WorldWideScience

Sample records for resonant coherent excitation

  1. Coherence-Resonance Chimeras in a Network of Excitable Elements.

    Science.gov (United States)

    Semenova, Nadezhda; Zakharova, Anna; Anishchenko, Vadim; Schöll, Eckehard

    2016-07-01

    We demonstrate that chimera behavior can be observed in nonlocally coupled networks of excitable systems in the presence of noise. This phenomenon is distinct from classical chimeras, which occur in deterministic oscillatory systems, and it combines temporal features of coherence resonance, i.e., the constructive role of noise, and spatial properties of chimera states, i.e., the coexistence of spatially coherent and incoherent domains in a network of identical elements. Coherence-resonance chimeras are associated with alternating switching of the location of coherent and incoherent domains, which might be relevant in neuronal networks.

  2. Energy harvesting from coherent resonance of horizontal vibration of beam excited by vertical base motion

    Energy Technology Data Exchange (ETDEWEB)

    Lan, C. B.; Qin, W. Y. [Department of Engineering Mechanics, Northwestern Polytechnical University, Xi' an 710072 (China)

    2014-09-15

    This letter investigates the energy harvesting from the horizontal coherent resonance of a vertical cantilever beam subjected to the vertical base excitation. The potential energy of the system has two symmetric potential wells. So, under vertical excitation, the system can jump between two potential wells, which will lead to the large vibration in horizontal direction. Two piezoelectric patches are pasted to harvest the energy. From experiment, it is found that the vertical excitation can make the beam turn to be bistable. The system can transform vertical vibration into horizontal vibration of low frequency when excited by harmonic motion. The horizontal coherence resonance can be observed when excited by a vertical white noise. The corresponding output voltages of piezoelectric films reach high values.

  3. Coherent secondary emission from resonantly excited two-exciton states

    DEFF Research Database (Denmark)

    Birkedal, Dan

    2000-01-01

    to the nonlinear susceptibility. The method exploits that emission from two-exciton coherences can occur in non-specular directions, with the recoil momentum taken up by an exciton left behind in the sample. Using ultrafast spectral interferometry we demonstrate the presence of this new coherent component...

  4. Reversible quantum optical data storage based on resonant Raman optical field excited spin coherence.

    Science.gov (United States)

    Ham, Byoung S

    2008-09-01

    A method of reversible quantum optical data storage is presented using resonant Raman field excited spin coherence, where the spin coherence is stored in an inhomogeneously broadened spin ensemble. Unlike the photon echo method, in the present technique, a 2pi Raman optical rephasing pulse area is used and multimode (parallel) optical channels are available in which the multimode access gives a great benefit to quantum information processors such as quantum repeaters.

  5. Vibronic resonances sustain excited state coherence in light harvesting proteins at room temperature

    CERN Document Server

    Novelli, Fabio; Roozbeh, Ashkan; Wilk, Krystyna E; Curmi, Paul M G; Davis, Jeffrey A

    2015-01-01

    Until recently it was believed that photosynthesis, a fundamental process for life on earth, could be fully understood with semi-classical models. However, puzzling quantum phenomena have been observed in several photosynthetic pigment-protein complexes, prompting questions regarding the nature and role of these effects. Recent attention has focused on discrete vibrational modes that are resonant or quasi-resonant with excitonic energy splittings and strongly coupled to these excitonic states. Here we report a series of experiments that unambiguously identify excited state coherent superpositions that dephase on the timescale of the excited state lifetime. Low energy (56 cm-1) oscillations on the signal intensity provide direct experimental evidence for the role of vibrational modes resonant with excitonic splittings in sustaining coherences involving different excited excitonic states at physiological temperature.

  6. Coherence-Resonance-Induced Neuronal Firing near a Saddle-Node and Homoclinic Bifurcation Corresponding to Type-I Excitability

    Institute of Scientific and Technical Information of China (English)

    JIA Bing; GU Hua-Guang; LI Yu-Ye

    2011-01-01

    @@ Excitability is an essential characteristic of excitable media such as nervous and cardiac systems.Different types of neuronal excitability are related to different bifurcation structures.We simulate the coherence resonance effect near a saddle-node and homoclinic bifurcation corresponding to type-I excitability in a theoretical neuron model,and recognize the obvious features of the corresponding firing pattern.Similar firing patterns are discovered in rat hippocampal CA1 pyramidal neurons.The results are not only helpful for understanding the dynamics of the saddle-node bifurcation and type-I excitability in a realistic nervous system,but also provide a practical indicator to identify types of excitability and bifurcation.%Excitability is an essential characteristic of excitable media such as nervous and cardiac systems. Different types of neuronal excitability are related to different bifurcation structures. We simulate the coherence resonance effect near a saddle-node and homoclinic bifurcation corresponding to type-I excitability in a theoretical neuron model, and recognize the obvious features of the corresponding firing pattern. Similar firing patterns are discovered in rat hippocampal CA1 pyramidal neurons. The results are not only helpful for understanding the dynamics of the saddle-node bifurcation and type-I excitability in a realistic nervous system, but also provide a practical indicator to identify types of excitability and bifurcation.

  7. Polarization-Dependent Interference of Coherent Scattering from Orthogonal Dipole Moments of a Resonantly Excited Quantum Dot

    Science.gov (United States)

    Chen, Disheng; Lander, Gary R.; Solomon, Glenn S.; Flagg, Edward B.

    2017-01-01

    Resonant photoluminescence excitation (RPLE) spectra of a neutral InGaAs quantum dot show unconventional line shapes that depend on the detection polarization. We characterize this phenomenon by performing polarization-dependent RPLE measurements and simulating the measured spectra with a three-level quantum model. The spectra are explained by interference between fields coherently scattered from the two fine structure split exciton states, and the measurements enable extraction of the steady-state coherence between the two exciton states.

  8. Coherent phonon spectroscopy of non-fully symmetric modes using resonant terahertz excitation

    Energy Technology Data Exchange (ETDEWEB)

    Huber, T., E-mail: tihuber@phys.ethz.ch; Huber, L.; Johnson, S. L. [Institute for Quantum Electronics, Physics Department, ETH Zurich, CH-8093 Zurich (Switzerland); Ranke, M. [The Hamburg Centre for Ultrafast Imaging, Luruper Chaussee 149, D-22761 Hamburg (Germany); Ferrer, A. [Institute for Quantum Electronics, Physics Department, ETH Zurich, CH-8093 Zurich (Switzerland); Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen PSI (Switzerland)

    2015-08-31

    We use intense terahertz (THz) frequency electromagnetic pulses generated via optical rectification in an organic crystal to drive vibrational lattice modes in single crystal Tellurium. The coherent modes are detected by measuring the polarization changes of femtosecond laser pulses reflecting from the sample surface, resulting in a phase-resolved detection of the coherent lattice motion. We compare the data to a model of Lorentz oscillators driven by the near-single-cycle broadband THz pulse. The demonstrated technique of optically probed coherent phonon spectroscopy with THz frequency excitation could prove to be a viable alternative to other time-resolved spectroscopic methods like standard THz time domain spectroscopy.

  9. Selective excitation of molecular mode in a mixture by femtosecond resonance-enhanced coherent anti-Stokes Raman scattering spectroscopy

    Institute of Scientific and Technical Information of China (English)

    He Ping; Li Si-Ning; Fan Rong-Wei; Li Xiao-Hui; Xia Yuan-Qin; Yu Xin; Chen De-Ying

    2012-01-01

    Femtosecond time-resolved coherent anti-Stokes Raman scattering (CARS) spectroscopy is used to investigate gaseous molecular dynamics.Due to the spectrally broad laser pulses,usually poorly resolved spectra result from this broad spectroscopy.However,it can be demonstrated that by the electronic resonance enhancement optimization control a selective excitation of specific vibrational mode is possible.Using an electronically resonance-enhanced effect,iodine molecule specific CARS spectroscopy can be obtained from a mixture of iodine-air at room temperature and a pressure of 1 atm (corresponding to a saturation iodine vapour as low as about 35 Pa).The dynamics on either the electronically excited state or the ground state of iodine molecules obtained is consistent with previous studies (vacuum,heated and pure iodine) in the femtosecond time resolved CARS spectroscopy,showing that an effective method of suppressing the non-resonant CARS background and other interferences is demonstrated.

  10. Combining THz laser excitation with resonant soft X-ray scattering at the Linac Coherent Light Source

    Energy Technology Data Exchange (ETDEWEB)

    Turner, Joshua J., E-mail: joshuat@slac.stanford.edu; Dakovski, Georgi L.; Hoffmann, Matthias C. [Linac Coherent Light Source, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025 (United States); Hwang, Harold Y. [Department of Chemistry, Massachusetts Institute of Technology, Cambridge, MA 02139 (United States); Zarem, Alex; Schlotter, William F.; Moeller, Stefan; Minitti, Michael P. [Linac Coherent Light Source, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025 (United States); Staub, Urs [Swiss Light Source, Paul Scherrer Institut, 5232 Villigen (Switzerland); Johnson, Steven [ETH Zurich, Institute for Quantum Electronics, Wolfgang-Pauli-Strasse 16, 8093 Zurich (Switzerland); Mitra, Ankush; Swiggers, Michele; Noonan, Peter; Curiel, G. Ivan; Holmes, Michael [Linac Coherent Light Source, SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, CA 94025 (United States)

    2015-04-11

    This paper describes new instrumentation developments at the LCLS for materials studies using THz laser excitation and resonant soft X-ray scattering. This paper describes the development of new instrumentation at the Linac Coherent Light Source for conducting THz excitation experiments in an ultra high vacuum environment probed by soft X-ray diffraction. This consists of a cantilevered, fully motorized mirror system which can provide 600 kV cm{sup −1} electric field strengths across the sample and an X-ray detector that can span the full Ewald sphere with in-vacuum motion. The scientific applications motivated by this development, the details of the instrument, and spectra demonstrating the field strengths achieved using this newly developed system are discussed.

  11. RESONANT CAVITY EXCITATION SYSTEM

    Science.gov (United States)

    Baker, W.R.; Kerns, Q.A.; Riedel, J.

    1959-01-13

    An apparatus is presented for exciting a cavity resonator with a minimum of difficulty and, more specifically describes a sub-exciter and an amplifier type pre-exciter for the high-frequency cxcitation of large cavities. Instead of applying full voltage to the main oscillator, a sub-excitation voltage is initially used to establish a base level of oscillation in the cavity. A portion of the cavity encrgy is coupled to the input of the pre-exciter where it is amplified and fed back into the cavity when the pre-exciter is energized. After the voltage in the cavity resonator has reached maximum value under excitation by the pre-exciter, full voltage is applied to the oscillator and the pre-exciter is tunned off. The cavity is then excited to the maximum high voltage value of radio frequency by the oscillator.

  12. Influence of optical coherence on the electron spin in singly charged InP quantum dots excited by resonant laser pulses

    Science.gov (United States)

    Tomimoto, Shinichi; Kawana, Keisuke; Murakami, Akira; Masumoto, Yasuaki

    2012-06-01

    We have experimentally studied the spin dynamics of excitons, electrons, and trions in charge-tunable InP/InGaP quantum dots (QDs) excited by picosecond resonant laser pulses by observing the time-resolved Kerr rotation. In singly charged QDs, inversion of the spin polarization direction of doped electrons is found to be caused simply by variation in the pulse intensity, which is accompanied by an abrupt change of the spin coherence time. This phenomenon is reproduced by density-matrix calculations allowing for the reaction on the QD electron-trion four-level system during its coherent radiation emission. This result means that the optical coherence is another critical factor affecting electron spin coherence.

  13. Resonance Radiation and Excited Atoms

    Science.gov (United States)

    Mitchell, Allan C. G.; Zemansky, Mark W.

    2009-06-01

    1. Introduction; 2. Physical and chemical effects connected with resonance radiation; 3. Absorption lines and measurements of the lifetime of the resonance state; 4. Collision processes involving excited atoms; 5. The polarization of resonance radiation; Appendix; Index.

  14. From Autonomous Coherence Resonance to Periodically Driven Stochastic Resonance

    Institute of Scientific and Technical Information of China (English)

    CAO Zhou-Jian; LI Peng-Fei; HU Gang

    2007-01-01

    In periodically driven nonlinear stochastic systems,noise may play a role of enhancing the output periodic signal (termed as stochastic resonance or SR).While in autonomous excitable systems,noise may play a role of increasing coherent motion(termed as coherence resonance or CR).So far the topics of SR and CR have been investigated separately as two major fields of studying the active roles of noise in nonlinear systems.We find that these two topics are closely related to each other.Specifically,SR occurs in such periodically driven systems that the corresponding autonomous systems show CR.The SR with sensitive frequency dependence can be observed when the corresponding autonomous system shows CR with finite characteristic frequency.Moreover,'resonant noise' and 'resonant frequency' of SR coincide with those of CR.

  15. Nuclear coherences in photosynthetic reaction centers following light excitation

    Energy Technology Data Exchange (ETDEWEB)

    Weber, S.; Norris, J.R. [Univ. of Chicago, IL (United States). Dept. of Chemistry; Berthold, T.; Ohmes, E.; Kothe, G. [Univ. of Freiburg (Germany). Dept. of Physical Chemistry; Thurnauer, M.C. [Argonne National Lab., IL (United States). Chemistry Div.

    1997-07-01

    Transient electron paramagnetic resonance is used to study the secondary radical pair in plant photosystem I. Nuclear coherences are observed in the transverse magnetization at lower temperatures following light excitation. Comparative studies of deuterated and deuterated {sup 15}N-substituted cyanobacteria S. lividus indicate assignment of these coherences to nitrogen nuclei in the primary donor and deuterons in the secondary acceptor. The modulation amplitude of a deuteron matrix line, as a function of the microwave power, reveals a distinct resonance behavior. The maximum amplitude is obtained when the Rabi frequency equals the nuclear Zeeman frequency.

  16. Electromagnetic Excitation of Nucleon Resonances

    CERN Document Server

    Tiator, L; Kamalov, S S; Vanderhaeghen, M

    2011-01-01

    Recent progress on the extraction of electromagnetic properties of nucleon resonance excitation through pion photo- and electroproduction is reviewed. Cross section data measured at MAMI, ELSA, and CEBAF are analyzed and compared to the analysis of other groups. On this basis, we derive longitudinal and transverse transition form factors for most of the four-star nucleon resonances. Furthermore, we discuss how the transition form factors can be used to obtain empirical transverse charge densities. Contour plots of the thus derived densities are shown for the Delta, Roper, S11, and D13 nucleon resonances.

  17. Coherent selection of invisible high-order electromagnetic excitations

    Science.gov (United States)

    Tseng, Ming Lun; Fang, Xu; Savinov, Vassili; Wu, Pin Chieh; Ou, Jun-Yu; Zheludev, Nikolay I.; Tsai, Din Ping

    2017-03-01

    Far-field spectroscopy and mapping of electromagnetic near-field distribution are the two dominant tools for analysis and characterization of the electromagnetic response in nanophotonics. Despite the widespread use, these methods can fail at identifying weak electromagnetic excitations masked by stronger neighboring excitations. This is particularly problematic in ultrafast nanophotonics, including optical sensing, nonlinear optics and nanolasers, where the broad resonant modes can overlap to a significant degree. Here, using plasmonic metamaterials, we demonstrate that coherent spectroscopy can conveniently isolate and detect such hidden high-order photonic excitations. Our results establish that the coherent spectroscopy is a powerful new tool. It complements the conventional methods for analysis of the electromagnetic response, and provides a new route to designing and characterizing novel photonic devices and materials.

  18. Quantum coherence in ion channels: Resonances, Transport and Verification

    CERN Document Server

    Vaziri, A

    2010-01-01

    Recently it was demonstrated that long-lived quantum coherence exists during excitation energy transport in photosynthesis. It is a valid question up to which length, time and mass scales quantum coherence may extend, how to one may detect this coherence and what if any role it plays for the dynamics of the system. Here we suggest that the selectivity filter of ion channels may exhibit quantum coherence which might be relevant for the process of ion selectivity and conduction. We show that quantum resonances could provide an alternative approch to ultrafast 2D spectroscopy to probe these quantum coherences. We demonstrate that the emergence of resonances in the conduction of ion channels that are modulated periodicallly by time dependent external electric fields can serve as signitures of quantum coherence in such a system. Assessments of experimental feasibility and specific paths towards the experimental realization of such experiments are presented. We show that this may be probed by direct 2-D spectroscop...

  19. Coherent acoustic excitation of cavity polaritons

    DEFF Research Database (Denmark)

    Poel, Mike van der; de Lima, M. M.; Hey, R.

    and highly nonlinear optical response.Our sample consists of epitaxially grown GaAs/AlGaAs QWs located at the anti-node ofa high Q lambda cavity, which is resonant with the QW excitonic transition3. The SAWfield, which is excited by an interdigital transducer on the piezoelectric GaAs samplesurface...

  20. Distributed coherent manipulation of qutrits by virtual excitation processes

    CERN Document Server

    Yang, Zhen-Biao; Serafini, Alessio; Zheng, Shi-Biao

    2009-01-01

    We propose a scheme for the deterministic coherent manipulation of two atomic qutrits, trapped in separate cavities coupled through a short optical fibre or optical resonator. We study such a system in the regime of dispersive atom-field interactions, where the dynamics of atoms, cavities and fibre operates through virtual population of both the atomic excited states and photonic states in the cavities and fibre. We show that the resulting effective dynamics allows for the creation of robust qutrit entanglement, and thoroughly investigate the influence of imperfections and dissipation, due to atomic spontaneous emission and photon leakage, on the entanglement of the two qutrits state.

  1. Distributed coherent manipulation of qutrits by virtual excitation processes

    Energy Technology Data Exchange (ETDEWEB)

    Yang Zhenbiao; Ye Saiyun; Zheng Shibiao [Department of Physics and State Key Laboratory Breeding Base of Photocatalysis, Fuzhou University, Fuzhou 350002 (China); Serafini, Alessio, E-mail: sbzheng@pub5.fz.fj.c [Department of Physics and Astronomy, University College London, Gower Street, London WC1E 6BT (United Kingdom)

    2010-04-28

    We propose a scheme for the deterministic coherent manipulation of two atomic qutrits, trapped in separate cavities coupled through a short optical fibre or optical resonator. We study such a system in the regime of dispersive atom-field interactions, where the dynamics of atoms, cavities and fibre operates through virtual population of both the atomic excited states and photonic states in the cavities and fibre. We show that the resulting effective dynamics allows for the creation of robust qutrit entanglement, and thoroughly investigate the influence of imperfections and dissipation, due to atomic spontaneous emission and photon leakage, on the entanglement of the two-qutrit state.

  2. Time-Resolved Speckle Analysis: A New Approach to Coherence and Dephasing of Optical Excitations in Solids

    DEFF Research Database (Denmark)

    Langbein, Wolfgang Werner; Hvam, Jørn Märcher; Zimmermann, R.

    1999-01-01

    A new method to measure the time-dependent coherence of both homogeneously and inhomogeneously broadened optical excitations in solids is presented. The coherence degree of resonantly excited light emission is deduced from the intensity fluctuations over the emission directions (speckles......). This method determines the decays of intensity and coherence separately, thus distinguishing lifetime from pure dephasing. The secondary emission of excitons in semiconductor quantum wells is investigated. Here the combination of static disorder and inelastic scattering leads to a partially coherent emission...

  3. Super-Resonant Intracavity Coherent Absorption

    CERN Document Server

    Malara, P; Giorgini, A; Avino, S; De Natale, P; Gagliardi, G

    2016-01-01

    The capability of optical resonators to extend the effective radiation-matter interaction length originates from a multipass effect, hence is intrinsically limited by the resonator quality factor. Here, we show that this constraint can be overcome by combining the concepts of resonant interaction and coherent perfect absorption. We demonstrate and investigate super-resonant coherent absorption in a coupled Fabry-Perot-ring cavity structure. At the FP resonant wavelengths, the described phenomenon gives rise to split modes with a nearly-transparent peak and a peak whose transmission is exceptionally sensitive to the intracavity loss. For small losses, the effective interaction pathlength of these modes is proportional respectively to the ratio and the product of the individual finesse coefficients of the two resonators. The results presented extend the conventional definition of resonant absorption and point to a way of circumventing the technological limitations of ultrahigh-quality resonators in spectroscopy...

  4. Spectrally tunable mollow triplet emission from a coherently excited quantum dot in a microcavity

    DEFF Research Database (Denmark)

    Ulrich, Sven M.; Ates, Serkan; Reitzenstein, Stephan

    2010-01-01

    Resonance fluorescence of excitonic s-shell emission from a coherently pumped single InGaAs/GaAs quantum dot inside a micropillar cavity has been investigated in dependence on optical pump power and laser detuning, respectively. For strong purely resonant excitation, Mollow triplet spectra...

  5. Generating Coherent Phonons and Spin Excitations with Ultrafast Light Pulses

    Science.gov (United States)

    Merlin, Roberto

    2006-03-01

    Recent work on the generation of coherent low-lying excitations by ultrafast laser pulses will be reviewed, emphasizing the microscopic mechanisms of light-matter interaction. The topics covered include long-lived phonons in ZnO [C. Aku-Leh, J. Zhao, R. Merlin, J. Men'endez and M. Cardona, Phys. Rev.B 71, 205211 (2005)], squeezed magnons [J. Zhao, A. V. Bragas, D. J. Lockwood and R. Merlin, Phys. Rev. Lett. 93, 107203 (2004)], spin- and charge-density fluctuations [J. M. Bao et al., Phys. Rev. Lett. 92, 236601 (2004)] and cyclotron resonance [J. K. Wahlstrand, D. M. Wang, P. Jacobs, J. M. Bao, R. Merlin, K. W. West and L. N. Pfeiffer, AIP Conference Proceedings 772 (2005), p. 1313] in GaAs quantum wells. In addition, unpublished results on surface -avoiding phonons in GaAs-AlAs superlattices [M. Trigo et al., unpublished] and magnons in ferromagnetic Ga1-xMnxAs [D. M. Wang et al., unpublished] will be discussed. It will also be shown that frequencies can be measured using pump-probe techniques with a precision comparable to that of Brillouin scattering. It is now widely accepted that stimulated Raman scattering (SRS) is (often but not always) the mechanism responsible for the coherent coupling. Results will be presented showing that SRS is described by two separate tensors, one of which accounts for the excitation-induced modulation of the susceptibility, and the other one for the dependence of the amplitude of the oscillation on the light intensity [T. E. Stevens, J. Kuhl and R. Merlin, Phys. Rev. B 65, 144304 (2002)]. These tensors have the same real component, associated with impulsive coherent generation, but different imaginary parts. If the imaginary term dominates, that is, for strongly absorbing substances, the mechanism for two-band processes becomes displacive in nature, as in the DECP (displacive excitation of coherent phonons) model. It will be argued that DECP is not a separate mechanism, but a particular case of SRS. In the final part of the talk, an

  6. Super-Resonant Intracavity Coherent Absorption

    Science.gov (United States)

    Malara, P.; Campanella, C. E.; Giorgini, A.; Avino, S.; de Natale, P.; Gagliardi, G.

    2016-07-01

    The capability of optical resonators to extend the effective radiation-matter interaction length originates from a multipass effect, hence is intrinsically limited by the resonator’s quality factor. Here, we show that this constraint can be overcome by combining the concepts of resonant interaction and coherent perfect absorption (CPA). We demonstrate and investigate super-resonant coherent absorption in a coupled Fabry-Perot (FP)/ring cavity structure. At the FP resonant wavelengths, the described phenomenon gives rise to split modes with a nearly-transparent peak and a peak whose transmission is exceptionally sensitive to the intracavity loss. For small losses, the effective interaction pathlength of these modes is proportional respectively to the ratio and the product of the individual finesse coefficients of the two resonators. The results presented extend the conventional definition of resonant absorption and point to a way of circumventing the technological limitations of ultrahigh-quality resonators in spectroscopy and optical sensing schemes.

  7. Coherent excitation of a single atom to a Rydberg state

    DEFF Research Database (Denmark)

    Miroshnychenko, Yevhen; Gaëtan, Alpha; Evellin, Charles

    2010-01-01

    We present the coherent excitation of a single Rubidium atom to the Rydberg state 58d3/2 using a two-photon transition. The experimental setup is described in detail, as are experimental techniques and procedures. The coherence of the excitation is revealed by observing Rabi oscillations between ...

  8. Coherent excitation of a single atom to a Rydberg state

    DEFF Research Database (Denmark)

    Miroshnychenko, Yevhen; Gaëtan, Alpha; Evellin, Charles

    2010-01-01

    We present the coherent excitation of a single Rubidium atom to the Rydberg state 58d3/2 using a two-photon transition. The experimental setup is described in detail, as are experimental techniques and procedures. The coherence of the excitation is revealed by observing Rabi oscillations between ...

  9. Floating Rydberg crystals formed by resonant excitation

    CERN Document Server

    Gärttner, M; Gasenzer, T; Evers, J

    2013-01-01

    The dynamics of a cloud of ultra-cold Rydberg atoms is studied at off-resonant laser driving. We find that excitation crystals are formed dynamically as a consequence of interaction-induced resonant excitations. These crystals have lattice constants independent of the trap length, are spatially not localized with respect to the trap, and sensitively depend on the shape of the interaction potential. Compared to previously proposed crystals, this leads to qualitatively different results for the spatial excitation density, the Mandel $Q$ parameter, and the total number of excitations.

  10. Wideband MEMS Resonator Using Multifrequency Excitation

    KAUST Repository

    Jaber, Nizar

    2016-03-09

    We demonstrate the excitation of combination resonances of additive and subtractive types and their exploitations to realize a large bandwidth micro-machined resonator of large amplitude even at higher harmonic modes of vibrations. The investigation is conducted on a Microelectromechanical systems (MEMS) clamped-clamped microbeam fabricated using polyimide as a structural layer coated with nickel from top and chromium and gold layers from bottom. The microbeam is excited by a two-source harmonic excitation, where the first frequency source is swept around the targeted resonance (first or third mode of vibration) while the second source frequency is kept fixed. We report for the first time a large bandwidth and large amplitude response near the higher order modes of vibration. Also, we show that by properly tuning the frequency and amplitude of the excitation force, the frequency bandwidth of the resonator is controlled.

  11. Efficient primary and parametric resonance excitation of bistable resonators

    KAUST Repository

    Ramini, Abdallah

    2016-09-12

    We experimentally demonstrate an efficient approach to excite primary and parametric (up to the 4th) resonance of Microelectromechanical system MEMS arch resonators with large vibrational amplitudes. A single crystal silicon in-plane arch microbeam is fabricated such that it can be excited axially from one of its ends by a parallel-plate electrode. Its micro/nano scale vibrations are transduced using a high speed camera. Through the parallel-plate electrode, a time varying electrostatic force is applied, which is converted into a time varying axial force that modulates dynamically the stiffness of the arch resonator. Due to the initial curvature of the structure, not only parametric excitation is induced, but also primary resonance. Experimental investigation is conducted comparing the response of the arch near primary resonance using the axial excitation to that of a classical parallel-plate actuation where the arch itself forms an electrode. The results show that the axial excitation can be more efficient and requires less power for primary resonance excitation. Moreover, unlike the classical method where the structure is vulnerable to the dynamic pull-in instability, the axial excitation technique can provide large amplitude motion while protecting the structure from pull-in. In addition to primary resonance, parametrical resonances are demonstrated at twice, one-half, and two-thirds the primary resonance frequency. The ability to actuate primary and/or parametric resonances can serve various applications, such as for resonator based logic and memory devices. (C) 2016 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license

  12. Spatially coherent surface resonance states derived from magnetic resonances

    CERN Document Server

    Wei, Zeyong; Cao, Yang; Wu, Chao; Ren, Jinzhi; Hang, Zhihong; Chen, Hong; Zhang, Daozhong; Chan, C T

    2010-01-01

    A thin metamaterial slab comprising a dielectric spacer sandwiched between a metallic grating and a ground plane is shown to possess spatially coherent surface resonance states that span a large frequency range and can be tuned by structural and material parameters. They give rise to nearly perfect angle-selective absorption and thus exhibit directional thermal emissivity. Direct numerical simulations show that the metamaterial slab supports spatially coherent thermal emission in a wide frequency range that is robust against structural disorder.

  13. Coherent blue emission generated by Rb two-photon excitation using diode and femtosecond lasers

    Science.gov (United States)

    Lopez, Jesus P.; Moreno, Marco P.; de Miranda, Marcio H. G.; Vianna, Sandra S.

    2017-04-01

    The coherent blue light generated in rubidium vapor due to the combined action of an ultrashort pulse train and a continuous wave diode laser is investigated. Each step of the two-photon transition 5S-5P{}3/2-5D is excited by one of the lasers, and the induced coherence between the 5S and 6P{}3/2 states is responsible for generating the blue beam. Measurements of the excitation spectrum reveal the frequency comb structure and allow us to identify the resonant modes responsible for inducing the nonlinear process. Further, each resonant mode excites a different group of atoms, making the process selective in atomic velocity. The signal dependency on the atomic density is characterized by a sharp growth and a rapid saturation. We also show that for high intensity of the diode laser, the Stark shift at resonance causes the signal suppression observed at low atomic density.

  14. Dynamic Coherence in Excitonic Molecular Complexes under Various Excitation Conditions

    CERN Document Server

    Chenu, Aurélia; Mancal, Tomáš

    2013-01-01

    In this paper, we investigate the relevance of dynamic electronic coherence under conditions natural to light-harvesting systems. We formulate the results of a quantum mechanical treatment of a weak light-matter interaction in terms of experimental observable, such as the incident light spectrum and the absorption spectrum of the material, and we derive the description of the incoherent F\\"orster type energy transfer fully from the wave function formalism. We demonstrate that excitation of a coherent superposition of electronic eigenstates of natural light-harvesting complexes by sunlight or by excitation transfer from a neighboring antenna is unlikely and that dynamical coherence therefore cannot play any significant role in natural photosynthesis, regardless of their life time. Dynamical coherence as a transient phenomenon must be strictly distinguished from the effect of excited state delocalization (also termed quantum coherence in the literature) which is established by interaction between the pigments a...

  15. Coherent and incoherent processes in resonant photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Magnuson, M.; Karis, O.; Weinelt, M. [Uppsala Univ. (Sweden)] [and others

    1997-04-01

    In this contribution the authors present the distinction between coherent and incoherent processes in resonant photoemission. As a first step they determine whether an autoionization process is photoemission-like or Auger-like. The discussion is based on measurements for a weakly bonded adsorption system, Ar/Pt(111). This type of system is well adapted to investigate these effects since it yields distinctly shifted spectral features depending on the nature of the process. After this, the question of resonance photoemission in metallic systems is addressed. This is done in connection with measurements at the 2p edges for Ni metal. Ni has been one of the prototype systems for resonant photoemission. The resonances have been discussed in connection with the strong correlation and d-band localization effects in this system. Based on the results some general comments about the appearance of resonant effects in metallic systems are made.

  16. Coherent versus incoherent excitation energy transfer in molecular systems.

    Science.gov (United States)

    Chang, Hung-Tzu; Cheng, Yuan-Chung

    2012-10-28

    We investigate the Markovian limit of a polaronic quantum master equation for coherent resonance energy transfer proposed recently by Jang et al. [J. Chem. Phys. 129, 101104 (2008)]. An expression for the rate of excitation energy transfer (EET) is derived and shown to exhibit both coherent and incoherent contributions. We then apply this theory to calculated EET rates for model dimer systems, and demonstrate that the small-polaron approach predicts a variety of dynamical behaviors. Notably, the results indicate that the EET dynamical behaviors can be understood by the interplay between noise-assisted EET and dynamical localization, while both are well captured by the polaron theory. Finally, we investigate bath correlation effects on the rate of EET and show that bath correlations (or anti-correlations) can either enhance or suppress EET rate depending on the strength of individual system-bath couplings. In summary, we introduce the small-polaron approach as an intuitive physical framework to consolidate our understanding of EET dynamics in the condensed phase.

  17. Coherent excitation of a single atom to a Rydberg state

    CERN Document Server

    Miroshnychenko, Y; Evellin, C; Grangier, P; Comparat, D; Pillet, P; Wilk, T; Browaeys, A

    2010-01-01

    We present the coherent excitation of a single Rubidium atom to the Rydberg state (58d3/2) using a two-photon transition. The experimental setup is described in detail, as well as experimental techniques and procedures. The coherence of the excitation is revealed by observing Rabi oscillations between ground and Rydberg states of the atom. We analyze the observed oscillations in detail and compare them to numerical simulations which include imperfections of our experimental system. Strategies for future improvements on the coherent manipulation of a single atom in our settings are given.

  18. Plasmon-polariton emission from a coherently p-excited quantum dot near a metal interface

    Science.gov (United States)

    Sanchez-Munoz, C.; Gonzalez-Tudela, A.; Tejedor, C.

    2012-03-01

    We study the emission of surface plasmon polaritons by the decay of the lowest excited state of a quantum emitter when the system is excited by a laser in resonance with a higher excited state (p-shell excitation). By solving a master equation and by using the quantum-regression theorem, we show how the emission is enhanced by the Purcell effect due to the weak coupling between the emitter and the structured spectral density of plasmon-polariton states of a metal surface. Measurable magnitudes, as the spectrum and the second-order coherence function, are extremely affected by the coherent p-shell excitation. In many cases, such coherent excitation completely masks the physical features of the emission under study. The coexistence between coherent p-shell excitation in the first step of the process and weak coupling in the final step is very important and completely general for any structured reservoir of final states. The advantage of our system is that, just by changing the distance from the quantum emitter to the metal surface, one can access a very rich set of regimes as purely dissipative direct photon emission or emission of plasmon polaritons.

  19. Double-excited resonant structure of photoionization

    Institute of Scientific and Technical Information of China (English)

    刘锦超; 杨向东; 王宗笠; 程延松

    1997-01-01

    The dominant diagrams were found in double-excited resonant structure of photoionization by using many-body perturbation theory.Based on the characteristics of these diagrams,the couple-equation method was improved,and the summation of specific classes of these diagrams is to an infinite order,and the resonant peaks with the widths are obtained first.The doubled-excited resonant structures (2p,3s)→(3p,np),(3p,nf),(3d,nd),(3d,ns) and (4s,ns) of the photoionization processes 2p→ks,kd are obtained.The photoionization with excitation process (2p,3s)→(3p,kp) was included in the calculations.The results of calculations are compared with the experimental data from 38.5 to 46.8 eV photon energies,which are in good agreement with the experiment.

  20. Excitation of multiple resonances in 1D Anderson localized systems for efficient light amplification.

    Science.gov (United States)

    Choi, Seung Ho; Byun, Kyung Min; Kim, Young L

    2015-03-01

    Excitation of hybridized multiple resonances can be an effective route for coherent light generation in irregular 1D systems larger than the localization length of light. Necklace states are often considered to have nonlocalized states. However, we propose that some hybridized/coupled states can have high-resonant tunneling with spatially extended fields. If strong localization properties are preserved in hybridized resonances, the excitation of such states allows for deposition of the excitation energy deep into the structure and spatial overlap with local gain regions. This result could allow for better utilizing hybridized resonances in biological or natural photonic systems.

  1. Observation of resonance fluorescence and the Mollow triplet from a coherently driven site-controlled quantum dot

    DEFF Research Database (Denmark)

    Unsleber, Sebastian; Maier, Sebastian; McCutcheon, Dara;

    2015-01-01

    Resonant excitation of solid state quantum emitters has the potential to deterministically excite a localized exciton while ensuring a maximally coherent emission. In this work, we demonstrate the coherent coupling of an exciton localized in a lithographically positioned, site-controlled semicond...

  2. Modeling noise-induced resonance in an excitable system: an alternative approach.

    Science.gov (United States)

    Nurujjaman, Md

    2010-03-01

    Recently, it has been observed [Md. Nurujjaman, Phy. Rev. E 80, 015201(R) (2009)] that in an excitable system, one can maintain noise-induced coherency in the coherence resonance by blocking the destructive effect of the noise on the system at higher noise level. This phenomenon of constant coherence resonance (CCR) cannot be explained by the existing way of simulation of the model equations of an excitable system with added noise. In this paper, we have proposed a general model which explains the noise-induced resonance phenomenon CCR as well as coherence resonance (CR) and stochastic resonance (SR). The simulation has been carried out considering the basic mechanism of noise-induced resonance phenomena: noise only perturbs the system control parameter to excite coherent oscillations, taking proper precautions so that the destructive effect of noise does not affect the system. In this approach, the CR has been obtained from the interference between the system output and noise and the SR has been obtained by adding noise and a subthreshold signal. This also explains the observation of the frequency shift of coherent oscillations in the CCR with noise level.

  3. Artificial Excitation of Schumann Resonance with HAARP

    Science.gov (United States)

    Streltsov, A. V.; Chang, C. L.

    2014-12-01

    We report results from the experiment aimed at the artificial excitation of extremely-low-frequency (ELF) electromagnetic waves with frequencies corresponding to the frequency of Schumann resonance (typically, 7.5 - 8.0 Hz frequency range). Electromagnetic waves with these frequencies can form a standing pattern inside the spherical cavity formed by the surface of the earth and the ionosphere. In the experiment the ELF waves were excited by heating the ionosphere with X-mode HF electromagnetic waves generated by the High Frequency Active Auroral Research Program (HAARP) facility in Alaska. The experiment demonstrates that heating of the ionosphere can excite relatively large-amplitude electromagnetic waves with frequencies in the range of the Schumann resonance, when the ionosphere has a strong F-layer and an electric field greater than 5 mV/m is present in the E-region.

  4. Interaction of coherent phonons with defects and elementary excitations

    Energy Technology Data Exchange (ETDEWEB)

    Hase, Muneaki [Institute of Applied Physics, University of Tsukuba, 1-1-1 Tennodai, Tsukuba 305-8573 (Japan); Kitajima, Masahiro, E-mail: mhase@bk.tsukuba.ac.j, E-mail: kitaji@nda.ac.j [Department of Applied Physics, School of Applied Science, National Defense Academy of Japan, Hashirimizu 1-10-20, Yokosuka, Kanagawa 239-8686 (Japan)

    2010-02-24

    We present an overview of the feasibility of using coherent phonon spectroscopy to study interaction dynamics of excited lattice vibrations with their environments. By exploiting the features of coherent phonons with a pump-probe technique, one can study lattice motions in a sub-picosecond time range. The dephasing properties tell us not only about interaction dynamics with carriers (electrons and holes) or thermal phonons but also about point defects in crystals. Modulations of the coherent phonon amplitude by more than two modes are closely related to phonon-carrier or phonon-phonon interferences. Related to this phenomenon, formation of coherent phonons at higher harmonics gives direct evidence for phonon-phonon couplings. A combined study of coherent phonons and ultrafast carrier response can be useful for understanding phonon-carrier interaction dynamics. For metals like zinc, nonequilibrium electrons may dominate the dynamics of both relaxation and generation of coherent phonons. The frequency chirp of coherent phonons can be a direct measure of how and when phonon-phonon and phonon-carrier couplings occur. Carbon nanotubes show some complicated behavior due to the existence of many modes with different symmetries, resulting in superposition or interference. To illustrate one of the most interesting applications, the selective excitation of specific phonon modes through the use of a pulse train technique is shown. (topical review)

  5. Intermolecular electron transfer from intramolecular excitation and coherent acoustic phonon generation in a hydrogen-bonded charge-transfer solid

    Science.gov (United States)

    Rury, Aaron S.; Sorenson, Shayne; Dawlaty, Jahan M.

    2016-03-01

    Organic materials that produce coherent lattice phonon excitations in response to external stimuli may provide next generation solutions in a wide range of applications. However, for these materials to lead to functional devices in technology, a full understanding of the possible driving forces of coherent lattice phonon generation must be attained. To facilitate the achievement of this goal, we have undertaken an optical spectroscopic study of an organic charge-transfer material formed from the ubiquitous reduction-oxidation pair hydroquinone and p-benzoquinone. Upon pumping this material, known as quinhydrone, on its intermolecular charge transfer resonance as well as an intramolecular resonance of p-benzoquinone, we find sub-cm-1 oscillations whose dispersion with probe energy resembles that of a coherent acoustic phonon that we argue is coherently excited following changes in the electron density of quinhydrone. Using the dynamical information from these ultrafast pump-probe measurements, we find that the fastest process we can resolve does not change whether we pump quinhydrone at either energy. Electron-phonon coupling from both ultrafast coherent vibrational and steady-state resonance Raman spectroscopies allows us to determine that intramolecular electronic excitation of p-benzoquinone also drives the electron transfer process in quinhydrone. These results demonstrate the wide range of electronic excitations of the parent of molecules found in many functional organic materials that can drive coherent lattice phonon excitations useful for applications in electronics, photonics, and information technology.

  6. Coherent excitation of vibrational levels using ultra short pulses

    CSIR Research Space (South Africa)

    De Clercq, LE

    2009-07-01

    Full Text Available The purpose of this study was to develop a model of the coherent excitation of the first few vibrational modes in the electronic ground state of the molecule. The model will be used in combination with an optimization algorithm to optimize a...

  7. Coherent and Incoherent Structural Dynamics in Laser-Excited Antimony

    CERN Document Server

    Waldecker, Lutz; Bertoni, Roman; Vasileiadis, Thomas; Garcia, Martin E; Zijlstra, Eeuwe S; Ernstorfer, Ralph

    2016-01-01

    We investigate the excitation of phonons in photoexcited antimony and demonstrate that the entire electron-lattice interactions, in particular coherent and incoherent electron-phonon coupling, can be probed simultaneously. Using femtosecond electron diffraction (FED) with high temporal resolution, we observe the coherent excitation of the fully symmetric \\Ag\\ optical phonon mode via the shift of the minimum of the atomic potential energy surface. Molecular dynamics simulations are performed to quantify the change in lattice potential and the associated real-space amplitude of the coherent atomic oscillations. In addition, our experimental configuration allows observing the energy transfer from electrons to phonons via incoherent electron-lattice scattering events. Applying a modified two-temperature model, the electron-phonon coupling is determined from the data as a function of electronic temperature.

  8. Resonance Raman excitation profiles of lycopene

    Science.gov (United States)

    Hoskins, L. C.

    1981-01-01

    The resonance Raman spectrum of lycopene has been examined in acetone solvent and excitation profiles of the three fundamentals ν1, ν2, and ν3 have been determined. The excitation data and the visible spectrum have been analyzed using two-mode and three-mode vibrational models, with the two-mode model involving virtual states of ν1 and ν2 giving the best fit to the data. This mode mixing or Duskinsky effect was not observed for β-carotene. The single-mode and three-mode theories which have been used to explain the corresponding data for β-carotene are shown to be inconsistent with the experimental data of lycopene. Equations for calculating excitation profiles and visible spectra are given.

  9. Excitation of field line resonances by sources outside the magnetosphere

    Directory of Open Access Journals (Sweden)

    A. D. M. Walker

    2005-11-01

    Full Text Available Field line resonances are thought to be excited by sources either at the magnetopause or outside it. Recent observations suggest that they may be associated with coherent oscillations or pressure pulses in the solar wind. In either case the excitation mechanism can be understood by considering the incidence of a harmonic wave on the magnetopause from outside the magnetosphere. Calculations are performed in a plane stratified model that consists of (i a magnetosheath region streaming tailward at uniform velocity (ii a sharp boundary representing the magnetopause, (iii a magnetosphere region in which the Alfvén speed increases monotonically with distance from the magnetopause. The structure implies the existence of a propagating region within the magnetopause bounded by a reflection level or turning point. Beyond this is a region in which waves are evanescent and a resonance level. The reflection and transmission of harmonic waves incident from the magnetosheath is considered in this model. It is shown that, in most cases, because of the mismatch between the magnetosphere and the magnetopause, the wave is reflected from the magnetopause with little penetration. At critical frequencies corresponding to the natural frequencies of the cavity formed between the magnetopause and turning point the signal excites the cavity and may leak evanescently to the resonance. The calculation includes the effect of the counter-streaming magnetosheath and magnetosphere plasmas on the wave. This can lead to amplification or attenuation. The nature of the processes that lead to transmission of the wave from magnetosheath to resonance are considered by synthesising the signal from plane wave spectra. A number of mechanisms for exciting cavity modes are reviewed and the relationship of the calculations to these mechanisms are discussed. Observations needed to discriminate between the mechanisms are specified.

  10. Coherent excitation with short electron pulses

    Science.gov (United States)

    Guertler, Andreas; Robicheaux, Francis; Noordam, Bart

    2000-06-01

    [1pt] The probability for a transition within an atom to be driven by a collision with a long pulse of electrons is proportional to the electron flux with the proportionality factor being the cross section for this transition. Recently it was shown [1] that for electron pulses shorter than the orbit time of the electron in the atom, a contribution of coherent scattering plays a role, which is proportional to the differential cross section in forward direction and the square of the electron flux. To investigate this effect, we are developing a picosecond electron gun [2]. Collision experiments will be done with Rydberg states in lithium around n=40 with Kepler orbit times in the order of 10 ps. For picosecond electron pulses, a quadratic dependance of the transition probability on the electron flux is expected in contrast to the linear dependance expected for nanosecond electron pulses. [1pt] References [1pt] [1] F. Robicheaux and L. D. Noordam, submitted to Phys. Rev. Lett. [1pt] [2] F. Robicheaux, G. M. Lankhuijzen, and L. D. Noordam, JOSA B 15, 1 (1998)

  11. Influence of coherent adiabatic excitation on femtosecond transient signals

    CERN Document Server

    Conde, A Peralta; Longarte, A

    2016-01-01

    The transient signals derived from femtosecond pump-probe experiments are analyzed in terms of the coherent evolution of the energy levels perturbed by the excitation pulse. The model system is treated as the sum of independent two-level subsystems that evolve adiabatically or are permanently excited, depending on the detuning from the central wavelength of the excitation laser. This approach will allow us to explain numerically and analytically the convergence between the coherent and incoherent (rate equations) treatments for complex multi-level systems. It will be also shown that the parameter that determines the validity of the incoherent treatment is the distribution of states outside and inside the laser bandwidth, rather than the density of states as it is commonly accepted.

  12. Nonradiative transfer of excitation in coherent decay from a Gaussian atomic distribution

    Energy Technology Data Exchange (ETDEWEB)

    Friedberg, Richard, E-mail: rfriedberg1@nyc.rr.com [Physics Department, Columbia University, NY (United States)

    2011-09-14

    Coherent decay of a spherically symmetric ensemble of initially resonantly phased two-level atoms is studied in the scalar photon model, in the continuum and Markov approximations. Emphasis is on the Gaussian distribution, where nonradiative transfer of excitation to excited states orthogonal to the initial one is found to be nonzero even in the limit of short wavelength, whether or not the scalar kernel exp(ik{sub 0}R)/ik{sub 0}R is replaced by its real part. Numerical results are compared to known values for the uniform distribution.

  13. Electromagnetic excitation of the Delta(1232) resonance

    Energy Technology Data Exchange (ETDEWEB)

    V. Pascalutsa; M. Vanderhaeghen; Shin Nan Yang

    2006-09-05

    We review the description of the lowest-energy nucleon excitation--the Delta(1232)-resonance. Much of the recent effort has been focused on the precision measurements of the nucleon to Delta transition by means of electromagnetic probes. We review the results of those measurements and confront them with the state-of-the-art calculations based on chiral effective-field theories (EFT), lattice QCD, and QCD-inspired models. Some of the theoretical approaches are reviewed in detail. In particular, we describe the chiral EFT of QCD in the energy domain of the Delta-resonance, and its applications to the electromagnetic nucleon-to-Delta transition (gamma N Delta). We also describe the recent dynamical and unitary-isobar models of pion electroproduction which are extensively used in the extraction of the gamma* N Delta form factors from experiment. Furthermore, we discuss the link of the gamma* N Delta form factors to generalized parton distributions (GPDs), as well as the predictions of perturbative QCD for these transition form factors. The present status of understanding the Delta-resonance properties and the nature of its excitation is summarized.

  14. Coherence resonance in bursting neural networks.

    Science.gov (United States)

    Kim, June Hoan; Lee, Ho Jun; Min, Cheol Hong; Lee, Kyoung J

    2015-10-01

    Synchronized neural bursts are one of the most noticeable dynamic features of neural networks, being essential for various phenomena in neuroscience, yet their complex dynamics are not well understood. With extrinsic electrical and optical manipulations on cultured neural networks, we demonstrate that the regularity (or randomness) of burst sequences is in many cases determined by a (few) low-dimensional attractor(s) working under strong neural noise. Moreover, there is an optimal level of noise strength at which the regularity of the interburst interval sequence becomes maximal-a phenomenon of coherence resonance. The experimental observations are successfully reproduced through computer simulations on a well-established neural network model, suggesting that the same phenomena may occur in many in vivo as well as in vitro neural networks.

  15. Subwavelength imaging and control of ultrafast optical near-field under resonant- and off-resonant excitation of bowtie nanostructures

    Science.gov (United States)

    Ji, Boyu; Qin, Jiang; Tao, Haiyan; Hao, Zuoqiang; Lin, Jingquan

    2016-09-01

    We demonstrate subwavelength imaging and control of localized near-field distribution under resonant and off-resonant excitation of identical gold bowtie nanostructures through photoemission electron microscopy. Control of the near-field distribution was realized by polarization rotation of single femtosecond laser pulse and variation of the phase delay of two orthogonally polarized femtosecond laser pulses. We show that the localized optical near-field distribution can be well controlled either among the corners of the nano-prisms in the bowtie for resonant excitation or the edges for off-resonant excitation. A better visualization of the PEEM image is achieved for resonant excitation than in the case of off-resonant excitation. The experimental results of the optical near-field distribution control are well reproduced by finite-difference time-domain simulations and understood by linear combination of electric charge distribution of the bowtie by s- and p- polarized light illumination. In addition, a shift of the near-field excitation position with inverted or unchanged phase, alternatively an un-shift of the excitation position but only with inverted phase of the near-field, can be realized by rotating the polarization angle of a single pulse and coherent control of two orthogonally polarized fs laser pulses.

  16. Two-Mode Excited Entangled Coherent State: Nonclassicality and Entanglement

    Science.gov (United States)

    Zhang, Hao-Liang; Wu, Jia-Ni; Liu, Cun-Jin; Hu, Yin-Quan; Hu, Li-Yun

    2017-03-01

    Two-mode excited entangled coherent states (TME-ECSs) are introduced by operating repeatedly the photon-excited operator on the ECSs. It is shown that the normalization constant is related to the product of two Laguerre polynomials. The influence of the operation on nonclassical behaviour of the ECSs is investigated in terms of cross-correlation function, anti-bunching effect and the negativity of Wigner function, which show that nonclassical properties can be enhanced. In addition, inseparability properties of the TME-ECSs are discussed by using Bell inequality and concurrence. It is found that the degree of quantum entanglement of even ECSs increases with the increase of the total excited photon number, and the violation of Bell inequality can be present for both even and odd case only when the total excited photon numbers are even and odd, respectively.

  17. Optical Generation of Single- or Two-Mode Excited Entangled Coherent States

    Institute of Scientific and Technical Information of China (English)

    REN Zhen-Zhong; JING Hui; ZHANG Xian-Zhou

    2008-01-01

    With nonlinear Mach-Zehnder interferometer (NLMZI) and a type-Ⅰ beta-barium borate (BBO) crystal, we optically generate single-mode excited entangled coherent states. This scheme can be easily generalized to generate two-mode excited entangled coherent states. We simply analyse different influences of single- and two-mode photon excitations on entangled coherent states.

  18. Nonlinear Resonance of Mechanically Excited Sessile Drops

    Science.gov (United States)

    Chang, Chun-Ti; Daniel, Susan; Steen, Paul

    2013-11-01

    The spectrum of frequencies and mode shapes for an inviscid drop on a planar substrate have recently been documented. For vertical excitation, zonal modes respond to the driving frequency harmonically and non-zonal modes subharmonically, consistent with the prior literature. In this study, we report observations from the regime of nonlinear response. Here, zonals can respond non-harmonically, both sub- and super-harmonic responses are reported. The principal challenge to generating and observing superharmonic resonances of higher zonal modes is a mode-mixing behavior. However, using a simple visual simulation based on the ray-tracing technique, the individual contributions to the mixed resonance behavior can be extracted. In summary, results from experiment and theory show that the zonal modes, which respond harmonically and can mix with non-zonal modes without interfering with one another in the linear regime, tend to respond sub- or superharmonically and compete with non-zonal modes in the nonlinear regime.

  19. Manipulating coherence resonance in a quantum dot semiconductor laser via electrical pumping.

    Science.gov (United States)

    Otto, Christian; Lingnau, Benjamin; Schöll, Eckehard; Lüdge, Kathy

    2014-06-02

    Excitability and coherence resonance are studied in a semiconductor quantum dot laser under short optical self-feedback. For low pump levels, these are observed close to a homoclinic bifurcation, which is in correspondence with earlier observations in quantum well lasers. However, for high pump levels, we find excitability close to a boundary crisis of a chaotic attractor. We demonstrate that in contrast to the homoclinic bifurcation the crisis and thus the excitable regime is highly sensitive to the pump current. The excitability threshold increases with the pump current, which permits to adjust the sensitivity of the excitable unit to noise as well as to shift the optimal noise strength, at which maximum coherence is observed. The shift adds up to more than one order of magnitude, which strongly facilitates experimental realizations.

  20. Nucleon Resonance Excitation with Virtual Photons

    CERN Document Server

    Tiator, L

    2007-01-01

    The unitary isobar model MAID is used for a partial wave analysis of pion photoproduction and electroproduction data on the nucleon. In particular we have taken emphasis on the region of the Delta(1232) resonance and have separated the resonance and background amplitudes with the K-matrix approach. This leads to electromagnetic properties of the dressed Delta resonance, where all multipole amplitudes become purely imaginary and all form factors and helicity amplitudes become purely real at the K-matrix pole of W=M_Delta=1232 MeV. The REM=E2/M1 and RSM=C2/M1 ratios of the quadrupole excitation are compared to recent data analysis of different groups. The REM ratio of MAID2005 agrees very well with the data and has a linear behavior over the whole experimentally explored Q^2 region with a small positive slope that predicts a zero crossing around 3.5 GeV^2. The recent RSM data for Q^2 < 0.2 GeV^2 indicate a qualitative change in the shape of the ratio which can be explained by the impact of the Siegert theore...

  1. Ultrafast spectral interferometry of resonant secondary emission from quantum wells: From Rayleigh scattering to coherent emission from biexcitons

    DEFF Research Database (Denmark)

    Birkedal, Dan; Shah, Jagdeep; Pfeiffer, L. N.

    1999-01-01

    Recent investigations of secondary emission from quantum well excitons following ultrafast resonant excitation have demonstrated an intricate interplay of coherent Rayleigh scattering and incoherent luminescence. We have very recently demonstrated that it is possible to isolate and time resolve...... invalidating the use of current theories using ensemble averages to describe our observations. Furthermore, we report here a new and hitherto unknown coherent scattering mechanism involving the two-photon coherence associated with the biexciton transition. The process leaves an exciton behind taking up...

  2. Femtosecond laser excitation of coherent optical phonons in ferroelectric LuMnO3

    Science.gov (United States)

    Lou, Shi-Tao; Zimmermann, Frank M.; Bartynski, Robert A.; Hur, Namjung; Cheong, Sang-Wook

    2009-06-01

    We have used femtosecond pump-probe spectroscopy to excite and probe coherent optical phonon vibrations in single crystals of hexagonal ferroelectric LuMnO3 . An optical phonon mode of A1 symmetry was coherently excited with 25 fs pump-laser pulses (λ≈800nm) . The phonon mode, involving Lu ion motion along the c axis, was identified as the soft mode driving the ferroelectric transition. The excitation mechanism was determined to be purely displacive in nature due to resonant excitation of a narrow intra-atomic dxy,x2-y2→d3z2-r2 transition in Mn. The lifetime of the Mndxy,x2-y2→d3z2-r2 excitation was measured to be 0.8 ps. A remarkable reversal of the sign of the oscillation amplitude ( π phase shift) of the reflectivity curve was observed upon comparing longitudinal-optical (LO) with transverse-optical (TO) mode geometries. The phase reversal is attributed to the macroscopic electric depolarization field accompanying infrared-active longitudinal phonon modes but absent in TO modes. In addition to the direct effect of the ion motion on the optical properties, which is the same in LO and TO modes, the longitudinal depolarization field of the LO mode gives rise to an additional modulation of the refractive index via the linear electro-optic effect which dominates the optical response.

  3. Observation of the 2p{sub 3/2}-2s{sub 1/2} radiative transition in Li-like uranium using the resonant coherent excitation in Si-crystal.

    Energy Technology Data Exchange (ETDEWEB)

    Ananyeva, Alena [Goethe Universitaet Frankfurt am Main (Germany); GSI Helmholtzzentrum fuer Schwerionenforschung, Darmstadt (Germany); Azuma, Toshiyuki; Nakano, Yuji [Tokyo Metropolitan University (Japan); RIKEN, Tokyo (Japan); Braeuning, Harald; Braeuning-Demian, Angela; Dimopoulou, Christina; Kleffner, Carl; Steck, Markus [GSI Helmholtzzentrum fuer Schwerionenforschung, Darmstadt (Germany); Dauvergne, Denis [IPNL - Institut de Physique Nucleaire de' Lyon (France); Kanai, Yasuyuki [RIKEN, Tokyo (Japan); Pivovarov, Yuri [National ResearchTomsk Polytechnic University (Russian Federation); Suda, Shintaro [Tokyo Metropolitan University (Japan); Yamazaki, Yasunori [RIKEN, Tokyo (Japan); University of Tokyo (Japan)

    2012-07-01

    Taking advantage of the cooled, relativistic ion beams delivered by the Experimental Storage Ring (ESR) at GSI, Darmstadt the energy of the 1s{sup 2}2p{sub 3/2}- 1s{sup 2}2s{sub 1/2} transition in Li-like U ions was measured by using the resonant excitation of ions in a Si-crystal in channelling conditions. The excitation of the projectile traversing a solid target with an ordered structure is induced with great probability by the periodic potential defined by the atoms of the crystal lattice when the oscillation frequency of the crystal field fits the energy difference between two levels of the ion. The resonant character of the process enables the determination of transition energy with high precision. The present scheme is quite universal being applicable for various ions and for a wide range of transition energies in the field of atomic as well as nuclear physics.

  4. Coherence depression in stochastic excitable systems with two-frequency forcing

    Science.gov (United States)

    Yu, Na; Longtin, André

    2011-12-01

    We study the response of two generic neuron models, the leaky integrate-and-fire (LIF) model and the leaky integrate-and-fire model with dynamic threshold (LIFDT) (i.e., with memory) to a stimulus consisting of two sinusoidal drives with incommensurate frequency, an amplitude modulation ("envelope") noise and a relatively weak additive noise. Spectral and coherence analysis of responses to such naturalistic stimuli reveals how the LIFDT model exhibits better correlation between modulation and spike train even in the presence of both noises. However, a resonance-induced synchrony, occurring when the beat frequency between the sinusoids is close to the intrinsic neuronal firing rate, decreases the coherence in the dynamic threshold case. Under suprathreshold conditions, the modulation noise simultaneously decreases the linear spectral coherence between the spikes and the whole stimulus, as well as between spikes and the stimulus envelope. Our study shows that the coefficient of variation of the envelope fluctuations is positively correlated with the degree of coherence depression. As the coherence function quantifies the linear information transmission, our findings indicate that under certain conditions, a transmission loss results when an excitable system with adaptive properties encodes a beat with frequency in the vicinity of its mean firing rate.

  5. Seeded excitation avalanches in off-resonantly driven Rydberg gases

    CERN Document Server

    Simonelli, Cristiano; Masella, Guido; Asteria, Luca; Arimondo, Ennio; Ciampini, Donatella; Morsch, Oliver

    2016-01-01

    We report an experimental investigation of the facilitated excitation dynamics in off-resonantly driven Rydberg gases by separating the initial off-resonant excitation phase from the facilitation phase, in which successive facilitation events lead to excitation avalanches. We achieve this by creating a controlled number of initial seed excitations. Greater insight into the avalanche mechanism is obtained from an analysis of the full counting distributions. We also present simple mathematical models and numerical simulations of the excitation avalanches that agree well with our experimental results.

  6. Coherent resonant Ka-band photonic microwave receiver

    CERN Document Server

    Ilchenko, Vladimir S; Savchenkov, Anatoliy A; Seidel, David; Matsko, Andrey B; Maleki, Lute

    2008-01-01

    We propose theoretically and demonstrate experimentally a coherent microwave photonic receiver operating at 35 GHz carrier frequency. The device is based on a lithium niobate or lithium tantalate optical whispering gallery mode resonator coupled to a microwave strip line resonator. Microwave local oscillator is fed into the microwave resonator along with the microwave signal. We show that the sensitivity of this receiver significantly exceeds the sensitivity of the incoherent quadratic receiver based on the same technology. The coherent receiver can possess a dynamic range in excess of 100 dB in 5 MHz band if a low noise laser is utilized.

  7. Coherent anti-Stokes Raman spectroscopy in the presence of strong resonant signal from background molecules

    CERN Document Server

    Bitter, Martin

    2012-01-01

    Optical spectroscopy with broadband femtosecond laser pulses often involves simultaneous excitation of multiple molecular species with close resonance frequencies. Interpreting the collective optical response from molecular mixtures typically requires Fourier analysis of the detected time-resolved signal. We propose an alternative method of separating coherent optical responses from two molecular species with neighboring excitation resonances (here, vibrational modes of oxygen and carbon dioxide). We utilize ro-vibrational coupling as a mechanism of suppressing the strong vibrational response from the dominating molecular species (O$_{2}$). Coherent ro-vibrational dynamics lead to long "silence windows" of zero signal from oxygen molecules. In these silence windows, the detected signal stems solely from the minority species (CO$_{2}$) enabling background-free detection and characterization of the O$_2$/CO$_2$ mixing ratio. In comparison to a Fourier analysis, our technique does not require femtosecond time re...

  8. Grid impedance detection via excitation of LCL-filter resonance

    DEFF Research Database (Denmark)

    Liserre, Marco; Blaabjerg, Frede; Teodorescu, Remus

    2005-01-01

    the resonance of the LCL-fiIter can be also excited in a controlled way in order to individuate the resonance frequency in the spectrum (using for example the FFn. This paper proposes to use a controlled excitation to measure the grid impedance, since this one influences also the resonance frequency. This paper...... will address some possible limits, some solutions and some implementation issues (e.g. how to obtain a controlled resonance in the filter without damaging the system) in order to use the resonant peak for grid impedance detection. The analysis is validated both by simulations and experimental results....

  9. Transition from double coherence resonances to single coherence resonance in a neuronal network with phase noise.

    Science.gov (United States)

    Jia, Yanbing; Gu, Huaguang

    2015-12-01

    The effect of phase noise on the coherence dynamics of a neuronal network composed of FitzHugh-Nagumo (FHN) neurons is investigated. Phase noise can induce dissimilar coherence resonance (CR) effects for different coupling strength regimes. When the coupling strength is small, phase noise can induce double CRs. One corresponds to the average frequency of phase noise, and the other corresponds to the intrinsic firing frequency of the FHN neuron. When the coupling strength is large enough, phase noise can only induce single CR, and the CR corresponds to the intrinsic firing frequency of the FHN neuron. The results show a transition from double CRs to single CR with the increase in the coupling strength. The transition can be well interpreted based on the dynamics of a single neuron stimulated by both phase noise and the coupling current. When the coupling strength is small, the coupling current is weak, and phase noise mainly determines the dynamics of the neuron. Moreover, the phase-noise-induced double CRs in the neuronal network are similar to the phase-noise-induced double CRs in an isolated FHN neuron. When the coupling strength is large enough, the coupling current is strong and plays a key role in the occurrence of the single CR in the network. The results provide a novel phenomenon and may have important implications in understanding the dynamics of neuronal networks.

  10. Stochastic and coherence resonance in an in silico neural model.

    Science.gov (United States)

    Chiu, Alan W L; Bardakjian, Berj L

    2004-05-01

    We show that it is possible for chaotic systems to display the main features of stochastic and coherence resonance. In particular, a model of coupled nonlinear oscillators which emulates the transmembrane voltage activities in CA3 neurons, operating in a chaotic regime and in the presence of noise, can exhibit coherence resonance and stochastic resonance. Certain firing frequencies become more "rhythmic" for some optimal values of noise intensity. The effect of noise in different coupling pathways is investigated. We found that the effect of coherence resonance and stochastic resonance are more prominent if noise is presented in either electric field or gap junction coupling pathways. Frequency sensitivity of the model is investigated as a preliminary step in illustrating the principles of possible epileptic seizure control strategies using "chaos control" concepts. Significant effects of stochastic resonance are observed in the 4-8 Hz range. Weaker effects can be found in the 1-4 Hz and 8-10 Hz ranges whereas 0.5 Hz does not exhibit any resonance phenomenon. Our results suggest that: (a) Stochastic resonance could enhance the intrinsic 4-8 Hz rhythms in CA3 neurons more prominently via field coupling pathways. It could also help explain why some reported seizure control strategies using pulse-trains would only be effective at 0.5 Hz. (b) Stochastic resonance-like behavior can occur in the gamma range only if noise is presented via chemical synaptic pathways.

  11. Ultrafast modulation of electronic structure by coherent phonon excitations

    Science.gov (United States)

    Weisshaupt, J.; Rouzée, A.; Woerner, M.; Vrakking, M. J. J.; Elsaesser, T.; Shirley, E. L.; Borgschulte, A.

    2017-02-01

    Femtosecond x-ray absorption spectroscopy with a laser-driven high-harmonic source is used to map ultrafast changes of x-ray absorption by femtometer-scale coherent phonon displacements. In LiBH4, displacements along an Ag phonon mode at 10 THz are induced by impulsive Raman excitation and give rise to oscillatory changes of x-ray absorption at the Li K edge. Electron density maps from femtosecond x-ray diffraction data show that the electric field of the pump pulse induces a charge transfer from the BH4- to neighboring Li+ ions, resulting in a differential Coulomb force that drives lattice vibrations in this virtual transition state.

  12. Mixed frequency excitation of an electrostatically actuated resonator

    KAUST Repository

    Ramini, Abdallah

    2015-04-24

    We investigate experimentally and theoretically the dynamics of a capacitive resonator under mixed frequency excitation of two AC harmonic signals. The resonator is composed of a proof mass suspended by two cantilever beams. Experimental measurements are conducted using a laser Doppler vibrometer to reveal the interesting dynamics of the system when subjected to two-source excitation. A nonlinear single-degree-of-freedom model is used for the theoretical investigation. The results reveal combination resonances of additive and subtractive type, which are shown to be promising to increase the bandwidth of the resonator near primary resonance frequency. Our results also demonstrate the ability to shift the combination resonances to much lower or much higher frequency ranges. We also demonstrate the dynamic pull-in instability under mixed frequency excitation. © 2015 Springer-Verlag Berlin Heidelberg

  13. Persistent spin excitations in doped antiferromagnets revealed by resonant inelastic light scattering

    Science.gov (United States)

    Jia, C. J.; Nowadnick, E. A.; Wohlfeld, K.; Kung, Y. F.; Chen, C.-C.; Johnston, S.; Tohyama, T.; Moritz, B.; Devereaux, T. P.

    2014-02-01

    How coherent quasiparticles emerge by doping quantum antiferromagnets is a key question in correlated electron systems, whose resolution is needed to elucidate the phase diagram of copper oxides. Recent resonant inelastic X-ray scattering (RIXS) experiments in hole-doped cuprates have purported to measure high-energy collective spin excitations that persist well into the overdoped regime and bear a striking resemblance to those found in the parent compound, challenging the perception that spin excitations should weaken with doping and have a diminishing effect on superconductivity. Here we show that RIXS at the Cu L3-edge indeed provides access to the spin dynamical structure factor once one considers the full influence of light polarization. Further we demonstrate that high-energy spin excitations do not correlate with the doping dependence of Tc, while low-energy excitations depend sensitively on doping and show ferromagnetic correlations. This suggests that high-energy spin excitations are marginal to pairing in cuprate superconductors.

  14. Coherent quantum control of internal conversion: {S}_{2}\\;\\leftrightarrow \\;{S}_{1} in pyrazine via {S}_{0}\\;\\to \\;{S}_{2}/{S}_{1} weak field excitation

    Science.gov (United States)

    Grinev, Timur; Shapiro, Moshe; Brumer, Paul

    2015-09-01

    Coherent control of internal conversion (IC) between the first (S1) and second (S2) singlet excited electronic states in pyrazine, where the S2 state is populated from the ground singlet electronic state S0 by weak field excitation, is examined. Control is implemented by shaping the laser which excites S2. Excitation and IC are considered simultaneously, using the recently introduced resonance-based control approach. Highly successful control is achieved by optimizing both the amplitude and phase profiles of the laser spectrum. The dependence of control on the properties of resonances in S2 is demonstrated.

