WorldWideScience

Sample records for nonlinear optical methods

  1. Nonlinear optics

    International Nuclear Information System (INIS)

    Boyd, R.W.

    1992-01-01

    Nonlinear optics is the study of the interaction of intense laser light with matter. This book is a textbook on nonlinear optics at the level of a beginning graduate student. The intent of the book is to provide an introduction to the field of nonlinear optics that stresses fundamental concepts and that enables the student to go on to perform independent research in this field. This book covers the areas of nonlinear optics, quantum optics, quantum electronics, laser physics, electrooptics, and modern optics

  2. Nonlinear optics

    CERN Document Server

    Bloembergen, Nicolaas

    1996-01-01

    Nicolaas Bloembergen, recipient of the Nobel Prize for Physics (1981), wrote Nonlinear Optics in 1964, when the field of nonlinear optics was only three years old. The available literature has since grown by at least three orders of magnitude.The vitality of Nonlinear Optics is evident from the still-growing number of scientists and engineers engaged in the study of new nonlinear phenomena and in the development of new nonlinear devices in the field of opto-electronics. This monograph should be helpful in providing a historical introduction and a general background of basic ideas both for expe

  3. Nonlinear optics

    CERN Document Server

    Boyd, Robert W

    2013-01-01

    Nonlinear Optics is an advanced textbook for courses dealing with nonlinear optics, quantum electronics, laser physics, contemporary and quantum optics, and electrooptics. Its pedagogical emphasis is on fundamentals rather than particular, transitory applications. As a result, this textbook will have lasting appeal to a wide audience of electrical engineering, physics, and optics students, as well as those in related fields such as materials science and chemistry.Key Features* The origin of optical nonlinearities, including dependence on the polarization of light* A detailed treatment of the q

  4. Kyropoulos method for growth of nonlinear optical organic crystal ABP (4-aminobenzophenone) from the melt

    Science.gov (United States)

    Pan, Shoukui; Okano, Y.; Tsunekawa, S.; Fukuda, T.

    1993-03-01

    The Kyropoulus method was used to grow nonlinear optical organic crystals ABP (4-aminobenzophenone). The crystals were characterized by nonlinear optical measurements and had a large effect of frequency doubling.

  5. Nonlinear Optical Terahertz Technology

    Data.gov (United States)

    National Aeronautics and Space Administration — We develop a new approach to generation of THz radiation. Our method relies on mixing two optical frequency beams in a nonlinear crystalline Whispering Gallery Mode...

  6. Advances in nonlinear optics

    CERN Document Server

    Chen, Xianfeng; Zeng, Heping; Guo, Qi; She, Weilong

    2015-01-01

    This book presents an overview of the state of the art of nonlinear optics from weak light nonlinear optics, ultrafast nonlinear optics to electro-optical theory and applications. Topics range from the fundamental studies of the interaction between matter and radiation to the development of devices, components, and systems of tremendous commercial interest for widespread applications in optical telecommunications, medicine, and biotechnology.

  7. Nonlinear optical properties measurement of polypyrrole -carbon nanotubes prepared by an electrochemical polymerization method

    Directory of Open Access Journals (Sweden)

    Shahriari

    2017-02-01

    Full Text Available In this work, the optical properties dependence of Multi-Walled Carbon Nanotubes (MWNT on concentration was discussed. MWNT samples were prepared in polypyrrole by an electrochemical polymerization of monomers, in the presence of different concentrations of MWNTs, using Sodium Dodecyl-Benzen-Sulfonate (SDBS as surfactant at room temperature. The nonlinear refractive and nonlinear absorbtion indices were measured using a low power CW laser beam operated at 532 nm using z-scan method. The results show that nonlinear refractive and nonlinear absorbtion indices tend to be increased with increasing the concentration of carbon nanotubes. Optical properties of  carbone nanotubes indicate that they are good candidates for nonlinear optical devices

  8. Structural, optical and nonlinear optical studies of AZO thin film prepared by SILAR method for electro-optic applications

    Science.gov (United States)

    Edison, D. Joseph; Nirmala, W.; Kumar, K. Deva Arun; Valanarasu, S.; Ganesh, V.; Shkir, Mohd.; AlFaify, S.

    2017-10-01

    Aluminium doped (i.e. 3 at%) zinc oxide (AZO) thin films were prepared by simple successive ionic layer adsorption and reaction (SILAR) method with different dipping cycles. The structural and surface morphology of AZO thin films were studied by using X-ray diffraction (XRD) and scanning electron microscopy (SEM). The optical parameters such as, transmittance, band gap, refractive index, extinction coefficient, dielectric constant and nonlinear optical properties of AZO films were investigated. XRD pattern revealed the formation of hexagonal phase ZnO and the intensity of the film was found to increase with increasing dipping cycle. The crystallite size was found to be in the range of 29-37 nm. Scanning Electron Microscope (SEM) images show the presence of small sized grains, revealing that the smoothest surface was obtained at all the films. The EDAX spectrum of AZO conforms the presence of Zn, O and Al. The optical transmittance in the visible region is high 87% and the band gap value is 3.23 eV. The optical transmittance is decreased with respect to dipping cycles. The room temperature PL studies revealed that the AZO films prepared at (30 cycles) has good film quality with lesser defect density. The third order nonlinear optical parameters were also studied using Z-scan technique to know the applications of deposited films in nonlinear devices. The third order nonlinear susceptibility value is found to be 1.69 × 10-7, 3.34 × 10-8, 1.33 × 10-7and 2.52 × 10-7 for AZO films deposited after 15, 20, 25 and 30 dipping cycles.

  9. Nonlinear fibre optics overview

    DEFF Research Database (Denmark)

    Travers, J. C.; Frosz, Michael Henoch; Dudley, J. M.

    2010-01-01

    The optical fiber based supercontinuum source has recently become a significant scientific and commercial success, with applications ranging from frequency comb production to advanced medical imaging. This one-of-a-kind book explains the theory of fiber supercontinuum broadening, describes......, provides a background to the associated nonlinear optical processes, treats the generation mechanisms from continuous wave to femtosecond pulse pump regimes and highlights the diverse applications. A full discussion of numerical methods and comprehensive computer code are also provided, enabling readers...

  10. Nonlinear Optics and Applications

    Science.gov (United States)

    Abdeldayem, Hossin A. (Editor); Frazier, Donald O. (Editor)

    2007-01-01

    Nonlinear optics is the result of laser beam interaction with materials and started with the advent of lasers in the early 1960s. The field is growing daily and plays a major role in emerging photonic technology. Nonlinear optics play a major role in many of the optical applications such as optical signal processing, optical computers, ultrafast switches, ultra-short pulsed lasers, sensors, laser amplifiers, and many others. This special review volume on Nonlinear Optics and Applications is intended for those who want to be aware of the most recent technology. This book presents a survey of the recent advances of nonlinear optical applications. Emphasis will be on novel devices and materials, switching technology, optical computing, and important experimental results. Recent developments in topics which are of historical interest to researchers, and in the same time of potential use in the fields of all-optical communication and computing technologies, are also included. Additionally, a few new related topics which might provoke discussion are presented. The book includes chapters on nonlinear optics and applications; the nonlinear Schrodinger and associated equations that model spatio-temporal propagation; the supercontinuum light source; wideband ultrashort pulse fiber laser sources; lattice fabrication as well as their linear and nonlinear light guiding properties; the second-order EO effect (Pockels), the third-order (Kerr) and thermo-optical effects in optical waveguides and their applications in optical communication; and, the effect of magnetic field and its role in nonlinear optics, among other chapters.

  11. Investigation of nonlinear optical properties of various organic materials by the Z-scan method

    Science.gov (United States)

    Ganeev, R. A.; Boltaev, G. S.; Tugushev, R. I.; Usmanov, T.

    2012-06-01

    We have studied the nonlinear optical properties of various organic materials (vegetable oil, juice, wine, cognac, Coca-Cola and Fanta drinks, Nescafé coffee, tea, gasoline, clock oil, glycerol, and polyphenyl ether) that are used in everyday life. Their nonlinearities have been studied by the Z-scan method in the near-IR and visible spectral ranges. We have shown that the majority of samples possess a nonlinear absorption; however, some of the studied materials show a strong saturated absorption and nonlinear refraction. Red wine and glycerol proved to be the most interesting materials. For these samples, we have observed a change in the sign of the nonlinear absorption with increasing laser intensity, which was attributed to the competition between two-photon absorption and saturated absorption.

  12. Quantum Nonlinear Optics

    CERN Document Server

    Hanamura, Eiichi; Yamanaka, Akio

    2007-01-01

    This graduate-level textbook gives an introductory overview of the fundamentals of quantum nonlinear optics. Based on the quantum theory of radiation, Quantum Nonlinear Optics incorporates the exciting developments in novel nonlinear responses of materials (plus laser oscillation and superradiance) developed over the past decade. It deals with the organization of radiation field, interaction between electronic system and radiation field, statistics of light, mutual manipulation of light and matter, laser oscillation, dynamics of light, nonlinear optical response, and nonlinear spectroscopy, as well as ultrashort and ultrastrong laser pulse. Also considered are Q-switching, mode locking and pulse compression. Experimental and theoretical aspects are intertwined throughout.

  13. Nonlinear optical systems

    CERN Document Server

    Lugiato, Luigi; Brambilla, Massimo

    2015-01-01

    Guiding graduate students and researchers through the complex world of laser physics and nonlinear optics, this book provides an in-depth exploration of the dynamics of lasers and other relevant optical systems, under the umbrella of a unitary spatio-temporal vision. Adopting a balanced approach, the book covers traditional as well as special topics in laser physics, quantum electronics and nonlinear optics, treating them from the viewpoint of nonlinear dynamical systems. These include laser emission, frequency generation, solitons, optically bistable systems, pulsations and chaos and optical pattern formation. It also provides a coherent and up-to-date treatment of the hierarchy of nonlinear optical models and of the rich variety of phenomena they describe, helping readers to understand the limits of validity of each model and the connections among the phenomena. It is ideal for graduate students and researchers in nonlinear optics, quantum electronics, laser physics and photonics.

  14. Polarization Nonlinear Optics of Quadratically Nonlinear Azopolymers

    International Nuclear Information System (INIS)

    Konorov, S.O.; Akimov, D.A.; Ivanov, A.A.; Petrov, A.N.; Alfimov, M.V.; Yakimanskii, A.V.; Smirnov, N.N.; Ivanova, V.N.; Kudryavtsev, V.V.; Podshivalov, A.A.; Sokolova, I.M.; Zheltikov, A.M.

    2005-01-01

    The polarization properties of second harmonic and sum-frequency signals generated by femtosecond laser pulses in films of polymers containing covalent groups of an azobenzothiazole chromophore polarized by an external electric field are investigated. It is shown that the methods of polarization nonlinear optics make it possible to determine the structure of oriented molecular dipoles and reveal important properties of the motion of collectivized πelectrons in organic molecules with strong optical nonlinearities. The polarization measurements show that the tensor of quadratic nonlinear optical susceptibility of chromophore fragments oriented by an external field in macromolecules of the noted azopolymers has a degenerate form. This is indicative of a predominantly one-dimensional character of motion of collectivized π electrons along an extended group of atoms in such molecules

  15. Photostable nonlinear optical polycarbonates

    NARCIS (Netherlands)

    Faccini, M.; Balakrishnan, M.; Diemeer, Mart; Torosantucci, Riccardo; Driessen, A.; Reinhoudt, David; Verboom, Willem

    2008-01-01

    Highly thermal and photostable nonlinear optical polymers were obtained by covalently incorporating the tricyanovinylidenediphenylaminobenzene (TCVDPA) chromophore to a polycarbonate backbone. NLO polycarbonates with different chromophore attachment modes and flexibilities were synthesized. In spite

  16. Geometrical optics analysis of the structural imperfection of retroreflection corner cubes with a nonlinear conjugate gradient method.

    Science.gov (United States)

    Kim, Hwi; Min, Sung-Wook; Lee, Byoungho

    2008-12-01

    Geometrical optics analysis of the structural imperfection of retroreflection corner cubes is described. In the analysis, a geometrical optics model of six-beam reflection patterns generated by an imperfect retroreflection corner cube is developed, and its structural error extraction is formulated as a nonlinear optimization problem. The nonlinear conjugate gradient method is employed for solving the nonlinear optimization problem, and its detailed implementation is described. The proposed method of analysis is a mathematical basis for the nondestructive optical inspection of imperfectly fabricated retroreflection corner cubes.

  17. 50 years of nonlinear optics

    International Nuclear Information System (INIS)

    Shen Yuanrang

    2011-01-01

    This article presents a brief introduction to the birth and early investigations of nonlinear optics, such as second harmonic generation,sum and difference frequency generation, stimulated Raman scattering,and self-action of light etc. Several important research achievements and applications of nonlinear optics are presented as well, including nonlinear optical spectroscopy, phase conjugation and adaptive optics, coherent nonlinear optics, and high-order harmonic generation. In the end, current and future research topics in nonlinear optics are summarized. (authors)

  18. Fundamentals of nonlinear optical materials

    Indian Academy of Sciences (India)

    Nonlinear optics; nonlinear polarization; optical fiber communication; optical switch- ing. PACS Nos 42.65Tg; ... The importance of nonlinear optics is to understand the nonlinear behavior in the induced polarization and to ..... but much work in material development and characterization remains to be done. 16. Conclusion.

  19. Nonlinear optics at interfaces

    International Nuclear Information System (INIS)

    Chen, C.K.

    1980-12-01

    Two aspects of surface nonlinear optics are explored in this thesis. The first part is a theoretical and experimental study of nonlinear intraction of surface plasmons and bulk photons at metal-dielectric interfaces. The second part is a demonstration and study of surface enhanced second harmonic generation at rough metal surfaces. A general formulation for nonlinear interaction of surface plasmons at metal-dielectric interfaces is presented and applied to both second and third order nonlinear processes. Experimental results for coherent second and third harmonic generation by surface plasmons and surface coherent antiStokes Raman spectroscopy (CARS) are shown to be in good agreement with the theory

  20. Ultrafast nonlinear optics

    CERN Document Server

    Leburn, Christopher; Reid, Derryck

    2013-01-01

    The field of ultrafast nonlinear optics is broad and multidisciplinary, and encompasses areas concerned with both the generation and measurement of ultrashort pulses of light, as well as those concerned with the applications of such pulses. Ultrashort pulses are extreme events – both in terms of their durations, and also the high peak powers which their short durations can facilitate. These extreme properties make them powerful experiment tools. On one hand, their ultrashort durations facilitate the probing and manipulation of matter on incredibly short timescales. On the other, their ultrashort durations can facilitate high peak powers which can drive highly nonlinear light-matter interaction processes. Ultrafast Nonlinear Optics covers a complete range of topics, both applied and fundamental in nature, within the area of ultrafast nonlinear optics. Chapters 1 to 4 are concerned with the generation and measurement of ultrashort pulses. Chapters 5 to 7 are concerned with fundamental applications of ultrasho...

  1. Nonlinear optical interactions in silicon waveguides

    Directory of Open Access Journals (Sweden)

    Kuyken B.

    2017-03-01

    Full Text Available The strong nonlinear response of silicon photonic nanowire waveguides allows for the integration of nonlinear optical functions on a chip. However, the detrimental nonlinear optical absorption in silicon at telecom wavelengths limits the efficiency of many such experiments. In this review, several approaches are proposed and demonstrated to overcome this fundamental issue. By using the proposed methods, we demonstrate amongst others supercontinuum generation, frequency comb generation, a parametric optical amplifier, and a parametric optical oscillator.

  2. Terahertz semiconductor nonlinear optics

    DEFF Research Database (Denmark)

    Turchinovich, Dmitry; Hvam, Jørn Märcher; Hoffmann, Matthias

    2013-01-01

    In this proceedings we describe our recent results on semiconductor nonlinear optics, investigated using single-cycle THz pulses. We demonstrate the nonlinear absorption and self-phase modulation of strong-field THz pulses in doped semiconductors, using n-GaAs as a model system. The THz...... nonlinearity in doped semiconductors originates from the near-instantaneous heating of free electrons in the ponderomotive potential created by electric field of the THz pulse, leading to ultrafast increase of electron effective mass by intervalley scattering. Modification of effective mass in turn leads...... to a decrease of plasma frequency in semiconductor and produces a substantial modification of THz-range material dielectric function, described by the Drude model. As a result, the nonlinearity of both absorption coefficient and refractive index of the semiconductor is observed. In particular we demonstrate...

  3. Calculations on nonlinear optical properties for large systems the elongation method

    CERN Document Server

    Gu, Feng Long; Springborg, Michael; Kirtman, Bernard

    2014-01-01

    For design purposes one needs to relate the structure of proposed materials to their NLO (nonlinear optical) and other properties, which is a situation where theoretical approaches can be very helpful in providing suggestions for candidate systems that subsequently can be synthesized and studied experimentally. This brief describes the quantum-mechanical treatment of the response to one or more external oscillating electric fields for molecular and macroscopic, crystalline systems. To calculate NLO properties of large systems, a linear scaling generalized elongation method for the efficient and accurate calculation is introduced. The reader should be aware that this treatment is particularly feasible for complicated three-dimensional and/or delocalized systems that are intractable when applied to conventional or other linear scaling methods.

  4. Nonlinear fiber optics

    CERN Document Server

    Agrawal, Govind

    2012-01-01

    Since the 4e appeared, a fast evolution of the field has occurred. The 5e of this classic work provides an up-to-date account of the nonlinear phenomena occurring inside optical fibers, the basis of all our telecommunications infastructure as well as being used in the medical field. Reflecting the big developments in research, this new edition includes major new content: slow light effects, which offers a reduction in noise and power consumption and more ordered network traffic-stimulated Brillouin scattering; vectorial treatment of highly nonlinear fibers; and a brand new chapter o

  5. Essentials of nonlinear optics

    CERN Document Server

    Murti, Y V G S

    2014-01-01

    Current literature on Nonlinear Optics varies widely in terms of content, style, and coverage of specific topics, relative emphasis of areas and the depth of treatment. While most of these books are excellent resources for the researchers, there is a strong need for books appropriate for presenting the subject at the undergraduate or postgraduate levels in Universities. The need for such a book to serve as a textbook at the level of the bachelors and masters courses was felt by the authors while teaching courses on nonlinear optics to students of both science and engineering during the past two decades. This book has emerged from an attempt to address the requirement of presenting the subject at college level. A one-semester course covering the essentials can effectively be designed based on this.

  6. Terahertz Nonlinear Optics in Semiconductors

    DEFF Research Database (Denmark)

    Turchinovich, Dmitry; Hvam, Jørn Märcher; Hoffmann, Matthias C.

    2013-01-01

    We demonstrate the nonlinear optical effects – selfphase modulation and saturable absorption of a single-cycle THz pulse in a semiconductor. Resulting from THz-induced modulation of Drude plasma, these nonlinear optical effects, in particular, lead to self-shortening and nonlinear spectral...... breathing of a single-cycle THz pulse in a semiconductor....

  7. A novel method to produce nonlinear empirical physical formulas for experimental nonlinear electro-optical responses of doped nematic liquid crystals: Feedforward neural network approach

    Energy Technology Data Exchange (ETDEWEB)

    Yildiz, Nihat, E-mail: nyildiz@cumhuriyet.edu.t [Cumhuriyet University, Faculty of Science and Literature, Department of Physics, 58140 Sivas (Turkey); San, Sait Eren; Okutan, Mustafa [Department of Physics, Gebze Institute of Technology, P.O. Box 141, Gebze 41400, Kocaeli (Turkey); Kaya, Hueseyin [Cumhuriyet University, Faculty of Science and Literature, Department of Physics, 58140 Sivas (Turkey)

    2010-04-15

    Among other significant obstacles, inherent nonlinearity in experimental physical response data poses severe difficulty in empirical physical formula (EPF) construction. In this paper, we applied a novel method (namely layered feedforward neural network (LFNN) approach) to produce explicit nonlinear EPFs for experimental nonlinear electro-optical responses of doped nematic liquid crystals (NLCs). Our motivation was that, as we showed in a previous theoretical work, an appropriate LFNN, due to its exceptional nonlinear function approximation capabilities, is highly relevant to EPF construction. Therefore, in this paper, we obtained excellently produced LFNN approximation functions as our desired EPFs for above-mentioned highly nonlinear response data of NLCs. In other words, by using suitable LFNNs, we successfully fitted the experimentally measured response and predicted the new (yet-to-be measured) response data. The experimental data (response versus input) were diffraction and dielectric properties versus bias voltage; and they were all taken from our previous experimental work. We conclude that in general, LFNN can be applied to construct various types of EPFs for the corresponding various nonlinear physical perturbation (thermal, electronic, molecular, electric, optical, etc.) data of doped NLCs.

  8. A novel method to produce nonlinear empirical physical formulas for experimental nonlinear electro-optical responses of doped nematic liquid crystals: Feedforward neural network approach

    International Nuclear Information System (INIS)

    Yildiz, Nihat; San, Sait Eren; Okutan, Mustafa; Kaya, Hueseyin

    2010-01-01

    Among other significant obstacles, inherent nonlinearity in experimental physical response data poses severe difficulty in empirical physical formula (EPF) construction. In this paper, we applied a novel method (namely layered feedforward neural network (LFNN) approach) to produce explicit nonlinear EPFs for experimental nonlinear electro-optical responses of doped nematic liquid crystals (NLCs). Our motivation was that, as we showed in a previous theoretical work, an appropriate LFNN, due to its exceptional nonlinear function approximation capabilities, is highly relevant to EPF construction. Therefore, in this paper, we obtained excellently produced LFNN approximation functions as our desired EPFs for above-mentioned highly nonlinear response data of NLCs. In other words, by using suitable LFNNs, we successfully fitted the experimentally measured response and predicted the new (yet-to-be measured) response data. The experimental data (response versus input) were diffraction and dielectric properties versus bias voltage; and they were all taken from our previous experimental work. We conclude that in general, LFNN can be applied to construct various types of EPFs for the corresponding various nonlinear physical perturbation (thermal, electronic, molecular, electric, optical, etc.) data of doped NLCs.

  9. Nonlinear optical methods for the analysis of protein nanocrystals and biological tissues

    Science.gov (United States)

    Dow, Ximeng You

    Structural biology underpins rational drug design and fundamental understanding of protein function. X-ray diffraction (XRD) has been the golden standard for solving for high-resolution protein structure. Second harmonic generation (SHG) microscopy has been developed by the Simpson lab as a sensitive, crystal-specific detection method for the identification of protein crystal and help optimize the crystallization condition. Protein nanocrystals has been widely used for structure determination of membrane proteins in serial femtosecond nanocrystallography. In this thesis work, novel nonlinear optical methods were developed to address the challenges associated with the detection and characterization of protein nanocrystals. SHG-correlation spectroscopy (SHG-CS) was developed to take advantage of the diffusing motion and retrieve the size distribution and crystal quality of the nanocrystals. Polarization-dependent SHG imaging technique was developed to measure the relative orientation as well as the internal structure of the sample. Two photon- excited fluorescence has been used in the Simpson lab as a complementary measurement besides the inherent SHG signal from the crystals. A novel instrumentation development was also introduced in this thesis work to greatly improve the speed of fluorescence lifetime imaging (FLIM).

  10. Nonlinear compression of optical solitons

    Indian Academy of Sciences (India)

    linear pulse propagation is the nonlinear Schrödinger (NLS) equation [1]. There are ... Optical pulse compression finds important applications in optical fibres. The pulse com ..... to thank CSIR, New Delhi for financial support in the form of SRF.

  11. Chirality in nonlinear optics and optical switching

    NARCIS (Netherlands)

    Meijer, E.W.; Feringa, B.L.

    1993-01-01

    Chirality in molecular opto-electronics is limited sofar to the use of optically active liquid crystals and a number of optical phenomena are related to the helical macroscopic structure obtained by using one enantiomer, only. In this paper, the use of chirality in nonlinear optics and optical

  12. Investigation of the dynamics of a nonlinear optical response in glassy chalcogenide semiconductors by the pump–probe method

    Science.gov (United States)

    Romanova, E. A.; Kuzyutkina, Yu S.; Shiryaev, V. S.; Guizard, S.

    2018-03-01

    An analysis of the results of measurements by using the pump–probe method with a femtosecond resolution in time and computer simulation of the charge carrier kinetics have revealed two types of a nonlinear optical response in samples of chalcogenide glasses belonging to the As – S – Se system, irradiated by 50-fs laser pulses with a wavelength of 0.79 μm. The difference in the nonlinear dynamics is due to the difference in the photoexcitation character, because laser radiation can be absorbed either through bound states in the band gap or without their participation, depending on the ratio of the pump photon energy to the bandgap energy.

  13. Applications of nonlinear fiber optics

    CERN Document Server

    Agrawal, Govind

    2008-01-01

    * The only book describing applications of nonlinear fiber optics * Two new chapters on the latest developments: highly nonlinear fibers and quantum applications* Coverage of biomedical applications* Problems provided at the end of each chapterThe development of new highly nonlinear fibers - referred to as microstructured fibers, holey fibers and photonic crystal fibers - is the next generation technology for all-optical signal processing and biomedical applications. This new edition has been thoroughly updated to incorporate these key technology developments.The bo

  14. Field guide to nonlinear optics

    CERN Document Server

    Powers, Peter E

    2013-01-01

    Optomechanics is a field of mechanics that addresses the specific design challenges associated with optical systems. This [i]Field Guide [/i]describes how to mount optical components, as well as how to analyze a given design. It is intended for practicing optical and mechanical engineers whose work requires knowledge in both optics and mechanics. This Field Guide is designed for those looking for a condensed and concise source of key concepts, equations, and techniques for nonlinear optics. Topics covered include technologically important effects, recent developments in nonlinear optics

  15. Non-linear optical materials

    CERN Document Server

    Saravanan, R

    2018-01-01

    Non-linear optical materials have widespread and promising applications, but the efforts to understand the local structure, electron density distribution and bonding is still lacking. The present work explores the structural details, the electron density distribution and the local bond length distribution of some non-linear optical materials. It also gives estimation of the optical band gap, the particle size, crystallite size, and the elemental composition from UV-Visible analysis, SEM, XRD and EDS of some non-linear optical materials respectively.

  16. New organic materials for optics: optical storage and nonlinear optics

    International Nuclear Information System (INIS)

    Gan, F.

    1996-01-01

    New organic materials have received considerable attention recently, due to their easy preparation and different variety. The most application fields in optics are optical storage and nonlinear optics. In optical storage the organic dyes have been used for example, in record able and erasable compact disks (CD-R, CD-E) nonlinear optical effects, such as nonlinear optical absorption, second and third order optical absorption, second and third order optical nonlinearities, can be applied for making optical limiters, optical modulators, as well as laser second and third harmonic generations. Due to high value of optical absorption and optical nonlinearity organic materials are always used as thin films in optical integration. In this paper the new experimental results have been presented, and future development has been also discussed. (author)

  17. Nonlinear Optics: Principles and Applications

    DEFF Research Database (Denmark)

    Rottwitt, Karsten; Tidemand-Lichtenberg, Peter

    of applications, Nonlinear Optics: Principles and Applications effectively bridges physics and mathematics with relevant applied material for real-world use. The book progresses naturally from fundamental aspects to illustrative examples, and presents a strong theoretical foundation that equips the reader...... and matter, this text focuses on the physical understanding of nonlinear optics, and explores optical material response functions in the time and frequency domain....

  18. Projection-reduction method applied to deriving non-linear optical conductivity for an electron-impurity system

    Directory of Open Access Journals (Sweden)

    Nam Lyong Kang

    2013-07-01

    Full Text Available The projection-reduction method introduced by the present authors is known to give a validated theory for optical transitions in the systems of electrons interacting with phonons. In this work, using this method, we derive the linear and first order nonlinear optical conductivites for an electron-impurity system and examine whether the expressions faithfully satisfy the quantum mechanical philosophy, in the same way as for the electron-phonon systems. The result shows that the Fermi distribution function for electrons, energy denominators, and electron-impurity coupling factors are contained properly in organized manners along with absorption of photons for each electron transition process in the final expressions. Furthermore, the result is shown to be represented properly by schematic diagrams, as in the formulation of electron-phonon interaction. Therefore, in conclusion, we claim that this method can be applied in modeling optical transitions of electrons interacting with both impurities and phonons.

  19. Nonlinear optics principles and applications

    CERN Document Server

    Li, Chunfei

    2017-01-01

    This book reflects the latest advances in nonlinear optics. Besides the simple, strict mathematical deduction, it also discusses the experimental verification and possible future applications, such as the all-optical switches. It consistently uses the practical unit system throughout. It employs simple physical images, such as "light waves" and "photons" to systematically explain the main principles of nonlinear optical effects. It uses the first-order nonlinear wave equation in frequency domain under the condition of “slowly varying amplitude approximation" and the classical model of the interaction between the light and electric dipole. At the same time, it also uses the rate equations based on the energy-level transition of particle systems excited by photons and the energy and momentum conservation principles to explain the nonlinear optical phenomenon. The book is intended for researchers, engineers and graduate students in the field of the optics, optoelectronics, fiber communication, information tech...

  20. Distributed nonlinear optical response

    DEFF Research Database (Denmark)

    Nikolov, Nikola Ivanov

    2005-01-01

    of bound states of out of phase bright solitons and dark solitons. Also, the newly introduced analogy between the nonlocal cubic nonlinear and the quadratic nonlinear media, presented in paper B and Chapter 3 is discussed. In particular it supplies intuitive physical meaning of the formation of solitons...... in quadratic nonlinear media. In the second part of the report (Chapter 4), the possibility to obtain light with ultrabroad spectrum due to the interplay of many nonlinear effects based on cubic nonlinearity is investigated thoroughly. The contribution of stimulated Raman scattering, a delayed nonlinear...... a modified nonlinear Schroedinger model equation. Chapter 4 and papers D and E are dedicated to this part of the research....

  1. Extreme Nonlinear Optics An Introduction

    CERN Document Server

    Wegener, Martin

    2005-01-01

    Following the birth of the laser in 1960, the field of "nonlinear optics" rapidly emerged. Today, laser intensities and pulse durations are readily available, for which the concepts and approximations of traditional nonlinear optics no longer apply. In this regime of "extreme nonlinear optics," a large variety of novel and unusual effects arise, for example frequency doubling in inversion symmetric materials or high-harmonic generation in gases, which can lead to attosecond electromagnetic pulses or pulse trains. Other examples of "extreme nonlinear optics" cover diverse areas such as solid-state physics, atomic physics, relativistic free electrons in a vacuum and even the vacuum itself. This book starts with an introduction to the field based primarily on extensions of two famous textbook examples, namely the Lorentz oscillator model and the Drude model. Here the level of sophistication should be accessible to any undergraduate physics student. Many graphical illustrations and examples are given. The followi...

  2. Nonlinear Optics of Hexaphenyl Nanofibers

    DEFF Research Database (Denmark)

    Balzer, Frank; Al-Shamery, Katharina; Neuendorf, Rolf

    2003-01-01

    The nonlinear optical response of films of needle-shaped para-hexaphenyl nanoaggregates on mica surfaces is investigated. Two-photon luminescence as well as optical second harmonic generation (SHG) are observed following excitation with femtosecond pulses at 770 nm. Polarization dependent...... measurements reveal that the nonlinear optical transition dipole moment is oriented with an angle of 75° with respect to the needles long axes. The absolute value of the macroscopic second-order susceptibility, averaged over a size distribution of p-6P nanoaggregates, is estimated to be of the order of 6...

  3. New exact solutions of the Tzitzéica-type equations in non-linear optics using the expa function method

    Science.gov (United States)

    Hosseini, K.; Ayati, Z.; Ansari, R.

    2018-04-01

    One specific class of non-linear evolution equations, known as the Tzitzéica-type equations, has received great attention from a group of researchers involved in non-linear science. In this article, new exact solutions of the Tzitzéica-type equations arising in non-linear optics, including the Tzitzéica, Dodd-Bullough-Mikhailov and Tzitzéica-Dodd-Bullough equations, are obtained using the expa function method. The integration technique actually suggests a useful and reliable method to extract new exact solutions of a wide range of non-linear evolution equations.

  4. Dispersive optical soliton solutions for the hyperbolic and cubic-quintic nonlinear Schrödinger equations via the extended sinh-Gordon equation expansion method

    Science.gov (United States)

    Seadawy, Aly R.; Kumar, Dipankar; Chakrabarty, Anuz Kumar

    2018-05-01

    The (2+1)-dimensional hyperbolic and cubic-quintic nonlinear Schrödinger equations describe the propagation of ultra-short pulses in optical fibers of nonlinear media. By using an extended sinh-Gordon equation expansion method, some new complex hyperbolic and trigonometric functions prototype solutions for two nonlinear Schrödinger equations were derived. The acquired new complex hyperbolic and trigonometric solutions are expressed by dark, bright, combined dark-bright, singular and combined singular solitons. The obtained results are more compatible than those of other applied methods. The extended sinh-Gordon equation expansion method is a more powerful and robust mathematical tool for generating new optical solitary wave solutions for many other nonlinear evolution equations arising in the propagation of optical pulses.

  5. Nonlinear optics an analytical approach

    CERN Document Server

    Mandel, Paul

    2010-01-01

    Based on the author's extensive teaching experience and lecture notes, this textbook provides a substantially analytical rather than descriptive presentation of nonlinear optics. Divided into five parts, with most chapters corresponding to a two-hour lecture, the book begins with a unique account of the historical development from Kirchhoff's law for the black-body radiation to Planck's quantum hypothesis and Einstein's discovery of spontaneous emission - providing all the explicit proofs. The subsequent sections deal with matter quantization, ultrashort pulse propagation in 2-level media, cavity nonlinear optics, chi(2) and chi(3) media. For graduate and PhD students in nonlinear optics or photonics, while also representing a valuable reference for researchers in these fields.

  6. Nonlinear optics principles and applications

    CERN Document Server

    Rottwitt, Karsten

    2014-01-01

    IntroductionReview of linear opticsInduced polarizationHarmonic oscillator modelLocal field correctionsEstimated nonlinear responseSummaryTime-domain material responseThe polarization time-response functionThe Born-Oppenheimer approximationRaman scattering response function of silicaSummaryMaterial response in the frequency domain, susceptibility tensorsThe susceptibility tensorThe induced polarization in the frequency domainSum of monochromatic fieldsThe prefactor to the induced polarizationThird-order polarization in the Born-Oppenheimer approximation in the frequency domainKramers-Kronig relationsSummarySymmetries in nonlinear opticsSpatial symmetriesSecond-order materialsThird-order nonlinear materialsCyclic coordinate-systemContracted notation for second-order susceptibility tensorsSummaryThe nonlinear wave equationMono and quasi-monochromatic beamsPlane waves - the transverse problemWaveguidesVectorial approachNonlinear birefringenceSummarySecond-order nonlinear effectsGeneral theoryCoupled wave theoryP...

  7. Oscillating solitons in nonlinear optics

    Indian Academy of Sciences (India)

    ... are derived, and the relevant properties and features of oscillating solitons are illustrated. Oscillating solitons are controlled by the reciprocal of the group velocity and Kerr nonlinearity. Results of this paper will be valuable to the study of dispersion-managed optical communication system and mode-locked fibre lasers.

  8. Exact solutions for the higher-order nonlinear Schoerdinger equation in nonlinear optical fibres

    International Nuclear Information System (INIS)

    Liu Chunping

    2005-01-01

    First, by using the generally projective Riccati equation method, many kinds of exact solutions for the higher-order nonlinear Schoerdinger equation in nonlinear optical fibres are obtained in a unified way. Then, some relations among these solutions are revealed

  9. Nonlinear optical properties of silicon waveguides

    International Nuclear Information System (INIS)

    Tsang, H K; Liu, Y

    2008-01-01

    Recent work on two-photon absorption (TPA), stimulated Raman scattering (SRS) and optical Kerr effect in silicon-on-insulator (SOI) waveguides is reviewed and some potential applications of these optical nonlinearities, including silicon-based autocorrelation detectors, optical amplifiers, high speed optical switches, optical wavelength converters and self-phase modulation (SPM), are highlighted. The importance of free carriers generated by TPA in nonlinear devices is discussed, and a generalized definition of the nonlinear effective length to cater for nonlinear losses is proposed. How carrier lifetime engineering, and in particular the use of helium ion implantation, can enhance the nonlinear effective length for nonlinear devices is also discussed

  10. Nonlinear fiber optics formerly quantum electronics

    CERN Document Server

    Agrawal, Govind

    1995-01-01

    The field of nonlinear fiber optics has grown substantially since the First Edition of Nonlinear Fiber Optics, published in 1989. Like the First Edition, this Second Edition is a comprehensive, tutorial, and up-to-date account of nonlinear optical phenomena in fiber optics. It synthesizes widely scattered research material and presents it in an accessible manner for students and researchers already engaged in or wishing to enter the field of nonlinear fiber optics. Particular attention is paid to the importance of nonlinear effects in the design of optical fiber communication systems. This is

  11. Investigation of inorganic nonlinear optical potassium penta borate tetra hydrate (PPBTH) single crystals grown by slow evaporation method

    Science.gov (United States)

    Arivuselvi, R.; Babu, P. Ramesh

    2018-03-01

    Borates family crystals were plays vital role in the field of non linear optics (NLO) due to needs of wide range of applications. In this report, NLO crystals (potassium penta borate tetra hydrate (KB5H8O12) are grown by slow evaporation method at room temperature (28° C) and studied their physical properties. The harvested single crystals are transparent with the dimension of 12 × 10 × 6 mm3 and colourless. X-ray diffraction of single crystals reveals that the grown crystal belongs to orthorhombic system with non-centrosymmetric space group Pba2. All the absorbed functional groups are present in the order of inorganic compounds expect 1688 cm-1 because of water (Osbnd H sbnd O blending) molecule present in the pristine. Crystals show transparent in the entire visible region with 5.9 eV optical band gap and also it shows excellence in both second and third order nonlinear optical properties. Crystals can withstand upto 154 °C without any phase changes which is observed using thermal (TGA/DTA) analysis.

  12. Infrared reduction, an efficient method to control the non-linear optical property of graphene oxide in femtosecond regime

    Science.gov (United States)

    Bhattacharya, S.; Maiti, R.; Saha, S.; Das, A. C.; Mondal, S.; Ray, S. K.; Bhaktha, S. B. N.; Datta, P. K.

    2016-04-01

    Graphene Oxide (GO) has been prepared by modified Hummers method and it has been reduced using an IR bulb (800-2000 nm). Both as grown GO and reduced graphene oxide (RGO) have been characterized using Raman spectroscopy and X-ray photoelectron spectroscopy (XPS). Raman spectra shows well documented Dband and G-band for both the samples while blue shift of G-band confirms chemical functionalization of graphene with different oxygen functional group. The XPS result shows that the as-prepared GO contains 52% of sp2 hybridized carbon due to the C=C bonds and 33% of carbon atoms due to the C-O bonds. As for RGO, increment of the atomic % of the sp2 hybridized carbon atom to 83% and rapid decrease in atomic % of C=O bonds confirm an efficient reduction with infrared radiation. UV-Visible absorption spectrum also confirms increment of conjugation with increased reduction. Non-linear optical properties of both GO and RGO are measured using single beam open aperture Z-Scan technique in femtosecond regime. Intensity dependent nonlinear phenomena are observed. Depending upon the intensity, both saturable absorption and two photon absorption contribute to the non-linearity of both the samples. Saturation dominates at low intensity (~ 127 GW/cm2) while two photon absorption become prominent at higher intensities (from 217 GW/cm2 to 302 GW/cm2). We have calculated the two-photon absorption co-efficient and saturation intensity for both the samples. The value of two photon absorption co-efficient (for GO~ 0.0022-0.0037 cm/GW and for RGO~ 0.0128-0.0143 cm/GW) and the saturation intensity (for GO~57 GW/cm2 and for RGO~ 194GW/cm2) is increased with reduction. Increase in two photon absorption coefficient with increasing intensity can also suggest that there may be multi-photon absorption is taking place.

  13. Synthesis of highly stable silver nanoparticles through a novel green method using Mirabillis jalapa for antibacterial, nonlinear optical applications

    Science.gov (United States)

    Pugazhendhi, S.; Palanisamy, P. K.; Jayavel, R.

    2018-05-01

    Green synthesis techniques are developing as more simplistic and eco-friendly approach for the synthesis of metal nanoparticles compared to chemical reduction methods. Herein we report Synthesis of highly stable silver nanoparticles using Mirabillis jalapa seed extract as a reducing and capping agent. The as-prepared silver nanoparticles were characterized by UV-vis spectroscopy (UV-vis) to confirm the formation of silver nanoparticles by its characteristic surface plasmon resonance peak observed at 420 nm. The Powder X-ray diffraction (P-XRD) revealed the structure and crystalline nature of synthesized silver nanoparticles, The Fourier transform infra-red spectroscopic (FT-IR) revealed the presence of the biomolecules in the extract that acted as reducing as well stabilizing agent. The high resolution transmission electron microscopic (HRTEM) images divulged that the synthesized silver nanoparticles were spherical in shape and poly dispersed. The energy dispersive X-ray diffraction (EDX) profile revealed the elements present in the as-synthesized colloidal silver nanoparticles and its percentages. The Zeta potential measured for silver nanoparticles evidenced that the prepared silver nanoparticles owned high stability in room temperature itself. The as-synthesized silver nanoparticles (AgNPs) in colloidal form were showed good antimicrobial effects and it's were found to exhibit third order optical nonlinearity as studied by Z-scan technique using 532 nm Nd:YAG (SHG) CW laser beam (COHERENT-Compass 215 M-50 diode pumped) output as source. The negative nonlinearity observed was well utilized for the study of optical limiting behavior of the silver nanoparticles.

  14. Nonlinear optical crystals a complete survey

    CERN Document Server

    Nikogosyan, David N

    2005-01-01

    Nonlinear optical crystals are widely used in modern optical science and technology for frequency conversion of laser light, i.e. to generate laser radiation at any specific wavelength in visible, UV or IR spectral regions. This unrivalled reference book contains the most complete and up-to-date information on properties of nonlinear optical crystals. It includes: * Database of 63 common and novel nonlinear optical crystals * Periodically-poled and self-frequency-doubling materials * Full description of linear and nonlinear optical properties * Significant amount of crystallophysical, thermophysical, spectroscopic, electro-optic and magneto-optic information * 7 mini-reviews on novel applications, such as deep-UV light generation, terahertz-wave generation, ultrashort laser pulse compression, photonic band-gap crystals, x3 nonlinearity, etc. * More than 1500 different references with full titles It is a vital source of information for scientists and engineers dealing with modern applications of nonlinear opti...

  15. Laser beam propagation in nonlinear optical media

    CERN Document Server

    Guha, Shekhar

    2013-01-01

    ""This is very unique and promises to be an extremely useful guide to a host of workers in the field. They have given a generalized presentation likely to cover most if not all situations to be encountered in the laboratory, yet also highlight several specific examples that clearly illustrate the methods. They have provided an admirable contribution to the community. If someone makes their living by designing lasers, optical parametric oscillators or other devices employing nonlinear crystals, or designing experiments incorporating laser beam propagation through linear or nonlinear media, then

  16. Nonlinear optical studies of surfaces

    International Nuclear Information System (INIS)

    Shen, Y.R.

    1994-07-01

    The possibly of using nonlinear optical processes for surface studies has attracted increasing attention in recent years. Optical second harmonic generation (SHG) and sum frequency generation (SFG), in particular, have been well accepted as viable surface probes. They have many advantages over the conventional techniques. By nature, they are highly surface-specific and has a submonolayer sensitivity. As coherent optical processes, they are capable of in-situ probing of surfaces in hostile environment as well as applicable to all interfaces accessible by light. With ultrafast pump laser pulses, they can be employed to study surface dynamic processes with a subpicosecond time resolution. These advantages have opened the door to many exciting research opportunities in surface science and technology. This paper gives a brief overview of this fast-growing new area of research. Optical SHG from a surface was first studied theoretically and experimentally in the sixties. Even the submonolayer surface sensitivity of the process was noticed fairly early. The success was, however, limited because of difficulties in controlling the experimental conditions. It was not until the early 1980's that the potential of the process for surface analysis was duly recognized. The first surface study by SHG was actually motivated by the then active search for an understanding of the intriguing surface enhanced Raman scattering (SERS). It had been suspected that the enhancement in SERS mainly came from the local-field enhancement due to local plasmon resonances and pointing rod effect on rough metal surfaces. In our view, Raman scattering is a two-photon process and is therefore a nonlinear optical effect

  17. Methods of nonlinear analysis

    CERN Document Server

    Bellman, Richard Ernest

    1970-01-01

    In this book, we study theoretical and practical aspects of computing methods for mathematical modelling of nonlinear systems. A number of computing techniques are considered, such as methods of operator approximation with any given accuracy; operator interpolation techniques including a non-Lagrange interpolation; methods of system representation subject to constraints associated with concepts of causality, memory and stationarity; methods of system representation with an accuracy that is the best within a given class of models; methods of covariance matrix estimation;methods for low-rank mat

  18. Nonlinear Optical Fiber Arrays for Limiting Application

    National Research Council Canada - National Science Library

    Khoo, Iam-Choon

    2006-01-01

    .... Measurements show that they possess desirable nonlinear optical such as low-freezing pint, non-volatile, transparent for low light level and possess large effective nonlinear absorption coefficients...

  19. Order and chaos in polarized nonlinear optics

    International Nuclear Information System (INIS)

    Holm, D.D.

    1990-01-01

    Methods for investigating temporal complexity in Hamiltonian systems are applied to the dynamics of a polarized optical laser beam propagating as a travelling wave in a medium with cubically nonlinear polarizability (i.e., a Kerr medium). The theory of Hamiltonian systems with symmetry is used to study the geometry of phase space for the optical problem, transforming from C 2 to S 2 x (J,θ), where (J,θ) is a symplectic action-angle pair. The bifurcations of the phase portraits of the Hamiltonian motion on S 2 are classified and shown graphically. These bifurcations create various saddle connections on S 2 as either J (the beam intensity), or the optical parameters of the medium are varied. After this bifurcation analysis, the Melnikov method is used to demonstrate analytically that the saddle connections break and intersect transversely in a Poincare map under spatially periodic perturbations of the optical parameters of the medium. These transverse intersections in the Poincare map imply intermittent polarization switching with extreme sensitivity to initial conditions characterized by a Smale horseshoe construction for the travelling waves of a polarized optical laser pulse. The resulting chaotic behavior in the form of sensitive dependence on initial conditions may have implications for the control and predictability of nonlinear optical polarization switching in birefringent media. 19 refs., 2 figs., 1 tab

  20. Nanoplasmonic solution for nonlinear optics

    DEFF Research Database (Denmark)

    Bache, Morten; Lavrinenko, Andrei; Lysenko, Oleg

    2014-01-01

    for the silicon dioxide cladding. The blue, cyan and magenta curves correspond to the transmission spectra for the gold waveguides with the width of 10 μm and length of 2, 3, and 4 mm.The polarization of laser beam was tuned to match the transverse magnetic mode of surface plasmonpolaritons in the gold waveguides...... and is being under investigation in recent years [3].The purpose of our research is to study nonlinear optical properties of gold waveguides embedded intodielectric medium (silicon dioxide) using picosecond laser spectroscopy. The work includes modeling ofoptical properties of gold waveguides, fabrication...... of prototype samples, and optical characterization ofsamples using a picosecond laser source.The prototype samples of gold waveguides embedded into silicon dioxide were fabricated at DTUDanchip. A silicon wafer with pre-made 6.5 μm layer of silicon dioxide was used as a substrate and goldwaveguides (films...

  1. Nonlinear Photonics and Novel Optical Phenomena

    CERN Document Server

    Morandotti, Roberto

    2012-01-01

    Nonlinear Photonics and Novel Optical Phenomena contains contributed chapters from leading experts in nonlinear optics and photonics, and provides a comprehensive survey of fundamental concepts as well as hot topics in current research on nonlinear optical waves and related novel phenomena. The book covers self-accelerating airy beams, integrated photonics based on high index doped-silica glass, linear and nonlinear spatial beam dynamics in photonic lattices and waveguide arrays, polariton solitons and localized structures in semiconductor microcavities, terahertz waves, and other novel phenomena in different nanophotonic and optical systems.

  2. Biological applications of novel nonlinear optical microscopy

    International Nuclear Information System (INIS)

    Kajiyama, Shin'ichiro; Ozeki, Yasuyuki; Itoh, Kazuyoshi; Fukui, Kiichi

    2010-01-01

    Two types of newly developed nonlinear optical microscopes namely stimulated parametric emission (SPE) microscope and stimulated Raman scattering (SRS) microscope were presented together with their biological applications.

  3. Cavity nonlinear optics with layered materials

    Directory of Open Access Journals (Sweden)

    Fryett Taylor

    2017-12-01

    Full Text Available Unprecedented material compatibility and ease of integration, in addition to the unique and diverse optoelectronic properties of layered materials, have generated significant interest in their utilization in nanophotonic devices. While initial nanophotonic experiments with layered materials primarily focused on light sources, modulators, and detectors, recent efforts have included nonlinear optical devices. In this paper, we review the current state of cavity-enhanced nonlinear optics with layered materials. Along with conventional nonlinear optics related to harmonic generation, we report on emerging directions of nonlinear optics, where layered materials can potentially play a significant role.

  4. Nonlinear optics quantum computing with circuit QED.

    Science.gov (United States)

    Adhikari, Prabin; Hafezi, Mohammad; Taylor, J M

    2013-02-08

    One approach to quantum information processing is to use photons as quantum bits and rely on linear optical elements for most operations. However, some optical nonlinearity is necessary to enable universal quantum computing. Here, we suggest a circuit-QED approach to nonlinear optics quantum computing in the microwave regime, including a deterministic two-photon phase gate. Our specific example uses a hybrid quantum system comprising a LC resonator coupled to a superconducting flux qubit to implement a nonlinear coupling. Compared to the self-Kerr nonlinearity, we find that our approach has improved tolerance to noise in the qubit while maintaining fast operation.

  5. Nonlinear super-resolution nano-optics and applications

    CERN Document Server

    Wei, Jingsong

    2015-01-01

    This book covers many advances in the subjects of nano-optics and nano photonics. The author describes the principle and technical schematics of common methods for breaking through the optical diffraction limit and focuses on realizing optical super-resolution with nonlinear effects of thin film materials. The applications of nonlinear optical super-resolution effects in nano-data storage, nanolithography, and nano-imaging are also presented. This book is useful to graduate students majoring in optics and nano science and also serves as a reference book for academic researchers, engineers, technical professionals in the fields of super-resolution optics and laser techniques, nano-optics and nano photonics, nano-data storage, nano imaging, micro/nanofabrication and nanolithography and nonlinear optics.

  6. Enhancement of nonlinear optical properties of compounds of silica

    Indian Academy of Sciences (India)

    The aim of this paper is to introduce a method for enhancing the nonlinear optical properties in silica glass by using metallic nanoparticles. First, the T-matrix method is developed to calculate the effective dielectric constant for the compound of silica glass and metallic nanoparticles, both of which possess nonlinear dielectric ...

  7. Nonlinear optics of liquid crystalline materials

    International Nuclear Information System (INIS)

    Khoo, Iam Choon

    2009-01-01

    Liquid crystals occupy an important niche in nonlinear optics as a result of their unique physical and optical properties. Besides their broadband birefringence and transparency, abilities to self-assemble into various crystalline phases and to conform to various flexible forms and shapes, liquid crystals are compatible with almost all other optoelectronic materials and technology platforms. In both isotropic and ordered phases, liquid crystals possess extraordinarily large optical nonlinearities that stretch over multiple time scales. To date, almost all conceivable nonlinear optical phenomena have been observed in a very broad spectrum spanning the entire visible to infrared and beyond. In this review, we present a self-contained complete discussion of the optical nonlinearities of liquid crystals, and a thorough review of a wide range of nonlinear optical processes and phenomena enabled by these unique properties. Starting with a brief historical account of the development of nonlinear optical studies of the mesophases of liquid crystals, we then review various liquid crystalline materials and structures, and their nonlinear optical properties. Emphasis is placed on the nematic phase, which best exemplifies the dual nature of liquid crystals, although frequent references to other phases are also made. We also delve into recent work on novel structures such as photonic crystals, metamaterials and nanostructures and their special characteristics and emergent properties. The mechanisms and complex nonlocal dynamics of optical nonlinearities associated with laser induced director axis reorientation, thermal, density, and order parameter fluctuations, space charge field formation and photorefractivity are critically reviewed as a foundation for the discussions of various nonlinear optical processes detailed in this paper

  8. Cascaded nonlinearities for ultrafast nonlinear optical science and applications

    DEFF Research Database (Denmark)

    Bache, Morten

    the cascading nonlinearity is investigated in detail, especially with focus on femtosecond energetic laser pulses being subjected to this nonlinear response. Analytical, numerical and experimental results are used to understand the cascading interaction and applications are demonstrated. The defocusing soliton...... observations with analogies in fiber optics are observed numerically and experimentally, including soliton self-compression, soliton-induced resonant radiation, supercontinuum generation, optical wavebreaking and shock-front formation. All this happens despite no waveguide being present, thanks...... is of particular interest here, since it is quite unique and provides the solution to a number of standing challenges in the ultrafast nonlinear optics community. It solves the problem of catastrophic focusing and formation of a filaments in bulk glasses, which even under controlled circumstances is limited...

  9. Nonlinear soliton matching between optical fibers

    DEFF Research Database (Denmark)

    Agger, Christian; Sørensen, Simon Toft; Thomsen, Carsten L.

    2011-01-01

    In this Letter, we propose a generic nonlinear coupling coefficient, η2 NL ¼ ηjγ=β2jfiber2=jγ=β2jfiber1, which gives a quantitative measure for the efficiency of nonlinear matching of optical fibers by describing how a fundamental soliton couples from one fiber into another. Specifically, we use η...

  10. Nuclear matter as a nonlinear optical medium

    International Nuclear Information System (INIS)

    Hefter, E.F.; Papini, G.

    1986-01-01

    This paper is concerned with the question whether nuclear matter should be considered as a nonlinear optical medium. Taking, in a pragmatic way, quality and quantity of the results of well-established linear and nonlinear approaches as the main criterion, an affirmative answer is seen to be consistent with long-standing practices adhered to in nuclear physics

  11. Nonlinear Multiantenna Detection Methods

    Directory of Open Access Journals (Sweden)

    Chen Sheng

    2004-01-01

    Full Text Available A nonlinear detection technique designed for multiple-antenna assisted receivers employed in space-division multiple-access systems is investigated. We derive the optimal solution of the nonlinear spatial-processing assisted receiver for binary phase shift keying signalling, which we refer to as the Bayesian detector. It is shown that this optimal Bayesian receiver significantly outperforms the standard linear beamforming assisted receiver in terms of a reduced bit error rate, at the expense of an increased complexity, while the achievable system capacity is substantially enhanced with the advent of employing nonlinear detection. Specifically, when the spatial separation expressed in terms of the angle of arrival between the desired and interfering signals is below a certain threshold, a linear beamformer would fail to separate them, while a nonlinear detection assisted receiver is still capable of performing adequately. The adaptive implementation of the optimal Bayesian detector can be realized using a radial basis function network. Two techniques are presented for constructing block-data-based adaptive nonlinear multiple-antenna assisted receivers. One of them is based on the relevance vector machine invoked for classification, while the other on the orthogonal forward selection procedure combined with the Fisher ratio class-separability measure. A recursive sample-by-sample adaptation procedure is also proposed for training nonlinear detectors based on an amalgam of enhanced -means clustering techniques and the recursive least squares algorithm.

  12. Microresonators for Nonlinear Quantum Optics

    Science.gov (United States)

    Vernon, Zachary

    In this thesis I study in detail the quantum dynamics of several nonlinear optical processes in microresonator systems. A Heisenberg-picture input-output formalism is developed from first principles that includes the effects of scattering losses and independent quality factors and coupling ratios for different resonances. The task of calculating the device output is then reduced to solving a set of driven, damped, ordinary differential equations for the resonator mode operators alone. This theoretical framework is used to study photon pair generation via spontaneous four-wave mixing in the weakly pumped regime, on which the effects of scattering losses are appraised. A more strongly driven regime is studied for continuous wave pumps, demonstrating when self- and cross-phase modulation and multi-photon pair generation become important, and their effects on the spectral and power scaling properties of the system are examined; A detuning strategy is presented that compensates for some of these effects. The results of the weak-pump regime are applied to study microresonator-based heralded single photon sources. The impact of scattering losses is studied, revealing that typical systems suffer from low heralding efficiency due to these losses. A technique to improve heralding efficiency is presented through over-coupling the resonator-channel system, and a resultant trade-off between heralding rate and heralding efficiency is uncovered. Limitations to the spectral purity of the heralded single photon output for conventional microresonator systems are also analysed, and a more sophisticated coupling scheme presented to overcome the upper bound for spectral purity of 93% that exists in typical systems, permitting the generation of single photons with spectral purity arbitrarily close to 100% without spectral filtering or sophisticated phase-matching techniques. The theory of quantum frequency conversion in microresonators using four-wave mixing is then developed in detail

  13. Nonlinear optical model for strip plasmonic waveguides

    DEFF Research Database (Denmark)

    Lysenko, Oleg; Bache, Morten; Lavrinenko, Andrei

    2016-01-01

    This paper presents a theoretical model of nonlinear optical properties for strip plasmonic waveguides. The particular waveguides geometry that we investigate contains a gold core, adhesion layers, and silicon dioxide cladding. It is shown that the third-order susceptibility of the gold core...... significantly depends on the layer thickness and has the dominant contribution to the effective third-order susceptibility of the long-range plasmon polariton mode. This results in two nonlinear optical effects in plasmonic waveguides, which we experimentally observed and reported in [Opt. Lett. 41, 317 (2016...... approaches. (C) 2016 Optical Society of America...

  14. Optical rogue waves and soliton turbulence in nonlinear fibre optics

    DEFF Research Database (Denmark)

    Genty, G.; Dudley, J. M.; de Sterke, C. M.

    2009-01-01

    We examine optical rogue wave generation in nonlinear fibre propagation in terms of soliton turbulence. We show that higher-order dispersion is sufficient to generate localized rogue soliton structures, and Raman scattering effects are not required.......We examine optical rogue wave generation in nonlinear fibre propagation in terms of soliton turbulence. We show that higher-order dispersion is sufficient to generate localized rogue soliton structures, and Raman scattering effects are not required....

  15. Oscillating solitons in nonlinear optics

    Indian Academy of Sciences (India)

    The study of solitons in those physical systems reveals some exciting .... With the following power series expansions for g(z,t) and f(z,t): g(z,t) = εg1(z,t) + ... If nonlinearity γ (z) is also taken as a function in figure 1b, the periodic and oscillation.

  16. Nonlinear optical techniques for surface studies

    International Nuclear Information System (INIS)

    Shen, Y.R.

    1981-09-01

    Recent effort in developing nonlinear optical techniques for surface studies is reviewed. Emphasis is on monolayer detection of adsorbed molecules on surfaces. It is shown that surface coherent antiStokes Raman scattering (CARS) with picosecond pulses has the sensitivity of detecting submonolayer of molecules. On the other hand, second harmonic or sum-frequency generation is also sensitive enough to detect molecular monolayers. Surface-enhanced nonlinear optical effects on some rough metal surfaces have been observed. This facilitates the detection of molecular monolayers on such surfaces, and makes the study of molecular adsorption at a liquid-metal interface feasible. Advantages and disadvantages of the nonlinear optical techniques for surface studies are discussed

  17. Nonlinear Optics with 2D Layered Materials.

    Science.gov (United States)

    Autere, Anton; Jussila, Henri; Dai, Yunyun; Wang, Yadong; Lipsanen, Harri; Sun, Zhipei

    2018-03-25

    2D layered materials (2DLMs) are a subject of intense research for a wide variety of applications (e.g., electronics, photonics, and optoelectronics) due to their unique physical properties. Most recently, increasing research efforts on 2DLMs are projected toward the nonlinear optical properties of 2DLMs, which are not only fascinating from the fundamental science point of view but also intriguing for various potential applications. Here, the current state of the art in the field of nonlinear optics based on 2DLMs and their hybrid structures (e.g., mixed-dimensional heterostructures, plasmonic structures, and silicon/fiber integrated structures) is reviewed. Several potential perspectives and possible future research directions of these promising nanomaterials for nonlinear optics are also presented. © 2018 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  18. Nonlinear programming analysis and methods

    CERN Document Server

    Avriel, Mordecai

    2012-01-01

    This text provides an excellent bridge between principal theories and concepts and their practical implementation. Topics include convex programming, duality, generalized convexity, analysis of selected nonlinear programs, techniques for numerical solutions, and unconstrained optimization methods.

