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Sample records for fission shape isomers

  1. Ternary fission of spontaneously fissile uranium isomers excited by neutrons

    International Nuclear Information System (INIS)

    Makarenko, V.E.; Molchanov, Y.D.; Otroshchenko, G.A.; Yan'kov, G.B.

    1989-01-01

    Spontaneously fissile isomers (SFI) of uranium were excited in the reactions 236,238 U(n,n') at an average neutron energy 4.5 MeV. A pulsed electrostatic accelerator and time analysis of the fission events were used. Fission fragments were detected by the scintillation method, and long-range particles from fission were detected by an ionization method. The relative probability of fission of nuclei through a spontaneously fissile isomeric state was measured: (1.30±0.01)·10 -4 ( 236 U) and (1.48±0.02)·10 -4 ( 238 U). Half-lives of the isomers were determined: 121±2 nsec (the SFI 236 U) and 267±13 nsec (the SFI 238 U). In study of the ternary fission of spontaneously fissile isotopes of uranium it was established that the probability of the process amounts to one ternary fission per 163±44 binary fissions of the SFI 236 U and one ternary fission per 49±14 binary fissions of the SFI 238 U. The substantial increase of the probability of ternary fission of SFI of uranium in comparison with the case of ternary fission of nuclei which are not in an isomeric state may be related to a special nucleon configuration of the fissile isomers of uranium

  2. Nuclear structure via isomer tagging of fission fragments

    Science.gov (United States)

    Wu, C. Y.; Cline, D.; Simon, M. W.; Stoyer, M. A.

    1997-10-01

    The high efficiency for detecting high-fold γ rays by large Ge arrays makes it possible to study the detailed spectroscopy of many neutron-rich nuclei produced by fission. Major progress has been made using sealed spontaneous fission sources. Considerable improvement in selectivity is provided, with an open source, both by gating on isomers and by detection of both fission fragments in coincidence with the deexcitation γ rays (see the preceding contribution). The reconstructed kinematics allows a measure of fragment mass and the Doppler shift correction of γ rays. In a recent experiment, fission fragments were detected using half of the CHICO array and an annular PPAC in coincidence with deexcitation γ rays detected by the Rochester array of eight Compton-suppressed Ge detectors. The annular PPAC was located only 1.0" from a 3.7 μCi ^252Cf source for efficient isomer tagging. The correlation was studied between delayed, within a time window between 150 ns and 10 μs after a fission occurring, and prompt γ rays. Several prominent feeding patterns to isomers in the mass region around 100 and 130 are identified by such correlation study. Experimental details and results will be presented.

  3. Analysis of shape isomer yields of Pu in the framework of dynamical ...

    Indian Academy of Sciences (India)

    February 2012 physics pp. 231–236. Analysis of shape isomer yields of ... the depth of the second potential well should be less than the results of statistical model calculations. Keywords. Fission; fission barrier ... (2) population of the second potential well and cooling via particle or γ emission (this event is interpreted as the ...

  4. Table of superdeformed nuclear bands and fission isomers

    Energy Technology Data Exchange (ETDEWEB)

    Firestone, R.B. [Lawrence Berkeley Lab., CA (United States); Singh, B. [McMaster Univ., Hamilton, ON (Canada)

    1994-06-01

    A minimum in the second potential well of deformed nuclei was predicted and the associated shell gaps are illustrated in the harmonic oscillator potential shell energy surface calculations shown in this report. A strong superdeformed minimum in {sup 152}Dy was predicted for {beta}{sub 2}-0.65. Subsequently, a discrete set of {gamma}-ray transitions in {sup 152}DY was observed and, assigned to the predicted superdeformed band. Extensive research at several laboratories has since focused on searching for other mass regions of large deformation. A new generation of {gamma}-ray detector arrays is already producing a wealth of information about the mechanisms for feeding and deexciting superdeformed bands. These bands have been found in three distinct regions near A=l30, 150, and 190. This research extends upon previous work in the actinide region near A=240 where fission isomers were identified and also associated with the second potential well. Quadrupole moment measurements for selected cases in each mass region are consistent with assigning the bands to excitations in the second local minimum. As part of our committment to maintain nuclear structure data as current as possible in the Evaluated Nuclear Structure Reference File (ENSDF) and the Table of Isotopes, we have updated the information on superdeformed nuclear bands. As of April 1994, we have complied data from 86 superdeformed bands and 46 fission isomers identified in 73 nuclides for this report. For each nuclide there is a complete level table listing both normal and superdeformed band assignments; level energy, spin, parity, half-life, magneto moments, decay branchings; and the energies, final levels, relative intensities, multipolarities, and mixing ratios for transitions deexciting each level. Mass excess, decay energies, and proton and neutron separation energies are also provided from the evaluation of Audi and Wapstra.

  5. Table of superdeformed nuclear bands and fission isomers

    International Nuclear Information System (INIS)

    Firestone, R.B.; Singh, B.

    1994-06-01

    A minimum in the second potential well of deformed nuclei was predicted and the associated shell gaps are illustrated in the harmonic oscillator potential shell energy surface calculations shown in this report. A strong superdeformed minimum in 152 Dy was predicted for β 2 -0.65. Subsequently, a discrete set of γ-ray transitions in 152 DY was observed and, assigned to the predicted superdeformed band. Extensive research at several laboratories has since focused on searching for other mass regions of large deformation. A new generation of γ-ray detector arrays is already producing a wealth of information about the mechanisms for feeding and deexciting superdeformed bands. These bands have been found in three distinct regions near A=l30, 150, and 190. This research extends upon previous work in the actinide region near A=240 where fission isomers were identified and also associated with the second potential well. Quadrupole moment measurements for selected cases in each mass region are consistent with assigning the bands to excitations in the second local minimum. As part of our committment to maintain nuclear structure data as current as possible in the Evaluated Nuclear Structure Reference File (ENSDF) and the Table of Isotopes, we have updated the information on superdeformed nuclear bands. As of April 1994, we have complied data from 86 superdeformed bands and 46 fission isomers identified in 73 nuclides for this report. For each nuclide there is a complete level table listing both normal and superdeformed band assignments; level energy, spin, parity, half-life, magneto moments, decay branchings; and the energies, final levels, relative intensities, multipolarities, and mixing ratios for transitions deexciting each level. Mass excess, decay energies, and proton and neutron separation energies are also provided from the evaluation of Audi and Wapstra

  6. Fission processes through compact and creviced shapes

    International Nuclear Information System (INIS)

    Royer, G.; Remaud, B.

    1984-01-01

    Using a one-parameter family of compact and creviced shapes the deformation energy of the liquid-drop model including the nuclear proximity energy has been calculated. The introduction of the proximity forces on such a shape sequence leads to the identification of fission and scission barriers since the rupture of the neck between the fragments is assumed before the barrier is crossed. The fission barrier heights are well reproduced and are much lower than those given by the liquid-drop model (without proximity) for the medium systems. It is shown that these low barriers are compatible with a strong enhancement of the critical angular momentum for cold fission. The translational kinetic energy of the fragments agrees with experimental data. Double-humped barriers are predicted for actinides; the inner barrier has essentially a microscopic origin while the outer one (which plays the role of a scission barrier) is governed mostly by the balance between Coulomb and nuclear forces. (author)

  7. Brownian shape motion: Fission fragment mass distributions

    Directory of Open Access Journals (Sweden)

    Sierk Arnold J.

    2012-02-01

    Full Text Available It was recently shown that remarkably accurate fission-fragment mass distributions can be obtained by treating the nuclear shape evolution as a Brownian walk on previously calculated five-dimensional potential-energy surfaces; the current status of this novel method is described here.

  8. Statistical model calculation of fission isomer excitation functions in (n,n') and (n,γ) reactions

    International Nuclear Information System (INIS)

    Chatterjee, A.; Athougies, A.L.; Mehta, M.K.

    1977-01-01

    A statistical model developed by Britt and others (1971, 1973) to analyze isomer excitation functions in spallation type reactions like (α,2n) has been adopted in fission isomer calculations for (n,n') and (n,γ) reactions. Calculations done for 235 U(n,n')sup(238m)U and 235 U(n,γ)sup(236m)U reactions have been compared with experimental measurements. A listing of the computer program ISOMER using FORTRAN IV to calculate the isomer to prompt ratios is given. (M.G.B.)

  9. Shape isomer excitation by mu-minus capture

    International Nuclear Information System (INIS)

    Kaplan, S.N.; Monard, J.A.; Nagamiya, S.

    1975-06-01

    In a search for back-decay gamma rays from the shape isomer in 238 U following mu-minus capture, no candidates have been found with yields greater than 2 percent of the muon stoppings. The intensities of the gamma rays are insufficient to permit definitive lifetime measurements of individual peaks; however, for 500-keV energy ranges of gamma ray pulses, lifetimes have been determined that give results consistent with recent electron lifetime measurements. (6 figures, 2 tables) (U.S.)

  10. Application of pulse shape discrimination in Si detector for fission ...

    Indian Academy of Sciences (India)

    Pulse shape discrimination (PSD) with totally depleted transmission type Si surface barrier detector in reverse mount has been investigated to identify fission fragments in the presence of elastic background in heavy ion-induced fission reactions by both numerical simulation and experimental studies. The PSD method is ...

  11. Shape-coexistence and shape-evolution studies for bismuth isotopes by insource laser spectroscopy and $\\beta$-delayed fission in $^{188}$Bi

    CERN Multimedia

    The proposal aims at the two main goals: \\\\ \\\\1) the studies of shape-coexistence and shape-evolution phenomena in the long chain of bismuth isotopes (Z=83) by in-source laser spectroscopy measurements of isotopic shifts (IS) and hyperfine structures (hfs), and \\\\ 2) $\\beta$-delayed fission ($\\beta$DF) of two isomeric states in $^{188}$Bi. \\\\ \\\\Isomer-selective $\\beta$DF studies for $^{188m1, 188m2}$Bi isomers will enable us for the first time to investigate the spin-dependence of the $\\beta$DF process and to check theoretical predictions of asymmetrical fission fragment mass-distribution in this region of nuclei. The measurements will be performed with the well-proven Windmill and MR-TOF MS/Penning Trap techniques.

  12. Low-lying level structure of the neutron-rich nucleus {sup 109}Nb: A possible oblate-shape isomer

    Energy Technology Data Exchange (ETDEWEB)

    Watanabe, H., E-mail: hiroshi@ribf.riken.j [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Sumikama, T. [Department of Physics, Faculty of Science and Technology, Tokyo University of Science, 2641 Yamazaki, Noda, Chiba (Japan); Nishimura, S. [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Yoshinaga, K. [Department of Physics, Faculty of Science and Technology, Tokyo University of Science, 2641 Yamazaki, Noda, Chiba (Japan); Li, Z. [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Miyashita, Y. [Department of Physics, Faculty of Science and Technology, Tokyo University of Science, 2641 Yamazaki, Noda, Chiba (Japan); Yamaguchi, K. [Department of Physics, Osaka University, Machikaneyama-machi 1-1, Osaka 560-0043 Toyonaka (Japan); Baba, H. [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Berryman, J.S. [Nuclear Science Division, Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Blasi, N. [INFN, Sezione di Milano, via Celoria 16, I-20133 Milano (Italy); Bracco, A.; Camera, F. [INFN, Sezione di Milano, via Celoria 16, I-20133 Milano (Italy); Dipartimento di Fisica, Universita di Milano, via Celoria 16, I-20133 Milano (Italy); Chiba, J. [Department of Physics, Faculty of Science and Technology, Tokyo University of Science, 2641 Yamazaki, Noda, Chiba (Japan); Doornenbal, P. [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Go, S.; Hashimoto, T.; Hayakawa, S. [Center for Nuclear Study, University of Tokyo, Hirosawa 2-1, Wako, Saitama 351-0198 (Japan); Hinke, C. [Physik Department, Technische Universitaet Muenchen, D-85748 Garching (Germany); Ideguchi, E. [Center for Nuclear Study, University of Tokyo, Hirosawa 2-1, Wako, Saitama 351-0198 (Japan); Isobe, T. [RIKEN Nishina Center, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan)

    2011-01-31

    The neutron-rich nuclei {sup 109}Nb and {sup 109}Zr have been populated using in-flight fission of a {sup 238}U beam at 345 MeV/nucleon at the RIBF facility. A T{sub 1/2}=150(30) ns isomer at 313 keV has been identified in {sup 109}Nb for the first time. The low-lying levels in {sup 109}Nb have been also populated following the {beta}-decay of {sup 109}Zr. Based on the difference in feeding pattern between the isomeric and {beta} decays, the decay scheme from the isomeric state in {sup 109}Nb was established. The observed hindrances of the electromagnetic transitions deexciting the isomeric state are discussed in terms of possible shape coexistence. Potential energy surface calculations for single-proton configurations predict the presence of low-lying oblate-deformed states in {sup 109}Nb.