  15. Transform analysis of the resonance Raman excitation profile of lycopene

    Science.gov (United States)

    Hoskins, L. C.

    1992-10-01

    The resonance Raman excitation profiles (RREPs) of the ν 1, ν 2 and ν 3 vibrations of lycopene in acetone, ethyl alcohol, toluene and carbon disulphide solvents have been analyzed using the transform method for calculating resonance Raman excitation profiles. The tests show excellent agreement between the calculated and observed profiles for the ν 2 and ν 3 RREPs, but greater difference between experiment and theory occurs for the ν 1 RREP, especially in carbon disulphide solvent.

  16. Coherent stochastic resonance in the presence of a field

    Science.gov (United States)

    Gitterman, Moshe; Weiss, George H.

    1995-11-01

    A recent paper by Bulsara, Lowen, and Rees [Phys. Rev. E 49, 4989 (1994)] presents a perturbation analysis of coherent stochastic resonance in a half-space in the presence of a field. We believe that the analysis there was flawed due to an improper use of the method of images and that a correct version of a perturbation analysis can be given by using a transformation of the underlying equations. The result still exhibits stochastic resonance.

  17. Single Element Excitation and Detection of (Micro-)Mechanical Resonators

    NARCIS (Netherlands)

    Tilmans, Harrie A.C.; IJntema, Dominicus .J.; Fluitman, Jan H.J

    1991-01-01

    The authors describe a single-element approach for the excitation and detection of the vibrational motion of (micro-)mechanical resonators. An equivalent electrical one-port network is derived for an electrostatically and a piezoelectrically driven resonator. In this way, the effect of the mechanica

  18. Population of highly excited intermediate resonance states by electron transfer and excitation

    Energy Technology Data Exchange (ETDEWEB)

    Schuch, R. (Manne Siegbahn Institute of Physics, S-104 05 Stockholm, Sweden (SE)); Justiniano, E. (Department of Physics, East Carolina University, Greenville, North Carolina 27858-4353 (USA)); Schulz, M.; Datz, S.; Dittner, P.F.; Giese, J.P.; Krause, H.F.; Schoene, H.; Vane, R. (Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831-6377 (USA)); Shafroth, S. (Department of Physics, North Carolina University, Chapel Hill, North Carolina 27599-3255 (USA))

    1991-05-01

    Coincidences between two sulfur {ital K} x rays were detected from collisions of hydrogenlike S ions with H{sub 2} gas in the projectile energy range between 150 and 225 MeV. These {ital K} x rays are emitted in the decay of doubly excited states formed in the collisions via transfer and excitation. The excitation function for two coincident {ital K}{beta} transitions peaks at about 175 MeV, slightly above the expected {ital KMM} resonance energy for resonant transfer and excitation (RTE). This demonstrates the occurrence of {Delta}{ital N}{ge}2 transitions (i.e., {ital KMM} and higher resonances) in the RTE process. The cross sections for the population of the very highly excited states are higher than those predicted by theoretical calculations that use dielectronic recombination rates folded with the Compton profile for the bound electrons.

  19. Resonator coupled Josephson junctions; parametric excitations and mutual locking

    DEFF Research Database (Denmark)

    Jensen, H. Dalsgaard; Larsen, A.; Mygind, Jesper

    1991-01-01

    Self-pumped parametric excitations and mutual locking in systems of Josephson tunnel junctions coupled to multimode resonators are reported. For the very large values of the coupling parameter, obtained with small Nb-Al2O3-Nb junctions integrated in superconducting microstrip resonators, the DC I......-V characteristic shows an equidistant series of current steps generated by subharmonic pumping of the fundamental resonator mode. This is confirmed by measurement of frequency and linewidth of the emitted Josephson radiation...

  20. Resonance flourescence in atomic coherent systems spectral features

    CERN Document Server

    Sandhya, S N

    1999-01-01

    We study resonance flourescence in a four level ladder system and illustrate some novel features due to quantum interference and atomic coherence effects. We find that under three photon resonant conditions, in some region of the parameter space of the rabi frequencies $\\Omega_1,\\Omega_2,\\Omega_3$, emission is dominantly by the level 4 at the line center even though there is an almost equal distribution of populations in all the levels. As one increases 'dynamically collapses' to a two level system. The steady state populations and the the resonance flourescence from all the levels provide adequate evidence to this effect.

  1. Coherent Dark Resonances in Atomic Barium

    CERN Document Server

    Dammalapati, U; Jungmann, K; Willmann, L

    2007-01-01

    The observation of dark-resonances in the two-electron atom barium and their influence on optical cooling is reported. In heavy alkali earth atoms, i.e. barium or radium, optical cooling can be achieved using n^1S_0-n^1P_1 transitions and optical repumping from the low lying n^1D_2 and n^3D_{1,2} states to which the atoms decay with a high branching ratio. The cooling and repumping transition have a common upper state. This leads to dark resonances and hence make optical cooling less inefficient. The experimental observations can be accurately modelled by the optical Bloch equations. Comparison with experimental results allows us to extract relevant parameters for effective laser cooling of barium.

  2. Plasmon-Induced Resonant Energy Transfer: a coherent dipole-dipole coupling mechanism

    Science.gov (United States)

    Bristow, Alan D.; Cushing, Scott K.; Li, Jiangtian; Wu, Nianqiang

    Metal-insulator-semiconductor core-shell nanoparticles have been used to demonstrate a dipole-dipole coupling mechanism that is entirely dependent on the dephasing time of the localized plasmonic resonance. Consequently, the short-time scale of the plasmons leads to broad energy uncertainty that allows for excitation of charge carriers in the semiconductor via stimulation of photons with energies below the energy band gap. In addition, this coherent energy transfer process overcomes interfacial losses often associated with direct charge transfer. This work explores the efficiency of the energy transfer process, the dipole-dipole coupling strength with dipole separation, shell thickness and plasmonic resonance overlap. We demonstrate limits where the coherent nature of the coupling is switched off and charge transfer processes can dominate. Experiments are performed using transient absorption spectroscopy. Results are compared to calculations using a quantum master equation. These nanostructures show strong potential for improving solar light-harvesting for power and fuel generation.

  3. Coherent molecule formation in anharmonic potentials near confinement-induced resonances.

    Science.gov (United States)

    Sala, S; Zürn, G; Lompe, T; Wenz, A N; Murmann, S; Serwane, F; Jochim, S; Saenz, A

    2013-05-17

    We perform a theoretical and experimental study of a system of two ultracold atoms with tunable interaction in an elongated trapping potential. We show that the coupling of center-of-mass and relative motion due to an anharmonicity of the trapping potential leads to a coherent coupling of a state of an unbound atom pair and a molecule with a center of mass excitation. By performing the experiment with exactly two particles we exclude three-body losses and can therefore directly observe coherent molecule formation. We find quantitative agreement between our theory of inelastic confinement-induced resonances and the experimental results. This shows that the effects of center-of-mass to relative-motion coupling can have a significant impact on the physics of quantum systems near center-of-mass to relative-motion coupling resonances.

  4. Stochastic Resonance on a Circle Without Periodic Excitation

    Institute of Scientific and Technical Information of China (English)

    QIAN Min; WANG Guan-Xiang

    2000-01-01

    We analyse the appearance of coherent motion in the dynamics of the Langevin equation in the subtle case of I<1, and show that stochastic resonance does exist even in the non-critical case I<1. Moreover, we show the monotonicity of the rotation number and discuss the relationship between the center frequency of the power spectrum peak and the rotation number

  5. Detection of a coherent population trapping resonance in a beam of 87Rb atoms by the Ramsey method

    Science.gov (United States)

    Sokolov, I. M.

    2015-10-01

    Formation of a coherent population trapping (CPT) resonance is studied in the interaction of a beam of 87Rb atoms with two spatially separated domains of the dichromatic field. Various resonance excitation schemes are compared depending on the choice of operation transitions and type of the polarisation scheme. In the case of a single-velocity atomic beam, the dependence of the CPT resonance profile is studied as a function of principal parameters of the system: beam velocity, distance between optical fields, laser beam dimensions and intensities, and applied permanent magnetic field. Influence of the atomic beam angular divergence and residual beam velocity spread on the resonance quality parameter is estimated.

  6. Electronically excited negative ion resonant states in chloroethylenes

    Energy Technology Data Exchange (ETDEWEB)

    Khvostenko, O.G., E-mail: khv@mail.ru; Lukin, V.G.; Tuimedov, G.M.; Khatymova, L.Z.; Kinzyabulatov, R.R.; Tseplin, E.E.

    2015-02-15

    Highlights: • Several novel dissociative negative ion channels were revealed in chloroethylenes. • The electronically excited resonant states were recorded in all chloroethylenes under study. • The states were assigned to the inter-shell types, but not to the core-excited Feshbach one. - Abstract: The negative ion mass spectra of the resonant electron capture by molecules of 1,1-dichloroethylene, 1,2-dichloroethylene-cis, 1,2-dichloroethylene-trans, trichloroethylene and tetrachloroethylene have been recorded in the 0–12 eV range of the captured electron energy using static magnetic sector mass spectrometer modified for operation in the resonant electron capture regime. As a result, several novel low-intensive dissociation channels were revealed in the compounds under study. Additionally, the negative ion resonant states were recorded at approximately 3–12 eV, mostly for the first time. These resonant states were assigned to the electronically excited resonances of the inter-shell type by comparing their energies with those of the parent neutral molecules triplet and singlet electronically excited states known from the energy-loss spectra obtained by previous studies.

  7. Unnatural parity resonance states in positron-excited hydrogen scattering

    Institute of Scientific and Technical Information of China (English)

    Ma Jia; Zhou Ya-Jun; Wang Yuan-Cheng

    2012-01-01

    The coupled-channels optical method for positron scattering has been applied to investigate resonance states with unnatural parities in a positron-excited hydrogen system.The positronium formation channels and continuum channel are included via a complex equivalent local potential.Resonance states with angular momenta L =1 to L =2 and parities (-1)L+1 are calculated.Resonance energies and widths are reported and compared with other theoretical calculations.We found that the opening positronium formation channels play an important role in forming nondipole Feshbach resonances.

  8. Vibration-assisted resonance in photosynthetic excitation energy transfer

    CERN Document Server

    Irish, E K; Lovett, B W

    2013-01-01

    Coherent quantum energy transfer, as observed in photosynthetic pigment-protein complexes, is inhibited by energetic disorder. While this difficulty can be overcome to some extent by the addition of environmental noise, it has recently has begun to be appreciated that discrete intra- and/or intermolecular vibrational modes may play an important role in quantum dynamics. We present a microscopic mechanism by which intramolecular vibrational modes create resonant energy transfer pathways, enhancing the efficiency of both coherent and dephasing-assisted transfer. The principles of this vibration-assisted resonance are illustrated in a simple model based on one energy-transfer branch of the well-characterised Fenna-Matthews-Olson complex. Despite its simplicity, this model captures the interplay between strong electronic coupling that produces delocalised exciton states and resonance-enhanced weak coupling to local vibrational modes. Analytical and numerical results show that intramolecular vibrations can enhance...

  9. Lifetime-vibrational interference effects in resonantly excited x-ray emission spectra of CO

    Energy Technology Data Exchange (ETDEWEB)

    Skytt, P.; Glans, P.; Gunnelin, K. [Uppsala Univ. (Sweden)] [and others

    1997-04-01

    The parity selection rule for resonant X-ray emission as demonstrated for O{sub 2} and N{sub 2} can be seen as an effect of interference between coherently excited degenerate localized core states. One system where the core state degeneracy is not exact but somewhat lifted was previously studied at ALS, namely the resonant X-ray emission of amino-substituted benzene (aniline). It was shown that the X-ray fluorescence spectrum resulting from excitation of the C1s at the site of the {open_quotes}aminocarbon{close_quotes} could be described in a picture separating the excitation and the emission processes, whereas the spectrum corresponding to the quasi-degenerate carbons could not. Thus, in this case it was necessary to take interference effects between the quasi-degenerate intermediate core excited states into account in order to obtain agreement between calculations and experiment. The different vibrational levels of core excited states in molecules have energy splittings which are of the same order of magnitude as the natural lifetime broadening of core excitations in the soft X-ray range. Therefore, lifetime-vibrational interference effects are likely to appear and influence the band shapes in resonant X-ray emission spectra. Lifetime-vibrational interference has been studied in non-resonant X-ray emission, and in Auger spectra. In this report the authors discuss results of selectively excited soft X-ray fluorescence spectra of molecules, where they focus on lifetime-interference effects appearing in the band shapes.

  10. Ultrafast spectral interferometry of resonant secondary emission from quantum wells: From Rayleigh scattering to coherent emission from biexcitons

    DEFF Research Database (Denmark)

    Birkedal, Dan; Shah, Jagdeep; Pfeiffer, L. N.

    1999-01-01

    Recent investigations of secondary emission from quantum well excitons following ultrafast resonant excitation have demonstrated an intricate interplay of coherent Rayleigh scattering and incoherent luminescence. We have very recently demonstrated that it is possible to isolate and time resolve...... the coherent field associated with Rayleigh component using ultrafast spectral interferometry or Tadpole, thus, obtaining substantial and new information of the nature of resonant secondary emission. Our observation demonstrates that Rayleigh scattering from static disorder is inherently a non-ergodic process...... invalidating the use of current theories using ensemble averages to describe our observations. Furthermore, we report here a new and hitherto unknown coherent scattering mechanism involving the two-photon coherence associated with the biexciton transition. The process leaves an exciton behind taking up...

  11. Selective Mode Excitation And Detection Of Micromachined Resonators

    NARCIS (Netherlands)

    Prak, Albert; Elwenspoek, Miko; Fluitman, Jan H.J

    1992-01-01

    Distributed mechanical systems such as micromachined resonant strain gages possess an infinite number of modes of vibration. Mostly, one is interested in only one or a few modes. A method is described with which only the desired modes are excited and detected. This is achieved by geometrically shapi

  12. Thermal pairing and giant dipole resonance in highly excited nuclei

    CERN Document Server

    Dang, Nguyen Dinh

    2014-01-01

    Recent results are reported showing the effects of thermal pairing in highly excited nuclei. It is demonstrated that thermal pairing included in the phonon damping model (PDM) is responsible for the nearly constant width of the giant dipole resonance (GDR) at low temperature $T $ 170 MeV.

  13. Direct excitation of resonant torsional Alfven waves by footpoint motions

    NARCIS (Netherlands)

    Ruderman, M. S.; Berghmans, D.; Goossens, M.; Poedts, S.

    1997-01-01

    The present paper studies the heating of coronal loops by linear resonant Alfven waves that are excited by the motions of the photospheric footpoints of the magnetic field lines. The analysis is restricted to torsionally polarised footpoint motions in an axially symmetric system so that only

  14. Resonance enhanced electron impact excitation of Cu-like gadolinium

    Science.gov (United States)

    Li, Shuang; Si, Ran; Zhang, Chun yu; Guo, Xue Ling; Chen, Zhan Bin; Wang, Kai; Chen, Chong Yang; Yan, Jun

    2017-06-01

    Employing the independent processes and isolated resonances approximation using distorted-waves (IPIRDW), we perform a large calculation and a detail investigation on resonance enhanced electron impact excitation (EIE) among the 27 singly excited levels from n ≤ 6 configurations of Cu-like gadolinium (Gd, Z = 64). We take into account the RE contributions from both the relevant Zn-like doubly excited series [Ne]3 l 18 n' l' n'' l'' with n' = 4-7, and the series [Ne]3 l 174 l4 l' n'' l''. Results show that the RE contributions are significant and enhance effective collision strengths ( Υ) of certain excitations by even up to an order of magnitude at low temperature (105.8 K), and still important at relative high temperature (106.8 K), where the fraction abundance of Gd XXXVI is expected at peak. We expect present resonance enhanced EIE results among the 27 levels, which is the first results with the RE contributions from n = 3 → 4 core excitation for Cu-like isoelectronic sequence, are more accurate due to our consideration of RE contributions for this ion for the first time.

  15. Effects of Herzberg--Teller vibronic coupling on coherent excitation energy transfer

    CERN Document Server

    Zhang, Hou-Dao; Xu, Rui-Xue; Yan, YiJing

    2016-01-01

    In this work, we study the effects of non-Condon vibronic coupling on the quantum coherence of excitation energy transfer, via the exact dissipaton-equation-of-motion (DEOM) evaluations on excitonic model systems. Field-triggered excitation energy transfer dynamics and two dimensional coherent spectroscopy are simulated for both Condon and non-Condon vibronic couplings. Our results clearly demonstrate that the non-Condon vibronic coupling intensifies the dynamical electronic-vibrational energy transfer and enhances the total system-and-bath quantum coherence. Moreover, the hybrid bath dynamics for non-Condon effects enriches the theoretical calculation, and further sheds light on the interpretation of the experimental nonlinear spectroscopy.

  16. Excitation of coherent oscillations in underdoped cuprate superconductors by intense THz pulses

    Science.gov (United States)

    Hoffmann, Matthias C.; Lee, Wei-Sheng; Dakovski, Georgi L.; Turner, Joshua J.; Gerber, Simon M.; Bonn, Doug; Hardy, Walter; Liang, Ruixing; Salluzzo, Marco

    2016-05-01

    We use intense broadband THz pulses to excite the cuprate superconductors YBCO and NBCO in their underdoped phase, where superconducting and charge density wave ground states compete. We observe pronounced coherent oscillations at attributed to renormalized low-energy phonon modes. These oscillation features are much more prominent than those observed in all-optical pump-probe measurements, suggesting a different excitation mechanism.

  17. Coherent excitation-selective spectroscopy in planar metamaterials

    OpenAIRE

    Fang, Xu; Tseng, Ming Lun; Tsai, Din Ping; Zheludev, Nikolay I.

    2013-01-01

    In a proof-of-principle experiment with metamaterials exhibiting electric dipolar and magnetic dipolar resonances, we demonstrated that the electric and magnetic resonances can be separately switches off and on by positioning the metamaterials along a standing wave, while both resonances are present in travelling-wave spectra.

  18. Coherent excitation-selective spectroscopy in planar metamaterials

    CERN Document Server

    Fang, Xu; Tsai, Din Ping; Zheludev, Nikolay I

    2013-01-01

    In a proof-of-principle experiment with metamaterials exhibiting electric dipolar and magnetic dipolar resonances, we demonstrated that the electric and magnetic resonances can be separately switches off and on by positioning the metamaterials along a standing wave, while both resonances are present in travelling-wave spectra.

  19. Oncotripsy: Targeting cancer cells selectively via resonant harmonic excitation

    CERN Document Server

    Heyden, Stefanie

    2015-01-01

    We investigate a method of selectively targeting cancer cells by means of ultrasound harmonic excitation at their resonance frequency, which we refer to as oncotripsy. The geometric model of the cells takes into account the cytoplasm, nucleus and nucleolus, as well as the plasma membrane and nuclear envelope. Material properties are varied within a pathophysiologically-relevant range. A first modal analysis reveals the existence of a spectral gap between the natural frequencies and, most importantly, resonant growth rates of healthy and cancerous cells. The results of the modal analysis are verified by simulating the fully-nonlinear transient response of healthy and cancerous cells at resonance. The fully nonlinear analysis confirms that cancerous cells can be selectively taken to lysis by the application of carefully tuned ultrasound harmonic excitation while simultaneously leaving healthy cells intact.

  20. Oncotripsy: Targeting cancer cells selectively via resonant harmonic excitation

    Science.gov (United States)

    Heyden, S.; Ortiz, M.

    2016-07-01

    We investigate a method of selectively targeting cancer cells by means of ultrasound harmonic excitation at their resonance frequency, which we refer to as oncotripsy. The geometric model of the cells takes into account the cytoplasm, nucleus and nucleolus, as well as the plasma membrane and nuclear envelope. Material properties are varied within a pathophysiologically-relevant range. A first modal analysis reveals the existence of a spectral gap between the natural frequencies and, most importantly, resonant growth rates of healthy and cancerous cells. The results of the modal analysis are verified by simulating the fully-nonlinear transient response of healthy and cancerous cells at resonance. The fully nonlinear analysis confirms that cancerous cells can be selectively taken to lysis by the application of carefully tuned ultrasound harmonic excitation while simultaneously leaving healthy cells intact.

  1. Coulomb and nuclear excitations of narrow resonances in 17Ne

    Directory of Open Access Journals (Sweden)

    J. Marganiec

    2016-08-01

    Full Text Available New experimental data for dissociation of relativistic 17Ne projectiles incident on targets of lead, carbon, and polyethylene targets at GSI are presented. Special attention is paid to the excitation and decay of narrow resonant states in 17Ne. Distributions of internal energy in the O15+p+p three-body system have been determined together with angular and partial-energy correlations between the decay products in different energy regions. The analysis was done using existing experimental data on 17Ne and its mirror nucleus 17N. The isobaric multiplet mass equation is used for assignment of observed resonances and their spins and parities. A combination of data from the heavy and light targets yielded cross sections and transition probabilities for the Coulomb excitations of the narrow resonant states. The resulting transition probabilities provide information relevant for a better understanding of the 17Ne structure.

  2. Single-pulse terahertz coherent control of spin resonance in the canted antiferromagnet YFeO3, mediated by dielectric anisotropy

    DEFF Research Database (Denmark)

    Jin, Zuanming; Mics, Zoltán; Ma, Guohong;

    2013-01-01

    We report on the coherent control of terahertz (THz) spin waves in a canted antiferromagnet yttrium orthoferrite, YFeO3, associated with a quasiferromagnetic (quasi-FM) spin resonance at a frequency of 0.3 THz, using a single-incident THz pulse. The spin resonance is excited impulsively...... by the magnetic field component of the THz pulse. The intrinsic dielectric anisotropy of YFeO3 in the THz range allows for coherent control of both the amplitude and the phase of the excited spin wave. The coherent control is based on simultaneous generation of two interfering phase-shifted spin waves whose...... amplitudes and relative phase, dictated by the dielectric anisotropy of the YFeO3 crystal, can be controlled by varying the polarization of the incident THz pulse with respect to the crystal axes. The spatially anisotropic decay of the THz-excited FM spin resonance in YFeO3, leading to an increasingly linear...

  3. Coherent resonance stop bands in alternating gradient beam transport

    Science.gov (United States)

    Ito, K.; Okamoto, H.; Tokashiki, Y.; Fukushima, K.

    2017-06-01

    An extensive experimental study is performed to confirm fundamental resonance bands of an intense hadron beam propagating through an alternating gradient linear transport channel. The present work focuses on the most common lattice geometry called "FODO" or "doublet" that consists of two quadrupoles of opposite polarities. The tabletop ion-trap system "S-POD" (Simulator of Particle Orbit Dynamics) developed at Hiroshima University is employed to clarify the parameter-dependence of coherent beam instability. S-POD can provide a non-neutral plasma physically equivalent to a charged-particle beam in a periodic focusing potential. In contrast with conventional experimental approaches relying on large-scale machines, it is straightforward in S-POD to control the doublet geometry characterized by the quadrupole filling factor and drift-space ratio. We verify that the resonance feature does not essentially change depending on these geometric factors. A few clear stop bands of low-order resonances always appear in the same pattern as previously found with the sinusoidal focusing model. All stop bands become widened and shift to the higher-tune side as the beam density is increased. In the space-charge-dominated regime, the most dangerous stop band is located at the bare betatron phase advance slightly above 90 degrees. Experimental data from S-POD suggest that this severe resonance is driven mainly by the linear self-field potential rather than by nonlinear external imperfections and, therefore, unavoidable at high beam density. The instability of the third-order coherent mode generates relatively weak but noticeable stop bands near the phase advances of 60 and 120 degrees. The latter sextupole stop band is considerably enhanced by lattice imperfections. In a strongly asymmetric focusing channel, extra attention may have to be paid to some coupling resonance lines induced by the Coulomb potential. Our interpretations of experimental data are supported by theoretical

  4. Resonant parametric excitations driven by lower-hybrid fields

    Energy Technology Data Exchange (ETDEWEB)

    Villalon, E.

    1980-11-01

    Three-wave parametric excitation in inhomogeneous plasmas is examined in a two-dimensional geometry relevant to supplementary rf heating of tokamaks. The stabilization of resonant parametric excitation due to a linear mismatch in wavenumbers and to the Landau-damping rates of the decay waves is analyzed, assuming that the magnitude of the pump field is constant in time and in the spatial region where the resonant interaction takes place. Both types of temporally growing modes and spatially amplified instabilities are studied, using a WKB analysis. It is shown that either by increasing the strength of the mismatch K' or the width of the pump L, the growth rate of the fastest growing normal mode will decrease. When the excited waves are slightly damped, it is shown that there exists a finite value of the product K'L, such that, above it, no temporal normal modes are excited. The amount of spatial amplification is also reduced by the mismatch in wavenumbers and by the damping rates of the excited waves. Because of the finite spatial extent of the pump electric field, the amplification length is found to be smaller than or equal to L, depending on the strength of the mismatch and damping rates.

  5. Origin of long-lived coherence and excitation dynamics in pigment-protein complexes

    CERN Document Server

    Zhang, Zhedong

    2015-01-01

    We uncover the mechanism of long-lived coherence that the discrete vibrational modes effectively weaken the exciton-environment interaction. This subsequently demonstrates the role of vibrational coherence which greatly contributes to long-lived feature of the excitonic coherence that has been observed in femtosecond experiments. To test the validity of our effective theory, we study the pigment-protein complex in details by exploring the energy transfer and coherence dynamics. The ground-state coherence generated by incoherent radiations is demonstrated to be significant to promote the excitation energy transfer. This on the other hand, seems to be natural from the point of view of nonequilibriumness, which funnels the downhill immigration of excitons. Moreover we also confirm that the considerable improvement of energy transfer is always accompanied by the long-lived oscillation of coherence.

  6. Origin of long-lived quantum coherence and excitation dynamics in pigment-protein complexes

    Science.gov (United States)

    Zhang, Zhedong; Wang, Jin

    2016-11-01

    We explore the mechanism for the long-lived quantum coherence by considering the discrete phonon modes: these vibrational modes effectively weaken the exciton-environment interaction, due to the new composite (polaron) formed by excitons and vibrons. This subsequently demonstrates the role of vibrational coherence which greatly contributes to long-lived feature of the excitonic coherence that has been observed in femtosecond experiments. The estimation of the timescale of coherence elongated by vibrational modes is given in an analytical manner. To test the validity of our theory, we study the pigment-protein complex in detail by exploring the energy transfer and coherence dynamics. The ground-state vibrational coherence generated by incoherent radiations is shown to be long-survived and is demonstrated to be significant in promoting the excitation energy transfer. This is attributed to the nonequilibriumness of the system caused by the detailed-balance-breaking, which funnels the downhill migration of excitons.

  7. Self-organization of a neural network with heterogeneous neurons enhances coherence and stochastic resonance

    Science.gov (United States)

    Li, Xiumin; Zhang, Jie; Small, Michael

    2009-03-01

    Most network models for neural behavior assume a predefined network topology and consist of almost identical elements exhibiting little heterogeneity. In this paper, we propose a self-organized network consisting of heterogeneous neurons with different behaviors or degrees of excitability. The synaptic connections evolve according to the spike-timing dependent plasticity mechanism and finally a sparse and active-neuron-dominant structure is observed. That is, strong connections are mainly distributed to the synapses from active neurons to inactive ones. We argue that this self-emergent topology essentially reflects the competition of different neurons and encodes the heterogeneity. This structure is shown to significantly enhance the coherence resonance and stochastic resonance of the entire network, indicating its high efficiency in information processing.

  8. Two-mode excited entangled coherent states and their entanglement properties

    Institute of Scientific and Technical Information of China (English)

    Zhou Dong-Lin; Kuang Le-Man

    2009-01-01

    This paper introduces two types of two-mode excited entangled coherent states(TMEECSs)|Ψ±(α,m,n)>,studies their entanglement characteristics,and investigates the influence of photon excitations on quantum entanglement.It shows that for the state|Ψ+(α,m,m)>the two-mode photon excitations affect seriously entanglement character while the state |Ψ-(α,m,m)>is always a maximally entangled state,and shows how such states can be produced by using cavity quantum electrodynamics and quantum measurements.It finds that the entanglement amount of the TMEECSs is larger than that of the single-mode excited entangled coherent states with the same photon excitation number.

  9. Enhanced entanglement of two different mechanical resonators via coherent feedback

    CERN Document Server

    Li, Jie; Zippilli, Stefano; Vitali, David; Zhang, Tiancai

    2016-01-01

    It is shown [New J. Phys. 17, 103037 (2015)] that extremely large and robust entanglement between two different mechanical resonators could be achieved, either dynamically or in the steady state, in an optomechanical system in which a single cavity mode driven by a suitably chosen two-tone field is coupled to two mechanical modes. The main limitation of the scheme is that the cavity decay rate must be much smaller than the two mechanical frequencies and their difference, allowing taking the rotating wave approximation where counter-rotating, non-resonant terms associated with the bichromatic driving are negligible. Here we show that, by simply adding a coherent feedback loop, the large entanglement can be remarkably enhanced and the effective cavity decay rate can be significantly reduced. Therefore, it improves the results of Ref. [New J. Phys. 17, 103037 (2015)] and meantime greatly extends the validity of the scheme.

  10. Resonant excitation of coupled skyrmions by spin-transfer torque

    Science.gov (United States)

    Dai, Y. Y.; Wang, H.; Yang, T.; Zhang, Z. D.

    2016-12-01

    Resonant excitations of coupled skyrmions in Co/Ru/Co nanodisks activated by spin-transfer torque (STT) have been studied by micromagnetic simulations. It is found that STT is an effective method to manipulate skyrmion dynamics. Unlike the dynamics driven by a microwave field, two skyrmions with opposite chiralities move synchronously in the same direction when they are driven by STT, which makes it easier to observe the dynamics of coupled skyrmions in experiments. Resonant excitations of coupled skyrmions can be controlled by changing the frequency or amplitude ratio of a dual-frequency alternating current (AC). In addition, the magnetostatic interaction between the two skyrmions plays an important role in the dynamics of coupled skyrmions.

  11. Artificial excitation of ELF waves with frequency of Schumann resonance

    Science.gov (United States)

    Streltsov, A. V.; Guido, T.; Tulegenov, B.; Labenski, J.; Chang, C.-L.

    2014-11-01

    We report results from the experiment aimed at the artificial excitation of extremely low-frequency (ELF) electromagnetic waves with frequencies corresponding to the frequency of Schumann resonance. Electromagnetic waves with these frequencies can form a standing pattern inside the spherical cavity formed by the surface of the Earth and the ionosphere. In the experiment the ELF waves were excited by heating the ionosphere with X-mode HF electromagnetic waves generated at the High Frequency Active Auroral Research Program (HAARP) facility in Alaska. The experiment demonstrates that heating of the ionosphere can excite relatively large-amplitude electromagnetic waves with frequencies in the range 7.8-8.0 Hz when the ionosphere has a strong F layer, the frequency of the HF radiation is in the range 3.20-4.57 MHz, and the electric field greater than 5 mV/m is present in the ionosphere.

  12. Coherent Zeeman resonance from electron spin coherence in a mixed-type GaAs/AlAs quantum well.

    Science.gov (United States)

    O'Leary, Shannon; Wang, Hailin; Prineas, John P

    2007-03-01

    Coherent Zeeman resonance from electron spin coherence is demonstrated in a Lambda-type three-level system, coupling electron spin states via trions. The optical control of electron density that is characteristic of a mixed-type quantum-well facilitates the study of trion formation as well as the effects of many-body interactions on the manifestation of electron spin coherence in the nonlinear optical response.

  13. Observation of Wakefields and Resonances in Coherent Synchrotron Radiation

    CERN Document Server

    Billinghurst, B E; Baribeau, C; Batten, T; Dallin, L; May, T E; Vogt, J M; Wurtz, W A; Warnock, R; Bizzizero, D A; Kramer, S

    2015-01-01

    We report on high resolution measurements of resonances in the spectrum of coherent synchrotron radiation (CSR) at the Canadian Light Source (CLS). The resonances permeate the spectrum at wavenumber intervals of $0.074 ~\\textrm{cm}^{-1}$, and are highly stable under changes in the machine setup (energy, bucket filling pattern, CSR in bursting or continuous mode). Analogous resonances were predicted long ago in an idealized theory as eigenmodes of a smooth toroidal vacuum chamber driven by a bunched beam moving on a circular orbit. A corollary of peaks in the spectrum is the presence of pulses in the wakefield of the bunch at well defined spatial intervals. Through experiments and further calculations we elucidate the resonance and wakefield mechanisms in the CLS vacuum chamber, which has a fluted form much different from a smooth torus. The wakefield is observed directly in the 30-110 GHz range by RF diodes, and indirectly by an interferometer in the THz range. The wake pulse sequence found by diodes is less ...

  14. Experimental Investigation on Selective Excitation of Two-Pulse Coherent Anti-Stokes Raman Scattering

    Institute of Scientific and Technical Information of China (English)

    LI Xia; ZHANG Hui; ZHANG Xiang-Yun; ZHANG Shi-An; WANG Zu-Geng; SUN Zhen-Rong

    2008-01-01

    Selective excitation of coherent anti-Stokes Raman scattering from the benzene solution is achieved by adaptive pulse shaping based on genetic algorithm, and second harmonic generation frequency-resolved optical gating (SHG-FROG) technique is adopted to characterize the original and optimal laser pulses. The mechanism for two-pulse coherent mode-selective excitation of Raman scattering is experimentally investigated by modulating the pump pulse in the frequency domain, and it is indicated that two-pulse coherent mode-selective excitation of Raman scattering mainly depends on the effective frequency components of the pump pulse related to specific vibrational mode. The experimental results suggest that two-pulse CARS has good signal-to-background ratio and high sensitivity, and it has attractive potential applications in the complicated molecular system.

  15. Vacuum-Induced Coherence in Ultracold Photoassociative Ro-Vibrational Excitations

    CERN Document Server

    Das, Sumanta; Deb, Bimalendu

    2011-01-01

    We show that coherence between two excited ro-vibrational states belonging to the same molecular electronic configuration arises quite naturally due to their interaction with electromagnetic vacuum. For initial preparation of a molecule in the desired ro-vibrational states, we propose to employ the method of ultracold photoassociation. Spontaneous decay of the excited molecule then gives rise to vacuum induced coherence between the excited ro-vibrational states. We demonstrate theoretically an interesting interplay of effects due to vacuum induced coherence and photoassociation. We apply our theory to photoassociation of bosonic Ytterbium (^{174}Yb) atoms which appear to be a promising system for exploring such interplay. The effects discussed here can be important for controlling decoherence and dissipation in molecular systems.

  16. Quenching of the Giant Dipole Resonance Strength at High Excitation Energy

    Energy Technology Data Exchange (ETDEWEB)

    Santonocito, D. [INFN - Laboratori Nazionali del Sud, via S. Sofia 62, I-95123 Catania (Italy); Blumenfeld, Y. [Institut de Physique Nucleaire, IN2P3-CNRS, F-91406 Orsay (France); Agodi, C. [INFN - Laboratori Nazionali del Sud, via S. Sofia 62, I-95123 Catania (Italy); Alba, R. [INFN - Laboratori Nazionali del Sud, via S. Sofia 62, I-95123 Catania (Italy); Bellia, G. [INFN - Laboratori Nazionali del Sud, via S. Sofia 62, I-95123 Catania (Italy); Dipartimento di Fisica e Astronomia dell' Universita di Catania, via S. Sofia 64, I-95123 Catania (Italy); Coniglione, R. [INFN - Laboratori Nazionali del Sud, via S. Sofia 62, I-95123 Catania (Italy); Delaunay, F. [Institut de Physique Nucleaire, IN2P3-CNRS, F-91406 Orsay (France); Del Zoppo, A. [INFN - Laboratori Nazionali del Sud, via S. Sofia 62, I-95123 Catania (Italy); Finocchiaro, P. [INFN - Laboratori Nazionali del Sud, via S. Sofia 62, I-95123 Catania (Italy); Frascaria, N. [Institut de Physique Nucleaire, IN2P3-CNRS, F-91406 Orsay (France); Hongmei, F. [INFN - Laboratori Nazionali del Sud, via S. Sofia 62, I-95123 Catania (Italy); Lima, V. [Institut de Physique Nucleaire, IN2P3-CNRS, F-91406 Orsay (France); Maiolino, C. [INFN - Laboratori Nazionali del Sud, via S. Sofia 62, I-95123 Catania (Italy); Migneco, E. [INFN - Laboratori Nazionali del Sud, via S. Sofia 62, I-95123 Catania (Italy); Dipartimento di Fisica e Astronomia dell' Universita di Catania, via S. Sofia 64, I-95123 Catania (Italy); Piattelli, P. [INFN - Laboratori Nazionali del Sud, via S. Sofia 62, I-95123 Catania (Italy); Sapienza, P. [INFN - Laboratori Nazionali del Sud, via S. Sofia 62, I-95123 Catania (Italy); Scarpaci, J.A. [Institut de Physique Nucleaire, IN2P3-CNRS, F-91406 Orsay (France)

    2007-05-15

    The evolution with excitation energy of the Giant Dipole Resonance features in nuclei of mass A{approx}108-136 is reviewed. We first discuss the results of the experiments performed with MEDEA studying the GDR gamma decay from hot nuclei populated at excitation energies above 300 MeV. The focus of the paper is on the excitation energy region between 160 and 290 MeV. This region has been investigated through the study of the reactions {sup 116}Sn + {sup 12}C at 17 and 23A MeV, and {sup 116}Sn + {sup 24}Mg at 17A MeV. Gamma-rays were detected using MEDEA in coincidence with evaporation residues detected in MACISTE. The analysis of the gamma-ray spectra and their comparison with statistical calculations are presented. The comparison with {gamma}-ray spectra from the reaction {sup 36}Ar + {sup 98}Mo at higher excitation energies shows a coherent scenario where a progressive reduction of {gamma} multiplicity relative to predictions for 100% of the Energy Weighted Sum Rule is observed above 200 MeV excitation energy. Finally, the existence of a link between disappearance of collective motion and the liquid-gas phase transitions is discussed.

  17. Experimental investigations on the splitting of coherent population trapping resonances by the nuclear magnetic moment

    Energy Technology Data Exchange (ETDEWEB)

    Lammegger, Roland; Vasari, Ivan; Neureiter, Christian; Windholz, Laurentius [Inst. f. Experimentalphysik, Techn. Univ. Graz (Austria)

    2007-07-01

    Coherent population trapping (CPT) is a resonance phenomenon due to a quantum mechanical interference effect within an atomic system. The resonantly driven atomic level population is being trapped into a superpositional dark state, yielding the atomic medium transparent for the exciting electromagnetic fields. The observation of this effect requires a special electronic structure ({lambda}-system) and suitable lifetimes which can be found e.g. in alkali atoms. We present experimental investigations on the behavior of the CPT resonances split by the nuclear magnetic moment under different external magnetic fields, laser polarizations and laser intensities. We focus our considerations on a special type of the {lambda}-System formation. In this case the center of gravity of the pair of split CPT resonances (called pseudoresonance) is sensitive to external magnetic fields only to second order in the magnetic field strength. The short term frequency stability of this pseudoresonance approaches the level of 10{sup -14}/{radical}({tau}). Thus such resonances seems to be a good candidate for applications in compact atomic clocks used e.g. in GPS receivers and Satellites.

  18. Coherent transport and energy flow patterns in photosynthesis under incoherent excitation.

    Science.gov (United States)

    Pelzer, Kenley M; Can, Tankut; Gray, Stephen K; Morr, Dirk K; Engel, Gregory S

    2014-03-13

    Long-lived coherences have been observed in photosynthetic complexes after laser excitation, inspiring new theories regarding the extreme quantum efficiency of photosynthetic energy transfer. Whether coherent (ballistic) transport occurs in nature and whether it improves photosynthetic efficiency remain topics of debate. Here, we use a nonequilibrium Green's function analysis to model exciton transport after excitation from an incoherent source (as opposed to coherent laser excitation). We find that even with an incoherent source, the rate of environmental dephasing strongly affects exciton transport efficiency, suggesting that the relationship between dephasing and efficiency is not an artifact of coherent excitation. The Green's function analysis provides a clear view of both the pattern of excitonic fluxes among chromophores and the multidirectionality of energy transfer that is a feature of coherent transport. We see that even in the presence of an incoherent source, transport occurs by qualitatively different mechanisms as dephasing increases. Our approach can be generalized to complex synthetic systems and may provide a new tool for optimizing synthetic light harvesting materials.

  19. Parametric excitation of multiple resonant radiations from localized wavepackets

    CERN Document Server

    Conforti, Matteo; Mussot, Arnaud; Kudlinski, Alexandre

    2015-01-01

    Fundamental physical phenomena such as laser-induced ionization, driven quantum tunneling, Faraday waves, Bogoliubov quasiparticle excitations, and the control of new states of matter rely on time-periodic driving of the system. A remarkable property of such driving is that it can induce the localized (bound) states to resonantly couple to the continuum. Therefore experiments that allow for enlightening and controlling the mechanisms underlying such coupling are of paramount importance. We implement such an experiment in a special fiber optics system characterized by a dispersion oscillating along the propagation coordinate, which mimics "time". The quasi-momentum associated with such periodic perturbation is responsible for the efficient coupling of energy from the localized wave-packets sustained by the fiber nonlinearity into free-running linear dispersive waves (continuum), at multiple resonant frequencies. Remarkably, the observed resonances can be explained by means of a unified approach, regardless of ...

  20. An Electromagnetically Excited Silicon Nitride Beam Resonant Accelerometer

    Directory of Open Access Journals (Sweden)

    2009-02-01

    Full Text Available A resonant microbeam accelerometer of a novel highly symmetric structure based on MEMS bulk-silicon technology is proposed and some numerical modeling results for this scheme are presented. The accelerometer consists of two proof masses, four supporting hinges, two anchors, and a vibrating triple beam, which is clamped at both ends to the two proof masses. LPCVD silicon rich nitride is chosen as the resonant triple beam material, and parameter optimization of the triple-beam structure has been performed. The triple beam is excited and sensed electromagnetically by film electrodes located on the upper surface of the beam. Both simulation and experimental results show that the novel structure increases the scale factor of the resonant accelerometer, and ameliorates other performance issues such as cross axis sensitivity of insensitive input acceleration, etc.

  1. Resonant Excitation of Terahertz Surface Plasmons in Subwavelength Metal Holes

    Directory of Open Access Journals (Sweden)

    Weili Zhang

    2007-01-01

    Full Text Available We present a review of experimental studies of resonant excitation of terahertz surface plasmons in two-dimensional arrays of subwavelength metal holes. Resonant transmission efficiency higher than unity was recently achieved when normalized to the area occupied by the holes. The effects of hole shape, hole dimensions, dielectric function of metals, polarization dependence, and array film thickness on resonant terahertz transmission in metal arrays were investigated by the state-of-the-art terahertz time-domain spectroscopy. In particular, extraordinary terahertz transmission was demonstrated in arrays of subwavelength holes made even from Pb, a generally poor metal, and having thickness of only one-third of skin depth. Terahertz surface plasmons have potential applications in terahertz imaging, biosensing, interconnects, and development of integrated plasmonic components for terahertz generation and detection.

  2. Nonlinear excitation kinetics of biased quantum wells. Coherent dynamical screening effect

    DEFF Research Database (Denmark)

    Turchinovich, Dmitry; Jepsen, Peter Uhd

    2006-01-01

    In this paper we describe a strongly nonlinear process of ultrafast photoexcitation of a biased quantum well. This process is governed by coherent dynamical screening, where the instantaneously polarized photoexcited carriers screen initial bias field. This results in a dynamic modification...... of the bandstructure of the quantum well, which is totally coherent with the temporal intensity distribution of the excitation laser pulse. We developed a time-resolved theoretical model of coherent dynamical screening, which predicts interesting fundamental consequences, such as nonlinear absorption and ultra......-broadband THz emission. The results of our THz and optical experiments are in good agreement with the theoretical model....

  3. Excited, bound and resonant positron-atom systems

    Energy Technology Data Exchange (ETDEWEB)

    Bromley, M W J [Department of Physics and Computational Science Research Center, San Diego State University, San Diego CA 92182 (United States); Mitroy, J, E-mail: mbromley@physics.sdsu.ed [ARC Centre for Antimatter-Matter Studies and Faculty of Education, Health and Science, Charles Darwin University, Darwin NT 0909 (Australia)

    2010-01-01

    Calculations have demonstrated that eleven neutral atoms can bind positrons, while many more can bind positronium. This is a short review of recent progress made in understanding some of the underlying mechanisms. The emphasis here being on configuration interaction calculations with excited state configurations. These have demonstrated the existence of a {sup 2}P{sup o} excited state of e{sup +}Ca, which consists predominantly of a positronium cluster orbiting the Ca{sup +} ion in the L = 1 partial wave. Preliminary results are presented of excited state positron binding to a model alkali atom, where the excited {sup 1}P{sup o} states are stable over a limited region. Implications for the unnatural parity, {sup 2,4}S{sup o}, states of PsH, LiPs, NaPs and KPs are also discussed. The e{sup +}Mg, e{sup +}Cu, e{sup +}Zn and e{sup +}Cd systems show a lack of a {sup 2}P{sup o} excited state, each instead possessing a low-energy p-wave shape resonance of varying strength.

  4. TOPICAL REVIEW: Interaction of coherent phonons with defects and elementary excitations

    Science.gov (United States)

    Hase, Muneaki; Kitajima, Masahiro

    2010-02-01

    We present an overview of the feasibility of using coherent phonon spectroscopy to study interaction dynamics of excited lattice vibrations with their environments. By exploiting the features of coherent phonons with a pump-probe technique, one can study lattice motions in a sub-picosecond time range. The dephasing properties tell us not only about interaction dynamics with carriers (electrons and holes) or thermal phonons but also about point defects in crystals. Modulations of the coherent phonon amplitude by more than two modes are closely related to phonon-carrier or phonon-phonon interferences. Related to this phenomenon, formation of coherent phonons at higher harmonics gives direct evidence for phonon-phonon couplings. A combined study of coherent phonons and ultrafast carrier response can be useful for understanding phonon-carrier interaction dynamics. For metals like zinc, nonequilibrium electrons may dominate the dynamics of both relaxation and generation of coherent phonons. The frequency chirp of coherent phonons can be a direct measure of how and when phonon-phonon and phonon-carrier couplings occur. Carbon nanotubes show some complicated behavior due to the existence of many modes with different symmetries, resulting in superposition or interference. To illustrate one of the most interesting applications, the selective excitation of specific phonon modes through the use of a pulse train technique is shown.

  5. Nanoscale femtosecond imaging of transient hot solid density plasmas with elemental and charge state sensitivity using resonant coherent diffraction

    CERN Document Server

    Kluge, Thomas; Chung, H -K; Gutt, C; Huang, L G; Zacharias, M; Schramm, U; Cowan, T E

    2015-01-01

    Here we propose to exploit the low energy bandwidth, small wavelength and penetration power of ultrashort pulses from XFELs for resonant Small Angle Scattering (SAXS) on plasma structures in laser excited plasmas. Small angle scattering allows to detect nanoscale density fluctuations in forward scattering direction. Typically, the SAXS signal from laser excited plasmas is expected to be dominated by the free electron distribution. We propose that the ionic scattering signal becomes visible when the X-ray energy is in resonance with an electron transition between two bound states (Resonant coherent X-ray diffraction, RCXD). In this case the scattering cross-section dramatically increases so that the signal of X-ray scattering from ions silhouettes against the free electron scattering background which allows to measure the opacity and derived quantities with high spatial and temporal resolution, being fundamentally limited only by the X-ray wavelength and timing. Deriving quantities such as ion spatial distribu...

  6. Resonant parametric excitations driven by lower-hybrid fields

    Science.gov (United States)

    Villalon, E.

    1980-11-01

    Three-wave parametric excitation in inhomogeneous plasmas is examined in a two-dimensional geometry relevant to supplementary rf heating of tokamaks. The stabilization of resonant parametric excitation due to a linear mismatch in wavenumbers and to the Landau-damping rates of the decay waves is analyzed, assuming that the magnitude of the pump field is constant in time and in the spatial region where the resonant interaction takes place. Both types of temporally growing modes and spatially amplified instabilities are studied, using a WKB analysis. It is shown that by increasing the strength of the mismatch K prime or the width of the pump L, the growth rate of the fastest growing normal mode will decrease. The amount of spatial amplification is also reduced by the mismatch in wavenumbers and by the damping rates of the excited waves. Because of the finite spatial extent of the pump electric field, the amplification length is smaller than or equal to L, depending on the strength of the mismatch and damping rates.

  7. Coherent phase control of excitation of atoms by bichromatic laser radiation in an electric field

    NARCIS (Netherlands)

    Astapenko, VA

    A new method for coherent phase control of excitation of atoms in a discrete spectrum under the action of bichromatic laser radiation with the frequency ratio 1 : 2 is analysed. An important feature of this control method is the presence of a electrostatic field, which removes the parity selection

  8. Solitonic excitations in linearly coherent channels of bilayer quantum Hall stripes

    Science.gov (United States)

    Doiron, C. B.; Côté, R.; Fertig, H. A.

    2005-09-01

    In some range of interlayer distances, the ground state of the two-dimensional electron gas at filling factor ν=4N+1 with N=0,1,2,… is a coherent stripe phase in the Hartree-Fock approximation. This phase has one-dimensional coherent channels that support charged excitations in the form of pseudospin solitons. In this work, we compute the transport gap of the coherent striped phase due to the creation of soliton-antisoliton pairs using a supercell microscopic unrestricted Hartree-Fock approach. We study this gap as a function of interlayer distance and tunneling amplitude. Our calculations confirm that the soliton-antisoliton excitation energy is lower than the corresponding Hartree-Fock electron-hole pair energy. We compare our results with estimates of the transport gap obtained from a field-theoretic model valid in the limit of slowly varying pseudospin textures.

  9. Excitation-energy dependence of the giant dipole resonance width

    Science.gov (United States)

    Enders, G.; Berg, F. D.; Hagel, K.; Kühn, W.; Metag, V.; Novotny, R.; Pfeiffer, M.; Schwalb, O.; Charity, R. J.; Gobbi, A.; Freifelder, R.; Henning, W.; Hildenbrand, K. D.; Holzmann, R.; Mayer, R. S.; Simon, R. S.; Wessels, J. P.; Casini, G.; Olmi, A.; Stefanini, A. A.

    1992-07-01

    High-energy γ rays have been measured in coincidence with heavy fragents in deeply inelastic reactions of 136Xe+48Ti at 18.5 MeV/nucleon. The giant dipole resonance (GDR) strength function is deduced from an analysis of the photon spectra within the statistical model. The GDR width Γ is studied as a function of the fragment excitation energy E*. A saturation at about Γ=10 MeV is observed for E*/A>=1.0 MeV/nucleon.

  10. Excitation-energy dependence of the giant dipole resonance width

    Energy Technology Data Exchange (ETDEWEB)

    Enders, G.; Berg, F.D.; Hagel, K.; Kuehn, W.; Metag, V.; Novotny, R.; Pfeiffer, M.; Schwalb, O. (II. Physikalisches Institut, Universitaet, Giessen, Giessen (Germany)); Charity, R.J.; Gobbi, A.; Freifelder, R.; Henning, W.; Hildenbrand, K.D.; Holzmann, R.; Mayer, R.S.; Simon, R.S.; Wessels, J.P. (Gesellschaft fuer Schwerionenforschung Darmstadt, Darmstadt (Germany)); Casini, G.; Olmi, A.; Stefanini, A.A. (Istituto Nazionale di Fisica Nucleare and University of Florence, Florence (Italy))

    1992-07-13

    High-energy {gamma} rays have been measured in coincidence with heavy fragents in deeply inelastic reactions of {sup 136}Xe+{sup 48}Ti at 18.5 MeV/nucleon. The giant dipole resonance (GDR) strength function is deduced from an analysis of the photon spectra within the statistical model. The GDR width {Gamma} is studied as a function of the fragment excitation energy {ital E}{sup *}. A saturation at about {Gamma}=10 MeV is observed for {ital E}{sup *}/{ital A}{ge}1.0 MeV/nucleon.

  11. Sensitivity of nonlinear photoionization to resonance substructure in collective excitation

    Science.gov (United States)

    Mazza, T.; Karamatskou, A.; Ilchen, M.; Bakhtiarzadeh, S.; Rafipoor, A. J.; O'Keeffe, P.; Kelly, T. J.; Walsh, N.; Costello, J. T.; Meyer, M.; Santra, R.

    2015-04-01

    Collective behaviour is a characteristic feature in many-body systems, important for developments in fields such as magnetism, superconductivity, photonics and electronics. Recently, there has been increasing interest in the optically nonlinear response of collective excitations. Here we demonstrate how the nonlinear interaction of a many-body system with intense XUV radiation can be used as an effective probe for characterizing otherwise unresolved features of its collective response. Resonant photoionization of atomic xenon was chosen as a case study. The excellent agreement between experiment and theory strongly supports the prediction that two distinct poles underlie the giant dipole resonance. Our results pave the way towards a deeper understanding of collective behaviour in atoms, molecules and solid-state systems using nonlinear spectroscopic techniques enabled by modern short-wavelength light sources.

  12. Control of coherent excitation of neon in the extreme ultraviolet regime.

    Science.gov (United States)

    Plenge, Jürgen; Wirsing, Andreas; Raschpichler, Christopher; Wassermann, Bernhard; Rühl, Eckart

    2011-01-01

    Coherent excitation of a superposition of Rydberg states in neon by the 13th harmonic of an intense 804 nm pulse and the formation of a wave packet is reported. Pump-probe experiments are performed, where the 3d-manifold of the 2p6-->2p5 (2P3/2) 3d [1/2]1- and 2p6-->2p5 (2P3/2) 3d [3/2]1-transitions are excited by an extreme ultraviolet (XUV) radiation pulse, which is centered at 20.05 eV photon energy. The temporal evolution of the excited state population is probed by ionization with a time-delayed 804 nm pulse. Control of coherent transient excitation and wave packet dynamics in the XUV-regime is demonstrated, where the spectral phase of the 13th harmonic is used as a control parameter. Modulation of the phase is achieved by propagation of the XUV-pulse through neon of variable gas density. The experimental results indicate that phase-shaped high-order harmonics can be used to control fundamental coherent excitation processes in the XUV-regime.

  13. Coherence and Decoherence of a Localized Excitation on a Surface Adatom

    Institute of Scientific and Technical Information of China (English)

    高世武; H.Petek; J.Aizpurua; P.Apell

    2002-01-01

    A theory of coherent excitation of a localized state on an adatom by two-photon photoemission spectroscopy(TR-2PPE) is presented within a microscopic model and the time-dependent formalism. Coherent oscillation and incoherent population decay of the excitation are obtained, and are shown to attain well-defined lifetime constants only in the long-delay limit. In addition, we have found a competing excitation channel via electron transfer. The theory is applied to Cs/Cu (111), which reproduces a few qualitative features observed in recent experiments. The effect of atomic motion on the 2PPE spectra, which manifests dominantly as a redshift in the spectrum, has been analysed.

  14. Enhancement of level-crossing resonances in rubidium atoms by frequency control of the exciting radiation field

    CERN Document Server

    Auzinsh, Marcis; Ferber, Ruvin; Gahbauer, Florian; Kalvans, Linards; Mozers, Arturs; Spiss, Agris

    2013-01-01

    We studied magneto-optical resonances caused by excited-state level crossings in a nonzero magnetic field. Experimental measurements were performed on the transitions of the $D_2$ line of rubidium. These measured signals were described by a theoretical model that takes into account all neighboring hyperfine transitions, the mixing of magnetic sublevels in an external magnetic field, the coherence properties of the exciting laser radiation, and the Doppler effect. Good agreement between the experimental measurements and the theoretical model could be achieved over a wide range of laser power densities. We further showed that the contrasts of the level-crossing peaks can be sensitive to changes in the frequency of the exciting laser radiation as small as several tens of megahertz when the hyperfine splitting of the exciting state is larger than the Doppler broadening.

  15. Sub-natural linewidth resonances in coherently-driven double system

    Indian Academy of Sciences (India)

    Niharika Singh; Q V Lawande; R D’souza; A Ray; B N Jagatap

    2010-12-01

    We investigate theoretically the pump-probe spectroscopy of coherently-driven four-level system with two closely spaced excited common levels, thereby forming a double system. Using the master equation approach, analytical results are obtained for the absorption spectrum of a weak probe in the presence of a strong pump. The model is applied to the double system 52 1/2 = 1, 2 → 523/2 ' = 1, 2 of 87Rb atom. It is shown that the absorption spectrum consists of a triplet, of which one resonance is of sub-natural linewidth depending on the atom–field interaction parameters. The effect of Doppler broadening on the absorption spectrum is also investigated.

  16. Coherent control of magnetization precession in electrically detected time domain ferromagnetic resonance

    Directory of Open Access Journals (Sweden)

    O. Wid

    2015-11-01

    Full Text Available We demonstrate coherent control of time domain ferromagnetic resonance by all electrical excitation and detection. Using two ultrashort magnetic field steps with variable time delay we control the induction decay in yttrium iron garnet (YIG. By setting suitable delay times between the two steps the precession of the magnetization can either be enhanced or completely stopped. The method allows for a determination of the precession frequency within a few precession periods and with an accuracy much higher than can be achieved using fast fourier transformation. Moreover it holds the promise to massively increase precession amplitudes in pulsed inductive microwave magnetometry (PIMM using low amplitude finite pulse trains. Our experiments are supported by micromagnetic simulations which nicely confirm the experimental results.

  17. Coherent control of magnetization precession in electrically detected time domain ferromagnetic resonance

    Energy Technology Data Exchange (ETDEWEB)

    Wid, O.; Wahler, M.; Homonnay, N.; Richter, T. [Institut für Physik, Martin-Luther-Universität Halle-Wittenberg, D-06099 (Germany); Schmidt, G., E-mail: georg.schmidt@physik.uni-halle.de [Institut für Physik, Martin-Luther-Universität Halle-Wittenberg, D-06099 (Germany); IZM, Martin-Luther-Universität Halle-Wittenberg, D-06099 (Germany)

    2015-11-15

    We demonstrate coherent control of time domain ferromagnetic resonance by all electrical excitation and detection. Using two ultrashort magnetic field steps with variable time delay we control the induction decay in yttrium iron garnet (YIG). By setting suitable delay times between the two steps the precession of the magnetization can either be enhanced or completely stopped. The method allows for a determination of the precession frequency within a few precession periods and with an accuracy much higher than can be achieved using fast fourier transformation. Moreover it holds the promise to massively increase precession amplitudes in pulsed inductive microwave magnetometry (PIMM) using low amplitude finite pulse trains. Our experiments are supported by micromagnetic simulations which nicely confirm the experimental results.

  18. Detection of a coherent population trapping resonance in a beam of {sup 87}Rb atoms by the Ramsey method

    Energy Technology Data Exchange (ETDEWEB)

    Sokolov, I M [Peter the Great St.Petersburg Polytechnic University, St.Petersburg (Russian Federation)

    2015-10-31

    Formation of a coherent population trapping (CPT) resonance is studied in the interaction of a beam of {sup 87}Rb atoms with two spatially separated domains of the dichromatic field. Various resonance excitation schemes are compared depending on the choice of operation transitions and type of the polarisation scheme. In the case of a single-velocity atomic beam, the dependence of the CPT resonance profile is studied as a function of principal parameters of the system: beam velocity, distance between optical fields, laser beam dimensions and intensities, and applied permanent magnetic field. Influence of the atomic beam angular divergence and residual beam velocity spread on the resonance quality parameter is estimated. (atomic beams)

  19. Role of coherent resonant nonlinear processes in the ultrashort KrF laser pulse propagation and filamentation in air

    Energy Technology Data Exchange (ETDEWEB)

    Smetanin, I.V.; Levchenko, A.O.; Shutov, A.V.; Ustinovskii, N.N. [P.N. Lebedev Physical Institute of Russian Academy of Sciences, 53 Leninskii pr., 119991 Moscow (Russian Federation); Zvorykin, V.D. [P.N. Lebedev Physical Institute of Russian Academy of Sciences, 53 Leninskii pr., 119991 Moscow (Russian Federation); National Research Nuclear University “MEPhI”, 31 Kashirskoe sh., 115409 Moscow (Russian Federation)

    2016-02-15

    Recent experiments on multiple filamentation of sub-picosecond terawatt-level KrF laser pulse in air and multi-photon ionization of air revealed an extremely low electron density in filaments, which is out of the conventional filamentation model considering Kerr self-focusing and plasma de-focusing. We propose here the coherent resonant scattering and ionization processes at the pulse durations significantly less than the polarization relaxation time to be possible explanation of the observed filamentation peculiarities. Namely, we argue that the plasma production results from the resonance enhanced (2+1)-photon ionization of the oxygen molecules through the two-photon excitation of the 3s metastable Rydberg state. Coherent Raman self-scattering at rotational transitions of nitrogen molecules provides self-induced focusing of the ultrashort UV laser pulse and filament formation.

  20. The separation of vibrational coherence from ground- and excited-electronic states in P3HT film

    KAUST Repository

    Song, Yin

    2015-06-07

    © 2015 AIP Publishing LLC. Concurrence of the vibrational coherence and ultrafast electron transfer has been observed in polymer/fullerene blends. However, it is difficult to experimentally investigate the role that the excited-state vibrational coherence plays during the electron transfer process since vibrational coherence from the ground- and excited-electronic states is usually temporally and spectrally overlapped. Here, we performed 2-dimensional electronic spectroscopy (2D ES) measurements on poly(3-hexylthiophene) (P3HT) films. By Fourier transforming the whole 2D ES datasets (S (λ 1, T∼ 2, λ 3)) along the population time (T∼ 2) axis, we develop and propose a protocol capable of separating vibrational coherence from the ground- and excited-electronic states in 3D rephasing and nonrephasing beating maps (S (λ 1, ν∼ 2, λ 3)). We found that the vibrational coherence from pure excited electronic states appears at positive frequency (+ ν∼ 2) in the rephasing beating map and at negative frequency (- ν∼ 2) in the nonrephasing beating map. Furthermore, we also found that vibrational coherence from excited electronic state had a long dephasing time of 244 fs. The long-lived excited-state vibrational coherence indicates that coherence may be involved in the electron transfer process. Our findings not only shed light on the mechanism of ultrafast electron transfer in organic photovoltaics but also are beneficial for the study of the coherence effect on photoexcited dynamics in other systems.

  1. Resonant tidal excitation of superfluid neutron stars in coalescing binaries

    CERN Document Server

    Yu, Hang

    2016-01-01

    We study the resonant tidal excitation of g-modes in coalescing superfluid neutron star binaries and investigate how such tidal driving impacts the gravitational-wave signal of the inspiral. Previous studies of this type treated the neutron star core as a normal fluid and thus did not account for its expected superfluidity. The source of buoyancy that supports the g-modes is fundamentally different in the two cases: in a normal fluid core the buoyancy is due to gradients in the proton-to-neutron fraction whereas in a superfluid core it is due to gradients in the muon-to-electron fraction. The latter yields a stronger stratification and a superfluid neutron star therefore has a denser spectrum of g-modes with frequencies above 10 Hz. As a result, many more g-modes undergo resonant tidal excitation as the binary sweeps through the bandwidth of gravitational-wave detectors such as LIGO. We find that roughly 10 times more orbital energy is transferred into g-mode oscillations if the neutron star has a superfluid ...

  2. Coherent Resonant Millenial-scale Climate Oscillations Triggered By Iceberg Surges

    Science.gov (United States)

    Timmermann, A.; Gildor, H.; Tziperman, E.; Schulz, M.

    We study the role of mean and stochastic freshwater forcing on the generation of millenial-scale climate variability in the North Atlantic using a low-order coupled atmosphere-ocean-sea-ice model. It is shown that millenial-scale oscillations can be excited stochastically, once the North Atlantic ocean is fresh enough. This finding is used in order to interpret the aftermath of iceberg surges (Heinrich events) in the glacial North Atlantic, which was characterized by an excitation of Dansgaard- Oeschger events. Based on our model results we hypothesize that Heinrich events trigger Dansgaard-Oeschger cycles, thereby explaining the existence of Bond cycles. The low order climate model is used in order to determine the mechanism of stochasti- cally excited millenial-scale variability in the North Atlantic. Sensitivity experiments reveal that the timescale of the oscillations can be decomposed into a stochastic and a diffusive component and that a generic homoclinic bifurcation acts as an organizing center for coherent resonant oscillations. Implications for interpreting paleo climatic records are discussed.

  3. Incoherent population mixing contributions to phase-modulation two-dimensional coherent excitation spectra

    Science.gov (United States)

    Grégoire, Pascal; Srimath Kandada, Ajay Ram; Vella, Eleonora; Tao, Chen; Leonelli, Richard; Silva, Carlos

    2017-09-01

    We present theoretical and experimental results showing the effects of incoherent population mixing on two-dimensional (2D) coherent excitation spectra that are measured via a time-integrated population and phase-sensitive detection. The technique uses four collinear ultrashort pulses and phase modulation to acquire two-dimensional spectra by isolating specific nonlinear contributions to the photoluminescence or photocurrent excitation signal. We demonstrate that an incoherent contribution to the measured line shape, arising from nonlinear population dynamics over the entire photoexcitation lifetime, generates a similar line shape to the expected 2D coherent spectra in condensed-phase systems. In those systems, photoexcitations are mobile such that inter-particle interactions are important on any time scale, including those long compared with the 2D coherent experiment. Measurements on a semicrystalline polymeric semiconductor film at low temperatures show that, in some conditions in which multi-exciton interactions are suppressed, the technique predominantly detects coherent signals and can be used, in our example, to extract homogeneous line widths. The same method used on a lead-halide perovskite photovoltaic cell shows that incoherent population mixing of mobile photocarriers can dominate the measured signal since carrier-carrier bimolecular scattering is active even at low excitation densities, which hides the coherent contribution to the spectral line shape. In this example, the intensity dependence of the signal matches the theoretical predictions over more than two orders of magnitude, confirming the incoherent nature of the signal. While these effects are typically not significant in dilute solution environments, we demonstrate the necessity to characterize, in condensed-phase materials systems, the extent of nonlinear population dynamics of photoexcitations (excitons, charge carriers, etc.) in the execution of this powerful population-detected coherent

  4. Iterative linearized density matrix propagation for modeling coherent excitation energy transfer in photosynthetic light harvesting.

    Science.gov (United States)

    Huo, P; Coker, D F

    2010-11-14

    Rather than incoherent hopping between chromophores, experimental evidence suggests that the excitation energy transfer in some biological light harvesting systems initially occurs coherently, and involves coherent superposition states in which excitation spreads over multiple chromophores separated by several nanometers. Treating such delocalized coherent superposition states in the presence of decoherence and dissipation arising from coupling to an environment is a significant challenge for conventional theoretical tools that either use a perturbative approach or make the Markovian approximation. In this paper, we extend the recently developed iterative linearized density matrix (ILDM) propagation scheme [E. R. Dunkel et al., J. Chem. Phys. 129, 114106 (2008)] to study coherent excitation energy transfer in a model of the Fenna-Matthews-Olsen light harvesting complex from green sulfur bacteria. This approach is nonperturbative and uses a discrete path integral description employing a short time approximation to the density matrix propagator that accounts for interference between forward and backward paths of the quantum excitonic system while linearizing the phase in the difference between the forward and backward paths of the environmental degrees of freedom resulting in a classical-like treatment of these variables. The approach avoids making the Markovian approximation and we demonstrate that it successfully describes the coherent beating of the site populations on different chromophores and gives good agreement with other methods that have been developed recently for going beyond the usual approximations, thus providing a new reliable theoretical tool to study coherent exciton transfer in light harvesting systems. We conclude with a discussion of decoherence in independent bilinearly coupled harmonic chromophore baths. The ILDM propagation approach in principle can be applied to more general descriptions of the environment.

  5. Storage of Multiple Coherent Microwave Excitations in an Electron Spin Ensemble

    DEFF Research Database (Denmark)

    Wu, Hua; George, Richard E.; Wesenberg, Janus H.;

    2010-01-01

    stored and retrieved. Here we employ holographic techniques to realize a coherent memory using a pulsed magnetic field gradient and demonstrate the storage and retrieval of up to 100 weak 10 GHz coherent excitations in collective states of an electron spin ensemble. We further show that such collective......Strong coupling between a microwave photon and electron spins, which could enable a long-lived quantum memory element for superconducting qubits, is possible using a large ensemble of spins. This represents an inefficient use of resources unless multiple photons, or qubits, can be orthogonally...

