WorldWideScience

Sample records for optically stimulated luminescence

  1. Optically stimulated luminescence in retrospective dosimetry

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.; Murray, A.S.

    2002-01-01

    Since the beginning of the 1990s the exploration of optically stimulated luminescence (OSL) in retrospective accident dosimetry has driven an intensive investigation and development programme at Riso into measurement facilities and techniques. This paper reviews some of the outcomes of this progr......Since the beginning of the 1990s the exploration of optically stimulated luminescence (OSL) in retrospective accident dosimetry has driven an intensive investigation and development programme at Riso into measurement facilities and techniques. This paper reviews some of the outcomes...

  2. Optically stimulated luminescence dating of rock surfaces

    DEFF Research Database (Denmark)

    Sohbati, Reza

    There are many examples of rock surfaces, rock art and stone structures whose ages are of great importance to the understanding of various phenomena in geology, climatology and archaeology. Optically stimulated luminescence (OSL) dating is a well-established chronological tool that has successfully...... of rock surfaces is successfully tested by application to two different quartz-rich rock types (sandstone and quartzite). Together with the measurement of infrared stimulated luminescence (IRSL) signals as a function of depth into the surface of different granites it is clear that both OSL and IRSL can....... Based on the studies of residual luminescence as a function of depth into a rock surface discussed above, a model is developed that relates this increase in residual luminescence to the exposure time. The model is then further developed using the quartz OSL signal from buried quartzite cobbles...

  3. Optically stimulated luminescence techniques in retrospective dosimetry

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.; Murray, A.S.

    2001-01-01

    Optically stimulated luminescence signals from natural quartz and feldspar are now used routinely in dating geological and archaeological materials. More recently they have also been employed in accident dosimetry, i.e. the retrospective assessment of doses received as a result of a nuclear...

  4. Optically stimulated luminescence dating of young sediments

    DEFF Research Database (Denmark)

    Madsen, A.T.; Murray, A.S.

    2009-01-01

    Optically stimulated luminescence (OSL) dating of young (< 1000 years) sediments is used increasingly in a wide variety of late-Holocene studies as a mean of establishing contemporary sedimentation rates or the timing of sediment deposition. This paper provides a summary of the basic principles o...

  5. Plasmon-enhanced optically stimulated luminescence

    Energy Technology Data Exchange (ETDEWEB)

    Guidelli, E. J.; Baffa, O. [Universidade de Sao Paulo, Faculdade de Filosofia, Ciencias e Letras de Ribeirao Preto, Departamento de Fisica, Av. Bandeirantes 3900, 14040-901 Ribeirao Preto, Sao Paulo (Brazil); Ramos, A. P., E-mail: ederguidelli@gmail.com [Universidade de Sao Paulo, Faculdade de Filosofia, Ciencias e Letras de Ribeirao Preto, Departamento de Quimica, Av. Bandeirantes 3900, 14040-901 Ribeirao Preto, Sao Paulo (Brazil)

    2015-10-15

    Full text: Optically Stimulated Luminescence dosimeters (OSLD) have been largely used for personal, medical, and industrial radiation dosimetry. Developing highly sensitive and small-sized radiation detectors and dosimeters is essential for improving spatial resolution and consequently diagnosis quality and treatment efficacy in the case of applications in radiodiagnosis and radiation therapy, for instance. Conventional methods to improve the OSLD sensitivity consist of doping and co-doping the host materials with atoms of other elements, thereby increasing the amount of trapping and/or luminescent centers. Our group is researching on the use of the plasmon properties of noble metal nanoparticles to increase OSL intensity. Upon incidence of a light beam with appropriate resonant wavelengths, the oscillation of the free electrons at the nanoparticle surface originates the Localized Surface Plasmons (LSP) and the consequent plasmon resonance band. The interaction between the LSP and the surrounding luminescent material leads to new optical properties largely employed for enhancing several luminescent processes. Here we will show our results regarding the use of LSP to increase OSLD sensitivity. The interaction between the traps/luminescent centers and the plasmons depends on the distance between them, on the plasmon resonance band intensity and position, as well as on the surrounding medium. Therefore, the plasmon-enhanced luminescence is a promising tool to develop more sensitive and miniaturized OSLD. (Author)

  6. Thermo-optical properties of optically stimulated luminescence in feldspars

    DEFF Research Database (Denmark)

    Poolton, N.R.J.; Bøtter-Jensen, L.; Johnsen, O.

    1995-01-01

    Optically stimulated luminescence processes in feldspars are subject to competing thermal enhancement and quenching processes: this article describes the thermal enhancement effects for orthoclase, albite and plagioclase feldspars. It is demonstrated that certain lattice vibrational modes can...

  7. Optically stimulated luminescence dating of rock surfaces

    DEFF Research Database (Denmark)

    Sohbati, Reza

    There are many examples of rock surfaces, rock art and stone structures whose ages are of great importance to the understanding of various phenomena in geology, climatology and archaeology. Optically stimulated luminescence (OSL) dating is a well-established chronological tool that has successfully...... determined the depositional age of a wide variety of fine-grained sediments, from several years to several hundred thousands of years. However, there is no routine OSL dating method applicable to larger clasts such as cobbles, boulders and other rock surfaces. Here the application of quartz OSL to the dating...... of rock surfaces is successfully tested by application to two different quartz-rich rock types (sandstone and quartzite). Together with the measurement of infrared stimulated luminescence (IRSL) signals as a function of depth into the surface of different granites it is clear that both OSL and IRSL can...

  8. Optically Stimulated Luminescence Fundamentals and Applications

    CERN Document Server

    McKeever, Stephen

    2011-01-01

    The book discusses advanced modern applications of optically stimulated luminescence including the appropriate fundamentals of the process. It features major chapters on the use of OSL in space radiation dosimetry, medical physics, personnel dosimetry, security, solid-state physics and other related applications. In each case, the underlying theory is discussed on an as-needed basis for a complete understanding of the phenomena, but with an emphasis of the practical applications of the technique. After an introductory chapter, Chapters 2 to 6 cover basic theory and practical aspects, personal

  9. Optically stimulated luminescence dating at Rose Cottage Cave

    CSIR Research Space (South Africa)

    Pienaar, M

    2008-01-01

    Full Text Available Six Optically stimulated luminescence (OSL) dates are compared with stratigraphically associated C-14 dates from Rose Cottage Cave. The OSL dates overlap the accepted C-14 chronology except for one sample that overestimates the expected age...

  10. Towards multi-exponential analysis in optically stimulated luminescence

    DEFF Research Database (Denmark)

    Ankjærgaard, Christina; Jain, Mayank; Hansen, Per Christian

    2010-01-01

    Optically stimulated luminescence (OSL) data from quartz can follow different mathematical forms depending on the stimulation mode. These data can be described in terms of different multi-exponential models and can be numerically fitted using several well-known methods. Here we make a comparative...

  11. Optically stimulated luminescence dosimetry using natural and synthetic materials

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.; McKeever, S.W.S.

    1996-01-01

    The application of optically stimulated luminescence (OSL) for use in radiation dosimetry is reviewed. A broad description is given of OSL techniques developed at Riso National Laboratory and at Oklahoma State University, and recent collaborative investigations on the properties of a variety...

  12. Optically stimulated luminescence dosimetry using natural and synthetic materials

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.; McKeever, S.W.S.

    1996-01-01

    The application of optically stimulated luminescence (OSL) for use in radiation dosimetry is reviewed. A broad description is given of OSL techniques developed at Riso National Laboratory and at Oklahoma State University, and recent collaborative investigations on the properties of a variety of n......, and unseparated materials such as bricks and porcelain items....

  13. Modelling of optically stimulated luminescence of zircon : assessment of the suitability for dating

    NARCIS (Netherlands)

    Turkin, A.A.; Vainshtein, D.I.; Hartog, H.W. den

    2006-01-01

    The mineral zircon, ZrSiO4, is a candidate material for optical dating because it exhibits luminescence after exposure to natural radioactivity. The kinetic model of zircon thermally stimulated luminescence proposed before has been modified and used to investigate optically Stimulated luminescence (

  14. Thermoluminescence and optically stimulated luminescence properties of natural barytes.

    Science.gov (United States)

    Kitis, G; Kiyak, N G; Polymeris, G S

    2010-12-01

    Heavy, baryte-loaded, concrete is commonly used as radiation shielding material around high energy particle accelerators. Concrete samples received from a shielding block located at CERN cite contain many crystalline inclusions which were identified as barytes by X-ray diffraction analysis and separated by their color, classified as white, orange and green. Basic properties of thermoluminescence (TL) and optically stimulated luminescence (OSL) signals of these barytes samples such as thermal and optical stability, repeatability and mainly the linearity of both their luminescence responses were investigated as a function of beta dose. These results are also discussed regarding detailed investigation on the correlation between TL and OSL signals and their implications for retrospective dosimetry.

  15. Dosimetry based on thermally and optically stimulated luminescence

    Energy Technology Data Exchange (ETDEWEB)

    Agersnap Larsen, Niels

    1999-01-01

    Thermally Stimulated Luminescence (TL) and Optically Stimulated Luminescence (OSL) properties of quartz and {alpha}-Al{sub 2}O{sub 3} have been investigated. Anneling-induced OSL and TL sensitivity changes in quartz has been investigated by experiments and modelling. This study does not support a pre-dose effect to account for the observed annealing-induced sensitivity change. The experimental data indicates a more simple mechanism that involves alteration of the concentration of the defect centers. Results from modelling of removal or creation of defect centers comparing well with experimentally obtained data. Thermal quenching of luminescence for the main emission center, the F-center, in {alpha}-Al{sub 2}O{sub 3}:C has been investigated by analysing TL curves obtained at different heating rates. The thermal quenching dependence of luminescence is found to follow the classical Mott-Seitz expression. Basic investigations of OSL properties of {alpha}Al{sub 2}O{sub 3}:C, including: the thermal depth of the OSL traps, the temperature dependence of OSL, and the OSL stimulation spectra. Simultaneous measurements of TL and thermally stimulated conductivity (TSC) are presented for {gamma}-irradiated {alpha}Al{sub 2}O{sub 3}:C. Activation energy analysis of the data reveals a superposition of several first-order TL and TSC peaks caused by release of charge carriers from a distribution of trapping states. Furthermore a description of an experimental method developed to determine the sign of the thermally released charge carriers has been presented. (au) 8 tabs., 59 ills., 90 refs.

  16. Systematic development of new thermoluminescence and optically stimulated luminescence materials

    Energy Technology Data Exchange (ETDEWEB)

    Yukihara, E.G., E-mail: eduardo.yukihara@okstate.edu [Physics Department, 145 Physical Sciences II, Oklahoma State University, Stillwater, OK 74078 (United States); Milliken, E.D.; Oliveira, L.C. [Physics Department, 145 Physical Sciences II, Oklahoma State University, Stillwater, OK 74078 (United States); Orante-Barron, V.R. [Departamento de Investigacion en Polimeros y Materiales, Universidad de Sonora, Hermosillo, Sonora 83000, Mexico (Mexico); Jacobsohn, L.G. [Center for Optical Materials Science and Engineering Technologies (COMSET), and School of Materials Science and Engineering, Clemson University, Clemson, SC (United States); Blair, M.W. [Materials Science and Technology Division, Los Alamos National Laboratory, Los Alamos, NM 87545 (United States)

    2013-01-15

    This paper presents an overview of a systematic study to develop new thermoluminescence (TL) and optically stimulated luminescence (OSL) materials using solution combustion synthesis (SCS) for applications such as personal OSL dosimetry, 2D dose mapping, and temperature sensing. A discussion on the material requirements for these applications is included. We present X-ray diffraction (XRD) data on single phase materials obtained with SCS, as well as radioluminescence (RL), TL and OSL data of lanthanide-doped materials. The results demonstrate the possibility of producing TL and OSL materials with sensitivity similar to or approaching those of commercial TL and OSL materials used in dosimetry (e.g., LiF:Mg,Ti and Al{sub 2}O{sub 3}:C) using SCS. The results also show that the luminescence properties can be improved by Li co-doping and annealing. The presence of an atypical TL background and anomalous fading are discussed and deserve attention in future investigations. We hope that these preliminary results on the use of SCS for production of TL and OSL materials are helpful to guide future efforts towards the development of new luminescence materials for different applications. - Highlights: Black-Right-Pointing-Pointer TL and OSL material produced with sensitivity similar to commercial materials. Black-Right-Pointing-Pointer Luminescence properties improved by Li co-doping and annealing. Black-Right-Pointing-Pointer The presence of atypical TL background and anomalous fading observed.

  17. Protocols for Thermoluninescence and Optically Stimulated Luminescence Research at DOSAR

    Energy Technology Data Exchange (ETDEWEB)

    Bernal, SM

    2004-10-11

    The Life Sciences Division (LSD) of Oak Ridge National Laboratory (ORNL) has a long record of radiation dosimetry research at the Dosimetry Applications Research (DOSAR) facility complex. These facilities have been used by a broad segment of the research community to perform a variety of experiments in areas including, but not limited to, radiobiology, radiation dosimeter and instrumentation development and calibration, and materials testing in a variety of radiation environments. Collaborations with the University of Tennessee-Knoxville (UTK) have also led to important contributions in the area of archaeometry, particularly as it relates to the use of radiation dosimetry to date archaeological artifacts. This manual is to serve as the primary instruction and operation manual for dosimetric and archaeometric research at DOSAR involving thermoluminescence (TL) and optically stimulated luminescence (OSL). Its purpose is to (1) provide protocols for common practices associated with the research, (2) outline the relevant organizational structure, (3) identify the Quality Assurance plan, and (4) describe all the procedures, operations, and responsibilities for safe and proper operation of associated equipment. Each person who performs research at DOSAR using TL/OSL equipment is required to read the latest revision of this manual and be familiar with its contents, and to sign and date the manual's master copy indicating that the manual has been read and understood. The TL/OSL Experimenter is also required to sign the manual after each revision to signify that the changes are understood. Each individual is responsible for completely understanding the proper operation of the TL/OSL equipment used and for following the guidance contained within this manual. The instructions, protocols, and operating procedures in this manual do not replace, supersede, or alter the hazard mitigation controls identified in the Research Safety Summary (''Thermoluminescence/Optically

  18. Influence of crystal structure on the optically stimulated luminescence properties of feldspars

    DEFF Research Database (Denmark)

    Poolton, N.R.J.; Bøtter-Jensen, L.; Ypma, P.J.M.

    1994-01-01

    Work is presented showing that the crystal structure of feldspar plays an important role in determining the energy positions at which optically stimulated luminescence transitions can occur, their thermo-optical behavior, the transport properties of charge in the conduction and valence bands, and......, and the time decay characteristics of the luminescence. First-order calculations of these effects are presented, and comparison is made with experimental results.......Work is presented showing that the crystal structure of feldspar plays an important role in determining the energy positions at which optically stimulated luminescence transitions can occur, their thermo-optical behavior, the transport properties of charge in the conduction and valence bands...

  19. Modelling the thermal quenching mechanism in quartz based on time-resolved optically stimulated luminescence

    DEFF Research Database (Denmark)

    Pagonis, V.; Ankjærgaard, Christina; Murray, Andrew

    2010-01-01

    . As the temperature of the sample is increased, more electrons are removed from the excited state via the non-radiative pathway. This reduction in the number of available electrons leads to both a decrease of the intensity of the luminescence signal and to a simultaneous decrease of the luminescence lifetime. Several...... simulations are carried out of time-resolved optically stimulated luminescence (TR-OSL) experiments, in which the temperature dependence of luminescence lifetimes in quartz is studied as a function of the stimulation temperature. Good quantitative agreement is found between the simulation results and new...

  20. Pottery versus sediment: Optically stimulated luminescence dating of the Neolithic Vinča culture, Serbia

    DEFF Research Database (Denmark)

    Bate, Stephen; Stevens, Thomas; Buylaert, Jan-Pieter

    2017-01-01

    Optically stimulated luminescence (OSL) dating was applied to the Neolithic Vinča culture's type-site, Vinča Belo-Brdo, to establish best protocols for routine luminescence dating of similar Holocene sites, critical in understanding Neolithic to Chalcolithic cultural development. Equivalent dose ...

  1. Optical stimulated Luminescence Signal on Modern Fluvial Deposit in Taiwan

    Science.gov (United States)

    Chen, Y. G.; Wu, T. S.; Chen, Y. W.; Kuo, Y. T.

    2014-12-01

    The river terraces overlain by fluvial and debris-flow deposit are widely distributed in Taiwan due to its active tectonic situation. They are not only critical in reconstructing the river evolution, but also of importance in understanding neotectonics. However, the age estimation for the terraces has their own problems by C-14 as well as OSL (Optical Stimulated Luminescence) dating method. For C-14 method, the major problem is the difficulty in discovering the suitable samples, but for OSL method the zeroing effect of the sediments becomes the major barrier if quartz SAR (Single Aliquot Regenerative) procedure is applied. In order to test the residual dose from different drainage areas in Taiwan, modern deposits were collected from 13 main rivers and 3 samples for each from upper-stream to downstream. The apparent dose of modern fluvial deposit was defined as residual dose and believed to be able to give a hint for estimating the zeroing effect for river terraces. Quartz SAR OSL procedure on small aliquot was adopted for all samples in this study. Our results show the residual dose in western Taiwan strongly relies on the source from. If we further apply the mean value of smallest 5% on samples from modern debris flow deposits in upper-stream, the residual dose rise up as high as ~40Gy but lower down to ~15Gy for samples collected from river mouth estuary. It implies that there will be a large error when evaluating the age of debris deposit terrace by quartz SAR OSL procedure. However, if the modern river does not suffer from debris flow in upper-stream, the residual dose is ~5Gy in upper stream and only -0.7~2Gy to the lower steam estuary, which provide better chance to derive relatively reliable ages. We also find that the luminescence characteristics is different between the samples in western and eastern Taiwan respectively. The quartz grains from eastern Taiwan are much dimer than those of the western Taiwan. We may therefore face severe challenge to approach

  2. The temperature dependence of optically stimulated luminescence from α-Al2O3:C

    DEFF Research Database (Denmark)

    Markey, B.G.; McKeever, S.W.S.; Akselrod, M.S.

    1996-01-01

    The results of experimental measurements and computer simulations on optically stimulated luminescence (OSL) from alpha-Al2O3:C are described. The intensity of the OSL observed during illumination of irradiated specimens with visible light is temperature dependent. Optical stimulation is observed...

  3. Review of optically stimulated luminescence (OSL) instrumental developments for retrospective dosimetry

    DEFF Research Database (Denmark)

    Bøtter-Jensen, Lars; Thomsen, Kristina Jørkov; Jain, Mayank

    2010-01-01

    This review describes 40 years of experience gained at Risø National Laboratory in the development of facilities for irradiation, thermal/optical stimulation and luminescence signal detection. These facilities have mainly been used in luminescence dating and nuclear accident dosimetry. We focus e...... especially on methods for light stimulation and irradiation, and developments of new portable TL/OSL readers for determining doses directly in the field on both Earth and the planet Mars....

  4. Optimising the separation of quartz and feldspar optically stimulated luminescence using pulsed excitation

    DEFF Research Database (Denmark)

    Ankjærgaard, Christina; Jain, Mayank; Thomsen, Kristina Jørkov;

    2010-01-01

    In luminescence dating, the two most commonly used natural minerals, quartz and feldspar, are exposed to different dose rates in the natural environment, and so record different doses. The luminescence signals also have different stabilities. For accurate dosimetry, the signals from these two...... minerals must be separated, either by physical separation of the mineral grains, or by instrumental separation of the luminescence signals. The luminescence signals from quartz and feldspar have different luminescence lifetimes under pulsed optical stimulation. This difference in lifetime can be used...... to discriminate between the two signals from a mixed quartz-feldspar sample. The purpose of this study is to identify optimum measurement conditions for the best separation of quartz OSL from that of feldspar in a mixed sample using pulsed stimulation and time-resolved OSL. We integrate the signal from 5 μs after...

  5. The temperature dependence of optically stimulated luminescence from α-Al2O3:C

    DEFF Research Database (Denmark)

    Markey, B.G.; McKeever, S.W.S.; Akselrod, M.S.;

    1996-01-01

    The results of experimental measurements and computer simulations on optically stimulated luminescence (OSL) from alpha-Al2O3:C are described. The intensity of the OSL observed during illumination of irradiated specimens with visible light is temperature dependent. Optical stimulation is observed...... from the main dosimetric traps, and from deep traps. The temperature dependence appears to be due to the presence of shallow traps, with a possible additional contribution from thermally assisted optical excitation....

  6. Feldspar, Infrared Stimulated Luminescence

    DEFF Research Database (Denmark)

    Jain, Mayank

    2014-01-01

    This entry primarily concerns the characteristics and the origins of infrared-stimulated luminescence in feldspars.......This entry primarily concerns the characteristics and the origins of infrared-stimulated luminescence in feldspars....

  7. Surface exposure dating of non-terrestrial bodies using optically stimulated luminescence

    DEFF Research Database (Denmark)

    Sohbati, Reza; Jain, Mayank; Murray, A.S.

    2012-01-01

    We propose a new method for in situ surface exposure dating of non-terrestrial geomorphological features using optically stimulated luminescence (OSL); our approach is based on the progressive emptying of trapped charge with exposure to light at depth into a mineral surface. A complete model...

  8. Developments in optically stimulated luminescence techniques for dating and retrospective dosimetry

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.; Murray, A.S.

    1999-01-01

    Optically stimulated luminescence signals from natural quartz and feldspar are now used routinely in dating geological and archaeological materials. More recently they have also been employed in accident dosimetry, i.e. the retrospective assessment of doses received as a result of a nuclear accid...

  9. Optically stimulated luminescence response to Al2O3 to beta radiation

    DEFF Research Database (Denmark)

    Akselrod, A.; Akselrod, M.S.; Agersnap Larsen, N.

    1999-01-01

    High sensitivity dosemeters based on Al2O3:C have been prepared and tested for use as beta dosemeters using optically stimulated luminescence (OSL). Two types of sample were prepared and tested, namely unpolished thick, single crystal chips and thin powder layers on aluminium substrates...

  10. Surface exposure dating of non-terrestrial bodies using optically stimulated luminescence: A new method

    DEFF Research Database (Denmark)

    Sohbati, Reza; Jain, Mayank; Murray, Andrew

    2012-01-01

    We propose a new method for in situ surface exposure dating of non-terrestrial geomorphological features using optically stimulated luminescence (OSL); our approach is based on the progressive emptying of trapped charge with exposure to light at depth into a mineral surface. A complete model of t...

  11. Optically stimulated luminescence of natural NaCl mineral from Dead Sea exposed to gamma radiation

    Energy Technology Data Exchange (ETDEWEB)

    Roman L, J.; Cruz Z, E. [UNAM, Instituto de Ciencias Nucleares, Ciudad Universitaria, 04510 Ciudad de Mexico (Mexico); Pina L, Y. I. [UNAM, Facultad de Ciencias, Ciudad Universitaria, 04510 Ciudad de Mexico (Mexico); Marcazzo, J., E-mail: jesus.roman@nucleares.unam.mx [Instituto de Fisica Arroyo Seco - UNICEN, Pinto 399, 7000 Tandil (Argentina)

    2016-10-15

    Luminescence properties such as radioluminescence, thermoluminescence and optically stimulated luminescence have been studied on natural sodium chloride (NaCl) for dosimetric purposes in retrospective dosimetry (Timar-Gabor et al., 2013; Druzhyna et al., 2016). In this work, the optically stimulated luminescence (Cw-OSL) emissions of natural salt minerals, collected from Dead Sea in summer of 2015, were studied. The Cw-OSL dose response of natural salt was analyzed in the range between 0.2 and 10 Gy gamma dose of {sup 60}Co. Samples exposed at 3 Gy exhibited good repeatability with a variation coefficient of 4.6%. The thermal stability of the Cw-OSL response was analyzed to different temperatures from 50 up to 250 degrees Celsius using a heating rate of 5 degrees Celsius. The results showed that the natural Dead Sea salt minerals could be applied as natural dosimeter of gamma radiation. (Author)

  12. Further investigations into pulsed optically stimulated luminescence from feldspars using blue and green light

    DEFF Research Database (Denmark)

    Ankjærgaard, Christina; Jain, Mayank; Kalchgruber, R.

    2009-01-01

    The purpose of this paper is to investigate characteristics of luminescence signals resulting from pulsed optical stimulation of feldspars and thereby to understand the underlying processes giving rise to the signal. Fourteen different feldspar specimens were investigated using time...... suggests that the TR-OSL signal decay is governed by the recombination process and not by the excited state lifetime. Furthermore data from the TR-OSL signal dependence on stimulation time and preheat temperature suggest that the recombination process may not be a sum of exponentials, although the model......-resolved optically stimulated luminescence (TR-OSL), and these signals can be mathematically described as a sum of 4 exponential components (a, b, c, d). The slowest component, d, increases with the duration of the light pulse as expected from the exponential model. The stimulation temperature dependence experiment...

  13. Photoluminescence and Optically Stimulated Luminescence Studies of LiAlO2 and LiGaO2 Crystals

    Science.gov (United States)

    2015-03-26

    PHOTOLUMINESCENCE AND OPTICALLY STIMULATED LUMINESCENCE STUDIES OF LiAlO2 AND LiGaO2 CRYSTALS THESIS Ian P. Ferguson, Second Lieutenant, USAF AFIT...STIMULATED LUMINESCENCE STUDIES OF LiAlO2 AND LiGaO2 CRYSTALS THESIS Presented to the Faculty Department of Engineering Physics Graduate School of...FOR PUBLIC RELEASE; DISTRIBUTION UNLIMITED. AFIT-ENP-MS-15-M-106 PHOTOLUMINESCENCE AND OPTICALLY STIMULATED LUMINESCENCE STUDIES OF LiAlO2 AND LiGaO2

  14. Optically stimulated luminescence (OSL) as a chronometer for surface exposure dating

    DEFF Research Database (Denmark)

    Sohbati, Reza; Murray, Andrew S.; Chapot, Melissa S.

    2012-01-01

    We pioneer a technique of surface-exposure dating based upon the characteristic form of an optically stimulated luminescence (OSL) bleaching profile beneath a rock surface; this evolves as a function of depth and time. As a field illustration of this new method, the maximum age of a premier examp......, at decadal to millennial timescales or perhaps longer (depending on the environmental dose rate) even for material subsequently buried. This has considerable potential in many archeological, geological and geo-hazard applications....

  15. A high sensitivity optically stimulated luminescence scanning system for measurement of single sand-sized grains

    DEFF Research Database (Denmark)

    Duller, G.A.T.; Bøtter-Jensen, L.; Kohsiek, P.;

    1999-01-01

    An instrument has been designed for the routine analysis of the optically stimulated luminescence signal from single grains of sand. The system is capable of analysing over 3000 individual grains in a single measurement sequence, and the OSL signal from each grain can be read in less than 3 s....... The design principles are described, along with preliminary measurements that illustrate the operation of the system and its capabilities....

  16. Thermoluminescence and optically stimulated luminescence dating of bricks from the Thung Tuk archaeological site, Southern Thailand

    Directory of Open Access Journals (Sweden)

    Santi Pailoplee

    2016-12-01

    Full Text Available Thermoluminescence (TL and optically stimulated luminescence (OSL based dating were applied to ancient fired bricks to derive the chronology of the Thung Tuk archaeological site (TT, southern Thailand. In order to test the feasibility of brick dating, the inside and outside portions of the brick mass were dated separately. From the obtained results, the outside portion of the brick mass was found to be more suitable for luminescence dating than the inside portion since the inside might be incompletely fired during the production process. Among the brick ages obtained using the outside portion, both the TL and OSL (with a minimum model analyses were all in agreement with the known ages of the TT, except for one sample that appeared to be much younger. This likely represents a subsequent renovation brick. Thus, the assessment of renovation and other imports into sites should be carefully considered in future luminescence dating.

  17. Optically stimulated luminescence (OSL) of dental enamel for retrospective assessment of radiation exposure

    Energy Technology Data Exchange (ETDEWEB)

    Yukihara, E.G. [Department of Physics, Oklahoma State University, Stillwater, OK 74078 (United States)], E-mail: eduardo.yukihara@okstate.edu; Mittani, J.; McKeever, S.W.S. [Department of Physics, Oklahoma State University, Stillwater, OK 74078 (United States); Simon, S.L. [Division of Cancer Epidemiology and Genetics, National Cancer Institute, National Institutes of Health, Bethesda, MD 20892-7238 (United States)

    2007-07-15

    This paper briefly reviews the optically stimulated luminescence (OSL) properties of dental enamel and discusses the potential and challenges of OSL for filling the technology gap in biodosimetry required for medical triage following a radiological/nuclear accident or terrorist event. The OSL technique uses light to stimulate a radiation-induced luminescence signal from materials previously exposed to ionizing radiation. This luminescence originates from radiation-induced defects in insulating crystals and is proportional to the absorbed dose of ionizing radiation. In our research conducted to date, we focused on fundamental investigations of the OSL properties of dental enamel using extracted teeth and tabletop OSL readers. The objective was to obtain information to support the development of the necessary instrumentation for retrospective dosimetry using dental enamel in laboratory, or for in situ and non-invasive accident dosimetry using dental enamel in emergency triage. An OSL signal from human dental enamel was detected using blue, green, or IR stimulation. Blue/green stimulation associated with UV emission detection seems to be the most appropriate combination in the sense that there is no signal from un-irradiated samples and the shape of the OSL decay is clear. Improvements in the minimum detection level were achieved by incorporating an ellipsoidal mirror in the OSL system to maximize light collection. Other possibilities to improve the sensitivity and research steps necessary to establish the feasibility of the technique for retrospective assessment of radiation exposure are also discussed.

  18. A new sensitive system for measurement of thermally and optically stimulated luminescence

    DEFF Research Database (Denmark)

    Markey, B.G.; Bøtter-Jensen, L.; Poolton, N.R.J.

    1996-01-01

    An automatic system developed at RisO National Laboratory for measuring thermally and optically stimulated luminescence (TL, OSL) is widely used for radiation dose measurements. In the present model, high excitation and detection efficiencies were attempted, but inevitably there is a constant...... optics of the system with a combination of ellipsoidal mirrors and light guides, which also serve to make the system more flexible in choice of excitation source when OSL measurements are required. A variety of new light sources might be employed, adapted to allow the most efficient wavelengths...

  19. A study on the real-time radiation dosimetry measurement system based on optically stimulated luminescence

    Institute of Scientific and Technical Information of China (English)

    LIU Yan-Ping; CHEN Zhao-Yang; BA Wei-Zhen; FAN Yan-Wei; DU Yan-Zhao; PAN Shi-Lie; GUO Qi

    2008-01-01

    The optically stimulated luminescent (OSL) radiation dosimeter technically surveys a wide dynamic measurement range and a high sensitivity.Optical fiber dosimeters provide capability for remote monitoring of the radiation in the locations which are difficult-to-acoess and hazardous.In addition.optical fiber dosimeters are immune to electrical and radio-frequency interference.In this paper,a novel remote optical fiber radiation dosimeter is described.The optical fiber dosimeter takes advantage of the charge trapping materials CaS:Ce, Sm that exhibit OSL.The measuring range of the dosimeter is from 0.1 to 100 Gy.The equipment is relatively simple and small in size,and has low power consumption.This device is suitable for measuring the space radiation dose and also can be used in high radiation dose condition and other dangerous radiation occasions.

  20. Optically stimulated luminescence from quartz measured using the linear modulation technique

    DEFF Research Database (Denmark)

    Bulur, E.; Bøtter-Jensen, L.; Murray, A.S.

    2000-01-01

    The optically stimulated luminescence (OSL) from heated natural quartz has been investigated using the linear modulation technique (LMT), in which the excitation light intensity is increased linearly during stimulation. In contrast to conventional stimulation, which usually produces a monotonically...... stimulated component occurs at a shorter time. This allows the separation of the overlapping OSL components, which are assumed to originate from different traps. The LM-OSL curve from quartz shows an initial peak Followed by a broad one. Deconvolution using curve fitting has shown that the composite OSL...... curve from quartz can be approximated well by using a linear combination of first-order peaks. In addition to the three known components, i.e. fast, medium and slow components from continuous-wave-OSL studies, an additional slow component is also identified for the first time. The dose responses...

  1. SEMICONDUCTOR PHYSICS Dose-rate dependence of optically stimulated luminescence signal

    Science.gov (United States)

    Pingqiang, Wei; Zhaoyang, Chen; Yanwei, Fan; Yurun, Sun; Yun, Zhao

    2010-10-01

    Optically stimulated luminescence (OSL) is the luminescence emitted from a semiconductor during its exposure to light. The OSL intensity is a function of the total dose absorbed by the sample. The dose-rate dependence of the OSL signal of the semiconductor CaS doped Ce and Sm was studied by numerical simulation and experiments. Based on a one-trap/one-center model, the whole OSL process was represented by a series of differential equations. The dose-rate properties of the materials were acquired theoretically by solving the equations. Good coherence was achieved between numerical simulation and experiments, both of which showed that the OSL signal was independent of dose rate. This result validates that when using OSL as a dosimetry technique, the dose-rate effect can be neglected.

  2. Optically stimulated luminescence in KCl:Cu x-irradiated at room temperature

    CERN Document Server

    Bandyopadhyay, P K; Chakrabarti, K

    1999-01-01

    Optically stimulated luminescence (OSL) has been observed in single crystals of KCl:Cu x-irradiated at room temperature. It is shown that electrons are liberated from anion sites during the OSL process. The OSL predominantly involves emission due to radiative transition (d s) of monovalent copper ions present in the lattice. The OSL emission shows a strong temperature dependence indicating a thermally assisted process. Electron-hole recombination followed by energy transfer to the Cu activator is suggested as a possible OSL mechanism in KCl:Cu. Preliminary results of OSL in KBr:Cu are also presented.

  3. Gamma response characterizations of optically stimulated luminescence (OSL) affects personal dosimetry

    Science.gov (United States)

    Monthonwattana, S.; Esor, J.; Rungseesumran, T.; Intang, A.

    2017-06-01

    Optically Stimulated Luminescence (OSL) is the current technique of personal dosimetry changed by Nuclear Technology Service Center instead of Thermoluminescence dosimetry (TLD) because OSL has more advantages, such as repeat reading and elimination of heating process. In this study, OSL was used to test the gamma response characterizations. Detailed OSL investigation on personal dosimetry was carried out in the dose range of 0.2 - 3.0 mSv. The batch homogeneity was 7.66%. R2 value of the linear regression was 0.9997. The difference ratio of angular dependence at ± 60° was 8.7%. Fading of the reading was about 3%.

  4. Surface exposure dating of non-terrestrial bodies using optically stimulated luminescence: A new method

    DEFF Research Database (Denmark)

    Sohbati, Reza; Jain, Mayank; Murray, Andrew

    2012-01-01

    We propose a new method for in situ surface exposure dating of non-terrestrial geomorphological features using optically stimulated luminescence (OSL); our approach is based on the progressive emptying of trapped charge with exposure to light at depth into a mineral surface. A complete model of t...... charge population. The potential dating applications for (a) include dust accumulation, volcanic rocks and impact-related sediments, and for (b) fault scarps, rock-falls, landslides and ice-scoured bedrock. Using assumptions based on terrestrial observations we expect that this approach...

  5. Optical fibre dosemeter systems for clinical applications based on radioluminescence and optically stimulated luminescence from Al2O3:C

    DEFF Research Database (Denmark)

    Marckmann, C.J.; Andersen, C.E.; Aznar, M.C.

    2006-01-01

    Optical fibre dosemeter systems based on radioluminescence and optically stimulated luminescence (OSL) from carbon-doped aluminium oxide (Al2O3:C) crystals were developed for in vivo real-time dose rate and absorbed dose measurements in radiotherapy and mammography. A technique was also developed...... for making ultra-small dosemeter probes that can easily be placed inside patients in radiation treatment. These probes have shown excellent properties in both head and neck intensity-modulated radiation therapy treatment and in mammography. The dose-response of the OSL signal for the new optical fibre...

  6. Developments in optically stimulated luminescence techniques for dating and retrospective dosimetry

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.; Murray, A.S.

    1999-01-01

    Optically stimulated luminescence signals from natural quartz and feldspar are now used routinely in dating geological and archaeological materials. More recently they have also been employed in accident dosimetry, i.e. the retrospective assessment of doses received as a result of a nuclear...... accident. Since 1990, the exploration of this wide variety of applications has driven an intensive investigation and development programme at Riso in measurement facilities and techniques. This paper reviews some of the outcomes of this programme, including (i) optimisation of stimulation and emission...... windows, and detection sensitivity, (ii) experience with various stimulation light sources, including filtered incandescent lamps and high intensity light emitting diodes and laser diodes (infrared at 830-850 nm, blue-green at 420-550 nm and blue at 470 nm). Also discussed are recently developed high...

  7. Charge recombination processes in minerals studied using optically stimulated luminescence and time-resolved exo-electrons

    DEFF Research Database (Denmark)

    Tsukamoto, Sumiko; Murray, Andrew; Ankjærgaard, Christina

    2010-01-01

    electron concentration in the conduction band. In this study, TR-OSE and time-resolved optically stimulated luminescence (TR-OSL) were measured for the first time using quartz, K-feldspar and NaCl by stimulating the samples using pulsed blue LEDs at different temperatures between 50 and 250 °C after beta...

  8. Thermally and optically stimulated luminescence of new ZnO nano phosphors exposed to beta radiation

    Energy Technology Data Exchange (ETDEWEB)

    Cruz V, C.; Burruel I, S.E.; Grijalva M, H.; Chernov, V.; Bernal, R. [Universidad de Sonora, A.P. 130, 83000 Hermosillo, Sonora (Mexico)

    2006-07-01

    In this work, we report the thermoluminescence (TL) and the optically stimulated luminescence (OSL) of ZnO nano phosphors obtained by thermal annealing of ZnS powders synthesized by precipitation in a chemical bath deposition reaction. To obtain nanocrystalline ZnO, ZnS pellet-shaped samples were subjected to a sintering process at 700 C during 24 under air atmosphere. Some samples were exposed to beta particles in the 0.15-10.15 kGy dose range and the integrated thermoluminescence as a function of dose increased as dose increased, with no saturation clue for the tested doses. Computerized glow-curve deconvolution of the experimental TL curves in individual peaks revealed a second order kinetics. In order to test the BOSL (Blue Optically Stimulated Luminescence) response, samples were beta irradiated with doses up to 600 Gy, showing an increasing OSL intensity as dose increases. From the experimental results that we have obtained, we conclude that the new ZnO phosphors under investigation are good candidates to be used as dosimetric materials. (Author)

  9. Luminescence optically stimulated: theory and applications; Luminiscencia opticamente estimulada: teoria y aplicaciones

    Energy Technology Data Exchange (ETDEWEB)

    Rivera M, T.; Azorin N, J. [Departamento de Fisica, Universidad Autonoma Metropolitana-Iztapalapa, 09340 Mexico D.F. (Mexico)

    2002-07-01

    The thermally stimulated luminescence (Tl) has occupied an important place in the Solid state physics (FES) by the flexibility of the phenomena, mainly for its applications in the fields of Radiation Physics (FR) and Medical Physics (MF). The reason of this phenomena lies in the fact of the electrons release by the action of heat. Under that same reason, it can be used the action of another stimulant agent for releasing the trapped electrons in the metastable states (EM), this agent is the light which has the same effect that the heat, giving as result the production of light photons at using light in the visible spectra, of different wavelength that the excitation light. This phenomena is called Luminescence optically stimulated (LOE). The LOE has a great impact in the Solid State Physics (FES), dating and now in the use of the phenomena as a dosimetric method, alternate to the Tl, for its use in the ionizing and non-ionizing radiations fields. (Author)

  10. Using soils for accident dosimetry: a preliminary study using optically stimulated luminescence from quartz

    DEFF Research Database (Denmark)

    Fujita, Hiroki; Jain, Mayank; Murray, Andrew S.

    2011-01-01

    The optimum conditions of preheat temperature, stimulation temperature, etc. in the single-aliquot regenerative optically stimulated luminescence (SAR OSL) method were examined specifically for measuring background dose in natural quartz extracted from soils collected around Tokai-mura in Japan....... The objective was to assess the potential of SAROSL dosimetry using soils for retrospective assessment of a radiation accident. Variation in dose with depth was also measured. The SAR data showed good reproducibility and dose recovery, and there was no evidence of fading of the quartz signal based on “delayed......, and no clear trend in dose depth profile was observed. From these results, we conclude that SAR OSL dosimetry using natural quartz extracted from soil could be used to evaluate the dose of an accident....

  11. Independent evaluation of optically stimulated luminescence (OSL) 'dot' dosemeters for environmental monitoring.

    Science.gov (United States)

    Timilsina, Bindu; Gesell, Thomas F

    2011-01-01

    Optically stimulated luminescence (OSL) 'dot' dosemeters (manufactured by Landauer®) are reported to have a high degree of environmental stability, high level of sensitivity and provide wide range of dose measuring capabilities from 0.05 mGy to 100 Gy. The optical read out method is fast and relatively simple and permits repeated read out, but few studies have been performed about its application in monitoring radiation in the environment. This study was initiated to independently test the performance of OSL dot dosemeters for the application of measuring doses of radiation in the outdoor environment. Testing was performed in the laboratory to evaluate reproducibility and stability and in the field to evaluate accuracy relative to calibrated high-pressure ionisation chambers. The results showed that OSL dot dosemeters had good reproducibility and stability in both laboratory and field tests and met the performance requirements of standards of the American National Standards Institute.

  12. Violet stimulated luminescence: geo- or thermochronometer?

    DEFF Research Database (Denmark)

    Ankjærgaard, Christina; Guralnik, Benny; Porat, N.

    2015-01-01

    The method of quartz optically stimulated luminescence (OSL) dating is widely used, but generally limited to the past ~0.1 million years (Ma) due to early saturation of the desired signal. Violet stimulated luminescence (VSL) of quartz has previously been shown as a promising alternative...

  13. Violet stimulated luminescence: geo- or thermochronometer?

    DEFF Research Database (Denmark)

    Ankjærgaard, Christina; Guralnik, Benny; Porat, N.;

    2015-01-01

    The method of quartz optically stimulated luminescence (OSL) dating is widely used, but generally limited to the past ~0.1 million years (Ma) due to early saturation of the desired signal. Violet stimulated luminescence (VSL) of quartz has previously been shown as a promising alternative...

  14. Kinetics of infrared stimulated luminescence from feldspars

    DEFF Research Database (Denmark)

    Jain, Mayank; Sohbati, Reza; Guralnik, Benny;

    2015-01-01

    thermal and optical, of the infrared stimulated luminescence signal from feldspar. Based on the application of this model, it is concluded that different infra-red stimulated luminescence emissions (UV, blue, yellow and far-red) follow the same kinetics, and, therefore, involve participation of the same...

  15. Soil development rates from an optically stimulated luminescence-dated beach ridge sequence in Northern Jutland, Denmark

    DEFF Research Database (Denmark)

    Nielsen, Asger Habekost; Elberling, Bo; Pejrup, Morten

    2010-01-01

    of each pedon and soil stratum was measured by optically stimulated luminescence (OSL) dating and used to estimate soil development rates. Soils were divided into five groups from Typic Haplorthods and Entic Alorthods with a mean OSL age of 29659294 yr to Typic Quartzipsamments with a mean OSL age...

  16. Optically stimulated luminescence dating of cave deposits at the Xiaogushan prehistoric site, northeastern China.

    Science.gov (United States)

    Zhang, Jia-Fu; Huang, Wei-Wen; Yuan, Bao-Yin; Fu, Ren-Yi; Zhou, Li-Ping

    2010-11-01

    The Xiaogushan cave site is one of the most important prehistoric sites in North China. The stone and bone artifacts found in the cave are similar to European contemporaneous artifacts. Cave deposits consist of five layers that have been dated from 46,353 ± 1179 to 4229 ± 135 cal. yr BP, using radiocarbon dating techniques on charcoal and bone samples collected from Layers 2-5. In this paper, optically stimulated luminescence (OSL) techniques were applied to date six samples taken from Layers 1-3. The luminescence properties of the fine-grained and coarse-grained quartz extracts indicate that the materials are suitable for OSL dating using a single-aliquot regeneration-dose (SAR) protocol. The OSL ages obtained are broadly consistent with the stratigraphy and the associated calibrated radiocarbon ages. The dating results show that the cave was first occupied by humans about 70 ka. The human occupation of the cave may be related to climate change. An occupation hiatus is inferred to between ∼ 17 to ∼ 10 ka. The stone and bone artifacts found in Layers 2 and 3 may indicate the Middle to Upper Paleolithic transitions in the region.

  17. An optically stimulated luminescence study of porcelain related to radiation dosimetry

    DEFF Research Database (Denmark)

    Poolton, N.R.J.; Bøtter-Jensen, L.; Jungner, H.

    1995-01-01

    This article describes the essential features regarding the photo-stimulated luminescence of porcelain: both the main ceramic and glazing materials are studied. In each case, radiation dose dependent signals are observed, superimposed on dose independent luminescence transitions that are both...... Stokes and anti-Stokes shifted in energy. Glazing is shown in some cases to be considerably more sensitive as a radiation dosemeter than the main porcelain ceramic. By comparison with the properties of artifical phosphors, the principal luminescent matrix is identified as being Al2O3...

  18. A new sensitive system for measurement of thermally and optically stimulated luminescence

    Energy Technology Data Exchange (ETDEWEB)

    Markey, B.G.; Boetter-Jensen, L.; Poolton, N.R.J.; Christensen, H.E.; Willumsen, F. [Risoe National Lab., Roskilde (Denmark)

    1996-12-31

    An automatic system developed at Riso National Laboratory for measuring thermally and optically stimulated luminescence (TL, OSL) is widely used for radiation dose measurements. In the present model, high excitation and detection efficiencies were attempted, but inevitably there is a constant demand for improvements that would allow lower doses (or less sensitive materials) to be measured, with increased accuracy. This article reports on a new generation of designs that are intended to meet these demands. Substantial increases in sensitivity of the instruments are made by replacing the lens optics of the system with a combination of ellipsoidal mirrors and light guides, which also serve to make the system more flexible in choice of excitation source when OSL measurements are required. A variety of new light sources might be employed, adapted to allow them most efficient wavelengths of excitation to be used for the particular dosemeter under study. The capabilities and characteristics of the new design are described, and comparison with the existing TL/OSL system is made throughout the article. (author).

  19. Dose-dependent optically stimulated luminescence of synthetic quartz at room temperature

    Energy Technology Data Exchange (ETDEWEB)

    Kale, Y.D. [Luminescence Research Laboratory, Applied Physics Department, Faculty of Technology and Engineering, M.S. University of Baroda, Vadodara (India); Gandhi, Y.H. [Luminescence Research Laboratory, Applied Physics Department, Faculty of Technology and Engineering, M.S. University of Baroda, Vadodara (India)], E-mail: yasheshgandhi@yahoo.co.in; Gartia, R.K. [Luminescence Dating Laboratory, Department of Physics, Manipur University, Imphal (India)

    2008-12-15

    Physical conditions such as annealing temperature, duration of annealing, ionizing radiation, etc., play a significant role in the applications of optically stimulated luminescence (OSL) dating as well as OSL dosimetry. Many efforts are made to understand the effect of these physical parameters on quartz specimens owing to its use in such applications. Such factors induce changes in OSL decay pattern. The definite correlation between color centers and luminescence sensitivity can be established on account of such pre-treatments to the specimen. The purpose of present investigations is to study the effect of ionizing radiation under identical physical conditions on OSL properties measured at room temperature. The shapes of decay curve and dose-response data are considered for this purpose. This study can reveal the changes in color centers in response to the pre-conditions to the specimen. It was found that the OSL decay remains slow and OSL properties change systematically with the rise in beta dose up to a critical dose; however, it changes the pattern when the beta exposure to the specimen was increased higher than the critical dose. This critical dose was found to be different for different temperature of annealing. The shape of decay curve up to the critical dose was also studied by considering the difference of OSL intensities between two successive durations from the observed OSL decay data. The results are explained based on the changes in available shallow traps during OSL measurement at room temperature with changes in pre-conditions to the specimens. The results also have been confirmed with the corresponding changes in ESR signals.

  20. Optically stimulated luminescence techniques in retrospective dosimetry using single grains of quartz extracted from unheated materials

    Energy Technology Data Exchange (ETDEWEB)

    Joerkov Thomsen, Kristina

    2004-02-01

    This work investigates the possibility of applying optically stimulated luminescence (OSL) in retrospective dose determinations using unheated materials. It focuses on identifying materials suitable for use in assessment of doses absorbed as a consequence of radiation accidents (i.e. accident dosimetry). Special attention has been paid to quartz extracted from unheated building materials such as concrete and mortar. The single-aliquot regeneration-dose (SAR) protocol has been used to determine absorbed doses in small aliquots as well as single grains of quartz. It is shown that OSL measurements of single grains of quartz extracted from poorly-bleached building materials can provide useful information on radiation accident doses, even when the luminescence sensitivity is low. Sources of variance in well-bleached single grain dose distributions have been investigated in detail and it is concluded that the observed variability in the data is consistent with the sum (in quadrature) of a component, which depends on the number of photons detected from each grain, and a fixed component independent of light level. Dose depth profiles through laboratory irradiated concrete bricks have successfully been measured and minimum detection limits of less than 100 mGy are derived. Measurements of thermal transfer in single grains of poorly-bleached quartz show that thermal transfer is variable on a grain-to-grain basis and that it can be a source of variance in single-grain dose distributions. Furthermore, the potential of using common household and workplace chemicals, such as table salt, washing powder and water softener, in retrospective dosimetry has been investigated. It is concluded that such materials should be considered as retrospective dosimeters in the event of a radiation accident. (au)

  1. Investigating quartz optically stimulated luminescence dose-response curves at high doses

    Energy Technology Data Exchange (ETDEWEB)

    Lowick, Sally E., E-mail: lowick@geo.unibe.c [Institut fuer Geologie, Universitaet Bern, Baltzerstrasse 1-3, 3012 Bern (Switzerland); Preusser, Frank [Institut fuer Geologie, Universitaet Bern, Baltzerstrasse 1-3, 3012 Bern (Switzerland); Wintle, Ann G. [Institute of Geography and Earth Sciences, Aberystwyth University, AberystwythSY23 3DB (United Kingdom)

    2010-10-15

    Despite the general expectation that optically stimulated luminescence (OSL) growth should be described by a simple saturating exponential function, an additional high dose component is often reported in the dose response of quartz. Although often reported as linear, it appears that this response is the early expression of a second saturating exponential. While some studies using equivalent doses that fall in this high dose region have produced ages that correlate well with independent dating, others report that it results in unreliable age determinations. Two fine grain sedimentary quartz samples that display such a response were used to investigate the origin of this additional high dose component: three experiments were conducted to examine their dose-response up to >1000 Gy. The high dose rates provided by laboratory irradiation were found not to induce a sensitivity change in the response to a subsequent test dose, with the latter not being significantly different from those generated following naturally acquired doses. The relative percentage contributions of the fast and medium OSL components remained fixed throughout the dose-response curve, suggesting that the electron traps that give rise to the initial OSL do not change with dose. An attempt was made to investigate a change in luminescence centre recombination probability by monitoring the depletion of the '325 {sup o}C' thermoluminescence (TL) during the optical stimulation that would result in depletion of the OSL signal. The emissions measured through both the conventional ultraviolet (UV), and a longer wavelength violet/blue (VB) window, displayed similar relative growth with dose, although it was not possible to resolve the origin of the VB emissions. No evidence was found to indicate whether the additional component at high doses occurs naturally or is a product of laboratory treatment. However, it appears that these samples display an increased sensitivity of quartz OSL to high doses

  2. Long persistent and optically stimulated luminescence behaviors of calcium aluminates with different trap filling processes

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, Buhao; Xu, Xuhui; Li, Qianyue; Wu, Yumei; Qiu, Jianbei; Yu, Xue, E-mail: yuyu6593@126.com

    2014-09-15

    Properties of long persistent luminescence (LPL) and optically stimulated luminescence (OSL) of CaAl{sub 2}O{sub 4}:Eu{sup 2+}, R{sup 3+} (R=Nd, Dy, Tm) materials were investigated. The observed phenomenon indicates that R{sup 3+} ions (R=Nd, Dy, Tm) have different effects on trap properties of CaAl{sub 2}O{sub 4}:Eu{sup 2+}. The greatly improved LPL performance was observed in Nd{sup 3+} co-doped samples, which indicates that the incorporation of Nd{sup 3+} creates suitable traps for LPL. While co-doping Tm{sup 3+} ions, the intensity of high temperature of thermoluminescence band in CaAl{sub 2}O{sub 4}:Eu{sup 2+} phosphors is enhanced for the formation of the most suitable traps which benefits the intense and stable OSL. These results suggest that the effective traps contributed to the LPL/OSL are complex, of which could be an aggregation formation with shallow and deep traps other than simple traps from co-doped R{sup 3+} ions. The mechanism presented in the end potentially provides explanations of why the OSL of CaAl{sub 2}O{sub 4}:Eu{sup 2+}, R{sup 3+} exhibits different read-in/read-out performance as well. - Graphical abstract: OSL emission spectra of Ca{sub 0.995}Al{sub 2}O{sub 4}:0.0025Eu{sup 2+}, 0.0025R{sup 3+} (R=Nd, Dy, Tm) taken under varying stimulation time (0, 25, 50, 75, 100 s). Inset: Blue emission pictures under varying stimulation time. - Highlights: • The LPL and OSL properties of CaAl{sub 2}O{sub 4}:Eu{sup 2+}, R{sup 3+} were investigated. • An alternative approach to control the trap depth of CaAl{sub 2}O{sub 4}:Eu{sup 2+} phosphor was proposed. • A new oxide ETM phosphor exhibiting intense and stable OSL was explored.

  3. Optically stimulated luminescence (OSL) dating of quartzite cobbles from the Tapada do Montinho archaeological site (east-central Portugal)

    DEFF Research Database (Denmark)

    Sohbati, Reza; Murray, Andrew S.; Buylaert, Jan-Pieter

    2012-01-01

    The burial age of an alluvially deposited cobble pavement at the Tapada do Montinho archaeological site (east-central Portugal) is investigated using optically stimulated luminescence (OSL) dating. Measurements on the cobbles (quartzite clasts) were carried out on intact slices and large aliquots...... luminescence characteristics. The variation in the natural OSL signal with depth below the cobble surface using intact slices from two different cobbles shows that both were bleached to a depth of at least similar to 2?mm before deposition. A model of the variation of dose with depth fitted to data from one...... contained within a single clast, and this suggests that the luminescence dating of rock surfaces may prove, in the future, to be at least as important as sand/silt sediment dating....

  4. Optically stimulated luminescence of common plastic materials for accident dose reconstruction

    Energy Technology Data Exchange (ETDEWEB)

    Chang, I.; Lee, J. I.; Kim, J. L. [Korea Atomic Energy Research Institute, Daejeon (Korea, Republic of); Chung, K. S. [Gyeongsang National Univ., Jinju (Korea, Republic of)

    2014-05-15

    Optically stimulate luminescence(OSL) has many applications in a variety of radiation dosimetry fields, including personal dosimetry, environmental radiation level monitor, retrospective dosimetry for dating, and reconstruction of radiation doses from radiation accident. In the reconstruction of radiation doses from radiation accident, OSL technique has been used to estimate the doses exposed to public area through analysis of housewares or house construing materials. Recently, many efforts have been carried out for dose reconstruction using personal electronic devices such as mobile phones and USB memory chips. Some of natural minerals such as quartz and feldspar have OSL properties. Quartz is the second most abundant mineral in continental crust of the Earth. In some of common plastics, inorganic fillers (quartz, alumina etc.) are added to make strengthen of their properties depends on applications areas. The aim of this research is to explore a possibility of use of the common plastic materials for dose reconstruction in radiation accident case. In this research the OSL dose response-curve and fading characteristics of the common plastics were tested and evaluated. Finally, we expect this work contribute to elevate the possibility of the dose reconstruction. The general conclusion of this work is that the possibility of dose reconstruction using common plastic materials is showed using the OSL characteristics of the materials. However, the tested common plastic materials have relatively low sensitivities. Further work is required to establish a database of OSL properties of common plastic materials for emergency dose reconstruction by using housewares.

  5. Optically stimulated luminescence dating of archaeological ceramics from Osvaldo and Lago Grande sites in central Amazon

    Energy Technology Data Exchange (ETDEWEB)

    Hazenfratz, Roberto; Tudela, Diego R.G.; Munita, Casimiro S., E-mail: robertohm@ipen.br [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP), Sao Paulo, SP (Brazil); Mittani, Juan C.R.; Tatumi, Sonia H. [Universidade Federal de Sao Paulo (UNIFESP), Santos, SP (Brazil)

    2013-07-01

    Thermoluminescence (TL) and optically stimulated luminescence (OSL) dating are two important techniques for dating archaeological and geological material, especially suitable for archaeological ceramics, where samples for {sup 14}C dating are not available. In this work, five pottery shards from Osvaldo and Lago Grande archaeological sites were dated by OSL. For measurements, it was used the SAR protocol. The annual dose rates were estimated by the contents of U, Th and K, determined by instrumental neutron activation analysis (INAA) of the pottery shards and clay samples near both sites. Lago Grande and Osvaldo represent a microcosm of the region, and their proximity and high density of archaeological record turn them interesting to study possible relations of cultural and/or commercial exchange. Calculations showed that the water content is an important variable that cannot be neglected in OSL dating of pottery shards from central Amazon, due to the high humidity in regional soils. The results between 867 ± 101 and 1154 ± 62 years AD agreed with the average time span for the archaeological sites occupation found in the literature. (author)

  6. Depth dose deposition measurement in electronics packages using optically stimulated luminescence films; Mesure du rendement en profondeur dans un boitier de composant electronique au moyen de films luminescents stimulables optiquement

    Energy Technology Data Exchange (ETDEWEB)

    Ranchoux, G.; Dusseau, L.; Gensanne, D.; Plattard, D.; Polge, G.; Saigne, F.; Fesquet, J.; Gasiot, J. [Montpellier-2 Univ., CEMM2, 34 (France); Menduina, X. [Universite Autonome de Barcelone (Spain); Bessiere, J.C. [CORAD P.I.T. Pompignane, 34 - Montpelliers (France)

    1999-07-01

    The energy deposited by electrons versus depth inside molded Epoxy packages is measured using optically stimulated luminescence (OSL) dose mapping technique. Longitudinal and transversal depth dose curves are investigated under various angles of irradiation. Experimental results are compared with PENELOPE transport code calculations. Preliminary results are in good agreement with simulations.

  7. Optically stimulated luminescence (OSL) as a chronometer for surface exposure dating

    Science.gov (United States)

    Sohbati, Reza; Murray, Andrew S.; Chapot, Melissa S.; Jain, Mayank; Pederson, Joel

    2012-09-01

    We pioneer a technique of surface-exposure dating based upon the characteristic form of an optically stimulated luminescence (OSL) bleaching profile beneath a rock surface; this evolves as a function of depth and time. As a field illustration of this new method, the maximum age of a premier example of Barrier Canyon Style (BCS) rock art in Canyonlands National Park, Utah, USA, is constrained. The natural OSL signal from quartz grains is measured from the surface to a depth of >10 mm in three different rock samples of the Jurassic Navajo Sandstone. Two samples are from talus with unknown daylight exposure histories; one of these samples was exposed at the time of sampling and one was buried and no longer light exposed. A third sample is known to have been first exposed 80 years ago and was still exposed at the time of sampling. First, the OSL-depth profile of the known-age sample is modeled to estimate material-dependent and environmental parameters. These parameters are then used to fit the model to the corresponding data for the samples of unknown exposure history. From these fits we calculate that the buried sample was light exposed for ˜700 years before burial and that the unburied sample has been exposed for ˜120 years. The shielded surface of the buried talus sample is decorated with rock art; this rock fell from the adjacent Great Gallery panel. Related research using conventional OSL dating suggests that this rockfall event occurred ˜900 years ago, and so we deduce that the rock art must have been created between ˜1600 and 900 years ago. Our results are the first credible estimates of exposure ages based on luminescence bleaching profiles. The strength of this novel OSL method is its ability to establish both ongoing and prior exposure times, at decadal to millennial timescales or perhaps longer (depending on the environmental dose rate) even for material subsequently buried. This has considerable potential in many archeological, geological and geo

  8. Optically stimulated luminescence dating of aeolian sand in the otindag dune field and holocene climate change

    Science.gov (United States)

    Zhou, Y.L.; Lu, H.Y.; Mason, J.; Miao, X.D.; Swinehart, J.; Goble, R.

    2008-01-01

    The dune system in Otindag sand field of northern China is sensitive to climate change, where effective moisture and related vegetation cover play a controlling role for dune activity and stability. Therefore, aeolian deposits may be an archive of past environmental changes, possibly at the millennial scale, but previous studies on this topic have rarely been reported. In this study, thirty-five optically stimulated luminescence (OSL) ages of ten representative sand-paleosol profiles in Otindag sand field are obtained, and these ages provide a relatively complete and well-dated chronology for wet and dry variations in Holocene. The results indicate that widespread dune mobilization occurred from 9.9 to 8.2 ka, suggesting a dry early Holocene climate. The dunes were mainly stabilized between 8.0 and 2.7 ka, implying a relatively wet climate, although there were short-term penetrations of dune activity during this wet period. After ???2.3 ka, the region became dry again, as inferred from widespread dune activity. The "8.2 ka" cold event and the Little Ice Age climatic deterioration are detected on the basis of the dune records and OSL ages. During the Medieval Warm Period and the Sui-Tang Warm Period (570-770 AD), climate in Otindag sand field was relatively humid and the vegetation was denser, and the sand dunes were stabilized again. These aeolian records may indicate climate changes at millennial time scale during Holocene, and these climatic changes may be the teleconnection to the climate changes elsewhere in the world. ?? Science in China Press and Springer-Verlag GmbH 2008.

  9. Optically stimulated luminescence dating of aeolian sand in the Otindag dune field and Holocene climate change

    Institute of Scientific and Technical Information of China (English)

    Joseph; MASON; James; SWINEHART; Ronald; GOBLE

    2008-01-01

    The dune system in Otindag sand field of northern China is sensitive to climate change, where effective moisture and related vegetation cover play a controlling role for dune activity and stability. Therefore, aeolian deposits may be an archive of past environmental changes, possibly at the millennial scale, but previous studies on this topic have rarely been reported. In this study, thirty-five optically stimulated luminescence (OSL) ages of ten representative sand-paleosol profiles in Otindag sand field are ob-tained, and these ages provide a relatively complete and well-dated chronology for wet and dry varia-tions in Holocene. The results indicate that widespread dune mobilization occurred from 9.9 to 8.2 ka, suggesting a dry early Holocene climate. The dunes were mainly stabilized between 8.0 and 2.7 ka, implying a relatively wet climate, although there were short-term penetrations of dune activity during this wet period. After ~2.3 ka, the region became dry again, as inferred from widespread dune activity. The "8.2 ka" cold event and the Little Ice Age climatic deterioration are detected on the basis of the dune records and OSL ages. During the Medieval Warm Period and the Sui-Tang Warm Period (570-770 AD), climate in Otindag sand field was relatively humid and the vegetation was denser, and the sand dunes were stabilized again. These aeolian records may indicate climate changes at millennial time scale during Holocene, and these climatic changes may be the teleconnection to the climate changes elsewhere in the world.

  10. Optically stimulated luminescence dating of aeolian sand in the Otindag dune field and Holocene climate change

    Institute of Scientific and Technical Information of China (English)

    ZHOU YaLi; LU HuaYu; Joseph MASON; MIAO XiaoDong; James SWINEHART; Ronald GOBLE

    2008-01-01

    The dune system in Otindag sand field of northern China is sensitive to climate change, where effective moisture and related vegetation cover play a controlling role for dune activity and stability. Therefore, aeolian deposits may be an archive of past environmental changes, possibly at the millennial scale, but previous studies on this topic have rarely been reported. In this study, thirty-five optically stimulated luminescence (OSL) ages of ten representative sand-paleosol profiles in Otindag sand field are ob-tained, and these ages provide a relatively complete and well-dated chronology for wet and dry varia-tions in Holocene. The results indicate that widespread dune mobilization occurred from 9.9 to 8.2 ka, suggesting a dry early Holocene climate. The dunes were mainly stabilized between 8.0 and 2.7 ka, implying a relatively wet climate, although there were short-term penetrations of dune activity during this wet period. After ~2.3 ka, the region became dry again, as inferred from widespread dune activity. The "8.2 ka" cold event and the Little Ice Age climatic deterioration are detected on the basis of the dune records and OSL ages. During the Medieval Warm Period and the Sui-Tang Warm Period (570-770 AD), climate in Otindag sand field was relatively humid and the vegetation was denser, and the sand dunes were stabilized again. These aeolian records may indicate climate changes at millennial time scale during Holocene, and these climatic changes may be the teleconnection to the climate changes elsewhere in the world.

  11. Optically stimulated luminescence (OSL) of Lu{sub 2}SiO{sub 5}:Ce powder: A preliminary study

    Energy Technology Data Exchange (ETDEWEB)

    Gartia, R.K., E-mail: rkgartia02@yahoo.i [Physics Department, Manipur University, Imphal 795003 (India); Singh, Th. Tejkumar [Physics Department, Manipur University, Imphal 795003 (India); Singh, Th. Basanta [Luminescence Dating Laboratory, Manipur University, Imphal 795003 (India)

    2011-01-01

    Optically stimulated luminescence (OSL) of Lu{sub 2}SiO{sub 5}:Ce powder (Phosphor Technology Ltd., UK) has been measured by Riso TL/OSL Reader (TL-DA-15). Upon blue photon stimulation ({lambda}{sub ex} {approx}470 nm) the material shows strong OSL signal that can detect {beta}-irradiation right up to the dose of {approx}0.2 Gy. A brief discussion on this finding is presented by comparing the thermoluminescence of the system with and without optical stimulation. The two key important parameters namely, trap-depth (E) and frequency factor (s) of the main peaks that occur at 85 and 232 {sup o}C are determined.

  12. KCl:Eu2+ as a solar UV-C radiation dosimeter.Optically stimulated luminescence and thermoluminescence analyses

    Institute of Scientific and Technical Information of China (English)

    I.Aguirre de Cáarcer; H.L.D'Antoni; M.Barboza-Flores; V.Correcher; F.Jaque

    2009-01-01

    The KCl:Eu2+ system response to UV-C was investigated by analyzing the optically stimulated luminescence (OSL) and thertoo-luminescence (TL) signal produced by ultraviolet light exposure at room temperature.It was found that after UV-C irradiation,OSL was produced on a wide band of visible wavelengths with decay time that varied by several orders of magnitude depending on the Eu2+ aggregation state.In spite of the low intensity of solar UV-C reaching the Earth's surface in Madrid (40° N,700 m a.s.l.),it was possible to measure the UV-C radiation dose at 6:48 solar time by using the TL response of the KCl:Eu2+ system and differentiate it from the ambient beta radiation dose.

  13. An optically stimulated luminescence study of flint related to radiation dosimetry

    DEFF Research Database (Denmark)

    Poolton, N.R.J.; Bøtter-Jensen, L.; Rink, W.J.

    1995-01-01

    This article describes the essential features of photo-stimulated luminescence in flint. The emission is shown to be complex, arising from a number of different aspects of the material. Under constant illumination, dose-dependent time-decaying anti-Stokes signals are superimposed on dose......-independent, time-stable emission that is both Stokes and anti-Stokes shifted in energy. It is argued that the dose-dependent signals arise from the crystalline quartz phase of the material, whereas the dose independent signals originate from an amorphous-like phase of SiO2. The microcrystallinity of the material...

  14. Optically stimulated luminescence sensitivity changes in quartz due to repeated use in single aliquot readout: Experiments and computer simulations

    DEFF Research Database (Denmark)

    McKeever, S.W.S.; Bøtter-Jensen, L.; Agersnap Larsen, N.

    1996-01-01

    As part of a study to examine sensitivity changes in single aliquot techniques using optically stimulated luminescence (OSL) a series of experiments has been conducted with single aliquots of natural quartz, and the data compared with the results of computer simulations of the type of processes...... believed to be occurring. The computer model used includes both shallow and deep ('hard-to-bleach') traps, OSL ('easy-to-bleach') traps, and radiative and non-radiative recombination centres. The model has previously been used successfully to account for sensitivity changes in quartz due to thermal...... trap and deep trap effects....

  15. Thermally and optically stimulated luminescence of AlN-Y2O3 ceramics after ionising irradiation

    DEFF Research Database (Denmark)

    Trinkler, L.; Bos, A.J.J.; Winkelman, A.J.M.;

    1999-01-01

    Thermally (TL) and optically stimulated luminescence (OSL) were studied in AlN-Y2O3 ceramics after irradiation with ionising radiation. The extremely high TL sensitivity (approximately 60 times the sensitivity of LiF:Mg,Tl (TLD-100)) makes AlN-Y2O3 ceramics attractive as a TLD material. However......, an essential drawback of AlN-Y2O3 is its high fading rate. Special attention has been focused on understanding and improving the fading properties. In particular, the influence of the ceramics production conditions and the additive concentration on the fading rate have been studied. Experimental results...

  16. Optically- and thermally-stimulated luminescences of Ce-doped SiO2 glasses prepared by spark plasma sintering

    Science.gov (United States)

    Okada, Go; Kasap, Safa; Yanagida, Takayuki

    2016-11-01

    Rare-earth doped phosphors have been used in many applications including radiation measurements. In the latter applications, the radiation photons are converted to light so that we can indirectly detect the radiation using a conventional photodetector. In this work, we have prepared and characterized a Ce-doped SiO2 glass for dosimeter applications. Unlike conventional techniques such as sol-gel synthesis, the sample was prepared by spark plasma sintering. Although the PL emission seems to be only from the Ce3+ ions in the structure, due to the X-ray induced luminescence, we have also observed optically-stimulated luminescence (OSL), and thermally-stimulated luminescence (TSL), owing to a pair of silylenes and a set of dioxasilirane and silylene in addition to Ce3+. We have measured the detector response vs irradiation dose for both the OSL and TSL. The detector response in both cases is linear over the dose range from at least 1 mGy to 2 Gy. Particularly, the sensitivity of TSL is so high that it should be considered to be a good candidate for practical applications.

  17. Recent developments of optically stimulated luminescence materials and techniques for radiation dosimetry and clinical applications

    Directory of Open Access Journals (Sweden)

    Pradhan A

    2008-01-01

    Full Text Available During the last 10 years, optically stimulated luminescence (OSL has emerged as a formidable competitor not only to thermoluminescence dosimetry (TLD but also to several other dosimetry systems. Though a large number of materials have been synthesized and studied for OSL, Al 2 O 3 :C continues to dominate the dosimetric applications. Re-investigations of OSL in BeOindicate that this material might provide an alternative to Al 2 O 3 :C. Study of OSL of electronic components of mobile phones and ID cards appears to have opened up a feasibility of dosimetry and dose reconstruction using the electronic components of gadgets of everyday use in the events of unforeseen situations of radiological accidents, including the event of a dirty bomb by terrorist groups. Among the newly reported materials, a very recent development of NaMgF 3 :Eu 2+ appears fascinating because of its high OSL sensitivity and tolerable tissue equivalence. In clinical dosimetry, an OSL as a passive dosimeter could do all that TLD can do, much faster with a better or at least the same efficiency; and in addition, it provides a possibility of repeated readout unlike TLD, in which all the dose information is lost in a single readout. Of late, OSL has also emerged as a practical real-time dosimeter for in vivo measurements in radiation therapy (for both external beams and brachytherapy and in various diagnostic radiological examinations including mammography and CT dosimetry. For in vivo measurements, a probe of Al 2 O 3 :C of size of a fraction of a millimeter provides the information on both the dose rate and the total dose from the readout of radioluminescence and OSL signals respectively, from the same probe. The availability of OSL dosimeters in various sizes and shapes and their performance characteristics as compared to established dosimeters such as plastic scintillation dosimeters, diode detectors, MOSFET detectors, radiochromic films, etc., shows that OSL may soon become

  18. A methodology for on-board CBCT imaging dose using optically stimulated luminescence detectors.

    Science.gov (United States)

    Mail, Noor; Yusuf, Muhammad; Alothmany, Nazeeh; Kinsara, A Abdulrahman; Abdulkhaliq, Fahad; Ghamdi, Suliman M; Saoudi, Abdelhamid

    2016-09-08

    Cone-beam computed tomography CBCT systems are used in radiation therapy for patient alignment and positioning. The CBCT imaging procedure for patient setup adds substantial radiation dose to patient's normal tissue. This study pre-sents a complete procedure for the CBCT dosimetry using the InLight optically-stimulated-luminescence (OSL) nanoDots. We report five dose parameters: the mean slice dose (DMSD); the cone beam dose index (CBDIW); the mean volume dose (DMVD); point-dose profile, D(FOV); and the off-field Dose. In addition, CBCT skin doses for seven pelvic tumor patients are reported. CBCT-dose mea-surement was performed on a custom-made cylindrical acrylic body phantom (50cm length, 32cm diameter). We machined 25 circular disks (2 cm thick) with grooves and holes to hold OSL-nanoDots. OSLs that showed similar sensitivities were selected and calibrated against a Farmer-type ionization-chamber (0.6 CT) before being inserted into the grooves and holes. For the phantom scan, a standard CBCT-imaging protocol (pelvic sites: 125 kVp, 80 mA and 25 ms) was used. Five dose parameters were quantified: DMSD, CBDIW, DMVD, D(FOV), and the off-field dose. The DMSD for the central slice was 31.1 ± 0.85 mGy, and CBDIW was 34.5± 0.6 mGy at 16cm FOV. The DMVD was 25.6 ± 1.1 mGy. The off-field dose was 10.5 mGy. For patients, the anterior and lateral skin doses attributable to CBCT imaging were 39.04 ± 4.4 and 27.1 ± 1.3 mGy, respectively.OSL nanoDots were convenient to use in measuring CBCT dose. The method of selecting the nanoDots greatly reduced uncertainty in the OSL measurements. Our detailed calibration procedure and CBCT dose measurements and calculations could prove useful in developing OSL routines for CBCT quality assessment, which in turn gives them the property of high spatial resolution, meaning that they have the potential for measurement of dose in regions of severe dose-gradients.

  19. Energy dependence and angular dependence of an optically stimulated luminescence dosimeter in the mammography energy range.