  13. Conversion-electron experiment to characterize the decay of the 237Np shape isomer

    International Nuclear Information System (INIS)

    Henry, E.A.; Becker, J.A.; Bauer, R.W.; Gardner, D.G.; Decman, D.J.; Meyer, R.A.; Roy, N.; Sale, K.E.

    1987-01-01

    Conversion electrons from the decay of low-lying levels of 237 Np have been measured to detect the population of these levels by gamma-ray decay of the 237 Np shape isomer. Analysis of the 208-keV transition L conversion-electron peak gives an upper limit of about 17 μb for the population of the 3/2 - 267-keV level in 237 Np from the shape isomer decay. Model calculations are compared with the measured limit. Improvements are suggested for this experiment. 9 refs., 4 figs

  14. High-spin isomer in 211Rn, and the shape of the yrast line

    International Nuclear Information System (INIS)

    Dracoulis, G.D.; Fahlander, C.; Poletti, A.R.

    1981-08-01

    High spin yrast states in 211 Rn have been identified. A 61/2 - , 380 ns isomer found at 8856 keV is characterised as a core-excited configuration. The average shape of the yrast line shows a smooth behaviour with spin, in contrast to its neighbour 212 Rn. This difference is attributed to the presence of the neutron hole

  15. Analysis of shape isomer yields of 237 Pu in the framework of ...

    Indian Academy of Sciences (India)

    Data on shape isomer yield for + 235U reaction at E lab = 20–29 MeV are analysed in the framework of a combined dynamical–statistical model. From this analysis, information on the double humped fission barrier parameters for some Pu isotopes has been obtained and it is shown that the depth of the second potential ...

  16. Single-molecule imaging reveals topological isomer-dependent diffusion by 4-armed star and dicyclic 8-shaped polymers

    KAUST Repository

    Habuchi, Satoshi

    2015-04-21

    Diffusion dynamics of topological isomers of polymer molecules was investigated at the single-molecule level in a melt state by employing the fluorophore-incorporated 4-armed star and the corresponding doubly-cyclized, 8-shaped poly(THF) chains. While the single-molecule fluorescence imaging experiment revealed that the diffusion of the 4-armed star polymer was described by a single Gaussian distribution, the diffusion of the 8-shaped polymer exhibited a double Gaussian distribution behaviour. We reasoned that the two 8-shaped polymeric isomers have distinct diffusion modes in the melt state, although ensemble-averaged experimental methods cannot detect differences in overall conformational state of the isomers. The single-molecule experiments suggested that one of the 8-shaped polymeric isomer, having the horizontally oriented form, causes an efficient threading with the linear matrix chains which leads to the slower diffusion compared with the corresponding 4-armed star polymer, while the other 8-shaped polymeric isomer, having the vertically oriented form, displayed faster diffusion by the suppression of effective threading with the linear matrix chains due to its contracted chain conformation.

  17. Pulse-shape discrimination in radioanalytical methods. Part I. Delayed fission neutron counting

    International Nuclear Information System (INIS)

    Posta, S.; Vacik, J.; Hnatowicz, V.; Cervena, J.

    1999-01-01

    In this study the principle of pulse shape discrimination (PSD) has been employed in delayed fission neutron counting (DNC) method. Effective elimination of unwanted gamma background signals in measured radiation spectra has been proved. (author)

  18. Predation risk shapes social networks in fission-fusion populations.

    Directory of Open Access Journals (Sweden)

    Jennifer L Kelley

    Full Text Available Predation risk is often associated with group formation in prey, but recent advances in methods for analysing the social structure of animal societies make it possible to quantify the effects of risk on the complex dynamics of spatial and temporal organisation. In this paper we use social network analysis to investigate the impact of variation in predation risk on the social structure of guppy shoals and the frequency and duration of shoal splitting (fission and merging (fusion events. Our analyses revealed that variation in the level of predation risk was associated with divergent social dynamics, with fish in high-risk populations displaying a greater number of associations with overall greater strength and connectedness than those from low-risk sites. Temporal patterns of organisation also differed according to predation risk, with fission events more likely to occur over two short time periods (5 minutes and 20 minutes in low-predation fish and over longer time scales (>1.5 hours in high-predation fish. Our findings suggest that predation risk influences the fine-scale social structure of prey populations and that the temporal aspects of organisation play a key role in defining social systems.

  19. Low energy nuclear fission

    International Nuclear Information System (INIS)

    Nifenecker, H.

    1982-02-01

    In these lectures we present the liquid drop model of fission and compare some of its prediction with experiment. The liquid drop analogy allows to define in a rather simple and intuitive way a number of useful concepts and possible observables. We then discuss, using the example of the oscillator model, the generality of shell effects. We show how a synthesis of the liquid drop model and of the shell model can be made using the Strutinsky shell averaging procedure. Some experimental data related to the existence of shape isomers are presented and discussed. We conclude by discussing some aspects, both experimental and theoretical, of fission dynamics

  20. Low energy nuclear fission

    International Nuclear Information System (INIS)

    Nifenecker, H.

    1980-08-01

    In these lectures the liquid drop model of fission is presented and some of its predictions compared with experiment. The liquid drop analogy allows to define in a rather simple and intuitive way a number of useful concepts and possible observables. It is shown how a synthesis of the liquid drop model and of the shell model can be made using the Strutinsky shell averaging procedure. Some experimental data related to the existence of shape isomers are presented and discussed. We conclude by discussing some aspects, both experimental and theoretical, of fission dynamics

  1. $\\beta$-delayed fission, laser spectroscopy and shape-coexistence studies with radioactive At beams

    CERN Multimedia

    We propose to study the $\\beta$-delayed fission, laser spectroscopy and radioactive decay of the newly available pure beams of neutron-deficient and neutron-rich astatine (Z=85) isotopes. The fission probability and the fission fragment distribution of the even-even isotopes $^{194,196}$Po following the $\\beta$-decay of the isotopes $^{194,196}$At will be studied with the Windmill setup. In-source laser spectroscopy will be performed on the entire astatine isotopic chain, using a combination of the Windmill setup, ISOLTRAP MR-ToF and ISOLDE Faraday. Radioactive decay data will be acquired at the Windmill setup throughout those studies and contribute to the global understanding of the phenomenon of shape coexistence in the neutron-deficient lead region.

  2. Nuclear structure and shapes from prompt gamma ray spectroscopy of fission products

    International Nuclear Information System (INIS)

    Ahmad, I.; Morss, L.R.; Durell, J.L.

    1996-01-01

    Many nuclear shape phenomena are predicted to occur in neutron-rich nuclei. The best source for the production of these nuclides is the spontaneous fission which produces practically hundreds of nuclides with yields of greater than 0.1 % per decay. Measurements of coincident gamma rays with large Ge arrays have recently been made to obtain information on nuclear structures and shapes of these neutron- rich nuclei. Among the important results that have been obtained from such measurements are octupole correlations in Ba isotopes, triaxial shapes in Ru nuclei, two-phonon vibrations in 106 Mo and level lifetimes and quadrupole moments in Nd isotopes and A=100 nuclei. These data have been used to test theoretical models

  3. Isomer shift and magnetic moment of the long-lived 1/2$^{+}$ isomer in $^{79}_{30}$Zn$_{49}$: signature of shape coexistence near $^{78}$Ni

    CERN Document Server

    Yang, X.F.; Xie, L.; Babcock, C.; Billowes, J.; Bissell, M.L.; Blaum, K.; Cheal, B.; Flanagan, K.T.; Garcia Ruiz, R. F.; Gins, W.; Gorges, C.; Grob, L.K.; Heylen, H.; Kaufmann, S.; Kowalska, M.; Kraemer, J.; Malbrunot-Ettenauer, S.; Neugart, R.; Neyens, G.; Nörtershäuser, W.; Papuga, J.; Sánchez, R.; Yordanov, D.T.

    2016-01-01

    Collinear laser spectroscopy has been performed on the $^{79}_{30}$Zn$_{49}$ isotope at ISOLDE-CERN. The existence of a long-lived isomer with a few hundred milliseconds half-life was confirmed, and the nuclear spins and moments of the ground and isomeric states in $^{79}$Zn as well as the isomer shift were measured. From the observed hyperfine structures, spins $I = 9/2$ and $I = 1/2$ are firmly assigned to the ground and isomeric states. The magnetic moment $\\mu$ ($^{79}$Zn) = $-$1.1866(10) $\\mu_{\\rm{N}}$, confirms the spin-parity $9/2^{+}$ with a $\

  4. Model of fission yeast cell shape driven by membrane-bound growth factors and the cytoskeleton.

    Directory of Open Access Journals (Sweden)

    Tyler Drake

    Full Text Available Fission yeast serves as a model for how cellular polarization machinery consisting of signaling molecules and the actin and microtubule cytoskeleton regulates cell shape. In this work, we develop mathematical models to investigate how these cells maintain a tubular shape of approximately constant diameter. Many studies identify active Cdc42, found in a cap at the inner membrane of growing cell tips, as an important regulator of local cell wall remodeling, likely through control of exocyst tethering and the targeting of other polarity-enhancing structures. First, we show that a computational model with Cdc42-dependent local cell wall remodeling under turgor pressure predicts a relationship between spatial extent of growth signal and cell diameter that is in agreement with prior experiments. Second, we model the consequences of feedback between cell shape and distribution of Cdc42 growth signal at cell tips. We show that stability of cell diameter over successive cell divisions places restrictions on their mutual dependence. We argue that simple models where the spatial extent of the tip growth signal relies solely on geometrical alignment of confined microtubules might lead to unstable width regulation. Third, we study a computational model that combines a growth signal distributed over a characteristic length scale (as, for example, by a reaction-diffusion mechanism with an axis-sensing microtubules system that places landmarks at positions where microtubule tips touch the cortex. A two-dimensional implementation of this model leads to stable cell diameter for a wide range of parameters. Changes to the parameters of this model reproduce straight, bent, and bulged cell shapes, and we discuss how this model is consistent with other observed cell shapes in mutants. Our work provides an initial quantitative framework for understanding the regulation of cell shape in fission yeast, and a scaffold for understanding this process on a more molecular

  5. Development of high sensitivity 4H-SiC detectors for fission neutron pulse shape measurements

    Science.gov (United States)

    Wu, Jian; Jiang, Yong; Li, Meng; Zeng, Lina; Li, Junjie; Gao, Hui; Zou, Dehui; Bai, Zhongxiong; Ye, Cenming; Liang, Wenfeng; Dai, Shaofeng; Lu, Yi; Rong, Ru; Du, Jinfeng; Fan, Xiaoqiang

    2017-08-01

    4H-silicon carbide (4H-SiC) detectors are well suited for measurements of fission neutron pulse shape for their compact size, excellent radiation resistance, and hydrogen free composition. The aim of this study is to improve the 4H-SiC detector's sensitivity to fission neutron pulses. 4H-SiC detectors with varied epilayer thicknesses are fabricated and then tested in the pulsed neutron field of the Chinese Fast Burst Reactor II (CFBR II). The sensitivity of the 4H-SiC detector to the CFBR II neutron pulse is increased by 139.8%, with the enlargement of epilayer thickness from 20 μm to 120 μm. By employing the proton-recoil method, the sensitivity of the 4H-SiC detector to the CFBR II neutron pulse is further increased by 11.6%. With enhanced sensitivity to fission neutron pulses, 4H-SiC detectors are promising devices for high intensity neutron pulse measurements.