  19. Benchmarking Post-Hartree–Fock Methods To Describe the Nonlinear Optical Properties of Polymethines: An Investigation of the Accuracy of Algebraic Diagrammatic Construction (ADC) Approaches

    KAUST Repository

    Knippenberg, Stefan

    2016-10-07

    Third-order nonlinear optical (NLO) properties of polymethine dyes have been widely studied for applications such as all-optical switching. However, the limited accuracy of the current computational methodologies has prevented a comprehensive understanding of the nature of the lowest excited states and their influence on the molecular optical and NLO properties. Here, attention is paid to the lowest excited-state energies and their energetic ratio, as these characteristics impact the figure-of-merit for all-optical switching. For a series of model polymethines, we compare several algebraic diagrammatic construction (ADC) schemes for the polarization propagator with approximate second-order coupled cluster (CC2) theory, the widely used INDO/MRDCI approach and the symmetry-adapted cluster configuration interaction (SAC-CI) algorithm incorporating singles and doubles linked excitation operators (SAC-CI SD-R). We focus in particular on the ground-to-excited state transition dipole moments and the corresponding state dipole moments, since these quantities are found to be of utmost importance for an effective description of the third-order polarizability γ and two-photon absorption spectra. A sum-overstates expression has been used, which is found to quickly converge. While ADC(3/2) has been found to be the most appropriate method to calculate these properties, CC2 performs poorly.

  20. Measurement-induced nonlinearity in linear optics

    International Nuclear Information System (INIS)

    Scheel, Stefan; Knight, Peter L.; Nemoto, Kae; Munro, William J.

    2003-01-01

    We investigate the generation of nonlinear operators with single-photon sources, linear optical elements, and appropriate measurements of auxiliary modes. We provide a framework for the construction of useful single-mode and two-mode quantum gates necessary for all-optical quantum information processing. We focus our attention generally on using minimal physical resources while providing a transparent and algorithmic way of constructing these operators

  1. Nonlinear microstructured polymer optical fibres

    DEFF Research Database (Denmark)

    Frosz, Michael Henoch

    is potentially the case for microstructured polymer optical fibres (mPOFs). Another advantage is that polymer materials have a higher biocompatibility than silica, meaning that it is easier to bond certain types of biosensor materials to a polymer surface than to silica. As with silica PCFs, it is difficult...

  2. Anisotropic and nonlinear optical waveguides

    CERN Document Server

    Someda, CG

    1992-01-01

    Dielectric optical waveguides have been investigated for more than two decades. In the last ten years they have had the unique position of being simultaneously the backbone of a very practical and fully developed technology, as well as an extremely exciting area of basic, forefront research. Existing waveguides can be divided into two sets: one consisting of waveguides which are already in practical use, and the second of those which are still at the laboratory stage of their evolution. This book is divided into two separate parts: the first dealing with anisotropic waveguides, an

  3. Quantum Information Processing using Nonlinear Optical Effects

    DEFF Research Database (Denmark)

    Andersen, Lasse Mejling

    This PhD thesis treats applications of nonlinear optical effects for quantum information processing. The two main applications are four-wave mixing in the form of Bragg scattering (BS) for quantum-state-preserving frequency conversion, and sum-frequency generation (SFG) in second-order nonlinear......-chirping the pumps. In the high-conversion regime without the effects of NPM, exact Green functions for BS are derived. In this limit, separability is possible for conversion efficiencies up to 60 %. However, the system still allows for selective frequency conversion as well as re-shaping of the output. One way...

  4. Lossy effects in a nonlinear nematic optical fiber

    Science.gov (United States)

    Rodríguez, R. F.; Reyes, J. A.

    2001-09-01

    We use the multiple scales method to derive a generalized nonlinear Schrödinger equation that takes into account the dissipative effects in the reorientation of a nematic confined in a cylindrical waveguide. This equation has soliton-like solutions and predicts a decrease in the penetration length of the optical solitons for each propagating mode with respect to the dissipationless case.

  5. Rigorous theory of molecular orientational nonlinear optics

    International Nuclear Information System (INIS)

    Kwak, Chong Hoon; Kim, Gun Yeup

    2015-01-01

    Classical statistical mechanics of the molecular optics theory proposed by Buckingham [A. D. Buckingham and J. A. Pople, Proc. Phys. Soc. A 68, 905 (1955)] has been extended to describe the field induced molecular orientational polarization effects on nonlinear optics. In this paper, we present the generalized molecular orientational nonlinear optical processes (MONLO) through the calculation of the classical orientational averaging using the Boltzmann type time-averaged orientational interaction energy in the randomly oriented molecular system under the influence of applied electric fields. The focal points of the calculation are (1) the derivation of rigorous tensorial components of the effective molecular hyperpolarizabilities, (2) the molecular orientational polarizations and the electronic polarizations including the well-known third-order dc polarization, dc electric field induced Kerr effect (dc Kerr effect), optical Kerr effect (OKE), dc electric field induced second harmonic generation (EFISH), degenerate four wave mixing (DFWM) and third harmonic generation (THG). We also present some of the new predictive MONLO processes. For second-order MONLO, second-order optical rectification (SOR), Pockels effect and difference frequency generation (DFG) are described in terms of the anisotropic coefficients of first hyperpolarizability. And, for third-order MONLO, third-order optical rectification (TOR), dc electric field induced difference frequency generation (EFIDFG) and pump-probe transmission are presented

  6. Interactive Nonlinear Multiobjective Optimization Methods

    OpenAIRE

    Miettinen, Kaisa; Hakanen, Jussi; Podkopaev, Dmitry

    2016-01-01

    An overview of interactive methods for solving nonlinear multiobjective optimization problems is given. In interactive methods, the decision maker progressively provides preference information so that the most satisfactory Pareto optimal solution can be found for her or his. The basic features of several methods are introduced and some theoretical results are provided. In addition, references to modifications and applications as well as to other methods are indicated. As the...

  7. Nonlinear optical studies of organic monolayers

    International Nuclear Information System (INIS)

    Shen, Y.R.

    1988-02-01

    Second-order nonlinear optical effects are forbidden in a medium with inversion symmetry, but are necessarily allowed at a surface where the inversion summary is broken. They are often sufficiently strong so that a submonolayer perturbation of the surface can be readily detected. They can therefore be used as effective tools to study monolayers adsorbed at various interfaces. We discuss here a number of recent experiments in which optical second harmonic generation (SHG) and sum-frequency generation (SFG) are employed to probe and characterize organic monolayers. 15 refs., 5 figs

  8. Statistical methods in nonlinear dynamics

    Indian Academy of Sciences (India)

    Sensitivity to initial conditions in nonlinear dynamical systems leads to exponential divergence of trajectories that are initially arbitrarily close, and hence to unpredictability. Statistical methods have been found to be helpful in extracting useful information about such systems. In this paper, we review briefly some statistical ...

  9. Nonlinear and quantum optics near nanoparticles

    Science.gov (United States)

    Dhayal, Suman

    We study the behavior of electric fields in and around dielectric and metal nanoparticles, and prepare the ground for their applications to a variety of systems viz. photovoltaics, imaging and detection techniques, and molecular spectroscopy. We exploit the property of nanoparticles being able to focus the radiation field into small regions and study some of the interesting nonlinear, and quantum coherence and interference phenomena near them. The traditional approach to study the nonlinear light-matter interactions involves the use of the slowly varying amplitude approximation (SVAA) as it simplifies the theoretical analysis. However, SVVA cannot be used for systems which are of the order of the wavelength of the light. We use the exact solutions of the Maxwell's equations to obtain the fields created due to metal and dielectric nanoparticles, and study nonlinear and quantum optical phenomena near these nanoparticles. We begin with the theoretical description of the electromagnetic fields created due to the nonlinear wavemixing process, namely, second-order nonlinearity in an nonlinear sphere. The phase-matching condition has been revisited in such particles and we found that it is not satisfied in the sphere. We have suggested a way to obtain optimal conditions for any type and size of material medium. We have also studied the modifications of the electromagnetic fields in a collection of nanoparticles due to strong near field nonlinear interactions using the generalized Mie theory for the case of many particles applicable in photovoltaics (PV). We also consider quantum coherence phenomena such as modification of dark states, stimulated Raman adiabatic passage (STIRAP), optical pumping in 4-level atoms near nanoparticles by using rotating wave approximation to describe the Hamiltonian of the atomic system. We also considered the behavior of atomic and the averaged atomic polarization in 7-level atoms near nanoparticles. This could be used as a prototype to study

  10. Advanced in Nonlinear Optics and Laser Research and Development

    International Nuclear Information System (INIS)

    Jackel, S.; Kotler, Z; Lavi, R.; Sternklar, S.

    1996-01-01

    The Nonlinear Optics Group (NLOG) at Soreq NRC is engaged in the development of fundamental and applied technology in the related fields of nonlinear optics and laser development. Our work in nonlinear optics started with the goal of improving laser performance. These efforts were successful and opened the way for R and D in nonlinear optics for other applications. Today we use nonlinear optics to enable continuous tunability of lasers, control the path of light beams, modulate a light signal rapidly, provide optical data storage, and supply new means of microscopically probing biological and inorganic samples. Technology maturation and interaction with users will show which aspects of nonlinear optics will make the most impact

  11. Progress in nonlinear nano-optics

    CERN Document Server

    Lienau, Christoph; Grunwald, Rüdiger

    2015-01-01

    This book presents the state of the art in nonlinear nanostructures for ultrafast laser applications. Most recent results in two emerging fields are presented: (i) generation of laser-induced nanostructures in materials like metals, metal oxides and semiconductors, and (ii) ultrafast excitation and energy transfer in nanoscale physical, chemical and hybrid systems. Particular emphasis is laid on the up-to-date controversially discussed mechanisms of sub-wavelength ripple formation including models of self-organized material transport and multiphoton excitation channels, nonlinear optics of plasmonic structures (nanotips, nanowires, 3D-metamaterials), and energy localization and transport on ultrafast time scale and spatial nanoscale. High-resolution spectroscopy, simulation and characterization techniques are reported. New applications of ultrashort-pulsed lasers for materials processing and the use of nanostructured materials for characterizing laser fields and laser-matter-interactions are discussed.

  12. ZnS/PVA nanocomposites for nonlinear optical applications

    Science.gov (United States)

    Ozga, K.; Michel, J.; Nechyporuk, B. D.; Ebothé, J.; Kityk, I. V.; Albassam, A. A.; El-Naggar, A. M.; Fedorchuk, A. O.

    2016-07-01

    We have found a correlation between ZnS nanocomposite nonlinear optical features and technological processing using electrolytic method. In the earlier researches this factor was neglected. However, it may open a new stage for operation by photovoltaic features of the well known semiconductors within a wide range of magnitudes. The titled nanostructured zinc sulfide (ZnS) was synthesized by electrolytic method. The obtained ZnS nano-crystallites possessed nano-particles sizes varying within 1.6 nm…1.8 nm. The titled samples were analyzed by XRD, HR-TEM, STEM, and nonlinear optical methods such as photo-induced two-photon absorption (TPA) and second harmonic generation (SHG). For this reason the nano-powders were embedded into the photopolymer poly(vinyl) alcohol (PVA) matrices. Role of aggregation in the mentioned properties is discussed. Possible origin of the such correlations are discussed.

  13. Performance emulation and parameter estimation for nonlinear fibre-optic links

    DEFF Research Database (Denmark)

    Piels, Molly; Porto da Silva, Edson; Zibar, Darko

    2016-01-01

    Fibre-optic communication systems, especially when operating in the nonlinear regime, generally do not perform exactly as theory would predict. A number of methods for data-based evaluation of nonlinear fibre-optic link parameters, both for accurate performance emulation and optimization...

  14. Homogenized description and retrieval method of nonlinear metasurfaces

    Science.gov (United States)

    Liu, Xiaojun; Larouche, Stéphane; Smith, David R.

    2018-03-01

    A patterned, plasmonic metasurface can strongly scatter incident light, functioning as an extremely low-profile lens, filter, reflector or other optical device. When the metasurface is patterned uniformly, its linear optical properties can be expressed using effective surface electric and magnetic polarizabilities obtained through a homogenization procedure. The homogenized description of a nonlinear metasurface, however, presents challenges both because of the inherent anisotropy of the medium as well as the much larger set of potential wave interactions available, making it challenging to assign effective nonlinear parameters to the otherwise inhomogeneous layer of metamaterial elements. Here we show that a homogenization procedure can be developed to describe nonlinear metasurfaces, which derive their nonlinear response from the enhanced local fields arising within the structured plasmonic elements. With the proposed homogenization procedure, we are able to assign effective nonlinear surface polarization densities to a nonlinear metasurface, and link these densities to the effective nonlinear surface susceptibilities and averaged macroscopic pumping fields across the metasurface. These effective nonlinear surface polarization densities are further linked to macroscopic nonlinear fields through the generalized sheet transition conditions (GSTCs). By inverting the GSTCs, the effective nonlinear surface susceptibilities of the metasurfaces can be solved for, leading to a generalized retrieval method for nonlinear metasurfaces. The application of the homogenization procedure and the GSTCs are demonstrated by retrieving the nonlinear susceptibilities of a SiO2 nonlinear slab. As an example, we investigate a nonlinear metasurface which presents nonlinear magnetoelectric coupling in near infrared regime. The method is expected to apply to any patterned metasurface whose thickness is much smaller than the wavelengths of operation, with inclusions of arbitrary geometry

  15. Nonlinear optics of fibre event horizons.

    Science.gov (United States)

    Webb, Karen E; Erkintalo, Miro; Xu, Yiqing; Broderick, Neil G R; Dudley, John M; Genty, Goëry; Murdoch, Stuart G

    2014-09-17

    The nonlinear interaction of light in an optical fibre can mimic the physics at an event horizon. This analogue arises when a weak probe wave is unable to pass through an intense soliton, despite propagating at a different velocity. To date, these dynamics have been described in the time domain in terms of a soliton-induced refractive index barrier that modifies the velocity of the probe. Here we complete the physical description of fibre-optic event horizons by presenting a full frequency-domain description in terms of cascaded four-wave mixing between discrete single-frequency fields, and experimentally demonstrate signature frequency shifts using continuous wave lasers. Our description is confirmed by the remarkable agreement with experiments performed in the continuum limit, reached using ultrafast lasers. We anticipate that clarifying the description of fibre event horizons will significantly impact on the description of horizon dynamics and soliton interactions in photonics and other systems.

  16. Unidirectional transmission in 1D nonlinear photonic crystal based on topological phase reversal by optical nonlinearity

    OpenAIRE

    Chong Li; Xiaoyong Hu; Hong Yang; Qihuang Gong

    2017-01-01

    We propose a scheme of unidirectional transmission in a 1D nonlinear topological photonic crystal based on the topological edge state and three order optical nonlinearity. The 1D photonic crystals consists of a nonlinear photonic crystal L and a linear photonic crystal R. In the backward direction, light is totally reflected for the photons transmission prohibited by the bandgap. While in the forward direction, light interacts with the nonlinear photonic crystal L by optical Kerr effect, brin...

  17. The Quest for the Ultimate Nonlinear Optical Material

    Science.gov (United States)

    Dagenais, M.

    1990-10-01

    The following sections are included: * Introduction * From Infancy to the Real World * Highly Efficient Nonlinear Optical Materials for Switching and Processing * The Era of Pragmatism * Conclusion * References

  18. Spin and diamagnetism in linear and nonlinear optics

    International Nuclear Information System (INIS)

    Andersen, Torsten; Keller, Ole; Huebner, Wolfgang; Johansson, Boerje

    2004-01-01

    We present a local-field theory for spin and diamagnetism in linear and nonlinear optics. We examine all the processes contained in the Pauli Hamiltonian and its corresponding microscopic current density, including the terms depending on the electron spin. The resulting general real-space conductivities are presented and discussed. To quantify the implications of including the spin, we study the linear and nonlinear optical properties of free-electron metals, represented by the screened homogeneous electron gas. The real-space formalism is transformed into Fourier space, and the symmetries of the linear and nonlinear optical conductivities in a homogeneous electron gas are discussed. Numerical results are presented for the homogeneous electron gas, in which we treat ω and q as independent variables, thereby opening the theory to near-field optics and the study of evanescent waves. We show that in regions of the ω-q spectrum, the presence of diamagnetism and spin dynamics significantly alters the response in comparison to considering only the paramagnetic response. Additionally, we discuss the effects of screening, and we finish our treatment by a discussion of how to connect the present theory to existing methods in ab initio solid-state physics

  19. Signaling on the continuous spectrum of nonlinear optical fiber.

    Science.gov (United States)

    Tavakkolnia, Iman; Safari, Majid

    2017-08-07

    This paper studies different signaling techniques on the continuous spectrum (CS) of nonlinear optical fiber defined by nonlinear Fourier transform. Three different signaling techniques are proposed and analyzed based on the statistics of the noise added to CS after propagation along the nonlinear optical fiber. The proposed methods are compared in terms of error performance, distance reach, and complexity. Furthermore, the effect of chromatic dispersion on the data rate and noise in nonlinear spectral domain is investigated. It is demonstrated that, for a given sequence of CS symbols, an optimal bandwidth (or symbol rate) can be determined so that the temporal duration of the propagated signal at the end of the fiber is minimized. In effect, the required guard interval between the subsequently transmitted data packets in time is minimized and the effective data rate is significantly enhanced. Moreover, by selecting the proper signaling method and design criteria a distance reach of 7100 km is reported by only singling on CS at a rate of 9.6 Gbps.

  20. Linear and nonlinear optical properties of borate crystals as ...

    Indian Academy of Sciences (India)

    Unknown

    crystal series, with an accuracy acceptable for materials development/design, and answer the questions often ... Optical property; nonlinear optical crystals; first principles calculation. 1. ..... system, and is not in concept suitable to excitation pro-.

  1. Non-linear optical imaging – Introduction and pharmaceutical applications

    NARCIS (Netherlands)

    Fussell, A.L.; Isomaki, Antti; Strachan, Clare J.

    2013-01-01

    Nonlinear optical imaging is an emerging technology with much potential in pharmaceutical analysis. The technique encompasses a range of optical phenomena, including coherent anti-Stokes Raman scattering (CARS), second harmonic generation (SHG), and twophoton excited fluorescence (TPEF). The

  2. Optical Chirality in Nonlinear Optics: Application to High Harmonic Generation.

    Science.gov (United States)

    Neufeld, Ofer; Cohen, Oren

    2018-03-30

    Optical chirality (OC)-one of the fundamental quantities of electromagnetic fields-corresponds to the instantaneous chirality of light. It has been utilized for exploring chiral light-matter interactions in linear optics, but has not yet been applied to nonlinear processes. Motivated to explore the role of OC in the generation of helically polarized high-order harmonics and attosecond pulses, we first separate the OC of transversal and paraxial beams to polarization and orbital terms. We find that the polarization-associated OC of attosecond pulses corresponds approximately to that of the pump in the quasimonochromatic case, but not in the multichromatic pump cases. We associate this discrepancy with the fact that the polarization OC of multichromatic pumps vary rapidly in time along the optical cycle. Thus, we propose new quantities, noninstantaneous polarization-associated OC, and time-scale-weighted polarization-associated OC, and show that these quantities link the chirality of multichromatic pumps and their generated attosecond pulses. The presented extension to OC theory should be useful for exploring various nonlinear chiral light-matter interactions. For example, it stimulates us to propose a tricircular pump for generation of highly elliptical attosecond pulses with a tunable ellipticity.

  3. Optical Chirality in Nonlinear Optics: Application to High Harmonic Generation

    Science.gov (United States)

    Neufeld, Ofer; Cohen, Oren

    2018-03-01

    Optical chirality (OC)—one of the fundamental quantities of electromagnetic fields—corresponds to the instantaneous chirality of light. It has been utilized for exploring chiral light-matter interactions in linear optics, but has not yet been applied to nonlinear processes. Motivated to explore the role of OC in the generation of helically polarized high-order harmonics and attosecond pulses, we first separate the OC of transversal and paraxial beams to polarization and orbital terms. We find that the polarization-associated OC of attosecond pulses corresponds approximately to that of the pump in the quasimonochromatic case, but not in the multichromatic pump cases. We associate this discrepancy with the fact that the polarization OC of multichromatic pumps vary rapidly in time along the optical cycle. Thus, we propose new quantities, noninstantaneous polarization-associated OC, and time-scale-weighted polarization-associated OC, and show that these quantities link the chirality of multichromatic pumps and their generated attosecond pulses. The presented extension to OC theory should be useful for exploring various nonlinear chiral light-matter interactions. For example, it stimulates us to propose a tricircular pump for generation of highly elliptical attosecond pulses with a tunable ellipticity.

  4. Evaluation of third order nonlinear optical parameters of CdS/PVA nanocomposite

    International Nuclear Information System (INIS)

    Sharma, Mamta; Tripathi, S. K.

    2015-01-01

    CdS nanoparticles dispersed in PVA are prepared by Chemical method at room temperature. The nonlinear optical parameters such as nonlinear absorption (β), nonlinear refractive index (n 2 ) and nonlinear susceptibility (χ 3 ) are calculated for this sample by using Z-scan technique. CdS/PVA samples show the two photon absorption mechanism. The third order nonlinear susceptibility is calculated from n 2 and β and is found to be of the order of 10 −7 – 10 −8 m 2 /V 2 . The larger value of third order nonlinear susceptibility is due to dielectric and quantum confinement effect

  5. Nonlinear and quantum optics with liquid crystals

    International Nuclear Information System (INIS)

    Lukishova, Svetlana G

    2014-01-01

    Thermotropic liquid crystals' usual application is display technology. This paper describes experiments on light interaction with pure and doped liquid crystals under for these materials unconventional incident light powers: (1) under high-power laser irradiation, and (2) at the single-photon level. In (1), I will outline several nonlinear optical effects under high-power, nanosecond laser irradiation which should be taken into account in the design of lasers with liquid crystal components and in fabrication of optical power limiters based on liquid crystals: (1.1) athermal helical pitch dilation and unwinding of cholesteric mirrors (both in free space and inside laser resonators); (1.2) some pitfalls in measurements of refractive nonlinearity using z-scan technique under two-photon or linear absorption of liquids; (1.3) the first observation of thermal lens effects in liquid crystals under several-nanosecond, low-pulse-repetition rate (2-10 Hz) laser irradiation in the presence of two-photon absorption; (1.4) feedback-free kaleidoscope of patterns (hexagons, stripes, etc.) in dye-doped liquid crystals. In (2), at the single-photon level, it will be shown that with a proper selection of liquid crystals and a single-emitter dopant spectral range, liquid crystal structures can be used to control emitted single photons (both polarization and count rate). The application of the latter research is absolutely secure quantum communication with polarization coding of information. In particular, in (2.1), definite handedness, circular polarized cholesteric microcavity resonance in quantum dot fluorescence is reported. In (2.2), definite linear polarization of single (antibunched) photons from single-dye-molecules in planar-aligned nematic host is discussed. In (2.3), some results on photon antibunching from NV-color center in nanodiamond in liquid crystal host and circularly polarized fluorescence of definite handedness from nanocrystals doped with trivalent ions of

  6. A Photonic Basis for Deriving Nonlinear Optical Response

    Science.gov (United States)

    Andrews, David L.; Bradshaw, David S.

    2009-01-01

    Nonlinear optics is generally first presented as an extension of conventional optics. Typically the subject is introduced with reference to a classical oscillatory electric polarization, accommodating correction terms that become significant at high intensities. The material parameters that quantify the extent of the nonlinear response are cast as…

  7. Evaluation of polymer based third order nonlinear integrated optics devices

    NARCIS (Netherlands)

    Driessen, A.; Hoekstra, Hugo; Blom, F.C.; Horst, F.; Horst, F.; Krijnen, Gijsbertus J.M.; van Schoot, J.B.P.; van Schoot, J.B.P.; Lambeck, Paul; Popma, T.J.A.; Diemeer, Mart

    Nonlinear polymers are promising materials for high speed active integrated optics devices. In this paper we evaluate the perspectives polymer based nonlinear optical devices can offer. Special attention is directed to the materials aspects. In our experimental work we applied mainly Akzo Nobel DANS

  8. Moment methods for nonlinear maps

    International Nuclear Information System (INIS)

    Pusch, G.D.; Atomic Energy of Canada Ltd., Chalk River, ON

    1993-01-01

    It is shown that Differential Algebra (DA) may be used to push moments of distributions through a map, at a computational cost per moment comparable to pushing a single particle. The algorithm is independent of order, and whether or not the map is symplectic. Starting from the known result that moment-vectors transform linearly - like a tensor - even under a nonlinear map, I suggest that the form of the moment transformation rule indicates that the moment-vectors are elements of the dual to DA-vector space. I propose several methods of manipulating moments and constructing invariants using DA. I close with speculations on how DA might be used to ''close the circle'' to solve the inverse moment problem, yielding an entirely DA-and-moment-based space-charge code. (Author)

  9. Semiclassical Path Integral Calculation of Nonlinear Optical Spectroscopy.

    Science.gov (United States)

    Provazza, Justin; Segatta, Francesco; Garavelli, Marco; Coker, David F

    2018-02-13

    Computation of nonlinear optical response functions allows for an in-depth connection between theory and experiment. Experimentally recorded spectra provide a high density of information, but to objectively disentangle overlapping signals and to reach a detailed and reliable understanding of the system dynamics, measurements must be integrated with theoretical approaches. Here, we present a new, highly accurate and efficient trajectory-based semiclassical path integral method for computing higher order nonlinear optical response functions for non-Markovian open quantum systems. The approach is, in principle, applicable to general Hamiltonians and does not require any restrictions on the form of the intrasystem or system-bath couplings. This method is systematically improvable and is shown to be valid in parameter regimes where perturbation theory-based methods qualitatively breakdown. As a test of the methodology presented here, we study a system-bath model for a coupled dimer for which we compare against numerically exact results and standard approximate perturbation theory-based calculations. Additionally, we study a monomer with discrete vibronic states that serves as the starting point for future investigation of vibronic signatures in nonlinear electronic spectroscopy.

  10. Nonlinear optical effects in pure and N-doped semiconductors

    International Nuclear Information System (INIS)

    Donlagic, N.S.

    2000-01-01

    Over the last decades, the nonlinear optical properties of condensed matter systems have been an attractive and fruitful field of research. While the linear response functions of solids provide information about the elementary excitations of the systems, nonlinear optical experiments give insight into the dynamics of the fundamental many-body processes which are initiated by the external excitations. Stimulated by the experimental results, new theoretical concepts and methods have been developed in order to relate the observed phenomena to the microscopic properties of the investigated materials. The present work deals with the study of the nonlinear dynamics of the optical interband polarization in pure and n-doped semiconductors.In the first part of the thesis, the relaxation behavior of optically excited electron-hole pairs in a one-dimensional semiconductor, which are coupled to longitudinal optical phonons with an initial lattice temperature T>0, is studied with the help of quantum kinetic equations. Apart from Hartree-Fock-like Coulomb contributions, these equations contain additional Coulomb terms, the so-called vertex corrections, by which the influence of the electron-electron interaction on the electron-phonon scattering processes is taken into account. The numerical studies indicate that the vertex corrections are essential for a correct description of the excitonic dynamics.In the second part of the thesis, the attention is shifted to the characteristics of the optical response of a one-dimensional n-doped two-band semiconductor whose conduction band has been linearized with respect to the two Fermi points. Due to the linearization it is possible to calculate the linear and nonlinear response functions of the interacting electron system exactly. These response functions are then used in order to determine the linear absorption spectrum and the time-integrated signal of a degenerated four-wave-mixing experiment. It is shown that the well-known features

  11. NONLINEAR OPTICAL MOLECULAR CRYSTAL BASED ON 2,6-DIAMINOPYRIDINE: SYNTHESIS AND CHARACTERIZATION

    Directory of Open Access Journals (Sweden)

    I. M. Pavlovetc

    2014-05-01

    Full Text Available The paper deals with investigation of a new nonlinear optical material based on nonlinear optical chromophore (4-Nitrophenol and aminopyridine (2,6-Diaminopyridine. Calculation results are presented for molecular packing in the crystalline compound, based on the given components. According to these results the finite material must have a noncentrosymmetric lattice, which determines the presence of the second order nonlinear optical response. Investigations carried out in this work confirm these calculations. Results of experiments are given describing the co-crystallization of these components and the following re-crystallization of the obtained material. In order to get a monocrystal form, the optimal conditions for the synthesis of molecular crystals based on these components are determined. Sufficiently large homogeneous crystals are obtained, that gave the possibility to record their spectra in the visible and near infrared parts of the spectrum, to determine their nonlinear optical properties and the level of homogeneity. Their optical (optical transmission and optical laser damage threshold and nonlinear optical properties are presented. For observation and measurement of the nonlinear optical properties an installation was built which implements the comparative method for measurements of nonlinear optical properties. A potassium titanyl oxide phosphate crystal was used as a sample for comparison. Results are given for the conversion efficiency of the primary laser radiation in the second optical harmonic relative to the signal obtained on the potassium titanyl oxide phosphate crystal. Obtained results show that the molecular co-crystal based on 2,6-Diaminopyridine is a promising nonlinear optical material for generating the second optical harmonic on the Nd: YAG laser (532 nm.

  12. Nonlinear optical characteristics of monolayer MoSe{sub 2}

    Energy Technology Data Exchange (ETDEWEB)

    Le, Chinh Tam; Ullah, Farman; Senthilkumar, Velusamy; Kim, Yong Soo [Department of Physics and Energy Harvest Storage Research Center, University of Ulsan (Korea, Republic of); Clark, Daniel J.; Jang, Joon I. [Department of Physics, Applied Physics and Astronomy, Binghamton University, Binghamton, NY (United States); Sim, Yumin; Seong, Maeng-Je [Department of Physics, Chung-Ang University, Seoul (Korea, Republic of); Chung, Koo-Hyun [School of Mechanical Engineering, University of Ulsan (Korea, Republic of); Park, Hyoyeol [Electronics, Communication and Semiconductor Applications Department, Ulsan College (Korea, Republic of)

    2016-08-15

    In this study, we utilized picosecond pulses from an Nd:YAG laser to investigate the nonlinear optical characteristics of monolayer MoSe{sub 2}. Two-step growth involving the selenization of pulsed-laser-deposited MoO{sub 3} film was employed to yield the MoSe{sub 2} monolayer on a SiO{sub 2}/Si substrate. Raman scattering, photoluminescence (PL) spectroscopy, and atomic force microscopy verified the high optical quality of the monolayer. The second-order susceptibility χ{sup (2)} was calculated to be ∝50 pm V{sup -1} at the second harmonic wavelength λ{sub SHG} ∝810 nm, which is near the optical gap of the monolayer. Interestingly, our wavelength-dependent second harmonic scan can identify the bound excitonic states including negatively charged excitons much more efficiently, compared with the PL method at room temperature. Additionally, the MoSe{sub 2} monolayer exhibits a strong laser-induced damage threshold ∝16 GW cm{sup -2} under picosecond-pulse excitation{sub .} Our findings suggest that monolayer MoSe{sub 2} can be considered as a promising candidate for high-power, thin-film-based nonlinear optical devices and applications. (copyright 2016 by WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  13. Characterizing the Statistics of a Bunch of Optical Pulses Using a Nonlinear Optical Loop Mirror

    Directory of Open Access Journals (Sweden)

    Olivier Pottiez

    2015-01-01

    Full Text Available We propose in this work a technique for determining the amplitude distribution of a wave packet containing a large number of short optical pulses with different amplitudes. The technique takes advantage of the fast response of the optical Kerr effect in a fiber nonlinear optical loop mirror (NOLM. Under some assumptions, the statistics of the pulses can be determined from the energy transfer characteristic of the packet through the NOLM, which can be measured with a low-frequency detection setup. The statistical distribution is retrieved numerically by approximating the solution of a system of nonlinear algebraic equations using the least squares method. The technique is demonstrated numerically in the case of a packet of solitons.

  14. Computational studies of third-order nonlinear optical properties of ...

    Indian Academy of Sciences (India)

    Anuj Kumar

    2017-06-20

    Jun 20, 2017 ... Department of Physics, Jaypee University of Engineering and Technology, Raghogarh,. Guna 473 226, India. ∗ ... properties and other molecular properties of the organic nonlinear optical crystal 2-aminopyridinium p- toluenesulphonate ... nal processing, optical limiting, optical logic gates, laser radiation ...

  15. Nonlinear optical studies of curcumin metal derivatives with cw laser

    Energy Technology Data Exchange (ETDEWEB)

    Henari, F. Z., E-mail: fzhenari@rcsi-mub.com; Cassidy, S. [Department of Basic Medical Sciences, Royal College of Surgeons in Ireland, Medical University of Bahrain (Bahrain)

    2015-03-30

    We report on measurements of the nonlinear refractive index and nonlinear absorption coefficients for curcumin and curcumin metal complexes of boron, copper, and iron at different wavelengths using the Z-scan technique. These materials are found to be novel nonlinear media. It was found that the addition of metals slightly influences its nonlinearity. These materials show a large negative nonlinear refractive index of the order of 10{sup −7} cm{sup 2}/W and negative nonlinear absorption of the order of 10{sup −6} cm/W. The origin of the nonlinearity was investigated by comparison of the formalism that is known as the Gaussian decomposition model with the thermal lens model. The optical limiting behavior based on the nonlinear refractive index was also investigated.

  16. Nonlinear optical studies of curcumin metal derivatives with cw laser

    International Nuclear Information System (INIS)

    Henari, F. Z.; Cassidy, S.

    2015-01-01

    We report on measurements of the nonlinear refractive index and nonlinear absorption coefficients for curcumin and curcumin metal complexes of boron, copper, and iron at different wavelengths using the Z-scan technique. These materials are found to be novel nonlinear media. It was found that the addition of metals slightly influences its nonlinearity. These materials show a large negative nonlinear refractive index of the order of 10 −7 cm 2 /W and negative nonlinear absorption of the order of 10 −6 cm/W. The origin of the nonlinearity was investigated by comparison of the formalism that is known as the Gaussian decomposition model with the thermal lens model. The optical limiting behavior based on the nonlinear refractive index was also investigated

  17. Topology optimization of nonlinear optical devices

    DEFF Research Database (Denmark)

    Jensen, Jakob Søndergaard

    2011-01-01

    This paper considers the design of nonlinear photonic devices. The nonlinearity stems from a nonlinear material model with a permittivity that depends on the local time-averaged intensity of the electric field. A finite element model is developed for time-harmonic wave propagation and an incremen......This paper considers the design of nonlinear photonic devices. The nonlinearity stems from a nonlinear material model with a permittivity that depends on the local time-averaged intensity of the electric field. A finite element model is developed for time-harmonic wave propagation...... limiter. Here, air, a linear and a nonlinear material are distributed so that the wave transmission displays a strong sensitivity to the amplitude of the incoming wave....

  18. Methods of stability analysis in nonlinear mechanics

    International Nuclear Information System (INIS)

    Warnock, R.L.; Ruth, R.D.; Gabella, W.; Ecklund, K.

    1989-01-01

    We review our recent work on methods to study stability in nonlinear mechanics, especially for the problems of particle accelerators, and compare our ideals to those of other authors. We emphasize methods that (1) show promise as practical design tools, (2) are effective when the nonlinearity is large, and (3) have a strong theoretical basis. 24 refs., 2 figs., 2 tabs

  19. Optical nonlinearity enhancement with graphene-decorated silicon waveguides

    Science.gov (United States)

    Ishizawa, Atsushi; Kou, Rai; Goto, Takahiro; Tsuchizawa, Tai; Matsuda, Nobuyuki; Hitachi, Kenichi; Nishikawa, Tadashi; Yamada, Koji; Sogawa, Tetsuomi; Gotoh, Hideki

    2017-04-01

    Broadband on-chip optical frequency combs (OFCs) are important for expanding the functionality of photonic integrated circuits. Here, we demonstrate a huge local optical nonlinearity enhancement using graphene. A waveguide is decorated with graphene by precisely manipulating graphene’s area and position. Our approach simultaneously achieves both an extremely efficient supercontinuum and ultra-short pulse generation. With our graphene-decorated silicon waveguide (G-SWG), we have achieved enhanced spectral broadening of femtosecond pump pulses, along with an eightfold increase in the output optical intensity at a wavelength approximately 200 nm shorter than that of the pump pulses. We also found that this huge nonlinearity works as a compressor that effectively compresses pulse width from 80 to 15.7 fs. Our results clearly show the potential for our G-SWG to greatly boost the speed and capacity of future communications with lower power consumption, and our method will further decrease the required pump laser power because it can be applied to decorate various kinds of waveguides with various two-dimensional materials.

  20. Optoelectronic and nonlinear optical processes in low dimensional ...

    Indian Academy of Sciences (India)

    Optoelectronic process; nonlinear optical process; semiconductor. Quest for ever faster and intelligent information processing technologies has sparked ..... Schematic energy level diagram for the proposed 4-level model. States other than the.

  1. Squeezing in multi-mode nonlinear optical state truncation

    International Nuclear Information System (INIS)

    Said, R.S.; Wahiddin, M.R.B.; Umarov, B.A.

    2007-01-01

    In this Letter, we show that multi-mode qubit states produced via nonlinear optical state truncation driven by classical external pumpings exhibit squeezing condition. We restrict our discussions to the two- and three-mode cases

  2. Field-enhanced nonlinear optical properties of organic nanofibers

    DEFF Research Database (Denmark)

    Kostiučenko, Oksana; Fiutowski, Jacek; Brewer, Jonathan R.

    2014-01-01

    Second harmonic generation in nonlinearly optically active organic nanofibers, generated via self-assembled surface growth from nonsymmetrically functionalized para-quarterphenylene (CNHP4) molecules, has been investigated. After the growth on mica templates, nanofibers have been transferred onto...

  3. Nonlinear optical beam manipulation, beam combining, and atmospheric propagation

    International Nuclear Information System (INIS)

    Fischer, R.A.

    1988-01-01

    These proceedings collect papers on optics: Topics include: diffraction properties of laser speckle, coherent beam combination by plasma modes, nonlinear responses, deformable mirrors, imaging radiometers, electron beam propagation in inhomogeneous media, and stability of laser beams in a structured environment

  4. The chemistry and physics of nonlinear optical materials

    International Nuclear Information System (INIS)

    Velsko, S.P.; Eimerl, D.

    1989-01-01

    Recent efforts to engineer new nonlinear optical materials with specific desired characteristics has engendered a need for a theoretical description of optical properties which is readily accessible to chemists, yet correctly treats the essential physics of dielectric response. This paper describes a simple empirical molecular orbital model which gives useful insights into the relationship between chemical composition, crystalline structure, and optical susceptibilities. The authors compare the probabilities of finding new harmonic generators in various chemical classes. Rigorous bounds on the magnitudes of linear and nonlinear optical coefficients and their anisotropies are also discussed

  5. Ultra-Fast Optical Signal Processing in Nonlinear Silicon Waveguides

    DEFF Research Database (Denmark)

    Oxenløwe, Leif Katsuo; Galili, Michael; Pu, Minhao

    2011-01-01

    We describe recent demonstrations of exploiting highly nonlinear silicon nanowires for processing Tbit/s optical data signals. We perform demultiplexing and optical waveform sampling of 1.28 Tbit/s and wavelength conversion of 640 Gbit/s data signals.......We describe recent demonstrations of exploiting highly nonlinear silicon nanowires for processing Tbit/s optical data signals. We perform demultiplexing and optical waveform sampling of 1.28 Tbit/s and wavelength conversion of 640 Gbit/s data signals....

  6. Ripple distribution for nonlinear fiber-optic channels.

    Science.gov (United States)

    Sorokina, Mariia; Sygletos, Stylianos; Turitsyn, Sergei

    2017-02-06

    We demonstrate data rates above the threshold imposed by nonlinearity on conventional optical signals by applying novel probability distribution, which we call ripple distribution, adapted to the properties of the fiber channel. Our results offer a new direction for signal coding, modulation and practical nonlinear distortions compensation algorithms.

  7. Nonlinear Fourier transform for dual-polarization optical communication system

    DEFF Research Database (Denmark)

    Gaiarin, Simone

    communication is considered an emerging paradigm in fiber-optic communications that could potentially overcome these limitations. It relies on a mathematical technique called “inverse scattering transform” or “nonlinear Fourier transform (NFT)” to exploit the “hidden” linearity of the nonlinear Schrödinger...

  8. A novel organic nonlinear optical crystal: Creatininium succinate

    Energy Technology Data Exchange (ETDEWEB)

    Thirumurugan, R.; Anitha, K., E-mail: singlecerystalxrd@gmail.ciom [School of Physics, Madurai Kamraj University, Madurai 625021 (India)

    2015-06-24

    A novel organic material complex of creatininium succinate (CS) has been synthesized and single crystals were grown by the reaction of creatinine and succinic acid from aqueous solution by employing the technique of slow evaporation at room temperature. The structure of the grown crystal has been elucidated using single crystal X-ray diffraction analysis and the structure was refined by least-squares method to R = 0.027 for 1840 reflections. FT-IR spectral investigation has been carried out to identify the various functional groups in the title compound. UV–Vis transmission was carried out which shows the crystal has a good optical transmittance in the visible region with lower cutoff wavelength around 220 nm. Nonlinear optical property of the crystal was confirmed by Kurtz-Perry powder technique.

  9. All-optical universal logic gates on nonlinear multimode interference coupler using tunable input intensity

    Science.gov (United States)

    Tajaldini, Mehdi; Jafri, Mohd Zubir Mat

    2015-04-01

    The theory of Nonlinear Modal Propagation Analysis Method (NMPA) have shown significant features of nonlinear multimode interference (MMI) coupler with compact dimension and when launched near the threshold of nonlinearity. Moreover, NMPA have the potential to allow studying the nonlinear MMI based the modal interference to explorer the phenomenon that what happen due to the natural of multimode region. Proposal of all-optical switch based NMPA has approved its capability to achieving the all-optical gates. All-optical gates have attracted increasing attention due to their practical utility in all-optical signal processing networks and systems. Nonlinear multimode interference devices could apply as universal all-optical gates due to significant features that NMPA introduce them. In this Paper, we present a novel Ultra-compact MMI coupler based on NMPA method in low intensity compared to last reports either as a novel design method and potential application for optical NAND, NOR as universal gates on single structure for Boolean logic signal processing devices and optimize their application via studding the contrast ratio between ON and OFF as a function of output width. We have applied NMPA for several applications so that the miniaturization in low nonlinear intensities is their main purpose.

  10. Explicit formulation of second and third order optical nonlinearity in the FDTD framework

    Science.gov (United States)

    Varin, Charles; Emms, Rhys; Bart, Graeme; Fennel, Thomas; Brabec, Thomas

    2018-01-01

    The finite-difference time-domain (FDTD) method is a flexible and powerful technique for rigorously solving Maxwell's equations. However, three-dimensional optical nonlinearity in current commercial and research FDTD softwares requires solving iteratively an implicit form of Maxwell's equations over the entire numerical space and at each time step. Reaching numerical convergence demands significant computational resources and practical implementation often requires major modifications to the core FDTD engine. In this paper, we present an explicit method to include second and third order optical nonlinearity in the FDTD framework based on a nonlinear generalization of the Lorentz dispersion model. A formal derivation of the nonlinear Lorentz dispersion equation is equally provided, starting from the quantum mechanical equations describing nonlinear optics in the two-level approximation. With the proposed approach, numerical integration of optical nonlinearity and dispersion in FDTD is intuitive, transparent, and fully explicit. A strong-field formulation is also proposed, which opens an interesting avenue for FDTD-based modelling of the extreme nonlinear optics phenomena involved in laser filamentation and femtosecond micromachining of dielectrics.

  11. Polarization dependent dispersion and its impact on optical parametric process in high nonlinear microstructure fibre

    International Nuclear Information System (INIS)

    Xiao Li; Zhang Wei; Huang Yidong; Peng Jiangde

    2008-01-01

    High nonlinear microstructure fibre (HNMF) is preferred in nonlinear fibre optics, especially in the applications of optical parametric effects, due to its high optical nonlinear coefficient. However, polarization dependent dispersion will impact the nonlinear optical parametric process in HNMFs. In this paper, modulation instability (MI) method is used to measure the polarization dependent dispersion of a piece of commercial HNMF, including the group velocity dispersion, the dispersion slope, the fourth-order dispersion and group birefringence. It also experimentally demonstrates the impact of the polarization dependent dispersion on the continuous wave supercontinuum (SC) generation. On one axis MI sidebands with symmetric frequency detunings are generated, while on the other axis with larger MI frequency detuning, SC is generated by soliton self-frequency shift

  12. Regularized linearization for quantum nonlinear optical cavities: application to degenerate optical parametric oscillators.

    Science.gov (United States)

    Navarrete-Benlloch, Carlos; Roldán, Eugenio; Chang, Yue; Shi, Tao

    2014-10-06

    Nonlinear optical cavities are crucial both in classical and quantum optics; in particular, nowadays optical parametric oscillators are one of the most versatile and tunable sources of coherent light, as well as the sources of the highest quality quantum-correlated light in the continuous variable regime. Being nonlinear systems, they can be driven through critical points in which a solution ceases to exist in favour of a new one, and it is close to these points where quantum correlations are the strongest. The simplest description of such systems consists in writing the quantum fields as the classical part plus some quantum fluctuations, linearizing then the dynamical equations with respect to the latter; however, such an approach breaks down close to critical points, where it provides unphysical predictions such as infinite photon numbers. On the other hand, techniques going beyond the simple linear description become too complicated especially regarding the evaluation of two-time correlators, which are of major importance to compute observables outside the cavity. In this article we provide a regularized linear description of nonlinear cavities, that is, a linearization procedure yielding physical results, taking the degenerate optical parametric oscillator as the guiding example. The method, which we call self-consistent linearization, is shown to be equivalent to a general Gaussian ansatz for the state of the system, and we compare its predictions with those obtained with available exact (or quasi-exact) methods. Apart from its operational value, we believe that our work is valuable also from a fundamental point of view, especially in connection to the question of how far linearized or Gaussian theories can be pushed to describe nonlinear dissipative systems which have access to non-Gaussian states.

  13. Effective-medium theory for nonlinear magneto-optics in magnetic granular alloys: cubic nonlinearity

    International Nuclear Information System (INIS)

    Granovsky, Alexander B.; Kuzmichov, Michail V.; Clerc, J.-P.; Inoue, Mitsuteru

    2003-01-01

    We propose a simple effective-medium approach for calculating the effective dielectric function of a magnetic metal-insulator granular alloy in which there is a weakly nonlinear relation between electric displacement D and electric field E for both constituent materials of the form D i =ε i (0) E i +χ i (3) |E i | 2 E i . We assume that linear ε i (0) and cubic nonlinear χ i (3) dielectric functions are diagonal and linear with magnetization non-diagonal components. For such metal-insulator composite magneto-optical effects depend on a light intensity and the effective cubic dielectric function χ eff (3) can be significantly greater (up to 10 3 times) than that for constituent materials. The calculation scheme is based on the Bergman and Stroud-Hui theory of nonlinear optical properties of granular matter. The giant cubic magneto-optical nonlinearity is found for composites with metallic volume fraction close to the percolation threshold and at a resonance of optical conductivity. It is shown that a composite may exhibit nonlinear magneto-optics even when both constituent materials have no cubic magneto-optical nonlinearity

  14. Effective-medium theory for nonlinear magneto-optics in magnetic granular alloys: cubic nonlinearity

    Energy Technology Data Exchange (ETDEWEB)

    Granovsky, Alexander B. E-mail: granov@magn.ru; Kuzmichov, Michail V.; Clerc, J.-P.; Inoue, Mitsuteru

    2003-03-01

    We propose a simple effective-medium approach for calculating the effective dielectric function of a magnetic metal-insulator granular alloy in which there is a weakly nonlinear relation between electric displacement D and electric field E for both constituent materials of the form D{sub i}={epsilon}{sub i}{sup (0)}E{sub i} +{chi}{sub i}{sup (3)}|E{sub i}|{sup 2}E{sub i}. We assume that linear {epsilon}{sub i}{sup (0)} and cubic nonlinear {chi}{sub i}{sup (3)} dielectric functions are diagonal and linear with magnetization non-diagonal components. For such metal-insulator composite magneto-optical effects depend on a light intensity and the effective cubic dielectric function {chi}{sub eff}{sup (3)} can be significantly greater (up to 10{sup 3} times) than that for constituent materials. The calculation scheme is based on the Bergman and Stroud-Hui theory of nonlinear optical properties of granular matter. The giant cubic magneto-optical nonlinearity is found for composites with metallic volume fraction close to the percolation threshold and at a resonance of optical conductivity. It is shown that a composite may exhibit nonlinear magneto-optics even when both constituent materials have no cubic magneto-optical nonlinearity.

  15. Intense laser effects on nonlinear optical absorption and optical rectification in single quantum wells under applied electric and magnetic field

    International Nuclear Information System (INIS)

    Duque, C.A.; Kasapoglu, E.; Sakiroglu, S.; Sari, H.; Soekmen, I.

    2011-01-01

    In this work the effects of intense laser on the electron-related nonlinear optical absorption and nonlinear optical rectification in GaAs-Ga 1-x Al x As quantum wells are studied under, applied electric and magnetic field. The electric field is applied along the growth direction of the quantum well whereas the magnetic field has been considered to be in-plane. The calculations were performed within the density matrix formalism with the use of the effective mass and parabolic band approximations. The intense laser effects are included through the Floquet method, by modifying the confining potential associated to the heterostructure. Results are presented for the nonlinear optical absorption, the nonlinear optical rectification and the resonant peak of these two optical processes. Several configurations of the dimensions of the quantum well, the applied electric and magnetic fields, and the incident intense laser radiation have been considered. The outcome of the calculation suggests that the nonlinear optical absorption and optical rectification are non-monotonic functions of the dimensions of the heterostructure and of the external perturbations considered in this work.

  16. Shocks, singularities and oscillations in nonlinear optics and fluid mechanics

    CERN Document Server

    Santo, Daniele; Lannes, David

    2017-01-01

    The book collects the most relevant results from the INdAM Workshop "Shocks, Singularities and Oscillations in Nonlinear Optics and Fluid Mechanics" held in Rome, September 14-18, 2015. The contributions discuss recent major advances in the study of nonlinear hyperbolic systems, addressing general theoretical issues such as symmetrizability, singularities, low regularity or dispersive perturbations. It also investigates several physical phenomena where such systems are relevant, such as nonlinear optics, shock theory (stability, relaxation) and fluid mechanics (boundary layers, water waves, Euler equations, geophysical flows, etc.). It is a valuable resource for researchers in these fields. .

  17. Renormgroup symmetries in problems of nonlinear geometrical optics

    International Nuclear Information System (INIS)

    Kovalev, V.F.

    1996-01-01

    Utilization and further development of the previously announced approach [1,2] enables one to construct renormgroup symmetries for a boundary value problem for the system of equations which describes propagation of a powerful radiation in a nonlinear medium in geometrical optics approximation. With the help of renormgroup symmetries new rigorous and approximate analytical solutions of nonlinear geometrical optics equations are obtained. Explicit analytical expressions are presented that characterize spatial evolution of laser beam which has an arbitrary intensity dependence at the boundary of the nonlinear medium. (author)

  18. Scalable Nonlinear AUC Maximization Methods

    OpenAIRE

    Khalid, Majdi; Ray, Indrakshi; Chitsaz, Hamidreza

    2017-01-01

    The area under the ROC curve (AUC) is a measure of interest in various machine learning and data mining applications. It has been widely used to evaluate classification performance on heavily imbalanced data. The kernelized AUC maximization machines have established a superior generalization ability compared to linear AUC machines because of their capability in modeling the complex nonlinear structure underlying most real world-data. However, the high training complexity renders the kernelize...

  19. Second-order nonlinear optical metamaterials: ABC-type nanolaminates

    International Nuclear Information System (INIS)

    Alloatti, L.; Kieninger, C.; Lauermann, M.; Köhnle, K.; Froelich, A.; Wegener, M.; Frenzel, T.; Freude, W.; Leuthold, J.; Koos, C.

    2015-01-01

    We demonstrate a concept for second-order nonlinear metamaterials that can be obtained from non-metallic centrosymmetric constituents with inherently low optical absorption. The concept is based on iterative atomic-layer deposition of three different materials, A = Al 2 O 3 , B = TiO 2 , and C = HfO 2 . The centrosymmetry of the resulting ABC stack is broken since the ABC and the inverted CBA sequences are not equivalent—a necessary condition for non-zero second-order nonlinearity. In our experiments, we find that the bulk second-order nonlinear susceptibility depends on the density of interfaces, leading to a nonlinear susceptibility of 0.26 pm/V at a wavelength of 800 nm. ABC-type nanolaminates can be deposited on virtually any substrate and offer a promising route towards engineering of second-order optical nonlinearities at both infrared and visible wavelengths

  20. Linear and non-linear optics of condensed matter

    International Nuclear Information System (INIS)

    McLean, T.P.

    1977-01-01

    Part I - Linear optics: 1. General introduction. 2. Frequency dependence of epsilon(ω, k vector). 3. Wave-vector dependence of epsilon(ω, k vector). 4. Tensor character of epsilon(ω, k vector). Part II - Non-linear optics: 5. Introduction. 6. A classical theory of non-linear response in one dimension. 7. The generalization to three dimensions. 8. General properties of the polarizability tensors. 9. The phase-matching condition. 10. Propagation in a non-linear dielectric. 11. Second harmonic generation. 12. Coupling of three waves. 13. Materials and their non-linearities. 14. Processes involving energy exchange with the medium. 15. Two-photon absorption. 16. Stimulated Raman effect. 17. Electro-optic effects. 18. Limitations of the approach presented here. (author)

  1. Ageing of the nonlinear optical susceptibility in soft matter

    International Nuclear Information System (INIS)

    Ghofraniha, N; Conti, C; Leonardo, R Di; Ruzicka, B; Ruocco, G

    2007-01-01

    We investigate the nonlinear optics response of a colloidal dispersion undergoing dynamics slowing down with age, by using Z-scan and dynamic light scattering measurements. We study the high optical nonlinearity of an organic dye (rhodamine B) dispersed in a water-clay (laponite) suspension. We consider different clay concentrations (2.0-2.6 wt%) experiencing dynamics arrest. We find that (i) the concentration dependent exponential growth of both mean relaxation time and nonlinear absorption coefficient can be individually scaled to a master curve and (ii) the scaling times are the same for the two physical quantities. These findings indicate that the optical nonlinear susceptibility exhibits the same ageing universal scaling behaviour, typical of disordered out of equilibrium systems

  2. Third-order optical nonlinearity of N-doped graphene oxide nanocomposites at different GO ratios

    Science.gov (United States)

    Kimiagar, Salimeh; Abrinaei, Fahimeh

    2018-05-01

    In the present work, the influence of GO ratios on the structural, linear and nonlinear optical properties of nitrogen-doped graphene oxide nanocomposites (N-GO NCs) has been studied. N-GO NCs were synthesized by hydrothermal method. The XRD, FTIR, SEM, and TEM results confirmed the reduction of GO by nitrogen doping. The energy band gaps of N-GO NCs calculated from UV-Vis analyzed by using Tauc plot. To obtain further insight into potential optical changes in the N-GO NCs by increasing GO contents, Z-scan analysis was performed with nanosecond Nd-YAG laser at 532 nm. The nonlinear absorption coefficient, β, and nonlinear refractive index, n2, for N-GO NCs at the laser intensity of 113 MW/cm were measured and an increase was observed in both parameters after addition of nitrogen to GO. The third-order nonlinear optical susceptibilities of N-GO NCs were measured in the order of 10-9 esu. The results showed that N-GO NCs have negative nonlinearity which can be controlled by GO contents to obtain the highest values for nonlinear optical parameters. The nonlinear optical results not only imply that N-GO NCs can serve as an important material in the advancing of optoelectronics but also open new possibilities for the design of new graphene-based materials by variation of N and GO ratios as well as manufacturing conditions.

  3. A variational approach to nonlinear evolution equations in optics

    Indian Academy of Sciences (India)

    optics. D ANDERSON, M LISAK and A BERNTSON£. Department of Electromagnetics, Chalmers University of Technology, SE-41296 Göteborg, Sweden. £Ericsson Telcom ... Many works in nonlinear optics have made efficient ...... focusing dynamics of a laser beam (or a Bose–Einstein condensate) in a parabolic external.

  4. Nonlinear Optics: Materials, Fundamentals, and Applications. Postdeadline papers

    Science.gov (United States)

    1992-08-01

    The Nonlinear Optics: Materials, Fundamentals, and Applications conference was held on 17-21 Aug. 1992. The following topics were addressed: subpicosecond time resolved four-wave mixing spectroscopy in heteroepitaxial ZnSe thin layers; anisotropic two-photon transition in GaAs/AlGaAs multiple quantum well waveguides; two picosecond, narrow-band, tunable, optical parametric systems using BBO and LBO; second generation in an optically active liquid: experimental observation of a fourth-order optical nonlinearity due to molecular chirality; optical image recognition system implemented with a 3-D memory disk; phase-matched second-harmonic generation in waveguides of polymeric Langmuir-Blodgett films; fluence dependent dynamics observed in the resonant third-order optical response of C60 and C70 films; temporal modulation of spatial optical solitons: a variational approach; measurements of light-scattering noise during two-wave mixing in a Kerr medium; excess noise introduced by beam propagation through an atomic vapor; an approach to all-optical switching based on second-order nonlinearities; multilayer, nonlinear ARROW waveguides for surface emitted sum-frequency mixing; energy scaling of SBS phase conjugate mirrors to 4J; vector versus scalar theory for the double phase conjugate mirror; cross-talk and error probability in counter-beam lambda-multiplexed digital holograms; and modal growth of SHG in doped silica thin film waveguides.

  5. Black phosphorus: broadband nonlinear optical absorption and application

    Science.gov (United States)

    Li, Ying; He, Yanliang; Cai, Yao; Chen, Shuqing; Liu, Jun; Chen, Yu; Yuanjiang, Xiang

    2018-02-01

    Black phosphorus (BP), 2D layered material with layered dependent direct bandgap (0.3 eV (bulk), 2.0 eV (single layer)) that has gained renewed attention, has been demonstrated as an extremely appropriate optical material for broadband optical applications from infrared to mid-infrared wavebands. Herein, by coupling multi-layer BP films with microfiber, we fabricated a nonlinear optical device with long light-matter interaction distance and enhanced damage threshold. Through taking full advantage of its fine nonlinear optical absorption property, we obtained stable mode-locking (51 ps) and Q-switched mode-locking states in Yb-doped or Er-doped (403.7 fs) all-fiber lasers and the single-longitudinal-mode operation (53 kHz) in an Er-doped fiber laser with enhanced power tolerance, using the same nonlinear optical device. Our results showed that BP could be a favorable nonlinear optical material for developing BP-enabled wave-guiding photonic devices, and revealed new insight into BP for high optical power unexplored optical devices.

  6. Nonlinear fiber-optic strain sensor based on four-wave mixing in microstructured optical fiber

    DEFF Research Database (Denmark)

    Gu, Bobo; Yuan, Scott Wu; Frosz, Michael H.

