed across a large range of eddy diffusivities (K zz ), gravities, material properties, and cloud formation pathways by fitting cloud distributions calculated by a more detailed cloud microphysics model. We find that f sed is dependent on K zz , but not gravity, when K zz is held constant. f sed is most sensitive to the nucleation rate of cloud particles, as determined by material properties like surface energy and molecular weight. High surface energy materials form fewer, larger cloud particles, leading to large f sed (>1), and vice versa for materials with low surface energy. For cloud formation via heterogeneous nucleation, f sed is sensitive to the condensation nuclei flux and radius, connecting cloud formation in substellar atmospheres to the objects’ formation environments and other atmospheric aerosols. These insights could lead to improved cloud models that help us better understand substellar atmospheres. For example, we demonstrate that f sed could increase with increasing cloud base depth in an atmosphere, shedding light on the nature of the brown dwarf L/T transition.

  9. Stratospheric Water and OzOne Satellite Homogenized (SWOOSH) data set

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — The Stratospheric Water and Ozone Satellite Homogenized (SWOOSH) data set is a merged record of stratospheric ozone and water vapor measurements taken by a number of...

  10. An ultrahot gas-giant exoplanet with a stratosphere.

    Science.gov (United States)

    Evans, Thomas M; Sing, David K; Kataria, Tiffany; Goyal, Jayesh; Nikolov, Nikolay; Wakeford, Hannah R; Deming, Drake; Marley, Mark S; Amundsen, David S; Ballester, Gilda E; Barstow, Joanna K; Ben-Jaffel, Lotfi; Bourrier, Vincent; Buchhave, Lars A; Cohen, Ofer; Ehrenreich, David; García Muñoz, Antonio; Henry, Gregory W; Knutson, Heather; Lavvas, Panayotis; Etangs, Alain Lecavelier des; Lewis, Nikole K; López-Morales, Mercedes; Mandell, Avi M; Sanz-Forcada, Jorge; Tremblin, Pascal; Lupu, Roxana

    2017-08-02

    Infrared radiation emitted from a planet contains information about the chemical composition and vertical temperature profile of its atmosphere. If upper layers are cooler than lower layers, molecular gases will produce absorption features in the planetary thermal spectrum. Conversely, if there is a stratosphere-where temperature increases with altitude-these molecular features will be observed in emission. It has been suggested that stratospheres could form in highly irradiated exoplanets, but the extent to which this occurs is unresolved both theoretically and observationally. A previous claim for the presence of a stratosphere remains open to question, owing to the challenges posed by the highly variable host star and the low spectral resolution of the measurements. Here we report a near-infrared thermal spectrum for the ultrahot gas giant WASP-121b, which has an equilibrium temperature of approximately 2,500 kelvin. Water is resolved in emission, providing a detection of an exoplanet stratosphere at 5σ confidence. These observations imply that a substantial fraction of incident stellar radiation is retained at high altitudes in the atmosphere, possibly by absorbing chemical species such as gaseous vanadium oxide and titanium oxide.

  11. The impact of a non-uniform land surface on the radiation environment over an Arctic fjord - a study with a 3D radiative transfer model for stratus clouds over the Hornsund fjord, Spitsbergen

    Directory of Open Access Journals (Sweden)

    Izabela Górecka

    2012-11-01

    Full Text Available This paper estimates the influence of land topography and cover on 3D radiativeeffects under overcast skies in the Arctic coastal environment, in particular in theHornsund fjord region, Spitsbergen. The authors focus on the impact of anon-uniform surface on: (1 the spatial distribution of solar fluxesreaching the fjord surface, (2 spectral shortwave cloud radiative forcing atthe fjord surface, (3 the solar flux anomaly at the domain surface resultingfrom the assumption of a uniform surface, i.e. the error due to plane parallelassumptions in climate models, and (4 remote sensing of cloud opticalthickness over the fjord. Their dependence on spectral channel, cloud opticalthickness, cloud type, cloud base height, surface albedo and solar zenithangle is discussed. The analysis is based on Monte Carlo simulations of solarradiation transfer over a heterogeneous surface for selected channels of theMODIS radiometer. The simulations showed a considerable impact of the landsurrounding the fjord on the solar radiation over the fjord. The biggestdifferences between atmospheric transmittances over the fjord surface and over theocean were found for a cloud optical thickness τ = 12, low solar zenith angle θ, high cloud base and snow-covered land. For τ = 12, θ = 53°, cloud base height 1.8 km andwavelength λ = 469 nm, the enhancement in irradiance transmittanceover the fjord was 0.19 for the inner fjords and 0.10 for the whole fjord(λ = 469 nm. The land surrounding the Hornsund fjord also hada considerable impact on the spectral cloud radiative forcing on the fjordsurface and the solar flux anomaly at the domain surface due to the uniformsurface assumption. For the mouth and central part of the fjord the error dueto the use of channel 2 of the MODIS radiometer (λ = 858 nm forcloud optical thickness retrieval was < 1 in the case of low-level clouds(cloud base height 1 km, nadir radiance, θ = 53°, cloudoptical thickness retrieved solely from MODIS

  12. Stratospheric Ozone Distribution and Tropospheric General Circulation: Interconnections in the UTLS Region

    Science.gov (United States)

    Barodka, S.; Krasovsky, A.; Shalamyansky, A.

    2014-12-01

    The height of the tropopause, which divided the stratosphere and the troposphere, is a result of two rival categories of processes: the tropospheric vertical convection and the radiative heating of the stratosphere resulting from the ozone cycle. Hence, it is natural that tropospheric and stratospheric phenomena can have effect each other in manifold processes of stratosphere-troposphere interactions. In the present study we focus our attention to the "top-down" side of the interaction: the impact of stratospheric ozone distribution on the features of tropospheric circulation and the associated weather patterns and regional climate conditions. We proceed from analyzes of the observational data performed at the A.I. Voeikov Main Geophysical Observatory, which suggest a distinct correlation between stratospheric ozone distribution, synoptic formations and air-masses boundaries in the upper troposphere and the temperature field of the lower stratosphere [1]. Furthermore, we analyze local features of atmospheric general circulation and stratospheric ozone distribution from the atmospheric reanalyses and general circulation model data, focusing our attention to instantaneous positions of subtropical and polar stationary atmospheric fronts, which define regional characteristics of the general circulation cells in the troposphere and separate global tropospheric air-masses, correspond to distinct meteorological regimes in the TOC field [2, 3]. We assume that by altering the tropopause height, stratospheric ozone-related processes can have an impact on the location of the stationary atmospheric fronts, thereby exerting influence on circulation processes in troposphere and lower stratosphere. For midlatitudes, the tropopause height controls the position of the polar stationary front, which has a direct impact on the trajectory of motion of active vortices on synoptic tropospheric levels, thereby controlling weather patterns in that region and the regional climate. This

  13. SWIFT: Semi-empirical and numerically efficient stratospheric ozone chemistry for global climate models

    OpenAIRE

    Kreyling, Daniel; Wohltmann, Ingo; Lehmann, Ralph; Rex, Markus

    2015-01-01

    The SWIFT model is a fast yet accurate chemistry scheme for calculating the chemistry of stratospheric ozone. It is mainly intended for use in Global Climate Models (GCMs), Chemistry Climate Models (CCMs) and Earth System Models (ESMs). For computing time reasons these models often do not employ full stratospheric chem- istry modules, but use prescribed ozone instead. This can lead to insufficient representation between stratosphere and troposphere. The SWIFT stratospheric ozone chem...

  14. Forcing of stratospheric chemistry and dynamics during the Dalton Minimum

    Science.gov (United States)

    Anet, J. G.; Muthers, S.; Rozanov, E.; Raible, C. C.; Peter, T.; Stenke, A.; Shapiro, A. I.; Beer, J.; Steinhilber, F.; Brönnimann, S.; Arfeuille, F.; Brugnara, Y.; Schmutz, W.

    2013-11-01

    The response of atmospheric chemistry and dynamics to volcanic eruptions and to a decrease in solar activity during the Dalton Minimum is investigated with the fully coupled atmosphere-ocean chemistry general circulation model SOCOL-MPIOM (modeling tools for studies of SOlar Climate Ozone Links-Max Planck Institute Ocean Model) covering the time period 1780 to 1840 AD. We carried out several sensitivity ensemble experiments to separate the effects of (i) reduced solar ultra-violet (UV) irradiance, (ii) reduced solar visible and near infrared irradiance, (iii) enhanced galactic cosmic ray intensity as well as less intensive solar energetic proton events and auroral electron precipitation, and (iv) volcanic aerosols. The introduced changes of UV irradiance and volcanic aerosols significantly influence stratospheric dynamics in the early 19th century, whereas changes in the visible part of the spectrum and energetic particles have smaller effects. A reduction of UV irradiance by 15%, which represents the presently discussed highest estimate of UV irradiance change caused by solar activity changes, causes global ozone decrease below the stratopause reaching as much as 8% in the midlatitudes at 5 hPa and a significant stratospheric cooling of up to 2 °C in the mid-stratosphere and to 6 °C in the lower mesosphere. Changes in energetic particle precipitation lead only to minor changes in the yearly averaged temperature fields in the stratosphere. Volcanic aerosols heat the tropical lower stratosphere, allowing more water vapour to enter the tropical stratosphere, which, via HOx reactions, decreases upper stratospheric and mesospheric ozone by roughly 4%. Conversely, heterogeneous chemistry on aerosols reduces stratospheric NOx, leading to a 12% ozone increase in the tropics, whereas a decrease in ozone of up to 5% is found over Antarctica in boreal winter. The linear superposition of the different contributions is not equivalent to the response obtained in a simulation

  15. Rain-shadow: An area harboring "Gray Ocean" clouds

    Science.gov (United States)

    Padmakumari, B.; Maheskumar, R. S.; Harikishan, G.; Morwal, S. B.; Kulkarni, J. R.

    2018-06-01

    The characteristics of monsoon convective clouds over the rain-shadow region of north peninsular India have been investigated using in situ aircraft cloud microphysical observations collected during Cloud Aerosol Interaction and Precipitation Enhancement EXperiment (CAIPEEX). The parameters considered for characterization are: liquid water content (LWC), cloud vertical motion (updraft, downdraft: w), cloud droplet number concentration (CDNC) and effective radius (Re). The results are based on 15 research flights which were conducted from the base station Hyderabad during summer monsoon season. The clouds studied were developing congestus. The clouds have low CDNC and low updraft values resembling the oceanic convective clouds. The super-saturation in clouds is found to be low (≤0.2%) due to low updrafts. The land surface behaves like ocean surface during monsoon as deduced from Bowen ratio. Microphysically the clouds showed oceanic characteristics. However, these clouds yield low rainfall due to their low efficiency (mean 14%). The cloud parameters showed a large variability; hence their characteristic values are reported in terms of median values. These values will serve the numerical models for rainfall simulations over the region and also will be useful as a scientific basis for cloud seeding operations to increase the rainfall efficiency. The study revealed that monsoon convective clouds over the rain-shadow region are of oceanic type over the gray land, and therefore we christen them as "Gray Ocean" clouds.

  16. Imaging gravity waves in lower stratospheric AMSU-A radiances, Part 2: Validation case study

    Directory of Open Access Journals (Sweden)

    S. D. Eckermann

    2006-01-01

    Full Text Available Two-dimensional radiance maps from Channel 9 (~60–90 hPa of the Advanced Microwave Sounding Unit (AMSU-A, acquired over southern Scandinavia on 14 January 2003, show plane-wave-like oscillations with a wavelength λh of ~400–500 km and peak brightness temperature amplitudes of up to 0.9 K. The wave-like pattern is observed in AMSU-A radiances from 8 overpasses of this region by 4 different satellites, revealing a growth in the disturbance amplitude from 00:00 UTC to 12:00 UTC and a change in its horizontal structure between 12:00 UTC and 20:00 UTC. Forecast and hindcast runs for 14 January 2003 using high-resolution global and regional numerical weather prediction (NWP models generate a lower stratospheric mountain wave over southern Scandinavia with peak 90 hPa temperature amplitudes of ~5–7 K at 12:00 UTC and a similar horizontal wavelength, packet width, phase structure and time evolution to the disturbance observed in AMSU-A radiances. The wave's vertical wavelength is ~12 km. These NWP fields are validated against radiosonde wind and temperature profiles and airborne lidar profiles of temperature and aerosol backscatter ratios acquired from the NASA DC-8 during the second SAGE III Ozone Loss and Validation Experiment (SOLVE II. Both the amplitude and phase of the stratospheric mountain wave in the various NWP fields agree well with localized perturbation features in these suborbital measurements. In particular, we show that this wave formed the type II polar stratospheric clouds measured by the DC-8 lidar. To compare directly with the AMSU-A data, we convert these validated NWP temperature fields into swath-scanned brightness temperatures using three-dimensional Channel 9 weighting functions and the actual AMSU-A scan patterns from each of the 8 overpasses of this region. These NWP-based brightness temperatures contain two-dimensional oscillations due to this resolved stratospheric mountain wave that have an amplitude, wavelength

  17. Impact of major volcanic eruptions on stratospheric water vapour

    Directory of Open Access Journals (Sweden)

    M. Löffler

    2016-05-01

    Full Text Available Volcanic eruptions can have a significant impact on the Earth's weather and climate system. Besides the subsequent tropospheric changes, the stratosphere is also influenced by large eruptions. Here changes in stratospheric water vapour after the two major volcanic eruptions of El Chichón in Mexico in 1982 and Mount Pinatubo on the Philippines in 1991 are investigated with chemistry–climate model simulations. This study is based on two simulations with specified dynamics of the European Centre for Medium-Range Weather Forecasts Hamburg – Modular Earth Submodel System (ECHAM/MESSy Atmospheric Chemistry (EMAC model, performed within the Earth System Chemistry integrated Modelling (ESCiMo project, of which only one includes the long-wave volcanic forcing through prescribed aerosol optical properties. The results show a significant increase in stratospheric water vapour induced by the eruptions, resulting from increased heating rates and the subsequent changes in stratospheric and tropopause temperatures in the tropics. The tropical vertical advection and the South Asian summer monsoon are identified as sources for the additional water vapour in the stratosphere. Additionally, volcanic influences on tropospheric water vapour and El Niño–Southern Oscillation (ENSO are evident, if the long-wave forcing is strong enough. Our results are corroborated by additional sensitivity simulations of the Mount Pinatubo period with reduced nudging and reduced volcanic aerosol extinction.

  18. Variability in modeled cloud feedback tied to differences in the climatological spatial pattern of clouds

    Science.gov (United States)

    Siler, Nicholas; Po-Chedley, Stephen; Bretherton, Christopher S.

    2018-02-01

    Despite the increasing sophistication of climate models, the amount of surface warming expected from a doubling of atmospheric CO_2 (equilibrium climate sensitivity) remains stubbornly uncertain, in part because of differences in how models simulate the change in global albedo due to clouds (the shortwave cloud feedback). Here, model differences in the shortwave cloud feedback are found to be closely related to the spatial pattern of the cloud contribution to albedo (α) in simulations of the current climate: high-feedback models exhibit lower (higher) α in regions of warm (cool) sea-surface temperatures, and therefore predict a larger reduction in global-mean α as temperatures rise and warm regions expand. The spatial pattern of α is found to be strongly predictive (r=0.84) of a model's global cloud feedback, with satellite observations indicating a most-likely value of 0.58± 0.31 Wm^{-2} K^{-1} (90% confidence). This estimate is higher than the model-average cloud feedback of 0.43 Wm^{-2} K^{-1}, with half the range of uncertainty. The observational constraint on climate sensitivity is weaker but still significant, suggesting a likely value of 3.68 ± 1.30 K (90% confidence), which also favors the upper range of model estimates. These results suggest that uncertainty in model estimates of the global cloud feedback may be substantially reduced by ensuring a realistic distribution of clouds between regions of warm and cool SSTs in simulations of the current climate.

  19. The natural stratosphere of 1974. CIAP monograph 1. Final report

    International Nuclear Information System (INIS)

    1975-09-01

    The Climatic Impact Assessment Program (CIAP) of the U.S. Department of Transportation is charged with the 'assessment' of the impact of future aircraft fleets and other vehicles operating in, or transiting through, the stratosphere. CIAP monograph 1 gives a survey, largely from an experimental standpoint, of what is known in 1974 about the unperturbed stratosphere with respect to an application to stratospheric flight. It reviews the overall structure of the stratosphere, its origin in terms of ozone photochemistry, solar irradiance and overall radiative energy balance, other chemically reactive minor species, and atmospheric motions on a variety of scales of time and distance. The limitations of our understanding are emphasized in the presentation. Also, the monograph examines briefly what is known about the effect of massive injections of nitrogen oxides (from atmospheric nuclear explosions) and sulfur oxides (from major volcanic eruptions)

  20. The Role of Emissivity in the Detection of Arctic Night Clouds

    Directory of Open Access Journals (Sweden)

    Filomena Romano

    2017-04-01

    Full Text Available Detection of clouds over polar areas from satellite radiometric measurements in the visible and IR atmospheric window region is rather difficult because of the high albedo of snow, possible ice covered surfaces, very low humidity, and the usual presence of atmospheric temperature inversion. Cold and highly reflective polar surfaces provide little thermal and visible contrast between clouds and the background surface. Moreover, due to the presence of temperature inversion, clouds are not always identifiable as being colder than the background. In addition, low humidity often causes polar clouds to be optically thin. Finally, polar clouds are usually composed of a mixture of ice and water, which leads to an unclear spectral signature. Single and bi-spectral threshold methods are sometimes inappropriate due to a large variability of surface emissivity and cloud conditions. The objective of this study is to demonstrate the crucial role played by surface emissivity in the detection of polar winter clouds and the potential improvement offered by infrared hyperspectral observations, such as from the Infrared Atmospheric Sounding Interferometer (IASI. In this paper a new approach for cloud detection is proposed and validated exploiting active measurements from satellite sensors, i.e., the CloudSat cloud profiling radar (CPR and the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP on board the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO. For a homogenous IASI field of view (FOVs, the proposed cloud detection scheme tallies with the combined CPR and CALIOP product in classifying 98.11% of the FOVs as cloudy and also classifies 97.54% of the FOVs as clear. The Hansen Kuipers discriminant reaches 0.95.

  1. The fate of atmospheric phosgene and the stratospheric chlorine loadings of its parent compounds: CCl4, C2Cl4, C2HCL3, CH3CCl3, and CHCl3

    Science.gov (United States)

    Kindler, T. P.; Chameides, W. L.; Wine, P. H.; Cunnold, D. M.; Alyea, F. N.; Franklin, J. A.

    1995-01-01

    A study of the tropospheric and stratospheric cycles of phosgene is carried out to determine its fate and ultimate role in controlling the ozone depletion potentials of its parent compounds. Tropospheric phosgene is produced from the OH-initiated oxidation of C2Cl4, CH3CCl3, CHCl3, and C2HCl3. Simulations using a two-dimensional model indicate that these processes produce about 90 pptv/yr of tropospheric phosgene with an average concentration of about 18 pptv, in reasonable agreement with observations. We estimate a residence time of about 70 days for tropospheric phosgene, with the vast majority being removed by hydrolysis in cloudwater. Only about 0.4% of the phosgene produced in the troposphere avoids wet removal and is transported to the stratosphere, where its chlorine can be released to participate in the catalytic destruction of ozone. Stratospheric phosgene is produced from the photochemical degradation of CCl4, C2Cl4, CHCl3, and CH3CCl3 and is removed by photolysis and downward transport to the troposphere. Model calculations, in good agreement with observations, indicate that these processes produce a peak stratospheric concentration of about 25-30 pptv at an altitude of about 25 km. In contrast to tropospheric phosgene, stratospheric phosgene is found to have a lifetime against photochemical removal of the order of years. As a result, a significant portion of the phosgene that is produced in the stratosphere is ultimately returned to the troposphere, where it is rapidly removed by clouds. This phenomenon effectively decreases the amount of reactive chlorine injected into the stratosphere and available for ozone depletion from phosgene's parent compounds. A similar phenomenon due to the downward transport of stratospheric COFCl produced from CFC-11 is estimated to cause a 7% decrease in the amount of reactive chlorine injected into the stratosphere from this compound. Our results are potentially sensitive to a variety of parameters, most notably the rate

  2. Stratospheric chlorine: Blaming it on nature

    International Nuclear Information System (INIS)

    Taube, G.

    1993-01-01

    Much of the bitter public debate over ozone depletion has centered on the claim that chlorofluorocarbons (CFCs) pale into insignificance alongside natural sources of chlorine in the stratosphere. If so, goes the argument, chlorine could not be depleting ozone as atmospheric scientists claim, because the natural sources have been around since time immemorial, and the ozone layer is still there. The claim, put forward in a book by Rogelio Maduro and Ralf Schauerhammer, has since been touted by former Atomic Energy Commissioner Dixy Lee Ray and talk-show host Rush Limbaugh, and it forms the basis of much of the backlash now being felt by atmospheric scientists. The argument is simple: Maduro and Schauerhammer calculate that 600 million tons of chlorine enters the atmosphere annually from seawater, 36 million tons from volcanoes, 8.4 million tons from biomass burning, and 5 million tons from ocean biota. In contrast, CFCs account for a mere 750,000 tons of atmospheric chlorine a year. Besides disputing the numbers, scientists have both theoretical and observational bases for doubting that much of this chlorine is getting into the stratosphere, where it could affect the ozone layer. Linwood Callis of the National Aeronautics and Space Administration's (NASA) Langley Research Center points out one crucial problem with the argument: Chlorine from natural sources is soluble, and so it gets rained out of the lower atmosphere. CFCs, in contrast, are insoluble and inert and thus make it to the stratosphere to release their chlorine. What's more, observations of stratospheric chemistry don't support the idea that natural sources are contributing much to the chlorine there

  3. Effects of Surface BRDF on the OMI Cloud and NO2 Retrievals: A New Approach Based on Geometry-Dependent Lambertian Equivalent Reflectivity (GLER) Derived from MODIS

    Science.gov (United States)

    Vasilkov, Alexander; Qin, Wenhan; Krotkov, Nickolay; Lamsal, Lok; Spurr, Robert; Haffner, David; Joiner, Joanna; Yang, Eun-Su; Marchenko, Sergey

    2017-01-01

    The Ozone Monitoring Instrument (OMI) cloud and NO2 algorithms use a monthly gridded surface reflectivity climatology that does not depend upon the observation geometry. In reality, reflection of incoming direct and diffuse solar light from land or ocean surfaces is sensitive to the sun sensor geometry. This dependence is described by the bidirectional reflectance distribution function (BRDF). To account for the BRDF, we propose to use a new concept of geometry-dependent Lambertian equivalent reflectivity (GLER). Implementation within the existing OMI cloud and NO2 retrieval infrastructure requires changes only to the input surface reflectivity database. GLER is calculated using a vector radiative transfer model with high spatial resolution BRDF information from MODIS over land and the Cox Munk slope distribution over ocean with a contribution from water-leaving radiance. We compare GLER and climatological LER at 466 nm, which is used in the OMI O2-O2cloud algorithm to derive effective cloud fractions. A detailed comparison of the cloud fractions and pressures derived with climatological and GLERs is carried out. GLER and corresponding retrieved cloud products are then used as input to the OMI NO2 algorithm. We find that replacing the climatological OMI-based LERs with GLERs can increase NO2 vertical columns by up to 50 % in highly polluted areas; the differences include both BRDF effects and biases between the MODIS and OMI-based surface reflectance data sets. Only minor changes to NO2 columns (within 5 %) are found over unpolluted and overcast areas.