  6. Nuclear Structure Studies of Microsecond Isomers Near A=100

    Science.gov (United States)

    Simpson, G.; Genevey, J.; Pinston, J. A.; Urban, W.; Zlomaniec, A.; Orlandi, R.; Scherillo, A.; Tsekhanovich, I.; Smith, A. G.; Thallon, A.; Varley, B. J.; Jolie, J.; Warr, N.

    2007-04-01

    A large variety of shapes may be observed in Sr and Zr nuclei of the A = 100 region when the number of neutrons increases from N = 58 to N = 64. The lighter isotopes are rather spherical. It is also well established that three shapes co-exist in the transitional odd-A, N = 59, Sr and Zr nuclei. For N > 59, strongly deformed axially symmetric bands are observed. Recently, a new isomer of half-life 1.4(2) mu s was observed in 95Kr, the odd-odd 96Rb has been reinvestigated and a new high-spin isomer observed in the even-even 98Zr. These nuclei were studied by means of prompt gamma -ray spectroscopy of the spontaneous fission of 248Cm using the EUROGAM 2 Ge array and/or measurements of mu s isomers produced by fission of 239,241Pu with thermal neutrons at the ILL (Grenoble). To allow spectroscopic studies of isomeric states with lifetimes around 100 ns, across a broad range of medium-heavy neutron-rich nuclei, an experiment was performed at a neutron guide of the ILL using thermal-neutron-induced fission. Fission fragments were identified using a small spectrometer consisting of a section to measure time-of-flight and an ionization chamber. Isomeric gamma rays emitted from complementary fragments were detected in an array of Ge detectors.

  7. Projected shell model description for nuclear isomers

    Energy Technology Data Exchange (ETDEWEB)

    Sun, Y. [Department of Physics, Shanghai Jiao Tong University, Shanghai 200240, Popular Republic (China)

    2008-12-15

    The study of nuclear isomer properties is a current research focus. To describe isomers, we present a method based on the Projected Shell Model. Two kinds of isomers, {kappa}-isomers and shape isomers, are discussed. For the {kappa}-isomer treatment, {kappa}-mixing is properly implemented in the model. It is found however that in order to describe the strong {kappa}-violation more efficiently, it may be necessary to further introduce triaxiality into the shell model basis. To treat shape isomers, a scheme is outlined which allows mixing those configurations belonging to different shapes. (Author)

  8. A new high-spin isomer in 195Bi

    International Nuclear Information System (INIS)

    Roy, T.; Mukherjee, G.; Rana, T.K.; Bhattacharya, Soumik; Asgar, Md.A.; Bhattacharya, C.; Bhattacharya, S.; Bhattacharyya, S.; Pai, H.; Madhavan, N.; Bala, I.; Gehlot, J.; Gurjar, R.K.; Jhingan, A.; Kumar, R.; Muralithar, S.; Nath, S.; Singh, R.P.; Varughese, T.; Basu, K.; Bhattacharjee, S.S.; Ghugre, S.S.; Raut, R.; Sinha, A.K.; Palit, R.

    2015-01-01

    A new high-spin isomer has been identified in 195 Bi at the focal plane of the HYbrid Recoil mass Analyser (HYRA) used in the gas-filled mode. The fusion evaporation reactions 169 Tm ( 30 Si, x n) 193, 195 Bi were used with the beam energies on targets of 168 and 146MeV for 6n and 4n channels, respectively. The evaporation residues, separated from the fission fragments, and their decays were detected at the focal plane of HYRA using MWPC, Si-Pad and clover HPGe detectors. The half-life of the new isomer in 195 Bi has been measured to be 1.6(1) μs. The configuration of the new isomer has been proposed and compared with the other isomers in this region. The Total Routhian Surface (TRS) calculations for the three-quasiparticle configurations corresponding to the new isomer suggest an oblate deformation for this isomeric state. The same calculations for different configurations in 195 Bi and for the even-even 194 Pb core indicate that the proton i 13/2 orbital has a large shape driving effect towards oblate shape in these nuclei. (orig.)

  9. A new high-spin isomer in {sup 195}Bi

    Energy Technology Data Exchange (ETDEWEB)

    Roy, T.; Mukherjee, G.; Rana, T.K.; Bhattacharya, Soumik; Asgar, Md.A.; Bhattacharya, C.; Bhattacharya, S.; Bhattacharyya, S.; Pai, H. [Variable Energy Cyclotron Centre, Kolkata (India); Madhavan, N.; Bala, I.; Gehlot, J.; Gurjar, R.K.; Jhingan, A.; Kumar, R.; Muralithar, S.; Nath, S.; Singh, R.P.; Varughese, T. [Inter University Acclerator Centre, New Delhi (India); Basu, K.; Bhattacharjee, S.S.; Ghugre, S.S.; Raut, R.; Sinha, A.K. [UGC-DAE-CSR Kolkata Centre, Kolkata (India); Palit, R. [Tata Institute of Fundamental Research, Department of Nuclear and Atomic Physics, Mumbai (India)

    2015-11-15

    A new high-spin isomer has been identified in {sup 195}Bi at the focal plane of the HYbrid Recoil mass Analyser (HYRA) used in the gas-filled mode. The fusion evaporation reactions {sup 169}Tm ({sup 30}Si, x n) {sup 193,} {sup 195}Bi were used with the beam energies on targets of 168 and 146MeV for 6n and 4n channels, respectively. The evaporation residues, separated from the fission fragments, and their decays were detected at the focal plane of HYRA using MWPC, Si-Pad and clover HPGe detectors. The half-life of the new isomer in {sup 195}Bi has been measured to be 1.6(1) μs. The configuration of the new isomer has been proposed and compared with the other isomers in this region. The Total Routhian Surface (TRS) calculations for the three-quasiparticle configurations corresponding to the new isomer suggest an oblate deformation for this isomeric state. The same calculations for different configurations in {sup 195}Bi and for the even-even {sup 194}Pb core indicate that the proton i{sub 13/2} orbital has a large shape driving effect towards oblate shape in these nuclei. (orig.)

  10. Experimental grounds for nuclear shape isomerism

    International Nuclear Information System (INIS)

    Makarenko, V.E.

    1995-11-01

    Experimental data on fission isomeric states of actinide nuclei - half lives, energies, quantum numbers, decay branches and spectroscopic properties - are discussed. Quite a few results find their explanation in the framework of nuclear shape isomerism hypothesis being the in-thing for about thirty years. Others seem to be the hints to the quasiparticle nature of fission isomers. The problem could be solved by direct measurement of nuclear spin for isomeric states. (author). 44 refs, 1 tab

  11. Study of scission shapes in spontaneous ternary fission of 252Cf

    International Nuclear Information System (INIS)

    Singer, P.; Schwalm, D.; Thirolf, P.; Goennenwein, F.; Hesse, M.

    1995-06-01

    A new kinematic study on the ternary fission of 252 Cf has been conducted by registering prompt neutrons and fission γ rays coincidence with light charged particles (LCP) and fission fragments. The aim is to investigate changes in fragment deformation energy between the binary and ternary fission modes from measured prompt neutron angular distributions and multiplicities, and to explore the influence of light particle emission on the energy distribution, multiplicity and angular anisotropy of γ rays emitted during fragment de-excitation. The experiment was performed at the MPI Heidelberg using the Darmstadt-Heidelberg crystal ball spectrometer as γ-ray and neutron detector. Fragments were identified by a double-E measurement with an angular sensitive twin ionization chamber (IC). Light charged particles from fission were measured by ΔE-E telescopes composed of ΔE ICs and silicon PIN diodes. The telescopes enable to identify various LCPs which are emitted much more rarely than ternary α particles. The parameters of the experiment and the method of data analysis are described and first results presented. (orig.)

  12. A Network of Multiple Regulatory Layers Shapes Gene Expression in Fission Yeast

    OpenAIRE

    Lackner, Daniel H.; Beilharz, Traude H.; Marguerat, Samuel; Mata, Juan; Watt, Stephen; Schubert, Falk; Preiss, Thomas; B?hler, J?rg

    2007-01-01

    Summary Gene expression is controlled at multiple layers, and cells may integrate different regulatory steps for coherent production of proper protein levels. We applied various microarray-based approaches to determine key gene-expression intermediates in exponentially growing fission yeast, providing genome-wide data for translational profiles, mRNA steady-state levels, polyadenylation profiles, start-codon sequence context, mRNA half-lives, and RNA polymerase II occupancy. We uncovered wide...

  13. Search for the gamma-branch of the shape isomers of separated U isotopes using muon for nuclide excitation

    International Nuclear Information System (INIS)

    Mireshghi, A.

    1982-12-01

    We have searched for back-decay gamma rays from the shape isomeric states in 235 U, 236 U, and 238 U possibly excited in muon radiationless transition. The energies and intensities of gamma rays following muon atomic capture were measured as a function of time after muon stopping. Background was suppressed by requiring that the candidate gamma ray be followed by another gamma ray (μ-capture gamma ray). The prompt gamma-ray spectra included the U-muonic x rays. The measured 235 U and 238 U x-ray energies were in good agreement with previously reported results. The x-ray spectrum from 236 U has not been previously reported. The 236 U spectrum is very similar to that of 238 U, except that the K x-rays exhibit an isotope shift of approximately 20 keV, the 236 U energies being higher. In the analysis of the delayed spectra of 236 U and 238 U using the GAMANL peak searching program, and with an effective lower-limit detection efficiency of .15% per stopping muon, no candidate gamma rays for the back decay transitions from the shape isomeric state were observed

  14. Part I: $\\beta$-delayed fission, laser spectroscopy and shape-coexistence studies with astatine beams; Part II: Delineating the island of deformation in the light gold isotopes by means of laser spectroscopy

    CERN Document Server

    Andreyev, Andrei

    2013-01-01

    Part I: $\\beta$-delayed fission, laser spectroscopy and shape-coexistence studies with astatine beams; Part II: Delineating the island of deformation in the light gold isotopes by means of laser spectroscopy

  15. Theory of nuclear fission: a review

    International Nuclear Information System (INIS)

    Mosel, U.

    1976-01-01

    General properties of nuclear fission are reviewed and related to our present knowledge of fission theory. For this purpose the basic reasons for the shape of the fission barriers are discussed and their consequences compared with experimental results on barrier shapes and structures. Special emphasis is put on the asymmetry of the fission barriers and mass-distributions and its relation to the shells of the nascent fragment shells. Finally the problem of calculating fission cross sections is discussed

  16. Intermediate energy nuclear fission

    International Nuclear Information System (INIS)

    Hylten, G.