  6. Thin film characterization by resonantly excited internal standing waves

    Energy Technology Data Exchange (ETDEWEB)

    Di Fonzio, S. [SINCROTRONE TRIESTE, Trieste (Italy)

    1996-09-01

    This contribution describes how a standing wave excited in a thin film can be used for the characterization of the properties of the film. By means of grazing incidence X-ray reflectometry one can deduce the total film thickness. On the other hand in making use of a strong resonance effect in the electric field intensity distribution inside a thin film on a bulk substrate one can learn more about the internal structure of the film. The profile of the internal standing wave is proven by diffraction experiments. The most appropriate non-destructive technique for the subsequent thin film characterization is angularly dependent X-ray fluorescence analysis. The existence of the resonance makes it a powerful tool for the detection of impurities and of ultra-thin maker layers, for which the position can be determined with very high precision (about 1% of the total film thickness). This latter aspect will be discussed here on samples which had a thin Ti marker layer at different positions in a carbon film. Due to the resonance enhancement it was still possible to perform these experiments with a standard laboratory x-ray tube and with standard laboratory tool for marker or impurity detection in thin films.

  7. Polarization of resonantly excited X-ray lines

    Science.gov (United States)

    Shah, Chintan; Amaro, Pedro; Steinbrügge, René; Bernitt, Sven; Fritzsche, Stephan; Surzhykov, Andrey; Crespo Lopez-Urrutia, José R.; Tashenov, Stanislav

    2017-08-01

    For a wide range of temperatures, resonantly captured electrons with energies below the excitation threshold are the strongest source of X-ray line excitation in hot plasmas containing highly charged Fe ions. The angular distribution and polarization of X-rays emitted due to these processes were experimentally studied using an electron beam ion trap. The electron-ion collision energy was scanned over the KLL dielectronic, trielectronic, and quadruelectronic recombination resonances of Fe18+..24+ and Kr28+..34+ with an exemplary resolution of ~6 eV. The angular distribution of induced X-ray fluorescence was measured along and perpendicular to the electron beam propagation direction [1]. Subsequently, the polarization of X-ray fluorescence was also measured using a novel Compton polarimeter [2, 3].The experimental data reveal the alignment of the populated excited states and exhibit a high sensitivity to the relativistic Breit interaction [2, 4]. We observed that most of the transitions lead to polarization, including hitherto-neglected trielectronic and quadruelectronic recombination channels. Furthermore, these channels dominate the polarization of the prominent Kα X-rays emitted by hot anisotropic plasmas in a wide temperature range. The present experimental results comprehensively benchmark full-order atomic calculations carried out with the FAC [5] and RATIP [6] codes. We conclude that accurate polarization diagnostics of hot anisotropic plasmas, e.~g., of solar flares and active galactic nuclei, and laboratory fusion plasmas of tokamaks can only be obtained under the premise of careful inclusion of relativistic effects and higher-order resonances which were often neglected in previous works [1]. The present experiments also demonstrate the suitability of the applied technique for accurate directional diagnostics of electron or ion beams in hot plasmas [7].[1] C. Shah et al., Phys. Rev. E 93, 061201 (R) (2016)[2] C. Shah et al., Phys. Rev. A 92, 042702 (2015

  8. A coherent modified Redfield theory for excitation energy transfer in molecular aggregates

    Energy Technology Data Exchange (ETDEWEB)

    Hwang-Fu, Yu-Hsien; Chen, Wei; Cheng, Yuan-Chung, E-mail: yuanchung@ntu.edu.tw

    2015-02-02

    Highlights: • A CMRT method for coherent energy transfer in molecular aggregates was developed. • Applicability of the method was verified in two-site systems with various parameters. • CMRT accurately describes population dynamics in the FMO-complex. • The method is accurate in a large parameter space and computationally efficient. - Abstract: Excitation energy transfer (EET) is crucial in photosynthetic light harvesting, and quantum coherence has been recently proven to be a ubiquitous phenomenon in photosynthetic EET. In this work, we derive a coherent modified Redfield theory (CMRT) that generalizes the modified Redfield theory to treat coherence dynamics. We apply the CMRT method to simulate the EET in a dimer system and compare the results with those obtained from numerically exact path integral calculations. The comparison shows that CMRT provides excellent computational efficiency and accuracy within a large EET parameter space. Furthermore, we simulate the EET dynamics in the FMO complex at 77 K using CMRT. The results show pronounced non-Markovian effects and long-lasting coherences in the ultrafast EET, in excellent agreement with calculations using the hierarchy equation of motion approach. In summary, we have successfully developed a simple yet powerful framework for coherent EET dynamics in photosynthetic systems and organic materials.

  9. Isoscalar monopole and dipole excitations of cluster states and giant resonances in 12C

    Science.gov (United States)

    Kanada-En'yo, Yoshiko

    2016-05-01

    The isoscalar monopole (ISM) and dipole (ISD) excitations in 12C are investigated theoretically with the shifted antisymmetrized molecular dynamics (AMD) plus 3 α -cluster generator coordinate method (GCM). The small-amplitude vibration modes are described by coherent one-particle one-hole excitations expressed by a small shift of single-nucleon Gaussian wave functions within the AMD framework, whereas the large-amplitude cluster modes are incorporated by superposing 3 α -cluster wave functions in the GCM. The coupling of the excitations in the intrinsic frame with the rotation and parity transformation is taken into account microscopically by the angular-momentum and parity projections. The present a calculation that describes the ISM and ISD excitations over a wide energy region covering cluster modes in the low-energy region and the giant resonances in the high-energy region, although the quantitative description of the high-energy part is not satisfactory. The low-energy ISM and ISD strengths of the cluster modes are enhanced by the distance motion between α clusters, and they split into a couple of states because of the angular motion of α clusters. The low-energy ISM strengths exhaust 26% of the energy-weighted sum rule, which is consistent with the experimental data for the 12C(02+; 7.65 MeV) and 12C(03+; 10.3 MeV) measured by (e ,e') ,(α ,α') , and (6Li,6Li' ) scatterings. In the calculated low-energy ISD strengths, two 1- states (the 11- and 12- states) with the significant strengths are obtained over E =10 -15 MeV. The results indicate that the ISD excitations can be a good probe to experimentally search for new cluster states such as the 12C(12-) obtained in the present calculation.

  10. Theme Article - Time-Resolved X-Ray Scattering from Coherent Excitations in Solids

    Energy Technology Data Exchange (ETDEWEB)

    Trigo, Mariano; Reis, David (SLAC)

    2010-10-22

    Recent advances in pulsed x-ray sources have opened up new opportunities to study the dynamics of matter directly in the time domain with picosecond to femtosecond resolution. In this article, we present recent results from a variety of ultrafast sources on time-resolved x-ray scattering from elementary excitations in periodic solids. A few representative examples are given on folded acoustic phonons, coherent optical phonons, squeezed phonons, and polaritons excited by femtosecond lasers. Next-generation light sources, such as the x-ray-free electron laser, will lead to improvements in coherence, flux, and pulse duration. These experiments demonstrate potential opportunities for studying matter far from equilibrium on the fastest time scales and shortest distances that will be available in the coming years.

  11. Peptide backbone orientation and dynamics in spider dragline silk and two-photon excitation in nuclear magnetic and quadrupole resonance

    Energy Technology Data Exchange (ETDEWEB)

    Eles, P.T

    2005-07-01

    In the first part of the dissertation, spider dragline silk is studied by solid state NMR techniques. The dependence of NMR frequency on molecular orientation is exploited using the DECODER experiment to determine the orientation of the protein backbone within the silk fibre. Practical experimental considerations require that the silk fibres be wound about a cylindrical axis perpendicular to the external magnetic field, complicating the reconstruction of the underlying orientation distribution and necessitating the development of numerical techniques for this purpose. A two-component model of silk incorporating static b-sheets and polyglycine II helices adequately fits the NMR data and suggests that the b-sheets are well aligned along the silk axis (20 FWHM) while the helices are poorly aligned (68 FWHM). The effects of fibre strain, draw rate and hydration on orientation are measured. Measurements of the time-scale for peptide backbone motion indicate that when wet, a strain-dependent fraction of the poorly aligned component becomes mobile. This suggests a mechanism for the supercontraction of silk involving latent entropic springs that undergo a local strain-dependent phase transition, driving supercontraction. In the second part of this dissertation a novel method is developed for exciting NMR and nuclear quadrupole resonance (NQR) by rf irradiation at multiple frequencies that sum to (or differ by) the resonance frequency. This is fundamentally different than traditional NMR experiments where irradiation is applied on-resonance. With excitation outside the detection bandwidth, two-photon excitation allows for detection of free induction signals during excitation, completely eliminating receiver dead-time. A theoretical approach to describing two-photon excitation is developed based on average Hamiltonian theory. An intuition for two-photon excitation is gained by analogy to the coherent absorption of multiple photons requiring conservation of total energy and

  12. Numerical simulation of the resonantly excited capillary-gravity waves

    Science.gov (United States)

    Hanazaki, Hideshi; Hirata, Motonori; Okino, Shinya

    2015-11-01

    Capillary gravity waves excited by an obstacle are investigated by a direct numerical simulation. In the flow without capillary effects, it is well known that large-amplitude upstream advancing solitary waves are generated periodically under the resonant condition, i.e., when the phase velocity of the long surface waves and the mean flow velocity agrees. With capillary effects, solutions of the Euler equations show the generation of very short waves further upstream of the solitary waves and also in the depression region downstream of the obstacle. The overall characteristics of these waves agree with the solutions of the forced fifth-order KdV equation, while the weakly nonlinear theory generally overestimates the wavelength of the short waves.

  13. Emergence and coherence of oscillations in star networks of stochastic excitable elements

    CERN Document Server

    Kromer, Justus A; Neiman, Alexander B

    2015-01-01

    We study the emergence and coherence of stochastic oscillations in star networks of excitable elements in which peripheral nodes receive independent random inputs. A biophysical model of a distal branch of sensory neuron in which peripheral nodes of Ranvier are coupled to a central node by myelinated cable segments is used along with a generic model of networked stochastic active rotators. We show that coherent oscillations can emerge due to stochastic synchronization of peripheral nodes and that the degree of coherence can be maximized by tuning the coupling strength and the size of the network. Analytical results are obtained for the strong coupling regime of the active rotator network. In particular, we show that in the strong coupling regime the network dynamics can be described by an effective single active rotator with rescaled parameters and noise.

  14. Decoherence of quantum excitation of even/odd coherent states in thermal environment

    Indian Academy of Sciences (India)

    Mohammadbeigi A; Tavassoly M K

    2016-04-01

    In this paper, we study the decoherence of quantum excitation (photon-added)even/odd coherent states, $((\\^{a})^m|\\alpha_{\\pm}\\rangle)$, in a thermal environment by investigating the variation of negative part of the Wigner quasidistribution function vs. the rescaled time. For this purpose, at first we obtain the time-dependent Wigner function corresponding to the mentioned states in the framework of standard master equation. Then, the time evolution of the Wigner function associated with photon-added even/odd coherent states, as well as the number of added photons $m$ are analysed. It is shown that, in both states, the negative part of the Wigner function decreases with time. By deriving the threshold value of the rescaled time for single photon-added even/odd coherent states, it is also found that, if the rescaled time exceeds the threshold value, the associated Wigner function becomes positive, i.e., the decoherence occurs completely.

  15. Double resonance spectroscopy of multiple-photon excited molecules

    Science.gov (United States)

    Steinfeld, J. I.; Melzer, J. E.

    1977-01-01

    Multiple infrared photon absorption is a quite general process which molecules can undergo when placed in a high flux of infrared energy, such as the focussed beam of a CO2 laser. In order to understand how this process works, one must be able to follow the evolution of the molecules through their internal states, populated by photon absorption. Double-resonance spectroscopy is the method of a choice for getting at this information. A system pumped by CO2 laser radiation can be examined with a tunable laser probe beam, such as that from a lead-salt diode laser. From such an experiment, one can directly observe Rabi modulation of the absorption lines, determine elementary state-to-state relaxation pathways, and locate higher excited vibrational states. Systems currently under investigation include SF6 and vinyl chloride. In suitable cases, the probe beam can be a tunable visible or UV source, such as a dye laser. Fluorescence spectroscopy can then be used to monitor the transient absorptions produced by multiple-photon excitation. Among the systems which can be examined are biacetyl and glyoxal.

  16. Resonances in nonlinear structure vibrations under multifrequency excitations

    Energy Technology Data Exchange (ETDEWEB)

    El-Bassiouny, A F [Faculty of Science, Mathematics Department, Benha University, Benha 1358 (Egypt); El-Latif, G M Abd [Faculty of Science, Mathematics Department, Sohag University, Sohag (Egypt)

    2006-10-15

    The response of a single-degree-of-freedom system with quadratic, cubic and quartic nonlinearities subjected to a sinusoidal excitation that involves multiple frequencies is considered. The method of multiple scales is used to construct a first order uniform expansion yielding two first-order nonlinear ordinary differential equations that are derived for the evolution of the amplitude and phase. These oscillations involve a subharmonic oscillation of order one-fourth and superharmonic oscillation of order two. Steady state responses and their stability are computed for selected values of the system parameters. The effects of these (quadratic, cubic, and quartic) nonlinearities on these oscillations are specifically investigated. With this study, it has been verified that the qualitative effects of these nonlinearities are different. Regions of hardening (softening) behaviour of the system exist for the case of subharmonic resonance. The response curve is not affected by decreasing the damping factor for the case of superharmonic resonance. It is shown that the response curve contracts or expands as the parameters vary. The multivalued region increases or decreases when some parameters vary.

  17. A Study of Resonant Excitation of Longitudinal HOMs in the Cryomodules of LCLS-II

    Energy Technology Data Exchange (ETDEWEB)

    Bane, Karl

    2015-09-23

    The Linac Coherent Light Source (LCLS) at SLAC, the world’s first hard X-ray FEL, is being upgraded to the LCLS-II. The major new feature will be the installation of 35 cryomodules (CMs) of TESLA-type, superconducting accelerating structures, to allow for high rep-rate operation. It is envisioned that eventually the LCLS-II will be able to deliver 300 pC, 1 kA pulses of beam at a rate of 1 MHz. At a cavity temperature of 2 K, any heat generated (even on the level of a few watts) is expensive to remove. In the last linac of LCLS-II, L3—where the peak current is highest—the power radiated by the bunches in the CMs is estimated at 13.8 W (charge 300 pC option, rep rate 1 MHz). But this calculation ignores resonances that can be excited between the bunch frequency and higher order mode (HOM) frequencies in the CMs, which in principle can greatly increase this number. In the present work we calculate the multi-bunch wakefields excited in a CM of LCLS-II, in order to estimate the probability of the beam losing a given amount of power. Along theway, we find some interesting properties of the resonant interaction. In detail, we begin this report by finding the wakes experienced by bunches far back in the bunch train. Then we present a complementary approach that calculates the field amplitude excited in steady-state by a train of bunches, and show that the two approaches agree. Next we obtain the properties of the 450 longitudinal HOMs that cover the range 3–5 GHz in the CMs of LCLS-II, where we include the effects of the inter-CM ceramic dampers. At the end we apply our method using these modes.

  18. Resonant vibrational excitation of ethylene molecules in laser-assisted diamond deposition

    Science.gov (United States)

    Fan, L. S.; Zhou, Y. S.; Wang, M. X.; Gao, Y.; Liu, L.; Silvain, J. F.; Lu, Y. F.

    2014-07-01

    The influence of resonant vibrational excitation of ethylene molecules in combustion chemical vapor deposition of diamond was investigated. Resonant vibrational excitation of the CH2-wagging mode (a type c fundamental band, υ7, at 949.3 cm-1) in ethylene molecules was achieved by using a wavelength-tunable CO2 laser with a matching wavelength at 10.532 µm. By comparing to laser irradiation at off-resonance wavelengths, an on-resonance vibrational excitation is more efficient in energy coupling, increasing flame temperatures, accelerating the combustion reactions, and promoting diamond deposition. An enhanced rate of 5.7 was achieved in terms of the diamond growth rate with an improved diamond quality index at a high flame temperature under a resonant excitation of the CH2-wagging mode. This study demonstrates that a resonant vibrational excitation is an effective route for coupling energy into the gas phase reactions and promoting the diamond synthesis process.

  19. Coherent Excitation of Lithium to Rydberg States and Application to Rydberg Atom Optics

    Science.gov (United States)

    Stevens, G.; Widmer, M.; Tudorica, F.; Iu, C.-H.; Metcalf, H.

    1996-05-01

    We present a theoretical analysis of several schemes for coherently exciting lithium atoms in a thermal beam to Rydberg states in a four level/three laser system, previously discussed by Oreg et al.(J. Oreg et al.), Phys. Rev. A 45, 4888 (1992). The time evolution of the dressed states and their populations are calculated numerically, solving the optical Bloch equations by a fourth order Runge-Kutta integration. Our code closely models actual experimental conditions, including spontaneous decay, beam profiles, intensities and detunings. Large Rydberg populations (50%) around n=15 may be obtained by non-adiabatic excitation, with each laser power on the order of 1 mW. We discuss the effects of an externally controlled time dependent detuning in the Rydberg state, for example as produced by atoms traversing an inhomogeneous electric field. An understanding of this excitation mechanism is important for large angle reflection of coherently excited atoms using field gradients. Some primitive ideas of Stark-Rydberg atom optics are presented.

  20. Subharmonic resonant optical excitation of confined acoustic modes in a free-standing semiconductor membrane at GHz frequencies with a high-repetition-rate femtosecond laser.

    Science.gov (United States)

    Bruchhausen, A; Gebs, R; Hudert, F; Issenmann, D; Klatt, G; Bartels, A; Schecker, O; Waitz, R; Erbe, A; Scheer, E; Huntzinger, J-R; Mlayah, A; Dekorsy, T

    2011-02-18

    We propose subharmonic resonant optical excitation with femtosecond lasers as a new method for the characterization of phononic and nanomechanical systems in the gigahertz to terahertz frequency range. This method is applied for the investigation of confined acoustic modes in a free-standing semiconductor membrane. By tuning the repetition rate of a femtosecond laser through a subharmonic of a mechanical resonance we amplify the mechanical amplitude, directly measure the linewidth with megahertz resolution, infer the lifetime of the coherently excited vibrational states, accurately determine the system's quality factor, and determine the amplitude of the mechanical motion with femtometer resolution.

  1. Heat dissipation and information flow for delayed bistable Langevin systems near coherence resonance

    Science.gov (United States)

    Xiao, Tiejun

    2016-11-01

    In this paper, stochastic thermodynamics of delayed bistable Langevin systems near coherence resonance is discussed. We calculate the heat dissipation rate and the information flow of a delayed bistable Langevin system under various noise intensities. Both the heat dissipation rate and the information flow are found to be bell-shaped functions of the noise intensity, which implies that coherence resonance manifests itself in the thermodynamic properties.

  2. Fröhlich's coherent excitations & the cancer problem--a retrospective overview of his guiding philosophy.

    Science.gov (United States)

    Hyland, G J

    2009-01-01

    The guiding philosophy underlying Fröhlich's approach to biology from the side of theoretical physics is summarized, and illustrated, in the context of his prediction of (dynamic) coherent excitations in living systems, based on their dielectric and elastic properties, and far-from-equilibrium (nonlinear) character. His envisaged role of these coherent excitations in cell division and its control is outlined, together with the associated implications for cancer--as understood both at the time of his work and subsequently.

  3. Collective State of Interwell Excitons in GaAs/AlGaAs Double Quantum Wells under Pulse Resonance Excitation

    DEFF Research Database (Denmark)

    Larionov, A. V.; Timofeev, V. B.; Hvam, Jørn Märcher

    2002-01-01

    The time evolution and kinetics of photoluminescence (PL) spectra of interwell excitons in double GaAs/AlGaAs quantum wells (n–i–n structures) have been investigated under the pulse resonance excitation of intrawell 1sHH excitons using a pulsed tunable laser. It is found that the collective exciton......, and a significant increase in the radiative decay rate of the condensed phase. The collective exciton phase arises at temperatures T properties of the collective phase of interwell excitons and experimental manifestations of this coherence...

  4. Coherent Fano resonances in a plasmonic nanocluster enhance optical four-wave mixing

    Science.gov (United States)

    Zhang, Yu; Wen, Fangfang; Zhen, Yu-Rong; Nordlander, Peter; Halas, Naomi J.

    2013-01-01

    Plasmonic nanoclusters, an ordered assembly of coupled metallic nanoparticles, support unique spectral features known as Fano resonances due to the coupling between their subradiant and superradiant plasmon modes. Within the Fano resonance, absorption is significantly enhanced, giving rise to highly localized, intense near fields with the potential to enhance nonlinear optical processes. Here, we report a structure supporting the coherent oscillation of two distinct Fano resonances within an individual plasmonic nanocluster. We show how this coherence enhances the optical four-wave mixing process in comparison with other double-resonant plasmonic clusters that lack this property. A model that explains the observed four-wave mixing features is proposed, which is generally applicable to any third-order process in plasmonic nanostructures. With a larger effective susceptibility χ(3) relative to existing nonlinear optical materials, this coherent double-resonant nanocluster offers a strategy for designing high-performance third-order nonlinear optical media. PMID:23690571

  5. Coherence resonance in globally coupled neuronal networks with different neuron numbers

    Institute of Scientific and Technical Information of China (English)

    Ning Wei-Lian; Zhang Zheng-Zhen; Zeng Shang-You; Luo Xiao-Shu; Hu Jin-Lin; Zeng Shao-Wen; Qiu Yi; Wu Hui-Si

    2012-01-01

    Because a brain consists of tremendous neuronal networks with different neuron numbers ranging from tens to tens of thousands,we study the coherence resonance due to ion channel noises in globally coupled neuronal networks with different neuron numbers.We confirm that for all neuronal networks with different neuron numbers there exist the array enhanced coherence resonance and the optimal synaptic conductance to cause the maximal spiking coherence.Furthermoremore,the enhancement effects of coupling on spiking coherence and on optimal synaptic conductance are almost the same,regardless of the neuron numbers in the neuronal networks.Therefore for all the neuronal networks with different neuron numbers in the brain,relative weak synaptic conductance (0.1 mS/cm2) is sufficient to induce the maximal spiking coherence and the best sub-threshold signal encoding.

  6. Coherent Terahertz Radiation from Multiple Electron Beams Excitation within a Plasmonic Crystal-like structure

    Science.gov (United States)

    Zhang, Yaxin; Zhou, Yucong; Gang, Yin; Jiang, Guili; Yang, Ziqiang

    2017-01-01

    Coherent terahertz radiation from multiple electron beams excitation within a plasmonic crystal-like structure (a three-dimensional holes array) which is composed of multiple stacked layers with 3 × 3 subwavelength holes array has been proposed in this paper. It has been found that in the structure the electromagnetic fields in each hole can be coupled with one another to construct a composite mode with strong field intensity. Therefore, the multiple electron beams injection can excite and efficiently interact with such mode. Meanwhile, the coupling among the electron beams is taken place during the interaction so that a very strong coherent terahertz radiation with high electron conversion efficiency can be generated. Furthermore, due to the coupling, the starting current density of this mechanism is much lower than that of traditional electron beam-driven terahertz sources. This multi-beam radiation system may provide a favorable way to combine photonics structure with electronics excitation to generate middle, high power terahertz radiation.

  7. Nonlinear TeraHertz Coherent Excitation of Vibrational Modes of Liquids

    CERN Document Server

    Allodi, Marco A; Blake, Geoffrey A

    2015-01-01

    We report the first coherent excitation of intramolecular vibrational modes via the nonlinear interaction of a TeraHertz (THz) light field with molecular liquids. A TeraHertz-TeraHertz-Raman pulse sequence prepares the coherences with a broadband, high-energy, (sub)picosecond TeraHertz pulse, that are then measured in a TeraHertz Kerr effect spectrometer via phase-sensitive, heterodyne detection with an optical pulse. The spectrometer reported here has broader TeraHertz frequency coverage and an increased sensitivity relative to previously reported TeraHertz Kerr effect experiments. Vibrational coherences are observed in liquid diiodomethane at 3.66 THz (122 cm$^{-1}$), and in carbon tetrachloride at 6.50 THz (217 cm$^{-1}$), in exact agreement with literature values of those intramolecular modes. This work opens the door to 2D spectroscopies, nonlinear in TeraHertz field, that can study the dynamics of condensed-phase molecular systems, as well as coherent control at TeraHertz frequencies.

  8. Ultrafast Optical Excitation of Coherent and Squeezed Phonons in SrTiO_3

    Science.gov (United States)

    Garrett, G. A.; Whitaker, J. F.; Merlin, R.

    1998-03-01

    We report on the impulsive excitation of coherent and squeezed phonon fields in SrTiO3 using, respectively, first-order and second-order stimulated Raman scattering.(osa.org/oearchive/source/2733.htm>Garrett et al)., Optics Express, to be published. Strontium titanate undergoes an antiferro-distortive phase transition at T_c≈ 110 K to a low temperature tetragonal structure. First-order Raman scattering is allowed only below T_c. Pump-probe spectra were obtained as a function of temperature and pump intensity. The frequency of the coherent (first-order) state is that of the A_1g-component of the soft mode associated with the phase transition. As in KTaO_3,(Garrett et al)., Science 275, 1638 (1997). the squeezed (second-order) field oscillates at a frequency corresponding to a strong, narrow peak in the density of states of the acoustic phonons.

  9. Ultra-wide-band accumulation of coherent undulator synchrotron radiation in a resonating cavity

    Directory of Open Access Journals (Sweden)

    Y. H. Seo

    2011-06-01

    Full Text Available Cavity accumulation of coherent undulator synchrotron radiation emitted by a train of periodic electron bunches is investigated. Phase-matching conditions for accumulation of radiation emitted by successive bunches are analyzed and numerically confirmed. While the coherent emission of a single bunch is optimal at grazing resonance, the accumulated radiation targeted at the upper resonant frequency of the waveguide mode is found to have much broader bandwidth and higher efficiency as the resonance steps away from the grazing condition. Numerical results confirm that stimulated superradiance is responsible for the accumulated radiation.

  10. Coherent triplet excitation suppresses the heading error of the avian compass

    Energy Technology Data Exchange (ETDEWEB)

    Katsoprinakis, G E; Dellis, A T; Kominis, I K, E-mail: ikominis@iesl.forth.g [Department of Physics, University of Crete, Heraklion 71103 (Greece); Institute of Electronic Structure and Laser, Foundation for Research and Technology, Heraklion 71110 (Greece)

    2010-08-15

    Radical-ion pair reactions are currently understood to underlie the biochemical magnetic compass of migratory birds. It was recently shown that radical-ion pair reactions form a rich playground for the application of quantum-information-science concepts and effects. We will show here that the intricate interplay between the quantum Zeno effect and the coherent excitation of radical-ion pairs leads to an exquisite angular sensitivity of the reaction yields. This results in a significant and previously unanticipated suppression of the avian compass heading error, opening the way to quantum engineering precision biological sensors.

  11. Investigation on driving characteristics of a piezoelectric stick–slip actuator based on resonant/off-resonant hybrid excitation

    Science.gov (United States)

    Cheng, Tinghai; Li, Hengyu; He, Meng; Zhao, Hongwei; Lu, Xiaohui; Gao, Haibo

    2017-03-01

    A resonant/off-resonant hybrid excitation of a piezoelectric stick–slip actuator is proposed in this paper. It is accomplished by a resonant sinusoidal friction regulation wave (RSFR-wave) and an off-resonant saw-tooth wave (ORST-wave). The RSFR-wave is applied to the rapid deformation stage of the ORST-wave. In this stage, the first-order longitudinal vibration mode of the stator can be obtained. By this longitudinal vibration mode, the kinetic friction between the slider and frictional rod is obviously decreased utilizing ultrasonic friction reduction. The backward displacement is remarkably restrained. The high velocity, large mass of load and smooth displacement are achieved. The operation principle of hybrid excitation was discussed in detail, and a prototype was simulated, designed, and fabricated. A series of experiments were carried out and the results indicate that the step efficiency under the saw-tooth excitation and resonant/off-resonant hybrid excitation can realize 36.9% and 91.2%, respectively. The output velocity is increased by 147.23% relative to saw-tooth excitation. The minimum input power and the minimum driving voltage are decreased by 89.56% and 58.33%, respectively. Besides, the maximum mass of load capacity is 2.88 times that of saw-tooth excitation. The driving capacity of the actuator is increased by 466.13%.

  12. Fast electronic relaxation in metal nanoclusters via excitation of coherent shape deformations: Circumventing a bottleneck

    CERN Document Server

    Kresin, V V; Kresin, Vitaly V.; Ovchinnikov, Yu. N.

    2006-01-01

    Electron-phonon relaxation in size-quantized systems may become inhibited when the spacing of discrete electron energy levels exceeds the magnitude of the phonon frequency. We show, however, that nanoclusters can support a fast nonradiative relaxation channel which derives from their distinctive ability to undergo Jahn-Teller shape deformations. Such a deformation represents a collective and coherent vibrational excitation and enables electronic transitions to occur without a multiphonon bottleneck. We analyze this mechanism for a metal cluster within the analytical framework of a three-dimensional potential well undergoing a spheroidal distortion. An expression for the time evolution of the distortion parameter is derived, the electronic level crossing condition formulated, and the probability of electronic transition at a level crossing is evaluated. An application to electron-hole recombination in a closed-shell aluminum cluster with 40 electrons shows that the short (~250 fs) excitation lifetime observed ...

  13. Off-resonant vibrational excitation: Orientational dependence and spatial control of photofragments

    DEFF Research Database (Denmark)

    Machholm, Mette; Henriksen, Niels Engholm

    2000-01-01

    -dependent response to the IR fields is due to the anharmonicity of the potential. A subsequent ultraviolet laser pulse in resonance at the outer turning point of the vibrational motion can then dissociate the oscillating molecules, all with the same orientation, leading to spatial control of the photofragment......Off-resonant and resonant vibrational excitation with short intense infrared (IR) laser pulses creates localized oscillating wave packets, but differs by the efficiency of the excitation and surprisingly by the orientational dependence. Orientational selectivity of the vibrational excitation...... of randomly oriented heteronuclear diatomic molecules can be obtained under simultaneous irradiation by a resonant and an off-resonant intense IR laser pulse: Molecules with one initial orientation will be vibrationally excited, while those with the opposite orientation will be at rest. The orientation...

  14. Synchronization and coherence resonance in chaotic neural networks

    Institute of Scientific and Technical Information of China (English)

    Wang Mao-Sheng; Hou Zhong-Huai; Xin Hou-Wen

    2006-01-01

    Synchronization and coherence of chaotic Morris-Lecar (ML) neural networks have been investigated by numerical methods. The synchronization of the neurons can be enhanced by increasing the number of the shortcuts, even though all neurons are chaotic when uncoupled. Moreover, the coherence of the neurons exhibits a non-monotonic dependence on the density of shortcuts. There is an optimal number of shortcuts at which the neurons' motion is most ordered, i.e. the order parameter (the characteristic correlation time) that is introduced to measure the coherence of the neurons has a maximum. These phenomena imply that stochastic shortcuts can tame spatiotemporal chaos. The effects of the coupling strength have also been studied. The value of the optimal number of shortcuts goes down as the coupling strength increases.

  15. Quadrupole lattice resonances in plasmonic crystal excited by cylindrical vector beams

    Science.gov (United States)

    Sakai, Kyosuke; Nomura, Kensuke; Yamamoto, Takeaki; Omura, Tatsuya; Sasaki, Keiji

    2016-10-01

    We report a scheme to exploit low radiative loss plasmonic resonance by combining a dark (subradiant) mode and a lattice resonance. We theoretically demonstrate that such dark-mode lattice resonances in periodic arrays of nanodisks or plasmonic crystals can be excited by vertically incident light beams. We investigate the excitation of lattice resonances in a finite sized, square-lattice plasmonic crystal by two types of cylindrical vector beams and a linearly polarized Gaussian beam. Quadrupole lattice resonances are excited by all three beams, and the largest peak intensity is obtained by using a specific type of cylindrical vector beam. Because of their lower radiative losses with many hotspots, the quadrupole lattice resonances in plasmonic crystal may pave the way for photonic research and applications that require strong light-matter interactions.

  16. Time-optimal excitation of maximum quantum coherence: Physical limits and pulse sequences

    Science.gov (United States)

    Köcher, S. S.; Heydenreich, T.; Zhang, Y.; Reddy, G. N. M.; Caldarelli, S.; Yuan, H.; Glaser, S. J.

    2016-04-01

    Here we study the optimum efficiency of the excitation of maximum quantum (MaxQ) coherence using analytical and numerical methods based on optimal control theory. The theoretical limit of the achievable MaxQ amplitude and the minimum time to achieve this limit are explored for a set of model systems consisting of up to five coupled spins. In addition to arbitrary pulse shapes, two simple pulse sequence families of practical interest are considered in the optimizations. Compared to conventional approaches, substantial gains were found both in terms of the achieved MaxQ amplitude and in pulse sequence durations. For a model system, theoretically predicted gains of a factor of three compared to the conventional pulse sequence were experimentally demonstrated. Motivated by the numerical results, also two novel analytical transfer schemes were found: Compared to conventional approaches based on non-selective pulses and delays, double-quantum coherence in two-spin systems can be created twice as fast using isotropic mixing and hard spin-selective pulses. Also it is proved that in a chain of three weakly coupled spins with the same coupling constants, triple-quantum coherence can be created in a time-optimal fashion using so-called geodesic pulses.

  17. Coherent photoproduction of eta mesons on the deuteron in the range of the $S_{1}_{1}(1535)$ resonance

    CERN Document Server

    Ritz, F

    2000-01-01

    In the present thesis the meaning of two-particle effects for the coherent photoproduction of eta mesons on the deuteron in the range of the S sub 1 sub 1 (1535) resonance was studied. For this on the hadronic side a coupled-channel calculation for the nucleon-nucleon and nucleon-resonance interaction regarding the P sub 1 sub 1 (1440), D sub 1 sub 3 (1520), and S sub 1 sub 1 (1535) resonances was performed, which is based on the Bonn OBEPQ potential. On the electromagnetic side beside the one-particle currents the isoscalar pi- and eta-meson exchange currents belonging to the OBEPQ potential. The analyses yield for the proton excitation strength vertical stroke A sub p vertical stroke the value 138 x 10 sup - sup 3 GeV sup - sup 1 sup / sup 2 and vertical stroke A sub s /A sub p vertical stroke approx 0.25 at the resonance point. For the ratio of the total resonant cross sections of neutron and proton results sigma sub n /sigma sub p approx 0. 68.

  18. Polaronic quasiparticle picture for generation dynamics of coherent phonons in semiconductors: Transient and nonlinear Fano resonance

    Science.gov (United States)

    Watanabe, Yohei; Hino, Ken-ichi; Hase, Muneaki; Maeshima, Nobuya

    2017-01-01

    We examine generation dynamics of coherent phonons in both polar and nonpolar semiconductors, such as GaAs and Si, based on a polaronic-quasiparticle (PQ) model. In this model, the PQ operator is composed of two kinds of operators: one is a quasiboson operator, defined as a linear combination of a set of pairs of electron operators, and the other is a longitudinal optical (LO) phonon operator. In particular, the problem of transient and nonlinear Fano resonance (FR) is tackled, where the vestige of this quantum interference effect was observed exclusively in lightly n -doped Si immediately after carriers were excited by an ultrashort pulse laser [M. Hase et al., Nature (London) 426, 51 (2003), 10.1038/nature02044], although not observed yet in GaAs. The PQ model enables us to show straightforwardly that the phonon energy state is embedded in continuum states formed by a set of adiabatic eigenstates of the quasiboson; this energy configuration is a necessary condition of the manifestation of the transient FR in the present optically nonlinear system. Numerical calculations are done for photoemission spectra relevant to the retarded longitudinal dielectric function of transient photoexcited states and for power spectra relevant to the LO-phonon displacement function of time. The photoemission spectra show that in undoped Si, an asymmetric spectral profile characteristic of FR comes into existence immediately after the instantaneous carrier excitation to fade out gradually, whereas in undoped GaAs, no asymmetry in spectra appears in the whole temporal region. The similar results are also obtained in the power spectra. These results are in harmony with the reported experimental results. It is found that the obtained difference in spectral profile between undoped Si and GaAs is attributed to a phase factor of an effective interaction between the LO phonon and the quasiboson. More detailed discussion of the FR dynamics is made in the text.

  19. [Research Progress on Laser-Induced Breakdown Spectroscopy Based on Resonance Excitation].

    Science.gov (United States)

    Wang, Xu-zhao; Hao, Zhong-qi; Guo, Lian-bo; Li, Xiang-you; Lu, Yong-feng; Zeng, Xiao-yan

    2015-05-01

    Laser-induced breakdown spectroscopy (LIBS), a new kind of atomic spectrum analysis technology, has attracted much atterition of the researchers due to its characteristics of real-time, simultaneous multi-element analysis, and no sample preparation. However, the poor analytical sensitivity has been an important factor that restricts the development of this technology. LIBS based on resonance excitation combines atomic fluorescence spectroscopy and laser-induced breakdown spectroscopy and selectively excites the target elements. In this way, the analytical sensitivity of LIBS can be improved substantially and its application for trace elements detection is greatly expanded. In this paper, the research development of LIBS based on resonance excitation is summarized. The generation of atomic, fluorescence spectrum in laser-induced plasma, the typical classification and the basic principle of LIBS based on resonance. excitation are introduced. The influence of ablation laser energy, resonant laser energy and wavelength, delay between the ablation laser and the resonant laser, and the gate width on spectral enhancement are analyzed in detail. The application status and deficiencies of LIBS based on resonance excitation in the fields of metallurgy, environmental monitoring and isotope detection are elaborated. Future prospects of LIBS based on resonance excitation are also described.

  20. Nanoscale femtosecond imaging of transient hot solid density plasmas with elemental and charge state sensitivity using resonant coherent diffraction

    Science.gov (United States)

    Kluge, T.; Bussmann, M.; Chung, H.-K.; Gutt, C.; Huang, L. G.; Zacharias, M.; Schramm, U.; Cowan, T. E.

    2016-03-01

    Here, we propose to exploit the low energy bandwidth, small wavelength, and penetration power of ultrashort pulses from XFELs for resonant Small Angle Scattering (SAXS) on plasma structures in laser excited plasmas. Small angle scattering allows to detect nanoscale density fluctuations in forward scattering direction. Typically, the SAXS signal from laser excited plasmas is expected to be dominated by the free electron distribution. We propose that the ionic scattering signal becomes visible when the X-ray energy is in resonance with an electron transition between two bound states (resonant coherent X-ray diffraction). In this case, the scattering cross-section dramatically increases so that the signal of X-ray scattering from ions silhouettes against the free electron scattering background which allows to measure the opacity and derived quantities with high spatial and temporal resolution, being fundamentally limited only by the X-ray wavelength and timing. Deriving quantities such as ion spatial distribution, charge state distribution, and plasma temperature with such high spatial and temporal resolution will make a vast number of processes in shortpulse laser-solid interaction accessible for direct experimental observation, e.g., hole-boring and shock propagation, filamentation and instability dynamics, electron transport, heating, and ultrafast ionization dynamics.

  1. Observation of Time-Invariant Coherence in a Nuclear Magnetic Resonance Quantum Simulator.

    Science.gov (United States)

    Silva, Isabela A; Souza, Alexandre M; Bromley, Thomas R; Cianciaruso, Marco; Marx, Raimund; Sarthour, Roberto S; Oliveira, Ivan S; Lo Franco, Rosario; Glaser, Steffen J; deAzevedo, Eduardo R; Soares-Pinto, Diogo O; Adesso, Gerardo

    2016-10-14

    The ability to live in coherent superpositions is a signature trait of quantum systems and constitutes an irreplaceable resource for quantum-enhanced technologies. However, decoherence effects usually destroy quantum superpositions. It was recently predicted that, in a composite quantum system exposed to dephasing noise, quantum coherence in a transversal reference basis can stay protected for an indefinite time. This can occur for a class of quantum states independently of the measure used to quantify coherence, and it requires no control on the system during the dynamics. Here, such an invariant coherence phenomenon is observed experimentally in two different setups based on nuclear magnetic resonance at room temperature, realizing an effective quantum simulator of two- and four-qubit spin systems. Our study further reveals a novel interplay between coherence and various forms of correlations, and it highlights the natural resilience of quantum effects in complex systems.

  2. Coherence Resonance and Noise-Induced Synchronization in Hindmarsh-Rose Neural Network with Different Topologies

    Institute of Scientific and Technical Information of China (English)

    2007-01-01

    In this paper, we investigate coherence resonance (CR) and noise-induced synchronization in Hindmarsh-Rose (HR) neural network with three different types of topologies: regular, random, and small-world. It is found that the additive noise can induce CR in HR neural network with different topologies and its coherence is optimized by a proper noise level. It is also found that as coupling strength increases the plateau in the measure of coherence curve becomes broadened and the effects of network topology is more pronounced simultaneously. Moreover, we find that increasing tie probability p of the network topology leads to an enhancement of noise-induced synchronization in HR neurons network.

  3. Autapse-induced multiple coherence resonance in single neurons and neuronal networks

    Science.gov (United States)

    Yilmaz, Ergin; Ozer, Mahmut; Baysal, Veli; Perc, Matjaž

    2016-08-01

    We study the effects of electrical and chemical autapse on the temporal coherence or firing regularity of single stochastic Hodgkin-Huxley neurons and scale-free neuronal networks. Also, we study the effects of chemical autapse on the occurrence of spatial synchronization in scale-free neuronal networks. Irrespective of the type of autapse, we observe autaptic time delay induced multiple coherence resonance for appropriately tuned autaptic conductance levels in single neurons. More precisely, we show that in the presence of an electrical autapse, there is an optimal intensity of channel noise inducing the multiple coherence resonance, whereas in the presence of chemical autapse the occurrence of multiple coherence resonance is less sensitive to the channel noise intensity. At the network level, we find autaptic time delay induced multiple coherence resonance and synchronization transitions, occurring at approximately the same delay lengths. We show that these two phenomena can arise only at a specific range of the coupling strength, and that they can be observed independently of the average degree of the network.

  4. Autapse-induced multiple coherence resonance in single neurons and neuronal networks.

    Science.gov (United States)

    Yilmaz, Ergin; Ozer, Mahmut; Baysal, Veli; Perc, Matjaž

    2016-08-02

    We study the effects of electrical and chemical autapse on the temporal coherence or firing regularity of single stochastic Hodgkin-Huxley neurons and scale-free neuronal networks. Also, we study the effects of chemical autapse on the occurrence of spatial synchronization in scale-free neuronal networks. Irrespective of the type of autapse, we observe autaptic time delay induced multiple coherence resonance for appropriately tuned autaptic conductance levels in single neurons. More precisely, we show that in the presence of an electrical autapse, there is an optimal intensity of channel noise inducing the multiple coherence resonance, whereas in the presence of chemical autapse the occurrence of multiple coherence resonance is less sensitive to the channel noise intensity. At the network level, we find autaptic time delay induced multiple coherence resonance and synchronization transitions, occurring at approximately the same delay lengths. We show that these two phenomena can arise only at a specific range of the coupling strength, and that they can be observed independently of the average degree of the network.

  5. Influence of the atomic-wall collision elasticity on the coherent population trapping resonance shape

    CERN Document Server

    Kazakov, G A; Matisov, B G; Romanenko, V I; Yatsenko, L P; Romanenko, A V

    2011-01-01

    We studied theoretically a coherent population trapping resonance formation in cylindrical cell without buffer gas irradiated by a narrow laser beam. We take into account non-zero probabilities of elastic ("specular") and inelastic ("sticking") collision between the atom and the cell wall. We have developed a theoretical model based on averaging over the random Ramsey pulse sequences of times that atom spent in and out of the beam. It is shown that the shape of coherent population trapping resonance line depends on the probability of elastic collision.

  6. Light-induced spatial gratings created by unipolar attosecond pulses coherently interacting with a resonant medium

    Science.gov (United States)

    Arkhipov, R. M.; Arkhipov, M. V.; Pakhomov, A. V.; Babushkin, I.; Rosanov, N. N.

    2017-09-01

    Recently, the possibility of the creation, erasing and ultrafast control of polarization and population inversion gratings by sequences of few-cycle bipolar pulses interacting with a medium in a resonant and coherent way was predicted. In this case, the overlapping of pulses in the medium is not needed for the creation of gratings. In this paper, we study the possibility of the ultrafast creation and control of spatial periodic gratings in a resonant medium when subcycle unipolar pulses (that is ones containing the constant spectral component of an electric field) propagate in the coherent regime.

  7. Coherent resonance of quantum plasmons in the graphene-gold cluster hybrid system.

    Science.gov (United States)

    Zhang, Kaibiao; Zhang, Hong; Li, Chikang

    2015-05-14

    Noble metal nanoparticles can modify the optical properties of graphene. Here we present a detailed theoretical analysis of the coherent resonance of quantum plasmons in the graphene-gold cluster hybrid system by using time dependent density functional theory (TDDFT). This plasmon coherent effect is mainly attributed to the electromagnetic field coupling between the graphene and the gold cluster. As a result, the optical response of the hybrid system exhibits a remarkably strong, selectable tuning and polarization dependent plasmon resonance enhanced in wide frequency regions. This investigation provides an improved understanding of the plasmon enhancement effect in a graphene-based photoelectric device.

  8. Ultra-short, off-resonant, strong excitation of two-level systems

    CERN Document Server

    Jha, Pankaj K; Grazioso, Fabio

    2013-01-01

    We present a model describing the use of ultra-short strong pulses to populate the excited level of a two-level quantum system. In particular, we study an off-resonance excitation with a few cycles pulse which presents a smooth phase jump i.e. a change of the pulse's phase which is not step-like, but happens over a finite time interval. A numerical solution is given for the time-dependent probability amplitude of the excited level. The enhancement of the excited level's population is optimized with respect to the shape of the phase transient, and to other parameters of the excitation pulse.

  9. Fluorescent resonant excitation energy transfer in linear polyenes.

    Science.gov (United States)

    Das, Mousumi; Ramasesha, S

    2010-03-28

    We have studied the dynamics of excitation transfer between two conjugated polyene molecules whose intermolecular separation is comparable to the molecular dimensions. We have employed a correlated electron model that includes both the charge-charge, charge-bond, and bond-bond intermolecular electron repulsion integrals. We have shown that the excitation transfer rate varies as inverse square of donor-acceptor separation R(-2) rather than as R(-6), suggested by the Forster type of dipolar approximation. Our time-evolution study also shows that the orientational dependence on excitation transfer at a fixed short donor-acceptor separation cannot be explained by Forster type of dipolar approximation beyond a certain orientational angle of rotation of an acceptor polyene with respect to the donor polyene. The actual excitation transfer rate beyond a certain orientational angle is faster than the Forster type of dipolar approximation rate. We have also studied the excitation transfer process in a pair of push-pull polyenes for different push-pull strengths. We have seen that, depending on the push-pull strength, excitation transfer could occur to other dipole coupled states. Our study also allows for the excitation energy transfer to optically dark states which are excluded by Forster theory since the one-photon transition intensity to these states (from the ground state) is zero.

  10. Fluorescent resonant excitation energy transfer in linear polyenes

    Science.gov (United States)

    Das, Mousumi; Ramasesha, S.

    2010-03-01

    We have studied the dynamics of excitation transfer between two conjugated polyene molecules whose intermolecular separation is comparable to the molecular dimensions. We have employed a correlated electron model that includes both the charge-charge, charge-bond, and bond-bond intermolecular electron repulsion integrals. We have shown that the excitation transfer rate varies as inverse square of donor-acceptor separation R-2 rather than as R-6, suggested by the Förster type of dipolar approximation. Our time-evolution study also shows that the orientational dependence on excitation transfer at a fixed short donor-acceptor separation cannot be explained by Förster type of dipolar approximation beyond a certain orientational angle of rotation of an acceptor polyene with respect to the donor polyene. The actual excitation transfer rate beyond a certain orientational angle is faster than the Förster type of dipolar approximation rate. We have also studied the excitation transfer process in a pair of push-pull polyenes for different push-pull strengths. We have seen that, depending on the push-pull strength, excitation transfer could occur to other dipole coupled states. Our study also allows for the excitation energy transfer to optically dark states which are excluded by Förster theory since the one-photon transition intensity to these states (from the ground state) is zero.

  11. Periodic coupling strength-dependent multiple coherence resonance by time delay in Newman-Watts neuronal networks.

    Science.gov (United States)

    Wu, Yanan; Gong, Yubing; Xu, Bo

    2013-12-01

    Recently, multiple coherence resonance induced by time delay has been observed in neuronal networks with constant coupling strength. In this paper, by employing Newman-Watts Hodgkin-Huxley neuron networks with time-periodic coupling strength, we study how the temporal coherence of spiking behavior and coherence resonance by time delay change when the frequency of periodic coupling strength is varied. It is found that delay induced coherence resonance is dependent on periodic coupling strength and increases when the frequency of periodic coupling strength increases. Periodic coupling strength can also induce multiple coherence resonance, and the coherence resonance occurs when the frequency of periodic coupling strength is approximately multiple of the spiking frequency. These results show that for periodic coupling strength time delay can more frequently optimize the temporal coherence of spiking activity, and periodic coupling strength can repetitively optimize the temporal coherence of spiking activity as well. Frequency locking may be the mechanism for multiple coherence resonance induced by periodic coupling strength. These findings imply that periodic coupling strength is more efficient for enhancing the temporal coherence of spiking activity of neuronal networks, and thus it could play a more important role in improving the time precision of information processing and transmission in neural networks.

  12. Ultra-coherent nanomechanical resonators via soft clamping and dissipation dilution

    CERN Document Server

    Tsaturyan, Yeghishe; Polzik, Eugene S; Schliesser, Albert

    2016-01-01

    The small mass and high coherence of nanomechanical resonators render them the ultimate force probe, with applications ranging from biosensing and magnetic resonance force microscopy, to quantum optomechanics. A notorious challenge in these experiments is thermomechanical noise related to dissipation through internal or external loss channels. Here, we introduce a novel approach to defining nanomechanical modes, which simultaneously provides strong spatial confinement, full isolation from the substrate, and dilution of the resonator material's intrinsic dissipation by five orders of magnitude. It is based on a phononic bandgap structure that localises the mode, without imposing the boundary conditions of a rigid clamp. The reduced curvature in the highly tensioned silicon nitride resonator enables mechanical $Q>10^{8}$ at $ 1 \\,\\mathrm{MHz}$, yielding the highest mechanical $Qf$-products ($>10^{14}\\,\\mathrm{Hz}$) yet reported at room temperature. The corresponding coherence times approach those of optically t...

  13. Vibronically coherent speed-up of the excitation energy transfer in the Fenna-Matthews-Olson complex

    Science.gov (United States)

    Nalbach, P.; Mujica-Martinez, C. A.; Thorwart, M.

    2015-02-01

    We show that underdamped molecular vibrations fuel the efficient excitation energy transfer in the Fenna-Matthews-Olson molecular aggregate under realistic physiological conditions. By employing an environmental fluctuation spectral function derived from experiments, we obtain numerically exact results for the exciton quantum dynamics in the presence of underdamped vibrationally coherent quantum states. Assuming the prominent 180 -cm-1 vibrational mode to be underdamped, additional coherent transport channels for the excitation energy transfer open up and we observe an increase of the transfer speed towards the reaction center by up to 24 % .

  14. Interface between light coupled to excited-states transition and ground-state coherence of rubidium atoms

    CERN Document Server

    Parniak, Michał; Wasilewski, Wojciech

    2015-01-01

    We demonstrate an interface between light coupled to transition between excited states of rubidium and long-lived ground-state atomic coherence. In our proof-of-principle experiment a non-linear process of four-wave mixing in an open-loop configuration is used to achieve light emission proportional to independently prepared ground-state atomic coherence. We demonstrate strong correlations between Raman light heralding generation of ground-state coherence and the new four-wave mixing signal. Dependance of the efficiency of the process on laser detunings is studied.

  15. Experimental demonstration of coherent perfect absorption in a silicon photonic racetrack resonator.

    Science.gov (United States)

    Rothenberg, Jacob M; Chen, Christine P; Ackert, Jason J; Dadap, Jerry I; Knights, Andrew P; Bergman, Keren; Osgood, Richard M; Grote, Richard R

    2016-06-01

    We present the first experimental demonstration of coherent perfect absorption (CPA) in an integrated device using a silicon racetrack resonator at telecommunication wavelengths. Absorption in the racetrack is achieved by Si+-ion-implantation, allowing for phase controllable amplitude modulation at the resonant wavelength. The device is measured to have an extinction of 24.5 dB and a quality-factor exceeding 3000. Our results will enable integrated CPA devices for data modulation and detection.

  16. Theory of deep ultraviolet generation at maximum coherence assisted by Stark-chirped two-photon resonance

    CERN Document Server

    Myslivets, S A; Kimberg, V V; George, T F; George, Thomas F.

    2003-01-01

    A scheme is analyzed for effcient generation of vacuum ultraviolet radiation through four-wave mixing processes assisted by the technique of Stark-chirped rapid adiabatic passage. These opportunities are associated with pulse excitation of laddertype short-wavelength two-photon atomic or molecular transitions so that relaxation processes can be neglected. In this three-laser technique, a delayed-pulse of strong oR-resonant infrared radiation sweeps the laser-induced Stark-shift of a two-photon transition in a such way that facilitates robust maximum two-photon coherence induced by the first ultraviolet laser. A judiciously delayed third pulse scatters at this coherence and generates short-wavelength radiation. A theoretical analysis of these problems based on the density matrix is performed. A numerical model is developed to carry out simulations of a typical experiment. The results illustrate a behavior of populations, coherence and generated radiation along the medium as well as opportunities of effcient ge...

  17. Resonance Analysis of High-Frequency Electrohydraulic Exciter Controlled by 2D Valve

    Directory of Open Access Journals (Sweden)

    Guojun Pan

    2015-01-01

    Full Text Available The resonant characteristic of hydraulic system has not been described yet because it is necessarily restricted by linear assumptions in classical fluid theory. A way of the resonance analysis is presented for an electrohydraulic exciter controlled by 2D valve. The block diagram of this excitation system is established by extracting nonlinear parts from the traditional linearization analysis; as a result the resonant frequency is obtained. According to input energy from oil source which is equal to the reverse energy to oil source, load pressure and load flow are solved analytically as the working frequency reaches the natural frequency. The analytical expression of resonant peak is also derived without damping. Finally, the experimental system is built to verify the theoretical analysis. The initial research on resonant characteristic will lay theoretical foundation and make useful complement for resonance phenomena of classical fluid theory in hydraulic system.

  18. Effects of inhomogeneous broadening on the resonance Raman excitation profile of lycopene

    Science.gov (United States)

    Cotting, J. E.; Hoskins, L. C.; Levan, M. E.

    1982-08-01

    The resonance Raman excitation profiles for the ν1, ν2, and ν3 vibrations of lycopene in ethyl alcohol, toluene, and carbon disulfide solvents have been measured. The results are interpreted in terms of a three-mode vibrational theory which includes both homogeneous and inhomogeneous broadening effects. Excellent agreement between calculated and observed excitation profiles and visible spectra was found, thus emphasizing the need to interpret resonance Raman data using a multimode vibrational model. The results indicate that the major broadening mechanism is homogeneous broadening, with about a 25% contribution from inhomogeneous broadening. The excitation profiles in carbon disulfide gave the largest inhomogeneous broadening.

  19. Angular dependent study on ferromagnetic resonance and spin excitations by spin rectification

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, Yichao; Fan, Xiaolong, E-mail: fanxiaolong@lzu.edu.cn; Zhao, Xiaobing; Rao, Jinwei; Zhou, Hengan; Guo, Dangwei; Xue, Desheng [The Key Lab for Magnetism and Magnetic Materials of Ministry of Education, Lanzhou University, Lanzhou 730000 (China); Gui, Y. S.; Hu, C.-M. [Department of Physics and Astronomy, University of Manitoba, Winnipeg, Manitoba R3T 2N2 (Canada)

    2015-01-14

    We report angular dependent spin rectification spectra which are applied to studying spin excitations in single permalloy stripe. Based on planar Hall effect, those spin excitations generate special resonant dc Hall voltages, which have been characterized as functions of the amplitude and direction of applied magnetic field. Through high angular resolution 2D mappings, the evolutions of different spin excitation can be directly presented, and the dynamic magnetic parameters such as the gyromagnetic ratio, effective exchange field, as well as the quantized numbers of standing spin waves can be accurately determined through fitting the angular evolution of each resonance.

  20. Suppression of electron spin-echo envelope modulation peaks in double quantum coherence electron spin resonance.

    Science.gov (United States)

    Bonora, Marco; Becker, James; Saxena, Sunil

    2004-10-01

    We show the use of the observer blind spots effect for the elimination of electron spin-echo envelope modulation (ESEEM) peaks in double quantum coherence (DQC) electron spin resonance (ESR). The suppression of ESEEM facilitates the routine and unambiguous extraction of distances from DQC-ESR spectra. This is also the first demonstration of this challenging methodology on commercial instrumentation.

  1. Coherence and anticoherence resonance in high-concentration erbium-doped fiber laser

    OpenAIRE

    Sergeyev, Sergey; O'Mahoney, Kieran; Popov, Sergei; Friberg, Ari T.

    2010-01-01

    We report an experimental study of low-frequency (~10 kHz) self-pulsing of the output intensity in a high- concentration erbium-doped fiber laser. We suggest that the fast intensity fluctuations caused by multimode and polarization instabilities play the role of an external noise source, leading to low-frequency auto-oscillations through a coherence resonance scenario.

  2. Resonant Enhancement of Coherent Phonons in Carbon Nanotubes Observed with Sub-10fs Time Resolution

    Directory of Open Access Journals (Sweden)

    Yanagi K.

    2013-03-01

    Full Text Available Using wavelength-resolved pump-probe spectroscopy with a sub-10-fs laser, we investigated resonant enhancement of radial breathing mode and G-mode coherent phonons in carbon nanotubes (CNTs, and successfully distinguished the electronic states of CNTs with different chiralities.

  3. Theoretical resonant electron-impact vibrational excitation, dissociative recombination and dissociative excitation cross sections of ro-vibrationally excited BeH+ ion

    Science.gov (United States)

    Laporta, V.; Chakrabarti, K.; Celiberto, R.; Janev, R. K.; Mezei, J. Zs; Niyonzima, S.; Tennyson, J.; Schneider, I. F.

    2017-02-01

    A theoretical study of resonant vibrational excitation, dissociative recombination and dissociative excitation processes of the beryllium monohydride cation, BeH+, induced by electron impact, is reported. Full sets of ro-vibrationally-resolved cross sections and of the corresponding Maxwellian rate coefficients are presented for the three processes. Particular emphasis is given to the high-energy behaviour. Potential curves of {}2{{{Σ }}}+, {}2{{\\Pi }} and {}2{{Δ }} symmetries and the corresponding resonance widths, obtained from R-matrix calculations, provide the input for calculations which use a local complex-potential model for resonant collisions in each of the three symmetries. Rotational motion of nuclei and isotopic effects are also discussed. The relevant results are compared with those obtained using a multichannel quantum defect theory method. Full results are available from the Phys4Entry database.

  4. Quantum Entanglement and Shannon Information Entropy for the Doubly Excited Resonance State in Positronium Negative Ion

    Directory of Open Access Journals (Sweden)

    Chien-Hao Lin

    2015-09-01

    Full Text Available In the present work, we report an investigation on quantum entanglement in the doubly excited 2s2 1Se resonance state of the positronium negative ion by using highly correlated Hylleraas type wave functions, determined by calculation of the density of resonance states with the stabilization method. Once the resonance wave function is obtained, the spatial (electron-electron orbital entanglement entropies (von Neumann and linear can be quantified using the Schmidt decomposition method. Furthermore, Shannon entropy in position space, a measure for localization (or delocalization for such a doubly excited state, is also calculated.

  5. Effect resonance radiation transfer of excitation porous silicon to I sub 2 molecules sorbed in pores

    CERN Document Server

    Zakharchenko, K V; Kuznetsov, M B; Chistyakov, A A; Karavanskij, V A

    2001-01-01

    One studies the effect of resonance radiation-free transfer of electronic excitation between silicon nanocrystals and iodine molecules sorbed in pores. The experiment procedure includes laser-induced luminescence and laser desorption mass spectrometry. One analyzes photoluminescence spectra prior to and upon iodine sorption. Excitation of iodine through the mechanism of resonance transfer is determined to result in desorption of the iodine sorbed molecules with relatively high kinetic energies (3-1 eV). One evaluated the peculiar distance of resonance transfer the approximate value of which was equal to 2 nm

  6. Nonideal rotations in nuclear magnetic resonance: Estimation of coherence transfer leakage

    Energy Technology Data Exchange (ETDEWEB)

    Jerschow, Alexej [Materials Sciences Division, 11-D62, Lawrence Berkeley Laboratory, Berkeley, California 94720 (United States); Chemistry Department, D62 Hildebrand, University of California at Berkeley, Berkeley, California 94720 (United States)

    2000-07-15

    When spherical tensors are rotated by certain angles, coherence transfer selection rules may apply. For example, a {pi} rotation cleanly inverts the coherence order. A {pi}/2 rotation of a T{sub 0}{sup 1} tensor creates only T{sub {+-}}{sub 1}{sup 1} tensors. In this work estimations are given for the coherence transfer leakage under the action of rotations with small errors in the rotation angle or axis. Although the theory is stated with particular applications to NMR (nuclear magnetic resonance) in mind it is equally applicable wherever nonideal rotations of spherical tensors are considered (e.g., quantum computing and relaxation theory). In NMR it is useful for the estimation of coherence transfer leakage, especially in pulse sequences with many n{pi} pulses. The results are also applicable to spinors and half-integer representations of the rotation group. (c) 2000 American Institute of Physics.

  7. Nuclear spin cooling by electric dipole spin resonance and coherent population trapping

    Science.gov (United States)

    Li, Ai-Xian; Duan, Su-Qing; Zhang, Wei

    2017-09-01

    Nuclear spin fluctuation suppression is a key issue in preserving electron coherence for quantum information/computation. We propose an efficient way of nuclear spin cooling in semiconductor quantum dots (QDs) by the coherent population trapping (CPT) and the electric dipole spin resonance (EDSR) induced by optical fields and ac electric fields. The EDSR can enhance the spin flip-flop rate and may bring out bistability under certain conditions. By tuning the optical fields, we can avoid the EDSR induced bistability and obtain highly polarized nuclear spin state, which results in long electron coherence time. With the help of CPT and EDSR, an enhancement of 1500 times of the electron coherence time can been obtained after a 500 ns preparation time.

  8. Dynamical resonance in F+H2 chemical reaction and rotational excitation effect

    Institute of Scientific and Technical Information of China (English)

    YANG XueMing; XIE DaiQian; ZHANG DongHui

    2007-01-01

    Reaction resonance is a frontier topic in chemical dynamics research, and it is also essential to the understanding of mechanisms of elementary chemical reactions. This short article describes an important development in the frontier of research. Experimental evidence of reaction resonance has been detected in a full quantum state resolved reactive scattering study of the F+H2 reaction. Highly accurate full quantum scattering theoretical modeling shows that the reaction resonance is caused by two Feshbach resonance states. Further studies show that quantum interference is present between the two resonance states for the forward scattering product. This study is a significant step forward in our understanding of chemical reaction resonance in the benchmark F+H2 system. Further experimental studies on the effect of H2 rotational excitation on dynamical resonance have been carried out. Dynamical resonance in the F+H2 (j = 1) reaction has also been observed.

  9. Contact resonance atomic force microscopy imaging in air and water using photothermal excitation

    Energy Technology Data Exchange (ETDEWEB)

    Kocun, Marta; Labuda, Aleksander; Gannepalli, Anil; Proksch, Roger, E-mail: Roger.Proksch@oxinst.com [Asylum Research, an Oxford Instruments Company, Santa Barbara, California 93117 (United States)

    2015-08-15

    Contact Resonance Force Microscopy (CR-FM) is a leading atomic force microscopy technique for measuring viscoelastic nano-mechanical properties. Conventional piezo-excited CR-FM measurements have been limited to imaging in air, since the “forest of peaks” frequency response associated with acoustic excitation methods effectively masks the true cantilever resonance. Using photothermal excitation results in clean contact, resonance spectra that closely match the ideal frequency response of the cantilever, allowing unambiguous and simple resonance frequency and quality factor measurements in air and liquids alike. This extends the capabilities of CR-FM to biologically relevant and other soft samples in liquid environments. We demonstrate CR-FM in air and water on both stiff silicon/titanium samples and softer polystyrene-polyethylene-polypropylene polymer samples with the quantitative moduli having very good agreement between expected and measured values.

  10. Reservoir-induced decoherence of resonantly excited confined polaritons

    Science.gov (United States)

    Ouellet-Plamondon, C.; Sallen, G.; Morier-Genoud, F.; Oberli, D. Y.; Portella-Oberli, M. T.; Deveaud, B.

    2017-02-01

    We report on the effect of decoherence on polariton bistability. The polariton hysteresis loop is shown to collapse in a similar way when increasing the temperature or under nonresonant excitation power. The hysteresis upward threshold is pulled to lower excitation power, whereas the downward threshold remains almost constant. This effect is explained by the population of an incoherent reservoir that induces dephasing and repulsive interaction that saturates at large densities. All experimental findings are accurately simulated with the excitonic Bloch equations and indicate that reservoir-induced dephasing can be dominant over the reservoir-induced energy blueshift.

  11. Decoupling of excitation and receive coils in pulsed magnetic resonance using sinusoidal magnetic field modulation

    Science.gov (United States)

    Tseytlin, Mark; Epel, Boris; Sundramoorthy, Subramanian; Tipikin, Dmitriy; Halpern, Howard J.

    2016-11-01

    In pulsed magnetic resonance, the excitation power is many orders of magnitude larger than that induced by the spin system in the receiving coil or resonator. The receiver must be protected during and immediately after the excitation pulse to allow for the energy stored in the resonator to dissipate to a safe level. The time during which the signal is not detected, the instrumental dead-time, can be shortened by using magnetically decoupled excitation and receive coils. Such coils are oriented, with respect to each other, in a way that minimizes the total magnetic flux produced by one coil in the other. We suggest that magnetically decoupled coils can be isolated to a larger degree by tuning them to separate frequencies. Spins are excited at one frequency, and the echo signal is detected at another. Sinusoidal magnetic field modulation that rapidly changes the Larmor frequency of the spins between the excitation and detection events is used to ensure the resonance conditions for both coils. In this study, the relaxation times of trityl-CD3 were measured in a field-modulated pulsed EPR experiment and compared to results obtained using a standard spin echo method. The excitation and receive coils were tuned to 245 and 256.7 MHz, respectively. Using an available rapid-scan, cross-loop EPR resonator, we demonstrated an isolation improvement of approximately 20-30 dB due to frequency decoupling. Theoretical analysis, numerical simulations, and proof-of-concept experiments demonstrated that substantial excitation-detection decoupling can be achieved. A pulsed L-band system, including a small volume bi-modal resonator equipped with modulation coils, was constructed to demonstrate fivefold dead-time reduction in comparison with the standard EPR experiment. This was achieved by detuning of the excitation and receive coils by 26 MHz and using sinusoidal modulation at 480 kHz.

  12. Rotational Diffusion of Plasmon-Resonant Gold Nanorods for Depth-Resolved Microrheology Using Optical Coherence Tomography

    Science.gov (United States)

    Oldenburg, Amy; Chhetri, Raghav; Kozek, Krystian; Johnston-Peck, Aaron; Tracy, Joseph

    2011-03-01

    The ability to perform microrheology in optically thick samples would enable analysis of bulk tissues. Optical coherence tomography (OCT) provides imaging several mean free scattering path lengths into tissue. In this study we report the use of plasmon-resonant gold nanorods as microrheological sensors in OCT. Nanorods exhibit a longitudinal mode that is excited when they are oriented parallel to the polarization of the incident light, which is favorable for passive microrheology using polarized light to monitor their rotational diffusion. We demonstrate measurements of the rotational diffusion of unconfined, colloidal gold nanorods using polarization-sensitive OCT, and validate the Stokes-Einstein relationship for the nanorods in simple fluids of varying viscosity. We then show that OCT provides depth-resolved imaging of fluid viscosity through measurements of the rotational diffusion rate of the nanorods. We acknowledge support from the Carolina Cancer Center for Nanotechnology Excellence (C-CCNE NIH (NCI) #U54CA119343).

  13. Optimally Coherent Kerr Combs Generated with Crystalline Whispering Gallery Mode Resonators for Ultrahigh Capacity Fiber Communications

    Science.gov (United States)

    Pfeifle, Joerg; Coillet, Aurélien; Henriet, Rémi; Saleh, Khaldoun; Schindler, Philipp; Weimann, Claudius; Freude, Wolfgang; Balakireva, Irina V.; Larger, Laurent; Koos, Christian; Chembo, Yanne K.