    Science.gov (United States)

    Kawaguchi, Ai; Matsunaga, Yuta; Suzuki, Shoichi; Chida, Koichi

    2017-03-01

    This study aimed to investigate the energy dependence and the angular dependence of commercially available optically stimulated luminescence (OSL) point dosimeters in the mammography energy range. The energy dependence was evaluated to calculate calibration factors (CFs). The half-value layer range was 0.31-0.60 mmAl (Mo/Mo 22-28 kV, Mo/Rh 28-32 kV, and W/Rh 30-34 kV at 2-kV intervals). Mo/Rh 28 kV was the reference condition. Angular dependence was tested by rotating the X-ray tube from -90° to 90° in 30° increments, and signal counts from angled nanoDots were normalized to the 0° signal counts. Angular dependence was compared with three tube voltage and target/filter combinations (Mo/Mo 26 kV, Mo/Rh 28 kV and W/Rh 32 kV). The CFs of energy dependence were 0.94-1.06. In Mo/Mo 26-28 kV and Mo/Rh 28-32 kV, the range of CF was 0.99-1.01, which was very similar. For angular dependence, the most deteriorated normalized values (Mo/Mo, 0.37; Mo/Rh, 0.43; and W/Rh, 0.58) were observed when the X-ray tube was rotated at a 90° angle, compared to 0°. The most angular dependences of ± 30°, 60°, and 90° decreased by approximately 4%, 14%, and 63% respectively. The mean deteriorated measurement 30° intervals from 0° to ± 30° was 2%, from ± 30° to ± 60° was 8%, and from ± 60° to ± 90° was 40%. The range of energy dependence in typical mammography energy range was not as much as that in general radiography and computed tomography. For accurate measurement using nanoDot, the tilt needs to be under 30°.

  20. Optically stimulated phosphorescence in quartz over the millisecond to second time scale: insights into the role of shallow traps in delaying luminescent recombination

    DEFF Research Database (Denmark)

    Ankjærgaard, Christina; Jain, Mayank

    2010-01-01

    Time-resolved optically stimulated luminescence (TR-OSL) curves from quartz are usually measured over a few hundred microseconds because this time range best illustrates the main component in quartz which lies in the range 30–45 µs. In this study we present the decay form of quartz TR-OSL and opt......Time-resolved optically stimulated luminescence (TR-OSL) curves from quartz are usually measured over a few hundred microseconds because this time range best illustrates the main component in quartz which lies in the range 30–45 µs. In this study we present the decay form of quartz TR...

  1. Application of the optically stimulated luminescence (OSL) technique for mouse dosimetry in micro-CT imaging

    Energy Technology Data Exchange (ETDEWEB)

    Vrigneaud, Jean-Marc; Courteau, Alan; Oudot, Alexandra; Collin, Bertrand [Department of Nuclear Medicine, Centre Georges-François Leclerc, 1 rue Professeur Marion, Dijon 21079 Cedex (France); Ranouil, Julien [Landauer Europe, 33 avenue du Général Leclerc, Fontenay-aux-Roses 92266 Cedex (France); Morgand, Loïc; Raguin, Olivier [Oncodesign, 20 rue Jean Mazen, Dijon 21076 Cedex (France); Walker, Paul [LE2i CNRS UMR 5158, Faculty of Medicine, BP 87900, 21079 Dijon Cedex (France); Brunotte, François [Department of Nuclear Medicine, Centre Georges-François Leclerc, 1 rue Professeur Marion, Dijon 21079 Cedex, France and LE2i CNRS UMR 5158, Faculty of Medicine, BP 87900, 21079 Dijon Cedex (France)

    2013-12-15

    Purpose: Micro-CT is considered to be a powerful tool to investigate various models of disease on anesthetized animals. In longitudinal studies, the radiation dose delivered by the micro-CT to the same animal is a major concern as it could potentially induce spurious effects in experimental results. Optically stimulated luminescence dosimeters (OSLDs) are a relatively new kind of detector used in radiation dosimetry for medical applications. The aim of this work was to assess the dose delivered by the CT component of a micro-SPECT (single-photon emission computed tomography)/CT camera during a typical whole-body mouse study, using commercially available OSLDs based on Al{sub 2}O{sub 3}:C crystals.Methods: CTDI (computed tomography dose index) was measured in micro-CT with a properly calibrated pencil ionization chamber using a rat-like phantom (60 mm in diameter) and a mouse-like phantom (30 mm in diameter). OSLDs were checked for reproducibility and linearity in the range of doses delivered by the micro-CT. Dose measurements obtained with OSLDs were compared to those of the ionization chamber to correct for the radiation quality dependence of OSLDs in the low-kV range. Doses to tissue were then investigated in phantoms and cadavers. A 30 mm diameter phantom, specifically designed to insert OSLDs, was used to assess radiation dose over a typical whole-body mouse imaging study. Eighteen healthy female BALB/c mice weighing 27.1 ± 0.8 g (1 SD) were euthanized for small animal measurements. OLSDs were placed externally or implanted internally in nine different locations by an experienced animal technician. Five commonly used micro-CT protocols were investigated.Results: CTDI measurements were between 78.0 ± 2.1 and 110.7 ± 3.0 mGy for the rat-like phantom and between 169.3 ± 4.6 and 203.6 ± 5.5 mGy for the mouse-like phantom. On average, the displayed CTDI at the operator console was underestimated by 1.19 for the rat-like phantom and 2.36 for the mouse

  2. Orbital surveys of solar stimulated luminescence

    Science.gov (United States)

    Hemphill, W. R.; Theisen, A. F.; Tyson, R. M.; Granata, J. S.

    The Fraunhofer line discriminator (FLD) is an electro-optical device for imaging natural and manmade materials which have been stimulated to luminesce by the sun. An airborne FLD has been used to detect geochemically stressed vegetation, drought-stressed agricultural crops, industrial and residential pollution effluents, marine oil seeps, phosphate rock, uranium-bearing sandstone, and bioluminescent ocean plankton. Three-dimensional perspective plots of excitation and emission spectra, measured with a laboratory spectrometer, graphically depict similarities and differences in luminescence properties between sample materials. The laboratory data also include luminescence intensities at six Fraunhofer lines in the visible and near-infrared regions of the electromagnetic spectrum. Both the airborne and laboratory data suggest the feasibility of delineating and monitoring at least some of these luminescing materials from orbital altitude, such as a test flight aboard the Space Shuttle using an improved third-generation FLD.

  3. Development of optically stimulated luminescence techniques using natural minerals and ceramics, and their application to retrospective dosimetry

    Energy Technology Data Exchange (ETDEWEB)

    Boetter-Jensen, L

    2000-09-01

    This thesis summarises research and development of optically stimulated luminescence (OSL) and its applications by the author at Risoe National Laboratory, up to 1999. These developments have been directed primarily at retrospective accident dosimetry and luminescence dating. Experimental investigations include the studies of OSL properties of the natural minerals quartz and feldspars and the artificial materials porcelain and aluminium oxide (Al{sub 2}O{sub 3}). Blue light emitting diodes and infrared laser diodes are shown to provide simple and practical alternatives to broad-band light and visible laser stimulation. The development of OSL apparatus designed for the rapid measurement of single grains of phosphors also opens up a new area of luminescence measurement, allowing the detailed examination of dose distributions within a multiple-grain sample. This is of particular importance to the studies of incompletely reset geological sediments, and to accident dosimetry measurements using unheated materials. Al{sub 2}O{sub 3}:C single crystals are tested as environmental OSL dosemeters for assessing both the natural background photon radiation dose rates in the field and the natural dose rates inside bricks collected for accident dose evaluation. Environmental doses of the order of few {mu}Gy are measured with high precision. UV photo-stimulated luminescence spectra obtained from porcelain samples are used to confirm that the main component responsible for the OSL signal from porcelain is Al{sub 2}O{sub 3}. OSL single-aliquot regenerative-dose (SAR) techniques are used with quartz extracted from Chernobyl bricks to determine the accrued dose after the accident. This has improved the measurement precision significantly, from about 5-6 % using traditional methods to now less than 2 %. Depth-dose profiles measured in Chernobyl bricks are compared with those obtained in the laboratory using different gamma sources and these comparisons show that the average energy of

  4. Optical, scintillation and thermally stimulated luminescence properties of Ce-doped yttrium-aluminum-indium garnet

    Science.gov (United States)

    Mori, Masaki; Okada, Go; Kawaguchi, Noriaki; Yanagida, Takayuki

    2017-01-01

    We have investigated the photoluminescence (PL), scintillation and thermally stimulated luminescence (TSL) properties of 1 mol % Ce-doped Y3(Al X In1- X )5O12 (X = 0-1 Ce:YAING). These samples showed strong and broad PL emission by Ce3+ ion appeared in the spectral range from 480 to 620 nm. The PL decay profiles can be represented by a first-order exponential function with the decay time ranging 39-62 ns. Furthermore, the scintillation spectra showed similar features with those observed in PL. The scintillation decay time profiles were approximated by second or third order exponential decay functions, and we observed 26-61 ns component due to Ce3+ emission. The X-ray induced afterglow levels of Ce:YAING were worse than that of Ce:Y3Al5O12. The pulse height spectra of Ce:Y3(Al0.26In0.74)5O12 showed a clear photoabsorption peak, and that of the scintillation light yield was around 6,700 photons/MeV. In TSL glow curves, Ce:YAING show the glow peak at around 110 °C.

  5. An assessment of cumulative external doses from Chernobyl fallout for a forested area in Russia using the optically stimulated luminescence from quartz inclusions in bricks

    DEFF Research Database (Denmark)

    Ramzaev, V.; Bøtter-Jensen, Lars; Thomsen, Kristina Jørkov

    2008-01-01

    Optically stimulated luminescence (OSL) has been used for estimation of the accumulated doses in quartz inclusions obtained from two fired bricks, extracted in July 2004 from a building located in the forested surroundings of the recreational area Novie Bobovichi, the Bryansk Region, Russia...

  6. Dose response of commercially available optically stimulated luminescent detector, Al2O3:C for megavoltage photons and electrons.

    Science.gov (United States)

    Kim, Dong Wook; Chung, Weon Kuu; Shin, Dong Oh; Yoon, Myonggeun; Hwang, Ui-Jung; Rah, Jeong-Eun; Jeong, Hojin; Lee, Sang Yeob; Shin, Dongho; Lee, Se Byeong; Park, Sung Yong

    2012-04-01

    This study examined the dose response of an optically stimulated luminescence dosemeter (OSLD) to megavoltage photon and electron beams. A nanoDot™ dosemeter was used to measure the dose response of the OSLD. Photons of 6-15 MV and electrons of 9-20 MeV were delivered by a Varian 21iX machine (Varian Medical System, Inc. Milpitas, CA, USA). The energy dependency was photons, the dose was linear until 200 cGy. The superficial dose measurements revealed photon irradiation to have an angular dependency. The nanoDot™ dosemeter has potential use as an in vivo dosimetric tool that is independent of the energy, has dose linearity and a rapid response compared with normal in vivo dosimetric tools, such as thermoluminescence detectors. However, the OSLD must be treated very carefully due to the high angular dependency of the photon beam.

  7. Study of optically stimulated luminescence (OSL) for radiation detection. Application to an optical fibre {gamma}-radiation sensor; Etude de la luminescence stimulee optiquement (OSL) pour la detection de rayonnements: application a un capteur a fibre optique de rayonnement {gamma}

    Energy Technology Data Exchange (ETDEWEB)

    Roy, O. [CEA Saclay, 91 - Gif-sur-Yvette (France). Dept. d`Electronique et d`Instrumentation Nucleaire]|[Paris-7 Univ., 75 (France)

    1998-12-31

    This work shows up the usefulness of the Optically Stimulated Luminescence (OSL) to resolve radioprotection problems. We study the use of OSL as a gamma dosimetric technique with respect to the ALARA`s concept (As Low As Reasonably Achievable). A new approach based on optical fibers and luminescent materials showing OSL properties (closely related to Thermoluminescence phenomena) is presented in order to improve the remote real time dosimetry monitoring. Like thermoluminescent materials (TLD), OSL materials can trap charges under an irradiation (UV, X, {gamma},...). Instead of heating, the charges trapped are released by light stimulation and produce a visible luminescence which amount is proportional to trap the `data stored` left by irradiation, enabling the dose measurement. The OSL phenomenon offers the same advantages as TLD plus the interesting possibility of a remote optical stimulation. The end-user objective deals with the development of a {gamma}-radiation Optical FIber Sensor (OFS) for dose measurement which can offer new functionalities based on OSL materials coupled with an optical fiber. Rare earth doped Alkaline Earth Sulphides (AES), BAFX:EU{sup 2+} (X = Cl, Br, I) and halogen alkaline have been studied (crystalline form, synthesis techniques, influence of dopants and color centers). Their characteristics are presented and extensively discussed. A specific experimental set-up to characterise various OSL phosphors has been developed. It allows the study of sensitivity, linearity, time decay behaviour of OSL signal and zeroing time. A joint study of OSL and TL has shown the technical limitations as well as the thermal fading and the origin of the long zeroing time. An Optical Fiber Sensor (OFS) based on OSL and using MgS:Sm has been developed for practical applications on nuclear fields. Its specifications are presented and discussed, moreover improvements are proposed. (author) 320 refs.

  8. Thermoluminescence, luminescence optically stimulated and creation of defects in alkaline halogenides contaminated with Europium; Termoluminiscencia, luminiscencia opticamente estimulada y creacion de defectos en halogenuros alcalinos contaminados con Europio

    Energy Technology Data Exchange (ETDEWEB)

    Barboza F, M. [Centro de Investigacion en Fisica, Universidad de Sonora, Apartado Postal 5-088, 83190 Hermosillo, Sonora (Mexico)

    1999-07-01

    The alkaline halogenides have been subject matter of investigations related with the search of sensor materials for X-ray bidimensional images or optical memories. The understanding of the damage formation processes generated by ionizing and non-ionizing radiations is important for the correct design of devices that working as detectors and dosemeters of both type of radiations. In this work we present the investigation results related with the defects produced by the ionizing radiation type X and ultraviolet light in the range of 200-360 nm in crystals of KCl: Eu{sup 2+} and KBr:Eu{sup 2+}. It is examined the thermoluminescence and luminescence spectra with the purpose of identifying the exciton processes, owing to the excitation of the halogenide ions in which the primary defects correspond to the F and H centers. It has been found that the 400-600 nm emission is associated with the luminescence type that in his turn can be associated with autotrapped excitons perturbed by the impurity. On the other hand, it is examined the emission spectra of the luminescence optically stimulated in crystals of KBr: Eu{sup 2+} and KCl: Eu{sup 2+} finding too that such materials would be used as optical memories susceptible of to store information, and through of photostimulation to read this. It was determined that the F centers participate in the luminescence optically stimulated in these crystals, as well as too in the recombination processes responsible by the thermoluminescent emission. (Author)

  9. Luminescence from potassium feldspars stimulated by infrared and green light

    DEFF Research Database (Denmark)

    Duller, G.A.T.; Bøtter-Jensen, L.

    1993-01-01

    A series of experiments are reported which investigate stimulated luminescence from potassium feldspar. The aim is to provide a basic phenomenological description of the response of the material to stimulation by heat, infrared radiation (875 DELTA 80 nm) and a green light wavelength band from 5 15...... to 560 nm. Two conclusions are drawn: firstly it is suggested that the majority of the trapped charge responsible for the infrared stimulated luminescence signal does not give rise to a thermoluminescence signal, and secondly that a large traction of the two optically stimulated luminescence signals...

  10. Optically stimulated luminescence of Tb{sup 3+}/Sm{sup 3+} doubly doped K{sub 2}YF{sub 5} single crystals

    Energy Technology Data Exchange (ETDEWEB)

    Camargo, L.; Marcazzo, J.; Santiago, M.; Caselli, E. [Universidad Nacional del Centro de la Provincia de Buenos Aires, Instituto de Fisica Arroyo Seco, Gral. Pinto 399, B7000GHG, Tandil (Argentina); Khaidukov, N. M., E-mail: jmarcass@exa.unicen.edu.ar [Kurnakov Institute of General and Inorganic Chemistry, RAS, Leninskii Prospekt 31, 119991 Moscow (Russian Federation)

    2014-08-15

    In this work optically stimulated luminescence (OSL) properties of K{sub 2}YF{sub 5} crystals doubly doped with Tb{sup 3+} and Sm{sup 3+} ions have been investigated for the first time. OSL responses for different dopant concentration and for optical stimulation with different wavelengths have been analyzed for each compound. Dosimetric properties of the most efficient composition, namely, K{sub 2}YF{sub 5}:1.0 at.% Tb{sup 3+}; 1.0 at.% Sm{sup 3+}, have been studied. Finally, the possible application of this single crystal as OSL dosimeter has been evaluated. (Author)

  11. Optically stimulated phosphorescence in quartz over the millisecond to second time scale: insights into the role of shallow traps in delaying luminescent recombination

    DEFF Research Database (Denmark)

    Ankjærgaard, Christina; Jain, Mayank

    2010-01-01

    Time-resolved optically stimulated luminescence (TR-OSL) curves from quartz are usually measured over a few hundred microseconds because this time range best illustrates the main component in quartz which lies in the range 30–45 µs. In this study we present the decay form of quartz TR......-OSL and optically stimulated phosphorescence (OSP) covering over 8 orders of magnitude from 50 ns to ~8 s. A detailed characterization of the previously unstudied slowly decaying signals (millisecond–second time scales) is undertaken to understand the origin of these components and the role of re-trapping following...... optical stimulation. We present preheat and stimulation temperature dependence for both the TR-OSL and OSP curves in these time ranges and use the latter data to determine the E and s values for the participating shallow traps. We observe an abnormal decay behaviour seen as a sudden increase in the decay...

  12. Identification of defects responsible for optically stimulated luminescence (OSL) from copper-diffused LiAlO{sub 2} crystals

    Energy Technology Data Exchange (ETDEWEB)

    Holston, M.S.; Ferguson, I.P.; Giles, N.C.; McClory, J.W. [Department of Engineering Physics, Air Force Institute of Technology, Wright-Patterson Air Force Base, OH 45433 (United States); Halliburton, L.E., E-mail: Larry.Halliburton@mail.wvu.edu [Department of Physics and Astronomy, West Virginia University, Morgantown, WV 26506 (United States)

    2015-08-15

    A large optically stimulated luminescence (CW-OSL) response has been observed from bulk lithium aluminate (LiAlO{sub 2}) crystals that have been copper-diffused. After introducing the copper, an optical absorption band peaking at 277 nm is present and is assigned to Cu{sup +} (3d{sup 10}) ions at Li{sup +} sites. Photoluminescence (PL and PLE) from copper-diffused samples shows an emission band near 359 nm and an excitation band near 273 nm. These PL bands are also assigned to the Cu{sup +} ions. After an irradiation at room temperature with x-rays, the copper-diffused crystals give an intense OSL signal when stimulated with light in the 425–500 nm region. The OSL emitted light has a peak near 357 nm and thus is directly associated with recombination at a Cu ion. Electron paramagnetic resonance (EPR) shows that the x-rays produce two distinct Cu{sup 2+} (3d{sup 9}) centers, both at Li{sup +} sites. One of the trapped-hole centers is a Cu{sup 2+} with no nearby defects and the other is a Cu{sup 2+} with a neighboring Li{sup +} vacancy. Monitoring the EPR spectra before and after OSL shows that only the isolated Cu{sup 2+} ions (i.e., those with no nearby defect) participate in the OSL process. The electron traps participating in the OSL are shown with EPR to be transition-metal ions that are unintentionally present. Specifically, Fe{sup 2+} ions replacing Li{sup +} ions, possibly with a nearby lithium vacancy, convert to Fe{sup +} (3d{sup 7}) ions when they trap an electron during irradiation. These electrons are optically released by the OSL exciting light and migrate to the holes trapped as isolated Cu{sup 2+} ions, where electron–hole recombination gives the characteristic Cu{sup +} emission. By combining OSL, PL, and EPR, we establish the general OSL mechanism in copper-diffused LiAlO{sub 2} crystals. - Highlights: • Copper is diffused into LiAlO{sub 2} crystals at high temperature. • Cu{sup +} ions at Li{sup +} sites cause PL at 359 nm and PLE at 273 nm

  13. Characterization of Al2O3 optically stimulated luminescence films for 2D dosimetry using a 6 MV photon beam

    Science.gov (United States)

    Ahmed, M. F.; Shrestha, N.; Schnell, E.; Ahmad, S.; Akselrod, M. S.; Yukihara, E. G.

    2016-11-01

    This work evaluates the dosimetric properties of newly developed optically stimulated luminescence (OSL) films, fabricated with either Al2O3:C or Al2O3:C,Mg, using a prototype laser scanning reader, a developed image reconstruction algorithm, and a 6 MV therapeutic photon beam. Packages containing OSL films (Al2O3:C and Al2O3:C,Mg) and a radiochromic film (Gafchromic EBT3) were irradiated using a 6 MV photon beam using different doses, field sizes, with and without wedge filter. Dependence on film orientation of the OSL system was also tested. Diode-array (MapCHECK) and ionization chamber measurements were performed for comparison. The OSLD film doses agreed with the MapCHECK and ionization chamber data within the experimental uncertainties (response was approximately linear from the MDD up to a few grays (the linearity correction was  response, resolution and dosimetric properties. The negligible background and potential simple calibration make these OSLD films suitable for remote audits. The characterization presented here may motivate further commercial development of a 2D dosimetry system based on the OSL from Al2O3:C or Al2O3:C,Mg.

  14. Detection of herbs and spices irradiated through optically stimulated luminescence; Deteccion de hierbas y especias irradiadas mediante luminiscencia opticamente estimulada

    Energy Technology Data Exchange (ETDEWEB)

    Preciado, S.; Agundez A, Z.; Barboza F, M. [Centro de Investigacion en Fisica, Universidad de Sonora, A.P. 5-088, 83190 Hermosillo, Sonora (Mexico); Cruz Z, E. [Instituto de Ciencias Nucleares de la UNAM, 04510 Mexico D.F. (Mexico)

    2003-07-01

    The irradiation of foods is one of the common practices in several countries of the American and European continents. In spite of the widespread use of irradiation methods and technics of nutritious products, it doesn't exist a method of general use at the present time for the detection of previously submitted foods to irradiation with pasteurization ends or sterilization. In the present work the results are presented obtained in the detection of herbs and spices exposed to radiation in the range of 0.1 - 3 KGy, by means of the photostimulation with light of 470 nm. It was used for it a RIS0 model team TL/OSL-GIVE-15 conditioned with a {beta} ray source, {sup 90}Sr/{sup 90}Y and a source of light of 50 mW/cm2. samples of chili guajillo were studied, pepper, cumin, mint and camomile; achieving you to detect exhibitions of the order of 8.33x10{sup -4} KGy that which is indicative of the high sensitivity of the luminescence technique optically stimulated. The answer of the samples with regard to the radiation dose presents a range of lineality for low dose of the order of 0.5 KGy; and supralineal for further dose without to arrive to a saturation stage. (Author)

  15. A new flexible system for measuring thermally and optically stimulated luminescence

    DEFF Research Database (Denmark)

    Markey, B.G.; Bøtter-Jensen, L.; Duller, G.A.T.

    1997-01-01

    The automated Riso TL/OSL reader system is used worldwide for luminescence dating, retrospective dosimetry environmental dosimetry and material characterization. In response to requests from many users we have re-designed the reader by incorporating a variety of new hardware and software features....... New hardware features include a two-speed sample turntable, a new detachable beta irradiator with a Be window vacuum interface and the incorporation of an on-board minicomputer.,A completely new software concept was developed that allows the user unlimited control of the reader and has, at the same...... time, made the new generation Riso TL/OSL readers extremely flexible and user friendly. A description of the new system is given and measurement results are presented to demonstrate its capabilities. (C) 1997 Elsevier Science Ltd....

  16. Characteristics of thermally transferred optically stimulated luminescence (TT-OSL) in quartz and its potential for dating sediments

    Energy Technology Data Exchange (ETDEWEB)

    Tsukamoto, Sumiko [Institute of Geography and Earth Sciences, Aberystwyth University, Aberystwyth SY23 3DB (United Kingdom); Duller, Geoff A.T. [Institute of Geography and Earth Sciences, Aberystwyth University, Aberystwyth SY23 3DB (United Kingdom)], E-mail: ggd@aber.ac.uk; Wintle, Ann G. [Institute of Geography and Earth Sciences, Aberystwyth University, Aberystwyth SY23 3DB (United Kingdom)

    2008-08-15

    The temperature dependence, dose response and bleaching characteristics of the thermally transferred optically stimulated luminescence (TT-OSL) of sedimentary quartz were studied, in order to assess the potential of the TT-OSL signal for dating. The TT-OSL was separated into two components; recuperated OSL (ReOSL) and basic transfer (BT-OSL) by annealing samples at 300 deg. C for 10 s as suggested in an earlier study. Four quartz extracts were studied, two from loess from China and two from coastal sands from South Africa. The equivalent doses of the two recent samples (one sand and one loess) were {approx}15Gy and this suggests that the signal can be bleached by sunlight but may not be totally zeroed. The sensitivity-corrected ReOSL from the older samples did not reach zero and gave doses of 14 and 52 Gy, respectively, after 7 days bleaching with a solar simulator. A single aliquot regenerative dose (SAR) protocol using ReOSL was proposed and tested. In this protocol, a blue light stimulation at 280 deg. C for 100 s at the end of each cycle resulted in the recovery of identical sensitivity-corrected ReOSL values, in spite of {approx}20 -30% loss in sensitivity for the four samples that were tested. Two dose response curves were constructed using the sensitivity-corrected ReOSL, one for the initial 2 s signal and the other for the fast component obtained by curve fitting. Using the additional high temperature bleach and the separated fast component of the ReOSL, it was possible to recover given doses within 10%, up to {approx}1000Gy for the loess and {approx}2000Gy for the coarse grained quartz. However, the natural dose obtained for the older sand was twice that obtained using the conventional SAR OSL method.

  17. Optically stimulated luminescence age controls on late Pleistocene and Holocene coastal lithosomes, North Carolina, USA

    Science.gov (United States)

    Mallinson, D.; Burdette, K.; Mahan, S.; Brook, G.

    2008-01-01

    Luminescence ages from a variety of coastal features on the North Carolina Coastal Plain provide age control for shoreline formation and relative sea-level position during the late Pleistocene. A series of paleoshoreline ridges, dating to Marine Isotope Stage (MIS) 5a and MIS 3 have been defined. The Kitty Hawk beach ridges, on the modern Outer Banks, yield ages of 3 to 2??ka. Oxygen-isotope data are used to place these deposits in the context of global climate and sea-level change. The occurrence of MIS 5a and MIS 3 shorelines suggests that glacio-isostatic adjustment (GIA) of the study area is large (ca. 22 to 26??m), as suggested and modeled by other workers, and/or MIS 3 sea level was briefly higher than suggested by some coral reef studies. Correcting the shoreline elevations for GIA brings their elevation in line with other sea-level indicators. The age of the Kitty Hawk beach ridges places the Holocene shoreline well west of its present location at ca. 3 to 2??ka. The age of shoreline progradation is consistent with the ages of other beach ridge complexes in the southeast USA, suggesting some regionally contemporaneous forcing mechanism. ?? 2007 University of Washington.

  18. Determination of average LET of therapeutic proton beams using Al2O3:C optically stimulated luminescence (OSL) detectors.

    Science.gov (United States)

    Sawakuchi, Gabriel O; Sahoo, Narayan; Gasparian, Patricia B R; Rodriguez, Matthew G; Archambault, Louis; Titt, Uwe; Yukihara, Eduardo G

    2010-09-07

    In this work we present a methodology and proof of concept to experimentally determine average linear energy transfer (LET) of therapeutic proton beams using the optically stimulated luminescence (OSL) of small Al(2)O(3):C detectors. Our methodology is based on the fact that the shape of the OSL decay curve of Al(2)O(3):C detectors depends on the LET of the radiation field. Thus, one can use the shape of the OSL decay curves to establish an LET calibration curve, which in turn permits measurements of LET. We performed irradiations at the M D Anderson Cancer Center Proton Therapy Center, Houston (PTCH), with passive scattering beams. We determined the average LET of the passive scattering beams using a validated Monte Carlo model of the PTCH passive scattering nozzle and correlated them with the shape of the OSL decay curve to obtain an LET calibration curve. Using this calibration curve and OSL measurements, we determined the averaged LET at various water-equivalent depths for therapeutic spread-out Bragg peaks and compared the results with averaged LETs determined using the Monte Carlo simulations. Agreement between measured and simulated fluence-averaged LET was within 24% for low energy spread-out Bragg peak (SOBP) fields and within 14% for high energy SOBP fields. Agreement between measured and simulated dose-averaged LET was within 12% for low energy SOBP fields and within 47% for high energy SOBP fields. The data presented in this work demonstrated the correlation between the OSL decay curve shapes and the average LET of the radiation fields, providing proof of concept of the feasibility of using OSL from Al(2)O(3):C detectors to measure average LET of therapeutic proton beams.

  19. SU-E-T-600: In Vivo Dosimetry for Total Body and Total Marrow Irradiations with Optically Stimulated Luminescence Dosimeters

    Energy Technology Data Exchange (ETDEWEB)

    Niedbala, M; Save, C [The Ottawa Hospital Cancer Ctr., Ottawa, ON (Canada); Cygler, J [The Ottawa Hospital Cancer Ctr., Ottawa, ON (Canada); University of Ottawa (Canada); Carleton University (Canada)

    2014-06-01

    Purpose: To evaluate the feasibility of using optically stimulated luminescence dosimeters (OSLDs) for in-vivo dosimetry of patients undergoing Total Body and Total Marrow Irradiations (TBI and TMI). Methods: TBI treatments of 12 Gy were delivered in 6 BID fractions with the patient on a moving couch under a static 10 MV beam (Synergy, Elekta). TMI treatments of 18 Gy in 9 BID fractions were planned and delivered using a 6 MV TomoTherapy unit (Accuray). To provide a uniform dose to the entire patient length, the treatment was split into 2 adjacent fields junctioned in the thigh region. Our standard clinical practice involves in vivo dosimetry with MOSFETs for each TBI fraction and TLDs for at least one fraction of the TMI treatment for dose verification. In this study we also used OSLDs. Individual calibration coefficients were obtained for the OSLDs based on irradiations in a solid water phantom to the dose of 50 cGy from Elekta Synergy 10 MV (TBI) and 6 MV (TMI) beams. Calibration coefficients were calculated based on the OSLDs readings taken 2 hrs post-irradiation. For in vivo dosimetry OSLDs were placed alongside MOSFETs for TBI patients and in approximately the same locations as the TLDs for TMI patients. OSLDs were read 2 hours post treatment and compared to the MOSFET and TLD results. Results: OSLD measured doses agreed within 5% with MOSFET and TLD results, with the exception of the junction region in the TMI patient due to very high dose gradient and difficulty of precise and reproducible detector placement. Conclusion: OSLDs are useful for in vivo dosimetry of TBI and TMI patients. The quick post-treatment readout is an advantage over TLDs, allowing the results to be obtained between BID fractions, while wireless detectors are advantageous over MOSFETs for treatments involving a moving couch.

  20. Evaluation of an X-Ray Dose Profile Derived from an Optically Stimulated Luminescent Dosimeter during Computed Tomographic Fluoroscopy.

    Directory of Open Access Journals (Sweden)

    Hiroaki Hasegawa

    Full Text Available The purpose of this study was to evaluate scatter radiation dose to the subject surface during X-ray computed tomography (CT fluoroscopy using the integrated dose ratio (IDR of an X-ray dose profile derived from an optically stimulated luminescent (OSL dosimeter. We aimed to obtain quantitative evidence supporting the radiation protection methods used during previous CT fluoroscopy. A multislice CT scanner was used to perform this study. OSL dosimeters were placed on the top and the lateral side of the chest phantom so that the longitudinal direction of dosimeters was parallel to the orthogonal axis-to-slice plane for measurement of dose profiles in CT fluoroscopy. Measurement of fluoroscopic conditions was performed at 120 kVp and 80 kVp. Scatter radiation dose was evaluated by calculating the integrated dose determined by OSL dosimetry. The overall percent difference of the integrated doses between OSL dosimeters and ionization chamber was 5.92%. The ratio of the integrated dose of a 100-mm length area to its tails (-50 to -6 mm, 50 to 6 mm was the lowest on the lateral side at 80 kVp and the highest on the top at 120 kVp. The IDRs for different measurement positions were larger at 120 kVp than at 80 kVp. Similarly, the IDRs for the tube voltage between the primary X-ray beam and scatter radiation was larger on the lateral side than on the top of the phantom. IDR evaluation suggested that the scatter radiation dose has a high dependence on the position and a low dependence on tube voltage relative to the primary X-ray beam for constant dose rate fluoroscopic conditions. These results provided quantitative evidence supporting the radiation protection methods used during CT fluoroscopy in previous studies.

  1. High resolution optically stimulated luminescence dating of a sediment core from the southwestern Sea of Okhotsk

    DEFF Research Database (Denmark)

    Sugisaki, S.; Buylaert, J. P.; Murray, A. S.;

    2012-01-01

    in application to a 19 m marine sediment core (MR0604-PC04A) taken from the southwestern Sea of Okhotsk, immediately to the north of Hokkaido, Japan. Fine-grained quartz (4 to 11 mu m) was chosen as the dosimeter, and a single-aliquot regenerative-dose protocol was used for the determination of equivalent dose...... (D-e), with stimulation by both infrared and blue light. The suitability of the measurement procedure was confirmed using dose recovery tests. A high resolution record (similar to 2 OSL ages/m) identified clear sedimentation rate changes down the core. The OSL ages are significantly dependent...

  2. Luminescence Instrumentation

    DEFF Research Database (Denmark)

    Jain, Mayank; Bøtter-Jensen, Lars

    2014-01-01

    This chapter gives an introduction to instrumentation for stimulated luminescence studies, with special focus on luminescence dating using the natural dosimeters, quartz and feldspars. The chapter covers basic concepts in luminescence detection, and thermal and optical stimulation, and reference...

  3. Thermally and optically stimulated luminescence in long persistent orthorhombic strontium aluminates doped with Eu, Dy and Eu, Nd

    Science.gov (United States)

    Zúñiga-Rivera, N. J.; Salas-Castillo, P.; Chernov, V.; Díaz-Torres, L. A.; Meléndrez, R.; García-Gutierrez, R.; Carrillo-Torres, R. C.; Barboza-Flores, M.

    2017-05-01

    The long persistent luminescence, thermoluminescence (TL) and IR stimulated luminescence properties of two orthorhombic strontium aluminates (Sr4Al14O25) co-doped with Eu2+, Dy3+ and Eu2+, Nd3+ exposed to beta radiation is reported. The phosphors were synthesized by the combustion method followed by a post-annealing treatment under a reductive carbon atmosphere. Photoluminescence emission spectra of both phosphors are typical for emission of Eu2+ ions with 7-fold and 10-fold coordination in Sr4Al14025 and consist of the main band at 480 nm and a weak band between 390 and 440 nm. After exposure to beta radiation the Sr4Al14025:Eu2+,Dy3+ phosphor exhibits two strongly overlapped TL peaks at about 70 and 100 °C while the low temperature TL of the Sr4Al14025:Eu2+,Nd3+ phosphor consist of two well separated peaks with maxima at about 60 and 130 °C. Additionally, both phosphors exhibit a weak TL between 180 and 400 °C. The traps responsible for the low temperature TL peaks are the Dy3+ and Nd3+ centers situated in two different Sr sites with 7-fold and 10-fold coordination. The thermal emptying of the Dy and Nd filled traps creates ultra-long intense afterglow, which gradually decays with time and remains detectable after 220 h storage in dark. IR stimulation of beta irradiated phosphors creates intense IR stimulated luminescence, which is related to the release of electrons from the filled Dy and Nd traps.

  4. Angular dependence of dose sensitivity of nanoDot optically stimulated luminescent dosimeters in different radiation geometries

    Energy Technology Data Exchange (ETDEWEB)

    Jursinic, Paul A., E-mail: pjursinic@wmcc.org [West Michigan Cancer Center, 200 North Park Street, Kalamazoo, Michigan 49007 (United States)

    2015-10-15

    Purpose: A type of in vivo dosimeter, an optically stimulated luminescent dosimeter, OSLD, may have dose sensitivity that depends on the angle of incidence of radiation. This work measures how angular dependence of a nanoDot changes with the geometry of the phantom in which irradiation occurs and with the intrinsic structure of the nanoDot. Methods: The OSLDs used in this work were nanoDot dosimeters (Landauer, Inc., Glenwood, IL), which were read with a MicroStar reader (Landauer, Inc., Glenwood, IL). Dose to the OSLDs was delivered by 6 MV x-rays. NanoDots with various intrinsic sensitivities were irradiated in numerous phantoms that had geometric shapes of cylinders, rectangles, and a cube. Results: No angular dependence was seen in cylindrical phantoms, cubic phantoms, or rectangular phantoms with a thickness to width ratio of 0.3 or 1.5. An angular dependence of 1% was observed in rectangular phantoms with a thickness to width of 0.433–0.633. A group of nanoDots had sensitive layers with mass density of 2.42–2.58 g/cm{sup 3} and relative sensitivity of 0.92–1.09 and no difference in their angular dependence. Within experimental uncertainty, nanoDot measurements agree with a parallel-plate ion chamber at a depth of maximum dose. Conclusions: When irradiated in cylindrical, rectangular, and cubic phantoms, nanoDots show a maximum angular dependence of 1% or less at an incidence angle of 90°. For a sample of 78 new nanoDots, the range of their relative intrinsic sensitivity is 0.92–1.09. For a sample of ten nanoDots, on average, the mass in the sensitive layer is 73.1% Al{sub 2}O{sub 3}:C and 26.9% polyester. The mass density of the sensitive layer of a nanoDot disc is between 2.42 and 2.58 g/cm{sup 3}. The angular dependence is not related to Al{sub 2}O{sub 3}:C loading of the nanoDot disc. The nanoDot at the depth of maximum dose has no more angular dependence than a parallel-plate ion chamber.

  5. Optically stimulated luminescence of ZnO obtained by thermal treatment of ZnS chemically synthesized; Luminiscencia opticamente estimulada de ZnO obtenido por tratamiento termico de ZnS sintetizado quimicamente

    Energy Technology Data Exchange (ETDEWEB)

    Cruz V, C.; Burruel I, S.E.; Orante B, V.R.; Grijalva M, H.; Perez S, R.; Bernal, R. [Universidad de Sonora, A.P. 130, Hermosillo (Mexico)

    2005-07-01

    In this work, we report the optically stimulated luminescence (OSL) dosimetry of new nano phosphors of ZnO obtained by thermal annealing of chemically synthesized ZnS powder. The synthesized ZnS nano powder was compressed in order to form pellet shaped pellets, which were afterwards subjected to a thermal annealing at 700 C during 24 h under air atmosphere. X-ray diffraction (XRD) patterns and energy-disperse X-ray Spectrometry (EDS) analyses confirmed the transformation of ZnS to ZnO. Samples were exposed to several doses of beta radiation up to 600 Gy, and the optically stimulated luminescence with 470 nm wavelength light was recorded as a function of dose. The intensity of the OSL signal increases by increasing dose, for what it is concluded that these new phosphor materials are suitable to be used in optically stimulated luminescence dosimetry. (Author)

  6. High resolution shallow geologic characterization of a late Pleistocene eolian environment using ground penetrating radar and optically stimulated luminescence techniques: North Carolina, USA

    Science.gov (United States)

    Mallinson, D.; Mahan, S.; Moore, Christine

    2008-01-01

    Geophysical surveys, sedimentology, and optically-stimulated luminescence age analyses were used to assess the geologic development of a coastal system near Swansboro, NC. This area is a significant Woodland Period Native American habitation and is designated the "Broad Reach" archaeological site. 2-d and 3-d subsurface geophysical surveys were performed using a ground penetrating radar system to define the stratigraphic framework and depositional facies. Sediment samples were collected and analyzed for grain-size to determine depositional environments. Samples were acquired and analyzed using optically stimulated luminescence techniques to derive the depositional age of the various features. The data support a low eolian to shallow subtidal coastal depositional setting for this area. Li-DAR data reveal ridge and swale topography, most likely related to beach ridges, and eolian features including low-relief, low-angle transverse and parabolic dunes, blowouts, and a low-relief eolian sand sheet. Geophysical data reveal dominantly seaward dipping units, and low-angle mounded features. Sedimentological data reveal mostly moderately-well to well-sorted fine-grained symmetrical to coarse skewed sands, suggesting initial aqueous transport and deposition, followed by eolian reworking and bioturbation. OSL data indicate initial coastal deposition prior to ca. 45,000 yBP, followed by eolian reworking and low dune stabilization at ca. 13,000 to 11,500 yBP, and again at ca. 10,000 yBP (during, and slightly after the Younger Dryas chronozone).

  7. Retrospective assessment of environmental dose rates using optically stimulated luminescence from Al2O3:C and quartz

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.; Banerjee, D.; Jungner, H.;

    1999-01-01

    As part of our continuing work on assessing the usefulness of natural and artificial dosemeters in retrospective accident dosimetry, the natural photon dose rates within bricks have been measured using the optically stimulated luminescence (OSL) from Al2O3:C single crystal dosemeters. These were...... placed in bricks in house walls for two weeks to integrate the environmental dose rates after which their OSL signals were measured. These results were compared with (1) OSL measurements of quartz samples extracted from the bricks and (2) dose rates determined from laboratory measurements of the natural...... crystals distributed in holes across a brick section and (2) quartz (extracted from the matrix of the brick) taken across the same section. These were compared with typical depth dose profiles found in bricks collected in the Chernobyl accident area and demonstrate retrospectively that the average energy...

  8. Investigation on heat sterilization of BeO-detectors for optical stimulated luminescence (OSL); Untersuchungen zur Hitzesterilisation von BeO-Detektoren fuer die optisch stimulierte Lumineszenz (OSL)

    Energy Technology Data Exchange (ETDEWEB)

    Schwarz, W.; Piehler, S.; Burgkhardt, B. [Duale Hochschule Baden-Wuerttemberg (DHBW), Karlsruhe (Germany). Sicherheitswesen

    2015-07-01

    BeO-Detectors show a high thermal stability when optically stimulated luminescence is measured. With respect to steam sterilization of extremity dosimeters in medicine this paper investigates the effect of heat treatments on the response at commonly used temperatures of 121 C and 134 C. A commercial OSL-dosimetry system with BeO detectors uses dosimeter trays made of none-heat resistant plastic. The detectors are welded with the tray. Constructing a tray which allowed the detectors to be taken out was essential to perform heat treatments in heat resistant holders. Up to 20 simulated heat treatments at 121 C as well as irradiations of one dosimeter during one month resulted in small changes of the detector response, within ±10%. Similar results were shown by one irradiation and one summed up heat treatment at 121 C and 134 C. This is also true for the characteristics of the response vs. time of the heat treatment.

  9. Dating human occupation at Toca do Serrote das Moendas, São Raimundo Nonato, Piauí-Brasil by electron spin resonance and optically stimulated luminescence.

    Science.gov (United States)

    Kinoshita, Angela; Skinner, Anne R; Guidon, Niede; Ignacio, Elaine; Felice, Gisele Daltrini; Buco, Cristiane de A; Tatumi, Sonia; Yee, Márcio; Figueiredo, Ana Maria Graciano; Baffa, Oswaldo

    2014-12-01

    Excavation of Toca do Serrote das Moendas, in Piauí state, Brazil revealed a great quantity of fossil wild fauna associated with human remains. In particular, fossils of a cervid (Blastocerus dichotomus) were found, an animal frequently pictured in ancient rock wall paintings. In a well-defined stratum, two loose teeth of this species were found in close proximity to human bones. The teeth were independently dated by electron spin resonance (ESR) in two laboratories. The ages obtained for the teeth were 29 ± 3 ka (thousands of years) and 24 ± 1 ka. The concretion layer capping this stratum was dated by optically stimulated luminescence (OSL) of the quartz grains to 21 ± 3 ka. As these values were derived independently in three different laboratories, using different methods and equipment, these results are compelling evidence of early habitation in this area.

  10. Energy levels in YPO{sub 4}:Ce{sup 3+},Sm{sup 3+} studied by thermally and optically stimulated luminescence

    Energy Technology Data Exchange (ETDEWEB)

    Bos, Adrie J.J., E-mail: a.j.j.bos@tudelft.n [Delft University of Technology, Mekelweg 15, NL 2629 JB Delft (Netherlands); Poolton, Nigel R.J. [Delft University of Technology, Mekelweg 15, NL 2629 JB Delft (Netherlands); Institute of Maths and Physics, Aberystwyth University, Aberystwyth SY23 3BZ (United Kingdom); Wallinga, Jakob [Netherlands Centre for Luminescence Dating, Delft University of Technology, Mekelweg 15, NL 2629 JB Delft (Netherlands); Bessiere, Aurelie [Ecole Nat. Superieure de Chimie de Paris, 11 Rue P et M Curie, 75231 Paris Cedex 05 (France); Dorenbos, Pieter [Delft University of Technology, Mekelweg 15, NL 2629 JB Delft (Netherlands)

    2010-03-15

    Energy-resolved optically stimulated luminescence (OSL) spectra and thermoluminescence (TL) glow curves of a powder sample of YPO{sub 4}:Ce{sup 3+},Sm{sup 3+} were measured to investigate the nature of the trapping centre and to locate its energy level relative to the valence and conduction bands of the YPO{sub 4} host. The high-temperature glow peak could unequivocally be assigned to Sm{sup 2+} (thus Sm{sup 3+} acts as an electron trap). The trap depth of this centre, as derived from the OSL excitation spectra, is in good agreement with the Dorenbos model prediction. The OSL excitation spectra also reveal excited states of Sm{sup 2+} well below the conduction band. These excited states produce a broadening of the high-temperature TL glow peak and also cause the activation energy determined by the Hoogenstraten method to underestimate the trap depth.

  11. Thermoluminescence and optically stimulated luminescence properties of the 0.5P₂O₅-xBaO-(0.5-x)Li₂O glass systems.

    Science.gov (United States)

    Timar-Gabor, A; Ivascu, C; Vasiliniuc, S; Daraban, L; Ardelean, I; Cosma, C; Cozar, O

    2011-05-01

    Thermoluminescence and optically stimulated luminescence properties of phosphate glasses doped with BaO and Li(2)O at various concentrations were studied. Lithium-doped glasses show a broad TL peak in the 200-300°C region with poor dosimetric characteristics. Barium-doped glasses feature at least two TL peaks, approximately at 200 and 400°C, which were attributed to Ba(2+) ions. They also produce a fast-decaying OSL signal correlated with the lower-temperature TL peak. Responses of both TL emissions to radiation doses up to 100 Gy are linear (R² >0.99). Due to its encouraging characteristics such as acceptable batch homogeneity, good measurement reproducibility and weak signal fading, the P₂O₅-xBaO glass can be considered as a candidate material for dosimetry in the high-dose range (>10 Gy).

  12. Infrared stimulated luminescence dating of an Eemian (MIS 5e) site in Denmark using K-feldspar

    DEFF Research Database (Denmark)

    Buylaert, Jan-Pieter; Huot, Sebastian; Murray, Andrew S.

    2011-01-01

    Infrared stimulated luminescence (IRSL) dating of K-feldspars may be an alternative to quartz optically stimulated luminescence (OSL) dating when the quartz OSL signal is too close to saturation or when the quartz luminescence characteristics are unsuitable. In this paper, Eemian (MIS 5e) coastal...

  13. Middle-Late Holocene earthquake history of the Gyrtoni Fault, Central Greece: Insight from optically stimulated luminescence (OSL) dating and paleoseismology

    Science.gov (United States)

    Tsodoulos, Ioannis M.; Stamoulis, Konstantinos; Caputo, Riccardo; Koukouvelas, Ioannis; Chatzipetros, Alexandros; Pavlides, Spyros; Gallousi, Christina; Papachristodoulou, Christina; Ioannides, Konstantinos

    2016-09-01

    The south-dipping Gyrtoni Fault defines the northeastern boundary of the Middle-Late Quaternary Tyrnavos Basin, Central Greece. The recognition and recent tectonic activity of the fault were previously based on mapping, remote sensing analyses and electrical resistivity tomography studies. To understand the Holocene seismotectonic behavior of the Gyrtoni Fault we excavated two paleoseismological trenches. To estimate the timing of past earthquakes using luminescence dating, we obtained twenty five fluvial-colluvial sediment and pottery samples from both the upthrown and the downthrown fault blocks. We applied the Optically Stimulated Luminescence (OSL) dating to coarse grain quartz using the single-aliquot regenerative-dose (SAR) protocol. Our investigations of luminescence characteristics using various tests confirmed the suitability of the material for OSL dating. We found that the estimated OSL ages were internally consistent and agreed well with the available stratigraphical data, archaeological evidence and radiocarbon dates. The performed paleoseismological analysis emphasized the occurrence of three surface faulting events in a time span between 1.42 ± 0.06 ka and 5.59 ± 0.13 ka. Also, we recognized an earlier faulting event (fourth) has been also recognized to be older than 5.59 ± 0.13 ka. The mean throw per event value of 0.50-0.60 m could correspond to a ca. Mw 6.5 earthquake. An average fault slip rate of 0.41 ± 0.01 mm/a and an average recurrence time of 1.39 ± 0.14 ka were also estimated. Our results suggest that the elapsed time from the most recent event (minimum age 1.42 ± 0.06 ka) is comparable with the mean return period.

  14. The origin of dose distributions in fluvial sediments, and the prospect of dating single grains from fluvial deposits using optically stimulated luminescence

    CERN Document Server

    Olley, J M; Roberts, R G

    1999-01-01

    We examine the causes of the asymmetric distributions of dose observed from measurements of the optically stimulated luminescence emitted by small aliquots of fluvial quartz, and deduce that the asymmetry arises as a result of samples being composed of a mix of mainly well bleached grains with grains that were effectively unbleached at the time of deposition. We demonstrate that the shapes of the dose distributions can be used to assess the likelihood that aliquots consist only of grains that were well-bleached at the time of deposition. The more asymmetric the distribution, the greater the probability that the aliquots with the lowest dose most closely represent the true burial dose. Single grains with differing doses are present in each of the samples examined, and the population with the lowest dose gives an optical age consistent with the expected burial age. This result implies that the beta-dose heterogeneity in these deposits is small, and that the effects of micro-dosimetric variations on optical dati...

  15. Stimulated luminescence emission from localized recombination in randomly distributed defects

    DEFF Research Database (Denmark)

    Jain, Mayank; Guralnik, Benny; Andersen, Martin Thalbitzer

    2012-01-01

    We present a new kinetic model describing localized electronic recombination through the excited state of the donor (d) to an acceptor (a) centre in luminescent materials. In contrast to the existing models based on the localized transition model (LTM) of Halperin and Braner (1960 Phys. Rev. 117...... that evolves only in the temporal domain. An excellent agreement is observed between thermally and optically stimulated luminescence (TL and OSL) results produced from the two models. In comparison to the first-order kinetic behaviour of the LTM of Halperin and Braner (1960 Phys. Rev. 117 408–15), our model...... results in a highly asymmetric TL peak; this peak can be understood to derive from a continuum of several first-order TL peaks. Our model also shows an extended power law behaviour for OSL (or prompt luminescence), which is expected from localized recombination mechanisms in materials with random...

  16. SU-E-T-315: The Change of Optically Stimulated Luminescent Dosimeters (OSLDs) Sensitivity by Accumulated Dose and High Dose

    Energy Technology Data Exchange (ETDEWEB)

    Han, S; Jung, H; Kim, M; Ji, Y; Kim, K [University of Science and Technology, Daejeon (Korea, Republic of); Korea Institute of Radiological and Medical Sciences, Seoul (Korea, Republic of); Choi, S; Park, S; Yoo, H [Korea Institute of Radiological and Medical Sciences, Seoul (Korea, Republic of); Yi, C [Korea Research Institute of Standards and Science, Daejeon (Korea, Republic of)

    2014-06-01

    Purpose: The objective of this study is to evaluate radiation sensitivity of optical stimulated luminance dosimeters (OSLDs) by accumulated dose and high dose. Methods: This study was carried out in Co-60 unit (Theratron 780, AECL, and Canada) and used InLight MicroStar reader (Landauer, Inc., Glenwood, IL) for reading. We annealed for 30 min using optical annealing system which contained fluorescent lamps (Osram lumilux, 24 W, 280 ∼780 nm). To evaluate change of OSLDs sensitivity by repeated irradiation, the dosimeters were repeatedly irradiated with 1 Gy. And whenever a repeated irradiation, we evaluated OSLDs sensitivity. To evaluate OSLDs sensitivity after accumulated dose with 5 Gy, We irradiated dose accumulatively (from 1 Gy to 5 Gy) without annealing. And OSLDs was also irradiated with 15, 20, 30 Gy to certify change of OSLDs sensitivity after high dose irradiation. After annealing them, they were irradiated with 1Gy, repeatedly. Results: The OSLDs sensitivity increased up to 3% during irradiating seven times and decreased continuously above 8 times. That dropped by about 0.35 Gy per an irradiation. Finally, after 30 times irradiation, OSLDs sensitivity decreased by about 7%. For accumulated dose from 1 Gy to 5 Gy, OSLDs sensitivity about 1 Gy increased until 4.4% after second times accumulated dose compared with before that. OSLDs sensitivity about 1 Gy decreased by 1.6% in five times irradiation. When OSLDs were irradiated ten times with 1Gy after irradiating high dose (10, 15, 20 Gy), OSLDs sensitivity decreased until 6%, 9%, 12% compared with it before high dose irradiation, respectively. Conclusion: This study certified OSLDs sensitivity by accumulated dose and high dose. When irradiated with 1Gy, repeatedly, OSLDs sensitivity decreased linearly and the reduction rate of OSLDs sensitivity after high dose irradiation had dependence on irradiated dose.

  17. Thermally stimulated luminescence of urine salts

    Science.gov (United States)

    Bordun, O.; Drobchak, O.

    2008-05-01

    The thermally stimulated luminescence (TSL) of normal and pathological urine was studied. The presence of pathological salts leads to extinguishing of TSL intensity and to the appearance of additional stripes with maxima nearly 118 and 205K, except of characteristic stripes with the maxima nearly 173 and 260K. TSL stripes depend on urine constituents. The comparison of TSL intensity of normal and pathological urine is carried out and energies of thermal activation are determined for most intensive TSL stripes.

  18. SU-E-T-585: Optically-Stimulated Luminescent Dosimeters for Monitoring Pacemaker Dose in Radiation Therapy

    Energy Technology Data Exchange (ETDEWEB)

    Apicello, L [Hofstra University, Hempstead, NY (United States); Riegel, A; Jamshidi, A [North Shore LIJ Health System, Lake Success, NY (United States)

    2015-06-15

    Purpose: A sufficient amount of ionizing radiation can cause failure to components of pacemakers. Studies have shown that permanent damage can occur after a dose of 10 Gy and minor damage to functionality occurs at doses as low as 2 Gy. Optically stimulated thermoluminescent dosimeters (OSLDs) can be used as in vivo dosimeters to predict dose to be deposited throughout the treatment. The purpose of this work is to determine the effectiveness of using OSLDs for in vivo dosimetry of pacemaker dose. Methods: As part of a clinical in vivo dosimetry experience, OSLDs were placed at the site of the pacemaker by the therapist for one fraction of the radiation treatment. OSLD measurements were extrapolated to the total dose to be received by the pacemaker during treatment. A total of 79 measurements were collected from November 2011 to December 2013 on six linacs. Sixty-six (66) patients treated in various anatomical sites had the dose of their pacemakers monitored. Results: Of the 79 measurements recorded, 76 measurements (96 %) were below 2 Gy. The mean and standard deviation were 50.12 ± 76.41 cGy. Of the 3 measurements that exceeded 2 Gy, 2 measurements matched the dose predicted in the treatment plan and 1 was repeated after an unexpectedly high Result. The repeated measurement yielded a total dose less than 2 Gy. Conclusion: This analysis suggests OSLDs may be used for in vivo monitoring of pacemaker dose. Further research should be performed to assess the effect of increased backscatter from the pacemaker device.

  19. The study on optically stimulated luminescence dosimeter based on the SrS:Eu, Sm and CaS:Eu, Sm

    Institute of Scientific and Technical Information of China (English)

    Liu Yan-Ping; Chen Zhao-Yang; Fan Yan-Wei; Ba Wei-Zhen; Gou Qi; Lu Wu; Tang Xin-Qiang; Du Yan-Zhao

    2008-01-01

    With the increasing use of nuclear energy, there is a need for a wider range of efficient dosimeters for radiation detection and assessment. There has been a tremendous growth in the development of radiation detectors and devices in the past few decades. In recent years, the development of new materials for radiation dosimetry has progressed significantly. Alkaline earth sulfides (AES) have been known for a long time as excellent and versatile phosphor materials.In the present investigation, a number of phosphor samples such as mono-, binary and ternary sulfides of alkaline earths (Ⅱa-Ⅵb) have been prepared and their TL properties have been studied with respect to exposure (x-ray) response and fading. In this paper, some results on SrS:Eu, Sm and CaS:Eu, Sm phosphors are presented. A type of novel OSL dosimeter is described. The dosimeter takes advantage of the characteristics of charge trapping materials SrS:Eu, Sm and CaS:Eu, Sm that exhibit optically stimulated luminescence (OSL). The measuring range of the dosimeter is from 0.01 to 1000 Gy. The OSL dosimeters provide capability for remote monitoring radiation locations which are difficult to access and hazardous. This equipment is relatively simple, small in size and has low power consumption. The device is suitable for space radiation dose exploration. In addition, it also can be used in IC and other radiation occasions and has good prospects.

  20. Energy absorption buildup factors, exposure buildup factors and Kerma for optically stimulated luminescence materials and their tissue equivalence for radiation dosimetry

    Science.gov (United States)

    Singh, Vishwanath P.; Badiger, N. M.

    2014-11-01

    Optically stimulated luminescence (OSL) materials are sensitive dosimetric materials used for precise and accurate dose measurement for low-energy ionizing radiation. Low dose measurement capability with improved sensitivity makes these dosimeters very useful for diagnostic imaging, personnel monitoring and environmental radiation dosimetry. Gamma ray energy absorption buildup factors and exposure build factors were computed for OSL materials using the five-parameter Geometric Progression (G-P) fitting method in the energy range 0.015-15 MeV for penetration depths up to 40 mean free path. The computed energy absorption buildup factor and exposure buildup factor values were studied as a function of penetration depth and incident photon energy. Effective atomic numbers and Kerma relative to air of the selected OSL materials and tissue equivalence were computed and compared with that of water, PMMA and ICRU standard tissues. The buildup factors and kerma relative to air were found dependent upon effective atomic numbers. Buildup factors determined in the present work should be useful in radiation dosimetry, medical diagnostics and therapy, space dosimetry, accident dosimetry and personnel monitoring.

  1. Optically stimulated luminescence (OSL) response of Al2O3:C, BaFCl:Eu and K2Ca2(SO4)3:Eu phosphors.

    Science.gov (United States)

    Kumar, Pratik; Bahl, Shaila; Sahare, P D; Kumar, Surender; Singh, Manveer

    2015-12-01

    This paper investigates the optically stimulated luminescence (OSL) response of BaFCl:Eu and K2Ca2(SO4)3:Eu phosphors for different doses and bleaching durations. The results have also been compared with the commercially available Landauer Al2O3:C (Luxel®) dosemeter. Nanocrystalline K2Ca2(SO4)3:Eu is known to be a sensitive thermoluminescent phosphor, but its OSL response is hardly reported. At first, pellets of nanocrystalline K2Ca2(SO4)3:Eu powder were prepared by adding Teflon as a binder. Their OSL signal was compared with that of the material in pure form, i.e. without adding the binder (in 100:1 ratio). It was observed that adding the binder does not appreciably affect the OSL intensity. On comparison with the commercially available Al2O3:C from Landauer, it was found that K2Ca2(SO4)3:Eu is around 15 times less sensitive than Al2O3:C. 'Homemade' BaFCl:Eu phosphor has also been studied. The intensity of BaFCl:Eu was ∼20 times more than the standard Al2O3:C dosemeter and ∼200 times more sensitive than K2Ca2(SO4)3:Eu in the dose range of 13-200 cGy. OSL dosemeters are believed to give luminescence signal even if they are read before, i.e. multiple reading may be possible under suitable conditions after single exposure. This was also checked for all the prepared dosemeters and it was found that Al2O3:C showed the least decrease of Eu of 15 % and K2Ca2(SO4)3:Eu with 20 %. Finally, Al2O3:C and BaFCl:Eu phosphors were also studied for their optical bleaching durations to which the respective signals get completely removed so that the phosphor can be re-used. It was observed that BaFCl:Eu is bleached faster and more easily than Al2O3:C.

  2. Slip rate determination along the Southern Dead Sea fault: optically stimulated luminescence, 10Be cosmogenic radionuclide, and 14C ages brought face to face

    Science.gov (United States)

    Le Beon, Maryline; Jaiswal, Manoj; Kunz, Alexander; Al-Qaryouti, Mahmoud; Burr, George; Klinger, Yann; Moumani, Khaled; Chen, Yue-Gau; Abdelghafoor, Mohammed; Suppe, John

    2014-05-01

    Active tectonics studies are often limited by difficulties in accurately and precisely dating Late Quaternary alluvial deposits that commonly lack organic matter or date beyond the 14C dating limit. This is illustrated at a site called Fidan, in arid southern Jordan, where a series of alluvial fans are laterally offset by the southern Dead Sea fault. Geodetic, geomorphic and geologic studies converge to a fault slip rate of 5 ± 2 mm/a. Yet, Late Pleistocene slip rate at Fidan cover a wide range due to the dispersion of 10Be cosmogenic radionuclide (CRN) ages. The maximum slip rate since ~100 ka is up to a value of 11 mm/a, possibly suggesting significant variations in fault activity with time. In order to reduce the uncertainty on the Late Pleistocene slip rate and draw further conclusions regarding the fault seismic behavior, we implement complementary dating using optically stimulated luminescence (OSL) techniques on both quartz and K-feldspar minerals and using 14C when possible. OSL measurements include a newly developed technique called post-infra-red infra-red stimulated luminescence at 290°C (pIR290). We extensively sampled surface levels F2 and F4, digging ~50-cm deep pits into the geomorphic surfaces. Annual dose rates were determined in the laboratory from both geochemical analysis of the sediment and gamma-ray spectrometry. Due to sediment heterogeneity, we consider gamma-ray spectrometry as more reliable because it is based on a larger volume of sediment. Quartz OSL ages and preliminary pIR290 results on K-feldspars give consistent Early Holocene ages of 9-14 ka for F2, also in agreement with a 14C age of 13 ka from a landsnail shell. 10Be CRN exposure ages on F2 were significantly older, with 37 ± 4 ka, probably due to inheritance. On F4, 10Be CRN exposure ages showed a scattered distribution, from ~50 ka to ~120 ka, with most samples comprised in the mean interval of 87 ± 26 ka. Quartz OSL ages from 5 locations on F4 are comprised between 32 ± 3

  3. Development and characterization of remote radiation dosimetry systems using optically stimulated luminescence of alumina:carbon and potassium bromide:europium

    Science.gov (United States)

    Klein, David Matthew

    Scope and Method of Study. To develop and test the performance of two different dosimetry systems; one for in situ, high-sensitivity, inexpensive environmental monitoring, and another for near-real-time medical dosimetry. The systems are based on remote interrogation of the optically stimulated luminescence (OSL) from Al2O3:C and KBr:Eu single crystal dosimeters (exposed to environmental and medical radiation fields, respectively) via fiber optic cables. The environmental system was tested in lab conditions using various radioactive sources including 60Co, 90 Sr, 137Cs, and 226Ra, as well as with 232Th-enriched soil stimulant. The medical system was tested under various diagnostic x-ray systems, including fluoroscopy and computed tomography (CT) machines, as well as with high dose rate 192Ir brachytherapy sources and 232 MeV proton therapy beams under simulated treatment conditions. Findings and Conclusions. The environmental system was shown to achieve sensitivity high enough for measuring an OSL signal resulting from a dose of ˜1 muGy, which is equivalent to ˜12 hours of natural background radiation. This sensitivity allows for monitoring of the radiation characteristics of a natural environment more rapidly and/or less expensively than existing methods, such as soil sampling and in situ gamma spectroscopy. The KBr:Eu-based medical system results show that the near-real-time data acquisition during irradiation allows for rapid quality assurance (QA) measurements that benefits from high spatial resolution. These features are not present in most current standard dosimeters such as thermoluminescent detectors and pencil ionization chambers. The dosimeter does exhibit energy dependence, and a sensitization during high dose rate procedures. As a result, a model has been proposed that provides a description of the possible mechanisms that govern the transfer of electrons and holes within KBr:Eu during OSL measurement at room temperature. Correction factors for these

  4. Investigation of neutron converters for production of optically stimulated luminescence (OSL) neutron dosimeters using Al{sub 2}O{sub 3}:C

    Energy Technology Data Exchange (ETDEWEB)

    Mittani, J.C.R. [Department of Physics, Oklahoma State University, Stillwater, OK 74078-3072 (United States); Silva, A.A.R. da [Department of Physics, Oklahoma State University, Stillwater, OK 74078-3072 (United States); Vanhavere, F. [SCK.CEN, Belgian Nuclear Research Centre, Boeretang 200, 2400 Mol (Belgium); Akselrod, M.S. [Landauer, Inc., Stillwater Crystal Growth Division, 723 1/2 Eastgate Rd., Stillwater, OK 74074 (United States); Yukihara, E.G. [Department of Physics, Oklahoma State University, Stillwater, OK 74078-3072 (United States)]. E-mail: eduardo.yukihara@okstate.edu

    2007-07-15

    This paper presents the optically stimulated luminescence (OSL) properties of neutron dosimeters in powder and in the form of pellets prepared with a mixture of Al{sub 2}O{sub 3}:C and neutron converters. The neutron converters investigated were high density polyethylene (HDPE), lithium fluoride (LiF), lithium fluoride 95% enriched with {sup 6}Li ({sup 6}LiF), lithium carbonate 95% enriched with {sup 6}Li ({sup 6}Li{sub 2}CO{sub 3}), boric acid enriched with 99% of {sup 10}B (H{sub 3}{sup 10}BO{sub 3}) and gadolinium oxide (Gd{sub 2}O{sub 3}). The proportion of Al{sub 2}O{sub 3}:C and neutron converter in the mixture was varied to optimize the total OSL signal and neutron sensitivity. The neutron sensitivity and dose-response were determined for the OSL dosimeters using a bare {sup 252}Cf source and compared to the response of Harshaw TLD-600 and TLD-700 dosimeters ({sup 6}LiF:Mg,Ti and {sup 7}LiF:Mg,Ti). The results demonstrate the possibility of developing an OSL dosimeter made of Al{sub 2}O{sub 3}:C powder and neutron converter with a neutron sensitivity (defined as the ratio between the {sup 60}Co equivalent gamma dose and the reference neutron absorbed dose) and neutron-gamma discrimination comparable to the TLD-600/TLD-700 combination. It was shown that the shape of the OSL decay curves varied with the type of the neutron converter, demonstrating the influence of the energy deposition mechanism and ionization density on the OSL process in Al{sub 2}O{sub 3}:C.

  5. The influence of radiation-induced defects on thermoluminescence and optically stimulated luminescence of α-Al{sub 2}O{sub 3}:C

    Energy Technology Data Exchange (ETDEWEB)

    Nyirenda, A.N., E-mail: anyirenda@gmail.com; Chithambo, M.L.

    2017-04-15

    It is known that when α-Al{sub 2}O{sub 3}:C is exposed to excessive amounts of ionising radiation, defects are induced within its matrix. We report the influence of radiation-induced defects on the thermoluminescence (TL) and optically stimulated luminescence (OSL) measured from α-Al{sub 2}O{sub 3}:C after irradiation to 1000 Gy. These radiation-induced defects are thermally unstable in the region 450–650 °C and result in TL peaks in this range when the TL is measured at 1 °C/s. Heating a sample to 700 °C obliterates the radiation-induced defects, that is, the TL peaks corresponding to the radiation induced defects are no longer observed in the subsequent TL measurements when moderate irradiation doses below 10 Gy are used. The charge traps associated with these radiation-induced defects are more stable than the dosimetric trap when the sample is exposed to either sunlight or 470-nm blue light from LEDs. TL glow curves measured following the defect-inducing irradiation produce a dosimetric peak that is broader and positioned at a higher temperature than observed in glow curves obtained before the heavy irradiation. In addition, sample sensitization/desensitization occurs due to the presence of these radiation-induced defects. Furthermore, both the activation energy and the kinetic order of the dosimetric peak evaluated when the radiation-induced defects are present in the sample are significantly lower in value than those obtained when these defects are absent. The radiation-induced defects also affect the shape and total light sum of the OSL signal as well as the position and width of the resultant residual phototransferred thermoluminescence main peak.

  6. The influence of radiation-induced defects on thermoluminescence and optically stimulated luminescence of α-Al2O3:C

    Science.gov (United States)

    Nyirenda, A. N.; Chithambo, M. L.

    2017-04-01

    It is known that when α-Al2O3:C is exposed to excessive amounts of ionising radiation, defects are induced within its matrix. We report the influence of radiation-induced defects on the thermoluminescence (TL) and optically stimulated luminescence (OSL) measured from α-Al2O3:C after irradiation to 1000 Gy. These radiation-induced defects are thermally unstable in the region 450-650 °C and result in TL peaks in this range when the TL is measured at 1 °C/s. Heating a sample to 700 °C obliterates the radiation-induced defects, that is, the TL peaks corresponding to the radiation induced defects are no longer observed in the subsequent TL measurements when moderate irradiation doses below 10 Gy are used. The charge traps associated with these radiation-induced defects are more stable than the dosimetric trap when the sample is exposed to either sunlight or 470-nm blue light from LEDs. TL glow curves measured following the defect-inducing irradiation produce a dosimetric peak that is broader and positioned at a higher temperature than observed in glow curves obtained before the heavy irradiation. In addition, sample sensitization/desensitization occurs due to the presence of these radiation-induced defects. Furthermore, both the activation energy and the kinetic order of the dosimetric peak evaluated when the radiation-induced defects are present in the sample are significantly lower in value than those obtained when these defects are absent. The radiation-induced defects also affect the shape and total light sum of the OSL signal as well as the position and width of the resultant residual phototransferred thermoluminescence main peak.

  7. Study of thermoluminescence (TL) and optically stimulated luminescence (OSL) from α-keratin protein found in human hairs and nails: potential use in radiation dosimetry.

    Science.gov (United States)

    Mishra, D R; Soni, A; Rawat, N S; Bokam, G

    2016-05-01

    The thermoluminescence (TL) and optically stimulated luminescence (OSL) properties of human nails and hairs containing α-keratin proteins have been investigated. For the present studies, black hairs and finger nails were selectively collected from individuals with ages between 25 and 35 years. The collected hairs/nails were cut to a size of TL glow peaks in the temperature range from 70 to 210 ° C. Continuous wave (CW)-OSL measurements of hair samples at a wavelength of 470 nm showed the presence of two distinct OSL components with photoionization cross section (PIC) values of about 1.65 × 10(-18) cm(2) and about 3.48 × 10(-19) cm(2), while measurements of nail samples showed PIC values of about 6.98 × 10(-18) cm(2) and about 8.7 × 10(-19) cm(2), respectively. This difference in PIC values for hair and nail samples from the same individual is attributed to different arrangement of α-keratin protein concentrations in the samples. The OSL sensitivity was found to vary ± 5 times among nail and hair samples from different individuals, with significant fading (60% in 11 h) at room temperature. The remaining signal (after fading) can be useful for dose estimation when a highly sensitive OSL reader is used. In the absorbed dose range of 100 mGy-100 Gy, both the TL and OSL signals of hair and nail samples showed linear dose dependence. The results obtained in the present study suggest that OSL using hair and nail samples may provide a supplementary method of dose estimation in radiological and nuclear emergencies.

  8. Quaternary glacial history of the Kanas Valley, Chinese Altai, NW China, constrained by electron spin resonance and optically stimulated luminescence datings

    Science.gov (United States)

    Yang, Jianqiang; Chen, Yixin; Xu, Xiangke; Cui, Zhijiu; Xiong, Heigang

    2017-10-01

    The Chinese Altai is located on the northern edge of Central Asia. Rich geological records of Quaternary glaciations are preserved in this area. However, the glacial history in the Chinese Altai has hardly been investigated. This study aims to rebuild the regional glacial history in the Kanas Valley of the Chinese Altai. We present 14 electron spin resonance (ESR) ages and 3 optically stimulated luminescence (OSL) ages from glacial landforms. By integrating with ages from previous studies, five major glacial advances are identified during Marine Oxygen Isotope Stages (MIS) 6, 5, 4, 3 and 2, with ages of 167.0 ± 16.0-123.0 ± 18.0 ka, 97.0 ± 19.0-78.0 ± 7.0 ka, 76.0 ± 16.0-73.1 ± 6.6 ka, 52.1 ± 7.8-34.4 ± 4.2 ka, and 28.0 ± 3.3-16.1 ± 1.5 ka respectively. The glacial advance during MIS 5 is the local Last Glacial Maximum, and glaciers became successively more restricted from MIS 5 to MIS 2. In addition, the extensive MIS 3 glacial advance in the Chinese Altai contrasts with the absence of MIS 3 glacial advance in the Mongolia Altai. These glacial patterns reflect that precipitation brought by the westerlies might play a primary role on driving glacial advances during the Last Glacial in the Chinese Altai. This glacial chronology is in reasonable agreement with existing glacial chronologies from other parts of the Altai, Tian Shan and Pamir, indicating similar climate controls on the patterns of Quaternary glaciation across Central Asia Highlands.

  9. The age of three Middle Palaeolithic sites: Single-grain optically stimulated luminescence chronologies for Pech de l'Azé I, II and IV in France.

    Science.gov (United States)

    Jacobs, Zenobia; Jankowski, Nathan R; Dibble, Harold L; Goldberg, Paul; McPherron, Shannon J P; Sandgathe, Dennis; Soressi, Marie

    2016-06-01

    Optically stimulated luminescence (OSL) measurements were made on individual, sand-sized grains of quartz from Middle Palaeolithic deposits at three sites (Pech de l'Azé I, II and IV) located close to one another in the Dordogne region of southwest France. We were able to calculate OSL ages for 69 samples collected from these three sites. These ages reveal periods of occupation between about 180 and 50 thousand years ago. Our single-grain OSL chronologies largely support previous age estimates obtained by thermoluminescence dating of burnt flints at Pech IV, electron spin resonance dating of tooth enamel at Pech I, II and IV and radiocarbon dating of bone at Pech I and IV, but provide a more complete picture due to the ubiquitous presence of sand-sized quartz grains used in OSL dating. These complete chronologies for the three sites have allowed us to compare the single-grain ages for similar lithic assemblages among the three sites, to test the correlations among them previously proposed by Bordes in the 1970s, and to construct our own correlative chronological framework for the three sites. This shows that similar lithic assemblages occur at around the same time, and that where a lithic assemblage is unique to one or found at two of the Pech sites, there are no deposits of chronologically equivalent age at the other Pech site(s). We interpret this to mean that, at least for these Pech de l'Azé sites, the Mousterian variants show temporal ordering. Whether or not this conclusion applies to the wider region and beyond, the hypothesis that Mousterian industrial variation is temporally ordered cannot be refuted at this time.