    2012-01-01

    We demonstrate a nonlinear fiber-optic strain sensor, which uses the shifts of four-wave mixing Stokes and anti-Stokes peaks caused by the strain-induced changes in the structure and refractive index of a microstructured optical fiber. The sensor thus uses the inherent nonlinearity of the fiber a...

  7. Nonlinear optical properties of ultrathin metal layers

    DEFF Research Database (Denmark)

    Lysenko, Oleg

    2016-01-01

    This thesis presents experimental and theoretical studies of nonlinear propagation of ultrashort long-range surface plasmon polaritons in gold strip waveguides. The strip plasmonic waveguides are fabricated in house, and contain a gold layer, adhesion layers, and silicon dioxide cladding. The opt......This thesis presents experimental and theoretical studies of nonlinear propagation of ultrashort long-range surface plasmon polaritons in gold strip waveguides. The strip plasmonic waveguides are fabricated in house, and contain a gold layer, adhesion layers, and silicon dioxide cladding......-order nonlinear susceptibility of the plasmonic mode in the gold strip waveguides significantly depends on the metal layer thickness and laser pulse duration. This dependence is explained in detail in terms of the free-electron temporal dynamics in gold. The third-order nonlinear susceptibility of the gold layer...

  8. Nonboson treatment of excitonic nonlinearity in optically excited media

    International Nuclear Information System (INIS)

    Nguyen Ba An.

    1990-11-01

    The present article shortly reviews some recent results in the study of excitonic nonlinearity in optically excited media using a nonboson treatment for many-exciton systems. After a brief discussion of the exciton nonbosonity the closed commutation relations are given for exciton operators which hold for any exciton density and type. The nonboson treatment is then applied to the problems of intrinsic optical bistability and nonlinear polariton yielding quite interesting and new effects, e.g. new shapes of hysteresis loops of intrinsic optical bistability or anomalies of polariton dispersion. (author). 71 refs, 4 figs

  9. Comparison of some nonlinear smoothing methods

    International Nuclear Information System (INIS)

    Bell, P.R.; Dillon, R.S.

    1977-01-01

    Due to the poor quality of many nuclear medicine images, computer-driven smoothing procedures are frequently employed to enhance the diagnostic utility of these images. While linear methods were first tried, it was discovered that nonlinear techniques produced superior smoothing with little detail suppression. We have compared four methods: Gaussian smoothing (linear), two-dimensional least-squares smoothing (linear), two-dimensional least-squares bounding (nonlinear), and two-dimensional median smoothing (nonlinear). The two dimensional least-squares procedures have yielded the most satisfactorily enhanced images, with the median smoothers providing quite good images, even in the presence of widely aberrant points

  10. Hofstadter butterflies in nonlinear Harper lattices, and their optical realizations

    International Nuclear Information System (INIS)

    Manela, Ofer; Segev, Mordechai; Christodoulides, Demetrios N; Kip, Detlef

    2010-01-01

    The ubiquitous Hofstadter butterfly describes a variety of systems characterized by incommensurable periodicities, ranging from Bloch electrons in magnetic fields and the quantum Hall effect to cold atoms in optical lattices and more. Here, we introduce nonlinearity into the underlying (Harper) model and study the nonlinear spectra and the corresponding extended eigenmodes of nonlinear quasiperiodic systems. We show that the spectra of the nonlinear eigenmodes form deformed versions of the Hofstadter butterfly and demonstrate that the modes can be classified into two families: nonlinear modes that are a 'continuation' of the linear modes of the system and new nonlinear modes that have no counterparts in the linear spectrum. Finally, we propose an optical realization of the linear and nonlinear Harper models in transversely modulated waveguide arrays, where these Hofstadter butterflies can be observed. This work is relevant to a variety of other branches of physics beyond optics, such as disorder-induced localization in ultracold bosonic gases, localization transition processes in disordered lattices, and more.

  11. Hofstadter butterflies in nonlinear Harper lattices, and their optical realizations

    Energy Technology Data Exchange (ETDEWEB)

    Manela, Ofer; Segev, Mordechai [Department of Physics and Solid State Institute, Technion, Haifa 32000 (Israel); Christodoulides, Demetrios N [College of Optics/CREOL, University of Central Florida, FL 32816-2700 (United States); Kip, Detlef, E-mail: msegev@tx.technion.ac.i [Department of Electrical Engineering, Helmut Schmidt University, 22043 Hamburg (Germany)

    2010-05-15

    The ubiquitous Hofstadter butterfly describes a variety of systems characterized by incommensurable periodicities, ranging from Bloch electrons in magnetic fields and the quantum Hall effect to cold atoms in optical lattices and more. Here, we introduce nonlinearity into the underlying (Harper) model and study the nonlinear spectra and the corresponding extended eigenmodes of nonlinear quasiperiodic systems. We show that the spectra of the nonlinear eigenmodes form deformed versions of the Hofstadter butterfly and demonstrate that the modes can be classified into two families: nonlinear modes that are a 'continuation' of the linear modes of the system and new nonlinear modes that have no counterparts in the linear spectrum. Finally, we propose an optical realization of the linear and nonlinear Harper models in transversely modulated waveguide arrays, where these Hofstadter butterflies can be observed. This work is relevant to a variety of other branches of physics beyond optics, such as disorder-induced localization in ultracold bosonic gases, localization transition processes in disordered lattices, and more.

  12. Nonlinear optics with coherent free electron lasers

    Science.gov (United States)

    Bencivenga, F.; Capotondi, F.; Mincigrucci, R.; Cucini, R.; Manfredda, M.; Pedersoli, E.; Principi, E.; Simoncig, A.; Masciovecchio, C.

    2016-12-01

    We interpreted the recent construction of free electron laser (FELs) facilities worldwide as an unprecedented opportunity to bring concepts and methods from the scientific community working with optical lasers into the domain of x-ray science. This motivated our efforts towards the realization of FEL-based wave-mixing applications. In this article we present new extreme ultraviolet transient grating (X-TG) data from vitreous SiO2, collected using two crossed FEL pulses (photon frequency 38 eV) to generate the X-TG and a phase matched optical probing pulse (photon frequency 3.1 eV). This experiment extends our previous investigation, which was carried out on a nominally identical sample using a different FEL photon frequency (45 eV) to excite the X-TG. The present data are featured by a peak intensity of the X-TG signal substantially larger than that previously reported and by slower modulations of the X-TG signal at positive delays. These differences could be ascribed to the different FEL photon energy used in the two experiments or to differences in the sample properties. A systematic X-TG study on the same sample as a function of the FEL wavelength is needed to draw a consistent conclusion. We also discuss how the advances in the performance of the FELs, in terms of generation of fully coherent photon pulses and multi-color FEL emission, may push the development of original experimental strategies to study matter at the femtosecond-nanometer time-length scales, with the unique option of element and chemical state specificity. This would allow the development of advanced experimental tools based on wave-mixing processes, which may have a tremendous impact in the study of a large array of phenomena, ranging from nano-dynamics in complex materials to charge and energy transfer processes.

  13. Symbolic-computation study of the perturbed nonlinear Schrodinger model in inhomogeneous optical fibers

    International Nuclear Information System (INIS)

    Tian Bo; Gao Yitian

    2005-01-01

    A realistic, inhomogeneous fiber in the optical communication systems can be described by the perturbed nonlinear Schrodinger model (also named as the normalized nonlinear Schrodinger model with periodically varying coefficients, dispersion managed nonlinear Schrodinger model or nonlinear Schrodinger model with variable coefficients). Hereby, we extend to this model a direct method, perform symbolic computation and obtain two families of the exact, analytic bright-solitonic solutions, with or without the chirp respectively. The parameters addressed include the shape of the bright soliton, soliton amplitude, inverse width of the soliton, chirp, frequency, center of the soliton and center of the phase of the soliton. Of optical and physical interests, we discuss some previously-published special cases of our solutions. Those solutions could help the future studies on the optical communication systems. ms

  14. Natural Silk as a Photonics Component: a Study on Its Light Guiding and Nonlinear Optical Properties

    OpenAIRE

    Kujala, Sami; Mannila, Anna; Karvonen, Lasse; Kieu, Khanh; Sun, Zhipei

    2016-01-01

    Silk fibers are expected to become a pathway to biocompatible and bioresorbable waveguides, which could be used to deliver localized optical power for various applications, e.g., optical therapy or imaging inside living tissue. Here, for the first time, the linear and nonlinear optical properties of natural silk fibers have been studied. The waveguiding properties of silk fibroin of largely unprocessed Bombyx mori silkworm silk are assessed using two complementary methods, and found to be on ...

  15. A nonlinear plasmonic waveguide based all-optical bidirectional switching

    Science.gov (United States)

    Bana, Xiaoqiang; Pang, Xingxing; Li, Xiaohui; Hu, Bin; Guo, Yixuan; Zheng, Hairong

    2018-01-01

    In this paper, an all-optical switching with a nanometer coupled ring resonator is demonstrated based on the nonlinear material. By adjusting the light intensity, we implement the resonance wavelength from 880 nm to 940 nm in the nonlinear material structure monocyclic. In the bidirectional switch structure, the center wavelength (i.e. 880 nm) is fixed. By changing the light intensity from I = 0 to I = 53 . 1 MW /cm2, the function of optical switching can be obtained. The results demonstrate that both the single-ring cavity and the T-shaped double-ring structure can realize the optical switching effect. This work takes advantage of the simple structure. The single-ring cavity plasmonic switches have many advantages, such as nanoscale size, low pumping light intensity, ultrafast response time (femtosecond level), etc. It is expected that the proposed all-optical integrated devices can be potentially applied in optical communication, signal processing, and signal sensing, etc.

  16. FDTD modeling of anisotropic nonlinear optical phenomena in silicon waveguides.

    Science.gov (United States)

    Dissanayake, Chethiya M; Premaratne, Malin; Rukhlenko, Ivan D; Agrawal, Govind P

    2010-09-27

    A deep insight into the inherent anisotropic optical properties of silicon is required to improve the performance of silicon-waveguide-based photonic devices. It may also lead to novel device concepts and substantially extend the capabilities of silicon photonics in the future. In this paper, for the first time to the best of our knowledge, we present a three-dimensional finite-difference time-domain (FDTD) method for modeling optical phenomena in silicon waveguides, which takes into account fully the anisotropy of the third-order electronic and Raman susceptibilities. We show that, under certain realistic conditions that prevent generation of the longitudinal optical field inside the waveguide, this model is considerably simplified and can be represented by a computationally efficient algorithm, suitable for numerical analysis of complex polarization effects. To demonstrate the versatility of our model, we study polarization dependence for several nonlinear effects, including self-phase modulation, cross-phase modulation, and stimulated Raman scattering. Our FDTD model provides a basis for a full-blown numerical simulator that is restricted neither by the single-mode assumption nor by the slowly varying envelope approximation.

  17. Nonlinear optical studies of single gold nanoparticles

    NARCIS (Netherlands)

    Dijk, Meindert Alexander van

    2007-01-01

    Gold nanoparticles are spherical clusters of gold atoms, with diameters typically between 1 and 100 nanometers. The applications of these particles are rather diverse, from optical labels for biological experiments to data carrier for optical data storage. The goal of my project was to develop new

  18. Method for conducting nonlinear electrochemical impedance spectroscopy

    Science.gov (United States)

    Adler, Stuart B.; Wilson, Jamie R.; Huff, Shawn L.; Schwartz, Daniel T.

    2015-06-02

    A method for conducting nonlinear electrochemical impedance spectroscopy. The method includes quantifying the nonlinear response of an electrochemical system by measuring higher-order current or voltage harmonics generated by moderate-amplitude sinusoidal current or voltage perturbations. The method involves acquisition of the response signal followed by time apodization and fast Fourier transformation of the data into the frequency domain, where the magnitude and phase of each harmonic signal can be readily quantified. The method can be implemented on a computer as a software program.

  19. Advances in iterative methods for nonlinear equations

    CERN Document Server

    Busquier, Sonia

    2016-01-01

    This book focuses on the approximation of nonlinear equations using iterative methods. Nine contributions are presented on the construction and analysis of these methods, the coverage encompassing convergence, efficiency, robustness, dynamics, and applications. Many problems are stated in the form of nonlinear equations, using mathematical modeling. In particular, a wide range of problems in Applied Mathematics and in Engineering can be solved by finding the solutions to these equations. The book reveals the importance of studying convergence aspects in iterative methods and shows that selection of the most efficient and robust iterative method for a given problem is crucial to guaranteeing a good approximation. A number of sample criteria for selecting the optimal method are presented, including those regarding the order of convergence, the computational cost, and the stability, including the dynamics. This book will appeal to researchers whose field of interest is related to nonlinear problems and equations...

  20. Evaluation of third order nonlinear optical parameters of CdS/PVA nanocomposite

    Energy Technology Data Exchange (ETDEWEB)

    Sharma, Mamta [Department of Physics, Center of Advanced Study in Physics, Panjab University, Chandigarh-160014 (India); Department of Applied Sciences (Physics), UIET, Panjab University, Chandigarh-160014 (India); Tripathi, S. K., E-mail: surya@pu.ac.in, E-mail: surya-tr@yahoo.com [Department of Physics, Center of Advanced Study in Physics, Panjab University, Chandigarh-160014 (India)

    2015-06-24

    CdS nanoparticles dispersed in PVA are prepared by Chemical method at room temperature. The nonlinear optical parameters such as nonlinear absorption (β), nonlinear refractive index (n{sub 2}) and nonlinear susceptibility (χ{sup 3}) are calculated for this sample by using Z-scan technique. CdS/PVA samples show the two photon absorption mechanism. The third order nonlinear susceptibility is calculated from n{sub 2} and β and is found to be of the order of 10{sup −7} – 10{sup −8} m{sup 2}/V{sup 2}. The larger value of third order nonlinear susceptibility is due to dielectric and quantum confinement effect.

  1. Unidirectional transmission in 1D nonlinear photonic crystal based on topological phase reversal by optical nonlinearity

    Directory of Open Access Journals (Sweden)

    Chong Li

    2017-02-01

    Full Text Available We propose a scheme of unidirectional transmission in a 1D nonlinear topological photonic crystal based on the topological edge state and three order optical nonlinearity. The 1D photonic crystals consists of a nonlinear photonic crystal L and a linear photonic crystal R. In the backward direction, light is totally reflected for the photons transmission prohibited by the bandgap. While in the forward direction, light interacts with the nonlinear photonic crystal L by optical Kerr effect, bringing a topological phase reversal and results the topological edge mode arising at the interface which could transmit photons through the bandgaps both of the photonic crystal L and R. When the signal power intensity larger than a moderate low threshold value of 10.0 MW/cm2, the transmission contrast ratio could remain at 30 steadily.

  2. Optical soliton solutions for two coupled nonlinear Schroedinger systems via Darboux transformation

    International Nuclear Information System (INIS)

    Zhang Haiqiang; Li Juan; Xu Tao; Zhang Yaxing; Hu Wei; Tian Bo

    2007-01-01

    In nonlinear optical fibers, the vector solitons can be governed by the systems of coupled nonlinear Schroedinger from polarized optical waves in an isotropic medium. Based on the Ablowitz-Kaup-Newell-Segur technology, the Darboux transformation method is successfully applied to two coupled nonlinear Schroedinger systems. With the help of symbolic computation, the bright vector one- and two-soliton solutions including one-peak and two-peak solitons are further constructed via the iterative algorithm of Darboux transformation. Through the figures for several sample solutions, the stable propagation and elastic collisions for these kinds of bright vector solitons are discussed and the possible applications are pointed out in optical communications and relevant optical experiments.In addition, the conserved quantities of such two systems, i.e., the energy, momentum and Hamiltonian, are also presented

  3. Label-free and selective nonlinear fiber-optical biosensing

    DEFF Research Database (Denmark)

    Ott, Johan Raunkjær; Heuck, Mikkel; Agger, Christian

    2008-01-01

    We demonstrate that the inherent nonlinearity of a microstructured optical fiber (MOF) may be used to achieve label-free selective biosensing, thereby eliminating the need for post-processing of the fiber. This first nonlinear biosensor utilizes a change in the modulational instability (MI) gain...... for optimizing the sensitivity. The nonlinear sensor shows a sensitivity of around 10.4nm/nm, defined as the shift in resonance wavelength per nm biolayer, which is a factor of 7.5 higher than the hitherto only demonstrated label-free MOF biosensor....

  4. Nonlinear optical microscopy for histology of fresh normal and cancerous pancreatic tissues.

    Directory of Open Access Journals (Sweden)

    Wenyan Hu

    Full Text Available BACKGROUND: Pancreatic cancer is a lethal disease with a 5-year survival rate of only 1-5%. The acceleration of intraoperative histological examination would be beneficial for better management of pancreatic cancer, suggesting an improved survival. Nonlinear optical methods based on two-photon excited fluorescence (TPEF and second harmonic generation (SHG of intrinsic optical biomarkers show the ability to visualize the morphology of fresh tissues associated with histology, which is promising for real-time intraoperative evaluation of pancreatic cancer. METHODOLOGY/PRINCIPAL FINDINGS: In order to investigate whether the nonlinear optical imaging methods have the ability to characterize pancreatic histology at cellular resolution, we studied different types of pancreatic tissues by using label-free TPEF and SHG. Compared with other routine methods for the preparation of specimens, fresh tissues without processing were found to be most suitable for nonlinear optical imaging of pancreatic tissues. The detailed morphology of the normal rat pancreas was observed and related with the standard histological images. Comparatively speaking, the preliminary images of a small number of chemical-induced pancreatic cancer tissues showed visible neoplastic differences in the morphology of cells and extracellular matrix. The subcutaneous pancreatic tumor xenografts were further observed using the nonlinear optical microscopy, showing that most cells are leucocytes at 5 days after implantation, the tumor cells begin to proliferate at 10 days after implantation, and the extracellular collagen fibers become disordered as the xenografts grow. CONCLUSIONS/SIGNIFICANCE: In this study, nonlinear optical imaging was used to characterize the morphological details of fresh pancreatic tissues for the first time. We demonstrate that it is possible to provide real-time histological evaluation of pancreatic cancer by the nonlinear optical methods, which present an

  5. Entropy viscosity method for nonlinear conservation laws

    KAUST Repository

    Guermond, Jean-Luc

    2011-05-01

    A new class of high-order numerical methods for approximating nonlinear conservation laws is described (entropy viscosity method). The novelty is that a nonlinear viscosity based on the local size of an entropy production is added to the numerical discretization at hand. This new approach does not use any flux or slope limiters, applies to equations or systems supplemented with one or more entropy inequalities and does not depend on the mesh type and polynomial approximation. Various benchmark problems are solved with finite elements, spectral elements and Fourier series to illustrate the capability of the proposed method. © 2010 Elsevier Inc.

  6. Entropy viscosity method for nonlinear conservation laws

    KAUST Repository

    Guermond, Jean-Luc; Pasquetti, Richard; Popov, Bojan

    2011-01-01

    A new class of high-order numerical methods for approximating nonlinear conservation laws is described (entropy viscosity method). The novelty is that a nonlinear viscosity based on the local size of an entropy production is added to the numerical discretization at hand. This new approach does not use any flux or slope limiters, applies to equations or systems supplemented with one or more entropy inequalities and does not depend on the mesh type and polynomial approximation. Various benchmark problems are solved with finite elements, spectral elements and Fourier series to illustrate the capability of the proposed method. © 2010 Elsevier Inc.

  7. Picosecond optical nonlinearities in symmetrical and unsymmetrical ...

    Indian Academy of Sciences (India)

    It is evident that the saturable absorption (SA) behaviour changed to reverse sat- urable absorption (RSA) and the nonlinear coefficients were obtained using the equation α = α0I/[1 + (I/Is)]. The open-aperture scans were fitted by solving the propagation equation for homogeneous medium dI/dz = {−α0I/[1+(I/Is)]}−βI2.

  8. Optical computation based on nonlinear total reflectional optical ...

    Indian Academy of Sciences (India)

    Optical computing; beam splitter; optical switch; polarized beams. ... main research direction called quantum information and quantum computation is .... above has several advantages: Firstly, it is easy to be integrated with appropriate.

  9. Third-order nonlinear optical properties of ADP crystal

    Science.gov (United States)

    Wang, Mengxia; Wang, Zhengping; Chai, Xiangxu; Sun, Yuxiang; Sui, Tingting; Sun, Xun; Xu, Xinguang

    2018-05-01

    By using the Z-scan method, we investigated the third-order nonlinear optical (NLO) properties of ADP crystal at different wavelengths (355, 532, and 1064 nm) and different orientations ([001], [100], [110], I and II). The experimental data were fitted by NLO theory, to give out the two photon absorption (TPA) coefficient β 2 and the nonlinear refractive index n 2. When the light source changed from a 40 ps, 1064 nm fundamental laser to a 30 ps, 355 nm third-harmonic-generation (THG) laser, the β 2 value increased about 5 times (0.2 × 10‑2 → 1 × 10‑2 cm GW‑1), and the n 2 value increased about 1.5 times (1.5 × 10‑16 → 2.2 × 10‑16 cm2 W‑1). Among all of the orientations, the [110] sample exhibits the smallest β 2, and the second smallest n 2. It indicates that this orientation and its surroundings will be the preferred directions for high-power laser applications of ADP crystal.

  10. Numerical simulation methods for wave propagation through optical waveguides

    International Nuclear Information System (INIS)

    Sharma, A.

    1993-01-01

    The simulation of the field propagation through waveguides requires numerical solutions of the Helmholtz equation. For this purpose a method based on the principle of orthogonal collocation was recently developed. The method is also applicable to nonlinear pulse propagation through optical fibers. Some of the salient features of this method and its application to both linear and nonlinear wave propagation through optical waveguides are discussed in this report. 51 refs, 8 figs, 2 tabs

  11. Nonlinear light-matter interactions in engineered optical media

    Science.gov (United States)

    Litchinitser, Natalia

    In this talk, we consider fundamental optical phenomena at the interface of nonlinear and singular optics in artificial media, including theoretical and experimental studies of linear and nonlinear light-matter interactions of vector and singular optical beams in metamaterials. We show that unique optical properties of metamaterials open unlimited prospects to ``engineer'' light itself. Thanks to their ability to manipulate both electric and magnetic field components, metamaterials open new degrees of freedom for tailoring complex polarization states and orbital angular momentum (OAM) of light. We will discuss several approaches to structured light manipulation on the nanoscale using metal-dielectric, all-dielectric and hyperbolic metamaterials. These new functionalities, including polarization and OAM conversion, beam magnification and de-magnification, and sub-wavelength imaging using novel non-resonant hyperlens are likely to enable a new generation of on-chip or all-fiber structured light applications. The emergence of metamaterials also has a strong potential to enable a plethora of novel nonlinear light-matter interactions and even new nonlinear materials. In particular, nonlinear focusing and defocusing effects are of paramount importance for manipulation of the minimum focusing spot size of structured light beams necessary for nanoscale trapping, manipulation, and fundamental spectroscopic studies. Colloidal suspensions offer as a promising platform for engineering polarizibilities and realization of large and tunable nonlinearities. We will present our recent studies of the phenomenon of spatial modulational instability leading to laser beam filamentation in an engineered soft-matter nonlinear medium. Finally, we introduce so-called virtual hyperbolic metamaterials formed by an array of plasma channels in air as a result of self-focusing of an intense laser pulse, and show that such structure can be used to manipulate microwave beams in a free space. This

  12. Transverse effects in nonlinear optics: Toward the photon superfluid

    Science.gov (United States)

    McCormick, Colin Fraser

    Nonlinear optics displays a wealth of transverse effects. These effects are particularly rich in the presence of an optical cavity. Many considerations suggest that in a Kerr nonlinear cavity a new state of light known as a "photon superfluid" can form, with strong analogies to atomic superfluids. The conditions for the formation of the photon superfluid include requirements on the cavity, input light fields and the nonlinear medium as well as various timescales. The most favorable candidate nonlinear medium for observing the photon super-fluid is an atomic vapor. With a strong and fast Kerr effect, atomic vapors also have the advantage of a Kerr coefficient that is tunable in both magnitude and sign. A series of z-scan experiments in far-detuned atomic rubidium vapor is reported, measuring the Kerr coefficient and determining its functional dependence on detuning to be that of a Doppler-broadened two-level model with adiabatic following of the electric field by the atom pseudomoment. Saturation effects are found to be important. Z-scan measurements for detunings within the Doppler profile are shown to agree well with numerical simulations based on the Doppler-broadened model. Agreement between absorptive and refractive non-linear coefficients is evidence of the Kramers-Kronig relations at work, even in this nonlinear system. The formation of the photon superfluid is discussed and the calculation of a new process, nearly collinear four-wave mixing, is presented. This process is essentially an inverse beam filamentation that is likely to be the underlying physical mechanism for transverse cooling and condensation of photons in a nonlinear optical cavity. Nearly collinear four-wave mixing may also be related to phenomena in general nonlinear physics, including modulation instability and Fermi-Pasta-Ulam recurrence.

  13. Mapping the nonlinear optical susceptibility by noncollinear second-harmonic generation.

    Science.gov (United States)

    Larciprete, M C; Bovino, F A; Giardina, M; Belardini, A; Centini, M; Sibilia, C; Bertolotti, M; Passaseo, A; Tasco, V

    2009-07-15

    We present a method, based on noncollinear second-harmonic generation, to evaluate the nonzero elements of the nonlinear optical susceptibility. At a fixed incidence angle, the generated signal is investigated by varying the polarization state of both fundamental beams. The resulting polarization charts allows us to verify if Kleinman's symmetry rules can be applied to a given material or to retrieve the absolute value of the nonlinear optical tensor terms, from a reference measurement. Experimental measurements obtained from gallium nitride layers are reported. The proposed method does not require an angular scan and thus is useful when the generated signal is strongly affected by sample rotation.

  14. Twistacene contained molecule for optical nonlinearity: Excited-state based negative refraction and optical limiting

    Science.gov (United States)

    Wu, Xingzhi; Xiao, Jinchong; Sun, Ru; Jia, Jidong; Yang, Junyi; Ao, Guanghong; Shi, Guang; Wang, Yuxiao; Zhang, Xueru; Song, Yinglin

    2018-06-01

    Spindle-type molecules containing twisted acenes (PyBTA-1 &PyBTA-2) are designed, synthesized characterized. Picosecond Z-scan experiments under 532 nm show reverse saturable absorption and negative nonlinear refraction, indicating large third-order optical nonlinearity in PyBTA-1. The mechanism of the optical nonlinearity is investigated and the results show that the nonlinear absorption and refraction in PyBTA-1 originates from a charge transfer (CT) state. Furthermore, relatively long lifetime and absorptive cross section of the CT state are measured. Based on the excited state absorption in PyBTA-1, strong optical limiting with ∼0.3 J/cm2 thresholds are obtained when excited by picoseconds and nanoseconds pulses. The findings on nonlinear optics suggest PyBTA-1 a promising material of all optical modulation and laser protection, which enrich the potential applications of these spindle-type molecules. Comparing to the previously reported spindle-type molecules with analogous structures, the introduction of ICT in PyBTA-1 &PyBTA-2 dramatically decreases the two-photon absorption while enhances the nonlinear refraction. The results could be used to selectively tailor the optical nonlinearity in such kind of compounds.

  15. All-optical image processing with nonlinear liquid crystals

    Science.gov (United States)

    Hong, Kuan-Lun

    Liquid crystals are fascinating materials because of several advantages such as large optical birefringence, dielectric anisotropic, and easily compatible to most kinds of materials. Compared to the electro-optical properties of liquid crystals widely applied in displays and switching application, transparency through most parts of wavelengths also makes liquid crystals a better candidate for all-optical processing. The fast response time of liquid crystals resulting from multiple nonlinear effects, such as thermal and density effect can even make real-time processing realized. In addition, blue phase liquid crystals with spontaneously self-assembled three dimensional cubic structures attracted academic attention. In my dissertation, I will divide the whole contents into six parts. In Chapter 1, a brief introduction of liquid crystals is presented, including the current progress and the classification of liquid crystals. Anisotropy and laser induced director axis reorientation is presented in Chapter 2. In Chapter 3, I will solve the electrostrictive coupled equation and analyze the laser induced thermal and density effect in both static and dynamic ways. Furthermore, a dynamic simulation of laser induced density fluctuation is proposed by applying finite element method. In Chapter 4, two image processing setups are presented. One is the intensity inversion experiment in which intensity dependent phase modulation is the mechanism. The other is the wavelength conversion experiment in which I can read the invisible image with a visible probe beam. Both experiments are accompanied with simulations to realize the matching between the theories and practical experiment results. In Chapter 5, optical properties of blue phase liquid crystals will be introduced and discussed. The results of grating diffractions and thermal refractive index gradient are presented in this chapter. In addition, fiber arrays imaging and switching with BPLCs will be included in this chapter

  16. Nonlinear Fourier transform for dual-polarization optical communication system

    OpenAIRE

    Gaiarin, Simone

    2018-01-01

    New services and applications are causing an exponential increase in the internet traffic. In a few years, the current fiber-optic communication system infrastructure will not be able to meet this demand because fiber nonlinearity dramatically limits the information transmission rate. Eigenvalue communication is considered an emerging paradigm in fiber-optic communications that could potentially overcome these limitations. It relies on a mathematical technique called “inverse scattering trans...

  17. Optical Beams in Nonlocal Nonlinear Media

    DEFF Research Database (Denmark)

    Królikowski, W.; Bang, Ole; Wyller, J.

    2003-01-01

    We discuss propagation of optical beams in nonlocal Kerr-like media with the nonlocality of general form. We study the effect of nonlocality on modulational instability of the plane wave fronts, collapse of finite beams and formation of spatial solitons....

  18. Rapid assessment of nonlinear optical propagation effects in dielectrics

    Science.gov (United States)

    Hoyo, J. Del; de La Cruz, A. Ruiz; Grace, E.; Ferrer, A.; Siegel, J.; Pasquazi, A.; Assanto, G.; Solis, J.

    2015-01-01

    Ultrafast laser processing applications need fast approaches to assess the nonlinear propagation of the laser beam in order to predict the optimal range of processing parameters in a wide variety of cases. We develop here a method based on the simple monitoring of the nonlinear beam shaping against numerical prediction. The numerical code solves the nonlinear Schrödinger equation with nonlinear absorption under simplified conditions by employing a state-of-the art computationally efficient approach. By comparing with experimental results we can rapidly estimate the nonlinear refractive index and nonlinear absorption coefficients of the material. The validity of this approach has been tested in a variety of experiments where nonlinearities play a key role, like spatial soliton shaping or fs-laser waveguide writing. The approach provides excellent results for propagated power densities for which free carrier generation effects can be neglected. Above such a threshold, the peculiarities of the nonlinear propagation of elliptical beams enable acquiring an instantaneous picture of the deposition of energy inside the material realistic enough to estimate the effective nonlinear refractive index and nonlinear absorption coefficients that can be used for predicting the spatial distribution of energy deposition inside the material and controlling the beam in the writing process.

  19. Nonlinear optical studies in semiconductor-doped glasses under ...

    Indian Academy of Sciences (India)

    Abstract. Nonlinear optical studies in semiconductor-doped glasses (SDGs) are per- formed under femtosecond laser pulse excitation. Z-scan experiments with 800 nm wave- length pulses are used to excite SDG samples in the resonance and non-resonance regimes. Schott colour glass filter OG 515 shows stronger ...

  20. Nonlinear Optics Approaches Towards Subdiffraction Resolution in CARS Imaging

    NARCIS (Netherlands)

    Boller, Klaus J.; Beeker, W.P.; Cleff, C.; Kruse, K.; Lee, Christopher James; Gross, P.; Offerhaus, Herman L.; Fallnich, Carsten; Herek, Jennifer Lynn; Fornasiero, E.F.; Rizzoli, S.O.

    2014-01-01

    In theoretical investigations, we review several nonlinear optical approaches towards subdiffraction-limited resolution in label-free imaging via coherent anti-Stokes Raman scattering (CARS). Using a density matrix model and numerical integration, we investigate various level schemes and

  1. Enhancement of nonlinear optical properties of compounds of silica ...

    Indian Academy of Sciences (India)

    Enhancement of nonlinear optical properties of compounds of silica glass and metallic nanoparticle. A GHARAATI1,∗ and A KAMALDAR1,2. 1Department of Physics, Payame Noor University, P.O. Box 19395-3697, Tehran, Iran. 2Department of Education 1, Shiraz, Iran. ∗. Corresponding author. E-mail: agharaati@pnu.ac.

  2. Printed organic smart devices characterized by nonlinear optical

    DEFF Research Database (Denmark)

    Pastorelli, Francesco; Accanto, Nicolo; Jørgensen, Mikkel

    2017-01-01

    In this study, we demonstrate that nonlinear optical microscopy is a promising technique to characterize organic printed electronics. Using ultrashort laser pulses we stimulate two-photon absorption in a roll coated polymer semiconductor and map the resulting two-photon induced photoluminescence...

  3. Optical activity via Kerr nonlinearity in a spinning chiral medium

    Energy Technology Data Exchange (ETDEWEB)

    Khan, Anwar Ali, E-mail: anwarali@uom.edu.pk [Department of Physics, University of Malakand at Chakdara Dir(L) (Pakistan); Bacha, Bakht Amin, E-mail: aminoptics@gmail.com [Department of Physics, University of Malakand at Chakdara Dir(L) (Pakistan); Khan, Rahmat Ali, E-mail: rahmat_alipk@yahoo.com [Department of Mathematics, University of Malakand (Pakistan)

    2016-11-11

    Optical activity is investigated in a chiral medium by employing the four level cascade atomic model, in which the optical responses of the atomic medium are studied with Kerr nonlinearity. Light entering into a chiral medium splits into circular birefringent beams. The angle of divergence between the circular birefringent beams and the polarization states of the two light beams is manipulated with Kerr nonlinearity. In the stationary chiral medium the angle of divergence between the circular birefringent beams is calculated to be 1.3 radian. Furthermore, circular birefringence is optically controlled in a spinning chiral medium, where the maximum rotary photon drag angle for left (right) circularly polarized beam is ±1.1 (±1.5) microradian. The change in the angle of divergence between circular birefringent beams by rotary photon drag is calculated to be 0.4 microradian. The numerical results may help to understand image designing, image coding, discovery of photonic crystals and optical sensing technology. - Highlights: • Coherent control of a circular birefringence in a chiral medium is studied. • Angle of divergence between birefringent beams is modified with Kerr nonlinearity. • Rotary photon drag is controlled for birefringent beams and enhanced with Kerr nonlinearity in a spinning medium. • Rotation of the angle of divergence is observed with mechanical rotation of the medium about an axis and modified with Kerr effect. • A change in the angle of divergence is calculated by about a microradian with rotary photon drag.

  4. Extra phase noise from thermal fluctuations in nonlinear optical crystals

    DEFF Research Database (Denmark)

    César, J. E. S.; Coelho, A.S.; Cassemiro, K.N.

    2009-01-01

    We show theoretically and experimentally that scattered light by thermal phonons inside a second-order nonlinear crystal is the source of additional phase noise observed in optical parametric oscillators. This additional phase noise reduces the quantum correlations and has hitherto hindered the d...

  5. Generalized dispersive wave emission in nonlinear fiber optics.

    Science.gov (United States)

    Webb, K E; Xu, Y Q; Erkintalo, M; Murdoch, S G

    2013-01-15

    We show that the emission of dispersive waves in nonlinear fiber optics is not limited to soliton-like pulses propagating in the anomalous dispersion regime. We demonstrate, both numerically and experimentally, that pulses propagating in the normal dispersion regime can excite resonant dispersive radiation across the zero-dispersion wavelength into the anomalous regime.

  6. Linear and nonlinear optical spectroscopy: Spectral, temporal and spatial resolution

    DEFF Research Database (Denmark)

    Hvam, Jørn Marcher

    1997-01-01

    Selected linear and nonlinear optical spectroscopies are being described with special emphasis on the possibility of obtaining simultaneous spectral, temporal and spatial resolution. The potential of various experimental techniques is being demonstrated by specific examples mostly taken from inve...... investigations of the electronic, and opto-electronic, properties of semiconductor nanostructures....

  7. Applied nonlinear optics in the journal 'Quantum Electronics'

    International Nuclear Information System (INIS)

    Grechin, Sergei G; Dmitriev, Valentin G; Chirkin, Anatolii S

    2011-01-01

    A brief historical review of the experimental and theoretical works on nonlinear optical frequency conversion (generation of harmonics, up- and down-conversion, parametric oscillation), which have been published in the journal 'Quantum Electronics' for the last 40 years, is presented.

  8. Instrumentation for Linear and Nonlinear Optical Device Characterization

    Science.gov (United States)

    2018-01-31

    distribution is Unlimited 13. SUPPLEMENTARY NOTES 14. ABSTRACT The Pl has acquired six pieces of equipment to extend capabilities for linear and nonlinear...optical spectral analysis • Frequency comb generation in mid-infrared Accomplishments Six major pieces of equipment have been ordered and received

  9. Linear and nonlinear optical properties of Sb-doped GeSe2 thin films

    Science.gov (United States)

    Zhang, Zhen-Ying; Chen, Fen; Lu, Shun-Bin; Wang, Yong-Hui; Shen, Xiang; Dai, Shi-Xun; Nie, Qiu-Hua

    2015-06-01

    Sb-doped GeSe2 chalcogenide thin films are prepared by the magnetron co-sputtering method. The linear optical properties of as-deposited films are derived by analyzing transmission spectra. The refractive index rises and the optical band gap decreases from 2.08 eV to 1.41 eV with increasing the Sb content. X-ray photoelectron spectra further confirm the formation of a covalent Sb-Se bond. The third-order nonlinear optical properties of thin films are investigated under femtosecond laser excitation at 800 nm. The results show that the third-order nonlinear optical properties are enhanced with increasing the concentration of Sb. The nonlinear refraction indices of these thin films are measured to be on the order of 10-18 m2/W with a positive sign and the nonlinear absorption coefficients are obtained to be on the order of 10-10 m/W. These excellent properties indicate that Sb-doped Ge-Se films have a good prospect in the applications of nonlinear optical devices. Project supported by the National Key Basic Research Program of China (Grant No. 2012CB722703), the National Natural Science Foundation of China (Grant No. 61377061), the Young Leaders of Academic Climbing Project of the Education Department of Zhejiang Province, China (Grant No. pd2013092), the Program for Innovative Research Team of Ningbo City, China (Grant No. 2009B217), and the K. C. Wong Magna Fund in Ningbo University, China.

  10. Tangled nonlinear driven chain reactions of all optical singularities

    Science.gov (United States)

    Vasil'ev, V. I.; Soskin, M. S.

    2012-03-01

    Dynamics of polarization optical singularities chain reactions in generic elliptically polarized speckle fields created in photorefractive crystal LiNbO3 was investigated in details Induced speckle field develops in the tens of minutes scale due to photorefractive 'optical damage effect' induced by incident beam of He-Ne laser. It was shown that polarization singularities develop through topological chain reactions of developing speckle fields driven by photorefractive nonlinearities induced by incident laser beam. All optical singularities (C points, optical vortices, optical diabolos,) are defined by instantaneous topological structure of the output wavefront and are tangled by singular optics lows. Therefore, they have develop in tangled way by six topological chain reactions driven by nonlinear processes in used nonlinear medium (photorefractive LiNbO3:Fe in our case): C-points and optical diabolos for right (left) polarized components domains with orthogonally left (right) polarized optical vortices underlying them. All elements of chain reactions consist from loop and chain links when nucleated singularities annihilated directly or with alien singularities in 1:9 ratio. The topological reason of statistics was established by low probability of far enough separation of born singularities pair from existing neighbor singularities during loop trajectories. Topology of developing speckle field was measured and analyzed by dynamic stokes polarimetry with few seconds' resolution. The hierarchy of singularities govern scenario of tangled chain reactions was defined. The useful space-time data about peculiarities of optical damage evolution were obtained from existence and parameters of 'islands of stability' in developing speckle fields.

  11. Progress in linear optics, non-linear optics and surface alignment of liquid crystals

    Science.gov (United States)

    Ong, H. L.; Meyer, R. B.; Hurd, A. J.; Karn, A. J.; Arakelian, S. M.; Shen, Y. R.; Sanda, P. N.; Dove, D. B.; Jansen, S. A.; Hoffmann, R.

    We first discuss the progress in linear optics, in particular, the formulation and application of geometrical-optics approximation and its generalization. We then discuss the progress in non-linear optics, in particular, the enhancement of a first-order Freedericksz transition and intrinsic optical bistability in homeotropic and parallel oriented nematic liquid crystal cells. Finally, we discuss the liquid crystal alignment and surface effects on field-induced Freedericksz transition.

  12. Slow light enhanced optical nonlinearity in a silicon photonic crystal coupled-resonator optical waveguide.

    Science.gov (United States)

    Matsuda, Nobuyuki; Kato, Takumi; Harada, Ken-Ichi; Takesue, Hiroki; Kuramochi, Eiichi; Taniyama, Hideaki; Notomi, Masaya

    2011-10-10

    We demonstrate highly enhanced optical nonlinearity in a coupled-resonator optical waveguide (CROW) in a four-wave mixing experiment. Using a CROW consisting of 200 coupled resonators based on width-modulated photonic crystal nanocavities in a line defect, we obtained an effective nonlinear constant exceeding 10,000 /W/m, thanks to slow light propagation combined with a strong spatial confinement of light achieved by the wavelength-sized cavities.

  13. Exploring lipids with nonlinear optical microscopy in multiple biological systems

    Science.gov (United States)

    Alfonso-Garcia, Alba

    Lipids are crucial biomolecules for the well being of humans. Altered lipid metabolism may give rise to a variety of diseases that affect organs from the cardiovascular to the central nervous system. A deeper understanding of lipid metabolic processes would spur medical research towards developing precise diagnostic tools, treatment methods, and preventive strategies for reducing the impact of lipid diseases. Lipid visualization remains a complex task because of the perturbative effect exerted by traditional biochemical assays and most fluorescence markers. Coherent Raman scattering (CRS) microscopy enables interrogation of biological samples with minimum disturbance, and is particularly well suited for label-free visualization of lipids, providing chemical specificity without compromising on spatial resolution. Hyperspectral imaging yields large datasets that benefit from tailored multivariate analysis. In this thesis, CRS microscopy was combined with Raman spectroscopy and other label-free nonlinear optical techniques to analyze lipid metabolism in multiple biological systems. We used nonlinear Raman techniques to characterize Meibum secretions in the progression of dry eye disease, where the lipid and protein contributions change in ratio and phase segregation. We employed similar tools to examine lipid droplets in mice livers aboard a spaceflight mission, which lose their retinol content contributing to the onset of nonalcoholic fatty-liver disease. We also focused on atherosclerosis, a disease that revolves around lipid-rich plaques in arterial walls. We examined the lipid content of macrophages, whose variable phenotype gives rise to contrasting healing and inflammatory activities. We also proposed new label-free markers, based on lifetime imaging, for macrophage phenotype, and to detect products of lipid oxidation. Cholesterol was also detected in hepatitis C virus infected cells, and in specific strains of age-related macular degeneration diseased cells by

  14. Materials for Nonlinear Optics Chemical Perspectives

    Science.gov (United States)

    1991-01-01

    potassium iodide for 15 h at reflux. The benzaldehyde product was then allowed to react with diethyl(4-nitrobenzyl)phosphonate in the presence of ...photocrosslinking of NLO-inactive polyacrylate monomers. Recent advances in optical technology have created great interest in the construction of second-order...might be potassium niobate.) Because of this, the value of finding an "improved" material can be accurately gauged in a relative sense, and compared to

  15. Automated seeding-based nuclei segmentation in nonlinear optical microscopy.

    Science.gov (United States)

    Medyukhina, Anna; Meyer, Tobias; Heuke, Sandro; Vogler, Nadine; Dietzek, Benjamin; Popp, Jürgen

    2013-10-01

    Nonlinear optical (NLO) microscopy based, e.g., on coherent anti-Stokes Raman scattering (CARS) or two-photon-excited fluorescence (TPEF) is a fast label-free imaging technique, with a great potential for biomedical applications. However, NLO microscopy as a diagnostic tool is still in its infancy; there is a lack of robust and durable nuclei segmentation methods capable of accurate image processing in cases of variable image contrast, nuclear density, and type of investigated tissue. Nonetheless, such algorithms specifically adapted to NLO microscopy present one prerequisite for the technology to be routinely used, e.g., in pathology or intraoperatively for surgical guidance. In this paper, we compare the applicability of different seeding and boundary detection methods to NLO microscopic images in order to develop an optimal seeding-based approach capable of accurate segmentation of both TPEF and CARS images. Among different methods, the Laplacian of Gaussian filter showed the best accuracy for the seeding of the image, while a modified seeded watershed segmentation was the most accurate in the task of boundary detection. The resulting combination of these methods followed by the verification of the detected nuclei performs high average sensitivity and specificity when applied to various types of NLO microscopy images.

  16. Nonlinear Quantum Optical Springs and Their Nonclassical Properties

    International Nuclear Information System (INIS)

    Faghihi, M.J.; Tavassoly, M.K.

    2011-01-01

    The original idea of quantum optical spring arises from the requirement of quantization of the frequency of oscillations in the Hamiltonian of harmonic oscillator. This purpose is achieved by considering a spring whose constant (and so its frequency) depends on the quantum states of another system. Recently, it is realized that by the assumption of frequency modulation of ω to ω√1+μa † a the mentioned idea can be established. In the present paper, we generalize the approach of quantum optical spring with particular attention to the dependence of frequency to the intensity of radiation field that naturally observes in the nonlinear coherent states, from which we arrive at a physical system has been called by us as nonlinear quantum optical spring. Then, after the introduction of the generalized Hamiltonian of nonlinear quantum optical spring and it's solution, we will investigate the nonclassical properties of the obtained states. Specially, typical collapse and revival in the distribution functions and squeezing parameters, as particular quantum features, will be revealed. (electromagnetism, optics, acoustics, heat transfer, classical mechanics, and fluid dynamics)

  17. Optical nonlinear absorption characteristics of Sb2Se3 nanoparticles

    Science.gov (United States)

    Muralikrishna, Molli; Kiran, Aditha Sai; Ravikanth, B.; Sowmendran, P.; Muthukumar, V. Sai; Venkataramaniah, Kamisetti

    2014-04-01

    In this work, we report for the first time, the nonlinear optical absorption properties of antimony selenide (Sb2Se3) nanoparticles synthesized through solvothermal route. X-ray diffraction results revealed the crystalline nature of the nanoparticles. Electron microscopy studies revealed that the nanoparticles are in the range of 10 - 40 nm. Elemental analysis was performed using EDAX. By employing open aperture z-scan technique, we have evaluated the effective two-photon absorption coefficient of Sb2Se3 nanoparticles to be 5e-10 m/W at 532 nm. These nanoparticles exhibit strong intensity dependent nonlinear optical absorption and hence could be considered to have optical power limiting applications in the visible range.

  18. Nonlinear Silicon Photonic Signal Processing Devices for Future Optical Networks

    Directory of Open Access Journals (Sweden)

    Cosimo Lacava

    2017-01-01

    Full Text Available In this paper, we present a review on silicon-based nonlinear devices for all optical nonlinear processing of complex telecommunication signals. We discuss some recent developments achieved by our research group, through extensive collaborations with academic partners across Europe, on optical signal processing using silicon-germanium and amorphous silicon based waveguides as well as novel materials such as silicon rich silicon nitride and tantalum pentoxide. We review the performance of four wave mixing wavelength conversion applied on complex signals such as Differential Phase Shift Keying (DPSK, Quadrature Phase Shift Keying (QPSK, 16-Quadrature Amplitude Modulation (QAM and 64-QAM that dramatically enhance the telecom signal spectral efficiency, paving the way to next generation terabit all-optical networks.

  19. Nonlinear ultrafast optical response in organic molecular crystals

    Science.gov (United States)

    Rahman, Talat S.; Turkowski, Volodymyr; Leuenberger, Michael N.

    2012-02-01

    We analyze possible nonlinear excitonic effects in the organic molecule crystals by using a combined time-dependent DFT and many-body approach. In particular, we analyze possible effects of the time-dependent (retarded)interaction between different types of excitations, Frenkel excitons, charge transfer excitons and excimers, on the electric and the optical response of the system. We pay special attention to the case of constant electric field and ultrafast pulses, including that of four-wave mixing experiments. As a specific application we examine the optical excitations of pentacene nanocrystals and compare the results with available experimental data.[1] Our results demostrate that the nonlinear effects can play an important role in the optical response of these systems. [1] A. Kabakchiev, ``Scanning Tunneling Luminescence of Pentacene Nanocrystals'', PhD Thesis (EPFL, Lausanne, 2010).

  20. Exact optical solitons in (n + 1)-dimensions with anti-cubic nonlinearity

    Science.gov (United States)

    Younis, Muhammad; Shahid, Iram; Anbreen, Sumaira; Rizvi, Syed Tahir Raza

    2018-02-01

    The paper studies the propagation of optical solitons in (n + 1)-dimensions under anti-cubic law of nonlinearity. The bright, dark and singular optical solitons are extracted using the extended trial equation method. The constraint conditions, for the existence of these solitons, are also listed. Additionally, a couple of other solutions known as singular periodic and Jacobi elliptic solutions, fall out as a by-product of this scheme. The obtained results are new and reported first time in (n + 1)-dimensions with anti-cubic law of nonlinearity.

  1. Measurements of nonlinear optical properties of PVDF/ZnO using Z-scan technique

    Energy Technology Data Exchange (ETDEWEB)

    Shanshool, Haider Mohammed, E-mail: haidshan62@gmail.com [Ministry of Science and Technology, Baghdad (Iraq); Yahaya, Muhammad [School of Applied Physics, Faculty of Science and Technology, Universiti Kebangsaan Malaysia, Selangor (Malaysia); Yunus, Wan Mahmood Mat [Department of Physics, Faculty of Science, University Putra Malaysia, Serdang (Malaysia); Abdullah, Ibtisam Yahya [Department of Physics, College of Science, University of Mosul, Mosul (Iraq)

    2015-10-15

    The nonlinear optical properties of ZnO nanoparticles dispersed in poly (vinylidene fluoride) (PVDF) polymer are investigated. PVDF/ZnO nanocomposites were prepared by mixing different concentrations of ZnO nanoparticles, as the filler, with PVDF, as the polymer matrix, using casting method. Acetone was used as a solvent for the polymer. FTIR spectra of the samples were analyzed thus confirming the formation of α and β phases. The absorbance spectra of the samples were obtained, thereby showing high absorption in the UV region. The linear absorption coefficient was calculated. The single-beam Z-scan technique was used to measure the nonlinear refractive index and the nonlinear absorption coefficient of the PVDF/ZnO nanocomposite samples. We observed that the nonlinear refractive index is in the order of 10{sup -13} cm{sup 2}/W with the negative sign, whereas the nonlinear absorption coefficient is in the order of 10{sup -8} cm/W. (author)

  2. Macroscopic quantum effects in nonlinear optical patterns

    International Nuclear Information System (INIS)

    Gatti, A.; Lugiato, L.A.; Oppo, G.L.; Barnett, S.M.; Marzoli, I.

    1998-01-01

    We display the results of the numerical simulations of a set of Langevin equations, which describe the dynamics of a degenerate optical parametric oscillator in the Wigner representation. The scan of the threshold region shows the gradual transformation of a quantum image into a classical roll pattern. Thus the quantum image behaves as a precursor of the roll pattern which appear above threshold. In the fax field, suitable spatial correlation functions of intensity and field quadratures show unambiguously the quantum nature of fluctuations that generate the image, leading to effects of quantum noise reduction below the shot noise level and to the formulation of an EPR paradox. (author)

  3. Third-order nonlinear optical properties of the poly(methyl methacrylate)-phenothiazinium dye hybrid thin films

    International Nuclear Information System (INIS)

    Sun, Ru; Lu, Yue-Ting; Yan, Bao-Long; Lu, Jian-Mei; Wu, Xing-Zhi; Song, Ying-Lin; Ge, Jian-Feng

    2014-01-01

    The third-order nonlinear optical properties of poly(methyl methacrylate) films doped with charge flowable 3,7-di(piperidinyl)phenothiazin-5-ium chloride, which tested by Z-scan method with nanosecond laser beam at 532 nm, are reported. Large third-order nonlinear optical susceptibilities (up to 10 −7 esu) and high second hyperpolarizabilities (up to 10 −27 esu) are found. The third-order nonlinear absorptions change from reverse saturated absorptions to saturated absorptions with different percentage of the phenothiazinium dye in the poly(methyl methacrylate) films, which can be explained by the accumulation phenomenon of the phenothiazinium. The results suggest that the phenothiazinium salt is a promising material for third order non-linear applications. - Highlights: • Phenothiazinium containing optical films • Strong third-order nonlinear optical (NLO) absorption • Large third-order NLO susceptibilities

  4. Second order nonlinear optical properties of zinc oxide films deposited by low temperature dual ion beam sputtering

    International Nuclear Information System (INIS)

    Larciprete, M.C.; Passeri, D.; Michelotti, F.; Paoloni, S.; Sibilia, C.; Bertolotti, M.; Belardini, A.; Sarto, F.; Somma, F.; Lo Mastro, S.

    2005-01-01

    We investigated second order optical nonlinearity of zinc oxide thin films, grown on glass substrates by the dual ion beam sputtering technique under different deposition conditions. Linear optical characterization of the films was carried out by spectrophotometric optical transmittance and reflectance measurements, giving the complex refractive index dispersion. Resistivity of the films was determined using the four-point probe sheet resistance method. Second harmonic generation measurements were performed by means of the Maker fringes technique where the fundamental beam was originated by nanosecond laser at λ=1064 nm. We found a relatively high nonlinear optical response, and evidence of a dependence of the nonlinear coefficient on the deposition parameters for each sample. Moreover, the crystalline properties of the films were investigated by x-ray diffraction measurements and correlation with second order nonlinearity were analyzed. Finally, we investigated the influence of the oxygen flow rate during the deposition process on both the second order nonlinearity and the structural properties of the samples

  5. Optical computation based on nonlinear total reflectional optical ...

    Indian Academy of Sciences (India)

    2School of Education Science, South China Normal University, Guangzhou, 510631, China. *Corresponding ... Before the computation, all the inputs are prepared in the polarization state. The key .... The all-optical computing system described.

  6. Cross-Kerr nonlinearities in an optically dressed periodic medium

    Energy Technology Data Exchange (ETDEWEB)

    Slowik, K; Raczynski, A; Zaremba, J [Instytut Fizyki, Uniwersytet Mikolaja Kopernika, ulica Grudziadzka 5, 87-100 Torun (Poland); Zielinska-Kaniasty, S [Instytut Matematyki i Fizyki, Uniwersytet Technologiczno-Przyrodniczy, Aleja Prof. S Kaliskiego 7, 85-789 Bydgoszcz (Poland); Artoni, M [Department of Physics and Chemistry of Materials, CNR-INFM Sensor Lab, Brescia University and European Laboratory for Nonlinear Spectroscopy, Firenze (Italy); La Rocca, G C, E-mail: karolina@fizyka.umk.pl [Scuola Normale Superiore and CNISM, Pisa (Italy)

    2011-02-15

    Cross-Kerr nonlinearities are analyzed for two light beams propagating in an atomic medium in the tripod configuration, dressed by a strong standing-wave laser field that induces periodic optical properties. The reflection and transmission spectra as well as the phases of both the reflected and transmitted components of the two beams are analyzed theoretically with nonlinearities up to third order being taken into account. Ranges of parameters are sought in which the cross-Kerr effect can be used as the basis of the phase gate.

  7. Second-order nonlinear optical microscopy of spider silk

    Science.gov (United States)

    Zhao, Yue; Hien, Khuat Thi Thu; Mizutani, Goro; Rutt, Harvey N.

    2017-06-01

    Asymmetric β-sheet protein structures in spider silk should induce nonlinear optical interaction such as second harmonic generation (SHG) which is experimentally observed for a radial line and dragline spider silk using an imaging femtosecond laser SHG microscope. By comparing different spider silks, we found that the SHG signal correlates with the existence of the protein β-sheets. Measurements of the polarization dependence of SHG from the dragline indicated that the β-sheet has a nonlinear response depending on the direction of the incident electric field. We propose a model of what orientation the β-sheet takes in spider silk.

  8. Second Harmonic Generation, Sum Frequency Generation, and χ(3): Dissecting Environmental Interfaces with a Nonlinear Optical Swiss Army Knife

    Science.gov (United States)

    Geiger, Franz M.

    2009-05-01

    This review discusses recent advances in the nonlinear optics of environmental interfaces. We discuss the quantitative aspects of the label-free approaches presented here and demonstrate that nonlinear optics has now assumed the role of a Swiss Army knife that can be used to dissect, with molecular detail, the fundamental and practical aspects of environmental interfaces and heterogeneous geochemical environments. In this work, nonlinear optical methods are applied to complex organic molecules, such as veterinary antibiotics, and to small inorganic anions and cations, such as nitrate and chromate, or cadmium, zinc, and manganese. The environmental implications of the thermodynamic, kinetic, spectroscopic, structural, and electrochemical data are discussed.

  9. Benchmarking Post-Hartree–Fock Methods To Describe the Nonlinear Optical Properties of Polymethines: An Investigation of the Accuracy of Algebraic Diagrammatic Construction (ADC) Approaches

    KAUST Repository

    Knippenberg, Stefan; Gieseking, Rebecca L.; Rehn, Dirk R.; Mukhopadhyay, Sukrit; Dreuw, Andreas; Bredas, Jean-Luc

    2016-01-01

    -of-merit for all-optical switching. For a series of model polymethines, we compare several algebraic diagrammatic construction (ADC) schemes for the polarization propagator with approximate second-order coupled cluster (CC2) theory, the widely used INDO

  10. Report of workshop on X-ray and nonlinear optics

    Energy Technology Data Exchange (ETDEWEB)

    Nasu, Keiichiro; Namikawa, Kazumichi [eds.

    1994-07-01

    As synchrotron radiation has advanced to high luminance, the possibility of realizing coherent light has heightened, and the nonlinear optical phenomena in soft and hard X-ray regions have become the object of the concern of X-ray researchers, and also the researchers in the fields of quantum electronics and optical properties. This workshop was held on September 21 and 22, 1993 at National Laboratory for High energy Physics. Lectures were given on the generation of second harmonic of X-ray by utilizing dynamic diffraction, X-ray parametric scattering induced by strong laser beam, the resonance enhancement of X-ray inelastic scattering induced by strong visible light, Raman scattering in soft X-ray region, the control of nonlinear optical processes by strong external field; the experiments, though they are fundamental, they have not been carried out; undulator radiation X-ray and X-ray free electron laser, the improvement of the coherence of X-ray laser, superradiance of Frenkel excitor system and the measurement of superhigh speed pulses in X-ray region. The comment from the standpoint of the research on nonlinear optics was given. In this document, the gists of these lectures are collected. (K.I.).

  11. Report of workshop on X-ray and nonlinear optics

    International Nuclear Information System (INIS)

    Nasu, Keiichiro; Namikawa, Kazumichi

    1994-07-01

    As synchrotron radiation has advanced to high luminance, the possibility of realizing coherent light has heightened, and the nonlinear optical phenomena in soft and hard X-ray regions have become the object of the concern of X-ray researchers, and also the researchers in the fields of quantum electronics and optical properties. This workshop was held on September 21 and 22, 1993 at National Laboratory for High energy Physics. Lectures were given on the generation of second harmonic of X-ray by utilizing dynamic diffraction, X-ray parametric scattering induced by strong laser beam, the resonance enhancement of X-ray inelastic scattering induced by strong visible light, Raman scattering in soft X-ray region, the control of nonlinear optical processes by strong external field; the experiments, though they are fundamental, they have not been carried out; undulator radiation X-ray and X-ray free electron laser, the improvement of the coherence of X-ray laser, superradiance of Frenkel excitor system and the measurement of superhigh speed pulses in X-ray region. The comment from the standpoint of the research on nonlinear optics was given. In this document, the gists of these lectures are collected. (K.I.)