  4. NASA/GEWEX Surface Radiation Budget: Integrated Data Product With Reprocessed Radiance, Cloud, and Meteorology Inputs, and New Surface Albedo Treatment

    Science.gov (United States)

    Cox, Stephen J.; Stackhouse, Paul W., Jr.; Gupta, Shashi K.; Mikovitz, J. Colleen; Zhang, Taiping

    2016-01-01

    The NASA/GEWEX Surface Radiation Budget (SRB) project produces shortwave and longwave surface and top of atmosphere radiative fluxes for the 1983-near present time period. Spatial resolution is 1 degree. The current release 3.0 (available at gewex-srb.larc.nasa.gov) uses the International Satellite Cloud Climatology Project (ISCCP) DX product for pixel level radiance and cloud information. This product is subsampled to 30 km. ISCCP is currently recalibrating and recomputing their entire data series, to be released as the H product, at 10km resolution. The ninefold increase in pixel number will allow SRB a higher resolution gridded product (e.g. 0.5 degree), as well as the production of pixel-level fluxes. In addition to the input data improvements, several important algorithm improvements have been made. Most notable has been the adaptation of Angular Distribution Models (ADMs) from CERES to improve the initial calculation of shortwave TOA fluxes, from which the surface flux calculations follow. Other key input improvements include a detailed aerosol history using the Max Planck Institut Aerosol Climatology (MAC), temperature and moisture profiles from HIRS, and new topography, surface type, and snow/ice. Here we present results for the improved GEWEX Shortwave and Longwave algorithm (GSW and GLW) with new ISCCP data, the various other improved input data sets and the incorporation of many additional internal SRB model improvements. As of the time of abstract submission, results from 2007 have been produced with ISCCP H availability the limiting factor. More SRB data will be produced as ISCCP reprocessing continues. The SRB data produced will be released as part of the Release 4.0 Integrated Product, recognizing the interdependence of the radiative fluxes with other GEWEX products providing estimates of the Earth's global water and energy cycle (I.e., ISCCP, SeaFlux, LandFlux, NVAP, etc.).

  5. ASTER cloud coverage reassessment using MODIS cloud mask products

    Science.gov (United States)

    Tonooka, Hideyuki; Omagari, Kunjuro; Yamamoto, Hirokazu; Tachikawa, Tetsushi; Fujita, Masaru; Paitaer, Zaoreguli

    2010-10-01

    In the Advanced Spaceborne Thermal Emission and Reflection radiometer (ASTER) Project, two kinds of algorithms are used for cloud assessment in Level-1 processing. The first algorithm based on the LANDSAT-5 TM Automatic Cloud Cover Assessment (ACCA) algorithm is used for a part of daytime scenes observed with only VNIR bands and all nighttime scenes, and the second algorithm based on the LANDSAT-7 ETM+ ACCA algorithm is used for most of daytime scenes observed with all spectral bands. However, the first algorithm does not work well for lack of some spectral bands sensitive to cloud detection, and the two algorithms have been less accurate over snow/ice covered areas since April 2008 when the SWIR subsystem developed troubles. In addition, they perform less well for some combinations of surface type and sun elevation angle. We, therefore, have developed the ASTER cloud coverage reassessment system using MODIS cloud mask (MOD35) products, and have reassessed cloud coverage for all ASTER archived scenes (>1.7 million scenes). All of the new cloud coverage data are included in Image Management System (IMS) databases of the ASTER Ground Data System (GDS) and NASA's Land Process Data Active Archive Center (LP DAAC) and used for ASTER product search by users, and cloud mask images are distributed to users through Internet. Daily upcoming scenes (about 400 scenes per day) are reassessed and inserted into the IMS databases in 5 to 7 days after each scene observation date. Some validation studies for the new cloud coverage data and some mission-related analyses using those data are also demonstrated in the present paper.

  6. Cloud detection, classification and motion estimation using geostationary satellite imagery for cloud cover forecast

    International Nuclear Information System (INIS)

    Escrig, H.; Batlles, F.J.; Alonso, J.; Baena, F.M.; Bosch, J.L.; Salbidegoitia, I.B.; Burgaleta, J.I.

    2013-01-01

    Considering that clouds are the greatest causes to solar radiation blocking, short term cloud forecasting can help power plant operation and therefore improve benefits. Cloud detection, classification and motion vector determination are key to forecasting sun obstruction by clouds. Geostationary satellites provide cloud information covering wide areas, allowing cloud forecast to be performed for several hours in advance. Herein, the methodology developed and tested in this study is based on multispectral tests and binary cross correlations followed by coherence and quality control tests over resulting motion vectors. Monthly synthetic surface albedo image and a method to reject erroneous correlation vectors were developed. Cloud classification in terms of opacity and height of cloud top is also performed. A whole-sky camera has been used for validation, showing over 85% of agreement between the camera and the satellite derived cloud cover, whereas error in motion vectors is below 15%. - Highlights: ► A methodology for detection, classification and movement of clouds is presented. ► METEOSAT satellite images are used to obtain a cloud mask. ► The prediction of cloudiness is estimated with 90% in overcast conditions. ► Results for partially covered sky conditions showed a 75% accuracy. ► Motion vectors are estimated from the clouds with a success probability of 86%

  7. A theoretical study of rotatable renewable energy system for stratospheric airship

    International Nuclear Information System (INIS)

    Lv, Mingyun; Li, Jun; Zhu, Weiyu; Du, Huafei; Meng, Junhui; Sun, Kangwen

    2017-01-01

    Highlights: • A new rotatable renewable energy system is designed for stratospheric airship. • A theoretical model of optimal rotation angle and required area are studied. • The effects of latitude and date on output energy per day are investigated. • The advantages of the rotatable renewable energy system are studied. - Abstract: Renewable energy system is very critical for solving the energy problem of a long endurance stratospheric airship. Output performance of the traditional solar array fixed on the upper surface of the airship remains to be improved to reduce the area and weight of renewable energy system. Inspired by the solar tracking system and kirigami, a rotatable renewable energy system (mainly including solar array) is designed to improve the current status of the energy system. The advantages of the rotatable solar array are studied using a MATLAB computer program based on the theoretical model established in this paper. The improvements in output energy and required area of the solar array were compared between the traditional airship and improved one. Studies had shown that the rotatable renewable energy system made the total weight of energy system decreased by 1000 kg when the maximum design speed of the airship was greater than 22 m/s. The results demonstrate that the rotatable renewable energy system for the airship can be a good way to improve the output performance of solar array, and the conceptual design and theoretical model suggest a pathway towards solving the energy problem of a stratospheric airship.

  8. Strategies for cloud-top phase determination: differentiation between thin cirrus clouds and snow in manual (ground truth) analyses

    Science.gov (United States)

    Hutchison, Keith D.; Etherton, Brian J.; Topping, Phillip C.

    1996-12-01

    Quantitative assessments on the performance of automated cloud analysis algorithms require the creation of highly accurate, manual cloud, no cloud (CNC) images from multispectral meteorological satellite data. In general, the methodology to create ground truth analyses for the evaluation of cloud detection algorithms is relatively straightforward. However, when focus shifts toward quantifying the performance of automated cloud classification algorithms, the task of creating ground truth images becomes much more complicated since these CNC analyses must differentiate between water and ice cloud tops while ensuring that inaccuracies in automated cloud detection are not propagated into the results of the cloud classification algorithm. The process of creating these ground truth CNC analyses may become particularly difficult when little or no spectral signature is evident between a cloud and its background, as appears to be the case when thin cirrus is present over snow-covered surfaces. In this paper, procedures are described that enhance the researcher's ability to manually interpret and differentiate between thin cirrus clouds and snow-covered surfaces in daytime AVHRR imagery. The methodology uses data in up to six AVHRR spectral bands, including an additional band derived from the daytime 3.7 micron channel, which has proven invaluable for the manual discrimination between thin cirrus clouds and snow. It is concluded that while the 1.6 micron channel remains essential to differentiate between thin ice clouds and snow. However, this capability that may be lost if the 3.7 micron data switches to a nighttime-only transmission with the launch of future NOAA satellites.

  9. Tropical stratospheric water vapor measured by the microwave limb sounder (MLS)

    Science.gov (United States)

    Carr, E. S.; Harwood, R. S.; Mote, P. W.; Peckham, G. E.; Suttie, R. A.; Lahoz, W. A.; O'Neill, A.; Froidevaux, L.; Jarnot, R. F.; Read, W. G.

    1995-01-01

    The lower stratospheric variability of equatorial water vapor, measured by the Microwave Limb Sounder (MLS), follows an annual cycle modulated by the quasi-biennial oscillation. At levels higher in the stratosphere, water vapor measurements exhibit a semi-annual oscillatory signal with the largest amplitudes at 2.2 and 1hPa. Zonal-mean cross sections of MLS water vapor are consistent with previous satellite measurements from the limb infrared monitor of the stratosphere (LIMS) and the stratospheric Aerosol and Gas Experiment 2 (SAGE 2) instruments in that they show water vapor increasing upwards and the polewards from a well defined minimum in the tropics. The minimum values vary in height between the retrieved 46 and 22hPa pressure levels.

  10. Sub-micrometer scale minor element mapping in interplanetary dust particles: a test for stratospheric contamination

    International Nuclear Information System (INIS)

    Flynn, G.J.; Keller, L.P.; Sutton, S.R.

    2006-01-01

    We mapped the spatial distribution of minor elements including K, Mn, and Zn in 3 IDPs and found no evidence for the surface coatings (rims) of these elements that would be expected if the enrichments previously reported were due to contamination. Combined X-ray microprobe (XRM), energy dispersive x-ray fluorescence using a Transmission Electron Microscope (TEM), and electron microprobe measurements have determined that the average bulk chemical composition of the interplanetary dust particles (IDPs) collected from the Earth's stratosphere is enriched relative to the CI meteorite composition by a factor of 2 to 4 for carbon and for the moderately volatile elements Na, K, P, Mn, Cu, Zn, Ga, Ge, and Se, and enriched to ∼30 times CI for Br. However, Jessberger et al., who have reported similar bulk enrichments using Proton Induced X-ray Emission (PIXE), attribute the enrichments to contamination by meteor-derived atmospheric aerosols during the several weeks these IDPs reside in the Earth's atmosphere prior to collection. Using scanning Auger spectroscopy, a very sensitive surface analysis technique, Mackinnon and Mogk have observed S contamination on the surface of IDPs, presumably due to the accretion of sulfate aerosols during stratospheric residence. But the S-rich layer they detected was so thin (∼100 angstroms thick) that the total amount of S on the surface was too small to significantly perturb the bulk S-content of a chondritic IDP. Stephan et al. provide support for the contamination hypothesis by reporting the enrichment of Br on the edges of the IDPs using Time-of-Flight Secondary-Ion Mass-Spectrometry (TOF-SIMS), but TOF-SIMS is notorious for producing false edge-effects, particularly on irregularly-shaped samples like IDPs. Sutton et al. mapped the spatial distribution of Fe, Ni, Zn, Br, and Sr, at the ∼2 (micro)m scale, in four IDPs using element-specific x-ray fluorescence (XRF) computed microtomography. They found the moderately volatile

  11. A refined method for calculating equivalent effective stratospheric chlorine

    Science.gov (United States)

    Engel, Andreas; Bönisch, Harald; Ostermöller, Jennifer; Chipperfield, Martyn P.; Dhomse, Sandip; Jöckel, Patrick

    2018-01-01

    Chlorine and bromine atoms lead to catalytic depletion of ozone in the stratosphere. Therefore the use and production of ozone-depleting substances (ODSs) containing chlorine and bromine is regulated by the Montreal Protocol to protect the ozone layer. Equivalent effective stratospheric chlorine (EESC) has been adopted as an appropriate metric to describe the combined effects of chlorine and bromine released from halocarbons on stratospheric ozone. Here we revisit the concept of calculating EESC. We derive a refined formulation of EESC based on an advanced concept of ODS propagation into the stratosphere and reactive halogen release. A new transit time distribution is introduced in which the age spectrum for an inert tracer is weighted with the release function for inorganic halogen from the source gases. This distribution is termed the release time distribution. We show that a much better agreement with inorganic halogen loading from the chemistry transport model TOMCAT is achieved compared with using the current formulation. The refined formulation shows EESC levels in the year 1980 for the mid-latitude lower stratosphere, which are significantly lower than previously calculated. The year 1980 is commonly used as a benchmark to which EESC must return in order to reach significant progress towards halogen and ozone recovery. Assuming that - under otherwise unchanged conditions - the EESC value must return to the same level in order for ozone to fully recover, we show that it will take more than 10 years longer than estimated in this region of the stratosphere with the current method for calculation of EESC. We also present a range of sensitivity studies to investigate the effect of changes and uncertainties in the fractional release factors and in the assumptions on the shape of the release time distributions. We further discuss the value of EESC as a proxy for future evolution of inorganic halogen loading under changing atmospheric dynamics using simulations from

  12. Accounting for the Effects of Surface BRDF on Satellite Cloud and Trace-Gas Retrievals: A New Approach Based on Geometry-Dependent Lambertian-Equivalent Reflectivity Applied to OMI Algorithms

    Science.gov (United States)

    Vasilkov, Alexander; Qin, Wenhan; Krotkov, Nickolay; Lamsal, Lok; Spurr, Robert; Haffner, David; Joiner, Joanna; Yang, Eun-Su; Marchenko, Sergey

    2017-01-01

    Most satellite nadir ultraviolet and visible cloud, aerosol, and trace-gas algorithms make use of climatological surface reflectivity databases. For example, cloud and NO2 retrievals for the Ozone Monitoring Instrument (OMI) use monthly gridded surface reflectivity climatologies that do not depend upon the observation geometry. In reality, reflection of incoming direct and diffuse solar light from land or ocean surfaces is sensitive to the sun-sensor geometry. This dependence is described by the bidirectional reflectance distribution function (BRDF). To account for the BRDF, we propose to use a new concept of geometry-dependent Lambertian equivalent reflectivity (LER). Implementation within the existing OMI cloud and NO2 retrieval infrastructure requires changes only to the input surface reflectivity database. The geometry-dependent LER is calculated using a vector radiative transfer model with high spatial resolution BRDF information from the Moderate Resolution Imaging Spectroradiometer (MODIS) over land and the Cox-Munk slope distribution over ocean with a contribution from water-leaving radiance. We compare the geometry-dependent and climatological LERs for two wavelengths, 354 and 466 nm, that are used in OMI cloud algorithms to derive cloud fractions. A detailed comparison of the cloud fractions and pressures derived with climatological and geometry-dependent LERs is carried out. Geometry-dependent LER and corresponding retrieved cloud products are then used as inputs to our OMI NO2 algorithm. We find that replacing the climatological OMI-based LERs with geometry-dependent LERs can increase NO2 vertical columns by up to 50% in highly polluted areas; the differences include both BRDF effects and biases between the MODIS and OMI-based surface reflectance data sets. Only minor changes to NO2 columns (within 5 %) are found over unpolluted and overcast areas.

  13. Accounting for the effects of surface BRDF on satellite cloud and trace-gas retrievals: a new approach based on geometry-dependent Lambertian equivalent reflectivity applied to OMI algorithms

    Science.gov (United States)

    Vasilkov, Alexander; Qin, Wenhan; Krotkov, Nickolay; Lamsal, Lok; Spurr, Robert; Haffner, David; Joiner, Joanna; Yang, Eun-Su; Marchenko, Sergey

    2017-01-01

    Most satellite nadir ultraviolet and visible cloud, aerosol, and trace-gas algorithms make use of climatological surface reflectivity databases. For example, cloud and NO2 retrievals for the Ozone Monitoring Instrument (OMI) use monthly gridded surface reflectivity climatologies that do not depend upon the observation geometry. In reality, reflection of incoming direct and diffuse solar light from land or ocean surfaces is sensitive to the sun-sensor geometry. This dependence is described by the bidirectional reflectance distribution function (BRDF). To account for the BRDF, we propose to use a new concept of geometry-dependent Lambertian equivalent reflectivity (LER). Implementation within the existing OMI cloud and NO2 retrieval infrastructure requires changes only to the input surface reflectivity database. The geometry-dependent LER is calculated using a vector radiative transfer model with high spatial resolution BRDF information from the Moderate Resolution Imaging Spectroradiometer (MODIS) over land and the Cox-Munk slope distribution over ocean with a contribution from water-leaving radiance. We compare the geometry-dependent and climatological LERs for two wavelengths, 354 and 466 nm, that are used in OMI cloud algorithms to derive cloud fractions. A detailed comparison of the cloud fractions and pressures derived with climatological and geometry-dependent LERs is carried out. Geometry-dependent LER and corresponding retrieved cloud products are then used as inputs to our OMI NO2 algorithm. We find that replacing the climatological OMI-based LERs with geometry-dependent LERs can increase NO2 vertical columns by up to 50 % in highly polluted areas; the differences include both BRDF effects and biases between the MODIS and OMI-based surface reflectance data sets. Only minor changes to NO2 columns (within 5 %) are found over unpolluted and overcast areas.

  14. Improved stratospheric atmosphere forecasts in the general circulation model through a methane oxidation parametrization

    Science.gov (United States)

    Wang, S.; Jun, Z.

    2017-12-01

    Climatic characteristics of tropical stratospheric methane have been well researched using various satellite data, and numerical simulations have furtherly conducted using chemical climatic models, while the impact of stratospheric methane oxidation on distribution of water vapor is not paid enough attention in general circulation models. Simulated values of water vapour in the tropical upper stratosphere, and throughout much of the extratropical stratosphere, were too low. Something must be done to remedy this deficiency in order to producing realistic stratospheric water vapor using a general circulation model including the whole stratosphere. Introduction of a simple parametrization of the upper-stratospheric moisture source due to methane oxidation and a sink due to photolysis in the mesosphere was conducted. Numerical simulations and analysis of the influence of stratospheric methane on the prediction of tropical stratospheric moisture and temperature fields were carried out. This study presents the advantages of methane oxidation parametrization in producing a realistic distribution of water vapour in the tropical stratosphere and analyzes the impact of methane chemical process on the general circulation model using two storm cases including a heavy rain in South China and a typhoon caused tropical storm.It is obvious that general circulation model with methane oxidation parametrization succeeds in simulating the water vapor and temperature in stratosphere. The simulating rain center value of contrast experiment is increased up to 10% than that of the control experiment. Introduction of methane oxidation parametrization has modified the distribution of water vapour and then producing a broadly realistic distribution of temperature. Objective weather forecast verifications have been performed using simulating results of one month, which demonstrate somewhat positive effects on the model skill. There is a certain extent impact of methane oxidation

  15. Changes in ultraviolet radiation reaching the earth's surface

    International Nuclear Information System (INIS)

    Madronich, S.; McKenzie, R.L.; Caldwell, M.M.; Bjorn, L.O.

    1995-01-01

    The quality and quantity of UV measurements have increased greatly in the last few years. Variations among measurements from different instruments are diminishing toward the 5 level. Long-term trend detection is still a problem, with little historical data available for baseline estimations. Enhanced UV levels are clearly associated with the antartic springtime ozone reductions. Measurements show that maximum UV levels at the South Pole are reached well before the summer solstice, and DNA-damaging radiation at Palmer Station, Antarctica (64§S) during the springtime ozone depletion can exceed maximum summer values at San Diego, USA (32§N). UV increases al mid-latitudes are smaller. However, increases associated with the record low ozone column of 1992-93 in the Northern Hemisphere are evident when examined on a wavelength-specific basis. Measurements in Argentina, Chile, New Zealand, and Australia show relatively high spheric latitudes, with differences in both stratospheric ozone and tropospheric pollutants likely to be playing a role. Tropospheric ozone and aerosols can reduce global UV-B irradiances appreciably. At some locations, tropospheric pollution has increased since pre-industrial times, leading to decreases in surface UV radiation. However, recent trends in tropospheric pollution probably had only minor effects on UV trends relative to the effect of stratospheric ozone reductions. Global ozone measurements from satellites over the period 1979-1993 imply significant UV-B increases at high and mid-latitudes of both hemispheres, but only small changes in the tropics. Such estimates however assume that cloud cover and tropospheric pollution have remained constant over this time period. Under the current CFC phase-out schedules, global UV levels are predicted to peak around the turn of the century in association with peak loading of chlorine in the stratosphere and the concomitant ozone reductions. The recovery to pre-ozone depletion levels is expected to

  16. Methanogenesis, Mesospheric Clouds, and Global Habitability

    Science.gov (United States)

    Pueschel, Rudolf F.; Condon, Estelle P. (Technical Monitor)

    2000-01-01

    Hyperthermophilic methanogens can exist in a deep hot biosphere up to 110 C, or 10 km deep. Methane (CH4) itself is thermodynamically stable to depths of 300 km. Geologic (microbial plus abiogenic thermal) methane is transported upward, attested to by its association with helium, to form petroleum pools. Near or at the surface, geologic CH4 mixes with other natural and with anthropogenic CH4 yielding annual emissions into the atmosphere of 500 Tg, of which 200 Tg are natural and 300 Tg are man-made. The atmospheric lifetime of CH4, a greenhouse gas 20 times more effective than CO2 in raising global temperatures, is approximately 10 years. It is removed from the atmosphere mainly by reactions with hydroxyl radical (OH) to form CO2, but also by dry soil and by conversion to H2O in the stratosphere and middle atmosphere. A sudden rise in atmospheric temperatures by 9-12 C some 55 million years ago has been explained by the release in a few thousand years of three trillion tons of CH4 out of 15 trillion tons that had formed beneath the sea floor. What prevented this CH4-induced greenhouse effect from running away? An analog to the CH4-burp of 55 million years ago is the CH4-doubling over the past century which resulted in a increase in upper level H2O from 4.3 ppmv to 6 ppmv. This 30% increase in H2O vapor yielded a tenfold increase in brightness of polar mesospheric clouds because of a strong dependence of the ice particle nucleation rate on the water saturation ratios. Models show that at a given temperature the optical depth of mesospheric clouds scales as [H2O]beta with beta varying between 4 and 8. Radiative transfer tools applied to mesospheric particles suggest that an optical depth of approximately one, or 1000 times the current mesospheric cloud optical depth, would result in tropospheric cooling of about 10 K. Assuming beta=6, a thousandfold increase in optical thickness would require a three-fold increase of H2O, or a 20-fold increase of CH4. At the current

  17. Efforts to reduce stratospheric ozone loss affect agriculture

    International Nuclear Information System (INIS)

    Weare, B.C.

    1995-01-01

    Research has shown that the increased ultraviolet radiation reaching the Earth's surface resulting from stratospheric ozone loss poses a danger to everyone. Concern about ozone loss prompted many nations to ratify the Montreal Protocol, the most comprehensive international environmental agreement ever enacted. Several provisions of this protocol will have substantial, long-term effects on the agricultural industry. Agriculture contributes substantially to ozone depletion, primarily through its use of chlorofluorocarbons (CFCs) for refrigeration in processing, storage and transport of meats and produce. This paper is meant to serve as an overview of the scientific basis for ozone depletion concerns, a description of the current international policy agreement, and the possible consequences of that policy for agriculture. (author)

  18. Comparison of Cloud Properties from CALIPSO-CloudSat and Geostationary Satellite Data

    Science.gov (United States)

    Nguyen, L.; Minnis, P.; Chang, F.; Winker, D.; Sun-Mack, S.; Spangenberg, D.; Austin, R.

    2007-01-01

    Cloud properties are being derived in near-real time from geostationary satellite imager data for a variety of weather and climate applications and research. Assessment of the uncertainties in each of the derived cloud parameters is essential for confident use of the products. Determination of cloud amount, cloud top height, and cloud layering is especially important for using these real -time products for applications such as aircraft icing condition diagnosis and numerical weather prediction model assimilation. Furthermore, the distribution of clouds as a function of altitude has become a central component of efforts to evaluate climate model cloud simulations. Validation of those parameters has been difficult except over limited areas where ground-based active sensors, such as cloud radars or lidars, have been available on a regular basis. Retrievals of cloud properties are sensitive to the surface background, time of day, and the clouds themselves. Thus, it is essential to assess the geostationary satellite retrievals over a variety of locations. The availability of cloud radar data from CloudSat and lidar data from CALIPSO make it possible to perform those assessments over each geostationary domain at 0130 and 1330 LT. In this paper, CloudSat and CALIPSO data are matched with contemporaneous Geostationary Operational Environmental Satellite (GOES), Multi-functional Transport Satellite (MTSAT), and Meteosat-8 data. Unlike comparisons with cloud products derived from A-Train imagers, this study considers comparisons of nadir active sensor data with off-nadir retrievals. These matched data are used to determine the uncertainties in cloud-top heights and cloud amounts derived from the geostationary satellite data using the Clouds and the Earth s Radiant Energy System (CERES) cloud retrieval algorithms. The CERES multi-layer cloud detection method is also evaluated to determine its accuracy and limitations in the off-nadir mode. The results will be useful for

  19. Models of gas-grain chemistry in interstellar cloud cores with a stochastic approach to surface chemistry

    Science.gov (United States)

    Stantcheva, T.; Herbst, E.