    1982-01-01

    Nuclear fission has been investigated with the double-kinetic-energy method using silicon surface barrier detectors. Fragment energy correlation measurements have been made for U, Th and Bi with bremsstrahlung of 600 MeV maximum energy. Distributions of kinetic energy as a function of fragment mass are presented. The results are compared with earlier photofission data and in the case of bismuth, with calculations based on the liquid drop model. The binary fission process in U, Yb, Tb, Ce, La, Sb, Ag and Y induced by 600 MeV protons has been investigated yielding fission cross sections, fragment kinetic energies, angular correlations and mass distributions. Fission-spallation competition calculations are used to deduce values of macroscopic fission barrier heights and nuclear level density parameter values at deformations corresponding to the saddle point shapes. We find macroscopic fission barriers lower than those predicted by macroscopic theories. No indication is found of the Businaro Gallone limit expected to occur somewhere in the mass range A = 100 to A = 140. For Ce and La asymmetric mass distributions similar to those in the actinide region are found. A method is described for the analysis of angular correlations between complementary fission products. The description is mainly concerned with fission induced by medium-energy protons but is applicable also to other projectiles and energies. It is shown that the momentum and excitation energy distributions of cascade residuals leading to fission can be extracted. (Author)

  17. Detection of Actinides via Nuclear Isomer De-Excitation

    Energy Technology Data Exchange (ETDEWEB)

    Francy, Christopher J. [Oregon State Univ., Corvallis, OR (United States)

    2009-07-01

    This dissertation discusses a data collection experiment within the Actinide Isomer Identification project (AID). The AID project is the investigation of an active interrogation technique that utilizes nuclear isomer production, with the goal of assisting in the interdiction of illicit nuclear materials. In an attempt to find and characterize isomers belonging to 235U and its fission fragments, a 232Th target was bombarded with a monoenergetic 6Li ion beam, operating at 45 MeV.

  18. Determination of the quadrupole moment of the fission-isomeric state in 238U by a modified charge-plunger method

    International Nuclear Information System (INIS)

    Pedersen, J.; Goerlach, U.; Habs, D.; Just, M.; Metag, V.; Mosler, E.; Schukraft, J.; Singer, P.; Specht, H.J.; Ulfert, G.

    1978-01-01

    A modified version of the charge plunger method has been developed which, by utilizing electrostatic fields, renders possible the separation of low- and high-charge recoil ions over short flight distances. With this technique the quadrupole moment of the 200 ns fission isomer in 238 U has been determined to be (29 +- 3) b. The corresponding deformation of c/a = (1.8 +- 0.1) provides another quantitative proof for shape isomerism in the actinide region. (orig.) [de

  19. Shapes and dynamics from the time-dependent mean field

    International Nuclear Information System (INIS)

    Stevenson, P.D.; Goddard, P.M.; Rios, A.

    2015-01-01

    Explaining observed properties in terms of underlying shape degrees of freedom is a well-established prism with which to understand atomic nuclei. Self-consistent mean-field models provide one tool to understand nuclear shapes, and their link to other nuclear properties and observables. We present examples of how the time-dependent extension of the mean-field approach can be used in particular to shed light on nuclear shape properties, particularly looking at the giant resonances built on deformed nuclear ground states, and at dynamics in highly-deformed fission isomers. Example calculations are shown of 28 Si in the first case, and 240 Pu in the latter case

  20. Fission fragment angular momentum

    International Nuclear Information System (INIS)

    Frenne, D. De

    1991-01-01

    Most of the energy released in fission is converted into translational kinetic energy of the fragments. The remaining excitation energy will be distributed among neutrons and gammas. An important parameter characterizing the scission configuration is the primary angular momentum of the nascent fragments. Neutron emission is not expected to decrease the spin of the fragments by more than one unit of angular momentum and is as such of less importance in the determination of the initial fragment spins. Gamma emission is a suitable tool in studying initial fragment spins because the emission time, number, energy, and multipolarity of the gammas strongly depend on the value of the primary angular momentum. The main conclusions of experiments on gamma emission were that the initial angular momentum of the fragments is large compared to the ground state spin and oriented perpendicular to the fission axis. Most of the recent information concerning initial fragment spin distributions comes from the measurement of isomeric ratios for isomeric pairs produced in fission. Although in nearly every mass chain isomers are known, only a small number are suitable for initial fission fragment spin studies. Yield and half-life considerations strongly limit the number of candidates. This has the advantage that the behavior of a specific isomeric pair can be investigated for a number of fissioning systems at different excitation energies of the fragments and fissioning nuclei. Because most of the recent information on primary angular momenta comes from measurements of isomeric ratios, the global deexcitation process of the fragments and the calculation of the initial fragment spin distribution from measured isomeric ratios are discussed here. The most important results on primary angular momentum determinations are reviewed and some theoretical approaches are given. 45 refs., 7 figs., 2 tabs

  1. Benzene and its Isomers

    Indian Academy of Sciences (India)

    Benzene and its Isomers atomic weights and availability of improved analytical methods. At this time the .... geometry. Forcing them in cyclic structures would lead to signifi- cant strain. Bicyclic structures do not easily accommodate double bonds at bridgehead positions (Bredt's rule). Many of the polycy- clic isomers clearly ...

  2. Short-lived isomers in 94Rb

    International Nuclear Information System (INIS)

    Tsekhanovich, I.; Dare, J. A.; Smith, A. G.; Varley, B. J.; Simpson, G. S.; Urban, W.; Soldner, T.; Jolie, J.; Linnemann, A.; Orlandi, R.; Smith, J. F.; Scherillo, A.; Rzaca-Urban, T.; Zlomaniec, A.; Dorvaux, O.; Gall, B. J. P.; Roux, B.

    2008-01-01

    The medium-spin structure of the neutron-rich, odd-odd nucleus 94 Rb was studied by means of γ-ray spectroscopy. Excited levels were populated in the neutron-induced fission of 235 U and in the spontaneous fission of 252 Cf and 248 Cm. Two isomeric states were found at 1485.2 and 2074.8 keV with half-lives of 18 and 107 ns, respectively. The probable structures of the two isomers involve the fully aligned, proton-neutron configurations [π(g 9/2 ) x ν(g 7/2 )] 8 + and [π(g 9/2 ) x ν(h 11/2 )] 10 - , respectively. These new data give information on the single-particle energies in the region

  3. Ternary fission

    International Nuclear Information System (INIS)

    Wagemans, C.

    1991-01-01

    Since its discovery in 1946, light (charged) particle accompanied fission (ternary fission) has been extensively studied, for spontaneous as well as for induced fission reactions. The reason for this interest was twofold: the ternary particles being emitted in space and time close to the scission point were expected to supply information on the scission point configuration and the ternary fission process was an important source of helium, tritium, and hydrogen production in nuclear reactors, for which data were requested by the nuclear industry. Significant experimental progress has been realized with the advent of high-resolution detectors, powerful multiparameter data acquisition systems, and intense neutron and photon beams. As far as theory is concerned, the trajectory calculations (in which scission point parameters are deduced from the experimental observations) have been very much improved. An attempt was made to explain ternary particle emission in terms of a Plateau-Rayleigh hydrodynamical instability of a relatively long cylindrical neck or cylindrical nucleus. New results have also been obtained on the so-called open-quotes trueclose quotes ternary fission (fission in three about-equal fragments). The spontaneous emission of charged particles has also clearly been demonstrated in recent years. This chapter discusses the main characteristics of ternary fission, theoretical models, light particle emission probabilities, the dependence of the emission probabilities on experimental variables, light particle energy distributions, light particle angular distributions, correlations between light particle accompanied fission observables, open-quotes trueclose quotes ternary fission, and spontaneous emission of heavy ions. 143 refs., 18 figs., 8 tabs

  4. Determination of shell energies. Nuclear deformations and fission barriers

    International Nuclear Information System (INIS)

    Koura, Hiroyuki; Tachibana, Takahiro; Uno, Masahiro; Yamada, Masami.

    1996-01-01

    We have been studying a method of determining nuclear shell energies and incorporating them into a mass formula. The main feature of this method lies in estimating shell energies of deformed nuclei from spherical shell energies. We adopt three assumptions, from which the shell energy of a deformed nucleus is deduced to be a weighted sum of spherical shell energies of its neighboring nuclei. This shell energy should be called intrinsic shell energy since the average deformation energy also acts as an effective shell energy. The ground-state shell energy of a deformed nucleus and its equilibrium shape can be obtained by minimizing the sum of these two energies with respect to variation of deformation parameters. In addition, we investigate the existence of fission isomers for heavy nuclei with use of the obtained shell energies. (author)

  5. Seniority isomers in nuclei

    International Nuclear Information System (INIS)

    Van Isacker, P

    2011-01-01

    Seniority isomers are nuclear states with an electromagnetic decay that is hindered by selection rules related to the seniority quantum number. A simple analysis is presented of their possible formation with reference to the nickel isotopes 70–76 Ni and the N = 50 isotones from molybdenum to cadmium. It is shown that the existence of seniority isomers in a j = 9/2 shell is predominantly governed by the quadrupole pairing matrix element of the nucleon-nucleon interaction. The analysis is generalized to shells with larger j.

  6. Benzene and its Isomers

    Indian Academy of Sciences (India)

    Home; Journals; Resonance – Journal of Science Education; Volume 6; Issue 5. Benzene and its Isomers - How many Structures can we Draw for C6H6? Gopalpur Nagendrappa. General Article Volume 6 Issue 5 May 2001 pp 74-78. Fulltext. Click here to view fulltext PDF. Permanent link:

  7. Fifty years of nuclear fission: Nuclear data and measurements series

    International Nuclear Information System (INIS)

    Lynn, J.E.

    1989-06-01

    This report is the written version of a colloquium first presented at Argonne National Laboratory in January 1989. The paper begins with an historical preamble about the events leading to the discovery of nuclear fission. This leads naturally to an account of early results and understanding of the fission phenomena. Some of the key concepts in the development of fission theory are then discussed. The main theme of this discussion is the topography of the fission barrier, in which the interplay of the liquid-drop model and nucleon shell effects lead to a wide range of fascinating phenomena encompassing metastable isomers, intermediate-structure effects in fission cross-sections, and large changes in fission product properties. It is shown how study of these changing effects and theoretical calculations of the potential energy of the deformed nucleus have led to broad qualitative understanding of the nature of the fission process. 54 refs., 35 figs

  8. FY2011 Annual Report for the Actinide Isomer Detection Project

    International Nuclear Information System (INIS)

    Warren, Glen A.; Francy, Christopher J.; Ressler, Jennifer J.; Erikson, Luke E.; Tatishvili, Gocha; Hatarik, R.

    2011-01-01

    This project seeks to identify a new signature for actinide element detection in active interrogation. This technique works by exciting and identifying long-lived nuclear excited states (isomers) in the actinide isotopes and/or primary fission products. Observation of isomers in the fission products will provide a signature for fissile material. For the actinide isomers, the decay time and energy of the isomeric state is unique to a particular isotope, providing an unambiguous signature for SNM. This project entails isomer identification and characterization and neutron population studies. This document summarizes activities from its third year - completion of the isomer identification characterization experiments and initialization of the neutron population experiments. The population and decay of the isomeric state in 235U remain elusive, although a number of candidate gamma rays have been identified. In the course of the experiments, a number of fission fragment isomers were populated and measured (Ressler 2010). The decays from these isomers may also provide a suitable signature for the presence of fissile material. Several measurements were conducted throughout this project. This report focuses on the results of an experiment conducted collaboratively by PNNL, LLNL and LBNL in December 2010 at LBNL. The measurement involved measuring the gamma-rays emitted from an HEU target when bombarded with 11 MeV neutrons. This report discussed the analysis and resulting conclusions from those measurements. There was one strong candidate, at 1204 keV, of an isomeric signature of 235U. The half-life of the state is estimated to be 9.3 μs. The measured time dependence fits the decay time structure very well. Other possible explanations for the 1204-keV state were investigated, but they could not explain the gamma ray. Unfortunately, the relatively limited statistics of the measurement limit, and the lack of understanding of some of the systematic of the experiment, limit

  9. Singlet Fission

    Czech Academy of Sciences Publication Activity Database

    Smith, M. B.; Michl, Josef

    2010-01-01

    Roč. 110, č. 11 (2010), s. 6891-6936 ISSN 0009-2665 Grant - others:Department of Energy(US) DE- FG36 -08GO18017 Institutional research plan: CEZ:AV0Z40550506 Keywords : solar energy conversion * photovoltaics * singlet fission Subject RIV: CF - Physical ; Theoretical Chemistry Impact factor: 33.033, year: 2010

  10. Ternary fission

    Indian Academy of Sciences (India)

    2015-08-05

    Aug 5, 2015 ... We present the ternary fission of 252Cf and 236U within a three-cluster model as well as in a level density approach. The competition between collinear and equatorial geometry is studied by calculating the ternary fragmentation potential as a function of the angle between the lines joining the stationary ...