  12. Ablation and optical third-order nonlinearities in Ag nanoparticles

    Directory of Open Access Journals (Sweden)

    Carlos Torres-Torres

    2010-11-01

    Full Text Available Carlos Torres-Torres1, Néstor Peréa-López2, Jorge Alejandro Reyes-Esqueda3, Luis Rodríguez-Fernández3, Alejandro Crespo-Sosa3, Juan Carlos Cheang-Wong3, Alicia Oliver31Section of Graduate Studies and Research, School of Mechanical and Electrical Engineering, National Polytechnic Institute, Zacatenco, Distrito Federal, Mexico; 2Laboratory for Nanoscience and Nanotechnology Research and Advanced Materials Department, IPICYT, Camino a la Presa San Jose, San Luis Potosi, Mexico; 3Instituto de Física, Universidad Nacional Autónoma de México, A.P. 20-364, México, D.F. 01000, MéxicoAbstract: The optical damage associated with high intensity laser excitation of silver nanoparticles (NPs was studied. In order to investigate the mechanisms of optical nonlinearity of a nanocomposite and their relation with its ablation threshold, a high-purity silica sample implanted with Ag ions was exposed to different nanosecond and picosecond laser irradiations. The magnitude and sign of picosecond refractive and absorptive nonlinearities were measured near and far from the surface plasmon resonance (SPR of the Ag NPs with a self-diffraction technique. Saturable optical absorption and electronic polarization related to self-focusing were identified. Linear absorption is the main process involved in nanosecond laser ablation, but nonlinearities are important for ultrashort picosecond pulses when the absorptive process become significantly dependent on the irradiance. We estimated that near the resonance, picosecond intraband transitions allow an expanded distribution of energy among the NPs, in comparison to the energy distribution resulting in a case of far from resonance, when the most important absorption takes place in silica. We measured important differences in the ablation threshold and we estimated that the high selectiveness of the SPR of Ag NPs as well as their corresponding optical nonlinearities can be strongly significant for laser

  13. FDTD method and models in optical education

    Science.gov (United States)

    Lin, Xiaogang; Wan, Nan; Weng, Lingdong; Zhu, Hao; Du, Jihe

    2017-08-01

    In this paper, finite-difference time-domain (FDTD) method has been proposed as a pedagogical way in optical education. Meanwhile, FDTD solutions, a simulation software based on the FDTD algorithm, has been presented as a new tool which helps abecedarians to build optical models and to analyze optical problems. The core of FDTD algorithm is that the time-dependent Maxwell's equations are discretized to the space and time partial derivatives, and then, to simulate the response of the interaction between the electronic pulse and the ideal conductor or semiconductor. Because the solving of electromagnetic field is in time domain, the memory usage is reduced and the simulation consequence on broadband can be obtained easily. Thus, promoting FDTD algorithm in optical education is available and efficient. FDTD enables us to design, analyze and test modern passive and nonlinear photonic components (such as bio-particles, nanoparticle and so on) for wave propagation, scattering, reflection, diffraction, polarization and nonlinear phenomena. The different FDTD models can help teachers and students solve almost all of the optical problems in optical education. Additionally, the GUI of FDTD solutions is so friendly to abecedarians that learners can master it quickly.

  14. Optical switching in nonlinear photonic crystals lightly doped with nanostructures

    Energy Technology Data Exchange (ETDEWEB)

    Singh, Mahi R [Department of Physics and Astronomy, University of Western Ontario, London, ON N6A 3K7 (Canada); Lipson, R H [Department of Chemistry, University of Western Ontario, London, ON N6A 5B7 (Canada)

    2008-01-14

    A possible switching mechanism has been investigated for nonlinear photonic crystals doped with an ensemble of non-interacting three-level nanoparticles. In this scheme, an intense pump laser field is used to change the refractive index of the nonlinear photonic crystal while a weaker probe field monitors an absorption transition in the nanoparticles. In the absence of the strong laser field the system transmits the probe field when the resonance energy of the nanoparticles lies near the edge of the photonic band gap due to strong coupling between the photonic crystal and the nanoparticles. However, upon application of an intense pump laser field the system becomes absorbing due to a band edge frequency shift that arises due to a nonlinear Kerr effect which changes the refractive index of the crystal. It is anticipated that the optical switching mechanism described in this work can be used to make new types of photonic devices.

  15. Determination of optical constants and nonlinear optical coefficients ...

    Indian Academy of Sciences (India)

    of single crystals of organic molecules [12,13], organic molecules in a liquid solution. [14,15] and organic ... valence band 'tail states' might have a strong effect on the optical absorption resulting in ..... cm/W). The negative sign of the third-order.

  16. Nonlinear optical polarization analysis in chemistry and biology

    CERN Document Server

    Simpson, Garth J

    2017-01-01

    This rigorous yet accessible guide presents a molecular-based description of nonlinear optical polarization analysis of chemical and biological assemblies. It includes discussion of the most common nonlinear optical microscopy and interfacial measurements used for quantitative analysis, specifically second harmonic generation (SHG), two-photon excited fluorescence (2PEF), vibrational sum frequency generation (SFG), and coherent anti-Stokes Raman spectroscopy/stimulated Raman spectroscopy (CARS/SRS). A linear algebra mathematical framework is developed, allowing step-wise systematic connections to be made between the observable measurements and the molecular response. Effects considered include local field corrections, the molecular orientation distribution, rotations between the molecular frame, the local frame and the laboratory frame, and simplifications from molecular and macromolecular symmetry. Specific examples are provided throughout the book, working from the common and relatively simple case studies ...

  17. Nonlinear optical localization in embedded chalcogenide waveguide arrays

    International Nuclear Information System (INIS)

    Li, Mingshan; Huang, Sheng; Wang, Qingqing; Chen, Kevin P.; Petek, Hrvoje

    2014-01-01

    We report the nonlinear optical localization in an embedded waveguide array fabricated in chalcogenide glass. The array, which consists of seven waveguides with circularly symmetric cross sections, is realized by ultrafast laser writing. Light propagation in the chalcogenide waveguide array is studied with near infrared laser pulses centered at 1040 nm. The peak intensity required for nonlinear localization for the 1-cm long waveguide array was 35.1 GW/cm 2 , using 10-nJ pulses with 300-fs pulse width, which is 70 times lower than that reported in fused silica waveguide arrays and with over 7 times shorter interaction distance. Results reported in this paper demonstrated that ultrafast laser writing is a viable tool to produce 3D all-optical switching waveguide circuits in chalcogenide glass

  18. Dynamic nonlinear thermal optical effects in coupled ring resonators

    Directory of Open Access Journals (Sweden)

    Chenguang Huang

    2012-09-01

    Full Text Available We investigate the dynamic nonlinear thermal optical effects in a photonic system of two coupled ring resonators. A bus waveguide is used to couple light in and out of one of the coupled resonators. Based on the coupling from the bus to the resonator, the coupling between the resonators and the intrinsic loss of each individual resonator, the system transmission spectrum can be classified by three different categories: coupled-resonator-induced absorption, coupled-resonator-induced transparency and over coupled resonance splitting. Dynamic thermal optical effects due to linear absorption have been analyzed for each category as a function of the input power. The heat power in each resonator determines the thermal dynamics in this coupled resonator system. Multiple “shark fins” and power competition between resonators can be foreseen. Also, the nonlinear absorption induced thermal effects have been discussed.

  19. Methods for Large-Scale Nonlinear Optimization.

    Science.gov (United States)

    1980-05-01

    STANFORD, CALIFORNIA 94305 METHODS FOR LARGE-SCALE NONLINEAR OPTIMIZATION by Philip E. Gill, Waiter Murray, I Michael A. Saunden, and Masgaret H. Wright...typical iteration can be partitioned so that where B is an m X m basise matrix. This partition effectively divides the vari- ables into three classes... attention is given to the standard of the coding or the documentation. A much better way of obtaining mathematical software is from a software library

  20. Nonlinear effect of the structured light profilometry in the phase-shifting method and error correction

    International Nuclear Information System (INIS)

    Zhang Wan-Zhen; Chen Zhe-Bo; Xia Bin-Feng; Lin Bin; Cao Xiang-Qun

    2014-01-01

    Digital structured light (SL) profilometry is increasingly used in three-dimensional (3D) measurement technology. However, the nonlinearity of the off-the-shelf projectors and cameras seriously reduces the measurement accuracy. In this paper, first, we review the nonlinear effects of the projector–camera system in the phase-shifting structured light depth measurement method. We show that high order harmonic wave components lead to phase error in the phase-shifting method. Then a practical method based on frequency domain filtering is proposed for nonlinear error reduction. By using this method, the nonlinear calibration of the SL system is not required. Moreover, both the nonlinear effects of the projector and the camera can be effectively reduced. The simulations and experiments have verified our nonlinear correction method. (electromagnetism, optics, acoustics, heat transfer, classical mechanics, and fluid dynamics)

  1. Femtosecond nonlinear fiber optics in the ionization regime.

    Science.gov (United States)

    Hölzer, P; Chang, W; Travers, J C; Nazarkin, A; Nold, J; Joly, N Y; Saleh, M F; Biancalana, F; Russell, P St J

    2011-11-11

    By using a gas-filled kagome-style photonic crystal fiber, nonlinear fiber optics is studied in the regime of optically induced ionization. The fiber offers low anomalous dispersion over a broad bandwidth and low loss. Sequences of blueshifted pulses are emitted when 65 fs, few-microjoule pulses, corresponding to high-order solitons, are launched into the fiber and undergo self-compression. The experimental results are confirmed by numerical simulations which suggest that free-electron densities of ∼10(17) cm(-3) are achieved at peak intensities of 10(14) W/cm(2) over length scales of several centimeters.

  2. Structure, Electronic and Nonlinear Optical Properties of Furyloxazoles and Thienyloxazoles

    International Nuclear Information System (INIS)

    Dagli, Ozlem; Gok, Rabia; Bahat, Mehmet; Ozbay, Akif

    2016-01-01

    Geometry optimization, electronic and nonlinear optical properties of isomers of furyloxazole and thienyloxazole molecules are carried out at the B3LYP/6-311++G(2d,p) level. The conformational analysis of 12 compounds have been studied as a function of torsional angle between rings. Electronic and NLO properties such as dipole moment, energy gap, polarizability and first hyperpolarizability were also calculated. (paper)

  3. Optical Nonlinearities and Ultrafast Carrier Dynamics in Semiconductor Quantum Dots

    Energy Technology Data Exchange (ETDEWEB)

    Klimov, V.; McBranch, D.; Schwarz, C.

    1998-08-10

    Low-dimensional semiconductors have attracted great interest due to the potential for tailoring their linear and nonlinear optical properties over a wide-range. Semiconductor nanocrystals (NC's) represent a class of quasi-zero-dimensional objects or quantum dots. Due to quantum cordhement and a large surface-to-volume ratio, the linear and nonlinear optical properties, and the carrier dynamics in NC's are significantly different horn those in bulk materials. napping at surface states can lead to a fast depopulation of quantized states, accompanied by charge separation and generation of local fields which significantly modifies the nonlinear optical response in NC's. 3D carrier confinement also has a drastic effect on the energy relaxation dynamics. In strongly confined NC's, the energy-level spacing can greatly exceed typical phonon energies. This has been expected to significantly inhibit phonon-related mechanisms for energy losses, an effect referred to as a phonon bottleneck. It has been suggested recently that the phonon bottleneck in 3D-confined systems can be removed due to enhanced role of Auger-type interactions. In this paper we report femtosecond (fs) studies of ultrafast optical nonlinearities, and energy relaxation and trap ping dynamics in three types of quantum-dot systems: semiconductor NC/glass composites made by high temperature precipitation, ion-implanted NC's, and colloidal NC'S. Comparison of ultrafast data for different samples allows us to separate effects being intrinsic to quantum dots from those related to lattice imperfections and interface properties.

  4. Optically nonlinear energy transfer in light-harvesting dendrimers

    OpenAIRE

    Andrews, David; Bradshaw, DS

    2004-01-01

    Dendrimeric polymers are the subject of intense research activity geared towards their implementation in nanodevice applications such as energy harvesting systems,organic light-emitting diodes, photosensitizers, low-threshold lasers, and quantum logic elements, etc. A recent development in this area has been the construction of dendrimers specifically designed to exhibit novel forms of optical nonlinearity, exploiting the unique properties of these materials at high levels of photon flux. Sta...

  5. Nonlinear response matrix methods for radiative transfer

    International Nuclear Information System (INIS)

    Miller, W.F. Jr.; Lewis, E.E.

    1987-01-01

    A nonlinear response matrix formalism is presented for the solution of time-dependent radiative transfer problems. The essential feature of the method is that within each computational cell the temperature is calculated in response to the incoming photons from all frequency groups. Thus the updating of the temperature distribution is placed within the iterative solution of the spaceangle transport problem, instead of being placed outside of it. The method is formulated for both grey and multifrequency problems and applied in slab geometry. The method is compared to the more conventional source iteration technique. 7 refs., 1 fig., 4 tabs

  6. Nonlinear optical effects of opening a gap in graphene

    Science.gov (United States)

    Carvalho, David N.; Biancalana, Fabio; Marini, Andrea

    2018-05-01

    Graphene possesses remarkable electronic, optical, and mechanical properties that have taken the research of two-dimensional relativistic condensed matter systems to prolific levels. However, the understanding of how its nonlinear optical properties are affected by relativisticlike effects has been broadly uncharted. It has been recently shown that highly nontrivial currents can be generated in free-standing samples, notably leading to the generation of even harmonics. Since graphene monolayers are centrosymmetric media, for which such harmonic generation at normal incidence is deemed inaccessible, this light-driven phenomenon is both startling and promising. More realistically, graphene samples are often deposited on a dielectric substrate, leading to additional intricate interactions. Here, we present a treatment to study this instance by gapping the spectrum and we show this leads to the appearance of a Berry phase in the carrier dynamics. We analyze the role of such a phase in the generated nonlinear current and conclude that it suppresses odd-harmonic generation. The pump energy can be tuned to the energy gap to yield interference among odd harmonics mediated by interband transitions, allowing even harmonics to be generated. Our results and general methodology pave the way for understanding the role of gap opening in the nonlinear optics of two-dimensional lattices.

  7. Synthesis of polymeric micro- and nanostructural materials for application in non-linear optics

    International Nuclear Information System (INIS)

    Kravets, Lyubov; Palistrant, Natalia; Bivol, Valerii; Robu, Stepan; Barba, Nikolai; Orelovitch, Oleg

    2007-01-01

    The present paper describes a new approach developed for the preparation of micro- and nanostructural materials on the basis of polymeric compositions used as a matrix in non-linear optics. This approach consists in filling the pores of poly(ethylene terephthalate) track membranes (PET TM) from polymeric compositions using an impregnation method. It is shown that depending on the concentration of polymeric compositions in the solution it is possible to form a variety of micro- and nanostructural materials (tubules and wires as well as composite membranes) with a wide spectrum of characteristics. The developed method of producing micro- and nanostructural materials provides a possible way for creating polymeric objects with non-linear optic properties which can be used to design electronic micro- and nanodevices and to obtain chemical and optical sensors

  8. Preparation, characterization, and nonlinear optical properties of hybridized graphene @ gold nanorods nanocomposites

    Science.gov (United States)

    Guo, Jia; Ning, Tingyin; Han, Yanshun; Sheng, Yingqiang; Li, Chonghui; Zhao, Xiaofei; Lu, Zhengyi; Man, Baoyuan; Jiao, Yang; Jiang, Shouzhen

    2018-03-01

    The methods of chemical vapor deposition (CVD) and seed-mediated growth were used to obtain graphene and gold nanorods (GNRs), respectively. We fabricate graphene @ gold nanorods (G@GNRs) nanocomposites by successively using dropping and transferring methods Through SEM, Raman spectra and TEM analysis, the number of graphene layers is 6-7. The diameter of gold nanorods (GNRs) is about 10 nm and the average aspect ratio is 6.5. In addition, we systematically investigate their nonlinear optical responses by using open-aperture Z-scan technique. In contrast with graphene and GNRs, the G@GNRs nanocomposites exhibit excellent nonlinear optical response with a modulation depth of about 51% and a saturable intensity of about 6.23 GW/cm2. The results suggest that the G@GNRs nanocomposites could potentially be used as an optical modulator in pulsed laser generation.

  9. Nonlinear ordinary differential equations analytical approximation and numerical methods

    CERN Document Server

    Hermann, Martin

    2016-01-01

    The book discusses the solutions to nonlinear ordinary differential equations (ODEs) using analytical and numerical approximation methods. Recently, analytical approximation methods have been largely used in solving linear and nonlinear lower-order ODEs. It also discusses using these methods to solve some strong nonlinear ODEs. There are two chapters devoted to solving nonlinear ODEs using numerical methods, as in practice high-dimensional systems of nonlinear ODEs that cannot be solved by analytical approximate methods are common. Moreover, it studies analytical and numerical techniques for the treatment of parameter-depending ODEs. The book explains various methods for solving nonlinear-oscillator and structural-system problems, including the energy balance method, harmonic balance method, amplitude frequency formulation, variational iteration method, homotopy perturbation method, iteration perturbation method, homotopy analysis method, simple and multiple shooting method, and the nonlinear stabilized march...

  10. Multi-crack imaging using nonclassical nonlinear acoustic method

    International Nuclear Information System (INIS)

    Zhang Lue; Zhang Ying; Liu Xiao-Zhou; Gong Xiu-Fen

    2014-01-01

    Solid materials with cracks exhibit the nonclassical nonlinear acoustical behavior. The micro-defects in solid materials can be detected by nonlinear elastic wave spectroscopy (NEWS) method with a time-reversal (TR) mirror. While defects lie in viscoelastic solid material with different distances from one another, the nonlinear and hysteretic stress—strain relation is established with Preisach—Mayergoyz (PM) model in crack zone. Pulse inversion (PI) and TR methods are used in numerical simulation and defect locations can be determined from images obtained by the maximum value. Since false-positive defects might appear and degrade the imaging when the defects are located quite closely, the maximum value imaging with a time window is introduced to analyze how defects affect each other and how the fake one occurs. Furthermore, NEWS-TR-NEWS method is put forward to improve NEWS-TR scheme, with another forward propagation (NEWS) added to the existing phases (NEWS and TR). In the added phase, scanner locations are determined by locations of all defects imaged in previous phases, so that whether an imaged defect is real can be deduced. NEWS-TR-NEWS method is proved to be effective to distinguish real defects from the false-positive ones. Moreover, it is also helpful to detect the crack that is weaker than others during imaging procedure. (electromagnetism, optics, acoustics, heat transfer, classical mechanics, and fluid dynamics)

  11. Optical rogue waves generation in a nonlinear metamaterial

    Science.gov (United States)

    Onana Essama, Bedel Giscard; Atangana, Jacques; Biya-Motto, Frederick; Mokhtari, Bouchra; Cherkaoui Eddeqaqi, Noureddine; Kofane, Timoleon Crepin

    2014-11-01

    We investigate the behavior of electromagnetic wave which propagates in a metamaterial for negative index regime. The optical pulse propagation is described by the nonlinear Schrödinger equation with cubic-quintic nonlinearities, second- and third-order dispersion effects. The behavior obtained for negative index regime is compared to that observed for positive index regime. The characterization of electromagnetic wave uses some pulse parameters obtained analytically and called collective coordinates such as amplitude, temporal position, width, chirp, frequency shift and phase. Six frequency ranges have been pointed out where a numerical evolution of collective coordinates and their stability are studied under a typical example to verify our analysis. It appears that a robust soliton due to a perfect compensation process between second-order dispersion and cubic-nonlinearity is presented at each frequency range for both negative and positive index regimes. Thereafter, the stability of the soliton pulse and physical conditions leading to optical rogue waves generation are discussed at each frequency range for both regimes, when third-order dispersion and quintic-nonlinearity come into play. We have demonstrated that collective coordinates give much useful information on external and internal behavior of rogue events. Firstly, we determine at what distance begins the internal excitation leading to rogue waves. Secondly, what kind of internal modification and how it modifies the system in order to build-up rogue events. These results lead to a best comprehension of the mechanism of rogue waves generation. So, it clearly appears that the rogue wave behavior strongly depends on nonlinearity strength of distortion, frequency and regime considered.

  12. Gallium nitride on gallium oxide substrate for integrated nonlinear optics

    KAUST Repository

    Awan, Kashif M.; Dolgaleva, Ksenia; Mumthaz Muhammed, Mufasila; Roqan, Iman S.

    2017-01-01

    Gallium Nitride (GaN), being a direct bandgap semiconductor with a wide bandgap and high thermal stability, is attractive for optoelectronic and electronic applications. Furthermore, due to its high optical nonlinearity — the characteristic of all 111-V semiconductors — GaN is also expected to be a suitable candidate for integrated nonlinear photonic circuits for a plethora of apphcations, ranging from on-chip wavelength conversion to quantum computing. Although GaN devices are in commercial production, it still suffers from lack of a suitable substrate material to reduce structural defects like high densities of threading dislocations (TDs), stacking faults, and grain boundaries. These defects significandy deteriorate the optical quality of the epi-grown GaN layer, since they act as non-radiative recombination centers. Recent studies have shown that GaN grown on (−201) β-Gallium Oxide (Ga2O3) has superior optical quality due to a better lattice matching as compared to GaN grown on Sapphire (Al2O3) [1-3]. In this work, we report on the fabrication of GaN waveguides on GaiOj substrate and their optical characterization to assess their feasibihty for efficient four-wave mixing (FWM).

  13. Polycarbonate-Based Blends for Optical Non-linear Applications

    Science.gov (United States)

    Stanculescu, F.; Stanculescu, A.

    2016-02-01

    This paper presents some investigations on the optical and morphological properties of the polymer (matrix):monomer (inclusion) composite materials obtained from blends of bisphenol A polycarbonate and amidic monomers. For the preparation of the composite films, we have selected monomers characterised by a maleamic acid structure and synthesised them starting from maleic anhydride and aniline derivatives with -COOH, -NO2, -N(C2H5)2 functional groups attached to the benzene ring. The composite films have been deposited by spin coating using a mixture of two solutions, one containing the matrix and the other the inclusion, both components of the composite system being dissolved in the same solvent. The optical transmission and photoluminescence properties of the composite films have been investigated in correlation with the morphology of the films. The scanning electron microscopy and atomic force microscopy have revealed a non-uniform morphology characterised by the development of two distinct phases. We have also investigated the generation of some optical non-linear (ONL) phenomena in these composite systems. The composite films containing as inclusions monomers characterised by the presence of one -COOH or two -NO2 substituent groups to the aromatic nucleus have shown the most intense second-harmonic generation (SHG). The second-order optical non-linear coefficients have been evaluated for these films, and the effect of the laser power on the ONL behaviour of these materials has also been emphasised.

  14. Gallium nitride on gallium oxide substrate for integrated nonlinear optics

    KAUST Repository

    Awan, Kashif M.

    2017-11-22

    Gallium Nitride (GaN), being a direct bandgap semiconductor with a wide bandgap and high thermal stability, is attractive for optoelectronic and electronic applications. Furthermore, due to its high optical nonlinearity — the characteristic of all 111-V semiconductors — GaN is also expected to be a suitable candidate for integrated nonlinear photonic circuits for a plethora of apphcations, ranging from on-chip wavelength conversion to quantum computing. Although GaN devices are in commercial production, it still suffers from lack of a suitable substrate material to reduce structural defects like high densities of threading dislocations (TDs), stacking faults, and grain boundaries. These defects significandy deteriorate the optical quality of the epi-grown GaN layer, since they act as non-radiative recombination centers. Recent studies have shown that GaN grown on (−201) β-Gallium Oxide (Ga2O3) has superior optical quality due to a better lattice matching as compared to GaN grown on Sapphire (Al2O3) [1-3]. In this work, we report on the fabrication of GaN waveguides on GaiOj substrate and their optical characterization to assess their feasibihty for efficient four-wave mixing (FWM).

  15. New methods of testing nonlinear hypothesis using iterative NLLS estimator

    Science.gov (United States)

    Mahaboob, B.; Venkateswarlu, B.; Mokeshrayalu, G.; Balasiddamuni, P.

    2017-11-01

    This research paper discusses the method of testing nonlinear hypothesis using iterative Nonlinear Least Squares (NLLS) estimator. Takeshi Amemiya [1] explained this method. However in the present research paper, a modified Wald test statistic due to Engle, Robert [6] is proposed to test the nonlinear hypothesis using iterative NLLS estimator. An alternative method for testing nonlinear hypothesis using iterative NLLS estimator based on nonlinear hypothesis using iterative NLLS estimator based on nonlinear studentized residuals has been proposed. In this research article an innovative method of testing nonlinear hypothesis using iterative restricted NLLS estimator is derived. Pesaran and Deaton [10] explained the methods of testing nonlinear hypothesis. This paper uses asymptotic properties of nonlinear least squares estimator proposed by Jenrich [8]. The main purpose of this paper is to provide very innovative methods of testing nonlinear hypothesis using iterative NLLS estimator, iterative NLLS estimator based on nonlinear studentized residuals and iterative restricted NLLS estimator. Eakambaram et al. [12] discussed least absolute deviation estimations versus nonlinear regression model with heteroscedastic errors and also they studied the problem of heteroscedasticity with reference to nonlinear regression models with suitable illustration. William Grene [13] examined the interaction effect in nonlinear models disused by Ai and Norton [14] and suggested ways to examine the effects that do not involve statistical testing. Peter [15] provided guidelines for identifying composite hypothesis and addressing the probability of false rejection for multiple hypotheses.

  16. Exact solitary wave solution for higher order nonlinear Schrodinger equation using He's variational iteration method

    Science.gov (United States)

    Rani, Monika; Bhatti, Harbax S.; Singh, Vikramjeet

    2017-11-01

    In optical communication, the behavior of the ultrashort pulses of optical solitons can be described through nonlinear Schrodinger equation. This partial differential equation is widely used to contemplate a number of physically important phenomena, including optical shock waves, laser and plasma physics, quantum mechanics, elastic media, etc. The exact analytical solution of (1+n)-dimensional higher order nonlinear Schrodinger equation by He's variational iteration method has been presented. Our proposed solutions are very helpful in studying the solitary wave phenomena and ensure rapid convergent series and avoid round off errors. Different examples with graphical representations have been given to justify the capability of the method.

  17. Nonlinear optical activity in Bridgman growth layered compounds

    Energy Technology Data Exchange (ETDEWEB)

    Miah, M.I., E-mail: m.miah@griffith.edu.au [Queensland Micro- and Nanotechnology Centre, Griffith University, Nathan, Brisbane, QLD 4111 (Australia); Biomolecular and Physical Sciences, Griffith University, Nathan, Brisbane, QLD 4111 (Australia); Department of Physics, University of Chittagong, Chittagong 4331 (Bangladesh)

    2010-02-15

    Layered semiconductor compound CdI{sub 2} has been grown with the Bridgman technique and studied by nonlinear transmittance spectroscopy. The optical absorption in CdI{sub 2} shows a nonlinear transmission of the incident laser power (P{sub 0}) within a lower power limit. The transmission, however, is found to saturate at high powers, giving a clamped output. The value of the incident power (P{sub 0C}) at which clamping starts is also found to depend on the crystal temperature (T{sub L}). The values of P{sub OC} ranges from 55 to 65 MW cm{sup -2} for T{sub L} = 4.2-180 K. The dynamic range (D{sub R}) as a function of T{sub L} is calculated and the values are found to range from D{sub R} = 2 to 1.6. The optical limiting mechanisms are discussed. The two-photon absorption (TPA) coefficient ({beta}) of the optical nonlinear process in CdI{sub 2} is estimated. The values are found to be within a range from {beta} = 47 to 25 cm GW{sup -1} and be decreasing with increasing T{sub L}. As expected for the TPA process, the experimental data within a certain range follows the linear relation: log (P{sub 0}/P{sub T}) = A{sub G} + {Omega}(P{sub 0} - P{sub T}), where P{sub T} is the transmitted power, A{sub G} is the absorbance of the ground state and {Omega} is a constant depending on the absorption cross-section and the relaxation time. The values of A{sub G} and {Omega} estimated from the fits to the measured data vary with T{sub L}. The findings resulting from this investigation might have potential applications in optical sensors protection.

  18. Analysis of Nonlinear Periodic and Aperiodic Media: Application to Optical Logic Gates

    Science.gov (United States)

    Yu, Yisheng

    This dissertation is about the analysis of nonlinear periodic and aperiodic media and their application to the design of intensity controlled all optical logic gates: AND, OR, and NOT. A coupled nonlinear differential equation that characterizes the electromagnetic wave propagation in a nonlinear periodic (and aperiodic) medium has been derived from the first principle. The equations are general enough that it reflects the effect of transverse modal fields and can be used to analyze both co-propagating and counter propagating waves. A numerical technique based on the finite differences method and absorbing boundary condition has been developed to solve the coupled differential equations here. The numerical method is simple and accurate. Unlike the method based on characteristics that has been reported in the literature, this method does not involve integration and step sizes of time and space coordinates are decoupled. The decoupling provides independent choice for time and space step sizes. The concept of "gap soliton" has also been re-examined. The dissertation consists of four manuscripts. Manuscript I reports on the design of all optical logic gates: AND, OR, and NOT based on the bistability property of nonlinear periodic and aperiodic waveguiding structures. The functioning of the logic gates has been shown by analysis. The numerical technique that has been developed to solve the nonlinear differential equations are addressed in manuscript II. The effect of transverse modal fields on the bistable property of nonlinear periodic medium is reported in manuscript III. The concept of "gap soliton" that are generated in a nonlinear periodic medium has been re-examined. The details on the finding of the re-examination are discussed in manuscript IV.

  19. Nonclassical properties of a contradirectional nonlinear optical coupler

    Energy Technology Data Exchange (ETDEWEB)

    Thapliyal, Kishore [Jaypee Institute of Information Technology, A-10, Sector-62, Noida, UP-201307 (India); Pathak, Anirban, E-mail: anirban.pathak@gmail.com [Jaypee Institute of Information Technology, A-10, Sector-62, Noida, UP-201307 (India); RCPTM, Joint Laboratory of Optics of Palacky University and Institute of Physics of Academy of Science of the Czech Republic, Faculty of Science, Palacky University, 17. listopadu 12, 771 46 Olomouc (Czech Republic); Sen, Biswajit [Department of Physics, Vidyasagar Teachers' Training College, Midnapore 721101 (India); Perřina, Jan [RCPTM, Joint Laboratory of Optics of Palacky University and Institute of Physics of Academy of Science of the Czech Republic, Faculty of Science, Palacky University, 17. listopadu 12, 771 46 Olomouc (Czech Republic); Department of Optics, Palacky University, 17. listopadu 12, 771 46 Olomouc (Czech Republic)

    2014-10-24

    We investigate the nonclassical properties of output fields propagated through a contradirectional asymmetric nonlinear optical coupler consisting of a linear waveguide and a nonlinear (quadratic) waveguide operated by second harmonic generation. In contrast to the earlier results, all the initial fields are considered weak and a completely quantum-mechanical model is used here to describe the system. Perturbative solutions of Heisenberg's equations of motion for various field modes are obtained using Sen–Mandal technique. Obtained solutions are subsequently used to show the existence of single-mode and intermodal squeezing, single-mode and intermodal antibunching, two-mode and multi-mode entanglement in the output of contradirectional asymmetric nonlinear optical coupler. Further, existence of higher order nonclassicality is also established by showing the existence of higher order antibunching, higher order squeezing and higher order entanglement. Variation of observed nonclassical characters with different coupling constants and phase mismatch is discussed. - Highlights: • Nonclassicalities in fields propagating through a directional coupler is studied. • Completely quantum-mechanical description of the coupler is provided. • Analytic solutions of Heisenberg equations of motion for various modes are obtained. • Existence of lower order and higher order entanglement is shown. • Variation of nonclassicalities with phase-mismatch and coupling constants is studied.

  20. Time-resolved analysis of nonlinear optical limiting for laser synthesized carbon nanoparticles

    Science.gov (United States)

    Chen, G. X.; Hong, M. H.

    2010-11-01

    Nonlinear optical limiting materials have attracted much research interest in recent years. Carbon nanoparticles suspended in liquids show a strong nonlinear optical limiting function. It is important to investigate the nonlinear optical limiting process of carbon nanoparticles for further improving their nonlinear optical limiting performance. In this study, carbon nanoparticles were prepared by laser ablation of a carbon target in tetrahydrofuran (THF). Optical limiting properties of the samples were studied with 532-nm laser light, which is in the most sensitive wavelength band for human eyes. The shape of the laser pulse plays an important role for initializing the nonlinear optical limiting effect. Time-resolved analysis of laser pulses discovered 3 fluence stages of optical limiting. Theoretical simulation indicates that the optical limiting is initialized by a near-field optical enhancement effect.

  1. PREFACE: Ultrafast and nonlinear optics in carbon nanomaterials

    Science.gov (United States)

    Kono, Junichiro

    2013-02-01

    Carbon-based nanomaterials—single-wall carbon nanotubes (SWCNTs) and graphene, in particular—have emerged in the last decade as novel low-dimensional systems with extraordinary properties. Because they are direct-bandgap systems, SWCNTs are one of the leading candidates to unify electronic and optical functions in nanoscale circuitry; their diameter-dependent bandgaps can be utilized for multi-wavelength devices. Graphene's ultrahigh carrier mobilities are promising for high-frequency electronic devices, while, at the same time, it is predicted to have ideal properties for terahertz generation and detection due to its unique zero-gap, zero-mass band structure. There have been a large number of basic optical studies on these materials, but most of them were performed in the weak-excitation, quasi-equilibrium regime. In order to probe and assess their performance characteristics as optoelectronic materials under device-operating conditions, it is crucial to strongly drive them and examine their optical properties in highly non-equilibrium situations and with ultrashot time resolution. In this section, the reader will find the latest results in this rapidly growing field of research. We have assembled contributions from some of the leading experts in ultrafast and nonlinear optical spectroscopy of carbon-based nanomaterials. Specific topics featured include: thermalization, cooling, and recombination dynamics of photo-generated carriers; stimulated emission, gain, and amplification; ultrafast photoluminescence; coherent phonon dynamics; exciton-phonon and exciton-plasmon interactions; exciton-exciton annihilation and Auger processes; spontaneous and stimulated emission of terahertz radiation; four-wave mixing and harmonic generation; ultrafast photocurrents; the AC Stark and Franz-Keldysh effects; and non-perturbative light-mater coupling. We would like to express our sincere thanks to those who contributed their latest results to this special section, and the

  2. Efficient control of ultrafast optical nonlinearity of reduced graphene oxide by infrared reduction

    Energy Technology Data Exchange (ETDEWEB)

    Bhattachraya, S.; Maiti, R.; Das, A. C.; Saha, S.; Mondal, S.; Ray, S. K.; Bhaktha, S. N. B.; Datta, P. K., E-mail: pkdatta.iitkgp@gmail.com [Department of Physics, Indian Institute of Technology Kharagpur, Kharagpur 721302 (India)

    2016-07-07

    Simultaneous occurrence of saturable absorption nonlinearity and two-photon absorption nonlinearity in the same medium is well sought for the devices like optical limiter and laser mode-locker. Pristine graphene sheet consisting entirely of sp{sup 2}-hybridized carbon atoms has already been identified having large optical nonlinearity. However, graphene oxide (GO), a precursor of graphene having both sp{sup 2} and sp{sup 3}-hybridized carbon atom, is increasingly attracting cross-discipline researchers for its controllable properties by reduction of oxygen containing groups. In this work, GO has been prepared by modified Hummers method, and it has been further reduced by infrared (IR) radiation. Characterization of reduced graphene oxide (RGO) by means of Raman spectroscopy, X-ray photoelectron spectroscopy, and UV-Visible absorption measurements confirms an efficient reduction with infrared radiation. Here, we report precise control of non-linear optical properties of RGO in femtosecond regime with increased degrees of IR reduction measured by open aperture z-scan technique. Depending on the intensity, both saturable absorption and two-photon absorption effects are found to contribute to the non-linearity of all the samples. Saturation dominates at low intensity (∼127 GW/cm{sup 2}) while two-photon absorption becomes prominent at higher intensities (from 217 GW/cm{sup 2} to 302 GW/cm{sup 2}). The values of two-photon absorption co-efficient (∼0.0022–0.0037 cm/GW for GO, and ∼0.0128–0.0143 cm/GW for RGO) and the saturation intensity (∼57 GW/cm{sup 2} for GO, and ∼194 GW/cm{sup 2} for RGO) increase with increasing reduction, indicating GO and RGO as novel tunable photonic devices. We have also explained the reason of tunable nonlinear optical properties by using amorphous carbon model.

  3. Efficient control of ultrafast optical nonlinearity of reduced graphene oxide by infrared reduction

    International Nuclear Information System (INIS)

    Bhattachraya, S.; Maiti, R.; Das, A. C.; Saha, S.; Mondal, S.; Ray, S. K.; Bhaktha, S. N. B.; Datta, P. K.

    2016-01-01

    Simultaneous occurrence of saturable absorption nonlinearity and two-photon absorption nonlinearity in the same medium is well sought for the devices like optical limiter and laser mode-locker. Pristine graphene sheet consisting entirely of sp"2-hybridized carbon atoms has already been identified having large optical nonlinearity. However, graphene oxide (GO), a precursor of graphene having both sp"2 and sp"3-hybridized carbon atom, is increasingly attracting cross-discipline researchers for its controllable properties by reduction of oxygen containing groups. In this work, GO has been prepared by modified Hummers method, and it has been further reduced by infrared (IR) radiation. Characterization of reduced graphene oxide (RGO) by means of Raman spectroscopy, X-ray photoelectron spectroscopy, and UV-Visible absorption measurements confirms an efficient reduction with infrared radiation. Here, we report precise control of non-linear optical properties of RGO in femtosecond regime with increased degrees of IR reduction measured by open aperture z-scan technique. Depending on the intensity, both saturable absorption and two-photon absorption effects are found to contribute to the non-linearity of all the samples. Saturation dominates at low intensity (∼127 GW/cm"2) while two-photon absorption becomes prominent at higher intensities (from 217 GW/cm"2 to 302 GW/cm"2). The values of two-photon absorption co-efficient (∼0.0022–0.0037 cm/GW for GO, and ∼0.0128–0.0143 cm/GW for RGO) and the saturation intensity (∼57 GW/cm"2 for GO, and ∼194 GW/cm"2 for RGO) increase with increasing reduction, indicating GO and RGO as novel tunable photonic devices. We have also explained the reason of tunable nonlinear optical properties by using amorphous carbon model.

  4. Theoretical analysis of open aperture reflection Z-scan on materials with high-order optical nonlinearities

    International Nuclear Information System (INIS)

    Petris, Adrian I.; Vlad, Valentin I.

    2010-03-01

    We present a theoretical analysis of open aperture reflection Z-scan in nonlinear media with third-, fifth-, and higher-order nonlinearities. A general analytical expression for the normalized reflectance when third-, fifth- and higher-order optical nonlinearities are excited is derived and its consequences on RZ-scan in media with high-order nonlinearities are discussed. We show that by performing RZ-scan experiments at different incident intensities it is possible to put in evidence the excitation of different order nonlinearities in the medium. Their contributions to the overall nonlinear response can be discriminated by using formulas derived by us. A RZ-scan numerical simulation using these formulas and data taken from literature, measured by another method for the third-, fifth-, and seventh-order nonlinear refractive indices of As 2 S 3 chalcogenide glass, is performed. (author)

  5. Nonlinear optical properties of colloidal silver nanoparticles produced by laser ablation in liquids

    International Nuclear Information System (INIS)

    Karavanskii, V A; Krasovskii, V I; Ivanchenko, P V; Simakin, Aleksandr V

    2004-01-01

    The optical and nonlinear optical properties of colloidal solutions of silver obtained by laser ablation in water and ethanol are studied. It is shown that freshly prepared colloids experience a full or partial sedimentation by changing their nonlinear optical properties. Aqueous colloids undergo a partial sedimentation and their nonlinear optical absorption changes to nonlinear optical transmission. The obtained results are interpreted using the Drude model for metal particles taking the particle size into account and can be explained by the sedimentation of larger silver particles accompanied by the formation of a stable colloid containing silver nanoparticles with a tentatively silver oxide shell. The characteristic size of particles forming such a stable colloid is determined and its optical nonlinearity is estimated. (nonlinear optical phenomena)

  6. A Versatile Nonlinear Method for Predictive Modeling

    Science.gov (United States)

    Liou, Meng-Sing; Yao, Weigang

    2015-01-01

    As computational fluid dynamics techniques and tools become widely accepted for realworld practice today, it is intriguing to ask: what areas can it be utilized to its potential in the future. Some promising areas include design optimization and exploration of fluid dynamics phenomena (the concept of numerical wind tunnel), in which both have the common feature where some parameters are varied repeatedly and the computation can be costly. We are especially interested in the need for an accurate and efficient approach for handling these applications: (1) capturing complex nonlinear dynamics inherent in a system under consideration and (2) versatility (robustness) to encompass a range of parametric variations. In our previous paper, we proposed to use first-order Taylor expansion collected at numerous sampling points along a trajectory and assembled together via nonlinear weighting functions. The validity and performance of this approach was demonstrated for a number of problems with a vastly different input functions. In this study, we are especially interested in enhancing the method's accuracy; we extend it to include the second-orer Taylor expansion, which however requires a complicated evaluation of Hessian matrices for a system of equations, like in fluid dynamics. We propose a method to avoid these Hessian matrices, while maintaining the accuracy. Results based on the method are presented to confirm its validity.

  7. Assessment of fibrotic liver disease with multimodal nonlinear optical microscopy

    Science.gov (United States)

    Lu, Fake; Zheng, Wei; Tai, Dean C. S.; Lin, Jian; Yu, Hanry; Huang, Zhiwei

    2010-02-01

    Liver fibrosis is the excessive accumulation of extracellular matrix proteins such as collagens, which may result in cirrhosis, liver failure, and portal hypertension. In this study, we apply a multimodal nonlinear optical microscopy platform developed to investigate the fibrotic liver diseases in rat models established by performing bile duct ligation (BDL) surgery. The three nonlinear microscopy imaging modalities are implemented on the same sectioned tissues of diseased model sequentially: i.e., second harmonic generation (SHG) imaging quantifies the contents of the collagens, the two-photon excitation fluorescence (TPEF) imaging reveals the morphology of hepatic cells, while coherent anti-Stokes Raman scattering (CARS) imaging maps the distributions of fats or lipids quantitatively across the tissue. Our imaging results show that during the development of liver fibrosis (collagens) in BDL model, fatty liver disease also occurs. The aggregated concentrations of collagen and fat constituents in liver fibrosis model show a certain correlationship between each other.

  8. Higher-order modulation instability in nonlinear fiber optics.

    Science.gov (United States)

    Erkintalo, Miro; Hammani, Kamal; Kibler, Bertrand; Finot, Christophe; Akhmediev, Nail; Dudley, John M; Genty, Goëry

    2011-12-16

    We report theoretical, numerical, and experimental studies of higher-order modulation instability in the focusing nonlinear Schrödinger equation. This higher-order instability arises from the nonlinear superposition of elementary instabilities, associated with initial single breather evolution followed by a regime of complex, yet deterministic, pulse splitting. We analytically describe the process using the Darboux transformation and compare with experiments in optical fiber. We show how a suitably low frequency modulation on a continuous wave field induces higher-order modulation instability splitting with the pulse characteristics at different phases of evolution related by a simple scaling relationship. We anticipate that similar processes are likely to be observed in many other systems including plasmas, Bose-Einstein condensates, and deep water waves. © 2011 American Physical Society

  9. Coherent Femtosecond Spectroscopy and Nonlinear Optical Imaging on the Nanoscale

    Science.gov (United States)

    Kravtsov, Vasily

    Optical properties of many materials and macroscopic systems are defined by ultrafast dynamics of electronic, vibrational, and spin excitations localized on the nanoscale. Harnessing these excitations for material engineering, optical computing, and control of chemical reactions has been a long-standing goal in science and technology. However, it is challenging due to the lack of spectroscopic techniques that can resolve processes simultaneously on the nanometer spatial and femtosecond temporal scales. This thesis describes the fundamental principles, implementation, and experimental demonstration of a novel type of ultrafast microscopy based on the concept of adiabatic plasmonic nanofocusing. Simultaneous spatio-temporal resolution on a nanometer-femtosecond scale is achieved by using a near-field nonlinear optical response induced by ultrafast surface plasmon polaritons nanofocused on a metal tip. First, we study the surface plasmon response in metallic structures and evaluate its prospects and limitations for ultrafast near-field microscopy. Through plasmon emission-based spectroscopy, we investigate dephasing times and interplay between radiative and non-radiative decay rates of localized plasmons and their modification due to coupling. We identify a new regime of quantum plasmonic coupling, which limits the achievable spatial resolution to several angstroms but at the same time provides a potential channel for generating ultrafast electron currents at optical frequencies. Next, we study propagation of femtosecond wavepackets of surface plasmon polaritons on a metal tip. In time-domain interferometric measurements we detect group delays that correspond to slowing of the plasmon polaritons down to 20% of the speed of light at the tip apex. This provides direct experimental verification of the plasmonic nanofocusing mechanism and suggests enhanced nonlinear optical interactions at the tip apex. We then measure a plasmon-generated third-order nonlinear optical

  10. Method and apparatus of highly linear optical modulation

    Science.gov (United States)

    DeRose, Christopher; Watts, Michael R.

    2016-05-03

    In a new optical intensity modulator, a nonlinear change in refractive index is used to balance the nonlinearities in the optical transfer function in a way that leads to highly linear optical intensity modulation.

  11. Fractals: Giant impurity nonlinearities in optics of fractal clusters

    International Nuclear Information System (INIS)

    Butenko, A.V.; Shalaev, V.M.; Stockman, M.I.

    1988-01-01

    A theory of nonlinear optical properties of fractals is developed. Giant enhancement of optical susceptibilities is predicted for impurities bound to a fractal. This enhancement occurs if the exciting radiation frequency lies within the absorption band of the fractal. The giant optical nonlinearities are due to existence of high local electric fields in the sites of impurity locations. Such fields are due to the inhomogeneously broadened character of a fractal spectrum, i.e. partial conservation of individuality of fractal-forming particles (monomers). The field enhancement is proportional to the Q-factor of the resonance of a monomer. The effects of coherent anti-Stokes Raman scattering (CARS) and phase conjugation (PC) of light waves are enhanced to a much greater degree than generation of higher harmonics. In a general case the susceptibility of a higher-order is enhanced in the maximum way if the process includes ''subtraction'' of photons (at least one of the strong field frequencies enters the susceptibility with the minus sign). Alternatively, enhancement for the highest-order harmonic generation (when all the photons are ''accumulated'') is minimal. The predicted phenomena bear information on spectral properties of both impurity molecules and a fractal. In particular, in the CARS spectra a narrow (with the natural width) resonant structure, which is proper to an isolated monomer of a fractal, is predicted to be observed. (orig.)

  12. On Madelung systems in nonlinear optics: A reciprocal invariance

    Science.gov (United States)

    Rogers, Colin; Malomed, Boris

    2018-05-01

    The role of the de Broglie-Bohm potential, originally established as central to Bohmian quantum mechanics, is examined for two canonical Madelung systems in nonlinear optics. In a seminal case, a Madelung system derived by Wagner et al. via the paraxial approximation and in which the de Broglie-Bohm potential is present is shown to admit a multi-parameter class of what are here introduced as "q-gaussons." In the limit, as the Tsallis parameter q → 1, the q-gaussons are shown to lead to standard gausson solitons, as admitted by the logarithmic nonlinear Schrödinger equation encapsulating the Madelung system. The q-gaussons are obtained for optical media with dual power-law refractive index. In the second case, a Madelung system originally derived via an eikonal approximation in the context of laser beam propagation and in which the de Broglie Bohm term is neglected is shown to admit invariance under a novel class of two-parameter class of reciprocal transformations. Model optical laws analogous to the celebrated Kármán-Tsien law of classical gas dynamics are introduced.

  13. Progress Toward Single-Photon-Level Nonlinear Optics in Crystalline Microcavities

    Science.gov (United States)

    Kowligy, Abijith S.

    Over the last two decades, the emergence of quantum information science has uncovered many practical applications in areas such as communications, imaging, and sensing where harnessing quantum features of Nature provides tremendous benefits over existing methods exploiting classical physical phenomena. In this effort, one of the frontiers of research has been to identify and utilize quantum phenomena that are not susceptible to environmental and parasitic noise processes. Quantum photonics has been at the forefront of these studies because it allows room-temperature access to its inherently quantum-mechanical features, and allows leveraging the mature telecommunication industry. Accompanying the weak environmental influence, however, are also weak optical nonlinearities. Efficient nonlinear optical interactions are indispensible for many of the existing protocols for quantum optical computation and communication, e.g. high-fidelity entangling quantum logic gates rely on large nonlinear responses at the one- or few-photon-level. While this has been addressed to a great extent by interfacing photons with single quantum emitters and cold atomic gases, scalability has remained elusive. In this work, we identify the macroscopic second-order nonlinear polarization as a robust platform to address this challenge, and utilize the recent advances in the burgeoning field of optical microcavities to enhance this nonlinear response. In particular, we show theoretically that by using the quantum Zeno effect, low-noise, single-photon-level optical nonlinearities can be realized in lithium niobate whispering-gallery-mode microcavities, and present experimental progress toward this goal. Using the measured strength of the second-order nonlinear response in lithium niobate, we modeled the nonlinear system in the strong coupling regime using the Schrodinger picture framework and theoretically demonstrated that the single-photon-level operation can be observed for cavity lifetimes in

  14. Numerical nonlinear complex geometrical optics algorithm for the 3D Calderón problem

    DEFF Research Database (Denmark)

    Delbary, Fabrice; Knudsen, Kim

    2014-01-01

    to the generalized Laplace equation. The 3D problem was solved in theory in late 1980s using complex geometrical optics solutions and a scattering transform. Several approximations to the reconstruction method have been suggested and implemented numerically in the literature, but here, for the first time, a complete...... computer implementation of the full nonlinear algorithm is given. First a boundary integral equation is solved by a Nystrom method for the traces of the complex geometrical optics solutions, second the scattering transform is computed and inverted using fast Fourier transform, and finally a boundary value...

  15. Nonlinear Optical Properties of Aluminum Doped Zinc Oxide

    Science.gov (United States)

    Otieno, Calford O.

    Nonlinear optical (NLO) materials are crucial to future progress in industrial and technological applications that involve intense light-matter interaction. While ZnO-related materials are known to possess good NLO properties, existing results on ZnO and AZO (Al-doped ZnO) are mostly available at a single wavelength or limited ranges. Therefore, NLO dispersions (wavelength dependences) are not entirely studied, especially at longer wavelengths far below the bandgap. It is important to explore wavelength dependences since doping can induce a drastic change in the NLO responses at varied spectral ranges via doping-induced subgap-state contributions. We present results of our studies on nonlinear harmonic generation from our samples, which include 1) second harmonic generation and 2) third harmonic generation precisely characterized by Maker fringes as a function of both Al doping and wavelength. We exhaustively discuss the possible cause for the modified optical nonlinearities observed in our AZO thin films and give detailed comparisons of our observations with the previous studies. We also present the results of open- and close-aperture Z-scans to characterize the two-photon absorption coefficient (TPA) and the nonlinear refractive index (NLR), respectively, of the AZO films. There was no clearcut evidence of monotonic dependence of TPA and NLR on doping. This presumably indicates that the overall effect is nontrivial and should be understood in terms of combined effects of bandgap shift and crystallinity upon varying the doping level. Most intriguingly, we found that NLR values from the closed-aperture Z-scan are very large by orders of magnitude when compared with the bulk counterparts. Similar observation was made for TPA values from the open-aperture Z-scan. To countercheck very large NLO absorption, we conducted simple intensity scan by varying the incident photon number on each sample but fixing the beam area to eliminate any possible errors related to optical

  16. Nonlinear Conservation Laws and Finite Volume Methods

    Science.gov (United States)

    Leveque, Randall J.

    Introduction Software Notation Classification of Differential Equations Derivation of Conservation Laws The Euler Equations of Gas Dynamics Dissipative Fluxes Source Terms Radiative Transfer and Isothermal Equations Multi-dimensional Conservation Laws The Shock Tube Problem Mathematical Theory of Hyperbolic Systems Scalar Equations Linear Hyperbolic Systems Nonlinear Systems The Riemann Problem for the Euler Equations Numerical Methods in One Dimension Finite Difference Theory Finite Volume Methods Importance of Conservation Form - Incorrect Shock Speeds Numerical Flux Functions Godunov's Method Approximate Riemann Solvers High-Resolution Methods Other Approaches Boundary Conditions Source Terms and Fractional Steps Unsplit Methods Fractional Step Methods General Formulation of Fractional Step Methods Stiff Source Terms Quasi-stationary Flow and Gravity Multi-dimensional Problems Dimensional Splitting Multi-dimensional Finite Volume Methods Grids and Adaptive Refinement Computational Difficulties Low-Density Flows Discrete Shocks and Viscous Profiles Start-Up Errors Wall Heating Slow-Moving Shocks Grid Orientation Effects Grid-Aligned Shocks Magnetohydrodynamics The MHD Equations One-Dimensional MHD Solving the Riemann Problem Nonstrict Hyperbolicity Stiffness The Divergence of B Riemann Problems in Multi-dimensional MHD Staggered Grids The 8-Wave Riemann Solver Relativistic Hydrodynamics Conservation Laws in Spacetime The Continuity Equation The 4-Momentum of a Particle The Stress-Energy Tensor Finite Volume Methods Multi-dimensional Relativistic Flow Gravitation and General Relativity References

  17. Z-scan: A simple technique for determination of third-order optical nonlinearity

    Energy Technology Data Exchange (ETDEWEB)

    Singh, Vijender, E-mail: chahal-gju@rediffmail.com [Department of Applied Science, N.C. College of Engineering, Israna, Panipat-132107, Haryana (India); Aghamkar, Praveen, E-mail: p-aghamkar@yahoo.co.in [Department of Physics, Chaudhary Devi Lal University, Sirsa-125055, Haryana (India)

    2015-08-28

    Z-scan is a simple experimental technique to measure intensity dependent nonlinear susceptibilities of third-order nonlinear optical materials. This technique is used to measure the sign and magnitude of both real and imaginary part of the third order nonlinear susceptibility (χ{sup (3)}) of nonlinear optical materials. In this paper, we investigate third-order nonlinear optical properties of Ag-polymer composite film by using single beam z-scan technique with Q-switched, frequency doubled Nd: YAG laser (λ=532 nm) at 5 ns pulse. The values of nonlinear absorption coefficient (β), nonlinear refractive index (n{sub 2}) and third-order nonlinear optical susceptibility (χ{sup (3)}) of permethylazine were found to be 9.64 × 10{sup −7} cm/W, 8.55 × 10{sup −12} cm{sup 2}/W and 5.48 × 10{sup −10} esu, respectively.

  18. Nonlinear polarization effects in a birefringent single mode optical fiber

    International Nuclear Information System (INIS)

    Ishiekwene, G.C.; Mensah, S.Y.; Brown, C.S.

    2001-04-01

    The nonlinear polarization effects in a birefringent single mode optical fiber is studied using Jacobi elliptic functions. We find that the polarization state of the propagating beam depends on the initial polarization as well as the intensity of the input light in a complicated way. The Stokes polarization parameters are either periodic or aperiodic depending on the value of the Jacobian modulus. Our calculations suggest that the effective beat length of the fiber can become infinite at a higher critical value of the input power when polarization dependent losses are considered. (author)

  19. Structure/property relationships in non-linear optical materials

    Energy Technology Data Exchange (ETDEWEB)

    Cole, J M [Institut Max von Laue - Paul Langevin (ILL), 38 - Grenoble (France); [Durham Univ. (United Kingdom); Howard, J A.K. [Durham Univ. (United Kingdom); McIntyre, G J [Institut Max von Laue - Paul Langevin (ILL), 38 - Grenoble (France)

    1997-04-01

    The application of neutrons to the study of structure/property relationships in organic non-linear optical materials (NLOs) is described. In particular, charge-transfer effects and intermolecular interactions are investigated. Charge-transfer effects are studied by charge-density analysis and an example of one such investigation is given. The study of intermolecular interactions concentrates on the effects of hydrogen-bonding and an example is given of two structurally similar molecules with very disparate NLO properties, as a result of different types of hydrogen-bonding. (author). 3 refs.

  20. Dispersive shock waves in nonlinear and atomic optics

    Directory of Open Access Journals (Sweden)

    Kamchatnov Anatoly

    2017-01-01

    Full Text Available A brief review is given of dispersive shock waves observed in nonlinear optics and dynamics of Bose-Einstein condensates. The theory of dispersive shock waves is developed on the basis of Whitham modulation theory for various situations taking place in these two fields. In particular, the full classification is established for types of wave structures evolving from initial discontinuities for propagation of long light pulses in fibers with account of steepening effect and for dynamics of the polarization mode in two-component Bose-Einstein condensates.

  1. Superradiance Effects in the Linear and Nonlinear Optical Response of Quantum Dot Molecules

    Science.gov (United States)

    Sitek, A.; Machnikowski, P.

    2008-11-01

    We calculate the linear optical response from a single quantum dot molecule and the nonlinear, four-wave-mixing response from an inhomogeneously broadened ensemble of such molecules. We show that both optical signals are affected by the coupling-dependent superradiance effect and by optical interference between the two polarizations. As a result, the linear and nonlinear responses are not identical.

  2. Integrated all optical transmodulator circuits with non-linear gain elements and tunable optical fibers

    NARCIS (Netherlands)

    Kuindersma, P.I.; Leijtens, X.J.M.; Zantvoort, van J.H.C.; Waardt, de H.

    2012-01-01

    We characterize integrated InP circuits for high speed ‘all-optical’ signal processing. Single chip circuits act as optical transistors. Transmodulation is performed by non-linear gain sections. Integrated tunable filters give signal equalization in time domain.

  3. Ab initio studies on the optical effects in the deep ultraviolet nonlinear optical crystals of the KBe2BO3F2 family

    International Nuclear Information System (INIS)

    Kang Lei; Luo Siyang; Huang Hongwei; Lin, Z S; Chen, C T; Zheng Tao

    2012-01-01

    Electronic structures of the deep ultraviolet nonlinear optical crystals of the KBe 2 BO 3 F 2 (KBBF) family, including KBBF, RbBe 2 BO 3 F 2 and CsBe 2 BO 3 F 2 , have been investigated based on a plane-wave pseudopotential method. Their linear and nonlinear optical coefficients are also calculated, and are in good agreement with the experimental results. A real-space atom-cutting method is adopted to analyze the respective contributions of the alkali metal cations and anionic groups to optical response. The results show that the contributions of anionic groups to the nonlinear optical anisotropic responses are dominant, but the influence of the A-site alkali metal cations becomes slightly more pronounced with the increase of their radius. Moreover, the birefringence difference among these crystals strongly depends on the volume effect, i.e., the spatial density of the (BO 3 ) 3- anionic groups. (paper)

  4. Nonlinear optical response of some Graphene oxide and Graphene fluoride derivatives

    OpenAIRE

    Liaros Nikolaos; Orfanos Ioannis; Papadakis Ioannis; Couris Stelios

    2016-01-01

    The nonlinear optical properties of two graphene derivatives, graphene oxide and graphene fluoride, are investigated by means of the Z-scan technique employing 35 ps and 4 ns, visible (532 nm) laser excitation. Both derivatives were found to exhibit significant third-order nonlinear optical response at both excitation regimes, with the nonlinear absorption being relatively stronger and concealing the presence of nonlinear refraction under ns excitation, while ps excita...

  5. First International Conference on Organic Nonlinear Optics. Section B: Nonlinear Optics, Principles, Materials, Phenomena, and Devices.