  10. Energy dependence measurement of small-type optically stimulated luminescence (OSL) dosimeter by means of characteristic X-rays induced with general diagnostic X-ray equipment.

    Science.gov (United States)

    Takegami, Kazuki; Hayashi, Hiroaki; Okino, Hiroki; Kimoto, Natsumi; Maehata, Itsumi; Kanazawa, Yuki; Okazaki, Tohru; Hashizume, Takuya; Kobayashi, Ikuo

    2016-01-01

    For X-ray inspections by way of general X-ray equipment, it is important to measure an entrance-skin dose. Recently, a small optically stimulated luminescence (OSL) dosimeter was made commercially available by Landauer, Inc. The dosimeter does not interfere with the medical images; therefore, it is expected to be a convenient detector for measuring personal exposure doses. In an actual clinical situation, it is assumed that X-rays of different energies will be detected by a dosimeter. For evaluation of the exposure dose measured by a dosimeter, it is necessary to know the energy dependence of the dosimeter. Our aim in this study was to measure the energy dependence of the OSL dosimeter experimentally in the diagnostic X-ray region. Metal samples weighing several grams were irradiated and, in this way, characteristic X-rays having energies ranging from 8 to 85 keV were generated. Using these mono-energetic X-rays, the dosimeter was irradiated. Simultaneously, the fluence of the X-rays was determined with a CdTe detector. The energy-dependent efficiency of the dosimeter was derived from the measured value of the dosimeter and the fluence. Moreover, the energy-dependent efficiency was calculated by Monte-Carlo simulation. The efficiency obtained in the experiment was in good agreement with that of the simulation. In conclusion, our proposed method, in which characteristic X-rays are used, is valuable for measurement of the energy dependence of a small OSL dosimeter in the diagnostic X-ray region.

  11. Radiation-induced growth and isothermal decay of infrared-stimulated luminescence from feldspar

    DEFF Research Database (Denmark)

    Guralnik, Benny; Li, Bo; Jain, Mayank

    2015-01-01

    Optically stimulated luminescence (OSL) ages can determine a wide range of geological events or processes, such as the timing of sediment deposition, the exposure duration of a rock surface, or the cooling rate of bedrock. The accuracy of OSL dating critically depends on our capability to describe...... the growth and decay of laboratory-regenerated luminescence signals. Here we review a selection of common models describing the response of infrared stimulated luminescence (IRSL) of feldspar to constant radiation and temperature as administered in the laboratory. We use this opportunity to introduce...

  12. Luminescence excitation characteristics of Ca-, Na- and K-aluminosilicates (feldspars), in the stimulation range 20-500 eV: optical detection of XAS

    CERN Document Server

    Poolton, N R J; Quinn, F M; Pantos, E; Andersen, C E; Bøtter-Jensen, L; Johnsen, O; Murray, A S

    2003-01-01

    We demonstrate that the visible/UV luminescence from common feldspar crystals (NaAlSi sub 3 O sub 8 , KAlSi sub 3 O sub 8 and CaAl sub 2 Si sub 2 O sub 8) can be used to detect detailed L-edge and associated near-edge absorption structure of the main constituent atoms (Ca, K, Na, Al, Si), when exciting in the energy range 20-500 eV. Comparisons of the spectral features are drawn with similar measurements made on the associated materials SiO sub 2 , Al sub 2 O sub 3 and CaCO sub 3. The potential for using optically detected x-ray absorption spectroscopy as a method for identifying the luminescent components of mixed mineral samples is considered.

  13. Luminescence excitation characteristics of Ca-, Na- and K-aluminosilicates (feldspars), in the stimulation range 20-500 eV: optical detection of XAS

    Energy Technology Data Exchange (ETDEWEB)

    Poolton, N R J [Synchrotron Radiation Department, Daresbury Laboratory, Warrington WA4 4AD, Cheshire (United Kingdom); Malins, A E R [Synchrotron Radiation Department, Daresbury Laboratory, Warrington WA4 4AD, Cheshire (United Kingdom); Quinn, F M [Synchrotron Radiation Department, Daresbury Laboratory, Warrington WA4 4AD, Cheshire (United Kingdom); Pantos, E [Synchrotron Radiation Department, Daresbury Laboratory, Warrington WA4 4AD, Cheshire (United Kingdom); Andersen, C E [Radiation Research Department, Riso National Laboratory, 4000 Roskilde (Denmark); Botter-Jensen, L [Radiation Research Department, Riso National Laboratory, 4000 Roskilde (Denmark); Johnsen, O [Geological Museum, University of Copenhagen, Oster Voldgade 5-7, 1350 Copenhagen (Denmark); Murray, A S [Nordic Laboratory for Luminescence Dating, Aarhus University, Riso National Laboratory, 4000 Roskilde (Denmark)

    2003-05-07

    We demonstrate that the visible/UV luminescence from common feldspar crystals (NaAlSi{sub 3}O{sub 8}, KAlSi{sub 3}O{sub 8} and CaAl{sub 2}Si{sub 2}O{sub 8}) can be used to detect detailed L-edge and associated near-edge absorption structure of the main constituent atoms (Ca, K, Na, Al, Si), when exciting in the energy range 20-500 eV. Comparisons of the spectral features are drawn with similar measurements made on the associated materials SiO{sub 2}, Al{sub 2}O{sub 3} and CaCO{sub 3}. The potential for using optically detected x-ray absorption spectroscopy as a method for identifying the luminescent components of mixed mineral samples is considered.

  14. Luminescent solar concentrator improvement by stimulated emission

    Science.gov (United States)

    Kaysir, Md Rejvi; Fleming, Simon; MacQueen, Rowan W.; Schmidt, Timothy W.; Argyros, Alexander

    2015-12-01

    Luminescent solar concentrators (LSCs) offer the prospect of reducing the cost of solar energy, and are a promising candidate for building integrated photovoltaic (PV) structures. However, the realization of commercially viable efficiency of LSCs is currently hindered by reabsorption losses. In this work, a method is introduced for reducing reabsorption as well as improving directional emission in LSCs by using stimulated emission. Light from a seed laser (potentially an inexpensive laser diode) passes through the entire length of the LSC panel, modifying the emission spectrum of excited dye molecules such that it is spectrally narrower, at wavelengths that minimize reabsorption, and directed by the seed laser towards a small target PV cell. A mathematical model of such a system is presented which identifies different physical parameters responsible for the power conversion efficiency and gives the net effective output power.

  15. Luminescent solar concentrators utilizing stimulated emission.

    Science.gov (United States)

    Kaysir, Md Rejvi; Fleming, Simon; MacQueen, Rowan W; Schmidt, Timothy W; Argyros, Alexander

    2016-03-21

    Luminescent solar concentrators (LSCs) are an emerging technology that aims primarily to reduce the cost of solar energy, with great potential for building integrated photovoltaic (PV) structures. However, realizing LSCs with commercially viable efficiency is currently hindered by reabsorption losses. Here, we introduce an approach to reducing reabsorption as well as improving directional emission in LSCs by using stimulated emission. Light from a seed laser (potentially an inexpensive laser diode) passes through the entire area of the LSC panel, modifying the emission spectrum of excited dye molecules such that it is spectrally narrower, at wavelengths that minimize reabsorption to allow net gain in the system, and directed towards a small PV cell. A mathematical model, taking into account thermodynamic considerations, of such a system is presented which identifies key parameters and allows evaluation in terms of net effective output power.

  16. Development and implementation of a remote audit tool for high dose rate (HDR) Ir-192 brachytherapy using optically stimulated luminescence dosimetry

    Energy Technology Data Exchange (ETDEWEB)

    Casey, Kevin E.; Kry, Stephen F.; Howell, Rebecca M.; Followill, David [Department of Radiation Physics, The University of Texas MD Anderson Cancer Center, Houston, Texas 77030 and The University of Texas Graduate School of Biomedical Sciences at Houston, Houston, Texas 77030 (United States); Alvarez, Paola; Lawyer, Ann [Department of Radiation Physics, The University of Texas MD Anderson Cancer Center, Houston, Texas 77030 (United States)

    2013-11-15

    Purpose: The aim of this work was to create a mailable phantom with measurement accuracy suitable for Radiological Physics Center (RPC) audits of high dose-rate (HDR) brachytherapy sources at institutions participating in National Cancer Institute-funded cooperative clinical trials. Optically stimulated luminescence dosimeters (OSLDs) were chosen as the dosimeter to be used with the phantom.Methods: The authors designed and built an 8 × 8 × 10 cm{sup 3} prototype phantom that had two slots capable of holding Al{sub 2}O{sub 3}:C OSLDs (nanoDots; Landauer, Glenwood, IL) and a single channel capable of accepting all {sup 192}Ir HDR brachytherapy sources in current clinical use in the United States. The authors irradiated the phantom with Nucletron and Varian {sup 192}Ir HDR sources in order to determine correction factors for linearity with dose and the combined effects of irradiation energy and phantom characteristics. The phantom was then sent to eight institutions which volunteered to perform trial remote audits.Results: The linearity correction factor was k{sub L}= (−9.43 × 10{sup −5}× dose) + 1.009, where dose is in cGy, which differed from that determined by the RPC for the same batch of dosimeters using {sup 60}Co irradiation. Separate block correction factors were determined for current versions of both Nucletron and Varian {sup 192}Ir HDR sources and these vendor-specific correction factors differed by almost 2.6%. For the Nucletron source, the correction factor was 1.026 [95% confidence interval (CI) = 1.023–1.028], and for the Varian source, it was 1.000 (95% CI = 0.995–1.005). Variations in lateral source positioning up to 0.8 mm and distal/proximal source positioning up to 10 mm had minimal effect on dose measurement accuracy. The overall dose measurement uncertainty of the system was estimated to be 2.4% and 2.5% for the Nucletron and Varian sources, respectively (95% CI). This uncertainty was sufficient to establish a ±5% acceptance

  17. Optically stimulated exoelectron emission processes in quartz: comparison of experiment and theory

    DEFF Research Database (Denmark)

    Pagonis, V.; Ankjærgaard, Christina; Murray, A.S.

    2009-01-01

    Recent experiments have demonstrated that it is possible to measure optically stimulated exoelectron emission (OSE) signals simultaneously with optically stimulated luminescence (OSL) from quartz samples. These experiments provide valuable information on the charge movement in quartz grains. Two...

  18. Comparative dose evaluations between XVI and OBI cone beam CT systems using Gafchromic XRQA2 film and nanoDot optical stimulated luminescence dosimeters

    Energy Technology Data Exchange (ETDEWEB)

    Giaddui, Tawfik; Cui Yunfeng; Galvin, James; Yu Yan; Xiao Ying [Department of Radiation Oncology, Thomas Jefferson University, Philadelphia, Pennsylvania 19107 (United States)

    2013-06-15

    Purpose: To investigate the effect of energy (kVp) and filters (no filter, half Bowtie, and full Bowtie) on the dose response curves of the Gafchromic XRQA2 film and nanoDot optical stimulated luminescence dosimeters (OSLDs) in CBCT dose fields. To measure surface and internal doses received during x-ray volume imager (XVI) (Version R4.5) and on board imager (OBI) (Version 1.5) CBCT imaging protocols using these two types of dosimeters. Methods: Gafchromic XRQA2 film and nanoDot OSLD dose response curves were generated at different kV imaging settings used by XVI (software version R4.5) and OBI (software version 1.5) CBCT systems. The settings for the XVI system were: 100 kVp/F0 (no filter), 120 kVp/F0, and 120 kVp/F1 (Bowtie filter), and for the OBI system were: 100 kVp/full fan, 125 kVp/full fan, and 125 kVp/half fan. XRQA2 film was calibrated in air to air kerma levels between 0 and 11 cGy and scanned using reflection scanning mode with the Epson Expression 10000 XL flat-bed document scanner. NanoDot OSLDs were calibrated on phantom to surface dose levels between 0 and 14 cGy and read using the inLight{sup TM} MicroStar reader. Both dosimeters were used to measure in field surface and internal doses in a male Alderson Rando Phantom. Results: Dose response curves of XRQA2 film and nanoDot OSLDs at different XVI and OBI CBCT settings were reported. For XVI system, the surface dose ranged between 0.02 cGy in head region during fast head and neck scan and 4.99 cGy in the chest region during symmetry scan. On the other hand, the internal dose ranged between 0.02 cGy in the head region during fast head and neck scan and 3.17 cGy in the chest region during chest M20 scan. The average (internal and external) dose ranged between 0.05 cGy in the head region during fast head and neck scan and 2.41 cGy in the chest region during chest M20 scan. For OBI system, the surface dose ranged between 0.19 cGy in head region during head scan and 4.55 cGy in the pelvis region during

  19. Red-IR stimulated luminescence in K-feldspar: Single or multiple trap origin?

    DEFF Research Database (Denmark)

    Andersen, Martin Thalbitzer; Jain, Mayank; Tidemand-Lichtenberg, Peter

    2012-01-01

    We investigate on the origins of the infra-red stimulated luminescence (IRSL) signals in 3 potassium feldspars based on IR-red spectroscopy (700–1050 nm) using a fiber-coupled tunable Ti:Sapphire laser, in combination with different thermal and optical (pre)treatments of the samples. We also...

  20. Thermal dependence of time-resolved blue light stimulated luminescence in α-Al2O3:C

    DEFF Research Database (Denmark)

    Pagonis, Vasilis; Ankjærgaard, Christina; Jain, Mayank

    2013-01-01

    This paper presents time-resolved optically stimulated luminescence (TR-OSL) experiments in the important dosimetric material Al2O 3:C. During these experiments short pulses (0.5 s) of light from blue LEDs (470 nm) are followed by relaxation periods (2.5 s) of the charge carriers at different......-dependent phosphorescence signal, the delayed-OSL described previously for this material. The temperature dependent luminescence lifetimes obtained from analysis of the optical stimulation period are identical to those obtained from the corresponding relaxation period. However, the values of these luminescence lifetimes...

  1. Stimulated luminescence of AlN ceramics induced by ultraviolet radiation

    DEFF Research Database (Denmark)

    Trinkler, L.; Bøtter-Jensen, L.; Christensen, P.

    2001-01-01

    Properties of thermally stimulated luminescence (TL) and optically stimulated luminescence (OSL) of the ceramic material A1N-Y2O3 have been studied after exposure to ultraviolet radiation (UVR). The dosemeter material Al2O3 : C has been used for comparative measurements. The spectral sensitivity...... than that of Al2O3 : C in a broad spectral region. The possibility of using A1N-Y2O3 ceramic for UVR dosimetry is discussed. (C) 2001 Elsevier Science Ltd. All rights reserved....

  2. Towards dating Quaternary sediments using the quartz Violet Stimulated Luminescence (VSL) signal

    DEFF Research Database (Denmark)

    Ankjærgaard, C.; Jain, Mayank; Wallinga, J.

    2013-01-01

    Quartz optically stimulated luminescence (OSL) dating is widely used to determine the time of deposition and burial of Late Quaternary sediments. Application of the method is usually limited to the past 150,000 years due to early saturation of the OSL signal. Here we explore the potential to date...... Quaternary sediments using the violet (402 nm) stimulated luminescence (VSL) signal of quartz.We develop and test a new post-blue VSL single aliquot regenerative dose dating protocol, and demonstrate that the VSL signal originates from a deep trap at about 1.9 eV with a thermal lifetime of 1011 years at 10...

  3. Luminescence from potassium feldspars stimulated by infrared and green light

    DEFF Research Database (Denmark)

    Duller, G.A.T.; Bøtter-Jensen, L.

    1993-01-01

    A series of experiments are reported which investigate stimulated luminescence from potassium feldspar. The aim is to provide a basic phenomenological description of the response of the material to stimulation by heat, infrared radiation (875 DELTA 80 nm) and a green light wavelength band from 5 15...

  4. Thermoluminescence and optically stimulated luminescence properties of the 0.5P{sub 2}O{sub 5}-xBaO-(0.5-x)Li{sub 2}O glass systems

    Energy Technology Data Exchange (ETDEWEB)

    Timar-Gabor, A., E-mail: alida.timar@ubbcluj.r [Faculty of Environmental Science, Babes-Bolyai University, Fantanele 30, 400294 Cluj Napoca (Romania); Ivascu, C. [Faculty of Physics, Babes-Bolyai University, Kogalniceanu 1, 400084 Cluj Napoca (Romania); Vasiliniuc, S. [Faculty of Environmental Science, Babes-Bolyai University, Fantanele 30, 400294 Cluj Napoca (Romania); Daraban, L.; Ardelean, I. [Faculty of Physics, Babes-Bolyai University, Kogalniceanu 1, 400084 Cluj Napoca (Romania); Cosma, C. [Faculty of Environmental Science, Babes-Bolyai University, Fantanele 30, 400294 Cluj Napoca (Romania); Cozar, O. [Faculty of Physics, Babes-Bolyai University, Kogalniceanu 1, 400084 Cluj Napoca (Romania)

    2011-05-15

    Thermoluminescence and optically stimulated luminescence properties of phosphate glasses doped with BaO and Li{sub 2}O at various concentrations were studied. Lithium-doped glasses show a broad TL peak in the 200-300 {sup o}C region with poor dosimetric characteristics. Barium-doped glasses feature at least two TL peaks, approximately at 200 and 400 {sup o}C, which were attributed to Ba{sup 2+} ions. They also produce a fast-decaying OSL signal correlated with the lower-temperature TL peak. Responses of both TL emissions to radiation doses up to 100 Gy are linear (R{sup 2}>0.99). Due to its encouraging characteristics such as acceptable batch homogeneity, good measurement reproducibility and weak signal fading, the P{sub 2}O{sub 5}-BaO glass can be considered as a candidate material for dosimetry in the high-dose range (>10 Gy).

  5. Modeling of stimulated emission based luminescent solar concentrators.

    Science.gov (United States)

    Kaysir, Md Rejvi; Fleming, Simon; Argyros, Alexander

    2016-12-26

    The efficiency improvement of luminescent solar concentrators (LSCs) necessary for practical realization is currently hindered by one major loss mechanism: reabsorption of emitted photons by the luminophores. Recently, we explored a promising technique for reducing reabsorption and also improving directional emission in LSCs utilizing stimulated emission, rather than only spontaneous emission, with an inexpensive seed laser. In this work, a model is developed to quantify the gain (i.e. the amount of amplification of a low power seed laser propagating through the solar-pumped concentrator) of stimulated-LSCs (s-LSCs) considering the effects of different important physical parameters. The net optical output power, available for a small PV cell, from the concentrator can also be determined from the model, which indicates the performance of s-LSCs. Finally, the performance of different existing material systems is investigated using literature values of the parameters required for the model, and a set of optimal parameters is suggested for practical realization of such a device.

  6. Thermoluminescence and optically stimulated luminescence properties of nanocrystalline Er{sup 3+} and Yb{sup 3+} doped Y{sub 3}Al{sub 5}O{sub 12} exposed to {beta}-rays

    Energy Technology Data Exchange (ETDEWEB)

    RodrIguez, R A [Universidad de Guadalajara en Lagos, Lagos de Moreno, Jalisco, 47460 (Mexico); Rosa, E de la [Centro de Investigaciones en Optica, A.P. 1-948, Leon, Gto. 37150 (Mexico); Salas, P [Instituto Mexicano del Petroleo, Eje Central Lazaro Cardenas 152, C.P. 07730, Mexico, D. F. (Mexico); Melendrez, R [Centro de Investigacion en Fisica, Universidad de Sonora, PO Box 5-088, Hermosillo, Sonora, 83190 (Mexico); Barboza-Flores, M [Centro de Investigacion en Fisica, Universidad de Sonora, PO Box 5-088, Hermosillo, Sonora, 83190 (Mexico)

    2005-11-07

    The thermoluminescence (TL) and optically stimulated luminescence (OSL) characterization of Er{sup 3+} and Yb{sup 3+} doped Y{sub 3}Al{sub 5}O{sub 12} nanocrystalline samples prepared by the precipitation process and exposed to {beta}-rays are discussed. The TL as well as the OSL were two orders of magnitude higher in Er{sup 3+} doped than in Yb{sup 3+} specimens. The charge trapping and the radiative thermally stimulated recombination processes in Y{sub 3}Al{sub 5}O{sub 12} : Er{sup 3+} involve four trapping states at 166, 243, 342 and 424 deg. C, but just two trapping levels at 219 and 413 deg. C for Y{sub 3}Al{sub 5}O{sub 12} : Yb{sup 3+} at a heating rate of 10 deg. C s{sup -1}. The photostimulation with 470 nm light causes in both phosphors a radiative recombination of the optically free charge carriers belonging to the same trapping states. The TL and the OSL as a function of radiation dose behaviour were linear in the 10-100 Gy dose range. The results provide evidence of the potential uses of these materials in radiation storage and dosimeter devices.

  7. Evaluation of environmental dose at JCO using luminescence from quartz stimulated by blue light.

    Science.gov (United States)

    Hong, D G; Galloway, R B; Takano, M; Hashimoto, T

    2001-01-01

    The environmental dose due to the recent nuclear accident at JCO, Japan, was estimated using luminescence optically stimulated from unheated quartz. Two methods originally developed for dating analysis, the single aliquot additive dose method and the single aliquot regeneration added dose method, were employed to confirm the dose rate. Consistent results were obtained from both methods and from thermoluminescence measurements. Although the dose rate values had lower precision than can be obtained from heated materials, it is suggested that luminescence from sedimentary quartz can usefully be employed in retrosepective dosimetry.

  8. Luminescent probes for optical in vivo imaging

    Science.gov (United States)

    Texier, Isabelle; Josserand, Veronique; Garanger, Elisabeth; Razkin, Jesus; Jin, Zhaohui; Dumy, Pascal; Favrot, Marie; Boturyn, Didier; Coll, Jean-Luc

    2005-04-01

    Going along with instrumental development for small animal fluorescence in vivo imaging, we are developing molecular fluorescent probes, especially for tumor targeting. Several criteria have to be taken into account for the optimization of the luminescent label. It should be adapted to the in vivo imaging optical conditions : red-shifted absorption and emission, limited overlap between absorption and emission for a good signal filtering, optimized luminescence quantum yield, limited photo-bleaching. Moreover, the whole probe should fulfill the biological requirements for in vivo labeling : adapted blood-time circulation, biological conditions compatibility, low toxicity. We here demonstrate the ability of the imaging fluorescence set-up developed in LETI to image the bio-distribution of molecular probes on short times after injection. Targeting with Cy5 labeled holo-transferrin of subcutaneous TS/Apc (angiogenic murine breast carcinoma model) or IGROV1 (human ovarian cancer) tumors was achieved. Differences in the kinetics of the protein uptake by the tumors were evidenced. IGROV1 internal metastatic nodes implanted in the peritoneal cavity could be detected in nude mice. However, targeted metastatic nodes in lung cancer could only be imaged after dissection of the mouse. These results validate our fluorescence imaging set-up and the use of Cy5 as a luminescent label. New fluorescent probes based on this dye and a molecular delivery template (the RAFT molecule) can thus be envisioned.

  9. Luminescence techniques: Instrumentation and methods

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.

    1997-01-01

    This paper describes techniques, instruments and methods used in luminescence dating and environmental dosimetry in many laboratories around the world. These techniques are based on two phenomena - thermally stimulated luminescence and optically stimulated luminescence. The most commonly used...... luminescence stimulation and detection techniques are reviewed and information is given on recent developments in instrument design and on the stale of the art in luminescence measurements and analysis. (C) 1998 Elsevier Science Ltd. All rights reserved....

  10. Optically stimulated luminescence and thermoluminescence in CVD diamond and dosimetric evaluation in fields of ionizing radiation; Luminiscencia opticamente estimulada y termoluminiscencia en diamante DQV y evaluacion dosimetrica en campos de radiacion ionizante

    Energy Technology Data Exchange (ETDEWEB)

    Barboza F, M.; Chernov, V.; Pedroza M, M. [Centro de Investigaciones en Fisica, Universidad de Sonora, A.P. 5-088, 83190 Hermosillo, Sonora (Mexico); Schreck, M. [Universitat Augsburg, Institut fur Physik D-86135, Augsburg (Germany); Preciado F, S.; Melendrez, R. [Universidad de Sonora, A.P. 130, 83000 Hermosillo, Sonora (Mexico)

    2006-07-01

    The optically stimulated luminescence (OSL) results a highly appropriate dosimetric technique for readings of absorbed radiation 'in alive' and 'in situ', as well as in real time. The CVD diamond on the other hand presents excellent qualities like radiation reader thanks to its reproducibility, radiation resistance, biocompatibility and non toxicity. The present work studies the answer of two diamond films pure and polluted with nitrogen (750 ppm) grown by the Chemical Vapor Deposition method (CVD) on silicon substrate (001) irradiated with beta (Sr-90) in the 0.833-100 Gy interval. The optical stimulation was carried out by 40 seconds with infrared laser (830 nm, 0.36 W/cm{sup 2}) and the filter BG-39 (300-600 nm) coupled the PM. The intensity and the decay of the hyperbolic type of the LOE curves were similar in both samples, for the non doped diamond were observed trapping states in 200-380 C being compared with those that it presents the polluted diamond with nitrogen in 80-277 C. The dosimetric behavior in the pure sample is observed lineal in two regions 0-16 Gy and in 30-100 Gy, only the doped sample didn't present linearity in the all range of the studied dose. The advantage is stood out of LOE on TL because the first one not requires of thermal stimulation in such a way that is more appropriate to detect and to measure radiation doses in biomedicine. (Author)

  11. Thermoluminescence and optically stimulated luminescence properties of Dy{sup 3+}-doped CaO–Al{sub 2}O{sub 3}–B{sub 2}O{sub 3}-based glasses

    Energy Technology Data Exchange (ETDEWEB)

    Yahaba, T., E-mail: takuma.yahaba.s1@dc.tohoku.ac.jp [Department of Applied Chemistry, Graduate School of Engineering, Tohoku University, 6-6-07 Aramaki Aza Aoba, Aoba-ku, Sendai 980-8579 (Japan); Fujimoto, Y. [Department of Applied Chemistry, Graduate School of Engineering, Tohoku University, 6-6-07 Aramaki Aza Aoba, Aoba-ku, Sendai 980-8579 (Japan); Yanagida, T. [Nara Institute of Science and Technology (NAIST), 8916-5 Takayama, Ikoma 630-0192 (Japan); Koshimizu, M.; Tanaka, H.; Saeki, K.; Asai, K. [Department of Applied Chemistry, Graduate School of Engineering, Tohoku University, 6-6-07 Aramaki Aza Aoba, Aoba-ku, Sendai 980-8579 (Japan)

    2017-02-01

    We developed Dy{sup 3+}-doped CaO–Al{sub 2}O{sub 3}–B{sub 2}O{sub 3} based glasses with Dy concentrations of 0.5, 1.0, and 2.0 mol% using a melt-quenching technique. The as-synthesized glasses were applicable as materials exhibiting thermoluminescence (TL) and optically stimulated luminescence (OSL). The optical and radiation response properties of the glasses were characterized. In the photoluminescence (PL) spectra, two emission bands due to the {sup 4}F{sub 9/2} → {sup 6}H{sub 15/2} and {sup 4}F{sub 9/2} → {sup 6}H{sub 13/2} transitions of Dy{sup 3+} were observed at 480 and 580 nm. In the OSL spectra, the emission band due to the {sup 4}F{sub 9/2} → {sup 6}H{sub 15/2} transition of Dy{sup 3+} was observed. Excellent TL and OSL responses were observed for dose ranges of 0.1–90 Gy. In addition, TL fading behavior was better than that of OSL in term of the long-time storage. These results indicate that the Dy{sup 3+}-doped CaO–Al{sub 2}O{sub 3}–B{sub 2}O{sub 3}-based glasses are applicable as TL materials.

  12. 荧光玻璃、热释光和光释光探测器性能比较%Comparison on Characteristics of Radiophotoluminescent Glass,Thermoluminescence and Optically Stimulated Luminescence

    Institute of Scientific and Technical Information of China (English)

    樊海军; 唐开勇; 崔辉; 刘正

    2011-01-01

    It is to review that the principle of radiophotoluminescence glass detectors( RPLCD) , thermolumines-cence detectors (TLD)and Optically Stimulated luminescence (OSL) detectors ,and compare their advantages and disadvantages and some recent developments in luminescence of detectors. The major advantage of RPLCD is long - term stability and capability of repeating readout. The major advantage of TLD and OSL detectors are high sensitivity, low detection threshold, good fading effect, good energy response after γ - ray irradiation (for materials with Zeff close to that of tissue) , resistance to high humidity and to high magnetic fields. Compare with IiF:Mg,Cu,P,however,the OSL of is very high sensitivity to visible light and relative high effective atomic number(10.2).%介绍了荧光玻璃探测器、热释光探测器和光释光探测器基本原理和近期发展,并总结了荧光玻璃、热释光探测器、光释光探测器的优缺点.荧光玻璃最大优点是长期稳定性好和可多次读取.热释光和光释光探测器具有灵敏度高、低探测阈、较好的稳定性和能量响应、环境适应性强等优点.但与LiF:Mg,Cu,P相比,α- Al2O3:C光释光探测器对可见光敏感和具有较高的有效原子序数(10.2).

  13. Discussions of Optical Stimulated Luminescence Dating about Colluvial Deposits in Lintong-chang'an Fault%临潼-长安断裂上断层崩积楔光释光测年的探讨

    Institute of Scientific and Technical Information of China (English)

    李晓妮; 田勤虎; 李高阳; 李苗; 李娟

    2011-01-01

    选择西安临潼-长安断裂带上韩峪乡范家村剖面的一个典型崩积楔样品进行测试.用3种不同的释光测试方法测出了9个不同的年龄数据.根据地层信息和矿物的释光生长曲线确定只有采用混合矿物简单多片再生法、纯石英矿物简单多片再生法以及纯石英矿物单片再生法的光释光测年法所得结果更接近于崩积楔的真实年龄.这些断层崩积楔年龄接近于围岩的形成年龄,并不能代表真正意义上的断层活动时代.因此,断层崩积楔年龄光释光测年结果无法给出该断层最真实的活动时代.%This article choosed Fanjiacun profile in Iintong-chang'an fault as a typical fault gouge samples testing and used three different methods to obtain nine different age data. According to stratum information and minerals luminescence growth curve, the paper determined only three dating method. They are mixed minerals multiple aliquot regenerative dose protocol, fine grained quartz multiple aliquot regenerative dose protocol and fine grained quartz single aliquot regenerative dose protocol. These fault wedge ages are close to collapse product of surrounding rock formation age but can't represent real fault activity era. So we conclude that optical stimulated luminescence age results of colluvial deposit can't give real activity age about fault.

  14. Violet stimulated luminescence dating of quartz from Luochuan (Chinese loess plateau)

    NARCIS (Netherlands)

    Ankjærgaard, C.; Guralnik, B.; Buylaert, J.P.; Reimann, T.; Yi, S.W.; Wallinga, J.

    2016-01-01

    Luminescence dating at the Luochuan loess type (China) section is at present limited to ∼0.1 Ma using quartz blue light stimulated luminescence (BLSL), but can be extended back in time to ∼0.5 Ma by resorting to the more developmental post-infrared infrared stimulated luminescence (post-IR IRSL)

  15. Red-IR stimulated luminescence in K-feldspar: Single or multiple trap origin?

    Science.gov (United States)

    Thalbitzer Andersen, Martin; Jain, Mayank; Tidemand-Lichtenberg, Peter

    2012-08-01

    We investigate on the origins of the infra-red stimulated luminescence (IRSL) signals in 3 potassium feldspars based on IR-red spectroscopy (˜700-1050 nm) using a fiber-coupled tunable Ti:Sapphire laser, in combination with different thermal and optical (pre)treatments of the samples. We also measure dose-response curves with different wavelengths and at different stimulation temperatures so as to be able to distinguish between traps based on their electron trapping cross-sections. Our data suggest that the dosimetric signals, IRSL, and the post IR-IRSL in K-feldspars arise from a single electron trapping centre.

  16. Measurement of Tumor Dose Using Optically Stimulated Luminescence Detectors (OSLDs) and Ionization Chambers for Primary and Metastatic Lymph Node Cancers with Head and Neck: Comparison of Beam Spoiler and Bolus

    Energy Technology Data Exchange (ETDEWEB)

    Lee, Jeong Ok [Dept. of Radiotechnology, Wonkwang Health Science University, Iksan (Korea, Republic of); Lee, Jae Seung [Dept. of Physics, Soonchunhyang University, Seoul (Korea, Republic of); Jeong, Dong Hyeok [Research center, Dongnam Inst. of Radiological and Medical Science, Busan (Korea, Republic of)

    2011-09-15

    This study conducts cross-comparison through verification of treatment planning of using beam spoiler and bolus, according to the dose variation of different tumor bed and metastatic lymph node cancers, against ionization and optically stimulated luminescence detectors(OSLDs), in head and neck radiotherapy. Verification of treatment planning examined the feasibility of inserting detectors through simulated solid dry water slabs under identical irradiated conditions from treatment planning system to measure beam spoiler and 0.5, 1 cm bolus. In addition, two detectors were cross-compared for verification of treatment planning accuracy and reliability within {+-} 2%. The study found that, given a beam spoiler thickness of 0.5 cm and beam spoiler-to-skin distance of 10 cm subjected to optimal dose distribution given for metastatic lymph node cancers, the bolus low-level skin dose was less, and the tumor bed dose reduced slightly. Additionally, two detectors were cross-compared for accuracy within {+-} 1%. Accordingly, The use of beam spoiler was determined that reduces skin side effects and can deliver an optimal dose distribution for tumor, and to apply to future clinical studies should be performed.

  17. Solid-state luminescence for the optical examination of archaeological glass beads

    Science.gov (United States)

    Zacharias, N.; Beltsios, K.; Oikonomou, A.; Karydas, A. G.; Bassiakos, Y.; Michael, C. T.; Zarkadas, Ch.

    2008-03-01

    The work pertains to the application of solid-state luminescence as a characterization tool for glassy ceramic cultural artefacts. An archaeological glass bead collection excavated at the city of Thebes, Greece and considered as unique in terms of typological variety and time span was examined with the application of luminescence techniques (thermoluminescence, optically stimulated luminescence). Additionally, X-rays fluorescence (XRF) was used to provide non-destructively the elemental concentration profile of the samples. The thermoluminescence signals following laboratory irradiation provided distinct groups of spectra types according to the color classification of the samples. For each sample, the signal sensitivity and growth were examined using both thermoluminescence and optically stimulated luminescence recording. The study provides evidence for the usefulness of the combined application of luminescence and non-destructive, XRF-based, elemental analysis for the characterization of glass assemblages. Finally, due to the satisfactory level of radiation-induced signal intensity, the work suggests the possibility of chronological estimation of ancient glass beads using luminescence dating protocols.

  18. Optically stimulated differential impedance spectroscopy

    Science.gov (United States)

    Maxey, Lonnie C; Parks, II, James E; Lewis, Sr., Samuel A; Partridge, Jr., William P

    2014-02-18

    Methods and apparatuses for evaluating a material are described. Embodiments typically involve use of an impedance measurement sensor to measure the impedance of a sample of the material under at least two different states of illumination. The states of illumination may include (a) substantially no optical stimulation, (b) substantial optical stimulation, (c) optical stimulation at a first wavelength of light, (d) optical stimulation at a second wavelength of light, (e) a first level of light intensity, and (f) a second level of light intensity. Typically a difference in impedance between the impedance of the sample at the two states of illumination is measured to determine a characteristic of the material.

  19. Concerning infrared-stimulated luminescence from K-feldspars: evidence from heating before stimulating

    CERN Document Server

    Galloway, R B

    1999-01-01

    Repeated heating and stimulation by infrared of feldspar samples causes a reduction in the luminescence signal. Two feldspars were investigated, one microcline and one orthoclase. Empirically the fraction of luminescence signal f(n) remaining after the nth cycle of heating and stimulation is given by f(n)=1-a ln(n) for laboratory dosed samples of both microcline and orthoclase feldspars, for heating temperatures of 150 deg. C, 180 deg. C and 220 deg. C, for heating durations per cycle ranging from 20 s to 2400 s and with the study covering 10 cycles of heating and stimulation. Logarithmic decay of luminescence with time has been explained previously, in other contexts, as due either to quantum tunnelling or to a continuous distribution of states being involved but it is shown that these explanations do not fit the present data. The measured data on f(n) were corrected for the loss of luminescence due to infrared stimulation to ensure that this did not account for the differences between the data and the expec...

  20. Ce doped hafniate scintillating glasses thermally stimulated luminescence and photoluminescence

    CERN Document Server

    Martini, M; Vedda, A; Dafinei, I; Lecoq, P; Nikl, M

    1995-01-01

    Thermally stimulated luminescence (TSL) and time resolved luminescence studies have been performed on undoped, and Ce3+ and Mn2+ doped fluoro-hafniate glasses (HFG). The X-ray induced TSL glow curve above room temperature features different broad structures extending up to 350 degree C; wavelength resolved measurements put in evidence the existence of two distinct emission peaks around 300 nm and 550 nm, attributed to Ce3+ and Mn2+ ions respectively. The role of Ce3+ and Mn2+ dopant ions in the trapping-recombination TSL processes was investigated, on the basis of the analysis of the spectral distribution of the emitted light at different dopant ions concentrations, and of the dose dependencies of the signals. Time resolved luminescence measurements allowed a detailed characterization of both Ce3+ and Mn2+ emissions. Their decay times were found to be 19.2 ns and 27 ms, respectively; the excitation spectrum of the 550 nm emission revealed the existence of a radiative energy transfer between Ce3+ and Mn2+ cent...

  1. Optically stimulated luminescence response to ionizing radiation of red bricks (SiO{sub 2}, Al{sub 2}O{sub 3} an Fe{sub 2}O{sub 3}) used as building materials

    Energy Technology Data Exchange (ETDEWEB)

    Espinosa, G.; Golzarri, J. I.; Santiago, P. [Instituto de Fisica, UNAM, Apartado Postal 20-364, 01000 Mexico D. F. (Mexico); Bogard, J. S. [Oak Ridge National Laboratory, P.O. Box 2008, Oak Ridge TN 37831-6426 (United States)]. e-mail: espinosa@fisica.unam.mx

    2008-02-15

    Quartz is the most common mineral in our environment. It is found in granite, hydrothermal veins and volcanic rocks, as well as in sedimentary deposits derived from such solid materials. These sediments are also made into building materials, such as bricks and pottery. Thus the potential use of a dose reconstruction technique based on quartz grains is enormous, whether as a dating tool in archaeology and quaternary geology, or in nuclear accident dosimetry. This work describes the Optically Stimulated Luminescence (OSL) response of red brick to ionizing radiation. The bricks, from the state of Puebla, Mexico, represent another class of materials that can be used in retrospective dosimetry following nuclear or radiological incidents. The chemical composition of fifteen bricks (three samples from five different brick factories) was determined, using energy dispersive spectroscopy, be primarily SiO{sub 2}, Al{sub 2}0{sub 3} and Fe{sub 2}O{sub 3} and is believed to be representative for this common building material. Individual aliquots from these bricks were powdered in agate mortars and thermally annealed. Replicate samples of the aliquots were then irradiated with beta particles from a sealed source of {sup 9}0Sr/{sup 9}0Y. The OSL response was measured with a Daybreak Model 2200 High-Capacity OSL Reader System. We present here for this material the characteristic OSL response to beta particles; the reproducibility of the OSL response; the linearity of the response in the dose range 0.47 Gy to 47 Gy; and the fading characteristics. (Author)

  2. Real-time optical-fibre luminescence dosimetry for radiotherapy: physical characteristics and applications in photon beams

    DEFF Research Database (Denmark)

    Aznar, M.C.; Andersen, C.E.; Bøtter-Jensen, L.;

    2004-01-01

    A new optical-fibre radiation dosimeter system, based on radioluminescence and optically stimulated luminescence from carbon-doped aluminium oxide, was developed and tested in clinical photon beams. This prototype offers several features, such as a small detector (1 x 1 x 2 mm), high sensitivity...

  3. 光释光测年在海岸风沙地貌研究中的新进展%PROGRESS IN OPTICAL STIMULATED LUMINESCENCE DATING FOR COASTAL AEOLIAN GEOMORPHOLOGY RESEARCH : A REVIEW

    Institute of Scientific and Technical Information of China (English)

    谢丽; 张振克

    2011-01-01

    Since the mid-1980's much progress has been made in the use of optical stimulated luminescence (OSL) dating method into the studies of coastal aeolian sediments. OSL is one of the important dating methods used in Quaternary geology and archeology. In this paper the main achievements and advances in OSL dating of coastal aeolian sediments were summarized. With the development of the stimulating light source and OSL dating methods itself, more accurate dating results of the coastal aeolian sediments could be obtained. The improvement of OSL dating methods, such as the single aliquot additive dose protocol and the single aliquot regenerative dose protocol,has expanded the dating range and enhanced the precision of OSL dating. The youngest age of coastal aeolian sediments,which have been dated by OSL dating,is within 10 years,and the oldest one is over 900 thousands years. A great deal of researches in this field focus on the evolution of coastal aeolian dune and its relationship with global climate changes in the past. With the ongoing development of OSL dating technology, sandy coast evolution, regional climatic changes and sea level changes will be studied deeply and widely in the near future.%20世纪80年代中期以来,光释光技术广泛应用于海岸风沙沉积物测年研究中,并取得了丰硕的成果.随着光释光测年激发光源和单片再生剂量方法的快速发展,海岸风沙光释光测年的时间范围不断扩大,测年的准确度逐渐提高,已测得最年轻的海岸风沙沉积物的年龄小于10年,最老的年龄达到90多万年.利用光释先年龄重建海岸风沙演化进程及其与全球气候变化关系的研究,正成为学术界关注的焦点,光释光测年方法在将来的砂质海岸演化、区域气候变化及海平面变化等全球变化问题的研究中具有广阔发展前景.

  4. Time-resolved luminescence from quartz

    NARCIS (Netherlands)

    Chithambo, M.L.; Ankjærgaard, C.; Pagonis, V.

    2016-01-01

    Time-resolved optical stimulation of luminescence has become established as a key method for measurement of optically stimulated luminescence from quartz, feldspar and α-Al2O3:C, all materials of interest in dosimetry. The aim of time-resolved optical stimulation is to separ

  5. Quantitative analysis of time-resolved infrared stimulated luminescence in feldspars

    DEFF Research Database (Denmark)

    Pagonis, Vasilis; Ankjærgaard, Christina; Jain, Mayank;

    2016-01-01

    Time-resolved infrared-stimulated luminescence (TR-IRSL) from feldspar samples is of importance in the field of luminescence dating, since it provides information on the luminescence mechanism in these materials. In this paper we present new analytical equations which can be used to analyze TR......-IRSL signals, both during and after short infrared stimulation pulses. The equations are developed using a recently proposed kinetic model, which describes localized electronic recombination via tunneling between trapped electrons and recombination centers in luminescent materials. Recombination is assumed...

  6. Thermally stimulated luminescence studies in combustion synthesized polycrystalline aluminum oxide

    Indian Academy of Sciences (India)

    K R Nagabhushana; B N Lakshminarasappa; D Revannasiddaiah; Fouran Singh

    2008-08-01

    Synthesis of materials by combustion technique results in homogeneous and fine crystalline product. Further, the technique became more popular since it not only saved time and energy but also was easy to process. Aluminum oxide phosphor was synthesized by using urea as fuel in combustion reaction. Photoluminescence (PL) and thermally stimulated luminescence (TSL) characteristics of -irradiated aluminum oxide samples were studied. A broad PL emission with a peak at ∼ 465 nm and a pair of strong and sharp emissions with peaks at 679 and 695 nm were observed in -rayed samples. The PL intensity was observed to increase with increase in -ray dose. Two prominent and well resolved TSL glows with peaks at 210°C and 365°C were observed in all -irradiated Al2O3 samples. The TSL intensity was also found to increase with increase in -ray dose. The TSL glow curves indicated second order kinetics.

  7. Identifying irradiated flours by photo-stimulated luminescence technique

    Science.gov (United States)

    Ramli, Ros Anita Ahmad; Yasir, Muhamad Samudi; Othman, Zainon; Abdullah, Wan Saffiey Wan

    2014-02-01

    Photo-stimulated luminescence (PSL) technique was used in this study to detect gamma irradiation treatment of five types of flours (corn, rice, tapioca, wheat and glutinous rice) at four different doses 0, 0.2, .05 and 1kGy. The signal level was compared with two threshold values (700 and 5000). With the exception of glutinous rice, all irradiated samples produced a strong signal above the upper threshold (5000 counts/60s). All control samples produced negative result with the signals below the lower threshold (700 counts/60s) suggesting that the samples have not been irradiated. Irradiated glutinous rice samples produced intermediate signals (700 - 5000 counts/60s) which were subsequently confirmed using calibrated PSL. The PSL signals remained stable after 90 days of storage. The findings of this study will be useful to facilitate control of food irradiation application in Malaysia.

  8. Identifying irradiated flours by photo-stimulated luminescence technique

    Energy Technology Data Exchange (ETDEWEB)

    Ramli, Ros Anita Ahmad; Yasir, Muhamad Samudi [Faculty of Science and Technology, National University of Malaysia, Bangi, 43000 Kajang, Selangor (Malaysia); Othman, Zainon; Abdullah, Wan Saffiey Wan [Malaysian Nuclear Agency, Bangi 43000 Kajang, Selangor (Malaysia)

    2014-02-12

    Photo-stimulated luminescence (PSL) technique was used in this study to detect gamma irradiation treatment of five types of flours (corn, rice, tapioca, wheat and glutinous rice) at four different doses 0, 0.2, .05 and 1kGy. The signal level was compared with two threshold values (700 and 5000). With the exception of glutinous rice, all irradiated samples produced a strong signal above the upper threshold (5000 counts/60s). All control samples produced negative result with the signals below the lower threshold (700 counts/60s) suggesting that the samples have not been irradiated. Irradiated glutinous rice samples produced intermediate signals (700 - 5000 counts/60s) which were subsequently confirmed using calibrated PSL. The PSL signals remained stable after 90 days of storage. The findings of this study will be useful to facilitate control of food irradiation application in Malaysia.

  9. Up-Conversion Photostimulated Luminescence of Mg2SnO4 for Optical Storage

    Institute of Scientific and Technical Information of China (English)

    ZHANG Jia-Chi; QIN Qing-Song; YU Ming-Hui; SUN Jia-Yao; SHI Liu-Rong; MA Xin-Long

    2011-01-01

    @@ We report the first observation of up-conversion photostimulated luminescence in non-doped Mg2SnO4.Stimulated by 980 nm infrared laser (reading) after ultraviolet irradiation (writing), the phosphor shows photostimulated emission band covering 470-550nm, which is due to the recombination of F centers with holes.After ceasing ultraviolet irradiation, the storage intensity would rapidly decrease to 59% of its original storage intensity in 2.5h and then would not degrade anymore.It is suggested that the Mg2SnO4 has potential applications for optical storage.Accordingly, the possible photostimulated luminescence mechanisms of Mg2SnO4 are proposed.%We report the first observation of up-conversion photostimulated luminescence in non-doped Mg2SnO4. Stimulated by 980 nm infrared laser (reading) after ultraviolet irradiation (writing), the phosphor shows photostimulated emission band covering 470-550nm, which is due to the recombination of F centers with holes. After ceasing ultraviolet irradiation, the storage intensity would rapidly decrease to 59% of its original storage intensity in 2.5 h and then would not degrade anymore. It is suggested that the Mg2SnO4 has potential applications for optical storage. Accordingly, the possible photostimulated luminescence mechanisms of Mg2SnO4 are proposed.

  10. Optically stimulated luminescence in retrospective dosimetry

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.; Murray, A.S.

    2002-01-01

    of this programme, including the evaluation of the single-aliquot regenerative-dose (SAR) measurement protocol with brick quartz and the determination of dose-depth profiles in building materials as a guide to determining the mean energy of the incident radiation. Investigations into heated materials are most...... advanced, and a lower detection limit for quartz extracted from Chernobyl bricks was determined to be aliquot and single-grain techniques have been used...

  11. Luminescence chronology of a second millenium BCE settlement near Porbandar on the Gujarat coast, India

    Digital Repository Service at National Institute of Oceanography (India)

    Gaur, A.S.; Thomas, P.J.; Vora, K.H.; Sundaresh

    ) and optically stimulated luminescence (OSL) dating of two potshards. The obtained luminescence ages are found to be in agreement with other archaeological findings. The implications of the luminescence ages on the maritime history of the area and the cultural...

  12. Electronic displays using optically pumped luminescent semiconductor nanocrystals

    Science.gov (United States)

    Weiss, Shimon; Schlamp, Michael C.; Alivisatos, A. Paul

    2011-09-27

    A multicolor electronic display is based on an array of luminescent semiconductor nanocrystals. Nanocrystals which emit light of different colors are grouped into pixels. The nanocrystals are optically pumped to produce a multicolor display. Different sized nanocrystals are used to produce the different colors. A variety of pixel addressing systems can be used.

  13. Electronic displays using optically pumped luminescent semiconductor nanocrystals

    Science.gov (United States)

    Weiss, Shimon; Schlam, Michael C; Alivisatos, A. Paul

    2014-03-25

    A multicolor electronic display is based on an array of luminescent semiconductor nanocrystals. Nanocrystals which emit tight of different colors are grouped into pixels. The nanocrystals are optically pumped to produce a multicolor display. Different sized nanocrystals are used to produce the different colors. A variety of pixel addressing systems can be used.

  14. Characterisation of blue-light stimulated luminescence components in different quartz samples: implications for dose measurement

    Energy Technology Data Exchange (ETDEWEB)

    Jain, M. E-mail: mayank.jain@risoe.dk; Murray, A.S.; Boetter-Jensen, L

    2003-10-01

    Over the last few years, we have become increasingly confident that quartz is a reliable natural dosimeter for sediment dating. Nevertheless, there is only a limited understanding of the behaviour of the different components of optically stimulated luminescence (OSL) from quartz. Recent single-aliquot dose-evaluation protocols seem to be relatively free of complications when applied to quartz dominated by the fast OSL component coming from 325 deg. C TL region, but this may not be true for quartz in which other components are more significant. An adequate understanding of how different OSL components behave during various measurement cycles is critical to ensuring that our dose evaluation protocols are robust and it is also important to our interpretation of the variation of apparent dose with optical stimulation time for identification of partial bleaching. We report here the principal results from measurement of (a) sensitisation, (b) thermal stability, (c) recuperation, and (d) infrared response as a function of stimulation temperature from 3 different samples of sedimentary quartz selected on the basis of relative OSL contribution from different blue light stimulated linearly modulated (LM-OSL) components. We then discuss the implications of these characteristics for dose assessment using the single aliquot regeneration dose protocol.

  15. Quantitative analysis of time-resolved infrared stimulated luminescence in feldspars

    Energy Technology Data Exchange (ETDEWEB)

    Pagonis, Vasilis, E-mail: vpagonis@mcdaniel.edu [McDaniel College, Physics Department, Westminster, MD 21157 (United States); Ankjærgaard, Christina [Soil Geography and Landscape Group & Netherlands Centre for Luminescence dating, Wageningen University, PO Box 47, 6700 AA Wageningen (Netherlands); Jain, Mayank [Center for Nuclear Technologies, Technical University of Denmark, DTU Risø Campus, Roskilde (Denmark); Chithambo, Makaiko L. [Department of Physics and Electronics, Rhodes University, PO BOX 94, Grahamstown 6140 (South Africa)

    2016-09-15

    Time-resolved infrared-stimulated luminescence (TR-IRSL) from feldspar samples is of importance in the field of luminescence dating, since it provides information on the luminescence mechanism in these materials. In this paper we present new analytical equations which can be used to analyze TR-IRSL signals, both during and after short infrared stimulation pulses. The equations are developed using a recently proposed kinetic model, which describes localized electronic recombination via tunneling between trapped electrons and recombination centers in luminescent materials. Recombination is assumed to take place from the excited state of the trapped electron to the nearest-neighbor center within a random distribution of luminescence recombination centers. Different possibilities are examined within the model, depending on the relative importance of electron de-excitation and recombination. The equations are applied to experimental TR-IRSL data of natural feldspars, and good agreement is found between experimental and modeling results.

  16. Luminescence and scintillation properties of YAG:Ce single crystal and optical ceramics

    CERN Document Server

    Mihóková, E; Mareš, J A; Beitlerová, A; Vedda, A; Nejezchleb, K; Blažek, K; D’Ambrosio, C

    2007-01-01

    We use various techniques to study optical and scintillation properties of Ce-doped yttrium aluminum garnet, Y3Al5O12 (YAG:Ce), in the form of a high-quality industrial single crystal. This was compared to optical ceramics prepared from YAG:Ce nanopowders. We present experimental data in the areas of optical absorption, radioluminescence, scintillation decay, photoelectron yield, thermally stimulated luminescence and radiation-induced absorption. The results point to an interesting feature—the absence of antisite (YAl, i.e. Y at the Al site) defects in optical ceramics. The scintillation decay of the ceramics is faster than that of the single crystal, but its photoelectron yield (measured with 1 μs integration time) is about 30–40% lower. Apart from the photoelectron yield value the YAG:Ce optical ceramic is fully comparable to a high quality industrial YAG:Ce single crystal and can become a competitive scintillator material.

  17. Measuring modulated luminescence using non-modulated stimulation: ramping the sample period

    Energy Technology Data Exchange (ETDEWEB)

    Poolton, N.R.J. E-mail: n.r.j.poolton@dl.ac.uk; Boetter-Jensen, L.; Andersen, C.E.; Jain, M.; Murray, A.S.; Malins, A.E.R.; Quinn, F.M

    2003-12-01

    Conventional methods of recording linearly modulated (LM) optically stimulated luminescence (OSL) require control over either the exciting light intensity, or the ability to pulse the source. For many light sources (e.g. constant-power CW lasers, arc lamps and synchrotrons) this can be problematic. Directly analogous results to LM-OSL can, however, be achieved with non-modulated excitation sources, by ramping the sample period (RSP) of luminescence detection. RSP-OSL has the distinct advantage over LM-OSL in that, since the excitation remains at full power, data accumulation times (that can be considerable) can be reduced by typically 50%. RSP methods are universally applicable and can be employed, for example, where the excitation source is constant heat, rather than light: here, iso-thermal decay of phosphorescence becomes recorded as a sequence of peaks, corresponding to de-trapping of charge from different defect levels, and is particularly useful for analysing shallow-trap effects. RSP methods are also useful in providing significant compaction of data sets, where signal analysis is required of overlapping systems having a wide range of decay kinetics.

  18. Dependence of (anomalous) fading of infra-red stimulated luminescence on trap occupancy in feldspars

    DEFF Research Database (Denmark)

    Morthekai, P.; Jain, Mayank; Gach, Grzegorz

    2013-01-01

    Dose dependency of anomalous fading of infra-red stimulated luminescence (IRSL) from feldspars has been investigated using radiations of different ionisation qualities. The rate of fading of the IRSL signal after proton irradiation (9.4–30%/decade) is on an average almost twice compared to that a......Dose dependency of anomalous fading of infra-red stimulated luminescence (IRSL) from feldspars has been investigated using radiations of different ionisation qualities. The rate of fading of the IRSL signal after proton irradiation (9.4–30%/decade) is on an average almost twice compared...

  19. Na-rich feldspar as a luminescence dosimeter in infrared stimulated luminescence (IRSL) dating

    DEFF Research Database (Denmark)

    Sohbati, Reza; Murray, Andrew; Jain, Mayank;

    2013-01-01

    on geological origin and erosion history, but the dosimetry of K-rich feldspar grains extracted from rocks is complicated because the internal dose rate is very dependent on the original feldspar grain size. The in situ grain size information is lost during the crushing process used to separate the grains...... are in agreement with the expected age control, raising the possibility that this signal originates mainly from K-rich feldspar contamination in our Na-rich fractions, and thus is not so useful in the luminescence dating of rock surfaces. On the other hand, the pIRIR290 fading-corrected ages based on the yellow......One of the challenges in dating rock surfaces is the choice of the luminescence mineral. Although quartz is the preferred dosimeter in sediment dating, it is often not sufficiently sensitive when extracted from solid rocks. The intensity of signals from feldspars tends to be much less dependent...

  20. Combining infrared- and green-laser stimulation sources in single-grain luminescence measurements of feldspar and quartz

    Energy Technology Data Exchange (ETDEWEB)

    Duller, G.A.T. E-mail: ggd@aber.ac.uk; Boetter-Jensen, L.; Murray, A.S

    2003-10-01

    A system designed for measurement of the optically stimulated luminescence (OSL) from individual sand-sized mineral grains has been constructed. Previously, this system was equipped only with a green laser emitting at 532 nm, but now an infrared (IR) laser at 830 nm has been added. It is now possible to interchangeably use the two laser sources for optical stimulation. This is especially valuable for the measurement of feldspars. The power density using the IR laser at the grain is {approx}500 W cm{sup -2}, and stimulation for 1 s reduces the OSL signal to near background level. Initial results on grains from two feldspar samples are described. These show that the ratio of the OSL signal under green and IR stimulation is similar for all the feldspar grains. As expected, the ratio for quartz grains is very different, with a much weaker signal when using IR stimulation. For the two feldspars, the distribution of OSL between the grains and the saturation of the dose response curve shows much less variability than is typically seen for quartz grains.

  1. Stimulation of mineral-specific luminescence from multi-mineral samples

    DEFF Research Database (Denmark)

    Duller, G.A.T.; Bøtter-Jensen, L.; Poolton, N.R.J.

    1995-01-01

    Grains of quartz and potassium-rich feldspar have been mixed in known ratios to produce samples of known mineralogical composition, analogous to those found in natural sedimentary deposits. The variation of the green light stimulated luminescence (GLSL), as a function of sample temperature......, was measured for each of these mixtures in order to attempt to isolate a luminescence signal that originates specifically from just one of the components. As the sample is heated from room temperature to 450 degrees C, thermal quenching reduces the signal from the quartz component to near zero, while that from...

  2. Method of measuring luminescence of a material

    Science.gov (United States)

    Miller, Steven D.

    2015-12-15

    A method of measuring luminescence of a material is disclosed. The method includes applying a light source to excite an exposed material. The method also includes amplifying an emission signal of the material. The method further includes measuring a luminescent emission at a fixed time window of about 10 picoseconds to about 10 nanoseconds. The luminescence may be radio photoluminescence (RPL) or optically stimulated luminescence (OSL).

  3. Optical characterization of luminescent silicon nanocrystals embedded in glass matrices

    Energy Technology Data Exchange (ETDEWEB)

    Debieu, Olivier

    2008-12-16

    Interstellar dust in nebulae and in the Diffuse Interstellar Medium (DISM) of galaxies contains a component which exhibits efficient visible-near infrared luminescence ranging from 500 to 1000 nm, known as Extended Red Emission (ERE). Silicon nanocrystals (nc-Si) are discussed as possible carriers of the ERE. We employed the accelerator facilities of the Institute of Solid State Physics of the University of Jena to implant Si ions into fused silica windows. An excess concentration of silicon atoms is thus produced in the host SiO{sub 2} matrix which, by applying an annealing at 1100 C, condensates to silicon nanoparticles and crystallizes. Although the condensation and crystallization occur after an annealing of one minute,10, 15 the samples were annealed during one hour in order to well-passivate the nc-Si, that means, to reduce effectively the number of Si-dangling bonds at the nc-Si surface that are efficient non-radiative recombination centers. 10, 16 Upon excitation with UV light, most of our nc-Si/SiO{sub 2} samples revealed strong PL. We implanted into our luminescent nc-Si/SiO{sub 2} systems other atomic elements, as for instance magnesium and calcium, which form silicates if their oxide is combined with SiO{sub 2}. The purpose is to simulate the conditions for silicates containing nc-Si. In order to understand the effect of the incorporation of foreign atoms on the PL properties of our nc-Si/SiO{sub 2} systems, we proceeded to similar experiments with Er and Ge. As has been demonstrated by several authors, 17, 18 the presence of nc-Si in a glass matrix enhances considerably the emission of Er{sup 3+} ions at 1.536{mu}m. At the same time, the PL of nc-Si is considerably quenched. Since the solubility of Er in crystalline silicon is about 2 orders of magnitude lower than in SiO{sub 2}, the optically active Er{sup 3+} ions are believed to be localized outside the nc-Si core, demonstrating that ions present in the host SiO{sub 2} matrix influence the PL

  4. Luminescence dating of Netherlands’ sediments

    OpenAIRE

    Wallinga, J.; Davids, F.; Dijkmans, J.W.A.

    2007-01-01

    Over the last decades luminescence dating techniques have been developed that allow earth scientists to determine the time of deposition of sediments. In this contribution we review: 1) the development of the methodology; 2) tests of the reliability of luminescence dating on Netherlands’ sediments; and 3) geological applications of the method in the Netherlands. Our review shows that optically stimulated luminescence dating of quartz grains using the single aliquot regenerative dose method yi...

  5. Optical stimulator for vision-based sensors

    DEFF Research Database (Denmark)

    Rössler, Dirk; Pedersen, David Arge Klevang; Benn, Mathias

    2014-01-01

    We have developed an optical stimulator system for vision-based sensors. The stimulator is an efficient tool for stimulating a camera during on-ground testing with scenes representative of spacecraft flights. Such scenes include starry sky, planetary objects, and other spacecraft. The optical...... precision and long-term stability. The system can be continuously used over several days. By facilitating a full camera including optics in the loop, the stimulator enables the more realistic simulation of flight maneuvers based on navigation cameras than pure computer simulations or camera stimulations...... stimulator is used as a test bench to simulate high-precision navigation by different types of camera systems that are used onboard spacecraft, planetary rovers, and for spacecraft rendezvous and proximity maneuvers. Careful hardware design and preoperational calibration of the stimulator result in high...

  6. Optical luminescence spectroscopy as a probe of the surface mineralogy of Mars

    Science.gov (United States)

    Treiman, A. H.

    1992-01-01

    Optical luminescence (OpL) spectroscopy is an attractive use of a visible-near-IR spectrometer on a Mars lander because mineral products of atmosphere-surface interactions on Mars will probably have characteristic OpL spectra. Optical luminescence spectra would be taken at night, when a spectrometer might otherwise sit idle. Also needed would be a source of exciting radiation, which could be shared with other experiments. Optical luminescence is emission of nonthermal optical photons (near-UV through near-IR) as a response to energy input. On absorption of energy, an atom (or ion) will enter an excited state. The favored decay of many such excited states involving valence-band electrons is emission of an optical photon. Optical luminescence spectra can be useful in determining mineralogy and mineral composition. Optical luminescence in crystals can arise from essential elements (or ions), trace-element substituents (activators), or defects. Common activators in salts of alkali and alkaline earth elements include Mn(2+)(VI), other transition metals, the rare earths, and the actinides. Trace substituents of other species can enhance or quench OpL (e.g., Pb(2+) vs. Fe(3+)). Optical luminescence can also arise from defects in crystal structures, including those caused by radiation and shock.

  7. Semiconducting Polymer Nanoparticles with Persistent Near-Infrared Luminescence for In Vivo Optical Imaging.

    Science.gov (United States)

    Palner, Mikael; Pu, Kanyi; Shao, Shirley; Rao, Jianghong

    2015-09-21

    Materials with persistent luminescence are attractive for in vivo optical imaging since they have a long lifetime that allows the separation of excitation of fluorophores and image acquisition for time-delay imaging, thus eliminating tissue autofluorescence associated with fluorescence imaging. Persistently luminescent nanoparticles have previously been fabricated from toxic rare-earth metals. This work reports that nanoparticles made of the conjugated polymer MEH-PPV can generate luminescence persisting for an hour upon single excitation. A near-infrared dye was encapsulated in the conjugated polymer nanoparticle to successfully generate persistent near-infrared luminescence through resonance energy transfer. This new persistent luminescence nanoparticles have been demonstrated for optical imaging applications in living mice.

  8. Hard X-ray-induced optical luminescence via biomolecule-directed metal clusters.

    Science.gov (United States)

    Osakada, Yasuko; Pratx, Guillem; Sun, Conroy; Sakamoto, Masanori; Ahmad, Moiz; Volotskova, Olga; Ong, Qunxiang; Teranishi, Toshiharu; Harada, Yoshie; Xing, Lei; Cui, Bianxiao

    2014-04-07

    Here, we demonstrate that biomolecule-directed metal clusters are applicable in the study of hard X-ray excited optical luminescence, promising a new direction in the development of novel X-ray-activated imaging probes.

  9. Synchrotron generated X-ray Excited Optical Luminescence (XEOL) from Quartz

    Science.gov (United States)

    King, Georgina; Finch, Adrian; Robinson, Ruth

    2010-05-01

    Quartz is the preferred mineral for optically stimulated luminescence (OSL) dating, due to its well constrained behaviour as a radiation dosimeter. However, despite the plethora of successful quartz OSL applications, no solution has been found to the problem that some quartz luminesce more brightly than others, which has limited the application of OSL in certain settings. This has been addressed through examination of the luminescence emission using a variety of excitation techniques and emission spectroscopy. X-ray Excited Optical Luminescence (XEOL) is luminescence excited by x-rays produced by a synchrotron. XEOL analyses were conducted upon a suite of quartz samples at Diamond, Great Britain, which had previously been analysed with Ionoluminescence (IL), at Sussex University. The samples were selected to include quartz of both poor and excellent OSL sensitivities. Therefore, two Scottish glacial outwash samples prepared at St Andrews, and a calibration quartz sample, prepared at the Risø National Laboratory in Denmark were analysed for these properties respectively. The XEOL emission spectra comprised three major emissions at 3.32, 3.81 and 4.05 eV, and one weaker emission at 1.94 eV in all samples. The calibration quartz sample had the most intense emission by an order of magnitude. Throughout increased exposure to x-rays, the intensity of the UV emission reduced, and an increase in the red (1.94 eV) emission was recorded. The derived XEOL spectra complement the IL spectra obtained previously. The IL spectra were dominated by only two broad emissions at 3.2-3.1 eV and 1.8-1.7 eV. However, throughout the IL experiments a dose dependent effect was also observed, whereby the UV emission was depleted to the benefit of the red with increasing exposure. Furthermore the gradient of the power law relationship between the UV and red emission change with dose is similar for both the IL and XEOL data: at -1.15 and -1.05 respectively for calibration quartz, when plotted

  10. The origin and dynamics of soft X-ray-excited optical luminescence of ZnO.

    Science.gov (United States)

    Armelao, Lidia; Heigl, Franziskus; Brunet, Sophie; Sammynaiken, Ramaswami; Regier, Tom; Blyth, Robert I R; Zuin, Lucia; Sankari, Rami; Vogt, Johannes; Sham, Tsun-Kong

    2010-12-03

    The distinct optical emission from ZnO materials, nanoneedles and microcrystallites synthesized with different sizes and morphologies by a flow deposition technique, is investigated with X-ray excited optical luminescence (XEOL) and time-resolved X-ray excited optical luminescence (TR-XEOL) from a synchrotron light source at the O K and Zn L(3,2) edges. The innovative use of XEOL, allowing site-specific chemical information and luminescence information at the same time, is fundamental to provide direct evidence for the different behaviour and the crucial role of bulk and surface defects in the origin of ZnO optical emission, including dynamics. XEOL from highly crystalline ZnO nanoneedles is characterized by a sharp band-gap emission (~380 nm) and a broad red luminescence (~680 nm) related to surface defects. Luminescence from ZnO microcrystallites is mostly dominated by green emission (~510 nm) associated with defects in the core. TR-XEOL experiments show considerably faster decay dynamics in nanoneedles compared to microcrystallites for both band-gap emission and visible luminescence. Herein we make a fundamental step forward correlating for the first time the interplay of size, crystallinity, morphology and excitation energy with luminescence from ZnO materials.

  11. A new luminescence detection and stimulation head for the Risø TL/OSL reader

    DEFF Research Database (Denmark)

    Lapp, Torben; Kook, Myung Ho; Murray, Andrew Sean

    2015-01-01

    A new automated Detection And Stimulation Head (DASH) has been developed for the Risø TL/OSL luminescence reader to provide easy access to new technologies, new signals and new measurement methods. The automated DASH includes a filter changer and a detector changer that makes it possible to change...... stimulation filters (4×4 filter combinations possible) and detectors (3 detectors possible) as part of a measurements sequence. The new automated DASH with dedicated driver electronics does not affect the use of other attachments, and can be retrospectively fitted to existing Risø TL/OSL readers....

  12. Multispectral Cerenkov luminescence tomography for small animal optical imaging.

    Science.gov (United States)

    Spinelli, Antonello E; Kuo, Chaincy; Rice, Brad W; Calandrino, Riccardo; Marzola, Pasquina; Sbarbati, Andrea; Boschi, Federico

    2011-06-20

    Quite recently Cerenkov luminescence imaging (CLI) has been introduced as a novel pre-clinical imaging for the in vivo imaging of small animals such as mice. The CLI method is based on the detection of Cerenkov radiation (CR) generated by beta particles as they travel into the animal tissues with an energy such that Cerenkov emission condition is satisfied. This paper describes an image reconstruction method called multi spectral diffuse Cerenkov luminescence tomography (msCLT) in order to obtain 3D images from the detection of CR. The multispectral approach is based on a set of 2D planar images acquired using a number of narrow bandpass filters, and the distinctive information content at each wavelength is used in the 3D image reconstruction process. The proposed msCLT method was tested both in vitro and in vivo using 32P-ATP and all the images were acquired by using the IVIS 200 small animal optical imager (Caliper Life Sciences, Alameda USA). Source depth estimation and spatial resolution measurements were performed using a small capillary source placed between several slices of chicken breast. The theoretical Cerenkov emission spectrum and optical properties of chicken breast were used in the modelling of photon propagation. In vivo imaging was performed by injecting control nude mice with 10 MBq of 32P-ATP and the 3D tracer bio-distribution was reconstructed. Whole body MRI was acquired to provide an anatomical localization of the Cerenkov emission. The spatial resolution obtained from the msCLT reconstructed images of the capillary source showed that the FWHM is about 1.5 mm for a 6 mm depth. Co-registered MRI images showed that the Cerenkov emission regions matches fairly well with anatomical regions, such as the brain, heart and abdomen. Ex vivo imaging of the different organs such as intestine, brain, heart and ribs further confirms these findings. We conclude that in vivo 3D bio-distribution of a pure beta-minus emitting radiopharmaceutical such as 32P

  13. Persistent luminescence induced by near infra-red photostimulation in chromium-doped zinc gallate for in vivo optical imaging

    Science.gov (United States)

    Sharma, Suchinder K.; Gourier, Didier; Teston, Eliott; Scherman, Daniel; Richard, Cyrille; Viana, Bruno

    2017-01-01

    The analysis of the optical spectroscopy of the Cr3+ doped spinel was initiated by Prof. Georges Boulon more than twenty years ago. More recently persistent luminescence nanoparticles of Cr doped zinc gallate have found interest for in vivo imaging of small animals. Here we evaluated near infra-red (NIR) excitation (or NIR photostimulation) via photo-transfer mechanism as an additional tool for in vivo optical imaging. Investigation of the persistent luminescence induced by NIR photostimulation is studied after either a primary UV (band-to-band excitation) or visible irradiation (direct Cr 3d-3d excitation). UV or visible pre-excited ZnGa2O4:Cr (ZGO:Cr) nanoparticles are kept active during several days thanks to deep traps (with depths 1 eV-1.2 eV) observed in these samples which can be probed through thermally stimulated luminescence (TSL) technique showing glow curve maximums at 470 K and 530 K upon visible light excitation. These deep traps are stable at room temperature but can be emptied by NIR light photostimulation. Experiments were carried out to study the photostimulation induced trapping-detrapping in the ZGO:Cr phosphor. Photostimulation was also tested in vivo for small animal optical imaging to offer new perspectives and modalities.

  14. Thermally stimulated luminescence and electron paramagnetic resonance studies on uranium doped calcium phosphate

    CERN Document Server

    Natarajan, V; Veeraraghavan, R; Sastry, M D

    2003-01-01

    Thermally stimulated luminescence (TSL) and electron paramagnetic resonance (EPR) studies on uranium doped calcium phosphate yielded mechanistic information on the observed glow peaks at 365, 410 and 450 K. TSL spectral studies of the glow peaks showed that UO sub 2 sup 2 sup + acts as the luminescent center. Electron paramagnetic resonance studies on gamma-irradiated samples revealed that the predominant radiation induced centers are H sup 0 , PO sub 4 sup 2 sup - , PO sub 3 sup 2 sup - and O sup - ion. Studies on the temperature dependence studies of the EPR spectra of samples annealed to different temperatures indicate the role of H sup 0 and PO sub 4 sup 2 sup - ions in the main glow peak at 410 K.

  15. Violet stimulated luminescence dating of quartz from Luochuan (Chinese loess plateau): Agreement with independent chronology up to ∼600 ka

    DEFF Research Database (Denmark)

    Ankjærgaard, C.; Guralnik, B.; Buylaert, Jan-Pieter

    2016-01-01

    Luminescence dating at the Luochuan loess type (China) section is at present limited to ∼0.1 Ma using quartz blue light stimulated luminescence (BLSL), but can be extended back in time to ∼0.5 Ma by resorting to the more developmental post-infrared infrared stimulated luminescence (post-IR IRSL) ......-1800 Gy) would correspond to the ability to date sediment up to ∼1 Ma back in time, offering a remarkable advance over existing methods.......Luminescence dating at the Luochuan loess type (China) section is at present limited to ∼0.1 Ma using quartz blue light stimulated luminescence (BLSL), but can be extended back in time to ∼0.5 Ma by resorting to the more developmental post-infrared infrared stimulated luminescence (post-IR IRSL...... demonstrate that the Multi-Aliquot Additive-Dose (MAAD) protocol produces a VSL chronology at Luochuan which is in agreement with independent ages up to ∼0.6 Ma. For a more representative environmental dose rate of ∼2 Gy/ka (∼35% lower than at Luochuan), the documented range of MAAD-VSL sensitivity (200...

  16. Use of scanning near-field optical microscope with an aperture probe for detection of luminescent nanodiamonds

    Science.gov (United States)

    Shershulin, V. A.; Samoylenko, S. R.; Shenderova, O. A.; Konov, V. I.; Vlasov, I. I.

    2017-02-01

    The suitability of scanning near-field optical microscopy (SNOM) to image photoluminescent diamond nanoparticles with nanoscale resolution is demonstrated. Isolated diamond nanocrystals with an average size of 100 nm, containing negatively charged nitrogen-vacancy (NV-) centers, were chosen as tested material. The NV- luminescence was stimulated by continuous 532 nm laser light. Sizes of analyzed crystallites were monitored by an atomic force microscope. The lateral resolution of the order of 100 nm was reached in SNOM imaging of diamond nanoparticles using 150 nm square aperture of the probe.