    2015-03-01

    Optical Kerr frequency combs are known to be effective coherent multiwavelength sources for ultrahigh capacity fiber communications. These combs are the frequency-domain counterparts of a wide variety of spatiotemporal dissipative structures, such as cavity solitons, chaos, or Turing patterns (rolls). In this Letter, we demonstrate that Turing patterns, which correspond to the so-called primary combs in the spectral domain, are optimally coherent in the sense that for the same pump power they provide the most robust carriers for coherent data transmission in fiber communications using advanced modulation formats. Our model is based on a stochastic Lugiato-Lefever equation which accounts for laser pump frequency jitter and amplified spontaneous emission noise induced by the erbium-doped fiber amplifier. Using crystalline whispering-gallery-mode resonators with quality factor Q ˜109 for the comb generation, we show that when the noise is accounted for, the coherence of a primary comb is significantly higher than the coherence of their solitonic or chaotic counterparts for the same pump power. In order to confirm this theoretical finding, we perform an optical fiber transmission experiment using advanced modulation formats, and we show that the coherence of the primary comb is high enough to enable data transmission of up to 144 Gbit /s per comb line, the highest value achieved with a Kerr comb so far. This performance evidences that compact crystalline photonic systems have the potential to play a key role in a new generation of coherent fiber communication networks, alongside fully integrated systems.

  14. Inactivation of viruses by coherent excitations with a low power visible femtosecond laser

    Directory of Open Access Journals (Sweden)

    Wu T-C

    2007-06-01

    Full Text Available Abstract Background Resonant microwave absorption has been proposed in the literature to excite the vibrational states of microorganisms in an attempt to destroy them. But it is extremely difficult to transfer microwave excitation energy to the vibrational energy of microorganisms due to severe absorption of water in this spectral range. We demonstrate for the first time that, by using a visible femtosecond laser, it is effective to inactivate viruses such as bacteriophage M13 through impulsive stimulated Raman scattering. Results and discussion By using a very low power (as low as 0.5 nj/pulse visible femtosecond laser having a wavelength of 425 nm and a pulse width of 100 fs, we show that M13 phages were inactivated when the laser power density was greater than or equal to 50 MW/cm2. The inactivation of M13 phages was determined by plaque counts and had been found to depend on the pulse width as well as power density of the excitation laser. Conclusion Our experimental findings lay down the foundation for an innovative new strategy of using a very low power visible femtosecond laser to selectively inactivate viruses and other microorganisms while leaving sensitive materials unharmed by manipulating and controlling with the femtosecond laser system.

  15. Inactivation of viruses by coherent excitations with a low power visible femtosecond laser.

    Science.gov (United States)

    Tsen, K T; Tsen, Shaw-Wei D; Chang, Chih-Long; Hung, Chien-Fu; Wu, T-C; Kiang, Juliann G

    2007-06-05

    Resonant microwave absorption has been proposed in the literature to excite the vibrational states of microorganisms in an attempt to destroy them. But it is extremely difficult to transfer microwave excitation energy to the vibrational energy of microorganisms due to severe absorption of water in this spectral range. We demonstrate for the first time that, by using a visible femtosecond laser, it is effective to inactivate viruses such as bacteriophage M13 through impulsive stimulated Raman scattering. By using a very low power (as low as 0.5 nj/pulse) visible femtosecond laser having a wavelength of 425 nm and a pulse width of 100 fs, we show that M13 phages were inactivated when the laser power density was greater than or equal to 50 MW/cm2. The inactivation of M13 phages was determined by plaque counts and had been found to depend on the pulse width as well as power density of the excitation laser. Our experimental findings lay down the foundation for an innovative new strategy of using a very low power visible femtosecond laser to selectively inactivate viruses and other microorganisms while leaving sensitive materials unharmed by manipulating and controlling with the femtosecond laser system.

  16. Hyperboloidal Multipass Resonator RF Discharge Excited Carbon Dioxide Lasers

    Science.gov (United States)

    Xin, Jian Guo

    1987-05-01

    Available from UMI in association with The British Library. In this thesis, we present a novel multipass optical resonator. This type of resonator consists of an ordinary linear, two mirror resonator enclosing a beam-folding optical system composed of a pair of spherical mirrors, which we refer to as "folding mirrors". In the beam folding system, the beam paths occupy a hyperboloidal shell, and therefore can in principle provide a good geometrical overlap with an annular gain medium. The important feature of this type of resonator is that not only does it have the potential to provide a high power output and compact device but also it produces a very good output mode which may be described by Laguerre Gaussian functions. In this thesis, we combine the multipass optical resonator with the RF coaxial discharge system which provides an annular gain medium to produce a compact and powerful laser system. In the experiments, 65 watts output with TEM_{rm oo} mode has been obtained from only 26cm gain length. It can be expected that even higher powers than those recorded in this thesis may be obtained while maintaining a compact laser head.

  17. Spiral Waves and Multiple Spatial Coherence Resonances Induced by Colored Noise in Neuronal Network

    Institute of Scientific and Technical Information of China (English)

    唐昭; 李玉叶; 惠磊; 贾冰; 吉华光

    2012-01-01

    Gaussian colored noise induced spatial patterns and spatial coherence resonances in a square lattice neuronal network composed of Morris-Lecar neurons are studied. Each neuron is at resting state near a saddle-node bifurcation on invariant circle, coupled to its nearest neighbors by electronic coupling. Spiral waves with different structures and disordered spatial structures can be alternately induced within a large range of noise intensity. By calculating spatial structure function and signal-to-noise ratio (SNR), it is found that SNR values are higher when the spiral structures are simple and are lower when the spatial patterns are complex or disordered, respectively. SNR manifest multiple local maximal peaks, indicating that the colored noise can induce multiple spatial coherence resonances. The maximal SNR values decrease as the correlation time of the noise increases. These results not only provide an example of multiple resonances, but also show that Gaussian colored noise play constructive roles in neuronal network.

  18. Cooling molecular vibrations with shaped laser pulses: Optimal control theory exploiting the timescale separation between coherent excitation and spontaneous emission

    CERN Document Server

    Reich, Daniel M

    2013-01-01

    Laser cooling of molecules employing broadband optical pumping involves a timescale separation between laser excitation and spontaneous emission. Here, we optimize the optical pumping step using shaped laser pulses. We derive two optimization functionals to drive population into those excited state levels that have the largest spontaneous emission rates to the target state. We show that, when using optimal control, laser cooling of molecules works even if the Franck-Condon map governing the transitions is preferential to heating rather than cooling. Our optimization functional is also applicable to the laser cooling of other degrees of freedom provided the cooling cycle consists of coherent excitation and dissipative deexcitation steps whose timescales are separated.

  19. Circular Dichroism in Multiphoton Ionization of Resonantly Excited He+ Ions

    Science.gov (United States)

    Ilchen, M.; Douguet, N.; Mazza, T.; Rafipoor, A. J.; Callegari, C.; Finetti, P.; Plekan, O.; Prince, K. C.; Demidovich, A.; Grazioli, C.; Avaldi, L.; Bolognesi, P.; Coreno, M.; Di Fraia, M.; Devetta, M.; Ovcharenko, Y.; Düsterer, S.; Ueda, K.; Bartschat, K.; Grum-Grzhimailo, A. N.; Bozhevolnov, A. V.; Kazansky, A. K.; Kabachnik, N. M.; Meyer, M.

    2017-01-01

    Intense, circularly polarized extreme-ultraviolet and near-infrared (NIR) laser pulses are combined to double ionize atomic helium via the oriented intermediate He+(3 p ) resonance state. Applying angle-resolved electron spectroscopy, we find a large photon helicity dependence of the spectrum and the angular distribution of the electrons ejected from the resonance by NIR multiphoton absorption. The measured circular dichroism is unexpectedly found to vary strongly as a function of the NIR intensity. The experimental data are well described by theoretical modeling and possible mechanisms are discussed.

  20. Linewidth broadening and emission saturation of a resonantly excited quantum dot monitored via an off-resonant cavity mode

    DEFF Research Database (Denmark)

    Ulhaq, A.; Ates, Serkan; Weiler, S.;

    2010-01-01

    We report on the robustness of a detuned mode channel for reading out the relevant s-shell properties of a resonantly excited coupled quantum dot (QD) in a pillar microcavity. The line broadening of the QD s-shell is “monitored” by the mode signal with high conformity to the directly measured QD ...

  1. Grid impedance estimation via excitation of LCL-filter resonance

    DEFF Research Database (Denmark)

    Liserre, M.; Blaabjerg, Frede; Teodorescu, Remus

    2007-01-01

    Inverters adopted in distributed power generation, active filter, and uninterruptible power supply are often connected to the grid through an inductance-capacitor-inductance (LCL) filter. The impedance of the LCL filter has a typical frequency characteristic with a resonance peak. Hence, the LCL...

  2. Theory of low energy excitations in resonant inelastic x-ray scattering for rare-earth systems: Yb compounds as typical examples

    Science.gov (United States)

    Kotani, A.

    2011-04-01

    Theoretical predictions are given for low energy excitations, such as crystal field excitations and Kondo resonance excitations, to be detected by high-resolution measurements of resonant inelastic x-ray scattering (RIXS) of rare-earth materials with Yb compounds as typical examples. Crystal field excitations in the Yb 3d RIXS of a Yb3+ ion in the cubic crystal field are formulated, and the calculation of RIXS spectra for YbN is done. Kondo resonance excitations revealed in the Yb 3d RIXS spectra are calculated for mixed-valence Yb compounds, Yb1-xLuxAl3, in the leading term approximation of the 1/Nf expansion method with a single impurity Anderson model. It is emphasized that the high-resolution RIXS with polarization dependence is a powerful tool to study the crystal field levels together with their symmetry and also the Kondo bound state in rare-earth compounds. Some in-depth discussions are given on the polarization effects of RIXS, including 4d and 2p RIXS spectra, the coherence effect of the Kondo bound states, and the importance of the high-resolution RIXS spectra for condensed matter physics under extreme conditions.

  3. Optimized resonating valence bond state in square lattice: correlations & excitations

    Directory of Open Access Journals (Sweden)

    Z Nourbakhsh

    2009-09-01

    Full Text Available We consider RVB state as a variational estimate for the ground state of Heisenberg antiferromagnet in square lattice. We present numerical calculation of energy, spin-spin correlation function and spin excitation spectrum. We show, that the quantum flactuations reduce of magnetization respect to Neel order. Our results are in good agreement with other methods such as spin-wave calculation and series expansions.

  4. Wakefield Resonant Excitation by Intense Laser Pulse in Capillary Plasma%Wakefield Resonant Excitation by Intense Laser Pulse in Capillary Plasma

    Institute of Scientific and Technical Information of China (English)

    周素云; 袁孝; 刘明萍

    2012-01-01

    The laser-induced plasma wakefield in a capillary is investigated on the basis of a simple two-dimensional analytical model. It is shown that as an intense laser pulse reshaped by the capillary wall propagates in capillary plasma, it resonantly excites a strong wakefield if a suitable laser pulse width and capillary radius are chosen for a certain plasma density. The dependence of the laser width and capillary radius on the plasma density for resonance conditions is considered. The wakefield amplitude and longitudinal scale of bubbles in capillary plasma are much larger than those in unbounded plasma, so the capillary guided plasma wakefield is more favorable to electron acceleration.

  5. Coherence resonance in a noise-driven gene network regulated by small RNA

    Directory of Open Access Journals (Sweden)

    Yanan Zhu

    2014-01-01

    Full Text Available Small RNA has recently drawn more and more attention. In this paper, we concentrate on the influence of noises on gene network regulated by small RNA using chemical Langevin equation. It shows that the noise can cause oscillation when the oscillate does not occur in the corresponding deterministic system. The coherence of the noise induced oscillation reaches a maximum for an optimal intensity of noise, and the coherence resonance appears accordingly. The findings imply probably omnipresent importance of noise in the functioning process of living organism.

  6. Probing the quantum coherence of a nanomechanical resonator using a superconducting qubit: I. Echo scheme

    Energy Technology Data Exchange (ETDEWEB)

    Armour, A D [School of Physics and Astronomy, University of Nottingham, Nottingham, NG7 2RD (United Kingdom); Blencowe, M P [Department of Physics and Astronomy, 6127 Wilder Laboratory, Dartmouth College, Hanover, NH 03755 (United States)], E-mail: andrew.armour@nottingham.ac.uk, E-mail: miles.p.blencowe@dartmouth.edu

    2008-09-15

    We propose a scheme in which the quantum coherence of a nanomechanical resonator can be probed using a superconducting qubit. We consider a mechanical resonator coupled capacitively to a Cooper pair box and assume that the superconducting qubit is tuned to the degeneracy point so that its coherence time is maximized and the electro-mechanical coupling can be approximated by a dispersive Hamiltonian. When the qubit is prepared in a superposition of states, this drives the mechanical resonator progressively into a superposition which in turn leads to apparent decoherence of the qubit. Applying a suitable control pulse to the qubit allows its population to be inverted resulting in a reversal of the resonator dynamics. However, the resonator's interactions with its environment mean that the dynamics is not completely reversible. We show that this irreversibility is largely due to the decoherence of the mechanical resonator and can be inferred from appropriate measurements on the qubit alone. Using estimates for the parameters involved based on a specific realization of the system, we show that it should be possible to carry out this scheme with existing device technology.

  7. Resonant Doppler imaging with Fourier domain optical coherence tomography

    Science.gov (United States)

    Leitgeb, Rainer A.; Szklumowska, Anna; Pircher, Michael; Gotzinger, Erich; Fercher, Adolf F.

    2005-04-01

    Fourier Domain Optical Coherene Tomography (FD OCT) is a high speed imaging modality with increased sensitivity as compared to standard time domain (TD) OCT. The higher sensitivity is especially important, if strongly scattering tissue such as blood is investigated. Recently it could be shown that retinal blood flow can be assessed in-vivo by high speed FD OCT. However the detection bandwidth of color Doppler (CD) FDOCT is strongly limited due to blurring of the detected interference fringes during exposure. This leads to a loss of sensitivity for detection of fast changes in tissue. Using a moving mirror as a reference one can effectively increase the detection bandwidth for CD FDOCT and perform perfusion sectioning. The modality is called resonant CD FDOCT imaging. The principle of the method is presented and experimentally verified.

  8. Electromagnetic excitation of the delta resonance in nuclei

    Energy Technology Data Exchange (ETDEWEB)

    O' Connell, J.S.; Dodge, W.R.; Lightbody J.W. Jr.; Maruyama, X.K.; Adler, J.h.; Hansen, K.; Schro-dash-barder, B.; Bernstein, A.M.; Blomqvist, K.I.; Cottman, B.H.; and others

    1987-03-01

    Inclusive cross sections for the proton and nuclear targets of A = 4, 9, 12, and 16 were measured for 537 and 730 MeV electrons scattered at 37.1 deg. Systematic features of the continuum scattering data are compared with other electron scattering data and with photoabsorption measurements. A model calculation based on the isobar-hole formalism is compared with the data in the delta resonance region.

  9. Asymmetric resonance response analysis of a thermally excited silicon microcantilever for mass-sensitive nanoparticle detection

    Science.gov (United States)

    Bertke, Maik; Hamdana, Gerry; Wu, Wenze; Wasisto, Hutomo Suryo; Peiner, Erwin

    2017-06-01

    The asymmetric resonance responses of a thermally actuated silicon microcantilever of a portable, cantilever-based nanoparticle detector (Cantor) is analysed. For airborne nanoparticle concentration measurements, the cantilever is excited in its first in-plane bending mode by an integrated p-type heating actuator. The mass-sensitive nanoparticle (NP) detection is based on the resonance frequency (f0) shifting due to the deposition of NPs. A homemade phase-locked loop (PLL) circuit is developed for tracking of f0. For deflection sensing the cantilever contains an integrated piezo-resistive Wheatstone bridge (WB). A new fitting function based on the Fano resonance is proposed for analysing the asymmetric resonance curves including a method for calculating the quality factor Q from the fitting parameters. To obtain a better understanding, we introduce an electrical equivalent circuit diagram (ECD) comprising a series resonant circuit (SRC) for the cantilever resonator and voltage sources for the parasitics, which enables us to simulate the asymmetric resonance response and discuss the possible causes. Furthermore, we compare the frequency response of the on-chip thermal excitation with an external excitation using an in-plane piezo actuator revealing parasitic heating of the WB as the origin of the asymmetry. Moreover, we are able to model the phase component of the sensor output using the ECD. Knowing and understanding the phase response is crucial to the design of the PLL and thus the next generation of Cantor.

  10. Selective excitation of bright and dark plasmonic resonances of single gold nanorods

    CERN Document Server

    Demichel, O; Francs, G Colas des; Bouhelier, A; Hertz, E; Billard, F; de Fornel, F; Cluzel, B

    2015-01-01

    Plasmonic dark modes are pure near-field resonances since their dipole moments are vanishing in far field. These modes are particularly interesting to enhance nonlinear light-matter interaction at the nanometer scale because radiative losses are mitigated therefore increasing the intrinsic lifetime of the resonances. However, the excitation of dark modes by standard far field approaches is generally inefficient because the symmetry of the electromagnetic near-field distribution has a poor overlap with the excitation field. Here, we demonstrate the selective optical excitation of bright and dark plasmonic modes of single gold nanorods by spatial phase-shaping the excitation beam. Using two-photon luminescence measurements, we unambiguously identify the symmetry and the order of the emitting modes and analyze their angular distribution by Fourier-space imaging.

  11. Angular distribution of hypersatellite and satellite radiation emitted after resonant and excitation into $U^{91+}$ ions

    CERN Document Server

    Zakowicz, S; Harman, Z; Scheid, W

    2003-01-01

    In collisions of heavy few-electron projectile ions with light targets, an electron can be transferred from the target with the simultaneous excitation of a projectile electron. We study the angular distribution of de-excitation X rays following the resonant capture process. Our results are compared to experimental values of Ma et al. [Phys. Rev. A (joint to this issue)] for collisions of U91+ ions with a hydrogen gas target.

  12. Magnification of photonic crystal fluorescence enhancement via TM resonance excitation and TE resonance extraction on a dielectric nanorod surface

    Energy Technology Data Exchange (ETDEWEB)

    Wu, Hsin-Yu; Cunningham, Brian T [Department of Electrical and Computer Engineering, University of Illinois at Urbana-Champaign, 1406 W Green Street, Urbana, IL 61801 (United States); Zhang Wei [Department of Material Science and Engineering, University of Illinois at Urbana-Champaign, 1304 W Green Street, Urbana, IL 61801 (United States); Mathias, Patrick C, E-mail: bcunning@illinois.edu [Department of Bioengineering, University of Illinois at Urbana-Champaign, 1304 W Springfield Avenue, Urbana, IL 61801 (United States)

    2010-03-26

    Using a one-dimensional grating surface photonic crystal (PC), we experimentally demonstrate that the detection of fluorescent molecules on a PC surface can be substantially magnified through the combined effects of resonance-enhanced excitation of the fluorescent dye, resonance-enhanced extraction of the fluorescence emission and a dielectric nanorod surface coating increasing the surface area available for fluorophore-PC interaction. Enhanced excitation is obtained by engineering a high-Q TM resonant mode to efficiently couple with an incident TM-polarized {lambda} = 633 nm laser for exciting Cyanine-5 (Cy5). Enhanced extraction results from a low-Q TE resonance designed to spectrally overlap the Cy5 emission spectrum for channeling TE-polarized emission towards the detection instrument. The entire PC surface is coated with a porous film of TiO{sub 2} nanorods that allows more fluorophores to penetrate into the region of enhanced near-electric fields. Experimental results reveal a 588-fold enhancement in fluorescence intensity relative to an unpatterned glass surface.

  13. Coherence resonance and synchronization of Hindmarsh-Rose neurons with noise

    Institute of Scientific and Technical Information of China (English)

    Shi Xia; Lu Qi-Shao

    2005-01-01

    Noise effects on coherence resonance and synchronization of Hindmarsh-Rose (HR) neuron model are studied. The coherence resonance of a single HR neuron with Gaussian white noise added to the membrane potential is investigated in situations before, near and after the Hopf bifurcation, separately, with the external direct current as a bifurcation parameter. It is shown that even though there is no coupling between neurons, uncoupled identical HR neurons driven by a common noise can achieve complete synchronization when the noise intensity is higher than a critical value. Furthermore, noise also enhances complete synchronization of weakly coupled neurons. It is concluded that synchronization in bursting neurons is easier to be induced than in spiking ones, and coupling enhances the sensitivity of synchronization of neurons to noise stimulus.

  14. Resonant and non-resonant internal kink modes excited by the energetic electrons on HL-2A tokamak

    Science.gov (United States)

    Yu, L. M.; Chen, W.; Jiang, M.; Shi, Z. B.; Ji, X. Q.; Ding, X. T.; Li, Y. G.; Ma, R. R.; Shi, P. W.; Song, S. D.; Yuan, B. S.; Zhou, Y.; Ma, R.; Song, X. M.; Dong, J. Q.; Xu, M.; Liu, Y.; Yan, L. W.; Yang, Q. W.; Xu, Y. H.; Duan, X. R.; HL-2A Team

    2017-03-01

    Strong resonant and non-resonant internal kink modes (abbreviated as RKs and NRKs, respectively), which are also called resonant and non-resonant fishbones, are observed on HL-2A tokamak with high-power ECRH  +  ECCD‑ (or ECRH) and ECRH  +  ECCD+, respectively. (‘Resonant’ derives from the existence of q  =  1 surface (the resonant surface), and ‘non-resonant’ originates from the absence of q  =  1 surface ({{q}\\text{min}}>1 ). ECCD+ and ECCD‑ mean the driving direction of energetic electrons is the same and opposite to plasma current, respectively.) RK has features of periodic strong bursting amplitude and rapid chirping-down frequency, but NRK usually has the saturated amplitude, slow changed or constant frequency and long-lasting time. The NRK excited by energetic electrons is found for the first time. The reversed q-profiles are formed, and q min decreases during plasma current ramp-up. The value of q min is slightly smaller and a bit bigger than unity for RK and NRK conditions, respectively. The internal kink mode (IKM) structures of RKs and NRKs are confirmed by the ECEI system. Although there are different current drive directions of ECCD for excitation of RK and NRK, they all propagate in electron diamagnetic directions in poloidal. The radial mode structures, frequency and growth rate for IKMs are obtained by solving the dispersion relationship. The NRK is stable when q min is larger than a certain value, and with the decreasing q min the frequency drops, but the growth rate almost keeps constant when {{q}\\text{min}}>1 . This result is in agreement with experimental observation. Studying IKMs excited by energetic electrons can provide important experimental experiences for ITER, because the NRKs may be excited by high-power non-inductive drive of ECCD or ECRH in the operation of hybrid scenarios.

  15. Coherence, energy and charge transfers in de-excitation pathways of electronic excited state of biomolecules in photosynthesis

    DEFF Research Database (Denmark)

    Bohr, Henrik; Malik, F. Bary

    2013-01-01

    The observed multiple de-excitation pathways of photo-absorbed electronic excited state in the peridinin–chlorophyll complex, involving both energy and charge transfers among its constituents, are analyzed using the bio-Auger (B-A) theory. It is also shown that the usually used F¨orster–Dexter th...

  16. Chaotic motions in the resonant separatrix band of a parametrically excited pendulum

    Institute of Scientific and Technical Information of China (English)

    AlbertC.J.LUO

    2000-01-01

    The energy increment spectrum method is developed for the numerical prediction of the appearance and disappearance of a primary (2M : 1)-librational or (M : 1)-rotational resonant separatrix band in a parametrically excited pendulum. The analytical conditions for the presence of such separatrix bands are also obtained. Illustrations of the analytical and numerical results for the appearance and destruction of the resonant bands are given for a comparison.

  17. Theory of double resonance parametric excitation in plasmas. II

    Science.gov (United States)

    Fried, B. D.; Adler, A.; Bingham, R.

    1980-10-01

    A simpler formalism than in the original paper on this subject is used to verify the earlier result that, for a pump frequency separation Delta approximately equal to twice the ion acoustic frequency Omega, the use of two long-wavelength pumps can reduce the threshold for parametric excitation of ion-acoustic waves when, and only when, the Langmuir wave damping rate gamma is much larger than Omega. The threshold is then reduced by a factor of order Omega/omega, the optimum value of Delta being 2 Omega-Gamma for equal pump amplitudes, where Gamma is the ion-acoustic wave damping rate and Gamma is much less than Omega. The analysis presented in a recent paper is shown to be valid only for gamma much less than Omega, where the threshold reduction is quite small, vanishing in the limit of weak ion-acoustic wave damping (Te/Ti much greater than 1).

  18. Electron emission induced by resonant coherent ion-surface interaction at grazing incidence

    Energy Technology Data Exchange (ETDEWEB)

    Garcia de Abajo, F.J. (Departamento de Ciencias de la Computacion e Inteligencia Artificial, Facultad de Informatica, Universidad del Pais Vasco, Apartado 649, 20080 San Sebastian (Spain)); Ponce, V.H. (Centro Atomico Bariloche, Comision Nacional de Energia Atomica, 8400 San Carlos de Bariloche, Rio Negro (Argentina)); Echenique, P.M. (Departamento de Fisica de Materiales, Facultad de Quimica, Universidad del Pais Vasco, Apartado 1072, 20080 San Sebastian (Spain))

    1992-10-19

    A new spectroscopy based on the resonant coherently induced electron loss to the continuum in ion-surface scattering under grazing incidence is proposed. A series of peaks, corresponding to the energy differences determined by the resonant interaction with the rows of atoms in the surface, is predicted to appear in the energy distribution of electrons emitted from electronic states bound to the probe. Calculations for MeV He{sup +} ions scattered at a W(001) surface along the {l angle}100{r angle} direction with a glancing angle of 0--2 mrad show a total yield close to 1.

  19. Coherent perfect absorption induced by the nonlinearity of a Helmholtz resonator.

    Science.gov (United States)

    Achilleos, V; Richoux, O; Theocharis, G

    2016-07-01

    In this work, coherent perfect absorption of sound waves induced by the nonlinear response of a Helmholtz Resonator side loaded to a waveguide, is reported. It is shown that this two-port system can perfectly absorb two high amplitude symmetric incident waves under a certain condition. For the one-sided incidence configuration, this condition leads to an absorption equal to 0.5. Experiments verify these results and are in agreement with an analytical nonlinear impedance model for the resonator. The nonlinear control of perfect absorption opens new possibilities in the design of high amplitude sound attenuators for aero-engine applications.

  20. Coherent quantum state storage and transfer between two phase qubits via a resonant cavity.

    Science.gov (United States)

    Sillanpää, Mika A; Park, Jae I; Simmonds, Raymond W

    2007-09-27

    As with classical information processing, a quantum information processor requires bits (qubits) that can be independently addressed and read out, long-term memory elements to store arbitrary quantum states, and the ability to transfer quantum information through a coherent communication bus accessible to a large number of qubits. Superconducting qubits made with scalable microfabrication techniques are a promising candidate for the realization of a large-scale quantum information processor. Although these systems have successfully passed tests of coherent coupling for up to four qubits, communication of individual quantum states between superconducting qubits via a quantum bus has not yet been realized. Here, we perform an experiment demonstrating the ability to coherently transfer quantum states between two superconducting Josephson phase qubits through a quantum bus. This quantum bus is a resonant cavity formed by an open-ended superconducting transmission line of length 7 mm. After preparing an initial quantum state with the first qubit, this quantum information is transferred and stored as a nonclassical photon state of the resonant cavity, then retrieved later by the second qubit connected to the opposite end of the cavity. Beyond simple state transfer, these results suggest that a high-quality-factor superconducting cavity could also function as a useful short-term memory element. The basic architecture presented here can be expanded, offering the possibility for the coherent interaction of a large number of superconducting qubits.

  1. State-selective high-energy excitation of nuclei by resonant positron annihilation

    Directory of Open Access Journals (Sweden)

    Nikolay A. Belov

    2015-02-01

    Full Text Available In the annihilation of a positron with a bound atomic electron, the virtual γ photon created may excite the atomic nucleus. We put forward this effect as a spectroscopic tool for an energy-selective excitation of nuclear transitions. This scheme can efficiently populate nuclear levels of arbitrary multipolarities in the MeV regime, including giant resonances and monopole transitions. In certain cases, it may have higher cross sections than the conventionally used Coulomb excitation and it can even occur with high probability when the latter is energetically forbidden.

  2. Quantum resonance, Anderson localisation and selective rotational excitation in periodically kicked molecules

    Directory of Open Access Journals (Sweden)

    Averbukh I. Sh.

    2013-03-01

    Full Text Available We show that molecules kicked periodically by laser pulses currently used in molecular alignment experiments allow to observe effects of the periodically kicked quantum rotor in a real rotational system. Among these effects are Anderson localisation in angular momentum and the scaling of the quantum resonance. Based on this, we propose a new scheme for selective molecular rotational excitation.

  3. Study of orbitally excited B mesons and evidence for a new Bπ resonance

    Science.gov (United States)

    Aaltonen, T.; Amerio, S.; Amidei, D.; Anastassov, A.; Annovi, A.; Antos, J.; Apollinari, G.; Appel, J. A.; Arisawa, T.; Artikov, A.; Asaadi, J.; Ashmanskas, W.; Auerbach, B.; Aurisano, A.; Azfar, F.; Badgett, W.; Bae, T.; Barbaro-Galtieri, A.; Barnes, V. E.; Barnett, B. A.; Barria, P.; Bartos, P.; Bauce, M.; Bedeschi, F.; Behari, S.; Bellettini, G.; Bellinger, J.; Benjamin, D.; Beretvas, A.; Bhatti, A.; Bland, K. R.; Blumenfeld, B.; Bocci, A.; Bodek, A.; Bortoletto, D.; Boudreau, J.; Boveia, A.; Brigliadori, L.; Bromberg, C.; Brucken, E.; Budagov, J.; Budd, H. S.; Burkett, K.; Busetto, G.; Bussey, P.; Butti, P.; Buzatu, A.; Calamba, A.; Camarda, S.; Campanelli, M.; Canelli, F.; Carls, B.; Carlsmith, D.; Carosi, R.; Carrillo, S.; Casal, B.; Casarsa, M.; Castro, A.; Catastini, P.; Cauz, D.; Cavaliere, V.; Cavalli-Sforza, M.; Cerri, A.; Cerrito, L.; Chen, Y. C.; Chertok, M.; Chiarelli, G.; Chlachidze, G.; Cho, K.; Chokheli, D.; Clark, A.; Clarke, C.; Convery, M. E.; Conway, J.; Corbo, M.; Cordelli, M.; Cox, C. A.; Cox, D. J.; Cremonesi, M.; Cruz, D.; Cuevas, J.; Culbertson, R.; d'Ascenzo, N.; Datta, M.; de Barbaro, P.; Demortier, L.; Deninno, M.; Devoto, F.; D'Errico, M.; Di Canto, A.; Di Ruzza, B.; Dittmann, J. R.; D'Onofrio, M.; Donati, S.; Dorigo, M.; Driutti, A.; Ebina, K.; Edgar, R.; Elagin, A.; Erbacher, R.; Errede, S.; Esham, B.; Farrington, S.; Feindt, M.; Fernández Ramos, J. P.; Field, R.; Flanagan, G.; Forrest, R.; Franklin, M.; Freeman, J. C.; Frisch, H.; Funakoshi, Y.; Galloni, C.; Garfinkel, A. F.; Garosi, P.; Gerberich, H.; Gerchtein, E.; Giagu, S.; Giakoumopoulou, V.; Gibson, K.; Ginsburg, C. M.; Giokaris, N.; Giromini, P.; Giurgiu, G.; Glagolev, V.; Glenzinski, D.; Gold, M.; Goldin, D.; Golossanov, A.; Gomez, G.; Gomez-Ceballos, G.; Goncharov, M.; González López, O.; Gorelov, I.; Goshaw, A. T.; Goulianos, K.; Gramellini, E.; Grinstein, S.; Grosso-Pilcher, C.; Group, R. C.; Guimaraes da Costa, J.; Hahn, S. R.; Han, J. Y.; Happacher, F.; Hara, K.; Hare, M.; Harr, R. F.; Harrington-Taber, T.; Hatakeyama, K.; Hays, C.; Heck, M.; Heinrich, J.; Herndon, M.; Hocker, A.; Hong, Z.; Hopkins, W.; Hou, S.; Hughes, R. E.; Husemann, U.; Hussein, M.; Huston, J.; Introzzi, G.; Iori, M.; Ivanov, A.; James, E.; Jang, D.; Jayatilaka, B.; Jeon, E. J.; Jindariani, S.; Jones, M.; Joo, K. K.; Jun, S. Y.; Junk, T. R.; Kambeitz, M.; Kamon, T.; Karchin, P. E.; Kasmi, A.; Kato, Y.; Ketchum, W.; Keung, J.; Kilminster, B.; Kim, D. H.; Kim, H. S.; Kim, J. E.; Kim, M. J.; Kim, S. B.; Kim, S. H.; Kim, Y. K.; Kim, Y. J.; Kimura, N.; Kirby, M.; Knoepfel, K.; Kondo, K.; Kong, D. J.; Konigsberg, J.; Kotwal, A. V.; Kreps, M.; Kroll, J.; Kruse, M.; Kuhr, T.; Kurata, M.; Laasanen, A. T.; Lammel, S.; Lancaster, M.; Lannon, K.; Latino, G.; Lee, H. S.; Lee, J. S.; Leo, S.; Leone, S.; Lewis, J. D.; Limosani, A.; Lipeles, E.; Lister, A.; Liu, H.; Liu, Q.; Liu, T.; Lockwitz, S.; Loginov, A.; Lucà, A.; Lucchesi, D.; Lueck, J.; Lujan, P.; Lukens, P.; Lungu, G.; Lys, J.; Lysak, R.; Madrak, R.; Maestro, P.; Malik, S.; Manca, G.; Manousakis-Katsikakis, A.; Marchese, L.; Margaroli, F.; Marino, P.; Martínez, M.; Matera, K.; Mattson, M. E.; Mazzacane, A.; Mazzanti, P.; McNulty, R.; Mehta, A.; Mehtala, P.; Mesropian, C.; Miao, T.; Mietlicki, D.; Mitra, A.; Miyake, H.; Moed, S.; Moggi, N.; Moon, C. S.; Moore, R.; Morello, M. J.; Mukherjee, A.; Muller, Th.; Murat, P.; Mussini, M.; Nachtman, J.; Nagai, Y.; Naganoma, J.; Nakano, I.; Napier, A.; Nett, J.; Neu, C.; Nigmanov, T.; Nodulman, L.; Noh, S. Y.; Norniella, O.; Oakes, L.; Oh, S. H.; Oh, Y. D.; Oksuzian, I.; Okusawa, T.; Orava, R.; Ortolan, L.; Pagliarone, C.; Palencia, E.; Palni, P.; Papadimitriou, V.; Parker, W.; Pauletta, G.; Paulini, M.; Paus, C.; Phillips, T. J.; Piacentino, G.; Pianori, E.; Pilot, J.; Pitts, K.; Plager, C.; Pondrom, L.; Poprocki, S.; Potamianos, K.; Prokoshin, F.; Pranko, A.; Ptohos, F.; Punzi, G.; Ranjan, N.; Redondo Fernández, I.; Renton, P.; Rescigno, M.; Rimondi, F.; Ristori, L.; Robson, A.; Rodriguez, T.; Rolli, S.; Ronzani, M.; Roser, R.; Rosner, J. L.; Ruffini, F.; Ruiz, A.; Russ, J.; Rusu, V.; Sakumoto, W. K.; Sakurai, Y.; Santi, L.; Sato, K.; Saveliev, V.; Savoy-Navarro, A.; Schlabach, P.; Schmidt, E. E.; Schwarz, T.; Scodellaro, L.; Scuri, F.; Seidel, S.; Seiya, Y.; Semenov, A.; Sforza, F.; Shalhout, S. Z.; Shears, T.; Shepard, P. F.; Shimojima, M.; Shochet, M.; Shreyber-Tecker, I.; Simonenko, A.; Sliwa, K.; Smith, J. R.; Snider, F. D.; Sorin, V.; Song, H.; Stancari, M.; St. Denis, R.; Stentz, D.; Strologas, J.; Sudo, Y.; Sukhanov, A.; Suslov, I.; Takemasa, K.; Takeuchi, Y.; Tang, J.; Tecchio, M.; Teng, P. K.; Thom, J.; Thomson, E.; Thukral, V.; Toback, D.; Tokar, S.; Tollefson, K.; Tomura, T.; Tonelli, D.; Torre, S.; Torretta, D.; Totaro, P.; Trovato, M.; Ukegawa, F.; Uozumi, S.; Vázquez, F.; Velev, G.; Vellidis, C.; Vernieri, C.; Vidal, M.; Vilar, R.; Vizán, J.; Vogel, M.; Volpi, G.; Wagner, P.; Wallny, R.; Wang, S. M.; Waters, D.; Wester, W. C.; Whiteson, D.; Wicklund, A. B.; Wilbur, S.; Williams, H. H.; Wilson, J. S.; Wilson, P.; Winer, B. L.; Wittich, P.; Wolbers, S.; Wolfe, H.; Wright, T.; Wu, X.; Wu, Z.; Yamamoto, K.; Yamato, D.; Yang, T.; Yang, U. K.; Yang, Y. C.; Yao, W.-M.; Yeh, G. P.; Yi, K.; Yoh, J.; Yorita, K.; Yoshida, T.; Yu, G. B.; Yu, I.; Zanetti, A. M.; Zeng, Y.; Zhou, C.; Zucchelli, S.; CDF Collaboration

    2014-07-01

    Using the full CDF Run II data sample, we report evidence for a new resonance, which we refer to as B(5970), found simultaneously in the B0π+ and B+π- mass distributions with a significance of 4.4 standard deviations. We further report the first study of resonances consistent with orbitally excited B+ mesons and an updated measurement of the properties of orbitally excited B0 and Bs0 mesons. We measure the masses and widths of all states, as well as the relative production rates of the B1, B2*, and B(5970) states and the branching fraction of the Bs2*0 state to either B*+K- and B+K-. Furthermore, we measure the production rates of the orbitally excited B0,+ states relative to the B0,+ ground state. The masses of the new B(5970) resonances are 5978±5(stat)±12(syst) MeV/c2 for the neutral state and 5961±5(stat)±12(syst) MeV /c2 for the charged state, assuming that the resonance decays into Bπ final states. The properties of the orbitally excited and the new B(59700,+) states are compatible with isospin symmetry.

  4. Electron beam excitation of coherent sub-terahertz radiation in periodic structures manufactured by 3D printing

    Science.gov (United States)

    Phipps, A. R.; MacLachlan, A. J.; Robertson, C. W.; Zhang, L.; Konoplev, I. V.; Cross, A. W.; Phelps, A. D. R.

    2017-07-01

    For the creation of novel coherent sub-THz sources excited by electron beams there is a requirement to manufacture intricate periodic structures to produce and radiate electromagnetic fields. The specification and the measured performance is reported of a periodic structure constructed by additive manufacturing and used successfully in an electron beam driven sub-THz radiation source. Additive manufacturing, or ;3D printing;, is promising to be quick and cost-effective for prototyping these periodic structures.

  5. Influence of environment induced correlated fluctuations in electronic coupling on coherent excitation energy transfer dynamics in model photosynthetic systems.

    Science.gov (United States)

    Huo, Pengfei; Coker, David F

    2012-03-21

    Two-dimensional photon-echo experiments indicate that excitation energy transfer between chromophores near the reaction center of the photosynthetic purple bacterium Rhodobacter sphaeroides occurs coherently with decoherence times of hundreds of femtoseconds, comparable to the energy transfer time scale in these systems. The original explanation of this observation suggested that correlated fluctuations in chromophore excitation energies, driven by large scale protein motions could result in long lived coherent energy transfer dynamics. However, no significant site energy correlation has been found in recent molecular dynamics simulations of several model light harvesting systems. Instead, there is evidence of correlated fluctuations in site energy-electronic coupling and electronic coupling-electronic coupling. The roles of these different types of correlations in excitation energy transfer dynamics are not yet thoroughly understood, though the effects of site energy correlations have been well studied. In this paper, we introduce several general models that can realistically describe the effects of various types of correlated fluctuations in chromophore properties and systematically study the behavior of these models using general methods for treating dissipative quantum dynamics in complex multi-chromophore systems. The effects of correlation between site energy and inter-site electronic couplings are explored in a two state model of excitation energy transfer between the accessory bacteriochlorophyll and bacteriopheophytin in a reaction center system and we find that these types of correlated fluctuations can enhance or suppress coherence and transfer rate simultaneously. In contrast, models for correlated fluctuations in chromophore excitation energies show enhanced coherent dynamics but necessarily show decrease in excitation energy transfer rate accompanying such coherence enhancement. Finally, for a three state model of the Fenna-Matthews-Olsen light

  6. Relaxation dynamics of a quantum emitter resonantly coupled to a coherent state of a localized surface plasmon.

    Science.gov (United States)

    Nerkararyan, Khachatur V; Bozhevolnyi, Sergey I

    2015-01-01

    We investigate the relaxation dynamics of a quantum dipole emitter (QDE), e.g., a molecule or quantum dot, located near a metal nanoparticle (MNP) exhibiting a dipolar localized surface plasmon (LSP) resonance at the frequency of the QDE radiative transition. A generic three-level QDE, which is pumped with an external laser pulse and thereby brought into an optically active excited state, is considered to be weakly coupled to the resonant LSP described by a coherent state. It is shown that, under the condition of the QDE-MNP characteristic relaxation time being much shorter than that of the QDE in free space but much longer than the LSP lifetime, the QDE relaxation dynamics can be described analytically and feature, in general, non-exponential decay with complicated transient behaviour. The main physical consequence of this relaxation process is that the emission, being largely determined by the MNP, comes out with a substantial delay. It is also shown that energy dissipation in the QDE-MNP system is relatively weak with the probability of the photon emission being ∼0.75, a number which, rather surprisingly, does not explicitly depend on the metal absorption characteristics. A large number of QDE-MNP system parameters in our analytical description open new possibilities for controlling quantum emitter dynamics.

  7. Resonance-enhanced photon excitation spectroscopy of the even-parity autoionizing Rydberg states of Kr

    Institute of Scientific and Technical Information of China (English)

    LI ChunYan; WANG TingTing; ZHEN JunFeng; ZHANG Qun; CHEN Yang

    2009-01-01

    Kr atoms were produced in their metastable states 4p55s [3/2]2 and 4p55s' [1/2]0 in a pulsed DC discharge in a beam, and subsequently excited to the even-parity autoionizing Rydberg states 4p5np' [3/2]1,2, [1/2]1 and 4p5nf' [5/2]3 using single photon excitation. The excitation spectra of the even-parity autoionizing resonance series from the metastable Kr were obtained by recording the autoionized Kr+ ions with time-of-flight ion detection in the photon energy range of 29000-40000 cm-1. A wealth of autoionizing resonances were newly observed, from which more precise and more systematic spec-troscopic data of the level energy and quantum defects were derived.

  8. Resonance-Enhanced Photon Excitation Spectroscopy of the Even-Parity Autoionizing Rydberg States of Xe

    Institute of Scientific and Technical Information of China (English)

    Chun-yan Li; Ting-ting Wang; Jun-feng Zhen; Qun Zhang; Yang Chen

    2008-01-01

    Xenon atoms were produced in their metastable states 5p56s[3/2]2 and 5p56s'[1/2]0 in a pulsed DC discharge in a beam, and subsequently excited to the even-parity autoionizing Rydberg states 5p5np' [3/2] 1 ,[1/2]1, t, and 5p5 nf'[5/2]3 using single photon excitation. The excitation spectra of the even-parity autoionizing resonance series from the metastable 129Xe were obtained by recording the autoionized Xe+ with time-of-flight ion detection in the photon energy range of 28000-42000 cm-1. A wealth of autoionizing resonances were newly observed, from which more precise and systematic spectroscopic data of the level energies and quantum defects were derived.

  9. Doubly excited 2s2p 1,3p1 resonances in photoionization of helium

    Institute of Scientific and Technical Information of China (English)

    Wan Jian-Jie; Dong Chen-Zhong

    2009-01-01

    The multi-configuration Dirac-Fock (MCDF) method is implemented to study doubly excited 2s2p 1,3P1 resonances of the helium atom and the interference between photoionization and photoexcitation autoionization processes.In order to reproduce the total photoionization sprectra,the excited energies from the ground ls2 1 S0 state to the doubly excited 2s2p 1'3P1 states and the relevant Auger decay rates and widths are calculated in detail. Furthermore,the interference profile determined by the so-called Fano parameters q and p2 is also reproduced. Good agreement is found between the present results and other available theoretical and experimental results. This indeed shows a promising way to investigate the Fano resonances in photoionization of atoms within the MCDF scheme,although there are some discrepancies in the present calculations of the 2s2p 3P1 state.

  10. Nonlinear Response of Vibrational Conveyers with Nonideal Vibration Exciter: Superharmonic and Subharmonic Resonance

    Directory of Open Access Journals (Sweden)

    H. Bayıroğlu

    2012-01-01

    Full Text Available Vibrational conveyers with a centrifugal vibration exciter transmit their load based on the jumping method. Common unbalanced-mass driver oscillates the trough. The motion is strictly related to the vibrational parameters. The transition over resonance of a vibratory system, excited by rotating unbalances, is important in terms of the maximum vibrational amplitude produced and the power demand on the drive for the crossover. The mechanical system is driven by the DC motor. In this study, the working ranges of oscillating shaking conveyers with nonideal vibration exciter have been analyzed analytically for superharmonic and subharmonic resonances by the method of multiple scales and numerically. The analytical results obtained in this study agree well with the numerical results.

  11. Resonance-enhanced photon excitation spectroscopy of the even-parity autoionizing Rydberg states of Kr

    Institute of Scientific and Technical Information of China (English)

    2009-01-01

    Kr atoms were produced in their metastable states 4p55s [3/2]2 and 4p55s’ [1/2]0 in a pulsed DC dis-charge in a beam,and subsequently excited to the even-parity autoionizing Rydberg states 4p5np’ [3/2]1,2,[1/2]1 and 4p5nf’ [5/2]3 using single photon excitation.The excitation spectra of the even-parity autoionizing resonance series from the metastable Kr were obtained by recording the autoionized Kr+ ions with time-of-flight ion detection in the photon energy range of 29000-40000 cm1.A wealth of autoionizing resonances were newly observed,from which more precise and more systematic spec-troscopic data of the level energy and quantum defects were derived.

  12. Coherent time evolution of highly excited Rydberg states in pulsed electric field Opening a stringent way to selectively field-ionize the highly excited states

    CERN Document Server

    Tada, M; Ogawa, I; Funahashi, H; Yamamoto, K; Matsuki, S

    2000-01-01

    Coherent time evolution of highly excited Rydberg states in Rb (98 < n < 150) under pulsed electric field in high slew-rate regime was investigated with the field ionization detection. The electric field necessary to ionize the Rydberg states was found to take discrete values successively depending on the slew rate. Specifically the slew-rate dependence of the ionization field varies with the quantum defect value of the states, i.e. with the energy position of the states relative to the adjacent manifold. This discrete transitional behavior of the ionization field observed for the first time is considered to be a manifestation of the strong coherence effect in the time evolution of the Rydberg states in pulsed electric field and opens a new effective way to stringently select a low-l state from the nearby states by field ionization.

  13. Instability analysis of resonant standing waves in a parametrically excited boxed basin

    Energy Technology Data Exchange (ETDEWEB)

    Sirwah, Magdy A [Department of Mathematics, Faculty of Science, Tanta University, Tanta (Egypt)], E-mail: magdysirwah@yahoo.com

    2009-06-15

    Two-mode parametric excited interfacial waves of incompressible immiscible liquids in an infinite boxed basin subjected to a vertical excitation are studied. The method of multiple time scales is used to obtain uniform solutions of the second-order system as well as the third-order one, which in turn leads to the solvability conditions of the two orders including the cubic interaction terms. The different cases of resonance that arise among the natural frequencies together with the frequency of the vertical vibration of the box are demonstrated theoretically and numerical computations of one of these cases (the two-to-one internal resonance and the principal parametric resonance) have been performed in detail in order to investigate the behavior of the resonant waves, especially the qualitative one. The autonomous system of four first-order differential equations for the modulation of the amplitudes and phases of the resonant waves is derived. Some numerical applications are achieved to show the stability criteria of the excited liquids inside the considered basin.

  14. Resonance-enhanced electron-impact excitation of Cu-like gold

    Science.gov (United States)

    Xia, L.; Zhang, C. Y.; Si, R.; Guo, X. L.; Chen, Z. B.; Yan, J.; Li, S.; Chen, C. Y.; Wang, K.

    2017-09-01

    Employing the independent-process and isolated-resonance approximations using distorted-waves (IPIRDW), we have performed a series of calculations of the resonance-enhanced electron-impact excitations (EIE) among 27 singly excited levels from the n ≤ 6 configurations of Cu-like gold (Au, Z = 79). Resonance excitation (RE) contributions from both the n = 4 → 4 - 7 and n = 3 → 4 core excitations have been considered. Our results demonstrate that RE contributions are significant and enhance the effective collision strengths (ϒ) of certain excitations by up to an order of magnitude at low temperature (106.1 K), and are still important at relatively high temperature (107.5 K). Results from test calculations of the resonance-enhanced EIE processes among 16 levels from the n ≤ 5 configurations using both the Dirac R-matrix (DRM) and IPIRDW approaches agree very well with each other. This means that the close-coupling effects are not important for this ion, and thus warrants the reliability of present resonance-enhanced EIE data among the 27 levels. The results from the collisional-radiative model (CRM) show that, at 3000 eV, near where Cu-like Au is most abundant, RE contributions have important effects (up to 25%) on the density diagnostic line intensity ratios, which are sensitive near 1020 cm-3. The present work is the first EIE research including RE contributions for Cu-like Au. Our EIE data are more accurate than previous results due to our consideration of RE contributions, and the data should be helpful for modeling and diagnosing a variety of plasmas.

  15. Exciting Molecules Close to the Rotational Quantum Resonance: Anderson Wall and Rotational Bloch Oscillations.

    Science.gov (United States)

    Floß, Johannes; Averbukh, Ilya Sh

    2016-05-19

    We describe a universal behavior of linear molecules excited by a periodic train of short laser pulses under conditions close to the quantum resonance. The quantum resonance effect causes an unlimited ballistic growth of the angular momentum. We show that a disturbance of the quantum resonance, either by the centrifugal distortion of the rotating molecules or a controlled detuning of the pulse train period from the so-called rotational revival time, eventually halts the growth by causing Anderson localization beyond a critical value of the angular momentum, the Anderson wall. Below the wall, the rotational excitation oscillates with the number of pulses due to a mechanism similar to Bloch oscillations in crystalline solids. We suggest optical experiments capable of observing the rotational Anderson wall and Bloch oscillations at near-ambient conditions with the help of existing laser technology.

  16. Vacuum ultraviolet resonance Raman studies of the excited electronic states of ethylene

    Science.gov (United States)

    Sension, Roseanne J.; Hudson, Bruce S.

    1989-02-01

    A resonance Raman study of ethylene has been performed with the use of excitation wavelengths ranging from 200 to 141 nm. Excitation resonant with the V(pi pi -asterisk) state results in Raman spectra exhibiting intensity in the C = C stretching vibration, the CH2 symmetric scissors vibration, the CH2 torsional vibration and the CH2 out-of-plane wagging vibrations. These spectra confirm that the V state is strongly twisted about the C-C bond. They also indicate that the C = CH2 groups are no longer planar in the V state. The spectrum obtained in resonance with the (pi 3d) Rydberg transitions once again exhibits activity in the CH2 symmetric scissors mode.

  17. Observation of the stimulated coherent diffraction radiation in an open resonator at LUCX facility

    Energy Technology Data Exchange (ETDEWEB)

    Aryshev, A., E-mail: alar@post.kek.jp [KEK: High Energy Accelerator Research Organization,1-1 Oho, Tsukuba, Ibaraki 305-0801 (Japan); Araki, S.; Fukuda, M. [KEK: High Energy Accelerator Research Organization,1-1 Oho, Tsukuba, Ibaraki 305-0801 (Japan); Karataev, P. [John Adams Institute at Royal Holloway, University of London, Egham, Surrey TW20 0EX (United Kingdom); Konkov, A.; Naumenko, G.; Potylitsyn, A. [Tomsk Polytechnic University, Institute of Physics and Technology, Lenin ave. 30, Tomsk 634050 (Russian Federation); Sakaue, K. [Waseda University, 3-4-1, Okubo, Shinjuku, Tokyo 169-8555 (Japan); Sukhikh, L. [Tomsk Polytechnic University, Institute of Physics and Technology, Lenin ave. 30, Tomsk 634050 (Russian Federation); Terunuma, N. [KEK: High Energy Accelerator Research Organization,1-1 Oho, Tsukuba, Ibaraki 305-0801 (Japan); Verigin, D. [Tomsk Polytechnic University, Institute of Physics and Technology, Lenin ave. 30, Tomsk 634050 (Russian Federation); Urakawa, J. [KEK: High Energy Accelerator Research Organization,1-1 Oho, Tsukuba, Ibaraki 305-0801 (Japan)

    2014-11-01

    We present an initial test of a new type of a pre-bunched beam pumped free electron maser based on Stimulated Coherent Diffraction Radiation (SCDR) generated in an open resonator. A fast Schottky Barrier Diode (time response <1ns) has enabled us to investigate the properties of the radiation stored in the cavity as well as the intrinsic properties of the cavity itself. We observed a turn-by-turn SCDR generated by a multibunch beam. When the cavity length was exactly a half of the bunch spacing a clear resonance was observed. Moreover, turn-by-turn measurements revealed the cavity quality factor of 72.88, which was rather high for an open resonator in the wavelength range of 3–5 mm. An exponential growth of the photon intensity as a function of the number of bunches was also demonstrated.

  18. Coherent X-ray radiation excited by a diverging relativistic electron beam in a single crystal

    Energy Technology Data Exchange (ETDEWEB)

    Blazhevich, S. V., E-mail: noskovbupk@mail.ru; Noskov, A. V. [Belgorod State National Research University (Russian Federation)

    2015-05-15

    We develop a dynamic theory of coherent X-rays generated in a single-crystal wafer by a diverging relativistic electron beam. The dependence of the spectral-angular density of coherent X-ray radiation on the angle of divergence is analyzed for the case when the angular spread can be described by the 2D Gaussian distribution. The theory constructed here makes it possible to analyze coherent radiation for an arbitrary angular distribution of electrons in the beam as well.

  19. Resonance between coherent whistler mode waves and electrons in the topside ionosphere

    Science.gov (United States)

    Neubert, T.; Bell, T. F.; Storey, L. R. O.

    1987-01-01

    Landau resonance and cyclotron resonance of coherent whistler mode waves and energetic electrons are explored for magnetoplasmas with appreciable gradients in the plasma density and magnetic field strength. It is shown that in the topside ionosphere of the earth near the ion transition height the gradients in plasma density and magnetic field strength along a magnetic field line may match in a way which enhances both Landau and cyclotron interactions between waves and electrons at the loss cone pitch angle. The pitch angle scattering induced by a signal from a ground-based VLF transmitter in the ionosphere above the transmitter has been estimated and compared to the pitch angle scattering induced by naturally occurring ELF hiss through cyclotron resonance. It is found that the expected scattering due to plasmapheric hiss is an order of magnitude larger than that due to Landau resonance in the topside ionosphere. Pitch angle scattering due to cyclotron resonance in the topside ionosphere, however, may be larger by a factor of 2. It is suggested that the 'fast Trimpi' effect may be caused by a cyclotron resonance interaction in the topside ionosphere.

  20. Excitation and Imaging of Resonant Optical Modes of Au Triangular Nano-Antennas Using Cathodoluminescence Spectroscopy

    CERN Document Server

    Kumar, Anil; Mabon, James C; Chow, Edmond; Fang, Nicholas X

    2010-01-01

    Cathodoluminescence (CL) imaging spectroscopy is an important technique to understand resonant behavior of optical nanoantennas. We report high-resolution CL spectroscopy of triangular gold nanoantennas designed with near-vacuum effective index and very small metal-substrate interface. This design helped in addressing issues related to background luminescence and shifting of dipole modes beyond visible spectrum. Spatial and spectral investigations of various plasmonic modes are reported. Out-of-plane dipole modes excited with vertically illuminated electron beam showed high-contrast tip illumination in panchromatic imaging. By tilting the nanostructures during fabrication, in-plane dipole modes of antennas were excited. Finite-difference time-domain simulations for electron and optical excitations of different modes showed excellent agreement with experimental results. Our approach of efficiently exciting antenna modes by using low index substrates is confirmed both with experiments and numerical simulations....

  1. Resonance search for quark excitation in the gamma + jet final state at CMS

    CERN Document Server

    Sharma, Varun

    2014-01-01

    This poster presents a search for excited quarks (q*) decaying into a $\\gamma$ + jet final state at $\\sqrt{\\rm s}$= 8 TeV with the CMS experiment, using the dataset corresponding to an integrated luminosity of 19.7 $\\,\\text{fb}^\\text{-1}$ collected during 2012 data taking at the LHC. Photons and jets with high transverse momentum are selected to search for a resonance peak in the $\\gamma$ + jet invariant mass distribution. The 95\\% confidence level upper limits on cross section times branching ratio are evaluated as a function of excited quark mass (Mq*). We exclude at 95\\% CL excited quarks with 0.7 $<$ Mq* $<$ 3.5 TeV for standard model couplings, and present exclusions of excited quark mass as a function of coupling strength.

  2. Triply resonant coherent four-wave mixing in silicon nitride microresonators.

    Science.gov (United States)

    Fülöp, Attila; Krückel, Clemens J; Castelló-Lurbe, David; Silvestre, Enrique; Torres-Company, Victor

    2015-09-01

    Generation of multiple tones using four-wave mixing (FWM) has been exploited for many applications, ranging from wavelength conversion to frequency comb generation. FWM is a coherent process, meaning that its dynamics strongly depend on the relative phase among the waves involved. The coherent nature of FWM has been exploited for phase-sensitive processing in different waveguide structures, but it has never been studied in integrated microresonators. Waveguides arranged in a resonant way allow for an effective increase in the wavelength conversion efficiency (at the expense of a reduction in the operational bandwidth). In this Letter, we show that phase shaping of a three-wave pump provides an extra degree of freedom for controlling the FWM dynamics in microresonators. We present experimental results in single-mode, normal-dispersion high-Q silicon nitride resonators, and numerical calculations of systems operating in the anomalous dispersion regime. Our results indicate that the wavelength conversion efficiency and modulation instability gain in microcavities pumped by multiple waves can be significantly modified with the aid of simple lossless coherent control techniques.

  3. Rectangular split-ring resonators with single-split and two-splits under different excitations at microwave frequencies

    Directory of Open Access Journals (Sweden)

    S. Zahertar

    2015-11-01

    Full Text Available In this work, transmission characteristics of rectangular split-ring resonators with single-split and two-splits are analyzed at microwave frequencies. The resonators are coupled with monopole antennas for excitation. The scattering parameters of the devices are investigated under different polarizations of E and H fields. The magnetic resonances induced by E and H fields are identified and the differences in the behavior of the resonators due to orientations of the fields are explained based on simulation and experimental results. The addition of the second split of the device is investigated considering different configurations of the excitation vectors. It is demonstrated that the single-split and the two-splits resonators exhibit identical transmission characteristics for a certain excitation configuration as verified with simulations and experiments. The presented resonators can effectively function as frequency selective media for varying excitation conditions.

  4. Excited superdeformed Kπ=0+ rotational bands in /β-vibrational fission resonances of 240Pu

    Science.gov (United States)

    Hunyadi, M.; Gassmann, D.; Krasznahorkay, A.; Habs, D.; Thirolf, P. G.; Csatlós, M.; Eisermann, Y.; Faestermann, T.; Graw, G.; Gulyás, J.; Hertenberger, R.; Maier, H. J.; Máté, Z.; Metz, A.; Chromik, M. J.

    2001-04-01

    The intermediate structure of fission resonances of 240Pu was observed with an experimental energy resolution of 7 keV in the excitation energy region of E*=3.8-5.6 MeV using the 239Pu(d,pf)240Pu reaction. Two-vibrational resonance groups centered at E*=4.6 MeV and 5.1 MeV, and attributed to the excitation of three and four /β-phonons, were resolved into individual substates, which could be assigned to the low-spin members of Kπ=0+ superdeformed (SD) rotational bands. In the region of the lower E*=4.6 MeV resonance individual moments of inertia of six well separated bands could be extracted for the first time with values of Θ/ℏ2 around 157 MeV-1, close to that of the ground state band in the second well. From the level density of these Kπ=0+ band heads the excitation energy of the SD ground state was determined to (/2.25+/-0.20) MeV, in agreement with earlier estimates from excitation functions.

  5. Electron spin coherence and electron nuclear double resonance of Bi donors in natural Si.

    Science.gov (United States)

    George, Richard E; Witzel, Wayne; Riemann, H; Abrosimov, N V; Nötzel, N; Thewalt, Mike L W; Morton, John J L

    2010-08-06

    Donors in silicon hold considerable promise for emerging quantum technologies, due to their uniquely long electron spin coherence times. Bismuth donors in silicon differ from more widely studied group V donors, such as phosphorous, in several significant respects: They have the strongest binding energy (70.98 meV), a large nuclear spin (I=9/2), and a strong hyperfine coupling constant (A=1475.4  MHz). These larger energy scales allow us to perform a detailed test of theoretical models describing the spectral diffusion mechanism that is known to govern the electron spin decoherence of P donors in natural silicon. We report the electron-nuclear double resonance spectra of the Bi donor, across the range 200 MHz to 1.4 GHz, and confirm that coherence transfer is possible between electron and nuclear spin degrees of freedom at these higher frequencies.

  6. Observation of intermolecular double-quantum coherence signal dips in nuclear magnetic resonance

    Institute of Scientific and Technical Information of China (English)

    Shen Gui-Ping; Cai Cong-Bo; Cai Shu-Hui; Chen Zhong

    2011-01-01

    The correlated spectroscopy revamped by asymmetric Z-gradient echo detection (CRAZED) sequence is modified to investigate intermolecular double-quantum coherence nuclear magnetic resonance signal dips in highly polarized spin systems.It is found that the occurrence of intermolecular double-quantum coherence signal dips is related to sample geometry,field inhomogeneity and dipolar correlation distance.If the field inhomogeneity is refocused,the signal dip occurs at a fixed position whenever the dipolar correlation distance approaches the sample dimension.However,the position is shifted when the field inhomogeneity exists.Experiments and simulations are performed to validate our theoretic analysis.These signal features may offer a unique way to investigate porous structures and may find applications in biomedicine and material science.

  7. Sectional model test study on vortex-excited resonance of vehicle-bridge system of Shanghai Bridge over Yangtse River

    Institute of Scientific and Technical Information of China (English)

    Li ZHOU; Yaojun GE

    2009-01-01

    It is necessary to study how vehicles influence the vortex-excited resonance of vehicle-bridge systems,because lock-in wind speed is low and vortex-excited resonance is sensitive to any change in the main girder sections. Based on the Shanghai Bridge over the Yangtse River, the vortex-excited resonance of a 1:60 scale sectional model was tested in a TJ-lwind tunnel, with or without vehicles at the attack angle of 0°, + 3 and -3°,respectively. The conversion relationships between the resonant amplitudes of the sectional model and that of the prototype bridge were also established by mode shape correction. The result indicates that: 1) for the bridge with vehicles, the vertical vortex-excited resonance is accom-panied by torsion vibration with the same frequency, and vice versa, 2) the amplitude of vortex-excited resonance of the bridge with vehicles is much larger than that of the bridge without vehicles, and 3) the lock-in wind speed of the vortex-excited resonance becomes smaller due to the disturbance of vehicles. It is obvious that vehicles bring about changes in the aerodynamic shape of the main girder.Therefore, the influence of vehicles on vortex-excited resonance performance of vehicle-bridge systems, in terms of both amplitude and mode, should not be ignored.

  8. Coherent resonance of quantum plasmons in Stone-Wales defected graphene-silver nanowire hybrid system

    Science.gov (United States)

    Liu, Tong; Zhang, Hong; Cheng, Xin-Lu; Xu, Yang

    2017-10-01

    Defected graphene has a more important practical significance than graphene. Silver nanoparticles can modify the optical properties of defected graphene. We present herein a detailed theoretical analysis about the coherent resonance of quantum plasmons in the Stone-Wales (SW) defected graphene-silver nanowire hybrid system by using time-dependent density functional theory. The plasmon coherent effect is mainly attributed to the electromagnetic field coupling between the Stone-Wales defected graphene and silver nanowires. As a result, the optical response of the hybrid system exhibits a remarkable enhancement. Plasmon resonance, which depends on polarization and selectable tuning, is enhanced in wide frequency regions. Moreover, it reveals that the resonance frequency of an optical absorption spectrum depends on the space configuration of the SW defected graphene in the hybrid system. This investigation provides a better understanding of the plasmon enhancement effect used in a graphene-based photoelectric device. The study also offers an effective means of detecting the defects existing in graphene.

  9. Circumferential resonance modes of solid elastic cylinders excited by obliquely incident acoustic waves.

    Science.gov (United States)

    Fan, Ying; Honarvar, Farhang; Sinclair, Anthony N; Jafari, Mohammad-Reza

    2003-01-01

    When an immersed solid elastic cylinder is insonified by an obliquely incident plane acoustic wave, some of the resonance modes of the cylinder are excited. These modes are directly related to the incidence angle of the insonifying wave. In this paper, the circumferential resonance modes of such immersed elastic cylinders are studied over a large range of incidence angles and frequencies and physical explanations are presented for singular features of the frequency-incidence angle plots. These features include the pairing of one axially guided mode with each transverse whispering gallery mode, the appearance of an anomalous pseudo-Rayleigh in the cylinder at incidence angles greater than the Rayleigh angle, and distortional effects of the longitudinal whispering gallery modes on the entire resonance spectrum of the cylinder. The physical explanations are derived from Resonance Scattering Theory (RST), which is employed to determine the interior displacement field of the cylinder and its dependence on insonification angle.

  10. Compound grating structures in photonic crystals for resonant excitation of azobenzene

    DEFF Research Database (Denmark)

    Jahns, Sabrina; Kallweit, Christine; Adam, Jost

    -difference time-domain (FDTD) calculations for determination of resonance positions and electric field strengths in compound grating structures. By superimposing two single-period gratings a photonic crystal can be designed supporting multiple guided mode resonances suitable to switch azobenzenes between...... is small and thus a high excitation light intensity is required. We investigate the enhancement of the local energy density using periodically nanostructured surfaces in a high refractive index material. Such photonic crystals support quasi-guided modes visible as resonances in the reflection as well...... as in the transmission light spectrum. These guided modes have field contributions decaying exponentially in the near field of the photonic crystal. Azobenzene immobilized on the photonic crystal surface will experience a significantly increased light intensity compared to non-resonant surfaces. We performed finite...

  11. Compound grating structures in photonic crystals for resonant excitation of azobenzene

    DEFF Research Database (Denmark)

    Jahns, Sabrina; Kallweit, Christine; Adam, Jost;

    -difference time-domain (FDTD) calculations for determination of resonance positions and electric field strengths in compound grating structures. By superimposing two single-period gratings a photonic crystal can be designed supporting multiple guided mode resonances suitable to switch azobenzenes between...... is small and thus a high excitation light intensity is required. We investigate the enhancement of the local energy density using periodically nanostructured surfaces in a high refractive index material. Such photonic crystals support quasi-guided modes visible as resonances in the reflection as well...... as in the transmission light spectrum. These guided modes have field contributions decaying exponentially in the near field of the photonic crystal. Azobenzene immobilized on the photonic crystal surface will experience a significantly increased light intensity compared to non-resonant surfaces. We performed finite...

  12. Coherence and population dynamics of chlorophyll excitations in FCP complex: Two-dimensional spectroscopy study.

    Science.gov (United States)

    Butkus, Vytautas; Gelzinis, Andrius; Augulis, Ramūnas; Gall, Andrew; Büchel, Claudia; Robert, Bruno; Zigmantas, Donatas; Valkunas, Leonas; Abramavicius, Darius

    2015-06-07

    Energy transfer processes and coherent phenomena in the fucoxanthin-chlorophyll protein complex, which is responsible for the light harvesting function in marine algae diatoms, were investigated at 77 K by using two-dimensional electronic spectroscopy. Experiments performed on femtosecond and picosecond timescales led to separation of spectral dynamics, witnessing evolutions of coherence and population states of the system in the spectral region of Qy transitions of chlorophylls a and c. Analysis of the coherence dynamics allowed us to identify chlorophyll (Chl) a and fucoxanthin intramolecular vibrations dominating over the first few picoseconds. Closer inspection of the spectral region of the Qy transition of Chl c revealed previously not identified, mutually non-interacting chlorophyll c states participating in femtosecond or picosecond energy transfer to the Chl a molecules. Consideration of separated coherent and incoherent dynamics allowed us to hypothesize the vibrations-assisted coherent energy transfer between Chl c and Chl a and the overall spatial arrangement of chlorophyll molecules.