  11. Ternary fission

    Indian Academy of Sciences (India)

    the energy minimization of all possible ternary breakups of a heavy radioactive nucleus. Further, within the TCM we have analysed the competition between different geometries as well as different positioning of the fragments. Also, an attempt was made to calculate the mass distribution of ternary fission process within the ...

  12. Spectroscopy of fission fragments using prompt-delayed ...

    Indian Academy of Sciences (India)

    2015-08-02

    Aug 2, 2015 ... The physics focus of INGA is to investigate the emergent properties of nuclear many- body system under varying rotational stress.These experimental ..... prompt spectrum are due to de-excitations from another fission fragment (a contaminant) having an isomer of similar half-life. To confirm the prompt γ-rays ...

  13. Investigation of exotic fission modes

    International Nuclear Information System (INIS)

    Poenaru, D. N.; Gherghescu, R. A.; Greiner, W.; Nagame, Y.; Hamilton, J. H.; Ramayya, A. V.

    2002-01-01

    Fission approach to the cluster radioactivities and α-decay has been systematically developed during the last two decades. A more complex process, the ternary fission, was observed since 1946 both in neutron-induced and spontaneous fission. We obtained interesting results concerning the binary fission saddle-point reflection asymmetric nuclear shapes, and we can explain how a possible nuclear quasimolecular state is formed during the 10 Be accompanied cold fission of 252 Cf. The equilibrium nuclear shapes in fission theory are usually determined by minimizing the deformation energy for a given surface equation. We developed a method allowing to obtain a very general saddle-point shape as a solution of a differential equation without an a priori introduction of a shape parametrization. In the approach based on a liquid drop model (LDM), saddle-point shapes are always reflection symmetric: the deformation energy increases with the mass-asymmetry parameter η = (A 1 - A 2 )/(A 1 + A 2 ). By adding the shell corrections to the LDM deformation energy, we obtained minima at a finite mass asymmetry for parent nuclei 238 U, 232,228 Th in agreement with experiments. This correction was calculated phenomenologically. A technique based on the fragment identification by using triple γ coincidences in the large arrays of Ge-detectors, like GAMMASPHERE, was employed at Vanderbilt University to discover new characteristics of the fission process, and new decay modes. The possibility of a whole family of new decay modes, the multicluster accompanied fission, was envisaged. Besides the fission into two or three fragments, a heavy or superheavy nucleus spontaneously breaks into four, five or six nuclei of which two are asymmetric or symmetric heavy fragments and the others are light clusters, e.g. α-particles, 10 Be, 14 C, or combinations of them. Examples were presented for the two-, three- and four cluster accompanied cold fission of 252 Cf and 262 Rf, in which the emitted

  14. Optimization of C20 isomers structure

    International Nuclear Information System (INIS)

    Ndjaka, J.M.B.; Charlier, J.C.

    2001-07-01

    We have performed geometry optimization of various possible planar and three-dimensional C 20 geometries. The planar structures considered include a linear chain, a monoclinic ring, and a bicyclic bow tie; while the three-dimensional geometric; consisted of a bowl or corranulene structure and a fullerene cage. In agreement with Wang et al MP2's calculations, our results predict the corranulene bowl to be the lowest energy structure. From the ground state geometry to the highest energy, considered C 20 structures, listed in increasing energy, are bowl, cage, bow tie, ring and chain. For the ring and bow tie isomers, the shape of the optimized structure deviates from that of the initial configuration; while the shape of the optimised bowl, cage and chain remain unchanged. (author)

  15. Energy released in fission

    International Nuclear Information System (INIS)

    James, M.F.

    1969-05-01

    The effective energy released in and following the fission of U-235, Pu-239 and Pu-241 by thermal neutrons, and of U-238 by fission spectrum neutrons, is discussed. The recommended values are: U-235 ... 192.9 ± 0.5 MeV/fission; U-238 ... 193.9 ± 0.8 MeV/fission; Pu-239 ... 198.5 ± 0.8 MeV/fission; Pu-241 ... 200.3 ± 0.8 MeV/fission. These values include all contributions except from antineutrinos and very long-lived fission products. The detailed contributions are discussed, and inconsistencies in the experimental data are pointed out. In Appendix A, the contribution to the total useful energy release in a reactor from reactions other than fission are discussed briefly, and in Appendix B there is a discussion of the variations in effective energy from fission with incident neutron energy. (author)

  16. Fission products collecting devices

    International Nuclear Information System (INIS)

    Matsumoto, Hiroshi

    1979-01-01

    Purpose: To enable fission products trap with no contamination to coolants and cover gas by the provision of a fission products trap above the upper part of a nuclear power plant. Constitution: Upon fuel failures in a reactor core, nuclear fission products leak into coolants and move along the flow of the coolants to the coolants above the reactor core. The fission products are collected in a trap container and guided along a pipeline into fission products detector. The fission products detector monitors the concentration of the fission products and opens the downstream valve of the detector when a predetermined concentration of the fission products is detected to introduce the fission products into a waste gas processing device and release them through the exhaust pipe. (Seki, T.)

  17. New isomers and medium-spin structure of the 95Y nucleus

    International Nuclear Information System (INIS)

    Urban, W.; Sieja, K.; Simpson, G. S.; Faust, H.; Rzaca-Urban, T.; Zlomaniec, A.; Lukasiewicz, M.; Smith, A. G.; Durell, J. L.; Smith, J. F.; Varley, B. J.; Nowacki, F.; Ahmad, I.

    2009-01-01

    Excited states in 95 Y, populated following the spontaneous fission of 248 Cm and 252 Cf and following fission of 235 U induced by thermal neutrons, were studied by means of γ spectroscopy using the EUROGAM2 and GAMMASPHERE multidetector Ge arrays and the LOHENGRIN fission-fragment separator, respectively. We have found a new (17/2 - ) isomer in 95 Y at 3142.2 keV with a half-life of T 1/2 =14.9(5) ns. Another isomer was identified in 95 Y at 5022.1 keV and it was assigned a spin-parity (27/2 - ). For this isomer a half-life of T 1/2 =65(4) ns was determined and four decay branches were found, including an E3 decay. A new E3 decay branch was also found for the known, 1087.5-keV isomer in 95 Y, for which we measured a half-life of 51.2(9) μs. The B(E3) and B(E1) transition rates, of 2.0 and 3.8x10 -7 W.u., respectively, observed in 95 Y are significantly lower than in the neighboring 96 Zr core, suggesting that octupole correlations in this region are mainly due to the coupling of proton Δj=3 orbitals. Shell-model calculations indicate that the (27/2 - ) isomer in 95 Y corresponds to the πg 9/2 ν(g 7/2 h 11/2 ) maximally aligned configuration and that all three isomers in 95 Y decay, primarily, by M2 transitions between proton g 9/2 and f 5/2 orbitals.

  18. Fission Research at IRMM

    Directory of Open Access Journals (Sweden)

    Al-Adili A.

    2010-03-01

    Full Text Available Fission Research at JRC-IRMM has a longstanding tradition. The present paper is discussing recent investigations of fission fragment properties of 238 U(n,f, 234 U(n,f, prompt neutron emission in fission of 252 Cf(SF as well as the prompt fission neutron spectrum of 235 U(n,f and is presenting the most important results.

  19. Can voltammetry distinguish glycan isomers?

    Czech Academy of Sciences Publication Activity Database

    Trefulka, Mojmír; Paleček, Emil

    2015-01-01

    Roč. 69, č. 1 (2015), s. 241-244 ISSN 0366-6352 R&D Projects: GA ČR(CZ) GAP301/11/2055 Institutional support: RVO:68081707 Keywords : oligosaccharide isomers * Os(VI) complexes * chemical modification Subject RIV: BO - Biophysics Impact factor: 1.326, year: 2015

  20. Spectroscopy of neutron-rich nuclei produced in the spontaneous fission of californium-252

    Science.gov (United States)

    Simon, Michael Wilhelm

    1999-10-01

    A new experimental technique has been developed for the spectroscopic investigation of the neutron-rich products of 252Cf(SF). The charged-particle detector CHICO was coupled to the Ge-detector array GAMMASPHERE and a thin fission source was used allowing the collection of high-statistics, high-fold γ-ray data in kinematic coincidence with the recoiling fission partners. The selectivity provided by this technique allows the γ-rays to be assigned unambiguously to the heavy or light fission partner. The added sensitivity allows many rotational bands to be extended to ~20 ħ, and a sensitivity to nuclei produced with a yield of 5 × 10-5 /fission was achieved by mass-gating the γ-ray spectra. The charged-particle detector CHICO was developed for this experiment and for studies utilizing other binary reactions, such as Coulomb excitation, transfer and fusion-fission reactions. The detector covers a total solid angle of 2.8 sr and has a time resolution of 500 ps, resulting in a mass resolution of Δm/m = 5% for beam experiments, or 8 mass units for spontaneous fission. This technique was used to set limits, in agreement with shell model predictions, on the E3 decay of the / - level in 135I. Rotational bands in 102,104,106,108Mo, 112Ru, 152,154,156 Nd, 156,158,160Sm were extended to higher spin. Band crossings were observed in the ground and γ-band in 104Mo. The γ-band of 112Ru shows continued tri-axial behavior at higher spin. The yrast rotational bands in 112,113,114,115,116 Pd were extended and rotational bands built on the low-lying isomeric levels in 113,115Pd were newly identified. The behavior of the observed band crossings in the ground and isomer bands of 113,115 Pd, when compared to the neighboring 111,113 Rh and cranked shell model calculations indicate that the predicted change from prolate to oblate shapes in the neutron-rich Pd does not occur before 116Pd. In a separate experiment, the lifetimes in 165Ho of the K=/ - ground band, up to spin / - ħ, and

  1. Fission dynamics in the proton induced fission of heavy nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Rubchenya, V.A. E-mail: rubchen@phys.jyu.fi; Trzaska, W.H.; Itkis, I.M.; Itkis, M.G.; Kliman, J.; Kniajeva, G.N.; Kondratiev, N.A.; Kozulin, E.M.; Krupa, L.; Pokrovski, I.V.; Voskressenski, V.M.; Hanappe, F.; Materna, T.; Dorvaux, O.; Stuttge, L.; Chubarian, G.; Khlebnikov, S.V.; Vakhtin, D.N.; Lyapin, V.G

    2004-04-05

    Multi-parameter correlation study of the reaction {sup 242}Pu(p, f) at E{sub p} 13, 20 and 55 MeV has been carried out. Fission fragment mass and kinetic energy distributions and the double differential neutron spectra have been measured. It was observed that the two-humped shape of mass distributions prevailed up to highest proton energy. Manifestation of the nuclear shell Z 28 near fragment mass A{sub fr} = 70 has been detected. The experimental results were analyzed in the framework of a time-dependent statistical model with inclusion of nuclear friction effects in the fission process. The multi-parameter correlation study of the reaction.

  2. Nuclear fission: What have we learned in 50 years?

    International Nuclear Information System (INIS)

    Vandenbosch, R.