  17. Irradiated integrated circuits dose-attenuation mapping using optically stimulated phosphors for packaging dosimetry

    Energy Technology Data Exchange (ETDEWEB)

    Dusseau, L.; Polge, G.; Albert, L.; Magnac, Y.; Fesquet, J.; Gasiot, J. [Univ. Montpellier II (France); Bessiere, J.C. [CORAD P.I.T. Pompignane, Montpellier (France)

    1998-12-01

    The feasibility of a dose mapping system using Optically Stimulated Luminescent (OSL) Phosphors is demonstrated. The OSL technique is briefly reviewed as well as its interest for calculation codes calibration. The sensors and the reading apparatus are presented. An example of attenuation dose map obtained for a Dual In Line Plastic Package (DIL) is given and the results compared to calculations with the code EGS4 PRESTA. Results obtained by experiment and simulation are discussed as well as the potentialities of the method.

  18. Blue light emitting diodes for optical stimulation of quartz in retrospective dosimetry and dating

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.; Duller, G.A.T.; Murray, A.S.

    1999-01-01

    (470 nm) gives order of magnitude greater rate of stimulation in quartz than that from conventional blue-green light filtered from a halogen lamp. A practical blue LED OSL configuration is described. From comparisons of OSL decay curves produced by green and blue light sources, and by examination......Recently developed blue light emitting diodes (LEDs) for the optical stimulation of quartz for use in routine optically stimulated luminescence (OSL) dating and retrospective dosimetry have been tested. For similar power densities, it was found that the higher energy light provided by the blue LEDs...... of the dependence of the blue LED OSL on preheat temperature, it is deduced that there is no evidence that the blue LEDs stimulate deep traps in a different manner from broadband filtered light. It is concluded that blue LEDs offer a practical alternative to existing stimulation sources. They have the significant...

  19. Stimulation of luminescence of mycelium of luminous fungus Neonothopanus nambi by ionizing radiation.

    Science.gov (United States)

    Kobzeva, Tatiana V; Melnikov, Anatoly R; Karogodina, Tatiana Y; Zikirin, Samat B; Stass, Dmitri V; Molin, Yuri N; Rodicheva, Emma K; Medvedeva, Svetlana E; Puzyr, Alexey P; Burov, Andrey A; Bondar, Vladimir S; Gitelson, Joseph I

    2014-11-01

    The luminescent system of higher luminous fungi is not fully understood and the enzyme/substrate pair of the light emission reaction has not been isolated. It was suggested that luminescence of fungi involves oxidase-type enzymes, and reactive oxygen species are important for fungal light production. Generation of reactive oxygen species can be stimulated by ionizing irradiation, which has not been studied for luminous fungi. We report the effect of X-irradiation on the luminescence of fungus Neonothopanus nambi. Experiments were performed with mycelium on a home-built setup based on an X-ray tube and monochromator/photomultiplier tube. Application of X-rays does not change the emission spectrum, but after approximately 20 min of continuous irradiation, light production from unsupported mycelium starts growing and increases up to approximately five times. After peaking, its level decreases irrespective of the presence of X-irradiation. After staying at a certain level, light production collapses to zero, which is not related to the drying of the mycelium or thermal impact of radiation. The observed shape of kinetics is characteristic of a multistage and/or chain reaction. The time profile of light production must reflect the current levels of radicals present in the system and/or the activity of enzyme complexes involved in light production.

  20. Thermally and optically stimulated radiative processes in Eu and Y co-doped LiCaAlF{sub 6} crystal

    Energy Technology Data Exchange (ETDEWEB)

    Fukuda, Kentaro, E-mail: ken-fukuda@tokuyama.co.jp [Tokuyama Corporation, 1-1 Mikage-cho, Shunan-shi, Yamaguchi 745-8648 (Japan); Yanagida, Takayuki; Fujimoto, Yutaka [Kyushu Institute of Technology, 2-4 Hibikino, Wakamatsu, Kitakyushu, Fukuoka 808-0196 (Japan)

    2015-06-01

    Yttrium co-doping was attempted to enhance dosimeter performance of Eu doped LiCaAlF{sub 6} crystal. Eu doped and Eu, Y co-doped LiCaAlF{sub 6} were prepared by the micro-pulling-down technique, and their dosimeter characteristics such as optically stimulated luminescence (OSL) and thermally stimulated luminescence (TSL) were investigated. By yttrium co-doping, emission intensities of OSL and TSL were enhanced by some orders of magnitude. In contrast, scintillation characteristics of yttrium co-doped crystal such as intensity of prompt luminescence induced by X-ray and light yield under neutron irradiation were degraded.

  1. Thermoluminescent dosimetry and of optically stimulated luminescence of diamond films grown up by the chemical vapor deposition technique exposed to beta radiation; Dosimetria termoluminiscente y de luminiscencia opticamente estimulada de peliculas de diamante crecidas por la tecnica de DVQ expuestas a radiacion beta

    Energy Technology Data Exchange (ETDEWEB)

    Melendrez A, R.; Barboza F, M. [Centro de Investigacion en Fisica, Universidad de Sonora, A.P. 5-88, Hermosillo, Sonora, 83190 (Mexico)

    2002-07-01

    A study of the dosimetric properties through the thermoluminescence (Tl) and Optically stimulated luminescence (Lobe) in diamond films grown up by the chemical vapor deposition (Dq) techniques was realized.The films under study have thickness of 6, 12, 180 and 500 microns. The dose range was from 0 to 1.5 KGy, observing for the case of the thermoluminescent dosimetry a linear behavior in the range 0-300 Gy and a supra linearity effect in the range from 300-1500 Gy. For the case of the dosimetry by means of LOE a linear behavior in the range (0-300 Gy) without be enough for the saturation was observed, although some samples exhibit a linear behavior until 1500 Gy (6 microns). The irradiation was realized with a source of Strontium 90 of (40 mCi) and the photoestimulation for realizing the measures of LOE was realized using diodes emitting of laser light (470 nm) which generate until 50 MW/cm{sup 2}. The Tl peak which was used to realize the dosimetry such Tl as LOE was that located around 340 C degrees in the brilliance curve which presents another peaks centered around of 110, 190, and 340 C degrees, depending on the film. It was realized a study of the Tl signal drop and it was observed that after 3 hours the signal was stable reaching a decay of 15 %. the analysis of the drop in the Tl signal, immediately after to irradiate and after to photoestimulate with the blue light laser for observing the LOE, indicated that exists a fall in all the Tl peaks, decaying in greater proportion those of more low temperature. (Author)

  2. Application of the thermoluminescent (TL) and optically stimulated luminescence (OSL) dosimetry techniques to determinate the isodose curves in a cancer treatment planning simulation using Volumetric Modulated Arc Therapy - VMAT; Aplicacao das tecnicas de dosimetria termoluminescente (TL) e luminescencia opticamente estimulada (OSL) na determinacao de curvas de isodose em uma simulacao de tratamento de cancer pela tecnica de radioterapia em arco modulado volumetrico - VMAT

    Energy Technology Data Exchange (ETDEWEB)

    Bravim, Amanda

    2015-07-01

    The Volumetric Modulated Arc Therapy (VMAT) is an advance technique of Intensity Modulated Radiation Therapy (IMRT). This progress is due to the continuous gantry rotation with the radiation beam modulation providing lower time of the patient treatment. This research aimed the verification of the isodose curves in a simulation of a vertebra treatment with spinal cord protection using the thermoluminescent (TL) and optically stimulated luminescence (OSL) dosimetry techniques and the LiF:Mg,Ti (TLD-100), CaS0{sub 4}:Dy and Al{sub 2}0{sub 3}:C dosimeters and LiF:Mg,Ti micro dosimeters (TLD-100). The dosimeters were characterized using PMMA plates of 30 x 30 x 30 cm{sup 3} and different thickness. All irradiations were done using Truebeam STx linear accelerator of Hospital Israelita Albert Einstein, with 6 MV photons beam. After the dosimeter characterization, they were irradiated according the specific planning simulation and using a PMMA phantom developed to VMAT measurements. This irradiation aimed to verify the isodose curves of the treatment simulation using the two dosimetry techniques. All types of dosimeters showed satisfactory results to determine the dose distribution but analysing the complexity of the isodose curves and the proximity of them, the LiF:Mg,Ti micro dosimeter showed the most appropriate for use due to its small dimensions. Regarding the best technique, as both technique showed satisfactory results, the TL technique presents less complex to be used because the most of the radiotherapy departments already have a TL laboratory. The OSL technique requires more care and greater investment in the hospital. (author)

  3. X-ray excited optical luminescence, photoluminescence, photostimulated luminescence and x-ray photoemission spectroscopy studies on BaFBr:Eu

    CERN Document Server

    Subramanian, N; Govinda-Rajan, K; Mohammad-Yousuf; Santanu-Bera; Narasimhan, S V

    1997-01-01

    The results of x-ray excited optical luminescence (XEOL), photoluminescence (PL), photostimulated luminescence (PSL) and x-ray photoemission spectroscopy (XPS) studies on the x-ray storage phosphor BaFBr:Eu are presented in this paper. Analyses of XEOL, PL and PSL spectra reveal features corresponding to the transitions from 4f sup 6 td sup 1 to 4f sup 7 configurations in different site symmetries of Eu sup 2 sup +. Increasing x-ray dose is seen to lead to a red shift in the maximum of the PL excitation spectrum for the 391 nm emission. The XEOL and XPS spectra do not show any signature of Eu sup 3 sup + in the samples studied by us, directly raising doubts about the model of Takahashi et al in which Eu sup 2 sup + is expected to ionize to Eu sup 3 sup + upon x-ray irradiation and remain stable until photostimulation. XEOL and PSL experiments with simultaneous x-ray irradiation and He - Ne laser excitation as well as those with sequential x-ray irradiation and laser stimulation bring out the competition betwe...

  4. Temperature lags of luminescence measurements in a commercial luminescence reader

    Energy Technology Data Exchange (ETDEWEB)

    Kitis, George [Aristotle University of Thessaloniki, Nuclear Physics Laboratory, 54124 Thessaloniki (Greece); Kiyak, Nafiye G. [ISIK University, Faculty of Science and Arts, Physics Department, Sile, 34980 Istanbul (Turkey); Polymeris, George S., E-mail: gspolymeris@ankara.edu.tr [Ankara University, Institute of Nuclear Sciences, Beşevler, 06100 Ankara (Turkey)

    2015-09-15

    The temperature recorded in thermoluminescence and optically stimulated luminescence equipments is not the temperature of the sample but that of the heating element on which the thermocouple is attached. Depending upon the rate of heating, a temperature difference appears between the samples and the heating element, termed as temperature lag, which could have serious effects on the curve shapes and trapping parameters. In the present work the temperature lag effect is studied in a newly developed luminescence equipment measuring both thermoluminescence and optically stimulated luminescence. It is found that the temperature lag could be large for heating rates above 2 K/s and it is strongly dependent upon the sample holder. A simple approximation method is proposed in order to both predict as well as correct for temperature lag effects in luminescence measurements.

  5. Ion beam induced luminescence of germano-silicate optical fiber preform

    Energy Technology Data Exchange (ETDEWEB)

    Jung, Hyunkyu; Kim, Jongyeol; Lee, Namho [Korea Atomic Energy Research Institute, Daejeon (Korea, Republic of); Kim, Youngwoong; Han, Wontaek [Gwangju Institute of Science and Technology, Gwangju (Korea, Republic of); Markovic, Nikola; Jaksic, Milko [Ruder Boskovic Institute, Zagred (Croatia)

    2014-05-15

    When an optical fiber is exposed to radiation, the attenuation (RIA, Radiation Induced Attenuation) in the optical fiber (OF) is increased because of the color centers which deteriorate the transmission property and generate the absorption loss. In order to understand the radiation induced defect, Ion Beam induced luminescence (IBIL) was introduced to investigate it. IBIL technique is to analyze IR/VIS/UV luminescence related to ion beam interaction with outer shell electrons involved in chemical bonds and structure defects of target atoms. So IBIL is sensitive to its chemical composition and has been used in analysis of material characterization, geological samples and cultural heritage objects. In silica material, four O atoms are surrounding one Si atom in tetrahedral coordination. In this study, the influence of Copper (Cu) and Cerium (Ce) dopants to germano silica core optical fibers were investigated under proton irradiation at RBI using Ion Beam induced luminescence (IBIL) method. To understand the radiation induced defect of optical fibers, IBIL were tested to a germano-silica core fiber under 2 MeV proton irradiation. Although a Cu or Ce dopant was not detected by IBIL technique, the relation between the amount of radiation and luminescence can be established. This experiment showed a potential technique of studying the effects and behavior of additive elements for silica core fiber. To increase the radiation resistance of optical fibers, further investigations are needed, i. e. the proper additives and its contents and an interaction mechanism between Ge-related defects and additives.

  6. Optical imaging as an expansion of nuclear medicine: Cerenkov-based luminescence vs fluorescence-based luminescence

    Energy Technology Data Exchange (ETDEWEB)

    Chin, Patrick T.K.; Welling, Mick M.; Leeuwen, Fijs W.B. van [Leiden University Medical Center, Interventional Molecular Imaging Laboratory, Department of Radiology, P.O. Box 9600, Leiden (Netherlands); Meskers, Stefan C.J. [Eindhoven University of Technology, Molecular Materials and Nanosystems, P.O. Box 513, Eindhoven (Netherlands); Valdes Olmos, Renato A. [Leiden University Medical Center, Interventional Molecular Imaging Laboratory, Department of Radiology, P.O. Box 9600, Leiden (Netherlands); Netherlands Cancer Institute-Antoni van Leeuwenhoek Hospital, Department of Nuclear Medicine, Amsterdam (Netherlands); Tanke, Hans [Leiden University Medical Center, Department of Molecular Cell Biology, P.O. Box 9600, Leiden (Netherlands)

    2013-08-15

    Integration of optical imaging technologies can further strengthen the field of radioguided surgery. Rather than using two separate chemical entities to achieve this extension, hybrid imaging agents can be used that contain both radionuclear and optical properties. Two types of such hybrid imaging agents are available: (1) hybrid imaging agents generated by Cerenkov luminescence imaging (CLI) of {beta}-emitters and (2) hybrid imaging agents that contain both a radioactive moiety and a fluorescent dye. One major challenge clinicians are now facing is to determine the potential value of these approaches. With this tutorial review we intend to clarify the differences between the two approaches and highlight the clinical potential of hybrid imaging during image-guided surgery applications. (orig.)

  7. Optical absorption and luminescence in neutron-irradiated, silica-based fibers

    Energy Technology Data Exchange (ETDEWEB)

    Cooke, D.W.; Farnum, E.H.; Clinard, F.W. [Los Alamos National Lab., CA (United States)] [and others

    1995-04-01

    The objectives of this work are to assess the effects of thermal annealing and photobleaching on the optical absorption of neutron-irradiated, silica fibers of the type proposed for use in ITER diagnostics, and to measure x-ray induced luminescence of unirradiated (virgin) and neutron-irradiated fibers.

  8. Material and Optical Design Rules for High Performance Luminescent Solar Concentrators

    Science.gov (United States)

    Bronstein, Noah Dylan

    This dissertation will highlight a path to achieve high photovoltaic conversion efficiency in luminescent solar concentrators, devices which absorb sunlight with a luminescent dye and then re-emit it into a waveguide where it is ultimately collected by a photovoltaic cell. Luminescent concentrators have been studied for more than three decades as potential low-cost but not high efficiency photovoltaics. Astute application of the blackbody radiation law indicates that photonic design is necessary to achieve high efficiency: a reflective filter must be used to trap luminescence at all angles while allowing higher energy photons to pass through. In addition, recent advances in the synthesis of colloidal nanomaterials have created the possibility for lumophores with broad absorption spectra, narrow-bandwidth emission, high luminescence quantum yield, tunable Stokes shifts and tunable Stokes ratios. Together, these factors allow luminescent solar concentrators to achieve the optical characteristics necessary for high efficiency. We have fabricated and tested the first generation of these devices. Our experiments demonstrate that the application of carefully matched photonic mirrors and luminescent quantum dots can allow luminescent concentration factors to reach record values while maintaining high photon collection efficiency. Finally, the photonic mirror dramatically mitigates the negative impact of scattering in the waveguide, allowing efficient photon collection over distances much longer than the scattering length of the waveguide. After demonstrating the possibility for high performance, we theoretically explore the efficacy of luminescent concentrators with dielectric reflectors as the high-bandgap top-junctions in two-junction devices. Simple thermodynamic calculations indicate that this approach can be nearly as good as a traditional vertically stacked tandem. The major barriers to such a device are the optical design of narrow-bandwidth, angle

  9. Detection of irradiated spices using photo-stimulated luminescence technique (PSL)

    Energy Technology Data Exchange (ETDEWEB)

    Ramli, Ros Anita Ahmad; Yasir, Muhamad Samudi [Faculty of Science and Technology, National University of Malaysia, Bangi, 43000 Kajang, Selangor (Malaysia); Othman, Zainon; Abdullah, Wan Saffiey Wan [Malaysian Nuclear Agency, Bangi 43000 Kajang, Selangor (Malaysia)

    2014-09-03

    Photo-stimulated luminescence (PSL) technique was applied to detect irradiated black pepper (Piper nigrum), cinnamon (Cinnamomum verum) and turmeric (Curcuma longa) after dark storage for 1 day, 3 and 6 months. Using screening and calibrated PSL, all samples were correctly discriminated between non-irradiated and spices irradiated with doses 1, 5 and 10 kGy. The PSL photon counts (PCs) of irradiated spices increased with increasing dose, with turmeric showing highest sensitivity index to irradiation compared to black pepper and cinnamon. The differences in response are possibly attributed to the varying quantity and quality of silicate minerals present in each spice sample. PSL signals of all irradiated samples reduced after 3 and 6 months storage. The results of this study provide a useful database on the applicability of PSL technique for the detection of Malaysian irradiated spices.

  10. Detection of irradiated spices using photo-stimulated luminescence technique (PSL)

    Science.gov (United States)

    Ramli, Ros Anita Ahmad; Yasir, Muhamad Samudi; Othman, Zainon; Abdullah, Wan Saffiey Wan

    2014-09-01

    Photo-stimulated luminescence (PSL) technique was applied to detect irradiated black pepper (Piper nigrum), cinnamon (Cinnamomum verum) and turmeric (Curcuma longa) after dark storage for 1 day, 3 and 6 months. Using screening and calibrated PSL, all samples were correctly discriminated between non-irradiated and spices irradiated with doses 1, 5 and 10 kGy. The PSL photon counts (PCs) of irradiated spices increased with increasing dose, with turmeric showing highest sensitivity index to irradiation compared to black pepper and cinnamon. The differences in response are possibly attributed to the varying quantity and quality of silicate minerals present in each spice sample. PSL signals of all irradiated samples reduced after 3 and 6 months storage. The results of this study provide a useful database on the applicability of PSL technique for the detection of Malaysian irradiated spices.

  11. Optical switching by stimulated thermal Rayleigh scattering

    Science.gov (United States)

    Peterson, Lauren M.

    1986-06-01

    Preliminary experiments were conducted whose ultimate goal is to develop all-optical control functions useful in an all-optical or optical-electronic hybrid digital computer or for optical interconnects. Stimulated thermal Rayleigh scattering (STRS) based upon generator experiments was pursued for scattering angles of 90 deg and 180 deg (backscattering). A pulsed nitrogen laser pumped dye laser served as the radiation source and the interaction medium was a liquid to which an absorbing dye was added. STRS amplifier experiments were successful and gain was observed and studied parametrically using eosine dye in ethanol. The gain was found to increase (although the gain coefficient decreased) with increasing pump power and the gain was found to be a maximum at an absorption coefficient of about 2.6 per cm. The generator experiments did not lead to stimulated scattering due to the limited output power of the laser and its multi-longitudinal spectral mode content. These studies will be continued along with analytical modeling in order to characterize the interaction and to enable the optimization of the scattering process.

  12. Photostimulated near-infrared persistent luminescence as a new optical read-out from Cr3+-doped LiGa5O8

    Science.gov (United States)

    Liu, Feng; Yan, Wuzhao; Chuang, Yen-Jun; Zhen, Zipeng; Xie, Jin; Pan, Zhengwei

    2013-01-01

    In conventional photostimulable storage phosphors, the optical information written by x-ray or ultraviolet irradiation is usually read out as a visible photostimulated luminescence (PSL) signal under the stimulation of a low-energy light with appropriate wavelength. Unlike the transient PSL, here we report a new optical read-out form, photostimulated persistent luminescence (PSPL) in the near-infrared (NIR), from a Cr3+-doped LiGa5O8 NIR persistent phosphor exhibiting a super-long NIR persistent luminescence of more than 1,000 h. An intense PSPL signal peaking at 716 nm can be repeatedly obtained in a period of more than 1,000 h when an ultraviolet-light (250–360 nm) pre-irradiated LiGa5O8:Cr3+ phosphor is repeatedly stimulated with a visible light or a NIR light. The LiGa5O8:Cr3+ phosphor has promising applications in optical information storage, night-vision surveillance, and in vivo bio-imaging. PMID:23532003

  13. Secure optical communication using stimulated Brillouin scattering in optical fiber

    Science.gov (United States)

    Yi, Lilin; Zhang, Tao; Li, Zhengxuan; Zhou, Junhe; Dong, Yi; Hu, Weisheng

    2013-03-01

    We propose to encrypt/decrypt high-speed optical signal using stimulated Brillouin scattering (SBS) effect in optical fiber for the first time. The broadened SBS gain or loss distorts the amplitude and phase of the optical signal so as to realize all-optical encryption. The corresponding SBS loss or gain with the same bandwidth and amplitude recovers the distorted signal to implement optical decryption. The encryption/decryption keys could be the SBS gain amplitude, bandwidth, central wavelength and the spectral shape, which are configurable and can be flexibly controlled by the users. The operation principle of the SBS based encryption and decryption is explained in detail. Complete encryption and error-free decryption for a 10.86-Gb/s on-off-keying signal has been experimentally demonstrated using broadband SBS amplification and absorption. The immunity of the proposed encryption method to the eavesdropper's attack is also analyzed. The SBS based secure optical communication is compatible with the current optical communication systems.

  14. Luminescence characteristics of dental ceramics for retrospective dosimetry: a preliminary study

    Energy Technology Data Exchange (ETDEWEB)

    Bailiff, I.K.; Correcher, V.; Delgado, A.; Goksu, Y.; Huebner, S

    2002-07-01

    Ceramic materials that are widely employed in dental prosthetics and repairs exhibit luminescent properties. Because of their use in the body, these materials are potentially of interest in situations where retrospective dosimetry for individuals is required but where monitoring was not planned. The luminescent properties of dental ceramics obtained in Germany, Spain and the UK were examined. Linear dose-response characteristics were obtained in the range <100 mGy to 10 Gy using thermoluminescence (TL), optically stimulated luminescence and infrared-stimulated luminescence measurement techniques. Measurements of time-resolved luminescence were also performed to examine the nature of the luminescence recombination under visible (470 nm) and IR (855 nm) stimulation. The results obtained by TL and optically stimulated techniques suggest that there may be deeper traps than previously observed in certain types of dental ceramic. Such traps may be less susceptible to optical and athermal fading than was reported in earlier studies. (author)

  15. Household and workplace chemicals as retrospective luminescence dosemeters

    DEFF Research Database (Denmark)

    Thomsen, Kristina Jørkov; Bøtter-Jensen, L.; Murray, A.S.

    2002-01-01

    , there are Other potential unheated crystalline materials found in the domestic and industrial environment which may also act as retrospective dosemeters, and may be considerably more sensitive. We have Surveyed the thermoluminescent and optically stimulated luminescent (OSL) characteristics of several...

  16. Limit of detection of a fiber optics gyroscope using a super luminescent radiation source

    CERN Document Server

    Sandoval, G E

    2003-01-01

    The main objective of this work is to establish the dependence of characteristics of the fiber optics gyroscope (FOG) with respect to the parameters of the super luminescent emission source based on doped optical fiber with rare earth elements (Super luminescent Fiber Source, SFS), argument the pumping rate election of the SFS to obtain characteristics limits of the FOG sensibility. By using this type of emission source in the FOG is recommend to use the rate when the direction of the pumping signal coincide with the super luminescent signal. The most results are the proposition and argumentation of the SFS election as emission source to be use in the FOG of the phase type. Such a decision allow to increase the characteristics of the FOG sensibility in comparison with the use of luminescent source of semiconductors emission which are extensively used in the present time. The use of emission source of the SFS type allow to come closer to the threshold of the obtained sensibility limit (detection limit) which i...

  17. New Nanomaterials and Luminescent Optical Sensors for Detection of Hydrogen Peroxide

    Directory of Open Access Journals (Sweden)

    Natalia A. Burmistrova

    2015-10-01

    Full Text Available Accurate methods that can continuously detect low concentrations of hydrogen peroxide (H2O2 have a huge application potential in biological, pharmaceutical, clinical and environmental analysis. Luminescent probes and nanomaterials are used for fabrication of sensors for H2O2 that can be applied for these purposes. In contrast to previous reviews focusing on the chemical design of molecular probes for H2O2, this mini-review highlights the latest luminescent nanoparticular materials and new luminescent optical sensors for H2O2 in terms of the nanomaterial composition and luminescent receptor used in the sensors. The nanomaterial section is subdivided into schemes based on gold nanoparticles, polymeric nanoparticles with embedded enzymes, probes showing aggregation-induced emission enhancement, quantum dots, lanthanide-based nanoparticles and carbon based nanomaterials, respectively. Moreover, the sensors are ordered according to the type of luminescent receptor used within the sensor membranes. Among them are lanthanide complexes, metal-ligand complexes, oxidic nanoparticles and organic dyes. Further, the optical sensors are confined to those that are capable to monitor the concentration of H2O2 in a sample over time or are reusable. Optical sensors responding to gaseous H2O2 are not covered. All nanomaterials and sensors are characterized with respect to the analytical reaction towards H2O2, limit of detection (LOD, analytical range, electrolyte, pH and response time/incubation time. Applications to real samples are given. Finally, we assess the suitability of the nanomaterials to be used in membrane-based sensors and discuss future trends and perspectives of these sensors in biomedical research.

  18. Understanding optically stimulated charge movement in quartz and feldspar using time-resolved measurements

    Energy Technology Data Exchange (ETDEWEB)

    Ankjaergaard, C.

    2010-02-15

    Thermoluminescence (TL) and optically stimulated luminescence (OSL) from quartz and feldspar are widely used in accident dosimetry and luminescence dating. In order to improve already existing methods or to develop new methods towards extending the current limits of the technique, it is important to understand the charge movement within these materials. Earlier studies have primarily focussed on examination of the trap behaviour; however, this only tells half of the story as OSL is a combination of charge stimulation and recombination. By using time-resolved OSL (TR-OSL), one can directly examine the recombination route(s), and thus obtain insight into the other half of the process involved in luminescence emission. This thesis studies the TR-OSL and optically stimulated phosphorescence signals from quartz and feldspars spanning several orders of magnitude in time (few ns to the seconds time scale) in order to identify various charge transport mechanisms in the different time regimes. The techniques employed are time-resolved OSL, continuous-wave OSL, TL, optically stimulated exo-electron (OSE) emission and time-resolved OSE. These different techniques are used in combination with variable thermal or optical stimulation energy. The thesis first delves into three main methodological developments, namely (i) research and development of the equipment for TR-OSL measurements, (ii) finding the best method for multiple-exponential analysis of a TR-OSL curve, and (iii) optimisation of the pulsing configuration for the best separation of quartz OSL from a mixed quarts-feldspar sample. It then proceeds to study the different charge transport mechanisms subsequent to an optical stimulation pulse in quartz and feldspars. The results obtained for quartz conclude that the main lifetime component in quartz represents an excited state lifetime of the recombination centre, and the more slowly decaying components on the millisecond to seconds time scale arise from charge recycling

  19. Luminescent Properties of Arylpolyene Organic Dyes and Cross-Conjugated Ketones Promising for Quantum Optics and Nanophotonics Applications

    Directory of Open Access Journals (Sweden)

    Naumova N. L.

    2015-01-01

    Full Text Available The spectral-luminescent properties of some dyes of substituted arylpolyenes and cross-conjugated ketones class in Shpolsky matrices, promising for using in solving quantum optics and nanophotonics, were studied.

  20. Modeling of the shape of infrared stimulated luminescence signals in feldspars

    DEFF Research Database (Denmark)

    Pagonis, Vasilis; Jain, Mayank; Murray, Andrew S.;

    2012-01-01

    This paper presents a new empirical model describing infrared (IR) stimulation phenomena in feldspars. In the model electrons from the ground state of an electron trap are raised by infrared optical stimulation to the excited state, and subsequently recombine with a nearest-neighbor hole via...... that the shape of the IRSL curves does not change significantly under different experimental conditions. The relationship between the simulated IRSL signal and the well-known power-law dependence of relaxation processes in solids is also explored, by fitting the IRSL signal at long times with a power-law type...

  1. Optical temperature sensing based on the luminescence from YAG:Pr transparent ceramics

    Science.gov (United States)

    Hu, Song; Lu, Chunhua; Liu, Xiaoxia; Xu, Zhongzi

    2016-10-01

    The YAG:Pr transparent ceramic was fabricated using a conventional solid-state reactive method to explore its possible application in optical thermometry. Photoluminescence and temperature-dependent luminescence were elaborately investigated under 452 nm excitation. The ceramic showed two intrinsic emission bands at 488 and 594 nm, which were attributed to characteristic Pr3+: 3P0 → 3H4 and 3P1 → 3H6 transitions, respectively. Down-conversion emissions from the two thermally coupled excited states of Pr3+ were recorded in the temperature range of 293-593 K. The Boltzmann distribution theory was adopted to interpret the temperature-dependent luminescence of Pr3+. The temperature sensitivity exhibited an increasing trend with the increase of temperature, typically, 0.0025 K-1 at 593 K. The results indicated that the present ceramic was a promising candidate for optical temperature sensor.

  2. Advances in luminescence instrument systems

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.; Bulur, E.; Duller, G.A.T.

    2000-01-01

    We report on recent advances in the development of luminescence measurement systems and techniques at Riso. These include: (1) optical stimulation units based on new-generation powerful blue light (470 nm) emitting diodes providing up to 28 mW/cm(2) for OSL measurements; (2) an infrared (830 nm...

  3. Radiation induced luminescence processes in c-BN

    DEFF Research Database (Denmark)

    Trinkler, L.; Berzina, B.; Benabdesselam, M.

    2004-01-01

    Spectral properties of cubic boron nitride have been studied using methods of photoluminescence (PL), X-ray excited luminescence (XL), thermoluminescence (TL) and optically stimulated luminescence. It is found that emission of cubic boron nitride is presented by 4 subbands, their relative yield...

  4. Thermal quenching of luminescence processes in feldspars

    DEFF Research Database (Denmark)

    Poolton, N.R.J.; Bøtter-Jensen, L.; Duller, G.A.T.

    1995-01-01

    The technique of optically stimulated luminescence has important uses in the dose evaluation of irradiated feldspars. The luminescence process involves the eviction of electrons from donor traps, charge transfer through the conduction band, and recombination at acceptor sites; each...... of these processes is, in general, thermally dependent, and leads either to enhancement or quenching of the luminescence with increasing temperature. Previous studies have measured the combined thermal activation characteristics of all three processes, and show a strong dependence on stimulation energy....... In this article, an initial attempt is made to isolate only the recombination part of the luminescence cycle, and determine its thermal characteristics separately. A Variety of luminescence transitions are examined in a range of both alkali and plagioclase feldspars; three distinct emission types are identified...

  5. X-ray excited optical luminescence studies on the system Ba (, =F, Cl, Br, I)

    Indian Academy of Sciences (India)

    K Govinda Rajan; A Jestin Lenus

    2005-08-01

    The present paper reports the experimental observations on the x-ray excited optical luminescence (XEOL) along with the afterglow and colour center features found for the barium salts, represented by the formula, Ba, where and are the halides. The system thus consists of four dihalides (BaF2, . . . ,BaI2) and six mixed halides (BaFCl,. . . ,BaBrI). To start with, it was found that on two of the binary halides of barium, BaClI and BaBrI, no literature exists, and so these were prepared for the first time and their crystal structures were determined. An x-ray generator of 3-kW rating was next coupled to a spectrometer via a high throughput fiberoptic sensor for recording the luminescence spectra under x-irradiation. Also presented in this paper are the observations on the Ba compounds in which about 0.1 mole% of Eu2+ was doped, in order to study the efficiency between the prompt luminescence and the photostimulated luminescence in these compounds. The crystal structure varies from fluorite (BaF2), to matlockite (BaF) and finally to orthorhombic (BaCl2, . . .,BaBrI) for these compounds. Hence searching for systematics and empirical relations in the observed XEOL behaviour of these compounds is still a challenging problem.

  6. Thermally stimulated luminescence of polycrystalline CdWO{sub 4} at low temperatures

    Energy Technology Data Exchange (ETDEWEB)

    Novais, S.M.V.; Silva, R.S. da [Laboratory of Advanced Ceramic Materials, Physics Department, Federal University of Sergipe, 49.100-000 Sao Cristovao, SE (Brazil); Macedo, Z.S., E-mail: zelia.macedo@gmail.co [Laboratory of Advanced Ceramic Materials, Physics Department, Federal University of Sergipe, 49.100-000 Sao Cristovao, SE (Brazil)

    2011-07-15

    CdWO{sub 4} scintillator powders were produced via solid state reaction and investigated by thermally stimulated luminescence technique after UV irradiation. Under a heating rate of 0.1 K/s, the glow curve presented a superposition of peaks at low temperatures. Four peaks were identified below 80 K by partial heating method and their kinetic parameters were evaluated from the initial rise analysis. Measurements were also performed for heating rates of 0.05 and 0.2 K/s and allowed the kinetic study by peak position method. Surface effects due to the polycrystalline feature of the sample were investigated by comparing the results with those reported for CdWO{sub 4} single crystals. - Highlights: {yields} TSL glow curve of CWO presented a superposition of at least 4 peaks below 80 K. {yields} Kinetic parameters were determined from initial rise and peak position methods. {yields} Concentrations of trapping centers related to nonstoichiometry were lowered. {yields} Surface effects caused peak widening and appearance of maximums at 117 and 160 K. {yields} For temperatures above 250 K, no TSL signal was detected.

  7. Anisotropy of optical absorption and luminescent properties of CaMoO{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Zakharko, Ya., E-mail: zakharko@electronics.wups.lviv.u [Faculty of Electronics, Ivan Franko National University of Lviv, 107 Tarnavskogo St., 79017 Lviv (Ukraine); Luchechko, A. [Faculty of Electronics, Ivan Franko National University of Lviv, 107 Tarnavskogo St., 79017 Lviv (Ukraine); Syvorotka, I.; Stryganyuk, G.; Solskii, I. [Institute for Materials, SRC ' Carat' , 202 Stryjska St., 79031 Lviv (Ukraine)

    2010-03-15

    Optical absorption, excitation and emission spectra, as well as photoluminescence decay time of CaMoO{sub 4} single crystals have been measured. It has been revealed that annealing of crystals in oxygen atmosphere leads to the disappearance of their anisotropic behavior in optical absorption, as well as in X-ray luminescence and decay time. Moreover, it has been found that annealing can significantly affect the value of the decay time. The relative intensity of the long-wavelength emission band increases under excitation in the region of indirect band-to-band transitions.

  8. Lanthanide upconversion luminescence at the nanoscale: fundamentals and optical properties.

    Science.gov (United States)

    Nadort, Annemarie; Zhao, Jiangbo; Goldys, Ewa M

    2016-07-01

    Upconversion photoluminescence is a nonlinear effect where multiple lower energy excitation photons produce higher energy emission photons. This fundamentally interesting process has many applications in biomedical imaging, light source and display technology, and solar energy harvesting. In this review we discuss the underlying physical principles and their modelling using rate equations. We discuss how the understanding of photophysical processes enabled a strategic influence over the optical properties of upconversion especially in rationally designed materials. We subsequently present an overview of recent experimental strategies to control and optimize the optical properties of upconversion nanoparticles, focussing on their emission spectral properties and brightness.

  9. Lanthanide upconversion luminescence at the nanoscale: fundamentals and optical properties

    Science.gov (United States)

    Nadort, Annemarie; Zhao, Jiangbo; Goldys, Ewa M.

    2016-07-01

    Upconversion photoluminescence is a nonlinear effect where multiple lower energy excitation photons produce higher energy emission photons. This fundamentally interesting process has many applications in biomedical imaging, light source and display technology, and solar energy harvesting. In this review we discuss the underlying physical principles and their modelling using rate equations. We discuss how the understanding of photophysical processes enabled a strategic influence over the optical properties of upconversion especially in rationally designed materials. We subsequently present an overview of recent experimental strategies to control and optimize the optical properties of upconversion nanoparticles, focussing on their emission spectral properties and brightness.

  10. Thermal History Using Microparticle Trap Luminescence

    Science.gov (United States)

    2012-06-01

    34 2008 IEEE/ LEOS Optical MEMS and Nanophotonics Conference, Freiburg Germany, August 2008, pp. 64- 65. 3. J. R. Hazelton, E. G. Yukihara, M. W. Blair...A.J.J. , Prokic, M. and Brouwer , J.C., 2006. Optically and thermally stimulated luminescence characteristics of MgO:Tb3+. Radiat. Prot. Dosim. 119

  11. Tuning the Upconversion Luminescence Lifetimes of KYb2 F7 :Ho(3+) Nanocrystals for Optical Multiplexing.

    Science.gov (United States)

    Ding, Mingye; Chen, Daqin; Ma, Danyang; Liu, Peng; Song, Kaixin; Lu, Hongwei; Ji, Zhenguo

    2015-12-21

    Conventional luminescent color coding is limited by spectral overlap and the interference of background fluorescence, thus restricting the number of distinguishable identities that can be used in practice. Here, we demonstrate the possibility of generating diverse time-domain codes, specially designed for a single emission band, using lanthanide-doped upconversion nanocrystals. Based on the knowledge of concentration quenching, the upconversion luminescence kinetics of KYb2 F7 : Ho(3+) nanocrystals can be precisely controlled by modifying the dopant concentration of Ho(3+) ions, resulting in a tunable emission lifetime from 75.8 to 1944.5 μs, which suggests the practicality of these time-domain codes for optical multiplexing. © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  12. Luminescence and optical absorption determination in porous silicon

    Energy Technology Data Exchange (ETDEWEB)

    Nogal, U.; Calderon, A.; Marin, E.; Rojas T, J. B.; Juarez, A. G., E-mail: u_nogal@hotmail.com [IPN, Centro de Investigacion en Ciencia Aplicada y Tecnologia Avanzada, Calz. Legaria No. 694, Col. Irrigacion, 11500 Mexico D. F. (Mexico)

    2012-10-15

    We applied the photoacoustic spectroscopy technique in order to obtain the optical absorption spectrum in porous silicon samples prepared by electrochemical anodic etching on n-type, phosphorous doped, (100)-oriented crystal-line silicon wafer with thickness of 300 {mu}m and 1-5 {omega}cm resistivity. The porous layers were prepared with etching times of 13, 20, 30, 40 and 60 minutes. Also, we realized a comparison among the optical absorption spectrum with the photoluminescence and photo reflectance ones, both obtained at room temperature. Our results show that the absorption spectrum of the samples of porous silicon depends notably of the etching time an it consist of two distinguishable absorption bands, one in the Vis region and the other one in the UV region. (Author)

  13. Luminescence sensitivity changes in quartz

    CERN Document Server

    Wintle, A G

    1999-01-01

    In the luminescence dating of sedimentary or heated quartz, some heat treatment is usually applied to the sample immediately prior to the measurement of the optically stimulated luminescence. In this paper we report experiments on a 30,000-year-old sedimentary quartz, in which we use the luminescence response to a test dose to monitor the changes in sensitivity that are caused by holding the quartz at temperatures from 160 to 280 deg. C for times from 10 s to 22 h. For an optically bleached sample, the monitoring is by both optically stimulated luminescence and the 110 deg. C TL peak; both luminescence signals are shown to have the same sensitisation (i.e. activation energy) characteristics. For natural or laboratory irradiated samples only the 110 deg. C TL peak can be used; sensitivity increases of up to a factor of 1.3 and 3 are observed for the natural and laboratory irradiated aliquots, respectively. Up to four exponential components are used to deconvolve the sensitivity change data; the dominant compon...

  14. Analysis of thermally stimulated luminescence and conductivity without quasi-equilibrium approximation

    Science.gov (United States)

    Opanowicz, A.

    2007-08-01

    Thermally stimulated luminescence (TSL) and conductivity (TSC) are considered using the classical insulator model that assumes one kind of active trap, one kind of inactive deep trap and one kind of recombination centre. Kinetic equations describing the model are solved numerically without and with the use of quasi-equilibrium (QE) approximation. The QE state is characterized by the parameter qI = (dnc/dt)/Ie, where dnc/dt is the rate of change of free electron density, and Ie is the TSL intensity. The QE state parameter qI, the relative recombination probability γ = Ie/(Ie + It) (It is the trapping intensity) and a new parameter called a quasi-stationary (QS) state parameter q* = qIγ = (dnc/dt)/(Ie + It) are used for the analysis of the TSL and TSC. The QE and QS states are determined by conditions |qI| Lt 1 and, respectively, |q*| Lt 1. The TSL and TSC curves and the temperature dependences of qI, q*, γ the recombination lifetime and the occupancies of active traps and recombination centres are numerically calculated for five sets of kinetic parameters and different heating rates. These calculation results show that (1) the upper limit of the heating rate for the presence of the QS state appears at a higher heating rate than that for the QE state when the retrapping process is present, and (2) the TSL (TSC) curves in the QS state have properties similar to those for the TSL (TSC) curves in the QE state. Approximate formulae for calculation of the parameters qI and q* in the initial range of the TSL and TSC curves are derived and used in the heating-rate methods, proposed in this work, for determination of those parameters from the calculated TSL curves.

  15. Investigation of Optical and Luminescence Properties of Soda Lime Borate Glasses Doped with Sm3+ Ion

    Institute of Scientific and Technical Information of China (English)

    FALAK; Zaman; GUL; Rooh; NATTAPON; Srisittipokakun; JACKRAPONG; Kaewkhao

    2016-01-01

    This paper was to investigate the optical and luminescence properties of Sm3+ doped SLB glasses by a melt quenching technique. The optical and luminescence properties of the prepared glass samples were investigated via absorption and photoluminescence spectra, respectively. The related physical and optical parameters were also calculated. From optical absorption measurements, the transition 6H5/2 → 6P3/2 at 403 nm has a higher spectral intensity and is a hypersensitive transition. From photoluminescence spectra, four prominent emission spectra appear. The most intense band is located at 4G5/2 →6H9/2(599 nm), which is the characteristic emission range of Sm3+ ions with the reddish orange color. The experimental decay time of the 4G5/2 level of Sm3+ SLB glasses was determined. The decay time decreases from 1.367 to 0.333 ms with increasing the content of Sm3+. The color coordinates(x, y) of the prepared glasses passes through the reddish-orange region in the CIE 1931 diagram and are suitable for orange LEDs, optoelectronics, and solidstate lighting. The further investigation on the optimization of the dopant content in the SLB glasses was suggested.

  16. Measurement and Optimization of Metal-Nanoparticle-Induced Luminescence Enhancement Factors in a Crossed-Optical Fiber Configuration

    Directory of Open Access Journals (Sweden)

    Maria Veronica Rigo

    2010-01-01

    Full Text Available A crossed-optical-fiber configuration comprised of silver nanoparticles covalently attached to the core of an optical fiber and labeled with luminescent ruthenium molecules is reported. A second optical fiber was placed at right angle of the fiber containing the nanoparticle/ruthenium, to form a fiber-fiber junction, and it was used to detect the luminescence from the ruthenium molecules bound to the first fiber. To employ the effect of metal-enhanced luminescence, the ruthenium complex was kept at an appropriate distance from the nanoparticles by polyelectrolyte spacer layers. For silver nanospheres, nanotriangles and nanorods and for spacer-layer thicknesses from 2–14 nm luminescence-enhancement factors were determined. A 27-fold luminescence enhancement was found when the ruthenium complex was placed 4 nm from silver nanotriangles. Finally, a calibration curve for the oxygen dependence of luminescence intensities and lifetimes of ruthenium complex is presented suggesting that the oxygen sensing capabilities of the nanoengineered-ruthenium complex are maintained.

  17. X-ray-excited optical luminescence of impurity atom in semiconductor.

    Science.gov (United States)

    Ishii, M; Tanaka, Y; Komuro, S; Morikawa, T; Aoyagi, Y; Ishikawa, T

    2001-03-01

    We observed the x-ray-excited optical luminescence (XEOL) of erbium-doped silicon (Si:Er) thin films to make a site-selective x-ray absorption fine structure (XAFS) measurement of an optically active Er atom. The undulator beam was used for the increment of the electron population in the excited state, and following XEOL at an infrared wavelength of 1.54 microm with minimum absorption loss in the host Si was detected. The edge-jump and XAFS oscillation were successfully obtained at the Er L(III)-edge. This spectrum originated from inner-shell excitation and relaxation of only the optically active Er atom, indicating that site-selectivity at an atomic level was achieved.

  18. Optical filtering and luminescence property of some molybdates prepared by combustion synthesis

    Energy Technology Data Exchange (ETDEWEB)

    Yadav, P. J., E-mail: yadav.pooja75@yahoo.in [Department of Electronics, RTM Nagpur University, Nagpur (India); Joshi, C. P. [Physics Department, RCOEM, Nagpur (India); Moharil, S. V., E-mail: svmoharil@yahoo.com [Physics Department, RTM Nagpur University, Nagpur (India)

    2014-10-15

    As an important class of lanthanide inorganic compounds, rare earth ions doped molybdates have gained much attention due to their attractive luminescence and structural properties, supporting various promising applications as phosphor materials in the fields such as white light-emitting diodes, optical fibers, biolabel, lasers, and so on. The molybdate family has promising trivalent cation conducting properties and most of the optical properties result from electron transitions of the 4f shell, which are greatly affected by the composition and structures of rare-earth compounds. In this paper we report the molybdate CaMoO{sub 4}:Eu{sup 3+} for red SSL and Bi{sub 1.4}Y{sub 0.6}MoO{sub 6}, Y{sub 6}MoO{sub 12} for optical filtering, prepared by one step combustion synthesis.

  19. Luminescent conjugated oligothiophenes: optical dyes for revealing pathological hallmarks of protein misfolding diseases

    Science.gov (United States)

    Hammarström, Per; Lindgren, Mikael; Nilsson, K. Peter R.

    2010-08-01

    Luminescent conjugated polymers (LCPs) have been frequently utilized for optical biosensors. The detection schemes of these sensors are employing the light harvesting properties or the conformation sensitive optical properties of the conjugated polymers. LCPs have been utilized as colorimetric and fluorescent sensing elements for the recording of biological processes. However, LCPs have several limitations for being used as real time in vivo imaging agents. In this regard, novel thiophene based molecular scaffolds, denoted luminescent conjugated oligothiophenes (LCOs) have been developed. These LCOs are chemically defined molecules having distinct side chain functionalizations and a precise number of thiophene units. Herein the utilization of LCOs as specific ligands for the pathological hallmarks underlying protein misfolding diseases, such as Alzheimer's disease, is described. The use of the conformation sensitive optical properties of the LCOs for spectral separation of these pathological entities in a diversity of in vitro, ex vivo or in vivo systems is demonstrated. The protein aggregates are easily identified due to the conformation-dependent emission profile from the LCOs and spectral assignment of protein aggregates can be obtained. Overall, these probes will offer practical research tools for studying protein misfolding diseases and facilitate the study of the molecular mechanism underlying these disorders.

  20. Glucose optical fibre sensor based on a luminescent molecularly imprinted polymer

    Science.gov (United States)

    Elosua, C.; Wren, S. P.; Sun, T.; Arregui, F. J.; Grattan, Kenneth T. V.

    2015-09-01

    An optrode able to detect glucose dissolved in water has been implemented. The device is based on the luminescence emission of a Molecularly Imprinted Polymer synthesized specifically for glucose detection, therefore its intensity changes in presence of glucose. This sensing material is attached onto a cleaved ended polymer-clad optical fibre and it is excited by light via 1x2 fibre coupler. The reflected fluorescence signal increases when it is immersed into glucose solutions and recovers to the baseline when it is dipped in ultrapure water. This reversible behaviour indicates the measurement repeatability of using such a glucose sensor.

  1. Developments in luminescence measurement techniques

    DEFF Research Database (Denmark)

    Thomsen, Kristina Jørkov; Bøtter-Jensen, L.; Denby, Phil M.

    2006-01-01

    We report on our continuing investigation and development of new measurement facilities for use in irradiation, optical stimulation and luminescence signal detection; these facilities have potential application to all forms of luminescence-based retrospective dosimetry, and are particularly...... intended for use with the Riso TL/OSL reader. We have investigated the potential of new more powerful blue (455 nm) and green (530nm) LEDs, and of gated counting combined with pulsed stimulation light techniques using conventional LEDs. Measurement of time-resolved OSL has resulted in a method of real......; both types are very stable and reproducible. Other recent developments include the modification of a Riso reader to measure both thermally and optically stimulated electrons (TSE and OSE) from granular or chip phosphors. (c) 2006 Elsevier Ltd. All rights reserved....

  2. Visible light stimulating dual-wavelength emission and O vacancy involved energy transfer behavior in luminescence for coaxial nanocable arrays

    Science.gov (United States)

    Yang, Lei; Dong, Jiazhang; Jiang, Zhongcheng; Pan, Anlian; Zhuang, Xiujuan

    2014-06-01

    We report a strategy to investigate O vacancy (VO) involved energy transfer and dual-wavelength yellow emission in coaxial nanocable. By electric field deposition and subsequent sol-gel template approach, ZnO:Tb/Y2O3:Eu coaxial nanocable arrays are synthesized. After visible light excitation, system is promoted to O vacancy charge transfer state of VO(0/+). In the following cross relaxation, energy transfer from VO to the excitation energy level of Tb3+ in ZnO:Tb core area. While in Y2O3:Eu shell area, energy transfer to the excitation energy level of Eu3+. Subsequently, dual-wavelength emission is observed. By constructing nanocable with dual-wavelength emission, yellow luminescence is obtained. Adjust doping concentration of Eu3+ or Tb3+ in the range of 0.01-0.05, chromaticity coordinates of ZnO:Tb/Y2O3:Eu nanocable stably stays at yellow region in color space except ZnO:Tb0.01/Y2O3:Eu0.01. As Vo states act as media in energy transfer process in nanocablers, visible light can stimulate dual-wavelength emissions. Yellow luminescent nanocable arrays will have great applications in light-emitting diode luminescence.

  3. A method to remove residual signals in fibre optic luminescence dosimeters.

    Science.gov (United States)

    Lee, J J; Liu, P Z Y; McKenzie, D R; Suchowerska, N

    2013-03-07

    Whenever a fibre optic is used to convey a light signal through a radiation field, it is likely that an unwanted background signal will arise from Cerenkov or fluorescent light which will contaminate the signal. In luminescence dosimetry of high energy beams, when a fibre optic is used to convey the signal from the radiation field to the detector, Cerenkov light is the dominant contributor to the background signal and must be corrected for. In this work, a novel method is demonstrated to separate the signal from the unwanted background. A remotely operated shutter is used to block the signal, allowing the residual background in the fibre optic to be quantified. This background is subtracted from the total measurement acquired in a subsequent irradiation, enabling the luminescence signal to be extracted. Two types of shutter mechanism are considered: an electro-mechanical device to intercept the light path and an LCD device to block the light by cross-polarization. Both shutters were characterized and incorporated into a fibre optic dosimetry system used to measure the radiation dose produced by external beam radiation linear accelerators. The dosimeter using each of the shutters in turn was exposed to a 6 MV photon beam to determine their performance, including the measurement of field size dependent output factors. The mechanical shutter determined the output factors to within 0.29% of those measured with an ionization chamber, whereas the LCD shutter gave results that deviated by up to 2.4%. The switching precision of both shutters was good with standard deviations of less than 0.25% and both were able to completely block the light signal when closed. The use of shutters could therefore be applied to any fibre optic based system to quantify and remove a reproducible background arising from any source including ambient, fluorescent and Cerenkov light.

  4. Measurement of solid-state optical refrigeration by two-band differential luminescence thermometry

    Energy Technology Data Exchange (ETDEWEB)

    Hehlen, Markus P [Los Alamos National Laboratory; Epstein, Richard I [Los Alamos National Laboratory; Patterson, Wendy M [UNM; Sheik - Bahae, Mansoor [UNM; Seletskiy, D V [UNM

    2009-01-01

    We present a non-contact spectroscopic teclmique for the measurement of laser-induced temperature changes in solids. Two-band differential luminescence thermometry (TBDLT) achieves a sensitivity of {approx}7 mK and enables precise measurement of the net quantum efficiency of optical refrigerator materials. TBDLT detects internal temperature changes by decoupling surface and bulk heating effects via time-resolved luminescence spectroscopy. Several Yb{sup 3+}-doped fluorozirconate (ZBLANI) glasses fabricated from precursors of varying purity and by different processes are analyzed in detail. A net quantum efficiency of 97.39% at 238 K (at a pump wavelength of 1020.5 nm) is found for a ZBLANI:1%Yb{sup 3+} laser-cooling sample produced from metal fluoride precursors that were purified by chelate-assisted solvent extraction and dried in hydrofluoric gas. In comparison, a ZBLANI:1%Yb{sup 3+} sample produced from commercial-grade metal fluoride precursors showed pronounced laser-induced heating that is indicative of a substantially higher impurity concentration. TBDLT enables rapid and sensitive benchmarking of laser-cooling materials and provides critical feedback to the development and optimization of high-performance optical cryocooler materials.

  5. On the shape of continuous wave infrared stimulated luminescence signals from feldspars: A case study

    DEFF Research Database (Denmark)

    Pagonis, V.; Jain, Mayank; Thomsen, Kristina Jørkov

    2014-01-01

    to guide future modeling work on luminescence processes in feldspars. Small statistical differences were found between K-rich and Na-rich fractions of the same sample. However, the experimental data shows that the parameters depend on the irradiation dose, but do not depend on the time elapsed after...

  6. Measuring modulated luminescence using non-modulated stimulation: Ramping the sample period

    DEFF Research Database (Denmark)

    Poolton, N.R.J.; Bøtter-Jensen, L.; Andersen, C.E.;

    2003-01-01

    . Directly analogous results to LM-OSL can, however, be achieved with non-modulated excitation sources, by ramping the sample period (RSP) of luminescence detection. RSP-OSL has the distinct advantage over LM-OSL in that, since the excitation remains at full power, data accumulation times (that can...

  7. Thermal and electron stimulated luminescence of natural bones, commercial hydroxyapatite and collagen.

    Science.gov (United States)

    Roman-Lopez, J; Correcher, V; Garcia-Guinea, J; Rivera, T; Lozano, I B

    2014-01-01

    The luminescence (cathodoluminescence and thermoluminescence) properties of natural bones (Siberian mammoth and adult elephant), commercial hydroxyapatite and collagen were analyzed. Chemical analyses of the natural bones were determined using by Electron Probe Micro-Analysis (EMPA). Structural, molecular and thermal characteristics were determined by X-ray Diffraction (XRD), Raman spectroscopy and Differential Thermal and Thermogravimetric analysis (DTA-TG). Cathodoluminescence (CL) spectra of natural bones and collagen showed similar intense broad bands at 440 and 490 nm related to luminescence of the tetrahedral anion [Formula: see text] or structural defects. A weaker luminescence exhibited at 310 nm could be attributed to small amount of rare earth elements (REEs). Four luminescent bands at 378, 424, 468 and 576 nm were observed in the commercial hydroxyapatite (HAP). Both natural bones and collagen samples exhibited natural thermoluminescence (NTL) with well-defined glow curves whereas that the induced thermoluminescence (ITL) only appears in the samples of commercial hydroxyapatite and collagen. Additional explanations for the TL anomalous fading of apatite, as a crucial difficulty performing dosimetry and dating, are also considered.

  8. Stimulation of the human auditory nerve with optical radiation

    Science.gov (United States)

    Fishman, Andrew; Winkler, Piotr; Mierzwinski, Jozef; Beuth, Wojciech; Izzo Matic, Agnella; Siedlecki, Zygmunt; Teudt, Ingo; Maier, Hannes; Richter, Claus-Peter

    2009-02-01

    A novel, spatially selective method to stimulate cranial nerves has been proposed: contact free stimulation with optical radiation. The radiation source is an infrared pulsed laser. The Case Report is the first report ever that shows that optical stimulation of the auditory nerve is possible in the human. The ethical approach to conduct any measurements or tests in humans requires efficacy and safety studies in animals, which have been conducted in gerbils. This report represents the first step in a translational research project to initiate a paradigm shift in neural interfaces. A patient was selected who required surgical removal of a large meningioma angiomatum WHO I by a planned transcochlear approach. Prior to cochlear ablation by drilling and subsequent tumor resection, the cochlear nerve was stimulated with a pulsed infrared laser at low radiation energies. Stimulation with optical radiation evoked compound action potentials from the human auditory nerve. Stimulation of the auditory nerve with infrared laser pulses is possible in the human inner ear. The finding is an important step for translating results from animal experiments to human and furthers the development of a novel interface that uses optical radiation to stimulate neurons. Additional measurements are required to optimize the stimulation parameters.

  9. Luminescence chronology of "Old Red Sand" in Jinjiang and its implications for optical dating of sediments in South China

    Institute of Scientific and Technical Information of China (English)

    ZHANG JiaFu; YUAN BaoYin; ZHOU LiPing

    2008-01-01

    A weathered deposit in South China is widespread on the coastal areas of Fujian and Guangdong provinces, China. This deposit consists of slightly cemented, medium- to fine-grained sands, and is characterized by its colors of red, brown red, light reddish brown or dark yellowish orange, and is usually called "Old Red Sand". The uncertainty in its formation age has been a major obstacle to the study of this type of deposit. In this paper, optically stimulated luminescence (OSL) techniques were used to date the "Old Red Sand" sediments from Jinjiang, Fujian Province, China. The effect of the geochemical behavior of uranium and thorium in sediment during chemical weathering on estimation of annual dose was investigated. The results show that the change in annual dose due to weathering poses a major problem for the optical,dating of such weathered sediments. The optical dating of these weathered deposits will produce erroneous ages if average annual dose during burial cannot be correctly estimated. For the profiles studied, the OSL dates obtained on samples from the upper part do not represent the burial age of the samples. It is highly likely that they are underestimated due mainly to the accumulated radioactive elements as a result of chemical weathering. It is concluded that changes in annual dose due to chemical weathering must be considered when dating similar sediments in South China. With a detailed analysis of the OSL dating results, the chronology of the marine terraces in this area was suggested. The lowest terrace was formed at -3.5 ka and the second terrace was dated to -74 ka. The age of the highest terrace may not be established accurately, but is inferred to be older than the apparent OSL date of ~77 ka and so is the Paleolithic artifacts from it.

  10. Time-resolved luminescence from quartz: An overview of contemporary developments and applications

    Energy Technology Data Exchange (ETDEWEB)

    Chithambo, M.L., E-mail: m.chithambo@ru.ac.za [Department of Physics and Electronics, Rhodes University, PO BOX 94, Grahamstown 6140 (South Africa); Ankjærgaard, C. [Soil Geography and Landscape Group, Wageningen University Netherlands Centre for Luminescence Dating, Droevendaalsesteeg 3, 6708 PB Wageningen, The Netherlands (Netherlands); Pagonis, V. [McDaniel College, Physics Department, Westminster, MD 21157 (United States)

    2016-01-15

    Time-resolved optical stimulation of luminescence has become established as a key method for measurement of optically stimulated luminescence from quartz, feldspar and α-Al{sub 2}O{sub 3}:C, all materials of interest in dosimetry. The aim of time-resolved optical stimulation is to separate in time the stimulation and emission of luminescence. The luminescence is stimulated from a sample using a brief light pulse and the emission monitored during stimulation in the presence of scattered stimulating light or after pulsing, over photomultiplier noise only. Although the use of the method in retrospective dosimetry has been somewhat limited, the technique has been successfully applied to study mechanisms in the processes leading up to luminescence emission. The main means for this has been the temperature dependence of the luminescence intensity as well as the luminescence lifetimes determined from time-resolved luminescence spectra. In this paper we review some key developments in theory and applications to quartz including methods of evaluating lifetimes, techniques of evaluating kinetic parameters using both the dependence of luminescence intensity and lifetime on measurement temperature, and of lifetimes on annealing temperature. We then provide an overview of some notable applications such as separation of quartz signals from a quartz–feldspar admixture and the utility of the dynamic throughput, a measure of luminescence measured as a function of the pulse width. The paper concludes with some suggestions of areas where further exploration would advance understanding of dynamics of luminescence in quartz and help address some outstanding problems in its application.

  11. Effects of heat treatment on physical, microstructural and optical characteristics of PbS luminescent nanocrystals

    Science.gov (United States)

    Mozafari, Masoud; Moztarzadeh, Fathollah; Vashaee, Dayoosh; Tayebi, Lobat

    2012-04-01

    The oxidation of lead sulfide (PbS) luminescent nanocrystals (NCs) considerably changes their luminescence characteristics. Hence, an understanding of the oxidation mechanism, the structure and properties of oxidized moieties is important. In this research, well-defined spherical PbS NCs were synthesized via a simple, effective and surfactant-free method and characterized. Then, the effects of heat treatment (at 250, 350, 450 and 550 °C) on the PbS NCs were investigated. The transmission electron microscope (TEM) micrographs of the synthesized PbS NCs revealed that they had a well-defined spherical morphology. In addition, the average crystallite size using Scherrer's formula was about 13 nm and the calculated lattice constant using Bragg's equation was 0.5950 nm, which was very close to the value in the standard card (JCPDS No. 5-592). Furthermore, the X-ray diffraction (XRD) revealed that the heat treatment of samples at temperatures of 250, 350,450 and 550 °C in air results in the formation of oxide sulfate phase of the compositions PbSO4 and PbO·PbSO4. The lattice parameter, crystallite size, average internal stress, micro-strain and optical properties of PbS NCs were calculated and correlated with the heat-treatment temperature.

  12. Tuning the luminescence and optical properties of graphene oxide and reduced graphene oxide functionnalized with PVA

    Science.gov (United States)

    Goumri, Meryem; Venturini, Jany Wéry; Bakour, Anass; Khenfouch, Mohammed; Baitoul, Mimouna

    2016-03-01

    The attractive optoelectronic properties of graphene are universally known. Also, their combination with polymer matrix added an exciting physical investigation. In the present work, nanocomposites based on poly (vinyl alcohol) (PVA) with low graphene oxide (GO) and partially reduced graphene oxide (PRGO) loadings (0.5, 1 and 2 wt%) were successfully prepared by a simple and environmentally friendly process using aqueous solution in both acidic (pH 4) and neutral media (pH 7)and optimized sonication time, in order to tailor the optical/electronic properties of the GO/PRGO nanosheets. FT-IR and Raman scattering spectroscopy reveal a strong interfacial interaction by hydrogen bonding between the two components. Steady-state photoluminescence results showed a pH-dependent fluorescence of these nanocomposites, and a significant luminescence over a wide range of the visible wavelengths was achieved at a concentration of 1 wt% GO and PRGO loading. A quenching of the PL started at 2 wt% suggesting the possibility of tuning the luminescence properties of GO/PRGO-based composites with PVA.

  13. Photo- and thermally stimulated luminescence of polyminerals extracted from herbs and spices

    Science.gov (United States)

    Cruz-Zaragoza, E.; Marcazzó, J.; Chernov, V.

    2012-08-01

    Ionizing radiation processing is a widely employed method for preservative treatment of foodstuffs. Usually it is possible to detect irradiated herbs and spices by resorting to luminescence techniques, in particular photo- and thermostimulated luminescence. For these techniques to be useful, it is necessary to characterize the response to radiation of each particular herb or spice. In this work, the thermoluminescence (TL) and photostimulated luminescence (PSL) properties of inorganic polymineral fractions extracted from commercial herbs and spices previously irradiated for disinfestation purposes have been analyzed. Samples of mint, cinnamon, chamomile, paprika, black pepper, coriander and Jamaica flower were irradiated from 50 to 400 Gy by using a beta source. The X-ray diffraction (XRD) analysis has shown that the mineral fractions consist mainly of quartz and feldspars. The PSL and TL response as a function of the absorbed dose, and their fading at room temperature have been determined. The TL glow curves have been deconvolved in order to obtain characteristic kinetics parameters in each case. The results of this work show that PSL and TL are reliable techniques for detection and analysis of irradiated foodstuffs.

  14. Testing the application of quartz and feldspar luminescence dating to MIS 5 Japanese marine deposits

    DEFF Research Database (Denmark)

    Thiel, Christine; Tsukamoto, Sumiko; Tokuyasu, Kayoko

    2015-01-01

    The applicability of both quartz and feldspar luminescence dating was tested on twenty-five samples from a marine succession now forming a coastal cliff at Oga Peninsula, Honshu Island, Japan. The quartz optically stimulated luminescence (OSL) signal shows thermal instability and linear modulated...

  15. Thermally stimulated luminescence and photoluminescence investigations of Eu3+ and Eu2+ doped SrBPO5

    Indian Academy of Sciences (India)

    Mithlesh Kumar; T K Seshagiri; S V Godbole

    2013-10-01

    Thermally stimulated luminescence (TSL) investigations of SrBPO5:Eu3+ and SrBPO5:Eu2+ phosphors were carried out in the temperature range of 300–650 K. In order to characterize the phosphors, X-ray diffraction and photoluminescence (PL) techniques were used. The emission spectrum of air heated SrBPO5:Eu3+ phosphor exhibited emission bands at 590, 614, 651 and 702 nm under 248 nm excitation, assigned to transitions of Eu3+ ion. In phosphor prepared in reducing (Ar + 8% H2) atmosphere, a broad emission band due to Eu2+ ranging from 350 to 400 nm was observed with 340 nm excitation. EPR studies have confirmed the presence of Eu2+ ions in the samples prepared in reducing atmosphere. TSL glow curve of SrBPO5:Eu3+ had shown intense peaks around 397, 510, 547 K and a weak peak around 440 K whereas in case of SrBPO5:Eu2+ system, glow peaks at 414, 478 and weak peak at 516 nm were observed. The shift in TSL glow pattern can be attributed to stabilization of different oxidation states of the dopant ion in the host lattice. Apart from this, TSL trap parameters such as trap depth and frequency factor were determined. Spectral characteristics of TSL emission have shown that Eu3+/Eu2+ ion acts as the luminescent centre in the respective phosphors.

  16. Time-resolved luminescence from feldspars: New insight into fading

    DEFF Research Database (Denmark)

    Tsukamoto, S.; Denby, P.M.; Murray, A.S.

    2006-01-01

    Time-resolved infrared optically stimulated luminescence (IR-OSL) signals of K- and Na-feldspar samples extracted from sediments were measured in UV, blue and red detection windows, using a fast photon counter and pulsed IR stimulation (lambda = 875 nm). We observe that the relative contribution...

  17. Synthesis, characterisation, optical and luminescence properties of CoAl{sub 2}O{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Agilandeswari, K.; Kumar, A. Ruban, E-mail: arubankumarvit@gmail.com [School of Advanced Sciences, VIT University, Vellore, Tamil Nadu, India-632014 (India)

    2015-06-24

    Solid state method has been used as an efficient method to synthesize blue pigment CoAl{sub 2}O{sub 4} at a temperature of 800°C. The products were characterized by powder X-ray diffraction (XRD), Fourier transformer infrared spectroscopy (FTIR), UV-Visible diffuse reflectance spectroscopy (DRS) and luminescent spectroscopy. X-ray diffraction pattern confirmed the formation of single phase CoAl{sub 2}O{sub 4}. Optical properties of CoAl{sub 2}O{sub 4} ceramic shows an energy band gap in the range of 3.10eV. The emission spectra of spinel CoAl{sub 2}O{sub 4} in the visible region confirmed the presence of tetrahedral coordinated Co{sup 2+} ions.

  18. In vivo X-Ray excited optical luminescence from phosphor-doped aerogel and Sylgard 184 composites

    Science.gov (United States)

    Allison, Stephen W.; Baker, Ethan S.; Lynch, Kyle J.; Sabri, Firouzeh

    2017-06-01

    X-Ray excited optical luminescence (XEOL) is a new and noninvasive diagnostic technique suitable for in situ biochemical imaging and disease detection. The X-Ray excited optical luminescence of phosphor doping in crosslinked silica aerogel and Sylgard 184 hosts was investigated in this study. Composite silica aerogels and Sylgard 184 samples of 5%, 15%, and 50% concentrations by weight of La2O2S:Eu phosphor were prepared and inserted subcutaneously in a Sprague-Dawley rat and excited by X-Ray emission at 70 and 100 kV. A fiber optic bundle positioned within 5 mm of the sample collected the luminescence signal and conveyed it to a photomultiplier detector. The signal intensity scaled with dopant concentration. The time dependence of the predominantly red luminescence consisted of 60 cycle bursts of approximately 8 ms duration. The amplitude was modulated at about 10 Hz with a 60% depth. This indicates the time dependence of the X-Ray source. A simulation showed how to observe phosphor decay between individual burst pulses. The emission from the two types of composite samples was easily detected from the outside of the skin layer. Both Sylgard 184 and crosslinked silica aerogels are biocompatible and bio stable materials that could serve a variety of potential XEOL applications. These very strong signals imply potential for creating new In-vivo sensing applications and diagnostic tools.

  19. Micro-modulated luminescence tomography

    CERN Document Server

    Cong, Wenxiang; Wang, Chao; Wang, Ge

    2013-01-01

    Imaging depth of optical microscopy has been fundamentally limited to millimeter or sub-millimeter due to light scattering. X-ray microscopy can resolve spatial details of few microns deeply inside a sample but the contrast resolution is still inadequate to depict heterogeneous features at cellular or sub-cellular levels. To enhance and enrich biological contrast at large imaging depth, various nanoparticles are introduced and become essential to basic research and molecular medicine. Nanoparticles can be functionalized as imaging probes, similar to fluorescent and bioluminescent proteins. LiGa5O8:Cr3+ nanoparticles were recently synthesized to facilitate luminescence energy storage with x-ray pre-excitation and the subsequently stimulated luminescence emission by visible/near-infrared (NIR) light. In this paper, we suggest a micro-modulated luminescence tomography (MLT) approach to quantify a nanophosphor distribution in a thick biological sample with high resolution. Our numerical simulation studies demonst...

  20. Evaluation of Dynamic Optical Projection of Acquired Luminescence for Sentinel Lymph Node Biopsy in Large Animals.

    Science.gov (United States)

    Ringhausen, Elizabeth; Wang, Tylon; Pitts, Jonathan; Sarder, Pinaki; Akers, Walter J

    2016-12-01

    Open surgery requiring cytoreduction still remains the primary treatment course for many cancers. The extent of resection is vital for the outcome of surgery, greatly affecting patients' follow-up treatment including need for revision surgery in the case of positive margins, choice of chemotherapy, and overall survival. Existing imaging modalities such as computed tomography, magnetic resonance imaging, and positron emission tomography are useful in the diagnostic stage and long-term monitoring but do not provide the level of temporal or spatial resolution needed for intraoperative surgical guidance. Surgeons must instead rely on visual evaluation and palpation in order to distinguish tumors from surrounding tissues. Fluorescence imaging provides high-resolution, real-time mapping with the use of a contrast agent and can greatly enhance intraoperative imaging. Here we demonstrate an intraoperative, real-time fluorescence imaging system for direct highlighting of target tissues for surgical guidance, optical projection of acquired luminescence (OPAL). Image alignment, accuracy, and resolution was determined in vitro prior to demonstration of feasibility for operating room use in large animal models of sentinel lymph node biopsy. Fluorescence identification of regional lymph nodes after intradermal injection of indocyanine green was performed in pigs with surgical guidance from the OPAL system. Acquired fluorescence images were processed and rapidly reprojected to highlight indocyanine green within the true surgical field. OPAL produced enhanced visualization for resection of lymph nodes at each anatomical location. Results show the optical projection of acquired luminescence system can successfully use fluorescence image capture and projection to provide aligned image data that is invisible to the human eye in the operating room setting. © The Author(s) 2015.

  1. Enhancing and quenching luminescence with gold nanoparticle films: the influence of substrate on the luminescent properties

    Science.gov (United States)

    José Guidelli, Eder; Ramos, Ana Paula; Baffa, Oswaldo

    2016-01-01

    Gold nanoparticle (AuNP) films were sputtered over glass and aluminum substrates to enhance optically stimulated luminescence (OSL), a luminescent technique employed for radiation detection, from x-ray irradiated NaCl nanocrystals. The AuNP films deposited over glass led to enhanced-OSL emission, whereas the AuNP films deposited on aluminum substrates quenched the OSL emission. The enhanced-OSL intensity is proportional to the optical density of the film's plasmon resonance band at the stimulation wavelength. For the case of the AuNP/aluminum films, the luminescence quenching diminishes, and OSL intensity partially recovers upon increasing the distance between the AuNPs and the aluminum substrates, and between the luminescent nanocrystals and the AuNP films. These results suggest that plasmonic interactions between the emitter nanocrystals, the localized surface plasmons (LSP) of the AuNPs, and the substrate are responsible for the OSL enhancement and quenching. In this sense, the substrate dictates whether LSP relaxation occurs by radiative or non-radiative transisitions, leading to enhanced or quenched OSL, respectively. Therefore, besides showing that AuNP films can enhance and/or tune the sensitivity of luminescent radiation detectors, and demonstrating OSL as a new technique to investigate mechanisms of plasmon-enhanced luminescence, these results bring insights on how substrates strongly modify the optical properties of AuNP films.

  2. Tailoring of the luminescent ions local environment in optical fibers, and applications

    CERN Document Server

    Dussardier, Bernard; Peterka, P

    2012-01-01

    The chapter is situated in the fields of fiber materials sciences and technologies (particularly dealing with the fiber glass compositions and luminescent ion doping, and transparent glass ceramic optical fibers), and applications such as fiber lasers and amplifiers. We propose to present a review of research activities on rare-earth (RE) and transition metals (TM) doped silica-based optical fibers, aiming at understanding theier spectral properties, and particularly some of their optical transitions that will allow interesting and alternative applications. Silica, as opposed to alternative, low temperature materials, is chosen for practical and economical reasons. Selected RE and TM ions are studied both as probes of their local environment and for their application potentials. In this chapter, we will focus on erbium (Er) ions for the potential spectral 'tailoring' of its gain curve at 1.55 $\\mu$m, thulium (Tm) as local environment probe along both near infrared transitions around 0.8 and 1.47 $\\mu$m, and c...