  13. Stochastic resonance, coherence resonance, and spike timing reliability of Hodgkin-Huxley neurons with ion-channel noise

    Science.gov (United States)

    Yu, Haitao; Galán, Roberto F.; Wang, Jiang; Cao, Yibin; Liu, Jing

    2017-04-01

    The random transitions of ion channels between open and closed states are a major source of noise in neurons. In this study, we investigate the stochastic dynamics of a single Hodgkin-Huxley (HH) neuron with realistic, physiological channel noise, which depends on the channel number and the voltage potential of the membrane. Without external input, the stochastic HH model can generate spontaneous spikes induced by ion-channel noise, and the variability of inter-spike intervals attains a minimum for an optimal membrane area, a phenomenon known as coherence resonance. When a subthreshold periodic input current is added, the neuron can optimally detect the input frequency for an intermediate membrane area, corresponding to the phenomenon of stochastic resonance. We also investigate spike timing reliability of neuronal responses to repeated presentations of the same stimulus with different realizations of channel noise. We show that, with increasing membrane area, the reliability of neuronal response decreases for subthreshold periodic inputs, and attains a minimum for suprathreshold inputs. Furthermore, Arnold tongues of high reliability arise in a two-dimensional plot of frequency and amplitude of the sinusoidal input current, resulting from the resonance effect of spike timing reliability.

  14. Multiple-Resonance Local Wave Functions for Accurate Excited States in Quantum Monte Carlo.

    Science.gov (United States)

    Zulfikri, Habiburrahman; Amovilli, Claudio; Filippi, Claudia

    2016-03-08

    We introduce a novel class of local multideterminant Jastrow-Slater wave functions for the efficient and accurate treatment of excited states in quantum Monte Carlo. The wave function is expanded as a linear combination of excitations built from multiple sets of localized orbitals that correspond to the bonding patterns of the different Lewis resonance structures of the molecule. We capitalize on the concept of orbital domains of local coupled-cluster methods, which is here applied to the active space to select the orbitals to correlate and construct the important transitions. The excitations are further grouped into classes, which are ordered in importance and can be systematically included in the Jastrow-Slater wave function to ensure a balanced description of all states of interest. We assess the performance of the proposed wave function in the calculation of vertical excitation energies and excited-state geometry optimization of retinal models whose π → π* state has a strong intramolecular charge-transfer character. We find that our multiresonance wave functions recover the reference values of the total energies of the ground and excited states with only a small number of excitations and that the same expansion can be flexibly used at very different geometries. Furthermore, significant computational saving can also be gained in the orbital optimization step by selectively mixing occupied and virtual orbitals based on spatial considerations without loss of accuracy on the excitation energy. Our multiresonance wave functions are therefore compact, accurate, and very promising for the calculation of multiple excited states of different character in large molecules.

  15. Dual-modality photothermal optical coherence tomography and magnetic-resonance imaging of carbon nanotubes.

    Science.gov (United States)

    Tucker-Schwartz, Jason M; Hong, Tu; Colvin, Daniel C; Xu, Yaqiong; Skala, Melissa C

    2012-03-01

    We demonstrate polyethylene-glycol-coated single-walled carbon nanotubes (CNTs) as contrast agents for both photothermal optical coherence tomography (OCT) and magnetic-resonance imaging (MRI). Photothermal OCT was accomplished with a spectral domain OCT system with an amplitude-modulated 750 nm pump beam using 10 mW of power, and T(2) MRI was achieved with a 4.7 T animal system. Photothermal OCT and T(2) MRI achieved sensitivities of nanomolar concentrations to CNTs dispersed in amine-terminated polyethylene glycol, thus establishing the potential for dual-modality molecular imaging with CNTs.

  16. Dual Modality Photothermal Optical Coherence Tomography and Magnetic Resonance Imaging of Carbon Nanotubes

    OpenAIRE

    Tucker – Schwartz, Jason M.; Hong, Tu; Colvin, Daniel C.; Xu, Yaqiong; Skala, Melissa C.

    2012-01-01

    We demonstrate polyethylene glycol coated single-walled carbon nanotubes (CNTs) as contrast agents for both photothermal optical coherence tomography (OCT) and magnetic resonance imaging. Photothermal OCT was accomplished with a spectral domain OCT system with an amplitude modulated 750 nm pump beam using 10 mW of power, and T2 MR imaging was achieved with a 4.7 T animal system. Photothermal OCT and T2 MR imaging achieved sensitivities of nM concentrations to CNTs dispersed in amine terminate...

  17. Resonant coherent ionization in grazing ion/atom-surface collisions at high velocities

    Energy Technology Data Exchange (ETDEWEB)

    Garcia de Abajo, F.J. (Dept. de Ciencias de la Computacion e Inteligencia Artificial, Facultad de Informatica, Univ. del Pais Vasco, San Sebastian (Spain)); Pitarke, J.M. (Materia Kondentsatuaren Fisika Saila, Zientzi Fakultatea, Euskal Herriko Univ., Bilbo (Spain))

    1994-05-01

    The resonant coherent interaction of a fast ion/atom with an oriented crystal surface under grazing incidence conditions is shown to contribute significantly to ionize the probe for high enough velocities and motion along a random direction. The dependence of this process on both the distance to the surface and the velocity of the projectile is studied in detail. We focus on the case of hydrogen moving with a velocity above 2 a.u. Comparison with other mechanisms of charge transfer, such as capture from inner shells of the target atoms, permits us to draw some conclusions about the charge state of the outgoing projectiles. (orig.)

  18. Noise-Induced Bursting and Coherence Resonance in Minimal Cytosolic Ca2+ Oscillation Model

    Institute of Scientific and Technical Information of China (English)

    JIA Ya; YANG Li-Jian; WU Dan; LIU Quan; ZHAN Xuan

    2004-01-01

    @@ A stochastic calcium oscillation model based on the minimal calcium oscillation model is investigated by numerical computation. When the extracellular stimulation is sub-threshold and random, the oscillations of cytosolic calcium show complex behaviour: a bursting-like phenomenon induced by noise, that is, the phase of glomerate spikes are separated by phase of quiescence (but fluctuations in the baseline values of calcium with small amplitude during the silent phase), in a pattern that occurs at irregular inter,ls. By using the histogram of interspike intervals of calcium concentration spikes, it is found that the noise-induced coherence resonance phenomenon occurs at the cellular level.

  19. Excitation of Giant Monopole Resonance in $^{208}$Pb and $^{116}$Sn Using Inelastic Deuteron Scattering

    CERN Document Server

    Patel, D; Itoh, M; Akimune, H; Berg, G P A; Fujiwara, M; Harakeh, M N; Iwamoto, C; Kawabata, T; Kawase, K; Matta, J T; Murakami, T; Okamoto, A; Sako, T; Schlax, K W; Takahashi, K; White, M; Yosoi, M

    2014-01-01

    The excitation of the isoscalar giant monopole resonance (ISGMR) in $^{116}$Sn and $^{208}$Pb has been investigated using small-angle (including $0^\\circ$) inelastic scattering of 100 MeV/u deuteron and multipole-decomposition analysis (MDA). The extracted strength distributions agree well with those from inelastic scattering of 100 MeV/u $\\alpha$ particles. These measurements establish deuteron inelastic scattering at E$_d \\sim$ 100 MeV/u as a suitable probe for extraction of the ISGMR strength with MDA, making feasible the investigation of this resonance in radioactive isotopes in inverse kinematics.

  20. Resonant transfer and excitation in Li-like F colliding with H/sub 2/

    Energy Technology Data Exchange (ETDEWEB)

    Schulz, M.; Schuch, R.; Datz, S.; Justiniano, E.L.B.; Miller, P.D.; Schoene, H.

    1988-11-15

    We have measured conicidences between x rays and projectiles that have captured one electron in F/sup 6+/+H/sub 2/ collisions at projectile energies between 15 and 33 MeV. The cross sections for capture and simultaneous x-ray emission as a function of projectile energy show clear structures. Indications of an unexpectedly high population of high-n states predominantly formed by resonant transfer and excitation (RTE) was found. Above the KLn (n>1) RTE resonance energies another maximum was observed.

  1. Carrier concentration dependence of the tunability of the dipole resonance peak in optically excited metamaterials

    Science.gov (United States)

    Chatzakis, Ioannis; Luo, Liang; Wang, Jigang; Shen, Nian Hai; Koschny, Thomas; Soukoulis, Costas

    2011-03-01

    Currently, there is strong interest to explore the dynamic control of the electromagnetic properties of metamaterials, which have important implications on their optoelectronic applications. While the design, fabrication and photo-doping of metamaterial/semiconductor structures have been actively pursued, some fundamental issues related to highly photo-excited states, their dynamic tuning and temporal evolution remain open. Using optical-pump terahertz probe spectroscopy, we report on the pump fluence dependence of the electric dipole resonance tunability in metamaterials. We find a previously undiscovered large non-monotonic variation on the strength of the dipole resonance peak with the photo-injected carrier concentration.

  2. The dissipative non-local oscillator in resonance with a periodic excitation

    Energy Technology Data Exchange (ETDEWEB)

    Maccari, A. [Istituto Tecnico `G. Cardano`, Monterotondo, Rome (Italy)

    1996-10-01

    The most important characteristic of a non-local and non-linear oscillator in resonance or in quasi-resonance with a periodic excitation are extensively examined by means of a new asymptotic perturbation method. The resultant motion is periodic or quasi-periodic, because in certain cases a motion given by the interference of even three different frequencies is observed. Comparison with the results deriving from the numerical integration confirms the validity of the asymptotic perturbation method employed in the calculation of the solution.

  3. Decay of the resonance fluorescence following pulsed excitation of a weakly disordered excitonic system

    Science.gov (United States)

    Boukahil, A.; Huber, D. L.

    1993-12-01

    A study is made of the decay of the resonance fluorescence following pulsed excitation of a weakly disordered system whose optical excitations are Frenkel excitons. The disorder is characterized by a Gaussian distribution of optical transition frequencies with no correlation between different sites. The duration of the resonant pulse is taken to be short in comparison with the reciprocal of the optical linewidth, and the wavelength of the light is assumed to be large in comparison with either the size of the array or the exciton mean free path associated with the disorder. In the limit where σ, the standard deviation of the Gaussian distribution, is much less than the exciton bandwidth, the integrated intensity of the fluorescence decays non-exponentially and is characterized by universal functions of σ xt, where x= 4/3, 2, and 4 in one, two, and three dimensions, respectively. Analytic approximations to the scaling functions in two and three dimensions are presented.

  4. The Giant Dipole Resonance built on highly excited states — results of the MEDEA experiment

    Science.gov (United States)

    Suomijärvi, T.; Le Faou, J. H.; Blumenfeld, Y.; Piattelli, P.; Agodi, C.; Alamanos, N.; Alba, R.; Auger, F.; Bellia, G.; Chomaz, Ph.; Coniglione, R.; Del Zoppo, A.; Finocchiaro, P.; Frascaria, N.; Gaardhøje, J. J.; Garron, J. P.; Gillibert, A.; Lamehi-Rachti, M.; Liguori-Neto, R.; Maiolino, C.; Migneco, E.; Russo, G.; Roynette, J. C.; Santonocito, D.; Sapienza, P.; Scarpaci, J. A.; Smerzi, A.

    1994-03-01

    Gamma-rays, light charged particles and evaporation residues emitted from hot nuclei formed in the 36Ar + 90Zr reaction at 27 MeV/u have been measured with a nearly 4π barium fluoride multidetector. It is shown that hot Sn-like nuclei with a range of excitation energies between 300 and 600 MeV are produced. The γ-ray yield from the decay of the Giant Dipole Resonance in these nuclei is shown to remain constant over this excitation energy range. The measured γ-ray spectra are compared with statistical calculations encompassing several recent theoretical models for the quenching of gamma-ray emission from the dipole resonance at very high temperatures.

  5. Parametric resonance of flexible footbridges under crowd-induced lateral excitation

    Science.gov (United States)

    Piccardo, Giuseppe; Tubino, Federica

    2008-03-01

    The excessive lateral sway motion caused by crowds walking across footbridges has attracted great public attention in the past few years. Three possible mechanisms responsible for such lateral vibrations have been investigated in the literature: direct resonance, dynamic interaction, and internal resonance. In this paper, starting from a critical review of the mechanisms proposed in the literature, a parametric excitation mechanism is analyzed, based on a forcing model whose amplitude is a function of deck oscillations. A stability criterion is identified, depending on the ratio between the structural and excitation frequencies, on the ratio of the structural and pedestrian masses, and on the structural damping. The proposed mechanism can be achieved for very flexible footbridges, with a lateral natural frequency around 0.5 Hz, corresponding to a half of the lateral walking frequency. This situation can occur in modern structures, such as in the case of the London Millennium Footbridge.

  6. Excited atoms in the free-burning Ar arc: treatment of the resonance radiation

    Science.gov (United States)

    Golubovskii, Yu; Kalanov, D.; Gortschakow, S.; Baeva, M.; Uhrlandt, D.

    2016-11-01

    The collisional-radiative model with an emphasis on the accurate treatment of the resonance radiation transport is developed and applied to the free-burning Ar arc plasma. This model allows for analysis of the influence of resonance radiation on the spatial density profiles of the atoms in different excited states. The comparison of the radial density profiles obtained using an effective transition probability approximation with the results of the accurate solution demonstrates the distinct impact of transport on the profiles and absolute densities of the excited atoms, especially in the arc fringes. The departures from the Saha-Boltzmann equilibrium distributions, caused by different radiative transitions, are analyzed. For the case of the DC arc, the local thermodynamic equilibrium (LTE) state holds close to the arc axis, while strong deviations from the equilibrium state on the periphery occur. In the intermediate radial positions the conditions of partial LTE are fulfilled.

  7. Small amplitude Dynamic AFM: quantifying interactions with different tip detection and excitation schemes in presence of additional resonances

    CERN Document Server

    Costa, Luca

    2014-01-01

    Quantifying the tip-sample interaction at the nanoscale in Amplitude Modulation mode AFM is challenging, especially when measuring in liquids. Here, we derive formulas for the tip-sample conservative and dissipative interactions and investigate the effect that spurious resonances have on the measured interaction. Both direct and acoustic excitation are considered. We also highlight the differences between measuring directly the tip position or the cantilever deflection. We show that, when probing the tip-sample forces, the acoustically excited cantilever behavior is insensitive to spurious resonances as long as the measured signal corresponds to the tip position, or if the excitation force is correctly taken into account. Since the effective excitation force may depend on the presence of such spurious resonances, we consider the cases where the frequency is kept constant during the measurement so that the proportionality between excitation signal and actual excitation force is kept constant. With the present ...

  8. Coherent Perfect Absorption induced by the nonlinearity of a Helmholtz resonator

    CERN Document Server

    Achilleos, V; Theocharis, G

    2016-01-01

    In this work, we analytically report Coherent Perfect Absorption induced by the acoustic nonlinear response of a Helmholtz Resonator side loaded to a waveguide. In particular, we show that this two-port acoustic system can perfectly absorb two high amplitude symmetric incident waves when the additive nonlinear losses in the HR, induced by the jet flow separation, together with the weak linear viscothermal losses of the HR balance the radiation losses to the waveguide. For the case of the one-sided incidence configuration, this condition leads to an absorption equal to 0.5. This result, which is verified experimentally, is in a good agreement with an analytical nonlinear model of the impedance of the HR. The nonlinear control of perfect absorption using resonators will open new possibilities in the design of high amplitude sound attenuators for aero-engine applications.

  9. Two types of coherence resonance in an intracellular calcium oscillation system

    Science.gov (United States)

    Ma, Juan; Gao, Qingyu

    2017-09-01

    Two types of noise induced oscillations (NIOs) near Hopf bifurcation and coherence resonance (CR) have been studied analytically in a calcium system. One is NIOs with small amplitude and internal signal stochastic resonance (CR type I) occurs, and the other is noise induced spike and the regularity of which reaches a maximum at an optimal noise level (CR type II). For the first type, stochastic normal form theory is employed to analyze the signal to noise ratio of the NIOs depending on the noise intensity. For the second type, based on the independent assumption, activation time and excursion time have been split, and the sum of which reach a minimum with the variation of noise intensity. The theoretical evidence is also explained in detail. Numerical simulations show good agreements with the theoretical results. It may indicate some kind of transmit mechanism involved in stochastic calcium dynamics.

  10. Frequency Stability of Atomic Clocks Based on Coherent Population Trapping Resonance in 85Rb

    Institute of Scientific and Technical Information of China (English)

    LIU Lu; GUO Tao; DENG Ke; LIU Xin-Yuan; CHEN Xu-Zong; WANG Zhong

    2007-01-01

    An atomic clock system based on coherent population trapping (CPT) resonance in 85Rb is reported, while most past works about the CPT clock are in 87Rb. A new modulation method (full-hyperfine-frequency-splitting modulation) is presented to reduce the effect of light shift to improve the frequency stability of the CPT clock in 85Rb. The experimental results show that the short-term frequency stability of the CPT clock in 85Rb is in the order of 10-10/s and the long-term frequency stability can achieve 1.5 × 10-11 /80000s, which performs as well as 87Rb in CPT resonance. This very good frequency stability performance associated with the low-cost and low-power properties of 85Rb indicates that an atomic clock based on CPT in 85 Rb should be a promising candidate for making the chip scale atomic clock.

  11. Ultrafast spectral interferometry of resonant secondary emmission from semiconductor quantum wells

    DEFF Research Database (Denmark)

    Birkedal, Dan; Shah, Jagdeep

    1999-01-01

    Recent investigations of secondary emission from quantum well excitons follwing resonant excitation have demonstrated an intricate interplay of coherent Rayleigh scattering and incoherent luminescence. We have very recently demonstrated that it is possible to isolate and time resolve the coherent...

  12. Low lying excitations in odd deformed nucleus studied by nuclear resonance fluorescence

    Energy Technology Data Exchange (ETDEWEB)

    Pinto, A.E. Almeida [Sao Paulo Univ., SP (Brazil). Inst. de Fisica; Margraf, J.; Nord, A. [Stuttgart Univ. (Germany). Inst. fuer Strahlenphysik] [and others

    1997-12-31

    Nuclear resonance fluorescence experiment was performed on {sup 153} Eu using the Bremsstrahlung beam of the Stuttgart Dynamitron and high resolution Ge-{gamma}-spectrometers. Detailed information was obtained on excitation energies, decay widths, transition probabilities, and branching ratios to study the fragmentation of the M1 scissors mode, and try establishing a systematics to explain the different fragmentation behavior of the dipole strengths in the odd isotopes recently studied. (author) 11 refs., 1 fig.; emilia at axpfep1.if.usp.br

  13. Stimulated excitation of resonant Cherenkov radiation at a large number of neighbouring waveguide modes

    CERN Document Server

    Grigoryan, L Sh; Khachatryan, H F; Grigoryan, M L

    2012-01-01

    The resonance Cherenkov radiation generated from a train of equally-spaced unidimensional electron bunches travelling along the axis of a hollow channel inside an infinite cylindrical waveguide filled with (weakly dispersing) transparent dielectric has been investigated. It was shown that its excitation might be stimulated at a large number of neighboring modes of the waveguide. A visual explanation of this effect is given and the possibility of its observation in the range of terahertz radiation is discussed.

  14. Coherence and population dynamics of chlorophyll excitations in FCP complex: Two-dimensional spectroscopy study

    CERN Document Server

    Butkus, Vytautas; Augulis, Ramūnas; Gall, Andrew; Büchel, Claudia; Robert, Bruno; Zigmantas, Donatas; Valkunas, Leonas; Abramavicius, Darius

    2015-01-01

    The energy transfer processes and coherent phenomena in the fucoxanthin-chlorophyll protein complex, which is responsible for the light harvesting function in marine algae diatoms, were investigated at 77 K by using two-dimensional electronic spectroscopy. Experiments performed on the femtosecond and picosecond timescales led to separation of spectral dynamics, witnessing evolutions of coherence and population states of the system in the spectral region of ${\\rm Q}_{y}$ transitions of chlorophylls $a$ and $c$. Analysis of the coherence dynamics allowed us to identify chlorophyll (Chl) $a$ and fucoxanthin intramolecular vibrations dominating over the first few picoseconds. Closer inspection of the spectral region of the ${\\rm Q}_{y}$ transition of Chl $c$ revealed previously not identified mutually non-interacting chlorophyll $c$ states participating in femtosecond or picosecond energy transfer to the Chl $a$ molecules. Consideration of separated coherent and incoherent dynamics allowed us to hypothesize the v...

  15. High-resolution magnetic resonance spectroscopy in unstable fields via intermolecular zero-quantum coherences.

    Science.gov (United States)

    Lin, Meijin; Chen, Xi; Cai, Shuhui; Chen, Zhong

    2010-06-21

    Intermolecular zero-quantum coherences (iZQCs) have been utilized to achieve high-resolution nuclear magnetic resonance (NMR) proton spectra under inhomogeneous and/or unstable fields. In this paper, we demonstrated that despite the insensitivity of iZQCs to B(0) variations, the influence of unstable fields on the observable single-quantum coherence signals causes strong t(1) noises in the high-resolution iZQC spectra. Short-time acquisition (STA) and phase spectrum schemes were proposed for noise suppression in in vivo iZQC magnetic resonance spectroscopy (MRS) under temporal B(0) variations. The feasibility of these schemes were verified by localized spectroscopic studies under B(0) variations generated by the Z0 coil current oscillations and by voxel position variations in the presence of field gradients, which simulate the field conditions of MRS in the presence of physiological motions. The phase scheme not only improves the signal-to-noise ratio but also further reduces the linewidth by half.

  16. Delay-induced coherence bi-resonance-like behavior in stochastic Hodgkin-Huxley neuron networks

    Institute of Scientific and Technical Information of China (English)

    2010-01-01

    In this paper,we study how information transmission delays affect the spiking behavior of electrically coupled stochastic Hodgkin-Huxley (HH) neurons on Newman-Watts networks.It is found that the spiking behavior becomes the most regular at an optimal time delay,indicating the occurrence of delay-induced coherence resonance-like (CR-like) behavior.Interestingly,there are different CR-like types,depending on the membrane patch size of the neuron.For a smaller patch size,only single CR-like behavior occurs;while for a larger patch size,coherence bi-resonance-like (CBR) behavior appears.These findings show that the delay-induced CR-like behavior is closely related to the channel noise strength,and the coupled neurons may exhibit different spiking behaviors under the interplay of the channel noise and time delay.Therefore,the channel noise should be taken into account in the study of time delay-related spiking activity in stochastic HH neurons.This work provides new insight into the role of channel noise and information transmission delays in realistic neural systems.

  17. Enhanced photoelectric detection of NV magnetic resonances in diamond under dual-beam excitation

    Science.gov (United States)

    Bourgeois, E.; Londero, E.; Buczak, K.; Hruby, J.; Gulka, M.; Balasubramaniam, Y.; Wachter, G.; Stursa, J.; Dobes, K.; Aumayr, F.; Trupke, M.; Gali, A.; Nesladek, M.

    2017-01-01

    The core issue for the implementation of NV center qubit technology is a sensitive readout of the NV spin state. We present here a detailed theoretical and experimental study of NV center photoionization processes, used as a basis for the design of a dual-beam photoelectric method for the detection of NV magnetic resonances (PDMR). This scheme, based on NV one-photon ionization, is significantly more efficient than the previously reported single-beam excitation scheme. We demonstrate this technique on small ensembles of ˜10 shallow NVs implanted in electronic grade diamond (a relevant material for quantum technology), on which we achieve a cw magnetic resonance contrast of 9%—three times enhanced compared to previous work. The dual-beam PDMR scheme allows independent control of the photoionization rate and spin magnetic resonance contrast. Under a similar excitation, we obtain a significantly higher photocurrent, and thus an improved signal-to-noise ratio, compared to single-beam PDMR. Finally, this scheme is predicted to enhance magnetic resonance contrast in the case of samples with a high proportion of substitutional nitrogen defects, and could therefore enable the photoelectric readout of single NV spins.

  18. Quanty for core level spectroscopy - excitons, resonances and band excitations in time and frequency domain

    Science.gov (United States)

    Haverkort, Maurits W.

    2016-05-01

    Depending on the material and edge under consideration, core level spectra manifest themselves as local excitons with multiplets, edge singularities, resonances, or the local projected density of states. Both extremes, i.e., local excitons and non-interacting delocalized excitations are theoretically well under control. Describing the intermediate regime, where local many body interactions and band-formation are equally important is a challenge. Here we discuss how Quanty, a versatile quantum many body script language, can be used to calculate a variety of different core level spectroscopy types on solids and molecules, both in the frequency as well as the time domain. The flexible nature of Quanty allows one to choose different approximations for different edges and materials. For example, using a newly developed method merging ideas from density renormalization group and quantum chemistry [1-3], Quanty can calculate excitons, resonances and band-excitations in x-ray absorption, photoemission, x-ray emission, fluorescence yield, non-resonant inelastic x-ray scattering, resonant inelastic x-ray scattering and many more spectroscopy types. Quanty can be obtained from: http://www.quanty.org.

  19. Acoustic resonance excitation of turbulent heat transfer and flow reattachment downstream of a fence

    Science.gov (United States)

    Selcan, Claudio; Cukurel, Beni; Shashank, Judah

    2016-10-01

    The current work investigates the aero-thermal impact of standing sound waves, excited in a straight channel geometry, on turbulent, separating and reattaching flow over a fence. Effects of distinct frequency resonant forcing (ReH = 10,050 and f = 122 Hz) are quantified by wall static pressure measurements and detailed convective heat transfer distributions via liquid crystal thermometry. Acoustic boundary conditions are numerically predicted and the computed longitudinal resonance mode shapes are experimentally verified by surface microphone measurements. Findings indicate the presence of a resonant sound field to exert strong influence on local heat transfer downstream of the fence, whereas the boundary layer upstream of the obstacle remains notable unaffected. Upstream shift of the maximum heat transfer location and an earlier pressure recovery indicate a reduction in time averaged flow reattachment length of up to 37 %. Although the streamwise peak Nusselt increased by only 5 %, the heat transfer level in the vicinity of the unexcited reattachment zone was locally enhanced up to 25 %. Despite prominent impact of resonant forcing on the fence wake flow, the total pressure drop penalty remained invariant. Observations demonstrate the significant aero-thermal implications of shear layer excitation by standing sound waves superimposed on the channel flow field.

  20. Resonance Raman enhancement optimization in the visible range by selecting different excitation wavelengths.

    Science.gov (United States)

    Wang, Zhong; Li, Yuee

    2015-09-01

    Resonance enhancement of Raman spectroscopy (RS) has been used to significantly improve the sensitivity and selectivity of detection for specific components in complicated environments. Resonance RS gives more insight into the biochemical structure and reactivity. In this field, selecting a proper excitation wavelength to achieve optimal resonance enhancement is vital for the study of an individual chemical/biological ingredient with a particular absorption characteristic. Raman spectra of three azo derivatives with absorption spectra in the visible range are studied under the same experimental conditions at 488, 532, and 633 nm excitations. Universal laws in the visible range have been concluded by analyzing resonance Raman (RR) spectra of samples. The long wavelength edge of the absorption spectrum is a better choice for intense enhancement and the integrity of a Raman signal. The obtained results are valuable for applying RR for the selective detection of biochemical constituents whose electronic transitions take place at energies corresponding to the visible spectra, which is much friendlier to biologial samples compared to ultraviolet.

  1. Electron Cloud Density Measurements in Accelerator Beam-pipe Using Resonant Microwave Excitation

    CERN Document Server

    Sikora, John P

    2013-01-01

    An accelerator beam can generate low energy electrons in the beam-pipe, generally called electron cloud, that can produce instabilities in a positively charged beam. One method of measuring the electron cloud density is by coupling microwaves into and out of the beam-pipe and observing the response of the microwaves to the presence of the electron cloud. This paper describes a technique in which the beam-pipe is resonantly excited with microwaves and the electron cloud density calculated from the change that it produces in the resonant frequency of the beam-pipe. The resonant technique has the advantage that measurements can be localized to sections of beam-pipe that are a meter or less in length, as well as greatly improving the signal to noise ratio.

  2. Realistic vs sudden turn-on of natural incoherent light: Coherences and dynamics in molecular excitation and internal conversion

    Energy Technology Data Exchange (ETDEWEB)

    Grinev, Timur; Brumer, Paul [Chemical Physics Theory Group, Department of Chemistry, and Center for Quantum Information and Quantum Control, University of Toronto, Toronto, Ontario M5S 3H6 (Canada)

    2015-12-28

    Molecular excitation with incoherent light is examined using realistic turn-on time scales, and results are compared to those obtained via commonly used sudden turn-on, or pulses. Two significant results are obtained. First, in contrast to prior studies involving sudden turn-on, realistic turn-on is shown to lead to stationary coherences for natural turn-on time scales. Second, the time to reach the final stationary mixed state, known to result from incoherent excitation, is shown to depend directly on the inverse of the molecular energy level spacings, in both sudden and realistic turn-on cases. The S{sub 0} → S{sub 2}/S{sub 1} internal conversion process in pyrazine is used as an example throughout. Implications for studies of natural light harvesting systems are noted.

  3. Realistic vs sudden turn-on of natural incoherent light: Coherences and dynamics in molecular excitation and internal conversion.

    Science.gov (United States)

    Grinev, Timur; Brumer, Paul

    2015-12-28

    Molecular excitation with incoherent light is examined using realistic turn-on time scales, and results are compared to those obtained via commonly used sudden turn-on, or pulses. Two significant results are obtained. First, in contrast to prior studies involving sudden turn-on, realistic turn-on is shown to lead to stationary coherences for natural turn-on time scales. Second, the time to reach the final stationary mixed state, known to result from incoherent excitation, is shown to depend directly on the inverse of the molecular energy level spacings, in both sudden and realistic turn-on cases. The S0 → S2/S1 internal conversion process in pyrazine is used as an example throughout. Implications for studies of natural light harvesting systems are noted.

  4. Femtosecond Twisting and Coherent Vibrational Motion in the Excited State of Tetraphenylethylene

    NARCIS (Netherlands)

    Lenderink, E; Duppen, K.; Wiersma, D. A.

    1995-01-01

    The initial dynamics after excitation to the S-1 state of tetraphenylethylene is studied using femtosecond pump-probe spectroscopy. From the rapid spectral changes during the first few hundred femtoseconds, we conclude that a fast ethylenic twisting motion occurs in the excited state within this tim

  5. Decay and coherence of two-photon excited yellow orthoexcitons in Cu2O

    NARCIS (Netherlands)

    Karpinska, Katarzyna; Mostovoy, M; van der Vegte, MA; Revcolevschi, A; van Loosdrecht, PHM

    2005-01-01

    Photoluminescence excitation spectroscopy has revealed a highly efficient two-photon excitation method to produce a cold, uniformly distributed high density excitonic gas in bulk cuprous oxide. A study of the time evolution of the density, temperature, and chemical potential of the exciton gas shows

  6. Coherence and population dynamics of chlorophyll excitations in FCP complex: Two-dimensional spectroscopy study

    Energy Technology Data Exchange (ETDEWEB)

    Butkus, Vytautas; Gelzinis, Andrius; Valkunas, Leonas [Department of Theoretical Physics, Faculty of Physics, Vilnius University, Sauletekio Ave. 9-III, 10222 Vilnius (Lithuania); Center for Physical Sciences and Technology, Savanoriu Ave. 231, 02300 Vilnius (Lithuania); Augulis, Ramūnas [Center for Physical Sciences and Technology, Savanoriu Ave. 231, 02300 Vilnius (Lithuania); Gall, Andrew; Robert, Bruno [Institut de Biologie et Technologies de Saclay, Bât 532, Commissariat à l’Energie Atomique Saclay, 91191 Gif sur Yvette (France); Büchel, Claudia [Institut für Molekulare Biowissenschaften, Universität Frankfurt, Max-von-Laue-Straße 9, Frankfurt (Germany); Zigmantas, Donatas [Department of Chemical Physics, Lund University, P.O. Box 124, 22100 Lund (Sweden); Abramavicius, Darius, E-mail: darius.abramavicius@ff.vu.lt [Department of Theoretical Physics, Faculty of Physics, Vilnius University, Sauletekio Ave. 9-III, 10222 Vilnius (Lithuania)

    2015-06-07

    Energy transfer processes and coherent phenomena in the fucoxanthin–chlorophyll protein complex, which is responsible for the light harvesting function in marine algae diatoms, were investigated at 77 K by using two-dimensional electronic spectroscopy. Experiments performed on femtosecond and picosecond timescales led to separation of spectral dynamics, witnessing evolutions of coherence and population states of the system in the spectral region of Q{sub y} transitions of chlorophylls a and c. Analysis of the coherence dynamics allowed us to identify chlorophyll (Chl) a and fucoxanthin intramolecular vibrations dominating over the first few picoseconds. Closer inspection of the spectral region of the Q{sub y} transition of Chl c revealed previously not identified, mutually non-interacting chlorophyll c states participating in femtosecond or picosecond energy transfer to the Chl a molecules. Consideration of separated coherent and incoherent dynamics allowed us to hypothesize the vibrations-assisted coherent energy transfer between Chl c and Chl a and the overall spatial arrangement of chlorophyll molecules.

  7. Spatial Coherence Properties of Organic Molecules Coupled to Plasmonic Surface Lattice Resonances in the Weak and Strong Coupling Regimes

    CERN Document Server

    Shi, L; Rekola, H T; Martikainen, J -P; Moerland, R J; Törmä, P

    2014-01-01

    We study spatial coherence properties of a system composed of periodic silver nanoparticle arrays covered with a fluorescent organic molecule (DiD) film. The evolution of spatial coherence of this composite structure from the weak to the strong coupling regime is investigated by systematically varying the coupling strength between the localized DiD excitons and the collective, delocalized modes of the nanoparticle array known as surface lattice resonances. A gradual evolution of coherence from the weak to the strong coupling regime is observed, with the strong coupling features clearly visible in interference fringes. A high degree of spatial coherence is demonstrated in the strong coupling regime, even when the mode is very excitonlike (80%), in contrast to the purely localized nature of molecular excitons. We show that coherence appears in proportion to the weight of the plasmonic component of the mode throughout the weak-to-strong coupling crossover, providing evidence for the hybrid nature of the normal m...

  8. Resonant Transparency and Non-Trivial Non-Radiating Excitations in Toroidal Metamaterials

    Science.gov (United States)

    Fedotov, V. A.; Rogacheva, A. V.; Savinov, V.; Tsai, D. P.; Zheludev, N. I.

    2013-01-01

    Engaging strongly resonant interactions allows dramatic enhancement of functionalities of many electromagnetic devices. However, resonances can be dampened by Joule and radiation losses. While in many cases Joule losses may be minimized by the choice of constituting materials, controlling radiation losses is often a bigger problem. Recent solutions include the use of coupled radiant and sub-radiant modes yielding narrow asymmetric Fano resonances in a wide range of systems, from defect states in photonic crystals and optical waveguides with mesoscopic ring resonators to nanoscale plasmonic and metamaterial systems exhibiting interference effects akin to electromagnetically-induced transparency. Here we demonstrate theoretically and confirm experimentally a new mechanism of resonant electromagnetic transparency, which yields very narrow isolated symmetric Lorentzian transmission lines in toroidal metamaterials. It exploits the long sought non-trivial non-radiating charge-current excitation based on interfering electric and toroidal dipoles that was first proposed by Afanasiev and Stepanovsky in [J. Phys. A Math. Gen. 28, 4565 (1995)]. PMID:24132231

  9. Excitation of the Roper resonance in single- and double-pion production

    Energy Technology Data Exchange (ETDEWEB)

    Skorodko, T.; Clement, H.; Bashkanov, M.; Doroshkevich, E.; Khakimova, O.; Kren, F.; Wagner, G. [Physikalisches Inst., Univ. Tuebingen (Germany); Kaskulov, M. [Inst. fuer Theoretische Physik, Univ. Giessen (Germany)

    2007-07-01

    The Roper resonance has been a puzzle ever since its detection in {pi}N phase shifts. In most investigations no apparent resonance signatures could be found in the observables. Not only its nature has been a matter of permanent debate, also its resonance parameters show a big scatter in their values. In the pp {yields} np{pi}{sup +} reaction measured at CELSIUS-WASA at several energies a pronounced resonance structure at M{sub n{pi}{sup +}} {approx} 1350 MeV with {gamma} {approx} 140 MeV has been found. These numbers agree very favourably with recent SAID {pi}N phase shift results for the Roper pole as well as with the very recent BES results from J/{psi} {yields} NN*. With the pole position being roughly 100 MeV below the previously believed value of the N*(1440), also its decay branchings (defined at the pole position) change dramatically. From near-threshold two-pion production, when Roper excitation is the only significant process, we find the decay N* {yields} N{sigma} to be the by far dominant process pointing to a breathing mode nature of the Roper resonance. (orig.)

  10. Shifted excitation resonance Raman difference spectroscopy using a microsystem light source at 488 nm

    Science.gov (United States)

    Maiwald, M.; Sowoidnich, K.; Schmidt, H.; Sumpf, B.; Erbert, G.; Kronfeldt, H.-D.

    2010-04-01

    Experimental results in shifted excitation resonance Raman difference spectroscopy (SERRDS) at 488 nm will be presented. A novel compact diode laser system was used as excitation light source. The device is based on a distributed feedback (DFB) diode laser as a pump light source and a nonlinear frequency doubling using a periodically poled lithium niobate (PPLN) waveguide crystal. All elements including micro-optics are fixed on a micro-optical bench with a footprint of 25 mm × 5 mm. An easy temperature management of the DFB laser and the crystal was used for wavelength tuning. The second harmonic generation (SHG) provides an additional suppression of the spontaneous emission. Raman spectra of polystyrene demonstrate that no laser bandpass filter is needed for the Raman experiments. Resonance-Raman spectra of the restricted food colorant Tartrazine (FD&C Yellow 5, E 102) in distilled water excited at 488 nm demonstrate the suitability of this light source for SERRDS. A limit of detection (LOD) of 0.4 μmol.l-1 of E102 enables SERRDS at 488 nm for trace detection in e.g. food safety control as an appropriate contactless spectroscopic technique.

  11. 4 f excitations in Ce Kondo lattices studied by resonant inelastic x-ray scattering

    Science.gov (United States)

    Amorese, A.; Dellea, G.; Fanciulli, M.; Seiro, S.; Geibel, C.; Krellner, C.; Makarova, I. P.; Braicovich, L.; Ghiringhelli, G.; Vyalikh, D. V.; Brookes, N. B.; Kummer, K.

    2016-04-01

    The potential of resonant inelastic soft x-ray scattering to measure 4 f crystal electric-field excitation spectra in Ce Kondo lattices has been examined. Spectra have been obtained for several Ce systems and show a well-defined structure determined by crystal-field, spin-orbit, and charge-transfer excitations only. The spectral shapes of the excitation spectra can be well understood in the framework of atomic multiplet calculations. For CeCu2Si2 we found notable disagreement between the inelastic x-ray-scattering spectra and theoretical calculations when using the crystal-field scheme proposed from inelastic neutron scattering. Modified sets of crystal-field parameters yield better agreement. Our results also show that, with the very recent improvements of soft x-ray spectrometers in resolution to below 30 meV at the Ce M4 ,5 edges, resonant inelastic x-ray scattering could be an ideal tool to determine the crystal-field scheme in Ce Kondo lattices and other rare-earth compounds.

  12. Charge-resonance excitations in symmetric molecules - Comparison of linear response DFT with CC3 for the excited states of a model dimer

    DEFF Research Database (Denmark)

    Kuhlman, Thomas Scheby; Mikkelsen, Kurt V.; Møller, Klaus Braagaard;

    2009-01-01

    We present a study on the excited states of an ethylene dimer as to investigate the presence of and perturbation from low-lying charge-resonance states calculated by linear response density functional theory (DFT) using the B3LYP and CAM-B3LYP functionals. The calculations are compared to a refer......We present a study on the excited states of an ethylene dimer as to investigate the presence of and perturbation from low-lying charge-resonance states calculated by linear response density functional theory (DFT) using the B3LYP and CAM-B3LYP functionals. The calculations are compared...

  13. Coherent oscillations of electrons in tunnel-coupled wells under ultrafast intersubband excitation

    Energy Technology Data Exchange (ETDEWEB)

    Hernandez-Cabrera, A [Departamento de FIsica Basica, Universidad de La Laguna, La Laguna 38206-Tenerife, Canary Islands (Spain); Aceituno, P [Departamento de FIsica Basica, Universidad de La Laguna, La Laguna 38206-Tenerife, Canary Islands (Spain); Vasko, F T [Institute of Semiconductor Physics, NAS of Ukraine, Kiev, 252650 (Ukraine)

    2004-07-28

    Ultrafast intersubband excitation of electrons in tunnel-coupled wells is studied in respect of its dependence on the structure parameters, the duration of the infrared pump and the detuning frequency. The temporal dependences of the photoinduced carrier concentration and dipole moment are obtained for two cases of transitions: from the single ground state to the tunnel-coupled excited states and from the tunnel-coupled states to the single excited state. The peculiarities of dephasing and population relaxation processes are also taken into account. The nonlinear regime of the response is also considered when the splitting energy between the tunnel-coupled levels is renormalized by the photoexcited electron concentration. The dependences of the period and the amplitude of oscillations on the excitation pulse are presented with a description of the damping of the nonlinear oscillations.

  14. Coherent Motion Reveals Non‐Ergodic Nature of Internal Conversion between Excited States

    DEFF Research Database (Denmark)

    Kuhlman, Thomas Scheby; Sølling, Theis I.; Møller, Klaus Braagaard

    2012-01-01

    for smaller molecules. Specifically, we focus on the S2→S1 internal conversion in cyclobutanone, cyclopentanone, and cyclohexanone. By means of time‐resolved mass spectrometry and photoelectron spectroscopy the relative rate of this transition is determined to be 13:2:1. Remarkably, we observe coherent...

  15. Coherent population trapping resonances at lower atomic levels of Doppler broadened optical lines

    Energy Technology Data Exchange (ETDEWEB)

    Şahin, E; Hamid, R; Çelik, M [National Metrology Institute of Turkey, Gebze, Kocaeli (Turkey); Özen, G [Istanbul Technical University, Faculty of Science and Letters, Engineering Physics Department Maslak, Istanbul (Turkey); Izmailov, A Ch [Institute of Physics, Azerbaijan National Academy of Sciences, H. Javid av. 33, Baku, Az-1143 (Azerbaijan)

    2014-11-30

    We have detected and analysed narrow high-contrast coherent population trapping (CPT) resonances, which are induced in absorption of a weak monochromatic probe light beam by counterpropagating two-frequency pump radiation in a cell with rarefied caesium vapour. The experimental investigations have been performed by the example of nonclosed three level Λ-systems formed by spectral components of the D{sub 2} line of caesium atoms. The applied method allows one to analyse features of the CPT phenomenon directly at a given low long-lived level of the selected Λ-system even in sufficiently complicated spectra of atomic gases with large Doppler broadening. We have established that CPT resonances in transmission of the probe beam exhibit not only a higher contrast but also a much lesser width in comparison with well- known CPT resonances in transmission of the corresponding two-frequency pump radiation. The results obtained can be used in selective photophysics, photochemistry and ultra-high resolution atomic (molecular) spectroscopy. (laser applications and other topics in quantum electronics)

  16. Resonantly excited precession motion of three-dimensional vortex core in magnetic nanospheres [corrected].

    Science.gov (United States)

    Kim, Sang-Koog; Yoo, Myoung-Woo; Lee, Jehyun; Lee, Ha-Youn; Lee, Jae-Hyeok; Gaididei, Yuri; Kravchuk, Volodymyr P; Sheka, Denis D

    2015-01-01

    We found resonantly excited precession motions of a three-dimensional vortex core in soft magnetic nanospheres and controllable precession frequency with the sphere diameter 2R, as studied by micromagnetic numerical and analytical calculations. The precession angular frequency for an applied static field HDC is given as ωMV = γeffHDC, where γeff = γ〈mΓ〉 is the effective gyromagnetic ratio in collective vortex dynamics, with the gyromagnetic ratio γ and the average magnetization component 〈mΓ〉 of the ground-state vortex in the core direction. Fitting to the micromagnetic simulation data for 〈mΓ〉 yields a simple explicit form of 〈mΓ〉 ≈ (73.6 ± 3.4)(lex/2R)(2.20±0.14), where lex is the exchange length of a given material. This dynamic behavior might serve as a foundation for potential bio-applications of size-specific resonant excitation of magnetic vortex-state nanoparticles, for example, magnetic particle resonance imaging.

  17. Multi-mode excitation of a clamped–clamped microbeam resonator

    KAUST Repository

    Younis, Mohammad I.

    2015-02-18

    We present modeling and simulation of the nonlinear dynamics of a microresonator subjected to two-source electrostatic excitation. The resonator is composed of a clamped–clamped beam excited by a DC voltage load superimposed to two AC voltage loads of different frequencies. One frequency is tuned close to the first natural frequency of the beam and the other is close to the third (second symmetric) natural frequency. A multi-mode Galerkin procedure is applied to extract a reduced-order model, which forms the basis of the numerical simulations. Time history response, Poincare’ sections, Fast Fourier Transforms FFT, and bifurcation diagrams are used to reveal the dynamics of the system. The results indicate complex nonlinear phenomena, which include quasiperiodic motion, torus bifurcations, and modulated chaotic attractors.

  18. An optically detected magnetic resonance spectrometer with tunable laser excitation and wavelength resolved infrared detection

    CERN Document Server

    Negyedi, M; Gyüre, B; Dzsaber, S; Kollarics, S; Rohringer, P; Pichler, T; Simon, F

    2016-01-01

    We present the development and performance of an optically detected magnetic resonance (ODMR) spectrometer. The spectrometer represents advances over similar instruments in three areas: i) the exciting light is a tunable laser source which covers much of the visible light range, ii) the optical signal is analyzed with a spectrograph, iii) the emitted light is detected in the near-infrared domain. The need to perform ODMR experiments on single-walled carbon nanotubes motivated the present development and we demonstrate the utility of the spectrometer on this material. The performance of the spectrometer is critically compared to similar instruments. The present development opens the way to perform ODMR studies on various new materials such as molecules and luminescent quantum dots where the emission is in the near-infrared range and requires a well-defined excitation wavelength and analysis of the scattered light.

  19. Dual Strip-Excited Dielectric Resonator Antenna with Parasitic Strips for Radiation Pattern Reconfigurability

    Directory of Open Access Journals (Sweden)

    M. Kamran Saleem

    2014-01-01

    Full Text Available A novel pattern reconfigurable antenna concept utilizing rectangular dielectric resonator antenna (DRA placed over dielectric substrate backed by a ground plane is presented. A dual strip excitation scheme is utilized and both excitation strips are connected together by means of a 50 Ω microstrip feed network placed over the substrate. The four vertical metallic parasitic strips are placed at corner of DRA each having a corresponding ground pad to provide a short/open circuit between the parasitic strip and antenna ground plane, through which a shift of 90° in antenna radiation pattern in elevation plane is achieved. A fractional bandwidth of approximately 40% at center frequency of 1.6 GHz is achieved. The DRA peak realized gain in whole frequency band of operation is found to be above 4 dB. The antenna configuration along with simulation and measured results are presented.

  20. Coherent control of non-resonant two-photon transition in molecular system

    Institute of Scientific and Technical Information of China (English)

    Zhang Hui; Zhang Shi-An; Wang Zu-Geng; Sun Zhen-Rong

    2010-01-01

    In this paper,we study theoretically and experimentally the coherent control of non-resonant two-photon transition in a molecular system (Perylene dissolved in chloroform solution) by shaping the femtosecond pulses with simple phase patterns (cosinusoidal and π phase step-function shape).The control efficiency of the two-photon transition probability is correlated with both the laser field and the molecular absorption bandwidth.Our results demonstrate that,the two-photon transition probability in a molecular system can be reduced but not completely eliminated by manipulating the laser field,and the control efficiency is minimal when the molecular absorption bandwidth is larger than twice the laser spectral bandwidth.

  1. Coherent dynamical recoupling of diffusion-driven decoherence in magnetic resonance

    CERN Document Server

    Alvarez, Gonzalo A; Frydman, Lucio

    2013-01-01

    During recent years, dynamical decoupling (DD) has gained relevance as a tool for manipulating quantum systems and extracting information from them. This is particularly relevant for spins involved in nuclear magnetic resonance (NMR), where DD sequences can be used to prolong quantum coherences, or for selectively couple/decouple the effects imposed by random environmental fluctuations. In this Letter, we show that one can exploit these concepts in order to selectively recouple diffusion processes in restricted spaces. The ensuing method provides a novel tool to measure restriction lengths in confined systems such as capillaries, pores or cells. The principles of this method for selectively recoupling diffusion-driven decoherence, its standing within the context of diffusion NMR, and corroborating experiments, are presented.

  2. Multidimensional resonant nonlinear spectroscopy with coherent broadband x-ray pulses

    Science.gov (United States)

    Bennett, Kochise; Zhang, Yu; Kowalewski, Markus; Hua, Weijie; Mukamel, Shaul

    2016-12-01

    New x-ray free electron laser (XFEL) and high harmonic generation (HHG) light sources are capable of generating short and intense pulses that make x-ray nonlinear spectroscopy possible. Multidimensional spectroscopic techniques, which have long been used in the nuclear magnetic resonance, infrared, and optical regimes to probe the electronic structure and nuclear dynamics of molecules by sequences of short pulses with variable delays, can thus be extended to the attosecond x-ray regime. This opens up the possibility of probing core-electronic structure and couplings, the real-time tracking of impulsively created valence-electronic wavepackets and electronic coherences, and monitoring ultrafast processes such as nonadiabatic electron-nuclear dynamics near conical-intersection crossings. We survey various possible types of multidimensional x-ray spectroscopy techniques and demonstrate the novel information they can provide about molecules.

  3. Exploring Electrical and Magnetic Resonances from Coherently Correlated Long-Lived Radical Pairs towards Development of Negative Refractive-Index Materials

    Science.gov (United States)

    2015-01-03

    Resonances from Coherently Correlated Long-Lived Radical Pairs towards Development of Negative Refractive - Index materials Grant/Contract Number AFOSR... Refractive - Index Materials Subtitle: Task 1: Radicals Based Molecular Metamaterials Task 2: Thin-Film Based Polymer Thermoelectric Devices 5a...and Magnetic Resonances from Coherently Correlated Long-Lived Radical Pairs towards Development of Negative - Index Materials Principle Investigator

  4. "Parallel factor analysis of multi-excitation ultraviolet resonance Raman spectra for protein secondary structure determination".

    Science.gov (United States)

    Oshokoya, Olayinka O; JiJi, Renee D

    2015-09-10

    Protein secondary structural analysis is important for understanding the relationship between protein structure and function, or more importantly how changes in structure relate to loss of function. The structurally sensitive protein vibrational modes (amide I, II, III and S) in deep-ultraviolet resonance Raman (DUVRR) spectra resulting from the backbone C-O and N-H vibrations make DUVRR a potentially powerful tool for studying secondary structure changes. Experimental studies reveal that the position and intensity of the four amide modes in DUVRR spectra of proteins are largely correlated with the varying fractions of α-helix, β-sheet and disordered structural content of proteins. Employing multivariate calibration methods and DUVRR spectra of globular proteins with varying structural compositions, the secondary structure of a protein with unknown structure can be predicted. A disadvantage of multivariate calibration methods is the requirement of known concentration or spectral profiles. Second-order curve resolution methods, such as parallel factor analysis (PARAFAC), do not have such a requirement due to the "second-order advantage." An exceptional feature of DUVRR spectroscopy is that DUVRR spectra are linearly dependent on both excitation wavelength and secondary structure composition. Thus, higher order data can be created by combining protein DUVRR spectra of several proteins collected at multiple excitation wavelengths to give multi-excitation ultraviolet resonance Raman data (ME-UVRR). PARAFAC has been used to analyze ME-UVRR data of nine proteins to resolve the pure spectral, excitation and compositional profiles. A three factor model with non-negativity constraints produced three unique factors that were correlated with the relative abundance of helical, β-sheet and poly-proline II dihedral angles. This is the first empirical evidence that the typically resolved "disordered" spectrum represents the better defined poly-proline II type structure.

  5. Excitation energy and strength of the pygmy dipole resonance in stable tin isotopes

    CERN Document Server

    Özel, B; Lenske, H; Von Neumann-Cosel, P; Poltoratska, I; Ponomarev, V Yu; Richter, A; Savran, D; Tsoneva, N

    2009-01-01

    The $^{112,120}$Sn$(\\gamma,\\gamma')$ reactions have been studied at the S-DALINAC. Electric dipole (E1) strength distributions have been determined including contributions from unresolved strength extracted by a fluctuation analysis. Together with available data on $^{116,124}$Sn, an experimental systematics of the pygmy dipole resonance (PDR) in stable even-mass tin isotopes is established. The PDR centroid excitation energies and summed strengths are in reasonable agreement with quasiparticle-phonon model calculations based on a nonrelativistic description of the mean field but disagree with relativistic quasiparticle random-phase approximation predictions.

  6. Quantum-Coherence-Assisted Tunable On- and Off-Resonance Tunneling through a Quantum-Dot-Molecule Dielectric Film

    Science.gov (United States)

    Shen, Jian Qi; Zeng, Rui Xi

    2017-02-01

    Quantum-dot-molecular phase coherence (and the relevant quantum-interference-switchable optical response) can be utilized to control electromagnetic wave propagation via a gate voltage, since quantum-dot molecules can exhibit an effect of quantum coherence (phase coherence) when quantum-dot-molecular discrete multilevel transitions are driven by an electromagnetic wave. Interdot tunneling of carriers (electrons and holes) controlled by the gate voltage can lead to destructive quantum interference in a quantum-dot molecule that is coupled to an incident electromagnetic wave, and gives rise to a quantum coherence effect (e.g., electromagnetically induced transparency, EIT) in a quantum-dot-molecule dielectric film. The tunable on- and off-resonance tunneling effect of an incident electromagnetic wave (probe field) through such a quantum-coherent quantum-dot-molecule dielectric film is investigated. It is found that a high gate voltage can lead to the EIT phenomenon of the quantum-dot-molecular systems. Under the condition of on-resonance light tunneling through the present quantum-dot-molecule dielectric film, the probe field should propagate without loss if the probe frequency detuning is zero. Such an effect caused by both EIT and resonant tunneling, which is sensitive to the gate voltage, can be utilized for designing devices such as photonic switching, transistors, and logic gates.

  7. Coherent motion of excited state cyclic ketones: The have and the have-nots

    Science.gov (United States)

    Larsen, M. A. B.; Stephansen, A. B.; Sølling, T. I.

    2017-09-01

    The internal conversion processes of four cyclic ketones; cyclopentanone, 2-methylcyclopentanone, 3-methylcyclopentanone and cyclohexanone are investigated by Velocity Map Imaging (VMI) photoelectron spectroscopy. A 201 nm pump accesses the second excited state (n,3s) and the ultrafast dynamics is mapped by subsequent ionization with a 350 nm probe. Three of the four investigated molecular systems show an oscillatory time-dependence in the peak position of the 3s photoelectron band, while the last one simply decays exponentially. We find that the most plausible reason for the absence of the oscillation is due to high structural similarity between the excited state and the ionic state along the active coordinate.

  8. Resonant Excitation of White Dwarf Oscillations in Compact Object Binaries: 1. The No Back Reaction Approximation

    Energy Technology Data Exchange (ETDEWEB)

    Rathore, Y.

    2004-06-14

    We consider the evolution of white dwarfs with compact object companions (specifically black holes with masses up to {approx} 10{sup 6} M{sub {circle_dot}}, neutron stars, and other white dwarfs). We suppose that the orbits are initially quite elliptical and then shrink and circularize under the action of gravitational radiation. During this evolution, the white dwarfs will pass through resonances when harmonics of the orbital frequency match the stellar oscillation eigenfrequencies. As a star passes through these resonances, the associated modes will be excited and can be driven to amplitudes that are so large that there is a back reaction on the orbit which, in turn, limits the growth of the modes. A formalism is presented for describing this dynamical interaction for a non-rotating star in the linear approximation when the orbit can be treated as non-relativistic. A semi-analytical expression is found for computing the resonant energy transfer as a function of stellar and orbital parameters for the regime where back reaction may be neglected. This is used to calculate the results of passage through a sequence of resonances for several hypothetical systems. It is found that the amplitude of the {ell} = m = 2 f-mode can be driven into the non-linear regime for appropriate initial conditions. We also discuss where the no back reaction approximation is expected to fail, and the qualitative effects of back reaction.

  9. Phase-noise-induced resonance in arrays of coupled excitable neural models.

    Science.gov (United States)

    Xiaoming Liang; Liang Zhao

    2013-08-01

    Recently, it is observed that, in a single neural model, phase noise (time-varying signal phase) arising from an external stimulating signal can induce regular spiking activities even if the signal is subthreshold. In addition, it is also uncovered that there exists an optimal phase noise intensity at which the spiking rhythm coincides with the frequency of the subthreshold signal, resulting in a phase-noise-induced resonance phenomenon. However, neurons usually do not work alone, but are connected in the form of arrays or blocks. Therefore, we study the spiking activity induced by phase noise in arrays of globally and locally coupled excitable neural models. We find that there also exists an optimal phase noise intensity for generating large neural response and such an optimal value is significantly decreased compared to an isolated single neuron case, which means the detectability in response to the subthreshold signal of neurons is sharply improved because of the coupling. In addition, we reveal two new resonance behaviors in the neuron ensemble with the presence of phase noise: there exist optimal values of both coupling strength and system size, where the coupled neurons generate regular spikes under subthreshold stimulations, which are called as coupling strength and system size resonance, respectively. Finally, the dependence of phase-noise-induced resonance on signal frequency is also examined.

  10. Low-energy d-d excitations in MnO studied by resonant x-ray fluorescence spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Butorin, S.M.; Guo, J.; Magnuson, M. [Uppsala Univ. (Sweden)] [and others

    1997-04-01

    Resonant soft X-ray emission spectroscopy has been demonstrated to possess interesting abilities for studies of electronic structure in various systems, such as symmetry probing, alignment and polarization dependence, sensitivity to channel interference, etc. In the present abstract the authors focus on the feasibility of resonant soft X-ray emission to probe low energy excitations by means of resonant electronic X-ray Raman scattering. Resonant X-ray emission can be regarded as an inelastic scattering process where a system in the ground state is transferred to a low excited state via a virtual core excitation. The energy closeness to a core excitation of the exciting radiation enhances the (generally) low probability for inelastic scattering at these wavelengths. Therefore soft X-ray emission spectroscopy (in resonant electronic Raman mode) can be used to study low energy d-d excitations in transition metal systems. The involvement of the intermediate core state allows one to use the selection rules of X-ray emission, and the appearance of the elastically scattered line in the spectra provides the reference to the ground state.

  11. Optical coherent control in semiconductors

    DEFF Research Database (Denmark)

    Østergaard, John Erland; Vadim, Lyssenko; Hvam, Jørn Märcher

    2001-01-01

    of quantum control including the recent applications to semiconductors and nanostructures. We study the influence of inhomogeneous broadening in semiconductors on CC results. Photoluminescence (PL) and the coherent emission in four-wave mixing (FWM) is recorded after resonant excitation with phase...

  12. Cross sections and coherence terms for associative ionization of two differently excited Na(3p) atoms

    NARCIS (Netherlands)

    Meijer, H.A.J.; Pelgrim, T.J.C.; Heideman, H.G.M.; Morgenstern, R.; Andersen, N.

    1989-01-01

    The associative ionization process in thermal Na(3p)-Na(3p) encounters has been studied in a series of crossed-beam experiments where the light polarization of the two laser beams preparing the excited atoms before collision was varied independently. It is shown how in this way maximum possible info

  13. Effects of molecular resonances on Rydberg blockade

    CERN Document Server

    Derevianko, Andrei; Topcu, Turker; Kroeze, Ronen M; Lukin, Mikhail D

    2015-01-01

    We study the effect of resonances associated with complex molecular interaction of Rydberg atoms on Rydberg blockade. We show that densely-spaced molecular potentials between doubly-excited atomic pairs become unavoidably resonant with the optical excitation at short interatomic separations. Such molecular resonances limit the coherent control of individual excitations in Rydberg blockade. As an illustration, we compute the molecular interaction potentials of Rb atoms near the $100s$ states asymptote to characterize such detrimental molecular resonances, determine the resonant loss rate to molecules and inhomogeneous light shifts. Techniques to avoid the undesired effect of molecular resonances are discussed.

  14. Electron emission induced by resonant coherent interaction in ion-surface scattering at grazing incidence

    Energy Technology Data Exchange (ETDEWEB)

    Garcia de Abajo, F.J. (Departamento de Ciencias de la Computacion e Inteligencia Artificial, Facultad de Informatica, Universidad del Pais Vasco, Apartado 649, 20080 San Sebastian (Spain)); Ponce, V.H.; Echenique, P.M. (Departamento de Fisica de Materiales, Facultad de Quimica, Universidad del Pais Vasco, Apartado 1072, 20080 San Sebastian (Spain))

    1994-01-15

    The resonant coherent interaction of an ion with an oriented crystal surface, under grazing-incidence conditions with respect to a special direction of the crystal, gives rise to electron loss to the continuum from electronic bound states of the ion. The calculations presented below predict large probabilities for electron emission due to this mechanism. The electrons are emitted with well defined energies, expressed in terms of the condition of resonance. Furthermore, the emission takes place around certain preferential directions, which are determined by both the latter condition and the symmetry of the surface lattice. Our calculations for MeV He[sup +] ions scattered at a W(001) surface along the [l angle]100[r angle] direction with glancing angle of 0--2 mrad indicate a yield of emission close to 1. Using heavier projectiles, one obtains smaller yields, but still large enough to be measurable in some cases (e.g., [approx]0.9 for 53 MeV B[sup 4+] and an angle of incidence of 1 mrad). Besides, the initial bound state is energy shifted due to the interaction with both the crystal potential and the velocity-dependent image potential. This results in a slight shift of the peaks of emission, which suggests a possible spectroscopy for analyzing the dynamical interaction of electronic bound states with solid surfaces.

  15. AlN-based piezoelectric bimorph microgenerator utilizing low-level non-resonant excitation

    Science.gov (United States)

    Hampl, Stefan; Cimalla, Volker; Polster, Tobias; Hoffmann, Martin

    2011-06-01

    This work aims for utilizing human ocular motion for the self-sufficient power supply of a minimally invasive implantable monitoring system for intraocular pressure (IOP). With a proven piezoelectric functionality (d33>5 pm/V), nanocrystalline thin films of aluminum nitride (AlN) provide a good capability for micromechanical energy harvesting (EH) in medical applications. Many d31-mode microcantilever architectures are poorly suited for human-induced EH: Resonant mass-spring-damper systems are tested under high, narrow-band excitation frequencies. However, human motions, e.g. vibrations of eyeballs are marked by their low frequency, unpredictable, mainly aperiodic and time-varying signature. Different vibration types and directions are 3-dimensionally superimposed. Saccadic eye movements are favorable for inertial microgenerators because of their high dynamic loading (ω<=1000°/s). Our generator concept (symmetric active/active-parallel-bimorph cantilever) enables a high structural compliance by maximizing the piezoactive volume at very low cantilever thicknesses (<1 μm). An increased length and seismic mass enable an effective excitation by low-level aperiodic vibrations such as saccadic acceleration impulses. Analytic calculations and FEA-simulations investigate the potential distribution and transient response of different bimorph structures (length 200- 1000 μm, width 20-200 μm) on broadband vibrations. First released monomorph and bimorph structures show very low resonant frequencies and an adequate robustness.

  16. Inclined slot-excited annular electron cyclotron resonance plasma source for hyperthermal neutral beam generation.

    Science.gov (United States)

    You, H-J; Kim, D-W; Koo, M; Jang, S-O; Jung, Y-H; Hong, S-H; Lee, B-J

    2011-01-01

    An inclined slot-excited antenna (ISLAN) electron cyclotron resonance (ECR) plasma source is newly designed and constructed for higher flux hyperthermal neutral beam (HNB) generation. The developed ISLAN source is modified from vertical slot-excited antenna (VSLAN) source in two aspects: one is the use of inclined slots instead of vertical slots, and the other is a cusp magnetic field configuration rather than a toroidal configuration. Such modifications allow us to have more uniform arrangement of slots and magnets, then enabling plasma generation more uniform and thinner. Moreover, ECR plasma allows higher ionization rate, enabling plasma density higher even in submillitorr pressures, therefore decreasing the collision rate and∕or the reionization rate of the reflected atoms while passing through the plasma, and eventually getting higher flux of HNBs. In this paper, we report the design features and the plasma characteristics of the ISLAN source by doing plasma measurements and electromagnetic simulations. It was found that ISLAN source can be a high potential source for larger flux HNB generation; the source was found to give higher plasma densities and better uniformities than inductively coupled plasma source, particularly in low pressure ranges. Also, it is important that using ISLAN gives easier matching and better stability, i.e., ISLAN shows similar field patterns and good plasma symmetries irrespective of the variations of the mean diameter of the ring resonator and∕or the presence of a limiter or a reflector, and the operating pressures.

  17. Multi frequency excited MEMS cantilever beam resonator for Mixer-Filter applications

    KAUST Repository

    Chandran, Akhil A.

    2016-09-15

    Wireless communication uses Radio Frequency waves to transfer information from one point to another. The modern RF front end devices are implementing MEMS in their designs so as to exploit the inherent properties of MEMS devices, such as its low mass, low power consumption, and small size. Among the components in the RF transceivers, band pass filters and mixers play a vital role in achieving the optimum RF performance. And this paper aims at utilizing an electrostatically actuated micro cantilever beam resonator\\'s nonlinear frequency mixing property to realize a Mixer-Filter configuration through multi-frequency excitation. The paper studies about the statics and dynamics of the device. Simulations are carried out to study the added benefits of multi frequency excitation. The modelling of the cantilever beam has been done using a Reduced Order Model of the Euler-Bernoulli\\'s beam equation by implementing the Galerkin discretization. The device is shown to be able to down-convert signals from 960 MHz of frequency to an intermediate frequency around 50 MHz and 70 MHz in Phase 1 and 2, respectively. The simulation showed promising results to take the project to the next level. © 2016 IEEE.

  18. Plane wave excitation-detection of non-resonant plasmons along finite-width graphene strips.

    Science.gov (United States)

    Gómez-Díaz, J S; Esquius-Morote, M; Perruisseau-Carrier, J

    2013-10-21

    An approach to couple free-space waves and non-resonant plasmons propagating along graphene strips is proposed based on the periodic modulation of the graphene strip width. The solution is technologically very simple, scalable in frequency, and provides customized coupling angle and intensity. Moreover, the coupling properties can be dynamically controlled at a fixed frequency via the graphene electrical field effect, enabling advanced and flexible plasmon excitation-detection strategies. We combine a previously derived scaling law for graphene strips with leaky-wave theory borrowed from microwaves to achieve rigorous and efficient modeling and design of the structure. In particular we analytically derive its dispersion, predict its coupling efficiency and radiated field structure, and design strip configurations able to fulfill specific coupling requirements. The proposed approach and developed methods are essential to the recent and fundamental problem of the excitation-detection of non-resonant plasmons propagating along a continuous graphene strip, and could pave the way to smart all-graphene sensors and transceivers.