    Science.gov (United States)

    1994-01-01

    HOSOTTE: Alignement and Orientation of Chromophores by Optical Pumping 327 CELINE FIORINI, FABRICE CHARRA, JEAN-MICHEL NUNZI and PAUL RAIMOND...Normandin, R. L. Williams and M. Dion , Electron. Lett., 28, 1540 (1992). 6. D. Vakhshoori and S. Wang, Appl. Phys. Lett., 53, 347 (1988). 7. D. Vakhshoori, J

  6. Molecular studies and plastic optical fiber device structures for nonlinear optical applications

    Science.gov (United States)

    Dirk, Carl W.; Nagarur, Aruna R.; Lu, Jin J.; Zhang, Lixia; Kalamegham, Priya; Fonseca, Joe; Gopalan, Saytha; Townsend, Scott; Gonzalez, Gabriel; Craig, Patrick; Rosales, Monica; Green, Leslie; Chan, Karen; Twieg, Robert J.; Ermer, Susan P.; Leung, Doris S.; Lovejoy, Steven M.; Lacroix, Suzanne; Godbout, Nicolas; Monette, Etienne

    1995-10-01

    Summarized are two project areas: First, the development of a quantitative structure property relationship for analyzing thermal decomposition differential scanning calorimetry data of electro-optic dyes is presented. The QSPR relationship suggest that thermal decomposition can be effectively correlated with structure by considering the kinds of atoms, their hybridization, and their nearest neighbor bonded atoms. Second, the simple preparation of clad plastic optical fibers (POF) is discussed with the intention of use for nonlinear optical applications. We discuss preparation techniques for single core and multiple core POF, and present some recent data on index profiles and the optimization of thermal stability in acrylate-based POF structures.

  7. Growth, spectral, linear and nonlinear optical characteristics of an efficient semiorganic acentric crystal: L-valinium L-valine chloride

    Energy Technology Data Exchange (ETDEWEB)

    Nageshwari, M.; Jayaprakash, P.; Kumari, C. Rathika Thaya [PG & Research Department of Physics, Arignar Anna Govt. Arts College, Cheyyar 604407, Tamil Nadu (India); Vinitha, G. [Department of Physics, School of Advanced Sciences, VIT Chennai, 600127 Tamil Nadu (India); Caroline, M. Lydia, E-mail: lydiacaroline2006@yahoo.co.in [PG & Research Department of Physics, Arignar Anna Govt. Arts College, Cheyyar 604407, Tamil Nadu (India)

    2017-04-15

    An efficient nonlinear optical semiorganic material L-valinium L-valine chloride (LVVCl) was synthesized and grown-up by means of slow evaporation process. Single crystal XRD evince that LVVCl corresponds to monoclinic system having acentric space group P2{sub 1}. The diverse functional groups existing in LVVCl were discovered with FTIR spectral investigation. The UV-Visible and photoluminescence spectrum discloses the optical and electronic properties respectively for the grown crystal. Several optical properties specifically extinction coefficient, reflectance, linear refractive index, electrical and optical conductivity were also determined. The SEM analysis was also carried out and it portrayed the surface morphology of LVVCl. The calculated value of laser damage threshold was 2.59 GW/cm{sup 2}. The mechanical and dielectric property of LVVCl was investigated employing microhardness and dielectric studies. The second and third order nonlinear optical characteristics of LVVCl was characterized utilizing Kurtz Perry and Z scan technique respectively clearly suggest its suitability in the domain of optics and photonics. - Graphical abstract: Good quality transparent single crystals of L-valinium L-valine chloride single crystal was grown by slow evaporation technique. The grown crystals were analyzed using different instrumentation methods to check its usefulness for the device fabrication. The determination of nonlinear refractive index (n{sub 2}), absorption coefficient (β) and third order nonlinear susceptibility was determined by Z scan technique, highlighted that LVVCl can serve as a promising candidate for opto electronic and nonlinear optical applications.

  8. Nonlinear optical oscillation dynamics in high-Q lithium niobate microresonators.

    Science.gov (United States)

    Sun, Xuan; Liang, Hanxiao; Luo, Rui; Jiang, Wei C; Zhang, Xi-Cheng; Lin, Qiang

    2017-06-12

    Recent advance of lithium niobate microphotonic devices enables the exploration of intriguing nonlinear optical effects. We show complex nonlinear oscillation dynamics in high-Q lithium niobate microresonators that results from unique competition between the thermo-optic nonlinearity and the photorefractive effect, distinctive to other device systems and mechanisms ever reported. The observed phenomena are well described by our theory. This exploration helps understand the nonlinear optical behavior of high-Q lithium niobate microphotonic devices which would be crucial for future application of on-chip nonlinear lithium niobate photonics.

  9. Nonlinear optical properties of ZnO/poly (vinyl alcohol) nanocomposite films

    International Nuclear Information System (INIS)

    Jeeju, P. P.; Jayalekshmi, S.; Chandrasekharan, K.

    2014-01-01

    Extensive studies have already been reported on the optical characteristics of ZnO/polymer nanocomposite films, using a variety of polymers including transparent polymers such as polystyrene, polymethyl methacrylate etc and many interesting results have been established regarding the non linear optical characteristics of these systems. Poly (vinyl alcohol)(PVA) is a water soluble polymer. Though the structural and optical studies of ZnO/PVA nanocomposite films have already been investigated, there are no detailed reports on the nonlinear optical characteristics of ZnO/PVA nanocomposite films, irrespective of the fact that these nanocomposite films can be synthesized using quite easy and cost effective methods. The present work is an attempt to study in detail the nonlinear optical behaviour of ZnO/PVA nanocomposite films using Z-scan technique. Highly transparent ZnO/PVA nanocomposite films were prepared from the ZnO incorporated PVA solution in water using spin coating technique. The ZnO nanoparticles were synthesized by the simple chemical route at room temperature. High-resolution transmission electron microscopy studies show that the ZnO nanoparticles are of size around 10 nm. The ZnO/PVA nanocomposite films were structurally characterized by X-ray diffraction technique, from which the presence of both PVA and ZnO in the nanocomposite was established. The optical absorptive nonlinearity in the nanocomposite films was investigated using open aperture Z-scan technique. The results indicate optical limiting type nonlinearity in the films due to two photon absorption in ZnO with efficiency more than 50%. These films also show a self defocusing type negative nonlinear refraction in closed aperture Z-scan experiment. The present studies indicate that, highly transparent and homogeneous films of ZnO/PVA nanocomposite can be obtained on glass substrates using simple methods, in a highly cost effective way, since PVA is water soluble. These nanocomposite films offer

  10. Spectral dependence of nonlinear optical absorption of silica glass with copper nanoparticles

    International Nuclear Information System (INIS)

    Golubev, A N; Nikitin, S I; Smirnov, M A; Stepanov, A L

    2011-01-01

    The nonlinear optical properties of silica glass with copper nanoparticles synthesized by ion implantation were investigated by z-scan method in nanosecond time scale. The reverse saturation absorption (RSA) at the wavelength range of 450–540 nm and saturation absorption (SA) at 550–585 nm were observed. It was supposed that the two-photon electron absorption from bound of d-states determined the RSA effect and the SA is due to saturation of plasmon excitation.

  11. Nonlinear light scattering in a two component medium: optical limiting application

    International Nuclear Information System (INIS)

    Joudrier, Valerie

    1998-01-01

    Scattering is a fundamental manifestation of the interaction between matter and radiation, resulting from inhomogeneities in the refractive index, which decrease transmission. This phenomenon is then especially attractive for sensor protection from laser light by optical limiting. One of the methods to induce scattering at high incident energy is to make use of the Kerr effect where the index of refraction is intensity dependent. Thus, the idea is to use a two component medium with a good index matching between the two components at low intensity, resulting in the medium transparency, and to modify it, at high intensity, due to the non linearity of one component making the medium highly scattering. Some of the experimental and theoretical investigations concerning a new material (here, a cell containing some liquid with small silica particles as inclusion in it) are presented in the visible domain (I=532 nm), for the nanosecond protection regime, beginning, with the chemical synthesis of the sample. The experimental results concerning the optical limiting process are presented, showing that nonlinear scattering is clearly the dominant mechanism in confrontation with other potential nonlinear effects. Several complementary experiments are then performed to complete the nonlinear scattering characterization, involving the measurement of the angular distribution of scattered energy and the integrating sphere measurement. Further information are also gained by studying the time response of the nonlinearities with a dual-beam (pulsed-pump, cw probe) technique. The previous experimental data is also analyzed with some simple theoretical models to evaluate the nonlinearity of the material from optical limiting, the angular scattering and the total scattering energy measurements. The good match between all the analytical results permits to delineate the physical mechanisms responsible for the nonlinear scattering effect and to direct the final conclusion. (author) [fr

  12. Nonlinear optical spectroscopy of isotropic and anisotropic metallic nanocomposites

    Energy Technology Data Exchange (ETDEWEB)

    Fernandez-Hernandez, R C; Gleason-Villagran, R; Cheang-Wong, J C; Crespo-Sosa, A; Rodriguez-Fernandez, L; Lopez-Suarez, A; Oliver, A; Reyes-Esqueda, J A [Instituto de Fisica, Universidad Nacional Autonoma de Mexico, Mexico, D. F. 04510 (Mexico); Torres-Torres, C [Seccion de Estudios de Posgrado e Investigacion, ESIME-Zacatenco, Instituto Politecnico Nacional, Mexico, D. F. 07338 (Mexico); Rangel-Rojo, R, E-mail: reyes@fisica.unam.mx [CICESE/Depto. de Optica, A.P. 360, Ensenada, B. C. 22860 (Mexico)

    2011-01-01

    In this work, we studied the nonlinear absorption and refraction of isotropic and anisotropic metallic nanocomposites, which consist of Au and Ag nanoparticles (NPs) embedded in matrices of SiO{sub 2}. We performed this study at different wavelengths using the Z-scan technique in the picosecond regime. The wavelengths were selected accordingly to the absorption spectra of the nanocomposites, choosing wavelengths into the inter- and intra-band transitions regions, including the surface plasmon (SP) resonance, as well as in the transparent region. For the anisotropic nanocomposites, the polarization and the incident angle were varied in order to evaluate the different components of the third order susceptibility tensor, {chi}{sup (3)}. We observed dramatic changes of sign for both, nonlinear refraction and absorption, when passing from Au to Ag and/or varying the wave length. The results accentuate the importance of the hot-electrons contribution to the nonlinear optical response at this temporal regime, when compared to inter-band and intra-band transitions contributions.

  13. Nonlinear optical spectroscopy of isotropic and anisotropic metallic nanocomposites

    International Nuclear Information System (INIS)

    Fernandez-Hernandez, R C; Gleason-Villagran, R; Cheang-Wong, J C; Crespo-Sosa, A; Rodriguez-Fernandez, L; Lopez-Suarez, A; Oliver, A; Reyes-Esqueda, J A; Torres-Torres, C; Rangel-Rojo, R

    2011-01-01

    In this work, we studied the nonlinear absorption and refraction of isotropic and anisotropic metallic nanocomposites, which consist of Au and Ag nanoparticles (NPs) embedded in matrices of SiO 2 . We performed this study at different wavelengths using the Z-scan technique in the picosecond regime. The wavelengths were selected accordingly to the absorption spectra of the nanocomposites, choosing wavelengths into the inter- and intra-band transitions regions, including the surface plasmon (SP) resonance, as well as in the transparent region. For the anisotropic nanocomposites, the polarization and the incident angle were varied in order to evaluate the different components of the third order susceptibility tensor, χ (3) . We observed dramatic changes of sign for both, nonlinear refraction and absorption, when passing from Au to Ag and/or varying the wave length. The results accentuate the importance of the hot-electrons contribution to the nonlinear optical response at this temporal regime, when compared to inter-band and intra-band transitions contributions.

  14. Fabrication of Metallic Quantum Dot Arrays For Nanoscale Nonlinear Optics

    Science.gov (United States)

    McMahon, M. D.; Hmelo, A. B.; Lopez Magruder, R., III; Weller Haglund, R. A., Jr.; Feldman, L. C.

    2003-03-01

    Ordered arrays of metal nanocrystals embedded in or sequestered on dielectric hosts have potential applications as elements of nonlinear or near-field optical circuits, as sensitizers for fluorescence emitters and photo detectors, and as anchor points for arrays of biological molecules. Metal nanocrystals are strongly confined electronic systems with size-, shape and spatial orientation-dependent optical responses. At the smallest scales (below about 15 nm diameter), their band structure is drastically altered by the small size of the system, and the reduced population of conduction-band electrons. Here we report on the fabrication of two-dimensional ordered metallic nanocrystal arrays, and one-dimensional nanocrystal-loaded waveguides for optical investigations. We have employed strategies for synthesizing metal nanocrystal composites that capitalize on the best features of focused ion beam (FIB) machining and pulsed laser deposition (PLD). The FIB generates arrays of specialized sites; PLD vapor deposition results in the directed self-assembly of Ag nanoparticles nucleated at the FIB generated sites on silicon substrates. We present results based on the SEM, AFM and optical characterization of prototype composites. This research has been supported by the U.S. Department of Energy under grant DE-FG02-01ER45916.

  15. Computational Modeling of Ultrafast Pulse Propagation in Nonlinear Optical Materials

    Science.gov (United States)

    Goorjian, Peter M.; Agrawal, Govind P.; Kwak, Dochan (Technical Monitor)

    1996-01-01

    There is an emerging technology of photonic (or optoelectronic) integrated circuits (PICs or OEICs). In PICs, optical and electronic components are grown together on the same chip. rib build such devices and subsystems, one needs to model the entire chip. Accurate computer modeling of electromagnetic wave propagation in semiconductors is necessary for the successful development of PICs. More specifically, these computer codes would enable the modeling of such devices, including their subsystems, such as semiconductor lasers and semiconductor amplifiers in which there is femtosecond pulse propagation. Here, the computer simulations are made by solving the full vector, nonlinear, Maxwell's equations, coupled with the semiconductor Bloch equations, without any approximations. The carrier is retained in the description of the optical pulse, (i.e. the envelope approximation is not made in the Maxwell's equations), and the rotating wave approximation is not made in the Bloch equations. These coupled equations are solved to simulate the propagation of femtosecond optical pulses in semiconductor materials. The simulations describe the dynamics of the optical pulses, as well as the interband and intraband.

  16. Mechanism of large optical nonlinearity in gold nanoparticle films.

    Science.gov (United States)

    Mirza, I; McCloskey, D; Blau, W J; Lunney, J G

    2018-04-01

    The Z-scan technique, using femtosecond (fs) laser pulses at 1480 nm laser pulses, was used to measure the nonlinear optical properties of gold (Au) nanoparticle (NP) films made by both nanosecond (ns) and fs pulsed laser deposition (PLD) in vacuum. At irradiance levels of 1×10 12   Wm -2 , the ns-PLD films displayed induced absorption with β=4×10 -5   mW -1 , and a negative lensing effect with n 2 =-4.7×10 -11   m 2  W -1 with somewhat smaller values for the fs-PLD films. These values of n 2 imply an unphysically large change in the real part of the refractive index, demonstrating the need to take account of nonlinear changes of the Fresnel coefficients and multiple beam interference in Z-scan measurements on nanoscale films. Following this approach, the Z-scan observations were analyzed to determine the effective complex refractive index of the NP film at high irradiance. It appears that at high irradiance the NP film behaves as a metal, while at low irradiance it behaves as a low-loss dielectric. Thus, it is conjectured that, for high irradiance near the waist of the Z-scan laser beam, laser driven electron tunneling between NPs gives rise to metal-like optical behavior.

  17. Structural, spectroscopic (FT-IR, NMR, UV-visible), nonlinear optical (NLO), cytotoxic and molecular docking studies of 4-nitro-isonitrosoacetophenone (ninapH) by DFT method

    Science.gov (United States)

    Kucuk, Ilhan; Kaya, Yunus; Kaya, A. Asli

    2017-07-01

    (4-Nitro-phenyl)-oxo-acetaldehyde oxime (ninapH) is a type of oxime, which has a oxime and α-carbonyl groups. This molecule has been synthesized from literature procedure. The structural properties and conformational behaviors were examined using the density functional theory (DFT) with the B3LYP method combined with the 6-311++G(d,p) basis set. As a result of the conformational studies, the most stable conformer was determined, and then this molecule was optimized with the same basis set. Comprehensive theoretical and experimental structural studies on the molecule have been carried out by FT-IR, NMR and UV-vis spectrometry. The calculated HOMO and LUMO energies show that charge transfer within the molecule. The first order hyperpolarizability and molecular electrostatic potential (MEP) were also performed. The thermodynamic properties (heat capacity, entropy, and enthalpy) of the ninapH have been calculated at different temperatures, 100-1000 K. In addition, the molecular docking studies have been performed with DNA and protein structures (downloaded from Protein Data Bank).

  18. How nonlinear optics can merge interferometry for high resolution imaging

    Science.gov (United States)

    Ceus, D.; Reynaud, F.; Tonello, A.; Delage, L.; Grossard, L.

    2017-11-01

    High resolution stellar interferometers are very powerful efficient instruments to get a better knowledge of our Universe through the spatial coherence analysis of the light. For this purpose, the optical fields collected by each telescope Ti are mixed together. From the interferometric pattern, two expected information called the contrast Cij and the phase information φij are extracted. These information lead to the Vij, called the complex visibility, with Vij=Cijexp(jφij). For each telescope doublet TiTj, it is possible to get a complex visibility Vij. The Zernike Van Cittert theorem gives a relationship between the intensity distribution of the object observed and the complex visibility. The combination of the acquired complex visibilities and a reconstruction algorithm allows imaging reconstruction. To avoid lots of technical difficulties related to infrared optics (components transmission, thermal noises, thermal cooling…), our team proposes to explore the possibility of using nonlinear optical techniques. This is a promising alternative detection technique for detecting infrared optical signals. This way, we experimentally demonstrate that frequency conversion does not result in additional bias on the interferometric data supplied by a stellar interferometer. In this presentation, we report on wavelength conversion of the light collected by each telescope from the infrared domain to the visible. The interferometric pattern is observed in the visible domain with our, so called, upconversion interferometer. Thereby, one can benefit from mature optical components mainly used in optical telecommunications (waveguide, coupler, multiplexer…) and efficient low-noise detection schemes up to the single-photon counting level.

  19. Non-linear optics of nano-scale pentacene thin film

    Science.gov (United States)

    Yahia, I. S.; Alfaify, S.; Jilani, Asim; Abdel-wahab, M. Sh.; Al-Ghamdi, Attieh A.; Abutalib, M. M.; Al-Bassam, A.; El-Naggar, A. M.

    2016-07-01

    We have found the new ways to investigate the linear/non-linear optical properties of nanostructure pentacene thin film deposited by thermal evaporation technique. Pentacene is the key material in organic semiconductor technology. The existence of nano-structured thin film was confirmed by atomic force microscopy and X-ray diffraction. The wavelength-dependent transmittance and reflectance were calculated to observe the optical behavior of the pentacene thin film. It has been observed the anomalous dispersion at wavelength λ 800. The non-linear refractive index of the deposited films was investigated. The linear optical susceptibility of pentacene thin film was calculated, and we observed the non-linear optical susceptibility of pentacene thin film at about 6 × 10-13 esu. The advantage of this work is to use of spectroscopic method to calculate the liner and non-liner optical response of pentacene thin films rather than expensive Z-scan. The calculated optical behavior of the pentacene thin films could be used in the organic thin films base advanced optoelectronic devices such as telecommunications devices.

  20. Designing Hybrids of Graphene Oxide and Gold Nanoparticles for Nonlinear Optical Response

    Science.gov (United States)

    Yadav, Rajesh Kumar; Aneesh, J.; Sharma, Rituraj; Abhiramnath, P.; Maji, Tuhin Kumar; Omar, Ganesh Ji; Mishra, A. K.; Karmakar, Debjani; Adarsh, K. V.

    2018-04-01

    Nonlinear optical absorption of light by materials is weak due to its perturbative nature, although a strong nonlinear response is of crucial importance to applications in optical limiting and switching. Here we demonstrate experimentally and theoretically an extremely efficient scheme of excited-state absorption by charge transfer between donor and acceptor materials as a method to enhance the nonlinear absorption by orders of magnitude. With this idea, we demonstrate a strong excited-state absorption (ESA) in reduced graphene oxide that otherwise shows an increased transparency at high fluence and enhancement of ESA by one order of magnitude in graphene oxide by attaching gold nanoparticles (Au NP) in the tandem configuration that acts as an efficient charge-transfer pair when excited at the plasmonic wavelength. To explain the unprecedented enhancement, we develop a five-level rate-equation model based on the charge transfer between the two materials and numerically simulate the results. To understand the correlation of interfacial charge transfer with the concentration and type of the functional ligands attached to the graphene oxide sheet, we investigate the Au-NP—graphene oxide interface with various possible ligand configurations from first-principles calculations. By using the strong ESA of our hybrid materials, we fabricate liquid cell-based high-performance optical limiters with important device parameters better than that of the benchmark optical limiters.

  1. Convergence of hybrid methods for solving non-linear partial ...

    African Journals Online (AJOL)

    This paper is concerned with the numerical solution and convergence analysis of non-linear partial differential equations using a hybrid method. The solution technique involves discretizing the non-linear system of PDE to obtain a corresponding non-linear system of algebraic difference equations to be solved at each time ...

  2. Bifurcation methods of dynamical systems for handling nonlinear ...

    Indian Academy of Sciences (India)

    physics pp. 863–868. Bifurcation methods of dynamical systems for handling nonlinear wave equations. DAHE FENG and JIBIN LI. Center for Nonlinear Science Studies, School of Science, Kunming University of Science and Technology .... (b) It can be shown from (15) and (18) that the balance between the weak nonlinear.

  3. Differential Polarization Nonlinear Optical Microscopy with Adaptive Optics Controlled Multiplexed Beams

    Directory of Open Access Journals (Sweden)

    Virginijus Barzda

    2013-09-01

    Full Text Available Differential polarization nonlinear optical microscopy has the potential to become an indispensable tool for structural investigations of ordered biological assemblies and microcrystalline aggregates. Their microscopic organization can be probed through fast and sensitive measurements of nonlinear optical signal anisotropy, which can be achieved with microscopic spatial resolution by using time-multiplexed pulsed laser beams with perpendicular polarization orientations and photon-counting detection electronics for signal demultiplexing. In addition, deformable membrane mirrors can be used to correct for optical aberrations in the microscope and simultaneously optimize beam overlap using a genetic algorithm. The beam overlap can be achieved with better accuracy than diffraction limited point-spread function, which allows to perform polarization-resolved measurements on the pixel-by-pixel basis. We describe a newly developed differential polarization microscope and present applications of the differential microscopy technique for structural studies of collagen and cellulose. Both, second harmonic generation, and fluorescence-detected nonlinear absorption anisotropy are used in these investigations. It is shown that the orientation and structural properties of the fibers in biological tissue can be deduced and that the orientation of fluorescent molecules (Congo Red, which label the fibers, can be determined. Differential polarization microscopy sidesteps common issues such as photobleaching and sample movement. Due to tens of megahertz alternating polarization of excitation pulses fast data acquisition can be conveniently applied to measure changes in the nonlinear signal anisotropy in dynamically changing in vivo structures.

  4. Crystal growth and characterization of a semiorganic nonlinear optical single crystal of gamma glycine

    International Nuclear Information System (INIS)

    Prakash, J. Thomas Joseph; Kumararaman, S.

    2008-01-01

    Gamma glycine has been successfully synthesized by taking glycine and potassium chloride and single crystals have been grown by solvent evaporation method for the first time. The grown single crystals have been analyzed with XRD, Fourier transform infrared (FTIR), and thermo gravimetric and differential thermal analyses (TG/DTA) measurements. Its mechanical behavior has been assessed by Vickers microhardness measurements. Its nonlinear optical property has been tested by Kurtz powder technique. Its optical behavior was examined by UV-vis., and found that the crystal is transparent in the region between 240 and 1200 nm. Hence, it may be very much useful for the second harmonic generation (SHG) applications

  5. Fabrication of highly nonlinear germano-silicate glass optical fiber incorporated with PbTe semiconductor quantum dots using atomization doping process and its optical nonlinearity.

    Science.gov (United States)

    Ju, Seongmin; Watekar, Pramod R; Han, Won-Taek

    2011-01-31

    Germano-silicate glass optical fiber incorporated with PbTe semiconductor quantum dots (SQDs) in the core was fabricated by using the atomization process in modified chemical vapor deposition (MCVD) process. The absorption bands attributed to PbTe semiconductor quantum dots in the fiber core were found to appear at around 687 nm and 1055 nm. The nonlinear refractive index measured by the long-period fiber grating (LPG) pair method upon pumping with laser diode at 976.4 nm was estimated to be ~1.5 × 10(-16) m2/W.

  6. The nonlinear Schrödinger equation singular solutions and optical collapse

    CERN Document Server

    Fibich, Gadi

    2015-01-01

    This book is an interdisciplinary introduction to optical collapse of laser beams, which is modelled by singular (blow-up) solutions of the nonlinear Schrödinger equation. With great care and detail, it develops the subject including the mathematical and physical background and the history of the subject. It combines rigorous analysis, asymptotic analysis, informal arguments, numerical simulations, physical modelling, and physical experiments. It repeatedly emphasizes the relations between these approaches, and the intuition behind the results. The Nonlinear Schrödinger Equation will be useful to graduate students and researchers in applied mathematics who are interested in singular solutions of partial differential equations, nonlinear optics and nonlinear waves, and to graduate students and researchers in physics and engineering who are interested in nonlinear optics and Bose-Einstein condensates. It can be used for courses on partial differential equations, nonlinear waves, and nonlinear optics. Gadi Fib...

  7. The third-order nonlinear optical susceptibility of C{sub 60}-derived nanotubes

    Energy Technology Data Exchange (ETDEWEB)

    Xiangang, Wan [Nanjing Univ. (China). National Lab. of Solid State Microstructures; [Center for Advanced Studies in Science and Technology of Microstructures, Nanjing (China); Jinming, Dong [Nanjing Univ. (China). National Lab. of Solid State Microstructures; [Center for Advanced Studies in Science and Technology of Microstructures, Nanjing (China); Jie, Jiang [Nanjing Univ., JS (China). Dept. of Physics; Xing, D Y [Nanjing Univ., JS (China). Dept. of Physics

    1997-02-01

    Using the extended Su-Schrieffer-Heeger (SSH) model and the sum-over-state (SOS) method, we have calculated the third-order nonlinear polarizability {gamma} and its dispersion spectra for C{sub 60}-derived nanotubes, which is one of the narrowest tubes. Our numerical calculations indicate that both symmetry and size of the nanotubes have great effect on the third-order nonlinear polarizability {gamma} spectra. We find that with increasing size, both static {gamma} values and dynamical response peak values increase. When the atom number of the C{sub 60}-derived nanotubes is 140, the static {gamma} value is about 65 times larger than that of C{sub 60}, and the highest peak value of {gamma} (at 3{omega} = 3.52 eV) is about three orders larger than that of C{sub 60}. So, C{sub 60}-derived nanotubes may become a kind of good nonlinear optical materials. (orig.)

  8. Investigation on the structural and nonlinear optical properties of Pt doped TiO2 nanoparticles

    International Nuclear Information System (INIS)

    Rahulan, K. Mani; Padmanathan, N.; Vinitha, G.; Kanakam, Charles Christopher

    2013-01-01

    Graphical abstract: The open aperture Z-scan traces of Pt doped TiO 2 nanoparticles at different Pt concentrations were carried out at an irradiation wavelength of 532 nm. It was numerically found that, two photon absorption (TPA) type process gives the best fit to the obtained open aperture Z-scan data. The nonlinear transmission was found to be of third order as it fits to a two-photon absorption. The optical limiting performances of nanoparticles were greatly enhanced with increased volume ratio of Pt. Increasing particle size reduced the limiting threshold and enhanced the optical limiting performance. - Highlights: • Pt doped TiO 2 nanoparticles with different concentrations of Pt have been synthesized by sol–gel method. • The average fluorescence lifetime decreases as the volume fraction of Pt dopant increases. • The effects of Pt content on the optical limiting property were investigated by open aperture Z-scan measurements done at 532 nm using 5 ns laser pulses. • The values of the third-order nonlinearities of nanoparticles are interesting from the application point of view which could be used as a potential candidate for the application of nonlinear optical device. - Abstract: Pt doped TiO 2 nanoparticles with different concentrations of Pt were prepared by sol–gel method. X-ray diffraction (XRD) study reveals that the samples have a homogeneous anatase phase tetragonal system and the lattice parameter analysis indicates that Pt ions substitute into the lattice of TiO 2 . The addition of dopant increases the growth of TiO 2 grains, agglomerates them and shifts the absorption band of TiO 2 from ultraviolet to visible region. The incorporation of Pt in TiO 2 is also confirmed by fluorescence quenching and the fluorescence lifetime decreases as the volume fraction of Pt dopant increases. Open aperture Z-scan measurements done at 532 nm using 7 ns laser pulses show nonlinear absorption which arises from an effective two photon absorption process

  9. Third order nonlinear optical properties of a paratellurite single crystal

    Science.gov (United States)

    Duclère, J.-R.; Hayakawa, T.; Roginskii, E. M.; Smirnov, M. B.; Mirgorodsky, A.; Couderc, V.; Masson, O.; Colas, M.; Noguera, O.; Rodriguez, V.; Thomas, P.

    2018-05-01

    The (a,b) plane angular dependence of the third-order nonlinear optical susceptibility, χ(3) , of a c-cut paratellurite (α-TeO2) single crystal was quantitatively evaluated here by the Z-scan technique, using a Ti:sapphire femtosecond laser operated at 800 nm. In particular, the mean value Re( ⟨χ(3)⟩a,b )(α-TeO2) of the optical tensor has been extracted from such experiments via a direct comparison with the data collected for a fused silica reference glass plate. A R e (⟨χ(3)⟩(a,b )(α-TeO2)):R e (χ(3))(SiO2 glass) ratio roughly equal to 49.1 is found, and our result compares thus very favourably with the unique experimental value (a ratio of ˜50) reported by Kim et al. [J. Am. Ceram. Soc. 76, 2486 (1993)] for a pure TeO2 glass. In addition, it is shown that the angular dependence of the phase modulation within the (a,b) plane can be fully understood in the light of the strong dextro-rotatory power known for TeO2 materials. Taking into account the optical activity, some analytical model serving to estimate the diagonal and non-diagonal components of the third order nonlinear susceptibility tensor has been thus developed. Finally, Re( χxxxx(3) ) and Re( χxxyy(3) ) values of 95.1 ×10-22 m 2/V2 and 42.0 ×10-22 m2/V2 , respectively, are then deduced for a paratellurite single crystal, considering fused silica as a reference.

  10. Linear and nonlinear optical properties of multilayered spherical quantum dots: Effects of geometrical size, hydrogenic impurity, hydrostatic pressure and temperature

    International Nuclear Information System (INIS)

    Karimi, M.J.; Rezaei, G.; Nazari, M.

    2014-01-01

    Based on the effective mass and parabolic one band approximations, simultaneous effects of the geometrical size, hydrogenic impurity, hydrostatic pressure, and temperature on the intersubband optical absorption coefficients and refractive index changes in multilayered spherical quantum dots are studied. Energy eigenvalues and eigenvectors are calculated using the fourth-order Runge–Kutta method and optical properties are obtained using the compact density matrix approach. The results indicate that the hydrogenic impurity, hydrostatic pressure, temperature and geometrical parameters such as the well and barrier widths have a great influence on the linear, the third-order nonlinear and the total optical absorption coefficients and refractive index changes. -- Highlights: • Hydrogenic impurity effects on the optical properties of a MSQD are investigated. • Hydrostatic pressure and temperature effects are also studied. • Hydrogenic impurity has a great influence on the linear and nonlinear ACs and RICs. • Hydrostatic pressure and temperature change the linear and nonlinear ACs and RICs

  11. Matter-wave two-dimensional solitons in crossed linear and nonlinear optical lattices

    International Nuclear Information System (INIS)

    Luz, H. L. F. da; Gammal, A.; Abdullaev, F. Kh.; Salerno, M.; Tomio, Lauro

    2010-01-01

    The existence of multidimensional matter-wave solitons in a crossed optical lattice (OL) with a linear optical lattice (LOL) in the x direction and a nonlinear optical lattice (NOL) in the y direction, where the NOL can be generated by a periodic spatial modulation of the scattering length using an optically induced Feshbach resonance is demonstrated. In particular, we show that such crossed LOLs and NOLs allow for stabilizing two-dimensional solitons against decay or collapse for both attractive and repulsive interactions. The solutions for the soliton stability are investigated analytically, by using a multi-Gaussian variational approach, with the Vakhitov-Kolokolov necessary criterion for stability; and numerically, by using the relaxation method and direct numerical time integrations of the Gross-Pitaevskii equation. Very good agreement of the results corresponding to both treatments is observed.

  12. Matter-wave two-dimensional solitons in crossed linear and nonlinear optical lattices

    Science.gov (United States)

    da Luz, H. L. F.; Abdullaev, F. Kh.; Gammal, A.; Salerno, M.; Tomio, Lauro

    2010-10-01

    The existence of multidimensional matter-wave solitons in a crossed optical lattice (OL) with a linear optical lattice (LOL) in the x direction and a nonlinear optical lattice (NOL) in the y direction, where the NOL can be generated by a periodic spatial modulation of the scattering length using an optically induced Feshbach resonance is demonstrated. In particular, we show that such crossed LOLs and NOLs allow for stabilizing two-dimensional solitons against decay or collapse for both attractive and repulsive interactions. The solutions for the soliton stability are investigated analytically, by using a multi-Gaussian variational approach, with the Vakhitov-Kolokolov necessary criterion for stability; and numerically, by using the relaxation method and direct numerical time integrations of the Gross-Pitaevskii equation. Very good agreement of the results corresponding to both treatments is observed.

  13. Vibrational spectroscopic and non-linear optical activity studies on nicotinanilide : A DFT approach

    Science.gov (United States)

    Premkumar, S.; Jawahar, A.; Mathavan, T.; Dhas, M. Kumara; Benial, A. Milton Franklin

    2015-06-01

    The molecular structure of nicotinanilide was optimized by the DFT/B3LYP method with cc-pVTZ basis set using Gaussian 09 program. The first order hyperpolarizability of the molecule was calculated, which exhibits the higher nonlinear optical activity. The natural bond orbital analysis confirms the presence of intramolecular charge transfer and the hydrogen bonding interaction, which leads to the higher nonlinear optical activity of the molecule. The Frontier molecular orbitals analysis of the molecule shows that the delocalization of electron density occurs within the molecule. The lower energy gap indicates that the hydrogen bond formation between the charged species. The vibrational frequencies were calculated and assigned on the basis of potential energy distribution calculation using the VEDA 4.0 program and the corresponding vibrational spectra were simulated. Hence, the nicotinanilide molecule can be a good candidate for second-order NLO material.

  14. Measurement and control of optical nonlinearities of importance to glass laser fusion systems

    International Nuclear Information System (INIS)

    Kurnit, N.A.; Shimada, T.; Sorem, M.S.; Taylor, A.J.; Rodriguez, G.; Clement, T.S.; James, D.F.V.; Milonni, P.W.

    1996-01-01

    Results of a number of studies carried out at Los Alamos, both experimental and theoretical, of nonlinear optical phenomena important to the design of the National Ignition Facility are summarized. These include measurements of nonlinear index coefficients, Raman scattering in atmospheric oxygen, and theoretical studies of harmonic conversion. The measurements were made by two different techniques in order to increase confidence in the results. One method was an application of a recently-developed technique for measuring the amplitude and phase of an ultrashort pulse by Frequency-Resolved Optical Gating (FROG). The other utilized a modified version of the Z-scan technique that measures beam distortion introduced by scanning a sample through the focus of a beam. The measurements by both techniques for fused silica were consistent with the lower range of previously measured values, indicating that it should not be necessary to further expand the beam size in the NIF to stay below the self-focusing threshold

  15. Effects of intermode nonlinearity and intramode nonlinearity on modulation instability in randomly birefringent two-mode optical fibers

    Science.gov (United States)

    Li, Jin Hua; Xu, Hui; Sun, Ting Ting; Pei, Shi Xin; Ren, Hai Dong

    2018-05-01

    We analyze in detail the effects of the intermode nonlinearity (IEMN) and intramode nonlinearity (IRMN) on modulation instability (MI) in randomly birefringent two-mode optical fibers (RB-TMFs). In the anomalous dispersion regime, the MI gain enhances significantly as the IEMN and IRMN coefficients increases. In the normal dispersion regime, MI can be generated without the differential mode group delay (DMGD) effect, as long as the IEMN coefficient between two distinct modes is above a critical value, or the IRMN coefficient inside a mode is below a critical value. This critical IEMN (IRMN) coefficient depends strongly on the given IRMN (IEMN) coefficient and DMGD for a given nonlinear RB-TMF structure, and is independent on the input total power, the power ratio distribution and the group velocity dispersion (GVD) ratio between the two modes. On the other hand, in contrast to the MI band arising from the pure effect of DMGD in the normal dispersion regime, where MI vanishes after a critical total power, the generated MI band under the combined effects of IEMN and IRMN without DMGD exists for any total power and enhances with the total power. The MI analysis is verified numerically by launching perturbed continuous waves (CWs) with wave propagation method.

  16. Design and optimization of carbon-nanotube-material/dielectric hybrid nonlinear optical waveguides

    International Nuclear Information System (INIS)

    Zhao, Xin; Zheng, Zheng; Lu, Zhiting; Zhu, Jinsong; Zhou, Tao

    2011-01-01

    The nonlinear optical characteristics of highly nonlinear waveguides utilizing carbon nanotube composite materials are investigated theoretically. The extremely high nonlinearity and relatively high loss of the carbon nanotube materials are shown to greatly affect the performance of such waveguides for nonlinear optical applications, in contrast to waveguides using conventional nonlinear materials. Different configurations based on applying the carbon nanotube materials to the popular ridge and buried waveguides are thoroughly studied, and the optimal geometries are derived through simulations. It is shown that, though the nonlinear coefficient is often huge for these waveguides, the loss characteristics can significantly limit the maximum achievable accumulated nonlinearity, e.g. the maximum nonlinear phase shift. Our results suggest that SOI-based high-index-contrast, carbon nanotube cladding waveguides, rather than the currently demonstrated low-contrast waveguides, could hold the promise of achieving significantly higher accumulated nonlinearity

  17. Linear and Non-Linear Optical Imaging of Cancer Cells with Silicon Nanoparticles

    Science.gov (United States)

    Tolstik, Elen; Osminkina, Liubov A.; Akimov, Denis; Gongalsky, Maksim B.; Kudryavtsev, Andrew A.; Timoshenko, Victor Yu.; Heintzmann, Rainer; Sivakov, Vladimir; Popp, Jürgen

    2016-01-01

    New approaches for visualisation of silicon nanoparticles (SiNPs) in cancer cells are realised by means of the linear and nonlinear optics in vitro. Aqueous colloidal solutions of SiNPs with sizes of about 10–40 nm obtained by ultrasound grinding of silicon nanowires were introduced into breast cancer cells (MCF-7 cell line). Further, the time-varying nanoparticles enclosed in cell structures were visualised by high-resolution structured illumination microscopy (HR-SIM) and micro-Raman spectroscopy. Additionally, the nonlinear optical methods of two-photon excited fluorescence (TPEF) and coherent anti-Stokes Raman scattering (CARS) with infrared laser excitation were applied to study the localisation of SiNPs in cells. Advantages of the nonlinear methods, such as rapid imaging, which prevents cells from overheating and larger penetration depth compared to the single-photon excited HR-SIM, are discussed. The obtained results reveal new perspectives of the multimodal visualisation and precise detection of the uptake of biodegradable non-toxic SiNPs by cancer cells and they are discussed in view of future applications for the optical diagnostics of cancer tumours. PMID:27626408

  18. Optical Asymmetry and Nonlinear Light Scattering from Colloidal Gold Nanorods.

    Science.gov (United States)

    Lien, Miao-Bin; Kim, Ji-Young; Han, Myung-Geun; Chang, You-Chia; Chang, Yu-Chung; Ferguson, Heather J; Zhu, Yimei; Herzing, Andrew A; Schotland, John C; Kotov, Nicholas A; Norris, Theodore B

    2017-06-27

    A systematic study is presented of the intensity-dependent nonlinear light scattering spectra of gold nanorods under resonant excitation of the longitudinal surface plasmon resonance (SPR). The spectra exhibit features due to coherent second and third harmonic generation as well as a broadband feature that has been previously attributed to multiphoton photoluminescence arising primarily from interband optical transitions in the gold. A detailed study of the spectral dependence of the scaling of the scattered light with excitation intensity shows unexpected scaling behavior of the coherent signals, which is quantitatively accounted for by optically induced damping of the SPR mode through a Fermi liquid model of the electronic scattering. The broadband feature is shown to arise not from luminescence, but from scattering of the second-order longitudinal SPR mode with the electron gas, where efficient excitation of the second order mode arises from an optical asymmetry of the nanorod. The electronic-temperature-dependent plasmon damping and the Fermi-Dirac distribution together determine the intensity dependence of the broadband emission, and the structure-dependent absorption spectrum determines the spectral shape through the fluctuation-dissipation theorem. Hence a complete self-consistent picture of both coherent and incoherent light scattering is obtained with a single set of physical parameters.

  19. Method for nonlinear exponential regression analysis

    Science.gov (United States)

    Junkin, B. G.

    1972-01-01

    Two computer programs developed according to two general types of exponential models for conducting nonlinear exponential regression analysis are described. Least squares procedure is used in which the nonlinear problem is linearized by expanding in a Taylor series. Program is written in FORTRAN 5 for the Univac 1108 computer.

  20. A study on linear and non-linear optical constants of Rhodamine B thin film deposited on FTO glass

    Science.gov (United States)

    Yahia, I. S.; Jilani, Asim; Abutalib, M. M.; AlFaify, S.; Shkir, M.; Abdel-wahab, M. Sh.; Al-Ghamdi, Attieh A.; El-Naggar, A. M.

    2016-06-01

    The aim of this research was to fabricate/deposit the good quality thin film of Rhodamine B dye on fluorine doped tin oxide glass substrate by the low cost spin coating technique and study their linear and nonlinear optical parameters. The thickness of the thin film was measured about 300 nm with alpha step system. The transmittance of the fabricated thin film was found to be above 75% corresponding to the fluorine doped tin oxide layer. The structural analysis was performed with X-rays diffraction spectroscopy. Atomic force microscope showed the topographic image of deposited thin film. Linear optical constant like absorption coefficient, band gap, and extinction index was calculated. The dielectric constant was calculated to know the optical response of Rhodamine B dye over fluorine doped tin oxide substrate. The nonlinear optical constant like linear optical susceptibility χ(1), nonlinear optical susceptibility χ(3), nonlinear refractive index (n2) were calculated by spectroscopic method. This method has advantage over the experimental method like Z-Scan for organic dye base semiconductors for future advance optoelectronics applications like dye synthesis solar cell.

  1. A study on linear and non-linear optical constants of Rhodamine B thin film deposited on FTO glass

    Energy Technology Data Exchange (ETDEWEB)

    Yahia, I.S. [Nano-Science & Semiconductor Labs, Physics Department, Faculty of Education, Ain Shams University, Roxy, Cairo (Egypt); Department of Physics, Faculty of Science, King Khalid University, P.O. Box 9004, Abha (Saudi Arabia); Jilani, Asim, E-mail: asim.jilane@gmail.com [Centre of Nanotechnology, Physics Department-Faculty of Science-AL Faisaliah Campus, King Abdulaziz University, P.O. Box 80200, Jeddah 21589 (Saudi Arabia); Abutalib, M.M. [Centre of Nanotechnology, Physics Department-Faculty of Science-AL Faisaliah Campus, King Abdulaziz University, P.O. Box 80200, Jeddah 21589 (Saudi Arabia); AlFaify, S. [Nano-Science & Semiconductor Labs, Physics Department, Faculty of Education, Ain Shams University, Roxy, Cairo (Egypt); Shkir, M. [Department of Physics, Faculty of Science, King Khalid University, P.O. Box 9004, Abha (Saudi Arabia); Abdel-wahab, M.Sh.; Al-Ghamdi, Attieh A. [Centre of Nanotechnology, Physics Department-Faculty of Science-AL Faisaliah Campus, King Abdulaziz University, P.O. Box 80200, Jeddah 21589 (Saudi Arabia); El-Naggar, A.M. [Exploitation of Renewable Energy Applications in Saudi Arabia, Physics & Astronomy Department, College of Science, King Saud University, P.O.Box 2455, Riyadh 11451 (Saudi Arabia)

    2016-06-01

    The aim of this research was to fabricate/deposit the good quality thin film of Rhodamine B dye on fluorine doped tin oxide glass substrate by the low cost spin coating technique and study their linear and nonlinear optical parameters. The thickness of the thin film was measured about 300 nm with alpha step system. The transmittance of the fabricated thin film was found to be above 75% corresponding to the fluorine doped tin oxide layer. The structural analysis was performed with X-rays diffraction spectroscopy. Atomic force microscope showed the topographic image of deposited thin film. Linear optical constant like absorption coefficient, band gap, and extinction index was calculated. The dielectric constant was calculated to know the optical response of Rhodamine B dye over fluorine doped tin oxide substrate. The nonlinear optical constant like linear optical susceptibility χ{sup (1)}, nonlinear optical susceptibility χ{sup (3)}, nonlinear refractive index (n{sub 2}) were calculated by spectroscopic method. This method has advantage over the experimental method like Z-Scan for organic dye base semiconductors for future advance optoelectronics applications like dye synthesis solar cell.

  2. Beam-Based Nonlinear Optics Corrections in Colliders

    CERN Document Server

    Pilat, Fulvia Caterina; Malitsky, Nikolay; Ptitsyn, Vadim

    2005-01-01

    A method has been developed to measure and correct operationally the non-linear effects of the final focusing magnets in colliders, which gives access to the effects of multi-pole errors by applying closed orbit bumps, and analyzing the resulting tune and orbit shifts. This technique has been tested and used during 3 years of RHIC (the Relativistic Heavy Ion Collider at BNL) operations. I will discuss here the theoretical basis of the method, the experimental set-up, the correction results, the present understanding of the machine model, the potential and limitations of the method itself as compared with other non linear correction techniques.

  3. Characterization of electrosynthesized conjugated polymer-carbon nanotube composite: optical nonlinearity and electrical property.

    Science.gov (United States)

    Bahrami, Afarin; Talib, Zainal Abidin; Shahriari, Esmaeil; Yunus, Wan Mahmood Mat; Kasim, Anuar; Behzad, Kasra

    2012-01-01

    The effects of multi-walled carbon nanotube (MWNT) concentration on the structural, optical and electrical properties of conjugated polymer-carbon nanotube composite are discussed. Multi-walled carbon nanotube-polypyrrole nanocomposites were synthesized by electrochemical polymerization of monomers in the presence of different amounts of MWNTs using sodium dodecylbenzensulfonate (SDBS) as surfactant at room temperature and normal pressure. Field emission scanning electron microscopy (FESEM) indicates that the polymer is wrapped around the nanotubes. Measurement of the nonlinear refractive indices (n(2)) and the nonlinear absorption (β) of the samples with different MWNT concentrations measurements were performed by a single Z-scan method using continuous wave (CW) laser beam excitation wavelength of λ = 532 nm. The results show that both nonlinear optical parameters increased with increasing the concentration of MWNTs. The third order nonlinear susceptibilities were also calculated and found to follow the same trend as n(2) and β. In addition, the conductivity of the composite film was found to increase rapidly with the increase in the MWNT concentration.

  4. Numerical approximations of nonlinear fractional differential difference equations by using modified He-Laplace method

    Directory of Open Access Journals (Sweden)

    J. Prakash

    2016-03-01

    Full Text Available In this paper, a numerical algorithm based on a modified He-Laplace method (MHLM is proposed to solve space and time nonlinear fractional differential-difference equations (NFDDEs arising in physical phenomena such as wave phenomena in fluids, coupled nonlinear optical waveguides and nanotechnology fields. The modified He-Laplace method is a combined form of the fractional homotopy perturbation method and Laplace transforms method. The nonlinear terms can be easily decomposed by the use of He’s polynomials. This algorithm has been tested against time-fractional differential-difference equations such as the modified Lotka Volterra and discrete (modified KdV equations. The proposed scheme grants the solution in the form of a rapidly convergent series. Three examples have been employed to illustrate the preciseness and effectiveness of the proposed method. The achieved results expose that the MHLM is very accurate, efficient, simple and can be applied to other nonlinear FDDEs.

  5. Growth, structural, optical, thermal and mechanical studies on 4-Aminopyridinium monophthalate: A novel nonlinear optical crystal

    Science.gov (United States)

    Marudhu, G.; Krishnan, S.; Palanichamy, M.

    2016-03-01

    A novel nonlinear optical crystal of 4-Aminopyridinium monophthalate (4-APMP) was grown by slow evaporation technique using methanol as solvent. Single crystal X-ray diffraction analysis confirms that the grown crystal belongs to orthorhombic system. The presence of functional groups was qualitatively determined by FTIR analysis. The optical absorption studies reveal very low absorption in the entire visible region. The fluorescence emission spectrum shows the emission is in blue region. The thermal stability of the grown crystal is found to be around 197.2 °C. The SHG efficiency of the grown crystal is found to be 1.1 times than that of KDP crystals.

  6. An integrated nonlinear optical loop mirror in silicon photonics for all-optical signal processing

    Directory of Open Access Journals (Sweden)

    Zifei Wang

    2018-02-01

    Full Text Available The nonlinear optical loop mirror (NOLM has been studied for several decades and has attracted considerable attention for applications in high data rate optical communications and all-optical signal processing. The majority of NOLM research has focused on silica fiber-based implementations. While various fiber designs have been considered to increase the nonlinearity and manage dispersion, several meters to hundreds of meters of fiber are still required. On the other hand, there is increasing interest in developing photonic integrated circuits for realizing signal processing functions. In this paper, we realize the first-ever passive integrated NOLM in silicon photonics and demonstrate its application for all-optical signal processing. In particular, we show wavelength conversion of 10 Gb/s return-to-zero on-off keying (RZ-OOK signals over a wavelength range of 30 nm with error-free operation and a power penalty of less than 2.5 dB, we achieve error-free nonreturn to zero (NRZ-to-RZ modulation format conversion at 10 Gb/s also with a power penalty of less than 2.8 dB, and we obtain error-free all-optical time-division demultiplexing of a 40 Gb/s RZ-OOK data signal into its 10 Gb/s tributary channels with a maximum power penalty of 3.5 dB.

  7. Superior optical nonlinearity of an exceptional fluorescent stilbene dye

    Energy Technology Data Exchange (ETDEWEB)

    He, Tingchao [College of Physics Science and Technology, Shenzhen University, Shenzhen 518060 (China); Division of Physics and Applied Physics, Centre for Disruptive Photonic Technologies (CDPT), School of Physical and Mathematical Sciences, Nanyang Technological University, 21 Nanyang Link, Singapore 637371 (Singapore); Sreejith, Sivaramapanicker; Zhao, Yanli [Division of Chemistry and Biological Chemistry, School of Physical and Mathematical Sciences, Nanyang Technological University, 21 Nanyang Link, Singapore 637371 (Singapore); Gao, Yang; Grimsdale, Andrew C. [School of Materials Science and Engineering, Nanyang Technological University, Singapore, Singapore 639798 (Singapore); Lin, Xiaodong, E-mail: linxd@szu.edu.cn, E-mail: hdsun@ntu.edu.sg [College of Physics Science and Technology, Shenzhen University, Shenzhen 518060 (China); Sun, Handong, E-mail: linxd@szu.edu.cn, E-mail: hdsun@ntu.edu.sg [Division of Physics and Applied Physics, Centre for Disruptive Photonic Technologies (CDPT), School of Physical and Mathematical Sciences, Nanyang Technological University, 21 Nanyang Link, Singapore 637371 (Singapore)

    2015-03-16

    Strong multiphoton absorption and harmonic generation in organic fluorescent chromophores are, respectively, significant in many fields of research. However, most of fluorescent chromophores fall short of the full potential due to the absence of the combination of such different nonlinear upconversion behaviors. Here, we demonstrate that an exceptional fluorescent stilbene dye could exhibit efficient two- and three-photon absorption under the excitation of femtosecond pulses in solution phase. Benefiting from its biocompatibility and strong excited state absorption behavior, in vitro two-photon bioimaging and superior optical limiting have been exploited, respectively. Simultaneously, the chromophore could generate efficient three-photon excited fluorescence and third-harmonic generation (THG) when dispersed into PMMA film, circumventing the limitations of classical fluorescent chromophores. Such chromophore may find application in the production of coherent light sources of higher photon energy. Moreover, the combination of three-photon excited fluorescence and THG can be used in tandem to provide complementary information in biomedical studies.

  8. Femtojoule-scale all-optical latching and modulation via cavity nonlinear optics.

    Science.gov (United States)

    Kwon, Yeong-Dae; Armen, Michael A; Mabuchi, Hideo

    2013-11-15

    We experimentally characterize Hopf bifurcation phenomena at femtojoule energy scales in a multiatom cavity quantum electrodynamical (cavity QED) system and demonstrate how such behaviors can be exploited in the design of all-optical memory and modulation devices. The data are analyzed by using a semiclassical model that explicitly treats heterogeneous coupling of atoms to the cavity mode. Our results highlight the interest of cavity QED systems for ultralow power photonic signal processing as well as for fundamental studies of mesoscopic nonlinear dynamics.

  9. Optically nonlinear energy transfer in light-harvesting dendrimers

    Science.gov (United States)

    Andrews, David L.; Bradshaw, David S.

    2004-08-01

    Dendrimeric polymers are the subject of intense research activity geared towards their implementation in nanodevice applications such as energy harvesting systems, organic light-emitting diodes, photosensitizers, low-threshold lasers, and quantum logic elements, etc. A recent development in this area has been the construction of dendrimers specifically designed to exhibit novel forms of optical nonlinearity, exploiting the unique properties of these materials at high levels of photon flux. Starting from a thorough treatment of the underlying theory based on the principles of molecular quantum electrodynamics, it is possible to identify and characterize several optically nonlinear mechanisms for directed energy transfer and energy pooling in multichromophore dendrimers. Such mechanisms fall into two classes: first, those where two-photon absorption by individual donors is followed by transfer of the net energy to an acceptor; second, those where the excitation of two electronically distinct but neighboring donor groups is followed by a collective migration of their energy to a suitable acceptor. Each transfer process is subject to minor dissipative losses. In this paper we describe in detail the balance of factors and the constraints that determines the favored mechanism, which include the excitation statistics, structure of the energy levels, laser coherence factors, chromophore selection rules and architecture, possibilities for the formation of delocalized excitons, spectral overlap, and the overall distribution of donors and acceptors. Furthermore, it transpires that quantum interference between different mechanisms can play an important role. Thus, as the relative importance of each mechanism determines the relevant nanophotonic characteristics, the results reported here afford the means for optimizing highly efficient light-harvesting dendrimer devices.

  10. Fiber Nonlinearity Post-Compensation by Optical Phase Conjugation for 40Gb/s CO-OFDM Systems

    International Nuclear Information System (INIS)

    Qiao Yao-Jun; Liu Xue-Jun; Ji Yue-Feng

    2011-01-01

    Fiber nonlinearity impairments in a 40-Gb/s coherent optical orthogonal frequency division multiplexing (COOFDM) system are post-compensated for by a new method of fiber nonlinearity post-compensation (FNPC). The FNPC located before the CO-OFDM receiver includes an optical phase conjugation (OPC) unit and a subsequent 80-km-high nonlinear fiber (HNLF) as a fiber nonlinearity compensator. The OPC unit is based on a four wave mixing effect in a semiconductor optical amplifier. The fiber nonlinearity impairments in the transmission link are post-compensated for after OPC by transmission through the HNLF with a large nonlinearity coefficient. Simulation results show that the nonlinear threshold (NLT) (for Q > 10 dB) can be increased by about 2.5 dB and the maximum Q factor is increased by about 1.2 dB for the single-channel 40-Gb/s CO-OFDM system with periodic dispersion maps. In the 50-GHz channel spacing wavelength-division-multiplexing system, the NLT increases by 1.1 dB, equating to a 0.7 dB improvement for the maximum Q factor. (fundamental areas of phenomenology(including applications))

  11. Nonlinear Optical Magnetism Revealed by Second-Harmonic Generation in Nanoantennas.

    Science.gov (United States)

    Kruk, Sergey S; Camacho-Morales, Rocio; Xu, Lei; Rahmani, Mohsen; Smirnova, Daria A; Wang, Lei; Tan, Hark Hoe; Jagadish, Chennupati; Neshev, Dragomir N; Kivshar, Yuri S

    2017-06-14

    Nonlinear effects at the nanoscale are usually associated with the enhancement of electric fields in plasmonic structures. Recently emerged new platform for nanophotonics based on high-index dielectric nanoparticles utilizes optically induced magnetic response via multipolar Mie resonances and provides novel opportunities for nanoscale nonlinear optics. Here, we observe strong second-harmonic generation from AlGaAs nanoantennas driven by both electric and magnetic resonances. We distinguish experimentally the contribution of electric and magnetic nonlinear response by analyzing the structure of polarization states of vector beams in the second-harmonic radiation. We control continuously the transition between electric and magnetic nonlinearities by tuning polarization of the optical pump. Our results provide a direct observation of nonlinear optical magnetism through selective excitation of multipolar nonlinear modes in nanoantennas.

  12. Resonantly enhanced nonlinear optics in semiconductor quantum wells: An application to sensitive infrared detection

    International Nuclear Information System (INIS)

    Yelin, S.F.; Hemmer, P.R.

    2002-01-01

    A novel class of coherent nonlinear optical phenomena, involving induced transparency in semiconductor quantum wells, is considered in the context of a particular application to sensitive long-wavelength infrared detection. It is shown that the strongest decoherence mechanisms can be suppressed or mitigated, resulting in substantial enhancement of nonlinear optical effects in semiconductor quantum wells

  13. Modulation stability and dispersive optical soliton solutions of higher order nonlinear Schrödinger equation and its applications in mono-mode optical fibers

    Science.gov (United States)

    Arshad, Muhammad; Seadawy, Aly R.; Lu, Dianchen

    2018-01-01

    In mono-mode optical fibers, the higher order non-linear Schrödinger equation (NLSE) describes the propagation of enormously short light pulses. We constructed optical solitons and, solitary wave solutions of higher order NLSE mono-mode optical fibers via employing modified extended mapping method which has important applications in Mathematics and physics. Furthermore, the formation conditions are also given on parameters in which optical bright and dark solitons can exist for this media. The moment of the obtained solutions are also given graphically, that helps to realize the physical phenomena's of this model. The modulation instability analysis is utilized to discuss the model stability, which verifies that all obtained solutions are exact and stable. Many other such types of models arising in applied sciences can also be solved by this reliable, powerful and effective method. The method can also be functional to other sorts of higher order nonlinear problems in contemporary areas of research.

  14. Optical nonlinearities and ultrafast all-optical switching of m-plane GaN in the near-infrared

    Energy Technology Data Exchange (ETDEWEB)

    Fang, Yu; Zhou, Feng; Yang, Junyi; Yang, Yong [College of Physics, Optoelectronics and Energy, Soochow University, 215006 Suzhou (China); Xiao, Zhengguo; Wu, Xingzhi [Department of Physics, Harbin Institute of Technology, 150001 Harbin (China); Song, Yinglin, E-mail: ylsong@hit.edu.cn [College of Physics, Optoelectronics and Energy, Soochow University, 215006 Suzhou (China); Department of Physics, Harbin Institute of Technology, 150001 Harbin (China)

    2015-06-22

    We reported a systematic investigation on the three-photon absorption (3PA) spectra and wavelength dispersion of Kerr refraction of bulk m-plane GaN crystal with both polarization E⊥c and E//c by femtosecond Z-scan technique in the near-infrared region from 760 to 1030 nm. Both 3PA spectra and Kerr refraction dispersion were in good agreement with two-band models. The calculated nonlinear figure of merit and measured ultrafast nonlinear refraction dynamics via femtosecond pump-probe with phase object method revealed that m-plane GaN would be a promising candidate for ultrafast all-optical switching and autocorrelation applications at telecommunication wavelengths.