  3. Optically stimulated phosphorescence in orthoclase feldspar over the millisecond to second time scale

    DEFF Research Database (Denmark)

    Ankjærgaard, Christina; Jain, Mayank

    2010-01-01

    In the past, time-resolved IR stimulated luminescence (TR-IRSL) curves from feldspar have mainly been measured over a few hundred μs with the purpose of estimating the lifetimes of the components. In this study, we present the decay form of time-resolved IRSL and IR stimulated phosphorescence (IRSP......) from orthoclase feldspar covering over 8 orders of magnitude (50 ns to 7 s). A detailed characterisation of the slowly decaying signals (ms to s time scales) from feldspar is undertaken to obtain further insight into the role of re-trapping in both the IR stimulated luminescence (IRSL...

  4. Enhancement of second-order nonlinear-optical signals by optical stimulation

    CERN Document Server

    Goodman, Aaron J

    2015-01-01

    Second-order nonlinear optical interactions such as sum- and difference-frequency generation are widely used for bioimaging and as selective probes of interfacial environments. However, inefficient nonlinear optical conversion often leads to poor signal-to-noise ratio and long signal acquisition times. Here, we demonstrate the dramatic enhancement of weak second-order nonlinear optical signals via stimulated sum- and difference-frequency generation. We present a conceptual framework to quantitatively describe the interaction and show that the process is highly sensitive to the relative optical phase of the stimulating field. To emphasize the utility of the technique, we demonstrate stimulated enhancement of second harmonic generation (SHG) from bovine collagen-I fibrils. Using a stimulating pulse fluence of only 3 nJ/cm2, we obtain an SHG enhancement >10^4 relative to the spontaneous signal. The stimulation enhancement is greatest in situations where spontaneous signals are the weakest - such as low laser pow...

  5. Implantable optical-electrode device for stimulation of spinal motoneurons

    Science.gov (United States)

    Matveev, M. V.; Erofeev, A. I.; Zakharova, O. A.; Pyatyshev, E. N.; Kazakin, A. N.; Vlasova, O. L.

    2016-08-01

    Recent years, optogenetic method of scientific research has proved its effectiveness in the nerve cell stimulation tasks. In our article we demonstrate an implanted device for the spinal optogenetic motoneurons activation. This work is carried out in the Laboratory of Molecular Neurodegeneration of the Peter the Great St. Petersburg Polytechnic University, together with Nano and Microsystem Technology Laboratory. The work of the developed device is based on the principle of combining fiber optic light stimulation of genetically modified cells with the microelectrode multichannel recording of neurons biopotentials. The paper presents a part of the electrode implant manufacturing technique, combined with the optical waveguide of ThorLabs (USA).

  6. Application of luminescence techniques in retrospective dosimetry

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.; Jungner, H.

    1999-01-01

    Luminescence signals measured from minerals within bricks or ceramic samples can provide information about the absorbed radiation dose. This feature has for several years been used in dating archaeological and geological samples and recently luminescence techniques have been intensively used far...... retrospective assessment of accident doses received by the population after a nuclear accident. The development of new luminescence techniques after the Chernobyl accident has considerably improved the sensitivity and precision in the evaluation of accident doses. This paper reviews the development work......, especially on optically stimulated luminescence methods for retrospective assessment of accident doses carried out at Riso National Laboratory in collaboration with the University of Helsinki as part bf a joint European Union research project. We demonstrate that doses lower than 100 mGy can be measured from...

  7. A device for obtaining stimulated optical emission

    Energy Technology Data Exchange (ETDEWEB)

    Kvaril, J.; Kubelka, J.; Kvapil, J.; Perner, B.

    1983-04-30

    A laser is proposed which is characterized by the use of a YAG active material in the laser with neodymium ion and/or ionic elements with atomic numbers of 58-59 and 61-71 used as the dopant. The ratio of the molar concentration of the yttrium oxide and dopant oxide in the initial mixture is equal to (3.001 to 3.030) to 5. Additionally, an optical active filter is used in the laser; this filter includes a methyl orange and rhodamine 6G solution or glass with a dopant of 1 percent cesium oxide and 2.5 percent titanium oxide.

  8. Characterisation of blue-light stimulated luminescence components in different quartz samples: Implications for dose measurement

    DEFF Research Database (Denmark)

    Jain, M.; Murray, A.S.; Bøtter-Jensen, L.

    2003-01-01

    results from measurement of (a) sensitisation, (b) thermal stability, (c) recuperation, and (d) infrared response as a function of stimulation temperature from 3 different samples of sedimentary quartz selected on the basis of relative OSL contribution from different blue light stimulated linearly...

  9. Optical, luminescence and thermal properties of radiopure ZnMoO{sub 4} crystals used in scintillating bolometers for double beta decay search

    Energy Technology Data Exchange (ETDEWEB)

    Chernyak, D.M. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); Centre de Sciences Nucléaires et de Sciences de la Matière, 91405 Orsay (France); Danevich, F.A. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); Degoda, V.Ya.; Dmitruk, I.M. [Kyiv National Taras Shevchenko University, MSP 03680 Kyiv (Ukraine); Ferri, F. [Dipartimento di Scienza e Alta Tecnologia dell' Università dell' Insubria, Como I-22100 (Italy); Galashov, E.N. [Nikolaev Institute of Inorganic Chemistry, 630090 Novosibirsk (Russian Federation); Giuliani, A., E-mail: Andrea.Giuliani@csnsm.in2p3.fr [Centre de Sciences Nucléaires et de Sciences de la Matière, 91405 Orsay (France); Dipartimento di Scienza e Alta Tecnologia dell' Università dell' Insubria, Como I-22100 (Italy); Sezione INFN di Milano-Bicocca, I-20126 Italy (Italy); Ivanov, I.M. [Nikolaev Institute of Inorganic Chemistry, 630090 Novosibirsk (Russian Federation); Kobychev, V.V. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); Mancuso, M.; Marnieros, S. [Centre de Sciences Nucléaires et de Sciences de la Matière, 91405 Orsay (France); Dipartimento di Scienza e Alta Tecnologia dell' Università dell' Insubria, Como I-22100 (Italy); Mokina, V.M. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); Nones, C.; Olivieri, E. [Service de Physique des Particules, CEA-Saclay, F-91191 Gif sur Yvette (France); Pessina, G. [Sezione INFN di Milano-Bicocca, I-20126 Italy (Italy); Rusconi, C. [Dipartimento di Scienza e Alta Tecnologia dell' Università dell' Insubria, Como I-22100 (Italy); Sezione INFN di Milano-Bicocca, I-20126 Italy (Italy); and others

    2013-11-21

    Zinc molybdate (ZnMoO{sub 4}) crystals are an excellent candidate material to fabricate scintillating bolometers for the study of neutrinoless double beta decay of {sup 100}Mo, provided that the crystal quality meets strict optical, thermal and radiopurity requirements. This paper addresses the characterization of improved crystalline samples grown by the low-thermal-gradient Czochralski technique. Transmittance measurements confirm significant improvement of the material with respect to previously developed samples. Luminescence properties (emission spectra, dependence of intensity on temperature, thermally stimulated luminescence and phosphorescence) have been studied under X-ray excitation from liquid-helium to room temperature. The index of refraction was measured in the wavelength interval 406–655 nm. Samples of ZnMoO{sub 4} crystals with masses of 5.07 g and 23.8 g were operated as scintillating bolometers at temperatures below 30 mK, with simultaneous detection of scintillation and heat signals, confirming an excellent alpha/beta rejection power. Background measurements allowed encouraging radiopurity level estimations. The light collection from ZnMoO{sub 4} scintillators was Monte Carlo simulated, analysing different crystal size, shape and surface properties and different photodetector sizes.

  10. Optical stimulation of the facial nerve: a surgical tool?

    Science.gov (United States)

    Richter, Claus-Peter; Teudt, Ingo Ulrik; Nevel, Adam E.; Izzo, Agnella D.; Walsh, Joseph T., Jr.

    2008-02-01

    One sequela of skull base surgery is the iatrogenic damage to cranial nerves. Devices that stimulate nerves with electric current can assist in the nerve identification. Contemporary devices have two main limitations: (1) the physical contact of the stimulating electrode and (2) the spread of the current through the tissue. In contrast to electrical stimulation, pulsed infrared optical radiation can be used to safely and selectively stimulate neural tissue. Stimulation and screening of the nerve is possible without making physical contact. The gerbil facial nerve was irradiated with 250-μs-long pulses of 2.12 μm radiation delivered via a 600-μm-diameter optical fiber at a repetition rate of 2 Hz. Muscle action potentials were recorded with intradermal electrodes. Nerve samples were examined for possible tissue damage. Eight facial nerves were stimulated with radiant exposures between 0.71-1.77 J/cm2, resulting in compound muscle action potentials (CmAPs) that were simultaneously measured at the m. orbicularis oculi, m. levator nasolabialis, and m. orbicularis oris. Resulting CmAP amplitudes were 0.3-0.4 mV, 0.15-1.4 mV and 0.3-2.3 mV, respectively, depending on the radial location of the optical fiber and the radiant exposure. Individual nerve branches were also stimulated, resulting in CmAP amplitudes between 0.2 and 1.6 mV. Histology revealed tissue damage at radiant exposures of 2.2 J/cm2, but no apparent damage at radiant exposures of 2.0 J/cm2.

  11. A robust feldspar luminescence dating method for Middle and Late Pleistocene sediments

    DEFF Research Database (Denmark)

    Buylaert, Jan-Pieter; Jain, Mayank; Murray, Andrew S.

    2012-01-01

    Luminescence dating is used extensively to provide absolute chronologies for Late Pleistocene sediments. Nowadays, most optical dates are based on quartz optically stimulated luminescence (OSL). However, the application of this signal is usually limited to the last ~100 ka because of saturation...... of the quartz luminescence signal with dose. In contrast, the feldspar infrared stimulated luminescence (IRSL) dose–response curve grows to much higher doses; this has the potential to extend the datable age range by a factor of 4–5 compared with quartz OSL. However, it has been known for several decades...... is widely applicable (feldspar of appropriate luminescence behaviour is even more ubiquitous than quartz). These characteristics make this a method of great importance for the dating of Middle and Late Pleistocene deposits....

  12. On the relationship between luminescence excitation spectra and feldspar mineralogy

    DEFF Research Database (Denmark)

    Poolton, N.R.J.; Bøtter-Jensen, L.; Johnsen, O.

    1996-01-01

    Feldspar minerals can be used as naturally occurring radiation dosemeters, with dose assessment commonly using luminescence techniques. Since many feldspars contain radioactive K-40, knowledge of the mineralogy of the luminescent samples being measured is of high importance. Most feldspars contain...... more than trace amounts of highly luminescent Fe3+ impurities, and this article examines the relationship between features of the luminescence excitation spectrum of this ion with sample mineralogy. It is demonstrated that there is a near linear correspondence between the plagioclase feldspar...... groups. The results are compared with properties of the excitation spectra dose-dependent optically stimulated luminescence (OSL) in order to compare the chemical environment of the OSL donor defect, and the isolated Fe3+ centres....

  13. Monte Carlo simulation of an x-ray luminescence optical tomography scanner prototype

    Energy Technology Data Exchange (ETDEWEB)

    Rosas-González, S., E-mail: sarahi@fisica.unam.mx, E-mail: arnulfo@fisica.unam.mx; Martínez-Dávalos, A., E-mail: sarahi@fisica.unam.mx, E-mail: arnulfo@fisica.unam.mx; Rodríguez-Villafuerte, M., E-mail: sarahi@fisica.unam.mx, E-mail: arnulfo@fisica.unam.mx; Murrieta-Rodríguez, T., E-mail: sarahi@fisica.unam.mx, E-mail: arnulfo@fisica.unam.mx [Instituto de Física, Universidad Nacional Autónoma de México, A.P. 20-364, 01000 (Mexico)

    2014-11-07

    In this work we report the calculation of the deposited energy distribution produced by an x-ray luminescence optical tomography (XLOT) system in a phantom containing different concentrations of Gd{sub 2}O{sub 2}S:Eu nanoparticles. The calculations were performed via Monte Carlo simulation considering spectra from a W target x-ray tube operating between 30 and 90 kVp, with 1.0 mm Al added filtration. CT and XLOT tomographic images were reconstructed from the same data. The results show that XLOT has better detectability than CT alone, that the dose scales linearly with kVp for a fixed concentration of Gd{sub 2}O{sub 2}S:Eu and air-kerma rate, the scattered radiation contribution to the total dose and signal is about 20% and that the dose ratio for a 3 mm diameter insert containing 10 mg/ml Gd{sub 2}O{sub 2}S embedded in a 30 mm diameter water phantom is 6:1. This ratio drops to less than 2:1 for a 1 mg/ml concentration. Finally we show that the method of conjugate images can be used to correct for artifacts due to attenuation effects in XLOT images.

  14. Insights on proximity effect and multiphoton induced luminescence from gold nanospheres in far field optical microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Borglin, Johan [Biomedical Photonics Group, Department of Chemistry and Molecular Biology, University of Gothenburg, Kemivägen 10, 412 96 Gothenburg (Sweden); Department of Physics, University of Gothenburg, Kemivägen 10, 412 96 Gothenburg (Sweden); Guldbrand, Stina [Department of Physics, University of Gothenburg, Kemivägen 10, 412 96 Gothenburg (Sweden); Evenbratt, Hanne [Pharmaceutical Technology, Department of Chemistry and Chemical Engineering, Chalmers University of Technology, Kemigården 4, 412 96 Gothenburg (Sweden); Kirejev, Vladimir; Ericson, Marica B., E-mail: marica.ericson@chem.gu.se [Biomedical Photonics Group, Department of Chemistry and Molecular Biology, University of Gothenburg, Kemivägen 10, 412 96 Gothenburg (Sweden); Grönbeck, Henrik [Department of Applied Physics, Chalmers University of Technology, Kemivägen 9, 412 96 Gothenburg (Sweden)

    2015-12-07

    Gold nanoparticles can be visualized in far-field multiphoton laser-scanning microscopy (MPM) based on the phenomena of multiphoton induced luminescence (MIL). This is of interest for biomedical applications, e.g., for cancer diagnostics, as MPM allows for working in the near-infrared (NIR) optical window of tissue. It is well known that the aggregation of particles causes a redshift of the plasmon resonance, but its implications for MIL applying far-field MPM should be further exploited. Here, we explore MIL from 10 nm gold nanospheres that are chemically deposited on glass substrates in controlled coverage gradients using MPM operating in NIR range. The substrates enable studies of MIL as a function of inter-particle distance and clustering. It was shown that MIL was only detected from areas on the substrates where the particle spacing was less than one particle diameter, or where the particles have aggregated. The results are interpreted in the context that the underlying physical phenomenon of MIL is a sequential two-photon absorption process, where the first event is driven by the plasmon resonance. It is evident that gold nanospheres in this size range have to be closely spaced or clustered to exhibit detectable MIL using far-field MPM operating in the NIR region.

  15. Stimulated luminescence property of Zn(BO{sub 2}){sub 2}:TbCl{sub 3}

    Energy Technology Data Exchange (ETDEWEB)

    Cedillo, G.; Cruz Z, E. [UNAM, Instituto de Ciencias Nucleares, Circuito Exterior, Ciudad Universitaria, 04510 Mexico D. F. (Mexico); Garcia H, M. [UNAM, Instituto de Investigaciones en Materiales, Posgrado en Ciencia e Ingenieria de Materiales, Apdo. Postal 70-360, 04510 Mexico D. F. (Mexico); Marcazzo, J. [Instituto de Fisica Arroyo Seco / UNICEN, Gral. Pinto 399, 7000 Tandil, Buenos Aires (Argentina); Hernandez A, J. M.; Murrieta S, H., E-mail: ecruz@nucleares.unam.mx [UNAM, Instituto de Fisica, Apdo. Postal 20-364, 01000 Mexico D. F. (Mexico)

    2015-10-15

    Zinc borate, Zn(BO{sub 2}){sub 2}, doped with TbCl{sub 3} at different concentration (0.5-8 mol %) was synthesized. The polycrystalline samples were characterized by Scanning Electron Microscopy (Sem/EDS) and X-ray Diffraction. The X-ray difractrograms of the pure samples sintered at 750 and 800 degrees C shown the evidence of the Zn(BO{sub 2}){sub 2} has the body centered cubic (bcc) structure and a ZnB{sub 4}O{sub 7} primitive orthorhombic phase of the crystal system. The thermoluminescent (Tl) intensity was dependent on the thermal treatment (250-500 degrees C) and also on the impurity concentration. The glow curves show four glow peaks at about 82, 164, 251, and 331 degrees C when the Tb{sup 3+} doped zinc borate samples were exposed to gamma or beta radiation. The structure of the glow curves was analyzed by CGCD deconvolution method. The kinetics parameters (activation energy, frequency factor and the kinetic order) were calculated assuming the general order kinetics model describing accurately the Tl process. The glow peaks were overlapped and then the whole glow curve was considered for dosimetric characteristics measurements. The linear Tl response as a function of gamma and beta doses was performed using a {sup 60}Co irradiator and a {sup 90}Sr, respectively. Zinc borate with 8 mol % of impurity concentration exhibited an intense radio luminescent (Rl) emission. The Rl spectra show their maximum bands at 370, 490, 545 and 700 nm. The linear dose-response was between 2.2 c Gy and 27.7 Gy when the samples were exposed to beta radiation. These results suggest that the Tb -doped zinc borate material is a good phosphor for use in radiation dosimetry because its high Tl sensitivity to the ionizing radiation and good dose-response. (Author)

  16. Power-penalty-free all-optical decryption using stimulated Brillouin scattering in optical fiber

    Science.gov (United States)

    Yi, L. L.; Zhang, T.; Li, Z. X.; Zhang, Y.; Dong, Y.; Hu, W. S.

    2013-04-01

    We propose to all-optically encrypt and decrypt high-speed optical signals using the stimulated Brillouin scattering (SBS) effect in optical fiber for the first time. The spectral-shaped SBS gain or loss distorts the broadband optical signal so as to realize optical encryption. A corresponding SBS loss or gain with the same spectral shape and amplitude recovers the distorted signal to implement optical decryption. We experimentally demonstrate the SBS encryption/decryption process on 10.86 Gb s-1 non-return-to-zero-on-off-keying (NRZ-OOK) data using phase-modulated Brillouin pumps to generate a spectral-shaped SBS gain/loss encryption key, and no power penalty is observed for the best decryption case. The proposed all-optical encryption/decryption method is completely compatible with existing fiber-optic communication systems.

  17. Evolution of photo-stimulated luminescence of EB-PVD/(Ni, Pt)Al thermal barrier coatings

    Energy Technology Data Exchange (ETDEWEB)

    Wen Mei [Department of Metallurgy and Materials Engineering, University of Connecticut, Storrs, CT 06269 (United States); Jordan, Eric H. [Department of Mechanical Engineering, University of Connecticut, Storrs, CT 06269 (United States)]. E-mail: jordan@engr.uconn.edu; Gell, Maurice [Department of Metallurgy and Materials Engineering, University of Connecticut, Storrs, CT 06269 (United States)

    2005-05-25

    Experiments are described which were designed to assess the suitability of photo-stimulated luminescence piezo-spectroscopy (PLPS) measurements as a basis for non-destructive inspection (NDI) and determination of life remaining of thermal barrier coatings (TBCs). Thermal cyclic tests were conducted on 7 wt.% Y{sub 2}O{sub 3} stabilized ZrO{sub 2} (YSZ) electron beam physical vapor deposited (EB-PVD)/(Ni, Pt)Al/CMSX-4 TBCs at two temperatures 1151 and 1121 deg. C. The evolution of PLPS spectral characteristics (peak frequency shift, peak width and area ratio of peaks) was studied as a function of thermal cycles. It was observed that the average thermally grown oxide (TGO) stress and its standard deviation, and the area ratio of peaks show systematic change with thermal cycling, indicating that these characteristics can be used for NDI and determination of life remaining. The average TGO stress increases initially and then decreases monotonically with thermal cycling. The rate of change in the stress can be related to specimen life: the shallower the slope, the higher the life. The peak area ratio also decreases monotonically with cycling. The average TGO stress changes in a systematic manner versus remaining life fraction independent of temperature. Remaining life predictions were made based on average stress versus life fraction, which resulted in life assessments within {+-}13% of actual values excluding one specimen with abnormal behavior.

  18. Characteristics of pulsed photo-stimulated luminescence and thermoluminescence for the identification of gamma irradiated poultry eggs

    Institute of Scientific and Technical Information of China (English)

    2007-01-01

    Pulsed photo-stimulated luminescence (PPSL) is a simple screening method that can be employed qualitatively at the spot for the detection of eggs treated with ionizing radiation. Due to the variations in the results during storage, the eggs of ostrich, duck, hen, and quail were irradiated to doses of 0, 1, 2, and 3 kGy. Most of the samples were incorrectly identified during storage after four months of irradiation. Thermoluminescence (TL)technique was also tried by using egg shells in order to confirm the irradiation treatment in eggs. TL glow curves were recorded between the temperatures 50℃ to 400℃ at the rate of 5°/s for all the control and irradiated samples. On the basis of integrated areas of first glow curves (TL1), the glow curve ratios (TL1/TL2) and the shapes of maxima of TL1,the irradiation treatment of all the eggs was confirmed. Furthermore, the presence of calcite and aragonite minerals that cause the TL signal in the egg shells were studied using X-ray diffraction spectrometry.

  19. Transformation optics simulation method for stimulated Brillouin scattering

    CERN Document Server

    Zecca, Roberto; Smith, David R; Larouche, Stéphane

    2016-01-01

    We develop a novel approach to enable the full-wave simulation of stimulated Brillouin scattering and related phenomena in a frequency-domain, finite-element environment. The method uses transformation optics techniques to implement a time-harmonic coordinate transform that reconciles the different frames of reference used by electromagnetic and mechanical finite-element solvers. We show how this strategy can be successfully applied to bulk and guided systems, comparing the results with the predictions of established theory.

  20. Effect of an electron beam irradiation on optical and luminescence properties of LiBaAlF6 single crystals

    Science.gov (United States)

    Ogorodnikov, I. N.; Pustovarov, V. A.; Omelkov, S. I.; Kirm, M.

    2017-07-01

    Paper reports the effect of a 10 keV, 110 keV and 10 MeV electron beam irradiation on optical and luminescence properties of LiBaAlF6 (LBAF) single crystals at 10, 90, and 293 K. Five absorption bands at 2.0, 3.2, 4.3, 4.9 and 5.5 eV were revealed in irradiated crystals in the energy range of 1.2-9.5 eV. Several PL emission bands (1.7-1.8, 2.2 and 2.5-3.5 eV) related to defects were found in the luminescence spectra at room temperature, while only one luminescence band at E = 2.2 eV appears at T = 90 K in LBAF crystals after a 10 MeV electron bombardment. The PL excitation spectra and time-response for these emission bands were studied at 10, 90, and 293 K. Thermoluminescence (TL) of irradiated crystals was studied in the temperature range of 90-740 K. New TL glow peaks at 166, 530 and 670 K were revealed and their parameters were determined. Temperature dependence of relative photoluminescence yield recorded monitoring emission at the 1.87 and 2.23 eV in the temperature range from 130 to 450 K, were fitted using five quenching processes related to TL glow peaks revealed in our research. Significant similarity in the manifestation of radiation-induced defects for LBAF and previously studied LiBaF3 single crystals is noted. The effect of an electron beam irradiation on optical and luminescence properties of LBAF single crystals and possible origin of the radiation defects were discussed.

  1. Optical gain and stimulated emission in periodic nanopatterned crystalline silicon.

    Science.gov (United States)

    Cloutier, Sylvain G; Kossyrev, Pavel A; Xu, Jimmy

    2005-12-01

    Persistent efforts have been made to achieve efficient light emission from silicon in the hope of extending the reach of silicon technology into fully integrated optoelectronic circuits, meeting the needs for high-bandwidth intrachip and interchip connects. Enhanced light emission from silicon is known to be theoretically possible, enabled mostly through quantum-confinement effects. Furthermore, Raman-laser conversion was demonstrated in silicon waveguides. Here we report on optical gain and stimulated emission in uniaxially nanopatterned silicon-on-insulator using a nanopore array as an etching mask. In edge-emission measurements, we observed threshold behaviour, optical gain, longitudinal cavity modes and linewidth narrowing, along with a collimated far-field pattern, all indicative of amplification and stimulated emission. The sub-bandgap 1,278 nm emission peak is attributed to A-centre mediated phononless direct recombination between trapped electrons and free holes. The controlled nanoscale silicon engineering, combined with the low material loss in this sub-bandgap spectral range and the long electron lifetime in such A-type trapping centres, gives rise to the measured optical gain and stimulated emission and provides a new pathway to enhance light emission from silicon.

  2. Limits to depletion of blue-green light stimulated luminescence in feldspars: Implications for quartz dating

    DEFF Research Database (Denmark)

    Jain, M.; Singhvi, A.K.

    2001-01-01

    -red stimulation at elevated temperature (220 degreesC) (ETIR) permits depletions of charges in Type (A) and Type (B) to the extent that the feldspar BGSL can be reduced by up to 97% in 5 min. These results offer prospects for (1) improved precision in paleodose estimates based on quartz; (2) BGSL dating of quartz...... in a polyminerallic fine grain samples; (3) age estimates based on both quartz and feldspars from the same aliquots, and (4) dating based on feldspar micro-inclusions. (C) 2001 Elsevier Science Ltd. All rights reserved....

  3. Luminescence, optical and laser Raman scattering studies on γ -irradiated terbium-doped potassium iodide crystals

    Science.gov (United States)

    Bangaru, S.

    2011-02-01

    This paper reports the thermoluminescence (TL), optical absorption and other laser Raman scattering studies performed on terbium-doped KI crystals γ-irradiated at room temperature. Photoluminescence studies confirm the presence of terbium ions in the KI matrix in their trivalent form. Formation of V3- and Z1-centres on F-bleaching of γ-irradiated crystals was observed. The characteristic emission due to Tb3+ ions in the spectral distribution under optically stimulated emission and TL emission confirms the participation of the Tb3+ ions in the recombination process. The Raman bands were identified as the totally symmetric vibration modes of f.c.c. species KI:Tb3+.

  4. Configurational coordinate diagram of Ni{sup 2+} doped silver halide crystals, as determined by optical and luminescence measurements

    Energy Technology Data Exchange (ETDEWEB)

    Zakosky-Neuberger, I., E-mail: yifat_z2@hotmail.com [Raymond and Beverly Sackler Faculty of Exact Sciences, School of Physics and Astronomy, Tel-Aviv University, Tel-Aviv 69978 (Israel); Shafir, I.; Nagli, L.; Katzir, A. [Raymond and Beverly Sackler Faculty of Exact Sciences, School of Physics and Astronomy, Tel-Aviv University, Tel-Aviv 69978 (Israel)

    2012-08-15

    Optical and luminescence measurements were carried out on Ni{sup 2+} doped silver halide crystals. The configurational coordinates of the ground and the first excited states made it possible to explain the important optical properties, such as the Stokes shift between the ground and excited states, the broadening of the bands with temperature and the thermal quenching. Determining the configurational coordinate diagram of the ground and first excited states is the first step for the design and fabrication of solid state and fiber lasers which are based on Ni{sup 2+} doped silver halides and which operate in the middle infrared. - Highlights: Black-Right-Pointing-Pointer Optical and luminescence measurements were carried out on Ni{sup 2+} doped silver halide crystals. Black-Right-Pointing-Pointer Configurational coordinates of the ground and the first excited state were calculated. Black-Right-Pointing-Pointer Optical properties of Ni{sup 2+} doped silver halide crystals can be obtained from the configurational coordinate diagram. Black-Right-Pointing-Pointer No emission signal was found above 220 K.

  5. New Nanomaterials and Luminescent Optical Sensors for Detection of Hydrogen Peroxide

    OpenAIRE

    Natalia A. Burmistrova; Olga A. Kolontaeva; Axel Duerkop

    2015-01-01

    Accurate methods that can continuously detect low concentrations of hydrogen peroxide (H2O2) have a huge application potential in biological, pharmaceutical, clinical and environmental analysis. Luminescent probes and nanomaterials are used for fabrication of sensors for H2O2 that can be applied for these purposes. In contrast to previous reviews focusing on the chemical design of molecular probes for H2O2, this mini-review highlights the latest luminescent nanoparticular materials and new lu...

  6. Mechanism of red-luminescence flash in CdS single crystals irradiated by electrons

    Energy Technology Data Exchange (ETDEWEB)

    Bogdanyuk, N.S.; Galushka, A.P.; Ostapenko, S.S.; Shejnkman, M.K. (AN Ukrainskoj SSR, Kiev. Inst. Poluprovodnikov)

    1984-02-01

    Results of investigations into ''red''-luminescence flash (lambdasub(x)=720 nm) in cadmium sulfide, irradiated by electrons at 77 K, are presented. Measurement of spectra of stationary photoluminescence and its excitation, as well as flash luminescence, its pumping and stimulation along with temperature flash dependences enabled to suggest a new mechanism of optical luminescence stimulation, based on the model of complex center of flash luminescense. The mechanism consists in modulation of probabilities of intercenter electron transitions, when charge state of one of components of the complex center changes.

  7. Enhancement of Second-Order Nonlinear-Optical Signals by Optical Stimulation

    Science.gov (United States)

    Goodman, A. J.; Tisdale, W. A.

    2015-05-01

    Second-order nonlinear optical interactions such as sum- and difference-frequency generation are widely used for bioimaging and as selective probes of interfacial environments. However, inefficient nonlinear optical conversion often leads to poor signal-to-noise ratio and long signal acquisition times. Here, we demonstrate the dramatic enhancement of weak second-order nonlinear optical signals via stimulated sum- and difference-frequency generation. We present a conceptual framework to quantitatively describe the interaction and show that the process is highly sensitive to the relative optical phase of the stimulating field. To emphasize the utility of the technique, we demonstrate stimulated enhancement of second harmonic generation (SHG) from bovine collagen-I fibrils. Using a stimulating pulse fluence of only 3 nJ /cm2 , we obtain an SHG enhancement >104 relative to the spontaneous signal. The stimulation enhancement is greatest in situations where spontaneous signals are the weakest—such as low laser power, small sample volume, and weak nonlinear susceptibility—emphasizing the potential for this technique to improve signal-to-noise ratios in biological imaging and interfacial spectroscopy.

  8. Exposure to static magnetic field stimulates quorum sensing circuit in luminescent Vibrio strains of the Harveyi clade.

    Science.gov (United States)

    Talà, Adelfia; Delle Side, Domenico; Buccolieri, Giovanni; Tredici, Salvatore Maurizio; Velardi, Luciano; Paladini, Fabio; De Stefano, Mario; Nassisi, Vincenzo; Alifano, Pietro

    2014-01-01

    In this study, the evidence of electron-dense magnetic inclusions with polyhedral shape in the cytoplasm of Harveyi clade Vibrio strain PS1, a bioluminescent bacterium living in symbiosis with marine organisms, led us to investigate the behavior of this bacterium under exposure to static magnetic fields ranging between 20 and 2000 Gauss. When compared to sham-exposed, the light emission of magnetic field-exposed bacteria growing on solid medium at 18°C ±0.1°C was increased up to two-fold as a function of dose and growth phase. Stimulation of bioluminescence by magnetic field was more pronounced during the post-exponential growth and stationary phase, and was lost when bacteria were grown in the presence of the iron chelator deferoxamine, which caused disassembly of the magnetic inclusions suggesting their involvement in magnetic response. As in luminescent Vibrio spp. bioluminescence is regulated by quorum sensing, possible effects of magnetic field exposure on quorum sensing were investigated. Measurement of mRNA levels by reverse transcriptase real time-PCR demonstrated that luxR regulatory gene and luxCDABE operon coding for luciferase and fatty acid reductase complex were significantly up-regulated in magnetic field-exposed bacteria. In contrast, genes coding for a type III secretion system, whose expression was negatively affected by LuxR, were down-regulated. Up-regulation of luxR paralleled with down-regulation of small RNAs that mediate destabilization of luxR mRNA in quorum sensing signaling pathways. The results of experiments with the well-studied Vibrio campbellii strain BB120 (originally classified as Vibrio harveyi) and derivative mutants unable to synthesize autoinducers suggest that the effects of magnetic fields on quorum sensing may be mediated by AI-2, the interspecies quorum sensing signal molecule.

  9. Highly luminescent and cytocompatible cationic Ag2S NIR-emitting quantum dots for optical imaging and gene transfection

    OpenAIRE

    Duman, Fatma Demir; Hocaoğlu, İbrahim; Hocaoglu, Ibrahim; Öztürk, Deniz Gülfem; Ozturk, Deniz Gulfem; Gözüaçık, Devrim; Gozuacik, Devrim; Kiraz, Alper; Yağcı Acar, Havva; Yagci Acar, Havva

    2015-01-01

    Nanoscale PAPER Cite this: Nanoscale, 2015, 7, 11352 Received 12th January 2015, Accepted 23rd May 2015 DOI: 10.1039/c5nr00189g www.rsc.org/nanoscale Highly luminescent and cytocompatible cationic Ag2S NIR-emitting quantum dots for optical imaging and gene transfection† Fatma Demir Duman,a Ibrahim Hocaoglu,a Deniz Gulfem Ozturk,b Devrim Gozuacik,b Alper Kiraza,c and Havva Yagci Acar*a,d,e The development of non-toxic theranostic nanoparticles capable of del...

  10. The manifestation of optical centers in UV-Vis absorption and luminescence spectra of white blood human cells

    Science.gov (United States)

    Terent'yeva, Yu G.; Yashchuk, V. M.; Zaika, L. A.; Snitserova, O. M.; Losytsky, M. Yu

    2016-12-01

    A white blood human cells spectral investigation is presented. The aim of this series of experiments was to obtain and analyze the absorption and luminescence (fluorescence and phosphorescence) spectra at room temperature and at 78 K of newly isolated white blood human cells and their organelles. As a result the optical centers and possible biochemical components that form the studied spectra where identified. Also the differences between the spectra of abnormal cells (B-cell chronic lymphocytic leukemia BCLL) and normal ones were studied for the whole cells and individual organelles.

  11. [Photo-stimulated and long persistent luminescence properties of Sr3SiO5 : Eu2+, RE3+ (RE = Nd3+, Ho3+, La3+)].

    Science.gov (United States)

    Zhang, Zhe; Xu, Xu-hui; Qiu, Jian-bei; Zhang, Xin; Yu, Xue

    2014-06-01

    A series of electron capture materials Sr3SiO5 : Eu2+, RE3+ (RE = Nd3+, Ho3+, La3+) were prepared by high temperature solid state method. The photo-stimulated luminescence (PSL) and long afterglow performance were evaluated. After excited by UV light, it showed a strong up-conversion photo-stimulated read-out response when stimulated by 980 nm laser, which is attributed to the existence of deep traps (438 K). This property was especially shown in Sr3 SiO5 : Eu2+, La3+ and Sr3SiO5 : EU2+, Ho3+. Subsequently, the trapping depth and carrier concentration were studied. In this way, we verified the cause of PSL. The calculation of parameters of trapping electron in the thermoluminescence spectrum is through the method of Chen's half width, getting the value of trapping depth under the temperature of 438 K, which contrasts to the energy of 980 nm laser radiation. At the same time, the afterglow performance after co-doping with rare earth ion was greatly improved. The afterglow time of Sr3 SiO5 : Eu2+ , La3+ is up to 12 hours. Research results show that the change in mixed trap structure is the primary cause of photo-stimulated and long persistent luminescence properties.

  12. EDITORIAL: Special issue on optical neural engineering: advances in optical stimulation technology Special issue on optical neural engineering: advances in optical stimulation technology

    Science.gov (United States)

    Shoham, Shy; Deisseroth, Karl

    2010-08-01

    Neural engineering, itself an 'emerging interdisciplinary research area' [1] has undergone a sea change over the past few years with the emergence of exciting new optical technologies for monitoring, stimulating, inhibiting and, more generally, modulating neural activity. To a large extent, this change is driven by the realization of the promise and complementary strengths that emerging photo-stimulation tools offer to add to the neural engineer's toolbox, which has been almost exclusively based on electrical stimulation technologies. Notably, photo-stimulation is non-contact, can in some cases be genetically targeted to specific cell populations, can achieve high spatial specificity (cellular or even sub-cellular) in two or three dimensions, and opens up the possibility of large-scale spatial-temporal patterned stimulation. It also offers a seamless solution to the problem of cross-talk generated by simultaneous electrical stimulation and recording. As in other biomedical optics phenomena [2], photo-stimulation includes multiple possible modes of interaction between light and the target neurons, including a variety of photo-physical and photo-bio-chemical effects with various intrinsic components or exogenous 'sensitizers' which can be loaded into the tissue or genetically expressed. Early isolated reports of neural excitation with light date back to the late 19th century [3] and to Arvanitaki and Chalazonitis' work five decades ago [4]; however, the mechanism by which these and other direct photo-stimulation, inhibition and modulation events [5-7] took place is yet unclear, as is their short- and long-term safety profile. Photo-chemical photolysis of covalently 'caged' neurotransmitters [8, 9] has been widely used in cellular neuroscience research for three decades, including for exciting or inhibiting neural activity, and for mapping neural circuits. Technological developments now allow neurotransmitters to be uncaged with exquisite spatial specificity (down to

  13. Luminescence sensitivity changes in quartz as a result of annealing

    DEFF Research Database (Denmark)

    Bøtter-Jensen, L.; Agersnap Larsen, N.; Mejdahl, V.

    1995-01-01

    Retrospective dosimetry using optically stimulated luminescence (OSL) on quartz extracted from (for example) bricks needs to account for strong OSL sensitivity changes that are known to occur depending on the previous thermal treatment of the sample. Non-heated quartz exhibits OSL orders of magni......Retrospective dosimetry using optically stimulated luminescence (OSL) on quartz extracted from (for example) bricks needs to account for strong OSL sensitivity changes that are known to occur depending on the previous thermal treatment of the sample. Non-heated quartz exhibits OSL orders...... of magnitude less per unit radiation than that for heated material. The reason these temperature-induced sensitivity changes occur in quartz is presently not well understood. This phenomenon is also seen in the related area of luminescence dating in which sedimentary quartz and quartz from heated...

  14. Optical stimulation of zebrafish hair cells expressing channelrhodopsin-2.

    Directory of Open Access Journals (Sweden)

    Bryan D Monesson-Olson

    Full Text Available Vertebrate hair cells are responsible for the high fidelity encoding of mechanical stimuli into trains of action potentials (spikes in afferent neurons. Here, we generated a transgenic zebrafish line expressing Channelrhodopsin-2 (ChR2 under the control of the hair-cell specific myo6b promoter, in order to examine the role of the mechanoelectrical transduction (MET channel in sensory encoding in afferent neurons. We performed in vivo recordings from afferent neurons of the zebrafish lateral line while activating hair cells with either mechanical stimuli from a waterjet or optical stimuli from flashes of ∼470-nm light. Comparison of the patterns of encoded spikes during 100-ms stimuli revealed no difference in mean first spike latency between the two modes of activation. However, there was a significant increase in the variability of first spike latency during optical stimulation as well as an increase in the mean number of spikes per stimulus. Next, we compared encoding of spikes during hair-cell stimulation at 10, 20, and 40-Hz. Consistent with the increased variability of first spike latency, we saw a significant decrease in the vector strength of phase-locked spiking during optical stimulation. These in vivo results support a physiological role for the MET channel in the high fidelity of first spike latency seen during encoding of mechanical sensory stimuli. Finally, we examined whether remote activation of hair cells via ChR2 activation was sufficient to elicit escape responses in free-swimming larvae. In transgenic larvae, 100-ms flashes of ∼470-nm light resulted in escape responses that occurred concomitantly with field recordings indicating Mauthner cell activity. Altogether, the myo6b:ChR2 transgenic line provides a platform to investigate hair-cell function and sensory encoding, hair-cell sensory input to the Mauthner cell, and the ability to remotely evoke behavior in free-swimming zebrafish.

  15. Comparative analysis of luminescent properties of germanate glass and double-clad optical fibers co-doped with Yb3+/Ho3+ ions

    Science.gov (United States)

    Pietrzycki, Marcin; Kochanowicz, Marcin; Romańczuk, Patryk; Żmojda, Jacek; Miluski, Piotr; Ragiń, Tomasz; Jeleń, Piotr; Sitarz, Maciej; Dorosz, Dominik

    2016-09-01

    The 2 μm and visible emission of low phonon (805 cm-1) germanate glasses and double - clad optical fiber co-doped with 0.7Yb2O3/(0.07-0.7)Ho2O3 ions have been investigated. Luminescence at 2 μm corresponding to Ho3+: 5I7 → 5I8 as well as upconversion luminescence in the visible spectral range corresponding to the Ho3+: 5S2(5F4)→5I8 (545 nm), and Ho3+: 5F5→5I8 (655 nm) transition, respectively were obtained. The optimization of the acceptor content and donor-acceptor ratio were conducted with the purpose of maximizing the luminescence intensity. The highest luminescence intensity in both spectral range was obtained in glass co-doped with 0.7Yb2O3/0.15 Ho2O3. Despite relatively small effective absorption coefficient of the optical fiber comparative analysis of luminescent properties of fabricated glasses (further core) and double - clad optical fiber showed significant contribution of reabsorption process of emitted ASE signal.

  16. Internal luminescence efficiencies in InGaP/GaAs/Ge triple-junction solar cells evaluated from photoluminescence through optical coupling between subcells

    Science.gov (United States)

    Tex, David M.; Imaizumi, Mitsuru; Akiyama, Hidefumi; Kanemitsu, Yoshihiko

    2016-12-01

    In-situ characterization is one of the most powerful techniques to improve material quality and device performance. Especially in view of highly efficient tandem solar cells this is an important issue for improving the cost-performance ratio. Optical techniques are suitable characterization methods, since they are non-destructing and contactless. In this work, we measured the power dependence of photoluminescence (PL) from the InGaP and GaAs subcells of an industry-standard triple-junction solar cell. High luminescence yields enhance the luminescence coupling, which was directly verified by time-resolved PL measurements. We present a new method to determine the internal luminescence efficiencies of InGaP and GaAs subcells with the aid of luminescence coupling. High luminescence efficiencies of 90% for GaAs and more than 20% for InGaP were found, which suggest that the material quality of the grown GaAs layer is excellent while the intrinsic luminescence limit of InGaP is still not reached even for high excitation conditions. The PL method is useful for probing the intrinsic material properties of the subcells in flat band condition, without influence of transport. Since no calibration of absolute PL is required, a fast screening of the material quality is possible, which should be extremely helpful for the solar cell industry.

  17. Optical and luminescence studies of ZnMoO 4 using vacuum ultraviolet synchrotron radiation

    Science.gov (United States)

    Mikhailik, V. B.; Kraus, H.; Wahl, D.; Ehrenberg, H.; Mykhaylyk, M. S.

    2006-06-01

    In this paper we present a characterisation of ZnMoO 4 using spectroscopic techniques. Reflection, luminescence and luminescence excitation spectra were measured over the temperature range 8-295 K using VUV synchrotron radiation. The emission spectrum of the crystal exhibits a broad band with a maximum around 1.95 eV at 80 K that is attributed to the radiative transitions within MO 42- oxyanion complex. An interpretation of the observed features of the electronic excitations in the crystal is given based on present knowledge of the electronic structure and emission properties of molybdate crystals. The results of this study suggest that ZnMoO 4 is a suitable candidate for further testing for implementation as a target material in cryogenic scintillation searches for rare events.

  18. Optical and luminescence studies of ZnMoO{sub 4} using vacuum ultraviolet synchrotron radiation

    Energy Technology Data Exchange (ETDEWEB)

    Mikhailik, V.B. [Department of Physics, University of Oxford, Keble Road, Oxford OX1 3RH (United Kingdom)]. E-mail: vmikhai@hotmail.com; Kraus, H. [Department of Physics, University of Oxford, Keble Road, Oxford OX1 3RH (United Kingdom); Wahl, D. [Department of Physics, University of Oxford, Keble Road, Oxford OX1 3RH (United Kingdom); Ehrenberg, H. [Material Science, Darmstadt University of Technology, Petersenstr. 23, Darmstadt 64287 (Germany); Mykhaylyk, M.S. [Physics Department, Lviv National University, 8 Kyryla and Mefodiya str., Lviv, 79005 (Ukraine)

    2006-06-15

    In this paper we present a characterisation of ZnMoO{sub 4} using spectroscopic techniques. Reflection, luminescence and luminescence excitation spectra were measured over the temperature range 8-295 K using VUV synchrotron radiation. The emission spectrum of the crystal exhibits a broad band with a maximum around 1.95 eV at 80 K that is attributed to the radiative transitions within MO{sub 4} {sup 2-} oxyanion complex. An interpretation of the observed features of the electronic excitations in the crystal is given based on present knowledge of the electronic structure and emission properties of molybdate crystals. The results of this study suggest that ZnMoO{sub 4} is a suitable candidate for further testing for implementation as a target material in cryogenic scintillation searches for rare events.

  19. X-ray absorption fine structure and X-ray excited optical luminescence studies of II-VI semiconducting nanostructures

    Science.gov (United States)

    Murphy, Michael Wayne

    2010-06-01

    Various II-VI semiconducting nanomaterials such as ZnO-ZnS nanoribbons (NRs), CdSxSe1-x nanostructures, ZnS:Mn NRs, ZnS:Mn,Eu nanoprsims (NPs), ZnO:Mn nanopowders, and ZnO:Co nanopowders were synthesized for study. These materials were characterized by techniques such as scanning electron microscopy, transmission electron microscopy, element dispersive X-ray spectroscopy, selected area electron diffraction, and X-ray diffraction. The electronic and optical properties of these nanomaterials were studied by X-ray absorption fine structure (XAFS) spectroscopy and X-ray excited optical luminescence (XEOL) techniques, using tuneable soft X-rays from a synchrotron light source. The complementary nature ofthe XAFS and XEOL techniques give site, element and chemical specific measurements which allow a better understanding of the interplay and role of each element in the system. Chemical vapour deposition (CVD) of ZnS powder in a limited oxygen environment resulted in side-by-side biaxial ZnO-ZnS NR heterostructures. The resulting NRs contained distinct wurtzite ZnS and wurtzite ZnO components with widths of 10--100 nm and 20 --500 nm, respectively and a uniform interface region of 5-15 nm. XAFS and XEOL measurements revealed the luminescence of ZnO-ZnS NRs is from the ZnO component. The luminescence of CdSxSe1-x nanostructures is shown to be dependent on the S to Se ratio, with the band-gap emission being tunable between that of pure CdS and CdSe. Excitation of the CdSxSe 1-x nanostructures by X-ray in XEOL has revealed new de-excitation channels which show a defect emission band not seen by laser excitation. CVD of Mn2+ doped ZnS results in nanostructures with luminescence dominated by the yellow Mn2+ emission due to energy transfer from the ZnS host to the Mn dopant sites. The addition of EuCl3 to the reactants in the CVD process results in a change in morphology from NR to NP. Zn1-xMnxO and Zn1-xCOxO nanopowders were prepared by sol-gel methods at dopant concentrations

  20. Multicolour optical coding from a series of luminescent lanthanide complexes with a unique antenna.

    Science.gov (United States)

    Wartenberg, Nicolas; Raccurt, Olivier; Bourgeat-Lami, Elodie; Imbert, Daniel; Mazzanti, Marinella

    2013-03-04

    The bis-tetrazolate-pyridine ligand H(2)pytz sensitises efficiently the visible and/or near-IR luminescence emission of ten lanthanide cations (Pr, Nd, Sm, Eu, Tb, Dy, Ho, Er, Tm, Yb). The Ln(III) complexes present sizeable quantum yields in both domains with a single excitation source. The wide range of possible colour combinations in water, organic solvents and the solid state makes the complexes very attractive for labelling and encoding.

  1. Improved properties of phosphor-filled luminescent down-shifting layers: reduced scattering, optical model, and optimization for PV application

    Science.gov (United States)

    Solodovnyk, Anastasiia; Lipovšek, Benjamin; Forberich, Karen; Stern, Edda; Krč, Janez; Batentschuk, Miroslaw; Topič, Marko; Brabec, Christoph J.

    2015-12-01

    We studied the optical properties of polymer layers filled with phosphor particles in two aspects. First, we used two different polymer binders with refractive indices n = 1.46 and n = 1.61 (λ = 600 nm) to decrease Δn with the phosphor particles (n = 1.81). Second, we prepared two particle size distributions D50 = 12 μm and D50 = 19 μm. The particles were dispersed in both polymer binders in several volume concentrations and coated onto glass with thicknesses of 150 - 600 μm. We present further a newly developed optical model for simulation and optimization of such luminescent down-shifting (LDS) layers. The model is developed within the ray tracing framework of the existing optical simulator CROWM (Combined Ray Optics / Wave Optics Model), which enables simulation of standalone LDS layers as well as complete solar cells (including thick and thin layers) enhanced by the LDS layers for an improved solar spectrum harvesting. Experimental results and numerical simulations show that the layers of the higher refractive index binder with larger particles result in the highest optical transmittance in the visible light spectrum. Finally we proved that scattering of the phosphor particles in the LDS layers may increase the overall light harvesting in the solar cell. We used numerical simulations to determine optimal layer composition for application in realistic thin-film photovoltaic devices. Surprisingly LDS layers with lower measured optical transmittance are more efficient when applied onto the solar cells due to graded refractive index and efficient light scattering. Therefore, our phosphor-filled LDS layers could possibly complement other light-coupling techniques in photovoltaics.

  2. Optogenetics Based Rat-Robot Control: Optical Stimulation Encodes "Stop" and "Escape" Commands.

    Science.gov (United States)

    Chen, SiCong; Zhou, Hong; Guo, SongChao; Zhang, JiaCheng; Qu, Yi; Feng, ZhouYan; Xu, KeDi; Zheng, XiaoXiang

    2015-08-01

    Electric brain stimulation is frequently used in bio-robot control. However, one possible limitation of electric stimulation is the resultant wide range of influences that may lead to unexpected side-effects. Although there has been prior research done towards optogenetics based brain activation, there has not been much development regarding the comparisons between electric and optical methods of brain activation. In this study, we first encode "Stop" and "Escape" commands by optical stimulation in the dorsal periaqueductal grey (dPAG). The rats behavioral comparisons are then noted down under these two methods. The dPAG neural activity recorded during optical stimulation suggests rate and temporal coding mechanisms in behavioral control. The behavioral comparisons show that rats exhibit anxiety under the "Stop" command conveyed through both optical and electric methods. However, rats are able to recover more quickly from freezing only under optical "Stop" command. Under "Escape" commands, also conveyed through optical means, the rat would move with lessened urgency but the results are more stable. Moreover, c-Fos study shows the optical stimulation activates restricted range in midbrain: the optical stimulation affected only dPAG and its downstreams but electric stimulation activates both the upstream and downstream circuits, in which the glutamatergic neurons are largely occupied and play important role in "Stop" and "Escape" behavior controls. We conclude that optical stimulation is more suited for encoding "Stop" and "Escape" commands for rat-robot control.

  3. Structure, optical and photoluminescence properties of LiGd1-xErx(WO4)2 green luminescence phosphor

    Science.gov (United States)

    Demiaï, A.; Derbal, M.; Guerbous, L.; Rekik, B.

    2017-03-01

    Double tungstate of lithium and trivalent gadolinium ions were prepared by mean of solid state reaction, and have been studied using X-ray diffraction, Raman scattering and photoluminescence analysis. The Er3+ concentration effects on the structural and optical properties were studied. The compounds crystallize in the scheelite like structure with space group I41/a, and Z = 2. Spectroscopic and structural properties of the Er3+ ions doping elements in LiGd(WO4)2 have been determined at room temperature. Steady and time resolved photoluminescence spectroscopies of the synthesized compounds are reported. Samples exhibit intense green emission of Er3+ (4S3/2 → 4I15/2 and 2H11/2 → 4I15/2 transitions) under 377 nm excitation wavelength and present luminescent quenching around 3 at% Er3+ concentration. The decay time decrease with increasing the Er3+ concentration.

  4. Ag7+ ion induced modification of morphology, optical and luminescence behaviour of charge compensated CaMoO4 nanophosphor

    Science.gov (United States)

    Dutta, S.; Som, S.; Kunti, A. K.; Sharma, S. K.; Kumar, Vijay; Swart, H. C.; Visser, H. G.

    2016-10-01

    The present paper reports on the swift heavy ion (SHI) induced structural, optical and luminescence properties of CaMoO4:Dy3+/K+ nanophosphor synthesized via hydrothermal route. Herein 100 MeV Ag7+ ion beam was used varying fluence from 1 × 1011 to 1 × 1013 ions/cm2. The depth profile of the Ag7+ ions was estimated using SRIM code. XRD and FESEM results revealed the loss of crystallinity and reduction in particle size after SHI irradiations. The XPS technique confirmed the stability of oxidation states of the elements. Reflectance spectra exhibited a red shift in the absorption band, followed by a decrease in band gap. Decrease in the intensity of the photoluminescence peaks without any change in band positions was also obtained after ion irradiation. The thermoluminescence (TL) characteristics were discussed in detail, and the trapping parameter was calculated. The results were compared on the grounds of linear energy transfer of the irradiated ions.

  5. X-ray-excited optical luminescence of protein crystals: a new tool for studying radiation damage during diffraction data collection.

    Science.gov (United States)

    Owen, Robin L; Yorke, Briony A; Pearson, Arwen R

    2012-05-01

    During X-ray irradiation protein crystals radiate energy in the form of small amounts of visible light. This is known as X-ray-excited optical luminescence (XEOL). The XEOL of several proteins and their constituent amino acids has been characterized using the microspectrophotometers at the Swiss Light Source and Diamond Light Source. XEOL arises primarily from aromatic amino acids, but the effects of local environment and quenching within a crystal mean that the XEOL spectrum of a crystal is not the simple sum of the spectra of its constituent parts. Upon repeated exposure to X-rays XEOL spectra decay non-uniformly, suggesting that XEOL is sensitive to site-specific radiation damage. However, rates of XEOL decay were found not to correlate to decays in diffracting power, making XEOL of limited use as a metric for radiation damage to protein crystals. © 2012 International Union of Crystallography

  6. Scintillation and storage luminescence properties of MgF2 transparent ceramics doped with Ce3+

    Science.gov (United States)

    Nakamura, Fumiya; Kato, Takumi; Okada, Go; Kawaguchi, Noriaki; Fukuda, Kentaro; Yanagida, Takayuki

    2017-10-01

    In this paper, we report basic optical properties and scintillation and storage luminescence properties of MgF2:Ce transparent ceramics with different doping concentrations of Ce (0.01, 0.1 and 1%) synthesized by spark plasma sintering (SPS). In scintillation, thermally-stimulated luminescence (TSL) and optically-stimulated luminescence (OSL), the dominant emissions were due to the 5d-4f transitions of Ce3+ which appeared in the near-UV region peaking around 320 and 360 nm. The scintillation was evaluated by X-ray irradiation while OSL was observed under 540 nm stimulation. In particular, the TSL sensitivity was high and showed a good linearity from 0.1 mGy to 1000 mGy.

  7. Mechanoresponsive Luminescent Molecular Assemblies: An Emerging Class of Materials.

    Science.gov (United States)

    Sagara, Yoshimitsu; Yamane, Shogo; Mitani, Masato; Weder, Christoph; Kato, Takashi

    2016-02-10

    The possibility to change the molecular assembled structures of organic and organometallic materials through mechanical stimulation is emerging as a general and powerful concept for the design of functional materials. In particular, the photophysical properties such as photoluminescence color, quantum yield, and emission lifetime of organic and organometallic fluorophores can significantly depend on the molecular packing, enabling the development of molecular materials with mechanoresponsive luminescence characteristics. Indeed, an increasing number of studies have shown in recent years that mechanical force can be utilized to change the molecular arrangement, and thereby the optical response, of luminescent molecular assemblies of π-conjugated organic or organometallic molecules. Here, the development of such mechanoresponsive luminescent (MRL) molecular assemblies consisting of organic or organometallic molecules is reviewed and emerging trends in this research field are summarized. After a brief introduction of mechanoresponsive luminescence observed in molecular assemblies, the concept of "luminescent molecular domino" is introduced, before molecular materials that show turn-on/off of photoluminescence in response to mechanical stimulation are reviewed. Mechanically stimulated multicolor changes and water-soluble MRL materials are also highlighted and approaches that combine the concept of MRL molecular assemblies with other materials types are presented in the last part of this progress report.

  8. Measurement of Solid-State Optical Refrigeration by Two-Band Differential Luminescence Thermometry

    Science.gov (United States)

    2010-03-01

    induced cooling of a solid in 1995 produced a mere 0.3 K of cooling in the Yb3+-doped fluorozirconate glass (ZrF4–BaF2–LaF3–AlF3–NaF, ZBLAN ) [1...sensitivity is indicative of what can be achieved for a Yb3+-doped ZBLAN glass . Other materials will have dif- ferent luminescence spectra with...Model of laser cooling in the Yb3+-doped fluorozirconate glass ZBLAN ,” Phys. Rev. B 75, 144302 (2007). Fig. 8. TBDLT parameter [measured in vacuum

  9. The use of the adding-doubling method for the optical optimization of planar luminescent down shifting layers for solar cells.

    Science.gov (United States)

    Leyre, Sven; Cappelle, Jan; Durinck, Guy; Abass, Aimi; Hofkens, Johan; Deconinck, Geert; Hanselaer, Peter

    2014-05-05

    To enhance the efficiency of solar cells, a luminescent down shifting layer can be applied in order to adapt the solar spectrum to the spectral internal quantum efficiency of the semiconductor. Optimization of such luminescent down shifting layers benefits from quick and direct evaluation methods. In this paper, the potential of the adding-doubling method is investigated to simulate the optical behavior of an encapsulated solar cell including a planar luminescent down shifting layer. The results of the adding-doubling method are compared with traditional Monte Carlo ray tracing simulations. The average relative deviation is found to be less than 1.5% for the absorptance in the active layer and the reflectance from the encapsulated cell, while the computation time can be decreased with a factor 52. Furthermore, the adding-doubling method is adopted to investigate the suitability of the SrB4O7:5%Sm2 + ,5%Eu2 + phosphor as a luminescent down shifting material in combination with a Copper Indium Gallium Selenide solar cell. A maximum increase of 9.0% in the short-circuit current can be expected if precautions are taken to reduce the scattering by matching the refractive index of host material to the phosphor particles. To be useful as luminescent down shifting material, the minimal value of the quantum yield of the phosphor is determined to be 0.64.

  10. FORMATION OF LUMINESCENT OPTICAL WAVEGUIDES IN SILICATE GLASS MATRIX BY THE ION-EXCHANGE TECHNIQUE

    Directory of Open Access Journals (Sweden)

    I. A. Dyomichev

    2015-01-01

    Full Text Available We present spectra of the alkali-silicate glasses with copper ions in near-surface area, introduced by ion exchange of different temperature and duration. It is shown that the reduction of Cu2+ in the near-surface area causes existence of Cu+ and neutral atoms in glass after the ion-exchange in divalent salt. The ion-exchange itself involves only Cu+ and Na+ ions. The formation of subnanometer clusters Cun is due to neutral copper atoms staying in near-surface zone. We have shown that the waveguide layer in near-surface area, made by ion-exchange, has а visible luminescence with the excitation by UVradiation. At the same time, the contribution to luminescence is made by Cu+ ions, molecular clusters Cun and by dimers Cu+ - Cu+ . During the high-temperature ion-exchange at 600 °С the formation and destruction equilibrium shift of molecular clusters Cun can be seen. An hour ion-exchange leads to molecular clusters Cun destruction, while at time periods less than 30 min and around 18 hours it leads to the formation of Cun. The sample turns green after 18,5 hours ion-exchange showing formation of a considerable amount of divalent copper ions Cu2+ therein.

  11. Identifying well-bleached quartz using the different bleaching rates of quartz and feldspar luminescence signals

    DEFF Research Database (Denmark)

    Murray, A.S.; Thomsen, Kristina Jørkov; Masuda, N.;

    2012-01-01

    When dating older sedimentary deposits using quartz, there are no unambiguous methods for identifying the presence of incomplete bleaching. Current statistical analysis of dose distributions depends entirely on the assumption that incomplete bleaching and mixing are the main causes of any excess...... in relative bleaching rates of quartz optically stimulated luminescence (OSL) and feldspar luminescence stimulated at 50 °C by infrared light (IR50) and feldspar luminescence stimulated at 290 °C by infrared light after a stimulation at 50 °C (pIRIR290), and use recently deposited samples to determine...... that the large aliquot data are more likely to be correct. We conclude that a comparison of quartz and feldspar doses provides a useful independent method for identifying well-bleached quartz samples, and that it is unwise to apply statistical models to dose distributions without clear evidence for the physical...

  12. Optically stimulated luminescence dating of large storm events in Northern Scotland

    Science.gov (United States)

    Sommerville, A. A.; Hansom, J. D.; Sanderson, D. C. W.; Housley, R. A.

    2003-05-01

    Climate changes over the Holocene have directly impacted on both coastal processes and human use of coastal areas. This paper presents results from the dating of wind blown sand deposits collected from coastal and archaeological sites in Northern Scotland. Archaeological remains are frequently found interspersed with sand deposits and represent distinct periods of occupation of settlement sites within the local landscapes. In some cases storm events sufficiently inundate the sites with sand to result in periodic abandonment. Storm events can also have dramatic results on adjacent rock coastlines, with storm boulder ridges emplaced by large waves, burying sand deposits on cliff-top sites. Work has been undertaken using a quartz SAR protocol to date sand deposition at two archaeological sites in Orkney and a cliff-top site in Shetland. These dates provide chronological information, which help to construct regional chronologies of climatic instability and environmental change and allow the SAR-OSL method to be assessed as an accurate sediment dating tool in this context.

  13. Optically stimulated luminescence techniques in retrospective dosimetry using single grains of quartz extracted from unheated materials

    DEFF Research Database (Denmark)

    Thomsen, Kristina Jørkov

    dosimetry). Special attention has been paid to quartz extracted from unheated building materials such as concrete and mortar. The single-aliquot regeneration-dose (SAR) protocol has been used to determine absorbeddoses in small aliquots as well as single grains of quartz. It is shown that OSL measurements...... that the observed variability in the data is consistent with the sum (in quadrature) of a component,which depends on the number of photons detected from each grain, and a fixed component independent of light level. Dose depth profiles through laboratory irradiated concrete bricks have successfully been measured...

  14. Organ dose measurement using Optically Stimulated Luminescence Detector (OSLD) during CT examination

    Science.gov (United States)

    Yusuf, Muhammad; Alothmany, Nazeeh; Abdulrahman Kinsara, Abdulraheem

    2017-10-01

    This study provides detailed information regarding the imaging doses to patient radiosensitive organs from a kilovoltage computed tomography (CT) scan procedure using OSLD. The study reports discrepancies between the measured dose and the calculated dose from the ImPACT scan, as well as a comparison with the dose from a chest X-ray radiography procedure. OSLDs were inserted in several organs, including the brain, eyes, thyroid, lung, heart, spinal cord, breast, spleen, stomach, liver and ovaries, of the RANDO phantom. Standard clinical scanning protocols were used for each individual site, including the brain, thyroid, lung, breast, stomach, liver and ovaries. The measured absorbed doses were then compared with the simulated dose obtained from the ImPACT scan. Additionally, the equivalent doses for each organ were calculated and compared with the dose from a chest X-ray radiography procedure. Absorbed organ doses measured by OSLD in the RANDO phantom of up to 17 mGy depend on the organ scanned and the scanning protocols used. A maximum 9.82% difference was observed between the target organ dose measured by OSLD and the results from the ImPACT scan. The maximum equivalent organ dose measured during this experiment was equal to 99.899 times the equivalent dose from a chest X-ray radiography procedure. The discrepancies between the measured dose with the OSLD and the calculated dose from the ImPACT scan were within 10%. This report recommends the use of OSLD for measuring the absorbed organ dose during CT examination.

  15. Cat Island Terrestrial Core Optically Stimulated Luminescence (OSL) Data from field activity 10BIM03

    Data.gov (United States)

    U.S. Geological Survey, Department of the Interior — Scientists from the U.S. Geological Survey (USGS), St. Petersburg Coastal and Marine Science Center (SPCMSC), in collaboration with the U.S. Army Corps of Engineers...

  16. Cat Island Terrestrial Core Optically Stimulated Luminescence (OSL) Data from field activity 10BIM03

    Data.gov (United States)

    U.S. Geological Survey, Department of the Interior — Scientists from the U.S. Geological Survey (USGS), St. Petersburg Coastal and Marine Science Center (SPCMSC), in collaboration with the U.S. Army Corps of Engineers...

  17. Influence of surface coating on structural, morphological and optical properties of upconversion-luminescent LaF3:Yb/Er nanoparticles

    Science.gov (United States)

    Ansari, Anees A.; Yadav, Ranvijay; Rai, S. B.

    2016-07-01

    LaF3:Yb/Er (core), LaF3:Yb/Er@LaF3 (core/shell) and LaF3:Yb/Er@LaF3@SiO2 (core/shell/SiO2) nanoparticles were synthesized using citric-acid-based complexation process. X-ray diffraction, transmission electron microscopy, energy-dispersive X-ray analysis, optical absorption, band-gap energy ( E g), Fourier transform infrared and upconversion emission spectroscopy were employed to investigate the structural, morphological and optical properties of the synthesized core and core/shell/SiO2 nanoparticles. These core/shell/SiO2 nanoparticles can be well dispersed in aqueous solvents to form clear colloidal solution. The optical band-gap energy was decreased after shell formation due to increase in the crystalline size. The growth of an inactive and porous silica layers simultaneously on the surface of luminescent core-nanoparticles resulting an increase in average crystalline size of the nanoparticles. As-prepared inert shell-coated core/shell nanoparticles show intensive upconversion-luminescence as compared to the seed-core and silica-surface-modified core/shell/SiO2 nanoparticles because luminescent ions (Yb3+ and Er3+) ions located at the particle surface were protected from the non-radiative decay arising from surface dangling bonds and capping agent. However, our study revealed that there was only a slight reduction in upconversion efficiency for the silica-modified core/shell nanoparticles, indicating that upconversion properties of the upconversion nanoparticles are largely preserved in the core/shell/SiO2 nanoparticles. Absorption and upconversion-luminescence properties were examined for future application in the development of optical devices as well as optical bioprobes.

  18. Synthetic Aspects and Electro-Optical Properties of Fluorinated Arylenevinylenes for Luminescence and Photovoltaics

    Directory of Open Access Journals (Sweden)

    Antonio Cardone

    2013-03-01

    Full Text Available In this review, the main synthetic aspects and properties of fluorinated arylenevinylene compounds, both oligomers and polymers, are summarized and analyzed. Starting from vinyl organotin derivatives and aryl halides, the Stille cross-coupling reaction has been successfully applied as a versatile synthetic protocol to prepare a wide series of π-conjugated compounds, selectively fluorinated on the aromatic and/or vinylene units. The impact of fluoro-functionalization on properties, the solid state organization and intermolecular interactions of the synthesized compounds are discussed, also in comparison with the non-fluorinated counterparts. Luminescent and photovoltaic applications are also discussed, highlighting the role of fluorine on the performance of devices.

  19. Electrical stimulation vs. pulsed and continuous-wave optical stimulation of the rat prostate cavernous nerves, in vivo

    Science.gov (United States)

    Perkins, William C.; Lagoda, Gwen A.; Burnett, Arthur; Fried, Nathaniel M.

    2015-07-01

    Identification and preservation of the cavernous nerves (CNs) during prostate cancer surgery is critical for post-operative sexual function. Electrical nerve stimulation (ENS) mapping has previously been tested as an intraoperative tool for CN identification, but was found to be unreliable. ENS is limited by the need for electrode-tissue contact, poor spatial precision from electrical current spreading, and stimulation artifacts interfering with detection. Alternatively, optical nerve stimulation (ONS) provides noncontact stimulation, improved spatial selectivity, and elimination of stimulation artifacts. This study compares ENS to pulsed/CW ONS to explore the ONS mechanism. A total of eighty stimulations were performed in 5 rats, in vivo. ENS (4 V, 5 ms, 10 Hz) was compared to ONS using a pulsed diode laser nerve stimulator (1873 nm, 5 ms, 10 Hz) or CW diode laser nerve stimulator (1455 nm). Intracavernous pressure (ICP) response and nerve compound action potentials (nCAPs) were measured. All three stimulation modes (ENS, ONS-CW, ONS-P) produced comparable ICP magnitudes. However, ENS demonstrated more rapid ICP response times and well defined nCAPs compared to unmeasurable nCAPs for ONS. Further experiments measuring single action potentials during ENS and ONS are warranted to further understand differences in the ENS and ONS mechanisms.

  20. Electronic structure and optical properties of CdS{sub x}Se{sub 1−x} solid solution nanostructures from X-ray absorption near edge structure, X-ray excited optical luminescence, and density functional theory investigations

    Energy Technology Data Exchange (ETDEWEB)

    Murphy, M. W. [DESY (Deutsches Elektronen-Synchrotron), FS-PEX, Notkestrasse 85, 22607 Hamburg (Germany); Yiu, Y. M., E-mail: yyiu@uwo.ca; Sham, T. K. [Department of Chemistry, University of Western Ontario, London, ON N6A5B7 (Canada); Ward, M. J. [Cornell High Energy Synchrotron Source (CHESS), Cornell University, Ithaca, NY 14853 (United States); Liu, L. [Institute of Functional Nano and Soft Materials (FUNSOM) and Soochow University-Western University Center for Synchrotron Radiation Research, Soochow University, Suzhou, Jiangsu, 215123 (China); Hu, Y. [Canadian Light Source, University of Saskatchewan, Saskatoon, SK S7N2V3 (Canada); Zapien, J. A. [Center Of Super-Diamond and Advanced Films (COSDAF) and Department of Physics and Materials Science, City University of Hong Kong, Hong Kong SAR (China); Liu, Yingkai [Institute of Physics and Electronic Information, Yunnan Normal University, Kunming, Yunnan, 650500 (China)

    2014-11-21

    The electronic structure and optical properties of a series of iso-electronic and iso-structural CdS{sub x}Se{sub 1−x} solid solution nanostructures have been investigated using X-ray absorption near edge structure, extended X-ray absorption fine structure, and X-ray excited optical luminescence at various absorption edges of Cd, S, and Se. It is found that the system exhibits compositions, with variable local structure in-between that of CdS and CdSe accompanied by tunable optical band gap between that of CdS and CdSe. Theoretical calculation using density functional theory has been carried out to elucidate the observations. It is also found that luminescence induced by X-ray excitation shows new optical channels not observed previously with laser excitation. The implications of these observations are discussed.

  1. Constraining the age of rock art by dating a rockfall event using sediment and rock-surface luminescence dating techniques

    DEFF Research Database (Denmark)

    Chapot, Melissa; Sohbati, Reza; Murray, A.S.

    2012-01-01

    Optically stimulated luminescence (OSL) is used to determine the age of a rockfall event that removed part of the pictograph figures at the Great Gallery rock art panel in Canyonlands National Park, Utah, USA. Analyses from the outer millimeter of the buried surface of a rockfall boulder and quar...... rock art with a controversial and unknown origin.......Optically stimulated luminescence (OSL) is used to determine the age of a rockfall event that removed part of the pictograph figures at the Great Gallery rock art panel in Canyonlands National Park, Utah, USA. Analyses from the outer millimeter of the buried surface of a rockfall boulder and quartz...

  2. Probing Luminescence Dating Of Archaeologically Significant Carved Rock Types

    Science.gov (United States)

    Liritzis, Ioannis; Kitis, George; Galloway, Robert B.; Vafiadou, Asimina; Tsirliganis, Nestoras C.; Polymeris, George S.

    The thermoluminescence (TL) and Optically Stimulated Luminescence (OSL) dating of crystalline materials, first applied to calcites (limestone buildings), has been extended to carved megalithic monuments made of granites, basalt and sandstones derived from archaeological sites. Various applied criteria for potential dating included pulsed blue light stimulation, different preheating and solar simulator bleaching, while the single (and multiple) aliquot regeneration and additive dose procedures were used for equivalent dose determination. The decay curves of signal loss follow a power law, n-p; for blue stimulation the signal loss of quartz and feldspar is better approached by an exponential law, 1-aln(n).

  3. Luminescence property of volcanic quartz and the use of red isothermal TL for dating tephras

    DEFF Research Database (Denmark)

    Tsukamoto, S.; Murray, A.S.; Huot, S.

    2007-01-01

    An optically stimulated luminescence (OSL) age obtained from a Japanese tephra using quartz phenocrysts severely underestimated the known age. The characteristics of the OSL signals were investigated in order to understand the cause of the underestimation; the main OSL component of volcanic quartz...

  4. Re-evaluating luminescence burial doses and bleaching of fluvial deposits using Bayesian computational statistics

    NARCIS (Netherlands)

    Cunningham, A. C.; Wallinga, J.; Hobo, N.; Versendaal, A. J.; Makaske, B.; Middelkoop, H.

    2015-01-01

    The optically stimulated luminescence (OSL) signal from fluvial sediment often contains a remnant from the previous deposition cycle, leading to a partially bleached equivalent-dose distribution. Although identification of the burial dose is of primary concern, the degree of bleaching could potentia

  5. Re-evaluating luminescence burial doses and bleaching of fluvial deposits using Bayesian computational statistics.

    NARCIS (Netherlands)

    Cunningham, A.C.; Wallinga, J.; Versendaal, Alice; Makaske, A.; Middelkoop, H.; Hobo, N.

    2015-01-01

    The optically stimulated luminescence (OSL) signal from fluvial sediment often contains a remnant from the previous deposition cycle, leading to a partially bleached equivalent-dose distribution. Although identification of the burial dose is of primary concern, the degree of bleaching could potentia

  6. Bandwidth-tunable narrowband rectangular optical filter based on stimulated Brillouin scattering in optical fiber.

    Science.gov (United States)

    Wei, Wei; Yi, Lilin; Jaouën, Yves; Hu, Weisheng

    2014-09-22

    We propose a rectangular optical filter based on stimulated Brillouin scattering (SBS) in optical fiber with bandwidth tuning from 50 MHz to 4 GHz at less than 15-MHz resolution. The rectangular shape of the filter is precisely achieved utilizing digital feedback control of the comb-like pump spectral lines. The passband ripple is suppressed to ~1 dB by mitigating the nonlinearity influences of the comb-like pump lines generated in electrical and optical components and fibers. Moreover a fiber with a single Brillouin peak is employed to further reduce the in-band ripple and the out-of-band SBS gain at the same time. Finally, we analyze the noise performance of the filter at different bandwidth cases and demonstrate the system performance of the proposed filter with 2.1-GHz bandwidth and 19-dB gain by amplifying a 2-GHz orthogonal frequency-division-multiplexing (OFDM) signal with quadrature-phase-shift-keying (QPSK) and 16-quadrature-amplitude-modulation (16-QAM) on each subscriber.