  19. Study of orbitally excited $B$ mesons and evidence for a new $B\\pi$ resonance

    CERN Document Server

    Aaltonen, Timo Antero; Amidei, Dante E; Anastassov, Anton Iankov; Annovi, Alberto; Antos, Jaroslav; Apollinari, Giorgio; Appel, Jeffrey A; Arisawa, Tetsuo; Artikov, Akram Muzafarovich; Asaadi, Jonathan A; Ashmanskas, William Joseph; Auerbach, Benjamin; Aurisano, Adam J; Azfar, Farrukh A; Badgett, William Farris; Bae, Taegil; Barbaro-Galtieri, Angela; Barnes, Virgil E; Barnett, Bruce Arnold; Barria, Patrizia; Bartos, Pavol; Bauce, Matteo; Bedeschi, Franco; Behari, Satyajit; Bellettini, Giorgio; Bellinger, James Nugent; Benjamin, Douglas P; Beretvas, Andrew F; Bhatti, Anwar Ahmad; Bland, Karen Renee; Blumenfeld, Barry J; Bocci, Andrea; Bodek, Arie; Bortoletto, Daniela; Boudreau, Joseph Francis; Boveia, Antonio; Brigliadori, Luca; Bromberg, Carl Michael; Brucken, Erik; Budagov, Ioulian A; Budd, Howard Scott; Burkett, Kevin Alan; Busetto, Giovanni; Bussey, Peter John; Butti, Pierfrancesco; Buzatu, Adrian; Calamba, Aristotle; Camarda, Stefano; Campanelli, Mario; Canelli, Florencia; Carls, Benjamin; Carlsmith, Duncan L; Carosi, Roberto; Carrillo Moreno, Salvador; Casal Larana, Bruno; Casarsa, Massimo; Castro, Andrea; Catastini, Pierluigi; Cauz, Diego; Cavaliere, Viviana; Cavalli-Sforza, Matteo; Cerri, Alessandro; Cerrito, Lucio; Chen, Yen-Chu; Chertok, Maxwell Benjamin; Chiarelli, Giorgio; Chlachidze, Gouram; Cho, Kihyeon; Chokheli, Davit; Clark, Allan Geoffrey; Clarke, Christopher Joseph; Convery, Mary Elizabeth; Conway, John Stephen; Corbo, Matteo; Cordelli, Marco; Cox, Charles Alexander; Cox, David Jeremy; Cremonesi, Matteo; Cruz Alonso, Daniel; Cuevas Maestro, Javier; Culbertson, Raymond Lloyd; D'Ascenzo, Nicola; Datta, Mousumi; de Barbaro, Pawel; Demortier, Luc M; Marchese, Luigi; Deninno, Maria Maddalena; Devoto, Francesco; D'Errico, Maria; Di Canto, Angelo; Di Ruzza, Benedetto; Dittmann, Jay Richard; D'Onofrio, Monica; Donati, Simone; Dorigo, Mirco; Driutti, Anna; Ebina, Koji; Edgar, Ryan Christopher; Elagin, Andrey L; Erbacher, Robin D; Errede, Steven Michael; Esham, Benjamin; Farrington, Sinead Marie; Feindt, Michael; Fernández Ramos, Juan Pablo; Field, Richard D; Flanagan, Gene U; Forrest, Robert David; Franklin, Melissa EB; Freeman, John Christian; Frisch, Henry J; Funakoshi, Yujiro; Galloni, Camilla; Garfinkel, Arthur F; Garosi, Paola; Gerberich, Heather Kay; Gerchtein, Elena A; Giagu, Stefano; Giakoumopoulou, Viktoria Athina; Gibson, Karen Ruth; Ginsburg, Camille Marie; Giokaris, Nikos D; Giromini, Paolo; Giurgiu, Gavril A; Glagolev, Vladimir; Glenzinski, Douglas Andrew; Gold, Michael S; Goldin, Daniel; Golossanov, Alexander; Gomez, Gervasio; Gomez-Ceballos, Guillelmo; Goncharov, Maxim T; González López, Oscar; Gorelov, Igor V; Goshaw, Alfred T; Goulianos, Konstantin A; Gramellini, Elena; Grinstein, Sebastian; Grosso-Pilcher, Carla; Group, Robert Craig; Barreiro Guimaraes da Costa, Joao; Hahn, Stephen R; Han, Ji-Yeon; Happacher, Fabio; Hara, Kazuhiko; Hare, Matthew Frederick; Harr, Robert Francis; Harrington-Taber, Timothy; Hatakeyama, Kenichi; Hays, Christopher Paul; Heinrich, Joel G; Herndon, Matthew Fairbanks; Hocker, James Andrew; Hong, Ziqing; Hopkins, Walter Howard; Hou, Suen Ray; Hughes, Richard Edward; Husemann, Ulrich; Hussein, Mohammad; Huston, Joey Walter; Introzzi, Gianluca; Iori, Maurizio; Ivanov, Andrew Gennadievich; James, Eric B; Jang, Dongwook; Jayatilaka, Bodhitha Anjalike; Jeon, Eun-Ju; Jindariani, Sergo Robert; Jones, Matthew T; Joo, Kyung Kwang; Jun, Soon Yung; Junk, Thomas R; Kambeitz, Manuel; Kamon, Teruki; Karchin, Paul Edmund; Kasmi, Azeddine; Kato, Yukihiro; Ketchum, Wesley Robert; Keung, Justin Kien; Kilminster, Benjamin John; Kim, DongHee; Kim, Hyunsoo; Kim, Jieun; Kim, Min Jeong; Kim, Soo Bong; Kim, Shin-Hong; Kim, Young-Kee; Kim, Young-Jin; Kimura, Naoki; Kirby, Michael H; Knoepfel, Kyle James; Kondo, Kunitaka; Kong, Dae Jung; Konigsberg, Jacobo; Kotwal, Ashutosh Vijay; Kreps, Michal; Kroll, IJoseph; Kruse, Mark Charles; Kuhr, Thomas; Kurata, Masakazu; Laasanen, Alvin Toivo; Lammel, Stephan; Lancaster, Mark; Lannon, Kevin Patrick; Latino, Giuseppe; Heck, Martin; Lee, Hyun Su; Lee, Jaison; Leo, Sabato; Leone, Sandra; Lewis, Jonathan D; Limosani, Antonio; Lipeles, Elliot David; Lister, Alison; Liu, Hao; Liu, Qiuguang; Liu, Tiehui Ted; Lockwitz, Sarah E; Loginov, Andrey Borisovich; Lucà, Alessandra; Lucchesi, Donatella; Lueck, Jan; Lujan, Paul Joseph; Lukens, Patrick Thomas; Lungu, Gheorghe; Lys, Jeremy E; Lysak, Roman; Madrak, Robyn Leigh; Maestro, Paolo; Malik, Sarah Alam; Manca, Giulia; Manousakis-Katsikakis, Arkadios; Margaroli, Fabrizio; Marino, Christopher Phillip; Martínez-Perez, Mario; Matera, Keith; Mattson, Mark Edward; Mazzacane, Anna; Mazzanti, Paolo; McNulty, Ronan; Mehta, Andrew; Mehtala, Petteri; Mesropian, Christina; Miao, Ting; Mietlicki, David John; Mitra, Ankush; Miyake, Hideki; Moed, Shulamit; Moggi, Niccolo; Moon, Chang-Seong; Moore, Ronald Scott; Morello, Michael Joseph; Mukherjee, Aseet; Muller, Thomas; Murat, Pavel A; Mussini, Manuel; Nachtman, Jane Marie; Nagai, Yoshikazu; Naganoma, Junji; Nakano, Itsuo; Napier, Austin; Nett, Jason Michael; Neu, Christopher Carl; Nigmanov, Turgun S; Nodulman, Lawrence J; Noh, Seoyoung; Norniella Francisco, Olga; Oakes, Louise Beth; Oh, Seog Hwan; Oh, Young-do; Oksuzian, Iuri Artur; Okusawa, Toru; Orava, Risto Olavi; Ortolan, Lorenzo; Pagliarone, Carmine Elvezio; Palencia, Jose Enrique; Palni, Prabhakar; Papadimitriou, Vaia; Parker, William Chesluk; Pauletta, Giovanni; Paulini, Manfred; Paus, Christoph Maria Ernst; Phillips, Thomas J; Piacentino, Giovanni M; Pianori, Elisabetta; Pilot, Justin Robert; Pitts, Kevin T; Plager, Charles; Pondrom, Lee G; Poprocki, Stephen; Potamianos, Karolos Jozef; Prokoshin, Fedor; Pranko, Aliaksandr Pavlovich; Ptohos, Fotios K; Punzi, Giovanni; Ranjan, Niharika; Redondo Fernández, Ignacio; Renton, Peter B; Rescigno, Marco; Rimondi, Franco; Ristori, Luciano; Robson, Aidan; Rodriguez, Tatiana Isabel; Rolli, Simona; Ronzani, Manfredi; Roser, Robert Martin; Rosner, Jonathan L; Ruffini, Fabrizio; Ruiz Jimeno, Alberto; Russ, James S; Rusu, Vadim Liviu; Sakumoto, Willis Kazuo; Sakurai, Yuki; Santi, Lorenzo; Sato, Koji; Saveliev, Valeri; Savoy-Navarro, Aurore; Schlabach, Philip; Schmidt, Eugene E; Schwarz, Thomas A; Scodellaro, Luca; Scuri, Fabrizio; Seidel, Sally C; Seiya, Yoshihiro; Semenov, Alexei; Sforza, Federico; Shalhout, Shalhout Zaki; Shears, Tara G; Shepard, Paul F; Shimojima, Makoto; Shochet, Melvyn J; Tecker-Shreyber, Irina; Simonenko, Alexander V; Sliwa, Krzysztof Jan; Smith, John Rodgers; Snider, Frederick Douglas; Sorin, Maria Veronica; Song, Hao; Stancari, Michelle Dawn; St Denis, Richard Dante; Stentz, Dale James; Strologas, John; Sudo, Yuji; Sukhanov, Alexander I; Suslov, Igor M; Takemasa, Ken-ichi; Takeuchi, Yuji; Tang, Jian; Tecchio, Monica; Teng, Ping-Kun; Thom, Julia; Thomson, Evelyn Jean; Thukral, Vaikunth; Toback, David A; Tokar, Stanislav; Tollefson, Kirsten Anne; Tomura, Tomonobu; Tonelli, Diego; Torre, Stefano; Torretta, Donatella; Totaro, Pierluigi; Trovato, Marco; Ukegawa, Fumihiko; Uozumi, Satoru; Vázquez-Valencia, Elsa Fabiola; Velev, Gueorgui; Vellidis, Konstantinos; Vernieri, Caterina; Vidal Marono, Miguel; Vilar Cortabitarte, Rocio; Vizán Garcia, Jesus Manuel; Vogel, Marcelo; Volpi, Guido; Wagner, Peter; Wallny, Rainer S; Wang, Song-Ming; Waters, David S; Wester, William Carl; Whiteson, Daniel O; Wicklund, Arthur Barry; Wilbur, Scott; Williams, Hugh H; Wilson, Jonathan Samuel; Wilson, Peter James; Winer, Brian L; Wittich, Peter; Wolbers, Stephen A; Wolfe, Homer; Wright, Thomas Roland; Wu, Xin; Wu, Zhenbin; Yamamoto, Kazuhiro; Yamato, Daisuke; Yang, Tingjun; Yang, Un-Ki; Yang, Yu Chul; Yao, Wei-Ming; Yeh, Gong Ping; Yi, Kai; Yoh, John; Yorita, Kohei; Yoshida, Takuo; Yu, Geum Bong; Yu, Intae; Zanetti, Anna Maria; Zeng, Yu; Zhou, Chen; Zucchelli, Stefano

    2014-07-28

    Using the full CDF Run II data sample, we report evidence for a new resonance, which we refer to as B(5970), found simultaneously in the $B^0\\pi^+$ and $B^+\\pi^-$ mass distributions with a significance of 4.4 standard deviations. We further report the first study of resonances consistent with orbitally excited $B^{+}$ mesons and an updated measurement of the properties of orbitally excited $B^0$ and $B_s^0$ mesons. Using samples of approximately 8400 $B^{**0}$, 3300 $B^{**+}$, 1350 $B^{**0}_s$, 2600 $B(5970)^0$, and 1400 $B(5970)^+$ decays, we measure the masses and widths of all states, as well as the product of the relative production rate of $B_1$ and $B_2^*$ states times the branching fraction into a $B^{0,+}$ meson and a charged particle. Furthermore, we measure the branching fraction of the $B_{s2}^{*0} \\rightarrow B^{*+} K^-$ decay relative to the $B_{s2}^{*0} \\rightarrow B^{+} K^-$ decay, the production rate times the branching fraction of the B(5970) state relative to the $B_{2}^{*0,+}$ state, and th...

  20. Ionospheric Alfvén resonator excitation due to nearby thunderstorms

    Science.gov (United States)

    Surkov, V. V.; Hayakawa, M.; Schekotov, A. Y.; Fedorov, E. N.; Molchanov, O. A.

    2006-01-01

    A theory of midlatitude Ionospheric Alfvén Resonator (IAR) excitation due to random cloud-to-ground lightning discharges is developed. Electromagnetic wave radiated from the lightning discharges penetrates into the ionosphere, thereby exciting the shear Alfvén and magnetosonic waves in the F region of ionosphere. The IAR arises due to wave reflection from the Alfvén velocity gradients in the topside ionosphere. Typically, the ionospheric resonance cavity accumulates the shear Alfvén wave energy with periods from 1 s to a few tenths of seconds. To proceed analytically, a suitably idealized plane-stratified model of the medium was used that ignores the magnetic field line curvature and dip angle but includes plasma conductivity variations with altitude. The thunderstorm centers distributed around a ground-recording station is assumed to be statistically independent sources of the lightning activity, which is a stochastic Poisson process. The lightning onset time and the current moment is supposed to be a random value, while the shape and duration of return strokes are deterministic. Model calculations of the IAR spectrum due to nearby thunderstorm activity were applied to interpret ULF observation made at Karimshino station (52.94°N, 158.25°E) in Kamchatka peninsula. It is shown that the sharp impulses which are in one-to-one correspondence with the appearance of the spectral resonance structure (SRS) in dynamic spectrograms can be the result from nearby lightning discharges followed by impulse IAR excitation. The correlation functions and power spectra of the IAR due to random lightning discharge process is studied both analytically and numerically. We found that the nearby thunderstorms in the range of 1000-2000 km make a main contribution to the SRS signature of the midlatitude IAR, whereas the remote/tropic thunderstorm activity is of minor importance. It is not inconceivable that there may exist other permanent mechanisms of the midlatitude IAR excitation

  1. Synchronization of three homodromy coupled exciters in a non-resonant vibrating system of plane motion

    Institute of Scientific and Technical Information of China (English)

    Xue-Liang Zhang; Bang-Chun Wen; Chun-Yu Zhao

    2012-01-01

    In this paper,the synchronization problem of three homodromy coupled exciters in a non-resonant vibrating system of plane motion is studied.By introducing the average method of modified small parameters,we deduced dimensionless coupling equation of three exciters,which converted the problem of synchronization into that of the existence and stability of zero solutions for the average differential equations of the small parameters.Based on the dimensionless coupling torques and characteristics of the corresponding limited functions,the synchronization criterion for three exciters was derived as the absolute value of dimensionless residual torque difference between arbitrary two motors being less than the maximum of their dimensionless coupling torques.The stability criterion of its synchronous state lies in the double-condition that the inertia coupling matrix is positive definite and all its elements are positive as well.The synchronization determinants are the coefficients of synchronization ability,also called as the general dynamical symmetry coefficients.The double-equilibrium state of the vibrating system is manifested by numeric method,and the numeric and simulation results derived thereof indicate the indispensable and crucial role the structural parameters of the vibrating system play in the stability criterion of synchronous operation.Besides,by adjusting its structural parameters,the elliptical motion of the vibrating system successfully met the requirements in engineering applications.

  2. Excitation of the ionospheric resonance cavity by neutral winds at middle latitudes

    Directory of Open Access Journals (Sweden)

    V. V. Surkov

    2004-09-01

    Full Text Available A new mechanism for the ionospheric Alfvén resonator (IAR excitation at middle latitudes is considered. It is shown that the ionosphere wind system in this region is capable of sustaining the generation of geomagnetic perturbations that can be detected by ground magnetometers. The general IAR dispersion relation describing the linear coupling of the shear Alfvén and fast magnetosonic/compressional modes is obtained. The dependence of the IAR eigenfrequencies and damping rates on the perpendicular wave number and on the ground conductivity during the day- and nighttime conditions is analyzed both analytically and numerically. In order to demonstrate the IAR excitation by neutral winds the power spectra of the geomagnetic perturbation on the ground surface are calculated. Furthermore, it is found that Kolmogorov spectra of the ionospheric turbulent neutral winds and the IAR eigenfrequencies lie in the same frequency range that make it possible to enhance the IAR excitation. The relevance of the developed theoretical model to the ground-based observations is stressed.

  3. Resonant indirect excitation of Gd{sup 3+} in AlN thin films

    Energy Technology Data Exchange (ETDEWEB)

    Ishizu, Yuta; Tsuji, Kazuma; Harada, Yukihiro; Kita, Takashi [Department of Electrical and Electronic Engineering, Graduate School of Engineering, Kobe University, 1-1 Rokkodai, Nada, Kobe 657-8501 (Japan); Chigi, Yoshitaka; Nishimoto, Tetsuro; Tanaka, Hiroyuki; Kobayashi, Mikihiro [YUMEX INC., 400 Itoda, Yumesaki, Himeji, Hyogo 671-2114 (Japan); Ishihara, Tsuguo; Izumi, Hirokazu [Hyogo Prefectural Institute of Technology, 3-1-12 Yukihira, Suma, Kobe 654-0037 (Japan)

    2014-05-07

    We studied the efficient indirect excitation of Gd{sup 3+} ions in AlN thin films. C-axis oriented polycrystalline thin films of Al{sub 0.997}Gd{sub 0.003}N/AlN were grown on fused silica substrates using a reactive radio-frequency magnetron sputtering technique. The intra-orbital electron transition in Gd{sup 3+} showed a narrow luminescence line at 3.9 eV. The photoluminescence (PL) excitation (PLE) spectrum exhibited a peak originating from efficient indirect energy transfer from the band edge of AlN to Gd{sup 3+} ions. The PLE peak shifted and the PL intensity showed a dramatic change when the AlN band gap was varied by changing the temperature. Energy scanning performed by changing the band-gap energy of AlN with temperature revealed several resonant channels of energy transfer into the higher excited states of Gd{sup 3+}.

  4. Resonant tidal excitation of internal waves in the Earth's fluid core

    Science.gov (United States)

    Tyler, Robert H.; Kuang, Weijia

    2014-07-01

    It has long been speculated that there is a stably stratified layer below the core-mantle boundary, and two recent studies have improved the constraints on the parameters describing this stratification. Here we consider the dynamical implications of this layer using a simplified model. We first show that the stratification in this surface layer has sensitive control over the rate at which tidal energy is transferred to the core. We then show that when the stratification parameters from the recent studies are used in this model, a resonant configuration arrives whereby tidal forces perform elevated rates of work in exciting core flow. Specifically, the internal wave speed derived from the two independent studies (150 and 155 m/s) are in remarkable agreement with the speed (152 m/s) required for excitation of the primary normal mode of oscillation as calculated from full solutions of the Laplace Tidal Equations applied to a reduced-gravity idealized model representing the stratified layer. In evaluating this agreement it is noteworthy that the idealized model assumed may be regarded as the most reduced representation of the stratified dynamics of the layer, in that there are no non-essential dynamical terms in the governing equations assumed. While it is certainly possible that a more realistic treatment may require additional dynamical terms or coupling, it is also clear that this reduced representation includes no freedom for coercing the correlation described. This suggests that one must accept either (1) that tidal forces resonantly excite core flow and this is predicted by a simple model or (2) that either the independent estimates or the dynamical model does not accurately portray the core surface layer and there has simply been an unlikely coincidence between three estimates of a stratification parameter which would otherwise have a broad plausible range.

  5. Resonant Tidal Excitation of Internal Waves in the Earth's Fluid Core

    Science.gov (United States)

    Tyler, Robert H.; Kuang, Weijia

    2014-01-01

    It has long been speculated that there is a stably stratified layer below the core-mantle boundary, and two recent studies have improved the constraints on the parameters describing this stratification. Here we consider the dynamical implications of this layer using a simplified model. We first show that the stratification in this surface layer has sensitive control over the rate at which tidal energy is transferred to the core. We then show that when the stratification parameters from the recent studies are used in this model, a resonant configuration arrives whereby tidal forces perform elevated rates of work in exciting core flow. Specifically, the internal wave speed derived from the two independent studies (150 and 155 m/s) are in remarkable agreement with the speed (152 m/s) required for excitation of the primary normal mode of oscillation as calculated from full solutions of the Laplace Tidal Equations applied to a reduced-gravity idealized model representing the stratified layer. In evaluating this agreement it is noteworthy that the idealized model assumed may be regarded as the most reduced representation of the stratified dynamics of the layer, in that there are no non-essential dynamical terms in the governing equations assumed. While it is certainly possible that a more realistic treatment may require additional dynamical terms or coupling, it is also clear that this reduced representation includes no freedom for coercing the correlation described. This suggests that one must accept either (1) that tidal forces resonantly excite core flow and this is predicted by a simple model or (2) that either the independent estimates or the dynamical model does not accurately portray the core surface layer and there has simply been an unlikely coincidence between three estimates of a stratification parameter which would otherwise have a broad plausible range.

  6. Resonant Tidal Excitation of Internal Waves in the Earth's Fluid Core

    Science.gov (United States)

    Tyler, Robert H.; Kuang, Weijia

    2014-01-01

    It has long been speculated that there is a stably stratified layer below the core-mantle boundary, and two recent studies have improved the constraints on the parameters describing this stratification. Here we consider the dynamical implications of this layer using a simplified model. We first show that the stratification in this surface layer has sensitive control over the rate at which tidal energy is transferred to the core. We then show that when the stratification parameters from the recent studies are used in this model, a resonant configuration arrives whereby tidal forces perform elevated rates of work in exciting core flow. Specifically, the internal wave speed derived from the two independent studies (150 and 155 m/s) are in remarkable agreement with the speed (152 m/s) required for excitation of the primary normal mode of oscillation as calculated from full solutions of the Laplace Tidal Equations applied to a reduced-gravity idealized model representing the stratified layer. In evaluating this agreement it is noteworthy that the idealized model assumed may be regarded as the most reduced representation of the stratified dynamics of the layer, in that there are no non-essential dynamical terms in the governing equations assumed. While it is certainly possible that a more realistic treatment may require additional dynamical terms or coupling, it is also clear that this reduced representation includes no freedom for coercing the correlation described. This suggests that one must accept either (1) that tidal forces resonantly excite core flow and this is predicted by a simple model or (2) that either the independent estimates or the dynamical model does not accurately portray the core surface layer and there has simply been an unlikely coincidence between three estimates of a stratification parameter which would otherwise have a broad plausible range.

  7. Plasma Dipole Oscillation Excited by Trapped Electrons Leading to Bursts of Coherent Radiation

    CERN Document Server

    Kwon, Kyu Been; Song, Hyung Seon; Kim, Young-Kuk; Ersfeld, Bernhard; Jaroszynski, Dino A; Hur, Min Sup

    2016-01-01

    Plasma dipole oscillation (PDO) depicted as harmonic motion of a spatially localized block of electrons has, until now, been hypothetical. In practice, the plasma oscillation occurs always as a part of a plasma wave. Studies on radiation burst from plasmas have focused only on coupling of the plasma wave and electromagnetic wave. Here we show that a very-high-field PDO can be generated by the electrons trapped in a moving train of potential wells. The electrons riding on the potential train coherently construct a local dipole moment by charge separation. The subsequent PDO is found to persist stably until its energy is emitted entirely via coherent radiation. In our novel method, the moving potentials are provided by two slightly-detuned laser pulses colliding in a non-magnetized plasma. The radiated energy reaches several millijoules in the terahertz spectral region. The proposed method provides a way of realizing the PDO as a new radiation source in the laboratory. PDO as a mechanism of astrophysical radio-...

  8. Circular periodic orbits, resonance capture and inclination excitation during type II migration

    Science.gov (United States)

    Antoniadou, K. I.; Voyatzis, G.

    2017-03-01

    We consider planetary systems evolving under the effect of a Stokes-type dissipative force mimicking the outcome of a type II migration process. As inward migration proceeds and the planets follow the circular family (they start on circular orbits) and even though they are initially almost coplanar, resonance capture can be realized. Then, at the vertical critical orbits (VCOs), that the circular family possesses, the inclination excitation can abruptly take place. The planets are now guided by the spatial elliptic families, which bifurcate from those critical orbits. We herein, perform a direct link of mutually inclined stable planetary systems on circular orbits trapped in mean-motion resonance (MMR) with the existence of VCOs of high values of multiplicity. It is shown that the more the multiplicity of the periodic orbits of the circular family increases, the more VCOs (corresponding to more MMRs) appear. In this way, we can provide a justification for the existence of resonant planets on circular orbits, which could, even further to that, evolve stably if they were mutually inclined.

  9. Three dimensional nuclear magnetic resonance spectroscopic imaging of sodium ions using stochastic excitation and oscillating gradients

    Energy Technology Data Exchange (ETDEWEB)

    Frederick, B.deB. [California Univ., Berkeley, CA (United States)]|[Lawrence Berkeley Lab., CA (United States)

    1994-12-01

    Nuclear magnetic resonance (NMR) spectroscopic imaging of {sup 23}Na holds promise as a non-invasive method of mapping Na{sup +} distributions, and for differentiating pools of Na{sup +} ions in biological tissues. However, due to NMR relaxation properties of {sup 23}Na in vivo, a large fraction of Na{sup +} is not visible with conventional NMR imaging methods. An alternate imaging method, based on stochastic excitation and oscillating gradients, has been developed which is well adapted to measuring nuclei with short T{sub 2}. Contemporary NMR imaging techniques have dead times of up to several hundred microseconds between excitation and sampling, comparable to the shortest in vivo {sup 23}Na T{sub 2} values, causing significant signal loss. An imaging strategy based on stochastic excitation has been developed which greatly reduces experiment dead time by reducing peak radiofrequency (RF) excitation power and using a novel RF circuit to speed probe recovery. Continuously oscillating gradients are used to eliminate transient eddy currents. Stochastic {sup 1}H and {sup 23}Na spectroscopic imaging experiments have been performed on a small animal system with dead times as low as 25{mu}s, permitting spectroscopic imaging with 100% visibility in vivo. As an additional benefit, the encoding time for a 32x32x32 spectroscopic image is under 30 seconds. The development and analysis of stochastic NMR imaging has been hampered by limitations of the existing phase demodulation reconstruction technique. Three dimensional imaging was impractical due to reconstruction time, and design and analysis of proposed experiments was limited by the mathematical intractability of the reconstruction method. A new reconstruction method for stochastic NMR based on Fourier interpolation has been formulated combining the advantage of a several hundredfold reduction in reconstruction time with a straightforward mathematical form.

  10. Gas phase proton affinities of molecules in excited electronic states by ion cyclotron resonance spectroscopy. [Benzaldehyde, cyanobenzene, and pyridine

    Energy Technology Data Exchange (ETDEWEB)

    Freiser, B.S.; Beauchamp, J.L.

    1976-01-07

    Ion cyclotron resonance spectroscopy is proposed as a method to determine acid-base properties of molecules in excited electronic states. Proton affinity in the excited state can be determined from the proton affinity in the ground state plus the difference in excitation energies of the base and its conjugate acid. The difference in excitation energies may be determined by analyzing the absorption spectra of the base and the photodissociation spectra of its conjugate acid. Gas phase absorption spectra of benzaldehyde, cyanobenzene and pyradine and their respective conjugate acids were presented and discussed. The greatest increase of proton affinity was reported in the excitation state of benzaldehyde with lesser increases reported for the excitation states of cyanobenzene and pyridine. (DDA)

  11. Dielectronic recombination and resonant transfer excitation processes for helium-like krypton

    Institute of Scientific and Technical Information of China (English)

    Hu Xiao-Li; Qu Yi-Zhi; Zhang Song-Bin; Zhang Yu

    2012-01-01

    The relativistic configuration interaction method is employed to calculate the dielectronic recombination (DR) cross sections of helium-like krypton via the 1s21nl' (n =2,3,...,15) resonances.Then,the resonant transfer excitation (RTE) processes of Kr34+ colliding with H,He,H2,and CHx (x =0-4) targets are investigated under the impulse approximation.The needed Compton profiles of targets are obtained from the Hartree-Fock wave functions.The RTE cross sections are strongly dependent on DR resonant energies and strengths,and the electron momentum distributions of the target.For H2 and H targets,the ratio of their RTE cross sections changes from 1.85 for the 1s2121' to 1.88 for other resonances,which demonstrates the weak molecular effects on the Compton profiles of H2.For CHx (x =0-4) targets,the main contribution to the RTE cross section comes from the carbon atom since carbon carries 6 electrons;as the number of hydrogen increases in CHx,the RTE cross section almost increases by the same value,displaying the strong separate atom character for the hydrogen.However,further comparison of the individual orbital contributions of C(2p,2s,ls) and CH4(1t2,2a1,1a1) to the RTE cross sections shows that the molecular effects induce differences of about 25.1%,19.9%,and 0.2% between 2p-1t2,2s-2a1,and 1s-1a1 orbitals,respectively.

  12. On the self-excitation mechanisms of Plasma Series Resonance oscillations in single- and multi-frequency capacitive discharges

    CERN Document Server

    Schuengel, Edmund; Korolov, Ihor; Derzsi, Aranka; Donko, Zoltan; Schulze, Julian

    2016-01-01

    The self-excitation of plasma series resonance (PSR) oscillations is a prominent feature in the current of low pressure capacitive radio frequency (RF) discharges. This resonance leads to high frequency oscillations of the charge in the sheaths and enhances electron heating. Up to now, the phenomenon has only been observed in asymmetric discharges. There, the nonlinearity in the voltage balance, which is necessary for the self-excitation of resonance oscillations with frequencies above the applied frequencies, is caused predominantly by the quadratic contribution to the charge-voltage relation of the plasma sheaths. Using PIC/MCC simulations of single- and multi- frequency capacitive discharges and an equivalent circuit model, we demonstrate that other mechanisms such as a cubic contribution to the charge-voltage relation of the plasma sheaths and the time dependent bulk electron plasma frequency can cause the self-excitation of PSR oscillations, as well. These mechanisms have been neglected in previous model...

  13. Resonance raman spectroscopic study of alumina-supported vanadium oxide catalysts with 220 and 287 nm excitation.

    Energy Technology Data Exchange (ETDEWEB)

    Kim, H. S.; Stair, P. C.; Chemical Sciences and Engineering Division; Northwestern Univ.

    2009-01-01

    We present detailed resonance Raman spectroscopic results excited at 220 and 287 nm for alumina-supported VO{sub x} catalysts. The anharmonic constant, harmonic wavenumber, anharmonic force constant, bond dissociation energy, and bond length change in the excited state for double bonded V{double_bond}O and single bonded V-O were obtained from fundamental and overtone frequencies. Totally symmetric and nontotally symmetric modes could be discerned and assigned on the basis of the overtone and combination progressions found in the resonance Raman spectra. Selective resonance enhancement of two different vibrational modes with two different excitation wavelengths was observed. This allowed us to establish a linear relationship between charge transfer energy and VO bond length and, consequently, to assign the higher-energy charge transfer band centered around 210?250 nm in the UV?vis spectra to the V{double_bond}O transition.

  14. Wave-packet dynamics in alkaline dimers. Investigation and control through coherent excitation with fs-pulses; Wellenpaketdynamik in Alkali-Dimeren. Untersuchung und Steuerung durch kohaerente Anregung mit fs-Pulsen

    Energy Technology Data Exchange (ETDEWEB)

    Sauer, F.N.B.

    2007-07-01

    During my PhD thesis I investigated alkaline dimers with coherent control in a molecular beam as well as with pump-probe spectroscopy in a magneto-optical trap (MOT). The aim of the coherent control experiments were the isotope selective ionization with phase- and amplitude-shaped fs-pulses. Chapter 4 described the gained results of isotope selective ionization of NaK and KRb in a molecular beam by using different pulse formers. For the NaK dimer was the reached optimization factor R{sub Ph} and {sub Ampl}{sup 770}=R{sub max}/R{sub min}=25 between maximization and minimization of the isotopomer ratio ({sup 23}Na{sup 39}K){sup +}/({sup 23}Na{sup 41}K){sup +} with phase and amplitude modulation of the fs-pulse with a central wavelength of {lambda}=770 nm. From the electronic ground-state X(1){sup 1}{sigma}{sup +};{nu}''=0 transfers a one-photon-excitation population in the first excited A(2) {sup 1}{sigma}{sup +} state. The coherent control experiment on KRb was used to maximize and minimize the isotopomer ratio ({sup 124}KRb){sup +}/({sup 126}KRb){sup +}. It was the first coherent control experiment with a spectral resolution of 1.84 cm{sup -1}/Pixel. For the phase and amplitude optimization was the received optimization factor between minimization and maximization of the isotopomer ratio R{sub Ph} and {sub Ampl}=R{sub max}/R{sub min}=7 at a central wavelength of 840 nm. The results showed a stepwise excitation process from the electronic ground-state in the first excited (2){sup 1}{sigma}{sup +} state with a further excitation, that is possible over three resonant energy potential curves into the ionic ground-state. In the second part of my thesis I realized pump-probe spectroscopy of Rb{sub 2} dimers in a dark SPOT. (orig.)

  15. Pygmy and Giant Dipole Resonances by Coulomb Excitation using a Quantum Molecular Dynamics model

    CERN Document Server

    Tao, C; Zhang, G Q; Cao, X G; Wang, D Q Fang H W

    2012-01-01

    Pygmy and Giant Dipole Resonance (PDR and GDR) in Ni isotopes have been investigated by Coulomb excitation in the framework of the Isospin-dependent Quantum Molecular Dynamics model (IQMD). The spectra of $\\gamma$ rays are calculated and the peak energy, the strength and Full Width at Half Maximum (FWHM) of GDR and PDR have been extracted. Their sensitivities to nuclear equation of state, especially to its symmetry energy term are also explored. By a comparison with the other mean-field calculations, we obtain the reasonable values for symmetry energy and its slope parameter at saturation, which gives an important constrain for IQMD model. In addition, we also studied the neutron excess dependence of GDR and PDR parameters for Ni isotopes and found that the energy-weighted sum rule (EWSR) $PDR_{m_1}/GDR_{m_1}%$ increases linearly with the neutron excess.

  16. Time Dependent Coupled Cluster Approach to Resonance Raman Excitation Profiles from General Anharmonic Surfaces

    Directory of Open Access Journals (Sweden)

    M. Durga Prasad

    2002-05-01

    Full Text Available Abstract: A time dependent coupled cluster approach to the calculation of Resonance Raman excitation profiles on general anharmonic surfaces is presented. The vibrational wave functions on the ground electronic surface are obtained by the coupled cluster method (CCM. It is shown that the propagation of the vibrational ground state on the upper surface is equivalent to propagation of the vacuum state by an effective hamiltonian generated by the similarity transformation of the vibrational hamiltonian of that surface by the CCM wave operator of the lower surface up to a normalization constant. This time propagation is carried out by the time-dependent coupled cluster method in a time dependent frame. Numerical studies are presented to asses the validity of the approach.

  17. Coherent excitation transferring via dark state in light-harvesting process

    CERN Document Server

    Dong, H; Sun, C P

    2011-01-01

    We study the light absorption and energy transferring in a donor-acceptor system with a bionic structure. In the optimal case with uniform couplings, it is found that the quantum dynamics of this seemingly complicated system is reduced as a three-level system of $\\Lambda$-type. With this observation, we show that the dark state based electromagnetically-induced transparency (EIT) effect could enhance the energy transfer efficiency, through a quantum interference effect suppressing the excited population of the donors. We estimate the optimal parameters of the system to achieve the maximum output power. The splitting behavior of maximum power may be used to explain the phenomenon that the photosynthesis systems mainly absorb two colors of light.

  18. The B850/B875 Photosynthetic Complex Ground and Excited State are Both Coherent

    CERN Document Server

    Squire, R H; Rubio, A; Ingles, J R; Cunningham, W A

    2016-01-01

    A bacterial photosynthetic light harvesting complex PLHC absorbs a photon and transfers this energy almost perfectly at room temperature RT to a Reaction Center RC, where charge separation occurs. While there are a number of possible light absorbers involved in this process, our focus is the B850 and B875 complexes. We propose that the dominant feature of the ground states in the B850 ring and the B875 open chain are pseudo one dimensional metals due to each bacteriochlorophyll a BChl containing a coordinated magnesium ion Mg2+. The Mg ion structure undergoes a static Peierls distortion that results in symmetry breaking that changes the even spacing of the Mg/BChl molecules comprising the chains to the experimentally observed Mg/BChl dimers. The results are charge density waves CDW, one for each type of the two complexes that result in an energy gap in the single particle electronic spectrum and coherent phonon s spanning the entire rings. The ground state CDWs seem to have two functions the first is to form ...

  19. Effect of Fermi surface nesting on resonant spin excitations in Ba(1-x)K(x)Fe2As2.

    Science.gov (United States)

    Castellan, J-P; Rosenkranz, S; Goremychkin, E A; Chung, D Y; Todorov, I S; Kanatzidis, M G; Eremin, I; Knolle, J; Chubukov, A V; Maiti, S; Norman, M R; Weber, F; Claus, H; Guidi, T; Bewley, R I; Osborn, R

    2011-10-21

    We report inelastic neutron scattering measurements of the resonant spin excitations in Ba(1-x)K(x)Fe(2)As(2) over a broad range of electron band filling. The fall in the superconducting transition temperature with hole doping coincides with the magnetic excitations splitting into two incommensurate peaks because of the growing mismatch in the hole and electron Fermi surface volumes, as confirmed by a tight-binding model with s(±)-symmetry pairing. The reduction in Fermi surface nesting is accompanied by a collapse of the resonance binding energy and its spectral weight, caused by the weakening of electron-electron correlations.

  20. Effect of Fermi surface nesting on resonant spin excitations in Ba{<_1-x}K{<_x}Fe{<_2}As{<_2}.

    Energy Technology Data Exchange (ETDEWEB)

    Castellan, J.-P.; Rosenkranz, S.; Goremychkin, E.A.; Chung, D.Y.; Todorov, I.S.; Kanatzidis, M.G.; Eremin, I.; Knolle, J.; Chubukov, A.V.; Maiti, s.; Norman, M.R.; Weber, F.; Claus, H.; Guidi, T.; Bewley, R.I.; Osborn, R. (Materials Science Division); (Northwestern Univ.); (Ruhr Univ.); (Max-Planck-Institut fur Physik komplexer Systeme); (Univ. Wisconsin-Madison); (Rutherford AppletonLab)

    2011-01-01

    We report inelastic neutron scattering measurements of the resonant spin excitations in Ba{sub 1-x}K{sub x}Fe{sub 2}As{sub 2} over a broad range of electron band filling. The fall in the superconducting transition temperature with hole doping coincides with the magnetic excitations splitting into two incommensurate peaks because of the growing mismatch in the hole and electron Fermi surface volumes, as confirmed by a tight-binding model with s{sub {+-}}-symmetry pairing. The reduction in Fermi surface nesting is accompanied by a collapse of the resonance binding energy and its spectral weight, caused by the weakening of electron-electron correlations.

  1. Feshbach Resonance due to Coherent {lambda}-{sigma} Coupling in {sup 7}{sub {lambda}}He

    Energy Technology Data Exchange (ETDEWEB)

    Mon, San San; Nwe, Tin Tin [Department of Physics, Mandalay University (Myanmar); Myint, Khin Swe [Pro-Rector, Mandalay University (Myanmar)], E-mail: pro-rector@mptmail.net.mm; Akaishi, Y. [College of Science and Technology, Nihon University, Chiba, Japan and RIKEN Nishina Center, Saitama (Japan)

    2010-04-01

    Coherent {lambda}-{sigma} coupling effect in {sup 7}{sub {lambda}}He is analyzed within three-body framework of two coupled channels, {lambda}-t-t and {sigma}-{tau}-t, where {tau} represents trinulceon which is either {sup 3}H or {sup 3}He. The hyperon-trinucleon (Y{tau}) and trinucleon-trinucleon ({tau}{tau}) interactions are derived by folding G-matrices of YN and NN interactions with trinucleon density distributions. It is found that the binding energy of {sup 7}{sub {lambda}}He is 4.04 MeV below the {lambda}+t+t threshold without {lambda}-{sigma} coupling and the binding energy is increased to 4.46 MeV when the coupling effect is included. This state is 7.85 MeV above the {sup 6}He+{lambda} threshold and it may have a chance to be observed as a Feshbach resonance in {sup 7}Li (e,e{sup '}K{sup +}){sup 7}{sub {lambda}}He experiment done at Jefferson Lab.

  2. Optical Coherence Tomography and Magnetic Resonance Imaging in Multiple Sclerosis and Neuromyelitis Optica Spectrum Disorder.

    Science.gov (United States)

    Manogaran, Praveena; Hanson, James V M; Olbert, Elisabeth D; Egger, Christine; Wicki, Carla; Gerth-Kahlert, Christina; Landau, Klara; Schippling, Sven

    2016-11-15

    Irreversible disability in multiple sclerosis (MS) and neuromyelitis optica spectrum disorder (NMOSD) is largely attributed to neuronal and axonal degeneration, which, along with inflammation, is one of the major pathological hallmarks of these diseases. Optical coherence tomography (OCT) is a non-invasive imaging tool that has been used in MS, NMOSD, and other diseases to quantify damage to the retina, including the ganglion cells and their axons. The fact that these are the only unmyelinated axons within the central nervous system (CNS) renders the afferent visual pathway an ideal model for studying axonal and neuronal degeneration in neurodegenerative diseases. Structural magnetic resonance imaging (MRI) can be used to obtain anatomical information about the CNS and to quantify evolving pathology in MS and NMOSD, both globally and in specific regions of the visual pathway including the optic nerve, optic radiations and visual cortex. Therefore, correlations between brain or optic nerve abnormalities on MRI, and retinal pathology using OCT, may shed light on how damage to one part of the CNS can affect others. In addition, these imaging techniques can help identify important differences between MS and NMOSD such as disease-specific damage to the visual pathway, trans-synaptic degeneration, or pathological changes independent of the underlying disease process. This review focuses on the current knowledge of the role of the visual pathway using OCT and MRI in patients with MS and NMOSD. Emphasis is placed on studies that employ both MRI and OCT to investigate damage to the visual system in these diseases.

  3. Quantum Generation Dynamics of Coherent Phonon in Semiconductors: Transient and Nonlinear Fano Resonance

    Science.gov (United States)

    Watanabe, Yohei; Hino, Ken-Ichi; Hase, Muneaki; Maeshima, Nobuya

    The coherent phonon (CP) generation is one of the representative phenomena induced by ultrashort pulsed laser. In particular, in the initial stage of the CP generation in lightly n-doped Si, the vestige of Fano resonance (FR) manifested in a flash was observed in time-resolved spectroscopy experiments, in which it was speculated that this phenomenon results from the birth of transient polaronic quasiparticles composed of electrons and phonons strongly interacting each other. This study is aimed at constructing a fully-quantum-mechanical model for the CP generation and tracking the origin of the transient FR. We calculate two physical quantities in both of polar and non-polar semiconductors such as GaAs and undoped Si. One is a retarded longitudinal susceptibility which allows one to calculate a transient induced photoemission spectrum. The other is the Fourier-transform of LO-phonon displacement into frequency domain. We have succeeded in showing that the transient FR is exclusively caused in Si in harmony with the experiments, though, not observed in GaAs.

  4. Theoretical investigation of nonlinear resonances in a carbon nanotube cantilever with a tip-mass under electrostatic excitation

    Science.gov (United States)

    Kim, I. K.; Lee, S. I.

    2013-09-01

    The nonlinear dynamics of a resonating carbon nanotube (CNT) cantilever having an attached mass at the tip ("tip mass") were investigated by incorporating electrostatic forces and intermolecular interactions between the CNT and a conducting plane surface. This work enables applications of CNT resonating sensors for tiny mass detection and provides a better understanding of the dynamics of CNT cantilevers. The effect of tip mass on a resonating CNT cantilever is normally characterized by the fundamental frequency shift in the linear resonance regime. However, there are more complex dynamics in the nonlinear resonance regime, such as secondary resonances with parametric excitation. The latter have been limited to nano-cantilevers without tip mass or to axially excited micro-beams. To analyze the nonlinear dynamics, we developed a differential equation model that includes both geometric and inertial nonlinear terms for the large vibration amplitudes at increasing drive forces. In our approach, we used Galerkin discretization techniques and numerical integration methods. The CNT cantilever exhibited complex nonlinear responses due to the applied AC and DC voltages and various tip masses. The nonlinear model had a softer response for increasing tip mass than those of the linear model with the same driving conditions. At low applied voltages, the cantilever had linear amplitude and phase responses at primary and secondary superharmonic resonance frequencies. The response branches were softened at the primary resonance through saddle-node (SN) bifurcation from harmonic electrostatic excitation at higher applied voltages. After SN bifurcation, the lower branch of the solution near resonance became unstable. In addition, theoretical analyses were performed on more complex nonlinear responses and stability changes with tip mass variations, such as period-doubling (PD) bifurcation at subharmonic resonance frequencies.

  5. Resonant transfer of one- and two-photon excitations in quantum dot-bacteriorhodopsin complexes

    Science.gov (United States)

    Krivenkov, V. A.; Samokhvalov, P. S.; Bilan, R. S.; Chistyakov, A. A.; Nabiev, I. R.

    2017-01-01

    Light-sensitive protein bacteriorhodopsin (BR), which is capable of electrical response upon exposure to light, is a promising material for photovoltaics and optoelectronics. However, the rather narrow absorption spectrum of BR does not allow achieving efficient conversion of the light energy in the blue and infrared spectral regions. This paper summarizes the results of studies showing the possibility of extending the spectral region of the BR function by means of the Förster resonance energy transfer (FRET) from CdSe/ZnS quantum dots (QDs), which have a broad spectrum of one-photon absorption and a large twophoton absorption cross section (TPACS), to BR upon one- and two-photon excitation. In particular, it is shown that, on the basis of QDs and BR-containing purple membranes, it is possible to create electrostatically associated bio-nano hybrid systems in which FRET is implemented. In addition, the large TPACS of QDs, which is two orders of magnitude larger than those of BR and organic dyes, opens up a means for selective two-photon excitation of synthesized bio-nano hybrid complexes. On the basis of the results of this work, the spectral region in which BR converts the light energy into electrical energy can be extended from the UV to near-IR region, creating new opportunities for the use of this material in photovoltaics and optoelectronics.

  6. Multispectral code excited linear prediction coding and its application in magnetic resonance images.

    Science.gov (United States)

    Hu, J H; Wang, Y; Cahill, P T

    1997-01-01

    This paper reports a multispectral code excited linear prediction (MCELP) method for the compression of multispectral images. Different linear prediction models and adaptation schemes have been compared. The method that uses a forward adaptive autoregressive (AR) model has been proven to achieve a good compromise between performance, complexity, and robustness. This approach is referred to as the MFCELP method. Given a set of multispectral images, the linear predictive coefficients are updated over nonoverlapping three-dimensional (3-D) macroblocks. Each macroblock is further divided into several 3-D micro-blocks, and the best excitation signal for each microblock is determined through an analysis-by-synthesis procedure. The MFCELP method has been applied to multispectral magnetic resonance (MR) images. To satisfy the high quality requirement for medical images, the error between the original image set and the synthesized one is further specified using a vector quantizer. This method has been applied to images from 26 clinical MR neuro studies (20 slices/study, three spectral bands/slice, 256x256 pixels/band, 12 b/pixel). The MFCELP method provides a significant visual improvement over the discrete cosine transform (DCT) based Joint Photographers Expert Group (JPEG) method, the wavelet transform based embedded zero-tree wavelet (EZW) coding method, and the vector tree (VT) coding method, as well as the multispectral segmented autoregressive moving average (MSARMA) method we developed previously.

  7. d-d excitations in bilayer manganites probed by resonant inelastic x-ray scattering.

    Energy Technology Data Exchange (ETDEWEB)

    Weber, F.; Rosenkranz, S.; Castellan, J.-P.; Osborn, R.; Mitchell, J. F.; Zheng, H.; Case, D.; Kim, J. H.; Gog, T.

    2010-01-01

    We report a high-resolution resonant inelastic x-ray scattering investigation of the bilayer manganites La{sub 2-2x}Sr{sub 1+2x}Mn{sub 2}O{sub 7} with x=0.36 and 0.5. The momentum dependence along the crystallographic (110) direction for energy losses 1 eV {le} {Delta}E {le} 15 eV has been measured in detail with the data analysis focusing on the energy-loss region 1 eV {le} {Delta}E {le} 5 eV, which includes a strong peak located at {Delta}E {approx} 2 eV. We observe a clear dispersion of up to 0.5 eV in the measured q range, which is direct evidence of the nonlocal character of this excitation. Further, we found that the intensity in this low-energy region strongly depends on both the reduced wave vector q=(h,h,0), h=0.1-0.5, and temperature, i.e., different ordered phases. Results can be explained via an intersite d-d charge-transfer excitation, proposed for pseudocubic manganites, where the hopping rate is strongly increased (decreased) by ferromagnetic (antiferromagnetic) alignment of neighboring in-plane Mn ion core spins.

  8. Resonantly excited exciton dynamics in two-dimensional MoSe2 monolayers

    Science.gov (United States)

    Scarpelli, L.; Masia, F.; Alexeev, E. M.; Withers, F.; Tartakovskii, A. I.; Novoselov, K. S.; Langbein, W.

    2017-07-01

    We report on the exciton and trion density dynamics in a single layer of MoSe2, resonantly excited and probed using three-pulse four-wave mixing (FWM), at temperatures from 300 K to 77 K. A multiexponential third-order response function for amplitude and phase of the heterodyne-detected FWM signal including four decay processes is used to model the data. We provide a consistent interpretation within the intrinsic band structure, not requiring the inclusion of extrinsic effects. We find an exciton radiative lifetime in the subpicosecond range consistent to what has been recently reported by Jakubczyk et al. [Nano Lett. 16, 5333 (2016), 10.1021/acs.nanolett.6b01060]. After the dominating radiative decay, the remaining exciton density, which has been scattered from the initially excited direct spin-allowed radiative state into dark states of different nature by exciton-phonon scattering or disorder scattering, shows a slower dynamics, covering 10-ps to 10-ns time scales. This includes direct spin-allowed transitions with larger in-plane momentum, as well as indirect and spin-forbidden exciton states. We find that exciton-exciton annihilation is not relevant in the observed dynamics, in variance from previous finding under nonresonant excitation. The trion density at 77 K reveals a decay of the order of 1 ps, similar to what is observed for the exciton. After few tens of picoseconds, the trion dynamics resembles the one of the exciton, indicating that trion ionization occurs on this time scale.

  9. Spectral narrowing of coherent population trapping resonance in laser-cooled and room-temperature atomic gas

    Indian Academy of Sciences (India)

    S Pradhan; S Mishra; R Behera; N Kawade; A K Das

    2014-02-01

    We have investigated coherent population trapping (CPT) in laser-cooled as well as room-temperature (with and without buffer gas) rubidium atoms. The characteristic broad signal profile emerging from the two-photon Raman resonance for room-temperature atomic vapour is consistent with the theoretical calculation incorporating associated thermal averaging. The spectral width of the dark resonance obtained with cold atoms is found to be broadened, compared to roomtemperature vapour cell, due to the feeble role played by thermal averaging, although the cold atomic sample significantly overcomes the limitation of the transit time broadening. An alternative way to improve transit time is to use a buffer gas, with which we demonstrate that the coherent population trapping signal width is reduced to < 540 Hz.

  10. Parameter Diversity Induced Multiple Spatial Coherence Resonances and Spiral Waves in Neuronal Network with and Without Noise

    Institute of Scientific and Technical Information of China (English)

    李玉叶; 贾冰; 古华光; 安书成

    2012-01-01

    Diversity in the neurons and noise are inevitable in the real neuronal network.In this paper,parameter diversity induced spiral waves and multiple spatial coherence resonances in a two-dimensional neuronal network without or with noise are simulated.The relationship between the multiple resonances and the multiple transitions between patterns of spiral waves are identified.The coherence degrees induced by the diversity are suppressed when noise is introduced and noise density is increased.The results suggest that natural nervous system might profit from both parameter diversity and noise,provided a possible approach to control formation and transition of spiral wave by the cooperation between the diversity and noise.

  11. Generation of highly vibrationally excited H2 and detection by 2+1 resonantly enhanced multiphoton ionization

    Science.gov (United States)

    Robie, Daniel C.; Jusinski, Leonard E.; Bischel, William K.

    1990-02-01

    We report the first detection by optical means of highly vibrationally excited H2 X1Σ+g(vx=6-11). Vibrationally excited H2 was generated using a recently discovered hot-wire effect in H2 gas, and was detected in 40 bands with 2+1 resonantly enhanced multiphoton ionization via the EF state (vEF=0-14). Rotational temperatures are in the range 200-650 K, well below that required for thermal excitation of the observed vibrational levels.

  12. A Resonantly-Excited Disk-Oscillation Model of High-Frequency QPOs of Microquasars

    CERN Document Server

    Kato, Shoji

    2012-01-01

    A possible model of twin high-frequency QPOs (HF QPOs) of microquasars is examined. The disk is assumed to have global magnetic fields and to be deformed with a two-armed pattern. In this deformed disk, set of a two-armed ($m=2$) vertical p-mode oscillation and an axisymmetric ($m=0$) g-mode oscillation are considered. They resonantly interact through the disk deformation when their frequencies are the same. This resonant interaction amplifies the set of the above oscillations in the case where these two oscillations have wave energies of opposite signs. These oscillations are assumed to be excited most efficiently in the case where the radial group velocities of these two waves vanish at the same place. The above set of oscillations is not unique, depending on the node number, $n$, of oscillations in the vertical direction. We consider that the basic two sets of oscillations correspond to the twin QPOs. The frequencies of these oscillations depend on disk parameters such as strength of magnetic fields. For o...

  13. Double resonant excitation of the second harmonic of terahertz raditation in dielectric-graphene layered metamaterials

    Science.gov (United States)

    Rapoport, Yu; Grimalsky, V.; Lavrinenko, A. V.; Boardman, A.

    2017-09-01

    Excitation of the second harmonic of THz radiation is investigated theoretically in the planar multilayered structure dielectric-graphene-dielectric-graphene-…. It is studied the case of the oblique incidence of the s-polarized fundamental wave, where the electric field is parallel to the interfaces, and generation of the p-type second harmonic wave occurs. The original concept is proposed to employ the double resonance arrangement for the effective generation of the second harmonic. The double resonant case can be realized when a high-permittivity dielectric is at the input of the structure and the vacuum is at the output. The high efficiency is demonstrated; the second harmonic reflectance coefficient is ≥0.01 under realistic values of the collision frequency in graphene >1012 s-1. Such a great efficiency, which is four-five orders of magnitude higher than reported for the graphene-dielectric structures previously, is proposed for the first time. To compute the nonlinear surface currents, two approaches were used, the kinetic and the hydrodynamic. A qualitative agreement between two approaches, proven in the present modeling, ensures an applicability of the results.

  14. Family of graphene-assisted resonant surface optical excitations for terahertz devices

    Science.gov (United States)

    Lin, I-Tan; Liu, Jia-Ming; Tsai, Hsin-Cheng; Wu, Kaung-Hsiung; Syu, Jheng-Yuan; Su, Ching-Yuan

    2016-01-01

    The majority of the proposed graphene-based THz devices consist of a metamaterial that can optically interact with graphene. This coupled graphene-metamaterial system gives rise to a family of resonant modes such as the surface plasmon polariton (SPP) modes of graphene, the geometrically induced SPPs, also known as the spoof SPP modes, and the Fabry-Perot (FP) modes. In the literature, these modes are usually considered separately as if each could only exist in one structure. By contrast, in this paper, we show that even in a simple metamaterial structure such as a one-dimensional (1D) metallic slit grating, these modes all exist and can potentially interact with each other. A graphene SPP-based THz device is also fabricated and measured. Despite the high scattering rate, the effective SPP resonances can still be observed and show a consistent trend between the effective frequency and the grating period, as predicted by the theory. We also find that the excitation of the graphene SPP mode is most efficient in the terahertz spectral region due to the Drude conductivity of graphene in this spectral region. PMID:27739504

  15. Real-time monitoring of human blood clotting using a lateral excited film bulk acoustic resonator

    Science.gov (United States)

    Chen, Da; Wang, Jingjng; Wang, Peng; Guo, Qiuquan; Zhang, Zhen; Ma, Jilong

    2017-04-01

    Frequent assay of hemostatic status is an essential issue for the millions of patients using anticoagulant drugs. In this paper, we presented a micro-fabricated film bulk acoustic sensor for the real-time monitoring of blood clotting and the measurement of hemostatic parameters. The device was made of an Au/ZnO/Si3N4 film stack and excited by a lateral electric field. It operated under a shear mode resonance with the frequency of 1.42 GHz and had a quality factor of 342 in human blood. During the clotting process of blood, the resonant frequency decreased along with the change of blood viscosity and showed an apparent step-ladder curve, revealing the sequential clotting stages. An important hemostatic parameter, prothrombin time, was quantitatively determined from the frequency response for different dilutions of the blood samples. The effect of a typical anticoagulant drug (heparin) on the prothrombin time was exemplarily shown. The proposed sensor displayed a good consistency and clinical comparability with the standard coagulometric methods. Thanks to the availability of direct digital signals, excellent potentials of miniaturization and integration, the proposed sensor has promising application for point-of-care coagulation technologies.

  16. Experimental and theoretical comparison of different optical excitation schemes for a compact coherent population trapping Rb vapor clock

    Science.gov (United States)

    Warren, Z.; Shahriar, M. S.; Tripathi, R.; Pati, G. S.

    2017-08-01

    We have investigated, theoretically as well as experimentally, the relative merits and demerits of using three different optical configurations for a compact coherent population trapping (CPT) vapor clock using 87Rb. These correspond to the following choices of polarizations for the two Raman beams: \\text{lin} \\parallel \\text{lin} , (σ,~σ ), and push-pull optical pumping (PPOP), applied on the D1 manifold. We have used a multi-level atomic model to study the dependence of the CPT spectrum on axial as well as transverse magnetic fields for these three schemes. Corresponding experimental studies have been performed using a laboratory scale CPT clock employing a two cm long, isotopically pure rubidium cell, loaded with a buffer gas. We observed a CPT contrast close to 20% with a sub-kilohertz linewidth by adopting the PPOP scheme. We discuss the strengths and weaknesses of each of the three optical excitation schemes, and present frequency-stability measurement data for the prototype clock.

  17. Coherent phonon excitation and linear thermal expansion in structural dynamics and ultrafast electron diffraction of laser-heated metals

    Science.gov (United States)

    Tang, Jau

    2008-04-01

    In this study, we examine the ultrafast structural dynamics of metals induced by a femtosecond laser-heating pulse as probed by time-resolved electron diffraction. Using the two-temperature model and the Grüneisen relationship we calculate the electron temperature, phonon temperature, and impulsive force at each atomic site in the slab. Together with the Fermi-Pasta-Ulam anharmonic chain model we calculate changes of bond distance and the peak shift of Bragg spots or Laue rings. A laser-heated thin slab is shown to exhibit "breathing" standing-wave behavior, with a period equal to the round-trip time for sound wave and a wavelength twice the slab thickness. The peak delay time first increases linearly with the thickness (<70nm for aluminum and <200nm for gold), but becomes less dependent if further thickness increases. Coherent phonon excitation and propagation from the stressed bulk atoms due to impulsive forces as well as the linear thermal expansion due to lattice temperature jump are shown to contribute to the overall structural changes. Differences between these two mechanisms and their dependence on film thickness and other factors are discussed.

  18. Vibrational spectroscopy of the electronically excited state. 4. Nanosecond and picosecond time-resolved resonance Raman spectroscopy of carotenoid excited states

    Energy Technology Data Exchange (ETDEWEB)

    Dallinger, R.F.; Farquharson, S.; Woodruff, W.H.; Rodgers, M.A.J.

    1981-12-16

    Resonance Raman and electronic absorption spectra are reported for the S/sub 0/ and T/sub 1/ states of the carotenoids ..beta..-carotene, zeaxanthin, echinenone, canthaxanthin, dihydroxylycopene, astaxanthin, decapreno(C/sub 50/)-..beta..-carotene, ..beta..-apo-8'-carotenal, and ethyl ..beta..-apo-8'-carotenoate. The results reveal qualitatively similar ground-state spectra and similar frequency shifts in all observed resonance Raman modes between S/sub 0/ and T/sub 1/, regardless of carotenoid structure. Examinations of the relationship of the putative C--C and C==C frequencies in S/sub 0/ and T/sub 1/ reveals anomalous shifts to lower frequency in the ''single-bond'' mode upon electronic excitation. These shifts may be due to molecular distortions in the excited state which force changes in molecular motions comprising the observed modes. However, another possibility requiring no distortion is that the interaction (off-diagonal) force constants connecting the C--C and C==C modes change sign upon electronic excitation. This latter phenomenon may provide a unitary explanation for the ''anomalous'' frequency shifts in the C--C and C==C modes, both in the T/sub 1/ states of carotenoids and in the S/sub 1/ states of simpler polyenes, without postulating large, unpredicted structural changes upon excitation or general errors in existing vibrational or theoretical analyses. Resonance Raman and absorbance studies with 35-ps time resolution suggest that S/sub 1/ lifetime (of the /sup 1/B/sub u/ and/or the /sup 1/A/sub g/* states) of ..beta..-carotene in benzene is less than 1 ps.

  19. Parallel ferromagnetic resonance and spin-wave excitation in exchange-biased NiFe/IrMn bilayers

    Energy Technology Data Exchange (ETDEWEB)

    Sousa, Marcos Antonio de, E-mail: marcossharp@gmail.com [Instituto de Física, Universidade Federal de Goiás, Goiânia, 74001-970 (Brazil); Pelegrini, Fernando [Instituto de Física, Universidade Federal de Goiás, Goiânia, 74001-970 (Brazil); Alayo, Willian [Departamento de Física, Universidade Federal de Pelotas, Pelotas, 96010-900 (Brazil); Quispe-Marcatoma, Justiniano; Baggio-Saitovitch, Elisa [Centro Brasileiro de Pesquisas Físicas, Rio de Janeiro, 22290-180 (Brazil)

    2014-10-01

    Ferromagnetic Resonance study of sputtered Ru(7 nm)/NiFe(t{sub FM})/IrMn(6 nm)/Ru(5 nm) exchange-biased bilayers at X and Q-band microwave frequencies reveals the excitation of spin-wave and NiFe resonance modes. Angular variations of the in-plane resonance fields of spin-wave and NiFe resonance modes show the effect of the unidirectional anisotropy, which is about twice larger for the spin-wave mode due to spin pinning at the NiFe/IrMn interface. At Q-band frequency the angular variations of in-plane resonance fields also reveal the symmetry of a uniaxial anisotropy. A modified theoretical model which also includes the contribution of a rotatable anisotropy provides a good description of the experimental results.

  20. Excitation of the Roper resonance in single- and double-pion production in nucleon-nucleon collisions⋆

    Science.gov (United States)

    Skorodko, T.; Bashkanov, M.; Bogoslawsky, D.; Calen, H.; Cappellaro, F.; Clement, H.; Demiroers, L.; Doroshkevich, E.; Duniec, D.; Ekström, C.; Franssen, K.; Gustafsson, L.; Höistad, B.; Ivanov, G.; Jacewicz, M.; Jiganov, E.; Johansson, T.; Khakimova, O.; Kaskulov, M.; Keleta, S.; Koch, I.; Kren, F.; Kullander, S.; Kupść, A.; Kuznetsov, A.; Marciniewski, P.; Meier, R.; Morosov, B.; Pauly, C.; Petterson, H.; Petukhov, Y.; Povtorejko, A.; Schönning, K.; Scobel, W.; Shwartz, B.; Sopov, V.; Stepeniak, J.; Thörngren-Engblom, P.; Tikhomirov, V.; Wagner, G. J.; Wolke, M.; Yamamoto, A.; Zabierowski, J.; Złomanczuk, J.

    2008-03-01

    In most investigations the Roper resonance is sensed only very indirectly via complex partial-wave analyses. We find indications for its excitation in the invariant nπ+ mass spectrum of the pp → npπ+ reaction at M ≈ 1360 MeV with a width of ≈ 150 MeV . The values fit very favorably to the most recent phase shift results as well as to the observations at BES. In the near-threshold two-pion production pp → ppπ0π0 , where the Roper excitation and its subsequent decays via the routes N * → Δπ → Nππ and N * → Nσ are the only dominant processes, we find its direct decay into the Nσ channel to be the by far dominating decay process --in favor of a monopole excitation of the Roper resonance.

  1. Excitation of the Roper resonance in single- and double-pion production in nucleon-nucleon collisions

    Science.gov (United States)

    Skorodko, T.; Bashkanov, M.; Bogoslawsky, D.; Calen, H.; Cappellaro, F.; Clement, H.; Demiroers, L.; Doroshkevich, E.; Duniec, D.; Ekström, C.; Franssen, K.; Gustafsson, L.; Höistad, B.; Ivanov, G.; Jacewicz, M.; Jiganov, E.; Johansson, T.; Khakimova, O.; Kaskulov, M.; Keleta, S.; Koch, I.; Kren, F.; Kullander, S.; Kupść, A.; Kuznetsov, A.; Marciniewski, P.; Meier, R.; Morosov, B.; Pauly, C.; Petterson, H.; Petukhov, Y.; Povtorejko, A.; Schönning, K.; Scobel, W.; Shwartz, B.; Sopov, V.; Stepeniak, J.; Thörngren-Engblom, P.; Tikhomirov, V.; Wagner, G. J.; Wolke, M.; Yamamoto, A.; Zabierowski, J.; Złomanczuk, J.

    In most investigations the Roper resonance is sensed only very indirectly via complex partial-wave analyses. We find indications for its excitation in the invariant nπ + mass spectrum of the pp → npπ + reaction at M ≈ 1360MeV with a width of ≈ 150 MeV. The values fit very favorably to the most recent phase shift results as well as to the observations at BES. In the near-threshold two-pion production pp → ppπ 0 π 0, where the Roper excitation and its subsequent decays via the routes N* → Δπ → Nππ and N* → Nσ are the only dominant processes, we find its direct decay into the Nσ channel to be the by far dominating decay process —in favor of a monopole excitation of the Roper resonance.

  2. X-Ray Polarization Optics and Coherent Nuclear Resonance Scattering Using Synchrotron Radiation.

    Science.gov (United States)

    Shastri, Sarvjit Devdat

    1995-01-01

    Two projects, both involving X-ray scattering with synchrotron radiation, are presented in this dissertation. (1) A system of diffracting perfect crystals for the generation of variable, elliptically polarized X-rays was tested at the Cornell High Energy Synchrotron Source under the conditions of a standard undulator source. The phase retarding optical component was a 4-bounce, Ge(220) Bragg reflection channel -cut crystal. The full polarization state (density matrix) of the output beam, including the circular polarization purity P_3, was determined using the multiple-beam Bragg diffraction technique with a GaAs crystal polarimeter and was found to agree with calculations. In addition to measuring the optics' efficiency, the ability to scan the system in energy, while frequently reversing the circular helicity, was demonstrated at the vicinity of the Fe K-edge at 7.1 keV. The setup was applied to a circular magnetic X-ray dichroism measurement. (2) The time distribution of delayed photons from resonant forward scattering of 14.4 keV synchrotron radiation pulses by ^{57}Fe nuclei was investigated over the temperature range from 9 K to just above the Curie point at 1043 K, with particular attention to precise measurements of the Lamb-Mossbauer factor f_{LM } ~ e^{- } , whose change was determined from its influence on the "speed-up" of coherent decay. Apart from its importance in Mossbauer effect studies, knowing the temperature dependence of f_{LM} can be valuable for studies of lattice dynamics and structural phase transitions. The change in the nuclear hyperfine splitting was also measured. The synchrotron technique has precision-enhancing advantages over conventional Mossbauer spectroscopy methods employing radioactive sources because dealing with source effects and absolute intensity measurements is eliminated. The results also straightforwardly illustrate an interesting principle concerning the temperature dependence of scattering --that for "slow" resonance

  3. Optical Coherence Tomography and Magnetic Resonance Imaging in Multiple Sclerosis and Neuromyelitis Optica Spectrum Disorder

    Science.gov (United States)

    Manogaran, Praveena; Hanson, James V. M.; Olbert, Elisabeth D.; Egger, Christine; Wicki, Carla; Gerth-Kahlert, Christina; Landau, Klara; Schippling, Sven

    2016-01-01

    Irreversible disability in multiple sclerosis (MS) and neuromyelitis optica spectrum disorder (NMOSD) is largely attributed to neuronal and axonal degeneration, which, along with inflammation, is one of the major pathological hallmarks of these diseases. Optical coherence tomography (OCT) is a non-invasive imaging tool that has been used in MS, NMOSD, and other diseases to quantify damage to the retina, including the ganglion cells and their axons. The fact that these are the only unmyelinated axons within the central nervous system (CNS) renders the afferent visual pathway an ideal model for studying axonal and neuronal degeneration in neurodegenerative diseases. Structural magnetic resonance imaging (MRI) can be used to obtain anatomical information about the CNS and to quantify evolving pathology in MS and NMOSD, both globally and in specific regions of the visual pathway including the optic nerve, optic radiations and visual cortex. Therefore, correlations between brain or optic nerve abnormalities on MRI, and retinal pathology using OCT, may shed light on how damage to one part of the CNS can affect others. In addition, these imaging techniques can help identify important differences between MS and NMOSD such as disease-specific damage to the visual pathway, trans-synaptic degeneration, or pathological changes independent of the underlying disease process. This review focuses on the current knowledge of the role of the visual pathway using OCT and MRI in patients with MS and NMOSD. Emphasis is placed on studies that employ both MRI and OCT to investigate damage to the visual system in these diseases. PMID:27854301

  4. Optical Coherence Tomography and Magnetic Resonance Imaging in Multiple Sclerosis and Neuromyelitis Optica Spectrum Disorder

    Directory of Open Access Journals (Sweden)

    Praveena Manogaran

    2016-11-01

    Full Text Available Irreversible disability in multiple sclerosis (MS and neuromyelitis optica spectrum disorder (NMOSD is largely attributed to neuronal and axonal degeneration, which, along with inflammation, is one of the major pathological hallmarks of these diseases. Optical coherence tomography (OCT is a non-invasive imaging tool that has been used in MS, NMOSD, and other diseases to quantify damage to the retina, including the ganglion cells and their axons. The fact that these are the only unmyelinated axons within the central nervous system (CNS renders the afferent visual pathway an ideal model for studying axonal and neuronal degeneration in neurodegenerative diseases. Structural magnetic resonance imaging (MRI can be used to obtain anatomical information about the CNS and to quantify evolving pathology in MS and NMOSD, both globally and in specific regions of the visual pathway including the optic nerve, optic radiations and visual cortex. Therefore, correlations between brain or optic nerve abnormalities on MRI, and retinal pathology using OCT, may shed light on how damage to one part of the CNS can affect others. In addition, these imaging techniques can help identify important differences between MS and NMOSD such as disease-specific damage to the visual pathway, trans-synaptic degeneration, or pathological changes independent of the underlying disease process. This review focuses on the current knowledge of the role of the visual pathway using OCT and MRI in patients with MS and NMOSD. Emphasis is placed on studies that employ both MRI and OCT to investigate damage to the visual system in these diseases.