    1989-01-01

    Nuclear fission has captured the imagination of chemists and physicists for half a century now. There are several reasons for this. One of course is that it represents the most drastic rearrangement of nuclear matter known, challenged only recently by collisions induced by very heavy ions. Another is that both statistical and dynamical features come into play. Perhaps one of the most compelling reasons is its never-ending capacity to surprise us: asymmetric mass distributions, the sawtooth dependence of neutron yields in fragment mass, spontaneously fissioning isomers and intermediate structure resonances. Finally, and perhaps most importantly, fission is a rich laboratory within which one can explore the delicate interplay between the macroscopic aspects of bulk nuclear matter and the quantal effects of a finite number of Fermions. It will of course be impossible for me to cover all aspects of fission. I have chosen a limited number of topics to cover, with particular topics being chosen either because the have been associated with persistent puzzles in fission or because they have, or hopefully will, tell us something special about how nuclei behave. After a brief historical note, I organize these topics sequentially according to the various stages of the fission process, starting first with the probability for fission to occur and ending with scission phenomena. 56 refs., 11 figs

  3. Treatment of isomers in nucleosynthesis codes

    Science.gov (United States)

    Reifarth, René; Fiebiger, Stefan; Göbel, Kathrin; Heftrich, Tanja; Kausch, Tanja; Köppchen, Christoph; Kurtulgil, Deniz; Langer, Christoph; Thomas, Benedikt; Weigand, Mario

    2018-03-01

    The decay properties of long-lived excited states (isomers) can have a significant impact on the destruction channels of isotopes under stellar conditions. In sufficiently hot environments, the population of isomers can be altered via thermal excitation or de-excitation. If the corresponding lifetimes are of the same order of magnitude as the typical time scales of the environment, the isomers have to be treated explicitly. We present a general approach to the treatment of isomers in stellar nucleosynthesis codes and discuss a few illustrative examples. The corresponding code is available online at http://exp-astro.de/isomers/.

  4. Fission fragment mass distributions via prompt γ-ray spectroscopy

    Indian Academy of Sciences (India)

    2015-07-24

    Jul 24, 2015 ... The distribution of fragment masses formed in nuclear fission is one of the most striking features of the process. Such measurements are very important to understand the shape evolution of the nucleus from ground state to scission through intermediate saddle points. The fission fragment mass distributions, ...

  5. Fission fragment mass distributions via prompt γ-ray spectroscopy

    Indian Academy of Sciences (India)

    Abstract. The distribution of fragment masses formed in nuclear fission is one of the most strik- ing features of the process. Such measurements are very important to understand the shape evolu- tion of the nucleus from ground state to scission through intermediate saddle points. The fission fragment mass distributions ...

  6. Isomers chart; Table des isomeres

    Energy Technology Data Exchange (ETDEWEB)

    Dupont-Gautier, P.; Chantelot, S.; Moisson, N. [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires

    1967-07-01

    The nuclear isomers are nuclides offering the same mass number and the same atomic number, but different energy levels. In the following chart the zero energy ground states are omitted and the metastable isomers, i.e. of non-zero energy, known and of measurable lifetime, are listed. The lower limit of this lifetime was set here to 0.1 x 10{sup -6} s. The various isomers were classified in increasing lifetimes. (authors) [French] Les isomeres nucleaires sont des nucleides presentant le meme nombre de masse et le meme numero atomique, mais des niveaux energetiques differents. Dans la table suivante, on a neglige les etats fondamentaux d'energie nulle et on a recense les isomeres metastables, c'est-a-dire d'energie non nulle, connus et de periode mesurable. La limite inferieure de cette periode a ete fixee ici a 0,1 x 10{sup -6} s. Les differents isomeres ont ete classes par periodes croissantes. (auteurs)

  7. Effects of high-order deformation on high-K isomers in superheavy nuclei

    International Nuclear Information System (INIS)

    Liu, H. L.; Bertulani, C. A.; Xu, F. R.; Walker, P. M.

    2011-01-01

    Using, for the first time, configuration-constrained potential-energy-surface calculations with the inclusion of β 6 deformation, we find remarkable effects of the high-order deformation on the high-K isomers in 254 No, the focus of recent spectroscopy experiments on superheavy nuclei. For shapes with multipolarity six, the isomers are more tightly bound and, microscopically, have enhanced deformed shell gaps at N=152 and Z=100. The inclusion of β 6 deformation significantly improves the description of the very heavy high-K isomers.

  8. "Star" morphologies of charged nanodrops comprised of conformational isomers

    Science.gov (United States)

    In Oh, Myong; Paliy, Maxim; Consta, Styliani

    2018-01-01

    We study the spatial distribution of conformational isomers surrounding a central macroion in a charged droplet with linear dimensions in the nanometer range. Dimethyl carbonate and formic acid are selected as typical solvents that undergo isomerization and a charged buckyball (C60) is selected as a representative example of a macroion. The study is performed by atomistic molecular dynamics simulations. We find that when the charge of the buckyball is above a threshold value, it induces the formation of concentric shells of different conformational isomers surrounding the macroion. The presence of layers with different dielectric properties necessitates the use of different state equations for the solvent polarization in each layer. We find that at a high charge state of the buckyball, the nearest layer to the macroion comprises the conformers with the highest dipole moment. The interface of the outer layers of conformers is characterized by "ray"-forming structures of the higher dielectric constant isomers penetrating into the layer of the lowest dielectric constant isomers. For high values of the solvent dielectric constant, the charged droplet acquires a "star"-like global shape. We demonstrate that these distinct droplet structures are a manifestation of charge-induced instability. We describe this simulation-based phenomenology by an analytical theory that supports this conclusion. The findings suggest new experimental research venues that may explore the reactivity and assembly of molecules within regions of different dielectric properties in droplets.

  9. Measurement of mass and isotopic fission yields for heavy fission products with the LOHENGRIN mass spectrometer

    International Nuclear Information System (INIS)

    Bail, A.

    2009-05-01

    In spite of the huge amount of fission yield data available in different libraries, more accurate values are still needed for nuclear energy applications and to improve our understanding of the fission process. Thus measurements of fission yields were performed at the mass spectrometer Lohengrin at the Institut Laue-Langevin in Grenoble, France. The mass separator Lohengrin is situated at the research reactor of the institute and permits the placement of an actinide layer in a high thermal neutron flux. It separates fragments according to their atomic mass, kinetic energy and ionic charge state by the action of magnetic and electric fields. Coupled to a high resolution ionization chamber the experiment was used to investigate the mass and isotopic yields of the light mass region. Almost all fission yields of isotopes from Th to Cf have been measured at Lohengrin with this method. To complete and improve the nuclear data libraries, these measurements have been extended in this work to the heavy mass region for the reactions 235 U(n th ,f), 239 Pu(n th ,f) and 241 Pu(n th ,f). For these higher masses an isotopic separation is no longer possible. So, a new method was undertaken with the reaction 239 Pu(n th ,f) to determine the isotopic yields by spectrometry. These experiments have allowed to reduce considerably the uncertainties. Moreover the ionic charge state and kinetic energy distributions were specifically studied and have shown, among others, nanosecond isomers for some masses. (author)

  10. New experimental approaches to investigate the fission dynamics

    Energy Technology Data Exchange (ETDEWEB)

    Benlliure, J., E-mail: j.benlliure@usc.es; Rodríguez-Sánchez, J. L.; Alvarez-Pol, H.; Ayyad, Y.; Cortina-Gil, D.; Paradela, C.; Pietras, B.; Ramos, D.; Vargas, J. [Universidade de Santiago de Compostela, 15782 Santiago de Compostela (Spain); Audouin, L.; Boutoux, G. [Institut de Physique Nucléaire d’Orsay, F-91406 Orsay (France); Bélier, G.; Chatillon, A.; Gorbinet, T.; Laurent, B.; Martin, J.-F.; Pellereau, E.; Taïeb, J. [CEA, DAM, DIF, F-91297 Arpajon (France); Casarejos, E. [Universidad de Vigo, E-36200 Vigo (Spain); Heinz, A. [Chalmers University of Technology, SE-412 96 Gothenburg (Sweden); and others

    2016-07-07

    The first ever achieved full identification of both fission fragments, in atomic and mass number, made it possible to define new observables sensitive to the fission dynamics along the fission path up to the scission point. Moreover, proton-induced fission of {sup 208}Pb at high energies offers optimal conditions for the investigation of dissipative, and transient effects, because of the high-excitation energy of the fissioning nuclei, its low angular momentum, and limited shape distortion by the reaction. In this work we show that the charge distribution of the final fission fragments can constrain the ground-to-saddle dynamics while the mass distribution is sensitive to the dynamics until the scission point.

  11. Atlas of nuclear isomers and their systematics

    International Nuclear Information System (INIS)

    Jain, Ashok Kumar; Maheshwari, Bhoomika

    2015-01-01

    Isomers can be viewed as a separate class of nuclei and offer interesting possibilities to study the behavior of nuclei under varied conditions of excitation energy, spin, life-time and particle configuration. We have completed a horizontal evaluation of nuclear isomers and the resulting data set contains a wealth of information which offers new insights in the nuclear structure of a wide range of configurations, nuclei approaching the drip lines etc. We now have reliable data on approximately 2460 isomers having a half-life ≥ 10 ns. A few of the systematics of the properties of nuclear isomers like excitation energy, half-life, spin, abundance etc. will be presented. The data set of semi-magic isomers strongly supports the existence of seniority isomers originating from the higher spin orbitals. (author)

  12. Generalization of Kramer's formula: Fission over a multidimensional potential barrier

    International Nuclear Information System (INIS)

    Jing-Shang, Z.; Weidenmueller, H.A.

    1983-01-01

    We generalize Kramers's rate expression for diffusion over a potential barrier to the case of a diffusion problem for n degrees of freedom. These can be thought of as the shape degrees of freedom of a fissioning nucleus. We present our formula for the fission width and discuss its dependence on the parameters: the mass tensor, the friction tensor, and the shape of the potential landscape

  13. Fission Spectrum Related Uncertainties

    Energy Technology Data Exchange (ETDEWEB)

    G. Aliberti; I. Kodeli; G. Palmiotti; M. Salvatores

    2007-10-01

    The paper presents a preliminary uncertainty analysis related to potential uncertainties on the fission spectrum data. Consistent results are shown for a reference fast reactor design configuration and for experimental thermal configurations. However the results obtained indicate the need for further analysis, in particular in terms of fission spectrum uncertainty data assessment.

  14. The nuclear fission

    International Nuclear Information System (INIS)

    Fiorentino, J.

    1983-01-01

    The nuclear fission process considering initially the formation of compound nucleus and finishing with radioactive decay of fission products is studied. The process is divided in three parts which consist of the events associated to the nucleus of intermediate transitional state, the scission configuration, and the phenomenum of post scission. (M.C.K.) [pt

  15. Optical absorption spectra of Ag-11 isomers

    DEFF Research Database (Denmark)

    Martinez, Jose Ignacio; Fernandez, E. M.

    2009-01-01

    The optical absorption spectra of the three most; stable structural isomers of the Ag-11 cluster were calculated using the time-dependent, density functional theory within the Casida formalism. The slightly different, spectra, of the isomers may permit the identification of the ground-stale confi......The optical absorption spectra of the three most; stable structural isomers of the Ag-11 cluster were calculated using the time-dependent, density functional theory within the Casida formalism. The slightly different, spectra, of the isomers may permit the identification of the ground...

  16. Evidences for magicity in superdeformed shapes

    Indian Academy of Sciences (India)

    inertia (0) and nuclear softness parameter (σ) for the SD bands in all the mass regions ... to a good understanding of the observed SD bands and fission isomers. .... to the positions of least level density, we expect the. SD bands near magic nucleon numbers to be more close to exact rigid rotor. The usual. 30 40. 50. 60. 70.