  7. New luminescence measurement facilities in retrospective dosimetry

    DEFF Research Database (Denmark)

    Lapp, Torben; Jain, Mayank; Thomsen, Kristina Jørkov

    2012-01-01

    thermoelectrically cooled NIR sensitive PMT (detection window peak at 855 nm, FWHM 27 nm). Software and electronics have been modified to allow standard TL and OSL measurements in the same sequence as RL measurements. Together with a new bleaching source based on a high-power UV LED (395 nm; 700 mW/cm2......This paper gives a review of recent developments in luminescence measurement facilities on the Risø TL/OSL reader including radio-luminescence (RL), exo-electron and violet stimulation attachments, and a method for characterising and if necessary correcting for beta irradiation source non......-uniformity.We first describe improvements to the existing RL option to allow near infra-red detection (NIR) during irradiation by the built-in 90Sr/90Y beta source. The RL optical signal is collected by a liquid light guide through an F34-901 interference filter and detection is based on a dedicated...

  8. In-body optical stimulation formed connective tissue vascular grafts, "biotubes," with many capillaries and elastic fibers.

    Science.gov (United States)

    Oie, Tomonori; Yamanami, Masashi; Ishibashi-Ueda, Hatsue; Kanda, Keiichi; Yaku, Hitoshi; Nakayama, Yasuhide

    2010-12-01

    The autologous biotube, developed by using in-body tissue architecture technology, is one of the most promising small-diameter vascular grafts in regenerative medicine. The walls of the biotubes obtained by a traditional silicone mold-based method were very thin, and this is still the primary obstacle while handling anastomosis, even though these biotubes have adequate pressure resistance ability. This pilot study showed the effect of optical stimulation of subcutaneous tissue formation in the body during the preparation of the biotubes. A blue light-emitting diode (LED) was embedded into a silicone rod as a mold. The biotube was prepared by placing the luminescent molds into the dorsal subcutaneous pouches of a pair of beagles (each weighing ~10 kg) for 2 weeks under photoirradiation. The wall thickness of the obtained biotubes was 506.9 ± 185.7 μm, which was remarkably more than that of the previous biotubes prepared by 2 months of embedding similarly in beagles' subcutaneous pouches (thickness, 77.2 ± 14.8 μm). Many capillaries with smooth muscle cells were infiltrated into the wall and concentrated in the internal layer. Interestingly, the formation of elastic fibers had already started along with collagen fibers, mostly with a regular circumferential orientation. The short-term in-body optical stimulation resulted in the rapid formation of a biotube. These phenomena will allow easy surgical handling and may induce vascular maturation in histology during the acute phase after implantation.

  9. Optical dating of single sand-sized grains of quartz: Sources of variability

    DEFF Research Database (Denmark)

    Duller, G.A.T.; Bøtter-Jensen, L.; Murray, A.S.

    2000-01-01

    Optically stimulated luminescence (OSL) measurements have been made of over 3000 sand-sized grains of quartz. Analysis at this scale highlights the variability in the luminescence sensitivity and the dose saturation characteristics of individual quartz grains. Using a new instrument capable of me...... intensity, dose saturation characteristics and instrument uncertainty in equivalent dose calculation. (C) 2000 Elsevier Science Ltd. All rights reserved....

  10. Optical fibre luminescence sensor for real-time LDR brachytherapy dosimetry

    Science.gov (United States)

    Woulfe, P.; Sullivan, F. J.; O'Keeffe, S.

    2016-05-01

    An optical fibre sensor for monitoring low dose radiation is presented. The sensor is based on a scintillation material embedded within the optical fibre core, which emits visible light when exposed to low level ionising radiation. The incident level of ionising radiation can be determined by analysing the optical emission. An optical fibre sensor is presented, based on radioluminescence whereby radiation sensitive scintillation material, terbium doped gadolinium oxysulphide (Gd2O2S:Tb), is embedded in a cavity of 250μm of a 500μm plastic optical fibre. The sensor is designed for in-vivo monitoring of the radiation dose during radio-active seed implantation for brachytherapy, in prostate cancer treatment, providing oncologists with real-time information of the radiation dose to the target area and/or nearby critical structures. The radiation from the brachytherapy seeds causes emission of visible light from the scintillation material through the process of radioluminescence, which penetrates the fibre, propagating along the optical fibre for remote detection using a multi-pixel photon counter. The sensor demonstrates a high sensitivity to Iodine-125, the radioactive source most commonly used in brachytherapy for treating prostate cancer.

  11. All-optical control of neuronal function via optical delivery of light-sensitive proteins and optogenetic stimulation

    Science.gov (United States)

    Villalobos, Alex; Gu, Ling; Mohanty, Samarendra

    2012-02-01

    While pulsed laser beams have been used for stimulation of neurons, cellular specificity during optical stimulation is achieved by photo-sensitization of genetically-targeted cells by optogenetic means. However, till date, the process of optogenetic-sensitization primarily involves use of viral vectors. In rare occasions, electroporation has been used. Here, we report an all-optical method in which pulsed laser beam is used for delivery of genes, encoding optogenetic probes, to spatially-targeted cells, followed by optogenetic stimulation and optical detection of the activation process. Use of laser microbeam enabled highly precise spatially-patterned delivery of optogenes, as confirmed by expression of conjugated fluorescent protein. Light-activation of opsin-expressing cells was confirmed by calcium-imaging. The laser-assisted expression of optogenetic probes in spatially-targeted regions in combination with light-assisted activation and optical detection of neural activity will help in better understanding of the neuronal circuitry.

  12. Luminescence dosimetry: recent developments in theory and applications

    Energy Technology Data Exchange (ETDEWEB)

    McKeever, S.W.S. [Department of Physics, Oklahoma State University, Stillwater, OK 74078-3072 (United States)

    2000-07-01

    Thermally and optically stimulated luminescence have been used in applications in solid state physics, radiation dosimetry and geological dating for several decades. This paper gives a generalized description of these methods in terms of non-equilibrium thermodynamics and in doing so highlights similarities and differences between the methods. Recent advances in both the theory and application of the techniques are highlighted with numerous specific examples. (Author)

  13. A concise synthesis of optically active solanacol, the germination stimulant for seeds of root parasitic weeds.

    Science.gov (United States)

    Kumagai, Hiroshi; Fujiwara, Mami; Kuse, Masaki; Takikawa, Hirosato

    2015-01-01

    Solanacol, isolated from tobacco (Nicotiana tabacum L.), is a germination stimulant for seeds of root parasitic weeds. A concise synthesis of optically active solanacol has been achieved by employing enzymatic resolution as a key step.

  14. Nanophosphor aluminum oxide: Luminescence response of a potential dosimetric material

    Energy Technology Data Exchange (ETDEWEB)

    Blair, Michael W., E-mail: mblair@lanl.go [Los Alamos National Laboratory, Los Alamos, NM (United States); Jacobsohn, Luiz G. [Center for Optical Materials Science and Engineering Technologies, and the School of Materials Science and Engineering, Clemson University, Anderson, SC 29625 (United States); Tornga, Stephanie C. [Los Alamos National Laboratory, Los Alamos, NM (United States); Ugurlu, Ozan [Characterization Facility, Institute of Technology, University of Minnesota, Minneapolis, MN 55455 (United States); Bennett, Bryan L. [Los Alamos National Laboratory, Los Alamos, NM (United States); Yukihara, Eduardo G. [Department of Physics, Oklahoma State University, Stillwater, OK (United States); Muenchausen, Ross E. [Los Alamos National Laboratory, Los Alamos, NM (United States)

    2010-05-15

    This work reports on the investigation of the radiation dosimetry properties of Al{sub 2}O{sub 3} nanopowders. Samples were produced by solution combustion synthesis using three different organic fuels to check for the effect of synthesis conditions on the properties of interest. Luminescence characteristics were studied by thermoluminescence and optically stimulated luminescence (OSL) techniques. We found that samples produced using urea have characteristics similar to bulk Al{sub 2}O{sub 3}:C and may be suitable for personal dosimetry, while samples produced using glycine and hexamethylenetetramine (HMT) may be more suitable for applications where fast OSL decay is advantageous. While these results are promising and warrant further investigation, much has to be done to overcome the greatly decreased luminescence intensity of the nanomaterials as compared to bulk Al{sub 2}O{sub 3}:C.

  15. Luminescence Dating of Sediments: An Increasingly Diverse Family of Methods and Range of Applications

    Science.gov (United States)

    Roberts, H. M.

    2015-12-01

    In recent years, the term 'luminescence dating' has expanded its meaning such that today it encompasses a range of luminescence dating methods and materials. Whilst the fundamental principles that underlie these different dating methods are essentially the same, namely that the event typically being recorded is the last exposure of the material to light or to heat, the various luminescence dating techniques do differ in their suitability in different situations. Today, in the field of luminescence dating of sediments, there are a number of minerals that can be used for dating (quartz and feldspar being the most commonly used), and for each mineral it is possible to obtain a number of different luminescence signals (some obtained using optical stimulation, and some obtained by heating). These different luminescence signals may build-up and deplete in the natural environment at different rates from each other, and can span quite different time ranges. Additionally, the scale of analysis used in luminescence dating can now be varied (ranging from single sand-sized grains to multiple grains), as can the size range of the materials used for dating (ranging from fine-silt, coarse-silt, and sand-sized grains, through to large clasts and rock surfaces). Having such flexibility in the range of minerals, luminescence signals, grain sizes, and the scales of analysis available for dating, means that it is now possible to optimise the materials and methods selected for dating in any particular study in response to the precise scientific question to be addressed, the time-range of interest, and the likely mechanisms of re-setting of the luminescence signal in the context that is to be dated. In this paper, the flexibility offered by the growing family of luminescence techniques will be outlined by considering some of the different minerals, luminescence signals, and dramatically different timescales (tens of years to millions of years) potentially available for sediment dating

  16. Synthesis, characterization, photoluminescence and thermally stimulated luminescence investigations of orange red-emitting Sm3+-doped ZnAl2O4 phosphor

    Indian Academy of Sciences (India)

    Mithlesh Kumar; V Natarajan; S V Godbole

    2014-10-01

    Sm3+-doped ZnAl2O4 phosphor was synthesized by citrate sol–gel method and characterized using X-ray diffraction and scanning electron microscopy to identify the crystalline phase and determine the particle size. Photoluminescence (PL) studies on the sample showed emission peaks at 563, 601, 646 and 707 nm with ex = 230 nm corresponding to the ${}^{4}G_{5/2} \\rightarrow {}^{6}H_{5/2}, {}^{4}G_{5/2} \\rightarrow {}^{6}H_{7/2}, {}^{4}G_{5/2} \\rightarrow {}^{6}H_{9/2}$ and ${}^{4}G_{5/2} \\rightarrow {}^{6}H_{11/2}$ transitions, respectively, due to Sm3+ ions. PL lifetime decay studies confirmed that Sm3+ ions partly entered into the lattice by replacing Al3+ ions and remaining located at the surface of ZnAl2O4 host matrix. Thermally stimulated luminescence (TSL) studies of -irradiated Sm3+-doped ZnAl2O4 sample showed two glow peaks at 440 and 495 K, the former being most intense than the latter. The trap parameters were determined using different heating rate methods. Spectral characteristics of the TSL glow showed emission around 565, 599 and 641 nm, indicating the role of Sm3+ ion as the luminescent centre. A probable mechanism for the prominent TSL glow peak, observed at 440 K, was proposed. CIE chromaticity coordinates for the system was evaluated, which suggested that Sm3+-doped ZnAl2O4 could be employed as a potential orange red-emitting phosphor.

  17. Syntheses, structural characterization, luminescence and optical studies of Ni(II) and Zn(II) complexes containing salophen ligand

    Science.gov (United States)

    More, M. S.; Pawal, S. B.; Lolage, S. R.; Chavan, S. S.

    2017-01-01

    Some Ni(II) (1a-d) and Zn(II) (2a-d) salophen complexes were prepared by the treatment of 5-bromosalicylaldehyde, 5-(trimethylsilylethynyl)salicylaldehyde, 5-(4-nitrophenyl)ethynylsalicylaldehyde or 5-(4-methoxyphenyl)ethynylsalicylaldehyde with nickel acetate or zinc acetate followed by addition of 2,3-diamino-5-bromopyridine. All complexes were characterized by elemental analyses, IR, 1H NMR and mass spectral studies. X-ray powder diffraction of representative complexes 1c and 2b and SEM studies of 1b and 2d are used to elucidate the crystal structure and morphology of the complexes. The electrochemical behavior reveals that the redox responses of Ni(II) complexes shifted to more negative potential in order to increase the π-conjugation in the complexes. Room temperature luminescence is observed for all complexes corresponding to π→π* ILCT transition with some MLCT character in DMF and is finely tuned by the degree of extended π-conjugation and variation of the substituent group with different electronic effects in the complexes. The second harmonic generation (SHG) efficiency of the complexes was screened by Kurtz-powder technique indicating that all complexes possesses promising potential for the application as a useful nonlinear optical material.

  18. Optical thermometry based on luminescence behavior of Dy{sup 3+}-doped transparent LaF{sub 3} glass ceramics

    Energy Technology Data Exchange (ETDEWEB)

    Bu, Y.Y. [Nanjing University of Posts and Telecommunications, College of Electronic Science and Engineering, Nanjing (China); Nanjing University of Posts and Telecommunications, College of Science, Nanjing (China); Cheng, S.J.; Wang, X.F. [Nanjing University of Posts and Telecommunications, College of Electronic Science and Engineering, Nanjing (China); Key Laboratory of Radio Frequency and Micro-Nano Electronics of Jiangsu Province, Nanjing, Jiangsu (China); Yan, X.H. [Nanjing University of Posts and Telecommunications, College of Electronic Science and Engineering, Nanjing (China); Key Laboratory of Radio Frequency and Micro-Nano Electronics of Jiangsu Province, Nanjing, Jiangsu (China); Nanjing University of Aeronautics and Astronautics, College of Science, Nanjing (China)

    2015-11-15

    Dy{sup 3+}-doped transparent LaF{sub 3} glass ceramics were fabricated, and its structures of resulting glass ceramics are studied by the X-ray diffraction and transmission electron microscopy. Optical temperature sensing of the resulting glass ceramics in the temperature range from 298 to 523 K is studied based on the down-conversion luminescence of Dy{sup 3+} ion. By using fluorescence intensity ratio method, the {sup 4}I{sub 15/2} and {sup 4}F{sub 9/2} of Dy{sup 3+} ions are verified as thermally coupled levels. A minimum S{sub R} = 1.16 x 10{sup -4} K{sup -1} is obtained at T = 294 K. By doping Eu{sup 3+} ion, the overall emission color of Eu{sup 3+}-Dy{sup 3+} co-doped transparent glass ceramics can be tuned from white to yellow with the temperature increase through energy transfer between Eu{sup 3+} and Dy{sup 3+}. Additionally, the thermal stability of the Dy{sup 3+} single-doped transparent glass ceramics becomes higher after doping Eu{sup 3+} ion. (orig.)

  19. Measurement of optically and thermally stimulated electron emission from natural minerals

    DEFF Research Database (Denmark)

    Ankjærgaard, C.; Murray, A.S.; Denby, P.M.

    2006-01-01

    Electron emission during thermal stimulation has been studied before in some detail, but there has been less work on the optically stimulated signal, especially in natural dosimeters. We report on measurements obtained using a windowless pancake Geiger-Nifiller electron detector attachment...

  20. Optical lattice-like cladding waveguides by direct laser writing: fabrication, luminescence, and lasing.

    Science.gov (United States)

    Nie, Weijie; He, Ruiyun; Cheng, Chen; Rocha, Uéslen; Rodríguez Vázquez de Aldana, Javier; Jaque, Daniel; Chen, Feng

    2016-05-15

    We report on the fabrication of optical lattice-like waveguide structures in an Nd:YAP laser crystal by using direct femtosecond laser writing. With periodically arrayed laser-induced tracks, the waveguiding cores can be located in either the regions between the neighbored tracks or the central zone surrounded by a number of tracks as outer cladding. The polarization of the femtosecond laser pulses for the inscription has been found to play a critical role in the anisotropic guiding behaviors of the structures. The confocal photoluminescence investigations reveal different stress-induced modifications of the structures inscribed by different polarization of the femtosecond laser beam, which are considered to be responsible for the refractive index changes of the structures. Under optical pump at 808 nm, efficient waveguide lasing at ∼1  μm wavelength has been realized from the optical lattice-like structure, which exhibits potential applications as novel miniature light sources.

  1. Time structure measurement of the storage ring with the time-resolved X-ray excited optical luminescence method at SSRF

    CERN Document Server

    Zhaohong, Zhang; Song, Xue; Lifang, Zheng

    2014-01-01

    Measuring the time structure of the storage ring on the sample spot inside the experimental hutch is a foundational step during the time-resolved experiments using the pulsed synchrotron X-rays with the time structure defined by the storage ring. In this work, the method of time-resolved X-ray excited optical luminescence was designed and implemented to do the measurement. This method is based on the principle of time-correlated single photon counting techniques. The measurement system consists of a spectrometer with a detector of photomultiplier tube, a timing system, a set of Nuclear Instrument Modules and a luminescent material of Zinc Oxide. The measurement was performed on the X-ray absorbed fine structure spectrum beamline at Shanghai Synchrotron Radiation Facility. The results show that this system can be used to measure the time structure of the storage ring with a precision of less than 1 ns.

  2. Complexation of lactate with neodymium(III) and europium(III) at variable temperatures: studies by potentiometry, microcalorimetry, optical absorption, and luminescence spectroscopy.

    Science.gov (United States)

    Tian, Guoxin; Martin, Leigh R; Rao, Linfeng

    2010-11-15

    The complexation of neodymium(III) and europium(III) with lactate was studied at variable temperatures by potentiometry, absorption spectrophotometry, luminescence spectroscopy, and microcalorimetry. The stability constants of three successive lactate complexes (ML(2+), ML(2)(+), and ML(3)(aq), where M stands for Nd and Eu and L stands for lactate) at 10, 25, 40, 55, and 70 °C were determined. The enthalpies of complexation at 25 °C were determined by microcalorimetry. Thermodynamic data show that the complexation of trivalent lanthanides (Nd(3+) and Eu(3+)) with lactate is exothermic and the complexation becomes weaker at higher temperatures. Results from optical absorption and luminescence spectroscopy suggest that the complexes are inner-sphere chelate complexes in which the protonated α-hydroxyl group of lactate participates in the complexation.

  3. Luminescence nanothermometry

    Science.gov (United States)

    Jaque, Daniel; Vetrone, Fiorenzo

    2012-07-01

    The current status of luminescence nanothermometry is reviewed in detail. Based on the main parameters of luminescence including intensity, bandwidth, bandshape, polarization, spectral shift and lifetime, we initially describe and compare the different classes of luminescence nanothermometry. Subsequently, the various luminescent materials used in each case are discussed and the mechanisms at the root of the luminescence thermal sensitivity are described. The most important results obtained in each case are summarized and the advantages and disadvantages of these approaches are discussed.The current status of luminescence nanothermometry is reviewed in detail. Based on the main parameters of luminescence including intensity, bandwidth, bandshape, polarization, spectral shift and lifetime, we initially describe and compare the different classes of luminescence nanothermometry. Subsequently, the various luminescent materials used in each case are discussed and the mechanisms at the root of the luminescence thermal sensitivity are described. The most important results obtained in each case are summarized and the advantages and disadvantages of these approaches are discussed. This work was supported by the Universidad Autónoma de Madrid and Comunidad Autónoma de Madrid (Project S2009/MAT-1756), by the Spanish Ministerio de Educacion y Ciencia (MAT2010-16161) and by Caja Madrid Foundation.

  4. Combining infrared- and green-laser stimulation sources in single-grain luminescence measurements of feldspar and quartz

    DEFF Research Database (Denmark)

    Duller, G.A.T.; Bøtter-Jensen, L.; Murray, A.S.

    2003-01-01

    on grains from two feldspar samples are described. These show that the ratio of the OSL signal under green and IR stimulation is similar for all the feldspar grains. As expected, the ratio for quartz grains is very different, with a much weaker signal when using IR stimulation. For the two feldspars......, the distribution of OSL between the grains and the saturation of the dose response curve shows much less variability than is typically seen for quartz grains. (C) 2003 Elsevier Science Ltd. All rights reserved....

  5. Coherent control of the optical absorption in a plasmonic lattice coupled to a luminescent layer

    CERN Document Server

    Pirruccio, Giuseppe; Rodriguez, Said Rahimzadeh-Kalaleh; Rivas, Jaime Gomez

    2016-01-01

    We experimentally demonstrate the coherent control, i.e., phase-dependent enhancement and suppression, of the optical absorption in an array of metallic nanoantennas covered by a thin lu- minescent layer. The coherent control is achieved by using two collinear, counter-propagating and phase-controlled incident waves with wavelength matching the absorption spectrum of dye molecules coupled to the array. Symmetry arguments shed light on the relation between the relative phase of the incident waves and the excitation efficiency of the optical resonances of the system. This coherent control is associated with a phase-dependent distribution of the electromagnetic near-fields in the structure which enables a significant reduction of the unwanted dissipation in the metallic structures.

  6. Implantable optogenetic device with CMOS IC technology for simultaneous optical measurement and stimulation

    Science.gov (United States)

    Haruta, Makito; Kamiyama, Naoya; Nakajima, Shun; Motoyama, Mayumi; Kawahara, Mamiko; Ohta, Yasumi; Yamasaki, Atsushi; Takehara, Hiroaki; Noda, Toshihiko; Sasagawa, Kiyotaka; Ishikawa, Yasuyuki; Tokuda, Takashi; Hashimoto, Hitoshi; Ohta, Jun

    2017-05-01

    In this study, we have developed an implantable optogenetic device that can measure and stimulate neurons by an optical method based on CMOS IC technology. The device consist of a blue LED array for optically patterned stimulation, a CMOS image sensor for acquiring brain surface image, and eight green LEDs surrounding the CMOS image sensor for illumination. The blue LED array is placed on the CMOS image sensor. We implanted the device in the brain of a genetically modified mouse and successfully demonstrated the stimulation of neurons optically and simultaneously acquire intrinsic optical images of the brain surface using the image sensor. The integrated device can be used for simultaneously measuring and controlling neuronal activities in a living animal, which is important for the artificial control of brain functions.

  7. Highly luminescent mono- and multilayers of immobilized CdTe nanocrystals: controlling optical properties through post chemical surface modification.

    Science.gov (United States)

    Tsuruoka, Takaaki; Takahashi, Rena; Nakamura, Toshihiro; Fujii, Minoru; Akamatsu, Kensuke; Nawafune, Hidemi

    2008-04-14

    The significant fluorescence enhancement of immobilized CdTe nanocrystals through chemical surface modifications is described, enabling us to fabricate stable, highly luminescent thin films and patterns of nanocrystal mono- and mutilayers.

  8. Luminescence dating at Rose cottage cave: a progress report

    CSIR Research Space (South Africa)

    Woodborne, S

    1997-10-01

    Full Text Available Deal with infrared-stimulated luminescence and thermoluminescence dates from Rose Cottage Cave in South Africa. Discrepancy between luminescence and radiocarbon dates; Concentration of radioactive elements in sediments before and after leaching...

  9. Fluorinated Poly(p-phenylenevinylenes: Synthesis and Optical Properties of an Intriguing Class of Luminescent Polymers

    Directory of Open Access Journals (Sweden)

    Gianluca M. Farinola

    2010-05-01

    Full Text Available This review is an overview of our previous work on the synthesis and properties of poly(p-phenylenevinylenes (PPVs selectively fluorinated in different positions of the conjugated backbone. Both the synthetic challenges and the effects of functionalization with fluorine atoms on the optical behavior are discussed, highlighting the peculiarities and the interest of this class of conjugated polymers. A general polymerization protocol for PPVs, that is based on the Pd-catalyzed Stille cross-coupling reaction of bis-stannylated vinylene monomers with aromatic bis-halides, has been successfully extended to the synthesis of selectively fluorinated poly(p-phenylenevinylenes. The properties of a series of these PPVs differing in the number and positions of the fluorine atoms on the conjugated backbone have been studied, even in comparison with the non-fluorinated counterparts. The intriguing optical features of the resulting materials are discussed considering not only the role of the electronic and steric effects induced by the fluorine substituents, but also the impact of the fluorination on the solid state organization and intermolecular interactions.

  10. Photoinduced (WO4)3--La3+ center in PbWO4: Electron spin resonance and thermally stimulated luminescence study

    Science.gov (United States)

    Laguta, V. V.; Martini, M.; Meinardi, F.; Vedda, A.; Hofstaetter, A.; Meyer, B. K.; Nikl, M.; Mihóková, E.; Rosa, J.; Usuki, Y.

    2000-10-01

    The localization of electrons at W6+ sites perturbed by lanthanum in PbWO4 is studied by electron spin resonance (ESR) and thermally stimulated luminescence (TSL) measurements. The (WO4)3--La3+ centers are created at the W6+ sites close to La3+ in two different ways: (i) direct trapping of electrons from the conduction band under ultraviolet or x-ray irradiation at T=60 K (ii) retrapping of electrons freed from unperturbed (WO4)3- centers after irradiation at Teffect, which gives rise to a rhombic distortion of (WO4)3- complex. At T~95-98 K the (WO4)3--La3+ centers are thermally ionized giving rise to a TSL glow peak due to the recombination of detrapped electrons with localized holes. The emission spectrum of the TSL features one band peaking at 2.8 eV. The temperature dependence of both TSL and ESR intensity is analyzed in the frame of a general order recombination model. The thermal ionization energy of (WO4)3--La3+ centers has been calculated to be approximately 0.27 eV.

  11. Spatial and temporal variability in response to hybrid electro-optical stimulation

    Science.gov (United States)

    Duke, Austin R.; Lu, Hui; Jenkins, Michael W.; Chiel, Hillel J.; Jansen, E. Duco

    2012-06-01

    Hybrid electro-optical neural stimulation is a novel paradigm combining the advantages of optical and electrical stimulation techniques while reducing their respective limitations. However, in order to fulfill its promise, this technique requires reduced variability and improved reproducibility. Here we used a comparative physiological approach to aid the further development of this technique by identifying the spatial and temporal factors characteristic of hybrid stimulation that may contribute to experimental variability and/or a lack of reproducibility. Using transient pulses of infrared light delivered simultaneously with a bipolar electrical stimulus in either the marine mollusk Aplysia californica buccal nerve or the rat sciatic nerve, we determined the existence of a finite region of excitability with size altered by the strength of the optical stimulus and recruitment dictated by the polarity of the electrical stimulus. Hybrid stimulation radiant exposures yielding 50% probability of firing (RE50) were shown to be negatively correlated with the underlying changes in electrical stimulation threshold over time. In Aplysia, but not in the rat sciatic nerve, increasing optical radiant exposures (J cm-2) beyond the RE50 ultimately resulted in inhibition of evoked potentials. Accounting for the sources of variability identified in this study increased the reproducibility of stimulation from 35% to 93% in Aplysia and 23% to 76% in the rat with reduced variability.

  12. Light amplification by stimulated emission from an optically pumped molecular junction in a scanning tunneling microscope

    CERN Document Server

    Braun, K; Wang, X; Adler, H; Peisert, H; Chasse, T; Zhang, D; Meixner, A J

    2013-01-01

    Here, we introduce and experimentally demonstrate optical amplification and stimulated emission from a single optically pumped molecular tunneling junction of a scanning tunneling microscope. The gap between a sharp gold tip and a flat gold substrate covered with a self-assembled monolayer of 5-chloro-2-mercaptobenzothiazole molecules forms an extremely small optical gain medium. When electrons tunnel from the molecules highest occupied molecular orbital to the tip, holes are left behind. These can be repopulated by hot electrons induced by the laser-driven plasmon oscillation on the metal surfaces enclosing the cavity. Solving the laser-rate equations for this system shows that the repopulation process can be efficiently stimulated by the gap modes near field, TERS scattering from neighboring molecules acting as an optical seed. Our results demonstrate how optical enhancement inside the plasmonic cavity can be further increased by a stronger localization via tunneling through molecules. We anticipate that st...

  13. Optical and radiation-induced luminescence properties of Ce-doped magnesium aluminoborate glasses

    Science.gov (United States)

    Nakauchi, Daisuke; Okada, Go; Fujimoto, Yutaka; Kawano, Naoki; Kawaguchi, Noriaki; Yanagida, Takayuki

    2017-10-01

    Optical, radioluminescence (RL) and thermoluminescence (TL) properties of magnesium aluminoborate glasses were evaluated. The samples were synthesized by the conventional melt-quenching technique using an alumina crucible under ambient atmosphere. After polishing, all the samples show good transparency. In photoluminescence, RL and TL, the emission is predominantly due to the 5d-4f transitions of Ce3+ appearing as a broad feature peaking around 300-500 nm, and the decay time constants are affected by concentration quenching but on the typical range for the 5d-4f transitions of Ce3+. TL glow curves are characterized as a single but broad glow peak over 100-300 °C, and the TL intensity monotonically increases with the X-ray dose irradiated over 1-10000 mGy.

  14. Luminescent, magnetic and optical properties of ZnO-ZnS nanocomposites

    Science.gov (United States)

    Raleaooa, Pule V.; Roodt, Andreas; Mhlongo, Gugu G.; Motaung, David E.; Kroon, Robin E.; Ntwaeaborwa, Odireleng M.

    2017-02-01

    The structure, particle morphology, optical and magnetic properties of ZnO, ZnS and ZnO-ZnS nanoparticles prepared by the sol-gel method are reported. ZnO and ZnS were combined at room temperature by an ex situ synthetic route to prepare ZnO-ZnS nanocomposites. The nanocomposites exhibited particle morphology different from that of ZnO and ZnS nanoparticles. The ZnO and ZnS nanoparticles exhibited quantum confinement as inferred from the widening of their respective bandgap energies. The electron paramagnetic resonance data provided evidence for the existence of magnetic clusters near the surface, electron to nuclei interactions and defect states. The ZnO-ZnS nanocomposites exhibited tunable emission that was dependent on the ratio of ZnO to ZnS. These composites were evaluated for application in different types of light emitting devices.

  15. Luminescent, magnetic and optical properties of ZnO-ZnS nanocomposites

    Energy Technology Data Exchange (ETDEWEB)

    Raleaooa, Pule V. [Department of Physics, University of the Free State, ZA 9300 Bloemfontein (South Africa); Department of Chemistry, University of the Free State, ZA 9300 (South Africa); Roodt, Andreas [Department of Chemistry, University of the Free State, ZA 9300 (South Africa); Mhlongo, Gugu G.; Motaung, David E. [DST/CSIR Nanotechnology Innovation Center, National Center for Nano-Structured Materials, Council for Scientific and Industrial Research, P.O. Box 395, ZA 0001 Pretoria (South Africa); Kroon, Robin E. [Department of Physics, University of the Free State, ZA 9300 Bloemfontein (South Africa); Ntwaeaborwa, Odireleng M., E-mail: ntwaeab@gmail.com [School of Physics, University of the Witwatersrand, Private Bag 3, Wits, ZA 2050 (South Africa)

    2017-02-15

    The structure, particle morphology, optical and magnetic properties of ZnO, ZnS and ZnO-ZnS nanoparticles prepared by the sol-gel method are reported. ZnO and ZnS were combined at room temperature by an ex situ synthetic route to prepare ZnO-ZnS nanocomposites. The nanocomposites exhibited particle morphology different from that of ZnO and ZnS nanoparticles. The ZnO and ZnS nanoparticles exhibited quantum confinement as inferred from the widening of their respective bandgap energies. The electron paramagnetic resonance data provided evidence for the existence of magnetic clusters near the surface, electron to nuclei interactions and defect states. The ZnO-ZnS nanocomposites exhibited tunable emission that was dependent on the ratio of ZnO to ZnS. These composites were evaluated for application in different types of light emitting devices.

  16. X-ray-sensitive storage phosphors with the optically stable luminescent centres

    CERN Document Server

    Gorin, G B; Zvezdova, N P; Kochubey, D I; Sedova, Y G; Kochubey, D I; Kulipanov, G N; Lyakh, V V; Pindyurin, V F

    2000-01-01

    NaCl, KCl, KBr and LiF crystals doped by In, Tl, Ni, Pd and Ca were investigated as X-ray-sensitive materials. Influence of the way of doping of an impurity and growing of a crystal on such parameters of a material as: sensitivity to ionising radiation; radiative, optical and thermal stability of the image, obtained after an irradiation is investigated. As a result of the work, media for recording of the X-ray images are developed. These allow to reproduce the images in a mode of a photoluminescence. Spatial resolution and the dynamic range of registration of the developed materials concede to similar parameters of commercial storage luminophores like 'Image Plates' based on BaFBr : La. At the same time, as distinct from 'Image Plates', the developed radiophotoluminophores allow a long storage and multiple readout of the information recorded.

  17. Study of optical and luminescence properties of silicon — semiconducting silicide — silicon multilayer nanostructures

    Science.gov (United States)

    Galkin, N. G.; Galkin, K. N.; Dotsenko, , S. A.; Goroshko, D. L.; Shevlyagin, A. V.; Chusovitin, E. A.; Chernev, I. M.

    2016-12-01

    By method of in situ differential spectroscopy it was established that at the formation of monolayer Fe, Cr, Ca, Mg silicide and Mg stannide islands on the atomically clean silicon surface an appearance of loss peaks characteristic for these materials in the energy range of 1.1-2.6 eV is observed. An optimization of growth processes permit to grow monolithic double nanoheterostructures (DNHS) with embedded Fe, Cr and Ca nanocrystals, and also polycrystalline DNHS with NC of Mg silicide and Mg stannide and Ca disilicide. By methods of optical spectroscopy and Raman spectroscopy it was shown that embedded NC form intensive peaks in the reflectance spectra at energies up to 2.5 eV and Raman peaks. In DNS with β-FeSi2 NC a photoluminescence and electroluminescence at room temperature were firstly observed.

  18. Luminescence quartz dating of lime mortars. A first research approach.

    Science.gov (United States)

    Zacharias, N; Mauz, B; Michael, C T

    2002-01-01

    Lime mortars mixed with sand are well suited for connecting structural materials, like stones and bricks, due to the mechanical properties this material exhibits. Their extensive use in architectural and decorative works during the last 4000 years motivated the introduction of the 'Luminescence clock' for age determination of mortars. The same principles as for quartz optically stimulated luminescence (OSL) dating of sediments were applied for age estimation of a mortar fragment removed from a Byzantine church monument dated by archaeological means to 1050-1100 years ago (the first half of the 10th century). The OSL from the quartz was monitored under blue light stimulation and UV detection, using a single-aliquot-regenerative-dose protocol. The quartz-OSL dating of the mortar resulted in 870 +/- 230 a. TL polymineral fine grain dating was also performed on a brick fragment which was connected to the mortar, resulting in a TL age of 1095 +/- 190 a.

  19. Time structure measurement of the storage ring with the time-resolved X-ray excited optical luminescence method at SSRF

    OpenAIRE

    Zhaohong, Zhang; Zheng, Jiang; Song, Xue; Lifang, Zheng

    2014-01-01

    Measuring the time structure of the storage ring on the sample spot inside the experimental hutch is a foundational step during the time-resolved experiments using the pulsed synchrotron X-rays with the time structure defined by the storage ring. In this work, the method of time-resolved X-ray excited optical luminescence was designed and implemented to do the measurement. This method is based on the principle of time-correlated single photon counting techniques. The measurement system consis...

  20. Effect of alkali metal oxides R2O (R=Na, K) on 1.53 μm luminescence of Er3+-doped Ga2O3-GeO2 glasses for optical amplification

    Institute of Scientific and Technical Information of China (English)

    赵营刚; 石冬梅

    2013-01-01

    This paper reported the thermal stability and spectroscopic properties of Ga2O3-GeO2-Na2O-K2O (GGNK) glasses doped with Er3+. The GGNK glasses were characterized by differential scanning calorimetry (DSC), Raman spectra, absorption and infra-red-visible fluorescence spectra. Measured DSC result showed that these glasses possessed an excellent stability (ΔT=188.6 oC). The relationship between glass composition and Judd-Ofelt intensity parameters and other optical properties of Er3+, such as the absorption and stimulated emission cross-sections, were clarified. Meanwhile an intense broadband 1.53-μm emission with a full width at half-maximum of 51 nm and peak emission cross-section of 9.32×10-21 cm2 of Er3+-doped GGNK glass was obtained upon 980 nm di-ode-laser excitation. Effects of K2O replacing Na2O on the thermal stability and spectroscopic properties were investigated. It was found that the incorporation of K2O into Er3+-doped Ga2O3-GeO2-Na2O glass could effectively improve the 1.53μm emission luminescence. The results showed that GGNK glass might be more attractive host material for their application in C-band optical fiber amplifiers.

  1. Improved differentiation between luminescence decay components by use of time-resolved optical activity measurements and selective lifetime modulation.

    Science.gov (United States)

    Schauerte, J A; Gafni, A; Steel, D G

    1996-01-01

    The analysis of luminescence decay experiments from proteins is typically modeled as a combination of independent first-order decay functions. However, Poisson noise in the photon counting experiment limits the ability of this approach to resolve decay components from separate lumiphores with similar lifetimes. To provide further differentiation, we incorporate time-resolved circular polarization of luminescence, an additional independent observable, into the analysis. In the simplest case, for example, each lumiphore's chirality is assumed to be time independent and is determined by the position of the lumiphore with respect to the surrounding chiral environment within the protein. In this paper, we describe the analysis of simultaneously recorded time-resolved luminescence and circularly polarized luminescence data to obtain improved temporal resolution. When combined with selective dynamic luminescence quenching, in a model system comprising a mixture of Tb/transferrin and Tb/conalbumin, we demonstrate resolution between two decay components with a lifetime difference of 7% and a difference in emission anisotropy of 5 X 10(-2). Evidence for the improved discrimination is further demonstrated by the increase in curvature of the chi 2 surface that results from the additional information. PMID:8785358

  2. Optical transistor action by nonlinear coupling of stimulated emission and coherent scattering

    Science.gov (United States)

    Andrews, David L.; Bradshaw, David S.

    2010-08-01

    In the pursuit of improved platforms for computing, communications and internet connectivity, all-optical systems offer excellent prospects for a speed and fidelity of data transmission that will greatly surpass conventional electronics, alongside the anticipated benefits of reduced energy loss. With a diverse range of sources and fiber optical connections already in production, much current effort is being devoted towards forging optical components for signal switching, such as an all-optical transistor. Achievement of the desired characteristics for any practicable device can be expected to depend crucially on the engagement of a strongly nonlinear optical response. The innovative scheme proposed in the present work is based upon a third-order nonlinearity - its effect enhanced by stimulated emission - operating within a system designed to exploit the highly nonlinear response observed at the threshold for laser emission. Here, stimulated emission is strongly driven by coupling to the coherent scattering of a signal input beam whose optical frequency is purposely off-set from resonance. An electrodynamical analysis of the all-optical coupling process shows that the signal beam can significantly modify the kinetics of emission, and so lead to a dramatically enhanced output of resonant radiation. The underlying nonlinear optical mechanism is analyzed, model calculations are performed for realizable three-level laser systems, and the results exhibited graphically. The advantages of implementing this all-optical transistor scheme, compared to several previously envisaged proposals, are then outlined.

  3. Postural adaptations to repeated optic flow stimulation in older adults.

    Science.gov (United States)

    O'Connor, Kathryn W; Loughlin, Patrick J; Redfern, Mark S; Sparto, Patrick J

    2008-10-01

    The purpose of this study is to understand the processes of adaptation (changes in within-trial postural responses) and habituation (reductions in between-trial postural responses) to visual cues in older and young adults. Of particular interest were responses to sudden increases in optic flow magnitude. The postural sway of 25 healthy young adults and 24 healthy older adults was measured while subjects viewed anterior-posterior 0.4 Hz sinusoidal optic flow for 45 s. Three trials for each of three conditions were performed: (1) constant 12 cm optic flow amplitude (24 cm peak-to-peak), (2) constant 4 cm amplitude (8 cm p-t-p), and (3) a transition in amplitude from 4 to 12 cm. The average power of head sway velocity (P(vel)) was calculated for consecutive 5s intervals during the trial to examine the changes in sway within and between trials. A mixed factor repeated measures ANOVA was performed to examine the effects of subject Group, Trial, and Interval on the P(vel). P(vel) was greater in older adults in all conditions (phabituation. P(vel) of the older adults decreased significantly between all 3 trials, but decreased only between Trials 1 and 2 in young adults. While the responses of the young adults to the transition in optic flow from 4 to 12 cm did not significantly change, older adults had an increase in P(vel) following the transition, ranging from 6.5 dB for the first trial to 3.4 dB for the third trial. These results show that older adults can habituate to repeated visual perturbation exposures; however, this habituation requires a greater number of exposures than young adults. This suggests aging impacts the ability to quickly modify the relative weighting of the sensory feedback for postural stabilization.

  4. High speed data encryption and decryption using stimulated Brillouin scattering effect in optical fiber

    Science.gov (United States)

    Yi, Lilin; Zhang, Tao; Hu, Weisheng

    2011-11-01

    A novel all-optical encryption/decryption method based on stimulated Brillouin scattering (SBS) effect in optical fiber is proposed for the first time. The operation principle is explained in detail and the encryption and decryption performance is experimentally evaluated. The encryption keys could be the SBS gain amplitude, bandwidth, central wavelength and spectral shape, which are configurable and flexibly controlled by the users. We experimentally demonstrate the SBS encryption/decryption process of a 10.86-Gb/s non-return-to-zero (NRZ) data by using both phase-modulated and current-dithered Brillouin pumps for proof-of-concept. Unlike the traditional optical encryption methods of chaotic communications and optical code-division-multiplexing access (OCDMA), the SBS based encryption/decryption technique can directly upgrade the current optical communication system to a secure communication system without changing the terminal transceivers, which is completely compatible with the current optical communication systems.

  5. Time-gated optical imaging through turbid media using stimulated Raman scattering: Studies on image contrast

    Indian Academy of Sciences (India)

    K Divakar Rao; H S Patel; B Jain; P K Gupta

    2005-02-01

    In this paper, we report the development of experimental set-up for timegated optical imaging through turbid media using stimulated Raman scattering. Our studies on the contrast of time-gated images show that for a given optical thickness, the image contrast is better for sample with lower scattering coefficient and higher physical thickness, and that the contrast improves with decreasing value of anisotropy parameters of the scatterers. These results are consistent with time-resolved Monte Carlo simulations.

  6. Analysis of optical neural stimulation effects on neural networks affected by neurodegenerative diseases

    Science.gov (United States)

    Zverev, M.; Fanjul-Vélez, F.; Salas-García, I.; Ortega-Quijano, N.; Arce-Diego, J. L.

    2016-03-01

    The number of people in risk of developing a neurodegenerative disease increases as the life expectancy grows due to medical advances. Multiple techniques have been developed to improve patient's condition, from pharmacological to invasive electrodes approaches, but no definite cure has yet been discovered. In this work Optical Neural Stimulation (ONS) has been studied. ONS stimulates noninvasively the outer regions of the brain, mainly the neocortex. The relationship between the stimulation parameters and the therapeutic response is not totally clear. In order to find optimal ONS parameters to treat a particular neurodegenerative disease, mathematical modeling is necessary. Neural networks models have been employed to study the neural spiking activity change induced by ONS. Healthy and pathological neocortical networks have been considered to study the required stimulation to restore the normal activity. The network consisted of a group of interconnected neurons, which were assigned 2D spatial coordinates. The optical stimulation spatial profile was assumed to be Gaussian. The stimulation effects were modeled as synaptic current increases in the affected neurons, proportional to the stimulation fluence. Pathological networks were defined as the healthy ones with some neurons being inactivated, which presented no synaptic conductance. Neurons' electrical activity was also studied in the frequency domain, focusing specially on the changes of the spectral bands corresponding to brain waves. The complete model could be used to determine the optimal ONS parameters in order to achieve the specific neural spiking patterns or the required local neural activity increase to treat particular neurodegenerative pathologies.

  7. An integrated optical coherence microscopy imaging and optical stimulation system for optogenetic pacing in Drosophila melanogaster (Conference Presentation)

    Science.gov (United States)

    Alex, Aneesh; Li, Airong; Men, Jing; Jerwick, Jason; Tanzi, Rudolph E.; Zhou, Chao

    2016-03-01

    Electrical stimulation is the clinical standard for cardiac pacing. Although highly effective in controlling cardiac rhythm, the invasive nature, non-specificity to cardiac tissues and possible tissue damage limits its applications. Optogenetic pacing of the heart is a promising alternative, which is non-invasive and more specific, has high spatial and temporal precision, and avoids the shortcomings in electrical stimulation. Drosophila melanogaster, which is a powerful model organism with orthologs of nearly 75% of human disease genes, has not been studied for optogenetic pacing in the heart. Here, we developed a non-invasive integrated optical pacing and optical coherence microscopy (OCM) imaging system to control the heart rhythm of Drosophila at different developmental stages using light. The OCM system is capable of providing high imaging speed (130 frames/s) and ultrahigh imaging resolutions (1.5 μm and 3.9 μm for axial and transverse resolutions, respectively). A light-sensitive pacemaker was developed in Drosophila by specifically expressing the light-gated cation channel, channelrhodopsin-2 (ChR2) in transgenic Drosophila heart. We achieved non-invasive and specific optical control of the Drosophila heart rhythm throughout the fly's life cycle (larva, pupa, and adult) by stimulating the heart with 475 nm pulsed laser light. Heart response to stimulation pulses was monitored non-invasively with OCM. This integrated non-invasive optogenetic control and in vivo imaging technique provides a novel platform for performing research studies in developmental cardiology.

  8. Emission of thermally stimulated luminescence in mixed monocrystals KCl-KBr: Pb{sup 2+}, KCl: Pb{sup 2+} and KBr: Pb{sup 2+} exposed at low doses; Emision de luminiscencia estimulada termicamente en monocristales mixtos KCl-KBr:Pb{sup 2+}, KCl:Pb{sup 2+} y KBr:Pb{sup 2+} expuestos a dosis bajas

    Energy Technology Data Exchange (ETDEWEB)

    Cruz Z, E.; Ramos B, S. [Instituto de Ciencias Nucleares UNAM, A.P. 70-543, 04510 Mexico D.F. (Mexico); Melendrez A, R.; Chernov, V.; Piters, T.M.; Barboza F, M. [Centro de Investigacion en Fisica, Universidad de Sonora, A.P. 5-88 Hermosillo, Sonora (Mexico); Hernandez A, J.; Murrieta S, H. [Instituto de Fisica UNAM, A.P. 20-364, 01000 Mexico D.F. (Mexico)

    2002-07-01

    It is reported the behavior of solid solutions of mixed crystals KCl{sub 1-x} KBr{sub x} doped with divalent lead which were exposed to gamma radiation. The mixtures of KCl-KBr were varied, with x equivalents at 2, 50, 65, and 85 % including the extremes KCl: Pb{sup 2+} and KBr: Pb{sup 2+}. It was maintained a concentration of divalent lead between 20 and 40 ppm in the crystalline lattice. The production of the generated defects by radiation have been correlated with the increase in the brilliance curves depending on the received dose by the mixed doped crystal. It has been used the thermal stimulation (Tl) for obtaining the crystal luminescence depending on the dose until 130 Gy with gammas of cobalt 60. The results shows that this mixed crystalline material of varied composition responds adequately to low doses which indicates that this would be a good detector of ionizing radiation. The results have been correlated with the optical properties of this mixed doped crystal, however it has been found that exists an important loss of luminescence depending on the halogen quantity presents in the mixed crystal. (Author)

  9. System for X-Ray excited optical luminescence (XEOL) measurements; Sistema para realizacao de medidas de luminescencia com excitacao por raios X

    Energy Technology Data Exchange (ETDEWEB)

    Cebim, Marco Aurelio; Oliveira, Higor Henrique de Souza; Barelli, Nilso; Davolos, Marian Rosaly [UNESP, Araraquara, SP (Brazil). Inst. de Quimica. Dept. de Quimica Geral e Inorganica

    2011-07-01

    In this work is presented a versatile system for X-ray excited optical luminescence (XEOL) measurements. The apparatus was assembled from a sample holder connected to an optical fiber responsibly for the acquisition of the scintillation signal. The spectrum is registered with a CCD coupled in a spectrograph provided with diffraction gratings. The system performance was analyzed by exciting GdAlO3:Eu{sup 3+} 3.0 at.% with X-rays from a diffractometer and measuring the emission spectra. The system can be used to obtain precise and reliable spectroscopic properties of samples with various conformations without the loss of the required safety when dealing with ionizing radiations. (author)

  10. Luminescence dating of Pleistocene alluvial sediments affected by the Alhama de Murcia fault (eastern Betics, Spain) – a comparison between OSL, IRSL and post-IRIRSL ages

    DEFF Research Database (Denmark)

    Sohbati, Reza; Murray, Andrew S.; Buylaert, Jan-Pieter

    2012-01-01

    The ages of nine alluvial units, identified by the integration of data obtained from five trenches at the southern termination of the Alhama de Murcia Fault (AMF) (eastern Betics, Spain), are constrained using luminescence dating based on the Optically Stimulated Luminescence (OSL) from quartz......, Infrared Stimulated Luminescence (IRSL) at 50°C, and post-IR elevated temperature (225°C) IRSL signals from K-feldspar. All signals pass the routine tests associated with the Single Aliquot Regenerative (SAR) protocol, including the recycling ratio, recuperation, and dose recovery tests. The equivalent...... of anomalous fading to a great extent, the resulting age cannot be regarded as necessarily accurate because of the limitations of the fading correction model used, and the absence of independent age control for the old samples. Nevertheless, our luminescence ages provide the first age constraints...

  11. Stimulated Raman scattering modes in highly elliptical-core optical fiber

    Institute of Scientific and Technical Information of China (English)

    王兆民; 顾春明; 林景全; 郑学彦

    1996-01-01

    Stimulated Raman scattering (SRS) transmission modes in highly elliptical-core optical fiber of three different structures are experimentally researched.The measuring setup,SRS spectrum and photographs of Stokes modes are given.The observed phenomena are completely different from those on circular-core graded-index optical fiber.The beam sizes of SRS remain constant and SRS light transmits with the characteristics of higher-order.mode.In addition,the experimental results are theoretically explained with fiber-optical dispersion theory and SRS phase matching conditions.Experimental results and theoretical analyses are in good agreement.

  12. Microprocessor-controlled optical stimulating device to improve the gait of patients with Parkinson's disease.

    Science.gov (United States)

    Ferrarin, M; Brambilla, M; Garavello, L; Di Candia, A; Pedotti, A; Rabuffetti, M

    2004-05-01

    Different types of visual cue for subjects with Parkinson's disease (PD) produced an improvement in gait and helped some of them prevent or overcome freezing episodes. The paper describes a portable gait-enabling device (optical stimulating glasses (OSGs) that provides, in the peripheral field of view, different types of continuous optic flow (backward or forward) and intermittent stimuli synchronised with external events. The OSGs are a programmable, stand-alone, augmented reality system that can be interfaced with a PC for program set-up. It consists of a pair of non-corrective glasses, equipped with two matrixes of 70 micro light emitting diodes, one on each side, controlled by a microprocessor. Two foot-switches are used to synchronise optical stimulation with specific gait events. A pilot study was carried out on three PD patients and three controls, with different types of optic flow during walking along a fixed path. The continuous optic flow in the forward direction produced an increase in gait velocity in the PD patients (up to + 11% in average), whereas the controls had small variations. The stimulation synchronised with the swing phase, associated with an attentional strategy, produced a remarkable increase in stride length for all subjects. After prolonged testing, the device has shown good applicability and technical functionality, it is easily wearable and transportable, and it does not interfere with gait.

  13. Understanding optically stimulated charge movement in quartz and feldspar using time-resolved measurements

    DEFF Research Database (Denmark)

    Ankjærgaard, Christina

    to identify various charge transport mechanisms in the different time regimes. The techniques employed are time-resolved OSL, continuous-wave OSL, TL, optically stimulated exo-electron (OSE) emission and time-resolved OSE. These different techniques are used in combination with variable thermal or optical...... and the conduction band in determining charge transport. It is suggested that unlike quartz, the excited state lifetime does not play an important role in our measurements. Finally, it is shown that one of these routes favors production if a least fading signal (due to quantum mechanical tunnelling) in feldspars...... the TR-OSL and optically stimulated phosphorescence signals from quartz and feldspars spanning several orders of magnitude in time (few ns to the seconds time scale) in order to identify various charge transport mechanisms in the different time regimes. The techniques employed are time-resolved OSL...

  14. Controlling plasmon-enhanced luminescence

    NARCIS (Netherlands)

    Mertens, H.

    2007-01-01

    Plasmons are collective oscillations of the free electrons in a metal or an ionized gas. Plasmons dominate the optical properties of noble-metal nanoparticles, which enables a variety of applications. This thesis focuses on plasmon-enhanced luminescence of silicon quantum dots (Si QDs) and optically

  15. Stored Luminescence Computed Tomography

    CERN Document Server

    Cong, Wenxiang; Wang, Ge

    2013-01-01

    The phosphor nanoparticles made of doped semiconductors, pre-excited by well-collimated X-ray radiation, were recently reported for their light emission upon NIR light stimulation. The characteristics of X-ray energy storage and NIR stimulated emission is highly desirable to design targeting probes and improve molecular and cellular imaging. Here we propose stored luminescence computed tomography (SLCT), perform realistic numerical simulation, and demonstrate a much-improved spatial resolution in a preclinical research context. The future opportunities are also discussed along this direction.

  16. Luminescence properties of Er3+ ions doped bismuth borate glasses for 1.53 \\xB5m broadband optical amplifiers

    Science.gov (United States)

    Mariyappan, M.; Suthanthirakumar, P.; Arunkumar, S.; Marimuthu, K.

    2017-05-01

    A new series of Er3+ ions doped bismuth borate glasses were prepared with the composition (40—x)B2O3 + 20Bi2O3+20Na2O+20CaF2+xEr2O3 (where x= 0.1, 0.25, 0.5, 1 and 2 in wt%). The spectroscopic behaviors of the titled glasses have been examined through absorption, luminescence and decay spectral analysis. Luminescence spectra along with the JO intensity parameters have been used to determine the various radiative properties like transition probability (A), stimulated emission cross-section (σp), lifetimes (τcal, τexp), branching ratios (βR) and effective bandwidth (Δλeff) for the 4S3/2 →4I15/2 and 4I13/2→4I15/2 emission transitions and the results were discussed and reported. By employing the McCumbar theory, absorption and emission cross-sections for the 4I13/2→4I15/2 transition (1.53 μm) were calculated for all the titled glasses. The decay curves of the 4I13/2 level have been measured and the fall in lifetime value with the increase in Er3+ ion content have been studied through the energy transfer process takes place between the nearby Er3+ ions.

  17. Nonlinear optical absorption and stimulated Mie scattering in metallic nanoparticle suspensions

    Science.gov (United States)

    He, Guang S.; Law, Wing-Cheung; Baev, Alexander; Liu, Sha; Swihart, Mark T.; Prasad, Paras N.

    2013-01-01

    The nonlinear optical properties of four metallic (Au-, Au/Ag-, Ag-, and Pt-) nanoparticle suspensions in toluene have been studied in both femtosecond and nanosecond regimes. Nonlinear transmission measurements in the femtosecond laser regime revealed two-photon absorption (2PA) induced nonlinear attenuation, while in the nanosecond laser regime a stronger nonlinear attenuation is due to both 2PA and 2PA-induced excited-state absorption. In the nanosecond regime, at input pump laser intensities above a certain threshold value, a new type of stimulated (Mie) scattering has been observed. Being essentially different from all other well known molecular (Raman, Brillouin) stimulated scattering effects, the newly observed stimulated Mie scattering from the metallic nanoparticles exhibits the features of no frequency shift and low pump threshold requirement. A physical model of induced Bragg grating initiated by the backward Mie scattering from metallic nanoparticles is proposed to explain the gain mechanism of the observed stimulated scattering effect.

  18. High temperature luminescence of Dy3+ in crystalline silicon in the optical communication and eye-safe spectral regions.

    Science.gov (United States)

    Lourenço, M A; Mustafa, Z; Ludurczak, W; Wong, L; Gwilliam, R M; Homewood, K P

    2013-09-15

    We report on photoluminescence in the 1.3 and 1.7 μm spectral ranges in silicon doped with dysprosium. This is attributed to the Dy3+ internal transitions between the second Dy3+ excited state and the ground state, and between the third Dy3+ excited state and the ground state. Luminescence is achieved by Dy implantation into Si substrates codoped with boron, to form dislocation loops, and show a strong dependence on fabrication process. The spectra consist of several sharp lines with the strongest emission at 1736 nm, observed up to 200 K. No Dy3+ luminescence is observed in samples without B codoping, showing the paramount importance of dislocation loops to enable the Dy emission.

  19. Biocompatible Optically Transparent MEMS for Micromechanical Stimulation and Multimodal Imaging of Living Cells.

    Science.gov (United States)

    Fior, Raffaella; Kwok, Jeanie; Malfatti, Francesca; Sbaizero, Orfeo; Lal, Ratnesh

    2015-08-01

    Cells and tissues in our body are continuously subjected to mechanical stress. Mechanical stimuli, such as tensile and contractile forces, and shear stress, elicit cellular responses, including gene and protein alterations that determine key behaviors, including proliferation, differentiation, migration, and adhesion. Several tools and techniques have been developed to study these mechanobiological phenomena, including micro-electro-mechanical systems (MEMS). MEMS provide a platform for nano-to-microscale mechanical stimulation of biological samples and quantitative analysis of their biomechanical responses. However, current devices are limited in their capability to perform single cell micromechanical stimulations as well as correlating their structural phenotype by imaging techniques simultaneously. In this study, a biocompatible and optically transparent MEMS for single cell mechanobiological studies is reported. A silicon nitride microfabricated device is designed to perform uniaxial tensile deformation of single cells and tissue. Optical transparency and open architecture of the device allows coupling of the MEMS to structural and biophysical assays, including optical microscopy techniques and atomic force microscopy (AFM). We demonstrate the design, fabrication, testing, biocompatibility and multimodal imaging with optical and AFM techniques, providing a proof-of-concept for a multimodal MEMS. The integrated multimodal system would allow simultaneous controlled mechanical stimulation of single cells and correlate cellular response.

  20. Understanding landscape dynamics of the Sierra de Juarez, southern Mexico: An exploratory approach using inherited luminescence signals

    Science.gov (United States)

    Muñoz-Salinas, Esperanza; Castillo, Miguel; Caballero, Lizeth; Lacan, Pierre

    2017-07-01

    We explore inherited luminescence signals to generate information about different mechanisms involved in mobilization of debris flows in rivers (n = 12) of the Sierra de Juárez (Oaxaca, Mexico), that flow across the Oaxaca and Donaji faults. Sediment samples composed of poly-mineral and poly-grain sizes were optically stimulated using a Pulsed-Photon Stimulated Luminescence unit. In most of the rivers, the luminescence signals intensities fall with increasing distance from their source and the luminescence of different grain size fractions were variable. Our results suggest that mineral grains were transported in the water column without any stratification based on grain sizes, indicating debris flows and/or hyper-concentrated flows. A correlation between the inherited luminescence signals and the mean basin slope provides information about the river basin topography. Our results suggest that mobilization of sediments is related to the steepness of topography produced by the Oaxaca fault formation and inherited luminescence signals has a good potential to unravel the processes involved in the transport of fluvial sediment in mountainous settings of southern Mexico.

  1. Luminescence and photo-thermally stimulated defects creation processes in PbWO{sub 4} crystals doped with trivalent rare-earth ions

    Energy Technology Data Exchange (ETDEWEB)

    Fabeni, P. [Institute of Applied Physics “N.Carrara” (IFAC) of CNR, Via Madonna del Piano 10, 50019 Sesto Fiorentino (Firenze) (Italy); Krasnikov, A.; Kärner, T. [Institute of Physics, University of Tartu, Riia 142, 51014 Tartu (Estonia); Laguta, V.V.; Nikl, M. [Institute of Physics AS CR, Cukrovarnicka 10, 16253 Prague (Czech Republic); Pazzi, G.P. [Institute of Applied Physics “N.Carrara” (IFAC) of CNR, Via Madonna del Piano 10, 50019 Sesto Fiorentino (Firenze) (Italy); Zazubovich, S., E-mail: svet@fi.tartu.ee [Institute of Physics, University of Tartu, Riia 142, 51014 Tartu (Estonia)

    2013-04-15

    In PbWO{sub 4} crystals, doped with various trivalent rare-earth A{sup 3+} ions (A{sup 3+}: La{sup 3+}, Lu{sup 3+}, Y{sup 3+}, Ce{sup 3+}, Gd{sup 3+}), electron (WO{sub 4}){sup 3−} and {(WO_4)"3"−–A"3"+} centers can be created under UV irradiation not only in the host absorption region but also in the energy range around 3.85 eV (Böhm et al., 1999; Krasnikov et al., 2010). Under excitation in the same energy range, the UV emission peak at 3.05–3.20 eV is observed. In the present work, the origin of this emission is investigated in detail by low-temperature time-resolved luminescence methods. Photo-thermally stimulated creation of (WO{sub 4}){sup 3−} and {(WO_4)"3"−–A"3"+} centers is studied also in PbWO{sub 4}:Mo,A{sup 3+} crystals. Various processes, which could explain both the appearance of the UV emission and the creation of the {(WO_4)"3"−–A"3"+}-type centers under irradiation of PbWO{sub 4}: A{sup 3+} crystals in the 3.85±0.35 eV energy range, are discussed. The radiative and non-radiative decay of the excitons localized near A{sup 3+} ions is considered as the most probable mechanism to explain the observed features. -- Highlights: ► UV emission of PbWO{sub 4}: A{sup 3+} (A{sup 3+}: La{sup 3+}, Lu{sup 3+}, Y{sup 3+}, Ce{sup 3+}, and Gd{sup 3+}) crystals is studied. ► The emission is ascribed to the radiative decay of excitons localized near A{sup 3+} ions. ► The excitons are created at 3.85 eV excitation by a two-step process. ► Non-radiative decay of the excitons leads to the creation of (WO{sub 4}){sup 3−}–A{sup 3+} centers.

  2. Optical parametric amplification and oscillation assisted by low-frequency stimulated emission

    CERN Document Server

    Longhi, Stefano

    2016-01-01

    Optical parametric amplification/oscillation provide a powerful tool for coherent light generation in spectral regions inaccessible to lasers. Parametric gain is based on a frequency {\\it down-conversion} process, and thus it can not be realized for signal waves at a frequency $\\omega_3$ {\\it higher} than the frequency of the pump wave $\\omega_1$. In this work we suggest a route toward the realization of {\\it up-conversion} optical parametric amplification and oscillation, i.e. amplification of the signal wave by a coherent pump wave of lower frequency, assisted by stimulated emission of the auxiliary idler wave. When the signal field is resonated in an optical cavity, parametric oscillation is obtained. Design parameters for the observation of up-conversion optical parametric oscillation at $\\lambda_3=465$ nm are given for a periodically-poled lithium-niobate (PPLN) crystal doped with Nd$^{3+}$ ions.

  3. Progress in chemical luminescence-based biosensors: A critical review.

    Science.gov (United States)

    Roda, Aldo; Mirasoli, Mara; Michelini, Elisa; Di Fusco, Massimo; Zangheri, Martina; Cevenini, Luca; Roda, Barbara; Simoni, Patrizia

    2016-02-15

    Biosensors are a very active research field. They have the potential to lead to low-cost, rapid, sensitive, reproducible, and miniaturized bioanalytical devices, which exploit the high binding avidity and selectivity of biospecific binding molecules together with highly sensitive detection principles. Of the optical biosensors, those based on chemical luminescence detection (including chemiluminescence, bioluminescence, electrogenerated chemiluminescence, and thermochemiluminescence) are particularly attractive, due to their high-to-signal ratio and the simplicity of the required measurement equipment. Several biosensors based on chemical luminescence have been described for quantitative, and in some cases multiplex, analysis of organic molecules (such as hormones, drugs, pollutants), proteins, and nucleic acids. These exploit a variety of miniaturized analytical formats, such as microfluidics, microarrays, paper-based analytical devices, and whole-cell biosensors. Nevertheless, despite the high analytical performances described in the literature, the field of chemical luminescence biosensors has yet to demonstrate commercial success. This review presents the main recent advances in the field and discusses the approaches, challenges, and open issues, with the aim of stimulating a broader interest in developing chemical luminescence biosensors and improving their commercial exploitation.

  4. Luminescence response of synthetic opal under femtosecond laser pumping

    Energy Technology Data Exchange (ETDEWEB)

    Vasnetsov, M.V., E-mail: vasnet@hotmail.com [Institute of Physics, National Academy of Sciences of Ukraine, Prospect Nauki 46, Kiev 03680 (Ukraine); Bazhenov, V.Yu.; Dmitruk, I.N. [Institute of Physics, National Academy of Sciences of Ukraine, Prospect Nauki 46, Kiev 03680 (Ukraine); Kudryavtseva, A.D.; Tcherniega, N.V. [P. N. Lebedev Physical Institute of Russian Academy of Sciences, Leninskii Prospect 53, Moscow 119991 (Russian Federation)

    2015-10-15

    Synthetic opal is an artificial photonic metamaterial composed from spherical globules of amorphous silica (SiO{sub 2}) about 300 nm in diameter. We report, for the first time to our knowledge, the origin of a narrow luminescence spectral peak (4 nm HWHM) and optical second and third harmonic generation in synthetic opal samples under femtosecond laser excitation (800 nm) at liquid-nitrogen temperature. Stimulated-emission effects are discussed related to the possibility of nanocavity lasing at the condition of the first Mie resonance in a dielectric sphere. - Highlights: • Second harmonic generation in a synthetic opal (amorphous material composed from spherical SiO{sub 2} globules) was observed. • Narrow luminescence peak which we assign to a Mie resonance in a globule was detected at liquid-nitrogen temperature.

  5. Synthesis, characterization and optical studies of highly luminescent ZnS nanoparticles associated with hypromellose matrix as a green and novel stabilizer.

    Science.gov (United States)

    Tiwari, Ashish; Khan, S A; Kher, R S; Dhoble, S J

    2014-09-01

    ZnS nanoparticles stabilized by a carbohydrate-based matrix, hypromellose (hydroxypropyl methylcellulose) were prepared via a wet chemical method. The nanocomposite was characterized by X-ray diffraction, transmission electon microscopy and Fourier transform infrared spectroscopy. X-Ray diffraction patterns revealed a zinc blende structure. Thermogravimetric analysis suggested that polymer attached to the surface decomposes at 700 °C. Absorption measurements were carried out and calculation of the diameter polydispersity index (DPI) suggests the formation of monodisperse nanoparticles. The optical properties of the as-prepared samples were studied by UV/vis spectroscopy and steady-state photoluminescence (PL) spectroscopy. The PL studies indicate the applicability of these nanoparticles as biocompatible sensors or luminescence markers in future.

  6. Hybrid electro-optical stimulation of the rat sciatic nerve induces force generation in the plantarflexor muscles

    Science.gov (United States)

    Duke, Austin R.; Peterson, Erik; Mackanos, Mark A.; Atkinson, James; Tyler, Dustin; Jansen, E. Duco

    2012-12-01

    Objective. Optical methods of neural activation are becoming important tools for the study and treatment of neurological disorders. Infrared nerve stimulation (INS) is an optical technique exhibiting spatially precise activation in the native neural system. While this technique shows great promise, the risk of thermal damage may limit some applications. Combining INS with traditional electrical stimulation, a method known as hybrid electro-optical stimulation, reduces the laser power requirements and mitigates the risk of thermal damage while maintaining spatial selectivity. Here we investigate the capability of inducing force generation in the rat hind limb through hybrid stimulation of the sciatic nerve. Approach. Hybrid stimulation was achieved by combining an optically transparent nerve cuff for electrical stimulation and a diode laser coupled to an optical fiber for infrared stimulation. Force generation in the rat plantarflexor muscles was measured in response to hybrid stimulation with 1 s bursts of pulses at 15 and 20 Hz and with a burst frequency of 0.5 Hz. Main results. Forces were found to increase with successive stimulus trains, ultimately reaching a plateau by the 20th train. Hybrid evoked forces decayed at a rate similar to the rate of thermal diffusion in tissue. Preconditioning the nerve with an optical stimulus resulted in an increase in the force response to both electrical and hybrid stimulation. Histological evaluation showed no signs of thermally induced morphological changes following hybrid stimulation. Our results indicate that an increase in baseline temperature is a likely contributor to hybrid force generation. Significance. Extraneural INS of peripheral nerves at physiologically relevant repetition rates is possible using hybrid electro-optical stimulation.

  7. Eu2+ luminescence in strontium aluminates

    OpenAIRE

    Dutczak, D.; Juestel, T.; Ronda, C.; Meijerink, A.|info:eu-repo/dai/nl/075044986

    2015-01-01

    The luminescence properties of Eu2+ doped strontium aluminates are reported and reviewed for a variety of aluminates, viz. SrAl12O19, SrAl4O7, Sr4Al14O25, SrAl2O4 and Sr3Al2O6. The aim of the research is to investigate the role of local coordination and covalency of the aluminate host lattice, related to the Sr/Al ratio, on the optical properties of the Eu2+ ion. The UV and VUV excited luminescence spectra as well as luminescence decay curves were recorded to characterize the luminescence pro...

  8. Mathematical model quantifies multiple daylight exposure and burial events for rock surfaces using luminescence dating

    DEFF Research Database (Denmark)

    Freiesleben, Trine Holm; Sohbati, Reza; Murray, Andrew

    2015-01-01

    Interest in the optically stimulated luminescence (OSL) dating of rock surfaces has increased significantly over the last few years, as the potential of the method has been explored. It has been realized that luminescence-depth profiles show qualitative evidence for multiple daylight exposure and...... to determine the length of a fossil exposure, using a known natural light exposure as calibration. © 2015 Published by Elsevier Ltd....... of the cobble and by fitting the new model to the luminescence profile, it is concluded that the cobble was well bleached before burial. This indicates that the OSL burial age is likely to be reliable. In addition, a recent known exposure event provides an approximate calibration for older daylight exposure...

  9. Optical absorption and luminescence characteristics of Dy{sup 3+} doped Zinc Alumino Bismuth Borate glasses for lasing materials and white LEDs

    Energy Technology Data Exchange (ETDEWEB)

    Swapna, K.; Mahamuda, Sk. [Department of Physics, K.L. University, Green Fields, Vaddeswaram 522502, A.P. (India); Srinivasa Rao, A., E-mail: drsrallam@yahoo.co.in [Department of Physics, K.L. University, Green Fields, Vaddeswaram 522502, A.P. (India); Department of Applied Physics, Delhi Technological University, Delhi 110042 (India); Jayasimhadri, M. [Department of Applied Physics, Delhi Technological University, Delhi 110042 (India); Sasikala, T.; Rama Moorthy, L. [Department of Physics, S.V. University, Tirupathi 517502, A.P. (India)

    2013-07-15

    Good optical quality Dy{sup 3+} doped Zinc Alumino Bismuth Borate (ZnAlBiB) glasses were prepared by the conventional melt quenching technique and characterized by optical absorption and luminescence studies. The glassy nature of these materials has been confirmed through XRD measurements. From the absorption spectra, the three phenomenological JO parameters Ω{sub λ} (λ=2,4 and 6) have been determined from the absorption spectral intensities by using the JO theory. Luminescence spectra were measured for different concentrations of Dy{sup 3+} ions doped glasses by exciting the glasses at 387 nm. The intensity of Dy{sup 3+} emission spectra increases from 0.5 mol% to 1 mol % and beyond 1 mol % the concentration quenching is observed. The suitable concentration of Dy{sup 3+} ions for ZnAlBiB glassy material to act as good lasing material has been discussed by measuring the branching ratios and emission cross-sections for two strong emission transitions such as {sup 4}F{sub 9/2}→{sup 6}H{sub 15/2} and {sup 4}F{sub 9/2}→{sup 6}H{sub 13/2} observed in visible region. By exciting these glassy materials at various excitation wavelengths in n-UV region, the CIE chromaticity coordinates were evaluated for the two sharp emissions observed in blue ({sup 4}F{sub 9/2}→{sup 6}H{sub 15/2}) and yellow ({sup 4}F{sub 9/2}→{sup 6}H{sub 13/2}) regions to understand the suitability of these materials for white light generation. -- Highlights: ► Successfully synthesized the transparent Zinc Alumino Bismuth Borate glasses. ► Measured the absorption and luminescence properties. ► Discussed the spectroscopic properties by using Judd–Ofelt analysis for ZnAlBiB glasses. ► Finally, suitability of these glasses for lasers and white LEDs has been discussed.

  10. Handbook of luminescent semiconductor materials

    CERN Document Server

    Bergman, Leah

    2011-01-01

    Photoluminescence spectroscopy is an important approach for examining the optical interactions in semiconductors and optical devices with the goal of gaining insight into material properties. With contributions from researchers at the forefront of this field, Handbook of Luminescent Semiconductor Materials explores the use of this technique to study semiconductor materials in a variety of applications, including solid-state lighting, solar energy conversion, optical devices, and biological imaging. After introducing basic semiconductor theory and photoluminescence principles, the book focuses

  11. Optical imaging of the retina in response to the electrical stimulation

    Science.gov (United States)

    Fujikado, Takashi; Okawa, Yoshitaka; Miyoshi, Tomomitsu; Hirohara, Yoko; Mihashi, Toshifumi; Tano, Yasuo

    2008-02-01

    Purposes: To determine if reflectance changes of the retina can be detected following electrical stimulation to the retina using a newly developed optical-imaging fundus camera. Methods: Eyes of cats were examined after pupil dilation. Retina was stimulated either focally by a ball-type electrode (BE) placed on the fenestrated sclera or diffusely using a ring-type electrode (RE) placed on the corneoscleral limbus. Electrical stimulation by biphasic pulse trains was applied for 4 seconds. Fundus images with near-infrared (800-880 nm) light were obtained between 2 seconds before and 20 seconds after the electrical stimulation (ES). A two-dimensional map of the reflectance changes (RCs) was constructed. The effect of Tetrodotoxin (TTX) was also investigated on RCs by ES using RE. Results: RCs were observed around the retinal locus where the stimulating electrodes were positioned (BE) or in the retina of the posterior pole (RE), in which the latency was about 0.5 to 1.0 sec and the peak time about 2 to 5 sec after the onset of ES. The intensity of the RCs increased with the increase of the stimulus current in both cases. RCs were completely suppressed after the injection of TTX. Conclusions: The functional changes of the retina either by focal or diffuse electrical stimulation were successfully detected by optical imaging of the retina. The contribution of retinal ganglion cells on RCs by ES was confirmed by TTX experiment. This method may be applied to the objective evaluation of the artificial retina.