  15. Ultrasensitive mass sensing with nonlinear optics in a doubly clamped suspended carbon nanotube resonator

    Energy Technology Data Exchange (ETDEWEB)

    Chen, Hua-Jun; Zhu, Ka-Di [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, 800 DongChuan Road, Shanghai 2 00240 (China)

    2013-12-07

    Nanomechanical resonator makes itself as an ideal system for ultrasensitive mass sensing due to its ultralow mass and high vibrational frequency. The mass sensing principle is due to the linear relationship of the frequency-shift and mass-variation. In this work, we will propose a nonlinear optical mass sensor based on a doubly clamped suspended carbon nanotube resonator in all-optical domain. The masses of external particles (such as nitric oxide molecules) landing onto the surface of carbon nanotube can be determined directly and accurately via using the nonlinear optical spectroscopy. This mass sensing proposed here may provide a nonlinear optical measurement technique in quantum measurements and environmental science.

  16. Variational iteration method for one dimensional nonlinear thermoelasticity

    International Nuclear Information System (INIS)

    Sweilam, N.H.; Khader, M.M.

    2007-01-01

    This paper applies the variational iteration method to solve the Cauchy problem arising in one dimensional nonlinear thermoelasticity. The advantage of this method is to overcome the difficulty of calculation of Adomian's polynomials in the Adomian's decomposition method. The numerical results of this method are compared with the exact solution of an artificial model to show the efficiency of the method. The approximate solutions show that the variational iteration method is a powerful mathematical tool for solving nonlinear problems

  17. New Architecture of Optical Interconnect for High-Speed Optical Computerized Data Networks (Nonlinear Response

    Directory of Open Access Journals (Sweden)

    El-Sayed A. El-Badawy

    2008-02-01

    Full Text Available Although research into the use of optics in computers has increased in the last and current decades, the fact remains that electronics is still superior to optics in almost every way. Research into the use of optics at this stage mirrors the research into electronics after the 2nd World War. The advantages of using fiber optics over wiring are the same as the argument for using optics over electronics in computers. Even through totally optical computers are now a reality, computers that combine both electronics and optics, electro-optic hybrids, have been in use for some time. In the present paper, architecture of optical interconnect is built up on the bases of four Vertical-Cavity Surface- Emitting Laser Diodes (VCSELD and two optical links where thermal effects of both the diodes and the links are included. Nonlinear relations are correlated to investigate the power-current and the voltage-current dependences of the four devices. The good performance (high speed of the interconnect is deeply and parametrically investigated under wide ranges of the affecting parameters. The high speed performance is processed through three different effects, namely the device 3-dB bandwidth, the link dispersion characteristics, and the transmitted bit rate (soliton. Eight combinations are investigated; each possesses its own characteristics. The best architecture is the one composed of VCSELD that operates at 850 nm and the silica fiber whatever the operating set of causes. This combination possesses the largest device 3-dB bandwidth, the largest link bandwidth and the largest soliton transmitted bit rate. The increase of the ambient temperature reduces the high-speed performance of the interconnect

  18. EDITORIAL: Nonlinear optical manipulation, patterning and control in nano- and micro-scale systems Nonlinear optical manipulation, patterning and control in nano- and micro-scale systems

    Science.gov (United States)

    Denz, Cornelia; Simoni, Francesco

    2009-03-01

    Nonlinearities are becoming more and more important for a variety of applications in nanosciences, bio-medical sciences, information processing and photonics. For applications at the crossings of these fields, especially microscopic and nanoscopic imaging and manipulation, nonlinearities play a key role. They may range from simple nonlinear parameter changes up to applications in manipulating, controlling and structuring material by light, or the manipulation of light by light itself. It is this area between basic nonlinear optics and photonic applications that includes `hot' topics such as ultra-resolution optical microscopy, micro- and nanomanipulation and -structuring, or nanophotonics. This special issue contains contributions in this field, many of them from the International Conference on Nonlinear Microscopy and Optical Control held in conjunction with a network meeting of the ESF COST action MP0604 `Optical Micromanipulation by Nonlinear Nanophotonics', 19-22 February 2008, Münster, Germany. Throughout this special issue, basic investigations of material structuring by nonlinear light--matter interaction, light-induced control of nanoparticles, and novel nonlinear material investigation techniques, are presented, covering the basic field of optical manipulation and control. These papers are followed by impressive developments of optical tweezers. Nowadays, optical phase contrast tweezers, twin and especially multiple beam traps, develop particle control in a new dimension: particles can be arranged, sorted and identified with high throughput. One of the most prominent forthcoming applications of optical tweezers is in the field of microfluidics. The action of light on fluids will open new horizons in microfluidic manipulation and control. The field of optical manipulation and control is a very broad field that has developed in an impressive way, in a short time, in Europe with the installation of the MP0604 network. Top researchers from 19 countries are

  19. Nonlinear atom optics and bright-gap-soliton generation in finite optical lattices

    International Nuclear Information System (INIS)

    Carusotto, Iacopo; Embriaco, Davide; La Rocca, Giuseppe C.

    2002-01-01

    We theoretically investigate the transmission dynamics of coherent matter wave pulses across finite optical lattices in both the linear and the nonlinear regimes. The shape and the intensity of the transmitted pulse are found to strongly depend on the parameters of the incident pulse, in particular its velocity and density: a clear physical picture of the main features observed in the numerical simulations is given in terms of the atomic band dispersion in the periodic potential of the optical lattice. Signatures of nonlinear effects due to the atom-atom interaction are discussed in detail, such as atom-optical limiting and atom-optical bistability. For positive scattering lengths, matter waves propagating close to the top of the valence band are shown to be subject to modulational instability. A scheme for the experimental generation of narrow bright gap solitons from a wide Bose-Einstein condensate is proposed: the modulational instability is seeded starting from the strongly modulated density profile of a standing matter wave and the solitonic nature of the generated pulses is checked from their shape and their collisional properties

  20. Auxiliary equation method for solving nonlinear partial differential equations

    International Nuclear Information System (INIS)

    Sirendaoreji,; Jiong, Sun

    2003-01-01

    By using the solutions of an auxiliary ordinary differential equation, a direct algebraic method is described to construct several kinds of exact travelling wave solutions for some nonlinear partial differential equations. By this method some physically important nonlinear equations are investigated and new exact travelling wave solutions are explicitly obtained with the aid of symbolic computation

  1. Brain plasticity and functionality explored by nonlinear optical microscopy

    Science.gov (United States)

    Sacconi, L.; Allegra, L.; Buffelli, M.; Cesare, P.; D'Angelo, E.; Gandolfi, D.; Grasselli, G.; Lotti, J.; Mapelli, J.; Strata, P.; Pavone, F. S.

    2010-02-01

    In combination with fluorescent protein (XFP) expression techniques, two-photon microscopy has become an indispensable tool to image cortical plasticity in living mice. In parallel to its application in imaging, multi-photon absorption has also been used as a tool for the dissection of single neurites with submicrometric precision without causing any visible collateral damage to the surrounding neuronal structures. In this work, multi-photon nanosurgery is applied to dissect single climbing fibers expressing GFP in the cerebellar cortex. The morphological consequences are then characterized with time lapse 3-dimensional two-photon imaging over a period of minutes to days after the procedure. Preliminary investigations show that the laser induced fiber dissection recalls a regenerative process in the fiber itself over a period of days. These results show the possibility of this innovative technique to investigate regenerative processes in adult brain. In parallel with imaging and manipulation technique, non-linear microscopy offers the opportunity to optically record electrical activity in intact neuronal networks. In this work, we combined the advantages of second-harmonic generation (SHG) with a random access (RA) excitation scheme to realize a new microscope (RASH) capable of optically recording fast membrane potential events occurring in a wide-field of view. The RASH microscope, in combination with bulk loading of tissue with FM4-64 dye, was used to simultaneously record electrical activity from clusters of Purkinje cells in acute cerebellar slices. Complex spikes, both synchronous and asynchronous, were optically recorded simultaneously across a given population of neurons. Spontaneous electrical activity was also monitored simultaneously in pairs of neurons, where action potentials were recorded without averaging across trials. These results show the strength of this technique in describing the temporal dynamics of neuronal assemblies, opening promising

  2. Multifunctional Bi2ZnOB2O6 single crystals for second and third order nonlinear optical applications

    International Nuclear Information System (INIS)

    Iliopoulos, K.; Kasprowicz, D.; Majchrowski, A.; Michalski, E.; Gindre, D.; Sahraoui, B.

    2013-01-01

    Bi 2 ZnOB 2 O 6 nonlinear optical single crystals were grown by means of the Kyropoulos method from stoichiometric melt. The second and third harmonic generation (SHG/THG) of Bi 2 ZnOB 2 O 6 crystals were investigated by the SHG/THG Maker fringes technique. Moreover, SHG microscopy studies were carried out providing two-dimensional SHG images as a function of the incident laser polarization. The high nonlinear optical efficiency combined with the possibility to grow high quality crystals make Bi 2 ZnOB 2 O 6 an excellent candidate for photonic applications

  3. Propagation of optical vortex beams and nucleation of vortex-antivortex pairs in disordered nonlinear photonic lattices

    International Nuclear Information System (INIS)

    Cho, Yeong-Kwon; Kim, Ki-Hong

    2014-01-01

    The propagation of optical vortex beams through disordered nonlinear photonic lattices is numerically studied. The vortex beams are generated by using a superposition of several Gaussian laser beams arranged in a radially-symmetric manner. The paraxial nonlinear Schroedinger equation describing the longitudinal propagation of the beam array through nonlinear triangular photonic lattices with two-dimensional disorder is solved numerically by using the split-step Fourier method. We find that due to the spatial disorder, the vortex beam is destabilized after propagating a finite distance and new vortex-antivortex pairs are nucleated at the positions of perfect destructive interference. We also find that in the presence of a self-focusing nonlinearity, the vortex-antivortex pair nucleation is suppressed and the vortex beam becomes more stable, while a self-defocusing nonlinearity enhances the vortex-antivortex pair nucleation.

  4. Dynamic neural network-based methods for compensation of nonlinear effects in multimode communication lines

    Science.gov (United States)

    Sidelnikov, O. S.; Redyuk, A. A.; Sygletos, S.

    2017-12-01

    We consider neural network-based schemes of digital signal processing. It is shown that the use of a dynamic neural network-based scheme of signal processing ensures an increase in the optical signal transmission quality in comparison with that provided by other methods for nonlinear distortion compensation.

  5. Optical Frequency Mixing in Periodically-Patterned and in Quasi-Periodically-Patterned Nonlinear media

    International Nuclear Information System (INIS)

    Arie, A.

    1999-01-01

    Nonlinear frequency mixing processes, e.g. second harmonic generation, sum and difference frequency generation, etc., require matching of the phases of the interacting waves. The traditional method to achieve it is by selecting a specific angle of propagation in a birefringent nonlinear crystal. The main limitation of the birefringent phase matching method stems from the fact that for many interesting interactions, the phase matching condition cannot be satisfied in a specific crystal. This obstacle can be removed by the technique of quasi-phase-matching (QPM), where the nonlinear coefficient of the material is modulated at a fixed spatial frequency that equals the wave-vector phase mismatch between the interacting waves. An important development in recent years is the ability to periodically reverse the sign of the nonlinear coefficient in ferroelectric crystals by applying a high electric field through a periodic electrode. Some recent QPM interactions in periodically-poled KTP that were recently achieved at Tel-Aviv University include continuous-wave optical parametric oscillations, as well as generation of tunable mid-infrared radiation by difference frequency generation. Periodic patterning of the nonlinear coefficient enables to phase match only a single interaction. It would be advantageous to further extend the applications of this technique in order to simultaneously satisfy several interactions on a single crystal. This cannot be usually achieved in a periodic pattern, however more sophisticated quasi-periodic structures can be designed in this case. An interesting analogy can be drawn between artificially-made quasi-periodically-patterned nonlinear crystals and quasi-crystals found in nature, in rapidly-cooled metallic alloys

  6. Synthesis, growth, and structural, optical, mechanical, electrical properties of a new inorganic nonlinear optical crystal: Sodium manganese tetrachloride (SMTC

    Directory of Open Access Journals (Sweden)

    M. Packiya raj

    2017-01-01

    Full Text Available A new inorganic nonlinear optical single crystal of sodium manganese tetrachloride (SMTC has been successfully grown from aqueous solution using the slow evaporation technique at room temperature. The crystals obtained using the aforementioned method were characterized using different techniques. The crystalline nature of the as-grown crystal of SMTC was analyzed using powder X-ray diffraction. Single-crystal X-ray diffraction revealed that the crystal belongs to an orthorhombic system with non-centrosymmetric space group Pbam. The optical transmission study of the SMTC crystal revealed high transmittance in the entire UV–vis region, and the lower cut-off wavelength was determined to be 240 nm. The mechanical strength of the as-grown crystal was estimated using the Vickers microhardness test. The second harmonic generation (SHG efficiency of the crystal was measured using Kurtz's powder technique, which indicated that the crystal has a nonlinear optical (NLO efficiency that is 1.32 times greater than that of KDP. The dielectric constant and dielectric loss of the compound were measured at different temperatures with varying frequencies. The photoconductivity study confirmed that the title compound possesses a negative photoconducting nature. The growth mechanism and surface features of the as-grown crystals were investigated using chemical etching analysis.

  7. Studies on nonlocal optical nonlinearity of Sr–CuO–polyvinyl alcohol nanocomposite thin films

    International Nuclear Information System (INIS)

    Tamgadge, Y.S.; Talwatkar, S.S.; Sunatkari, A.L.; Pahurkar, V.G.; Muley, G.G.

    2015-01-01

    Thermally induced nonlocal nonlinear optical properties of strontium (Sr) doped CuO-polyvinyl alcohol (PVA) nanocomposite thin films under continuous wave Helium–Neon laser illumination are investigated by single beam Z-scan method. Undoped and Sr doped CuO nanoparticles (NPs) using L-arginine as surface modifying agent have been synthesized by wet chemical method and their thin films with PVA as host matrix have been obtained by spin coating technique. Structure, morphology and purity of prepared CuO NPs and thin films have been studied by X-ray diffraction, high-resolution transmission electron microscopy, field emission scanning electron microscopy and energy dispersive X-ray absorption spectroscopy. Fourier transform infra-red spectrum attests the role of L-arginine as surface modifier and ultraviolet–visible absorption studies reveal that the excitonic absorption wavelengths are blue shifted for strontium doped CuO NPs. Sr doped CuO NPs with average particle size of 7 nm and calculated optical band gap up to 2.54 eV have been reported. All Sr doped CuO–PVA nanocomposite thin films show enhanced nonlinear refraction and absorption best suited for optical limiting applications. Observed effects have been attributed to thermal lensing effect. - Highlights: • Pure and strontium doped CuO–polyvinyl alcohol nanocomposite thin films are prepared. • Z-scan studies of thin films are performed under continuous wave helium–neon laser. • Enhanced values of third order nonlinear optical coefficients are obtained for all films. • Thermally induced self-defocusing and reverse saturable absorption have been discussed.

  8. Studies on nonlocal optical nonlinearity of Sr–CuO–polyvinyl alcohol nanocomposite thin films

    Energy Technology Data Exchange (ETDEWEB)

    Tamgadge, Y.S. [Department of Physics, Mahatma Fule Arts, Commerce and S C Science Mahavidyalaya, Warud, Dist. Amravati (MS), 444906 (India); Talwatkar, S.S. [Department of Physics, D K Marathe and N G Acharya College, Chembur, Mumbai (MS) 440071 (India); Sunatkari, A.L. [Department of Physics, Siddharth College of Arts, Science and Commerce, Fort, Mumbai (MS) 440001 (India); Pahurkar, V.G. [Department of Physics, Sant Gadge Baba Amravati University, Amravati (MS), 444602 (India); Muley, G.G., E-mail: gajananggm@yahoo.co.in [Department of Physics, Sant Gadge Baba Amravati University, Amravati (MS), 444602 (India)

    2015-11-30

    Thermally induced nonlocal nonlinear optical properties of strontium (Sr) doped CuO-polyvinyl alcohol (PVA) nanocomposite thin films under continuous wave Helium–Neon laser illumination are investigated by single beam Z-scan method. Undoped and Sr doped CuO nanoparticles (NPs) using L-arginine as surface modifying agent have been synthesized by wet chemical method and their thin films with PVA as host matrix have been obtained by spin coating technique. Structure, morphology and purity of prepared CuO NPs and thin films have been studied by X-ray diffraction, high-resolution transmission electron microscopy, field emission scanning electron microscopy and energy dispersive X-ray absorption spectroscopy. Fourier transform infra-red spectrum attests the role of L-arginine as surface modifier and ultraviolet–visible absorption studies reveal that the excitonic absorption wavelengths are blue shifted for strontium doped CuO NPs. Sr doped CuO NPs with average particle size of 7 nm and calculated optical band gap up to 2.54 eV have been reported. All Sr doped CuO–PVA nanocomposite thin films show enhanced nonlinear refraction and absorption best suited for optical limiting applications. Observed effects have been attributed to thermal lensing effect. - Highlights: • Pure and strontium doped CuO–polyvinyl alcohol nanocomposite thin films are prepared. • Z-scan studies of thin films are performed under continuous wave helium–neon laser. • Enhanced values of third order nonlinear optical coefficients are obtained for all films. • Thermally induced self-defocusing and reverse saturable absorption have been discussed.

  9. Third order nonlinear optical properties and optical limiting behavior of alkali metal complexes of p-nitrophenol

    Science.gov (United States)

    Thangaraj, M.; Vinitha, G.; Sabari Girisun, T. C.; Anandan, P.; Ravi, G.

    2015-10-01

    Optical nonlinearity of metal complexes of p-nitrophenolate (M=Li, Na and K) in ethanol is studied by using a continuous wave (cw) diode pumped Nd:YAG laser (532 nm, 50 mW). The predominant mechanism of observed nonlinearity is thermal in origin. The nonlinear refractive index and the nonlinear absorption coefficient of the samples were found to be in the order of 10-8 cm2/W and 10-3 cm/W respectively. Magnitude of third-order optical parameters varies according to the choice of alkali metal chosen for metal complex formation of p-nitrophenolate. The third-order nonlinear susceptibility was found to be in the order of 10-6 esu. The observed saturable absorption and the self-defocusing effect were used to demonstrate the optical limiting action at 532 nm by using the same cw laser beam.

  10. Studies on third-order optical nonlinearity and power limiting of conducting polymers using the z-scan technique for nonlinear optical applications

    Science.gov (United States)

    Pramodini, S.; Sudhakar, Y. N.; SelvaKumar, M.; Poornesh, P.

    2014-04-01

    We present the synthesis and characterization of third-order optical nonlinearity and optical limiting of the conducting polymers poly (aniline-co-o-anisidine) and poly (aniline-co-pyrrole). Nonlinear optical studies were carried out by employing the z-scan technique using a He-Ne laser operating in continuous wave mode at 633 nm. The copolymers exhibited a reverse saturable absorption process and self-defocusing properties under the experimental conditions. The estimated values of βeff, n2 and χ(3) were found to be of the order of 10-2 cm W-1, 10-5 esu and 10-7 esu respectively. Self-diffraction rings were observed due to refractive index change when exposed to the laser beam. The copolymers possess a lower limiting threshold and clamping level, which is essential to a great extent for power limiting devices. Therefore, copolymers of aniline emerge as a potential candidate for nonlinear optical device applications.

  11. A method for nonlinear exponential regression analysis

    Science.gov (United States)

    Junkin, B. G.

    1971-01-01

    A computer-oriented technique is presented for performing a nonlinear exponential regression analysis on decay-type experimental data. The technique involves the least squares procedure wherein the nonlinear problem is linearized by expansion in a Taylor series. A linear curve fitting procedure for determining the initial nominal estimates for the unknown exponential model parameters is included as an integral part of the technique. A correction matrix was derived and then applied to the nominal estimate to produce an improved set of model parameters. The solution cycle is repeated until some predetermined criterion is satisfied.

  12. Robust methods and asymptotic theory in nonlinear econometrics

    CERN Document Server

    Bierens, Herman J

    1981-01-01

    This Lecture Note deals with asymptotic properties, i.e. weak and strong consistency and asymptotic normality, of parameter estimators of nonlinear regression models and nonlinear structural equations under various assumptions on the distribution of the data. The estimation methods involved are nonlinear least squares estimation (NLLSE), nonlinear robust M-estimation (NLRME) and non­ linear weighted robust M-estimation (NLWRME) for the regression case and nonlinear two-stage least squares estimation (NL2SLSE) and a new method called minimum information estimation (MIE) for the case of structural equations. The asymptotic properties of the NLLSE and the two robust M-estimation methods are derived from further elaborations of results of Jennrich. Special attention is payed to the comparison of the asymptotic efficiency of NLLSE and NLRME. It is shown that if the tails of the error distribution are fatter than those of the normal distribution NLRME is more efficient than NLLSE. The NLWRME method is appropriate ...

  13. Nonlinear optical response of chalcogenide glassy semiconductors in the IR and THz ranges studied with the femtosecond resolution in time

    DEFF Research Database (Denmark)

    Romanova, E.; Guizard, S.; Wang, Tianwu

    2017-01-01

    Two time-resolved experimental methods have been used for characterization of the non-linear optical response of chalcogenide glasses of the system As-S-Se-Te in IR and THz ranges upon excitation by femtosecond laser pulses at 800 nm wavelength. Photoinduced conductivity and refractivity were stu...

  14. Creating large second-order optical nonlinearity in optical waveguides written by femtosecond laser pulses in boro-aluminosilicate glass

    Science.gov (United States)

    An, Hong-Lin; Arriola, Alexander; Gross, Simon; Fuerbach, Alexander; Withford, Michael J.; Fleming, Simon

    2014-01-01

    The thermal poling technique was applied to optical waveguides embedded in a commercial boro-aluminosilicate glass, resulting in high levels of induced second-order optical nonlinearity. The waveguides were fabricated using the femtosecond laser direct-write technique, and thermally poled samples were characterized with second harmonic optical microscopy to reveal the distribution profile of the induced nonlinearity. It was found that, in contrast to fused silica, the presence of waveguides in boro-aluminosilicate glass led to an enhancement of the creation of the second-order nonlinearity, which is larger in the laser written waveguiding regions when compared to the un-modified substrate. The magnitude of the nonlinear coefficient d33 achieved in the core of the laser-written waveguides, up to 0.2 pm/V, was comparable to that in thermally poled fused silica, enabling the realization of compact integrated electro-optic devices in boro-aluminosilicate glasses.

  15. Numerical Methods for Nonlinear PDEs in Finance

    DEFF Research Database (Denmark)

    Mashayekhi, Sima

    Nonlinear Black-Scholes equations arise from considering parameters such as feedback and illiquid markets eects or large investor preferences, volatile portfolio and nontrivial transaction costs into option pricing models to have more accurate option price. Here some nite dierence schemes have be...

  16. MECHANISM OF OPTICAL NONLINEARITY IN “LYOTROPIC LIQUID CRYSTAL — VIOLOGEN” SYSTEM

    Directory of Open Access Journals (Sweden)

    Hanna Bordyuh

    2014-06-01

    Full Text Available In the present work we analyze the characteristics of holographic grating recording and consider a mechanism of optical nonlinearity in the lyotropic liquid crystal (LLC — viologen samples. Taking into account structural and electrooptical properties of the admixture molecules it is possible to suggest that the recording is realized due to the change of polarizability of π-electron system of coloured viologen derivatives under the action of laser radiation. The main nonlinear optical parameters such as nonlinear refraction coefficient n2, cubic nonlinear susceptibility χ(3, and hyperpolarizability γ were calculated.

  17. Optical nonlinearities in Ag/BaTiO{sub 3} multi-layer nanocomposite films

    Energy Technology Data Exchange (ETDEWEB)

    Yang Guang [Wuhan National Laboratory for Optoelectronics and School of Optoelectronics Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074 (China)], E-mail: gyang@hust.edu.cn; Zhou Youhua [Wuhan National Laboratory for Optoelectronics and School of Optoelectronics Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074 (China); School of Physics and Information Engineering, Jianghan University, Wuhan 430056 (China); Long Hua; Li Yuhua; Yang Yifa [Wuhan National Laboratory for Optoelectronics and School of Optoelectronics Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074 (China)

    2007-07-31

    The multi-layer structure of barium titanate composite thin films containing Ag nanoparticles were grown on MgO (100) substrates using pulsed laser deposition technique under the nitrogen pressure of 7.4 Pa. The X-ray photoelectron spectroscopy analysis indicated that the samples were composed of metal Ag embedded in the BaTiO{sub 3} matrices. The optical absorption properties were measured from 300 nm to 800 nm, and the absorption peaks due to the surface plasmon resonance of Ag particles were observed. With the increasing of Ag concentration in composite films, the peak absorption increased and shifted to longer wavelength (red-shift). Furthermore, the third-order optical nonlinearities of the films were determined by z-scan method and the nonlinear refractive index, n{sub 2}, and nonlinear absorption coefficient, {beta}, were determined to be about - 1.91 x 10{sup -13} m{sup 2}/W and - 5.80 x 10{sup -7} m/W, respectively.

  18. Optimizing optical nonlinearities in GaInAs/AlInAs quantum cascade lasers

    Directory of Open Access Journals (Sweden)

    Gajić Aleksandra D.

    2014-01-01

    Full Text Available Regardless of the huge advances made in the design and fabrication of mid-infrared and terahertz quantum cascade lasers, success in accessing the ~3-4 mm region of the electromagnetic spectrum has remained limited. This fact has brought about the need to exploit resonant intersubband transitions as powerful nonlinear oscillators, consequently enabling the occurrence of large nonlinear optical susceptibilities as a means of reaching desired wavelengths. In this work, we present a computational model developed for the optimization of second-order optical nonlinearities in In0.53Ga0.47As/Al0.48In0.52As quantum cascade laser structures based on the implementation of the Genetic algorithm. The carrier transport and the power output of the structure were calculated by self-consistent solutions to the system of rate equations for carriers and photons. Both stimulated and simultaneous double-photon absorption processes occurring between the second harmonic generation-relevant levels are incorporated into rate equations and the material-dependent effective mass and band non-parabolicity are taken into account, as well. The developed method is quite general and can be applied to any higher order effect which requires the inclusion of the photon density equation. [Projekat Ministarstva nauke Republike Srbije, br. III 45010

  19. Photo-physics of third-order nonlinear optical processes in organic dyes

    International Nuclear Information System (INIS)

    Delysse, Stephane

    1997-01-01

    We study some aspects of the nonlinear picosecond photo-physics in organic dyes using Kerr ellipsometry. The aim is to establish link between the photo-physics and nonlinear optics in these compounds. First, we study coherent processes directly linked to the third-order susceptibility. Thus, we measure two-photon absorption spectra of large internal charge transfer dyes. We take into account all coupling between three electronic states which can interfere to explain the particular response of some stilbene dyes. On the second hand, we expose a more photophysical approach to determine the S 1 → S n transition energies and moments using the measurement of excited state absorption cross sections. These results allow the prediction of the susceptibilities relevant to alternative nonlinear optical methods. Nevertheless, the stationary approach hides the complex relaxation processes which can take place in organic dyes. As an illustration, we study the formation and disappearance of a TICT (Twisted intramolecular charge transfer) in a pyrylium salt in solvents of increasing viscosity. (author) [fr

  20. Nonlinear-Optical and Fluorescent Properties of Ag Aqueous Colloid Prepared by Silver Nitrate Reduction

    Directory of Open Access Journals (Sweden)

    Xiaoqiang Zhang

    2010-01-01

    Full Text Available The nonlinear-optical properties of metal Ag colloidal solutions, which were prepared by the reduction of silver nitrate, were investigated using Z-scan method. Under picosecond 532 nm excitation, the Ag colloidal solution exhibited negative nonlinear refractive index (n2=−5.17×10−4 cm2/W and reverse saturable absorption coefficient (β=4.32 cm/GW. The data fitting result of optical limiting (OL response of metal Ag colloidal solution indicated that the nonlinear absorption was attributed to two-photon absorption effect at 532 nm. Moreover, the fluorescence emission spectra of Ag colloidal solution were recorded under excitations at both 280 nm and 350 nm. Two fluorescence peaks, 336 nm and 543 nm for 280 nm excitation, while 544 nm and 694 nm for 350 nm excitation, were observed.

  1. Modulation Instability of Copropagating Optical Beams in Fractional Coupled Nonlinear Schrödinger Equations

    Science.gov (United States)

    Zhang, Jinggui

    2018-06-01

    In this paper, we investigate the dynamical behaviors of the modulation instability (MI) of copropagating optical beams in fractional coupled nonlinear Schrödinger equations (NLSE) with the aim of revealing some novel properties different from those in the conventional coupled NLSE. By applying the standard linear stability method, we first derive an expression for the gain resulting from the instability induced by cross-phase modulation (CPM) in the presence of the Lévy indexes related to fractional effects. It is found that the modulation instability of copropagating optical beams still occurs even in the fractional NLSE with self-defocusing nonlinearity. Then, the analysis of our results further reveals that such Lévy indexes increase the fastest growth frequency and the bandwidth of conventional instability not only for the self-focusing case but also for the self-defocusing case, but do not influence the corresponding maximum gain. Numerical simulations are performed to confirm theoretical predictions. These findings suggest that the novel fractional physical settings may open up new possibilities for the manipulation of MI and nonlinear waves.

  2. HOMES - Holographic Optical Method for Exoplanet Spectroscopy

    Data.gov (United States)

    National Aeronautics and Space Administration — HOMES (Holographic Optical Method for Exoplanet Spectroscopy) is a space telescope that employs a double dispersion architecture, using a holographic optical element...

  3. Participation of the Third Order Optical Nonlinearities in Nanostructured Silver Doped Zinc Oxide Thin Solid Films

    Directory of Open Access Journals (Sweden)

    C. Torres-Torres

    2012-01-01

    Full Text Available We report the transmittance modulation of optical signals in a nanocomposite integrated by two different silver doped zinc oxide thin solid films. An ultrasonic spray pyrolysis approach was employed for the preparation of the samples. Measurements of the third-order nonlinear optical response at a nonresonant 532 nm wavelength of excitation were performed using a vectorial two-wave mixing. It seems that the separated contribution of the optical nonlinearity associated with each film noticeable differs in the resulting nonlinear effects with respect to the additive response exhibited by the bilayer system. An enhancement of the optical Kerr nonlinearity is predicted for prime number arrays of the studied nanoclusters in a two-wave interaction. We consider that the nanostructured morphology of the thin solid films originates a strong modification of the third-order optical phenomena exhibited by multilayer films based on zinc oxide.

  4. Third-order nonlinear optical studies of anthraquinone dyes using a CW He–Ne laser

    International Nuclear Information System (INIS)

    Pramodini, S; Poornesh, P

    2014-01-01

    We present investigations on the third-order optical nonlinearity and optical power limiting of anthraquinone dyes. Z-scan measurements were performed using a continuous wave He–Ne laser at 633 nm wavelength as an excitation source. The nonlinear refraction studies exhibited self-defocusing behavior of the dyes. The nonlinear absorption in the dyes was dominated by a reverse saturable absorption process. Self-diffraction ring patterns were observed due to the change in refractive index and thermal lensing. Increase of the electron donating ability of the substituents resulted in enhanced values of the nonlinear optical parameters, establishing the structure–property relationship. The optical limiting study revealed that the dyes possess a lower limiting threshold and clamping level which is very important for eye and sensor protection. Hence, the dyes investigated here emerge as promising candidates for future opto-electronic and photonic device applications such as optical power limiters. (paper)

  5. Third-order nonlinear optical studies of anthraquinone dyes using a CW He-Ne laser

    Science.gov (United States)

    Pramodini, S.; Poornesh, P.

    2014-05-01

    We present investigations on the third-order optical nonlinearity and optical power limiting of anthraquinone dyes. Z-scan measurements were performed using a continuous wave He-Ne laser at 633 nm wavelength as an excitation source. The nonlinear refraction studies exhibited self-defocusing behavior of the dyes. The nonlinear absorption in the dyes was dominated by a reverse saturable absorption process. Self-diffraction ring patterns were observed due to the change in refractive index and thermal lensing. Increase of the electron donating ability of the substituents resulted in enhanced values of the nonlinear optical parameters, establishing the structure-property relationship. The optical limiting study revealed that the dyes possess a lower limiting threshold and clamping level which is very important for eye and sensor protection. Hence, the dyes investigated here emerge as promising candidates for future opto-electronic and photonic device applications such as optical power limiters.

  6. A modal method for finite amplitude, nonlinear sloshing

    Indian Academy of Sciences (India)

    A modal method is used to calculate the two-dimensional sloshing motion of an inviscid liquid in a rectangular container. The full nonlinear problem is reduced to the solution of a system of nonlinear ordinary differential equations for the time varying coefficients in the expansions of the interface and the potential. The effects ...

  7. A modal method for finite amplitude, nonlinear sloshing

    Indian Academy of Sciences (India)

    Abstract. A modal method is used to calculate the two-dimensional sloshing motion of an inviscid liquid in a rectangular container. The full nonlinear problem is reduced to the solution of a system of nonlinear ordinary differential equations for the time varying coefficients in the expansions of the interface and the potential.

  8. Symbolic computation and solitons of the nonlinear Schroedinger equation in inhomogeneous optical fiber media

    International Nuclear Information System (INIS)

    Li Biao; Chen Yong

    2007-01-01

    In this paper, the inhomogeneous nonlinear Schroedinger equation with the loss/gain and the frequency chirping is investigated. With the help of symbolic computation, three families of exact analytical solutions are presented by employing the extended projective Riccati equation method. From our results, many previous known results of nonlinear Schroedinger equation obtained by some authors can be recovered by means of some suitable selections of the arbitrary functions and arbitrary constants. Of optical and physical interests, soliton propagation and soliton interaction are discussed and simulated by computer, which include snake-soliton propagation and snake-solitons interaction, boomerang-like soliton propagation and boomerang-like solitons interaction, dispersion managed (DM) bright (dark) soliton propagation and DM solitons interaction

  9. Design considerations for multi component molecular-polymeric nonlinear optical materials

    Energy Technology Data Exchange (ETDEWEB)

    Singer, K.D. (Case Western Reserve Univ., Cleveland, OH (USA). Dept. of Physics); Kuzyk, M.G. (Washington State Univ., Pullman, WA (USA). Dept. of Physics); Fang, T.; Holland, W.R. (AT and T Bell Labs., Princeton, NJ (USA)); Cahill, P.A. (Sandia National Labs., Albuquerque, NM (USA))

    1990-01-01

    We review our work on multi component polymeric nonlinear optical materials. These materials consist of nonlinear optical molecules incorporated in a polymeric host. A cross-linked triazine polymer incorporating a dicyanovinyl terminated azo dye was found to be relatively stable at 85{degree} and posses an electro-optic coefficient of 11pm/V. We have also observed the zero dispersion condition in a new anomalous dispersion dye for phase matched second harmonic generation, and expect efficient conversion to the blue. A squarylium dye, ISQ, has been found to posses a large third order nonlinearity, and may display two-level behavior. 24 refs., 11 figs.

  10. Optical polarization based logic functions (XOR or XNOR) with nonlinear Gallium nitride nanoslab.

    Science.gov (United States)

    Bovino, F A; Larciprete, M C; Giardina, M; Belardini, A; Centini, M; Sibilia, C; Bertolotti, M; Passaseo, A; Tasco, V

    2009-10-26

    We present a scheme of XOR/XNOR logic gate, based on non phase-matched noncollinear second harmonic generation from a medium of suitable crystalline symmetry, Gallium nitride. The polarization of the noncollinear generated beam is a function of the polarization of both pump beams, thus we experimentally investigated all possible polarization combinations, evidencing that only some of them are allowed and that the nonlinear interaction of optical signals behaves as a polarization based XOR. The experimental results show the peculiarity of the nonlinear optical response associated with noncollinear excitation, and are explained using the expression for the effective second order optical nonlinearity in noncollinear scheme.

  11. Thermally Stable Heterocyclic Imines as New Potential Nonlinear Optical Materials

    Science.gov (United States)

    Nesterov, Volodymyr V.; Antipin, Mikhail Y.; Nesterov, Vladimir N.; Moore, Craig E.; Cardelino, Beatriz H.; Timofeeva, Tatiana V.

    2004-01-01

    In the course of a search for new thermostable acentric nonlinear optical crystalline materials, several heterocyclic imine derivatives were designed, with the general structure D-pi-A(D'). Introduction of a donor amino group (D') into the acceptor moiety was expected to bring H-bonds into their crystal structures, and so to elevate their melting points and assist in an acentric molecular packing. Six heterocycle-containing compounds of this type were prepared, single crystals were grown for five of them, and these crystals were characterized by X-ray analysis. A significant melting temperature elevation was found for all of the synthesized compounds. Three of the compounds were also found to crystallize in acentric space groups. One of the acentric compounds is built as a three-dimensional H-bonded molecular network. In the other two compounds, with very similar molecular structure, the molecules form one-dimensional H-bonded head-to-head associates (chains). These chains are parallel in two different crystallographic directions and form very unusual interpenetrating chain patterns in an acentric crystal. Two of the compounds crystallized with centrosymmetric molecular packing.

  12. Nonlinear optical properties of Sn+ ion-implanted silica glass

    International Nuclear Information System (INIS)

    Takeda, Y.; Hioki, T.; Motohiro, T.; Noda, S.; Kurauchi, T.

    1994-01-01

    The absolute value of the third-order nonlinear optical susceptibility, vertical stroke χ (3) vertical stroke , of Sn + ion-implanted silica glass was found to be similar 10 -6 esu. This value is as large as those reported for semiconductor-doped glasses. Silica glass substrates were implanted with Sn + ions at an acceleration energy of 400 keV to a dose of 2x10 17 ions/cm 2 at room temperature. Metallic Sn microcrystallites of 4-20 nm in diameter were found to be embedded in the silica glass matrix. The average volume fraction of the Sn microcrystallites was evaluated to be 28%. vertical stroke χ (3) vertical stroke and the imaginary part of the dielectric function, Im ε, had peaks at the same wavelength of 500 nm owing to surface plasmon resonance. The peak width of vertical stroke χ (3) vertical stroke was nearly half of that of Im ε, which can be explained by an effective medium theory. ((orig.))

  13. Second-Order Nonlinear Optical Dendrimers and Dendronized Hyperbranched Polymers.

    Science.gov (United States)

    Tang, Runli; Li, Zhen

    2017-01-01

    Second-order nonlinear optical (NLO) dendrimers with a special topological structure were regarded as the most promising candidates for practical applications in the field of optoelectronic materials. Dendronized hyperbranched polymers (DHPs), a new type of polymers with dendritic structures, proposed and named by us recently, demonstrated interesting properties and some advantages over other polymers. Some of our work concerning these two types of polymers are presented herein, especially focusing on the design idea and structure-property relationship. To enhance their comprehensive NLO performance, dendrimers were designed and synthesized by adjusting their isolation mode, increasing the number of the dendritic generation, modifying their topological structure, introducing isolation chromophores, and utilizing the Ar-Ar F self-assembly effect. To make full use of the advantages of both the structural integrity of dendrimers and the convenient one-pot synthesis of hyperbranched polymers, DHPs were explored by utilizing low-generation dendrons as big monomers to construct hyperbranched polymers. These selected works could provide valuable information to deeply understand the relationship between the structure and properties of functional polymers with dendritic structures, but not only limited to the NLO ones, and might contribute much to the further development of functional polymers with rational design. © 2017 The Chemical Society of Japan & Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

  14. Analysis of nonlinear optical properties in donor–acceptor materials

    Energy Technology Data Exchange (ETDEWEB)

    Day, Paul N. [Air Force Research Laboratory, Wright-Patterson Air Force Base, Ohio 45433 (United States); General Dynamics Information Technology, Inc., Dayton, Ohio 45431 (United States); Pachter, Ruth [Air Force Research Laboratory, Wright-Patterson Air Force Base, Ohio 45433 (United States); Nguyen, Kiet A. [Air Force Research Laboratory, Wright-Patterson Air Force Base, Ohio 45433 (United States); UES, Inc., Dayton, Ohio 45432 (United States)

    2014-05-14

    Time-dependent density functional theory has been used to calculate nonlinear optical (NLO) properties, including the first and second hyperpolarizabilities as well as the two-photon absorption cross-section, for the donor-acceptor molecules p-nitroaniline and dimethylamino nitrostilbene, and for respective materials attached to a gold dimer. The CAMB3LYP, B3LYP, PBE0, and PBE exchange-correlation functionals all had fair but variable performance when compared to higher-level theory and to experiment. The CAMB3LYP functional had the best performance on these compounds of the functionals tested. However, our comprehensive analysis has shown that quantitative prediction of hyperpolarizabilities is still a challenge, hampered by inadequate functionals, basis sets, and solvation models, requiring further experimental characterization. Attachment of the Au{sub 2}S group to molecules already known for their relatively large NLO properties was found to further enhance the response. While our calculations show a modest enhancement for the first hyperpolarizability, the enhancement of the second hyperpolarizability is predicted to be more than an order of magnitude.

  15. Low-cost nonlinear optics experiment for undergraduate instructional laboratory and lecture demonstration

    Science.gov (United States)

    Turchiello, Rozane de F.; Pereira, Luiz A. A.; Gómez, Sergio L.

    2017-07-01

    This paper presents a simple and affordable experiment on the thermal lens effect, suitable for an undergraduate educational laboratory or as a tabletop demonstration in a lecture on nonlinear optics. Such an experiment exploits the formation of a lens in an absorbing medium illuminated by a laser beam with a Gaussian intensity profile. As an absorber, we use a commercial soy sauce, which exhibits a strong thermal lensing effect. Additionally, we show how to measure the radius of a Gaussian beam using the knife-edge method, and how to estimate the focal length of the induced thermal lens.

  16. SOLVING NONLINEAR KLEIN-GORDON EQUATION WITH A QUADRATIC NONLINEAR TERM USING HOMOTOPY ANALYSIS METHOD

    Directory of Open Access Journals (Sweden)

    H. Jafari

    2010-07-01

    Full Text Available In this paper, nonlinear Klein-Gordon equation with quadratic term is solved by means of an analytic technique, namely the Homotopy analysis method (HAM.Comparisons are made between the Adomian decomposition method (ADM, the exact solution and homotopy analysis method. The results reveal that the proposed method is very effective and simple.

  17. Nonlinear Optical Response of Polar Semiconductors in the Terahertz Range

    Science.gov (United States)

    Roman, Eric; Yates, Jonathan; Veithen, Marek; Vanderbilt, David; Souza, Ivo

    2006-03-01

    Using the Berry-phase finite-field method, we compute from first-principles the recently measured infrared (IR) dispersion of the nonlinear susceptibility (2)circ in III-V zincblende semiconductors. At far-IR (terahertz) frequencies, in addition to the purely electronic response (2)circ∞, the total (2)circ depends on three other parameters, C1, C2, and C3, describing the contributions from ionic motion. They relate to the TO Raman polarizability and the second-order displacement-induced dielectric polarization and forces, respectively. Contrary to a widely-accepted model, but in agreement with the recent experiments on GaAs, ^1 we find that the contribution from mechanical anharmonicity dominates over electrical anharmonicity. By using Richardson extrapolation to evaluate the Berry's phase in k-space by finite differences, we are able to improve the convergence of the nonlinear susceptibility from the usual O[(δk)^2] to O[(δk)^4], dramatically reducing the computational cost. T. Dekorsy, V. A. Yakovlev, W. Seidel, M. Helm, and F. Keilmann, Phys. Rev. Lett. 90, 055508 (2003). C. Flytzanis, Phys. Rev. B 6, 1264 (1972). R. Umari and A. Pasquarello, Phys. Rev. B 68, 085114 (2003).

  18. GHM method for obtaining rationalsolutions of nonlinear differential equations.

    Science.gov (United States)

    Vazquez-Leal, Hector; Sarmiento-Reyes, Arturo

    2015-01-01

    In this paper, we propose the application of the general homotopy method (GHM) to obtain rational solutions of nonlinear differential equations. It delivers a high precision representation of the nonlinear differential equation using a few linear algebraic terms. In order to assess the benefits of this proposal, three nonlinear problems are solved and compared against other semi-analytic methods or numerical methods. The obtained results show that GHM is a powerful tool, capable to generate highly accurate rational solutions. AMS subject classification 34L30.

  19. Non-linear programming method in optimization of fast reactors

    International Nuclear Information System (INIS)

    Pavelesku, M.; Dumitresku, Kh.; Adam, S.

    1975-01-01

    Application of the non-linear programming methods on optimization of nuclear materials distribution in fast reactor is discussed. The programming task composition is made on the basis of the reactor calculation dependent on the fuel distribution strategy. As an illustration of this method application the solution of simple example is given. Solution of the non-linear program is done on the basis of the numerical method SUMT. (I.T.)

  20. Linear and nonlinear optical characteristics of Te nanoparticles-doped germanate glasses

    Science.gov (United States)

    Xu, Zhousu; Guo, Qiangbing; Liu, Chang; Ma, Zhijun; Liu, Xiaofeng; Qiu, Jianrong

    2016-10-01

    Te nanoparticles (NPs)-doped GeO2-MgO-B2O3-Al2O3-TeO2 glasses were prepared by the conventional melt-quenching method. Based on X-ray photoelectron spectroscopy, Raman spectroscopy and transmission electron microscope observation, the coloration of the glass at high TeO2 concentration is ascribed to the precipitation of elemental Te NPs with a size of 5-10 nm in the germanate glass. Optical absorption spectra and nonlinear optical (NLO) properties of the glass samples were analyzed by UV-3600 spectrophotometry and Z-scan technique, respectively. The nonlinear absorption coefficient ( β) and the imaginary part of the third-order NLO susceptibility (Im χ (3)) were estimated to be 1.74 cm/GW and 1.142 × 10-12 esu for laser power of 95 μW, respectively. Due to the excellent NLO properties, the Te NPs-doped germanate glasses may have potential applications for ultrafast optical switch and photonics.

  1. Homogenous smooth sol gel films doped with organic compounds for nonlinear optics

    Energy Technology Data Exchange (ETDEWEB)

    Vasiliu, I.C. [INOE 2000 — National Institute for Optoelectronics, 409 Atomistilor Str., Magurele, Bucharest, RO 077125 (Romania); Ionita, I., E-mail: i_ionita@yahoo.com [UB — University of Bucharest, 405 Atomistilor Str., Magurele, Bucharest, RO 077125 (Romania); Matei, A. [INFLPR — National Institute for Laser, Plasma and Radiation Physics, 409 Atomistilor Str., Magurele, Bucharest, RO 077125 (Romania); Elisa, M.; Iordanescu, R.; Feraru, I.; Emandi, A. [INOE 2000 — National Institute for Optoelectronics, 409 Atomistilor Str., Magurele, Bucharest, RO 077125 (Romania)

    2016-02-29

    The demand for protection of various types of optical sensors from laser-beam pulses has resulted in the search for optical limiting devices that have the property of being transparent at low intensity of light (normal light), but no transparent towards high intensity (laser) light. Organic material with nonlinear optical (NLO) properties as reverse saturable absorption and two-photon absorption can be used for optical limiting with the advantage of a very fast response and self-activation. A promising approach in the fabrication of thin films by low cost/easy use deposition methods for second-order nonlinear optics is sol–gel technique. The present paper reports on the sol–gel synthesis of some pyrazolone derivative doped SiO{sub 2}–P{sub 2}O{sub 5} smooth and homogenous films (Root mean square roughness (Rq) = 1.1 nm) using as precursors tetraethylorthosilicate (TEOS) and phosphoric acid (H{sub 3}PO{sub 4}). The structure of the deposited azo-derivatives doped thin films was examined by Fourier transform infrared spectroscopy and atomic force microscopy, while their optical properties of the films by UV–VIS spectroscopy. The nonlinear optical efficiencies due to the interaction of the NLO-active chromophores with the inorganic matrix have a significant influence on the second harmonic generation capabilities that was measured using a femtosecond Ti:Sapphire laser. The properties of the films were investigated and correlated with the concentration of the organic dopant and the thermal treatment temperature. - Highlights: • We obtained pyrazolone derivative doped SiO{sub 2}–P{sub 2}O{sub 5} smooth and homogenous films. • The pyrazolone derivative presents SHG characteristics by itself. • Thin sol gel films doped with organic compounds with NLO properties. • Temperature of thermal treatment and aging time can improve NLO properties of films. • We found that 150 °C and 28 h aging time give the maximum performance in SHG response.

  2. ROTAX: a nonlinear optimization program by axes rotation method

    International Nuclear Information System (INIS)

    Suzuki, Tadakazu

    1977-09-01

    A nonlinear optimization program employing the axes rotation method has been developed for solving nonlinear problems subject to nonlinear inequality constraints and its stability and convergence efficiency were examined. The axes rotation method is a direct search of the optimum point by rotating the orthogonal coordinate system in a direction giving the minimum objective. The searching direction is rotated freely in multi-dimensional space, so the method is effective for the problems represented with the contours having deep curved valleys. In application of the axes rotation method to the optimization problems subject to nonlinear inequality constraints, an improved version of R.R. Allran and S.E.J. Johnsen's method is used, which deals with a new objective function composed of the original objective and a penalty term to consider the inequality constraints. The program is incorporated in optimization code system SCOOP. (auth.)

  3. An iterative kernel based method for fourth order nonlinear equation with nonlinear boundary condition

    Science.gov (United States)

    Azarnavid, Babak; Parand, Kourosh; Abbasbandy, Saeid

    2018-06-01

    This article discusses an iterative reproducing kernel method with respect to its effectiveness and capability of solving a fourth-order boundary value problem with nonlinear boundary conditions modeling beams on elastic foundations. Since there is no method of obtaining reproducing kernel which satisfies nonlinear boundary conditions, the standard reproducing kernel methods cannot be used directly to solve boundary value problems with nonlinear boundary conditions as there is no knowledge about the existence and uniqueness of the solution. The aim of this paper is, therefore, to construct an iterative method by the use of a combination of reproducing kernel Hilbert space method and a shooting-like technique to solve the mentioned problems. Error estimation for reproducing kernel Hilbert space methods for nonlinear boundary value problems have yet to be discussed in the literature. In this paper, we present error estimation for the reproducing kernel method to solve nonlinear boundary value problems probably for the first time. Some numerical results are given out to demonstrate the applicability of the method.

  4. Enhanced nonlinear optical absorption and optical limiting properties of superparamagnetic spinel zinc ferrite decorated reduced graphene oxide nanostructures

    International Nuclear Information System (INIS)

    Saravanan, M.; Sabari Girisun, T.C.

    2017-01-01

    Highlights: • Nanospindle and nanosphere ZnFe_2O_4 were decorated upon GO by hydrothermal method. • All the samples show superparamagnetism with almost zero coercivity and remanence. • The observed nonlinearity arises due to effective two photon absorption process. • Tuning of NLO behavior with variation in amount of ZnFe_2O_4 upon GO were achieved. • ZnFe_2O_4-(15 wt%)GO show higher NLO coefficients and superior limiting actions. - Abstract: Nonlinear absorption and optical limiting properties of ZnFe_2O_4-rGO magnetic nanostructures was investigated by the Z-scan technique using Q-switched Nd:YAG laser (5 ns, 532 nm, 10 Hz) as an excitation source. Excited state absorption was the dominant process responsible for the observed nonlinearity in ZnFe_2O_4 decorated rGO which arises due to photo-generated charge carriers in the conduction band of zinc ferrite and increases in defects at the surface of rGO due to the incorporation of ZnFe_2O_4. The magnitude of the nonlinear absorption co-efficient was found to be in the order of 10"−"1"0 m/W. A noteworthy enhancement in the third-order NLO properties in ZnFe_2O_4-(15 wt%) rGO with those of individual counter parts and well known graphene composites was reported. Role of induced defects states (sp"3) arising from the functionalization of rGO in the enhancement of NLO response was explained through Raman studies. Earlier incorporation and distribution of ZnFe_2O_4 upon GO through one-step hydrothermal method was analyzed by XRD and FTIR. Formation of (nanospheres/nanospindles) ZnFe_2O_4 along with reduction of graphene oxide was confirmed through TEM analysis. VSM studies showed zinc ferrite decorated rGO posseses superparamagnetic behavior. The tuning of nonlinear optical and magnetic behavior with variation in the content of spinel ferrites upon reduced graphene oxide provides an easy way to attain tunable properties which are exceedingly required in both optoelectronics and photothermal therapy

  5. Enhanced nonlinear optical absorption and optical limiting properties of superparamagnetic spinel zinc ferrite decorated reduced graphene oxide nanostructures

    Energy Technology Data Exchange (ETDEWEB)

    Saravanan, M.; Sabari Girisun, T.C., E-mail: sabarigirisun@bdu.ac.in

    2017-01-15

    Highlights: • Nanospindle and nanosphere ZnFe{sub 2}O{sub 4} were decorated upon GO by hydrothermal method. • All the samples show superparamagnetism with almost zero coercivity and remanence. • The observed nonlinearity arises due to effective two photon absorption process. • Tuning of NLO behavior with variation in amount of ZnFe{sub 2}O{sub 4} upon GO were achieved. • ZnFe{sub 2}O{sub 4}-(15 wt%)GO show higher NLO coefficients and superior limiting actions. - Abstract: Nonlinear absorption and optical limiting properties of ZnFe{sub 2}O{sub 4}-rGO magnetic nanostructures was investigated by the Z-scan technique using Q-switched Nd:YAG laser (5 ns, 532 nm, 10 Hz) as an excitation source. Excited state absorption was the dominant process responsible for the observed nonlinearity in ZnFe{sub 2}O{sub 4} decorated rGO which arises due to photo-generated charge carriers in the conduction band of zinc ferrite and increases in defects at the surface of rGO due to the incorporation of ZnFe{sub 2}O{sub 4}. The magnitude of the nonlinear absorption co-efficient was found to be in the order of 10{sup −10} m/W. A noteworthy enhancement in the third-order NLO properties in ZnFe{sub 2}O{sub 4}-(15 wt%) rGO with those of individual counter parts and well known graphene composites was reported. Role of induced defects states (sp{sup 3}) arising from the functionalization of rGO in the enhancement of NLO response was explained through Raman studies. Earlier incorporation and distribution of ZnFe{sub 2}O{sub 4} upon GO through one-step hydrothermal method was analyzed by XRD and FTIR. Formation of (nanospheres/nanospindles) ZnFe{sub 2}O{sub 4} along with reduction of graphene oxide was confirmed through TEM analysis. VSM studies showed zinc ferrite decorated rGO posseses superparamagnetic behavior. The tuning of nonlinear optical and magnetic behavior with variation in the content of spinel ferrites upon reduced graphene oxide provides an easy way to attain tunable

  6. Microscopic investigations of the terahertz and the extreme nonlinear optical response of semiconductors

    Energy Technology Data Exchange (ETDEWEB)

    Golde, Daniel

    2010-06-22

    In the major part of this Thesis, we discuss the linear THz response of semiconductor nanostructures based on a microscopic theory. Here, two different problems are investigated: intersubband transitions in optically excited quantum wells and the THz plasma response of two-dimensional systems. In the latter case, we analyze the response of correlated electron and electron-hole plasmas. Extracting the plasma frequency from the linear response, we find significant deviations from the commonly accepted two-dimensional plasma frequency. Besides analyzing the pure plasma response, we also consider an intermediate regime where the response of the electron-hole plasma consists of a mixture of plasma contributions and excitonic transitions. A quantitative experiment-theory comparison provides novel insights into the behavior of the system at the transition from one regime to the other. The discussion of the intersubband transitions mainly focuses on the coherent superposition of the responses from true THz transitions and the ponderomotively accelerated carriers. We present a simple method to directly identify ponderomotive effects in the linear THz response. Apart from that, the excitonic contributions to intersubband transitions are investigated. The last part of the present Thesis deals with a completely different regime. Here, the extreme nonlinear optical response of low-dimensional semiconductor structures is discussed. Formally, extreme nonlinear optics describes the regime of light-matter interaction where the exciting field is strong enough such that the Rabi frequency is comparable to or larger than the characteristic transition frequency of the investigated system. Here, the Rabi frequency is given by the product of the electrical field strength and the dipole-matrix element of the respective transition. Theoretical investigations have predicted a large number of novel nonlinear effects arising for such strong excitations. Some of them have been observed in

  7. Non-linear optical techniques and optical properties of condensed molecular systems

    Science.gov (United States)

    Citroni, Margherita

    2013-06-01

    Structure, dynamics, and optical properties of molecular systems can be largely modified by the applied pressure, with remarkable consequences on their chemical stability. Several examples of selective reactions yielding technologically attractive products can be cited, which are particularly efficient when photochemical effects are exploited in conjunction with the structural conditions attained at high density. Non-linear optical techniques are a basic tool to unveil key aspects of the chemical reactivity and dynamic properties of molecules. Their application to high-pressure samples is experimentally challenging, mainly because of the small sample dimensions and of the non-linear effects generated in the anvil materials. In this talk I will present results on the electronic spectra of several aromatic crystals obtained through two-photon induced fluorescence and two-photon excitation profiles measured as a function of pressure (typically up to about 25 GPa), and discuss the relationship between the pressure-induced modifications of the electronic structure and the chemical reactivity at high pressure. I will also present the first successful pump-probe infrared measurement performed as a function of pressure on a condensed molecular system. The system under examination is liquid water, in a sapphire anvil cell, up to 1 GPa along isotherms at 298 and 363 K. These measurements give a new enlightening insight into the dynamical properties of low- and high-density water allowing a definition of the two structures.

  8. COMPARISON OF NONLINEAR DYNAMICS OPTIMIZATION METHODS FOR APS-U

    Energy Technology Data Exchange (ETDEWEB)

    Sun, Y.; Borland, Michael

    2017-06-25

    Many different objectives and genetic algorithms have been proposed for storage ring nonlinear dynamics performance optimization. These optimization objectives include nonlinear chromaticities and driving/detuning terms, on-momentum and off-momentum dynamic acceptance, chromatic detuning, local momentum acceptance, variation of transverse invariant, Touschek lifetime, etc. In this paper, the effectiveness of several different optimization methods and objectives are compared for the nonlinear beam dynamics optimization of the Advanced Photon Source upgrade (APS-U) lattice. The optimized solutions from these different methods are preliminarily compared in terms of the dynamic acceptance, local momentum acceptance, chromatic detuning, and other performance measures.

  9. Computational Study of Chalcopyrite Semiconductors and Their Non-Linear Optical Properties

    National Research Council Canada - National Science Library

    Lambrecht, Walter R

    2007-01-01

    ... (Including cation antisites, cation and anion vacancies) and CdGeAs2; a study of the feasibility of nonciritical phase matching and associated nonlinear optical parameters in CdSiP2 and CdSIAs2...

  10. Self-Assembly of Nanocomposite Nonlinear Optical Materials for Photonic Devices, Phase I

    Data.gov (United States)

    National Aeronautics and Space Administration — This program targets the development of new highly anisotropic nonlinear optical nanocomposite materials for NASA and non-NASA applications in advanced photonic and...

  11. Studies of Second Order Optical Nonlinearities of 4-Aminobenzophenone (ABP) Single Crystal Films

    Science.gov (United States)

    Bhowmik, Achintya; Thakur, Mrinal

    1998-03-01

    Specific organic materials exhibit very high second order optical susceptibilities. Growth of single crystal films of these materials and characterization of nonlinear optical properties are necessary for implementation of device applications. We have grown large-area films ( 1 cm^2 area, 4 μm thick) of ABP by a modification of the shear method. Single crystal nature of the films was confirmed by polarized optical microscopy. X-ray diffraction analysis showed a [100] surface orientation. The absorption spectra revealed transparency from 390 nm to 1940 nm. Significant elements of the second order optical susceptibility tensor were measured by detailed SHG experiments using a Nd:YAG laser (1064 nm, 100 ps, 82 MHz). Second-harmonic power was measured using lock-in detection with carefully selected polarization conditions while the film was rotated about the propagation direction. Using LiNbØas the reference, d-coefficients of ABP were found to be d_23=7.2 pm/V and d_22=0.7 pm/V. Type-I and type-II phase-matching directions were identified on the film by analyzing the optical indicatrix surfaces at fundamental and second-harmonic frequencies.