  17. The nuclear fission process

    International Nuclear Information System (INIS)

    Wagemans, C.

    1991-01-01

    Fifty years after its discovery, the nuclear fission phenomenon is of recurring interest. When its fundamental physics aspects are considered, fission is viewed in a very positive way, which is reflected in the great interest generated by the meetings and large conferences organized for the 50th anniversary of its discovery. From a purely scientific and practical point of view, a new book devoted to the (low energy) nuclear fission phenomenon was highly desirable considering the tremendous amount of new results obtained since the publication of the book Nuclear Fission by Vandenbosch and Huizenga in 1973 (Academic Press). These new results could be obtained thanks to the growth of technology, which enabled the construction of powerful new neutron sources, particle and heavy ion accelerators, and very performant data-acquisition and computer systems. The re-invention of the ionization chamber, the development of large fission fragment spectrometers and sophisticated multiparameter devices, and the production of exotic isotopes also contributed significantly to an improved understanding of nuclear fission. This book is written at a level to introduce graduate students to the exciting subject of nuclear fission. The very complete list of references following each chapter also makes the book very useful for scientists, especially nuclear physicists. The book has 12 chapters covering the fission barrier and the various processes leading to fission as well as the characteristics of the various fission reaction products. In order to guarantee adequate treatment of the very specialized research fields covered, several distinguished scientists actively involved in some of these fields were invited to contribute their expertise as authors or co-authors of the different chapters

  18. Fission 2009 4. International Workshop on Nuclear Fission and Fission Product Spectroscopy - Compilation of slides

    International Nuclear Information System (INIS)

    2009-01-01

    This conference is dedicated to the last achievements in experimental and theoretical aspects of the nuclear fission process. The topics include: mass, charge and energy distribution, dynamical aspect of the fission process, nuclear data evaluation, quasi-fission and fission lifetime in super heavy elements, fission fragment spectroscopy, cross-section and fission barrier, and neutron and gamma emission. This document gathers the program of the conference and the slides of the presentations

  19. Structural-based differences in ecotoxicity of benzoquinoline isomers to the zebra mussel (Dreissena polymorpha)

    Energy Technology Data Exchange (ETDEWEB)

    Kraak, M.H.S.; Wijnands, P.; Govers, H.A.J.; Admiraal, W.; Voogt, P. de [Univ. of Amsterdam (Netherlands)

    1997-10-01

    Effects of four benzoquinoline isomers on the filtration rate of the zebra mussel (Dreissena polymorpha) were analyzed, to study the effect of minor differences in chemical structure on adverse biological effects. Filtration rates were measured after 48 h of exposure to different concentrations of acridine, phenanthridine, benzo[f]quinoline, and benzo[h]quinoline in the water. The 50% effective concentration (EC50) values for filtration rate of the four isomers differed significantly. Effects increased in the order benzo[f], -[h], -[b], and -[c]quinoline, and the difference between the most toxic isomer and the least toxic isomer amounted to a factor of 30. Attempts were made to relate these differences in toxicity to the structure of the isomers. Size- or topology-related molecular descriptors provided insufficient resolution to distinguish between the benzoquinoline isomers, and none of the electronic descriptors separately provided a significant correlation with the observed effects. In an alternative approach, molecular shape, accessibility, and minimum agent-macromolecule distance were used to represent repulsive and attractive forces between the benzoquinoline isomers and biological membranes. This approach could tentatively explain the observed effects and is supported by a high correlation between the EC50 data and the reversed-phase C18-HPLC behavior of the benzoquinolines (k{sub 0}), which is likely to be governed by similar processes.

  20. Mitochondrial morphological features are associated with fission and fusion events.

    Directory of Open Access Journals (Sweden)

    Laura M Westrate

    Full Text Available Mitochondria are dynamic organelles that undergo constant remodeling through the regulation of two opposing processes, mitochondrial fission and fusion. Although several key regulators and physiological stimuli have been identified to control mitochondrial fission and fusion, the role of mitochondrial morphology in the two processes remains to be determined. To address this knowledge gap, we investigated whether morphological features extracted from time-lapse live-cell images of mitochondria could be used to predict mitochondrial fate. That is, we asked if we could predict whether a mitochondrion is likely to participate in a fission or fusion event based on its current shape and local environment. Using live-cell microscopy, image analysis software, and supervised machine learning, we characterized mitochondrial dynamics with single-organelle resolution to identify features of mitochondria that are predictive of fission and fusion events. A random forest (RF model was trained to correctly classify mitochondria poised for either fission or fusion based on a series of morphological and positional features for each organelle. Of the features we evaluated, mitochondrial perimeter positively correlated with mitochondria about to undergo a fission event. Similarly mitochondrial solidity (compact shape positively correlated with mitochondria about to undergo a fusion event. Our results indicate that fission and fusion are positively correlated with mitochondrial morphological features; and therefore, mitochondrial fission and fusion may be influenced by the mechanical properties of mitochondrial membranes.

  1. Comparative aerobic soil metabolism of fenvalerate isomers

    International Nuclear Information System (INIS)

    Lee, P.W.; Powell, W.R.; Stearns, S.M.; McConnell, O.J.

    1987-01-01

    An aerobic soil metabolism study was conducted to determine the degradation rate of individual isomer of fenvalerate and to assess the potential influence of the RS, SR, and RR isomers to the metabolism of the most insecticidally active SS isomer. Individual [phenoxyphenyl- 14 C]fenvalerate isomers degraded at different rates. The calculated half-lives for the SR, RS, SS, and RR isomers in fenvalerate (racemic mixture) were 155, 89, 108, and 178 days, respectively. The resolved SS isomer degraded at a faster rate with a calculated half-life of 74 days. Racemization of the resolved SS isomer did not occur. A qualitative difference in the chemical nature of soil metabolites between fenvalerate and the resolved SS isomer was not observed. Soil degradation products, phenoxybenzoic acid, 3-(4-hydroxyphenoxy)benzoic acid, and 4'-OH- and CONH 2 -fenvalerate, each accounted for less than 2% of the applied radioactivity. Extensive degradation of these soil metabolites was evident since approximately 50% of the applied radioactivity was recovered as 14 C 2 and as unextractable bound residues

  2. Rupturing the hemi-fission intermediate in membrane fission under tension: Reaction coordinates, kinetic pathways, and free-energy barriers

    Science.gov (United States)

    Zhang, Guojie; Müller, Marcus

    2017-08-01

    Membrane fission is a fundamental process in cells, involved inter alia in endocytosis, intracellular trafficking, and virus infection. Its underlying molecular mechanism, however, is only incompletely understood. Recently, experiments and computer simulation studies have revealed that dynamin-mediated membrane fission is a two-step process that proceeds via a metastable hemi-fission intermediate (or wormlike micelle) formed by dynamin's constriction. Importantly, this hemi-fission intermediate is remarkably metastable, i.e., its subsequent rupture that completes the fission process does not occur spontaneously but requires additional, external effects, e.g., dynamin's (unknown) conformational changes or membrane tension. Using simulations of a coarse-grained, implicit-solvent model of lipid membranes, we investigate the molecular mechanism of rupturing the hemi-fission intermediate, such as its pathway, the concomitant transition states, and barriers, as well as the role of membrane tension. The membrane tension is controlled by the chemical potential of the lipids, and the free-energy landscape as a function of two reaction coordinates is obtained by grand canonical Wang-Landau sampling. Our results show that, in the course of rupturing, the hemi-fission intermediate undergoes a "thinning → local pinching → rupture/fission" pathway, with a bottle-neck-shaped cylindrical micelle as a transition state. Although an increase of membrane tension facilitates the fission process by reducing the corresponding free-energy barrier, for biologically relevant tensions, the free-energy barriers still significantly exceed the thermal energy scale kBT.

  3. Rupture of the neck in nuclear fission

    International Nuclear Information System (INIS)

    Davies, K.T.R.; Managan, R.A.; Nix, J.R.; Sierk, A.J.

    1977-01-01

    We introduce a degree of freedom to describe the rupture of the neck in nuclear fission and calculate the point at which the neck ruptures as the nucleus descends dynamically from its fission saddle point. This is done by mentally slicing the system into two portions at its minimum neck radius and calculating the force required to separate the two portions while keeping their shapes fixed. This force is obtained by differentiating with respect to separation the sum of the Coulomb and nuclear interaction energies between the two portions. For nuclei throughout the Periodic Table we calculate this force along dynamical paths leading from the fission saddle point. The force is initially attractive but becomes repulsive when the neck reaches a critical size. For actinide nuclei the neck radius at which rupture occurs is about 2 fm. This increases the calculated translational kinetic energy of the fission fragments at infinity relative to that calculated for scission occurring at zero neck radius. With the effect of neck rupture taken into account, we calculate and compare with experimental results fission-fragment kinetic energies for two types of nuclear dissipation: ordinary two-body viscosity and one-body dissipation

  4. Some aspects of the nuclear fission process

    International Nuclear Information System (INIS)

    Netter, F.

    1961-01-01

    In the following report one can find first a short general view on the present situation of our knowledge concerning the nuclear fission process, namely on the nucleus going through the saddle-point. Then there are some aspects connected with the excitation energy of the fissioning nucleus. The measurements made at Saclay on the fast neutron fission cross-section of U 233 , U 235 , Pu 239 , U 238 are described at the beginning of this work. It appears that for U 233 there is some characteristic shape modulation of the cross-section curve, in relation with the collective excited state of the deformed nucleus at the saddle-point. Good evidence of this is also given by the study of the relative fission rate with emission of long-range particles; it appears also that this ternary fission rate does not change substantially for neutron between thermal energy and 2 MeV, but that is very lower for the compound nucleus U 239 than for even-even compound nuclei. At the end there are some experiments on the strong 4,5 MeV gamma-ray originated by slow neutron absorption in U 235 . Time-of-flight device is used to establish that this 4,5 MeV gamma-ray seems mostly connected with radiative capture. (author) [fr

  5. Fission in a Plasma

    Energy Technology Data Exchange (ETDEWEB)

    Younes, W. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

    2016-10-26

    A three-year theory project was undertaken to study the fission process in extreme astrophysical environments, such as the crust of neutron stars. In the first part of the project, the effect of electron screening on the fission process was explored using a microscopic approach. For the first time, these calculations were carried out to the breaking point of the nucleus. In the second part of the project, the population of the fissioning nucleus was calculated within the same microscopic framework. These types of calculations are extremely computer-intensive and have seldom been applied to heavy deformed nuclei, such as fissioning actinides. The results, tools and methodologies produced in this work will be of interest to both the basic-science and nuclear-data communities.

  6. Prompt γ rays and neutrons from fission

    Science.gov (United States)

    Kwan, E.; Wu, C. Y.; Chyzh, A.; Gostic, J.; Henderson, R.; Haight, R. C.; Lee, H. Y.; O'Donnell, J. M.; Perdue, B. A.; Taddeucci, T. N.

    2011-10-01

    Nuclear data are needed to test the accuracy of calculations from nuclear reaction codes. Information on the prompt γ-ray distributions from fission is sparse and only a handful of published experiments data that measured the prompt γ-ray distribution above incident neutron energies of 1 MeV can be found. In addition, improvement on the accuracy and shape of neutron spectrum from the fission of actinides been requested by the nuclear data community. An investigation on the shapes of the neutron and γ-ray distributions from the spontaneous fission of 252Cf and the neutron-induced fission of 235U was undertaken using the Chi-Nu detector array at the Weapons Neutron Research Facility of the Los Alamos Neutron Science Center. Preliminary results will be presented. This work is performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344 and the Los Alamos National Laboratory under Contract DE-AC52-06NA25396.