  12. Thermal dependence of luminescence lifetimes and radioluminescence in quartz

    Energy Technology Data Exchange (ETDEWEB)

    Pagonis, V., E-mail: vpagonis@mcdaniel.edu [McDaniel College, Physics Department, Westminster, MD 21157 (United States); Chithambo, M.L. [Department of Physics and Electronics, Rhodes University, PO BOX 94, Grahamstown 6140 (South Africa); Chen, R. [Raymond and Beverly Sackler School of Physics and Astronomy, Tel-Aviv University, Tel-Aviv 69978 (Israel); Chruścińska, A. [Institute of Physics, Nicholas Copernicus University, 87-100 Toruń (Poland); Fasoli, M. [Department of Materials Science, University of Milano-Bicocca, Via Cozzi 53, 20125 Milano (Italy); Li, S.H. [Department of Earth Sciences, The University of Hong Kong (Hong Kong); Martini, M. [Department of Materials Science, University of Milano-Bicocca, Via Cozzi 53, 20125 Milano (Italy); Ramseyer, K. [Institut für Geologie, Baltzerstrasse 1-3, 3012 Bern (Switzerland)

    2014-01-15

    During time-resolved optical stimulation experiments (TR-OSL), one uses short light pulses to separate the stimulation and emission of luminescence in time. Experimental TR-OSL results show that the luminescence lifetime in quartz of sedimentary origin is independent of annealing temperature below 500 °C, but decreases monotonically thereafter. These results have been interpreted previously empirically on the basis of the existence of two separate luminescence centers L{sub H} and L{sub L} in quartz, each with its own distinct luminescence lifetime. Additional experimental evidence also supports the presence of a non-luminescent hole reservoir R, which plays a critical role in the predose effect in this material. This paper extends a recently published analytical model for thermal quenching in quartz, to include the two luminescence centers L{sub H} and L{sub L}, as well as the hole reservoir R. The new extended model involves localized electronic transitions between energy states within the two luminescence centers, and is described by a system of differential equations based on the Mott–Seitz mechanism of thermal quenching. It is shown that by using simplifying physical assumptions, one can obtain analytical solutions for the intensity of the light during a TR-OSL experiment carried out with previously annealed samples. These analytical expressions are found to be in good agreement with the numerical solutions of the equations. The results from the model are shown to be in quantitative agreement with published experimental data for commercially available quartz samples. Specifically the model describes the variation of the luminescence lifetimes with (a) annealing temperatures between room temperature and 900 °C, and (b) with stimulation temperatures between 20 and 200 °C. This paper also reports new radioluminescence (RL) measurements carried out using the same commercially available quartz samples. Gaussian deconvolution of the RL emission spectra was

  13. Household and workplace chemicals as retrospective luminescence dosemeters

    DEFF Research Database (Denmark)

    Thomsen, Kristina Jørkov; Bøtter-Jensen, L.; Murray, A.S.

    2002-01-01

    In the development of techniques for the retrospective assessment of the close absorbed by communities living and working adjacent to the site of a nuclear accident, attention has concentrated on the use Of natural minerals such as quartz and feldspar as dosemeters. These minerals are widely found......, there are Other potential unheated crystalline materials found in the domestic and industrial environment which may also act as retrospective dosemeters, and may be considerably more sensitive. We have Surveyed the thermoluminescent and optically stimulated luminescent (OSL) characteristics of several...

  14. A luminescence imaging system based on a CCD camera

    DEFF Research Database (Denmark)

    Duller, G.A.T.; Bøtter-Jensen, L.; Markey, B.G.

    1997-01-01

    to photographic systems, in order to obtain spatially resolved data. However, the former option is extremely expensive and it is difficult to obtain quantitative data from the latter. This paper describes the use of a CCD camera for imaging both thermoluminescence and optically stimulated luminescence. The system...... described here has a maximum spatial resolution of 17 mu m; though this may be varied under software control to alter the signal-to-noise ratio. The camera has been mounted on a Riso automated TL/OSL reader, and both the reader and the CCD are under computer control. In the near u.v and blue part...

  15. Signal and response properties indicate an optoacoustic effect underlying the intra-cochlear laser-optical stimulation

    Science.gov (United States)

    Kallweit, Nicole; Baumhoff, Peter; Krueger, Alexander; Tinne, Nadine; Heisterkamp, Alexander; Kral, Andrej; Maier, Hannes; Ripken, Tammo

    2016-02-01

    Optical cochlea stimulation is under investigation as a potential alternative to conventional electric cochlea implants in treatment of sensorineural hearing loss. If direct optical stimulation of spiral ganglion neurons (SGNs) would be feasible, a smaller stimulation volume and, therefore, an improved frequency resolution could be achieved. However, it is unclear whether the mechanism of optical stimulation is based on direct neuronal stimulation or on optoacoustics. Animal studies on hearing vs. deafened guinea pigs already identified the optoacoustic effect as potential mechanism for intra-cochlear optical stimulation. In order to characterize the optoacoustic stimulus more thoroughly the acoustic signal along the beam path of a pulsed laser in water was quantified and compared to the neuronal response properties of hearing guinea pigs stimulated with the same laser parameters. Two pulsed laser systems were used for analyzing the influence of variable pulse duration, pulse energy, pulse peak power and absorption coefficient. Preliminary results of the experiments in water and in vivo suggesta similar dependency of response signals on the applied laser parameters: Both datasets show an onset and offset signal at the beginning and the end of the laser pulse. Further, the resulting signal amplitude depends on the pulse peak power as well as the temporal development of the applied laser pulse. The data indicates the maximum of the first derivative of power as the decisive factor. In conclusion our findings strengthen the hypothesis of optoacoustics as the underlying mechanism for optical stimulation of the cochlea.

  16. Elimination of Cerenkov interference in a fibre-optic-coupled radiation dosemeter.

    Science.gov (United States)

    Justus, Brian L; Falkenstein, Paul; Huston, Alan L; Plazas, Maria C; Ning, Holly; Miller, Robert W

    2006-01-01

    An optical fibre point dosemeter based on the gated detection of the luminescence from a Cu(1+)-doped fused quartz detector effectively eliminated errors due to Cerenkov radiation and native fibre fluorescence. The gated optical fibre dosemeter overcomes serious problems faced by scintillation and optically stimulated luminescence approaches to optical fibre point dosimetry. The dosemeter was tested using an external beam radiotherapy machine that provided pulses of 6 MV X rays. Gated detection was used to discriminate the signal collected during the radiation pulses, which included contributions from Cerenkov radiation and native fibre fluorescence, from the signal collected between the radiation pulses, which contained only the long-lived luminescence from the Cu(1+)-doped fused quartz detector. Gated detection of the luminescence provided accurate, real-time dose measurements that were linear with absorbed dose, independent of dose rate and that were accurate for all field sizes studied.

  17. Non-Gaussian statistics and optical rogue waves in stimulated Raman scattering.

    Science.gov (United States)

    Monfared, Yashar E; Ponomarenko, Sergey A

    2017-03-20

    We explore theoretically and numerically optical rogue wave formation in stimulated Raman scattering inside a hydrogen filled hollow core photonic crystal fiber. We assume a weak noisy Stokes pulse input and explicitly construct the input Stokes pulse ensemble using the coherent mode representation of optical coherence theory, thereby providing a link between optical coherence and rogue wave theories. We show that the Stokes pulse peak power probability distribution function (PDF) acquires a long tail in the limit of nearly incoherent input Stokes pulses. We demonstrate a clear link between the PDF tail magnitude and the source coherence time. Thus, the latter can serve as a convenient parameter to control the former. We explain our findings qualitatively using the concepts of statistical granularity and global degree of coherence.

  18. Stimulated Brillouin scattering gain bandwidth reduction and applications in microwave photonics and optical signal processing

    Science.gov (United States)

    Preussler, Stefan; Schneider, Thomas

    2016-03-01

    Stimulated Brillouin scattering (SBS) is one of the most dominant nonlinear effects in standard single-mode fibers and its unique spectral characteristics, especially the narrow bandwidth, enable many different applications. Most of the applications would benefit from a narrower bandwidth. Different methods for the bandwidth reduction of SBS in optical fibers are presented and discussed. A bandwidth reduction down to 17% of the natural gain can be achieved by the superposition of the gain with two losses or the utilization of a multistage system. Furthermore, applications in the field of microwave photonics and optical signal processing like high-resolution spectroscopy of communication signals, the storage of optical data packets as well as the processing of frequency combs including generation of millimeter waves and ideal sinc-shaped Nyquist pulses are presented.

  19. Alternating Current Stimulation for Vision Restoration after Optic Nerve Damage: A Randomized Clinical Trial

    Science.gov (United States)

    Schittkowski, Michael P.; Antal, Andrea; Ambrus, Géza Gergely; Paulus, Walter; Dannhauer, Moritz; Michalik, Romualda; Mante, Alf; Bola, Michal; Lux, Anke; Kropf, Siegfried; Brandt, Stephan A.; Sabel, Bernhard A.

    2016-01-01

    Background Vision loss after optic neuropathy is considered irreversible. Here, repetitive transorbital alternating current stimulation (rtACS) was applied in partially blind patients with the goal of activating their residual vision. Methods We conducted a multicenter, prospective, randomized, double-blind, sham-controlled trial in an ambulatory setting with daily application of rtACS (n = 45) or sham-stimulation (n = 37) for 50 min for a duration of 10 week days. A volunteer sample of patients with optic nerve damage (mean age 59.1 yrs) was recruited. The primary outcome measure for efficacy was super-threshold visual fields with 48 hrs after the last treatment day and at 2-months follow-up. Secondary outcome measures were near-threshold visual fields, reaction time, visual acuity, and resting-state EEGs to assess changes in brain physiology. Results The rtACS-treated group had a mean improvement in visual field of 24.0% which was significantly greater than after sham-stimulation (2.5%). This improvement persisted for at least 2 months in terms of both within- and between-group comparisons. Secondary analyses revealed improvements of near-threshold visual fields in the central 5° and increased thresholds in static perimetry after rtACS and improved reaction times, but visual acuity did not change compared to shams. Visual field improvement induced by rtACS was associated with EEG power-spectra and coherence alterations in visual cortical networks which are interpreted as signs of neuromodulation. Current flow simulation indicates current in the frontal cortex, eye, and optic nerve and in the subcortical but not in the cortical regions. Conclusion rtACS treatment is a safe and effective means to partially restore vision after optic nerve damage probably by modulating brain plasticity. This class 1 evidence suggests that visual fields can be improved in a clinically meaningful way. Trial Registration ClinicalTrials.gov NCT01280877 PMID:27355577

  20. Limit of detection of a fiber optics gyroscope using a super luminescent radiation source; Limite de deteccion de un giroscopio de fibra optica usando una fuente de radiacion superluminiscente

    Energy Technology Data Exchange (ETDEWEB)

    Sandoval R, G.E. [Laboratorio de Optica Aplicada, Centro de Ciencias Aplicadas y Desarrollo Tecnologico, Universidad Nacional Autonoma de Mexico, Apartado Postal 70-186, 04510 Mexico D.F. (Mexico); Nikolaev, V.A. [Departamento de Optica y Radiofisica Cuantica, Universidad Estatal de Telecomunicaciones de San Petersburgo, M.A. Bonch-Bruyevich, Kanal Moika 61, Saint Petersburg 191186, (Russian Federation)

    2003-07-01

    The main objective of this work is to establish the dependence of characteristics of the fiber optics gyroscope (FOG) with respect to the parameters of the super luminescent emission source based on doped optical fiber with rare earth elements (Super luminescent Fiber Source, SFS), argument the pumping rate election of the SFS to obtain characteristics limits of the FOG sensibility. By using this type of emission source in the FOG is recommend to use the rate when the direction of the pumping signal coincide with the super luminescent signal. The most results are the proposition and argumentation of the SFS election as emission source to be use in the FOG of the phase type. Such a decision allow to increase the characteristics of the FOG sensibility in comparison with the use of luminescent source of semiconductors emission which are extensively used in the present time. The use of emission source of the SFS type allow to come closer to the threshold of the obtained sensibility limit (detection limit) which is determined with the shot noise. (Author)

  1. Laboratory fading rates of various luminescence signals from feldspar-rich sediment extracts

    DEFF Research Database (Denmark)

    Thomsen, Kristina Jørkov; Murray, A.S.; Jain, Mayank;

    2008-01-01

    ) and optically stimulated luminescence (OSL) signals exhibit anomalous (athermal) fading. Much of the OSL work carried out on feldspars in recent years has focussed on determining fading rates and correcting for them. Almost all work has been carried out using IR stimulation at 50 degrees C detected in the blue...... region of the spectrum. In contrast, we have determined fading rates for various sedimentary feldspar samples using different stimulation and detection windows. If the initial part of the OSL signal is used the lowest fading rate is observed with post-IR blue stimulation (UV detection), but if a later...... part of the signal is used the lowest fading rate is obtained for IR stimulation (blue detection). Daylight bleaching experiments show that, unlike quartz, the initial and final parts of the feldspar OSL signal bleach at approximately the same rate. Stimulation at elevated temperatures significantly...

  2. Optical path of infrared neural stimulation in the guinea pig and cat cochlea

    Science.gov (United States)

    Rajguru, Suhrud M.; Hwang, Margaret; Moreno, Laura E.; Matic, Agnella I.; Stock, Stuart R.; Richter, Claus-Peter

    2011-03-01

    It has been demonstrated previously that infrared neural stimulation (INS) can be used to stimulate spiral ganglion cells in the cochlea. With INS, neural stimulation can be achieved without direct contact of the radiation source and the tissue and is spatially well resolved. The presence of fluids or bone between the target structure and the radiation source may lead to absorption or scattering of the radiation and limit the efficacy of INS. To develop INS based cochlear implants, it is critical to determine the beam path of the radiation in the cochlea. In the present study, we utilized noninvasive X-ray microtomography (microCT) to visualize the orientation and location of the optical fiber within the guinea pig and cat cochlea. Overall, the results indicated that the optical fiber was directed towards the spiral ganglion cells in the cochlea and not the nerve fibers in the center of the modiolus. The fiber was approximately 300 μm away from the target structures. In future studies, results from the microCT will be correlated with physiology obtained from recordings in the midbrain.

  3. Persistent Luminescence Nanophosphor Involved Near-Infrared Optical Bioimaging for Investigation of Foodborne Probiotics Biodistribution in Vivo: A Proof-of-Concept Study.

    Science.gov (United States)

    Liu, Yaoyao; Liu, Jing-Min; Zhang, Dongdong; Ge, Kun; Wang, Peihua; Liu, Huilin; Fang, Guozhen; Wang, Shuo

    2017-09-20

    Probiotics has attracted great attention in food nutrition and safety research field, but thus far there are limited analytical techniques for visualized and real-time monitoring of the probiotics when they are ingested in vivo. Herein, the optical bioimaging technique has been introduced for investigation of foodborne probiotics biodistribution in vivo, employing the near-infrared (NIR) emitting persistent luminescence nanophosphors (PLNPs) of Cr(3+)-doped zinc gallogermanate (ZGGO) as the contrast nanoprobes. The ultrabrightness, super long afterglow, polydispersed size, low toxicity, and excellent photostability and biocompatibility of PLNPs were demonstrated to be qualified as a tracer for labeling probiotics via antibody (anti-Gram positive bacteria LTA antibody) recognition as well as contrast agent for long-term bioimaging the probiotics. In vivo optical bioimaging assay showed that the LTA antibody functionalized ZGGO nanoprobes that could be efficiently tagged to the probiobics were successfully applied for real-time monitoring and nondamaged probing of the biodistribution of probiotics inside the living body after oral administration. This work presents a proof-of-concept that exploited the bioimaging methodology for real-time and nondamaged researching the foodborne probiotics behaviors in vivo, which would open up a novel way of food safety detection and nutrition investigation.

  4. Testing a luminescence surface-exposure dating technique

    Science.gov (United States)

    Gliganic, Luke A.; Meyer, Michael; Gehring, Sebastian

    2016-04-01

    Recent work has shown that the relationship between the luminescence signal (optically stimulated [OSL] and infra-red stimulated [IRSL]) and depth into a rock surface can be used to estimate the length of time since that rock surface has been exposed to sunlight (Sohbati et al., 2012), thus serving as a means for surface-exposure dating. Despite the potential of this new dating tool, few published studies have tested or used this technique. Here, we present the results of two tests of the method. First, we perform laboratory bleaching experiments using two unexposed bedrock samples of different lithologies (granite and quartzite). Sub-samples were bleached for various durations (0 to 100,000 s) in a solar simulator, and IRSL/OSL-depth profiles were measured and fitted using the model of Sohbati et al. (2012). Results of fitting for each sub-sample were then compared. Second, we used a granite boulder from a known age moraine (1850 CE) to test the reproducibility of bleaching depth curves. Multiple cores were collected from the same ~5 cm2 surface area of the boulder, and IRSL-depth profiles were measured and modelled. While our systematic tests confirm the general physical basis of luminescence surface-exposure dating method, we found unexpected scatter in both adjacent bleaching depth curves and the fitting parameters of isochronous rock surfaces for some of our samples. Potential sources of error, including small-scale lithological variabilities and implications for accuracy and precision of the method are discussed. Sohbati, R., Murray, A.S., Chapot, M.S., Jain, M., Pederson, J. (2012) Optically stimulated luminescence (OSL) as a chronometer for surface exposure dating. Journal of Geophysical Research 117 (B9), B09202. doi.org/10.1029/2012JB009383.

  5. Long-term optical stimulation of channelrhodopsin-expressing neurons to study network plasticity

    Science.gov (United States)

    Lignani, Gabriele; Ferrea, Enrico; Difato, Francesco; Amarù, Jessica; Ferroni, Eleonora; Lugarà, Eleonora; Espinoza, Stefano; Gainetdinov, Raul R.; Baldelli, Pietro; Benfenati, Fabio

    2013-01-01

    Neuronal plasticity produces changes in excitability, synaptic transmission, and network architecture in response to external stimuli. Network adaptation to environmental conditions takes place in time scales ranging from few seconds to days, and modulates the entire network dynamics. To study the network response to defined long-term experimental protocols, we setup a system that combines optical and electrophysiological tools embedded in a cell incubator. Primary hippocampal neurons transduced with lentiviruses expressing channelrhodopsin-2/H134R were subjected to various photostimulation protocols in a time window in the order of days. To monitor the effects of light-induced gating of network activity, stimulated transduced neurons were simultaneously recorded using multi-electrode arrays (MEAs). The developed experimental model allows discerning short-term, long-lasting, and adaptive plasticity responses of the same neuronal network to distinct stimulation frequencies applied over different temporal windows. PMID:23970852

  6. Long-term optical stimulation of channelrhodopsin-expressing neurons to study network plasticity

    Directory of Open Access Journals (Sweden)

    Gabriele eLignani

    2013-08-01

    Full Text Available Neuronal plasticity produces changes in excitability, synaptic transmission, and network architecture in response to external stimuli. Network adaptation to environmental conditions takes place in time scales ranging from few seconds to days, and modulates the entire network dynamics. To study the network response to defined long-term experimental protocols, we setup a system that combines optical and electrophysiological tools embedded in a cell incubator. Primary hippocampal neurons transduced with lentiviruses expressing channelrhodopsin-2/H134R were subjected to various photostimulation protocols in a time window in the order of days. To monitor the effects of light-induced gating of network activity, stimulated transduced neurons were simultaneously recorded using multi-electrode arrays. The developed experimental model allows discerning short-term, long-lasting and adaptive plasticity responses of the same neuronal network to distinct stimulation frequencies applied over different temporal windows.

  7. Reproducibility of optically stimulated luminescence measurements from single grains of Al2O3: C and annealed quartz

    DEFF Research Database (Denmark)

    Truscott, A.J.; Duller, G.A.T.; Bøtter-Jensen, L.;

    2000-01-01

    of nine-by-nine holes, which are drilled in the sample disc, We report on tests carried out to determine the precision with which the laser beam can be directed at individual grains in these holes. Single grains of aluminium oxide (Al2O3:C) (90-180 mum) and annealed quartz (90-120 mum) were used to test...

  8. Optically stimulated luminescence dating as a tool for calculating sedimentation rates in Chinese loess: comparisons with grain-size records

    DEFF Research Database (Denmark)

    Stevens, Thomas; Lu, HY

    2009-01-01

    over the late Pleistocene and Holocene. The results demonstrate that sedimentation rates are site specific, extremely variable over millennial timescales and that this variation is often not reflected in grain-size changes. In the central part of the Loess Plateau, the relationship between grain...

  9. Introduction of a new dosimetry system based on optically stimulated luminescence (OSL) in our personal monitoring service

    Energy Technology Data Exchange (ETDEWEB)

    Hubner, S., E-mail: stephan.huebner@helmholtz-muenchen.de [Helmholtz Zentrum Munchen, German Research Center for Environmental Health, D-80219, Munich (Georgia)

    2014-08-15

    The personal monitoring service named Auswertungsstelle is part of the Helmholtz Zentrum Munchen, a non-profit-making research center in Germany. As one of the four monitoring services in Germany, we have been a reliable partner in radiation protection for more than 60 years. With about 1.9 million dose assessments per year, we are the largest monitoring service in Europe. For dozens of years, our main dosimeter used in whole-body dosimetry has been a film dosimeter. Although its dosimetric properties are still up to date, film dosimetry won.t be a sustainable technique for the use in monitoring services. Therefore, a project with the objective of investigating alternative dosimetric materials and methods was launched in the late 1990 at the Helmholtz Zentrum Munchen. Based on this research work, the use of Be O as an OSL dosimeter was studied by the radiation physics group of the Tu Dresden, by order and on account of the Auswertungsstelle at the Helmholtz Zentrum Munchen. It was shown, that ceramic Be O features promising dosimetric properties, making Be O detectors particularly suitable for being used in all applications in whole-body dosimetry measuring photons. Ceramic Be O material has an excellent resistance to environmental influences. The Be O chips are almost tissue equivalent. Therefore, these detectors show low photon energy dependence. A new personal dosimetry system based on the OSL dosimetry of Be O was developed. Applying this system, the Auswertungsstelle offers OSL-dosimeters for official monitoring of the Personal Dose Equivalent Hp(10) since 2011. This OSL-System is accredited according to DIN IEC 62387 and we obtained the corresponding type approval by the Ptb, the national metrology institute in Germany. Sophisticated logistics was developed and installed. High degree of automation was achieved by robots for dosimeter assembly and machines for packing, labelling and unpacking of the dosimeters. To become a sustainable dosimetry system not only appropriate dosimetric properties and perfect logistics are required. The new OSL system needs to be well established in personal dosimetry in order to ensure substantial maintenance and further development of the system. As at January 2014, already six monitoring services scattered all over the world are carrying out personal dosimetry using these OSL-Systems. According to respective national regulations both personal dose equivalents Hp(10) and Hp(0.07) can be measured. To meet that essential target to continuously increase the market share, a subsidiary company called Dosimetric s was launched in 2013 with the objective of performing the related commercial business, such as promotion and selling as well as ensuring further development and maintenance of the OSL-system. (Author)

  10. Paleoseismology of the Mejillones Fault, northern Chile: Insights from cosmogenic 10Be and optically stimulated luminescence determinations

    Science.gov (United States)

    CortéS A., J.; GonzáLez L., Gabriel; Binnie, S. A.; Robinson, R.; Freeman, S. P. H. T.; Vargas E., G.

    2012-04-01

    We have undertaken the first paleoseismological study on an upper plate fault in Chile. The selected structure was the Mejillones Fault, which is marked by a conspicuous fault-scarp. Using cosmogenic 10Be and OSL dating and detailed sedimentary logging of trenches, we have constrained the abandonment of two alluvial surfaces by fault activity at ca. 35 ka and ca.14 ka. Based on stratigraphic observation we characterized the fault evolution in four intervals over the last ca. 35 ka. During the first three intervals the fault had a steady slip rate of 0.61 ± 0.26 m/ka. The fourth interval is delineated by the last vertical fault slip and the accumulation of un-deformed hillslope deposits after ca. 3.3 ka and has a slip rate of 0.22 ± 0.06 m/ka. The younger surface abandonment was caused by two Mw ˜ 7 paleoearthquakes with a recurrence interval of 5.0 ± 3.5 ka. The third interval is characterized by the interaction of hillslope deposits and aseismic slip and/or centimeter scale seismic slip events. At ca. 3.5 ka, a last large (Mw ˜ 6.6) earthquake took place. The recurrence intervals of large (Mw > 8.5) subduction earthquakes do not appear to be the same as the recurrence intervals of the Mw ˜ 7 events on the upper plate Mejillones Fault.

  11. Late Quaternary floods and droughts in the Nile valley, Sudan: new evidence from optically stimulated luminescence and AMS radiocarbon dating

    Science.gov (United States)

    Williams, M. A. J.; Williams, F. M.; Duller, G. A. T.; Munro, R. N.; El Tom, O. A. M.; Barrows, T. T.; Macklin, M.; Woodward, J.; Talbot, M. R.; Haberlah, D.; Fluin, J.

    2010-05-01

    Our results show that the late Pleistocene Nile in northern Sudan was shifting position and actively aggrading at 145 ± 20 kyr, 83 ± 24 kyr, 32 ± 8 kyr and 20.7 ± 0.2 kyr and indicate, for the first time, a phase of high-energy flow in the White Nile at 27.8 ± 3.2 kyr, with still high but somewhat reduced flow in that river at 13.3 kyr, 10 kyr and 4.8-4.0 kyr. Beach ridges associated with a 386 m strandline of the White Nile have OSL ages of 27.5 ± 2.7 kyr and 14.5 ± 1.6 kyr. The Holocene terraces and former channels of the main Nile have ages of 11 kyr, 6.5-5.0 kyr and 4.8-4.0 kyr, after which there was a general decline in flood discharge. The now arid main Nile valley in northern Sudan was significantly wetter during the early to middle Holocene, with a lake up to 450 km 2 in area, fed by an overflow channel from the early Holocene Nile between 9.5 kyr and 7.5 kyr. Previously stable late Pleistocene dunes were reactivated at intervals during the Holocene, with five samples from the White Nile valley indicating brief phases of Holocene dune activity at 9.9 ± 2.0 kyr, 9.0 ± 2.8 kyr, 6.6 ± 0.9 kyr, 4.8 ± 0.9 kyr and 2.9 ± 0.5 kyr, the earliest of which occurred within periods of generally wetter climate and higher Nile flow. The youngest freshwater shells on the Khor Abu Habl alluvial fan west of the White Nile correspond to a time of regionally wetter climate between 1.7 and 1.0 kyr. Our results suggest that millennial scale climatic instability may have been characteristic of Holocene climates in this region.

  12. Jak/Stat Signaling Stimulates Zebrafish Optic Nerve Regeneration and Overcomes the Inhibitory Actions of Socs3 and Sfpq

    Science.gov (United States)

    Elsaeidi, Fairouz; Bemben, Michael A.; Zhao, Xiao-Feng

    2014-01-01

    The regenerative failure of mammalian optic axons is partly mediated by Socs3-dependent inhibition of Jak/Stat signaling (Smith et al., 2009, 2011). Whether Jak/Stat signaling is part of the normal regenerative response observed in animals that exhibit an intrinsic capacity for optic nerve regeneration, such as zebrafish, remains unknown. Nor is it known whether the repression of regenerative inhibitors, such as Socs3, contributes to the robust regenerative response of zebrafish to optic nerve damage. Here we report that Jak/Stat signaling stimulates optic nerve regeneration in zebrafish. We found that IL-6 family cytokines, acting via Gp130-coupled receptors, stimulate Jak/Stat3 signaling in retinal ganglion cells after optic nerve injury. Among these cytokines, we found that CNTF, IL-11, and Clcf1/Crlf1a can stimulate optic axon regrowth. Surprisingly, optic nerve injury stimulated the expression of Socs3 and Sfpq (splicing factor, proline/glutamine rich) that attenuate optic nerve regeneration. These proteins were induced in a Jak/Stat-dependent manner, stimulated each other's expression and suppressed the expression of regeneration-associated genes. In vivo, the injury-dependent induction of Socs3 and Sfpq inhibits optic nerve regeneration but does not block it. We identified a robust induction of multiple cytokine genes in zebrafish retinal ganglion cells that may contribute to their ability to overcome these inhibitory factors. These studies not only identified mechanisms underlying optic nerve regeneration in fish but also suggest new molecular targets for enhancing optic nerve regeneration in mammals. PMID:24523552

  13. Inflammatory stimulation preserves physiological properties of retinal ganglion cells after optic nerve injury

    Directory of Open Access Journals (Sweden)

    Henrike eStutzki

    2014-02-01

    Full Text Available Axonal injury in the optic nerve is associated with retinal ganglion cell (RGC degeneration and irreversible loss of vision. However, inflammatory stimulation (IS by intravitreal injection of Pam3Cys transforms RGCs into an active regenerative state enabling these neurons to survive injury and to regenerate axons into the injured optic nerve. Although morphological changes have been well studied, the functional correlates of RGCs transformed either into a de- or regenerating state at a sub-cellular level remain unclear. In the current study, we investigated the signal propagation in single intraretinal axons as well as characteristic activity features of RGCs in a naive, a degenerative or a regenerative state in ex vivo retinae one week after either optic nerve cut alone (ONC or additional inflammatory stimulation (ONC+IS. Recordings of single RGCs using high-density microelectrode arrays demonstrate that the mean intraretinal axonal conduction velocity significantly decreased within the first week after ONC. In contrast, when ONC was accompanied by regenerative Pam3Cys treatment the mean intraretinal velocity was undistinguishable from control RGCs, indicating a protective effect on the proximal axon. Spontaneous RGC activity decreased for the two most numerous RGC types (ON- and OFF-sustained cells within one post-operative week, but did not significantly increase in RGCs after inflammatory stimulation. The analysis of light-induced activity revealed that RGCs in ONC animals respond on average later and with fewer spikes than control RGCs. IS significantly improved the responsiveness of the two studied RGC types.These results show that the transformation into a regenerative state by IS preserves, at least transiently, the physiological functional properties of injured RGCs.

  14. Luminescence and structural properties of oxyorthosilicate and Al2O3 nanophosphors

    Energy Technology Data Exchange (ETDEWEB)

    Blair, Michael W [Los Alamos National Laboratory; Jacobsohn, Luiz G [Los Alamos National Laboratory; Bennett, Bryan L [Los Alamos National Laboratory; Tornga, Stephanie C [Los Alamos National Laboratory; Muenchausen, Ross E [Los Alamos National Laboratory; Yukihara, Eduardo G [OK STATE

    2008-01-01

    A large amount of research has been conducted on semiconducting quantum dots exploring quantum confinement effects. On the other hand, nanophosphors -- inorganic insulating nanostructured luminescent materials -- have received considerably less attention. Our research involving nanomaterials has then focused on the question: How does reduced dimensionality affect the physical and chemical behavior of nanophosphors? In order to partially answer this fundamental question, we have produced numerous oxides, among them Lu{sub 2}SiO{sub 5}Ce (LSO), Y{sub 2}SiO{sub 5}:Ce (YSO), Gd{sub 2}SiO{sub 5}:Ce (GSO), and Al{sub 2}O{sub 3}, and characterized their structural and luminescent properties. Structure, grain size, phase purity and chemical homogeneity in the nanoscale were determined using x-ray diffraction, transmission electron microscopy, and electron paramagnetic resonance. The luminescent properties of the nanophosphors were characterized by thermoluminescence, radioluminescence, photoluminescence, and optically stimulated luminescence. In this work, we present an overview of the nascent field of nanophosphors, and summarize the results obtained in our laboratory with particular emphasis on the luminescent properties.

  15. Interplay between chromium content and lattice disorder on persistent luminescence of ZnGa{sub 2}O{sub 4}:Cr{sup 3+} for in vivo imaging

    Energy Technology Data Exchange (ETDEWEB)

    Sharma, Suchinder K.; Bessière, Aurelie [Institut de Recherche de Chimie-Paris, CNRS – Chimie-ParisTech, 11 rue Pierre et Marie Curie, 75005 Paris (France); Basavaraju, Neelima; Priolkar, Kaustubh R. [Department of Physics, Goa University, Goa 403206 (India); Binet, Laurent; Viana, Bruno [Institut de Recherche de Chimie-Paris, CNRS – Chimie-ParisTech, 11 rue Pierre et Marie Curie, 75005 Paris (France); Gourier, Didier, E-mail: didier.gourier@chimie-paristech.fr [Institut de Recherche de Chimie-Paris, CNRS – Chimie-ParisTech, 11 rue Pierre et Marie Curie, 75005 Paris (France)

    2014-11-15

    In the quest of bright and long persistent far-red/near-infrared phosphors for in vivo optical imaging, the interest in the family of ZnGa{sub 2}O{sub 4} spinel compounds doped with Cr{sup 3+} has been aroused in the most recent years. We show that the dopant concentration plays an important role in the total persistent luminescence output of the material. ZnGa{sub 2}O{sub 4} doped with 0.25%, 0.50% and 0.75% Cr relative to (Ga+Cr) was prepared by solid state synthesis. 0.50% Cr was found optimal to obtain the most intense persistent luminescence after matrix excitation with X-rays or localized excitation in Cr{sup 3+} absorption band with 550 nm wavelength. Up to 0.5% Cr content, persistent luminescence increases as a consequence of an increased number of Cr{sup 3+} luminescent centers and associated defects. With 0.75% Cr content, a too large number of defects locally concentrated around Cr{sup 3+} ions are detrimental to the long-term persistent luminescence intensity. We supplement long lasting phosphorescence investigation with laser excited photoluminescence and thermally stimulated luminescence results. - Highlights: • The red persistent luminescence of ZnGa{sub 2}O{sub 4}:Cr is optimum for 0.50% Cr{sup 3+} doping. • Higher doping introduces lattice disorder. • The phenomenon is studied by correlating photoluminescence, EPR and thermoluminescence.

  16. Application of pulsed OSL to the separation of the luminescence components from a mixed quartz/feldspar sample

    DEFF Research Database (Denmark)

    Denby, Phil M.; Bøtter-Jensen, L.; Murray, A.S.

    2006-01-01

    this stimulation source, and hi.-h-speed photon timing, the OSL yield can be monitored throughout the pulsing cycle and subsequent OSL decay. It is found that the total photon yield per unit stimulation power in pulsed mode is, for quartz, twice and, for feldspar, nearly four times, that in continuous wave mode......It is known that the pulsed optically stimulated luminescence (OSL) characteristics of quartz and feldspars are very different. These differences can be used to preferentially discriminate against the feldspar signal in mixed quartz\\feldspar mineral assemblages, or in separated quartz contaminated...

  17. Evaluation of Effects of Electrical Stimulation in the Retina with Optical Coherence Tomography*

    Science.gov (United States)

    Gonzalez-Calle, A.; Weiland, J.D.

    2017-01-01

    Retinal prostheses provide the capability to blind patients to detect motion and locate large objects. To avoid activating axons of passage, which can create streak-like perceptions, long pulse stimulation can be used to bypass axons and achieve focal retinal activation. Safety is a concern because long pulses require more charge than short pulses to elicit a response from neural tissue. Future implants will require smaller electrodes to improve resolution, but increased charge density may result, which is another safety concern. We developed a method to study the effects of electrical stimulation in the retina in real time using OCT (Optical Coherence Tomography) imaging combined with micropositioning of a stimulating electrode over the retina in an animal model. When using a 250-micron diameter electrode and stimulating for 30 minutes (frequency: 333 Hz), charge density: 1.22 mC/cm2, we observed an increase in retinal thickness from 154.3 μm ± 7.04 μm to 179.67 μm ± 0.47μm, a 16.66 % ± 5.49% increase compared to baseline. The region of increased thickness extended laterally for 0.56 mm ± 0.009 mm. When stimulating with a charge density of 1.63 mC/cm2, we observed an increase in retinal thickness from 160.3 μm ± 2.05 μm to 190 μm ± 0.81μm, a 19.52 % ± 1.86% increase compared to baseline. The region of increased thickness expanded laterally for 1.27 mm ± 0.19 mm. PMID:28261012

  18. Evaluation of Effects of Electrical Stimulation in the Retina with Optical Coherence Tomography.

    Science.gov (United States)

    Gonzalez-Calle, A; Weiland, J D

    2016-08-01

    Retinal prostheses provide the capability to blind patients to detect motion and locate large objects. To avoid activating axons of passage, which can create streak-like perceptions, long pulse stimulation can be used to bypass axons and achieve focal retinal activation. Safety is a concern because long pulses require more charge than short pulses to elicit a response from neural tissue. Future implants will require smaller electrodes to improve resolution, but increased charge density may result, which is another safety concern. We developed a method to study the effects of electrical stimulation in the retina in real time using OCT (Optical Coherence Tomography) imaging combined with micropositioning of a stimulating electrode over the retina in an animal model. When using a 250-micron diameter electrode and stimulating for 30 minutes (frequency: 333 Hz), charge density: 1.22 mC/cm(2), we observed an increase in retinal thickness from 154.3 μm ± 7.04 μm to 179.67 μm ± 0.47μm, a 16.66 % ± 5.49% increase compared to baseline. The region of increased thickness extended laterally for 0.56 mm ± 0.009 mm. When stimulating with a charge density of 1.63 mC/cm(2), we observed an increase in retinal thickness from 160.3 μm ± 2.05 μm to 190 μm ± 0.81μm, a 19.52 % ± 1.86% increase compared to baseline. The region of increased thickness expanded laterally for 1.27 mm ± 0.19 mm.

  19. Investigation of linear optical absorption coefficients in core-shell quantum dot (QD) luminescent solar concentrators (LSCs)

    Science.gov (United States)

    Ebrahimipour, Bahareh Alsadat; Askari, Hassan Ranjbar; Ramezani, Ali Behjat

    2016-09-01

    The interlevel absorption coefficient of CdSe/ZnS and ZnS/CdSe core-shell Quantum Dot (QD) in luminescent solar concentrators (LSCs) is reported. By considering the quantum confinement effects, the wave functions and eigenenergies of electrons in the nonperturebative system consists of a core-shell QD have been numerically calculated under the frame work of effective-mass approximation by solving a three-dimensional Schrӧdinger equation. And then the absorption coefficient is obtained under density matrix approximation considering in the polymer sheets of the concentrator including the core-shell QDs. The effect of the hetero-structure geometry upon the energy spectrum and absorption coefficient associated to interlevel transitions was also considered. The results show that the core-shell QDs can absorb the photons with higher energy in solar spectrum as compared to the inverted core-shell. And with a small shell layer diameter, the core-shell QDs produce larger linear absorption coefficients and consequently higher efficiency values, however it is inversed for inverted core-shell QDs. The work described here gives a detailed insight into the promise of QD-based LSCs and the optoelectronic devices applications.

  20. Luminescence dating of aeolian sands from archaeological sites in Northern Britain: a preliminary study

    Science.gov (United States)

    Sommerville, A. A.; Sanderson, D. C. W.; Hansom, J. D.; Housley, R. A.

    2001-12-01

    Luminescence dating of aeolian sands from archaeological sites has potential to contribute to regional chronologies for sediment deposition and to provide a greater understanding of climatic influences on early communities. The Northern and Western Isles of Scotland provide important opportunities for sampling archaeologically intercalated sands for these purposes, and to provide constrained samples for method validation. A wide range of modern beaches have been sampled in the Western and Orkney Isles of Scotland to examine regional variations in luminescence sensitivity, residuals and ease of bleaching. These modern sands have negligible residuals for infra-red stimulated luminescence (IRSL), small optically stimulated luminescence (OSL) residuals and significant thermoluminescence residuals. The relationship between these signals and laboratory bleaching results may indicate the initial depositional environment, and hence lead to a means of identifying well-bleached dating samples. Both sensitivities and residuals show regional differences, reflecting local geology. Preliminary ages obtained from aeolian sands associated with archaeological sites at Amble (Northumbria) and Tofts Ness (Sanday, Orkney) using regenerative blue OSL techniques on extracted quartz are broadly consistent with external age controls from the first and third millennium BC.

  1. Optical processes in the formation of stimulated emission from ZnO nanowires

    Institute of Scientific and Technical Information of China (English)

    Liu Rui-Bin; Pan An-Lian; Wang Fei-Fei; Zou Bing-Suo

    2007-01-01

    This paper studies power dependent photoluminescence spectra, the stimulated emission occurring at ultraviolet (UV) band instead of the green emission band of ZnO nanowires, which are prepared with a chemical reduction method.The dynamics of the UV emission and green emission is given to demonstrate the reason of stimulated emission occurring at UV band but not the green emission band under high excitation, which indicates that the slow decay rate of trap state makes it easy to be fully filled and saturated, while the fast decay rate of near-band-edge exciton state makes the UV emission dominate the radiative recombination under high excitation. The UV emission, as well as the corresponding stimulated emission, occurs in competition with the green deep-trap emission. In addition, when pump fluence further increases, the multiple lasing modes appear. The dependence of these lasing modes on the pump fluence is first discussed.This diagram should be helpful to understand and design the optical nanodevices of ZnO nanowires.

  2. Transcorneal electrical stimulation alters morphology and survival of retinal ganglion cells after optic nerve damage.

    Science.gov (United States)

    Henrich-Noack, Petra; Voigt, Nadine; Prilloff, Sylvia; Fedorov, Anton; Sabel, Bernhard A

    2013-05-24

    Traumatic optic nerve injury leads to retrograde death of retinal ganglion cells (RGCs), but transcorneal electrical stimulation (TES) can increase the cell survival rate. To understand the mechanisms and to further define the TES-induced effects we monitored in living animals RGC morphology and survival after optic nerve crush (ONC) in real time by using in vivo confocal neuroimaging (ICON) of the retina. ONC was performed in rats and ICON was performed before crush and on post-lesion days 3, 7 and 15 which allowed us to repeatedly record RGC number and size. TES or sham-stimulation were performed immediately after the crush and on post-injury day 11. Three days after ONC we detected a higher percentage of surviving RGCs in the TES group as compared to sham-treated controls. However, the difference was below significance level on day 7 and disappeared completely by day 15. The death rate was more variable amongst the TES-treated rats than in the control group. Morphological analysis revealed that average cell size changed significantly in the control group but not in stimulated animals and the morphological alterations of surviving neurons were smaller in TES-treated compared to control cells. In conclusion, TES delays post-traumatic cell death significantly. Moreover, we found "responder animals" which also benefited in the long-term from the treatment. Our in vivo cellular imaging results provide evidence that TES reduces ONC-associated neuronal swelling and shrinkage especially in RGCs which survived long-term. Further studies are now needed to determine the differences of responders vs. non-responders.

  3. Dose response of hydrazine - Deproteinated tooth enamel under blue light stimulation

    Energy Technology Data Exchange (ETDEWEB)

    Yuece, Ulkue Rabia, E-mail: ulkuyuce@hotmail.co [Ankara University, Faculty of Engineering, Department of Engineering Physics, 06100, Tandogan - Ankara (Turkey); Meric, Niyazi, E-mail: meric@ankara.edu.t [Ankara University, Faculty of Engineering, Department of Engineering Physics, 06100, Tandogan - Ankara (Turkey); Atakol, Orhan, E-mail: atakol@science.ankara.edu.t [Ankara University, Science Faculty, Department of Chemistry, 06100, Tandogan - Ankara (Turkey); Yasar, Fusun, E-mail: ab121310@adalet.gov.t [Council of Forensic Medicine, Ankara Branch, Ankara (Turkey)

    2010-08-15

    The beta dose response and Optically Stimulated Luminescence (OSL) signal stability characteristics of human tooth enamel deproteinated by hydrazine reagent under blue photon stimulation are reported. Removal of the protein organic component of tooth enamel resulted in a higher OSL sensitivity and slower fading of OSL signals. The effect of chemical sample preparation on the enamel sample sensitivity is discussed and further steps to make this deproteinization treatment suitable for in vitro dose reconstruction studies are suggested.

  4. Long-persistent luminescence in the near-infrared from Nd3+-doped Sr2SnO4 for in vivo optical imaging

    Science.gov (United States)

    Kamimura, Sunao; Xu, Chao-Nan; Yamada, Hiroshi; Terasaki, Nao; Fujihala, Masayoshi

    2014-09-01

    We discovered a new near-infrared (NIR) persistent luminescent material Sr2SnO4:Nd3+, which exhibited NIR luminescence ranging from 850 to 1400 nm. Furthermore, we successfully enhanced the intensity of NIR persistent luminescence by increasing the firing temperature. The intensity of NIR persistent luminescence, which penetrates through a human finger and can be used to visualize a finger vein pattern by using a charge-coupled device camera, reached approximately 1.1 mW/m2 (λ = 900 nm) at a decay time of 10 s after ceasing the excitation. We proposed the enhancement process of the NIR persistent luminescence for Sr2SnO4:Nd3+ in conjunction with photoluminescence, absorption, thermoluminescence, and structural properties.

  5. Stochastic optical reconstruction microscopy (STORM) in comparison with stimulated emission depletion (STED) and other imaging methods.

    Science.gov (United States)

    Tam, Johnny; Merino, David

    2015-11-01

    Stochastic optical reconstruction microscopy (STORM) and stimulated emission depletion (STED) microscopy are two super-resolution optical microscopy approaches that have rapidly gained popularity in recent years. Both modalities offer super-resolution imaging capabilities with the potential for imaging in multiple colors, three-dimensions, and the possibility to image in live cells. In this review, we focus on the specific advantages and disadvantages of each technique in the context of each other. STORM has been reported to achieve higher spatial resolution when compared to STED, but a lengthy acquisition may be required. STED utilizes relatively higher laser intensities, but is able to generate a super-resolution image immediately after acquisition without the need for any additional data processing. Ultimately, the choice between STORM and STED will depend not only on the specific application, but also on the users' ability to understand and optimize the various parameters ranging from sample preparation to image acquisition, which determine the quality of the final image. Stochastic optical reconstruction microscopy (STORM) and stimulated emission depletion (STED) are two super-resolution microscopy approaches that have rapidly gained popularity in recent years. STORM is based on the precise localization of a large number of individual molecules that together form a super-resolved image (bottom), whereas STED is based on the scanning of two super-imposed light sources which together allow for a super-resolved spot on the sample to be imaged (top). We discuss the specific advantages and disadvantages of each technique and explain the various parameters that affect image quality, which should be taken into consideration when planning experiments.

  6. [3+3] Cyclocondensation of Disubstituted Biphenyl Dialdehydes: Access to Inherently Luminescent and Optically Active Hexa-substituted C3-Symmetric and Asymmetric Trianglimine Macrocycles.

    Science.gov (United States)

    Wang, Zhenzhen; Nour, Hany F; Roch, Loïc M; Guo, Minjie; Li, Wenjiao; Baldridge, Kim K; Sue, Andrew C H; Olson, Mark A

    2017-03-03

    A general synthetic route to inherently luminescent and optically active 6-fold substituted C3-symmetric and asymmetric biphenyl-based trianglimines has been developed. The synthesis of these hexa-substituted triangular macrocycles takes advantage of a convenient method for the synthesis of symmetrically and asymmetrically difunctionalized biphenyl dialdehydes through a convergent two-step aromatic nucleophilic substitution-one-pot Suzuki-coupling reaction protocol. A modular [3+3] diamine-dialdehyde cyclocondensation reaction between both the symmetrically and asymmetrically difunctionalized-4,4'-biphenyldialdehydes with enantiomerically pure (1R,2R)-1,2-diaminocyclohexane was employed to construct the hexa-substituted triangular macrocycles. B97-D/6-311G(2d,p) density functional theory determined structures and X-ray crystallographic analysis reveal that the six substituents appended to the biphenyl legs of the trianglimine macrocycles adopt an alternating conformation not unlike the 1,3,5-alternate conformation observed for calix[6]arenes. Reduction of the imine bonds using NaBH4 afforded the corresponding 6-fold substituted trianglamine without the need to alkylate the amine nitrogen atoms which could hinder their later use as metal coordination sites and without having to introduce asymmetric carbons.

  7. Luminescence imaging using radionuclides: a potential application in molecular imaging

    Energy Technology Data Exchange (ETDEWEB)

    Park, Jeong Chan [Department of Molecular Medicine, School of Medicine, Kyungpook National University, Daegu 700-422 (Korea, Republic of); Il An, Gwang [Molecular Imaging Research Center, Korea Institute of Radiological and Medical Sciences, Seoul 139-706 (Korea, Republic of); Park, Se-Il [Department of Molecular Medicine, School of Medicine, Kyungpook National University, Daegu 700-422 (Korea, Republic of); Oh, Jungmin [Korea Basic Science Institute Chuncheon Center, Gangwon-do 200-701 (Korea, Republic of); Kim, Hong Joo [Department of Physics and Energy Science, Kyungpook National University, Daegu 702-710 (Korea, Republic of); Su Ha, Yeong; Wang, Eun Kyung [Department of Molecular Medicine, School of Medicine, Kyungpook National University, Daegu 700-422 (Korea, Republic of); Min Kim, Kyeong; Kim, Jung Young [Molecular Imaging Research Center, Korea Institute of Radiological and Medical Sciences, Seoul 139-706 (Korea, Republic of); Lee, Jaetae [Department of Nuclear Medicine, School of Medicine, Kyungpook National University, Daegu 700-422 (Korea, Republic of); Welch, Michael J. [Department of Radiology, Washington University School of Medicine, St. Louis, MO 63110 (United States); Yoo, Jeongsoo, E-mail: yooj@knu.ac.k [Department of Molecular Medicine, School of Medicine, Kyungpook National University, Daegu 700-422 (Korea, Republic of)

    2011-04-15

    Introduction: Nuclear and optical imaging are complementary in many aspects and there would be many advantages when optical imaging probes are prepared using radionuclides rather than classic fluorophores, and when nuclear and optical dual images are obtained using single imaging probe. Methods: The luminescence intensities of various radionuclides having different decay modes have been assayed using luminescence imaging and in vitro luminometer. Radioiodinated Herceptin was injected into a tumor-bearing mouse, and luminescence and microPET images were obtained. The plant dipped in [{sup 32}P]phosphate solution was scanned in luminescence mode. Radio-TLC plate was also imaged in the same imaging mode. Results: Radionuclides emitting high energy {beta}{sup +}/{beta}{sup -} particles showed higher luminescence signals. NIH3T6.7 tumors were detected in both optical and nuclear imaging. The uptake of [{sup 32}P]phosphate in plant was easily followed by luminescence imaging. Radio-TLC plate was visualized and radiochemical purity was quantified using luminescence imaging. Conclusion: Many radionuclides with high energetic {beta}{sup +} or {beta}{sup -} particles during decay were found to be imaged in luminescence mode due mainly to Cerenkov radiation. 'Cerenkov imaging' provides a new optical imaging platform and an invaluable bridge between optical and nuclear imaging. New optical imaging probes could be easily prepared using well-established radioiodination methods. Cerenkov imaging will have more applications in the research field of plant science and autoradiography.

  8. Optical limiting effect based on stimulated Brillouin scattering in CCl4

    Institute of Scientific and Technical Information of China (English)

    LueZhi-Wei; LueYue-Lan; YangJun

    2003-01-01

    The optical limiting effect based on stimulated Brillouin scattering(SBS) in a nonlinear medium was investigated. We numerically treated the nonlinear propagation process with a theoretical model, which includes the spontansous nature of the initiation of SBS, and obtained optical limiting effect in the process. Energy limiting,pulse reshaping and stabilization have been demonstrated on SBS mechanism with the nonlinear medium CCl4. The input optical signals were Nd:YAG nanosecond laser pulses with width varying from 16ns to 7ns then to 2ns, the relationship between the transmitted signal and launched pump signal was shown. In the experimental regime, the most stable pulse the transmitted signal and launched pump signal was shown. In the experimental regime, the most stable pulse and a superior energy stabilization of the transmitted pulse were obtained when the laser pulse-width became as short as 2ns. For the energy variation of laser pulses in a wide range of 14-88mJ, the output energy was limited in a quite narrow range 4.5-5.5mJ.

  9. Up-conversion luminescence and optical temperature sensing behaviour of Yb3+/Er3+ codoped CaWO4 material

    Science.gov (United States)

    Cheng, Xuerui; Yang, Kun; Wang, Jiankun; Yang, Linfu; Cheng, Xiaoshuai

    2016-08-01

    Present article report on structural and optical properties of Er3+/Yb3+ codoped CaWO4 phosphors. Structural properties are explored using XRD and Raman technologies. The upconversion emission has been investigated with 980 nm excitation. The upconversion emission intensity is dependent on the concentrations of Yb3+ ions and reaches a maximum at 7%. Logarithmic plots of power dependencies reveal that the green and red emissions originate from a two-photon upconversion process. Based on the photon energy and the emission spectra, the possible upconversion processes and emission mechanisms are discussed. Finally, the optical temperature sensing properties has been performed using the fluorescence intensity ratio technique based on green upconversion emissions. Its temperature sensitivity is found to be above 0.0025 K-1 in the whole temperature range of 300-540 K, revealing this phosphor to be a promising optical temperature sensing material.

  10. Multifunctionality in bimetallic Ln(III)[W(V)(CN)8]3- (Ln = Gd, Nd) coordination helices: optical activity, luminescence, and magnetic coupling.

    Science.gov (United States)

    Chorazy, Szymon; Nakabayashi, Koji; Arczynski, Mirosław; Pełka, Robert; Ohkoshi, Shin-ichi; Sieklucka, Barbara

    2014-06-02

    Two chiral luminescent derivatives of pyridine bis(oxazoline) (Pybox), (SS/RR)-iPr-Pybox (2,6-bis[4-isopropyl-2-oxazolin-2-yl]pyridine) and (SRSR/RSRS)-Ind-Pybox (2,6-bis[8H-indeno[1,2-d]oxazolin-2-yl]pyridine), have been combined with lanthanide ions (Gd(3+), Nd(3+)) and octacyanotungstate(V) metalloligand to afford a remarkable series of eight bimetallic CN(-)-bridged coordination chains: {[Ln(III)(SS/RR-iPr-Pybox)(dmf)4]3[W(V)(CN)8]3}n ⋅dmf⋅4 H2O (Ln = Gd, 1-SS and 1-RR; Ln = Nd, 2-SS and 2-RR) and {[Ln(III)(SRSR/RSRS-Ind-Pybox)(dmf)4][W(V)(CN)8]}n⋅5 MeCN⋅4 MeOH (Ln = Gd, 3-SRSR and 3-RSRS; Ln = Nd, 4-SRSR and 4-RSRS). These materials display enantiopure structural helicity, which results in strong optical activity in the range 200-450 nm, as confirmed by natural circular dichroism (NCD) spectra and the corresponding UV/Vis absorption spectra. Under irradiation with UV light, the Gd(III)-W(V) chains show dominant ligand-based red phosphorescence, with λmax ≈660 nm for 1-(SS/RR) and 680 nm for 3-(SRSR/RSRS). The Nd(III)-W(V) chains, 2-(SS/RR) and 4-(SRSR/RSRS), exhibit near-infrared luminescence with sharp lines at 986, 1066, and 1340 nm derived from intra-f (4)F3/2 → (4)I9/2,11/2,13/2 transitions of the Nd(III) centers. This emission is realized through efficient ligand-to-metal energy transfer from the Pybox derivative to the lanthanide ion. Due to the presence of paramagnetic lanthanide(III) and [W(V)(CN)8](3-) moieties connected by cyanide bridges, 1-(SS/RR) and 3-(SRSR/RSRS) are ferrimagnetic spin chains originating from antiferromagnetic coupling between Gd(III) (SGd = 7/2) and W(V) (SW = 1/2) centers with J1-(SS) = -0.96(1) cm(-1), J1-(RR) =-0.95(1) cm(-1), J3-(SRSR) = -0.91(1) cm(-1), and J3-(RSRS) =-0.94(1) cm(-1). 2-(SS/RR) and 4-(SRSR/RSRS) display ferromagnetic coupling within their Nd(III)-NC-W(V) linkages.

  11. Characteristics of stimulated emission from optically pumped freestanding GaN grown by hydride vapor-phase epitaxy

    CERN Document Server

    Lee, M H; Kim, S T; Chung, S H; Moon, D C

    1999-01-01

    In this study, we observed optically pumped stimulated emission at room temperature in quasi-bulk GaN prepared from thick-film GaN grown on a sapphire substrate by using hydride vapor-phase epitaxy and subsequent mechanical removal of the sapphire substrate. The stimulated emission from the surface and 1-mm-wide-cleaved cavity of the GaN was red-shifted compared to the spontaneous emission by increasing the optical pumping-power density, and the full width at half maximum (FWHM) of the peak decreased. The stimulated emission was demonstrated to have a highly TE-mode polarized nature, and the super-linear dependence of the integrated emission intensity on the excitation power indicated a threshold pump-power density of I sub t sub h = 2 MW/cm sup 2 for one set of stimulated emissions.

  12. New Opportunities for Lanthanide Luminescence

    Institute of Scientific and Technical Information of China (English)

    Jean-Claude G. Bünzli; Steve Comby; Anne-Sophie Chauvin; Caroline D. B. Vandevyver

    2007-01-01

    Trivalent lanthanide ions display fascinating optical properties. The discovery of the corresponding elements and their first industrial uses were intimately linked to their optical properties. This relationship has been kept alive until today when many high-technology applications of lanthanide-containing materials such as energy-saving lighting devices, displays, optical fibers and amplifiers, lasers, responsive luminescent stains for biomedical analyses and in cellulo sensing and imaging, heavily rely on the brilliant and pure-color emission of lanthanide ions. In this review we first outlined the basics of lanthanide luminescence with emphasis on f-f transitions, the sensitization mechanisms, and the assessment of the luminescence efficiency of lanthanide-containing emissive molecular edifices. Emphasis was then put on two fast developing aspects of lanthanide luminescence: materials for telecommunications and light emitting diodes, and biomedical imaging and sensing. Recent advances in NIR-emitting materials for plastic amplifiers and waveguides were described, together with the main solutions brought by researchers to minimize non-radiative deactivation of excited states. The demonstration in 1999 that erbium tris(8-hydroxyquinolinate) displayed a bright green emission suitable for organic light emitting diodes (OLEDs) was followed by realizing that in OLEDs, 25% of the excitation energy leads to singlet states and 75% to triplet states. Since lanthanide ions are good triplet quenchers, they now also play a key role in the development of these lighting devices. Luminescence analyses of biological molecules are among the most sensitive analytical techniques known. The long lifetime of the lanthanide excited states allows time-resolved spectroscopy to be used, suppressing the sample autofluorescence and reaching very low detection limits. Not only visible lanthanide sensors are now ubiquitously provided in medical diagnosis and in cell imaging, but the

  13. CW-OSL measurement protocols using optical fibre Al2O3:C dosemeters

    DEFF Research Database (Denmark)

    Edmund, J.M.; Andersen, C.E.; Marckmann, C.J.

    2006-01-01

    A new system for in vivo dosimetry during radiotherapy has been introduced. Luminescence signals from a small crystal of carbon-doped aluminium oxide (Al2O3:C) are transmitted through an optical fibre cable to an instrument that contains optical filters, a photomultiplier tube and a green (532 nm......) laser. The prime output is continuous wave optically stimulated luminescence (CW-OSL) used for the measurement of the integrated dose. We demonstrate a measurement protocol with high reproducibility and improved linearity, which is suitable for clinical dosimetry. A crystal-specific minimum pre...

  14. Octopaminergic modulation of a fly visual motion-sensitive neuron during stimulation with naturalistic optic flow

    Directory of Open Access Journals (Sweden)

    Diana eRien

    2013-10-01

    Full Text Available In a variety of species locomotor activity, like walking or flying, has been demonstrated to alter visual information processing. The neuromodulator octopamine was shown to change the response characteristics of optic-flow processing neurons in the fly’s visual system in a similar way as locomotor activity. This modulation resulted in enhanced neuronal responses, in particular during sustained stimulation with high temporal frequencies, and in shorter latencies of responses to abrupt onsets of pattern motion. These state-dependent changes were interpreted to adjust neuronal tuning to the range of high velocities encountered during locomotion. Here we assess the significance of these changes for the processing of optic flow as experienced during flight. Naturalistic image sequences were reconstructed based on measurements of the head position and gaze direction of Calliphora vicina flying in an arena. We recorded the responses of the V1 neuron during presentation of these image sequences on a panoramic stimulus device (FliMax. Consistent with previous accounts, we found that spontaneous as well as stimulus-induced spike rates were increased by an octopamine agonist and decreased by an antagonist. Moreover, a small but consistent decrease in response latency upon octopaminergic activation was present, which might support fast responses to optic flow cues and limit instabilities during closed-loop optomotor regulation. However, apart from these effects the similarities between the dynamic response properties in the different pharmacologically induced states were surprisingly high, indicating that the processing of naturalistic optic flow is not fundamentally altered by octopaminergic modulation.

  15. Optical absorption, luminescence, and energy transfer processes studies for Dy3+/Tb3+-codoped borate glasses for solid-state lighting applications

    Science.gov (United States)

    Lakshminarayana, G.; Kaky, Kawa M.; Baki, S. O.; Lira, A.; Caldiño, U.; Kityk, I. V.; Mahdi, M. A.

    2017-10-01

    By using melt quenching technique, good optical quality singly doped Dy3+ or Tb3+ and Dy3+/Tb3+-codoped borate glasses were synthesized and studied by optical absorption, excitation, emission and decay lifetimes curve analysis. Following the absorption spectrum, the evaluated Judd-Ofelt (J-O) intensity parameters (Ωλ (λ = 2, 4 and 6)) were used to calculate the transition probability (AR), the branching ratio (βR), and the radiative lifetime (τR) for different luminescent transitions such as 4I15/2 → 6H15/2, 4F9/2 → 6H15/2, 4F9/2 → 6H13/2, 4F9/2 → 6H11/2 and 4F9/2 → 6H9/2,6F11/2 for the 0.5 mol % singly Dy3+-doped glass. The βR calculated (65%) indicates that for lasing applications, 4F9/2 → 6H13/2 emission transition is highly suitable. For all the Dy3+/Tb3+-codoped glasses, Tb3+: 5D3→7F6 emission decay lifetime curves are found to be non-exponential in nature for different concentrations of Dy3+ codoping. Using the Inokuti-Hirayama model, these nonexponential decay curves were analyzed to identify the nature of the energy transfer (ET) processes and here the electric dipole-dipole interaction is dominant for the ET. Based on the excitation and emission spectra and decay lifetimes curve analysis, the cross relaxation and ET processes between Dy3+ and Tb3+ were confirmed. For the 0.5 mol % Tb3+ and 2.0 mol % Dy3+-codoped glass, the evaluated Tb3+→Dy3+ ET efficiency (η) is found to be 45% under 369 nm excitation. Further, for Tb3+/Dy3+ -codoped glasses, an enhancement of Tb3+ green emission is observed up to 1.5 mol % Dy3+ codoping, and this is due to the non-radiative resonant ET from Dy3+ to Tb3+ upon 395 nm excitation. For singly 0.5 mol % Dy3+ or 0.5 mol % Tb3+-doped glass, the calculated color coordinates (x,y) and correlated color temperatures (CCT) represent the neutral white or warm white light regions, whereas Dy3+/Tb3+-codoped glasses (x,y) and CCT values fall in the yellowish green region with respect to the different Dy3

  16. Optical Stark effect in the four-wave mixing and stimulated Raman spectra of N2

    Science.gov (United States)

    Moosmuller, H.; She, C. Y.; Huo, Winifred M.

    1989-01-01

    The influence of the optical Stark effect on spectral line shapes in four-wave-mixing Raman spectroscopy (FWMRS) and stimulated Raman spectroscopy (SRS) is investigated experimentally and theoretically. Using an experimental setup capable of rapid alternation between the simultaneous measurement of coherent Stokes Raman spectroscopy and inverse Raman spectroscopy at low and high intensities, together with a sophisticated frequency reference scheme, it was possible to perform a rather direct comparison between Stark-broadened and non-Stark-broadened spectra of both classes of Raman spectroscopies. The results demonstrate that SRS spectra show more Stark shift and broadening than their FWMRS counterparts. A discrepancy with theoretical results is pointed out, and an attempt is made to explain it.

  17. Stimulated Brillouin scattering continuous wave phase conjugation in step-index fiber optics.

    Science.gov (United States)

    Massey, Steven M; Spring, Justin B; Russell, Timothy H

    2008-07-21

    Continuous wave (CW) stimulated Brillouin scattering (SBS) phase conjugation in step-index optical fibers was studied experimentally and modeled as a function of fiber length. A phase conjugate fidelity over 80% was measured from SBS in a 40 m fiber using a pinhole technique. Fidelity decreases with fiber length, and a fiber with a numerical aperture (NA) of 0.06 was found to generate good phase conjugation fidelity over longer lengths than a fiber with 0.13 NA. Modeling and experiment support previous work showing the maximum interaction length which yields a high fidelity phase conjugate beam is inversely proportional to the fiber NA(2), but find that fidelity remains high over much longer fiber lengths than previous models calculated. Conditions for SBS beam cleanup in step-index fibers are discussed.

  18. Two-photon luminescence contrast by tip-sample coupling in femtosecond near-field optical microscopy

    Science.gov (United States)

    Horneber, Anke; Wackenhut, Frank; Braun, Kai; Wang, Xiao; Wang, Jiyong; Zhang, Dai; Meixner, Alfred J.

    2017-01-01

    We investigate the role of tip-sample interaction in nonlinear optical scanning near-field microscopy. The experiment was performed by tightly focusing femtosecond laser pulses onto a sharp gold tip that was positioned in close proximity to the surface of a sample with gold nanostructures on a Si-substrate by shear force feedback. The nonlinear optical signal consists of two-photon photoluminescence and second harmonic signal from the gold tip and the gold nanostructures. These signals can be used to characterize different coupling parameters such as geometry, material and width of the tip-sample gap and enable to reveal the mechanism responsible for the image contrast. Under the excitation with 776-nm and 110-fs laser pulses nonlinear imaging is almost background free and yields super resolution showing features with dimensions significantly below the diffraction limit with a signal intensity following quadratic excitation power law.

  19. Effects of temperature and ionization density in medical luminescence dosimetry using Al2O3:C

    DEFF Research Database (Denmark)

    Edmund, Jens Morgenthaler

    2007-01-01

    A new system containing small crystals of aluminum oxide doped with carbon (Al2O3:C) attached to optical fiber cables has recently been introduced. During irradiation, the system monitors the radioluminescence (RL) from the crystals and after irradiation, an optically stimulated luminescence (OSL......) signal can be read out by stimulating the crystal with light. This thesis applies the initial part and the total area of the resulting OSL decay curve for dosimetry measurements and investigates the effects of temperature and proton energy, i.e. ionization density, on the RL and OSL signals from Al2O3:C...... temperature is kept constant, one can find an integration time which provides an OSL signal independent of stimulation temperature. Overall, the RL and OSL signals vary between -0.2 to 0.6% per C. Thermal effects were simulated with a band structure model and indicated that the temperature effects are caused...

  20. Luminescence dating: methodological research and application to volcanism in the Laschamp environment; Datation par luminescence: recherches methodologiques et applications au volcanisme dans l'environnement de Laschamp

    Energy Technology Data Exchange (ETDEWEB)

    Bassinet, C

    2007-03-15

    The aim of this work was to date lava flows from the Chaine des Puys (Massif Central, France) which were chronologically situated during the period of the Laschamp paleo-magnetic event (30-50 ka). The methods used were thermoluminescence and optically stimulated luminescence applied to quartz grains and quartz pebbles extracted from sediments baked by the lava flows. These minerals often emit luminescence signals exhibiting erratic behaviour. Thus, their radiation doses were tentatively determined by various methods to select those which were most likely to yield reliable results. These intercomparisons highlighted a dispersion of results beyond what could be expected from the uncertainties usually associated with each measurement. In the majority of cases, these observations forced us to propose a relatively wide interval in which the most probable age of the sample is included. (author)

  1. Establishing age constraints for Middle Pleistocene glaciofluvial sediments in the European Alpine foreland - new insights from luminescence dating

    Science.gov (United States)

    Lüthgens, Christopher; Rades, Eike F.; Bickel, Lukas; Fiebig, Markus

    2017-04-01

    This presentation summarises the outcome of a project funded by the Austrian Science Fund (FWF) which aimed at establishing new age constraints of deposits and landforms (glaciofluvial terraces) of the northern Alpine foreland (NAF) usually assigned to the Middle Pleistocene. The sediments under investigation were mostly deposited when large piedmont glaciers reached far into the Alpine foreland. Based on the concept of four Quaternary glacial advances to the NAF, which was already developed at the beginning of the 20th century by Penck and Brückner, specific morphostratigraphic units which can spatially be connected over the complete NAF area have been assigned to different glacial cycles and were subsequently correlated with the marine isotope record. However, numerical dating of the respective sediments had only been conducted to a limited extent, and previous studies report several methodological issues that limited the outcome with respect to the geochronological and chronostratigraphical value. In the course of the project, it became clear that the applicability of different optically stimulated luminescence (OSL) dating techniques for the targeted sediments was strongly dependent on the varying luminescence properties for samples from different catchment areas. By conducting a comparative luminescence dating approach, using different luminescence signals (quartz OSL, and feldspar infrared stimulated luminescence at 50°C (IR50) as well as post IR infrared stimulated luminescence at an elevated temperature (225°C, pIRIR225)), as well as using single aliquot and single grain dating techniques, it was i) possible to confirm but also to overcome prior problems of luminescence dating with the respective sediments ii) discern between samples that were well bleached prior to deposition and samples for which the luminescence signals were not properly reset, and iii) possible to establish reliable geochronological age constraints for the deposition of the sediments

  2. Luminescence and optical absorption studies of submicro-dimensional cerium ortho- and metaphosphates doped with Eu{sup 3+} ions

    Energy Technology Data Exchange (ETDEWEB)

    Matraszek, A. [Department of Inorganic Chemistry, Faculty of Engineering and Economics, Wroclaw University of Economics, 118/120 Komandorska str., 53-345 Wroclaw (Poland); Macalik, L. [Institute of Low Temperature and Structure Research, Polish Academy of Sciences, P.O. Box 1410, 50-950 Wroclaw (Poland); Szczygiel, I. [Department of Inorganic Chemistry, Faculty of Engineering and Economics, Wroclaw University of Economics, 118/120 Komandorska str., 53-345 Wroclaw (Poland); Godlewska, P. [Department of Bioorganic Chemistry, Faculty of Engineering and Economics, Wroclaw University of Economics, 118/120 Komandorska str., 53-345 Wroclaw (Poland); Solarz, P. [Institute of Low Temperature and Structure Research, Polish Academy of Sciences, P.O. Box 1410, 50-950 Wroclaw (Poland); Hanuza, J. [Institute of Low Temperature and Structure Research, Polish Academy of Sciences, P.O. Box 1410, 50-950 Wroclaw (Poland)], E-mail: j.hanuza@int.pan.wroc.pl

    2008-02-28

    Pechini method has been applied for synthesis of the phosphates in the submicro-state. Dimensions of the obtained grains by this method fall into the 100-1000 nm range. The following samples have been synthesised: stoichiometric orthophosphate Na{sub 3}Ce(PO{sub 4}){sub 2} and metaphosphate NaCe(PO{sub 3}){sub 4} both doped with 2 and 5% of Eu{sup 3+}. Optical absorption and emission studies have been performed to characterise the properties and structure of the compounds studied. The electronic characteristics of the Ce{sup 3+} and Eu{sup 3+} ions in these materials have been discussed.

  3. Luminescence dating of interglacial coastal depositional systems: Recent developments and future avenues of research

    Science.gov (United States)

    Lamothe, Michel

    2016-08-01

    Luminescence dating offers new opportunities to explore the evolution of Quaternary marine coastal facies and landforms. This review highlights the main advances in luminescence geochronology of interglacial coastal sediments through the analysis of 547 luminescence ages, most of which were published during the last decade. The majority of these reported luminescence investigations have been carried out along passive margin coasts. Since the turn of the century, the discovery of a normalization procedure known as Single Aliquot Regeneration (SAR) has drastically reduced data scatter and improved precision, with the consequence that quartz SAR optically-stimulated luminescence OSL has become the dating protocol of choice for the Last Interglacial (LIG) period. A more complex technique, known as thermally-transferred OSL (TT-OSL), is presumably proposed for dating older interglacials of the Mid-Pleistocene and beyond. Feldspar luminescence is increasingly being applied to dating Pleistocene sea level high stands due to a much higher dose saturation level than quartz OSL. The use of feldspar IRSL (Infrared-stimulated luminescence) is limited by the occurrence of variable, but ubiquitous anomalous fading (AF). Following the advent of AF-correction methods, several Middle Pleistocene sites have been amenable to dating, albeit with significant related uncertainties. Recently, new protocols involving the measurement of post-IR IRSL at elevated temperatures have yielded relatively coherent ages for interglacial sediments up to ca. 300 ka. Quartz OSL/TT-OSL, AF-corrected IRSL, and post-IR IRSL ages are generally correlated with periods of sea level high stands. A few ages are reported from the early and middle part of the Middle Pleistocene, as MIS11, 9 and more commonly MIS7 high stands are documented in strongly uplifting active margin coasts. However, by far the most obvious age peak corresponds to the end of the LIG. The MIS5e shoreline is probably the most studied and

  4. Optical enhanced luminescent measurements and sequential reagent mixing on a centrifugal microfluidic device for multi-analyte point-of-care applications

    Science.gov (United States)

    Bartholomeusz, Daniel A.; Davies, Rupert H.; Andrade, Joseph D.

    2006-02-01

    A centrifugal-based microfluidic device1 was built with lyophilized bioluminescent reagents for measuring multiple metabolites from a sample of less than 15 μL. Microfluidic channels, reaction wells, and valves were cut in adhesive vinyl film using a knife plotter with features down to 30 μm and transferred to metalized polycarbonate compact disks (CDs). The fabrication method was simple enough to test over 100 prototypes within a few months. It also allowed enzymes to be packaged in microchannels without exposure to heat or chemicals. The valves were rendered hydrophobic using liquid phase deposition. Microchannels were patterned using soft lithography to make them hydrophilic. Reagents and calibration standards were deposited and lyophilized in different wells before being covered with another adhesive film. Sample delivery was controlled by a modified CD ROM. The CD was capable of distributing 200 nL sample aliquots to 36 channels, each with a different set of reagents that mixed with the sample before initiating the luminescent reactions. Reflection of light from the metalized layer and lens configuration allowed for 20% of the available light to be collected from each channel. ATP was detected down to 0.1 μM. Creatinine, glucose, and galactose were also measured in micro and milliMolar ranges. Other optical-based analytical assays can easily be incorporated into the device design. The minimal sample size needed and expandability of the device make it easier to simultaneously measure a variety of clinically relevant analytes in point-of-care settings.