  5. Relaxation Process of Excitonic Molecules in CuCl under the Two-Photon Resonant Excitation. II. Transverse Relaxation

    Science.gov (United States)

    Itoh, Tadashi; Katohno, Takashi; Kirihara, Toshio; Ueta, Masayasu

    1984-02-01

    Under the off-resonant excitation at the slightly higher energy side of the giant two-photon absorption band (GTA) for the direct generation of excitonic molecules (EM) in CuCl, new narrow emission bands designated as XT and XL have been found in the energy region of the MT and ML broad bands, respectively. Their photon energies increase with the decrease of the pump photon energy from the higher-energy side of the resonance and finally, at the on-resonant excitation, their bands merge into MT0 and ML0 bands, respectively, previously reported by Mita et al. Based on the detailed studies on these bands, it is found that there exists a certain kind of transverse relaxation process which acts on the EM just after their generation by the GTA and brings about the X emission as a hot luminescence.

  6. Ultrafast fluorescence resonance energy transfer in a bile salt aggregate: Excitation wavelength dependence

    Indian Academy of Sciences (India)

    Ujjwal Mandal; Subhadip Ghosh; Dibyendu Kumar Das; Aniruddha Adhikari; Shantanu Dey; Kankan Bhattacharyya

    2008-01-01

    Fluorescence resonance energy transfer (FRET) from Coumarin 153 (C153) to Rhodamine 6G (R6G) in a secondary aggregate of a bile salt (sodium deoxycholate, NaDC) is studied by femtosecond up-conversion. The emission spectrum of C153 in NaDC is analysed in terms of two spectra-one with emission maximum at 480 nm which corresponds to a non-polar and hydrophobic site and another with maximum at ∼ 530 nm which arises from a polar hydrophilic site. The time constants of FRET were obtained from the rise time of the emission of the acceptor (R6G). In the NaDC aggregate, FRET occurs in multiple time scales -4 ps and 3700 ps. The 4 ps component is assigned to FRET from a donor (D) to an acceptor (A) held at a close distance (DA ∼ 17 Å) inside the bile salt aggregate. The 3700 ps component corresponds to a donor-acceptor distance ∼ 48 Å. The long (3700 ps) component may involve diffusion of the donor. With increase in the excitation wavelength (ex) from 375 to 435 nm, the relative contribution of the ultrafast component of FRET (∼ 4 ps) increases from 3 to 40% with a concomitant decrease in the contribution of the ultraslow component (∼3700 ps) from 97 to 60%. The ex dependence is attributed to the presence of donors at different locations. At a long ex (435 nm) donors in the highly polar peripheral region are excited. A short ex (375 nm) `selects’ donor at a hydrophobic location.

  7. Multidimensional Time-Resolved Spectroscopy of Vibrational Coherence in Biopolyenes

    Science.gov (United States)

    Buckup, Tiago; Motzkus, Marcus

    2014-04-01

    Multidimensional femtosecond time-resolved vibrational coherence spectroscopy allows one to investigate the evolution of vibrational coherence in electronic excited states. Methods such as pump-degenerate four-wave mixing and pump-impulsive vibrational spectroscopy combine an initial ultrashort laser pulse with a nonlinear probing sequence to reinduce vibrational coherence exclusively in the excited states. By carefully exploiting specific electronic resonances, one can detect vibrational coherence from 0 cm-1 to over 2,000 cm-1 and map its evolution. This review focuses on the observation and mapping of high-frequency vibrational coherence for all-trans biological polyenes such as β-carotene, lycopene, retinal, and retinal Schiff base. We discuss the role of molecular symmetry in vibrational coherence activity in the S1 electronic state and the interplay of coupling between electronic states and vibrational coherence.

  8. Multidimensional time-resolved spectroscopy of vibrational coherence in biopolyenes.

    Science.gov (United States)

    Buckup, Tiago; Motzkus, Marcus

    2014-01-01

    Multidimensional femtosecond time-resolved vibrational coherence spectroscopy allows one to investigate the evolution of vibrational coherence in electronic excited states. Methods such as pump-degenerate four-wave mixing and pump-impulsive vibrational spectroscopy combine an initial ultrashort laser pulse with a nonlinear probing sequence to reinduce vibrational coherence exclusively in the excited states. By carefully exploiting specific electronic resonances, one can detect vibrational coherence from 0 cm(-1) to over 2,000 cm(-1) and map its evolution. This review focuses on the observation and mapping of high-frequency vibrational coherence for all-trans biological polyenes such as β-carotene, lycopene, retinal, and retinal Schiff base. We discuss the role of molecular symmetry in vibrational coherence activity in the S1 electronic state and the interplay of coupling between electronic states and vibrational coherence.

  9. Theoretical vibrational-excitation cross sections and rate coefficients for electron-impact resonant collisions involving rovibrationally excited N2 and NO molecules

    CERN Document Server

    Laporta, V; Wadehra, J M

    2012-01-01

    Electron-impact vi->vf vibrational excitations cross sections, involving rovibrationally excited N_{2}(v_{i}, J) and NO(v_{i}, J) molecules (fixed J), are calculated for collisions occurring through the nitrogen resonant electronic state N_{2}^{-} (X ^{2}\\Pi_{g}), and the three resonant states of nitric oxide NO^{-}(^{3}\\Sigma^{-},^{1} \\Delta,^{1} \\Sigma^{+}). Complete sets of cross sections have been obtained for all possible transitions involving 68 vibrational levels of N2(X ^{1}\\Sigma^{+}_{g}) and 55 levels of NO(X ^{2}\\Pi), for the incident electron energy between 0.1 and 10 eV. In order to study the rotational motion in the resonant processes, cross sections have been also computed for rotationally elastic transitions characterized by the rotational quantum number J running from 0 through 150. The calculations are performed within the framework of the local complex potential model, by using potentials energies and widths optimized in order to reproduce the experimental cross sections available in litera...

  10. Resonant excitation of waves by a spiraling ion beam on the large plasma device

    Science.gov (United States)

    Tripathi, Shreekrishna

    2015-11-01

    The resonant interaction between energetic-ions and plasma waves is a fundamental topic of importance in the space, controlled magnetic-fusion, and laboratory plasma physics. We report new results on the spontaneous generation of traveling shear Alfvén waves and high-harmonic beam-modes in the lower-hybrid range of frequencies by an intense ion beam. In particular, the role of Landau and Doppler-shifted ion-cyclotron resonances (DICR) in extracting the free-energy from the ion-beam and destabilizing Alfvén waves was explored on the Large Plasma Device (LAPD). In these experiments, single and dual-species magnetized plasmas (n ~1010 -1012 cm-3, Te ~ 5.0-10.0 eV, B = 0.6-1.8 kG, He+ and H+ ions, 19.0 m long, 0.6 m diameter) were produced and a spiraling hydrogen ion beam (5-15 keV, 2-10 A, beam-speed/Alfvén-speed = 0.2-1.5, J ~ 50-150 mA/cm2, pitch-angle ~53°) was injected into the plasma. The interaction of the beam with the plasma was diagnosed using a retarding-field energy analyzer, three-axis magnetic-loop, and Langmuir probes. The resonance conditions for the growth of shear Alfvén waves were examined by varying the parameters of the ion-beam and ambient plasma. The experimental results demonstrate that the DICR process is particularly effective in exciting left-handed polarized shear Alfvén waves that propagate in the direction opposite to the ion beam. The high-harmonic beam modes were detected in the vicinity of the spiraling ion beam and contained more than 80 harmonics of Doppler-shifted gyro-frequency of the beam. Work jointly supported by US DOE and NSF and performed at the Basic Plasma Science Facility, UCLA.

  11. Isoscalar giant monopole resonance in Sn isotopes by Coulomb excitations using a quantum molecular dynamics model

    CERN Document Server

    Tao, C; Zhang, G Q; Cao, X G; Fang, D Q; Wang, H W; Xu, J

    2013-01-01

    The isoscalar giant monopole resonance (ISGMR) in Sn isotopes and other nuclei has been investigated by Coulomb excitations in the framework of the isospin-dependent quantum molecular dynamics (IQMD) model. The spectrum of GMR has been calculated by taking the root-mean-square (RMS) radius of a nucleus as its monopole moment. The peak energy, the full width at half maximum (FWHM), and the strength of GMR extracted by a Gaussian fit to the spectrum have been studied. The GMR peak energies for Sn isotopes from the calculations using a mass-number dependent Gaussian wave-packet width $\\sigma_r$ for nucleons are found to be overestimated and show a weak dependence on the mass number compared with the experimental data. However, it has been found that experimental data of the GMR peak energies for $^{40}$Ca, $^{56}$Ni, $^{90}$Zr and $^{208}$Pb as well as Sn isotopes can be nicely reproduced after taking into account the isospin dependence in isotope chains in addition to the mass number dependence of $\\sigma_r$ fo...

  12. Analysis of probabilities for nuclear excitation by near-resonant electronic transitions

    CERN Document Server

    Harston, M R

    2001-01-01

    Theoretical results are presented for nuclear excitation of low-lying isometric states of sup 1 sup 9 sup 7 Au, sup 1 sup 8 sup 9 Os and sup 2 sup 3 sup 7 Np by a near-resonant electronic deexcitation process known as NEET. A detailed comparison is made between current and previous theoretical results in order to clarify a number of anomalies. For sup 1 sup 9 sup 7 Au, the only case in which the current experimental precision appears to be sufficient to provide a stringent test of theory, the theoretical result for the NEET probability is P sub N sub E sub E sub T =3.6x10 sup - sup 8. This is a factor of three lower than previous theoretical results and reduces the difference between theory and the recent experimental result, P sub N sub E sub E sub T =(5.0+-0.6)x10 sup - sup 8 , to a level of approximately 2 sigma.

  13. Measurement of resonance parameters of orbitally excited narrow B0 mesons.

    Science.gov (United States)

    Aaltonen, T; Adelman, J; Akimoto, T; Albrow, M G; González, B Alvarez; Amerio, S; Amidei, D; Anastassov, A; Annovi, A; Antos, J; Apollinari, G; Apresyan, A; Arisawa, T; Artikov, A; Ashmanskas, W; Attal, A; Aurisano, A; Azfar, F; Azzurri, P; Badgett, W; Barbaro-Galtieri, A; Barnes, V E; Barnett, B A; Bartsch, V; Bauer, G; Beauchemin, P-H; Bedeschi, F; Beecher, D; Behari, S; Bellettini, G; Bellinger, J; Benjamin, D; Beretvas, A; Beringer, J; Bhatti, A; Binkley, M; Bisello, D; Bizjak, I; Blair, R E; Blocker, C; Blumenfeld, B; Bocci, A; Bodek, A; Boisvert, V; Bolla, G; Bortoletto, D; Boudreau, J; Boveia, A; Brau, B; Bridgeman, A; Brigliadori, L; Bromberg, C; Brubaker, E; Budagov, J; Budd, H S; Budd, S; Burke, S; Burkett, K; Busetto, G; Bussey, P; Buzatu, A; Byrum, K L; Cabrera, S; Calancha, C; Campanelli, M; Campbell, M; Canelli, F; Canepa, A; Carls, B; Carlsmith, D; Carosi, R; Carrillo, S; Carron, S; Casal, B; Casarsa, M; Castro, A; Catastini, P; Cauz, D; Cavaliere, V; Cavalli-Sforza, M; Cerri, A; Cerrito, L; Chang, S H; Chen, Y C; Chertok, M; Chiarelli, G; Chlachidze, G; Chlebana, F; Cho, K; Chokheli, D; Chou, J P; Choudalakis, G; Chuang, S H; Chung, K; Chung, W H; Chung, Y S; Chwalek, T; Ciobanu, C I; Ciocci, M A; Clark, A; Clark, D; Compostella, G; Convery, M E; Conway, J; Cordelli, M; Cortiana, G; Cox, C A; Cox, D J; Crescioli, F; Almenar, C Cuenca; Cuevas, J; Culbertson, R; Cully, J C; Dagenhart, D; Datta, M; Davies, T; de Barbaro, P; De Cecco, S; Deisher, A; De Lorenzo, G; Dell'orso, M; Deluca, C; Demortier, L; Deng, J; Deninno, M; Derwent, P F; di Giovanni, G P; Dionisi, C; Di Ruzza, B; Dittmann, J R; D'Onofrio, M; Donati, S; Dong, P; Donini, J; Dorigo, T; Dube, S; Efron, J; Elagin, A; Erbacher, R; Errede, D; Errede, S; Eusebi, R; Fang, H C; Farrington, S; Fedorko, W T; Feild, R G; Feindt, M; Fernandez, J P; Ferrazza, C; Field, R; Flanagan, G; Forrest, R; Frank, M J; Franklin, M; Freeman, J C; Furic, I; Gallinaro, M; Galyardt, J; Garberson, F; Garcia, J E; Garfinkel, A F; Genser, K; Gerberich, H; Gerdes, D; Gessler, A; Giagu, S; Giakoumopoulou, V; Giannetti, P; Gibson, K; Gimmell, J L; Ginsburg, C M; Giokaris, N; Giordani, M; Giromini, P; Giunta, M; Giurgiu, G; Glagolev, V; Glenzinski, D; Gold, M; Goldschmidt, N; Golossanov, A; Gomez, G; Gomez-Ceballos, G; Goncharov, M; González, O; Gorelov, I; Goshaw, A T; Goulianos, K; Gresele, A; Grinstein, S; Grosso-Pilcher, C; Grundler, U; da Costa, J Guimaraes; Gunay-Unalan, Z; Haber, C; Hahn, K; Hahn, S R; Halkiadakis, E; Han, B-Y; Han, J Y; Happacher, F; Hara, K; Hare, D; Hare, M; Harper, S; Harr, R F; Harris, R M; Hartz, M; Hatakeyama, K; Hays, C; Heck, M; Heijboer, A; Heinrich, J; Henderson, C; Herndon, M; Heuser, J; Hewamanage, S; Hidas, D; Hill, C S; Hirschbuehl, D; Hocker, A; Hou, S; Houlden, M; Hsu, S-C; Huffman, B T; Hughes, R E; Husemann, U; Huston, J; Incandela, J; Introzzi, G; Iori, M; Ivanov, A; James, E; Jayatilaka, B; Jeon, E J; Jha, M K; Jindariani, S; Johnson, W; Jones, M; Joo, K K; Jun, S Y; Jung, J E; Junk, T R; Kamon, T; Kar, D; Karchin, P E; Kato, Y; Kephart, R; Keung, J; Khotilovich, V; Kilminster, B; Kim, D H; Kim, H S; Kim, H W; Kim, J E; Kim, M J; Kim, S B; Kim, S H; Kim, Y K; Kimura, N; Kirsch, L; Klimenko, S; Knuteson, B; Ko, B R; Kondo, K; Kong, D J; Konigsberg, J; Korytov, A; Kotwal, A V; Kreps, M; Kroll, J; Krop, D; Krumnack, N; Kruse, M; Krutelyov, V; Kubo, T; Kuhr, T; Kulkarni, N P; Kurata, M; Kusakabe, Y; Kwang, S; Laasanen, A T; Lami, S; Lammel, S; Lancaster, M; Lander, R L; Lannon, K; Lath, A; Latino, G; Lazzizzera, I; Lecompte, T; Lee, E; Lee, H S; Lee, S W; Leone, S; Lewis, J D; Lin, C-S; Linacre, J; Lindgren, M; Lipeles, E; Lister, A; Litvintsev, D O; Liu, C; Liu, T; Lockyer, N S; Loginov, A; Loreti, M; Lovas, L; Lucchesi, D; Luci, C; Lueck, J; Lujan, P; Lukens, P; Lungu, G; Lyons, L; Lys, J; Lysak, R; Macqueen, D; Madrak, R; Maeshima, K; Makhoul, K; Maki, T; Maksimovic, P; Malde, S; Malik, S; Manca, G; Manousakis-Katsikakis, A; Margaroli, F; Marino, C; Marino, C P; Martin, A; Martin, V; Martínez, M; Martínez-Ballarín, R; Maruyama, T; Mastrandrea, P; Masubuchi, T; Mathis, M; Mattson, M E; Mazzanti, P; McFarland, K S; McIntyre, P; McNulty, R; Mehta, A; Mehtala, P; Menzione, A; Merkel, P; Mesropian, C; Miao, T; Miladinovic, N; Miller, R; Mills, C; Milnik, M; Mitra, A; Mitselmakher, G; Miyake, H; Moggi, N; Moon, C S; Moore, R; Morello, M J; Morlok, J; Fernandez, P Movilla; Mülmenstädt, J; Mukherjee, A; Muller, Th; Mumford, R; Murat, P; Mussini, M; Nachtman, J; Nagai, Y; Nagano, A; Naganoma, J; Nakamura, K; Nakano, I; Napier, A; Necula, V; Nett, J; Neu, C; Neubauer, M S; Neubauer, S; Nielsen, J; Nodulman, L; Norman, M; Norniella, O; Nurse, E; Oakes, L; Oh, S H; Oh, Y D; Oksuzian, I; Okusawa, T; Orava, R; Griso, S Pagan; Palencia, E; Papadimitriou, V; Papaikonomou, A; Paramonov, A A; Parks, B; Pashapour, S; Patrick, J; Pauletta, G; Paulini, M; Paus, C; Peiffer, T; Pellett, D E; Penzo, A; Phillips, T J; Piacentino, G; Pianori, E; Pinera, L; Pitts, K; Plager, C; Pondrom, L; Poukhov, O; Pounder, N; Prakoshyn, F; Pronko, A; Proudfoot, J; Ptohos, F; Pueschel, E; Punzi, G; Pursley, J; Rademacker, J; Rahaman, A; Ramakrishnan, V; Ranjan, N; Redondo, I; Rekovic, V; Renton, P; Renz, M; Rescigno, M; Richter, S; Rimondi, F; Ristori, L; Robson, A; Rodrigo, T; Rodriguez, T; Rogers, E; Rolli, S; Roser, R; Rossi, M; Rossin, R; Roy, P; Ruiz, A; Russ, J; Rusu, V; Safonov, A; Sakumoto, W K; Saltó, O; Santi, L; Sarkar, S; Sartori, L; Sato, K; Savoy-Navarro, A; Schlabach, P; Schmidt, A; Schmidt, E E; Schmidt, M A; Schmidt, M P; Schmitt, M; Schwarz, T; Scodellaro, L; Scribano, A; Scuri, F; Sedov, A; Seidel, S; Seiya, Y; Semenov, A; Sexton-Kennedy, L; Sforza, F; Sfyrla, A; Shalhout, S Z; Shears, T; Shepard, P F; Shimojima, M; Shiraishi, S; Shochet, M; Shon, Y; Shreyber, I; Sidoti, A; Sinervo, P; Sisakyan, A; Slaughter, A J; Slaunwhite, J; Sliwa, K; Smith, J R; Snider, F D; Snihur, R; Soha, A; Somalwar, S; Sorin, V; Spalding, J; Spreitzer, T; Squillacioti, P; Stanitzki, M; St Denis, R; Stelzer, B; Stelzer-Chilton, O; Stentz, D; Strologas, J; Strycker, G L; Stuart, D; Suh, J S; Sukhanov, A; Suslov, I; Suzuki, T; Taffard, A; Takashima, R; Takeuchi, Y; Tanaka, R; Tecchio, M; Teng, P K; Terashi, K; Thom, J; Thompson, A S; Thompson, G A; Thomson, E; Tipton, P; Ttito-Guzmán, P; Tkaczyk, S; Toback, D; Tokar, S; Tollefson, K; Tomura, T; Tonelli, D; Torre, S; Torretta, D; Totaro, P; Tourneur, S; Trovato, M; Tsai, S-Y; Tu, Y; Turini, N; Ukegawa, F; Vallecorsa, S; van Remortel, N; Varganov, A; Vataga, E; Vázquez, F; Velev, G; Vellidis, C; Veszpremi, V; Vidal, M; Vidal, R; Vila, I; Vilar, R; Vine, T; Vogel, M; Volobouev, I; Volpi, G; Wagner, P; Wagner, R G; Wagner, R L; Wagner, W; Wagner-Kuhr, J; Wakisaka, T; Wallny, R; Wang, S M; Warburton, A; Waters, D; Weinberger, M; Weinelt, J; Wester, W C; Whitehouse, B; Whiteson, D; Wicklund, A B; Wicklund, E; Wilbur, S; Williams, G; Williams, H H; Wilson, P; Winer, B L; Wittich, P; Wolbers, S; Wolfe, C; Wright, T; Wu, X; Würthwein, F; Wynne, S M; Xie, S; Yagil, A; Yamamoto, K; Yamaoka, J; Yang, U K; Yang, Y C; Yao, W M; Yeh, G P; Yoh, J; Yorita, K; Yoshida, T; Yu, G B; Yu, I; Yu, S S; Yun, J C; Zanello, L; Zanetti, A; Zhang, X; Zheng, Y; Zucchelli, S

    2009-03-13

    We report a measurement of resonance parameters of the orbitally excited (L=1) narrow B0 mesons in decays to B;{(*)+}pi;{-} using 1.7 fb;{-1} of data collected by the CDF II detector at the Fermilab Tevatron. The mass and width of the B_{2};{*0} state are measured to be m(B_{2};{*0})=5740.2_{-1.8};{+1.7}(stat)-0.8+0.9(syst) MeV/c;{2} and Gamma(B_{2};{*0})=22.7_{-3.2};{+3.8}(stat)-10.2+3.2(syst) MeV/c;{2}. The mass difference between the B_{2};{*0} and B10 states is measured to be 14.9_{-2.5};{+2.2}(stat)-1.4+1.2(syst) MeV/c;{2}, resulting in a B10 mass of 5725.3_{-2.2};{+1.6}(stat)-1.5+1.4(syst) MeV/c;{2}. This is currently the most precise measurement of the masses of these states and the first measurement of the B_{2};{*0} width.

  14. First Measurement of the Neutral Current Excitation of the Delta Resonance on a Proton Target

    CERN Document Server

    Androic, D; Arvieux, J; Bailey, S L; Beck, D H; Beise, E J; Benesch, J; Benmokhtar, F; Bimbot, L; Birchall, J; Bosted, P; Breuer, H; Capuano, C L; Chao, Y -C; Coppens, A; Davis, C A; Ellis, C; Flores, G; Franklin, G; Furget, C; Gaskell, D; Grames, J; Gericke, M T W; Guillard, G; Hansknecht, J; Horn, T; Jones, M K; King, P M; Korsch, W; Kox, S; Lee, L; Liu, J; Lung, A; Mammei, J; Martin, J W; McKeown, R D; Micherdzinska, A; Mihovilovic, M; Mkrtchyan, H; Muether, M; Page, S A; Papavassiliou, V; Pate, S F; Phillips, S K; Pillot, P; Pitt, M L; Poelker, M; Quinn, B; Ramsay, W D; Real, J -S; Roche, J; Roos, P; Schaub, J; Seva, T; Simicevic, N; Smith, G R; Spayde, D T; Stutzman, M; Suleiman, R; Tadevosyan, V; van Oers, W T H; Versteegen, M; Voutier, E; Vulcan, W; Wells, S P; Williamson, S E; Wood, S A

    2012-01-01

    The parity-violating asymmetry arising from inelastic electron-nucleon scattering at backward angle (~95 degrees) near the Delta(1232) resonance has been measured using a hydrogen target. From this asymmetry, we extracted the axial transition form factor G^A_{N\\Delta}, a function of the axial Adler form factors C^A_i. Though G^A_{N\\Delta} has been previously studied using charged current reactions, this is the first measurement of the weak neutral current excitation of the Delta using a proton target. For Q^2 = 0.34 (GeV/c)^2 and W = 1.18 GeV, the asymmetry was measured to be -33.4 \\pm (5.3)_{stat} \\pm (5.1)_{sys} ppm. The value of G^A_{N\\Delta} determined from the hydrogen asymmetry was -0.05 \\pm (0.35)_{stat} \\pm (0.34)_{sys} \\pm (0.06)_{theory}. These findings agree within errors with theoretical predictions for both the total asymmetry and the form factor. In addition to the hydrogen measurement, the asymmetry was measured at the same kinematics using a deuterium target. The asymmetry for deuterium was de...

  15. Excitation and tuning of Fano-like cavity plasmon resonances in dielectric-metal core-shell resonators

    Science.gov (United States)

    Gu, Ping; Wan, Mingjie; Wu, Wenyang; Chen, Zhuo; Wang, Zhenlin

    2016-05-01

    Fano resonances have been realized in plasmonic systems and have found intriguing applications, in which, however, precisely controlled symmetry breaking or particular arrangement of multiple constituents is usually involved. Although simple core-shell type architectures composed of a spherical dielectric core and a concentric metallic shell layer have been proposed as good candidates that support inherent Fano resonances, these theoretical predictions have rarely seen any detailed experimental investigation. Here, we report on the experimental investigation of the magnetic and electric-based multipolar plasmonic Fano resonances in the dielectric-metal core-shell resonators that are formed by wrapping a nearly perfect metal shell layer around a dielectric sphere. We demonstrate that these Fano resonances originate from the interference between the Mie cavity and sphere plasmon resonances. Moreover, we present that the variation on either the dielectric core size or core refractive index allows for easily tuning the observed Fano resonances over a wide spectral range. Our findings are supported by excellent agreement with analytical calculations, and offer unprecedented opportunities for realizing ultrasensitive bio-sensors, lasing and nonlinear optical devices.Fano resonances have been realized in plasmonic systems and have found intriguing applications, in which, however, precisely controlled symmetry breaking or particular arrangement of multiple constituents is usually involved. Although simple core-shell type architectures composed of a spherical dielectric core and a concentric metallic shell layer have been proposed as good candidates that support inherent Fano resonances, these theoretical predictions have rarely seen any detailed experimental investigation. Here, we report on the experimental investigation of the magnetic and electric-based multipolar plasmonic Fano resonances in the dielectric-metal core-shell resonators that are formed by wrapping a

  16. Resonant excitation of ethylene molecules in the combustion flame CVD of diamond using a wavelength tunable CO2 laser

    Science.gov (United States)

    Xie, Z. Q.; Park, J. B.; He, X. N.; Gao, Y.; Zhou, Y. S.; Lu, Y. F.

    2010-02-01

    CO2 laser resonant excitations of precursor molecules were applied in combustion flame synthesis of diamond films. The combustion flame was produced from a mixture of ethylene (C2H4), acetylene (C2H2) and oxygen (O2). A wavelength-tunable CO2 laser with wavelength range from 9.2 to 10.9 μm was used for wavelength-matched excitation of the ethylene molecules. By irradiating the flame using CO2 laser at 10.532 μm, the ethylene molecules were resonantly excited through the CH2 wagging vibrational mode (ν7, 949.3 cm-1). Irradiation of the flame using the common CO2 laser wavelength at 10.591 μm was also carried out for comparison. It was found that diamond synthesis was more obviously enhanced by the CO2 laser resonant excitation at 10.532 μm as compared to that at 10.591 μm. Firstly, the flame was shortened by 50%, indicating a promoted reaction in the process. Secondly, the diamond grain sizes as well as the diamond film thicknesses were increased by 200~300% and 160% respectively, indicating a higher growth rate of diamond films. Finally, Raman spectra of the diamond sample showed a sharp diamond peak at 1334 cm-1 and a suppressed G-band, indicating higher diamond quality.

  17. A unified view of coherent and incoherent dihydrogen exchange in transition metal hydrides by nuclear resonance and inelastic neutron scattering

    Energy Technology Data Exchange (ETDEWEB)

    Limbach, H.H.; Ulrich, S.; Buntkowsky, G. [Freie Univ. Berlin (Germany). Inst. fuer Organische Chemie; Sabo-Etienne, S.; Chaudret, B. [Toulouse-3 Univ., 31 (France). Lab. de Chimie de Coordination du C.N.R.S.; Kubas, G.J.; Eckert, J. [Los Alamos National Lab., NM (United States)

    1995-08-12

    In this paper a unified view of coherent and incoherent dihydrogen exchange in transition metal hydrides by nuclear magnetic resonance (NMR) and inelastic neutron scattering (INS) is presented. It is shown that both exchange processes coexist i.e. do not transform into each other although they may dominate the spectra in different temperature ranges. This superposition is the consequence of the incorporation of the tunnel frequency J of the coherent process into the nuclear two-spin hamiltonian of hydrogen pairs which allows to treat the problem using the well known density matrix theory of NMR line-shapes developed by Alexander and Binsch. It is shown that this theory can also be used to predict the line-shapes of the rotational tunneling transitions observed in the INS spectra of transition metal dihydrogen complexes and that both NMR and INS spectra depend on similar parameters.

  18. Coherent exciton dynamics in a dissipative environment maintained by an off-resonant vibrational mode

    Science.gov (United States)

    Levi, E. K.; Irish, E. K.; Lovett, B. W.

    2016-04-01

    The interplay between an open quantum system and its environment can lead to both coherent and incoherent behavior. We explore the extent to which strong coupling to a single bosonic mode can alter the coherence properties of a two-level system in a structured environment. This mode is treated exactly, with the rest of the environment comprising a Markovian bath of bosonic modes. The strength of the coupling between the two-level system and the single mode is varied for a variety of forms for the bath spectral density in order to assess whether the coherent dynamics of the two-level system are modified. We find a clear renormalization of the site population oscillation frequency that causes an altered interaction with the bath. This leads to enhanced or reduced coherent behavior of the two-level system, depending on the form of the spectral density function. We present an intuitive interpretation, based on an analytical model, to explain the behavior.

  19. Cooling a mechanical resonator with nitrogen-vacancy centres using a room temperature excited state spin-strain interaction

    Science.gov (United States)

    Macquarrie, E. R.; Otten, M.; Gray, S. K.; Fuchs, G. D.

    2017-02-01

    Cooling a mechanical resonator mode to a sub-thermal state has been a long-standing challenge in physics. This pursuit has recently found traction in the field of optomechanics in which a mechanical mode is coupled to an optical cavity. An alternate method is to couple the resonator to a well-controlled two-level system. Here we propose a protocol to dissipatively cool a room temperature mechanical resonator using a nitrogen-vacancy centre ensemble. The spin ensemble is coupled to the resonator through its orbitally-averaged excited state, which has a spin-strain interaction that has not been previously studied. We experimentally demonstrate that the spin-strain coupling in the excited state is 13.5+/-0.5 times stronger than the ground state spin-strain coupling. We then theoretically show that this interaction, combined with a high-density spin ensemble, enables the cooling of a mechanical resonator from room temperature to a fraction of its thermal phonon occupancy.

  20. Coherent coupling of molecular resonators with a micro-cavity mode

    CERN Document Server

    Shalabney, Atef; Hutchison, James A; Pupillo, Guido; Genet, Cyriaque; Ebbesen, Thomas W

    2014-01-01

    Strong coupling is at the heart of optomechanics where it enables coherent quantum state transfer between light and micromechanical oscillators. Strongly coupled molecule-cavity systems have also revealed unique properties enabling even the control of chemical rates through the optical hybridization of the electronic states. Here we combine these notions to show that molecular vibrational modes of the electronic ground state can be coherently coupled with a micro-cavity mode at room temperature, given the low vibrational thermal occupation factors n_{\

  1. Excitation of giant monopole resonance in {sup 208}Pb and {sup 116}Sn using inelastic deuteron scattering

    Energy Technology Data Exchange (ETDEWEB)

    Patel, D.; Garg, U. [Department of Physics, University of Notre Dame, Notre Dame, IN 46556 (United States); Joint Institute for Nuclear Astrophysics, University of Notre Dame, Notre Dame, IN 46556 (United States); Itoh, M. [Cyclotron and Radioisotope Center, Tohoku University, Sendai 980-8578 (Japan); Akimune, H. [Department of Physics, Konan University, Kobe 568-8501 (Japan); Berg, G.P.A. [Department of Physics, University of Notre Dame, Notre Dame, IN 46556 (United States); Joint Institute for Nuclear Astrophysics, University of Notre Dame, Notre Dame, IN 46556 (United States); Fujiwara, M. [Research Center for Nuclear Physics, Osaka University, Osaka 567-0047 (Japan); Harakeh, M.N. [Kernfysisch Versneller Instituut, University of Groningen, 9747 AA Groningen (Netherlands); GANIL, CEA/DSM-CNRS/IN2P3, 14076 Caen (France); Iwamoto, C. [Department of Physics, Konan University, Kobe 568-8501 (Japan); Kawabata, T. [Division of Physics and Astronomy, Kyoto University, Kyoto 606-8502 (Japan); Kawase, K. [Japan Atomic Energy Agency, Kyoto 619-0215 (Japan); Matta, J.T. [Department of Physics, University of Notre Dame, Notre Dame, IN 46556 (United States); Joint Institute for Nuclear Astrophysics, University of Notre Dame, Notre Dame, IN 46556 (United States); Murakami, T. [Division of Physics and Astronomy, Kyoto University, Kyoto 606-8502 (Japan); Okamoto, A. [Department of Physics, Konan University, Kobe 568-8501 (Japan); Sako, T. [Japan Atomic Energy Agency, Kyoto 619-0215 (Japan); Schlax, K.W. [Department of Physics, University of Notre Dame, Notre Dame, IN 46556 (United States); Takahashi, F. [Research Center for Nuclear Physics, Osaka University, Osaka 567-0047 (Japan); White, M. [Department of Physics, University of Notre Dame, Notre Dame, IN 46556 (United States); Yosoi, M. [Research Center for Nuclear Physics, Osaka University, Osaka 567-0047 (Japan)

    2014-07-30

    The excitation of the isoscalar giant monopole resonance (ISGMR) in {sup 208}Pb and {sup 116}Sn has been investigated using small-angle (including 0°) inelastic scattering of 100 MeV/u deuteron and multipole-decomposition analysis (MDA). The extracted strength distributions agree well with those from inelastic scattering of 100 MeV/u α particles. These measurements establish deuteron inelastic scattering at E{sub d}∼100 MeV/u as a suitable probe for extraction of the ISGMR strength with MDA, making feasible the investigation of this resonance in radioactive isotopes in inverse kinematics.

  2. Formation and erasure of population difference gratings in the coherent interaction of a resonant medium with extremely short optical pulses

    Science.gov (United States)

    Arkhipov, R. M.; Arkhipov, M. V.; Babushkin, I.; Rosanov, N. N.

    2016-11-01

    In the regime of coherent interaction of short optical pulses with a resonant medium, which is implemented with a pulse duration shorter than the relaxation times in the medium, the formation of population gratings can occur without overlapping the pulses therein. In this case, there are new possibilities for controlling optical pulses, which are especially pronounced for extremely short pulses. It is shown that, with the proper choice of the parameters of a sequence of extremely short optical pulses, not only the formation of population gratings, but also their erasure are possible. It is demonstrated that this effect can be used for the creation of an ultrahigh-speed optical deflector.

  3. Coherent dynamics of exciton and biexciton resonances in InGaAs/GaAs single quantum wells

    DEFF Research Database (Denmark)

    Borri, Paola; Langbein, Wolfgang; Hvam, Jørn Märcher

    1999-01-01

    The coherent dynamics of both exciton and biexciton resonances have been investigated in In0.18Ga0.82As/GaAs single quantum wells with thicknesses ranging from 1 to 4 nm, using time-integrated and spectrally-resolved transient four-wave mixing. From the temperature dependence of the exciton...... dephasing time we obtain linewidth broadening coefficients for acoustic and optical phonons. Biexciton binding energies are extracted from the four-wave mixing response in the spectral domain, and are found to be between 1.5 and 2.6 meV. The temperature dempendence of the dephasing of the exciton...

  4. Resonant excitation of coupled Rayleigh waves in a short and narrow fluid channel clad between two identical metal plates

    Directory of Open Access Journals (Sweden)

    Victor M. García-Chocano

    2011-12-01

    Full Text Available Transmission of ultrasonic waves through a slit between two water immersed brass plates is studied for sub-wavelength plate thicknesses and slit apertures. Extraordinary high absorption is observed at discrete frequencies corresponding to resonant excitation of Rayleigh waves on the both sides of the channel. The coupling of the Rayleigh waves occurs through the fluid and the corresponding contribution to the dispersion has been theoretically derived and also experimentally confirmed. Symmetric and anti-symmetric modes are predicted but only the symmetric mode resonances have been observed. It follows from the dispersion equation that the coupled Rayleigh waves cannot be excited in a channel with apertures less than the critical one. The calculated critical aperture is in a good agreement with the measured acoustic spectra. These findings could be applied to design a broadband absorptive metamaterial.

  5. Pulsed microwave-driven argon plasma jet with distinctive plume patterns resonantly excited by surface plasmon polaritons

    Institute of Scientific and Technical Information of China (English)

    陈兆权; 殷志祥; 夏广庆; 洪伶俐; 胡业林; 刘明海; 胡希伟

    2015-01-01

    Atmospheric lower-power pulsed microwave argon cold plasma jets are obtained by using coaxial transmission line resonators in ambient air. The plasma jet plumes are generated at the end of a metal wire placed in the middle of the dielec-tric tubes. The electromagnetic model analyses and simulation results suggest that the discharges are excited resonantly by the enhanced electric field of surface plasmon polaritons. Moreover, for conquering the defect of atmospheric argon filamentation discharges excited by 2.45-GHz continued microwave, the distinctive patterns of the plasma jet plumes can be maintained by applying different gas flow rates of argon gas, frequencies of pulsed modulator, duty cycles of pulsed microwave, peak values of input microwave power, and even by using different materials of dielectric tubes. In addition, the emission spectrum, the plume temperature, and other plasma parameters are measured, which shows that the proposed pulsed microwave plasma jets can be adjusted for plasma biomedical applications.

  6. Nature of low-lying electric dipole resonance excitations in 74Ge

    CERN Document Server

    Negi, D; Lanza, E G; Litvinova, E; Vitturi, A; Bark, R A; Bernstein, L A; Bleuel, D L; Bvumbi, S; Bucher, T D; Daub, B H; Dinoko, T S; Easton, J L; Gorgen, A; Guttormsen, M; Jones, P; Kheswa, B V; Khumalo, N A; Larsen, A C; Lawrie, E A; Lawrie, J J; Majola, S N T; Masiteng, L P; Nchodu, M R; Ndayishimye, J; Newman, R T; Noncolela, S P; Orce, J N; Papka, P; Pellegri, L; Renstrøm, T; Roux, D G; Schwengner, R; Shirinda, O; Siem, S

    2016-01-01

    Isospin properties of dipole excitations in 74 Ge are investigated using the ({\\alpha},{\\alpha}'{\\gamma}) reaction and compared to ({\\gamma},{\\gamma}) data. The results indicate that the dipole excitations in the energy region of 6 to 9 MeV adhere to the scenario of the recently found splitting of the region of dipole excitations into two separated parts: one at low energy, being populated by both isoscalar and isovector probes, and the other at high energy, excited only by the electromagnetic probe. Relativistic quasiparticle time blocking approximation (RQTBA) calculations show a reduction in the isoscalar E1 strength with an increase in excitation energy, which is consistent with the measurement.

  7. Developing a hybrid wind instrument: using a loudspeaker to couple a theoretical exciter to a real resonator

    OpenAIRE

    Buys, K.; D. Sharp; Laney, R.

    2014-01-01

    A hybrid wind instrument generates self-sustained sounds via a real-time interaction between a computed physical model of an exciter (such as human lips interacting with a mouthpiece) and a real acoustic resonator. Successful implementation of a hybrid wind instrument will not only open up new musical possibilities but will also provide a valuable research tool. However, attempts to produce a hybrid instrument have so far fallen short, in terms of both the accuracy and the variation in the so...

  8. Isoscalar Giant Resonance Strengths in $^{32}$S and possible excitations of superdeformed and $^{28}$Si + $\\alpha$ cluster bandheads

    CERN Document Server

    Itoh, M; Sakaguchi, H; Akimune, H; Fujiwara, M; Garg, U; Hara, K; Hashimoto, H; Hoffman, J; Kawabata, T; Kawase, K; Murakami, T; Nakanishi, K; Nayak, B K; Terashima, S; Uchida, M; Yasuda, Y; Yosoi, M

    2013-01-01

    Isoscalar giant resonances and low spin states in $^{32}$S have been measured with inelastic $\\alpha$ scattering at extremely forward angles including zero degrees at E$_{\\alpha}$ = 386 MeV. By applying the multipole decomposition analysis, various excited states are classified according to their spin and parities (J$^{\\pi}$), and are discussed in relation to the super deformed and $^{28}$Si + $\\alpha$ cluster bands.

  9. The Influence of Thermal Conditions on the Thermomechanics of Particulate-Composite, Mock Explosive Samples under Near-Resonant Excitation

    OpenAIRE

    2016-01-01

    Vapor detection is one of the most effective ways to find hidden plastic-bonded explosives in the field today. In recent years, it has been demonstrated that providing near-resonant vibratory excitation to explosives dramatically increases their vapor pressure, allowing for easier detection. Unfortunately, there currently exists a limited understanding of the thermomechanics of energetic material. This study seeks to help fill this technical void by exploring the thermomechanics of mock plast...

  10. Experimental Verification of Isotropic Radiation from a Coherent Dipole Source via Electric-Field-Driven LC Resonator Metamaterials

    Science.gov (United States)

    Tichit, Paul-Henri; Burokur, Shah Nawaz; Qiu, Cheng-Wei; de Lustrac, André

    2013-09-01

    It has long been conjectured that isotropic radiation by a simple coherent source is impossible due to changes in polarization. Though hypothetical, the isotropic source is usually taken as the reference for determining a radiator’s gain and directivity. Here, we demonstrate both theoretically and experimentally that an isotropic radiator can be made of a simple and finite source surrounded by electric-field-driven LC resonator metamaterials designed by space manipulation. As a proof-of-concept demonstration, we show the first isotropic source with omnidirectional radiation from a dipole source (applicable to all distributed sources), which can open up several possibilities in axion electrodynamics, optical illusion, novel transformation-optic devices, wireless communication, and antenna engineering. Owing to the electric- field-driven LC resonator realization scheme, this principle can be readily applied to higher frequency regimes where magnetism is usually not present.

  11. Fast high-resolution nuclear magnetic resonance spectroscopy through indirect zero-quantum coherence detection in inhomogeneous fields

    Science.gov (United States)

    Ke, Han-Ping; Chen, Hao; Lin, Yan-Qin; Wei, Zhi-Liang; Cai, Shu-Hui; Zhang, Zhi-Yong; Chen, Zhong

    2014-06-01

    In many cases, high-resolution nuclear magnetic resonance (NMR) spectra are virtually impossible to obtain by conventional nuclear magnetic resonance methods because of inhomogeneity of magnetic field and inherent heterogeneity of sample. Although conventional intramolecular zero-quantum coherence (ZQC) can be used to obtain high-resolution spectrum in inhomogeneous field, the acquisition takes rather long time. In this paper, a spatially encoded intramolecular ZQC technique is proposed to fast acquire high-resolution NMR spectrum in inhomogeneous field. For the first time, the gradient-driven decoding technique is employed to selectively acquire intramolecular ZQC signals. Theoretical analyses and experimental observations demonstrate that high-resolution NMR spectral information can be retrieved within several scans even when the field inhomogeneity is severe enough to erase most spectral information. This work provides a new way to enhance the acquisition efficiency of high-resolution intramolecular ZQC spectroscopy in inhomogeneous fields.

  12. How a single stretched polymer responds coherently to a minute oscillation in fluctuating environments: An entropic stochastic resonance

    CERN Document Server

    Kim, Won Kyu; 10.1063/1.4746118

    2012-01-01

    Within the cell, biopolymers are often situated in constrained, fluid environments, e.g., cytoskeletal networks, stretched DNAs in chromatin. It is of paramount importance to understand quantitatively how they, utilizing their flexibility, optimally respond to a minute signal, which is, in general, temporally fluctuating far away from equilibrium. To this end, we analytically study viscoelastic response and associated stochastic resonance in a stretched single semi-flexible chain to an oscillatory force or electric field. Including hydrodynamic interactions between chain segments, we evaluate dynamics of the polymer extension in coherent response to the force or field. We find power amplification factor of the response at a noise-strength (temperature) can attain the maximum that grows as the chain length increases, indicative of an entropic stochastic resonance (ESR). In particular for a charged chain under an electric field, we find that the maximum also occurs at an optimal chain length, a new feature of E...

  13. A study on the complexity of a business cycle model with great excitements in non-resonant condition

    Energy Technology Data Exchange (ETDEWEB)

    Ma Junhai [School of Management, Tianjin University, Tianjin 300072 (China); Tianjin University of Finance and Economics, Tianjin 300222 (China)], E-mail: mjhtju@yahoo.com.cn; Cui Yaqiang; Liulixia [School of Management, Tianjin University, Tianjin 300072 (China)

    2009-03-15

    Based on the researches of Szydlowski and Krawiec, we studied the inherent complexity of a chaotic business cycle with great excitements in non-resonant condition. First, we got the first-order and second-order approximate solutions of the system by using multiple scale method. Then deduced the formulation reflecting the complex relations between vibration, phase, bifurcation parameter {mu} and excite frequency {omega} of first-order solution. As the great excitement F varied, the global changes of the system solutions were analyzed. We also explored the different paths leading the systems with different parameter combinations into catastrophe region, fuzzy region or chaos region. Finally, we discussed the evolution trends of business cycle models under the above-mentioned conditions. Hence, this paper has some theoretical and practical significance.

  14. Analysis of asymmetric resonance response of thermally excited silicon micro-cantilevers for mass-sensitive nanoparticle detection

    Science.gov (United States)

    Bertke, Maik; Hamdana, Gerry; Wu, Wenze; Suryo Wasisto, Hutomo; Uhde, Erik; Peiner, Erwin

    2017-06-01

    In this paper, the asymmetric resonance frequency (f 0) responses of thermally in-plane excited silicon cantilevers for a pocket-sized, cantilever-based airborne nanoparticle detector (Cantor) are analysed. By measuring the shift of f 0 caused by the deposition of nanoparticles (NPs), the cantilevers are used as a microbalance. The cantilever sensors are low cost manufactured from silicon by bulk-micromachining techniques and contain an integrated p-type heating actuator and a sensing piezoresistive Wheatstone bridge. f 0 is tracked by a homemade phase-locked loop (PPL) for real-time measurements. To optimize the sensor performance, a new cantilever geometry was designed, fabricated and characterized by its frequency responses. The most significant characterisation parameters of our application are f 0 and the quality factor (Q), which have high influences on sensitivity and efficiency of the NP detector. Regarding the asymmetric resonance signal, a novel fitting function based on the Fano resonance replacing the conventionally used function of the simple harmonic oscillator and a method to calculate Q by its fitting parameters were developed for a quantitative evaluation. To obtain a better understanding of the resonance behaviours, we analysed the origin of the asymmetric line shapes. Therefore, we compared the frequency response of the on-chip thermal excitation with an external excitation using an in-plane piezo actuator. In correspondence to the Fano effect, we could reconstruct the measured resonance curves by coupling two signals with constant amplitude and the expected signal of the cantilever, respectively. Moreover, the phase of the measurement signal can be analysed by this method, which is important to understand the locking process of the PLL circuit. Besides the frequency analysis, experimental results and calibration measurements with different particle types are presented. Using the described analysis method, decent results to optimize a next

  15. Hanle effect in coherent backscattering

    CERN Document Server

    Labeyrie, G; Müller, C A; Sigwarth, O; Delande, D; Kaiser, R

    2002-01-01

    We study the shape of the coherent backscattering (CBS) cone obtained when resonant light illuminates a thick cloud of laser-cooled rubidium atoms in presence of a homogenous magnetic field. We observe new magnetic field-dependent anisotropies in the CBS signal. We show that the observed behavior is due to the modification of the atomic radiation pattern by the magnetic field (Hanle effect in the excited state).

  16. Strong and Coherent Coupling of a Plasmonic Nanoparticle to a Subwavelength Fabry-Pérot Resonator.

    Science.gov (United States)

    Konrad, Alexander; Kern, Andreas M; Brecht, Marc; Meixner, Alfred J

    2015-07-08

    A major aim in experimental nano- and quantum optics is observing and controlling the interaction between light and matter on a microscopic scale. Coupling molecules or atoms to optical microresonators is a prominent method to alter their optical properties such as luminescence spectra or lifetimes. Until today strong coupling of optical resonators to such objects has only been observed with atom-like systems in high quality resonators. We demonstrate first experiments revealing strong coupling between individual plasmonic gold nanorods (GNR) and a tunable low quality resonator by observing cavity-length-dependent nonlinear dephasing and spectral shifts indicating spectral anticrossing of the luminescent coupled system. These phenomena and experimental results can be described by a model of two coupled oscillators representing the plasmon resonance of the GNR and the optical fields of the resonator. The presented reproducible and accurately tunable resonator allows us to precisely control the optical properties of individual particles.

  17. Heteronuclear intermolecular single-quantum coherences in liquid nuclear magnetic resonance

    Institute of Scientific and Technical Information of China (English)

    Chen Song; Zhu Xiao-Qin; Cai Shu-Hui; Chen Zhong

    2008-01-01

    This paper analyses the heteronuclear Cosy Revamped by Asymmetric Z-gradient Echo Detection pulse sequence.General theoretical expressions of the pulse sequence with arbitrary flip angles were derived by using dipolar field treatment and signals originating from heteronuclear intermolecular single-quantum coherences (iSQCs) in highly-polarized two spin-1/2 systems were mainly discussed in order to find the optimal flip angles.The results show that signals from heteronuclear iSQCs decay slower than those from intermolecular double-quantum coherences or intermolecular zero-quantum coherences. Magical angle experiments validate that the signals are from heteronuclear iSQCs and insensitive to the imperfection of radio-frequency flip angles. All experimental observations are in excellent agreement with theoretical predictions. The quantum-mechanical treatment leads to similar predictions to the dipolar field treatment.

  18. Effects of time delay and random rewiring on the stochastic resonance in excitable small-world neuronal networks.

    Science.gov (United States)

    Yu, Haitao; Wang, Jiang; Du, Jiwei; Deng, Bin; Wei, Xile; Liu, Chen

    2013-05-01

    The effects of time delay and rewiring probability on stochastic resonance and spatiotemporal order in small-world neuronal networks are studied in this paper. Numerical results show that, irrespective of the pacemaker introduced to one single neuron or all neurons of the network, the phenomenon of stochastic resonance occurs. The time delay in the coupling process can either enhance or destroy stochastic resonance on small-world neuronal networks. In particular, appropriately tuned delays can induce multiple stochastic resonances, which appear intermittently at integer multiples of the oscillation period of the pacemaker. More importantly, it is found that the small-world topology can significantly affect the stochastic resonance on excitable neuronal networks. For small time delays, increasing the rewiring probability can largely enhance the efficiency of pacemaker-driven stochastic resonance. We argue that the time delay and the rewiring probability both play a key role in determining the ability of the small-world neuronal network to improve the noise-induced outreach of the localized subthreshold pacemaker.

  19. Excitation of half-integer resonances by random quadrupole field errors in the BETA-BEAM RCS

    CERN Document Server

    Lachaize, A

    The Rapid Cycling Synchrotron of the Beta-Beam facility has been designed to operatewith horizontal and vertical tunes between 6 and 7 in order to avoid systematicresonances up to the fourth order. Nevertheless, unavoidable magnet imperfections mayexcite non systematic second order resonances which may pertub particle motion.In this paper an Hamiltonian treatment based on a well established formalism [1-3] is used to analyze the resonance excitation and to suggest correction schemes minimizing their effects.[1] A. Schoch. Theory of linear and non linear perturbations of betatron oscillations inalternating gradient synchrotrons. CERN 52-21, 1958.[2] G. Guignard. A general treatment of resonances in accelerators. CERN 78-11, 1978.[3] J-L. Laclare, G. Leleux, and A. Tkatchenko. Resonnances quadrupolaires- aleatoiresquadrupolaires et corrections. DSS-GERS- 74-91/TP-06, 1974.

  20. Resonant and nonresonant vibrational excitation of ammonia molecules in the growth of gallium nitride using laser-assisted metal organic chemical vapour deposition

    Science.gov (United States)

    Golgir, Hossein Rabiee; Zhou, Yun Shen; Li, Dawei; Keramatnejad, Kamran; Xiong, Wei; Wang, Mengmeng; Jiang, Li Jia; Huang, Xi; Jiang, Lan; Silvain, Jean Francois; Lu, Yong Feng

    2016-09-01

    The influence of exciting ammonia (NH3) molecular vibration in the growth of gallium nitride (GaN) was investigated by using an infrared laser-assisted metal organic chemical vapor deposition method. A wavelength tunable CO2 laser was used to selectively excite the individual vibrational modes. Resonantly exciting the NH-wagging mode (v2) of NH3 molecules at 9.219 μm led to a GaN growth rate of 84 μm/h, which is much higher than the reported results. The difference between the resonantly excited and conventional thermally populated vibrational states was studied via resonant and nonresonant vibrational excitations of NH3 molecules. Resonant excitation of various vibrational modes was achieved at 9.219, 10.35, and 10.719 μm, respectively. Nonresonant excitation was conducted at 9.201 and 10.591 μm, similar to conventional thermal heating. Compared to nonresonant excitation, resonant excitation noticeably promotes the GaN growth rate and crystalline quality. The full width at half maximum value of the XRD rocking curves of the GaN (0002) and GaN (10-12) diffraction peaks decreased at resonant depositions and reached its minimum value of 45 and 53 arcmin, respectively, at the laser wavelength of 9.219 μm. According to the optical emission spectroscopic studies, resonantly exciting the NH3 v2 mode leads to NH3 decomposition at room temperature, reduces the formation of the TMGa:NH3 adduct, promotes the supply of active species in GaN formation, and, therefore, results in the increased GaN growth rate.

  1. Acoustic excitation of diffusion flames with coherent structure in a plane shear layer.; Effects of acoustic excitation on combustion properties; Soshiki kozo wo tomonau sendan kakusan kaen no onkyo reiki.; Onkyo reiki ni yoru nensho tokusei no henka

    Energy Technology Data Exchange (ETDEWEB)

    Ishino, Y.; Kojima, T.; Oiwa, N.; Yamaguchi, S. [Nagoya Institute of Technology, Nagoya (Japan)

    1993-10-25

    This paper reports on experiments for acoustic excitation of plane shear structured flame. Flows of air separated into the higher velocity side and the lower velocity side by a partition on the center of a flow path merge at the measuring point to form a mixed layer with coherent structure. Fuel is supplied to this mixed layer with the flows so adjusted that the generated flame will attach to the partition on the lower velocity side. Acoustic excitation (at a sound pressure level of 100 dB to 120 dB) is performed in a speaker fitted on a wall on the higher velocity side. The paper mentions the results of the experiments as follows: the acoustic excitation produces such changes to diffusion flame in the plane shear layer as shorter flame and blue flame combustion and clarification of flame structures; as seen from spectral characteristics of temperature change in the flames, a flame acoustically excited strongly presents remarkable improvements in periodicity of the structure; as seen from sound pressure distribution in the flow direction at the measuring point, the flame zone of the flame acoustically excited strongly is positioned at the middle of the node and loop of a standing wave. 6 refs., 9 figs., 1 tab.

  2. Multiple-resonance local wave functions for accurate excited states in quantum Monte Carlo

    NARCIS (Netherlands)

    Zulfikri, Habiburrahman; Amovilli, Claudio; Filippi, Claudia

    2016-01-01

    We introduce a novel class of local multideterminant Jastrow–Slater wave functions for the efficient and accurate treatment of excited states in quantum Monte Carlo. The wave function is expanded as a linear combination of excitations built from multiple sets of localized orbitals that correspond to

  3. Traveling Wave Resonance and Simplified Analysis Method for Long-Span Symmetrical Cable-Stayed Bridges under Seismic Traveling Wave Excitation

    Directory of Open Access Journals (Sweden)

    Zhong-ye Tian

    2014-01-01

    Full Text Available The seismic responses of a long-span cable-stayed bridge under uniform excitation and traveling wave excitation in the longitudinal direction are, respectively, computed. The numerical results show that the bridge’s peak seismic responses vary significantly as the apparent wave velocity decreases. Therefore, the traveling wave effect must be considered in the seismic design of long-span bridges. The bridge’s peak seismic responses do not vary monotonously with the apparent wave velocity due to the traveling wave resonance. A new traveling wave excitation method that can simplify the multisupport excitation process into a two-support excitation process is developed.

  4. Excited state structures and decay dynamics of 1,3-dimethyluracils in solutions: resonance Raman and quantum mechanical calculation study.

    Science.gov (United States)

    Li, Ming-Juan; Liu, Ming-Xia; Zhao, Yan-Ying; Pei, Ke-Mei; Wang, Hui-Gang; Zheng, Xuming; Fang, Wei Hai

    2013-10-03

    The resonance Raman spectroscopic study of the excited state structural dynamics of 1,3-dimethyluracil (DMU), 5-bromo-1,3-dimethyluracil (5BrDMU), uracil, and thymine in water and acetonitrile were reported. Density functional theory calculations were carried out to help elucidate the ultraviolet electronic transitions associated with the A-, and B-band absorptions and the vibrational assignments of the resonance Raman spectra. The effect of the methylation at N1, N3 and C5 sites of pyrimidine ring on the structural dynamics of uracils in different solvents were explored on the basis of the resonance Raman intensity patterns. The relative resonance Raman intensities of DMU and 5BrDMU are computed at the B3LYP-TD level. Huge discrepancies between the experimental resonance Raman intensities and the B3LYP-TD predicted ones were observed. The underlying mechanism was briefly discussed. The decay channel through the S1((1)nπ*)/S2((1)ππ*) conical intersection and the S1((1)nπ*)/T1((3)ππ*) intersystem crossing were revealed by using the CASSCF(8,7)/6-31G(d) level of theory calculations.

  5. Excitation of the Roper resonance in single- and double-pion production in nucleon-nucleon collisions

    Energy Technology Data Exchange (ETDEWEB)

    Skorodko, T.; Bashkanov, M.; Clement, H.; Doroshkevich, E.; Khakimova, O.; Kaskulov, M.; Keleta, S.; Kren, F.; Meier, R.; Wagner, G.J. [Physikalisches Institut der Universitaet Tuebingen, Tuebingen (Germany); Bogoslawsky, D.; Ivanov, G.; Jiganov, E.; Kuznetsov, A.; Morosov, B.; Petukhov, Y.; Povtorejko, A.; Tikhomirov, V. [Joint Institute for Nuclear Research, Dubna (Russian Federation); Calen, H.; Ekstroem, C.; Franssen, K.; Kupsc, A.; Marciniewski, P. [The Svedberg Laboratory, Uppsala (Sweden); Cappellaro, F.; Duniec, D.; Gustafsson, L.; Hoeistad, B.; Jacewicz, M.; Johansson, T.; Koch, I.; Kullander, S.; Petterson, H.; Schoenning, K.; Thoerngren-Engblom, P.; Zlomanczuk, J. [Uppsala University, Uppsala (Sweden); Demiroers, L.; Pauly, C.; Scobel, W. [Hamburg University, Hamburg (Germany); Shwartz, B. [Budker Institute of Nuclear Physics, Novosibirsk (Russian Federation); Sopov, V. [Institute of Theoretical and Experimental Physics, Moscow (Russian Federation); Stepeniak, J. [Soltan Institute of Nuclear Studies, Warsaw (Poland); Wolke, M. [Forschungszentrum Juelich (Germany); Yamamoto, A. [High Energy Accelerator Research Organization, Tsukuba (Japan); Zabierowski, J. [Soltan Institute of Nuclear Studies, Lodz (Poland)

    2008-03-15

    In most investigations the Roper resonance is sensed only very indirectly via complex partial-wave analyses. We find indications for its excitation in the invariant n{pi}{sup +} mass spectrum of the pp{yields}np{pi}{sup +} reaction at M{approx}1360 MeV with a width of {approx} 150 MeV. The values fit very favorably to the most recent phase shift results as well as to the observations at BES. In the near-threshold two-pion production pp{yields}pp{pi}{sup 0}{pi}{sup 0}, where the Roper excitation and its subsequent decays via the routes N{sup *}{yields}{delta}{pi}{yields} N{pi}{pi} and N{sup *}{yields}N{sigma} are the only dominant processes, we find its direct decay into the N{sigma} channel to be the by far dominating decay process -in favor of a monopole excitation of the Roper resonance. (orig.)

  6. Interplay between relativistic energy corrections and resonant excitations in x-ray multiphoton ionization dynamics of Xe atoms

    Science.gov (United States)

    Toyota, Koudai; Son, Sang-Kil; Santra, Robin

    2017-04-01

    In this paper, we theoretically study x-ray multiphoton ionization dynamics of heavy atoms taking into account relativistic and resonance effects. When an atom is exposed to an intense x-ray pulse generated by an x-ray free-electron laser (XFEL), it is ionized to a highly charged ion via a sequence of single-photon ionization and accompanying relaxation processes, and its final charge state is limited by the last ionic state that can be ionized by a single-photon ionization. If x-ray multiphoton ionization involves deep inner-shell electrons in heavy atoms, energy shifts by relativistic effects play an important role in ionization dynamics, as pointed out in Phys. Rev. Lett. 110, 173005 (2013), 10.1103/PhysRevLett.110.173005. On the other hand, if the x-ray beam has a broad energy bandwidth, the high-intensity x-ray pulse can drive resonant photoexcitations for a broad range of ionic states and ionize even beyond the direct one-photon ionization limit, as first proposed in Nat. Photon. 6, 858 (2012), 10.1038/nphoton.2012.261. To investigate both relativistic and resonance effects, we extend the xatom toolkit to incorporate relativistic energy corrections and resonant excitations in x-ray multiphoton ionization dynamics calculations. Charge-state distributions are calculated for Xe atoms interacting with intense XFEL pulses at a photon energy of 1.5 keV and 5.5 keV, respectively. For both photon energies, we demonstrate that the role of resonant excitations in ionization dynamics is altered due to significant shifts of orbital energy levels by relativistic effects. Therefore, it is necessary to take into account both effects to accurately simulate multiphoton multiple ionization dynamics at high x-ray intensity.

  7. Simulation of Coherent Diffraction Radiation Generation by Pico-Second Electron Bunches in an Open Resonator

    Science.gov (United States)

    Sukhikh, L. G.; Potylitsyn, A. P.; Verigin, D. A.

    2016-07-01

    In this report we present new approach for calculation of processes of diffraction radiation generation, storage and decay in an open resonator based on generalized surface current method. The radiation characteristics calculated using the developed approach were compared with those calculated using Gaussian-Laguerre modes method. The comparison shows reasonable coincidence of the results that allows to use developed method for investigation of more complicated resonators.

  8. Fluorescence resonance-energy-transfer in systems of Rhodamine 6G with ionic liquid showing emissions by excitation at wide wavelength areas.

    Science.gov (United States)

    Izawa, Hironori; Wakizono, Satoshi; Kadokawa, Jun-ichi

    2010-09-14

    Fluorescence resonance-energy-transfer occurred in a solution of Rhodamine 6G in an ionic liquid by excitation at wide wavelength areas owing to specific fluorescent behavior of the ionic liquid to show emissions at each excitation wavelength, which was also observed in the guar gum/ionic liquid gel material containing Rhodamine 6G.

  9. Artifical Excitation of Ferro-Resonance for Testing Electrotechnical Equipment in Distribution Devices with Increased Voltage

    Directory of Open Access Journals (Sweden)

    Ye. V. Dmitriev

    2006-01-01

    Full Text Available On the basis of the developed device for protection against of ferro-resonant and high-frequency cumulative over-voltages an algorithm for obtaining a voltage imitating ferro-resonant over-voltages is proposed in the paper. This algorithm presupposes to apply a voltage to the secondary transformer side from an extraneous source is proposed.

  10. Nonlinear optical sub-bandgap excitation of ZnO-based photonic resonators

    Energy Technology Data Exchange (ETDEWEB)

    Bader, Christina A.; Zeuner, Franziska; Bader, Manuel H. W.; Zentgraf, Thomas; Meier, Cedrik [Department of Physics and Center for Optoelectronics and Photonics Paderborn (CeOPP), Universität Paderborn, Warburger Str. 100, 33098 Paderborn (Germany)

    2015-12-07

    Zinc oxide (ZnO) is a versatile candidate for photonic devices due to its highly efficient optical emission. However, for pumping of ZnO photonic devices UV-sources are required. Here, we investigate the alternative usage of widely available pulsed near-infrared (NIR)-sources and compare the efficiency of linear and nonlinear excitation processes. We found that bulk ZnO, ZnO thin films grown by molecular beam epitaxy, and ZnO/SiO{sub 2} microdisk devices exhibit strong nonlinear response when excited with NIR pulses (λ ≈ 1060 nm). In addition, we show that the ZnO/SiO{sub 2} microdisks exhibit sharp whispering gallery modes over the blue-yellow part of the visible spectrum for both excitation conditions and high Q-factors up to Q = 4700. The results demonstrate that nonlinear excitation is an efficient way to pump ZnO photonic devices.

  11. Anti-Stokes resonant x-ray Raman scattering for atom specific and excited state selective dynamics

    Science.gov (United States)

    Kunnus, Kristjan; Josefsson, Ida; Rajkovic, Ivan; Schreck, Simon; Quevedo, Wilson; Beye, Martin; Grübel, Sebastian; Scholz, Mirko; Nordlund, Dennis; Zhang, Wenkai; Hartsock, Robert W.; Gaffney, Kelly J.; Schlotter, William F.; Turner, Joshua J.; Kennedy, Brian; Hennies, Franz; Techert, Simone; Wernet, Philippe; Odelius, Michael; Föhlisch, Alexander

    2016-10-01

    Ultrafast electronic and structural dynamics of matter govern rate and selectivity of chemical reactions, as well as phase transitions and efficient switching in functional materials. Since x-rays determine electronic and structural properties with elemental, chemical, orbital and magnetic selectivity, short pulse x-ray sources have become central enablers of ultrafast science. Despite of these strengths, ultrafast x-rays have been poor at picking up excited state moieties from the unexcited ones. With time-resolved anti-Stokes resonant x-ray Raman scattering (AS-RXRS) performed at the LCLS, and ab initio theory we establish background free excited state selectivity in addition to the elemental, chemical, orbital and magnetic selectivity of x-rays. This unparalleled selectivity extracts low concentration excited state species along the pathway of photo induced ligand exchange of Fe(CO)5 in ethanol. Conceptually a full theoretical treatment of all accessible insights to excited state dynamics with AS-RXRS with transform-limited x-ray pulses is given—which will be covered experimentally by upcoming transform-limited x-ray sources.