    2004-08-01

    We present a gas-grain model of homogeneous cold cloud cores with time-independent physical conditions. In the model, the gas-phase chemistry is treated via rate equations while the diffusive granular chemistry is treated stochastically. The two phases are coupled through accretion and evaporation. A small network of surface reactions accounts for the surface production of the stable molecules water, formaldehyde, methanol, carbon dioxide, ammonia, and methane. The calculations are run for a time of 107 years at three different temperatures: 10 K, 15 K, and 20 K. The results are compared with those produced in a totally deterministic gas-grain model that utilizes the rate equation method for both the gas-phase and surface chemistry. The results of the different models are in agreement for the abundances of the gaseous species except for later times when the surface chemistry begins to affect the gas. The agreement for the surface species, however, is somewhat mixed. The average abundances of highly reactive surface species can be orders of magnitude larger in the stochastic-deterministic model than in the purely deterministic one. For non-reactive species, the results of the models can disagree strongly at early times, but agree to well within an order of magnitude at later times for most molecules. Strong exceptions occur for CO and H2CO at 10 K, and for CO2 at 20 K. The agreement seems to be best at a temperature of 15 K. As opposed to the use of the normal rate equation method of surface chemistry, the modified rate method is in significantly better agreement with the stochastic-deterministic approach. Comparison with observations of molecular ices in dense clouds shows mixed agreement.

  20. On polluted by admixtures plasma cloud state diagnostics

    International Nuclear Information System (INIS)

    Temko, S.W.; Temko, K.W.; Kuz'min, S.K.

    1993-01-01

    The state of bounded plasma is dependent on perturbations which are caused from changing of inner and outer thermodynamical parameters. The authors describe interactions in a plasma cloud by potential functions. Potential functions are mathematical models of real interactions of particles with each others and with ionized cloud surface. Potential functions define potential energy of corresponding interactions at ionized cloud. Potential functions are sums of far-action and near-action potentials. An ionized cloud is formed under action of inner, outer and surface forces nearly connected with each others. The result of the indicated forces joint action is geometrical form and dimensions of the weakly ionized plasma cloud. Geometrical form of the cloud and its dimensions are able to be changed. They consider only the small changing of small perturbations type. Surface geometrical form and dimensions of the cloud are not given a priori. They are to be obtained by self-consistent problem solving. The self-consistent problem is solved by space non-linear statistical thermodynamics proposed before by the authors. They use abstract potential theory, distribution theory, results by N.M. Krylov and N.N. Bogoljubov and known N.N. Bogoljubov methods of statistical physics. To choose potential functions, their numerical parameters, surface form and dimensions of the cloud, they use optimal experiment planning, likelihood method, Monte-Carlo, directed random search and computer experiment methods. To be likelihood function they used free energy of ionized cloud with admixtures. They refuse describing single particle behavior at small volume. They consider particles to be washed spots and describe particles by distributions. According to R. Feinman it is lawful. Bounded plasma state is described by vector-density of particles distribution. Term distribution is used in Sobolev-Schwartc sence. To precipitate admixtures is effective ultrasound coagulation

  1. Planning, Implementation, and Scientific Goals of the Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS) Field Missions

    Science.gov (United States)

    Toon, Owen B.; Maring, Hal; Dibb, Jack; Ferrare, Richard A.; Jacob, Daniel J.; Jensen, Eric J.; Luo, Z. Johnny; Mace, Gerald G.; Pan, Laura L.; Pfister, Leonhard; hide

    2016-01-01

    The Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS) field mission based at Ellington Field, Texas, during August and September 2013 employed the most comprehensive airborne payload to date to investigate atmospheric composition over North America. The NASA ER-2, DC-8, and SPEC Inc. Learjet flew 57 science flights from the surface to 20 km. The ER-2 employed seven remote sensing instruments as a satellite surrogate and eight in situ instruments. The DC-8 employed 23 in situ and five remote sensing instruments for radiation, chemistry, and microphysics. The Learjet used 11 instruments to explore cloud microphysics. SEAC4RS launched numerous balloons, augmented Aerosol RObotic NETwork, and collaborated with many existing ground measurement sites. Flights investigating convection included close coordination of all three aircraft. Coordinated DC-8 and ER-2 flights investigated the optical properties of aerosols, the influence of aerosols on clouds, and the performance of new instruments for satellite measurements of clouds and aerosols. ER-2 sorties sampled stratospheric injections of water vapor and other chemicals by local and distant convection. DC-8 flights studied seasonally evolving chemistry in the Southeastern U.S., atmospheric chemistry with lower emissions of NOx and SO2 than in previous decades, isoprene chemistry under high and low NOx conditions at different locations, organic aerosols, air pollution near Houston and in petroleum fields, smoke from wildfires in western forests and from agricultural fires in the Mississippi Valley, and the ways in which the chemistry in the boundary layer and the upper troposphere were influenced by vertical transport in convective clouds.

  2. A radiation closure study of Arctic stratus cloud microphysical properties using the collocated satellite-surface data and Fu-Liou radiative transfer model

    Science.gov (United States)

    Dong, Xiquan; Xi, Baike; Qiu, Shaoyue; Minnis, Patrick; Sun-Mack, Sunny; Rose, Fred

    2016-09-01

    Retrievals of cloud microphysical properties based on passive satellite imagery are especially difficult over snow-covered surfaces because of the bright and cold surface. To help quantify their uncertainties, single-layered overcast liquid-phase Arctic stratus cloud microphysical properties retrieved by using the Clouds and the Earth's Radiant Energy System Edition 2 and Edition 4 (CERES Ed2 and Ed4) algorithms are compared with ground-based retrievals at the Atmospheric Radiation Measurement North Slope of Alaska (ARM NSA) site at Barrow, AK, during the period from March 2000 to December 2006. A total of 206 and 140 snow-free cases (Rsfc ≤ 0.3), and 108 and 106 snow cases (Rsfc > 0.3), respectively, were selected from Terra and Aqua satellite passes over the ARM NSA site. The CERES Ed4 and Ed2 optical depth (τ) and liquid water path (LWP) retrievals from both Terra and Aqua are almost identical and have excellent agreement with ARM retrievals under snow-free and snow conditions. In order to reach a radiation closure study for both the surface and top of atmosphere (TOA) radiation budgets, the ARM precision spectral pyranometer-measured surface albedos were adjusted (63.6% and 80% of the ARM surface albedos for snow-free and snow cases, respectively) to account for the water and land components of the domain of 30 km × 30 km. Most of the radiative transfer model calculated SW↓sfc and SW↑TOA fluxes by using ARM and CERES cloud retrievals and the domain mean albedos as input agree with the ARM and CERES flux observations within 10 W m-2 for both snow-free and snow conditions. Sensitivity studies show that the ARM LWP and re retrievals are less dependent on solar zenith angle (SZA), but all retrieved optical depths increase with SZA.

  3. Artificially ionized region as a source of ozone in the stratosphere

    International Nuclear Information System (INIS)

    Gurevich, Aleksandr V; Litvak, Aleksandr G; Vikharev, A L; Ivanov, O A; Borisov, Nikolai D; Sergeichev, Konstantin F

    2000-01-01

    A set of physical and chemical processes occurring in a microwave stratospheric discharge of nanosecond duration is discussed in connection with the effect they may have locally on the ozone layer in the artificially ionized region (AIR) in the stratosphere. The AIR, to be created at altitudes of 18 - 20 km by the microwave breakdown of air with ground-produced powerful electromagnetic wave beams, is planned for use in the natural physical experiment aimed at active monitoring of the ozone layer (its internal state and a set of plasma-chemical and photochemical processes) by controllably generating a considerable amount of ozone in the stratosphere. Results of relevant theoretical studies are presented, as are those of a large series of laboratory experiments performed under conditions similar to those prevailing in the stratosphere. Discharge regimes securing the efficient growth of ozone concentration are identified and studied in detail. It is demonstrated that such a stratospheric ozonizer is about as efficient as the best ground-based ozonizers used at present. For typical stratospheric conditions (low pressures and temperatures T ∼ 200 - 220 K), it is shown that the intense generation of ozone in a microwave breakdown effected by groups of short nanosecond pulses does not virtually increase the density of nitrogen oxides - gases that play a vital role in catalytic ozone-decomposing reactions. The possibility of effectively producing ozone in prebreakdown electric fields is established experimentally. It is demonstrated that due to its long lifetime, ozone produced locally at altitudes of 18 - 20 km may spread widely under the action of winds and turbulent diffusion, thus leading to an additional - artificial - ozonization of the stratosphere. (reviews of topical problems)

  4. Pinatubo Emulation in Multiple Models (POEMs): co-ordinated experiments in the ISA-MIP model intercomparison activity component of the SPARC Stratospheric Sulphur and it's Role in Climate initiative (SSiRC)

    Science.gov (United States)

    Lee, Lindsay; Mann, Graham; Carslaw, Ken; Toohey, Matthew; Aquila, Valentina

    2016-04-01

    The World Climate Research Program's SPARC initiative has a new international activity "Stratospheric Sulphur and its Role in Climate" (SSiRC) to better understand changes in stratospheric aerosol and precursor gaseous sulphur species. One component of SSiRC involves an intercomparison "ISA-MIP" of composition-climate models that simulate the stratospheric aerosol layer interactively. Within PoEMS each modelling group will run a "perturbed physics ensemble" (PPE) of interactive stratospheric aerosol (ISA) simulations of the Pinatubo eruption, varying several uncertain parameters associated with the eruption's SO2 emissions and model processes. A powerful new technique to quantify and attribute sources of uncertainty in complex global models is described by Lee et al. (2011, ACP). The analysis uses Gaussian emulation to derive a probability density function (pdf) of predicted quantities, essentially interpolating the PPE results in multi-dimensional parameter space. Once trained on the ensemble, a Monte Carlo simulation with the fast Gaussian emulator enabling a full variance-based sensitivity analysis. The approach has already been used effectively by Carslaw et al., (2013, Nature) to quantify the uncertainty in the cloud albedo effect forcing from a 3D global aerosol-microphysics model allowing to compare the sensitivy of different predicted quantities to uncertainties in natural and anthropogenic emissions types, and structural parameters in the models. Within ISA-MIP, each group will carry out a PPE of runs, with the subsequent analysis with the emulator assessing the uncertainty in the volcanic forcings predicted by each model. In this poster presentation we will give an outline of the "PoEMS" analysis, describing the uncertain parameters to be varied and the relevance to further understanding differences identified in previous international stratospheric aerosol assessments.

  5. Lidar observations and transfer of stratospheric aerosol over Tomsk in summer period

    Science.gov (United States)

    Novikov, P. V.; Cheremisin, A. A.; Marichev, V. N.; Barashkov, T. O.

    2015-11-01

    The analysis of the stratospheric aerosol origin was carried out by the method of Lagrangian particle trajectories. Stratospheric aerosol was registered by lidar sounding of atmosphere above Tomsk in 2008-2013 in summer time. The analysis of the results had shown that the aerosol content at altitudes of 13-125 km with maximum at 16-18 km can be associated with aerosol transfer from tropical stratospheric reservoir.

  6. Measurement of the Arctic UTLS composition in presence of clouds using millimetre-wave heterodyne spectroscopy

    Directory of Open Access Journals (Sweden)

    E. Castelli

    2013-10-01

    Full Text Available MARSCHALS (Millimetre-wave Airborne Receivers for Spectroscopic CHaracterisation in Atmospheric Limb Sounding is a limb viewing instrument working in the millimetre and sub-millimetre spectral regions (from 294 to 349 GHz. The scientific rationale of MARSCHALS is the study of the Upper Troposphere and Lower Stratosphere region. In March 2010 MARSCHALS was deployed on-board the M-55 Geophysica stratospheric aircraft during the PREMIER(PRocess Exploration through Measurements of Infrared and millimetre-wave Emitted Radiation-Ex field campaign. From the campaign base at Kiruna, Sweden, a research flight to investigate the Arctic atmosphere was conducted. For the first time the instrument fully exploited the three spectral bands. In this paper, we present results of the analysis of MARSCHALS measurements acquired during the PREMIER-Ex flight as processed by the Millimetre-wave Atmospheric Retrieval Code. For the second time after the SCOUT-O3 flight in 2005, MARSCHALS measured vertical distributions of temperature, water vapour, ozone and nitric acid over an altitude range of 4 to 24 km. In addition, vertical profiles of carbon monoxide and nitrous oxide were obtained for the first time. The measurements were performed in clear sky conditions and in presence of low and high altitude clouds (that were able to obscure measurements in the middle infrared spectroscopic region and some information about thick clouds were extracted from the data. The capabilities to derive information on upper tropospheric and lower stratospheric vertical profiles of temperature and minor constituents from millimetre-wave limb sounding observations in the northern polar region are presented and discussed for each of the individual targets. The results of MARSCHALS data analysis contributed to demonstrate the scientific relevance and technical feasibility of millimetre-wave limb-sounding of the UTLS proposed for the ESA Earth Explorer 7 candidate Core Mission PREMIER

  7. The Role of the Stratosphere in Explosive Deepening of Extratropical Cyclones

    Science.gov (United States)

    Knippertz, Peter; Wilbraham, Robert; Trzeciak, Tomek; Owen, Jenny; Odell, Luke; Fink, Andreas H.; Pinto, Joaquim G.

    2014-05-01

    Using a combination of an automatic cyclone tracking method and a special version of the classical pressure tendency equation (PTE), changes in surface core pressure of extra-tropical cyclones can be related to contributions from horizontal temperature advection, vertical motion and diabatic processes, i.e. mainly latent heat release in clouds. Here, the PTE is evaluated in 3°x3° boxes located over the cyclone positions at 6-hourly basis, thus following the movement of a given storm at each time step. PTE calculations are performed from the surface to 100 hPa. Previous work has shown that this approach can be used to quantify the contribution of diabatic processes to cyclone deepening in an automated way, and can easily be applied to large gridded datasets, in this case ERA-Interim reanalyses. In order to close the mass budget in the PTE, geopotential height tendencies at the upper integration boundary (usually 100 hPa) need to be taken into account. Older studies have assumed this term to be negligible, and this has been confirmed with modern re-analysis data for many explosively deepening storms. However, some historical storms show a remarkable contribution from this term, indicating a substantial warming of the levels above 100hPa. An outstanding example is the Braer Storm of January 1993, which reached a record minimum core pressure of 914 hPa near Iceland. A stepwise increase of the upper integration boundary reveals that substantial geopotential height tendencies reach above 1 hPa. This unusual behaviour appears to be related to the propagation of a deep planetary wave trough from North America towards the North Atlantic basin. A similar but somewhat less dramatic behaviour was found for cyclone Wiebke. Another interesting example is storm Emma, which managed to sustain substantial deepening rates despite adverse positive geopotential height tendencies at 100 hPa. Future work will include a more robust statistical analysis of this problem and a better

  8. Reduction of photosynthetically active radiation under extreme stratospheric-aerosol loads

    International Nuclear Information System (INIS)

    Gerstl, S.A.W.; Zardecki, A.

    1981-01-01

    The recently published hypothesis that the Cretaceous-Tertiary extinctions might be caused by an obstruction of sunlight is tested by model calculations. First we compute the total mass of stratospheric aerosols under normal atmospheric conditions for four different (measured) aerosol size distributions and vertical profiles. For comparison, the stratospheric dust masses after four volcanic eruptions are also evaluated. Detailed solar radiative transfer calculations are then performed for artificially increased aerosol amounts until the postulated darkness scenario is obtained. Thus we find that a total stratospheric aerosol mass between 1 and 4 times 10 16 g is sufficient to reduce photosynthesis to 10 3 of normal. We also infer from this result that the impact of a 0.4- to 3-km-diameter asteroid or a close encounter with a Halley-size comet may deposit that amount of particulates into the stratosphere. The darkness scenario of Alvarez et al., is thus shown to be a possible extinction mechanism, even with smaller size asteroids or comets than previously estimated

  9. Reduction of photosynthetically active radiation under extreme stratospheric aerosol loads

    International Nuclear Information System (INIS)

    Gerstl, S.A.W.; Zardecki, A.

    1981-08-01

    The recently published hypothesis that the Cretaceous-Tertiary extinctions might be caused by an obstruction of sunlight is tested by model calculations. First we compute the total mass of stratospheric aerosols under normal atmospheric conditions for four different (measured) aerosol size distributions and vertical profiles. For comparison, the stratospheric dust masses after four volcanic eruptions are also evaluated. Detailed solar radiative transfer calculations are then performed for artificially increased aerosol amounts until the postulated darkness scenario is obtained. Thus we find that a total stratospheric aerosol mass between 1 and 4 times 10 1 g is sufficient to reduce photosynthesis to 10 -3 of normal. We also infer from this result tha the impact of a 0.4- to 3-km-diameter asteroid or a close encounter with a Halley-size comet may deposit that amount of particulates into the stratosphere. The darkness scenario of Alvarez et al. is thus shown to be a possible extinction mechanism, even with smaller size asteroids of comets than previously estimated

  10. Possible effects of volcanic eruptions on stratospheric minor constituent chemistry

    Science.gov (United States)

    Stolarski, R. S.; Butler, D. M.

    1979-01-01

    Although stratosphere penetrating volcanic eruptions have been infrequent during the last half century, periods have existed in the last several hundred years when such eruptions were significantly more frequent. Several mechanisms exist for these injections to affect stratospheric minor constituent chemistry, both on the long-term average and for short-term perturbations. These mechanisms are reviewed and, because of the sensitivity of current models of stratospheric ozone to chlorine perturbations, quantitative estimates are made of chlorine injection rates. It is found that, if chlorine makes up as much as 0.5 to 1% of the gases released and if the total gases released are about the same magnitude as the fine ash, then a major stratosphere penetrating eruption could deplete the ozone column by several percent. The estimate for the Agung eruption of 1963 is just under 1% an amount not excluded by the ozone record but complicated by the peak in atmospheric nuclear explosions at about the same time.

  11. The annual cycle of stratospheric water vapor in a general circulation model

    Science.gov (United States)

    Mote, Philip W.

    1995-01-01

    The application of general circulation models (GCM's) to stratospheric chemistry and transport both permits and requires a thorough investigation of stratospheric water vapor. The National Center for Atmospheric Research has redesigned its GCM, the Community Climate Model (CCM2), to enable studies of the chemistry and transport of tracers including water vapor; the importance of water vapor to the climate and chemistry of the stratosphere requires that it be better understood in the atmosphere and well represented in the model. In this study, methane is carried as a tracer and converted to water; this simple chemistry provides an adequate representation of the upper stratospheric water vapor source. The cold temperature bias in the winter polar stratosphere, which the CCM2 shares with other GCM's, produces excessive dehydration in the southern hemisphere, but this dry bias can be ameliorated by setting a minimum vapor pressure. The CCM2's water vapor distribution and seasonality compare favorably with observations in many respects, though seasonal variations including the upper stratospheric semiannual oscillation are generally too small. Southern polar dehydration affects midlatitude water vapor mixing ratios by a few tenths of a part per million, mostly after the demise of the vortex. The annual cycle of water vapor in the tropical and northern midlatitude lower stratosphere is dominated by drying at the tropical tropopause. Water vapor has a longer adjustment time than methane and had not reached equilibrium at the end of the 9 years simulated here.

  12. Update of the Polar SWIFT model for polar stratospheric ozone loss (Polar SWIFT version 2)

    Science.gov (United States)

    Wohltmann, Ingo; Lehmann, Ralph; Rex, Markus

    2017-07-01

    The Polar SWIFT model is a fast scheme for calculating the chemistry of stratospheric ozone depletion in polar winter. It is intended for use in global climate models (GCMs) and Earth system models (ESMs) to enable the simulation of mutual interactions between the ozone layer and climate. To date, climate models often use prescribed ozone fields, since a full stratospheric chemistry scheme is computationally very expensive. Polar SWIFT is based on a set of coupled differential equations, which simulate the polar vortex-averaged mixing ratios of the key species involved in polar ozone depletion on a given vertical level. These species are O3, chemically active chlorine (ClOx), HCl, ClONO2 and HNO3. The only external input parameters that drive the model are the fraction of the polar vortex in sunlight and the fraction of the polar vortex below the temperatures necessary for the formation of polar stratospheric clouds. Here, we present an update of the Polar SWIFT model introducing several improvements over the original model formulation. In particular, the model is now trained on vortex-averaged reaction rates of the ATLAS Chemistry and Transport Model, which enables a detailed look at individual processes and an independent validation of the different parameterizations contained in the differential equations. The training of the original Polar SWIFT model was based on fitting complete model runs to satellite observations and did not allow for this. A revised formulation of the system of differential equations is developed, which closely fits vortex-averaged reaction rates from ATLAS that represent the main chemical processes influencing ozone. In addition, a parameterization for the HNO3 change by denitrification is included. The rates of change of the concentrations of the chemical species of the Polar SWIFT model are purely chemical rates of change in the new version, whereas in the original Polar SWIFT model, they included a transport effect caused by the

  13. Comparison of Cloud and Aerosol Detection between CERES Edition 3 Cloud Mask and CALIPSO Version 2 Data Products

    Science.gov (United States)

    Trepte, Qing; Minnis, Patrick; Sun-Mack, Sunny; Trepte, Charles

    Clouds and aerosol play important roles in the global climate system. Accurately detecting their presence, altitude, and properties using satellite radiance measurements is a crucial first step in determining their influence on surface and top-of-atmosphere radiative fluxes. This paper presents a comparison analysis of a new version of the Clouds and Earth's Radiant Energy System (CERES) Edition 3 cloud detection algorithms using Aqua MODIS data with the recently released Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) Version 2 Vertical Feature Mask (VFM). Improvements in CERES Edition 3 cloud mask include dust detection, thin cirrus tests, enhanced low cloud detection at night, and a smoother transition from mid-latitude to polar regions. For the CALIPSO Version 2 data set, changes to the lidar calibration can result in significant improvements to its identification of optically thick aerosol layers. The Aqua and CALIPSO satellites, part of the A-train satellite constellation, provide a unique opportunity for validating passive sensor cloud and aerosol detection using an active sensor. In this paper, individual comparison cases will be discussed for different types of clouds and aerosols over various surfaces, for daytime and nighttime conditions, and for regions ranging from the tropics to the poles. Examples will include an assessment of the CERES detection algorithm for optically thin cirrus, marine stratus, and polar night clouds as well as its ability to characterize Saharan dust plumes off the African coast. With the CALIPSO lidar's unique ability to probe the vertical structure of clouds and aerosol layers, it provides an excellent validation data set for cloud detection algorithms, especially for polar nighttime clouds.

  14. Influence of carbon dioxide clouds on early martian climate.

    Science.gov (United States)

    Mischna, M A; Kasting, J F; Pavlov, A; Freedman, R

    2000-06-01

    Recent studies have shown that clouds made of carbon dioxide ice may have warmed the surface of early Mars by reflecting not only incoming solar radiation but upwelling IR radiation as well. However, these studies have not treated scattering self-consistently in the thermal IR. Our own calculations, which treat IR scattering properly, confirm these earlier calculations but show that CO2 clouds can also cool the surface, especially if they are low and optically thick. Estimating the actual effect of CO2 clouds on early martian climate will require three-dimensional models in which cloud location, height, and optical depth, as well as surface temperature and pressure, are determined self-consistently. Our calculations further confirm that CO2 clouds should extend the outer boundary of the habitable zone around a star but that there is still a finite limit beyond which above-freezing surface temperatures cannot be maintained by a CO2-H2O atmosphere. For our own Solar System, the absolute outer edge of the habitable zone is at approximately 2.4 AU.