  5. Optical Characteristics and Math-physical Model of Bioluminescence of Oceanic Organism Stimulated by Flow%流场刺激下海洋生物发光的光学特性及数理模型

    Institute of Scientific and Technical Information of China (English)

    曹静; 宗思光; 王江安; 马治国; 吴荣华

    2012-01-01

    The detection of stimulated bioluminescence is the new technology and method of target detection in water. Three representative luminescent alga, such as lingulodinium polyedrum, pyro-cystis noctiluca and pyrocystis lunula, are studied. The platform of stimulated bioluminescence is built by the use of spectrometer, photon counter, Couette flow device and so on. The optical characteristics of bioluminescenee stimulated by flow are researched. Based on the experimental study, probabilistic and mathematic statistic theory, the math-physical model of stimulated bioluminescence is built. The experiment results showed that the light spectrum of luminescence alga is a single wavelength with about 472 nm of the maximum wavelength and 30~40 nm of full width at half maximum. Furthermore, the intensities of bioluminescence are different with different organisms and attenuated with the decrease of the energy of organisms, but it will be recovered after a rest. On the basis of their bioluminescence response in the same stimulated condition, these species were ranked in order of decreasing sensitivity as I( pyrocystis lunula) > I( pyrocystis noctiluca) >I( lingulodinium polyedrum)%生物受激发光探测是一种感知水中目标的新技术、新手段.选取多边膝沟藻、夜光虫和月芽形梨甲藻3种典型海洋受激发光生物体为对象,采用光谱仪、光子计数器、库埃特流场旋转圆筒等装置搭建了生物受激发光实验平台,研究了不同刺激下生物体受激发光的光学特性,并在此基础上结合概率论和数理统计理论,建立了流场刺激下的生物发光的数理模型.结果表明:发光藻的发光具有较好的单色谱特性,峰值波长集中在472 nm左右,谱线的半波宽度为30 ~40 nm.发光藻的发光随着机体的疲劳而变弱,但发光能力随着机体的休息会慢慢恢复.同种刺激条件下,3种藻发光强度的强弱依次为月芽形梨甲藻、夜光虫、多边膝沟藻.

  6. Optical and morphological characterization by atomic force microscopy of luminescent 2-styrylpyridine derivative compounds with Poly(N-vinylcarbazole) films

    Energy Technology Data Exchange (ETDEWEB)

    Perez-Gutierrez, E., E-mail: cuper_enrique@msn.com [Centro de Quimica, Instituto de Ciencias, Universidad Autonoma de Puebla, Complejo de Ciencias, ICUAP, Edif. 103-F, 22 Sur y San Claudio, C.P. 72570 Puebla, Puebla (Mexico); Percino, M.J.; Chapela, V.M. [Centro de Quimica, Instituto de Ciencias, Universidad Autonoma de Puebla, Complejo de Ciencias, ICUAP, Edif. 103-F, 22 Sur y San Claudio, C.P. 72570 Puebla, Puebla (Mexico); Maldonado, J.L. [Centro de Investigaciones en Optica A.C. (CIO), Lomas del Bosque 115, Col. Lomas del Campestre, C.P. 37150, Leon Guanajuato (Mexico)

    2011-07-01

    The present work addresses the optical and morphological properties of organic films based on low molecular weight dyes styrylpyridine derivatives 2-styrylpyridine (A), 4-chlorophenyl-2-vinylpyridine (B) and 4-fluorophenyl-2-vinylpyridine (C), embedded in a polymeric matrix poly(N-vinylcarbazole) (PVK). The films were prepared by a spin-coating technique from solutions with dye:PVK ratios of 0.25:1, 0.5:1 and 1:1. Solvents were chloroform and toluene. The molar absorption coefficient ({epsilon}) spectra for a dye:PVK mixture in solution were a combination of the absorptions of both components separately, but for the deposited films, the shape of the spectrum showed that the poly(N-vinylcarbazole) absorption dominated. However, when the same films were dissolved again in CHCl{sub 3}, their spectra showed an absorption shape similar to that of the solution mixture before the deposition. Solution viscosity measurements were carried out with an Ubbelohde glass capillary viscometer to corroborate the results that showed a better mixture of the dye with the host in chloroform. The morphology of the prepared films was analyzed by atomic force microscopy and exhibited a solvent effect, with a pinhole-free, smooth surface when toluene was used and a wavy surface with chloroform. The ratio dye:matrix was the principal parameter for obtaining optical quality films; for 0.25:1 and 0.5:1 ratios, the films were of good quality, but for 1:1, the dye was expelled from the PVK and a crystallization was present over the surface of the films. Film thickness was also measured and films deposited from toluene solutions gave an average thickness of 54 nm while films from chloroform solutions had an average thickness greater than 160 nm that increased depending on chromophore concentration.

  7. Preparation, theory, and biological applications of highly luminescent cadmium selenide/zinc sulfide quantum dots in optical and electron microscopy

    Science.gov (United States)

    Bouwer, James Christopher

    This dissertation describes the preparation, theory, and applications of ZnS overcoated CdSe (core) quantum dots for applications as fluorescent probes in optical microscopy and as electron energy loss spectroscopy (EELS) probes in electron microscopy, with applications to the biological sciences. The dissertation begins with a brief overview of quantum dots and their history. Next, a brief overview of the necessary semiconductor theory is discussed including the origin of the band gap, the origin of holes, the concepts of phonons, and trap states. Then, the role of the confinement potential in the quantum dot fluorescent spectrum is discussed in the context of the 3-dimensional spherical well. Included in this discussion is the role of excitonic electron-hole bound states. To provide a complete document useful to anyone who wishes to continue work along these lines, included is a methods section which describes the complete process of synthesis of the CdSe cores, overcoating the cores with ZnS, size selection of nanocrystals, water solubilization, and protein conjugation. The methods used in live cell labeling are included as well. In the section that follows, a discussion of the mathematical methods of image correlation spectroscopy (ICS) for extracting dynamic constants such as flow rates and diffusion constants from time lapse optical image data is discussed in the context of quantum dot fluorescent probes. Dynamic constants were obtained using live NIH3T3 mouse fibroblast cells labeled with IgG-anti-EGF conjugated quantum dots. These same cells were then fixed, imbedded in resin, sectioned to 100nm thick sections and imaged under the electron microscope. The electron dense cadmium selinide provides the contrast necessary to perform direct imaging of EGF receptor sites. In order to improve the data and move toward multi-channel imaging in the electron microscope, EELS spectroscopy and elemental mapping of quantum dots was performed. The theory along with a

  8. Luminescent hyperbolic metasurfaces

    Science.gov (United States)

    Smalley, J. S. T.; Vallini, F.; Montoya, S. A.; Ferrari, L.; Shahin, S.; Riley, C. T.; Kanté, B.; Fullerton, E. E.; Liu, Z.; Fainman, Y.

    2017-01-01

    When engineered on scales much smaller than the operating wavelength, metal-semiconductor nanostructures exhibit properties unobtainable in nature. Namely, a uniaxial optical metamaterial described by a hyperbolic dispersion relation can simultaneously behave as a reflective metal and an absorptive or emissive semiconductor for electromagnetic waves with orthogonal linear polarization states. Using an unconventional multilayer architecture, we demonstrate luminescent hyperbolic metasurfaces, wherein distributed semiconducting quantum wells display extreme absorption and emission polarization anisotropy. Through normally incident micro-photoluminescence measurements, we observe absorption anisotropies greater than a factor of 10 and degree-of-linear polarization of emission >0.9. We observe the modification of emission spectra and, by incorporating wavelength-scale gratings, show a controlled reduction of polarization anisotropy. We verify hyperbolic dispersion with numerical simulations that model the metasurface as a composite nanoscale structure and according to the effective medium approximation. Finally, we experimentally demonstrate >350% emission intensity enhancement relative to the bare semiconducting quantum wells.

  9. Thermally stimulated luminescence and electron paramagnetic resonance studies of {sup 147}Pm doped K{sub 3}Na(SO{sub 4}){sub 2}

    Energy Technology Data Exchange (ETDEWEB)

    Murali, S.; Natarajan, V. E-mail: agpage@magnum.barc.ernet.in; Seshagiri, T.K.; Kadam, R.M.; Venkataramani, R.; Sastry, M.D

    2003-06-01

    Rare earth and actinide doped alkali and alkaline earth sulphates, exhibit a variety of point defects stabilized due to the charge imbalance/self-irradiation and they play an important role in luminescence properties. In this paper, we report the point defects formed in the mixed sulphate K{sub 3}Na(SO{sub 4}){sub 2} on doping with the radio-active rare earth element {sup 147}Pm as studied by TSL and EPR techniques. EPR studies on self and gamma irradiated samples showed the signal due to the radical pair, SO{sub 4}{sup -}-SO{sub 3}{sup -} in addition to the signals from SO{sub 4}{sup -}, SO{sub 3}{sup -} and O{sub 2}{sup -} ions. However EPR spectra of electron beam irradiated (undoped) K{sub 3}Na(SO{sub 4}){sub 2} samples did not show the presence of the radical pair SO{sub 4}{sup -}-SO{sub 3}{sup -}, indicating the importance of dopant per se, in stabilizing the radical pair. EPR studies of {sup 147}Pm doped samples annealed at different temperatures after gamma irradiation showed that SO{sub 4}{sup -}-SO{sub 3}{sup -} radical pair gets destroyed around 550 K, whereas SO{sub 4}{sup -} ion gets annealed in the temperature range 375-450 K. SO{sub 3}{sup -} ion was found to be stable upto 600 K. From TSL-EPR correlation, it is inferred that the release of trapped hole at SO{sub 4}{sup -} ion on heating leads to the formation of SO{sub 4}{sup 2-{sup *}} and energy transfer to Pm{sup 3+} ion, results in the glow peak at 415 K.

  10. Luminescent Processes Elucidated by Simple Experiments on ZnS.

    Science.gov (United States)

    Schwankner, R.; And Others

    1981-01-01

    Describes some impurity-related optical properties of semiconductors, with special emphasis on the luminescence of zinc sulfide (ZnS). Presents and interprets five experiments using a ZnS screen, ultraviolet lamp, transparent Dewar liquid nitrogen, and a helium/neon gas base. Includes application of luminescence measurements to archaeology. (SK)

  11. Optical transmission radiation damage and recovery stimulation of DSB: Ce3+ inorganic scintillation material

    Science.gov (United States)

    Borisevich, A.; Dormenev, V.; Korjik, M.; Kozlov, D.; Mechinsky, V.; Novotny, R. W.

    2015-02-01

    Recently, a new scintillation material DSB: Ce3+ was announced. It can be produced in a form of glass or nano-structured glass ceramics with application of standard glass production technology with successive thermal annealing. When doped with Ce3+, material can be applied as scintillator. Light yield of scintillation is near 100 phe/MeV. Un-doped material has a wide optical window from 4.5eV and can be applied to detect Cherenkov light. Temperature dependence of the light yield LY(T) is 0.05% which is 40 times less than in case of PWO. It can be used for detectors tolerant to a temperature variation between -20° to +20°C. Several samples with dimensions of 15x15x7 mm3 have been tested for damage effects on the optical transmission under irradiation with γ-quanta. It was found that the induced absorption in the scintillation range depends on the doping concentration and varies in range of 0.5-7 m-1. Spontaneous recovery of induced absorption has fast initial component. Up to 25% of the damaged transmission is recuperated in 6 hours. Afterwards it remains practically constant if the samples are kept in the dark. However, induced absorption is reduced by a factor of 2 by annealing at 50°C and completely removed in a short time when annealing at 100°C. A significant acceleration of the induced absorption recovery is observed by illumination with visible and IR light. This effect is observed for the first time in a Ce-doped scintillation material. It indicates, that radiation induced absorption in DSB: Ce scintillation material can be retained at the acceptable level by stimulation with light in a strong irradiation environment of collider experiments.

  12. Multifocus optical-resolution photoacoustic microscopy using stimulated Raman scattering and chromatic aberration.

    Science.gov (United States)

    Hajireza, Parsin; Forbrich, Alexander; Zemp, Roger J

    2013-08-01

    In this Letter, multifocus optical-resolution photoacoustic microscopy is demonstrated using wavelength tuning and chromatic aberration for depth scanning. Discrete focal zones at several depth locations were created by refocusing light from a polarization-maintaining single-mode fiber pumped by a nanosecond fiber laser. The fiber and laser parameters were chosen to take advantage of stimulated Raman scattering (SRS) in the fiber to create a multiwavelength output that could then be bandpass filtered. The collimator lens and objective lens are chosen to take advantage of chromatic aberration in which each generated SRS wavelength peak focuses at a slightly different depth. The maximum amplitude of photoacoustic signals is mapped to form C-scan images. Additionally, all wavelength peaks fired simultaneously offers improved depth-of-field structural imaging at the cost of slight degradation of mainlobe-to-sidelobe ratios. Wavelength-tuned depth scanning over more than 440 μm is demonstrated, significantly greater than the ~100 μm depth of field predicted from our focused Gaussian beams. The improved depth of focus could be valuable for structural imaging of microvascular morphology without the need for mechanical scanning in the depth direction.

  13. Stimulated penetrating keratoplasty using real-time virtual intraoperative surgical optical coherence tomography

    Science.gov (United States)

    Lee, Changho; Kim, Kyungun; Han, Seunghoon; Kim, Sehui; Lee, Jun Hoon; Kim, Hong kyun; Kim, Chulhong; Jung, Woonggyu; Kim, Jeehyun

    2014-01-01

    Abstract. An intraoperative surgical microscope is an essential tool in a neuro- or ophthalmological surgical environment. Yet, it has an inherent limitation to classify subsurface information because it only provides the surface images. To compensate for and assist in this problem, combining the surgical microscope with optical coherence tomography (OCT) has been adapted. We developed a real-time virtual intraoperative surgical OCT (VISOCT) system by adapting a spectral-domain OCT scanner with a commercial surgical microscope. Thanks to our custom-made beam splitting and image display subsystems, the OCT images and microscopic images are simultaneously visualized through an ocular lens or the eyepiece of the microscope. This improvement helps surgeons to focus on the operation without distraction to view OCT images on another separate display. Moreover, displaying the OCT live images on the eyepiece helps surgeon’s depth perception during the surgeries. Finally, we successfully processed stimulated penetrating keratoplasty in live rabbits. We believe that these technical achievements are crucial to enhance the usability of the VISOCT system in a real surgical operating condition. PMID:24604471

  14. Using Optically Stimulated Electron Emission as an Inspection Method to Monitor Surface Contamination

    Science.gov (United States)

    Lingbloom, Mike S.

    2008-01-01

    During redesign of the Space Shuttle reusable solid rocket motor (RSRM), NASA amended the contract with ATK Launch Systems (then Morton Thiokol Inc.) with Change Order 966 to implement a contamination control and cleanliness verification method. The change order required: (1) A quantitative inspection method (2) A written record of actual contamination levels versus a known reject level (3) A method that is more sensitive than existing methods of visual and black light inspection. Black light inspection is only useful for inspection of contaminants that fluoresce near the 365 nm spectral line and is not useful for inspection of most silicones that will not produce strong fluorescence. Black light inspection conducted by a qualified inspector under controlled light is capable of detecting Conoco HD-2 grease in gross amounts and is very subjective due to operator sensitivity. Optically stimulated electron emission (OSEE), developed at the Materials and Process Laboratory at Marshall Space Flight Center (MSFC), was selected to satisfy Change Order 966. OSEE offers several important advantages over existing laboratory methods with similar sensitivity, e.g., spectroscopy and nonvolatile residue sampling, which provide turn around time, real time capability, and full coverage inspection capability. Laboratory methods require sample gathering and in-lab analysis, which sometimes takes several days to get results. This is not practical in a production environment. In addition, these methods do not offer full coverage inspection of the large components

  15. A Portable Surface Contamination Monitor Based on the Principle of Optically Stimulated Electron Emission (OSEE)

    Science.gov (United States)

    Perey, D. F.

    1996-01-01

    Many industrial and aerospace processes involving the joining of materials, require sufficient surface cleanliness to insure proper bonding. Processes as diverse as painting, welding, or the soldering of electronic circuits will be compromised if prior inspection and removal of surface contaminants is inadequate. As process requirements become more stringent and the number of different materials and identified contaminants increases, various instruments and techniques have been developed for improved inspection. One such technique, based on the principle of Optically Stimulated Electron Emission (OSEE), has been explored for a number of years as a tool for surface contamination monitoring. Some of the benefits of OSEE are: it is non-contacting; requires little operator training; and has very high contamination sensitivity. This paper describes the development of a portable OSEE based surface contamination monitor. The instrument is suitable for both hand-held and robotic inspections with either manual or automated control of instrument operation. In addition, instrument output data is visually displayed to the operator and may be sent to an external computer for archiving or analysis.

  16. Spatio-temporal characteristics of inhibition mapped by optical stimulation in mouse olfactory bulb

    Directory of Open Access Journals (Sweden)

    Alexander eLehmann

    2016-03-01

    Full Text Available Mitral and tufted cells (MTCs of the mammalian olfactory bulb (OB are connected via dendrodendritic synapses with inhibitory interneurons in the external plexiform layer. The range, spatial layout and temporal properties of inhibitory interactions between MTCs mediated by inhibitory interneurons remain unclear. Therefore we tested for inhibitory interactions using an optogenetic approach. We optically stimulated MTCs expressing channelrhodopsin-2 in transgenic mice, while recording from individual MTCs in juxtacellular or whole-cell configuration in vivo. We used a spatial noise stimulus for mapping interactions between MTCs belonging to different glomeruli in the dorsal bulb. Analyzing firing responses of MTCs to the stimulus, we did not find robust lateral inhibitory effects that were spatially specific. However, analysis of sub-threshold changes in the membrane potential revealed evidence for inhibitory interactions between MTCs that belong to different glomerular units. These lateral inhibitory effects were short-lived and spatially specific. MTC response maps showed hyperpolarizing effects radially extending over more than 5 glomerular diameters. The inhibitory maps exhibited non-symmetrical yet distance-dependent characteristics.

  17. Recent progress in biomedical applications of persistent luminescence nanoparticles.

    Science.gov (United States)

    Wang, Jie; Ma, Qinqin; Wang, Yingqian; Shen, Haijing; Yuan, Quan

    2017-05-18

    Persistent luminescence nanoparticles (PLNPs) are an emerging group of promising luminescent materials that can remain luminescent after the excitation ceases. In the past decade, PLNPs with intriguing optical properties have been developed and their applications in biomedicine have been widely studied. Due to the ultra-long decay time of persistent luminescence, autofluorescence interference in biosensing and bioimaging can be efficiently eliminated. Moreover, PLNPs can remain luminescent for hours, making them valuable in bio-tracing. Also, persistent luminescence imaging can guide cancer therapy with a high signal-to-noise ratio (SNR) and superior sensitivity. Briefly, PLNPs are demonstrated to be a newly-emerging class of functional materials with unprecedented advantages in biomedicine. In this review, we summarized recent advances in the preparation of PLNPs and the applications of PLNPs in biosensing, bioimaging and cancer therapy.

  18. Broadband true time delay for microwave signal processing, using slow light based on stimulated Brillouin scattering in optical fibers.

    Science.gov (United States)

    Chin, Sanghoon; Thévenaz, Luc; Sancho, Juan; Sales, Salvador; Capmany, José; Berger, Perrine; Bourderionnet, Jérôme; Dolfi, Daniel

    2010-10-11

    We experimentally demonstrate a novel technique to process broadband microwave signals, using all-optically tunable true time delay in optical fibers. The configuration to achieve true time delay basically consists of two main stages: photonic RF phase shifter and slow light, based on stimulated Brillouin scattering in fibers. Dispersion properties of fibers are controlled, separately at optical carrier frequency and in the vicinity of microwave signal bandwidth. This way time delay induced within the signal bandwidth can be manipulated to correctly act as true time delay with a proper phase compensation introduced to the optical carrier. We completely analyzed the generated true time delay as a promising solution to feed phased array antenna for radar systems and to develop dynamically reconfigurable microwave photonic filters.

  19. 基于受激发光实验的生物光尾流特性%Characteristics of bioluminescent wake based on stimulated luminescence laboratory experiments

    Institute of Scientific and Technical Information of China (English)

    曹静; 王江安; 何友; 吴荣华

    2011-01-01

    Abstract: Based on the relative characteristics of stimulated bioluminescence and hydrodynamic flow, the experimental plat-form of stimulated bioluminescence in Couette flow was built. The hydrodynamic elements stimulated bioluminescence were analy-sised. The threshold of shear stress for stimulated bioluminescence of Lingulodinium polyedrum is 0. 1 N/m2. And biolumines-cence emission is the function of shear stress and increases with it when the shear stress exceeds the threshold. The shear stress distributions of submarine were simulated by FLUENT software. The results of calculation illustrate that the shear stress decrea-ses with the increased length of wake of submarine and it can be decreased as the oscillation of sine wave in the near area. The shear stress of wake decreases rapidly and widely with the higher speed of submarine, when the speed of submarine is above 4. 1 m/s, the shear stress of wake in 2 000 m length is still over the threshold.%基于生物受激发光与流场机械刺激间的相关性,构建了库埃特流场刺激下的生物受激发光实验平台,分析了影响生物发光的水动力因素剪应力.实验结果显示:引起多边膝沟藻受激发光的剪应力阈值为0.1 N/m2;当流场中的剪应力大于发光阈值后,生物发光强度随着剪应力的增大而增强.采用FLUENT软件模拟计算了不同航速下某潜艇尾流场中的剪应力,计算结果表明:剪应力随着尾流长度的增加而减小,在近场区域剪应力出现了类似正弦波振荡的减小,且航速越大减幅越大,减速越快;当潜艇航速大于4.1 m/s航行时,2 000 m处尾流的剪应力仍然大于引起生物发光的剪应力阈值.

  20. Luminescence dating and palaeomagnetic age constraint on hominins from Sima de los Huesos, Atapuerca, Spain.

    Science.gov (United States)

    Arnold, Lee J; Demuro, Martina; Parés, Josep M; Arsuaga, Juan Luis; Aranburu, Arantza; Bermúdez de Castro, José María; Carbonell, Eudald

    2014-02-01

    Establishing a reliable chronology on the extensive hominin remains at Sima de los Huesos is critical for an improved understanding of the complex evolutionary histories and phylogenetic relationships of the European Middle Pleistocene hominin record. In this study, we use a combination of 'extended-range' luminescence dating techniques and palaeomagnetism to provide new age constraint on sedimentary infills that are unambiguously associated with the Sima fossil assemblage. Post-infrared-infrared stimulated luminescence (pIR-IR) dating of K-feldspars and thermally transferred optically stimulated luminescence (TT-OSL) dating of individual quartz grains provide weighted mean ages of 433 ± 15 ka (thousands of years) and 416 ± 19 ka, respectively, for allochthonous sedimentary horizons overlying the hominin-bearing clay breccia. The six replicate luminescence ages obtained for this deposit are reproducible and provide a combined minimum age estimate of 427 ± 12 ka for the underlying hominin fossils. Palaeomagnetic directions for the luminescence dated sediment horizon and underlying fossiliferous clays display exclusively normal polarities. These findings are consistent with the luminescence dating results and confirm that the hominin fossil horizon accumulated during the Brunhes Chron, i.e., within the last 780 ka. The new bracketing age constraint for the Sima hominins is in broad agreement with radiometrically dated Homo heidelbergensis fossil sites, such as Mauer and Arago, and suggests that the split of the H. neanderthalensis and H. sapiens lineages took place during the early Middle Pleistocene. More widespread numerical dating of key Early and Middle Pleistocene fossil sites across Europe is needed to test and refine competing models of hominin evolution. The new luminescence chronologies presented in this study demonstrate the versatility of TT-OSL and pIR-IR techniques and the potential role they could play in helping to refine evolutionary

  1. High Speed Signal Wavelength Conversion Using Stimulated Raman Effect in Ultrasmall Silicon-on-Insulator Optical Waveguides

    Institute of Scientific and Technical Information of China (English)

    WU Jian-Wei; LUO Feng-Guang; GALLEP Cristiano de Mello

    2008-01-01

    We propose the high speed signal wavelength conversion based on stimulated Raman effect on silicon waveguides.Simulation results of non-return-to-zero(NRZ)pseudorandom bit sequence(27-1 code)at 500-Gb/s rate of conversion in an ultrasmall silicon-on-insulator(SOI)optical wavegnide are presented by co-propagating pump optical field.The most attractive issue is that the inverted converted signal can be obtained at the same wavelength as that of primary signal.In addition,the conversion performances,including extinction ratio(ER)and average peak power of conversion signal,depend strongly on the launching pump intensity.

  2. Performance of a novel multiple-signal luminescence sediment tracing method

    Science.gov (United States)

    Reimann, Tony

    2014-05-01

    Optically Stimulated Luminescence (OSL) is commonly used for dating sediments. Luminescence signals build up due to exposure of mineral grains to natural ionizing radiation, and are reset when these grains are exposed to (sun)light during sediment transport and deposition. Generally, luminescence signals can be read in two ways, potentially providing information on the burial history (dating) or the transport history (sediment tracing) of mineral grains. In this study we use a novel luminescence measurement procedure (Reimann et al., submitted) that simultaneously monitors six different luminescence signals from the same sub-sample (aliquot) to infer the transport history of sand grains. Daylight exposure experiments reveal that each of these six signals resets (bleaches) at a different rate, thus allowing to trace the bleaching history of the sediment in six different observation windows. To test the feasibility of luminescence sediment tracing in shallow-marine coastal settings we took eight sediment samples from the pilot mega-nourishment Zandmotor in Kijkduin (South-Holland). This site provides relatively controlled conditions as the morphological evolution of this nourishment is densely monitored (Stive et al., 2013). After sampling the original nourishment source we took samples along the seaward facing contour of the spit that was formed from August 2011 (start of nourishment) to June 2012 (sampling). It is presumed that these samples originate from the source and were transported and deposited within the first year after construction. The measured luminescence of a sediment sample was interpolated onto the daylight bleaching curve of each signal to assign the Equivalent Exposure Time (EET) to a sample. The EET is a quantitative measure of the full daylight equivalent a sample was exposed to during sediment transport, i.e. the higher the EET the longer the sample has been transported or the more efficient it has been exposed to day-light during sediment

  3. Testing the potential of OSL, TT-OSL, IRSL and post-IR IRSL luminescence dating on a Middle Pleistocene sediment record of Lake El'gygytgyn, Russia

    Directory of Open Access Journals (Sweden)

    A. Zander

    2012-09-01

    Full Text Available Lake El'gygytgyn is a 12 km wide crater lake located in remote Chukotka in the far East Russian Arctic about 100 km to the north of the Arctic Circle. It was formed by a meteorite impact about 3.58 Ma ago. This study tests the paleomagnetic and proxy data-based Mid- to Late-Pleistocene sediment deposition history using novel luminescence dating techniques of sediment cores taken from the centre of the 175 m deep lake. For dating polymineral and quartz fine grains (4–11 μm grain size range were extracted from nine different levels from the upper 28 m of sediment cores 5011-1A and 5011-1B. Polymineral sub-samples were analysed by infra-red stimulated luminescence (IRSL and post-IR infra-red stimulated luminescence (post-IR IRSL using single aliquot regenerative dose (SAR sequences. SAR protocols were further applied to measure the blue light optically stimulated luminescence (OSL and thermally-transferred OSL (TT-OSL of fine-grained quartz supplemented by a multiple aliquot TT-OSL approach. According to an independent age model, the lowest sample from 27.8–27.9 m below lake bottom level correlates to the Brunhes-Matuyama (B/M reversal. Finally, the SAR post-IR-IRSL protocol applied to polymineral fine grains was the only luminescence technique able to provide dating results of acceptable accuracy up to ca. 700 ka. Major factors limiting precision and accuracy of the luminescence chronology are, for some samples, natural signals already approaching saturation level, and overall the uncertainty related to the sediment water content and its variations over geological times.

  4. Phenomenological model of stochastic, spatiotemporal, intensity dynamics of stimulated Brillouin scattering in a two-mode optical fiber.

    Science.gov (United States)

    Armstrong, Cameron R; David, John A; Thompson, John R

    2015-07-13

    We present a simple numerical model that is used in conjunction with a systematic algorithm for parameter optimization to understand the three-dimensional stochastic intensity dynamics of stimulated Brillouin scattering in a two-mode optical fiber. The primary factors driving the complex dynamics appear to be thermal density fluctuations, transverse pump fluctuations, and asymmetric transverse mode fractions over the beam cross-section.

  5. Stimulated recovery of the optical transmission of PbWO 4 scintillation crystals for electromagnetic calorimeters after radiation damage

    Science.gov (United States)

    Dormenev, V.; Kuske, T.; Novotny, R. W.; Borisevich, A.; Fedorov, A.; Korjik, M.; Mechinski, V.; Missevitch, O.; Lugert, S.

    2010-11-01

    In this paper we describe the phenomenon of the stimulated recovery of radiation damage in lead tungstate scintillation crystals achieved via illumination by visible and infrared light. It allows fast and efficient in-situ recovery of the optical transmission either during beam-off periods or on-line during data accumulation. The application can substantially improve or extend the running period of the experiment by keeping the damage at a tolerable level.

  6. Extending the area of investigation of fine versus coarse quartz optical ages from the Lower Danube to the Carpathian Basin

    DEFF Research Database (Denmark)

    Timar-Gabor, Alida; Constantin, Daniela; Marković, S.B.;

    2015-01-01

    Despite the general satisfactory performance of quartz in the single aliquot regeneration protocol (SAR), previous optically stimulated luminescence (OSL) dating studies of key loess sections in Romania, Lower Danube region, revealed a disturbing disagreement among the ages obtained on fine (4e11...

  7. Dispersion-based stimulated Raman scattering spectroscopy, holography, and optical coherence tomography (Conference Presentation)

    Science.gov (United States)

    Robles, Francisco E.; Fischer, Martin C.; Warren, Warren S.

    2016-03-01

    Stimulated Raman scattering (SRS) enables fast, high resolution imaging of chemical constituents important to biological structures and functional processes. While this technology has shown remarkable potential, it is currently limited to point scanning and can only probe a few Raman bands at a time. In this work we take a fundamentally different approach to detecting the small nonlinear signals based on dispersion effects that accompany the loss/gain processes in SRS. We use a modified pump-probe system (pulses with duration of ~0.5 ps and 75 fs, respectively) with interferometric detection in the Fourier-domain to demonstrate that the dispersive measurements are more robust to noise (e.g., laser noise) compared to conventional amplitude measurements, which in turn permits facile spectral and spatial multiplexing. Results show that it is possible to assess a broadband dispersion spectrum (currently limited to ~400 cm-1) with a single laser shot or spectrometer acquisition (20-50 µs). For molecular imaging with broadband spectral information, we achieve spatial pixel rates of 2.5 kHz, and will discuss how this can be further improved to 20-50 kHz. We also combine SRS with optical coherence tomography (OCT) (molecular and structural information are rendered from the same data), which enables axial multiplexing by coherence gating and paves the way for volumetric biochemical imaging. The approach is tested on a thin water-and-oil phantom, a thick scattering polystyrene bead phantom, and thick freshly excised human adipose tissue. Finally, we will outline other opportunities for spatial multiplexing using wide-field holography and spectroscopic-OCT, which would massively parallelize the spatial and spectral information. The combination of dispersion-based SRS and phase imaging has the potential to enable faster wide-area and volumetric molecular imaging. Such methods would be valuable in a clinical setting for many applications.

  8. The effects of electrical and optical stimulation of midbrain dopaminergic neurons on rat 50-kHz ultrasonic vocalizations

    Directory of Open Access Journals (Sweden)

    Tina eScardochio

    2015-12-01

    Full Text Available AbstractRationale Adult rats emit ultrasonic vocalizations (USVs at around 50-kHz ; these commonly occur in contexts that putatively engender positive affect. While several reports indicate that dopaminergic (DAergic transmission plays a role in the emission of 50-kHz calls, the pharmacological evidence is mixed. Different modes of dopamine (DA release (i.e. tonic and phasic could potentially explain this discrepancy.Objective To investigate the potential role of phasic DA release in 50-kHz call emission.Methods In Experiment 1, USVs were recorded in adult male rats following unexpected electrical stimulation of the medial forebrain bundle (MFB. In parallel, phasic DA release in the nucleus accumbens (NAcc was recorded using fast-scan cyclic voltammetry. In Experiment 2, USVs were recorded following response-contingent or non-contingent optogenetic stimulation of midbrain DAergic neurons. Four 20-s schedules of optogenetic stimulation were used: fixed-interval, fixed-time, variable-interval and variable-time.Results Brief electrical stimulation of the MFB increased both 50-kHz call rate and phasic DA release in the NAcc. During optogenetic stimulation sessions, rats initially called at a high rate comparable to that observed following reinforcers such as psychostimulants. Although optogenetic stimulation maintained reinforced responding throughout the 2-hour session, the call rate declined to near zero within the first 30 minutes. The trill call subtype predominated following both electrical and optical stimulation.Conclusion The occurrence of electrically-evoked 50-kHz calls, time-locked to phasic DA (Experiment 1, provides correlational evidence supporting a role for phasic DA in USV production. However, in Experiment 2, the temporal dissociation between calling and optogenetic stimulation of midbrain DAergic neurons suggests that phasic mesolimbic DA release is not sufficient to produce 50-kHz calls. The emission of the trill subtype of 50-k

  9. Dock3 overexpression and p38 MAPK inhibition synergistically stimulate neuroprotection and axon regeneration after optic nerve injury.

    Science.gov (United States)

    Semba, Kentaro; Namekata, Kazuhiko; Kimura, Atsuko; Harada, Chikako; Katome, Takashi; Yoshida, Hiroshi; Mitamura, Yoshinori; Harada, Takayuki

    2014-10-03

    The dedicator of cytokinesis 3 (Dock3) is an atypical guanine nucleotide exchange factor that is predominantly expressed in the CNS. Dock3 exerts neuroprotective effects and stimulates optic nerve regeneration. The p38 mitogen-activated protein kinase acts downstream of apoptosis signal-regulating kinase 1 (ASK1) signaling and plays an important role in neural cell death. We assessed a therapeutic efficacy of Dock3 stimulation and p38 inhibition in retinal degeneration induced by optic nerve injury (ONI). In vivo retinal imaging using optical coherence tomography revealed that ONI-induced retinal degeneration was ameliorated in SB203580 (a p38 inhibitor)-treated WT mice and PBS-treated Dock3 overexpressing (Dock3 Tg) mice, and SB203580 further stimulated retinal protection in Dock3 Tg mice. In addition, SB203580 increased the number of regenerating axons after ONI in both WT and Dock3 Tg mice. ONI-induced phosphorylation of ASK1, p38 and the N-methyl-d-aspartate receptor 2B subunit were suppressed in the retina of Dock3 Tg mice. Inhibition of the ASK1 pathway in Dock3 Tg mice suggests that Dock3 may have an antioxidant-like property. These results indicate that overexpression of Dock3 and pharmacological interruption of p38 have synergistic effects for both neuroprotection and axon regeneration, thus combined application may be beneficial for the treatment of ONI. Copyright © 2014 Elsevier Ireland Ltd. All rights reserved.

  10. Large delay tunable slow-light based on high-gain stimulated-Brillouin-scattering amplification in optical fibers

    Institute of Scientific and Technical Information of China (English)

    XING Liang; ZHAN Li; XIA YuXing

    2009-01-01

    Tunable stimulated-Brillouin-scattering (SBS)-based slow-light in optical fibers has potential applications in optical buffering in the future all-optical router commutation systems.However,due to the low SBS threshold and relatively high realistic signal power,the gain in the usual SBS systems is limited at~30 dB.This paper presents a high-gain SBS scheme to realize large delay slow-light,which benefits from avoiding the depletion of the pump power in a short fiber as SBS media.The experiment demon strates that,up to 50 dB non-saturated gain has been observed in the single-stage 591.8 m fiber SBS amplification.The slow-light delay can be obtained 52 ns,and the fractional delay can exceed 1.

  11. NIR luminescent Er{sup 3+}/Yb{sup 3+} co-doped SiO{sub 2}-ZrO{sub 2} nanostructured planar and channel waveguides: Optical and structural properties

    Energy Technology Data Exchange (ETDEWEB)

    Cunha, Cesar dos Santos [Departamento de Quimica, Faculdade de Filosofia, Ciencias e Letras de Ribeirao Preto, Universidade de Sao Paulo, Av. Bandeirantes, 3900, 14040-901, Ribeirao Preto/SP (Brazil); Ferrari, Jefferson Luis [Grupo de Pesquisa em Quimica de Materiais - (GPQM), Departamento de Ciencias Naturais, Universidade Federal de Sao Joao Del Rei, Campus Dom Bosco, Praca Dom Helvecio, 74, 36301-160, Sao Joao Del Rei, MG (Brazil); Oliveira, Drielly Cristina de [Departamento de Quimica, Faculdade de Filosofia, Ciencias e Letras de Ribeirao Preto, Universidade de Sao Paulo, Av. Bandeirantes, 3900, 14040-901, Ribeirao Preto/SP (Brazil); Maia, Lauro June Queiroz [Grupo Fisica de Materiais, Instituto de Fisica, UFG, Campus Samambaia, Caixa Postal 131, 74001-970, Goiania/GO (Brazil); Gomes, Anderson Stevens Leonidas [Departamento de Fisica, Universidade Federal de Pernambuco, Cidade Universitaria, Recife/PE, 50670-901 (Brazil); Ribeiro, Sidney Jose Lima [Laboratorio de Materiais Fotonicos, Instituto de Quimica, UNESP, Caixa Postal 355, 14801-970, Araraquara/SP (Brazil); and others

    2012-09-14

    Optical and structural properties of planar and channel waveguides based on sol-gel Er{sup 3+} and Yb{sup 3+} co-doped SiO{sub 2}-ZrO{sub 2} are reported. Microstructured channels with high homogeneous surface profile were written onto the surface of multilayered densified films deposited on SiO{sub 2}/Si substrates by a femtosecond laser etching technique. The densification of the planar waveguides was evaluated from changes in the refractive index and thickness, with full densification being achieved at 900 Degree-Sign C after annealing from 23 up to 500 min, depending on the ZrO{sub 2} content. Crystal nucleation and growth took place together with densification, thereby producing transparent glass ceramic planar waveguides containing rare earth-doped ZrO{sub 2} nanocrystals dispersed in a silica-based glassy host. Low roughness and crack-free surface as well as high confinement coefficient were achieved for all the compositions. Enhanced NIR luminescence of the Er{sup 3+} ions was observed for the Yb{sup 3+}-codoped planar waveguides, denoting an efficient energy transfer from the Yb{sup 3+} to the Er{sup 3+} ion. Highlights: Black-Right-Pointing-Pointer Sol-gel high NIR luminescent nanostructured planar and channel waveguides. Black-Right-Pointing-Pointer Microstructured channels written by a femtosecond laser etching technique. Black-Right-Pointing-Pointer Transparent glass ceramic with rare earth-doped ZrO{sub 2} nanocrystals in a silica host. Black-Right-Pointing-Pointer Enhanced NIR luminescence, efficient energy transfer from the Yb{sup 3+} to the Er{sup 3+} ion. Black-Right-Pointing-Pointer New planar channel waveguides to be applied as EDWA in the C telecommunication band.

  12. Using independent component analysis to remove artifacts in visual cortex responses elicited by electrical stimulation of the optic nerve

    Science.gov (United States)

    Lu, Yiliang; Cao, Pengjia; Sun, Jingjing; Wang, Jing; Li, Liming; Ren, Qiushi; Chen, Yao; Chai, Xinyu

    2012-04-01

    In visual prosthesis research, electrically evoked potentials (EEPs) can be elicited by one or more biphasic current pulses delivered to the optic nerve (ON) through penetrating electrodes. Multi-channel EEPs recorded from the visual cortex usually contain large stimulus artifacts caused by instantaneous electrotonic current spread through the brain tissue. These stimulus artifacts contaminate the EEP waveform and often make subsequent analysis of the underlying neural responses difficult. This is particularly serious when investigating EEPs in response to electrical stimulation with long duration and multi-pulses. We applied independent component analysis (ICA) to remove these electrical stimulation-induced artifacts during the development of a visual prosthesis. Multi-channel signals were recorded from visual cortices of five rabbits in response to ON electrical stimulation with various stimulus parameters. ON action potentials were then blocked by lidocaine in order to acquire cortical potentials only including stimulus artifacts. Correlation analysis of reconstructed artifacts by ICA and artifacts recorded after blocking the ON indicates successful removal of artifacts from electrical stimulation by the ICA method. This technique has potential applications in studies designed to optimize the electrical stimulation parameters used by visual prostheses.

  13. Luminescence and the light emitting diode the basics and technology of leds and the luminescence properties of the materials

    CERN Document Server

    Williams, E W; Pamplin, BR

    2013-01-01

    Luminescence and the Light Emitting Diode: The Basics and Technology of LEDS and the Luminescence Properties of the Materials focuses on the basic physics and technology of light emitting diodes (LEDS) and pn junction lasers as well as their luminescence properties. Optical processes in semiconductors and the useful devices which can be made are discussed. Comprised of 10 chapters, this book begins with an introduction to the crystal structure and growth, as well as the optical and electrical properties of LED materials. The detailed fabrication of the LED is then considered, along with the lu

  14. Luminescence dating of ancient Darhad basin, Mongolia

    Science.gov (United States)

    Cheul Kim, Jin; Yi, Sangheon; Lim, Jaesoo; Kim, Ju-Yong

    2016-04-01

    . Thus, age control on existing 14C ages from this site is limited, chronological interpretation based on the 14C ages is still incomplete in Hodon outcrop sediments. OSL (Optically Stimulated Luminescence) is an alternative method for dating to overcome the problems associated with 14C methods. OSL has been extensively used for dating arctic sediments (Thomas et al., 2006; more). Previous optical ages on Darhad paleolake sediments obtained using IRSL (Infrared-stimulated luminescence) on feldspars (Gillespie et al., 2008; Batbaatar et al., 2009). Feldspar has much brighter luminescence than quartz, while the OSL signal of feldspars bleaches at least one order of magnitude slower than the OSL signal of quartz (Godfrey-Smith et al., 1988; Huntly and Lamothe, 2001; Mauz and Bungenstock, 2007; Kim et al., 2012). In glaciofluvial, glaciolacustrine environments, inadequate bleaching of the OSL signal is known to be a potential problem of burial ages (Thomas et al., 2006). OSL dating of permafrost deposits may also involve uncertainty about the inhomogeneous radiation field surrounding the dosimeter and the absorption of ionizing energy alternately by water and ice in a not-constant pore volume (Haeberli et al., 2003). In this study, we test the applicability of quartz OSL dating for the uppermost paleolake sediments in the Hodon outcrop of the Darhad basin. The OSL results were systematically compared with additional radiocarbon ages from wood fragments to conclude the reliability of the OSL dates and to construct intensive chronology for Late-Pleistocene Darhad paleolake. To evaluate the time of recent expansion of the paleolake, the northern piedmont (Talyn outcrop) of the basin was dated by OSL.

  15. Optically pumped infrared stimulated radiation in pr3+:Y2SiO5

    Institute of Scientific and Technical Information of China (English)

    Yanliang Zhang(张衍亮); Zhenrong Sun(孙真荣); Yuqiong Li(李玉琼); Liang'en Ding(丁良恩); Zugeng Wang(王祖赓)

    2003-01-01

    The infrared stimulated radiation of 1D2 → 3F.2 and 1D2 → 3H6 transitions in Pr3+:Y2SiO5 (YSO) viapulsed laser pumping has been observed. The threshold energy, temperature dependence and divergenceangle for the stimulated radiation are also measured.

  16. Cerenkov luminescence imaging of medical isotopes

    OpenAIRE

    Ruggiero, Alessandro; Holland, Jason P.; Lewis, Jason S.; Grimm, Jan

    2010-01-01

    The development of novel multimodality imaging agents and techniques represents the current frontier of research in the field of medical imaging science. However, the combination of nuclear tomography with optical techniques has yet to be established. Here, we report the use of the inherent optical emissions from the decay of radiopharmaceuticals for Cerenkov luminescence imaging (CLI) of tumors in vivo and correlate the results with those obtained from concordant immuno-PET studies.

  17. Heterodyne-detected stimulated photon echo: applications to optical dynamics in solution : applications to optical dynamics in solution

    NARCIS (Netherlands)

    de Boeij, W.P.; Pshenichnikov, M.S; Wiersma, D. A.

    1998-01-01

    Heterodyne detection of the stimulated photon echo (HSPE) is discussed and applied to explore molecular solvation dynamics. With this technique the in-phase and in-quadrature parts of the induced transient nonlinear polarization can be time-gated. A third-order perturbative description of the HSPE i

  18. A novel orange emitting Sm3+ ions doped NaCaAlPO4F3 phosphor: Optical and luminescence properties

    Science.gov (United States)

    Nagaraja, R.; Pushpa Manjari, V.; Sailaja, B.; Ravikumar, R. V. S. S. N.

    2017-02-01

    A novel orange light emitting Sm3+ ions doped NaCaAlPO4F3 phosphor was synthesized via solid state reaction. The prepared sample was characterized by powder X-ray diffraction (PXRD), Optical absorption, Photoluminescence (PL) and Fourier Transform Infrared Spectroscopy (FT-IR) techniques. From powder XRD data, the average crystallite size and structural parameters are estimated. Absorption spectra consist of ten absorption peaks corresponding to the transitions from the 6H5/2 ground state to various excited energy levels. Transition probabilities, branching ratios and radiative lifetime were evaluated by using Judd-Ofelt analysis. Photoluminescence spectrum show three prominent emission bands centered at 562, 597 and 643 nm corresponding to the 4G5/2 → 6HJ (J = 5/2, 7/2 and 9/2) transitions respectively. From the emission transitions, stimulated emission cross-section (σe) and gain bandwidth (GBW) were predicted. The decay profiles of the prepared phosphor reveals the single exponential nature and the experimental lifetime is calculated. The colorimetric parameters CIE coordinates, Correlated color temperature of the prepared phosphor are also evaluated. FT-IR spectrum demonstrates the characteristic vibration bands of the prepared phosphor material.

  19. Photo-stimulated electro-optic response of liquid-crystalline system with trans-cis photo-isomerizable agent

    Science.gov (United States)

    Hadjichristov, G. B.; Marinov, Y. G.; Yelamaggad, C. V.

    2014-12-01

    A rather strong photo-stimulated enhancement of photo-induced bend flexoelectric effect based on trans-cis photoisomerization of azo bond was found in a guest-host system formed from the nematic liquid crystal (LC) N-(4-methoxybenzylidene)-4-butylaniline (MBBA) as a host, and the azobenzene LC 4-hexyloxybenzoloxy-4'-cyanoazobenzene, as a guest photoactive agent at 1 wt.% concentration. Upon application of electric field, thin homeotropic layers of thickness 100 pm containing this photo-sensitized LC mixture were investigated as subjected to a relatively weak illumination with UV light (λ = 375 nm, from narrow-band light-emitting diode, LED). The stimulation of the photoactive electro-optic response of azobenzene-doped MBBA (owing to enhanced photo-induced bend flexoelectric effect driven by the photo-isomerizable dopants) was achieved by pre-resonant excitation of the photoactive agent. The degree of the effect measured is of potential interest for thin-film photoactive electro-optic applications. The UV light-induced effect in azobenzene-doped MBBA was reversible; the back (relaxation) process was stimulated by light in the blue from a LED with broadband spectrum centered at 455 nm.

  20. An Ideal System for Analysis and Interpretation of Ion Beam Induced Luminescence

    Science.gov (United States)

    Townsend, P. D.; Crespillo, M. L.

    Luminescence is produced during ion beam implantation or ion-solid interaction for most insulators, and contains rich information. Surprisingly, the information extracted is often far from optimum. Rather than summarizing literature work, the focus here is to design an optimized and feasible target chamber that could offer far more information than what has currently been obtained. Such an improved and multi-probe approach opens a range of options to simultaneously record luminescence spectra generated by the ion beam, explore transient and excited state signals via probes of secondary excitation methods (such as ionisation or photo-stimulation). In addition, one may monitor optical absorption, reflectivity and lifetime dependent features, plus stress and polarization factors. A particularly valuable addition to conventional measurements is to have the ability to modulate both the ion beam and the probes. These features allow separation of transient lifetimes, as well as sensing intermediate steps in the defect formation and/or relaxation, and growth of new phases and nanoparticle inclusions. While luminescence methods are the most sensitive probes of defect and imperfection sites in optically active materials, less work has been performed at controlled low and high temperatures. Measurement with controlled cooling or heating of the samples is effective to reveal phase transitions (both of host and inclusions). Furthermore, simultaneous excitations (e.g. ions and photons) at different temperatures may lead to different end-phase or stale structure under extreme ionization conditions and enable fabrication of unique material structures. References to the existing literature will underline that the overall benefits of studying ion beam induced luminescence can be far more fruitful than that has normally been considered.

  1. Optical dating of fluvio-deltaic clastic lake-fill sediments - A feasibility study in the Holocene Rhine delta (western Netherlands)

    NARCIS (Netherlands)

    Wallinga, J.; Bos, I.J.

    2010-01-01

    We test the applicability of quartz optically stimulated luminescence (OSL) dating on clastic lake sediments to investigate whether this dating method can be applied to study the timing and rate of deposition in Holocene fluvio-deltaic lakes. Our study concerns the filling of a lake by the Angstel-V

  2. Synthesis, luminescence and nonlinear optical properties of homoleptic tetracyanamidogermanates ARE[Ge(CN{sub 2}){sub 4}] (A = K, Cs, and RE = La, Ce, Pr, Nd, Sm, Eu, Gd)

    Energy Technology Data Exchange (ETDEWEB)

    Dolabdjian, Konstantin; Schedel, Christine; Meyer, Hans-Juergen [Abteilung fuer Festkoerperchemie und Theoretische Anorganische Chemie, Institut fuer Anorganische Chemie, Universitaet Tuebingen (Germany); Enseling, David; Juestel, Thomas [Fachbereich Chemieingenieurwesen, FH Muenster, Steinfurt (Germany)

    2017-04-04

    Two new series of tetracyanamidogermanates were prepared by solid-state reaction of appropriate amounts of REF{sub 3} (RE = rare earth), A{sub 2}[GeF{sub 6}] (A = alkaline), and Li{sub 2}(CN{sub 2}) in evacuated silica tubes. Powder X-ray diffraction patterns of crystalline samples of KRE[Ge(CN{sub 2}){sub 4}] and CsRE[Ge(CN{sub 2}){sub 4}] were indexed isotypically to KRE[Si(CN{sub 2}){sub 4}] and RbRE[Ge(CN{sub 2}){sub 4}], respectively. Luminescence properties of Ce{sup 3+}, Eu{sup 3+}, and Tb{sup 3+} doped compounds and non-linear optical properties (NLO) of KRE[Ge(CN{sub 2}){sub 4}] are reported. (copyright 2017 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  3. Optical stimulation of the hearing and deaf cochlea under thermal and stress confinement condition

    Science.gov (United States)

    Schultz, M.; Baumhoff, P.; Kallweit, N.; Sato, M.; Krüger, A.; Ripken, T.; Lenarz, T.; Kral, A.

    2014-03-01

    There is a controversy, to which extend cochlear stimulation with near infrared laser pulses at a wavelength of 1860 nm is based on optoacoustic stimulation of intact hair cells or -in contrast- is based on direct stimulation of the nerve cells in absence of functional hair cells. Thermal and stress confinement conditions apply, because of the pulse duration range (5 ns, 10 μs-20 ms) of the two lasers used. The dependency of the signal characteristics on pulse peak power and pulse duration was investigated in this study. The compound action potential (CAP) was measured during stimulation of the cochlea of four anaesthetized guinea pigs, which were hearing at first and afterwards acutely deafened using intracochlear neomycin-rinsing. For comparison hydrophone measurements in a water tank were performed to investigate the optoacoustic signals at different laser interaction regimes. With rising pulse peak power CAPs of the hearing animals showed first a threshold, then a positively correlated and finally a saturating dependency. CAPs also showed distinct responses at laser onset and offset separated with the pulse duration. At pulse durations shorter than physiological response times the signals merged. Basically the same signal characteristics were observed in the optoacoustic hydrophone measurements, scaled with the sensitivity and response time of the hydrophone. Taking together the qualitative correspondence in the signal response and the absence of any CAPs in deafened animals our results speak in favor of an optoacoustic stimulation of intact hair cells rather than a direct stimulation of nerve cells.

  4. Photostimulated luminescence properties of Eu2+ -doped barium aluminate phosphor.

    Science.gov (United States)

    He, Quanlong; Qiu, Guangyu; Xu, Xuhui; Qiu, Jianbei; Yu, Xue

    2015-03-01

    An intense green photostimulated luminescence in BaAl2 O4 :Eu(2+) phosphor was prepared. The thermoluminescence results indicate that there are at least three types of traps (T1 , T2 , T3 ) with different trap depths in BaAl2 O4 :Eu(2+) phosphor according to the bands located at 327, 361 and 555 K, respectively, which are closely associated with the phosphor's long persistent luminescence and photostimulated luminescence properties. In addition, as a novel optical read-out form, a photostimulated persistent luminescence signal can be repeatedly obtained in BaAl2 O4 :Eu(2+) phosphor. This shows that re-trapping of the electron released from a deep trap plays an important role in photostimulated persistent luminescence.

  5. The influence of Ag{sup 9+} ion irradiation on the structural, optical and luminescence properties of Sm{sup 3+} doped NaSrBO{sub 3}: Stability of color emission

    Energy Technology Data Exchange (ETDEWEB)

    Bedyal, A.K. [School of Physics, Shri Mata Vaishno Devi University, Katra 182320 - J& K (India); Kumar, Vinay, E-mail: vinaykumar@smvdu.ac.in [School of Physics, Shri Mata Vaishno Devi University, Katra 182320 -J& K (India); Department of Physics, University of the Free State, P.O. Box 339, Bloemfontein, ZA 9300 (South Africa); Singh, Vivek K. [School of Physics, Shri Mata Vaishno Devi University, Katra 182320 - J& K (India); Singh, Fouran; Lochab, S.P. [Inter University Accelerator Centre, Anura Asaf Ali Marg, P.O. Box 10502, New Delhi 110067 (India); Ntwaeaborwa, O.M.; Swart, H.C. [Department of Physics, University of the Free State, P.O. Box 339, Bloemfontein, ZA 9300 (South Africa)

    2015-05-15

    Highlights: •120 MeV Ag{sup 9+} ion irradiation modified the structure, optical and luminescence properties of NaSrBO{sub 3}: Sm{sup 3+} phosphor. •The phosphor is synthesized by the solid state reaction and combustion method. •Colour statibilty confirmed by CIE coordinates after ion irradiations. -- Abstract: This paper reports on the effect of 120 MeV Ag{sup 9+} ion irradiation on the structure, optical and luminescence properties of NaSr{sub 1−x}BO{sub 3}: xSm{sup 3+} (x = 0.5–2.5 mol.%) phosphor, synthesized by the solid state reaction and combustion method. The samples were irradiated with Ag{sup 9+} swift heavy ions (SHIs) using fluences of 1 × 10{sup 12} ions cm{sup −2}, 5 × 10{sup 12} ions cm{sup −2} and 1 × 10{sup 13} ions cm{sup −2}. The as-prepared as well as irradiated samples were characterized by X-ray diffraction (XRD), diffuse reflectance (DR) and photoluminescence (PL) techniques. After irradiation, the structure of the phosphor did not change except that the loss of crystallinity which may be due to the fragmentation caused by the SHI. DR spectra reflect a blue shift in the absorption band with increasing fluences, for phosphors prepared using both solid state reaction and combustion method, resulting in an increase in the band gap from 5.64 to 6.06 eV. The PL intensity of the phosphors was enhanced with an increase in ion fluences, with the samples prepared using a combustion method exhibiting prominent intensity. The CIE coordinates were calculated and they correspond to the shade of orange–red emission of the Sm{sup 3+} ions.

  6. Investigation on the effect of beam divergence angle upon output waveform based on stimulated Brillouin scattering optical limiting

    Institute of Scientific and Technical Information of China (English)

    Hasi Wu-Li-Ji; Lu Huan-Huan; Gong Sheng; Fu Mei-Ling; Lin Zhi-Wei; Lin Dian-Yang; He Wei-Ming

    2009-01-01

    This paper investigates the effect of beam divergence angle on output waveform based on stimulated Brillouin scattering optical limiting. Output waveforms in the case of different pump divergence angles are numerically simulated,and validated in a Nd:YAG seed-injected laser system. The results indicate that a small pump divergence angle can lead to good interaction between pump and Stokes, and a platform can be easily realized in the transmitted waveform.In contrast, a peak followed by the platform appears when the divergence angle becomes large.

  7. Construction and use of a zebrafish heart voltage and calcium optical mapping system, with integrated electrocardiogram and programmable electrical stimulation.

    Science.gov (United States)

    Lin, Eric; Craig, Calvin; Lamothe, Marcel; Sarunic, Marinko V; Beg, Mirza Faisal; Tibbits, Glen F

    2015-05-01

    Zebrafish are increasingly being used as a model of vertebrate cardiology due to mammalian-like cardiac properties in many respects. The size and fecundity of zebrafish make them suitable for large-scale genetic and pharmacological screening. In larger mammalian hearts, optical mapping is often used to investigate the interplay between voltage and calcium dynamics and to investigate their respective roles in arrhythmogenesis. This report outlines the construction of an optical mapping system for use with zebrafish hearts, using the voltage-sensitive dye RH 237 and the calcium indicator dye Rhod-2 using two industrial-level CCD cameras. With the use of economical cameras and a common 532-nm diode laser for excitation, the rate dependence of voltage and calcium dynamics within the atrial and ventricular compartments can be simultaneously determined. At 140 beats/min, the atrial action potential duration was 36 ms and the transient duration was 53 ms. With the use of a programmable electrical stimulator, a shallow rate dependence of 3 and 4 ms per 100 beats/min was observed, respectively. In the ventricle the action potential duration was 109 ms and the transient duration was 124 ms, with a steeper rate dependence of 12 and 16 ms per 100 beats/min. Synchronous electrocardiograms and optical mapping recordings were recorded, in which the P-wave aligns with the atrial voltage peak and R-wave aligns with the ventricular peak. A simple optical pathway and imaging chamber are detailed along with schematics for the in-house construction of the electrocardiogram amplifier and electrical stimulator. Laboratory procedures necessary for zebrafish heart isolation, cannulation, and loading are also presented.

  8. NIR luminescence studies on Er{sup 3+}:Yb{sup 3+} co-doped sodium telluroborate glasses for lasers and optical amplifer applications

    Energy Technology Data Exchange (ETDEWEB)

    Annapoorani, K.; Marimuthu, K., E-mail: mari-ram2000@yahoo.com [Department of Physics, Gandhigram Rural Institute - Deemed University, Gandhigram – 624 302 (India); Murthy, N. Suriya [Radiological Safety Division, Indira Gandhi Centre for Atomic Research, Kalpakkam–603 102 (India)

    2016-05-23

    Er{sup 3+}:Yb{sup 3+} co-doped Sodium telluroborate glasses were prepared with the chemical composition (49.5–x)B{sub 2}O{sub 3}+25TeO{sub 2}+5Li{sub 2}CO{sub 3}+10ZnO+10NaF+0.5Er{sub 2}O{sub 3}+xYb{sub 2}O{sub 3} (where x= 0.1, 0.5, 1.0 and 2.0 in mol %) following the melt quenching technique. With the addition of Yb{sup 3+} ions into Er{sup 3+} ions in the prepared glasses, the absorption cross-section values were found to increase due to the effective energy transfer from {sup 2}F{sub 5/2} level of Yb{sup 3+} ions to the {sup 4}I{sub 11/2} level of Er{sup 3+} ions. The fluorescence around 1550 nm correspond to the {sup 4}I{sub 13/2}→{sup 4}I{sub 15/2} transition was observed under 980 nm pumping. Among the present glasses, integrated intensity was found to be higher for 1.0 mol% Yb{sup 3+} ion glass. The parameters such as stimulated emission cross- section, Gain bandwidth and quantum efficiency of the {sup 4}I{sub 13/2}→{sup 4}I{sub 15/2} transition was found to be higher for the NTBE1.0Y glass and the same is suggested for potential NIR lasers and optical amplifier applications.

  9. Photoluminescence of an Yb3+/Al3+-codoped microstructured optical fibre

    Institute of Scientific and Technical Information of China (English)

    Xia Chang-Ming; Zhou Gui-Yao; Han Ying; Hou Lan-Tian

    2011-01-01

    An Yb3+/Al3+-codoped microstructured optical fibre is prepared based on photonic crystal fibre technology.The characteristic spectra of preforms and fibres are experimentally investigated.The results show that under a 971 nm excitation,besides the known infrared fluorescence luminescence around 1050 nm,a blue luminescence peak at 486 nm is obtained.Moreover,an unexpected emission peak at 730 nm is also observed.The photoluminescence mechanism of an Yb3+/Al3+-codoped microstructured optical fibre is discussed.The emission peak at 486 nm is attributed to the cooperative upconversion resulting from pairs of Yb3+ions,and the emission peak around 730 nm is ascribed to the stimulated Raman scattering because of nonlinear effects of microstructured optical fibre.The Yb3+/Al3+-codoped microstructured optical fibre is promising for varieties of applications from laser printing and optical recording to cancer treatments,such as photodynamic therapy.

  10. Optical dating of the anastasia formation, northeastern florida, USA

    Science.gov (United States)

    Burdette, K.E.; Rink, J.W.; Means, G.H.; Portell, R.W.

    2009-01-01

    The single-aliquot regenerative-dose (SAR) procedure was used to obtain optically stimulated luminescence ages to determine the depositional age of the upper part of the Anastasia Formation. This unit, which crops out along the east coast of Florida, is one of the most culturally and economically important coquina deposits in North America. Rock samples from the upper three meters of exposure at three locations were collected. Additional materials for paleontological analysis were also taken. Based on our samples, the luminescence ages of the Anastasia Formation are well within marine isotope stage 5, which is supported by the results of Osmond et al. (1970) based on U/Th ages. The associated fossil assemblages support our luminescence age determinations. Associated fossils fall within the Rancholabrean North American Land Mammal Age (300 10 ka) and the fossil mollusk assemblage consists entirely of modern species.

  11. Optical response of the graded-gap Al sub x Ga sub 1 sub - sub x As X-ray detector

    CERN Document Server

    Pozela, K; Dapkus, L; Jasutis, V; Silenas, A; Smith, K M; Bendorius, R A

    2001-01-01

    It has been observed that only a part of the Al sub x Ga sub 1 sub - sub x As graded-gap layer with the energy gap gradient g>20 eV/cm is active as a X-ray luminescence source. The thickness of the active layer is 30-50 mu m. To increase the detectors optical response efficiency, the following methods are proposed and tested: - Reflection of the X-ray luminescence light, generated in the bulk Al sub x Ga sub 1 sub - sub x As layer, inside the total reflection angle theta; - Optical stimulation of the electron-hole radiative recombination.

  12. Luminescence Dating of Marine Terrace Sediments Between Trabzon and Rize, Eastern Black Sea Basin: Preliminary Results

    Science.gov (United States)

    Softa, Mustafa; Spencer, Joel Q. G.; Emre, Tahir; Sözbilir, Hasan; Turan, Mehmet

    2016-04-01

    Quaternary marine terraces in the coastal region of Pontides in Northeastern Turkey are valuable archives of past sea level change. Until recently, dates of raised marine terraces undeciphered in the coastal region between Trabzon and Rize because of chronologic limitations. In this paper was to determine ages of the terrace deposits by applying optically stimulated luminescence (OSL) dating methods using single aliquot regenerative dose (SAR) techniques on quartz minerals from extracted marine terraces. Several samples were collected from three orders of Quaternary marine terraces which are reproducible at all sampling location in between cities of Trabzon and Rize, Turkey, coastal of Eastern Pontides, at the front of the thrust system. The terrace deposits mainly consist of clays, silts, sands and gravels. The sediments in these deposits are mainly derived from basaltic, andesitic, and limestone geology, and have elipsoid, square and flat shapes. The terrace deposits have heights ranging from 1 to 17 meters and increases in height and thickness from west to east. Initial OSL results from 1 mm and 3 mm quartz aliquots demonstrate good luminescence characteristics. Preliminary equivalent dose analysis results ranging from 17.6 Gy to 79.6 Gy have been calculated using the Central Age Model (CAM) and Minimum Age Model (MAM). According to ages obtained from three separate terrace is ~8 ka, ~42 ka and ~78 ka, respectively. Results of marine terrace sediments indicate this region has three sedimentation periods and coastal region of Pontides has been remarkably tectonically active since latest Pleistocene to earlier Holocene. This study will present preliminary OSL dating results obtained from samples of Quaternary marine terrace formation. Keywords: optically stimulated luminescence (OSL) dating, single grain, marine terraces, Eastern Pontides.

  13. Local analysis of stimulated Brillouin interaction in installed fiber optics cables

    OpenAIRE

    Nikles, M.; Thévenaz, Luc; Salina, P.; Robert, P. A.

    1996-01-01

    Brillouin gain spectrum measurement along an optical fiber has recently gained a lot of interests owing to its potentiality for strain monitoring in installed telecom cables. The purpose of the paper is to show that this potentiality is now effective, since field measurements of installed fiber optics cables currently in operation are demonstrated. A portable instrument has been developed, based on an original experimental configuration developed in our Institute which is briefly described

  14. Luminescence properties of common salt (NaCl available in Nigeria for use as accident dosimeter in radiological emergency situation

    Directory of Open Access Journals (Sweden)

    Janet Ayobami Ademola

    2017-04-01

    Full Text Available In the event of a radiological accident or attack, it is important to assess and quantify radiation dose to the population. This could be done using materials in the vicinity that are sensitive to ionizing radiation. Common salt (NaCl is known to be a sensitive thermoluminescence (TL phosphor. Luminescence properties of common salt (NaCl used in Nigeria were investigated using an automated luminescence reader Risø TL/OSL-DA-15, with attention focused more on the Optically Stimulated Luminescence (OSL. Strong radiation-induced TL and OSL signals were observed. The TL peaks occurred at about 100 °C, 240 °C and 280 °C. The dose response of both the TL and OSL signals showed a linear relationship. From the OSL pulse anneal curve with TL curve, a preheat temperature of 190 °C for 10 s was found adequate for the OSL measurements. There was no significant difference in the OSL decay for stimulation temperatures of 100 and 120 °C. Fading experiment over a storage period of 14 days showed about 13 and 3% decrease in the OSL signal of sample 1 and sample 2, respectively. The ratios of measured to given dose for dose recovery test were within ±19% of unity. Within the limit of error the samples could be used as a complementary emergency dosimeter in radiological accident situation.

  15. 无线光刺激与神经传感系统%Wireless neural sensing system integrated optical stimulation

    Institute of Scientific and Technical Information of China (English)

    袁明军; 岳森; 张云鹏; 赵晓东; 王守岩

    2016-01-01

    Neuromodulation based on optogenetics is developed toward closed-loop control,a wireless light stimulation and neural sensing system is developed for requirements of free moving of test animal which has functions of larger range of optical stimulation,synchronous record,wireless programmable,which contains light stimulation-electric record neural interface,a stimulating and sensing module,a wireless transceiver module and upper PC software. The device can adjust light stimulation frequency,amplitude,duty ratio wirelessly and in real-time and synchronously acquire neural signal. The animal experiment shows that 30 Hz light stimulation at motor cortex movement of the mice is obviously enhanced,and EEG signal provoked by stimulation is recorded simultaneously. The system provides a multifunction neural regulation platform for optogenetics,which is beneficial to long schedule research for neural circuit and neural disease.%光遗传神经调控正在向闭环技术发展,针对实验动物可自由活动的需求,研发具有大范围光刺激、神经信号同步记录、无线程控等功能的无线光刺激与神经传感系统。该系统包括光刺激—电记录神经接口、刺激传感模块、无线收发模块以及上位机软件。可无线实时调节光刺激频率、幅度和占空比等参数,并同步采集神经信号。给予小鼠刺激运动皮层30Hz光刺激,小鼠运动明显增强,同时记录到刺激诱发的脑电信号。系统为光遗传技术提供多功能神经调控平台,有助于神经环路和神经疾病的长时程研究。

  16. Modeling Light Propagation in Luminescent Media

    Science.gov (United States)

    Sahin, Derya

    This study presents physical, computational and analytical modeling approaches for light propagation in luminescent random media. Two different approaches are used, namely (i) a statistical approach: Monte-Carlo simulations for photon transport and (ii) a deterministic approach: radiative transport theory. Both approaches account accurately for the multiple absorption and reemission of light at different wavelengths and for anisotropic luminescence. The deterministic approach is a generalization of radiative transport theory for solving inelastic scattering problems in random media. We use the radiative transport theory to study light propagation in luminescent media. Based on this theory, we also study the optically thick medium. Using perturbation methods, a corrected diffusion approximation with asymptotically accurate boundary conditions and a boundary layer solution are derived. The accuracy and the efficacy of this approach is verified for a plane-parallel slab problem. In particular, we apply these two approaches (MC and radiative transport theory) to model light propagation in semiconductor-based luminescent solar concentrators (LSCs). The computational results for both approaches are compared with each other and found to agree. The results of this dissertation present practical and reliable techniques to use for solving forward/inverse inelastic scattering problems arising in various research areas such as optics, biomedical engineering, nuclear engineering, solar science and material science.

  17. Yellow luminescence of gallium nitride generated by carbon defect complexes.

    Science.gov (United States)

    Demchenko, D O; Diallo, I C; Reshchikov, M A

    2013-02-22

    We demonstrate that yellow luminescence often observed in both carbon-doped and pristine GaN is the result of electronic transitions via the C(N)-O(N) complex. In contrast to common isolated defects, the C(N)-O(N) complex is energetically favorable, and its calculated optical properties, such as absorption and emission energies, a zero phonon line, and the thermodynamic transition level, all show excellent agreement with measured luminescence data. Thus, by combining hybrid density functional theory and experimental measurements, we propose a solution to a long-standing problem of the GaN yellow luminescence.

  18. LUMINESCENCE OF CADMIUM SULFIDE QUANTUM DOTS IN FLUOROPHOSPHATE GLASSES

    OpenAIRE

    Z. O. Lipatova; E. V. Kolobkova; V. A. Aseev

    2015-01-01

    Cadmium sulfide quantum dots are perspective materials in optics, medicine, biology and optoelectronics. Fluorophosphate glasses, doped with cadmium sulfide quantum dots, were examined in the paper. Heat treatment led to the formation of quantum dots with diameters equal to 2.8 nm, 3.0 nm and 3.8 nm. In view of such changes in the quantum dots size the fundamental absorption edge shift and the luminescence band are being displaced to the long wavelengths. Luminescence lifetime has been fou...

  19. Study of optical absorption, visible emission and NIR–vis luminescence spectra of Tm{sup 3+}/Yb{sup 3+}, Ho{sup 3+}/Yb{sup 3+} and Tm{sup 3+}/Ho{sup 3+}/Yb{sup 3+} doped tellurite glasses

    Energy Technology Data Exchange (ETDEWEB)

    Seshadri, M., E-mail: seshumeruva@gmail.com [Institute of Physics, University of Campinas, UNICAMP, P.O. Box 6165, Campinas 13083-970 (Brazil); Barbosa, L.C.; Cordeiro, C.M.B.; Radha, M. [Institute of Physics, University of Campinas, UNICAMP, P.O. Box 6165, Campinas 13083-970 (Brazil); Sigoli, F.A. [Institute of Chemistry, University of Campinas, UNICAMP, P.O. Box 6154, Campinas 13083-970 (Brazil); Ratnakaram, Y.C. [Department of Physics, Sri Venkateswara University, SVU, Tirupat 517502 (India)

    2015-10-15

    Tm{sup 3+}/Yb{sup 3+}, Ho{sup 3+}/Yb{sup 3+} co-doped and Tm{sup 3+}/Ho{sup 3+}/Yb{sup 3+} triply doped TeO{sub 2}–Bi{sub 2}O{sub 3}–ZnO–Li{sub 2}O–Nb{sub 2}O{sub 5} (TBZLN) tellurite glasses were prepared by melt quenching method. Judd–Ofelt intensity parameters (Ω{sub λ}, λ=2, 4 and 6), radiative transition probabilities, branching ratios and radiative lifetimes of Tm{sup 3+}, Ho{sup 3+} ions in co-doped TBZLN glasses were calculated from the optical absorption spectra. Excitation, visible luminescence and decay lifetimes in visible region were also investigated. The stimulated emission and gain cross-sections for the Tm{sup 3+}:{sup 3}F{sub 4}→{sup 3}H{sub 6} (1700 nm) and Ho{sup 3+}:{sup 5}I{sub 7}→{sup 5}I{sub 8} (1956 nm) transitions in co-doped TBZLN glasses have been analyzed and compared with those of other reported glasses. Up-conversion luminescence was observed in TBZLN glasses under 980 nm laser excitation and energy transfer mechanisms have been discussed. Finally, CIE color co-ordinates were calculated and it is observed that the color co-ordinates fall in blue and green regions for Tm{sup 3+}/Yb{sup 3+} and Ho{sup 3+}/Yb{sup 3+} co-doped TBZLN glasses, respectively. A subsequent shift in color co-ordinates from green to greenish-yellow region has been observed with an increase in the concentration (0.1, 0.5 and 1.0 mol%) of Tm{sup 3+} ions in Tm{sup 3+}/Ho{sup 3+}/Yb{sup 3+} triply doped TBZLN glasses. - Highlights: • High degree of covalecy of RE–O bond in co-doped TBZLN glasses was observed. • Tm{sup 3+}:{sup 1}D{sub 2}→{sup 3}F{sub 4} and Ho{sup 3+}:{sup 5}F{sub 4}({sup 5}S{sub 2})→{sup 5}I{sub 8} transitions show high emission cross-section. • Visible and strong 793 nm emission was observed when pumped by 980 nm diode laser. • Triply doped glasses exhibits tunable emission intensity by increasing Tm{sup 3+} ions.

  20. Chemically engineered persistent luminescence nanoprobes for bioimaging

    Science.gov (United States)

    Lécuyer, Thomas; Teston, Eliott; Ramirez-Garcia, Gonzalo; Maldiney, Thomas; Viana, Bruno; Seguin, Johanne; Mignet, Nathalie; Scherman, Daniel; Richard, Cyrille

    2016-01-01

    Imaging nanoprobes are a group of nanosized agents developed for providing improved contrast for bioimaging. Among various imaging probes, optical sensors capable of following biological events or progresses at the cellular and molecular levels are actually actively developed for early detection, accurate diagnosis, and monitoring of the treatment of diseases. The optical activities of nanoprobes can be tuned on demand by chemists by engineering their composition, size and surface nature. This review will focus on researches devoted to the conception of nanoprobes with particular optical properties, called persistent luminescence, and their use as new powerful bioimaging agents in preclinical assays. PMID:27877248