  12. Method of lightening radiation darkened optical elements

    International Nuclear Information System (INIS)

    Reich, F.R.; Schwankoff, A.R.

    1980-01-01

    A method of lightening a radiation-darkened optical element in which visible optical energy or electromagnetic radiation having a wavelength in the range of from about 2000 to about 20,000 angstroms is directed into the radiation-darkened optical element; the method may be used to lighten radiation-darkened optical element in-situ during the use of the optical element to transmit data by electronically separating the optical energy from the optical output by frequency filtering, data cooling, or interlacing the optic energy between data intervals

  13. Optical-Gravitation Nonlinearity: A Change of Gravitational Coefficient G induced by Gravitation Field

    OpenAIRE

    R. Vlokh; M. Kostyrko

    2006-01-01

    Nonlinear effect of the gravitation field of spherically symmetric mass on the gravitational coefficient G has been analysed. In frame of the approaches of parametric optics and gravitation nonlinearity we have shown that the gravitation field of spherically symmetric mass can lead to changes in the gravitational coefficient G.

  14. Measurement of picometre non-linearity in an optical grating encoder using x-ray interferometry

    Science.gov (United States)

    Yacoot, Andrew; Cross, Nigel

    2003-01-01

    X-ray interferometry has been used to characterize the non-linearity in an optical encoder displacement measuring system. Traceable measurements of the non-linearity have been made and an estimation of the uncertainty associated with the measurements is given. Cyclic errors with a magnitude of up to 50 pm and periodicity of the encoder system (128 nm) have been recorded.

  15. Dual-polarization nonlinear Fourier transform-based optical communication system

    DEFF Research Database (Denmark)

    Gaiarin, Simone; Perego, A. M.; da Silva, Edson Porto

    2018-01-01

    communication could potentially overcome these limitations. It relies on a mathematical technique called “nonlinear Fourier transform (NFT)” to exploit the “hidden” linearity of the nonlinear Schrödinger equation as the master model for signal propagation in an optical fiber. We present here the theoretical...

  16. Nonlinear optics with broad-band lasers: Progress report, July 15, 1987-April 14, 1988

    International Nuclear Information System (INIS)

    Raymer, M.G.

    1988-01-01

    During this reporting period several important results were obtained on the fluctuation dynamics of both continuous-wave (cw) and pulsed dye lasers, as well as their effects in certain nonlinear optical processes: (1) A new method discovered for producing optical pulses with broad bandwidths (5 GHz) and smooth, slowly varying amplitude. The bandwidth is determined purely by phase fluctuations. (2) A theoretical treatment of pulsed dye lasers was developed to explain intensity autocorrelation measurements. (3) The effects of laser bandwidth on the resonance fluorescence spectrum of a two-level atom were calculated. (4) The source of mode intensity fluctuations in a multimode, cw dye laser were shown, both experimentally and theoretically, to be caused by deterministic chaos, rather than quantum noise as had been previously assumed in the literature

  17. Analysis of adjusting effects of mounting force on frequency conversion of mounted nonlinear optics.

    Science.gov (United States)

    Su, Ruifeng; Liu, Haitao; Liang, Yingchun; Lu, Lihua

    2014-01-10

    Motivated by the need to increase the second harmonic generation (SHG) efficiency of nonlinear optics with large apertures, a novel mounting configuration with active adjusting function on the SHG efficiency is proposed and mechanically and optically studied. The adjusting effects of the mounting force on the distortion and stress are analyzed by the finite element methods (FEM), as well as the contribution of the distortion and stress to the change in phase mismatch, and the SHG efficiency are theoretically stated. Further on, the SHG efficiency is calculated as a function of the mounting force. The changing trends of the distortion, stress, and the SHG efficiency with the varying mounting force are obtained, and the optimal ones are figured out. Moreover, the mechanism of the occurrence of the optimal values is studied and the adjusting strategy is put forward. Numerical results show the robust adjustment of the mounting force, as well as the effectiveness of the mounting configuration, in increasing the SHG efficiency.

  18. Inverse operator theory method and its applications in nonlinear physics

    International Nuclear Information System (INIS)

    Fang Jinqing

    1993-01-01

    Inverse operator theory method, which has been developed by G. Adomian in recent years, and its applications in nonlinear physics are described systematically. The method can be an unified effective procedure for solution of nonlinear and/or stochastic continuous dynamical systems without usual restrictive assumption. It is realized by Mathematical Mechanization by us. It will have a profound on the modelling of problems of physics, mathematics, engineering, economics, biology, and so on. Some typical examples of the application are given and reviewed

  19. Impressive nonlinear optical response exhibited by Poly(vinylidene fluoride) (PVDF)/reduced graphene oxide (RGO) nanocomposite films

    Science.gov (United States)

    Sabira, K.; Saheeda, P.; Divyasree, M. C.; Jayalekshmi, S.

    2017-12-01

    In the present work, the nonlinear optical properties of free-standing films of Poly(vinylidene fluoride) (PVDF)/reduced graphene oxide (RGO) nanocomposite are investigated to assess their suitability as efficient optical limiters. The PVDF/RGO nanocomposite films are generated by mixing different concentrations of RGO as the filler, with PVDF, using solution casting method. The XRD and FTIR data of these nanocomposite films confirm the enhancement in the β phase of PVDF when RGO is added to PVDF, which is one of the prime factors, enhancing the nonlinear response of the nanocomposite. The open aperture and closed aperture Z-scan technique under nanosecond excitation (532 nm, 7 ns) is used to investigate the nonlinear optical characteristics of the PVDF/RGO nanocomposite films. These films are found to exhibit two photon absorption assisted optical non linearity in the nanosecond regime. The highlight of the present work is the observation of quite low values of the normalized transmittance and low optical limiting threshold power in free standing films of PVDF/RGO nanocomposite. These flexible, free-standing and stable nanocomposite films offer high application prospects in the design of efficient optical limiting devices of any desired size or shape.

  20. In situ 3D characterization of historical coatings and wood using multimodal nonlinear optical microscopy

    OpenAIRE

    Latour , Gaël; Echard , Jean-Philippe; Didier , Marie; Schanne-Klein , Marie-Claire

    2012-01-01

    International audience; We demonstrate multimodal nonlinear optical imaging of historical artifacts by combining Second Harmonic Generation (SHG) and Two-Photon Excited Fluorescence (2PEF) microscopies. We first identify the nonlinear optical response of materials commonly encountered in coatings of cultural heritage artifacts by analyzing one- and multi-layered model samples. We observe 2PEF signals from cochineal lake and sandarac and show that pigments and varnish films can be discriminate...

  1. Characterization of the bistable wideband optical filter on the basis of nonlinear 2D photonic crystal

    Energy Technology Data Exchange (ETDEWEB)

    Guryev, I. V., E-mail: guryev@ieee.org; Sukhoivanov, I. A., E-mail: guryev@ieee.org; Andrade Lucio, J. A., E-mail: guryev@ieee.org; Manzano, O. Ibarra, E-mail: guryev@ieee.org; Rodriguez, E. Vargaz, E-mail: guryev@ieee.org; Gonzales, D. Claudio, E-mail: guryev@ieee.org; Chavez, R. I. Mata, E-mail: guryev@ieee.org; Gurieva, N. S., E-mail: guryev@ieee.org [University of Guanajuato, Engineering division (Mexico)

    2014-05-15

    In our work, we investigated the wideband optical filter on the basis of nonlinear photonic crystal. The all-optical flip-flop using ultra-short pulses with duration lower than 200 fs is obtained in such filters. Here we pay special attention to the stability problem of the nonlinear element. To investigate this problem, the temporal response demonstrating the flip-flop have been computed within the certain range of the wavelengths as well as at different input power.

  2. An ultra-efficient nonlinear planar integrated platform for optical signal processing and generation

    DEFF Research Database (Denmark)

    Pu, Minhao; Ottaviano, Luisa; Semenova, Elizaveta

    2017-01-01

    This paper will discuss the recently developed integrated platform: AlGaAs-oninsulator and its broad range of nonlinear applications. Recent demonstrations of broadband optical signal processing and efficient frequency comb generations in this platform will be reviewed.......This paper will discuss the recently developed integrated platform: AlGaAs-oninsulator and its broad range of nonlinear applications. Recent demonstrations of broadband optical signal processing and efficient frequency comb generations in this platform will be reviewed....

  3. Focus scanning with feedback control for fiber-optic nonlinear endomicroscopy (Conference Presentation)

    Science.gov (United States)

    Li, Ang; Liang, Wenxuan; Li, Xingde

    2017-02-01

    Fiber-optic nonlinear endomicroscopy represents a strong promise to enable translation of nonlinear microscopy technologies to in vivo applications, particularly imaging of internal organs. Two-dimensional imaging beam scanning has been accomplished by using fiber-optic scanners or MEMS scanners. Yet nonlinear endomicroscopy still cannot perform rapid and reliable depth or focus scanning while maintaining a small form factor. Shape memory alloy (SMA) wire had shown promise in extending 2D endoscopic imaging to the third dimension. By Joule heating, the SMA wire would contract and move the endomicroscope optics to change beam focus. However, this method suffered from hysteresis, and was susceptible to change in ambient temperature, making it difficult to achieve accurate and reliable depth scanning. Here we present a feedback-controlled SMA actuator which addressed these challenges. The core of the feedback loop was a Hall effect sensor. By measuring the magnetic flux density from a tiny magnet attached to the SMA wire, contraction distance of the SMA wire could be tracked in real time. The distance was then fed to the PID algorithm running in a microprocessor, which computed the error between the command position and the current position of the actuator. The current running through the SMA wire was adjusted accordingly. Our feedback-controlled SMA actuator had a tube-like shape with outer diameter of 5.5 mm and length of 25 mm, and was designed to house the endomicroscope inside. Initial test showed that it allowed more than 300 microns of travel distance, with an average positioning error of less than 2 microns. 3D imaging experiments with the endomicroscope is underway, and its imaging performance will be assessed and discussed.

  4. Gradiometer Based on Nonlinear Magneto-Optic Rotation, Phase I

    Data.gov (United States)

    National Aeronautics and Space Administration — This Phase I SBIR project will demonstrate sensitive measurements of magnetic field gradients by nonlinear atomic spectroscopy. The gradients are determined by...

  5. Nonlinear optical and electroabsorption spectra of polydiacetylene crystals and films

    Science.gov (United States)

    Mukhopadhyay, D.; Soos, Z. G.

    1996-01-01

    Vibronic structure of nonlinear optical (NLO) coefficients is developed within the Condon approximation, displaced harmonic oscillators, and crude adiabatic states. The displacements of backbone modes of conjugated polymers are taken from vibrational data on the ground and 1B excited state. NLO resonances are modeled by three excitations and transition moments taken from Pariser-Parr-Pople (PPP) theory and optimized to polydiacetylene (PDA) spectra in crystals and films, with blue-shifted 1B exciton. The joint analysis of third-harmonic-generation, two-photon absorption, and nondegenerate four-wave-mixing spectra of PDA crystals and films shows weak two-photon absorption to 2A below 1B, leading to overlapping resonances in the THG spectrum, strong two-photon absorption to an nA state some 35% above 1B, and weak Raman resonances in nondegenerate FWM spectra. The full π-π* spectrum contributes to Stark shifts and field-induced transitions, as shown by PPP results for PDA oligomers. The Stark shift dominates high-resolution electroabsorption (EA) spectra of PDA crystals below 10 K. The close correspondence between EA and the first-derivative I'(ω) of the linear absorption above the 1B exciton in PDA crystals provides an experimental separation of vibrational and electronic contributions that limits any even-parity state in this 0.5 eV interval. An oscillator-strength sum rule is applied to the convergence of PDA oligomers with increasing length, N, and the crystal oscillator strengths are obtained without adjustable parameters. The sum rule for the 1B exciton implies large transition moments to higher-energy Ag states, whose locations in recent models are contrasted to PPP results. Joint analysis of NLO and EA spectra clarifies when a few electronic excitations are sufficient, distinguishes between vibrational and electronic contributions, and supports similar π-electron interactions in conjugated molecules and polymers.

  6. Nonlinear optics for the study of human scar tissue

    Science.gov (United States)

    Ferro, D. P.; Vieira-Damiani, G.; Adam, R. L.; Cesar, C. L.; Metze, Konradin

    2012-03-01

    Collagen fibers are an essential component of the dynamic process of scarring, which accompanies various diseases. Scar tissue may reveal different morphologic expressions, such as hypertrophic scars or keloids. Collagen fibers can be visualized by fluorescent light when stained with eosin. Second Harmonic Generation (SHG) creates a non linear signal that occurs only in molecules without inversion symmetry and is particularly strong in the collagen fibers arranged in triple helices. The aim of this study was to describe the methodology for the analysis of the density and texture of collagen in keloids, hypertrophic scars and conventional scars. Samples were examined in the National Institute of Science and Technology on Photonics Applied to Cell Biology (INFABIC) at the State University of Campinas. The images were acquired in a multiphoton microscopy LSM 780-NLO Zeiss 40X. Both signals, two-photon fluorescence (TPEF) and SHG, were excited by a Mai-Tai Ti:Sapphire laser at 940 nm. We used a LP490/SP485 NDD filter for SHG, and a BP565-610 NDD filter for fluorescence In each case, ten images were acquired serially (512×512 μm) in Z-stack and joined together to one patchwork-image . Image analysis was performed by a gliding-box-system with in-house made software. Keloids, hypertrophic scars and normal scar tissue show different collagen architecture. Inside an individual case differences of the scar process may be found between central and peripheral parts. In summary, the use of nonlinear optics is a helpful tool for the study of scars tissue.

  7. Relative permittivity in the electrical double layer from nonlinear optics

    Science.gov (United States)

    Boamah, Mavis D.; Ohno, Paul E.; Geiger, Franz M.; Eisenthal, Kenneth B.

    2018-06-01

    Second harmonic generation (SHG) spectroscopy has been applied to probe the fused silica/water interface at pH 7 and the uncharged 11 ¯ 02 sapphire/water interface at pH 5.2 in contact with aqueous solutions of NaCl, NaBr, NaI, KCl, RbCl, and CsCl as low as several 10 μM. For ionic strengths up to about 0.1 mM, the SHG responses were observed to increase, reversibly for all salts surveyed, when compared to the condition of zero salt added. Further increases in the salt concentration led to monotonic decreases in the SHG response. The SHG increases followed by decreases are found to be consistent with recent reports of phase interference and phase matching in nonlinear optics. By varying the relative permittivity employed in common mean field theories used to describe electrical double layers and by comparing our results to available literature data, we find that models recapitulating the experimental observations are the ones in which (1) the relative permittivity of the diffuse layer is that of bulk water, with other possible values as low as 30, (2) the surface charge density varies with salt concentration, and (3) the charge in the Stern layer or its thickness varies with salt concentration. We also note that the experimental data exhibit sensitivity depending on whether the salt concentration is increased from low to high values or decreased from high to low values, which, however, is not borne out in the fits, at least within the current uncertainties associated with the model point estimates.

  8. Nonlinear adaptive optics: aberration correction in three photon fluorescence microscopy for mouse brain imaging

    Science.gov (United States)

    Sinefeld, David; Paudel, Hari P.; Wang, Tianyu; Wang, Mengran; Ouzounov, Dimitre G.; Bifano, Thomas G.; Xu, Chris

    2017-02-01

    Multiphoton fluorescence microscopy is a well-established technique for deep-tissue imaging with subcellular resolution. Three-photon microscopy (3PM) when combined with long wavelength excitation was shown to allow deeper imaging than two-photon microscopy (2PM) in biological tissues, such as mouse brain, because out-of-focus background light can be further reduced due to the higher order nonlinear excitation. As was demonstrated in 2PM systems, imaging depth and resolution can be improved by aberration correction using adaptive optics (AO) techniques which are based on shaping the scanning beam using a spatial light modulator (SLM). In this way, it is possible to compensate for tissue low order aberration and to some extent, to compensate for tissue scattering. Here, we present a 3PM AO microscopy system for brain imaging. Soliton self-frequency shift is used to create a femtosecond source at 1675 nm and a microelectromechanical (MEMS) SLM serves as the wavefront shaping device. We perturb the 1020 segment SLM using a modified nonlinear version of three-point phase shifting interferometry. The nonlinearity of the fluorescence signal used for feedback ensures that the signal is increasing when the spot size decreases, allowing compensation of phase errors in an iterative optimization process without direct phase measurement. We compare the performance for different orders of nonlinear feedback, showing an exponential growth in signal improvement as the nonlinear order increases. We demonstrate the impact of the method by applying the 3PM AO system for in-vivo mouse brain imaging, showing improvement in signal at 1-mm depth inside the brain.

  9. Third-order nonlinear optical response of Ag-CdSe/PVA hybrid nanocomposite

    Energy Technology Data Exchange (ETDEWEB)

    Tripathi, S.K.; Kaur, Ramneek; Kaur, Jaspreet; Sharma, Mamta [Panjab University, Department of Physics, Center of Advanced Study in Physics, Chandigarh (India)

    2015-09-15

    Hybrid nanocomposites of II-VI semiconductor nanoparticles are gaining great interest in nonlinear optoelectronic devices. Present work includes the characterization of CdSe polymer nanocomposite prepared by chemical in situ technique. From X-ray diffraction, the hexagonal wurtzite structure of nanoparticles has been confirmed with spherical morphology from transmission electron microscopy. Ag-CdSe hybrid polymer nanocomposite has been prepared chemically at different Ag concentrations. The presence of Ag in hybrid nanocomposite has been confirmed with energy-dispersive X-ray spectroscopy. The effect of varying Ag concentration on the linear and nonlinear optical properties of the nanocomposites has been studied. In linear optical parameters, the linear absorption coefficient, refractive index, extinction coefficient and optical conductivity have been calculated. The third-order nonlinear optical properties have been observed with open- and closed-aperture Z-scan technique. The large nonlinear refractive index ∝10{sup -5} cm{sup 2}/W with self-focusing behaviour is due to the combined effect of quantum confinement and thermo-optical effects. The enhanced nonlinearity with increasing Ag content is due to the surface plasmon resonance, which enhances the local electric field near the nanoparticle surface. Thus, Ag-CdSe hybrid polymer nanocomposite has favourable nonlinear optical properties for various optoelectronic applications. (orig.)

  10. Third-order nonlinear optical response of Ag-CdSe/PVA hybrid nanocomposite

    International Nuclear Information System (INIS)

    Tripathi, S.K.; Kaur, Ramneek; Kaur, Jaspreet; Sharma, Mamta

    2015-01-01

    Hybrid nanocomposites of II-VI semiconductor nanoparticles are gaining great interest in nonlinear optoelectronic devices. Present work includes the characterization of CdSe polymer nanocomposite prepared by chemical in situ technique. From X-ray diffraction, the hexagonal wurtzite structure of nanoparticles has been confirmed with spherical morphology from transmission electron microscopy. Ag-CdSe hybrid polymer nanocomposite has been prepared chemically at different Ag concentrations. The presence of Ag in hybrid nanocomposite has been confirmed with energy-dispersive X-ray spectroscopy. The effect of varying Ag concentration on the linear and nonlinear optical properties of the nanocomposites has been studied. In linear optical parameters, the linear absorption coefficient, refractive index, extinction coefficient and optical conductivity have been calculated. The third-order nonlinear optical properties have been observed with open- and closed-aperture Z-scan technique. The large nonlinear refractive index ∝10 -5 cm 2 /W with self-focusing behaviour is due to the combined effect of quantum confinement and thermo-optical effects. The enhanced nonlinearity with increasing Ag content is due to the surface plasmon resonance, which enhances the local electric field near the nanoparticle surface. Thus, Ag-CdSe hybrid polymer nanocomposite has favourable nonlinear optical properties for various optoelectronic applications. (orig.)

  11. Surface plasmon enhanced third-order optical nonlinearity of Ag nanocomposite film

    Energy Technology Data Exchange (ETDEWEB)

    Singh, Vijender [Department of Applied Science, N.C. College of Engineering, Israna, Panipat 132107, Haryana (India); Aghamkar, Praveen, E-mail: p-aghamkar@yahoo.in [Department of Physics, Chaudhary Devi Lal University, Sirsa 125055, Haryana (India)

    2014-03-17

    We obtain a large third-order optical nonlinearity (χ{sup (3)} ≈ 10{sup −10}esu) of silver nanoparticles dispersed in polyvinyl alcohol/tetraethyl orthosilicate matrix using single beam z-scan technique at 532 nm by Q-switched Nd:YAG laser. We have shown that mechanisms responsible for third-order optical nonlinearity of Ag nanocomposite film are reverse saturable absorption (RSA) and self-defocusing in the purlieu of surface plasmon resonance (SPR). Optical band-gap and width of SPR band of Ag nanocomposite film decrease with increasing silver concentration, which leads to enhancement of local electric field and hence third-order optical nonlinearity. Optical limiting, due to RSA has also been demonstrated at 532 nm.

  12. Surface plasmon enhanced third-order optical nonlinearity of Ag nanocomposite film

    International Nuclear Information System (INIS)

    Singh, Vijender; Aghamkar, Praveen

    2014-01-01

    We obtain a large third-order optical nonlinearity (χ (3)  ≈ 10 −10 esu) of silver nanoparticles dispersed in polyvinyl alcohol/tetraethyl orthosilicate matrix using single beam z-scan technique at 532 nm by Q-switched Nd:YAG laser. We have shown that mechanisms responsible for third-order optical nonlinearity of Ag nanocomposite film are reverse saturable absorption (RSA) and self-defocusing in the purlieu of surface plasmon resonance (SPR). Optical band-gap and width of SPR band of Ag nanocomposite film decrease with increasing silver concentration, which leads to enhancement of local electric field and hence third-order optical nonlinearity. Optical limiting, due to RSA has also been demonstrated at 532 nm

  13. Single-step emulation of nonlinear fiber-optic link with gaussian mixture model

    DEFF Research Database (Denmark)

    Borkowski, Robert; Doberstein, Andy; Haisch, Hansjörg

    2015-01-01

    We use a fast and low-complexity statistical signal processing method to emulate nonlinear noise in fiber links. The proposed emulation technique stands in good agreement with the numerical NLSE simulation for 32 Gbaud DP-16QAM nonlinear transmission.......We use a fast and low-complexity statistical signal processing method to emulate nonlinear noise in fiber links. The proposed emulation technique stands in good agreement with the numerical NLSE simulation for 32 Gbaud DP-16QAM nonlinear transmission....

  14. Photoconductivity, photoluminescence and optical Kerr nonlinear effects in zinc oxide films containing chromium nanoclusters

    International Nuclear Information System (INIS)

    Torres-Torres, C.; García-Cruz, M.L.; Castañeda, L.; Rangel Rojo, R.; Tamayo-Rivera, L.; Maldonado, A.; Avendaño-Alejo, M.

    2012-01-01

    Chromium doped zinc oxide thin solid films were deposited on soda–lime glass substrates. The photoconductivity of the material and its influence on the optical behavior was evaluated. A non-alkoxide sol–gel synthesis approach was used for the preparation of the samples. An enhancement of the photoluminescence response exhibited by the resulting photoconductive films with embedded chromium nanoclusters is presented. The modification in the photoconduction induced by a 445 nm wavelength was measured and then associated with the participation of the optical absorptive response. In order to investigate the third order optical nonlinearities of the samples, a standard time-resolved Optical Kerr Gate configuration with 80 fs pulses at 830 nm was used and a quasi-instantaneous pure electronic nonlinearity without the contribution of nonlinear optical absorption was observed. We estimate that from the inclusion of Cr nanoclusters into the sample results a strong optical Kerr effect originated by quantum confinement. The large photoluminescence response and the important refractive nonlinearity of the photoconductive samples seem to promise potential applications for the development of multifunctional all-optical nanodevices. - Highlights: ► Enhancement in photoluminescence for chromium doped zinc oxide films is presented. ► A strong and ultrafast optical Kerr effect seems to result from quantum confinement. ► Photoconductive properties for optical and optoelectronic functions were observed.

  15. Photoconductivity, photoluminescence and optical Kerr nonlinear effects in zinc oxide films containing chromium nanoclusters

    Energy Technology Data Exchange (ETDEWEB)

    Torres-Torres, C., E-mail: crstorres@yahoo.com.mx [Seccion de Estudios de Posgrado e Investigacion, ESIME-Z, Instituto Politecnico Nacional, Mexico, DF 07738 (Mexico); Garcia-Cruz, M.L. [Centro de Investigacion en Dispositivos Semiconductores, Benemerita Universidad Autonoma de Puebla, A. P. J-48, Puebla 72570, Mexico (Mexico); Castaneda, L., E-mail: luisca@sirio.ifuap.buap.mx [Instituto de Fisica, Benemerita Universidad Autonoma de Puebla, A. P. J-48, Puebla 72570, Mexico (Mexico); Rangel Rojo, R. [CICESE/Depto. de Optica, A. P. 360, Ensenada, BC 22860 (Mexico); Tamayo-Rivera, L. [Instituto de Fisica, Universidad Nacional Autonoma de Mexico, Mexico, DF 01000 (Mexico); Maldonado, A. [Depto. de Ing. Electrica, CINVESTAV IPN-SEES, A. P. 14740, Mexico DF 07000 (Mexico); Avendano-Alejo, M., E-mail: imax_aa@yahoo.com.mx [Centro de Ciencias Aplicadas y Desarrollo Tecnologico, Universidad Nacional Autonoma de Mexico, A. P. 70-186, 04510, DF (Mexico); and others

    2012-04-15

    Chromium doped zinc oxide thin solid films were deposited on soda-lime glass substrates. The photoconductivity of the material and its influence on the optical behavior was evaluated. A non-alkoxide sol-gel synthesis approach was used for the preparation of the samples. An enhancement of the photoluminescence response exhibited by the resulting photoconductive films with embedded chromium nanoclusters is presented. The modification in the photoconduction induced by a 445 nm wavelength was measured and then associated with the participation of the optical absorptive response. In order to investigate the third order optical nonlinearities of the samples, a standard time-resolved Optical Kerr Gate configuration with 80 fs pulses at 830 nm was used and a quasi-instantaneous pure electronic nonlinearity without the contribution of nonlinear optical absorption was observed. We estimate that from the inclusion of Cr nanoclusters into the sample results a strong optical Kerr effect originated by quantum confinement. The large photoluminescence response and the important refractive nonlinearity of the photoconductive samples seem to promise potential applications for the development of multifunctional all-optical nanodevices. - Highlights: Black-Right-Pointing-Pointer Enhancement in photoluminescence for chromium doped zinc oxide films is presented. Black-Right-Pointing-Pointer A strong and ultrafast optical Kerr effect seems to result from quantum confinement. Black-Right-Pointing-Pointer Photoconductive properties for optical and optoelectronic functions were observed.

  16. Nonlinear Pulse Shaping in Fibres for Pulse Generation and Optical Processing

    Directory of Open Access Journals (Sweden)

    Sonia Boscolo

    2012-01-01

    Full Text Available The development of new all-optical technologies for data processing and signal manipulation is a field of growing importance with a strong potential for numerous applications in diverse areas of modern science. Nonlinear phenomena occurring in optical fibres have many attractive features and great, but not yet fully explored, potential in signal processing. Here, we review recent progress on the use of fibre nonlinearities for the generation and shaping of optical pulses and on the applications of advanced pulse shapes in all-optical signal processing. Amongst other topics, we will discuss ultrahigh repetition rate pulse sources, the generation of parabolic shaped pulses in active and passive fibres, the generation of pulses with triangular temporal profiles, and coherent supercontinuum sources. The signal processing applications will span optical regeneration, linear distortion compensation, optical decision at the receiver in optical communication systems, spectral and temporal signal doubling, and frequency conversion.

  17. Solitary wave for a nonintegrable discrete nonlinear Schrödinger equation in nonlinear optical waveguide arrays

    Science.gov (United States)

    Ma, Li-Yuan; Ji, Jia-Liang; Xu, Zong-Wei; Zhu, Zuo-Nong

    2018-03-01

    We study a nonintegrable discrete nonlinear Schrödinger (dNLS) equation with the term of nonlinear nearest-neighbor interaction occurred in nonlinear optical waveguide arrays. By using discrete Fourier transformation, we obtain numerical approximations of stationary and travelling solitary wave solutions of the nonintegrable dNLS equation. The analysis of stability of stationary solitary waves is performed. It is shown that the nonlinear nearest-neighbor interaction term has great influence on the form of solitary wave. The shape of solitary wave is important in the electric field propagating. If we neglect the nonlinear nearest-neighbor interaction term, much important information in the electric field propagating may be missed. Our numerical simulation also demonstrates the difference of chaos phenomenon between the nonintegrable dNLS equation with nonlinear nearest-neighbor interaction and another nonintegrable dNLS equation without the term. Project supported by the National Natural Science Foundation of China (Grant Nos. 11671255 and 11701510), the Ministry of Economy and Competitiveness of Spain (Grant No. MTM2016-80276-P (AEI/FEDER, EU)), and the China Postdoctoral Science Foundation (Grant No. 2017M621964).

  18. The effect of quintic nonlinearity on the propagation characteristics of dispersion managed optical solitons

    International Nuclear Information System (INIS)

    Konar, S.; Mishra, Manoj; Jana, S.

    2006-01-01

    The role of quintic nonlinearity on the propagation characteristics of optical solitons in dispersion managed optical communication systems has been presented in this paper. It has been shown that quintic nonlinearity has only marginal influence on single pulse propagation. However, numerical simulation has been undertaken to reveal that quintic nonlinearity reduces collision distance between neighbouring pulses of the same channel. It is found that for lower map strength the collapse distance between intra channel pulses is very much sensitive to the dispersion map strength

  19. Experimental investigations of optical nonlinearities in semiconductor-doped glass waveguides

    International Nuclear Information System (INIS)

    Dannberg, P.; Possner, T.; Braeuer, A.; Bartuch, U.

    1988-01-01

    Both, thermal and electronic optical nonlinearities are studied in semiconductor-doped glass (SDG) waveguides which are fabricated in commercially available sharp-cut filters by Cs + -K + ion exchange. The relaxation time in photodarkened substrates is measured to be 30 ps. By means of a prism coupling set-up the saturation value of the nonlinear index change is determined. Furthermore, a high stability dual-beam interferometer is presented for the measurement of both, thermal and electronic nonlinear refractive index n 2 in planar waveguides. Conclusions about the application of SDG to opto-optical switching are given. (author)

  20. Investigation of the spatial distribution of second-order nonlinearity in thermally poled optical fibers.

    Science.gov (United States)

    An, Honglin; Fleming, Simon

    2005-05-02

    The spatial distribution of second-order nonlinearity in thermally poled optical fibers was characterized by second-harmonic microscopy. The second-order nonlinearity was found to be confined to a thin layer close to the anode surface and progressed further into the silica as the poling time increased. Position uncertainty of the anode metal wire was observed to have an effect, as the nonlinear layers were found not always symmetrically located around the nearest points between the anode and cathode. Optical microscopy results were obtained on etched poled fiber cross-sections and compared with those from second-harmonic microscopy.

  1. A generalized auxiliary equation method and its application to nonlinear Klein-Gordon and generalized nonlinear Camassa-Holm equations

    International Nuclear Information System (INIS)

    Yomba, Emmanuel

    2008-01-01

    With the aid of symbolic computation, a generalized auxiliary equation method is proposed to construct more general exact solutions to two types of NLPDEs. First, we present new family of solutions to a nonlinear Klein-Gordon equation, by using this auxiliary equation method including a new first-order nonlinear ODE with six-degree nonlinear term proposed by Sirendaoreji. Then, we apply an indirect F-function method very close to the F-expansion method to solve the generalized Camassa-Holm equation with fully nonlinear dispersion and fully nonlinear convection C(l,n,p). Taking advantage of the new first-order nonlinear ODE with six degree nonlinear term, this indirect F-function method is used to map the solutions of C(l,n,p) equations to those of that nonlinear ODE. As a result, we can successfully obtain in a unified way, many exact solutions

  2. The spectral cell method in nonlinear earthquake modeling

    Science.gov (United States)

    Giraldo, Daniel; Restrepo, Doriam

    2017-12-01

    This study examines the applicability of the spectral cell method (SCM) to compute the nonlinear earthquake response of complex basins. SCM combines fictitious-domain concepts with the spectral-version of the finite element method to solve the wave equations in heterogeneous geophysical domains. Nonlinear behavior is considered by implementing the Mohr-Coulomb and Drucker-Prager yielding criteria. We illustrate the performance of SCM with numerical examples of nonlinear basins exhibiting physically and computationally challenging conditions. The numerical experiments are benchmarked with results from overkill solutions, and using MIDAS GTS NX, a finite element software for geotechnical applications. Our findings show good agreement between the two sets of results. Traditional spectral elements implementations allow points per wavelength as low as PPW = 4.5 for high-order polynomials. Our findings show that in the presence of nonlinearity, high-order polynomials (p ≥ 3) require mesh resolutions above of PPW ≥ 10 to ensure displacement errors below 10%.

  3. NLO 󈨞. Nonlinear Optics: Materials, Phenomena and Devices Digest. Internation Meeting on Nonlinear Optics (1st) Held in Kauai, Hawaii on 16-20 July 1990

    Science.gov (United States)

    1991-03-13

    combination50 with a dynamic grating diffraction modelO . Considering o 0 a polarlsatlon grating on a homoetropic aligned nematlc ’-i 40 filmi the optical...nonlinearities of solutions of chloroaluminumphthalocyanine (CAP) in methanol and a silicon naphthalocyanine (Nc) derivative, SiNc( OSi (hexyl)3)2 or

  4. Optical nonlinearities of excitonic states in atomically thin 2D transition metal dichalcogenides

    Energy Technology Data Exchange (ETDEWEB)

    Soh, Daniel Beom Soo [Sandia National Lab. (SNL-CA), Livermore, CA (United States). Proliferation Signatures Discovery and Exploitation Department

    2017-08-01

    We calculated the optical nonlinearities of the atomically thin monolayer transition metal dichalcogenide material (particularly MoS2), particularly for those linear and nonlinear transition processes that utilize the bound exciton states. We adopted the bound and the unbound exciton states as the basis for the Hilbert space, and derived all the dynamical density matrices that provides the induced current density, from which the nonlinear susceptibilities can be drawn order-by-order via perturbative calculations. We provide the nonlinear susceptibilities for the linear, the second-harmonic, the third-harmonic, and the kerr-type two-photon processes.

  5. Fiber optic sensor and method for making

    Science.gov (United States)

    Vartuli, James Scott; Bousman, Kenneth Sherwood; Deng, Kung-Li; McEvoy, Kevin Paul; Xia, Hua

    2010-05-18

    A fiber optic sensor including a fiber having a modified surface integral with the fiber wherein the modified surface includes an open pore network with optical agents dispersed within the open pores of the open pore network. Methods for preparing the fiber optic sensor are also provided. The fiber optic sensors can withstand high temperatures and harsh environments.

  6. NOLB: Nonlinear Rigid Block Normal Mode Analysis Method

    OpenAIRE

    Hoffmann , Alexandre; Grudinin , Sergei

    2017-01-01

    International audience; We present a new conceptually simple and computationally efficient method for nonlinear normal mode analysis called NOLB. It relies on the rotations-translations of blocks (RTB) theoretical basis developed by Y.-H. Sanejouand and colleagues. We demonstrate how to physically interpret the eigenvalues computed in the RTB basis in terms of angular and linear velocities applied to the rigid blocks and how to construct a nonlinear extrapolation of motion out of these veloci...

  7. Performance of a nonlinear receiver for the ultrashort-pulse optical CDMA system

    Science.gov (United States)

    Ni, Bin; Lehnert, James S.

    2005-09-01

    At the receiver of an ultrashort-pulse optical code-division multiple-access (OCDMA) system, a nonlinear thresholder is needed to discriminate between the correctly decoded short pulse and the interference that appears to be a pseudorandom signal. It has been demonstrated that the self phase modulation (SPM) effect can be used to realize this nonlinear thresholder. The performance of a system that exploits this phenomenon is analyzed in this paper. If the spreading code is random, the electrical field of the interfering signal from the multiple users can be shown to be a complex Gaussian random process. The broadened power spectral density (PSD) function caused by the SPM effect can be calculated. When "1" is transmitted, the correctly decoded signal from the desired user, which is a deterministic waveform, is added to the Gaussian random process. Beating between the two signals causes random fluctuations in the power. Since the strength of the SPM effect is proportional to the variation rate of power, the broadened signal spectrum will appear random. The Monte Carlo method is used to obtain the properties of the decision statistic. Finally, the bit-error rate (BER) is calculated, and the simulation results are presented. The result reveals that the performance of the SPM-based nonlinear receiver can outperform the ideal linear receiver in some circumstances.

  8. Nonlinear optical spectra having characteristics of Fano interferences in coherently coupled lowest exciton biexciton states in semiconductor quantum dots

    Directory of Open Access Journals (Sweden)

    Hideki Gotoh

    2014-10-01

    Full Text Available Optical nonlinear effects are examined using a two-color micro-photoluminescence (micro-PL method in a coherently coupled exciton-biexciton system in a single quantum dot (QD. PL and photoluminescence excitation spectroscopy (PLE are employed to measure the absorption spectra of the exciton and biexciton states. PLE for Stokes and anti-Stokes PL enables us to clarify the nonlinear optical absorption properties in the lowest exciton and biexciton states. The nonlinear absorption spectra for excitons exhibit asymmetric shapes with peak and dip structures, and provide a distinct contrast to the symmetric dip structures of conventional nonlinear spectra. Theoretical analyses with a density matrix method indicate that the nonlinear spectra are caused not by a simple coherent interaction between the exciton and biexciton states but by coupling effects among exciton, biexciton and continuum states. These results indicate that Fano quantum interference effects appear in exciton-biexciton systems at QDs and offer important insights into their physics.

  9. Nonlinear laser dynamics induced by frequency shifted optical feedback: application to vibration measurements.

    Science.gov (United States)

    Girardeau, Vadim; Goloni, Carolina; Jacquin, Olivier; Hugon, Olivier; Inglebert, Mehdi; Lacot, Eric

    2016-12-01

    In this article, we study the nonlinear dynamics of a laser subjected to frequency shifted optical reinjection coming back from a vibrating target. More specifically, we study the nonlinear dynamical coupling between the carrier and the vibration signal. The present work shows how the nonlinear amplification of the vibration spectrum is related to the strength of the carrier and how it must be compensated to obtain accurate (i.e., without bias) vibration measurements. The theoretical predictions, confirmed by numerical simulations, are in good agreement with the experimental data. The main motivation of this study is the understanding of the nonlinear response of a laser optical feedback imaging sensor for quantitative phase measurements of small vibrations in the case of strong optical feedback.

  10. Theoretical investigation of intensity-dependent optical nonlinearity in graphene-aided D-microfiber

    Science.gov (United States)

    Shah, Manoj Kumar; Lu, Rongguo; Zhang, Yali; Ye, Shengwei; Zhang, Shangjian; Liu, Yong

    2018-01-01

    We theoretically investigate the intensity-dependent optical nonlinearity in graphene-aided D-microfiber, by tuning the chemical potential of graphene and varying radial distance and radii of the D-microfiber. Utilizing an interplay between graphene and the enhanced evanescent field of a guided mode in the waveguide of interest, the net utility of nonlinear coefficient is harnessed up to a very high value of 106 W-1m-1. Importantly, which is ∼ two orders of magnitude larger than in PMMA-graphene-PMMA waveguide. The highly dispersive nature of the waveguide, D ∼ 103 ps/nm-km, and large nonlinear figure-of-merit, FOMNL ∼ 1.29, have raised the possibilities of utilizing slow light structures to operate devices at few watts power level with microscale length. These studies have opened one window towards the next-generation all fiber-optic graphene nonlinear optical devices.

  11. A Modified Lindstedt–Poincaré Method for a Strongly Nonlinear System with Quadratic and Cubic Nonlinearities

    Directory of Open Access Journals (Sweden)

    S.H. Chen

    1996-01-01

    Full Text Available A modified Lindstedt–Poincaré method is presented for extending the range of the validity of perturbation expansion to strongly nonlinear oscillations of a system with quadratic and cubic nonlinearities. Different parameter transformations are introduced to deal with equations with different nonlinear characteristics. All examples show that the efficiency and accuracy of the present method are very good.

  12. A Modified Conjugacy Condition and Related Nonlinear Conjugate Gradient Method

    Directory of Open Access Journals (Sweden)

    Shengwei Yao

    2014-01-01

    Full Text Available The conjugate gradient (CG method has played a special role in solving large-scale nonlinear optimization problems due to the simplicity of their very low memory requirements. In this paper, we propose a new conjugacy condition which is similar to Dai-Liao (2001. Based on this condition, the related nonlinear conjugate gradient method is given. With some mild conditions, the given method is globally convergent under the strong Wolfe-Powell line search for general functions. The numerical experiments show that the proposed method is very robust and efficient.

  13. Perturbation method for periodic solutions of nonlinear jerk equations

    International Nuclear Information System (INIS)

    Hu, H.

    2008-01-01

    A Lindstedt-Poincare type perturbation method with bookkeeping parameters is presented for determining accurate analytical approximate periodic solutions of some third-order (jerk) differential equations with cubic nonlinearities. In the process of the solution, higher-order approximate angular frequencies are obtained by Newton's method. A typical example is given to illustrate the effectiveness and simplicity of the proposed method

  14. Nonlinear optical switching behavior in the solid state: A theoretical investigation on anils

    KAUST Repository

    Ségerie, Audrey

    2011-09-13

    The linear (π(1)) and second-order nonlinear (π(2)) optical properties of two anil crystals, [N-(4-hydroxy)-salicylidene-amino-4-(methylbenzoate) and N-(3,5-di-tert- butylsalicylidene)-4-aminopyridine, denoted 4A and 4P, respectively], as well as the optical contrasts upon switching between their enol (E) and keto (K) forms, have been investigated by combining the molecular responses calculated using quantum chemistry methods and an electrostatic interaction scheme to account for the local field effects. It is found that intermolecular interactions impact differently the K/E optical contrasts in the two systems, which illustrates the importance of the supramolecular organization on the macroscopic responses. In 4A, the surrounding effects on the (hyper)polarizabilities are similar in the enol and keto forms, leading to optical contrasts very close to those of the isolated molecule. In contrast, an enhancement of the second-order susceptibility is observed in the keto form of 4P, leading to a large π(2)(K)/π(2)(E) contrast. Moreover, the π(2)(4A)/π(2)(4P) ratio for the most stable enol forms is obtained to be in good agreement with previous experimental investigations, which supports the reliability of the computational procedure. © 2011 American Chemical Society.

  15. Nonlinear optical switching behavior in the solid state: A theoretical investigation on anils

    KAUST Repository

    Sé gerie, Audrey; Castet, Fré dé ric; Kanoun, Mohammed; Plaquet, Auré lie; Lié geois, Vincent; Champagne, Benoit

    2011-01-01

    The linear (π(1)) and second-order nonlinear (π(2)) optical properties of two anil crystals, [N-(4-hydroxy)-salicylidene-amino-4-(methylbenzoate) and N-(3,5-di-tert- butylsalicylidene)-4-aminopyridine, denoted 4A and 4P, respectively], as well as the optical contrasts upon switching between their enol (E) and keto (K) forms, have been investigated by combining the molecular responses calculated using quantum chemistry methods and an electrostatic interaction scheme to account for the local field effects. It is found that intermolecular interactions impact differently the K/E optical contrasts in the two systems, which illustrates the importance of the supramolecular organization on the macroscopic responses. In 4A, the surrounding effects on the (hyper)polarizabilities are similar in the enol and keto forms, leading to optical contrasts very close to those of the isolated molecule. In contrast, an enhancement of the second-order susceptibility is observed in the keto form of 4P, leading to a large π(2)(K)/π(2)(E) contrast. Moreover, the π(2)(4A)/π(2)(4P) ratio for the most stable enol forms is obtained to be in good agreement with previous experimental investigations, which supports the reliability of the computational procedure. © 2011 American Chemical Society.

  16. Structural, electronic, linear, and nonlinear optical properties of ZnCdTe{sub 2} chalcopyrite

    Energy Technology Data Exchange (ETDEWEB)

    Ouahrani, Tarik [Laboratoire de Physique Theorique, Universite de Tlemcen, B.P. 230, Tlemcen 13000 (Algeria); Reshak, Ali H. [Institute of Physical Biology, South Bohemia University, Nove Hrady 37333 (Czech Republic); School of Microelectronic Engineering, University of Malaysia Perlis (UniMAP), Block A, Kompleks Pusat Pengajian, 02600 Arau Jejawi, Perlis (Malaysia); Khenata, R. [Laboratoire de Physique Quantique et de Modelisation Mathematique, Universite de Mascara, Mascara 29000 (Algeria); Department of Physics and Astronomy, Faculty of Science, King Saud University, P.O. Box 2455, Riyadh 11451 (Saudi Arabia); Baltache, H.; Amrani, B. [Laboratoire de Physique Quantique et de Modelisation Mathematique, Universite de Mascara, Mascara 29000 (Algeria); Bouhemadou, A. [Department of Physics and Astronomy, Faculty of Science, King Saud University, P.O. Box 2455, Riyadh 11451 (Saudi Arabia); Faculty of Sciences, Department of Physics, University of Setif, Setif 19000 (Algeria)

    2011-03-15

    We report results of first-principles density functional calculations using the full-potential linearized augmented plane wave method. The generalized gradient approximation (GGA) and the Engel-Vosko-GGA (EV-GGA) formalism were used for the exchange-correlation energy to calculate the structural, electronic, linear, and nonlinear optical properties of the chalcopyrite ZnCdTe{sub 2} compound. The valence band maximum and the conduction band minimum are located at the {gamma}-point, resulting in a direct band gap of about 0.71 eV for GGA and 1.29 eV for EV-GGA. The results of bulk properties, such as lattice parameters (a, c, and u), bulk modulus B, and its pressure derivative B' are evaluated. The optical properties of this compound, namely the real and the imaginary parts of the dielectric function, reflectivity, and refractive index, show a considerable anisotropy as a consequence ZnCdTe{sub 2} posseses a strong birefringence. In addition, the extinction coefficient, the electron energy loss function, and the nonlinear susceptibility are calculated and their spectra are analyzed. (Copyright copyright 2011 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  17. Growth and characterization of new nonlinear optical 1-phenyl-3-(4-dimethylamino phenyl) prop-2-en-1-one (PDAC) single crystals

    Science.gov (United States)

    Ravindraswami, K.; Janardhana, K.; Gowda, Jayaprakash; Moolya, B. Narayana

    2018-04-01

    Non linear optical 1-phenyl-3-(4-dimethylamino phenyl) prop-2-en-1-one (PDAC) was synthesized using Claisen - Schmidt condensation method and studied for optical nonlinearity with an emphasis on structure-property relationship. The structural confirmation studies were carried out using 1H-NMR, FT-IR and single crystal XRD techniques. The nonlinear absorption and nonlinear refraction parameters in z-scan with nano second laser pulses were obtained by measuring the profile of propagated beam through the samples. The real and imaginary parts of third-order bulk susceptibility χ(3) were evaluated. Thermo gravimetric analysis is carried out to investigate the thermal stability.

  18. Nonlinear optics at the single-photon level inside a hollow core fiber

    DEFF Research Database (Denmark)

    Hofferberth, Sebastian; Peyronel, Thibault; Liang, Qiyu

    2011-01-01

    Cold atoms inside a hollow core fiber provide an unique system for studying optical nonlinearities at the few-photon level. Confinement of both atoms and photons inside the fiber core to a diameter of just a few wavelengths results in high electric field intensity per photon and large optical...

  19. Aggregation induced enhancement of linear and nonlinear optical emission from a hexaphenylene derivative

    NARCIS (Netherlands)

    Duan, Y.; Ju, C.G.; Yang, G.; Fron, E.; Coutino-Gonzalez, E.; Semin, S.V.; Fan, C.C.; Balok, R.S.; Cremers, J.; Tinnemans, P.T.; Feng, Y.Q.; Li, Y.L.; Hofkens, J.; Rowan, A.E.; Rasing, T.H.M.; Xu, J.L.

    2016-01-01

    The discovery of the phenomenon known as aggregation-induced emission (AIE) has opened the door to a variety of brilliant organic solid-state light-emitting materials. While AIE is well established in linear optics, the development of AIE luminogens (AIEgens) with highly efficient nonlinear optical

  20. Growth and characterizaion of urea p-nitrophenol crystal: an organic nonlinear optical material for optoelectronic device application

    Science.gov (United States)

    Suresh, A.; Manikandan, N.; Jauhar, RO. MU.; Murugakoothan, P.; Vinitha, G.

    2018-06-01

    Urea p-nitrophenol, an organic nonlinear optical crystal was synthesized and grown adopting slow evaporation and seed rotation method. Single crystal X-ray diffraction study confirmed the formation of the desired crystal. High resolution X-ray diffraction study showed the defect nature of the crystal. The presence of functional groups in the material was confirmed by FTIR analysis. UV-Vis-NIR study indicates that the grown crystal has a wider transparency region with the lower cutoff wavelength at 423 nm. The grown crystal is thermally stable up to 120 °C as assessed by TG-DTA analysis. The optical homogeneity of the grown crystal was confirmed by birefringence study. The 1064 nm Nd-YAG laser was used to obtain laser induced surface damage threshold which was found to be 0.38, 0.25 and 0.33 GW/cm2 for (0 1 0), (1 1 - 1) and (0 1 1) planes, respectively. The dielectric study was performed to find the charge distribution inside the crystal. The hardness property of the titular material has been found using Vicker's microhardness study. The optical nonlinearity obtained from third order nonlinear optical measurements carried out using Z-scan technique showed that these samples could be exploited for optical limiting studies.

  1. Synthesis, crystal growth, optical, thermal, and mechanical properties of a nonlinear optical single crystal: ammonium sulfate hydrogen sulphamate (ASHS)

    Science.gov (United States)

    Sudhakar, K.; Nandhini, S.; Muniyappan, S.; Arumanayagam, T.; Vivek, P.; Murugakoothan, P.

    2018-04-01

    Ammonium sulfate hydrogen sulphamate (ASHS), an inorganic nonlinear optical crystal, was grown from the aqueous solution by slow evaporation solution growth technique. The single-crystal XRD confirms that the grown single crystal belongs to the orthorhombic system with the space group of Pna21. Powder XRD confirms the crystalline nature and the diffraction planes were indexed. Crystalline perfection of grown crystal was analysed by high-resolution X-ray diffraction rocking curve technique. UV-Vis-NIR studies revealed that ASHS crystal has optical transparency 65% and lower cut-off wavelength at 218 nm. The violet light emission of the crystal was identified by photoluminescence studies. The particle size-dependent second-harmonic generation efficiency for ASHS crystal was evaluated by Kurtz-Perry powder technique using Nd:YAG laser which established the existence of phase matching. Surface laser damage threshold value was evaluated using Nd:YAG laser. Optical homogeneity of the crystal was evaluated using modified channel spectrum method through birefringence study. Thermal analysis reveals that ASHS crystal is stable up to 213 °C. The mechanical behaviour of the ASHS crystal was analysed using Vickers microhardness study.

  2. Synthesis, crystal structure, growth, optical and third order nonlinear optical studies of 8HQ2C5N single crystal - An efficient third-order nonlinear optical material

    Energy Technology Data Exchange (ETDEWEB)

    Divya Bharathi, M.; Ahila, G.; Mohana, J. [Department of Physics, Presidency College, Chennai 600005 (India); Chakkaravarthi, G. [Department of Physics, CPCL Polytechnic College, Chennai 600068 (India); Anbalagan, G., E-mail: anbu24663@yahoo.co.in [Department of Nuclear Physics, University of Madras, Chennai 600025 (India)

    2017-05-01

    A neoteric organic third order nonlinear optical material 8-hydroxyquinolinium 2-chloro-5-nitrobenzoate dihydrate (8HQ2C5N) was grown by slow cooling technique using ethanol: water (1:1) mixed solvent. The calculated low value of average etch pit solidity (4.12 × 10{sup 3} cm{sup −2}) indicated that the title crystal contain less defects. From the single crystal X-ray diffraction data, it was endowed that 8HQ2C5N crystal belongs to the monoclinic system with centrosymmetric space group P2{sub 1}/c and the cell parameters values, a = 9.6546 (4) Ǻ, b = 7.1637(3) Ǻ, c = 24.3606 (12) Ǻ, α = γ = 90°, β = 92.458(2)° and volume = 1683.29(13) Ǻ{sup 3}. The FT-IR and FT-Raman spectrum were used to affirm the functional group of the title compound. The chemical structure of 8HQ2C5N was scrutinized by {sup 13}C and {sup 1}H NMR spectral analysis and thermal stability through the differential scanning calorimetry study. Using optical studies the lower cut-off wavelength and optical band gap of 8HQ2C5N were found to be 364 nm and 3.17 eV respectively. Using the single oscillator model suggested by Wemple – Didomenico, the oscillator energy (E{sub o}), the dispersion energy (E{sub d}) and static dielectric constant (ε{sub o}) were estimated. The third-order susceptibility were determined as Im χ{sup (3)} = 2.51 × 10{sup −5} esu and Re χ{sup (3)} = 4.46 × 10{sup −7} esu. The theoretical third-order nonlinear optical susceptibility χ{sup (3)} was calculated and the results were compared with experimental value. Photoluminescence spectrum of 8HQ2C5N crystal showed the yellow emission. The crystal had the single shot laser damage threshold of 5.562 GW/cm{sup 2}. Microhardness measurement showed that 8HQ2C5N belongs to a soft material category. - Highlights: • A new organic single crystals were grown and the crystal structure was reported. • Crystal possess, good transmittance, thermal and mechanical stability. • Single shot LDT value is found to be

  3. All-optical signal processing in quadratic nonlinear materials

    DEFF Research Database (Denmark)

    Johansen, Steffen Kjær

    2002-01-01

    of materials with a second order nonlinearity, the so-called X(2) materials, is faster and stronger than that of more conventional materials with a cubic nonlinearity. The X(2) materials support spatial solitons consisting of two coupled components, the fundamental wave (FW) and its second harmonic (SH......). During this project the interaction between such spatial solitons has been investigated theoretically through perturbation theory and experimentally via numerical simulations. The outcome of this research isnew theoretical tools for quantitatively predicting the escape angle, i.e. the angle of incidence...... are dedicated to this part of the research. In chapter 4 the generality of the theoretical approach is emphasised with the derivation and verification of equivalent tools for media with a saturable nonlinearity. The strength of the X(2) nonlinearity strongly depends on the phase mismatch between the FW...

  4. Synthesis, characterization and third-order nonlinear optical ...

    Indian Academy of Sciences (India)

    2016-09-20

    Sep 20, 2016 ... the past, several strategies have been evolved to enhance the third-order nonlinear ..... retical fit using the formulation given in ref. [22]. Fit param- ..... Acknowledgement. The corresponding author acknowledges the financial.

  5. Polaron effects on nonlinear optical rectification in asymmetrical Gaussian potential quantum wells with applied electric fields

    International Nuclear Information System (INIS)

    Wu, Jinghe; Guo, Kangxian; Liu, Guanghui

    2014-01-01

    Polaron effects on nonlinear optical rectification in asymmetrical Gaussian potential quantum wells are studied by the effective mass approximation and the perturbation theory. The numerical results show that nonlinear optical rectification coefficients are strongly dependent on the barrier hight V 0 of the Gaussian potential quantum wells, the range L of the confinement potential and the electric field F. Besides, the numerical results show that no matter how V 0 , L and F change, taking into consideration polaron effects, the optical rectification coefficients χ 0 (2) get greatly enhanced.

  6. CW all optical self switching in nonlinear chalcogenide nano plasmonic directional coupler

    Science.gov (United States)

    Motamed-Jahromi, Leila; Hatami, Mohsen

    2018-04-01

    In this paper we obtain the coupling coefficient of plasmonic directional coupler (PDC) made up of two parallel monolayer waveguides filled with high nonlinear chalcogenide material for TM mode in continues wave (CW) regime. In addition, we assume each waveguides acts as a perturbation to other waveguide. Four nonlinear-coupled equations are derived. Transfer distances are numerically calculated and used for deriving length of all optical switch. The length of designed switch is in the range of 10-1000 μm, and the switching power is in the range of 1-100 W/m. Obtained values are suitable for designing all optical elements in the integrated optical circuits.

  7. Alkali-Responsive Absorption Spectra and Third-Order Optical Nonlinearities of Imino Squaramides

    International Nuclear Information System (INIS)

    Li Zhong-Yu; Xu Song; Zhou Xin-Yu; Zhang Fu-Shi

    2012-01-01

    Third-order optical nonlinearities and dynamic responses of two imino squaramides under neutral and base conditions were studied using the femtosecond degenerate four-wave mixing technique at 800 nm. Ultrafast optical responses have been observed and the magnitude of the second-order hyperpolarizabilities of the squaramides has been measured to be as large as 10 −31 esu. The absorption spectra, color of solution, and third-order optical nonlinearities of two imino squaramides change with the addition of sodium hydroxide. The γ value under the base condition for each dye is approximately 1.25 times larger than that under neutral conditions. (fundamental areas of phenomenology(including applications))

  8. Nonlinear optical behaviour of absorbing CdSxSe1-x interference filters

    International Nuclear Information System (INIS)

    Ferencz, K.; Szipoecs, R.

    1988-01-01

    First experimental results of nonlinear, thin film interference filter wedges with mixed CdS x Se 1-x as spacer material at the 633 nm wavelength of He-Ne laser are reported. Optical bistability is observed with less than 7.5 mW of optical power in single-cavity structures. The change in refractive index is found to be positive which is in accordance with the thermal mechanism of nonlinearity. Producing a double-cavity structure a device is obtained which works as an optical astable multivibrator having periodical change of transmission as the function of time. (author)

  9. Light-induced second-order nonlinear optical properties of molecular materials

    International Nuclear Information System (INIS)

    Fiorini, Celine

    1995-01-01

    We present a theoretical and experimental study of all-optical orientation. The work focusses more particularly on the realization of poled polymers for quadratic nonlinear optics. It is shown that the coherent superposition of two beams at fundamental and second harmonic frequencies results in the breaking of the former centro-symmetry of the material. The source is a Neodymium-YAG laser delivering 25 ps pulses at 1064 nm. The incident second-harmonic beam is obtained by frequency doubling in a KDP crystal. Using a phase conjugation configuration based on six-wave mixing interactions, we have Investigated in detail the mechanism of photo-induced second-harmonic generation in initially centrosymmetric materials. It is shown that the light-induced non-centro-symmetry is due to an orientational hole burning of the molecules. The process involves interference effects between one and two photon absorptions. Experiments are performed in various solutions of an azo-dye molecule (Disperse Red One). The possibility of inducing quasi-permanent second-order susceptibility in a PMMA polymer matrix doped with the azo-dye molecule of Disperse Red One is also demonstrated. The method of all-optical poling consists in a seeding type process with alternate writing and probing phases. Permanent orientation of the molecules can be described in terms of photo-isomerization processes. It leads to a poling of the molecules with a spatial modulation which is phase-matched for frequency doubling. Relevant parameters leading to an efficient polarisation of the sample are identified. A theoretical modelling of the different phenomena observed is proposed. Last part of the study is devoted to an enlarged study of the potentialities offered by this dual-frequency holography technique: orientation of octupolar molecules, polarisation of highly transparent materials. We also show that the new techniques developed during this work can also reveal to be complementary methods for nonlinear

  10. Nonlinear Methods in Riemannian and Kählerian Geometry

    CERN Document Server

    Jost, Jürgen

    1991-01-01

    In this book, I present an expanded version of the contents of my lectures at a Seminar of the DMV (Deutsche Mathematiker Vereinigung) in Düsseldorf, June, 1986. The title "Nonlinear methods in complex geometry" already indicates a combination of techniques from nonlinear partial differential equations and geometric concepts. In older geometric investigations, usually the local aspects attracted more attention than the global ones as differential geometry in its foundations provides approximations of local phenomena through infinitesimal or differential constructions. Here, all equations are linear. If one wants to consider global aspects, however, usually the presence of curvature Ieads to a nonlinearity in the equations. The simplest case is the one of geodesics which are described by a system of second ordernonlinear ODE; their linearizations are the Jacobi fields. More recently, nonlinear PDE played a more and more pro~inent röle in geometry. Let us Iist some of the most important ones: - harmonic maps ...