  15. Observation of an unusual mid-stratospheric aerosol layer in the Arctic: possible sources and implications for polar vortex dynamics

    Directory of Open Access Journals (Sweden)

    M. Gerding

    Full Text Available By the beginning of winter 2000/2001, a mysterious stratospheric aerosol layer had been detected by four different Arctic lidar stations. The aerosol layer was observed first on 16 November 2000, at an altitude of about 38 km near Søndre Strømfjord, Greenland (67° N, 51° W and on 19 November 2000, near Andenes, Norway (69°  N, 16°  E. Subsequently, in early December 2000, the aerosol layer was observed near Kiruna, Sweden (68°  N, 21°  E and Ny-Ålesund, Spitsbergen (79°  N, 12°  E. No mid-latitude lidar station observed the presence of aerosols in this altitude region. The layer persisted throughout the winter 2000/2001, at least up to 12 February 2001. In November 2000, the backscatter ratio at a wavelength of 532 nm was up to 1.1, with a FWHM of about 2.5 km. By early February 2001, the layer had sedimented from an altitude of 38 km to about 26 km. Measurements at several wavelengths by the ALOMAR and Koldewey lidars indicate the particle size was between 30 and 50 nm. Depolarisation measurements reveal that the particles in the layer are aspherical, hence solid. In the mid-stratosphere, the ambient atmospheric temperature was too high to support in situ formation or existence of cloud particles consisting of ice or an acid-water solution. Furthermore, in the year 2000 there was no volcanic eruption, which could have injected aerosols into the upper stratosphere. Therefore, other origins of the aerosol, such as meteoroid debris, condensed rocket fuel, or aerosols produced under the influence of charged solar particles, will be discussed in the paper. Trajectory calculations illustrate the path of the aerosol cloud within the polar vortex and are used to link the observations at the different lidar sites. From the descent rate of  the layer and particle sedimentation rates, the mean down-ward motion of air within the polar vortex was estimated to be about 124 m/d between 35 and 30 km, with higher values at the edge of the

  16. Observation of an unusual mid-stratospheric aerosol layer in the Arctic: possible sources and implications for polar vortex dynamics

    Directory of Open Access Journals (Sweden)

    M. Gerding

    2003-04-01

    Full Text Available By the beginning of winter 2000/2001, a mysterious stratospheric aerosol layer had been detected by four different Arctic lidar stations. The aerosol layer was observed first on 16 November 2000, at an altitude of about 38 km near Søndre Strømfjord, Greenland (67° N, 51° W and on 19 November 2000, near Andenes, Norway (69°  N, 16°  E. Subsequently, in early December 2000, the aerosol layer was observed near Kiruna, Sweden (68°  N, 21°  E and Ny-Ålesund, Spitsbergen (79°  N, 12°  E. No mid-latitude lidar station observed the presence of aerosols in this altitude region. The layer persisted throughout the winter 2000/2001, at least up to 12 February 2001. In November 2000, the backscatter ratio at a wavelength of 532 nm was up to 1.1, with a FWHM of about 2.5 km. By early February 2001, the layer had sedimented from an altitude of 38 km to about 26 km. Measurements at several wavelengths by the ALOMAR and Koldewey lidars indicate the particle size was between 30 and 50 nm. Depolarisation measurements reveal that the particles in the layer are aspherical, hence solid. In the mid-stratosphere, the ambient atmospheric temperature was too high to support in situ formation or existence of cloud particles consisting of ice or an acid-water solution. Furthermore, in the year 2000 there was no volcanic eruption, which could have injected aerosols into the upper stratosphere. Therefore, other origins of the aerosol, such as meteoroid debris, condensed rocket fuel, or aerosols produced under the influence of charged solar particles, will be discussed in the paper. Trajectory calculations illustrate the path of the aerosol cloud within the polar vortex and are used to link the observations at the different lidar sites. From the descent rate of  the layer and particle sedimentation rates, the mean down-ward motion of air within the polar vortex was estimated to be about 124 m/d between 35 and 30 km, with higher values at the edge of the

  17. Space-time patterns of trends in stratospheric constituents derived from UARS measurements

    Science.gov (United States)

    Randel, William J.; Wu, Fei; Russell, James M.; Waters, Joe

    1999-02-01

    The spatial and temporal behavior of low-frequency changes (trends) in stratospheric constituents measured by instruments on the Upper Atmosphere Research Satellite (UARS) during 1991-98 is investigated. The data include CH4, H2O, HF, HCl, O3, and NO2 from the Halogen Occultation Experiment (HALOE), and O3, ClO, and HNO3 from the Microwave Limb Sounder (MLS). Time series of global anomalies are analyzed by linear regression and empirical orthogonal function analysis. Each of the constituents show significant linear trends over at least some region of the stratosphere, and the spatial patterns exhibit coupling between the different species. Several of the constituents (namely CH4, H2O, HF, HCl, O3, and NO2) exhibit a temporal change in trend rates, with strong changes prior to 1996 and weaker (or reversed) trends thereafter. Positive trends are observed in upper stratospheric ClO, with a percentage rate during 1993-97 consistent with stratospheric HCl increases and with tropospheric chlorine emission rates. Significant negative trends in ozone in the tropical middle stratosphere are found in both HALOE and MLS data during 1993-97, together with positive trends in the tropics near 25 km. These trends are very different from the decadal-scale ozone trends observed since 1979, and this demonstrates the variability of trends calculated over short time periods. Positive trends in NO2 are found in the tropical middle stratosphere, and spatial coincidence to the observed ozone decreases suggests the ozone is responding to the NO2 increase. Significant negative trends in HNO3 are found in the lower stratosphere of both hemispheres. These coupled signatures offer a fingerprint of chemical evolution in the stratosphere for the UARS time frame.

  18. Plane-parallel biases computed from inhomogeneous Arctic clouds and sea ice

    Science.gov (United States)

    Rozwadowska, Anna; Cahalan, Robert F.

    2002-10-01

    Monte Carlo simulations of the expected influence of nonuniformity in cloud structure and surface albedo on shortwave radiative fluxes in the Arctic atmosphere are presented. In particular, plane-parallel biases in cloud albedo and transmittance are studied for nonabsorbing, low-level, all-liquid stratus clouds over sea ice. The "absolute bias" is defined as the difference between the cloud albedo or transmittance for the uniform or plane-parallel case, and the albedo or transmittance for nonuniform conditions with the same mean cloud optical thickness and the same mean surface albedo, averaged over a given area (i.e., bias > 0 means plane-parallel overestimates). Ranges of means and standard deviations of input parameters typical of Arctic conditions are determined from the First International Satellite Cloud Climatology Project (ISCCP) Regional Experiment Artic Cloud Experiment (FIRE/ACE)/Surface Heat Budget of the Arctic Ocean (SHEBA)/Atmospheric Radiation Measurement Program (ARM) experiment, a cooperative effort of the Department of Energy, NASA, NSF, the National Oceanic and Atmospheric Administration, the Office of Naval Research, and the Atmospheric Environment Service. We determine the sensitivity of the bias with respect to the following: domain averaged means and spatial variances of cloud optical thickness and surface albedo, shape of the surface reflectance function, presence of a scattering layer under the clouds, and solar zenith angle. The simulations show that the biases in Arctic conditions are generally lower than in subtropical stratocumulus. The magnitudes of the absolute biases are unlikely to exceed 0.02 for albedo and 0.05 for transmittance. The "relative bias" expresses the absolute bias as a percentage of the actual cloud albedo or transmittance. The magnitude of the relative bias in albedo is typically below 2% over the reflective Arctic surface, while the magnitude of the relative bias in transmittance can exceed 10%.

  19. ON THE STAR FORMATION RATES IN MOLECULAR CLOUDS

    International Nuclear Information System (INIS)

    Lada, Charles J.; Lombardi, Marco; Alves, Joao F.

    2010-01-01

    In this paper, we investigate the level of star formation activity within nearby molecular clouds. We employ a uniform set of infrared extinction maps to provide accurate assessments of cloud mass and structure and compare these with inventories of young stellar objects within the clouds. We present evidence indicating that both the yield and rate of star formation can vary considerably in local clouds, independent of their mass and size. We find that the surface density structure of such clouds appears to be important in controlling both these factors. In particular, we find that the star formation rate (SFR) in molecular clouds is linearly proportional to the cloud mass (M 0.8 ) above an extinction threshold of A K ∼ 0.8 mag, corresponding to a gas surface density threshold of Σ gas ∼ 116 M sun pc 2 . We argue that this surface density threshold corresponds to a gas volume density threshold which we estimate to be n(H 2 ) ∼ 10 4 cm -3 . Specifically, we find SFR (M sun yr -1 ) = 4.6 ± 2.6 x 10 -8 M 0.8 (M sun ) for the clouds in our sample. This relation between the rate of star formation and the amount of dense gas in molecular clouds appears to be in excellent agreement with previous observations of both galactic and extragalactic star-forming activity. It is likely the underlying physical relationship or empirical law that most directly connects star formation activity with interstellar gas over many spatial scales within and between individual galaxies. These results suggest that the key to obtaining a predictive understanding of the SFRs in molecular clouds and galaxies is to understand those physical factors which give rise to the dense components of these clouds.

  20. Polar clouds and radiation in satellite observations, reanalyses, and climate models

    NARCIS (Netherlands)

    Lenaerts, JTM; Van Tricht, Kristof; Lhermitte, S.L.M.; L'Ecuyer, T.S.

    2017-01-01

    Clouds play a pivotal role in the surface energy budget of the polar regions. Here we use two largely independent data sets of cloud and surface downwelling radiation observations derived by satellite remote sensing (2007–2010) to evaluate simulated clouds and radiation over both polar ice sheets

  1. Equatorial waves in the stratosphere of Uranus

    Science.gov (United States)

    Hinson, David P.; Magalhaes, Julio A.

    1991-01-01

    Analyses of radio occultation data from Voyager 2 have led to the discovery and characterization of an equatorial wave in the Uranus stratosphere. The observed quasi-periodic vertical atmospheric density variations are in close agreement with theoretical predictions for a wave that propagates vertically through the observed background structure of the stratosphere. Quantitative comparisons between measurements obtained at immersion and at emersion yielded constraints on the meridional and zonal structure of the wave; the fact that the two sets of measurements are correlated suggests a wave of planetary scale. Two equatorial wave models are proposed for the wave.

  2. On the detection of the solar signal in the tropical stratosphere

    Directory of Open Access Journals (Sweden)

    G. Chiodo

    2014-06-01

    Full Text Available We investigate the relative role of volcanic eruptions, El Niño–Southern Oscillation (ENSO, and the quasi-biennial oscillation (QBO in the quasi-decadal signal in the tropical stratosphere with regard to temperature and ozone commonly attributed to the 11 \\unit{yr} solar cycle. For this purpose, we perform transient simulations with the Whole Atmosphere Community Climate Model forced from 1960 to 2004 with an 11 yr solar cycle in irradiance and different combinations of other forcings. An improved multiple linear regression technique is used to diagnose the 11 yr solar signal in the simulations. One set of simulations includes all observed forcings, and is thereby aimed at closely reproducing observations. Three idealized sets exclude ENSO variability, volcanic aerosol forcing, and QBO in tropical stratospheric winds, respectively. Differences in the derived solar response in the tropical stratosphere in the four sets quantify the impact of ENSO, volcanic events and the QBO in attributing quasi-decadal changes to the solar cycle in the model simulations. The novel regression approach shows that most of the apparent solar-induced lower-stratospheric temperature and ozone increase diagnosed in the simulations with all observed forcings is due to two major volcanic eruptions (i.e., El Chichón in 1982 and Mt. Pinatubo in 1991. This is caused by the alignment of these eruptions with periods of high solar activity. While it is feasible to detect a robust solar signal in the middle and upper tropical stratosphere, this is not the case in the tropical lower stratosphere, at least in a 45 yr simulation. The present results suggest that in the tropical lower stratosphere, the portion of decadal variability that can be unambiguously linked to the solar cycle may be smaller than previously thought.

  3. Modeling of biomass smoke injection into the lower stratosphere by a large forest fire (Part I: reference simulation

    Directory of Open Access Journals (Sweden)

    J. Trentmann

    2006-01-01

    Full Text Available Wildland fires in boreal regions have the potential to initiate deep convection, so-called pyro-convection, due to their release of sensible heat. Under favorable atmospheric conditions, large fires can result in pyro-convection that transports the emissions into the upper troposphere and the lower stratosphere. Here, we present three-dimensional model simulations of the injection of fire emissions into the lower stratosphere by pyro-convection. These model simulations are constrained and evaluated with observations obtained from the Chisholm fire in Alberta, Canada, in 2001. The active tracer high resolution atmospheric model (ATHAM is initialized with observations obtained by radiosonde. Information on the fire forcing is obtained from ground-based observations of the mass and moisture of the burned fuel. Based on radar observations, the pyro-convection reached an altitude of about 13 km, well above the tropopause, which was located at about 11.2 km. The model simulation yields a similarly strong convection with an overshoot of the convection above the tropopause. The main outflow from the pyro-convection occurs at about 10.6 km, but a significant fraction (about 8% of the emitted mass of the smoke aerosol is transported above the tropopause. In contrast to regular convection, the region with maximum updraft velocity in the pyro-convection is located close to the surface above the fire. This results in high updraft velocities >10 m s−1 at cloud base. The temperature anomaly in the plume decreases rapidly with height from values above 50 K at the fire to about 5 K at about 3000 m above the fire. While the sensible heat released from the fire is responsible for the initiation of convection in the model, the release of latent heat from condensation and freezing dominates the overall energy budget. Emissions of water vapor from the fire do not significantly contribute to the energy budget of the convection.

  4. Long-term trends in stratospheric ozone, temperature, and water vapor over the Indian region

    Science.gov (United States)

    Thankamani Akhil Raj, Sivan; Venkat Ratnam, Madineni; Narayana Rao, Daggumati; Venkata Krishna Murthy, Boddam

    2018-01-01

    We have investigated the long-term trends in and variabilities of stratospheric ozone, water vapor and temperature over the Indian monsoon region using the long-term data constructed from multi-satellite (Upper Atmosphere Research Satellite (UARS MLS and HALOE, 1993-2005), Aura Microwave Limb Sounder (MLS, 2004-2015), Sounding of the Atmosphere using Broadband Emission Radiometry (SABER, 2002-2015) on board TIMED (Thermosphere Ionosphere Mesosphere Energetics Dynamics)) observations covering the period 1993-2015. We have selected two locations, namely, Trivandrum (8.4° N, 76.9° E) and New Delhi (28° N, 77° E), covering northern and southern parts of the Indian region. We also used observations from another station, Gadanki (13.5° N, 79.2° E), for comparison. A decreasing trend in ozone associated with NOx chemistry in the tropical middle stratosphere is found, and the trend turned to positive in the upper stratosphere. Temperature shows a cooling trend in the stratosphere, with a maximum around 37 km over Trivandrum (-1.71 ± 0.49 K decade-1) and New Delhi (-1.15 ± 0.55 K decade-1). The observed cooling trend in the stratosphere over Trivandrum and New Delhi is consistent with Gadanki lidar observations during 1998-2011. The water vapor shows a decreasing trend in the lower stratosphere and an increasing trend in the middle and upper stratosphere. A good correlation between N2O and O3 is found in the middle stratosphere (˜ 10 hPa) and poor correlation in the lower stratosphere. There is not much regional difference in the water vapor and temperature trends. However, upper stratospheric ozone trends over Trivandrum and New Delhi are different. The trend analysis carried out by varying the initial year has shown significant changes in the estimated trend.

  5. Lidar observations of stratospheric aerosol layer after the Mt. Pinatubo volcanic eruption

    International Nuclear Information System (INIS)

    Nagai, Tomohiro; Uchino, Osamu; Fujimoto, Toshifumi.

    1992-01-01

    The volcano Mt. Pinatubo located on the Luzon Island, Philippines, had explosively erupted on June 15, 1991. The volcanic eruptions such as volcanic ash, SO2 and H2O reached into the stratosphere over 30 km altitude by the NOAA-11 satellite observation and this is considered one of the biggest volcanic eruptions in this century. A grandiose volcanic eruption influences the atmosphere seriously and causes many climatic effects globally. There had been many impacts on radiation, atmospheric temperature and stratospheric ozone after some past volcanic eruptions. The main cause of volcanic influence depends on stratospheric aerosol, that stay long enough to change climate and other meteorological conditions. Therefore it is very important to watch stratospheric aerosol layers carefully and continuously. Standing on this respect, we do not only continue stratospheric aerosol observation at Tsukuba but also have urgently developed another lidar observational point at Naha in Okinawa Island. This observational station could be thought valuable since there is no lidar observational station in this latitudinal zone and it is much nearer to Mt. Pinatubo. Especially, there is advantage to link up these two stations on studying the transportation mechanism in the stratosphere. In this paper, we present the results of lidar observations at Tsukuba and Naha by lidar systems with Nd:YAG laser

  6. Lidar Observations of Stratospheric Aerosol Layer After the Mt. Pinatubo Volcanic Eruption

    Science.gov (United States)

    Nagai, Tomohiro; Uchino, Osamu; Fujimoto, Toshifumi

    1992-01-01

    The volcano Mt. Pinatubo located on the Luzon Island, Philippines, had explosively erupted on June 15, 1991. The volcanic eruptions such as volcanic ash, SO2 and H2O reached into the stratosphere over 30 km altitude by the NOAA-11 satellite observation and this is considered one of the biggest volcanic eruptions in this century. A grandiose volcanic eruption influences the atmosphere seriously and causes many climatic effects globally. There had been many impacts on radiation, atmospheric temperature and stratospheric ozone after some past volcanic eruptions. The main cause of volcanic influence depends on stratospheric aerosol, that stay long enough to change climate and other meteorological conditions. Therefore it is very important to watch stratospheric aerosol layers carefully and continuously. Standing on this respect, we do not only continue stratospheric aerosol observation at Tsukuba but also have urgently developed another lidar observational point at Naha in Okinawa Island. This observational station could be thought valuable since there is no lidar observational station in this latitudinal zone and it is much nearer to Mt. Pinatubo. Especially, there is advantage to link up these two stations on studying the transportation mechanism in the stratosphere. In this paper, we present the results of lidar observations at Tsukuba and Naha by lidar systems with Nd:YAG laser.

  7. Impact of Surface Active Ionic Liquids on the Cloud Points of Nonionic Surfactants and the Formation of Aqueous Micellar Two-Phase Systems.

    Science.gov (United States)

    Vicente, Filipa A; Cardoso, Inês S; Sintra, Tânia E; Lemus, Jesus; Marques, Eduardo F; Ventura, Sónia P M; Coutinho, João A P

    2017-09-21

    Aqueous micellar two-phase systems (AMTPS) hold a large potential for cloud point extraction of biomolecules but are yet poorly studied and characterized, with few phase diagrams reported for these systems, hence limiting their use in extraction processes. This work reports a systematic investigation of the effect of different surface-active ionic liquids (SAILs)-covering a wide range of molecular properties-upon the clouding behavior of three nonionic Tergitol surfactants. Two different effects of the SAILs on the cloud points and mixed micelle size have been observed: ILs with a more hydrophilic character and lower critical packing parameter (CPP formation of smaller micelles and concomitantly increase the cloud points; in contrast, ILs with a more hydrophobic character and higher CPP (CPP ≥ 1) induce significant micellar growth and a decrease in the cloud points. The latter effect is particularly interesting and unusual for it was accepted that cloud point reduction is only induced by inorganic salts. The effects of nonionic surfactant concentration, SAIL concentration, pH, and micelle ζ potential are also studied and rationalized.

  8. Water Vapor in Titan's Stratosphere from Cassini CIRS Far-Infrared Spectra

    Science.gov (United States)

    Cottini, V.; Nixon, C. A.; Jennings, D. E.; Anderson, C. M.; Gorius, N.; Bjoraker, G. L.; Coustenis, A.; Teanby, N. A.; Achterberg, R. K.; Bezard, B.; hide

    2012-01-01

    Here we report the measurement of water vapor in Titan's stratosphere using the Cassini Composite Infrared Spectrometer (CIRS). CIRS senses water emissions in the far infrared spectral region near 50 micron, which we have modeled using two independent radiative transfer codes. From the analysis of nadir spectra we have derived a mixing ratio of 0.14 +/- 0.05 ppb at an altitude of 97 km, which corresponds to an integrated (from 0 to 600 km) surface normalized column abundance of 3.7 +/- 1.3 1014 molecules/cm2. In the latitude range 80S to 30N we see no evidence for latitudinal variations in these abundances within the error bars. Using limb observations, we obtained mixing ratios of 0.13 +/- 0.04 ppb at an altitude of 115 km and 0.45 +/- 0.15 ppb at an altitude of 230 km, confirming that the water abundance has a positive vertical gradient as predicted by photochemical models. We have also fitted our data using scaling factors of 0.1-0.6 to these photochemical model profiles, indicating that the models over-predict the water abundance in Titan's lower stratosphere.

  9. Extreme ozone depletion in the 2010–2011 Arctic winter stratosphere as observed by MIPAS/ENVISAT using a 2-D tomographic approach

    Directory of Open Access Journals (Sweden)

    E. Arnone

    2012-10-01

    Full Text Available We present observations of the 2010–2011 Arctic winter stratosphere from the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS onboard ENVISAT. Limb sounding infrared measurements were taken by MIPAS during the Northern polar winter and into the subsequent spring, giving a continuous vertically resolved view of the Arctic dynamics, chemistry and polar stratospheric clouds (PSCs. We adopted a 2-D tomographic retrieval approach to account for the strong horizontal inhomogeneity of the atmosphere present under vortex conditions, self-consistently comparing 2011 to the 2-D analysis of 2003–2010. Unlike most Arctic winters, 2011 was characterized by a strong stratospheric vortex lasting until early April. Lower stratospheric temperatures persistently remained below the threshold for PSC formation, extending the PSC season up to mid-March, resulting in significant chlorine activation leading to ozone destruction. On 3 January 2011, PSCs were detected up to 30.5 ± 0.9 km altitude, representing the highest PSCs ever reported in the Arctic. Through inspection of MIPAS spectra, 83% of PSCs were identified as supercooled ternary solution (STS or STS mixed with nitric acid trihydrate (NAT, 17% formed mostly by NAT particles, and only two cases by ice. In the lower stratosphere at potential temperature 450 K, vortex average ozone showed a daily depletion rate reaching 100 ppbv day−1. In early April at 18 km altitude, 10% of vortex measurements displayed total depletion of ozone, and vortex average values dropped to 0.6 ppmv. This corresponds to a chemical loss from early winter greater than 80%. Ozone loss was accompanied by activation of ClO, associated depletion of its reservoir ClONO2, and significant denitrification, which further delayed the recovery of ozone in spring. Once the PSC season halted, ClO was reconverted primarily into ClONO2. Compared to MIPAS observed 2003–2010 Arctic average values

  10. CERES Monthly Gridded Single Satellite TOA and Surfaces/Clouds (SFC) data in HDF (CER_SFC_TRMM-PFM-VIRS_Beta4)

    Science.gov (United States)

    Wielicki, Bruce A. (Principal Investigator)

    The Monthly Gridded TOA/Surface Fluxes and Clouds (SFC) product contains a month of space and time averaged Clouds and the Earth's Radiant Energy System (CERES) data for a single scanner instrument. The SFC is also produced for combinations of scanner instruments. All instantaneous shortwave, longwave, and window fluxes at the Top-of-the-Atmosphere (TOA) and surface from the CERES SSF product for a month are sorted by 1-degree spatial regions and by the local hour of observation. The mean of the instantaneous fluxes for a given region-hour bin is determined and recorded on the SFC along with other flux statistics and scene information. These average fluxes are given for both clear-sky and total-sky scenes. The regional cloud properties are column averaged and are included on the SFC. [Location=GLOBAL] [Temporal_Coverage: Start_Date=1998-01-01; Stop_Date=2000-03-31] [Spatial_Coverage: Southernmost_Latitude=-90; Northernmost_Latitude=90; Westernmost_Longitude=-180; Easternmost_Longitude=100] [Data_Resolution: Latitude_Resolution=1 degree; Longitude_Resolution=1 degree; Horizontal_Resolution_Range=100 km - < 250 km or approximately 1 degree - < 2.5 degrees; Temporal_Resolution=1 hour; Temporal_Resolution_Range=Hourly - < Daily].

  11. Cloud Statistics and Discrimination in the Polar Regions

    Science.gov (United States)

    Chan, M.; Comiso, J. C.