  12. Collective state of interwall excitons on GaAs/AlGaAs double quantum wells under pulse resonant excitation

    CERN Document Server

    Larionov, A V; Hvam, J; Soerensen, K

    2002-01-01

    The time evolution and kinetics of the photoluminescence (PL) spectra of the interwall excitons under the pulse resonant excitation of the interwall excitons are studied in the GaAs/AlGaAs binary quantum well. It is established, that the collective exciton phase originates with the time delay relative to the exciting pulse (several nanoseconds), which is conditioned by the density and temperature relaxation to the equilibrium values.The origination of the collective phase of the interwall excitons is accompanied by the strong narrowing of the corresponding photoluminescence line, the superlinear growth of its intensity and large time of change in the degree of the circular polarization.The collective exciton phase originates at the temperatures < 6 K and the interwall excitons densities 3 x 10 sup 1 sup 0 cm sup - sup 2

  13. EXCITATION OF GIANT-RESONANCES IN PB-208, SN-120, ZR-90 AND NI-60 BY 84 MEV/NUCLEON O-17 IONS

    NARCIS (Netherlands)

    NETO, RL; ROUSSELCHOMAZ, P; ROCHAIS, L; ALAMANOS, N; AUGER, F; GASTEBOIS, J; GILLIBERT, A; LACEY, R; MICZAIKA, A; PIERROUTSAKOU, D; BARRETTE, J; MARK, SK; TURCOTTE, R; BLUMENFELD, Y; FRASCARIA, N; GARRON, JP; ROYNETTE, JC; SCARPACI, JA; SUOMIJARVI, T; VANDERWOUDE, A; VANDENBERG, AM

    1993-01-01

    Elastic and inelastic scattering of 1435 MeV 170 ions on Pb-208, Sn-120, Zr-90 and Ni-60 have been measured. Hindrance in the excitation of the first 3- states is observed. Parameters of the isoscalar giant monopole and quadrupole resonances are obtained. The quadrupole resonance exhausts approximat

  14. Highly adaptive RF excitation scheme based on conformal resonant CRLH metamaterial ring antennas for 7-Tesla traveling-wave magnetic resonance imaging.

    Science.gov (United States)

    Erni, Daniel; Liebig, Thorsten; Rennings, Andreas; Koster, Norbert H L; Fröhlich, Jürg

    2011-01-01

    We propose an adaptive RF antenna system for the excitation (and manipulation) of the fundamental circular waveguide mode (TE(11)) in the context of high-field (7T) traveling-wave magnetic resonance imaging (MRI). The system consists of composite right-/left-handed (CRLH) meta-material ring antennas that fully conforms to the inner surface of the MRI bore. The specific use of CRLH metamaterials is motivated by its inherent dispersion engineering capabilities, which is needed when designing resonant ring structures for virtually any predefined diameter operating at the given Larmor frequency (i.e. 298 MHz). Each functional group of the RF antenna system consists of a pair of subsequently spaced and correspondingly fed CRLH ring antennas, allowing for the unidirectional excitation of propagating, circularly polarized B(1) mode fields. The same functional group is also capable to simultaneously mold an incoming, counter-propagating mode. Given these functionalities we are proposing now a compound scheme (i.e. periodically arranged multiple antenna pairs)--termed as "MetaBore"--that is apt to provide a tailored RF power distribution as well as full wave reflection compensation virtually at any desired location along the bore.

  15. Effect of spike-timing-dependent plasticity on coherence resonance and synchronization transitions by time delay in adaptive neuronal networks

    Science.gov (United States)

    Xie, Huijuan; Gong, Yubing; Wang, Qi

    2016-06-01

    In this paper, we numerically study how time delay induces multiple coherence resonance (MCR) and synchronization transitions (ST) in adaptive Hodgkin-Huxley neuronal networks with spike-timing dependent plasticity (STDP). It is found that MCR induced by time delay STDP can be either enhanced or suppressed as the adjusting rate Ap of STDP changes, and ST by time delay varies with the increase of Ap, and there is optimal Ap by which the ST becomes strongest. It is also found that there are optimal network randomness and network size by which ST by time delay becomes strongest, and when Ap increases, the optimal network randomness and optimal network size increase and related ST is enhanced. These results show that STDP can either enhance or suppress MCR and optimal STDP can enhance ST induced by time delay in the adaptive neuronal networks. These findings provide a new insight into STDP's role for the information processing and transmission in neural systems.

  16. Effect of Autaptic Activity on Intrinsic Coherence Resonance in Newman-Watts Networks of Stochastic Hodgkin-Huxley Neurons

    Science.gov (United States)

    Wang, Qi; Gong, Yubing

    2016-06-01

    In this paper, we study the effect of autaptic activity on intrinsic coherence resonance (CR) induced by channel noise in Newman-Watts (NW) networks of stochastic Hodgkin-Huxley (HH) neurons. It is found that autaptic strength and autaptic delay have a big effect on the intrinsic CR. As autaptic strength increases, there is optimal autaptic strength by which the intrinsic CR is most highly enhanced. Autaptic delay can enhance, reduce, or destroy the intrinsic CR, depending on the delay length. Moreover, there are optimal coupling strength and network randomness by which autaptic activity can most highly enhance the intrinsic CR. These results show that autaptic activity has different effects on the intrinsic CR in the neuronal networks, and it can most highly enhance the intrinsic CR at optimal coupling strength and network randomness. These findings could find potential implications of channel noise and autaptic activity for the information processing and transmission in neural systems.

  17. Ionization potentials, electron affinities, resonance excitation energies, oscillator strengths, and ionic radii of element Uus (Z = 117) and astatine.

    Science.gov (United States)

    Chang, Zhiwei; Li, Jiguang; Dong, Chenzhong

    2010-12-30

    Multiconfiguration Dirac-Fock (MCDF) method was employed to calculate the first five ionization potentials, electron affinities, resonance excitation energies, oscillator strengths, and radii for the element Uus and its homologue At. Main valence correlation effects were taken into account. The Breit interaction and QED effects were also estimated. The uncertainties of calculated IPs, EAs, and IR for Uus and At were reduced through an extrapolation procedure. The good consistency with available experimental and other theoretical values demonstrates the validity of the present results. These theoretical data therefore can be used to predict some unknown physicochemical properties of element Uus, Astatine, and their compounds.

  18. An analytical study on excitation of nuclear-coupled thermal-hydraulic instability due to seismically induced resonance in BWR

    Energy Technology Data Exchange (ETDEWEB)

    Hirano, Masashi [Japan Atomic Energy Research Institute, Ibaraki-ken (Japan)

    1997-07-01

    This paper describes the results of a scoping study on seismically induced resonance of nuclear-coupled thermal-hydraulic instability in BWRs, which was conducted by using TRAC-BF1 within a framework of a point kinetics model. As a result of the analysis, it is shown that a reactivity insertion could occur accompanied by in-surge of coolant into the core resulted from the excitation of the nuclear-coupled instability by the external acceleration. In order to analyze this phenomenon more in detail, it is necessary to couple a thermal-hydraulic code with a three-dimensional nuclear kinetics code.

  19. Evidence of resonant surface wave excitation in the relativistic regime through measurements of proton acceleration from grating targets

    CERN Document Server

    Ceccotti, T; Sgattoni, A; Bigongiari, A; Raynaud, M; Riconda, C; Heron, A; Baffigi, F; Labate, L; Gizzi, L A; Vassura, L; Fuchs, J; Passoni, M; Kveton, M; Novotny, F; Possolt, M; Prokupek, J; Proska, J; Psikal, J; Stolcova, L; Velyhan, A; Bougeard, M; D'Oliveira, P; Tcherbakoff, O; Reau, F; Martin, P; Macchi, A

    2013-01-01

    The interaction of laser pulses with thin grating targets, having a periodic groove at the irradiated surface, has been experimentally investigated. Ultrahigh contrast ($\\sim 10^{12}$) pulses allowed to demonstrate an enhanced laser-target coupling for the first time in the relativistic regime of ultra-high intensity $>10^{19} \\mbox{W/cm}^{2}$. A maximum increase by a factor of 2.5 of the cut-off energy of protons produced by Target Normal Sheath Acceleration has been observed with respect to plane targets, around the incidence angle expected for resonant excitation of surface waves. A significant enhancement is also observed for small angles of incidence, out of resonance.

  20. Active coated nano-particle excited by an arbitrarily located electric Hertzian dipole — resonance and transparency effects

    DEFF Research Database (Denmark)

    Arslanagic, Samel; Ziolkowski, Richard W.

    2010-01-01

    The present work investigates the optical properties of active coated spherical nano-particles excited by an arbitrarily located electric Hertzian dipole. The nano-particles are made of specific dielectric and plasmonic materials. The spatial near-field distribution as well as the normalized...... radiation resistance is examined. Both enhanced as well as reduced radiation effects are demonstrated. In particular, it is shown that specific active coated nano-particles can be designed to be resonant, leading to much larger values of the normalized radiation resistance than is the case...... with the corresponding passive coated nano-particles, thereby overcoming the intrinsic losses present in the plasmonic materials. Moreover, it is shown that other active coated nano-particle designs can significantly reduce the normalized radiation resistance; thus both the resonant as well as non...

  1. Dynamic nuclear spin polarization in the resonant laser excitation of an InGaAs quantum dot.

    Science.gov (United States)

    Högele, A; Kroner, M; Latta, C; Claassen, M; Carusotto, I; Bulutay, C; Imamoglu, A

    2012-05-11

    Resonant optical excitation of lowest-energy excitonic transitions in self-assembled quantum dots leads to nuclear spin polarization that is qualitatively different from the well-known optical orientation phenomena. By carrying out a comprehensive set of experiments, we demonstrate that nuclear spin polarization manifests itself in quantum dots subjected to finite external magnetic field as locking of the higher energy Zeeman transition to the driving laser field, as well as the avoidance of the resonance condition for the lower energy Zeeman branch. We interpret our findings on the basis of dynamic nuclear spin polarization originating from noncollinear hyperfine interaction and find excellent agreement between experiment and theory. Our results provide evidence for the significance of noncollinear hyperfine processes not only for nuclear spin diffusion and decay, but also for buildup dynamics of nuclear spin polarization in a coupled electron-nuclear spin system.

  2. Selective Two-Photon Absorptive Resonance Femtosecond-Laser Electronic-Excitation Tagging (STARFLEET) Velocimetry in Flow and Combustion Diagnostics

    Science.gov (United States)

    Jiang, Naibo; Halls, Benjamin R.; Stauffer, Hans U.; Roy, Sukesh; Danehy, Paul M.; Gord, James R.

    2016-01-01

    Selective Two-Photon Absorptive Resonance Femtosecond-Laser Electronic-Excitation Tagging (STARFLEET), a non-seeded ultrafast-laser-based velocimetry technique, is demonstrated in reactive and non-reactive flows. STARFLEET is pumped via a two-photon resonance in N2 using 202.25-nm 100-fs light. STARFLEET greatly reduces the per-pulse energy required (30 µJ/pulse) to generate the signature FLEET emission compared to the conventional FLEET technique (1.1 mJ/pulse). This reduction in laser energy results in less energy deposited in the flow, which allows for reduced flow perturbations (reactive and non-reactive), increased thermometric accuracy, and less severe damage to materials. Velocity measurements conducted in a free jet of N2 and in a premixed flame show good agreement with theoretical velocities and further demonstrate the significantly less-intrusive nature of STARFLEET.

  3. A Theoretical Distinction Between Time-Resolved Resonance Raman andResonance Fluorescence

    Institute of Scientific and Technical Information of China (English)

    LU Jing; DU Si-De; FAN Kang-Nian; Lee Soo-Ying

    2000-01-01

    Based on the time-dependent theory, an analysis of the distinction between resonance Raman (RR) and resonance fluorescence (RF) with pulse excitation was presented. The real population of the intermediate state gives two optical components-the independent time evolution of intermediate ket and bra states generates RR while RF originates from the phase coherent between ket and bra states. In cw limit, the transition probability of spontaneous emission with pulse excitation can be reduced to the classical theory.

  4. Resonant vibrational-excitation cross sections and rate constants for low-energy electron scattering by molecular oxygen

    CERN Document Server

    Laporta, V; Tennyson, J

    2016-01-01

    Resonant vibrational-excitation cross sections and rate constants for electron scattering by molecular oxygen are presented. Transitions between all 42 vibrational levels of O$_2(\\textrm{X}\\ ^3\\Sigma_g^- $) are considered. Molecular rotations are parameterized by the rotational quantum number $J$ which is considered in the range 1 to 151. The lowest four resonant states of O$_2^-$, $^2\\Pi_g$, $^2\\Pi_u$, $^4\\Sigma_u^-$ and $^2\\Sigma_u^-$, are taken into account. The calculations are performed using the fixed-nuclei R-matrix approach to determine the resonance positions and widths, and the boomerang model to characterize the nuclei motion. Two energy regions below and above 4~eV are investigated: the first one is characterized by sharp structures in the cross section, and the second by a broad resonance peaked at 10~eV. The computed cross sections are compared with theoretical and experimental results available in literature for both the energy regions, and are made available for use by modelers. The effect of ...

  5. Bright broadband coherent fiber sources emitting strongly blue-shifted resonant dispersive wave pulses

    DEFF Research Database (Denmark)

    Tu, Haohua; Lægsgaard, Jesper; Zhang, Rui;

    2013-01-01

    We predict and realize the targeted wavelength conversion from the 1550-nm band of a fs Er:fiber laser to an isolated band inside 370-850 nm, corresponding to a blue-shift of 700-1180 nm. The conversion utilizes resonant dispersive wave generation in widely available optical fibers with good...

  6. Extended coherence lifetimes in microcavities under angle-resonant pumping conditions

    DEFF Research Database (Denmark)

    Østergaard, John Erland; Birkedal, Dan; Mizeikis, V.;

    2001-01-01

    processes by the final-state polariton population. Strong enhancements of the scattering processes have been observed as a result of up to several 100 polaritons per final k-state under angle-resonant pumping conditions (Erland et al, 2000; Stevenson et al, 2000). Energy and wave vector are conserved...

  7. Coherent propagation of a short polarised radiation pulse in a one-dimensional resonance Bragg grating

    NARCIS (Netherlands)

    Maimistov, A. I.; Polikarpov, V. V.

    2006-01-01

    The propagation of an optical ultrashort pulse in a resonance Bragg grating is considered taking into account the polarisation of electromagnetic radiation. It is assumed that the grating is formed by thin films containing two-level atoms with the triply degenerate upper energy level. The system of

  8. Photon-statistics excitation spectroscopy of a single two-level system

    Science.gov (United States)

    Strauß, Max; Placke, Marlon; Kreinberg, Sören; Schneider, Christian; Kamp, Martin; Höfling, Sven; Wolters, Janik; Reitzenstein, Stephan

    2016-06-01

    We investigate the influence of the photon statistics on the excitation dynamics of a single two-level system. A single semiconductor quantum dot represents the two-level system and is resonantly excited either with coherent laser light, or excited with chaotic light, with photon statistics corresponding to that of thermal radiation. Experimentally, we observe a reduced absorption cross section under chaotic excitation in the steady state. In the transient regime, the Rabi oscillations observable under coherent excitation disappear under chaotic excitation. Likewise, in the emission spectrum, the well-known Mollow triplet, which we observe under coherent drive, disappears under chaotic excitation. Our observations are fully consistent with theoretical predictions based on the semiclassical Bloch equation approach.

  9. Photon-Statistics Excitation Spectroscopy of a Single Two Level System

    CERN Document Server

    Strauß, M; Kreinberg, S; Schneider, C; Kamp, M; Höfling, S; Wolters, J; Reitzenstein, S

    2016-01-01

    We investigate the influence of the photon statistics on the excitation dynamics of a single two level system. A single semiconductor quantum dot represents the two level system and is resonantly excited either with coherent laser light, or excited with chaotic light, with photon statistics corresponding to that of thermal radiation. Experimentally, we observe a reduced absorption cross-section under chaotic excitation in the steady-state. In the transient regime, the Rabi oscillations observable under coherent excitation disappear under chaotic excitation. Likewise, in the emission spectrum the well-known Mollow triplet, which we observe under coherent drive, disappears under chaotic excitation. Our observations are fully consistent with theoretical predictions based on the semi-classical Bloch equation approach.

  10. Pulsed microwave-driven argon plasma jet with distinctive plume patterns resonantly excited by surface plasmon polaritons

    Science.gov (United States)

    Chen, Zhao-Quan; Yin, Zhi-Xiang; Xia, Guang-Qing; Hong, Ling-Li; Hu, Ye-Lin; Liu, Ming-Hai; Hu, Xi-Wei; A. Kudryavtsev, A.

    2015-02-01

    Atmospheric lower-power pulsed microwave argon cold plasma jets are obtained by using coaxial transmission line resonators in ambient air. The plasma jet plumes are generated at the end of a metal wire placed in the middle of the dielectric tubes. The electromagnetic model analyses and simulation results suggest that the discharges are excited resonantly by the enhanced electric field of surface plasmon polaritons. Moreover, for conquering the defect of atmospheric argon filamentation discharges excited by 2.45-GHz of continued microwave, the distinctive patterns of the plasma jet plumes can be maintained by applying different gas flow rates of argon gas, frequencies of pulsed modulator, duty cycles of pulsed microwave, peak values of input microwave power, and even by using different materials of dielectric tubes. In addition, the emission spectrum, the plume temperature, and other plasma parameters are measured, which shows that the proposed pulsed microwave plasma jets can be adjusted for plasma biomedical applications. Project supported by the National Natural Science Foundation of China (Grant Nos. 11105002 and 61170172), the Natural Science Foundation of Anhui Province, China (Grant Nos. 1408085QA16 and 1408085ME101), the China Postdoctoral Science Foundation (Grant No. 2014M551788), and the Open-end Fund of State Key Laboratory of Advanced Electromagnetic Engineering and Technology (HUST), China (Grant No. GZ1301).

  11. Coherent Population Trapping Resonances in Buffer Gas-filled Cs Vapor Cells with Push-Pull Optical Pumping

    CERN Document Server

    Liu, Xiaochi; Guérandel, Stéphane; Gorecki, Christophe; de Clercq, Emeric; Boudot, Rodolphe

    2013-01-01

    We report on a theoretical study and experimental characterization of coherent population trapping (CPT) resonances in buffer gas-filled vapor cells with push-pull optical pumping (PPOP) on Cs D1 line. We point out that the push-pull interaction scheme is identical to the so-called lin per lin polarization scheme. Expressions of the relevant dark states, as well as of absorption, are reported. The experimental setup is based on the combination of a distributed feedback (DFB) diode laser, a pigtailed intensity Mach-Zehnder electro-optic modulator (MZ EOM) for optical sidebands generation and a Michelson-like interferometer. A microwave technique to stabilize the transfer function operating point of the MZ EOM is implemented for proper operation. A CPT resonance contrast as high as 78% is reported in a cm-scale cell for the magnetic-field insensitive clock transition. The impact of the laser intensity on the CPT clock signal key parameters (linewidth - contrast - linewidth/contrast ratio) is reported for three ...

  12. Resonant Excitation of a Truncated Metamaterial Cylindrical Shell by a Thin Wire Monopole

    DEFF Research Database (Denmark)

    Kim, Oleksiy S.; Erentok, Aycan; Breinbjerg, Olav

    2009-01-01

    A truncated metamaterial cylindrical shell excited by a thin wire monopole is investigated using the integral equation technique as well as the finite element method. Simulations reveal a strong field singularity at the edge of the truncated cylindrical shell, which critically affects the matching...

  13. Coherent zero-field magnetization resonance in a dipolar spin-1 Bose-Einstein condensate

    Science.gov (United States)

    Zhang, Wenxian; Yi, S.; Chapman, M. S.; You, J. Q.

    2015-08-01

    With current magnetic-field shielding and high-precision detection in dipolar spinor Bose-Einstein condensates, it is possible to experimentally detect the low- or zero-field nonsecular dipolar dynamics. Here we analytically investigate the zero-field nonsecular magnetic dipolar interaction effect, with an emphasis on magnetization dynamics in a spin-1 Bose-Einstein condensate under the single spatial mode approximation within the mean-field theory. Due to the biaxial nature of the dipolar interaction, a novel resonance occurs in the condensate magnetization oscillation, in contrast to the previous assumption of a conserved magnetization in strong magnetic fields. Furthermore, we propose a dynamical-decoupling detection method for such a resonance, which cancels the stray magnetic fields in experiment but restores the magnetization dynamics. Our results shed light on the dipolar systems and may find potential applications beyond cold atoms.

  14. Probing the quantum coherence of a nanomechanical resonator using a superconducting qubit: II. Implementation

    Energy Technology Data Exchange (ETDEWEB)

    Blencowe, M P [Department of Physics and Astronomy, 6127 Wilder Laboratory, Dartmouth College, Hanover, NH 03755 (United States); Armour, A D [School of Physics and Astronomy, University of Nottingham, Nottingham, NG7 2RD (United Kingdom)], E-mail: miles.p.blencowe@dartmouth.edu, E-mail: andrew.armour@nottingham.ac.uk

    2008-09-15

    We describe a possible implementation of the nanomechanical quantum superposition generation and detection scheme described in the preceding, companion paper (Armour A D and Blencowe M P 2008 New. J. Phys. 10 095004). The implementation is based on the circuit quantum electrodynamics (QED) set-up, with the addition of a mechanical degree of freedom formed out of a suspended, doubly-clamped segment of the superconducting loop of a dc SQUID located directly opposite the centre conductor of a coplanar waveguide (CPW). The relative merits of two SQUID based qubit realizations are addressed, in particular a capacitively coupled charge qubit and inductively coupled flux qubit. It is found that both realizations are equally promising, with comparable qubit-mechanical resonator mode as well as qubit-microwave resonator mode coupling strengths.

  15. Enhancement of Coherent THz Smith-Purcell Radiation by Resonance Overlapping

    Science.gov (United States)

    Li, Weiwei; Xu, Yuanfang; Lu, Yalin; He, Zhigang; Jia, Qika; Wang, Lin

    2017-01-01

    Frequency-locked coherent Smith-Purcell Radiation (SPR) is emitted when a train of pre-bunched electron beam passes close to the surface of a metallic grating, which develops an energy density spectrum restricted to harmonics of the bunching frequency. For the lamellar grating with narrow grooves, the radiation spectrum from a single electron can also have a feature of narrow band, which is related to the grating structure and the beam energy. The combination of them is proposed in this paper. By properly choosing the parameters, the peak frequency of single electron radiation can be overlapped with the harmonics of the bunching frequency of the electron bunch train, leading to the generation of extremely intense narrow-band THz radiation.

  16. Enhancement of Coherent THz Smith-Purcell Radiation by Resonance Overlapping

    Science.gov (United States)

    Li, Weiwei; Xu, Yuanfang; Lu, Yalin; He, Zhigang; Jia, Qika; Wang, Lin

    2016-08-01

    Frequency-locked coherent Smith-Purcell Radiation (SPR) is emitted when a train of pre-bunched electron beam passes close to the surface of a metallic grating, which develops an energy density spectrum restricted to harmonics of the bunching frequency. For the lamellar grating with narrow grooves, the radiation spectrum from a single electron can also have a feature of narrow band, which is related to the grating structure and the beam energy. The combination of them is proposed in this paper. By properly choosing the parameters, the peak frequency of single electron radiation can be overlapped with the harmonics of the bunching frequency of the electron bunch train, leading to the generation of extremely intense narrow-band THz radiation.

  17. Characterizing passive coherent population trapping resonance in a cesium vapor cell filled with neon buffer gas

    Institute of Scientific and Technical Information of China (English)

    Liu Zhi; Wang Jie-Ying; Diao Wen-Ting; He Jun; Wang Jun-Min

    2013-01-01

    We present a pair of phase-locked lasers with a 9.2-GHz frequency difference through the injection locking of a master laser to the RF-modulation sideband of a slave diode laser.Using this laser system,a coherent population trapping (CPT)signal with a typical linewidth of ~ 182 Hz is obtained in a cesium vapor cell filled with 30 Torr (4 kPa) of neon as the buffer gas.We investigate the influence of the partial pressure of the neon buffer gas on the CPT linewidth,amplitude,and frequency shift.The results may offer some references for CPT atomic clocks and CPT atomic magnetometers.

  18. Resonant Excitation of Disk Oscillations in Deformed Disks VII: Stability Criterion in MHD Systems

    CERN Document Server

    Kato, Shoji

    2013-01-01

    In a disk with an oscillatory deformation from an axisymmetric state with frequency $\\omega_{\\rm D}$ and azimuthal wavenumber $m_{\\rm D}$, a set of two normal mode oscillations with frequency and azimuthal wavenumber being ($\\omega_1$, $m_1$) and ($\\omega_2$, $m_2$) resonantly couple through the disk deformation, when the resonant conditions ($\\omega_1+\\omega_2+\\omega_{\\rm D}=0$ and $m_1+m_2+m_{\\rm D}=0$) are satisfied. In the case of hydrodynamical disks, the resonance amplifies the set of the oscillations if $(E_1/\\omega_1)(E_2/\\omega_2)>0$ (Kato 2013b), where $E_1$ and $E_2$ are wave energies of the two oscillations with $\\omega_1$ and $\\omega_2$, respectively. In this paper we show that this instability criterion is still valid even when the oscillations are ideal MHD ones in magnetized disks, if the displacements associated with the oscillations vanish on the boundary of the system.

  19. Electron heating via the self-excited plasma series resonance in geometrically symmetric multi-frequency capacitive plasmas

    CERN Document Server

    Schuengel, E; Donko, Z; Korolov, I; Derzsi, A; Schulze, J

    2016-01-01

    The self-excitation of Plasma Series Resonance (PSR) oscillations plays an important role in the electron heating dynamics in Capacitively Coupled Radio Frequency (CCRF) plasmas. In a combined approach of PIC/MCC simulations and a theoretical model based on an equivalent circuit, we investigate the self-excitation of PSR oscillations and their effect on the electron heating in geometrically symmetric CCRF plasmas driven by multiple consecutive harmonics. The discharge symmetry is controlled via the Electrical Asymmetry Effect, i.e. by varying the total number of harmonics and tuning the phase shifts between them. It is demonstrated that PSR oscillations will be self-excited under both symmetric and asymmetric conditions, if (i) the charge-voltage relation of the plasma sheaths deviates from a simple quadratic behavior and if (ii) the inductance of the plasma bulk exhibits a temporal modulation. These two effects have been neglected up to now, but we show that they must be included in the model in order to pro...

  20. Resonance Raman spectra of TNT and RDX using vibronic theory, excited-state gradient, and complex polarizability approximations.

    Science.gov (United States)

    Al-Saidi, W A; Asher, Sanford A; Norman, Patrick

    2012-08-02

    Geometries, UV absorption bands, and resonance Raman (RR) cross sections of TNT and RDX are investigated using density functional theory (DFT) in conjunction with the Coulomb attenuated B3LYP exchange-correlation functional. The absorption and RR spectra are determined with use of vibronic (VB) theory, excited-state gradient, and complex polarizability (CPP) approximations. We examined low-energy isomers (two for TNT and four for RDX) whose energies differ by less than 1 kcal/mol, such that they would appreciably be populated at room temperature. The two TNT isomers differ by an internal rotation of the methyl group, while the four conformers of RDX differ by the arrangements of the nitro group relative to the ring. Our theoretical optical properties of the TNT and RDX isomers are in excellent agreement with experimental and recent CCSD-EOM results, respectively. For the two TNT isomers, the ultraviolet RR (UVRR) spectra are similar and in good agreement with recently measured experimental results. Additionally, the UVRR spectra computed using the excited-state and CPP approaches compare favorably with the VB theory results. On the other hand, the RR spectra of the RDX conformers differ from one another, reflecting the importance of the positioning of the NO2 groups with respect to the ring. In the gas phase or in solution, RDX would give a spectrum associated with a conformationally averaged structure. It is encouraging that the computed spectra of the conformers show similarities to recent measured RDX spectra in acetonitrile solution, and reproduce the 10-fold decrease in the absolute Raman cross sections of RDX compared to TNT for the observed 229 nm excitation. We show that in TNT and RDX vibrational bands that couple to NO2 or the ring are particularly resonance enhanced. Finally, the computed RDX spectra of the conformers present a benchmark for understanding the RR spectra of the solid-phase polymorphs of RDX.

  1. Resonant generation of an electron–positron pair by two photons to excited Landau levels

    Energy Technology Data Exchange (ETDEWEB)

    Diachenko, M. M., E-mail: dyachenko.michail@mail.ru; Novak, O. P.; Kholodov, R. I. [National Academy of Sciences of Ukraine, Institute of Applied Physics (Ukraine)

    2015-11-15

    We consider the resonant generation of an electron–positron pair by two polarized photons to arbitrarily low Landau levels. The resonance occurs when the energy of one photon exceeds the one-photon generation threshold, and the energy of the other photon is multiple to the spacing between the levels. The cross section of the process is determined taking into account the spins of particles. The order of magnitude of the cross section is the highest when the magnetic moments of the particles are oriented along the magnetic field.

  2. Tunable repetition rate VECSEL for resonant acoustic-excitation of nanostructures

    Science.gov (United States)

    Chen Sverre, T.; Head, C. R.; Turnbull, A. P.; Shaw, E. A.; Tropper, A. C.; Muskens, O. L.

    2016-03-01

    We report a passively mode-locked InGaAs-quantum well VECSEL, emitting a constant pulse train at an average output power of 18 mW and emission wavelength of 1035 nm, with a continuously tunable pulse repetitionfrequency (PRF) between 0.88 - 1.88 GHz. Pulse duration was 230 fs over 80% of that range. Here we propose a technique making use of the demonstrated VECSEL PRF tunability for a resonant frequency-domain pumpprobe spectroscopic technique for acoustic interrogation of nanostructures. Simulation of suitable GHz acoustic resonators to demonstrate this technique is described.

  3. Ultrahigh-Resolution Magnetic Resonance in Inhomogeneous Magnetic Fields: Two-Dimensional Long-Lived-Coherence Correlation Spectroscopy

    Science.gov (United States)

    Chinthalapalli, Srinivas; Bornet, Aurélien; Segawa, Takuya F.; Sarkar, Riddhiman; Jannin, Sami; Bodenhausen, Geoffrey

    2012-07-01

    A half-century quest for improving resolution in Nuclear Magnetic Resonance (NMR) and Magnetic Resonance Imaging (MRI) has enabled the study of molecular structures, biological interactions, and fine details of anatomy. This progress largely relied on the advent of sophisticated superconducting magnets that can provide stable and homogeneous fields with temporal and spatial variations below ΔB0/B0lungs, tissue-air interfaces, surgical implants, etc., lead to fluctuations and losses of local homogeneity. A new method dubbed “long-lived-coherence correlation spectroscopy” (LLC-COSY) opens the way to overcome both inhomogeneous and homogeneous broadening, which arise from local variations in static fields and fluctuating dipole-dipole interactions, respectively. LLC-COSY makes it possible to obtain ultrahigh resolution two-dimensional spectra, with linewidths on the order of Δν=0.1 to 1 Hz, even in very inhomogeneous fields (ΔB0/B0>10ppm or 5000 Hz at 9.7 T), and can improve resolution by a factor up to 9 when the homogeneous linewidths are determined by dipole-dipole interactions. The resulting LLC-COSY spectra display chemical shift differences and scalar couplings in two orthogonal dimensions, like in “J spectroscopy.” LLC-COSY does not require any sophisticated gradient switching or frequency-modulated pulses. Applications to in-cell NMR and to magnetic resonance spectroscopy (MRS) of selected volume elements in MRI appear promising, particularly when susceptibility variations tend to preclude high resolution.

  4. Resonance raman and absorption spectra of isomeric retinals in their lowest excited triplet states

    DEFF Research Database (Denmark)

    Wilbrandt, Robert Walter; Jensen, N.-H.; Houee-Levin, C.

    1985-01-01

    implications about the size of the energy barriers separating the various triplet species are discussed. The resonance Raman spectra obtained by using either anthracene (ET = 177.7 kJ mol-1) or naphthalene (ET = 254.8 kJ mol-1) as sensitizers were virtually identical for the corresponding triplet states from...

  5. Resonant circuit which provides dual-frequency excitation for rapid cycling of an electromagnet

    Science.gov (United States)

    Praeg, W.F.

    1982-03-09

    Disclosed is a novel ring-magnet control circuit that permits synchrotron repetition rates much higher than the frequency of the sinusoidal guide field of the ring magnet during particle acceleration. The control circuit generates sinusoidal excitation currents of different frequencies in the half waves. During radio-frequency acceleration of the synchrotron, the control circuit operates with a lower frequency sine wave and, thereafter, the electromagnets are reset with a higher-frequency half sine wave.

  6. Spin-locking of half-integer quadrupolar nuclei in nuclear magnetic resonance of solids: creation and evolution of coherences.

    Science.gov (United States)

    Ashbrook, Sharon E; Wimperis, Stephen

    2004-02-08

    Spin-locking of half-integer quadrupolar nuclei, such as 23Na (I=3/2) and 27Al (I=5/2), is of renewed interest owing to the development of variants of the multiple-quantum and satellite-transition magic angle spinning (MAS) nuclear magnetic resonance experiments that either utilize spin-locking directly or offer the possibility that spin-locked states may arise. However, the large magnitude and, under MAS, the time dependence of the quadrupolar interaction often result in complex spin-locking phenomena that are not widely understood. Here we show that, following the application of a spin-locking pulse, a variety of coherence transfer processes occur on a time scale of approximately 1/omegaQ before the spin system settles down into a spin-locked state which may itself be time dependent if MAS is performed. We show theoretically for both spin I=3/2 and 5/2 nuclei that the spin-locked state created by this initial rapid dephasing typically consists of a variety of single- and multiple-quantum coherences and nonequilibrium population states and we discuss the subsequent evolution of these under MAS. In contrast to previous work, we consider spin-locking using a wide range of radio frequency field strengths, i.e., a range that covers both the "strong-field" (omega1 > omegaQPAS and "weak-field" (omega1 spin-locking experiments on NaNO2, NaNO3, and Al(acac)3, under both static and MAS conditions, are used to illustrate and confirm the results of the theoretical discussion.

  7. Unquenching the meson spectrum: a model study of excited $\\rho$ resonances

    CERN Document Server

    Rupp, George; van Beveren, Eef

    2016-01-01

    Quark models taking into account the dynamical effects of hadronic decay often produce very different predictions for mass shifts in the hadron spectrum. The consequences for meson spectroscopy can be dramatic and completely obscure the underlying confining force. Recent unquenched lattice calculations of mesonic resonances that also include meson-meson interpolators provide a touchstone for such models, despite the present limitations in applicability. On the experimental side, the $\\rho(770)$ meson and its several observed radial recurrences are a fertile testing ground for both quark models and lattice computations. Here we apply a unitarised quark model that has been successful in the description of many enigmatic mesons to these vector $\\rho$ resonances and the corresponding $P$-wave $\\pi\\pi$ phase shifts. This work is in progress, with encouraging preliminary results.

  8. Excitation of pygmy dipole resonance in neutron-rich nuclei via Coulomb and nuclear fields

    Indian Academy of Sciences (India)

    A Vitturi; E G Lanza; M V Andrés; F Catara; D Gambacurta

    2010-07-01

    We study the nature of the low-lying dipole strength in neutron-rich nuclei, often associated with the pygmy dipole resonance. The states are described within the Hartree–Fock plus RPA formalism, using different parametrizations of the Skyrme inter-action. We show how the information from combined reaction processes involving the Coulomb and different mixtures of isoscalar and isovector nuclear interactions can provide a clue to reveal the characteristic features of these states.

  9. Evidence for resonance electron transfer in photon excited X-ray satellite spectra of fluorine compounds

    Indian Academy of Sciences (India)

    K Ram Narayana; B Seetharami Reddy; S S Raju; T Seshi Reddy; S Lakshmi Narayana; K Premachand; B M Rao; M V R Murti; L S Mombasawala

    2005-08-01

    The KL1/KL0 intensity ratio of fluorine is measured in five fluorine compounds with a crystal spectrometer. An anomalous reduction of this intensity ratio was observed in KF and SrF2, which is attributed to resonance electron transfer from the metal ion to the spectator vacancy in the fluorine ion. KL2/KL0 intensity ratio of fluorine is also measured. The measured relative intensities are compared with the theoretical estimates of Aberg.

  10. Identical synchronization of chaotic secure communication systems with channel induced coherence resonance

    Science.gov (United States)

    Sepantaie, Marc M.; Namazi, Nader M.; Sepantaie, Amir M.

    2016-05-01

    This paper is devoted to addressing the synchronization, and detection of random binary data exposed to inherent channel variations existing in Free Space Optical (FSO) communication systems. This task is achieved by utilizing the identical synchronization methodology of Lorenz chaotic communication system, and its synergetic interaction in adversities imposed by the FSO channel. Moreover, the Lorenz system has been analyzed, and revealed to induce Stochastic Resonance (SR) once exposed to Additive White Gaussian Noise (AWGN). In particular, the resiliency of the Lorenz chaotic system, in light of channel adversities, has been attributed to the success of the proposed communication system. Furthermore, this paper advocates the use of Haar wavelet transform for enhanced detection capability of the proposed chaotic communication system, which utilizes Chaotic Parameter Modulation (CPM) technique for means of transmission.

  11. Noise-induced multimode behavior in excitable systems

    DEFF Research Database (Denmark)

    Postnov, D E; Sosnovtseva, Olga; Han, S K;

    2002-01-01

    Based on experiments with electronic circuits, we show how a system of coupled excitable units can possess several noise-induced oscillatory modes. We characterize the multimode organization in terms of the coherence resonance effect. Multiple gain of regularity is found to be related to different...

  12. Extreme secular excitation of eccentricity inside mean motion resonance. Small bodies driven into star-grazing orbits by planetary perturbations

    Science.gov (United States)

    Pichierri, Gabriele; Morbidelli, Alessandro; Lai, Dong

    2017-09-01

    Context. It is well known that asteroids and comets fall into the Sun. Metal pollution of white dwarfs and transient spectroscopic signatures of young stars like β-Pic provide growing evidence that extra solar planetesimals can attain extreme orbital eccentricities and fall into their parent stars. Aims: We aim to develop a general, implementable, semi-analytical theory of secular eccentricity excitation of small bodies (planetesimals) in mean motion resonances with an eccentric planet valid for arbitrary values of the eccentricities and including the short-range force due to General Relativity. Methods: Our semi-analytic model for the restricted planar three-body problem does not make use of series expansion and therefore is valid for any eccentricity value and semi-major axis ratio. The model is based on the application of the adiabatic principle, which is valid when the precession period of the longitude of pericentre of the planetesimal is much longer than the libration period in the mean motion resonance. In resonances of order larger than 1 this is true except for vanishingly small eccentricities. We provide prospective users with a Mathematica notebook with implementation of the model allowing direct use. Results: We confirm that the 4:1 mean motion resonance with a moderately eccentric (e' ≲ 0.1) planet is the most powerful one to lift the eccentricity of planetesimals from nearly circular orbits to star-grazing ones. However, if the planet is too eccentric, we find that this resonance is unable to pump the planetesimal's eccentricity to a very high value. The inclusion of the General Relativity effect imposes a condition on the mass of the planet to drive the planetesimals into star-grazing orbits. For a planetesimal at 1 AU around a solar mass star (or white dwarf), we find a threshold planetary mass of about 17 Earth masses. We finally derive an analytical formula for this critical mass. Conclusions: Planetesimals can easily fall into the central star

  13. Nonlinear Resonant Excitation of Fast Sausage Waves in Current-Carrying Coronal Loops

    Science.gov (United States)

    Mikhalyaev, B. B.; Bembitov, D. B.

    2014-11-01

    We consider a model of a coronal loop that is a cylindrical magnetic tube with two surface electric currents. Its principal sausage mode has no cut-off in the long-wavelength limit. For typical coronal conditions, the period of the mode is between one and a few minutes. The sausage mode of flaring loops could cause long-period pulsations observed in microwave and hard X-ray ranges. There are other examples of coronal oscillations: long-period pulsations of active-region quiet loops in the soft X-ray emission are observed. We assume that these can also be caused by sausage waves. The question arises of how the sausage waves are generated in quiet loops. We assume that they can be generated by torsional oscillations. This process can be described in the framework of the nonlinear three-wave interaction formalism. The periods of interacting torsional waves are similar to the periods of torsional oscillations observed in the solar atmosphere. The timescale of the sausage-wave excitation is not much longer than the periods of interacting waves, so that the sausage wave is excited before torsional waves are damped.

  14. Evidence for nucleon-resonance excitation in omega-meson photoproduction.

    Science.gov (United States)

    Ajaka, J; Assafiri, Y; Bouchigny, S; Didelez, J P; Fichen, L; Guidal, M; Hourany, E; Kouznetsov, V; Kunne, R; Mushkarenkov, A N; Nedorezov, V; Rudnev, N; Turinge, A; Zhao, Q

    2006-04-01

    The photoproduction of the omega meson has been studied at GRAAL from threshold up to a photon energy of 1.5 GeV. The differential cross sections and beam asymmetries have been measured precisely at all angles. The total cross section is also obtained. Systematic enhancements of the differential cross section at large angles and nonzero beam asymmetries at intermediate angles provide clear evidence for s- and u-channel resonant processes. The data are compared to the results of hadron and quark models.

  15. Excited states

    CERN Document Server

    Lim, Edward C

    1974-01-01

    Excited States, Volume I reviews radiationless transitions, phosphorescence microwave double resonance through optical spectra in molecular solids, dipole moments in excited states, luminescence of polar molecules, and the problem of interstate interaction in aromatic carbonyl compounds. The book discusses the molecular electronic radiationless transitions; the double resonance techniques and the relaxation mechanisms involving the lowest triplet state of aromatic compounds; as well as the optical spectra and relaxation in molecular solids. The text also describes dipole moments and polarizab

  16. Stimulated Emission Pumping by Two-Color Resonant Four-Wave Mixing: Rotational Characterization of Vibrationally Excited HCO

    Energy Technology Data Exchange (ETDEWEB)

    Radi, P.P.; Tulej, M.; Knopp, G.; Beaud, P.; Gerber, T.

    2004-03-01

    Stimulated emission pumping by applying two-color resonant four-wave mixing is used to measure rotationally resolved spectra of the HCO (0,0,0) B {sup 2}A' - (0,3,1) X {sup 2}A' transition. The formyl radical is produced by photodissociation of formaldehyde at 31710.8 cm{sup -1} under thermalized conditions in a low pressure cell. In contrast to the highly congested one-color spectrum of HCO at room temperature, the doubleresonance method yields well isolated transitions which are assigned unambiguously due to intermediate level labeling. 89 rotational transitions have been assigned and yield accurate rotational constants for the vibrationally excited (0,3,1) band of the electronic ground state X {sup 2}A' of HCO. The determined rotational constant A = 25.84{+-}0.01 cm-1 is considerably higher than that for the vibrationless ground state and reflects the structural change due to excitation of the bending mode of the formyl radical. (author)

  17. Excitation of internal m = 1 mode during application of resonant magnetic perturbations on J-TEXT tokamak

    Science.gov (United States)

    Li, Jianchao; Hu, Qiming; Ding, Yonghua; Zhang, Xiaoqing; Yu, Qingquan; Yang, Zhoujun; Chen, Zhipeng; Li, Da; Rao, Bo; Wang, Nengchao; Zhuang, Ge; the J-TEXT Team

    2017-08-01

    The excitation of internal m = 1 mode during application of resonant magnetic perturbations (RMPs) is observed on J-TEXT tokamak. It is found that the sawtooth oscillation disappears after RMPs penetration, and subsequently an internal m = 1 mode with a frequency around 2 kHz appears, were m and n are the poloidal and toroidal mode numbers, respectively. In addition, the internal m = 1 mode often coexists with a rotating m/n = 2/1 tearing mode, and its frequency increases by about 0.5 kHz when the 2/1 tearing mode is locked by RMPs. The bispectrum analysis proves that the m = 1 mode interacts with the rotating 2/1 tearing mode, which implies the mode coupling between these two modes. The frequency of m = 1 mode increases for higher electron density. These results reveal that, the internal m = 1 mode can be excited by RMPs and coexist with both locked and rotating 2/1 mode due to toroidal mode coupling.

  18. Waveguide slot-excited long racetrack electron cyclotron resonance plasma source for roll-to-roll (scanning) processing.

    Science.gov (United States)

    You, H-J

    2013-07-01

    We present a SLot-excited ANtenna (SLAN) long racetrack ECR plasma source that is utilized for roll-to-roll plasma processing such as thin film encapsulation of large-area OLED (organic light emitting diode) panel or modification of fabric surfaces. This source is designed to be long, and to operate under high density uniform plasma with sub-milli-torr pressures. The above features are accomplished by a slot-excited long racetrack resonator with a toroidal geometry of magnetic field ECR configuration, and reinforced microwave electric distributions along the central region of plasma chamber. Also, a new feature has been added to the source. This is to employ a tail plunger, which allows the microwave electric field and the uniformity of the plasma profile to be easily adjustable. We have successfully generated Ar plasmas operating with the microwave power of 0.5-3 kW in the pressure range of 0.2-10 mTorr. The plasma is uniform (racetrack-SLAN source.

  19. Advances in high-resolution nuclear magnetic resonance methods in inhomogeneous magnetic fields using intermolecular multiple quantum coherences

    Institute of Scientific and Technical Information of China (English)

    2009-01-01

    Strong and extremely homogeneous static magnetic field is usually required for high-resolution nu-clear magnetic resonance (NMR). However, in the cases of in vivo and so on, the magnetic field inho-mogeneity owing to magnetic susceptibility variation in samples is unavoidable and hard to eliminate by conventional methods such as shimming. Recently, intermolecular multiple quantum coherences (iMQCs) have been employed to eliminate inhomogeneous broadening and obtain high-resolution NMR spectra, especially for in vivo samples. Compared to other high-resolution NMR methods, iMQC method exhibits its unique feature and advantage. It simultaneously holds information of chemical shifts, multiplet structures, coupling constants, and relative peak areas. All the information is often used to analyze and characterize molecular structures in conventional one-dimensional NMR spec-troscopy. In this work, recent technical developments including our results in this field are summarized; the high-resolution mechanism is analyzed and comparison with other methods based on interactions between spins is made; comments on the current situation and outlook on the research directions are also made.

  20. Coupled cavity QED for coherent control of photon transmission (II): Slowing light in coupled resonator waveguide doped with $\\Lambda $ Atoms

    CERN Document Server

    Zhou, L; Sun, C P; Lu, Jing; Zhou, Lan

    2006-01-01

    In the first paper of our series of articles on photon transmission in the coupled resonator optical waveguide (CROW), we used the two time Green function approach to study the physical mechanism for the coherent control by doping two-level atoms. In present paper, we propose and study a hybrid mechanism for photon transmission in the CROW by incorporating the electromagnetically induced transparency (EIT) effect in the doping artificial atoms and the band structure of the CROW. Here, the configuration setup of system, similar to that in the first paper, consists of a CROW with homogeneous couplings and the artificial atoms with $\\Lambda$-type three levels doped in each cavity. Unlike the stimulated Raman process used in the first paper to reduce the three level systems into the two level ones, the roles of three levels are completely considered based on a kind of mean field approach where the collection of three-level atoms collectively behave as two-mode spin waves. Then the total system is reduced into an ...

  1. A Compact Dielectric Resonator Antenna Excited by a Planar Monopole Patch for Wideband Applications

    Directory of Open Access Journals (Sweden)

    Xuping Li

    2016-01-01

    Full Text Available A compact dielectric resonator antenna (DRA suitable for wideband applications is presented in this paper. The proposed antenna is mainly composed by a notched cylindrical dielectric resonator (DR coated with a metal surface on the top and a finite ground plane where the presented DR is placed. This antenna is very simple in structure and has a very low overall height of 0.14λmin at its lowest operation frequency. A comprehensive parametric study is carried out based on Ansoft HFSS to optimize the bandwidth. The proposed antenna has been successfully simulated, optimized, fabricated, and measured. The measurement results demonstrate that the proposed design produces an impedance bandwidth of more than 75%, ranging from 2.9 GHz to 6.7 GHz for the reflection coefficient less than −10 dB. In particular, consistent broadside radiation patterns, stable gain, and high radiation efficiency are also obtained within the operation frequency band.

  2. Eccentricity Excitation and Apsidal Resonance Capture in the Planetary System Upsilon Andromedae

    CERN Document Server

    Chiang, E I

    2002-01-01

    The orbits of the outer two known planets orbiting Upsilon Andromedae are remarkably eccentric. Planet C possesses an orbital eccentricity of e1 = 0.253. For the more distant planet D, e2 = 0.308. Previous dynamical analyses strongly suggest that the two orbits are nearly co-planar and are trapped in an apsidal resonance in which the difference between their longitudes of periastron undergoes a bounded oscillation about 0 degrees. Here we elucidate the origin of these large eccentricities and of the apsidal alignment. Resonant interactions between a remnant circumstellar disk of gas lying exterior to the orbits of both planets can smoothly grow e2. Secular interactions between planets D and C can siphon off the eccentricity of the former to grow that of the latter. Externally amplifying e2 during the phase of the apsidal oscillation when e2/e1 is smallest drives the oscillation amplitude towards zero. Thus, the substantial eccentricity of planet C and the locking of orbital apsides are both consequences of ex...

  3. Ejected-electron spectroscopy of autoionizing resonances of helium excited by fast-electron impact

    Science.gov (United States)

    Zhang, Zhe; Shan, Xu; Wang, Enliang; Chen, Xiangjun

    2012-06-01

    The autoionizing resonances (2s2)1S, (2p2)1D, and (2s2p)1P of helium have been investigated employing ejected-electron spectroscopy by fast-electron impact at incident energies of 250-2000 eV and ejected angles of 26°-116°. Shore parameters of the line shapes for these three resonances have been obtained in such high incident energy regime except at 250 eV. Distinct discrepancies between the present results at 250 eV and those of McDonald and Crowe at 200 eV [D. G. McDonald and A. Crowe, J. Phys. BJPAMA40953-407510.1088/0953-4075/25/9/018 25, 2129 (1992); D. G. McDonald and A. Crowe, J. Phys. BJPAMA40953-407510.1088/0953-4075/25/20/024 25, 4313 (1992)] and Sise at 250 eV [O. Sise, M. Dogan, I. Okur, and A. Crowe, Phys. Rev. APLRAAN1050-294710.1103/PhysRevA.84.022705 84, 022705 (2011)], especially for 1D and 1P states, are also observed.

  4. Resonant circuit which provides dual frequency excitation for rapid cycling of an electromagnet

    Science.gov (United States)

    Praeg, Walter F.

    1984-01-01

    Disclosed is a ring magnet control circuit that permits synchrotron repetition rates much higher than the frequency of the cosinusoidal guide field of the ring magnet during particle acceleration. the control circuit generates cosinusoidal excitation currents of different frequencies in the half waves. During radio frequency acceleration of the particles in the synchrotron, the control circuit operates with a lower frequency cosine wave and thereafter the electromagnets are reset with a higher frequency half cosine wave. Flat-bottom and flat-top wave shaping circuits maintain the magnetic guide field in a relatively time-invariant mode during times when the particles are being injected into the ring magnets and when the particles are being ejected from the ring magnets.

  5. Pulsed excitation dynamics of an optomechanical crystal resonator near its quantum ground-state of motion

    CERN Document Server

    Meenehan, Sean M; MacCabe, Gregory S; Marsili, Francesco; Shaw, Matthew D; Painter, Oskar

    2015-01-01

    Using pulsed optical excitation and read-out along with single phonon counting techniques, we measure the transient back-action, heating, and damping dynamics of a nanoscale silicon optomechanical crystal cavity mounted in a dilution refrigerator at a base temperature of 11mK. In addition to observing a slow (~740ns) turn-on time for the optical-absorption-induced hot phonon bath, we measure for the 5.6GHz `breathing' acoustic mode of the cavity an initial phonon occupancy as low as 0.021 +- 0.007 (mode temperature = 70mK) and an intrinsic mechanical decay rate of 328 +- 14 Hz (mechanical Q-factor = 1.7x10^7). These measurements demonstrate the feasibility of using short pulsed measurements for a variety of quantum optomechanical applications despite the presence of steady-state optical heating.

  6. Effect of the coherent cancellation of the two-photon resonance on the generation of vacuum ultraviolet light by two-photon reasonantly enhanced four-wave mixing

    Energy Technology Data Exchange (ETDEWEB)

    Payne, M.G.; Garrett, W.R.; Judish, J.P.; Wunderlich, R.

    1988-11-01

    Many of the most impressive demonstrations of the efficient generation of vacuum ultraviolet (VUV) light have made use of two- photon resonantly enhanced four-wave mixing to generate light at ..omega../sub VUV/ = 2..omega../sub L1/ +- ..omega../sub L2/. The two-photon resonance state is coupled to the ground state both by two photons from the first laser, or by a photon from the second laser and one from the generated VUV beam. We show here that these two coherent pathways destructively interfere once the second laser is made sufficiently intense, thereby leading to an important limiting effect on the achievable conversion efficiency. 4 refs.

  7. Principal Resonance of Parametrically Excited Moving Viscoelastic Belts with Geometrical Nonlinearity

    Institute of Scientific and Technical Information of China (English)

    侯之超; 祖武争

    2004-01-01

    Nonlinear dynamic analysis is performed on moving belts subjected to geometric nonlinearity and initial tension fluctuation.To incorporate more accurately the damping mechanism of belt material, linear viscoelastic models are adopted in a unified form of differential operators.To circumvent high-order differential vibration equation of time-varying coefficients and with gyroscopic and nonlinear terms, where analytical solution is almost impossible, a systematic approach is presented by reforming the motion equation and directly using the method of multiple scales.To exemplify the procedure, the solutions at principal resonance are obtained and their stability conditions are derived for employing a Kelvin-Voigt model to reflect the property of the belt material.The solutions and stability conditions successfully reduce to those for using Kelvin model and elastic model, which validate the present approaches.Numerical simulations highlight the effects of tension fluctuations and translating speeds on the stability of the belt vibration.

  8. A Practical Control Strategy for the Maglev Self-Excited Resonance Suppression

    Directory of Open Access Journals (Sweden)

    Jinhui Li

    2016-01-01

    Full Text Available This paper addresses the control strategy for the suppression of maglev vehicle-bridge interaction resonance, which worsens the ride comfort of vehicle and degrades the safety of the bridge. Firstly, a minimum model containing a flexible bridge and ten levitation units is presented. Based on the minimum model, we pointed out that magnetic flux feedback instead of the traditional current feedback is capable of simplifying the block diagram of the interaction system. Furthermore, considering the uncertainty of the bridge’s modal frequency, the stability of the interaction system is explored according to an improved root-locus technique. Motivated by the positive effects of the mechanical damping of bridges and the feedback channels’ difference between the levitation subsystem and the bridge subsystem, the increment of electrical damping by the additional feedback of vertical velocity of bridge is proposed and several related implementation issues are addressed. Finally, the numerical and experimental results illustrating the stability improvement are provided.

  9. Nanotubular J-aggregates and quantum dots coupled for efficient resonance excitation energy transfer.

    Science.gov (United States)

    Qiao, Yan; Polzer, Frank; Kirmse, Holm; Steeg, Egon; Kühn, Sergei; Friede, Sebastian; Kirstein, Stefan; Rabe, Jürgen P

    2015-02-24

    Resonant coupling between distinct excitons in organic supramolecular assemblies and inorganic semiconductors is supposed to offer an approach to optoelectronic devices. Here, we report on colloidal nanohybrids consisting of self-assembled tubular J-aggregates decorated with semiconductor quantum dots (QDs) via electrostatic self-assembly. The role of QDs in the energy transfer process can be switched from a donor to an acceptor by tuning its size and thereby the excitonic transition energy while keeping the chemistry unaltered. QDs are located within a close distance (energy transfer coupling, which is around 92% in the case of energy transfer from the QD donor to the J-aggregate acceptor and approximately 20% in the reverse case. This system provides a model of an organic-inorganic light-harvesting complex using methods of self-assembly in aqueous solution, and it highlights a route toward hierarchical synthesis of structurally well-defined supramolecular objects with advanced functionality.

  10. X-Ray Emission Spectrometer Design with Single-Shot Pump-Probe and Resonant Excitation Capabilities

    Energy Technology Data Exchange (ETDEWEB)

    Spoth, Katherine; /SUNY, Buffalo /SLAC

    2012-08-28

    Core-level spectroscopy in the soft X-ray regime is a powerful tool for the study of chemical bonding processes. The ultrafast, ultrabright X-ray pulses generated by the Linac Coherent Light Source (LCLS) allow these reactions to be studied in greater detail than ever before. In this study, we investigated a conceptual design of a spectrometer for the LCLS with imaging in the non-dispersive direction. This would allow single-shot collection of X-ray emission spectroscopy (XES) measurements with varying laser pump X-ray probe delay or a variation of incoming X-ray energy over the illuminated area of the sample. Ray-tracing simulations were used to demonstrate how the components of the spectrometer affect its performance, allowing a determination of the optimal final design. These simulations showed that the spectrometer's non-dispersive focusing is extremely sensitive to the size of the sample footprint; the spectrometer is not able to image a footprint width larger than one millimeter with the required resolution. This is compatible with a single shot scheme that maps out the laser pump X-ray probe delay in the non-dispersive direction as well as resonant XES applications at normal incidence. However, the current capabilities of the Soft X-Ray (SXR) beamline at the LCLS do not produce the required energy range in a small enough sample footprint, hindering the single shot resonant XES application at SXR for chemical dynamics studies at surfaces. If an upgraded or future beamline at LCLS is developed with lower monochromator energy dispersion the width can be made small enough at the required energy range to be imaged by this spectrometer design.

  11. Calculation of vibrational excitation cross-sections in resonant electron-molecule scattering using the time-dependent wave packet (TDWP) approach with application to the 2 CO- shape resonance

    Indian Academy of Sciences (India)

    Raman Kumar Singh; Manabendra Sarma; Ankit Jain; Satrajit Adhikari; Manoj K Mishra

    2007-09-01

    Results from application of a new implementation of the time-dependent wave packet (TDWP) approach to the calculation of vibrational excitation cross-sections in resonant e-CO scattering are presented to examine its applicability in the treatment of e-molecule resonances. The results show that the SCF level local complex potential (LCP) in conjunction with the TDWP approach can reproduce experimental features quite satisfactorily.

  12. On the excited-state multi-dimensionality in cyanines

    Science.gov (United States)

    Dietzek, Benjamin; Brüggemann, Ben; Persson, Petter; Yartsev, Arkady

    2008-03-01

    Vibrational coherences in a photoexcited cyanine dye are preserved for the time-scale of diffusive torsional motion to the bottom of the excited-state potential. The coherently excited modes are virtually unaffected by solvent friction and thus distinct from the bond-twisting motion, which is strongly coupled to the surrounding solvent. We correlate the modes apparent in the resonance Raman and the four-wave mixing signal of 1,1'-diethyl-2,2'-cyanine with the understanding of optimal control of isomerization. In turn, the experimental results illustrate that optimal control might be used to obtain vibrational information complementary to conventional spectroscopic data.

  13. Effects of spontaneously induced coherence on absorption of a ladder-type atom

    Institute of Scientific and Technical Information of China (English)

    Ma Hong-Mei; Gong Shang-Qing; Sun Zhen-Rong; Li Ru-Xin; Xu Zhi-Zhan

    2006-01-01

    This paper investigates the effects of spontaneously induced coherence on absorption properties in a nearly equispaced three-level ladder-type system driven by two coherent fields. It find that the absorption properties of this system with the probe field applied on the lower transition can be significantly modified if this coherence is optimized. In the case of small spontaneous decay rate in the upper excited state, it finds that such coherence does not destroy the electromagnetically induced transparency (EIT). Nevertheless, the absorption peak on both sides of zero detuning and the linewidth of absorption line become larger and narrower than those in the case corresponding to the effects of spontaneously induced coherence; while in the case of large decay rate, it finds that, instead of EIT with low resonant absorption, a sharp absorption peak at resonance appears. That is, electromagnetically induced absorption in the nearly equispaced ladder-type system can occur due to such coherent effects.

  14. Effect of a resonant excitation on the evolution of the beam emittance and halo population

    CERN Document Server

    Fitterer, Miriam; Valishev, Alexander; Bruce, Roderik; Papadopoulou, Parthena Stefania; Papotti, Giulia; Pellegrini, Dario; Redaelli, Stefano; Trad, Georges; Valuch, Daniel; Valentino, Gianluca; Wagner, Joschka; Xu, Chen; CERN. Geneva. ATS Department

    2017-01-01

    Collimation with hollow electron beams or lenses (HEL) is currently one of the most promising concepts for active halo control in HL-LHC. In previous studies it has been shown that the halo can be efficiently removed with a hollow electron lens. Equally important as an efficient removal of the halo, is to demonstrate that the core stays unperturbed. In the case of an ideal hollow electron lens without bends, the field at the location of the beam core vanishes and the core remains unperturbed. In reality, the field at the beam core does not vanish entirely due to imperfections in the electron beam profile and the electron lens bends necessary to guide the electron in and out of the proton aperture. In particular, in the case of a pulsed operation of the electron lens the non-vanishing residual field induces noise on the proton beam. To identify the most sensitive pulsing patterns for the resonant mode and derive tolerances on the profile imperfections, a first MD was carried out of which the first results...

  15. Four-dimensional coherent electronic Raman spectroscopy

    Science.gov (United States)

    Harel, Elad

    2017-04-01

    The correlations between different quantum-mechanical degrees of freedom of molecular species dictate their chemical and physical properties. Generally, these correlations are reflected in the optical response of the system but in low-order or low-dimensionality measurement the signals are highly averaged. Here, we describe a novel four-dimensional coherent spectroscopic method that directly correlates within and between the manifold of electronic and vibrational states. The optical response theory is developed in terms of both resonant and non-resonant field-matter interactions. Using resonance to select coherences on specific electronic states creates opportunities to directly distinguish coherent dynamics on the ground and electronically excited potentials. Critically, this method is free from lower-order signals that have plagued other electronically non-resonant vibrational spectroscopies. The theory presented here compliments recent work on the experimental demonstration of the 4D spectroscopic method described. We highlight specific means by which non-trivial effects such as anharmonicity (diagonal and off-diagonal), mode-specific vibronic coupling, and curvature of the excited states manifest in different projections of the 4D spectrum.

  16. Resonant excitation of precursor molecules in improving the particle crystallinity, growth rate and optical limiting performance of carbon nano-onions

    Energy Technology Data Exchange (ETDEWEB)

    Gao, Y; Zhou, Y S; Park, J B; Wang, H; He, X N; Lu, Y F [Department of Electrical Engineering, University of Nebraska-Lincoln, Lincoln, NE 68588-0511 (United States); Luo, H F; Jiang, L, E-mail: ylu2@unl.edu [Department of Mechanical and Automation Engineering, Beijing Institute of Technology, Beijing 10008 (China)

    2011-04-22

    A catalyst-free and highly efficient synthetic method for growing carbon nano-onions (CNOs) in open air has been developed through the laser resonant excitation of a precursor molecule, ethylene, in a combustion process. Highly concentric CNO particles with improved crystallinity were obtained at a laser wavelength of 10.532 {mu}m through the resonant excitation of the CH{sub 2} wagging mode of the ethylene molecules. A higher growth rate up to 2.1 g h{sup -1} was obtained, compared with that without a laser (1.3 g h{sup -1}). Formation of the CNOs with ordered graphitic shells is ascribed to the decomposition of polycyclic aromatic hydrocarbons (PAHs) into C{sub 2} species. The optical limiting performances of the CNOs grown by the combustion processes were investigated. CNOs grown at 10.532 {mu}m laser excitation demonstrated improved optical limiting properties due to the improved crystallinity.

  17. Waveguide coupled resonance fluorescence from on-chip quantum emitter.

    Science.gov (United States)

    Makhonin, Maxim N; Dixon, James E; Coles, Rikki J; Royall, Ben; Luxmoore, Isaac J; Clarke, Edmund; Hugues, Maxime; Skolnick, Maurice S; Fox, A Mark

    2014-12-10

    Resonantly driven quantum emitters offer a very promising route to obtain highly coherent sources of single photons required for applications in quantum information processing (QIP). Realizing this for on-chip scalable devices would be important for scientific advances and practical applications in the field of integrated quantum optics. Here we report on-chip quantum dot (QD) resonance fluorescence (RF) efficiently coupled into a single-mode waveguide, a key component of a photonic integrated circuit, with a negligible resonant laser background and show that the QD coherence is enhanced by more than a factor of 4 compared to off-resonant excitation. Single-photon behavior is confirmed under resonant excitation, and fast fluctuating charge dynamics are revealed in autocorrelation g((2)) measurements. The potential for triggered operation is verified in pulsed RF. These results pave the way to a novel class of integrated quantum-optical devices for on-chip quantum information processing with embedded resonantly driven quantum emitters.

  18. Neutral current coherent pion production

    CERN Document Server

    Alvarez-Ruso, L; Vacas, M J Vicente

    2007-01-01

    We investigate the neutrino induced coherent pion production reaction at low and intermediate energies. The model includes pion, nucleon and Delta(1232) resonance as the relevant hadronic degrees of freedom. Nuclear medium effects on the production mechanisms and pion distortion are taken into account. We obtain that the dominance of the Delta excitation holds due to large cancellations among the background contributions. We consider two sets of vector and axial-vector N-Delta transition form-factors, evidencing the strong sensitivity of the results to the axial coupling C5A(0). The differences between neutrino and antineutrino cross sections, emerging from interference terms, are also discussed.

  19. Structural dynamics of phenylisothiocyanate in the light-absorbing excited states: Resonance Raman and complete active space self-consistent field calculation study

    Energy Technology Data Exchange (ETDEWEB)

    Ouyang, Bing, E-mail: ouyangbing.zj@foxmail.com; Xue, Jia-Dan, E-mail: jenniexue@126.com; Zheng, Xuming, E-mail: zhengxuming126@126.com, E-mail: zxm@zstu.edu.cn, E-mail: fangwh@dnu.edu.cn [Department of Chemistry, Zhejiang Sci-Tech University, Hangzhou 310018 (China); Fang, Wei-Hai, E-mail: zxm@zstu.edu.cn, E-mail: fangwh@dnu.edu.cn, E-mail: fangwh@dnu.edu.cn [Department of Chemistry, Beijing Normal University, Beijing 100875 (China)

    2014-05-21

    The excited state structural dynamics of phenyl isothiocyanate (PITC) after excitation to the light absorbing S{sub 2}(A′), S{sub 6}(A′), and S{sub 7}(A′) excited states were studied by using the resonance Raman spectroscopy and complete active space self-consistent field method calculations. The UV absorption bands of PITC were assigned. The vibrational assignments were done on the basis of the Fourier transform (FT)-Raman and FT-infrared measurements, the density-functional theory computations, and the normal mode analysis. The A-, B-, and C-bands resonance Raman spectra in cyclohexane, acetonitrile, and methanol solvents were, respectively, obtained at 299.1, 282.4, 266.0, 252.7, 228.7, 217.8, and 208.8 nm excitation wavelengths to probe the corresponding structural dynamics of PITC. The results indicated that the structural dynamics in the S{sub 2}(A′), S{sub 6}(A′), and S{sub 7}(A′) excited states were very different. The conical intersection point CI(S{sub 2}/S{sub 1}) were predicted to play important role in the low-lying excited state decay dynamics. Two major decay channels were predicted for PITC upon excitation to the S{sub 2}(A′) state: the radiative S{sub 2,min} → S{sub 0} transition and the nonradiative S{sub 2} → S{sub 1} internal conversion via CI(S{sub 2}/S{sub 1}). The differences in the decay dynamics between methyl isothiocyanate and PITC in the first light absorbing excited state were discussed. The role of the intersystem crossing point ISC(S{sub 1}/T{sub 1}) in the excited state decay dynamics of PITC is evaluated.

  20. Structural dynamics of phenylisothiocyanate in the light-absorbing excited states: resonance Raman and complete active space self-consistent field calculation study.

    Science.gov (United States)

    Ouyang, Bing; Xue, Jia-Dan; Zheng, Xuming; Fang, Wei-Hai

    2014-05-21

    The excited state structural dynamics of phenyl isothiocyanate (PITC) after excitation to the light absorbing S2(A'), S6(A'), and S7(A') excited states were studied by using the resonance Raman spectroscopy and complete active space self-consistent field method calculations. The UV absorption bands of PITC were assigned. The vibrational assignments were done on the basis of the Fourier transform (FT)-Raman and FT-infrared measurements, the density-functional theory computations, and the normal mode analysis. The A-, B-, and C-bands resonance Raman spectra in cyclohexane, acetonitrile, and methanol solvents were, respectively, obtained at 299.1, 282.4, 266.0, 252.7, 228.7, 217.8, and 208.8 nm excitation wavelengths to probe the corresponding structural dynamics of PITC. The results indicated that the structural dynamics in the S2(A'), S6(A'), and S7(A') excited states were very different. The conical intersection point CI(S2/S1) were predicted to play important role in the low-lying excited state decay dynamics. Two major decay channels were predicted for PITC upon excitation to the S2(A') state: the radiative S(2,min) → S0 transition and the nonradiative S2 → S1 internal conversion via CI(S2/S1). The differences in the decay dynamics between methyl isothiocyanate and PITC in the first light absorbing excited state were discussed. The role of the intersystem crossing point ISC(S1/T1) in the excited state decay dynamics of PITC is evaluated.