  11. Nonlinear optical rectification in a vertically coupled lens-shaped InAs/GaAs quantum dots with wetting layers under hydrostatic pressure and temperature

    Energy Technology Data Exchange (ETDEWEB)

    Ben Mahrsia, R.; Choubani, M., E-mail: mohsenchoubani3@yahoo.fr; Bouzaiene, L.; Maaref, H.

    2016-06-25

    In this paper we explore the structure parameters, hydrostatic pressure and temperature effects on Nonlinear optical rectification (NOR) in an asymmetric vertically coupled lens-shaped InAs/GaAs quantum dots. During epitaxial growth, lens-shaped quantum dots (QDs) are formed on the wetting layer (WL). Many theoretical works have neglected WL and its effect on nonlinear optical properties of QD-based systems for sake of simplicity. However, in this work the WL has been shown to be so influential in the intersubband energy and nonlinear optical rectification magnitude. Also, a detailed and comprehensive study of the nonlinear optical rectification is theoretical investigated within the framework of the compact density-matrix approach and finite difference method (FDM). It's found that nonlinear optical rectification coefficient is strongly affected not only by the WL, but also by the pressure, temperature and the coupled width between the QDs. Obtained results revealed that a red or a blue shift cane be observed. This behavior in the NOR gives a new degree of freedom in regions of interest for device applications. - Highlights: • Vertically coupled lens-shaped InAs/GaAs quantum dots is investigated. • Photon energy shifts towards the red with increasing pressure. • Photon energy shifts towards the blue with increasing temperature. • Intersubband energy decreases with increasing the wetting layer width. • Nonlinear optical rectification magnitude is controlled and adjusted.

  12. Achieving nonlinear optical modulation via four-wave mixing in a four-level atomic system

    Science.gov (United States)

    Li, Hai-Chao; Ge, Guo-Qin; Zubairy, M. Suhail

    2018-05-01

    We propose an accessible scheme for implementing tunable nonlinear optical amplification and attenuation via a synergetic mechanism of four-wave mixing (FWM) and optical interference in a four-level ladder-type atomic system. By constructing a cyclic atom-field interaction, we show that two reverse FWM processes can coexist via optical transitions in different branches. In the suitable input-field conditions, strong interference effects between the input fields and the generated FWM fields can be induced and result in large amplification and deep attenuation of the output fields. Moreover, such an optical modulation from enhancement to suppression can be controlled by tuning the relative phase. The quantum system can be served as a switchable optical modulator with potential applications in quantum nonlinear optics.

  13. Linear and Nonlinear Optical Properties of Micrometer-Scale Gold Nanoplates

    International Nuclear Information System (INIS)

    Liu Xiao-Lan; Peng Xiao-Niu; Yang Zhong-Jian; Li Min; Zhou Li

    2011-01-01

    Micrometer-scale gold nanoplates have been synthesized in high yield through a polyol process. The morphology, crystal structure and linear optical extinction of the gold nanoplates have been characterized. These gold nanoplates are single-crystalline with triangular, truncated triangular and hexagonal shapes, exhibiting strong surface plasmon resonance (SPR) extinction in the visible and near-infrared (NIR) region. The linear optical properties of gold nanoplates are also investigated by theoretical calculations. We further investigate the nonlinear optical properties of the gold nanoplates in solution by Z-scan technique. The nonlinear absorption (NLA) coefficient and nonlinear refraction (NLR) index are measured to be 1.18×10 2 cm/GW and −1.04×10 −3 cm 2 /GW, respectively. (condensed matter: electronic structure, electrical, magnetic, and optical properties)

  14. Nonlinear optics response of semiconductor quantum wells under high magnetic fields

    International Nuclear Information System (INIS)

    Chemla, D.S.

    1993-07-01

    Recent investigations on the nonlinear optical response of semiconductor quantum wells in a strong perpendicular magnetic field, H, are reviewed. After some introductory material the evolution of the linear optical properties of GaAs QW's as a function of H is discussed; an examination is made of how the magneto-excitons (MX) extrapolate continuously between quasi-2D QW excitons (X) when H = 0, and pairs of Landau levels (LL) when H → ∞. Next, femtosecond time resolved investigations of their nonlinear optical response are presented; the evolution of MX-MX interactions with increasing H is stressed. Finally, how, as the dimensionality is reduced by application of H, the number of scattering channels is limited and relaxation of electron-hole pairs is affected. How nonlinear optical spectroscopy can be exploited to access the relaxation of angular momentum within magneto-excitons is also discussed

  15. A nonlinear plasmonic resonator for three-state all-optical switching

    KAUST Repository

    Amin, Muhammad

    2014-01-01

    A nonlinear plasmonic resonator design is proposed for three-state all-optical switching at frequencies including near infrared and lower red parts of the spectrum. The tri-stable response required for three-state operation is obtained by enhancing nonlinearities of a Kerr medium through multiple (higher order) plasmons excited on resonator\\'s metallic surfaces. Indeed, simulations demonstrate that exploitation of multiple plasmons equips the proposed resonator with a multi-band tri-stable response, which cannot be obtained using existing nonlinear plasmonic devices that make use of single mode Lorentzian resonances. Multi-band three-state optical switching that can be realized using the proposed resonator has potential applications in optical communications and computing. © 2014 Optical Society of America.

  16. Nonlinear optical measurements of conducting copolymers of aniline under CW laser excitation

    Science.gov (United States)

    Pramodini, S.; Poornesh, P.

    2015-08-01

    Synthesis and measurements of third-order optical nonlinearity and optical limiting of conducting copolymers of aniline are presented. Single beam z-scan technique was employed for the nonlinear optical studies. Continuous wave He-Ne laser operating at 633 nm was used as the source of excitation. Copolymer samples exhibited reverse saturable absorption (RSA) process. The nonlinear refraction studies depict that the copolymers exhibit self-defocusing property. The estimated values of βeff, n2 and χ(3) were found to be of the order of 10-2 cm/W, 10-5 esu and 10-7 esu respectively. Self-diffraction rings were observed due to refractive index change when exposed to the laser beam. A good optical limiting and clamping of power of ∼0.9 mW and ∼0.05 mW was observed. Therefore, copolymers of aniline emerge as a potential candidate for photonic device applications.

  17. Optical super-resolution effect induced by nonlinear characteristics of graphene oxide films

    Science.gov (United States)

    Zhao, Yong-chuang; Nie, Zhong-quan; Zhai, Ai-ping; Tian, Yan-ting; Liu, Chao; Shi, Chang-kun; Jia, Bao-hua

    2018-01-01

    In this work, we focus on the optical super-resolution effect induced by strong nonlinear saturation absorption (NSA) of graphene oxide (GO) membranes. The third-order optical nonlinearities are characterized by the canonical Z-scan technique under femtosecond laser (wavelength: 800 nm, pulse width: 100 fs) excitation. Through controlling the applied femtosecond laser energy, NSA of the GO films can be tuned continuously. The GO film is placed at the focal plane as a unique amplitude filter to improve the resolution of the focused field. A multi-layer system model is proposed to present the generation of a deep sub-wavelength spot associated with the nonlinearity of GO films. Moreover, the parameter conditions to achieve the best resolution (˜λ/6) are determined entirely. The demonstrated results here are useful for high density optical recoding and storage, nanolithography, and super-resolution optical imaging.

  18. A nonlinear plasmonic resonator for three-state all-optical switching

    KAUST Repository

    Amin, Muhammad; Farhat, Mohamed; Bagci, Hakan

    2014-01-01

    A nonlinear plasmonic resonator design is proposed for three-state all-optical switching at frequencies including near infrared and lower red parts of the spectrum. The tri-stable response required for three-state operation is obtained by enhancing nonlinearities of a Kerr medium through multiple (higher order) plasmons excited on resonator's metallic surfaces. Indeed, simulations demonstrate that exploitation of multiple plasmons equips the proposed resonator with a multi-band tri-stable response, which cannot be obtained using existing nonlinear plasmonic devices that make use of single mode Lorentzian resonances. Multi-band three-state optical switching that can be realized using the proposed resonator has potential applications in optical communications and computing. © 2014 Optical Society of America.

  19. Modulation stability and optical soliton solutions of nonlinear Schrödinger equation with higher order dispersion and nonlinear terms and its applications

    Science.gov (United States)

    Arshad, Muhammad; Seadawy, Aly R.; Lu, Dianchen

    2017-12-01

    In optical fibers, the higher order non-linear Schrödinger equation (NLSE) with cubic quintic nonlinearity describes the propagation of extremely short pulses. We constructed bright and dark solitons, solitary wave and periodic solitary wave solutions of generalized higher order NLSE in cubic quintic non Kerr medium by applying proposed modified extended mapping method. These obtained solutions have key applications in physics and mathematics. Moreover, we have also presented the formation conditions on solitary wave parameters in which dark and bright solitons can exist for this media. We also gave graphically the movement of constructed solitary wave and soliton solutions, that helps to realize the physical phenomena's of this model. The stability of the model in normal dispersion and anomalous regime is discussed by using the modulation instability analysis, which confirms that all constructed solutions are exact and stable. Many other such types of models arising in applied sciences can also be solved by this reliable, powerful and effective method.

  20. Observation and measurement of interaction-induced dispersive optical nonlinearities in an ensemble of cold rydberg atoms

    DEFF Research Database (Denmark)

    Parigi, V.; Bimbard, E.; Stanojevic, J.

    2012-01-01

    We observe and measure dispersive optical nonlinearities in an ensemble of cold Rydberg atoms placed inside an optical cavity. The experimental results are in agreement with a simple model where the optical nonlinearities are due to the progressive appearance of a Rydberg blockaded volume within...

  1. Non-linear M -sequences Generation Method

    Directory of Open Access Journals (Sweden)

    Z. R. Garifullina

    2011-06-01

    Full Text Available The article deals with a new method for modeling a pseudorandom number generator based on R-blocks. The gist of the method is the replacement of a multi digit XOR element by a stochastic adder in a parallel binary linear feedback shift register scheme.

  2. New Efficient Fourth Order Method for Solving Nonlinear Equations

    Directory of Open Access Journals (Sweden)

    Farooq Ahmad

    2013-12-01

    Full Text Available In a paper [Appl. Math. Comput., 188 (2 (2007 1587--1591], authors have suggested and analyzed a method for solving nonlinear equations. In the present work, we modified this method by using the finite difference scheme, which has a quintic convergence. We have compared this modified Halley method with some other iterative of fifth-orders convergence methods, which shows that this new method having convergence of fourth order, is efficient.

  3. New Conjugacy Conditions and Related Nonlinear Conjugate Gradient Methods

    International Nuclear Information System (INIS)

    Dai, Y.-H.; Liao, L.-Z.

    2001-01-01

    Conjugate gradient methods are a class of important methods for unconstrained optimization, especially when the dimension is large. This paper proposes a new conjugacy condition, which considers an inexact line search scheme but reduces to the old one if the line search is exact. Based on the new conjugacy condition, two nonlinear conjugate gradient methods are constructed. Convergence analysis for the two methods is provided. Our numerical results show that one of the methods is very efficient for the given test problems

  4. Harnessing mode-selective nonlinear optics for on-chip multi-channel all-optical signal processing

    Directory of Open Access Journals (Sweden)

    Ming Ma

    2016-11-01

    Full Text Available All-optical signal processing based on nonlinear optical effects allows for the realization of important functions in telecommunications including wavelength conversion, optical multiplexing/demultiplexing, Fourier transformation, and regeneration, amongst others, on ultrafast time scales to support high data rate transmission. In integrated photonic subsystems, the majority of all-optical signal processing systems demonstrated to date typically process only a single channel at a time or perform a single processing function, which imposes a serious limitation on the functionality of integrated solutions. Here, we demonstrate how nonlinear optical effects can be harnessed in a mode-selective manner to perform simultaneous multi-channel (two and multi-functional optical signal processing (i.e., regenerative wavelength conversion in an integrated silicon photonic device. This approach, which can be scaled to a higher number of channels, opens up a new degree of freedom for performing a broad range of multi-channel nonlinear optical signal processing functions using a single integrated photonic device.

  5. Design and Development of Nonlinear Optical Microscope System: Simple Implementation with epi-Illumination Platform

    Directory of Open Access Journals (Sweden)

    Ryu Jiheun

    2015-01-01

    Full Text Available During the research using fluorescence-tagged or auto-fluorescence molecules, meaningful information is often buried deep inside the tissue, not its surface. Therefore, especially in the field of biomedical imaging, acquiring optically sectioned images from deep inside the tissue is very important. As well know already, confocal laser scanning microscopy (the most well-known optical sectioning microscopy gives axially-resolved fluorescence information using the physical background blocking component called pinhole. However, the axial range of imaging is practically limited due to such optical phenomena as the light scattered and absorbed in the tissue. However, nonlinear optical microscopy (e.g. Multiphoton microscopy, harmonic generation microscopy, coherent anti-Stokes Raman spectroscopy realized by the development of ultrafast light sources has been used for visualizing various tissues, especially in vivo, because of their low sensitivity to the limitation caused by the scattering and the absorption of light. Although nonlinear optical microscopy gives deep tissue image, it is not easy for many researcher to build customized nonlinear system. Here, we introduce an easy and simple way designing and developing such nonlinear optical microscope with upright or inverted epi-illumination platform using commercial optical components only.

  6. Large third-order optical nonlinearity in vertically oriented mesoporous silica thin films embedded with Ag nanoparticles

    Energy Technology Data Exchange (ETDEWEB)

    Tan, Min; Liu, Qiming, E-mail: qmliu@whu.edu.cn [Wuhan University, Key Laboratory of Artificial Micro- and Nano-structures of Ministry of Education, School of Physics and Technology (China)

    2016-12-15

    Taking advantage of the channel confinement of mesoporous films to prevent the agglomeration of Ag nanoparticles to achieve large third-order optical nonlinearity in amorphous materials, Ag-loaded composite mesoporous silica film was prepared by the electrochemical deposition method on ITO substrate. Ag ions were firstly transported into the channels of mesoporous film by the diffusion and binding force of channels, which were reduced to nanoparticles by applying suitable voltage. The existence and uniform distribution of Ag nanoparticles ranging in 1–10 nm in the mesoporous silica thin films were exhibited by UV spectrophotometer, X-ray powder diffraction (XRD), transmission electron microscopy (TEM), and X-ray photoelectron spectroscopy (XPS) measurements. The third-order optical nonlinearity induced by Ag nanoparticles was studied by the Z-scan technique. Due to the local field surface plasmon resonance, the maximum third-order nonlinear optical susceptibility of Ag-loaded composite mesoporous silica film is 1.53×10{sup −10} esu, which is 1000 times larger than that of the Ag-contained chalcogenide glasses which showed large nonlinearity in amorphous materials.

  7. Effects of high light intensities on the optical Kerr nonlinearity of semiconducting polymers

    International Nuclear Information System (INIS)

    Charra, Fabrice

    1990-01-01

    Experimental investigations, in the picosecond time scale, of the Kerr type optical nonlinearity (or pump and probe) are presented. The nonlinear molecules semiconducting polymers of the type poly-diacetylene. The degenerate case (pump and probe at the same frequency) has been studied by four wave mixing at 1064 nm, in the configuration of phase conjugation. It is shown that the response is dominated by high orders of nonlinearity. The results are analysed in terms of two photon resonance. The non-degenerate case is studied by two wave mixing or in the optical Kerr gate experiment. The optical Stark effect and the differential spectra of photoinduced species are analysed. Two photon excitations at 1064 nm and one photon excitations at 532 nm are compared. A consequence of the mechanism of the nonlinearity is the possibility of generating phase conjugate waves at double frequency. The theoretical analysis and the experimental demonstration of this process are presented. The experiment is only sensitive to nonlinearities of the fifth order or more and thus allows to clarify its origins and dynamics. Finally, quantum modelling and calculations of the nonlinear optical responses, developed for the interpretations of the above experiments, are presented. (author) [fr

  8. Input signal shaping based on harmonic frequency response function for suppressing nonlinear optical frequency in frequency-scanning interferometry

    Science.gov (United States)

    Zhu, Yu; Liu, Zhigang; Deng, Wen; Deng, Zhongwen

    2018-05-01

    Frequency-scanning interferometry (FSI) using an external cavity diode laser (ECDL) is essential for many applications of the absolute distance measurement. However, owing to the hysteresis and creep of the piezoelectric actuator inherent in the ECDL, the optical frequency scanning exhibits a nonlinearity that seriously affects the phase extraction accuracy of the interference signal and results in the reduction of the measurement accuracy. To suppress the optical frequency nonlinearity, a harmonic frequency synthesis method for shaping the desired input signal instead of the original triangular wave is presented. The effectiveness of the presented shaping method is demonstrated through the comparison of the experimental results. Compared with an incremental Renishaw interferometer, the standard deviation of the displacement measurement of the FSI system is less than 2.4 μm when driven by the shaped signal.

  9. Variation Iteration Method for The Approximate Solution of Nonlinear ...

    African Journals Online (AJOL)

    In this study, we considered the numerical solution of the nonlinear Burgers equation using the Variational Iteration Method (VIM). The method seeks to examine the convergence of solutions of the Burgers equation at the expense of the parameters x and t of which the amount of errors depends. Numerical experimentation ...

  10. Interior Point Methods for Large-Scale Nonlinear Programming

    Czech Academy of Sciences Publication Activity Database

    Lukšan, Ladislav; Matonoha, Ctirad; Vlček, Jan

    2005-01-01

    Roč. 20, č. 4-5 (2005), s. 569-582 ISSN 1055-6788 R&D Projects: GA AV ČR IAA1030405 Institutional research plan: CEZ:AV0Z10300504 Keywords : nonlinear programming * interior point methods * KKT systems * indefinite preconditioners * filter methods * algorithms Subject RIV: BA - General Mathematics Impact factor: 0.477, year: 2005

  11. Mathematical optics classical, quantum, and computational methods

    CERN Document Server

    Lakshminarayanan, Vasudevan

    2012-01-01

    Going beyond standard introductory texts, Mathematical Optics: Classical, Quantum, and Computational Methods brings together many new mathematical techniques from optical science and engineering research. Profusely illustrated, the book makes the material accessible to students and newcomers to the field. Divided into six parts, the text presents state-of-the-art mathematical methods and applications in classical optics, quantum optics, and image processing. Part I describes the use of phase space concepts to characterize optical beams and the application of dynamic programming in optical wave

  12. Nonlinear conjugate gradient methods in micromagnetics

    Directory of Open Access Journals (Sweden)

    J. Fischbacher

    2017-04-01

    Full Text Available Conjugate gradient methods for energy minimization in micromagnetics are compared. The comparison of analytic results with numerical simulation shows that standard conjugate gradient method may fail to produce correct results. A method that restricts the step length in the line search is introduced, in order to avoid this problem. When the step length in the line search is controlled, conjugate gradient techniques are a fast and reliable way to compute the hysteresis properties of permanent magnets. The method is applied to investigate demagnetizing effects in NdFe12 based permanent magnets. The reduction of the coercive field by demagnetizing effects is μ0ΔH = 1.4 T at 450 K.

  13. An analog model for quantum lightcone fluctuations in nonlinear optics

    International Nuclear Information System (INIS)

    Ford, L.H.; De Lorenci, V.A.; Menezes, G.; Svaiter, N.F.

    2013-01-01

    We propose an analog model for quantum gravity effects using nonlinear dielectrics. Fluctuations of the spacetime lightcone are expected in quantum gravity, leading to variations in the flight times of pulses. This effect can also arise in a nonlinear material. We propose a model in which fluctuations of a background electric field, such as that produced by a squeezed photon state, can cause fluctuations in the effective lightcone for probe pulses. This leads to a variation in flight times analogous to that in quantum gravity. We make some numerical estimates which suggest that the effect might be large enough to be observable. - Highlights: ► Lightcone fluctuations, quantum fluctuations of the effective speed of light, are a feature of quantum gravity. ► Nonlinear dielectrics have a variable speed of light, analogous to the effects of gravity. ► Fluctuating electric fields create the effect of lightcone fluctuations in a nonlinear material. ► We propose to use squeezed light in a nonlinear material as an analog model of lightcone fluctuations. ► Variation in the speed of propagation of pulses is the observational signature of lightcone fluctuations.

  14. Studies on third-order optical nonlinearity and power limiting of conducting polymers using the z-scan technique for nonlinear optical applications

    International Nuclear Information System (INIS)

    Pramodini, S; Poornesh, P; Sudhakar, Y N; SelvaKumar, M

    2014-01-01

    We present the synthesis and characterization of third-order optical nonlinearity and optical limiting of the conducting polymers poly (aniline-co-o-anisidine) and poly (aniline-co-pyrrole). Nonlinear optical studies were carried out by employing the z-scan technique using a He–Ne laser operating in continuous wave mode at 633 nm. The copolymers exhibited a reverse saturable absorption process and self-defocusing properties under the experimental conditions. The estimated values of β eff , n 2 and χ (3) were found to be of the order of 10 −2  cm W −1 , 10 -5  esu and 10 −7  esu respectively. Self-diffraction rings were observed due to refractive index change when exposed to the laser beam. The copolymers possess a lower limiting threshold and clamping level, which is essential to a great extent for power limiting devices. Therefore, copolymers of aniline emerge as a potential candidate for nonlinear optical device applications. (paper)

  15. Dynamics of Nonlinear Excitation of the High-Order Mode in a Single-Mode Step-Index Optical Fiber

    Science.gov (United States)

    Burdin, V.; Bourdine, A.

    2018-04-01

    This work is concerned with approximate model of higher-order mode nonlinear excitation in a singlemode silica optical fiber. We present some results of simulation for step-index optical fiber under femtosecond optical pulse launching, which confirm ability of relatively stable higher-order mode excitation in such singlemode optical fiber over sufficiently narrow range of launched optical power variation.

  16. Analysis of Nonlinear Dynamics by Square Matrix Method

    Energy Technology Data Exchange (ETDEWEB)

    Yu, Li Hua [Brookhaven National Lab. (BNL), Upton, NY (United States). Energy and Photon Sciences Directorate. National Synchrotron Light Source II

    2016-07-25

    The nonlinear dynamics of a system with periodic structure can be analyzed using a square matrix. In this paper, we show that because the special property of the square matrix constructed for nonlinear dynamics, we can reduce the dimension of the matrix from the original large number for high order calculation to low dimension in the first step of the analysis. Then a stable Jordan decomposition is obtained with much lower dimension. The transformation to Jordan form provides an excellent action-angle approximation to the solution of the nonlinear dynamics, in good agreement with trajectories and tune obtained from tracking. And more importantly, the deviation from constancy of the new action-angle variable provides a measure of the stability of the phase space trajectories and their tunes. Thus the square matrix provides a novel method to optimize the nonlinear dynamic system. The method is illustrated by many examples of comparison between theory and numerical simulation. Finally, in particular, we show that the square matrix method can be used for optimization to reduce the nonlinearity of a system.

  17. Exponential function method for solving nonlinear ordinary ...

    Indian Academy of Sciences (India)

    [14] introduced a new system of rational. 79 ..... Also, for k-power of function f (η), by induction, we have ..... reliability and efficiency of the method. .... electric field and the polarization effects are negligible and B(x) is assumed by Chaim [8] as.

  18. Nonlinear structural analysis using integrated force method

    Indian Academy of Sciences (India)

    A new formulation termed the Integrated Force Method (IFM) was proposed by Patnaik ... nated ``Structure (nY m)'' where (nY m) are the force and displacement degrees of ..... Patnaik S N, Yadagiri S 1976 Frequency analysis of structures.

  19. New nonlinear methods for linear transport calculations

    International Nuclear Information System (INIS)

    Adams, M.L.

    1993-01-01

    We present a new family of methods for the numerical solution of the linear transport equation. With these methods an iteration consists of an 'S N sweep' followed by an 'S 2 -like' calculation. We show, by analysis as well as numerical results, that iterative convergence is always rapid. We show that this rapid convergence does not depend on a consistent discretization of the S 2 -like equations - they can be discretized independently from the S N equations. We show further that independent discretizations can offer significant advantages over consistent ones. In particular, we find that in a wide range of problems, an accurate discretization of the S 2 -like equation can be combined with a crude discretization of the S N equations to produce an accurate S N answer. We demonstrate this by analysis as well as numerical results. (orig.)

  20. Synthesis and characterization of silver nanoparticles from Alpinia calcarata by Green approach and its applications in bactericidal and nonlinear optics

    Energy Technology Data Exchange (ETDEWEB)

    Pugazhendhi, S.; Kirubha, E. [Department of Physics, Anna University, Chennai 600 025 (India); Palanisamy, P.K. [Department of Medical Physics, Anna University, Chennai 600 025 (India); Gopalakrishnan, R., E-mail: krgkrishnan@yahoo.com [Department of Physics, Anna University, Chennai 600 025 (India)

    2015-12-01

    Graphical abstract: - Highlights: • Alpinia calcarata root extract was used for the synthesis Ag nanoparticle. • AgNPs show remarkable stability at 25–30 °C. • The morphologies of the AgNPs were analyzed using HRTEM. • AgNPs exhibit good nonlinear optical behaviour and antimicrobial activities. - Abstract: Development of green route for the synthesis of nanoparticles with plant extracts plays a very important role in nanotechnology without any toxicity chemicals. Herein we report a new approach to synthesize silver nanoparticles (AgNPs) using aqueous extract of Alpinia calcarata root as a reducing as well as stabilizing agent. The crystal structure and purity of the synthesized AgNPs were studied using Powder X-ray Diffraction analysis. The Surface Plasmon Resonance bands of synthesized silver nanoparticles have been obtained and monitored using UV–Visible spectrum. The morphologies of the AgNPs were analyzed using High resolution transmission electron microscopy (HRTEM). The elements present in the A. calcarata extract were determined by the inductively coupled plasma-optical emission Spectrometry (ICP-OES) and Fourier transform infrared spectroscopy (FTIR). Silver nanoparticles from A. calcarata possess very good antimicrobial activity which was confirmed by resazurin dye reduction assay method and thus it is a potential source of antimicrobial agent. The synthesized Ag nanoparticles exhibit good optical nonlinearity and the nonlinear optical studies have been carried out by Z-scan technique.

  1. Synthesis and characterization of silver nanoparticles from Alpinia calcarata by Green approach and its applications in bactericidal and nonlinear optics

    International Nuclear Information System (INIS)

    Pugazhendhi, S.; Kirubha, E.; Palanisamy, P.K.; Gopalakrishnan, R.

    2015-01-01

    Graphical abstract: - Highlights: • Alpinia calcarata root extract was used for the synthesis Ag nanoparticle. • AgNPs show remarkable stability at 25–30 °C. • The morphologies of the AgNPs were analyzed using HRTEM. • AgNPs exhibit good nonlinear optical behaviour and antimicrobial activities. - Abstract: Development of green route for the synthesis of nanoparticles with plant extracts plays a very important role in nanotechnology without any toxicity chemicals. Herein we report a new approach to synthesize silver nanoparticles (AgNPs) using aqueous extract of Alpinia calcarata root as a reducing as well as stabilizing agent. The crystal structure and purity of the synthesized AgNPs were studied using Powder X-ray Diffraction analysis. The Surface Plasmon Resonance bands of synthesized silver nanoparticles have been obtained and monitored using UV–Visible spectrum. The morphologies of the AgNPs were analyzed using High resolution transmission electron microscopy (HRTEM). The elements present in the A. calcarata extract were determined by the inductively coupled plasma-optical emission Spectrometry (ICP-OES) and Fourier transform infrared spectroscopy (FTIR). Silver nanoparticles from A. calcarata possess very good antimicrobial activity which was confirmed by resazurin dye reduction assay method and thus it is a potential source of antimicrobial agent. The synthesized Ag nanoparticles exhibit good optical nonlinearity and the nonlinear optical studies have been carried out by Z-scan technique.

  2. Spectral dependence of third-order nonlinear optical properties in InN

    International Nuclear Information System (INIS)

    Ahn, H.; Lee, M.-T.; Chang, Y.-M.

    2014-01-01

    We report on the nonlinear optical properties of InN measured in a wide near-infrared spectral range with the femtosecond Z-scan technique. The above-bandgap nonlinear absorption in InN is found to originate from the saturation of absorption by the band-state-filling and its cross-section increases drastically near the bandgap energy. With below-bandgap excitation, the nonlinear absorption undergoes a transition from saturation absorption (SA) to reverse-SA (RSA), attributed to the competition between SA of band-tail states and two-photon-related RSA. The measured large nonlinear refractive index of the order of 10 −10 cm 2 /W indicates InN as a potential material for all-optical switching and related applications

  3. Ultrafast Relaxation Dynamics of the Optical Nonlinearity in Nanometric Gold Particles

    International Nuclear Information System (INIS)

    Puech, K.; Blau, W.J.

    2001-01-01

    Measurements of the resonantly enhanced, third-order nonlinear optical properties of gold nanostructures exhibiting reduced charge-carrier mobility in three dimensions were performed with a number of ultrafast nonlinear optical techniques. The size of the particles investigated was varied between 5 and 40 nm. The magnitude of the nonlinear susceptibility is of the order of 5.10 -16 m 2 V -2 at resonance and an order of magnitude lower off-resonance. The response time of the nonlinearity is found to be extremely fast and could not be resolved in the experiments undertaken here. The only statement that can be made in this regard is that the phase relaxation time is of the order of or less than 20 fs while the energy relaxation time is of the order of or less than 75 fs

  4. Structural control of nonlinear optical absorption and refraction in dense metal nanoparticle arrays.

    Science.gov (United States)

    Kohlgraf-Owens, Dana C; Kik, Pieter G

    2009-08-17

    The linear and nonlinear optical properties of a composite containing interacting spherical silver nanoparticles embedded in a dielectric host are studied as a function of interparticle separation using three dimensional frequency domain simulations. It is shown that for a fixed amount of metal, the effective third-order nonlinear susceptibility of the composite chi((3))(omega) can be significantly enhanced with respect to the linear optical properties, due to a combination of resonant surface plasmon excitation and local field redistribution. It is shown that this geometry-dependent susceptibility enhancement can lead to an improved figure of merit for nonlinear absorption. Enhancement factors for the nonlinear susceptibility of the composite are calculated, and the complex nature of the enhancement factors is discussed.

  5. Physical origin of third order non-linear optical response of porphyrin nanorods

    International Nuclear Information System (INIS)

    Mongwaketsi, N.; Khamlich, S.; Pranaitis, M.; Sahraoui, B.; Khammar, F.; Garab, G.; Sparrow, R.; Maaza, M.

    2012-01-01

    The non-linear optical properties of porphyrin nanorods were studied using Z-scan, Second and Third harmonic generation techniques. We investigated in details the heteroaggregate behaviour formation of [H 4 TPPS 4 ] 2- and [SnTPyP] 2+ mixture by means of the UV-VIS spectroscopy and aggregates structure and morphology by transmission electron microscopy. The porphyrin nanorods under investigation were synthesized by self assembly and molecular recognition method. They have been optimized in view of future application in the construction of the light harvesting system. The focus of this study was geared towards understanding the influence of the type of solvent used on these porphyrins nanorods using spectroscopic and microscopic techniques. Highlights: ► We synthesized porphyrin nanorods by self assembly and molecular recognition method. ► TEM images confirmed solid cylindrical shapes. ► UV-VIS spectroscopy showed the decrease in the absorbance peaks of the precursors. ► The enhanced third-order nonlinearities were observed.

  6. A new promising nonlinear optical (NLO) crystal for visible and ultraviolet (UV) regions

    Science.gov (United States)

    Gheorghe, L.; Achim, A.; Voicu, F.

    2012-08-01

    Different La1-xGdxSc3(BO3)4 compounds with 0 ≤ x ≤ 0.5 were synthesized by solid-state reaction method. The X-ray diffraction studies revealed that the compounds containing more than 30 at.% Gd3+ ions have non-centrosymmetric trigonal structure (space group R32) and, consequently they are optically nonlinear. A crystal of LaxGdyScz(BO3)4 (x+y+z = 4) - LGSB with La0.75Gd0.5Sc2.75(BO3)4 starting melt composition and relatively small dimensions (about 10 mm in diameter and 25 mm in length) was grown by the Czochralski method. In order to confirm the NLO property, the as-grown crystal was subjected to second-harmonic generation (SHG) test. The nonlinear coefficient d11 of LGSB crystal has been preliminary estimated to be about 1.9 pm/V, which is larger than that of YAl3(BO3)4 (YAB) crystal. This article has been formally retracted, please refer to the article PDF for the full retraction notice.

  7. Propagation and Interactions of Ultrahigh Power Light: Relativistic Nonlinear Optics

    Science.gov (United States)

    2014-09-30

    force of the ROS causes the bucket to constantly expand, trapping copious unwanted electrons, polluting the electron spectrum with a high-charge, low...Laser Wakefield Accelerator,” Conference on Lasers and Electro-Optics/Pacific Rim , C1094, Optical Society of America (2011). 19. Bunkers, K., Kalmykov

  8. Rational solitons in deep nonlinear optical Bragg grating

    NARCIS (Netherlands)

    Alatas, H.; Iskandar, A.A.; Tjia, M.O.; Valkering, T.P.

    2006-01-01

    We have examined the rational solitons in the Generalized Coupled Mode model for a deep nonlinear Bragg grating. These solitons are the degenerate forms of the ordinary solitons and appear at the transition lines in the parameter plane. A simple formulation is presented for the investigation of the

  9. Extreme non-linear elasticity and transformation optics

    DEFF Research Database (Denmark)

    Gersborg, Allan Roulund; Sigmund, Ole

    2010-01-01

    realizations correspond to minimizers of elastic energy potentials for extreme values of the mechanical Poisson's ratio ν . For TE (Hz) polarized light an incompressible transformation ν = 1/2 is ideal and for TM (E z) polarized light one should use a compressible transformation with negative Poissons's ratio......Transformation optics is a powerful concept for designing novel optical components such as high transmission waveguides and cloaking devices. The selection of specific transformations is a non-unique problem. Here we reveal that transformations which allow for all dielectric and broadband optical...... ν = -1. For the TM polarization the mechanical analogy corresponds to a modified Liao functional known from the transformation optics literature. Finally, the analogy between ideal transformations and solid mechanical material models automates and broadens the concept of transformation optics...

  10. Nonlinear optical properties of TeO$_2$ crystalline phases from first principles

    OpenAIRE

    Berkaine, Nabil; Orhan, Emmanuelle; Masson, Olivier; Thomas, Philippe; Junquera, Javier

    2010-01-01

    We have computed second and third nonlinear optical susceptibilities of two crystalline bulk tellurium oxide polymorphs: $\\alpha$-TeO$_{2}$ (the most stable crystalline bulk phase) and $\\gamma$-TeO$_{2}$ (the crystalline phase that ressembles the more to the glass phase. Third order nonlinear susceptibilities of the crystalline phases are two orders of magnitude larger than $\\alpha$-SiO$_{2}$ cristoballite, thus extending the experimental observations on glasses to the case of crystalline com...

  11. Matter-wave solitons and finite-amplitude Bloch waves in optical lattices with spatially modulated nonlinearity

    Science.gov (United States)

    Zhang, Jie-Fang; Li, Yi-Shen; Meng, Jianping; Wu, Lei; Malomed, Boris A.

    2010-09-01

    We investigate solitons and nonlinear Bloch waves in Bose-Einstein condensates trapped in optical lattices (OLs). By introducing specially designed localized profiles of the spatial modulation of the attractive nonlinearity, we construct an infinite set of exact soliton solutions in terms of Mathieu and elliptic functions, with the chemical potential belonging to the semi-infinite gap of the OL-induced spectrum. Starting from the particular exact solutions, we employ the relaxation method to construct generic families of soliton solutions in a numerical form. The stability of the solitons is investigated through the computation of the eigenvalues for small perturbations, and also by direct simulations. Finally, we demonstrate a virtually exact (in the numerical sense) composition relation between nonlinear Bloch waves and solitons.

  12. Matter-wave solitons and finite-amplitude Bloch waves in optical lattices with spatially modulated nonlinearity

    International Nuclear Information System (INIS)

    Zhang Jiefang; Meng Jianping; Wu Lei; Li Yishen; Malomed, Boris A.

    2010-01-01

    We investigate solitons and nonlinear Bloch waves in Bose-Einstein condensates trapped in optical lattices (OLs). By introducing specially designed localized profiles of the spatial modulation of the attractive nonlinearity, we construct an infinite set of exact soliton solutions in terms of Mathieu and elliptic functions, with the chemical potential belonging to the semi-infinite gap of the OL-induced spectrum. Starting from the particular exact solutions, we employ the relaxation method to construct generic families of soliton solutions in a numerical form. The stability of the solitons is investigated through the computation of the eigenvalues for small perturbations, and also by direct simulations. Finally, we demonstrate a virtually exact (in the numerical sense) composition relation between nonlinear Bloch waves and solitons.

  13. Pump-probe nonlinear magneto-optical rotation with frequency-modulated light

    International Nuclear Information System (INIS)

    Pustelny, S.; Gawlik, W.; Jackson Kimball, D. F.; Rochester, S. M.; Yashchuk, V. V.; Budker, D.

    2006-01-01

    Specific types of atomic coherences between Zeeman sublevels can be generated and detected using a method based on nonlinear magneto-optical rotation with frequency-modulated light. Linearly polarized, frequency-modulated light is employed to selectively generate ground-state coherences between Zeeman sublevels for which Δm=2 and Δm=4 in 85 Rb and 87 Rb atoms, and additionally Δm=6 in 85 Rb. The atomic coherences are detected with a separate, unmodulated probe light beam. Separation of the pump and probe beams enables independent investigation of the processes of creation and detection of the atomic coherences. With the present technique the transfer of the Zeeman coherences, including high-order coherences, from excited to ground state by spontaneous emission has been observed

  14. Nonlinear magneto-optical rotation with modulated light in tilted magnetic fields

    International Nuclear Information System (INIS)

    Pustelny, S.; Gawlik, W.; Rochester, S. M.; Kimball, D. F. Jackson; Yashchuk, V. V.; Budker, D.

    2006-01-01

    Larmor precession of laser-polarized atoms contained in antirelaxation-coated cells, detected via nonlinear magneto-optical rotation (NMOR), is a promising technique for a new generation of ultrasensitive atomic magnetometers. For magnetic fields directed along the light propagation direction, resonances in NMOR appear when linearly polarized light is frequency or amplitude modulated at twice the Larmor frequency. Because the frequency of these resonances depends on the magnitude but not the direction of the field, they are useful for scalar magnetometry. Additional NMOR resonances at the Larmor frequency appear when the magnetic field is tilted away from the light propagation direction in the plane defined by the light propagation and polarization vectors. These resonances, studied both experimentally and with a density matrix calculation in the present work, offer a convenient method of achieving additional information about a direction of the magnetic field

  15. Ultra-fast dynamics in the nonlinear optical response of silver nanoprism ordered arrays.

    Science.gov (United States)

    Sánchez-Esquivel, Héctor; Raygoza-Sanchez, Karen Y; Rangel-Rojo, Raúl; Kalinic, Boris; Michieli, Niccolò; Cesca, Tiziana; Mattei, Giovanni

    2018-03-15

    In this work we present the study of the ultra-fast dynamics of the nonlinear optical response of a honeycomb array of silver triangular nanoprisms, performed using a femtosecond pulsed laser tuned with the dipolar surface plasmon resonance of the nanoarray. Nonlinear absorption and refraction, and their time-dependence, were explored using the z-scan and time-resolved excite-probe techniques. Nonlinear absorption is shown to change sign with the input irradiance and the behavior was explained on the basis of a three-level model. The response time was determined to be in the picosecond regime. A technique based on a variable frequency chopper was also used in order to discriminate the thermal and electronic contributions to the nonlinearity, which were found to have opposite signs. All these findings propel the investigated nanoprism arrays as good candidates for applications in advanced ultra-fast nonlinear nanophotonic devices.

  16. Taylor's series method for solving the nonlinear point kinetics equations

    International Nuclear Information System (INIS)

    Nahla, Abdallah A.

    2011-01-01

    Highlights: → Taylor's series method for nonlinear point kinetics equations is applied. → The general order of derivatives are derived for this system. → Stability of Taylor's series method is studied. → Taylor's series method is A-stable for negative reactivity. → Taylor's series method is an accurate computational technique. - Abstract: Taylor's series method for solving the point reactor kinetics equations with multi-group of delayed neutrons in the presence of Newtonian temperature feedback reactivity is applied and programmed by FORTRAN. This system is the couples of the stiff nonlinear ordinary differential equations. This numerical method is based on the different order derivatives of the neutron density, the precursor concentrations of i-group of delayed neutrons and the reactivity. The r th order of derivatives are derived. The stability of Taylor's series method is discussed. Three sets of applications: step, ramp and temperature feedback reactivities are computed. Taylor's series method is an accurate computational technique and stable for negative step, negative ramp and temperature feedback reactivities. This method is useful than the traditional methods for solving the nonlinear point kinetics equations.

  17. Digital nonlinearity compensation in high-capacity optical communication systems considering signal spectral broadening effect.

    Science.gov (United States)

    Xu, Tianhua; Karanov, Boris; Shevchenko, Nikita A; Lavery, Domaniç; Liga, Gabriele; Killey, Robert I; Bayvel, Polina

    2017-10-11

    Nyquist-spaced transmission and digital signal processing have proved effective in maximising the spectral efficiency and reach of optical communication systems. In these systems, Kerr nonlinearity determines the performance limits, and leads to spectral broadening of the signals propagating in the fibre. Although digital nonlinearity compensation was validated to be promising for mitigating Kerr nonlinearities, the impact of spectral broadening on nonlinearity compensation has never been quantified. In this paper, the performance of multi-channel digital back-propagation (MC-DBP) for compensating fibre nonlinearities in Nyquist-spaced optical communication systems is investigated, when the effect of signal spectral broadening is considered. It is found that accounting for the spectral broadening effect is crucial for achieving the best performance of DBP in both single-channel and multi-channel communication systems, independent of modulation formats used. For multi-channel systems, the degradation of DBP performance due to neglecting the spectral broadening effect in the compensation is more significant for outer channels. Our work also quantified the minimum bandwidths of optical receivers and signal processing devices to ensure the optimal compensation of deterministic nonlinear distortions.

  18. Variable-coefficient higher-order nonlinear Schroedinger model in optical fibers: Variable-coefficient bilinear form, Baecklund transformation, brightons and symbolic computation

    International Nuclear Information System (INIS)

    Tian Bo; Gao Yitian; Zhu Hongwu

    2007-01-01

    Symbolically investigated in this Letter is a variable-coefficient higher-order nonlinear Schroedinger (vcHNLS) model for ultrafast signal-routing, fiber laser systems and optical communication systems with distributed dispersion and nonlinearity management. Of physical and optical interests, with bilinear method extend, the vcHNLS model is transformed into a variable-coefficient bilinear form, and then an auto-Baecklund transformation is constructed. Constraints on coefficient functions are analyzed. Potentially observable with future optical-fiber experiments, variable-coefficient brightons are illustrated. Relevant properties and features are discussed as well. Baecklund transformation and other results of this Letter will be of certain value to the studies on inhomogeneous fiber media, core of dispersion-managed brightons, fiber amplifiers, laser systems and optical communication links with distributed dispersion and nonlinearity management

  19. Linear Algebraic Method for Non-Linear Map Analysis

    International Nuclear Information System (INIS)

    Yu, L.; Nash, B.

    2009-01-01

    We present a newly developed method to analyze some non-linear dynamics problems such as the Henon map using a matrix analysis method from linear algebra. Choosing the Henon map as an example, we analyze the spectral structure, the tune-amplitude dependence, the variation of tune and amplitude during the particle motion, etc., using the method of Jordan decomposition which is widely used in conventional linear algebra.

  20. Synthesis, characterization and non-linear optical response of organophilic carbon dots

    KAUST Repository

    Bourlinos, Athanasios B.; Karakassides, Michael A.; Kouloumpis, Antonios; Gournis, Dimitrios; Bakandritsos, Aristides; Papagiannouli, Irene; Aloukos, Panagiotis; Couris, Stelios; Hola, Katerina; Zboril, Radek; Krysmann, Marta; Giannelis, Emmanuel P.

    2013-01-01

    For the first time ever we report the nonlinear optical (NLO) properties of carbon dots (C-dots). The C-dots for these experiments were synthesized by mild pyrolysis of lauryl gallate. The resulting C-dots bear lauryl chains and, hence, are highly dispersible in polar organic solvents, like chloroform. Dispersions in CHCl3 show significant NLO response. Specifically, the C-dots show negative nonlinear absorption coefficient and negative nonlinear refraction. Using suspensions with different concentrations these parameters are quantified and compared to those of fullerene a well-known carbon molecule with proven NLO response. © 2013 Elsevier Ltd. All rights reserved.

  1. Synthesis, characterization and non-linear optical response of organophilic carbon dots

    KAUST Repository

    Bourlinos, Athanasios B.

    2013-09-01

    For the first time ever we report the nonlinear optical (NLO) properties of carbon dots (C-dots). The C-dots for these experiments were synthesized by mild pyrolysis of lauryl gallate. The resulting C-dots bear lauryl chains and, hence, are highly dispersible in polar organic solvents, like chloroform. Dispersions in CHCl3 show significant NLO response. Specifically, the C-dots show negative nonlinear absorption coefficient and negative nonlinear refraction. Using suspensions with different concentrations these parameters are quantified and compared to those of fullerene a well-known carbon molecule with proven NLO response. © 2013 Elsevier Ltd. All rights reserved.

  2. Nonlinear optical properties of an electromagnetically induced transparency medium interacting with two quantized fields

    CERN Document Server

    Kuang-Leman; Wu Yong Shi

    2003-01-01

    We study linear and nonlinear optical properties of an electromagnetically induced transparency (EIT) medium interacting with two quantized laser fields in the adiabatic EIT case. We show that the EIT medium exhibits normal dispersion. Kerr and higher-order nonlinear refractive index coefficients are also calculated in a completely analytical form. It is indicated that the EIT medium exhibits giant resonantly enhanced nonlinearities. We discuss the response of the EIT medium to nonclassical light fields and find that the polarization vanishes when the probe laser is initially in a nonclassical state of no single-photon coherence.

  3. Defect solitons in saturable nonlinearity media with parity-time symmetric optical lattices

    Energy Technology Data Exchange (ETDEWEB)

    Hu, Sumei [Department of Physics, Guangdong University of Petrochemical Technology, Maoming 525000 (China); Laboratory of Nanophotonic Functional Materials and Devices, South China Normal University, Guangzhou 510631 (China); Hu, Wei, E-mail: huwei@scnu.edu.cn [Laboratory of Nanophotonic Functional Materials and Devices, South China Normal University, Guangzhou 510631 (China)

    2013-11-15

    We reported the existence and stability of defect solitons in saturable nonlinearity media with parity-time (PT) symmetric optical lattices. Families of fundamental and dipole solitons are found in the semi-infinite gap and the first gap. The power of solitons increases with the increasing of the propagation constant and saturation parameter. The existence areas of fundamental and dipole solitons shrink with the growth of saturation parameter. The instability of dipole solitons for positive and no defect induced by the imaginary part of PT symmetric potentials can be suppressed by the saturation nonlinearity, but for negative defect it cannot be suppressed by the saturation nonlinearity.

  4. Nonlinear tunneling of optical soliton in 3 coupled NLS equation with symbolic computation

    Energy Technology Data Exchange (ETDEWEB)

    Mani Rajan, M.S., E-mail: senthilmanirajanofc@gmail.com [Department of Physics, Anna University, Madurai Region, Ramanathapuram (India); Mahalingam, A. [Department of Physics, Anna University, Chennai - 600 025 (India); Uthayakumar, A. [Department of Physics, Presidency College, Chennai - 600 005 (India)

    2014-07-15

    We investigated the soliton solution for N coupled nonlinear Schrödinger (CNLS) equations. These equations are coupled due to the cross-phase-modulation (CPM). Lax pair of this system is obtained via the Ablowitz–Kaup–Newell–Segur (AKNS) scheme and the corresponding Darboux transformation is constructed to derive the soliton solution. One and two soliton solutions are generated. Using two soliton solutions of 3 CNLS equation, nonlinear tunneling of soliton for both with and without exponential background has been discussed. Finally cascade compression of optical soliton through multi-nonlinear barrier has been discussed. The obtained results may have promising applications in all-optical devices based on optical solitons, study of soliton propagation in birefringence fiber systems and optical soliton with distributed dispersion and nonlinearity management. -- Highlights: •We consider the nonlinear tunneling of soliton in birefringence fiber. •3-coupled NLS (CNLS) equation with variable coefficients is considered. •Two soliton solutions are obtained via Darboux transformation using constructed Lax pair. •Soliton tunneling through dispersion barrier and well are investigated. •Finally, cascade compression of soliton has been achieved.

  5. The impact of LED transfer function nonlinearity on high-speed optical wireless communications based on discrete-multitone modulation

    NARCIS (Netherlands)

    Inan, B.; Lee, S.C.J.; Randel, S.; Neokosmidis, L.; Koonen, A.M.J.; Walewski, J.

    2009-01-01

    The nonlinear dependence of the optical power from white LEDs on the applied driving current and its impact on discrete-multitone modulation was investigated by use of numerical simulations for the case of optical wireless communications.

  6. Projection-iteration methods for solving nonlinear operator equations

    International Nuclear Information System (INIS)

    Nguyen Minh Chuong; Tran thi Lan Anh; Tran Quoc Binh

    1989-09-01

    In this paper, the authors investigate a nonlinear operator equation in uniformly convex Banach spaces as in metric spaces by using stationary and nonstationary generalized projection-iteration methods. Convergence theorems in the strong and weak sense were established. (author). 7 refs

  7. An approximation method for nonlinear integral equations of Hammerstein type

    International Nuclear Information System (INIS)

    Chidume, C.E.; Moore, C.

    1989-05-01

    The solution of a nonlinear integral equation of Hammerstein type in Hilbert spaces is approximated by means of a fixed point iteration method. Explicit error estimates are given and, in some cases, convergence is shown to be at least as fast as a geometric progression. (author). 25 refs

  8. Application of the trial equation method for solving some nonlinear ...

    Indian Academy of Sciences (India)

    Therefore, our aim is just to find the function F. Liu has obtained a number of exact solutions to many nonlinear differential equations when F(u) is a polynomial or a rational function. ... In this study, we apply the trial equation method to seek exact solutions of the ... twice and setting the integration constant to zero, we have.

  9. Nonlinear realizations, the orbit method and Kohn's theorem

    OpenAIRE

    Andrzejewski, K.; Gonera, J.; Kosinski, P.

    2012-01-01

    The orbit method is used to describe the centre of mass motion of the system of particles with fixed charge to mass ratio moving in homogeneous magnetic field and confined by harmonic potential. The nonlinear action of symmetry group on phase space is identified and compared with the one obtained with the help of Eisenhart lift.

  10. Convergence of spectral methods for nonlinear conservation laws. Final report

    International Nuclear Information System (INIS)

    Tadmor, E.

    1987-08-01

    The convergence of the Fourier method for scalar nonlinear conservation laws which exhibit spontaneous shock discontinuities is discussed. Numerical tests indicate that the convergence may (and in fact in some cases must) fail, with or without post-processing of the numerical solution. Instead, a new kind of spectrally accurate vanishing viscosity is introduced to augment the Fourier approximation of such nonlinear conservation laws. Using compensated compactness arguments, it is shown that this spectral viscosity prevents oscillations, and convergence to the unique entropy solution follows

  11. Method for Measuring Small Nonlinearities of Electric Characteristics

    DEFF Research Database (Denmark)

    Guldbrandsen, Tom; Meyer, Niels I; Schjær-Jacobsen, Jørgen

    1965-01-01

    A method is described for measuring very small deviations from linearity in electric characteristics. The measurement is based on the harmonics generated by the nonlinear element when subjected to a sine wave signal. A special bridge circuit is used to balance out the undesired harmonics...... of the signal generator together with the first harmonic frequency. The set-up measures the small-signal value and the first and second derivative with respect to voltage. The detailed circuits are given for measuring nonlinearities in Ohmic and capacitive components. In the Ohmic case, a sensitivity...

  12. Growth and characterization of benzaldehyde 4-nitro phenyl hydrazone (BPH) single crystal: A proficient second order nonlinear optical material

    Science.gov (United States)

    Saravanan, M.; Abraham Rajasekar, S.

    2016-04-01

    The crystals (benzaldehyde 4-nitro phenyl hydrazone (BPH)) appropriate for NLO appliance were grown by the slow cooling method. The solubility and metastable zone width measurement of BPH specimen was studied. The material crystallizes in the monoclinic crystal system with noncentrosymmetric space group of Cc. The optical precision in the whole visible region was found to be excellent for non-linear optical claim. Excellence of the grown crystal is ascertained by the HRXRD and etching studies. Laser Damage Threshold and Photoluminescence studies designate that the grown crystal contains less imperfection. The mechanical behaviour of BPH sample at different temperatures was investigated to determine the hardness stability of the grown specimen. The piezoelectric temperament and the relative Second Harmonic Generation (for diverse particle sizes) of the material were also studied. The dielectric studies were executed at varied temperatures and frequencies to investigate the electrical properties. Photoconductivity measurement enumerates consummate of inducing dipoles due to strong incident radiation and also divulge the nonlinear behaviour of the material. The third order nonlinear optical properties of BPH crystals were deliberate by Z-scan method.

  13. Structural, vibrational and theoretical studies of anilinium trichloroacetate: New hydrogen bonded molecular crystal with nonlinear optical properties

    Science.gov (United States)

    Tanak, H.; Pawlus, K.; Marchewka, M. K.; Pietraszko, A.

    2014-01-01

    In this work, we report a combined experimental and theoretical study on molecular structure, vibrational spectra and NBO analysis of the potential nonlinear optical (NLO) material anilinium trichloroacetate. The FT-IR and FT-Raman spectra of the compound have been recorded together between 4000-80 cm-1 and 3600-80 cm-1 regions, respectively. The compound crystallizes in the noncentrosymmetric space group of monoclinic system. The optimized molecular structure, vibrational wavenumbers, IR intensities and Raman activities have been calculated by using density functional method (B3LYP) with 6-311++G(d,p) as higher basis set. The obtained vibrational wavenumbers and optimized geometric parameters were seen to be in good agreement with the experimental data. DSC measurements on powder samples do not indicate clearly on the occurrence of phase transitions in the temperature 113-293 K. The Kurtz and Perry powder reflection technique appeared to be very effective in studies of second-order nonlinear optical properties of the molecule. The non-linear optical properties are also addressed theoretically. The predicted NLO properties of the title compound are much greater than ones of urea. In addition, DFT calculations of the title compound, molecular electrostatic potential, frontier orbitals and thermodynamic properties were also performed at 6-311++G(d,p) level of theory. For title crystal the SHG efficiency was estimated by Kurtz-Perry method to be deff = 0.70 deff (KDP).

  14. Optical tsunamis: shoaling of shallow water rogue waves in nonlinear fibers with normal dispersion

    International Nuclear Information System (INIS)

    Wabnitz, Stefan

    2013-01-01

    In analogy with ocean waves running up towards the beach, shoaling of pre-chirped optical pulses may occur in the normal group-velocity dispersion regime of optical fibers. We present exact Riemann wave solutions of the optical shallow water equations and show that they agree remarkably well with the numerical solutions of the nonlinear Schrödinger equation, at least up to the point where a vertical pulse front develops. We also reveal that extreme wave events or optical tsunamis may be generated in dispersion tapered fibers in the presence of higher-order dispersion. (paper)

  15. Comprehensive experimental analysis of nonlinear dynamics in an optically-injected semiconductor laser

    Directory of Open Access Journals (Sweden)

    Kevin Schires

    2011-09-01

    Full Text Available We present the first comprehensive experimental study, to our knowledge, of the routes between nonlinear dynamics induced in a semiconductor laser under external optical injection based on an analysis of time-averaged measurements of the optical and RF spectra and phasors of real-time series of the laser output. The different means of analysis are compared for several types of routes and the benefits of each are discussed in terms of the identification and mapping of the nonlinear dynamics. Finally, the results are presented in a novel audio/video format that describes the evolution of the dynamics with the injection parameters.

  16. Web Platform for Sharing Modeling Software in the Field of Nonlinear Optics

    Science.gov (United States)

    Dubenskaya, Julia; Kryukov, Alexander; Demichev, Andrey

    2018-02-01

    We describe the prototype of a Web platform intended for sharing software programs for computer modeling in the rapidly developing field of the nonlinear optics phenomena. The suggested platform is built on the top of the HUBZero open-source middleware. In addition to the basic HUBZero installation we added to our platform the capability to run Docker containers via an external application server and to send calculation programs to those containers for execution. The presented web platform provides a wide range of features and might be of benefit to nonlinear optics researchers.

  17. Web Platform for Sharing Modeling Software in the Field of Nonlinear Optics

    Directory of Open Access Journals (Sweden)

    Dubenskaya Julia

    2018-01-01

    Full Text Available We describe the prototype of a Web platform intended for sharing software programs for computer modeling in the rapidly developing field of the nonlinear optics phenomena. The suggested platform is built on the top of the HUBZero open-source middleware. In addition to the basic HUBZero installation we added to our platform the capability to run Docker containers via an external application server and to send calculation programs to those containers for execution. The presented web platform provides a wide range of features and might be of benefit to nonlinear optics researchers.

  18. Universal continuous-variable quantum computation: Requirement of optical nonlinearity for photon counting

    International Nuclear Information System (INIS)

    Bartlett, Stephen D.; Sanders, Barry C.

    2002-01-01

    Although universal continuous-variable quantum computation cannot be achieved via linear optics (including squeezing), homodyne detection, and feed-forward, inclusion of ideal photon-counting measurements overcomes this obstacle. These measurements are sometimes described by arrays of beam splitters to distribute the photons across several modes. We show that such a scheme cannot be used to implement ideal photon counting and that such measurements necessarily involve nonlinear evolution. However, this requirement of nonlinearity can be moved ''off-line,'' thereby permitting universal continuous-variable quantum computation with linear optics

  19. Nonlinear optics and solid-state lasers advanced concepts, tuning-fundamentals and applications

    CERN Document Server

    Yao, Jianquan

    2012-01-01

    This book covers the complete spectrum of nonlinear optics and all solid state lasers.The book integrates theory, calculations and practical design, technology, experimental schemes and applications. With the expansion and further development of Laser technology, the wavelength spectrum of Lasers had to be enlarged, even to be tunable which requires the use of nonlinear optical and Laser tunable technology. It systematically summarizes and integrates the analysis of international achievements within the last 20 years in this field. It will be helpful for university teachers, graduate students as well as engineers.

  20. Quantum electronics and Moscow State University's Khokhlov-Akhmanov school of coherent and nonlinear optics

    International Nuclear Information System (INIS)

    Makarov, V.A.

    2004-01-01

    The aim of the report is to describe the history of the Moscow University Coherent and Nonlinear Optics School headed by R.V. Khokhlov and S.A. Akhmanov being a part of the history of the Russian efforts to investigate into quantum electronics. The reports describes briefly the most significant results of the mentioned School activity, in particular, thermonuclear reactions initiated by laser pulses in plasma; the procedure to accelerate electrons up to 1 GeV using the present-day lasers; the nonlinear-optical analogues of the Faraday and the Kerr effects [ru