    2012-12-01

    Despite their important role in the climate system, cloud cover and their statistics are poorly known, especially in the polar regions, where clouds are difficult to discriminate from snow covered surfaces. The advent of the A-train, which included Aqua/MODIS, CALIPSO/CALIOP and CloudSat/CPR sensors has provided an opportunity to improve our ability to accurately characterize the cloud cover. MODIS provides global coverage at a relatively good temporal and spatial resolution while CALIOP and CPR provide limited nadir sampling but accurate characterization of the vertical structure and phase of the cloud cover. Over the polar regions, cloud detection from a passive sensors like MODIS is challenging because of the presence of cold and highly reflective surfaces such as snow, sea-ice, glaciers, and ice-sheet, which have surface signatures similar to those of clouds. On the other hand, active sensors such as CALIOP and CPR are not only very sensitive to the presence of clouds but can also provide information about its microphysical characteristics. However, these nadir-looking sensors have sparse spatial coverage and their global data can have data spatial gaps of up to 100 km. We developed a polar cloud detection system for MODIS that is trained using collocated data from CALIOP and CPR. In particular, we employ a machine learning system that reads the radiative profile observed by MODIS and determine whether the field of view is cloudy or clear. Results have shown that the improved cloud detection scheme performs better than typical cloud mask algorithms using a validation data set not used for training. A one-year data set was generated and results indicate that daytime cloud detection accuracies improved from 80.1% to 92.6% (over sea-ice) and 71.2% to 87.4% (over ice-sheet) with CALIOP data used as the baseline. Significant improvements are also observed during nighttime, where cloud detection accuracies increase by 19.8% (over sea-ice) and 11.6% (over ice

  12. Drift-corrected Odin-OSIRIS ozone product: algorithm and updated stratospheric ozone trends

    Directory of Open Access Journals (Sweden)

    A. E. Bourassa

    2018-01-01

    Full Text Available A small long-term drift in the Optical Spectrograph and Infrared Imager System (OSIRIS stratospheric ozone product, manifested mostly since 2012, is quantified and attributed to a changing bias in the limb pointing knowledge of the instrument. A correction to this pointing drift using a predictable shape in the measured limb radiance profile is implemented and applied within the OSIRIS retrieval algorithm. This new data product, version 5.10, displays substantially better both long- and short-term agreement with Microwave Limb Sounder (MLS ozone throughout the stratosphere due to the pointing correction. Previously reported stratospheric ozone trends over the time period 1984–2013, which were derived by merging the altitude–number density ozone profile measurements from the Stratospheric Aerosol and Gas Experiment (SAGE II satellite instrument (1984–2005 and from OSIRIS (2002–2013, are recalculated using the new OSIRIS version 5.10 product and extended to 2017. These results still show statistically significant positive trends throughout the upper stratosphere since 1997, but at weaker levels that are more closely in line with estimates from other data records.

  13. Nonlinear Response of the Stratosphere and the North Atlantic-European Climate to Global Warming

    Science.gov (United States)

    Manzini, E.; Karpechko, A. Yu.; Kornblueh, L.

    2018-05-01

    The response of the northern winter atmospheric circulation for two consecutive global warming periods of 2 K is examined in a grand ensemble (68 members) of idealized CO2 increase experiments performed with the same climate model. The comparison of the atmospheric responses for the two periods shows remarkable differences, indicating the nonlinearity of the response. The nonlinear signature of the atmospheric and surface responses is reminiscent of the positive phase of the annular mode of variability. The stratospheric vortex response shifts from an easterly wind change for the first 2 K to a westerly wind change for the second 2 K. The North Atlantic storm track shifts poleward only in the second period. A weaker November Arctic amplification during the second period suggests that differences in Arctic sea ice changes can act to trigger the atmospheric nonlinear response. Stratosphere-troposphere coupling thereafter can provide for the persistence of this nonlinearity throughout the winter.

  14. Co-ordinated field measurements on the influnce of leewaves on polar stratospheric clouds; Koordinierte Feldmessungen zum Einfluss von Leewellen auf Wolkenfelder in der polaren Stratosphaere

    Energy Technology Data Exchange (ETDEWEB)

    Reichardt, J.; Behrendt, A.; Baumgart, R.; Weitkamp, C. [GKSS-Forschungszentrum Geesthacht GmbH (Germany). Inst. fuer Physikalische und Chemische Analytik

    1999-07-01

    Within the framework of the project presented, the GKSS Raman lidar was deployed at the Swedish research facility ESRANGE (67.9 N, 21.1 E) in winters 1996/7 and 1997/8 for simultaneous measurements of ozone, polar stratospheric cloud (PSC) particle properties, and temperature. Both synoptic and mesoscale PSCs were observed under various meteorological conditions. On 16 Jan 1997 the complete life cycle of a leewave-induced PSC was measured. Four days later backscatter and depolarization ratios of a PSC Ia-enhanced were observed at UV wavelengths for the first time. A model was developed to compute 532 nm particle properties from these Raman lidar measurements. The calculated optical parameters agreed well with lidar measurements of this PSC type at 532 nm. Ozone profiles in PSCs were obtained during two PSC events. In winter 1997/8 temperature profiles were measured in PSCs and leewaves with the newly developed rotational Raman receiver without critical a-priori assumptions. The comparison of lidar temperatures with the European Centre for Medium Range Weather Forecast temperature analysis proved the values at the 10 hPa model level erroneous by up to 25 K. Optical and geometrical properties of arctic-winter cirrus clouds were analyed as well. Surprising spatial homogeneity in the parameter profiles was found. (orig.) [German] Im Rahmen des hier vorgestellten Projekts wurden mit dem GKSS-Ramanlidar in den Wintern 1996/7 und 1997/8 auf der schwedischen Forschungsstation ESRANGE (67.9 N, 21.1 E) gleichzeitig Ozonkonzentration, Partikeleigenschaften polarer stratosphaerischer Wolken (PSCs) und Temperatur bestimmt. Unter verschiedenen meteorologischen Bedingungen wurden sowohl synoptische als auch mesoskalige PSCs gemessen. Am 16. Januar 1997 wurde der vollstaendige Lebenszyklus einer leerwelleninduzierten PSC beobachtet. Vier Tage spaeter wurden erstmalig bei UV-Wellenlaengen Rueckstreu- und Depolarisationsverhaeltnisse der PSC Ia-enhanced gemessen. Zur Berechnung der

  15. Effects of 3-D clouds on atmospheric transmission of solar radiation: Cloud type dependencies inferred from A-train satellite data

    Science.gov (United States)

    Ham, Seung-Hee; Kato, Seiji; Barker, Howard W.; Rose, Fred G.; Sun-Mack, Sunny

    2014-01-01

    Three-dimensional (3-D) effects on broadband shortwave top of atmosphere (TOA) nadir radiance, atmospheric absorption, and surface irradiance are examined using 3-D cloud fields obtained from one hour's worth of A-train satellite observations and one-dimensional (1-D) independent column approximation (ICA) and full 3-D radiative transfer simulations. The 3-D minus ICA differences in TOA nadir radiance multiplied by π, atmospheric absorption, and surface downwelling irradiance, denoted as πΔI, ΔA, and ΔT, respectively, are analyzed by cloud type. At the 1 km pixel scale, πΔI, ΔA, and ΔT exhibit poor spatial correlation. Once averaged with a moving window, however, better linear relationships among πΔI, ΔA, and ΔT emerge, especially for moving windows larger than 5 km and large θ0. While cloud properties and solar geometry are shown to influence the relationships amongst πΔI, ΔA, and ΔT, once they are separated by cloud type, their linear relationships become much stronger. This suggests that ICA biases in surface irradiance and atmospheric absorption can be approximated based on ICA biases in nadir radiance as a function of cloud type.

  16. Estimates for the Probabilities of Surface-to-Air Cloud-Free Lines-of-Sight and Low Cloud Statistics from Ship Observations. Part 1. Fifteen Marine Locations.

    Science.gov (United States)

    1980-11-24

    time before and after) or cumulus fractus of bad weath’er, or both ( pannus ), usually below altostratus or nimbostratus. 8 = Cumulus and stratocumulus...vibrous upper part by cumulus, stratocumulus, stratus or pannus . + . from Surface Marine Observations Tape Deck TDF-11 *Fog All clouds in the 0-50...Fractus of bad weather, cr V both ( pannus ), usually below Alto- stratus or N~imbostratus. The term "bad weather* denotes the conditions which coenerally

  17. The photoevaporation of interstellar clouds

    International Nuclear Information System (INIS)

    Bertoldi, F.

    1989-01-01

    The dynamics of the photoevaporation of interstellar clouds and its consequences for the structure and evolution of H II regions are studied. An approximate analytical solution for the evolution of photoevaporating clouds is derived under the realistic assumption of axisymmetry. The effects of magnetic fields are taken into account in an approximate way. The evolution of a neutral cloud subjected to the ionizing radiation of an OB star has two distinct stages. When a cloud is first exposed to the radiation, the increase in pressure due to the ionization at the surface of the cloud leads to a radiation-driven implosion: an ionization front drives a shock into the cloud, ionizes part of it and compresses the remaining into a dense globule. The initial implosion is followed by an equilibrium cometary stage, in which the cloud maintains a semistationary comet-shaped configuration; it slowly evaporates while accelerating away from the ionizing star until the cloud has been completely ionized, reaches the edge of the H II region, or dies. Expressions are derived for the cloud mass-loss rate and acceleration. To investigate the effect of the cloud photoevaporation on the structure of H II regions, the evolution of an ensemble of clouds of a given mass distribution is studied. It is shown that the compressive effect of the ionizing radiation can induce star formation in clouds that were initially gravitationally stable, both for thermally and magnetically supported clouds

  18. Radiative budget and cloud radiative effect over the Atlantic from ship-based observations

    Directory of Open Access Journals (Sweden)

    J. Kalisch

    2012-10-01

    Full Text Available The aim of this study is to determine cloud-type resolved cloud radiative budgets and cloud radiative effects from surface measurements of broadband radiative fluxes over the Atlantic Ocean. Furthermore, based on simultaneous observations of the state of the cloudy atmosphere, a radiative closure study has been performed by means of the ECHAM5 single column model in order to identify the model's ability to realistically reproduce the effects of clouds on the climate system.

    An extensive database of radiative and atmospheric measurements has been established along five meridional cruises of the German research icebreaker Polarstern. Besides pyranometer and pyrgeometer for downward broadband solar and thermal radiative fluxes, a sky imager and a microwave radiometer have been utilized to determine cloud fraction and cloud type on the one hand and temperature and humidity profiles as well as liquid water path for warm non-precipitating clouds on the other hand.

    Averaged over all cruise tracks, we obtain a total net (solar + thermal radiative flux of 144 W m−2 that is dominated by the solar component. In general, the solar contribution is large for cirrus clouds and small for stratus clouds. No significant meridional dependencies were found for the surface radiation budgets and cloud effects. The strongest surface longwave cloud effects were shown in the presence of low level clouds. Clouds with a high optical density induce strong negative solar radiative effects under high solar altitudes. The mean surface net cloud radiative effect is −33 W m−2.

    For the purpose of quickly estimating the mean surface longwave, shortwave and net cloud effects in moderate, subtropical and tropical climate regimes, a new parameterisation was created, considering the total cloud amount and the solar zenith angle.

    The ECHAM5 single column model provides a surface net cloud effect that is more

  19. The 'surf zone' in the stratosphere

    Science.gov (United States)

    McIntyre, M. E.; Palmer, T. N.

    Synoptic, coarse-grain, isentropic maps of Ertel's potential vorticity Q for the northern middle stratosphere, estimated using a large-Richardson-number approximation, are presented for a number of days in January-February 1979, together with some related isentropic trajectory calculations The effects of substituting FGGE for NMC base data are noted, as well as some slight corrections to maps published earlier. The combined evidence from the observations and from dynamical models strongly indicates the existence of planetary-wave breaking, a process in which material contours are rapidly and irreversibly deformed. In the winter stratosphere this occurs most spectacularly in a gigantic 'nonlinear critical layer', or 'surf zone', which surrounds the main polar vortex, and which tends to erode the vortex when wave amplitudes become large. Some of the FGGE-based Q maps suggest that we may be seeing glimpses of local dynamical instabilities and vortex-rollup phenomena within breaking planetary waves. Related phenomena in the troposphere are discussed. An objective definition of the area A( t) of the main vortex, as it appears on isentropic Q maps, is proposed. A smoothed time series of daily values of A( t) should be a statistically powerful 'circulation index' for the state of the winter-time middle stratosphere, which avoids the loss of information incurred by Eulerian space and time averaging.

  20. Simultaneous observations of solar MeV particles in a magnetic cloud and in the earth's northern tail lobe - Implications for the global field line topology of magnetic clouds and for the entry of solar particles into the magnetosphere during cloud passage

    Science.gov (United States)

    Farrugia, C. J.; Richardson, I. G.; Burlaga, L. F.; Lepping, R. P.; Osherovich, V. A.

    1993-01-01

    Simultaneous ISEE 3 and IMP 8 spacecraft observations of magnetic fields and flow anisotropies of solar energetic protons and electrons during the passage of an interplanetary magnetic cloud show various particle signature differences at the two spacecraft. These differences are interpretable in terms of the magnetic line topology of the cloud, the connectivity of the cloud field lines to the solar surface, and the interconnection between the magnetic fields of the magnetic clouds and of the earth. These observations are consistent with a magnetic cloud model in which these mesoscale configurations are curved magnetic flux ropes attached at both ends to the sun's surface, extending out to 1 AU.

  1. Update of the Polar SWIFT model for polar stratospheric ozone loss (Polar SWIFT version 2

    Directory of Open Access Journals (Sweden)

    I. Wohltmann

    2017-07-01

    Full Text Available The Polar SWIFT model is a fast scheme for calculating the chemistry of stratospheric ozone depletion in polar winter. It is intended for use in global climate models (GCMs and Earth system models (ESMs to enable the simulation of mutual interactions between the ozone layer and climate. To date, climate models often use prescribed ozone fields, since a full stratospheric chemistry scheme is computationally very expensive. Polar SWIFT is based on a set of coupled differential equations, which simulate the polar vortex-averaged mixing ratios of the key species involved in polar ozone depletion on a given vertical level. These species are O3, chemically active chlorine (ClOx, HCl, ClONO2 and HNO3. The only external input parameters that drive the model are the fraction of the polar vortex in sunlight and the fraction of the polar vortex below the temperatures necessary for the formation of polar stratospheric clouds. Here, we present an update of the Polar SWIFT model introducing several improvements over the original model formulation. In particular, the model is now trained on vortex-averaged reaction rates of the ATLAS Chemistry and Transport Model, which enables a detailed look at individual processes and an independent validation of the different parameterizations contained in the differential equations. The training of the original Polar SWIFT model was based on fitting complete model runs to satellite observations and did not allow for this. A revised formulation of the system of differential equations is developed, which closely fits vortex-averaged reaction rates from ATLAS that represent the main chemical processes influencing ozone. In addition, a parameterization for the HNO3 change by denitrification is included. The rates of change of the concentrations of the chemical species of the Polar SWIFT model are purely chemical rates of change in the new version, whereas in the original Polar SWIFT model, they included a transport effect

  2. Cloud's Center of Gravity – a compact approach to analyze convective cloud development

    Directory of Open Access Journals (Sweden)

    I. Koren

    2009-01-01

    Full Text Available As cloud resolving models become more detailed, with higher resolution outputs, it is often complicated to isolate the physical processes that control the cloud attributes. Moreover, due to the high dimensionality and complexity of the model output, the analysis and interpretation of the results can be very complicated. Here we suggest a novel approach to convective cloud analysis that yields more insight into the physical and temporal evolution of clouds, and is compact and efficient. The different (3-D cloud attributes are weighted and projected onto a single point in space and in time, that has properties of, or similar to, the Center Of Gravity (COG. The location, magnitude and spread of this variable are followed in time. The implications of the COG approach are demonstrated for a study of aerosol effects on a warm convective cloud. We show that in addition to reducing dramatically the dimensionality of the output, such an approach often enhances the signal, adds more information, and makes the physical description of cloud evolution clearer, allowing unambiguous comparison of clouds evolving in different environmental conditions. This approach may also be useful for analysis of cloud data retrieved from surface or space-based cloud radars.

  3. Stratospheric mean ages and transport rates from observations of CO{sub 2} and N{sub 2}O

    Energy Technology Data Exchange (ETDEWEB)

    Boering, K A; Wofsy, S C; Daube, B C; Schneider, H R [Harvard Univ., Cambridge, MA (United States). Div. of Engineering and Applied Sciences; Loewenstein, M; Podolske, J R [NASA Ames Research Center, Moffett Field, CA (United States); Conway, T J [National Oceanic and Atmospheric Administration, Boulder, CO (United States)

    1998-12-31

    Measurements of CO{sub 2} and N{sub 2}O concentrations are reported and analyzed to investigate stratospheric transport rates. Temporal variations in tropospheric CO{sub 2} are observed to propagate into the stratosphere, showing that tropospheric air enters the lower tropical stratosphere continuously, ascends, and is transported rapidly (in less than 1 month) to both hemispheres. The mean age of stratospheric air determined from CO{sub 2} data is approximately 5 years in the mid-stratosphere. It is shown that the mean age is mathematically equivalent to a conserved tracer analogous to exhaust from stratospheric aircraft. Comparison of the mean age from models and observations indicates that current model simulations likely underestimate pollutant concentrations from proposed stratospheric aircraft by 25-100%. (author) 36 refs.

  4. Stratospheric mean ages and transport rates from observations of CO{sub 2} and N{sub 2}O

    Energy Technology Data Exchange (ETDEWEB)

    Boering, K.A.; Wofsy, S.C.; Daube, B.C.; Schneider, H.R. [Harvard Univ., Cambridge, MA (United States). Div. of Engineering and Applied Sciences; Loewenstein, M.; Podolske, J.R. [NASA Ames Research Center, Moffett Field, CA (United States); Conway, T.J. [National Oceanic and Atmospheric Administration, Boulder, CO (United States)

    1997-12-31

    Measurements of CO{sub 2} and N{sub 2}O concentrations are reported and analyzed to investigate stratospheric transport rates. Temporal variations in tropospheric CO{sub 2} are observed to propagate into the stratosphere, showing that tropospheric air enters the lower tropical stratosphere continuously, ascends, and is transported rapidly (in less than 1 month) to both hemispheres. The mean age of stratospheric air determined from CO{sub 2} data is approximately 5 years in the mid-stratosphere. It is shown that the mean age is mathematically equivalent to a conserved tracer analogous to exhaust from stratospheric aircraft. Comparison of the mean age from models and observations indicates that current model simulations likely underestimate pollutant concentrations from proposed stratospheric aircraft by 25-100%. (author) 36 refs.

  5. Cloud vertical structure, precipitation, and cloud radiative effects over Tibetan Plateau

    Science.gov (United States)

    Liu, Y.; Yan, Y.; Lu, J.

    2017-12-01

    The vertical structure of clouds and its connection with precipitation and cloud radiative effects (CRE) over the Tibetan Plateau (TP) are analyzed and compared with its neighboring land and tropical oceans based on CloudSat and Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) products and the Tropical Rainfall Measuring Mission (TRMM) precipitation data. Unique characteristics of cloud vertical structure and CRE over the TP are found. The cloud amount shows seasonal variation over the TP, which presents a single peak (located in 7-11 km) during January to April and two peaks (located in 5-8 km and 11-17 km separately) after mid-June, and then resumes to one peak (located in 5-10 km) after mid-August. Topography-induced restriction on moisture supply leads to a compression effect on clouds, i.e., the reduction in both cloud thickness and number of cloud layers, over the TP. The topography-induced compression effect is also shown in the range in the variation of cloud thickness and cloud-top height corresponding to different precipitation intensity, which is much smaller over the TP than its neighboring regions. In summer, cloud ice particles over the TP are mostly located at lower altitude (5-10 km) with richer variety of sizes and aggregation in no rain conditions compared to other regions. Ice water content becomes abundant and the number concentration tends to be dense at higher levels when precipitation is enhanced. The longwave CRE in the atmosphere over the TP is a net cooling effect. The vertical structure of CRE over the TP is unique compared to other regions: there exists a strong cooling layer of net CRE at the altitude of 8 km, from June to the beginning of October; the net radiative heating layer above the surface is shallower but stronger underneath 7 km and with a stronger seasonal variation over the TP.

  6. Synchrotron x-ray fluorescence analyses of stratospheric cosmic dust: New results for chondritic and nickel-depleted particles

    International Nuclear Information System (INIS)

    Flynn, G.J.; Sutton, S.R.

    1989-06-01

    Trace element abundance determinations were performed using synchrotron x-ray fluorescence on nine particles collected from the stratosphere and classified as ''cosmic''. Improvements to the Synchrotron Light Source allowed the detection of all elements between Cr and Mo, with the exceptions of Co and As, in our largest particle. The minor and trace element abundance patterns of three Ni-depleted particles were remarkably similar to those of extraterrestrial igneous rocks. Fe/Ni and Fe/Mn ratios suggest that one of these may be of lunar origin. All nine particles exhibited an enrichment in Br, ranging form 1.3 to 38 times the Cl concentration. Br concentrations were uncorrelated with particle size, as would be expected for a surface correlated component acquires from the stratosphere. 27 refs., 4 figs., 2 tabs

  7. Stratospheric ozone chemistry in the Antarctic: what determines the lowest ozone values reached and their recovery?

    Directory of Open Access Journals (Sweden)

    J.-U. Grooß

    2011-12-01

    Full Text Available Balloon-borne observations of ozone from the South Pole Station have been reported to reach ozone mixing ratios below the detection limit of about 10 ppbv at the 70 hPa level by late September. After reaching a minimum, ozone mixing ratios increase to above 1 ppmv on the 70 hPa level by late December. While the basic mechanisms causing the ozone hole have been known for more than 20 yr, the detailed chemical processes determining how low the local concentration can fall, and how it recovers from the minimum have not been explored so far. Both of these aspects are investigated here by analysing results from the Chemical Lagrangian Model of the Stratosphere (CLaMS. As ozone falls below about 0.5 ppmv, a balance is maintained by gas phase production of both HCl and HOCl followed by heterogeneous reaction between these two compounds in these simulations. Thereafter, a very rapid, irreversible chlorine deactivation into HCl can occur, either when ozone drops to values low enough for gas phase HCl production to exceed chlorine activation processes or when temperatures increase above the polar stratospheric cloud (PSC threshold. As a consequence, the timing and mixing ratio of the minimum ozone depends sensitively on model parameters, including the ozone initialisation. The subsequent ozone increase between October and December is linked mainly to photochemical ozone production, caused by oxygen photolysis and by the oxidation of carbon monoxide and methane.

  8. Long-term trends in stratospheric ozone, temperature, and water vapor over the Indian region

    Directory of Open Access Journals (Sweden)

    S. T. Akhil Raj

    2018-01-01

    Full Text Available We have investigated the long-term trends in and variabilities of stratospheric ozone, water vapor and temperature over the Indian monsoon region using the long-term data constructed from multi-satellite (Upper Atmosphere Research Satellite (UARS MLS and HALOE, 1993–2005, Aura Microwave Limb Sounder (MLS, 2004–2015, Sounding of the Atmosphere using Broadband Emission Radiometry (SABER, 2002–2015 on board TIMED (Thermosphere Ionosphere Mesosphere Energetics Dynamics observations covering the period 1993–2015. We have selected two locations, namely, Trivandrum (8.4° N, 76.9° E and New Delhi (28° N, 77° E, covering northern and southern parts of the Indian region. We also used observations from another station, Gadanki (13.5° N, 79.2° E, for comparison. A decreasing trend in ozone associated with NOx chemistry in the tropical middle stratosphere is found, and the trend turned to positive in the upper stratosphere. Temperature shows a cooling trend in the stratosphere, with a maximum around 37 km over Trivandrum (−1.71 ± 0.49 K decade−1 and New Delhi (−1.15 ± 0.55 K decade−1. The observed cooling trend in the stratosphere over Trivandrum and New Delhi is consistent with Gadanki lidar observations during 1998–2011. The water vapor shows a decreasing trend in the lower stratosphere and an increasing trend in the middle and upper stratosphere. A good correlation between N2O and O3 is found in the middle stratosphere (∼ 10 hPa and poor correlation in the lower stratosphere. There is not much regional difference in the water vapor and temperature trends. However, upper stratospheric ozone trends over Trivandrum and New Delhi are different. The trend analysis carried out by varying the initial year has shown significant changes in the estimated trend.

  9. Electron Cloud Parameterization Studies in the LHC

    CERN Document Server

    Dominguez, O; Baglin, V; Bregliozzi, G; Jimenez, J M; Metral, E; Rumolo, G; Schulte, D; Zimmermann, F

    2011-01-01

    During LHC beam commissioning with 150, 75 and 50-ns bunch spacing, important electron-cloud effects, like pressure rise, cryogenic heat load, beam instabilities or emittance growth, were observed. The main strategy to combat the LHC electron cloud, defined about ten years ago, relies on the surface conditioning arising from the chamber-surface bombardment with cloud electrons. In a standard model, the conditioning state of the beam-pipe surface is characterized by three parameters: 1. most importantly, the secondary emission yield δmax; 2. the incident electron energy at which the yield is maximum, ε_max; and 3. the probability of elastic reflection of low-energy primary electrons hitting the chamber wall, R. Since at the LHC no in-situ secondary-yield measurements are available, we compare the relative local pressure-rise measurements taken for different beam configurations against simulations in which surface parameters are scanned. This benchmarking of measurements and simulations is used to infer the s...

  10. Molecular clouds without detectable CO

    International Nuclear Information System (INIS)

    Blitz, L.; Bazell, D.; Desert, F.X.

    1990-01-01

    The clouds identified by Desert, Bazell, and Boulanger (DBB clouds) in their search for high-latitude molecular clouds were observed in the CO (J = 1-0) line, but only 13 percent of the sample was detected. The remaining 87 percent are diffuse molecular clouds with CO abundances of about 10 to the -6th, a typical value for diffuse clouds. This hypothesis is shown to be consistent with Copernicus data. The DBB clouds are shown to be an essentially complete catalog of diffuse molecular clouds in the solar vicinity. The total molecular surface density in the vicinity of the sun is then only about 20 percent greater than the 1.3 solar masses/sq pc determined by Dame et al. (1987). Analysis of the CO detections indicates that there is a sharp threshold in extinction of 0.25 mag before CO is detectable and is derived from the IRAS I(100) micron threshold of 4 MJy/sr. This threshold is presumably where the CO abundance exhibits a sharp increase 18 refs

  11. A global, space-based stratospheric aerosol climatology: 1979 to 2014

    Science.gov (United States)

    Thomason, L. W.; Vernier, J. P.; Bourassa, A. E.; Millan, L.; Manney, G. L.

    2016-12-01

    Herein, we report on a global space-based stratospheric aerosol climatology (GloSSAC) that has been developed to support Coupled Model Intercomparison Project Phase 6 (CMIP6) (REF to CMIP6 and ETH work). GloSSAC is most closely related to the ASAP[SPARC, 2006] and CCMI data sets and follows a similar approach used to produce those data sets. It is primarily built using space-based measurements by a number of instruments including the SAGE series, OSIRIS, CALIPSO, CLAES and HALOE. The data set is presented as monthly depictions for 80S to 80N and from at least the tropopause to 40 km. The data set consists primarily of measurements by the instruments at their native wavelength and measurement type (e.g., extinction coefficient). However, every bin in these monthly grids receives measured or indirectly inferred values for aerosol extinction coefficient at 525 and 1020 nm. Generally, bins where no data are available are filled via simple linear interpolation in time only. The exceptions are in the SAGE I/II gap from 1982 to 1984 where data from SAM II and ground-based and airborne lidar data sets are used to span the 3 years between the end of the SAGE I mission in November 1981 and the beginning of the SAGE II mission in October 1984. Ground-based lidar also supplements space-based data in the months following the Pinatubo eruption when much of the lower stratosphere is too optically opaque for occultation measurements. This data set includes total aerosol surface area density and volume estimates based on Thomason et al.[2008] though these should be interpreted as bounding values (low and high) rather than functional aerosol parameters that are generally produced from this and predecessor data sets by other parties. Unlike previous versions of this data set, GloSSAC has been permanently archived at NASA's Atmospheric Science Data Center and a digital object identifier (doi) for GloSSAC is available. SPARC (2006), Assessment of Stratospheric Aerosol Properties (ASAP

  12. GEWEX cloud assessment: A review

    Science.gov (United States)

    Stubenrauch, Claudia; Rossow, William B.; Kinne, Stefan; Ackerman, Steve; Cesana, Gregory; Chepfer, Hélène; Di Girolamo, Larry; Getzewich, Brian; Guignard, Anthony; Heidinger, Andy; Maddux, Brent; Menzel, Paul; Minnis, Patrick; Pearl, Cindy; Platnick, Steven; Poulsen, Caroline; Riedi, Jérôme; Sayer, Andrew; Sun-Mack, Sunny; Walther, Andi; Winker, Dave; Zeng, Shen; Zhao, Guangyu

    2013-05-01

    Clouds cover about 70% of the Earth's surface and play a dominant role in the energy and water cycle of our planet. Only satellite observations provide a continuous survey of the state of the atmosphere over the entire globe and across the wide range of spatial and temporal scales that comprise weather and climate variability. Satellite cloud data records now exceed more than 25 years; however, climatologies compiled from different satellite datasets can exhibit systematic biases. Questions therefore arise as to the accuracy and limitations of the various sensors. The Global Energy and Water cycle Experiment (GEWEX) Cloud Assessment, initiated in 2005 by the GEWEX Radiation Panel, provides the first coordinated intercomparison of publicly available, global cloud products (gridded, monthly statistics) retrieved from measurements of multi-spectral imagers (some with multi-angle view and polarization capabilities), IR sounders and lidar. Cloud properties under study include cloud amount, cloud height (in terms of pressure, temperature or altitude), cloud radiative properties (optical depth or emissivity), cloud thermodynamic phase and bulk microphysical properties (effective particle size and water path). Differences in average cloud properties, especially in the amount of high-level clouds, are mostly explained by the inherent instrument measurement capability for detecting and/or identifying optically thin cirrus, especially when overlying low-level clouds. The study of long-term variations with these datasets requires consideration of many factors. The monthly, gridded database presented here facilitates further assessments, climate studies, and the evaluation of climate models.

  13. Decade of stratospheric sulfate measurements compared with observations of volcanic eruptions

    International Nuclear Information System (INIS)

    Sedlacek, W.A.; Mroz, E.J.; Lazrus, A.L.; Gandrud, B.W.

    1983-01-01

    Sulfate aerosol concentrations in the stratosphere have been measured for 11 years (1971--1981) using portions of filters collected by the Department of Energy's High Altitude Sampling Program. Data collected seasonally at altitudes between 13 km and 20 km spanning latitudes from 75 0 N to 51 0 S are reported. These data are compared with the reported altitudes of volcanic eruption plumes during the same decade. From this comparison it is concluded that (1) several unreported volcanic eruptions or eruptions to altitudes higher than reported did occur during the decade, (2) the e-fold removal time for sulfate aerosol from the stratosphere following the eruption of Volcan Fuego in 1974 was 11.2 +- 1.2 months, (3) the volcanic contribution to the average stratospheric sulfate concentration over the decade was greater than 50%, and (4) there may be evidence for an anthropogenic contribution to stratospheric sulfate that increases at the rate of 6 to 8% per year

  14. Uncertainty in stratiform cloud optical thickness inferred from pyranometer measurements at the sea surface

    Directory of Open Access Journals (Sweden)

    Anna Rozwadowska

    2004-06-01

    Full Text Available The relative "plane-parallel" error in a mean cloud optical thickness retrieved from ground-based pyranometer measurements is estimated. The plane-parallel error is defined as the bias introduced by the assumption in the radiative transfer model used in cloud optical thickness retrievals that the atmosphere, including clouds, is horizontally homogeneous on the scale of an individual retrieval. The error is estimated for the optical thickness averaged over the whole domain, which simulates the mean cloud optical thickness obtained from a time series of irradiance measurements. The study is based on 3D Monte Carlo radiative transfer simulations for non-absorbing, all-liquid, layer clouds. Liquid water path distributions in the clouds are simulated by a bounded cascade fractal model. The sensitivity of the error is studied with respect to the following factors: averaging time of irradiance used in an individual retrieval, mean cloud optical thickness, cloud variability, cloud base height and solar zenith angle. In the simulations presented in this paper, the relative bias in the domain averaged cloud optical thickness retrieved from pyranometer measurements varies from +1% for optically thin clouds to nearly -20%. The highest absolute value of the relative bias is expected for thick and variable clouds with high bases (e.g. 1 km and retrievals based on long-term mean irradiances (averaging time of the order of several tens of minutes or hours. The bias can be diminished by using short-term irradiance averages, e.g. of one minute, and by limiting retrievals to low-level clouds.

  15. Mie lidar and radiosonde observations at Gadanki (13.5°N, 79.2°E) during sudden stratospheric warming of 2009

    Science.gov (United States)

    Sridharan, S.; Raghunath, K.; Sathishkumar, S.; Nath, D.

    2011-03-01

    During a major sudden stratospheric warming event (21-27 January 2009), Mie-lidar observations at Gadanki (13.5°N, 79.2°E) show persistent occurrence of cirrus clouds. Outgoing long-wave radiation averaged for 70°E-90°E, decreases to a low value (170 W/m2) on 27 January 2009 over equator indicating deep convection. The zonal mean ERA-Interim data reveal large northward and upward circulation over equatorial upper troposphere. The latitude-longitude map of ERA-Interim zonal mean potential vorticity (PV) indicates two tongues of high PV emanating from polar latitudes and extending further down to equator. Radiosonde observations at Gadanki show the presence of ∼40% relative humidity at 11-13 km and lower tropopause temperature. It is inferred that the tropical circulation change due to PV intrusion leads to deep convection, which along with high humidity and low tropopause temperature leading to the formation of persistent cirrus clouds, the occurrence frequency of which is normally less during winter season over Gadanki.

  16. Clouds and Hazes in Exoplanet Atmospheres

    OpenAIRE

    Marley, Mark S.; Ackerman, Andrew S.; Cuzzi, Jeffrey N.; Kitzmann, Daniel

    2013-01-01

    Clouds and hazes are commonplace in the atmospheres of solar system planets and are likely ubiquitous in the atmospheres of extrasolar planets as well. Clouds affect every aspect of a planetary atmosphere, from the transport of radiation, to atmospheric chemistry, to dynamics and they influence - if not control - aspects such as surface temperature and habitability. In this review we aim to provide an introduction to the role and properties of clouds in exoplanetary atmospheres. We consider t...

  17. Global cloud database from VIRS and MODIS for CERES

    Science.gov (United States)

    Minnis, Patrick; Young, David F.; Wielicki, Bruce A.; Sun-Mack, Sunny; Trepte, Qing Z.; Chen, Yan; Heck, Patrick W.; Dong, Xiquan

    2003-04-01

    The NASA CERES Project has developed a combined radiation and cloud property dataset using the CERES scanners and matched spectral data from high-resolution imagers, the Visible Infrared Scanner (VIRS) on the Tropical Rainfall Measuring Mission (TRMM) satellite and the Moderate Resolution Imaging Spectroradiometer (MODIS) on Terra and Aqua. The diurnal cycle can be well-characterized over most of the globe using the combinations of TRMM, Aqua, and Terra data. The cloud properties are derived from the imagers using state-of-the-art methods and include cloud fraction, height, optical depth, phase, effective particle size, emissivity, and ice or liquid water path. These cloud products are convolved into the matching CERES fields of view to provide simultaneous cloud and radiation data at an unprecedented accuracy. Results are available for at least 3 years of VIRS data and 1 year of Terra MODIS data. The various cloud products are compared with similar quantities from climatological sources and instantaneous active remote sensors. The cloud amounts are very similar to those from surface observer climatologies and are 6-7% less than those from a satellite-based climatology. Optical depths are 2-3 times smaller than those from the satellite climatology, but are within 5% of those from the surface remote sensing. Cloud droplet sizes and liquid water paths are within 10% of the surface results on average for stratus clouds. The VIRS and MODIS retrievals are very consistent with differences that usually can be explained by sampling, calibration, or resolution differences. The results should be extremely valuable for model validation and improvement and for improving our understanding of the relationship between clouds and the radiation budget.

  18. Cloud-radiation interactions - Effects of cirrus optical thickness feedbacks

    Science.gov (United States)

    Somerville, Richard C. J.; Iacobellis, Sam

    1987-01-01

    The paper is concerned with a cloud-radiation feedback mechanism which may be an important component of the climate changes expected from increased atmospheric concentrations of carbon dioxide and other trace greenhouse gases. A major result of the study is that cirrus cloud optical thickness feedbacks may indeed tend to increase the surface warming due to trace gas increases. However, the positive feedback from cirrus appears to be generally weaker than the negative effects due to lower clouds. The results just confirm those of earlier research indicating that the net effect of cloud optical thickness feedbacks may be a negative feedback which may substantially (by a factor of about 2) reduce the surface warming due to the doubling of CO2, even in the presence of cirrus clouds.

  19. Small volcanic eruptions and the stratospheric sulfate aerosol burden

    Science.gov (United States)

    Pyle, David M.

    2012-09-01

    Understanding of volcanic activity and its impacts on the atmosphere has evolved in discrete steps, associated with defining eruptions. The eruption of Krakatau, Indonesia, in August 1883 was the first whose global reach was recorded through observations of atmospheric phenomena around the world (Symons 1888). The rapid equatorial spread of Krakatau's ash cloud revealed new details of atmospheric circulation, while the vivid twilights and other optical phenomena were soon causally linked to the effects of particles and gases released from the volcano (e.g. Stothers 1996, Schroder 1999, Hamilton 2012). Later, eruptions of Agung, Bali (1963), El Chichón, Mexico (1982) and Pinatubo, Philippines (1991) led to a fuller understanding of how volcanic SO2 is transformed to a long-lived stratospheric sulfate aerosol, and its consequences (e.g. Meinel and Meinel 1967, Rampino and Self 1982, Hoffman and Rosen 1983, Bekki and Pyle 1994, McCormick et al 1995). While our ability to track the dispersal of volcanic emissions has been transformed since Pinatubo, with the launch of fleets of Earth-observing satellites (e.g. NASA's A-Train; ESA's MetOp) and burgeoning networks of ground-based remote-sensing instruments (e.g. lidar and sun-photometers; infrasound and lightning detection systems), there have been relatively few significant eruptions. Thus, there have been limited opportunities to test emerging hypotheses including, for example, the vexed question of the role of 'smaller' explosive eruptions in perturbations of the atmosphere—those that may just be large enough to reach the stratosphere (of size 'VEI 3', Newhall and Self 1982, Pyle 2000). Geological evidence, from ice-cores and historical eruptions, suggests that small explosive volcanic eruptions with the potential to transport material into the stratosphere should be frequent (5-10 per decade), and responsible for a significant proportion of the long-term time-averaged flux of volcanic sulfur into the stratosphere

  20. Key aspects of stratospheric tracer modeling using assimilated winds

    Directory of Open Access Journals (Sweden)

    B. Bregman

    2006-01-01

    Full Text Available This study describes key aspects of global chemistry-transport models and their impact on stratospheric tracer transport. We concentrate on global models that use assimilated winds from numerical weather predictions, but the results also apply to tracer transport in general circulation models. We examined grid resolution, numerical diffusion, air parcel dispersion, the wind or mass flux update frequency, and time interpolation. The evaluation is performed with assimilated meteorology from the "operational analyses or operational data" (OD from the European Centre for Medium-Range Weather Forecasts (ECMWF. We also show the effect of the mass flux update frequency using the ECMWF 40-year re-analyses (ERA40. We applied the three-dimensional chemistry-transport Tracer Model version 5 (TM5 and a trajectory model and performed several diagnoses focusing on different transport regimes. Covering different time and spatial scales, we examined (1 polar vortex dynamics during the Arctic winter, (2 the large-scale stratospheric meridional circulation, and (3 air parcel dispersion in the tropical lower stratosphere. Tracer distributions inside the Arctic polar vortex show considerably worse agreement with observations when the model grid resolution in the polar region is reduced to avoid numerical instability. The results are sensitive to the diffusivity of the advection. Nevertheless, the use of a computational cheaper but diffusive advection scheme is feasible for tracer transport when the horizontal grid resolution is equal or smaller than 1 degree. The use of time interpolated winds improves the tracer distributions, particularly in the middle and upper stratosphere. Considerable improvement is found both in the large-scale tracer distribution and in the polar regions when the update frequency of the assimilated winds is increased from 6 to 3 h. It considerably reduces the vertical dispersion of air parcels in the tropical lower stratosphere. Strong

  1. A Semi-empirical Model of the Stratosphere in the Climate System

    Science.gov (United States)

    Sodergren, A. H.; Bodeker, G. E.; Kremser, S.; Meinshausen, M.; McDonald, A.

    2014-12-01

    Chemistry climate models (CCMs) currently used to project changes in Antarctic ozone are extremely computationally demanding. CCM projections are uncertain due to lack of knowledge of future emissions of greenhouse gases (GHGs) and ozone depleting substances (ODSs), as well as parameterizations within the CCMs that have weakly constrained tuning parameters. While projections should be based on an ensemble of simulations, this is not currently possible due to the complexity of the CCMs. An inexpensive but realistic approach to simulate changes in stratospheric ozone, and its coupling to the climate system, is needed as a complement to CCMs. A simple climate model (SCM) can be used as a fast emulator of complex atmospheric-ocean climate models. If such an SCM includes a representation of stratospheric ozone, the evolution of the global ozone layer can be simulated for a wide range of GHG and ODS emissions scenarios. MAGICC is an SCM used in previous IPCC reports. In the current version of the MAGICC SCM, stratospheric ozone changes depend only on equivalent effective stratospheric chlorine (EESC). In this work, MAGICC is extended to include an interactive stratospheric ozone layer using a semi-empirical model of ozone responses to CO2and EESC, with changes in ozone affecting the radiative forcing in the SCM. To demonstrate the ability of our new, extended SCM to generate projections of global changes in ozone, tuning parameters from 19 coupled atmosphere-ocean general circulation models (AOGCMs) and 10 carbon cycle models (to create an ensemble of 190 simulations) have been used to generate probability density functions of the dates of return of stratospheric column ozone to 1960 and 1980 levels for different latitudes.

  2. Evidence for Dynamical Coupling of Stratosphere-MLT during recent minor Stratospheric Warmings in Southern Hemisphere

    Science.gov (United States)

    Kim, Yongha; Sunkara, Eswaraiah; Hong, Junseok; Ratnam, Venkat; Chandran, Amal; Rao, Svb; Riggin, Dennis

    2015-04-01

    The mesosphere-lower thermosphere (MLT) response to extremely rare minor sudden stratospheric warming (SSW) events was observed for the first time in the southern hemisphere (SH) during 2010 and is investigated using the meteor radar located at King Sejong Station (62.22°S, 58.78°W), Antarctica. Three episodic SSWs were noticed from early August to late October 2010. The mesospheric wind field was found to significantly differ from normal years due to enhanced planetary wave (PW) activity before the SSWs and secondary PWs in the MLT afterwards. The zonal winds in the mesosphere reversed approximately a week before the SSW occurrence in the stratosphere as has been observed 2002 major SSW, suggesting the downward propagation of disturbance during minor SSWs as well. Signatures of mesospheric cooling (MC) in association with SSWs are found in the Microwave Limb Sounder (MLS) measurements. SD-WACCM simulations are able to produce these observed features.

  3. Detecting Super-Thin Clouds With Polarized Light

    Science.gov (United States)

    Sun, Wenbo; Videen, Gorden; Mishchenko, Michael I.

    2014-01-01

    We report a novel method for detecting cloud particles in the atmosphere. Solar radiation backscattered from clouds is studied with both satellite data and a radiative transfer model. A distinct feature is found in the angle of linear polarization of solar radiation that is backscattered from clouds. The dominant backscattered electric field from the clear-sky Earth-atmosphere system is nearly parallel to the Earth surface. However, when clouds are present, this electric field can rotate significantly away from the parallel direction. Model results demonstrate that this polarization feature can be used to detect super-thin cirrus clouds having an optical depth of only 0.06 and super-thin liquid water clouds having an optical depth of only 0.01. Such clouds are too thin to be sensed using any current passive satellite instruments.

  4. Airborne Arctic Stratospheric Expedition II: An overview

    Science.gov (United States)

    Anderson, James G.; Toon, Owen B.

    1993-11-01

    The sudden onset of ozone depletion in the antarctic vortex set a precedent for both the time scale and the severity of global change. The Airborne Antarctic Ozone Experiment (AAOE), staged from Punta Arenas, Chile, in 1987, established that CFCs, halons, and methyl bromide, the dominant sources of chlorine and bromine radicals in the stratosphere, control the rate of ozone destruction over the Antarctic; that the vortex is depleted in reactive nitrogen and water vapor; and that diabatic cooling during the Antarctic winter leads to subsidence within the vortex core, importing air from higher altitudes and lower latitudes. This last conclusion is based on observed dramatic distortion in the tracer fields, most notably N2O.In 1989, the first Airborne Arctic Stratospheric Expedition (AASE-I), staged from Stavanger, Norway, and using the same aircraft employed for AAOE (the NASA ER-2 and the NASA DC-8), discovered that while NOx and to some degree NOy were perturbed within the arctic vortex, there was little evidence for desiccation. Under these (in contrast to the antarctic) marginally perturbed conditions, however, ClO was found to be dramatically enhanced such that a large fraction of the available (inorganic) chlorine resided in the form of ClO and its dimer ClOOCl.This leaves two abiding issues for the northern hemisphere and the mission of the second Airborne Arctic Stratospheric Expedition (AASE-II): (1) Will significant ozone erosion occur within the arctic vortex in the next ten years as chlorine loading in the stratosphere exceeds four parts per billion by volume? (2) Which mechanisms are responsible for the observed ozone erosion poleward of 30°N in the winter/spring northern hemisphere reported in satellite observations?

  5. Stratospheric aerosol effects from Soufriere Volcano as measured by the SAGE satellite system

    Science.gov (United States)

    Mccormick, M. P.; Kent, G. S.; Yue, G. K.; Cunnold, D. M.

    1982-01-01

    During its April 1979 eruption series, Soufriere Volcano produced two major stratospheric plumes that the SAGE (Stratospheric Aerosol and Gas Experiment) satellite system tracked to West Africa and the North Atlantic Ocean. The total mass of these plumes, whose movement and dispersion are in agreement with those deduced from meteorological data and dispersion theory, was less than 0.5 percent of the global stratospheric aerosol burden; no significant temperature or climate perturbation is therefore expected.

  6. Clouds enhance Greenland ice sheet mass loss

    Science.gov (United States)

    Van Tricht, Kristof; Gorodetskaya, Irina V.; L'Ecuyer, Tristan; Lenaerts, Jan T. M.; Lhermitte, Stef; Noel, Brice; Turner, David D.; van den Broeke, Michiel R.; van Lipzig, Nicole P. M.

    2015-04-01

    Clouds have a profound influence on both the Arctic and global climate, while they still represent one of the key uncertainties in climate models, limiting the fidelity of future climate projections. The potentially important role of thin liquid-containing clouds over Greenland in enhancing ice sheet melt has recently gained interest, yet current research is spatially and temporally limited, focusing on particular events, and their large scale impact on the surface mass balance remains unknown. We used a combination of satellite remote sensing (CloudSat - CALIPSO), ground-based observations and climate model (RACMO) data to show that liquid-containing clouds warm the Greenland ice sheet 94% of the time. High surface reflectivity (albedo) for shortwave radiation reduces the cloud shortwave cooling effect on the absorbed fluxes, while not influencing the absorption of longwave radiation. Cloud warming over the ice sheet therefore dominates year-round. Only when albedo values drop below ~0.6 in the coastal areas during summer, the cooling effect starts to overcome the warming effect. The year-round excess of energy due to the presence of liquid-containing clouds has an extensive influence on the mass balance of the ice sheet. Simulations using the SNOWPACK snow model showed not only a strong influence of these liquid-containing clouds on melt increase, but also on the increased sublimation mass loss. Simulations with the Community Earth System Climate Model for the end of the 21st century (2080-2099) show that Greenland clouds contain more liquid water path and less ice water path. This implies that cloud radiative forcing will be further enhanced in the future. Our results therefore urge the need for improving cloud microphysics in climate models, to improve future projections of ice sheet mass balance and global sea level rise.

  7. MJO-Related Tropical Convection Anomalies Lead to More Accurate Stratospheric Vortex Variability in Subseasonal Forecast Models.

    Science.gov (United States)

    Garfinkel, C I; Schwartz, C

    2017-10-16

    The effect of the Madden-Julian Oscillation (MJO) on the Northern Hemisphere wintertime stratospheric polar vortex in the period preceding stratospheric sudden warmings is evaluated in operational subseasonal forecasting models. Reforecasts which simulate stronger MJO-related convection in the Tropical West Pacific also simulate enhanced heat flux in the lowermost stratosphere and a more realistic vortex evolution. The time scale on which vortex predictability is enhanced lies between 2 and 4 weeks for nearly all cases. Those stratospheric sudden warmings that were preceded by a strong MJO event are more predictable at ∼20 day leads than stratospheric sudden warmings not preceded by a MJO event. Hence, knowledge of the MJO can contribute to enhanced predictability, at least in a probabilistic sense, of the Northern Hemisphere polar stratosphere.

  8. A simple method to compute the change in earth-atmosphere radiative balance due to a stratospheric aerosol layer

    Science.gov (United States)

    Lenoble, J.; Tanre, D.; Deschamps, P. Y.; Herman, M.

    1982-01-01

    A computer code was developed in terms of a three-layer model for the earth-atmosphere system, using a two-stream approximation for the troposphere and stratosphere. The analysis was limited to variable atmosphere loading by solar radiation over an unperturbed section of the atmosphere. The scattering atmosphere above a Lambertian ground layer was considered in order to derive the planar albedo and the spherical albedo. Attention was given to the influence of the aerosol optical thickness in the stratosphere, the single scattering albedo and asymmetry factor, and the sublayer albedo. Calculations were performed of the zonal albedo and the planetary radiation balance, taking into account a stratospheric aerosol layer containing H2SO4 droplets and volcanic ash. The resulting ground temperature disturbance was computed using a Budyko (1969) climate model. Local decreases in the albedo in the summer were observed in high latitudes, implying a heating effect of the aerosol. An accompanying energy loss of 23-27 W/sq m was projected, which translates to surface temperature decreases of either 1.1 and 0.45 C, respectively, for background and volcanic aerosols.

  9. An Automatic Cloud Detection Method for ZY-3 Satellite

    Directory of Open Access Journals (Sweden)

    CHEN Zhenwei

    2015-03-01

    Full Text Available Automatic cloud detection for optical satellite remote sensing images is a significant step in the production system of satellite products. For the browse images cataloged by ZY-3 satellite, the tree discriminate structure is adopted to carry out cloud detection. The image was divided into sub-images and their features were extracted to perform classification between clouds and grounds. However, due to the high complexity of clouds and surfaces and the low resolution of browse images, the traditional classification algorithms based on image features are of great limitations. In view of the problem, a prior enhancement processing to original sub-images before classification was put forward in this paper to widen the texture difference between clouds and surfaces. Afterwards, with the secondary moment and first difference of the images, the feature vectors were extended in multi-scale space, and then the cloud proportion in the image was estimated through comprehensive analysis. The presented cloud detection algorithm has already been applied to the ZY-3 application system project, and the practical experiment results indicate that this algorithm is capable of promoting the accuracy of cloud detection significantly.

  10. The influences of wildfires and stratospheric-tropospheric exchange on ozone during seacions mission over St. Louis

    Science.gov (United States)

    Wilkins, Joseph L.

    The influence of wildfire biomass burning and stratospheric air mass transport on tropospheric ozone (O3) concentrations in St. Louis during the SEAC4RS and SEACIONS-2013 measurement campaigns has been investigated. The Lagrangian particle dispersion model FLEXPART-WRF analysis reveals that 55% of ozonesonde profiles during SEACIONS were effected by biomass burning. Comparing ozonesonde profiles with numerical simulations show that as biomass burning plumes age there is O3 production aloft. A new plume injection height technique was developed based on the Naval Research Laboratory's (NRL) detection algorithm for pyro-convection. The NRL method identified 29 pyro-cumulonimbus events that occurred during the summer of 2013, of which 13 (44%) impacted the SEACIONS study area, and 4 (14%) impacted the St. Louis area. In this study, we investigate wildfire plume injection heights using model simulations and the FLAMBE emissions inventory using 2 different algorithms. In the first case, wildfire emissions are injected at the surface and allowed to mix within the boundary layer simulated by the meteorological model. In the second case, the injection height of wildfire emissions is determined by a guided deep-convective pyroCb run using the NRL detection algorithm. Results show that simulations using surface emissions were able to represent the transport of carbon monoxide plumes from wildfires when the plumes remained below 5 km or occurred during large convective systems, but that the surface effects were over predicted. The pyroCb cases simulated the long-range transport of elevated plumes above 5 km 68% of the time. In addition analysis of potential vorticity suggests that stratospheric intrusions or tropopause folds affected 13 days (48%) when there were sonde launches and 27 days (44%) during the entire study period. The largest impact occurred on September 12, 2013 when ozone-rich air impacted the nocturnal boundary layer. By analyzing ozonesonde profiles with

  11. The Cloud Condensation Nuclei (CCN properties of 2-methyltetrols and C3-C6 polyols from osmolality and surface tension measurements

    Directory of Open Access Journals (Sweden)

    S. Ekström

    2009-02-01

    Full Text Available A significant fraction of the organic material in aerosols is made of highly soluble compounds such as sugars (mono- and polysaccharides and polyols such as the 2-methyltetrols, methylerythritol and methyltreitol. Because of their high solubility these compounds are considered as potentially efficient CCN material. For the 2-methyltetrols, this would have important implications for cloud formation at global scale because they are thought to be produced by the atmospheric oxidation of isoprene. To investigate this question, the complete Köhler curves for C3-C6 polyols and the 2-methyltetrols have been determined experimentally from osmolality and surface tension measurements. Contrary to what was expected, none of these compounds displayed a higher CCN efficiency than organic acids. Their Raoult terms show that this limited CCN efficiency is due to their absence of dissociation in water, this in spite of slight surface-tension effects for the 2-methyltetrols. Thus, compounds such as saccharides and polyols would not contribute more to cloud formation than other organic compounds studied so far. In particular, the presence of 2-methyltetrols in aerosols would not particularly enhance cloud formation in the atmosphere, in contrary to recently suggested.

  12. Characterization of AVHRR global cloud detection sensitivity based on CALIPSO-CALIOP cloud optical thickness information: demonstration of results based on the CM SAF CLARA-A2 climate data record

    Science.gov (United States)

    Karlsson, Karl-Göran; Håkansson, Nina

    2018-02-01

    The sensitivity in detecting thin clouds of the cloud screening method being used in the CM SAF cloud, albedo and surface radiation data set from AVHRR data (CLARA-A2) cloud climate data record (CDR) has been evaluated using cloud information from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) onboard the CALIPSO satellite. The sensitivity, including its global variation, has been studied based on collocations of Advanced Very High Resolution Radiometer (AVHRR) and CALIOP measurements over a 10-year period (2006-2015). The cloud detection sensitivity has been defined as the minimum cloud optical thickness for which 50 % of clouds could be detected, with the global average sensitivity estimated to be 0.225. After using this value to reduce the CALIOP cloud mask (i.e. clouds with optical thickness below this threshold were interpreted as cloud-free cases), cloudiness results were found to be basically unbiased over most of the globe except over the polar regions where a considerable underestimation of cloudiness could be seen during the polar winter. The overall probability of detecting clouds in the polar winter could be as low as 50 % over the highest and coldest parts of Greenland and Antarctica, showing that a large fraction of optically thick clouds also remains undetected here. The study included an in-depth analysis of the probability of detecting a cloud as a function of the vertically integrated cloud optical thickness as well as of the cloud's geographical position. Best results were achieved over oceanic surfaces at mid- to high latitudes where at least 50 % of all clouds with an optical thickness down to a value of 0.075 were detected. Corresponding cloud detection sensitivities over land surfaces outside of the polar regions were generally larger than 0.2 with maximum values of approximately 0.5 over the Sahara and the Arabian Peninsula. For polar land surfaces the values were close to 1 or higher with maximum values of 4.5 for the parts

  13. The Global and Local Characters of Mars Perihelion Cloud Trails

    Science.gov (United States)

    Clancy, R. T.; Wolff, M. J.; Smith, M. D.; Cantor, B. A.; Spiga, A.

    2014-12-01

    We present the seasonal and spatial distribution of Mars perihelion cloud trails as mapped from Mars Reconnaissance Orbiter (MRO) MARCI (Mars Color Imager) imaging observations in 2 ultraviolet and 3 visible filters. The extended 2007-2013 period of MARCI daily global image maps reveals the widespread distribution of these high altitude clouds, which are somewhat paradoxically associated with specific surface regions. They appear as longitudinally extended (300-700 km) cloud trails with distinct leading plumes of substantial ice cloud optical depths (0.02-0.2) for such high altitudes of occurrence (40-50 km, from cloud surface shadow measurements). These plumes generate small ice particles (Reff~1 to reflect locally elevated mesospheric water ice formation that may impact the global expression of mesospheric water ice aerosols.

  14. Impacts of Stratospheric Black Carbon on Agriculture

    Science.gov (United States)

    Xia, L.; Robock, A.; Elliott, J. W.

    2017-12-01

    A regional nuclear war between India and Pakistan could inject 5 Tg of soot into the stratosphere, which would absorb sunlight, decrease global surface temperature by about 1°C for 5-10 years and have major impacts on precipitation and the amount of solar radiation reaching Earth's surface. Using two global gridded crop models forced by one global climate model simulation, we investigate the impacts on agricultural productivity in various nations. The crop model in the Community Land Model 4.5 (CLM-crop4.5) and the parallel Decision Support System for Agricultural Technology (pDSSAT) in the parallel System for Integrating Impact Models and Sectors are participating in the Global Gridded Crop Model Intercomparison. We force these two crop models with output from the Whole Atmospheric Community Climate Model to characterize the global agricultural impact from climate changes due to a regional nuclear war. Crops in CLM-crop4.5 include maize, rice, soybean, cotton and sugarcane, and crops in pDSSAT include maize, rice, soybean and wheat. Although the two crop models require a different time frequency of weather input, we downscale the climate model output to provide consistent temperature, precipitation and solar radiation inputs. In general, CLM-crop4.5 simulates a larger global average reduction of maize and soybean production relative to pDSSAT. Global rice production shows negligible change with climate anomalies from a regional nuclear war. Cotton and sugarcane benefit from a regional nuclear war from CLM-crop4.5 simulation, and global wheat production would decrease significantly in the pDSSAT simulation. The regional crop yield responses to a regional nuclear conflict are different for each crop, and we present the changes in production on a national basis. These models do not include the crop responses to changes in ozone, ultraviolet radiation, or diffuse radiation, and we would like to encourage more modelers to improve crop models to account for those

  15. Does a Relationship Between Arctic Low Clouds and Sea Ice Matter?

    Science.gov (United States)

    Taylor, Patrick C.

    2016-01-01

    Arctic low clouds strongly affect the Arctic surface energy budget. Through this impact Arctic low clouds influence important aspects of the Arctic climate system, namely surface and atmospheric temperature, sea ice extent and thickness, and atmospheric circulation. Arctic clouds are in turn influenced by these elements of the Arctic climate system, and these interactions create the potential for Arctic cloud-climate feedbacks. To further our understanding of potential Arctic cloudclimate feedbacks, the goal of this paper is to quantify the influence of atmospheric state on the surface cloud radiative effect (CRE) and its covariation with sea ice concentration (SIC). We build on previous research using instantaneous, active remote sensing satellite footprint data from the NASA A-Train. First, the results indicate significant differences in the surface CRE when stratified by atmospheric state. Second, there is a weak covariation between CRE and SIC for most atmospheric conditions. Third, the results show statistically significant differences in the average surface CRE under different SIC values in fall indicating a 3-5 W m(exp -2) larger LW CRE in 0% versus 100% SIC footprints. Because systematic changes on the order of 1 W m(exp -2) are sufficient to explain the observed long-term reductions in sea ice extent, our results indicate a potentially significant amplifying sea ice-cloud feedback, under certain meteorological conditions, that could delay the fall freeze-up and influence the variability in sea ice extent and volume. Lastly, a small change in the frequency of occurrence of atmosphere states may yield a larger Arctic cloud feedback than any cloud response to sea ice.

  16. A Report of Clouds on Titan

    Science.gov (United States)

    Corlies, Paul; Hayes, Alexander; Adamkovics, Mate; Rodriguez, Sebastien; Kelland, John; Turtle, Elizabeth P.; Mitchell, Jonathan; Lora, Juan M.; Rojo, Patricio; Lunine, Jonathan I.

    2017-10-01

    We present in this work a detailed analysis of many of the clouds in the Cassini Visual and Infrared Mapping Spectrometer (VIMS) dataset in order to understand their global and seasonal properties. Clouds are one of the few direct observables in Titan’s atmosphere (Griffith et al 2009, Rodriguez et al 2009, Adamkovics et al 2010), and so determining their characteristics allows for a better understanding of surface atmosphere interactions, winds, transport of volatile material, and general circulation. We find the clouds on Titan generally reside in at 5-15km altitude, which agrees with previous modelling efforts (Rafkin et al. 2015), as well as a power law distribution for cloud optical depth. We assume an average cloud droplet size of 100um. No seasonal dependence is observed with either cloud altitude or optical depth, suggesting there is no preferred seasonal formation mechanisms. Combining these characteristics with cloud size (Kelland et al 2017) can trace the transport of volatiles in Titan’s atmosphere, which can be compared against general circulation models (GCMs) (Lora et al 2015). We also present some specific analysis of interesting cloud systems including hypothesized surface fogs (Brown et al 2009) and orographic cloud formation (Barth et al 2010, Corlies et al 2017). In this analysis we use a correlation between Cassini VIMS and RADAR observations as well as an updated topographic map of Titan’s southern hemisphere to better understand the role that topography plays in influencing and driving atmospheric phenomena.Finally, with the end of the Cassini mission, ground based observing now acts as the only means with which to observe clouds on Titan. We present an update of an ongoing cloud campaign to search for clouds on Titan and to understand their seasonal evolution.References:Adamkovics et al. 2010, Icarus 208:868Barth et al. 2010, Planet. Space Sci. 58:1740Corlies et al. 2017, 48th LPSC, 2870CGriffith et al. 2009, ApJ 702:L105Kelland et al

  17. Cloud Type Classification (cldtype) Value-Added Product

    Energy Technology Data Exchange (ETDEWEB)

    Flynn, Donna [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Shi, Yan [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Lim, K-S [Korean Atomic Energy Research Inst., Daejeon (South Korea); Riihimaki, Laura [Pacific Northwest National Lab. (PNNL), Richland, WA (United States)

    2017-08-15

    The Cloud Type (cldtype) value-added product (VAP) provides an automated cloud type classification based on macrophysical quantities derived from vertically pointing lidar and radar. Up to 10 layers of clouds are classified into seven cloud types based on predetermined and site-specific thresholds of cloud top, base and thickness. Examples of thresholds for selected U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Climate Research Facility sites are provided in Tables 1 and 2. Inputs for the cldtype VAP include lidar and radar cloud boundaries obtained from the Active Remotely Sensed Cloud Location (ARSCL) and Surface Meteorological Systems (MET) data. Rain rates from MET are used to determine when radar signal attenuation precludes accurate cloud detection. Temporal resolution and vertical resolution for cldtype are 1 minute and 30 m respectively and match the resolution of ARSCL. The cldtype classification is an initial step for further categorization of clouds. It was developed for use by the Shallow Cumulus VAP to identify potential periods of interest to the LASSO model and is intended to find clouds of interest for a variety of users.

  18. Brief communication "Stratospheric winds, transport barriers and the 2011 Arctic ozone hole"

    Directory of Open Access Journals (Sweden)

    M. J. Olascoaga

    2012-12-01

    Full Text Available The Arctic stratosphere throughout the late winter and early spring of 2011 was characterized by an unusually severe ozone loss, resulting in what has been described as an ozone hole. The 2011 ozone loss was made possible by unusually cold temperatures throughout the Arctic stratosphere. Here we consider the issue of what constitutes suitable environmental conditions for the formation and maintenance of a polar ozone hole. Our discussion focuses on the importance of the stratospheric wind field and, in particular, the importance of a high latitude zonal jet, which serves as a meridional transport barrier both prior to ozone hole formation and during the ozone hole maintenance phase. It is argued that stratospheric conditions in the boreal winter/spring of 2011 were highly unusual inasmuch as in that year Antarctic-like Lagrangian dynamics led to the formation of a boreal ozone hole.

  19. An investigation of the processes controlling ozone in the upper stratosphere

    International Nuclear Information System (INIS)

    Patten, K.O. Jr.; Connell, P.S.; Kinnison, D.E.; Wuebbles, D.J.; Waters, J.; Froidevaux, L.; Slanger, T.G.

    1992-01-01

    Photolysis of vibrationally excited oxygen produced by ultraviolet photolysis of ozone in the upper stratosphere is incorporated into the Lawrence Livermore National Laboratory 2-D zonally averaged chemical-radiative-transport model of the troposphere and stratosphere. The importance of this potential contributor of odd oxygen to the concentration of ozone is evaluated based upon recent information on vibrational distributions of excited oxygen and upon preliminary studies of energy transfer from the excited oxygen. When the energy transfer rate constants of previous work are assumed, increases in model ozone concentrations of up to 40 percent in the upper stratosphere are found, and the ozone concentrations of the model agree with measurements, including data from the Upper Atmosphere Research Satellite. However, the increase is about 0.4 percent when the larger energy transfer rate constants suggested by more recent experimental work are applied in the model. This indicates the importance of obtaining detailed information on vibrationally excited oxygen properties, particularly the state-specific energy transfer rate constants, to evaluation of tills precess for stratospheric modeling

  20. Net Influence of an Internally Generated Guasi-biennial Oscillation on Modelled Stratospheric Climate and Chemistry

    Science.gov (United States)

    Hurwitz, Margaret M.; Oman, Luke David; Newman, Paul A.; Song, InSun

    2013-01-01

    A Goddard Earth Observing System Chemistry- Climate Model (GEOSCCM) simulation with strong tropical non-orographic gravity wave drag (GWD) is compared to an otherwise identical simulation with near-zero tropical non-orographic GWD. The GEOSCCM generates a quasibiennial oscillation (QBO) zonal wind signal in response to a tropical peak in GWD that resembles the zonal and climatological mean precipitation field. The modelled QBO has a frequency and amplitude that closely resembles observations. As expected, the modelled QBO improves the simulation of tropical zonal winds and enhances tropical and subtropical stratospheric variability. Also, inclusion of the QBO slows the meridional overturning circulation, resulting in a generally older stratospheric mean age of air. Slowing of the overturning circulation, changes in stratospheric temperature and enhanced subtropical mixing all affect the annual mean distributions of ozone, methane and nitrous oxide. Furthermore, the modelled QBO enhances polar stratospheric variability in winter. Because tropical zonal winds are easterly in the simulation without a QBO, there is a relative increase in tropical zonal winds in the simulation with a QBO. Extratropical differences between the simulations with and without a QBO thus reflect the westerly shift in tropical zonal winds: a relative strengthening of the polar stratospheric jet, polar stratospheric cooling and a weak reduction in Arctic lower stratospheric ozone.

  1. Clouds and the earth's radiation balance

    Energy Technology Data Exchange (ETDEWEB)

    Schmetz, J; Raschke, E

    1986-01-01

    Cloud formation mechanisms and cloud effects must be known for all regions of the earth for two important purposes of weather and climate research: First, the circulation characteristics of the atmosphere can be defined and understood only if the energy transfer between the atmosphere and the earth's surface is known; secondly, the energy transfer calculations should be as realistic as possible. The article discusses the influence of clouds on the radiation balance of the earth/atmosphere radiation balance, and the effects on weather and climate.

  2. Stratospheric ozone reduction and its relation to natural and man made sources

    Energy Technology Data Exchange (ETDEWEB)

    Isaksen, I S [Oslo Univ. (Norway). Dept. of Geophysics

    1996-12-31

    Approximately 90 % of the total ozone mass is in the stratosphere (between approximately 12 and 50 km), the rest is in the troposphere (below 12 km). The global distribution of ozone in the stratosphere and its variation over time have been studied extensively over several decades. These studies include observations by ground based instruments (e.g. Dobson instruments), instruments on airborne platforms (e.g. ozone sondes) and on satellites, and model studies which simulate the chemical and dynamical behaviour of the stratosphere. These studies have given good information about the processes which determine the ozone distribution, and how man made emissions affect the distribution. Observations have revealed that there are large year to year variations in stratospheric ozone above a particular location. These variations are difficult to predict as they are connected to irregular weather patterns. However, the observations have shown that there has been a long term decrease in stratospheric ozone on a global scale during the last two decades. The decrease has been most pronounced during the last five to six years and is seen both in the Northern and the Southern Hemispheres. The strong decrease in stratospheric ozone over the Antarctic continent, which has been observed since the mid 80s, and which has reduced the total ozone column with more than 50 % compared with earlier observations, is proven to be a result of increased man made emissions of CFCs. There are also mounting evidences that Northern Hemispheric ozone reductions observed since 1980 are connected to man made emissions of CFCs

  3. Stratospheric ozone reduction and its relation to natural and man made sources

    Energy Technology Data Exchange (ETDEWEB)

    Isaksen, I.S. [Oslo Univ. (Norway). Dept. of Geophysics

    1995-12-31

    Approximately 90 % of the total ozone mass is in the stratosphere (between approximately 12 and 50 km), the rest is in the troposphere (below 12 km). The global distribution of ozone in the stratosphere and its variation over time have been studied extensively over several decades. These studies include observations by ground based instruments (e.g. Dobson instruments), instruments on airborne platforms (e.g. ozone sondes) and on satellites, and model studies which simulate the chemical and dynamical behaviour of the stratosphere. These studies have given good information about the processes which determine the ozone distribution, and how man made emissions affect the distribution. Observations have revealed that there are large year to year variations in stratospheric ozone above a particular location. These variations are difficult to predict as they are connected to irregular weather patterns. However, the observations have shown that there has been a long term decrease in stratospheric ozone on a global scale during the last two decades. The decrease has been most pronounced during the last five to six years and is seen both in the Northern and the Southern Hemispheres. The strong decrease in stratospheric ozone over the Antarctic continent, which has been observed since the mid 80s, and which has reduced the total ozone column with more than 50 % compared with earlier observations, is proven to be a result of increased man made emissions of CFCs. There are also mounting evidences that Northern Hemispheric ozone reductions observed since 1980 are connected to man made emissions of CFCs

  4. Precipitation-generated oscillations in open cellular cloud fields.

    Science.gov (United States)

    Feingold, Graham; Koren, Ilan; Wang, Hailong; Xue, Huiwen; Brewer, Wm Alan

    2010-08-12

    Cloud fields adopt many different patterns that can have a profound effect on the amount of sunlight reflected back to space, with important implications for the Earth's climate. These cloud patterns can be observed in satellite images of the Earth and often exhibit distinct cell-like structures associated with organized convection at scales of tens of kilometres. Recent evidence has shown that atmospheric aerosol particles-through their influence on precipitation formation-help to determine whether cloud fields take on closed (more reflective) or open (less reflective) cellular patterns. The physical mechanisms controlling the formation and evolution of these cells, however, are still poorly understood, limiting our ability to simulate realistically the effects of clouds on global reflectance. Here we use satellite imagery and numerical models to show how precipitating clouds produce an open cellular cloud pattern that oscillates between different, weakly stable states. The oscillations are a result of precipitation causing downward motion and outflow from clouds that were previously positively buoyant. The evaporating precipitation drives air down to the Earth's surface, where it diverges and collides with the outflows of neighbouring precipitating cells. These colliding outflows form surface convergence zones and new cloud formation. In turn, the newly formed clouds produce precipitation and new colliding outflow patterns that are displaced from the previous ones. As successive cycles of this kind unfold, convergence zones alternate with divergence zones and new cloud patterns emerge to replace old ones. The result is an oscillating, self-organized system with a characteristic cell size and precipitation frequency.

  5. Tharsis Limb Cloud

    Science.gov (United States)

    2005-01-01

    [figure removed for brevity, see original site] Annotated image of Tharsis Limb Cloud 7 September 2005 This composite of red and blue Mars Global Surveyor (MGS) Mars Orbiter Camera (MOC) daily global images acquired on 6 July 2005 shows an isolated water ice cloud extending more than 30 kilometers (more than 18 miles) above the martian surface. Clouds such as this are common in late spring over the terrain located southwest of the Arsia Mons volcano. Arsia Mons is the dark, oval feature near the limb, just to the left of the 'T' in the 'Tharsis Montes' label. The dark, nearly circular feature above the 'S' in 'Tharsis' is the volcano, Pavonis Mons, and the other dark circular feature, above and to the right of 's' in 'Montes,' is Ascraeus Mons. Illumination is from the left/lower left. Season: Northern Autumn/Southern Spring

  6. BAECC Biogenic Aerosols - Effects on Clouds and Climate

    Energy Technology Data Exchange (ETDEWEB)

    Petäjä, Tuukka [Univ. of Helsinki (Finland); Moisseev, Dmitri [Univ. of Helsinki (Finland); Sinclair, Victoria [Univ. of Helsinki (Finland); O' Connor, Ewan J. [Finnish Meteorological Institute, Helsinki (Finland); Manninen, Antti J. [Univ. of Helsinki (Finland); Levula, Janne [Univ. of Helsinki (Finland); Väänänen, Riikka [Univ. of Helsinki (Finland); Heikkinen, Liine [Univ. of Helsinki (Finland); Äijälä, Mikko [Univ. of Helsinki (Finland); Aalto, Juho [Univ. of Helsinki (Finland); Bäck, Jaana [University of Helsinki, Finland

    2015-11-01

    “Biogenic Aerosols - Effects on Clouds and Climate (BAECC)”, featured the U.S. Department of Energy’s Atmospheric Radiation Measurement (ARM) Program’s 2nd Mobile Facility (AMF2) in Hyytiälä, Finland. It operated for an 8-month intensive measurement campaign from February to September 2014. The main research goal was to understand the role of biogenic aerosols in cloud formation. One of the reasons to perform BAECC study in Hyytiälä was the fact that it hosts SMEAR-II (Station for Measuring Forest Ecosystem-Atmosphere Relations), which is one of the world’s most comprehensive surface in-situ observation sites in a boreal forest environment. The station has been measuring atmospheric aerosols, biogenic emissions and an extensive suite of parameters relevant to atmosphere-biosphere interactions continuously since 1996. The BAECC enables combining vertical profiles from AMF2 with surface-based in-situ SMEAR-II observations and allows the processes at the surface to be directly related to processes occurring throughout the entire tropospheric column. With the inclusion of extensive surface precipitation measurements, and intensive observation periods involving aircraft flights and novel radiosonde launches, the complementary observations of AMF2 and SMEAR-II provide a unique opportunity for investigating aerosol-cloud interactions, and cloud-to-precipitation processes. The BAECC dataset will initiate new opportunities for evaluating and improving models of aerosol sources and transport, cloud microphysical processes, and boundary-layer structures.

  7. Modelling micro- and macrophysical contributors to the dissipation of an Arctic mixed-phase cloud during the Arctic Summer Cloud Ocean Study (ASCOS

    Directory of Open Access Journals (Sweden)

    K. Loewe

    2017-06-01

    Full Text Available The Arctic climate is changing; temperature changes in the Arctic are greater than at midlatitudes, and changing atmospheric conditions influence Arctic mixed-phase clouds, which are important for the Arctic surface energy budget. These low-level clouds are frequently observed across the Arctic. They impact the turbulent and radiative heating of the open water, snow, and sea-ice-covered surfaces and influence the boundary layer structure. Therefore the processes that affect mixed-phase cloud life cycles are extremely important, yet relatively poorly understood. In this study, we present sensitivity studies using semi-idealized large eddy simulations (LESs to identify processes contributing to the dissipation of Arctic mixed-phase clouds. We found that one potential main contributor to the dissipation of an observed Arctic mixed-phase cloud, during the Arctic Summer Cloud Ocean Study (ASCOS field campaign, was a low cloud droplet number concentration (CDNC of about 2 cm−3. Introducing a high ice crystal concentration of 10 L−1 also resulted in cloud dissipation, but such high ice crystal concentrations were deemed unlikely for the present case. Sensitivity studies simulating the advection of dry air above the boundary layer inversion, as well as a modest increase in ice crystal concentration of 1 L−1, did not lead to cloud dissipation. As a requirement for small droplet numbers, pristine aerosol conditions in the Arctic environment are therefore considered an important factor determining the lifetime of Arctic mixed-phase clouds.

  8. The Impact of Cloud Properties on Young Sea Ice during Three Winter Storms at N-ICE2015

    Science.gov (United States)

    Murphy, S. Y.; Walden, V. P.; Cohen, L.; Hudson, S. R.

    2017-12-01

    The impact of clouds on sea ice varies significantly as cloud properties change. Instruments deployed during the Norwegian Young Sea Ice field campaign (N-ICE2015) are used to study how differing cloud properties influence the cloud radiative forcing at the sea ice surface. N-ICE2015 was the first campaign in the Arctic winter since SHEBA (1997/1998) to study the surface energy budget of sea ice and the associated effects of cloud properties. Cloud characteristics, surface radiative and turbulent fluxes, and meteorological properties were measured throughout the field campaign. Here we explore how cloud macrophysical and microphysical properties affect young, thin sea ice during three winter storms from 31 January to 15 February 2015. This time period is of interest due to the varying surface and atmospheric conditions, which showcase the variety of conditions the newly-formed sea ice can experience during the winter. This period was characterized by large variations in the ice surface and near-surface air temperatures, with highs near 0°C when warm, moist air was advected into the area and lows reaching -40°C during clear, calm periods between storms. The advection of warm, moist air into the area influenced the cloud properties and enhanced the downwelling longwave flux. For most of the period, downwelling longwave flux correlates closely with the air temperature. However, at the end of the first storm, a drop in downwelling longwave flux of about 50 Wm-2 was observed, independent of any change in surface or air temperature or cloud fraction, indicating a change in cloud properties. Lidar data show an increase in cloud height during this period and a potential shift in cloud phase from ice to mixed-phase. This study will describe the cloud properties during the three winter storms and discuss their impacts on surface energy budget.

  9. Solar wind control of stratospheric temperatures in Jupiter's auroral regions?

    Science.gov (United States)

    Sinclair, James Andrew; Orton, Glenn; Kasaba, Yasumasa; Sato, Takao M.; Tao, Chihiro; Waite, J. Hunter; Cravens, Thomas; Houston, Stephen; Fletcher, Leigh; Irwin, Patrick; Greathouse, Thomas K.

    2017-10-01

    Auroral emissions are the process through which the interaction of a planet’s atmosphere and its external magnetosphere can be studied. Jupiter exhibits auroral emission at a multitude of wavelengths including the X-ray, ultraviolet and near-infrared. Enhanced emission of CH4 and other stratospheric hydrocarbons is also observed coincident with Jupiter’s shorter-wavelength auroral emission (e.g. Caldwell et al., 1980, Icarus 44, 667-675, Kostiuk et al., 1993, JGR 98, 18823). This indicates that auroral processes modify the thermal structure and composition of the auroral stratosphere. The exact mechanism responsible for this auroral-related heating of the stratosphere has however remained elusive (Sinclair et al., 2017a, Icarus 292, 182-207, Sinclair et al., 2017b, GRL, 44, 5345-5354). We will present an analysis of 7.8-μm images of Jupiter measured by COMICS (Cooled Mid-Infrared Camera and Spectrograph, Kataza et al., 2000, Proc. SPIE(4008), 1144-1152) on the Subaru telescope. These images were acquired on January 11th, 12th, 13th, 14th, February 4, 5th and May 17th, 18th, 19th and 20th in 2017, allowing the daily variability of Jupiter’s auroral-related stratospheric heating to be tracked. Preliminary results suggest lower stratospheric temperatures are directly forced by the solar wind dynamical pressure. The southern auroral hotspot exhibited a significant increase in brightness temperature over a 24-hour period. Over the same time period, a solar wind propagation model (Tao et al. 2005, JGR 110, A11208) predicts a strong increase in the solar wind dynamical pressure at Jupiter.

  10. A consistent definition of the Arctic polar vortex breakup in both the lower and upper stratosphere

    Science.gov (United States)

    Choi, W.; Seo, J.

    2014-12-01

    Breakup of the polar vortex is a dominant feature of the seasonal transition from winter to summer in the stratosphere, which significantly affects stratospheric O3 concentration and tropospheric weather. Previously several criteria for the vortex breakup have been suggested based on the potential vorticity (PV) and wind speed, however, those mainly have focused on the lower stratospheric vortex of which spatiotemporal evolution and decay are more continuous than those of the upper stratospheric vortex. To find a consistent criterion for the vortex breakup in both the lower and upper stratosphere, the present study defined a polar vortex breakup day as when PV gradient at the polar vortex edge becomes lower than that at the subtropical edge on the area equivalent latitude based on PV. With applying the new definition to the UK Met Office reanalysis data, the breakup days of the Arctic polar vortices on 18 isentropic levels from 450 K to 1300 K were calculated for the period of 1993-2005. In comparison with CH4, N2O and O3 measured by the ILAS and POAM II/III satellite instruments, the breakup days are well consistent with changes in the distribution of such tracers as well as their zonal standard deviations associated with the vortex structure breaking and irreversible mixing. The vortex breakup in the upper stratosphere occurs more or less a month prior to that in the middle and lower stratosphere while the stratospheric final warming events occurs simultaneously in the upper and lower stratosphere.

  11. Trends and solar cycle effects in mesospheric ice clouds

    Science.gov (United States)

    Lübken, Franz-Josef; Berger, Uwe; Fiedler, Jens; Baumgarten, Gerd; Gerding, Michael

    Lidar observations of mesospheric ice layers (noctilucent clouds, NLC) are now available since 12 years which allows to study solar cycle effects on NLC parameters such as altitudes, bright-ness, and occurrence rates. We present observations from our lidar stations in Kuehlungsborn (54N) and ALOMAR (69N). Different from general expectations the mean layer characteris-tics at ALOMAR do not show a persistent anti-correlation with solar cycle. Although a nice anti-correlation of Ly-alpha and occurrence rates is detected in the first half of the solar cycle, occurrence rates decreased with decreasing solar activity thereafter. Interestingly, in summer 2009 record high NLC parameters were detected as expected in solar minimum conditions. The morphology of NLC suggests that other processes except solar radiation may affect NLC. We have recently applied our LIMA model to study in detail the solar cycle effects on tempera-tures and water vapor concentration the middle atmosphere and its subsequent influence on mesospheric ice clouds. Furthermore, lower atmosphere effects are implicitly included because LIMA nudges to the conditions in the troposphere and lower stratosphere. We compare LIMA results regarding solar cycle effects on temperatures and ice layers with observations at ALO-MAR as well as satellite borne measurements. We will also present LIMA results regarding the latitude variation of solar cycle and trends, including a comparison of northern and southern hemisphere. We have adapted the observation conditions from SBUV (wavelength and scatter-ing angle) in LIMA for a detailed comparison with long term observations of ice clouds from satellites.

  12. Cloud Infrastructure & Applications - CloudIA

    Science.gov (United States)

    Sulistio, Anthony; Reich, Christoph; Doelitzscher, Frank

    The idea behind Cloud Computing is to deliver Infrastructure-as-a-Services and Software-as-a-Service over the Internet on an easy pay-per-use business model. To harness the potentials of Cloud Computing for e-Learning and research purposes, and to small- and medium-sized enterprises, the Hochschule Furtwangen University establishes a new project, called Cloud Infrastructure & Applications (CloudIA). The CloudIA project is a market-oriented cloud infrastructure that leverages different virtualization technologies, by supporting Service-Level Agreements for various service offerings. This paper describes the CloudIA project in details and mentions our early experiences in building a private cloud using an existing infrastructure.

  13. Tritium Records to Trace Stratospheric Moisture Inputs in Antarctica

    Science.gov (United States)

    Fourré, E.; Landais, A.; Cauquoin, A.; Jean-Baptiste, P.; Lipenkov, V.; Petit, J.-R.

    2018-03-01

    Better assessing the dynamic of stratosphere-troposphere exchange is a key point to improve our understanding of the climate dynamic in the East Antarctica Plateau, a region where stratospheric inputs are expected to be important. Although tritium (3H or T), a nuclide naturally produced mainly in the stratosphere and rapidly entering the water cycle as HTO, seems a first-rate tracer to study these processes, tritium data are very sparse in this region. We present the first high-resolution measurements of tritium concentration over the last 50 years in three snow pits drilled at the Vostok station. Natural variability of the tritium records reveals two prominent frequencies, one at about 10 years (to be related to the solar Schwabe cycles) and the other one at a shorter periodicity: despite dating uncertainty at this short scale, a good correlation is observed between 3H and Na+ and an anticorrelation between 3H and δ18O measured on an individual pit. The outputs from the LMDZ Atmospheric General Circulation Model including stable water isotopes and tritium show the same 3H-δ18O anticorrelation and allow further investigation on the associated mechanism. At the interannual scale, the modeled 3H variability matches well with the Southern Annular Mode index. At the seasonal scale, we show that modeled stratospheric tritium inputs in the troposphere are favored in winter cold and dry conditions.

  14. Reduction of secondary electron yield for E-cloud mitigation by laser ablation surface engineering

    Energy Technology Data Exchange (ETDEWEB)

    Valizadeh, R., E-mail: reza.valizadeh@stfc.ac.uk [ASTeC, STFC Daresbury Laboratory, Warrington WA4 4AD (United Kingdom); Malyshev, O.B. [ASTeC, STFC Daresbury Laboratory, Warrington WA4 4AD (United Kingdom); Wang, S. [ASTeC, STFC Daresbury Laboratory, Warrington WA4 4AD (United Kingdom); Department of Physics, Loughborough University, Loughborough LE11 3TU (United Kingdom); Sian, T. [ASTeC, STFC Daresbury Laboratory, Warrington WA4 4AD (United Kingdom); The Photon Science Institute, The University of Manchester, Manchester M13 9PL (United Kingdom); Cropper, M.D. [Department of Physics, Loughborough University, Loughborough LE11 3TU (United Kingdom); Sykes, N. [Micronanics Ltd., Didcot, Oxon OX11 0QX (United Kingdom)

    2017-05-15

    Highlights: • SEY below 1 can be achieved with Laser ablation surface engineering. • SEY <1 surface can be produced with different types of nanosecond lasers. • Both microstructure (groves) and nano-structures are playing a role in reducing SEY. - Abstract: Developing a surface with low Secondary Electron Yield (SEY) is one of the main ways of mitigating electron cloud and beam-induced electron multipacting in high-energy charged particle accelerators. In our previous publications, a low SEY < 0.9 for as-received metal surfaces modified by a nanosecond pulsed laser was reported. In this paper, the SEY of laser-treated blackened copper has been investigated as a function of different laser irradiation parameters. We explore and study the influence of micro- and nano-structures induced by laser surface treatment in air of copper samples as a function of various laser irradiation parameters such as peak power, laser wavelength (λ = 355 nm and 1064 nm), number of pulses per point (scan speed and repetition rate) and fluence, on the SEY. The surface chemical composition was determined by x-ray photoelectron spectroscopy (XPS) which revealed that heating resulted in diffusion of oxygen into the bulk and induced the transformation of CuO to sub-stoichiometric oxide. The surface topography was examined with high resolution scanning electron microscopy (HRSEM) which showed that the laser-treated surfaces are dominated by microstructure grooves and nanostructure features.

  15. Aerosol properties and their impacts on surface CCN at the ARM Southern Great Plains site during the 2011 Midlatitude Continental Convective Clouds Experiment

    Science.gov (United States)

    Logan, Timothy; Dong, Xiquan; Xi, Baike

    2018-02-01

    Aerosol particles are of particular importance because of their impacts on cloud development and precipitation processes over land and ocean. Aerosol properties as well as meteorological observations from the Department of Energy Atmospheric Radiation Measurement (ARM) platform situated in the Southern Great Plains (SGP) are utilized in this study to illustrate the dependence of continental cloud condensation nuclei (CCN) number concentration ( N CCN) on aerosol type and transport pathways. ARM-SGP observations from the 2011 Midlatitude Continental Convective Clouds Experiment field campaign are presented in this study and compared with our previous work during the 2009-10 Clouds, Aerosol, and Precipitation in the Marine Boundary Layer field campaign over the current ARM Eastern North Atlantic site. Northerly winds over the SGP reflect clean, continental conditions with aerosol scattering coefficient ( σ sp) values less than 20 Mm-1 and N CCN values less than 100 cm-3. However, southerly winds over the SGP are responsible for the observed moderate to high correlation ( R) among aerosol loading ( σ sp moisture via the Gulf of Mexico, indicating a strong dependence on air mass type. NASA MERRA-2 reanalysis aerosol and chemical data are moderately to highly correlated with surface ARM-SGP data, suggesting that this facility can represent surface aerosol conditions in the SGP, especially during strong aerosol loading events that transport via the Gulf of Mexico. Future long-term investigations will help to understand the seasonal influences of air masses on aerosol, CCN, and cloud properties over land in comparison to over ocean.

  16. Cloud-Resolving Model Simulations of Aerosol-Cloud Interactions Triggered by Strong Aerosol Emissions in the Arctic

    Science.gov (United States)

    Wang, H.; Kravitz, B.; Rasch, P. J.; Morrison, H.; Solomon, A.

    2014-12-01

    Previous process-oriented modeling studies have highlighted the dependence of effectiveness of cloud brightening by aerosols on cloud regimes in warm marine boundary layer. Cloud microphysical processes in clouds that contain ice, and hence the mechanisms that drive aerosol-cloud interactions, are more complicated than in warm clouds. Interactions between ice particles and liquid drops add additional levels of complexity to aerosol effects. A cloud-resolving model is used to study aerosol-cloud interactions in the Arctic triggered by strong aerosol emissions, through either geoengineering injection or concentrated sources such as shipping and fires. An updated cloud microphysical scheme with prognostic aerosol and cloud particle numbers is employed. Model simulations are performed in pure super-cooled liquid and mixed-phase clouds, separately, with or without an injection of aerosols into either a clean or a more polluted Arctic boundary layer. Vertical mixing and cloud scavenging of particles injected from the surface is still quite efficient in the less turbulent cold environment. Overall, the injection of aerosols into the Arctic boundary layer can delay the collapse of the boundary layer and increase low-cloud albedo. The pure liquid clouds are more susceptible to the increase in aerosol number concentration than the mixed-phase clouds. Rain production processes are more effectively suppressed by aerosol injection, whereas ice precipitation (snow) is affected less; thus the effectiveness of brightening mixed-phase clouds is lower than for liquid-only clouds. Aerosol injection into a clean boundary layer results in a greater cloud albedo increase than injection into a polluted one, consistent with current knowledge about aerosol-cloud interactions. Unlike previous studies investigating warm clouds, the impact of dynamical feedback due to precipitation changes is small. According to these results, which are dependent upon the representation of ice nucleation

  17. Ten Years of Cloud Optical and Microphysical Retrievals from MODIS

    Science.gov (United States)

    Platnick, Steven; King, Michael D.; Wind, Galina; Hubanks, Paul; Arnold, G. Thomas; Amarasinghe, Nandana

    2010-01-01

    The MODIS cloud optical properties algorithm (MOD06/MYD06 for Terra and Aqua MODIS, respectively) has undergone extensive improvements and enhancements since the launch of Terra. These changes have included: improvements in the cloud thermodynamic phase algorithm; substantial changes in the ice cloud light scattering look up tables (LUTs); a clear-sky restoral algorithm for flagging heavy aerosol and sunglint; greatly improved spectral surface albedo maps, including the spectral albedo of snow by ecosystem; inclusion of pixel-level uncertainty estimates for cloud optical thickness, effective radius, and water path derived for three error sources that includes the sensitivity of the retrievals to solar and viewing geometries. To improve overall retrieval quality, we have also implemented cloud edge removal and partly cloudy detection (using MOD35 cloud mask 250m tests), added a supplementary cloud optical thickness and effective radius algorithm over snow and sea ice surfaces and over the ocean, which enables comparison with the "standard" 2.1 11m effective radius retrieval, and added a multi-layer cloud detection algorithm. We will discuss the status of the MOD06 algorithm and show examples of pixellevel (Level-2) cloud retrievals for selected data granules, as well as gridded (Level-3) statistics, notably monthly means and histograms (lD and 2D, with the latter giving correlations between cloud optical thickness and effective radius, and other cloud product pairs).

  18. Stratospheric aerosols and precursor gases

    Science.gov (United States)

    1982-01-01

    Measurements were made of the aerosol size, height and geographical distribution, their composition and optical properties, and their temporal variation with season and following large volcanic eruptions. Sulfur-bearing gases were measured in situ in the stratosphere, and studied of the chemical and physical processes which control gas-to-particle conversion were carried out in the laboratory.

  19. Thermodynamic control of anvil cloud amount

    Science.gov (United States)

    Bony, Sandrine; Stevens, Bjorn; Coppin, David; Becker, Tobias; Reed, Kevin A.; Voigt, Aiko

    2016-01-01

    General circulation models show that as the surface temperature increases, the convective anvil clouds shrink. By analyzing radiative–convective equilibrium simulations, we show that this behavior is rooted in basic energetic and thermodynamic properties of the atmosphere: As the climate warms, the clouds rise and remain at nearly the same temperature, but find themselves in a more stable atmosphere; this enhanced stability reduces the convective outflow in the upper troposphere and decreases the anvil cloud fraction. By warming the troposphere and increasing the upper-tropospheric stability, the clustering of deep convection also reduces the convective outflow and the anvil cloud fraction. When clouds are radiatively active, this robust coupling between temperature, high clouds, and circulation exerts a positive feedback on convective aggregation and favors the maintenance of strongly aggregated atmospheric states at high temperatures. This stability iris mechanism likely contributes to the narrowing of rainy areas as the climate warms. Whether or not it influences climate sensitivity requires further investigation. PMID:27412863

  20. Sulfate Aerosols from Non-Explosive Volcanoes: Chemical-Radiative Effects in the Troposphere and Lower Stratosphere

    Directory of Open Access Journals (Sweden)

    Giovanni Pitari

    2016-06-01

    Full Text Available SO2 and H2S are the two most important gas-phase sulfur species emitted by volcanoes, with a global amount from non-explosive emissions of the order 10 Tg-S/yr. These gases are readily oxidized forming SO42− aerosols, which effectively scatter the incoming solar radiation and cool the surface. They also perturb atmospheric chemistry by enhancing the NOx to HNO3 heterogeneous conversion via hydrolysis on the aerosol surface of N2O5 and Br-Cl nitrates. This reduces formation of tropospheric O3 and the OH to HO2 ratio, thus limiting the oxidation of CH4 and increasing its lifetime. In addition to this tropospheric chemistry perturbation, there is also an impact on the NOx heterogeneous chemistry in the lower stratosphere, due to vertical transport of volcanic SO2 up to the tropical tropopause layer. Furthermore, the stratospheric O3 formation and loss, as well as the NOx budget, may be slightly affected by the additional amount of upward diffused solar radiation and consequent increase of photolysis rates. Two multi-decadal time-slice runs of a climate-chemistry-aerosol model have been designed for studying these chemical-radiative effects. A tropopause mean global net radiative flux change (RF of −0.23 W·m−2 is calculated (including direct and indirect aerosol effects with a 14% increase of the global mean sulfate aerosol optical depth. A 5–15 ppt NOx decrease is found in the mid-troposphere subtropics and mid-latitudes and also from pole to pole in the lower stratosphere. The tropospheric NOx perturbation triggers a column O3 decrease of 0.5–1.5 DU and a 1.1% increase of the CH4 lifetime. The surface cooling induced by solar radiation scattering by the volcanic aerosols induces a tropospheric stabilization with reduced updraft velocities that produce ice supersaturation conditions in the upper troposphere. A global mean 0.9% decrease of the cirrus ice optical depth is calculated with an indirect RF of −0.08 W·m−2.