  7. Shape evolution in neutron-rich A ~ 140 nuclei beyond the doubly-magic nucleus 132Sn

    Science.gov (United States)

    Odahara, Atsuko; Eurica Collaboration

    2014-09-01

    Study for the shape evolution enables us to disentangle competition between spherical (single-particle like) shape and deformed (collective-like) shape as a function of neutron number. Neutron-rich nuclei in the northeast region of the doubly-magic 132Sn locates in one of the best mass region where a variety of collective modes, not only prolate deformation but also octupole collectivity, are expected to appear. These neutron-rich A ~140 nuclei were produced by using in-flight fission reaction of the 345 MeV/u 238U86+ beam at RIKEN RI Beam Factory. This experiment was performed in the framework of the EURICA (EUroball RIken Cluster Array) project based on the highly-efficient β- and isomer-decay spectroscopy methods. Around 20 extremely neutron-rich nuclei with Z=51--55 have been studied in this work. New isomers with half lives of longer than hundreds ns were found in some nuclei, such as the neutron-rich Cs isotopes. Also, preliminary results for the β decay of neutron-rich I and Xe isotopes have been obtained. Systematic change of the shape evolution for these neutron-rich isotopes will be discussed.

  8. Neutron angular distribution in plutonium-240 spontaneous fission

    Energy Technology Data Exchange (ETDEWEB)

    Marcath, Matthew J., E-mail: mmarcath@umich.edu [Department of Nuclear Engineering and Radiological Sciences, University of Michigan, 2355 Bonisteel Boulevard, Ann Arbor, MI 48109 (United States); Shin, Tony H.; Clarke, Shaun D. [Department of Nuclear Engineering and Radiological Sciences, University of Michigan, 2355 Bonisteel Boulevard, Ann Arbor, MI 48109 (United States); Peerani, Paolo [European Commission at the Joint Research Centre, Ispra (Italy); Pozzi, Sara A. [Department of Nuclear Engineering and Radiological Sciences, University of Michigan, 2355 Bonisteel Boulevard, Ann Arbor, MI 48109 (United States)

    2016-09-11

    Nuclear safeguards applications require accurate fission models that exhibit prompt neutron anisotropy. In the laboratory reference frame, an anisotropic neutron angular distribution is observed because prompt fission neutrons carry momentum from fully accelerated fission fragments. A liquid organic scintillation detector array was used with pulse shape discrimination techniques to produce neutron-neutron cross-correlation time distributions and angular distributions from spontaneous fission in a {sup 252}Cf, a 0.84 g {sup 240}Pu{sub eff} metal, and a 1.63 g {sup 240}Pu{sub eff} metal sample. The effect of cross-talk, estimated with MCNPX-PoliMi simulations, is removed from neutron-neutron coincidences as a function of the angle between detector pairs. Fewer coincidences were observed at detector angles near 90°, relative to higher and lower detector angles. As light output threshold increases, the observed anisotropy increases due to spectral effects arising from fission fragment momentum transfer to emitted neutrons. Stronger anisotropy was observed in Cf-252 spontaneous fission prompt neutrons than in Pu-240 neutrons. - Highlights: • Pu-240 prompt fission fast-neutron anisotropy was quantified for the first time. • MCNPX-PoliMi and MPPost codes were used to remove cross-talk neutron detections from experiment results. • Cf-252 spontaneous fission neutrons were found to be more anisotropic than Pu-240 neutrons.

  9. Correlated fission data measurements with DANCE and NEUANCE

    Science.gov (United States)

    Jandel, M.; Baramsai, B.; Bredeweg, T. A.; Couture, A.; Favalli, A.; Hayes, A. C.; Ianakiev, K. D.; Iliev, M. L.; Kawano, T.; Mosby, S.; Rusev, G.; Stetcu, I.; Talou, P.; Ullmann, J. L.; Vieira, D. J.; Walker, C. L.; Wilhelmy, J. B.

    2018-02-01

    To enhance the capabilities of the DANCE array, a new detector array NEUANCE was developed to enable simultaneous measurements of prompt fission neutrons and γ rays. NEUANCE was designed and constructed using 21 stilbene organic scintillator crystals. It was installed in the central cavity of the DANCE array. Signals from the 160 BaF2 detectors of DANCE and the 21 detectors of NEUANCE were merged into a newly designed high-density high-throughput data acquisition system. The excellent pulse shape discrimination properties of stilbene enabled detection of neutrons with energy thresholds as low as 30-40 keVee. A fission reaction tagging method was developed using a NEUANCE γ-ray or neutron signal. The probability of detecting a neutron from the spontaneous fission of 252Cf using NEUANCE is ∼47%. New correlated data for prompt fission neutrons and prompt fission γ rays were obtained for 252Cf using this high detection efficiency experimental setup. Average properties of prompt fission neutron emission as a function of prompt fission γ-ray quantities were also obtained, suggesting that neutron and γ-ray emission in fission are correlated.

  10. Microscopic description of 258Fm fission dynamic with pairing

    Directory of Open Access Journals (Sweden)

    Scamps Guillaume

    2016-01-01

    Full Text Available Fission dynamic remains a challenge for nuclear microscopic theories. In order to understand the dynamic of the last stage of the fission process, the time-dependent Hartree-Fock approach with BCS pairing is applied to the describe the fission of the 258Fm. A good agreement is found for the one-body observables: the total kinetic energy and the average mass asymmetry. The non-physical dependence of two-body observables with the initial shape is discussed.

  11. Scission neutron emission and prompt fission neutron spectrum

    CERN Document Server

    Kornilov, N V

    2001-01-01

    The mass, energy and angular integrated spectra of prompt fission neutrons for sup 2 sup 3 sup 5 U induced fission in the energy range from thermal to 5 MeV were analyzed. It allows assume that about 0.362+-0.025 neutrons per fission are emitted due to another mechanism then neutron emission from excited fragments after full acceleration. The spectrum of scission neutrons consists of two components with average energy 0.98 MeV and 2.74 MeV. The share of scission neutrons and their spectrum shape estimated in this work does not contradict to results of differential experiments analyzed in previous papers.

  12. Isomer effect on the near-infrared electrochromism of anthraquinone imides

    International Nuclear Information System (INIS)

    Yao, Bin; Chen, Fengkun; Jiang, Hong; Zhang, Jie; Wan, Xinhua

    2015-01-01

    Graphical abstract: Display Omitted - Highlights: • Two pairs of unsubstituted isomers (Ia and Ib) and nitro-substituted isomers (IIa and IIb) of anthraquinone imides (AQIs), which are a unique type of cathodically-colouring NIR electrochromic materials bearing both quinone and imide moieties, were synthesized. • Isomer effect on the NIR electrochromism of n-type optoelectric materials was first approached. • A meaningful reference to design cathodically active NIR EC materials, in which the molecular planarity and the orientation of polar groups are two key elements must to be carefully considered, is provided. - Abstract: To deeply explore the interplay between molecular structure and near-infrared electrochromism of anthraquinone imides, two pairs of unsubstituted isomers (Ia and Ib) and nitro-substituted isomers (IIa and IIb) of anthraquinone imides were synthesized, in which the molecules Ia and IIa took more linear shapes than Ib and IIb. Cyclic voltammetry and spectroelectrochemistry were combined to investigate their electrochemical properties. Cyclic voltammetry showed that Ib and IIb revealed decreased first reduction potentials and low cyclic stability compared to their isomers, indicating that the isomerization weakened the stabilization effect. Upon one-electron reduction, both the absorption wavelengths and absorption intensities of radical anions were greatly dependent on the structures of isomers. The radical anions of Ia, IIa, and IIb illustrated NIR absorptions peaked at 820, 1260, and 1380 nm, respectively, but that of Ib exhibited only weak absorption in the visible region centered at 660 nm. Gaussian calculations suggested that the electrons were delocalized over the whole molecular skeletons of Ia and IIa radical anions, but the effective conjugation length was interrupted on the imide section in both Ib and IIb. The isomer effects on the effective conjugation length and electron density distribution were considered to rationalize the

  13. Angular Momentum in Fission

    Science.gov (United States)

    Gönnenwein, F.; Bunakov, V.; Dorvaux, O.; Gagarski, A.; Guseva, I.; Hanappe, F.; Kadmensky, S.; von Kalben, J.; Khlebnikov, S.; Kinnard, V.; Kopatch, Yu.; Mutterer, M.; Nesvizhevsky, V.; Petrov, G.; Prokhorova, E.; Rubchenya, V.; Sillanpää, M.; Simpson, G.; Sokolov, V.; Soldner, T.; Stuttgé, L.; Tiourine, G.; Trzaska, W.; Tsekhanovich, I.; Wagemans, C.; Wollersheim, H.-J.; Zavarukhina, T.; Zimmer, O.

    2008-04-01

    Three novel experiments in spontaneous and thermal neutron induced fission all with a bearing on angular momentum in fission are reviewed. In the first experiment it was observed that, in the reaction 235U(n, f) with incident polarized cold neutrons, the nucleus undergoing scission is rotating. This was inferred from the shift in angular distributions of ternary particles being dependent on the orientation of neutron spin. In the second study the properties of the angular momentum of spherical fission fragments was investigated. Current theories trace the spin of fragments to their deformations allowing for collective rotational vibrations at scission. However, in particular the spherical 132Te isotope exhibits a large spin at variance with theory. Exploiting the specific properties of cold deformed fission it could be proven that, for 132Te, single particle excitations instead of collective modes are responsible for the large spin observed. In a third project a pilot study was exploring the possibility to search for an evaporation of neutrons from fragments being anisotropic in their own cm-system. Due to fragment spin this anisotropy is claimed since decades to exist. It was so far never observed. A scheme has been devised and tested were triple coincidences between a fragment and two neutrons are evaluated in a way to bring the cm-anisotropy into the foreground while getting rid of the kinematical anisotropy in the lab-system due to evaporation from moving fragments. The test was run for spontaneous fission of 252Cf.

  14. Fixed-bed adsorption separation of xylene isomers over sio2/silicallite-1 core-shell adsorbents

    KAUST Repository

    Khan, Easir A.

    2013-12-29

    SiO2/Silicalite-1 core-shell material has been demonstrated as potential shape selective adsorbent in gas phase separation of p-xylene from a mixture of p/o-xylene isomers. The core-shell composite comprised of large silica core and thin polycrystalline silicalite-1 shell which was synthesized via a self-assembly of silicalite-1 nanocrystals on core silica surface followed by a secondary seeded growth method. The core materials, SiO2 used in this study has mesoporosity with an average pore diameter of 60Å and hence offers no shape selectivity for xylene isomers. However, the shell, silicalite-1 contains rigid pore structures and preferentially adsorbs p-xylene from their isomers mixtures. A series of adsorption fixed bed breakthrough adsorption/desorption experiment was performed to obtain the equilibrium isotherms and adsorption isotherm parameters of xylene isomers. The equilibrium isotherms of xylene isomers follow the Langmuir\\'s model. A chromatographic adsorption model has been used to describe the fixed-bed breakthrough profiles of xylene isomers. The model has successfully predicted the responses of the binary mixtures of p/o-xylene isomers. The SiO2/silicalite-1 core-shell adsorbents have shown para-selectivity as high as 15. © Bangladesh Uni. of Engg. & Tech.

  15. Analysis of prompt fission neutrons in 235U(nth,f) and fission fragment distributions for the thermal neutron induced fission of 234U

    Science.gov (United States)

    Al-Adili, A.; Tarrío, D.; Hambsch, F.-J.; Göök, A.; Jansson, K.; Solders, A.; Rakopoulos, V.; Gustafsson, C.; Lantz, M.; Mattera, A.; Oberstedt, S.; Prokofiev, A. V.; Vidali, M.; Österlund, M.; Pomp, S.

    2016-06-01

    This paper presents the ongoing analysis of two fission experiments. Both projects are part of the collaboration between the nuclear reactions group at Uppsala and the JRC-IRMM. The first experiment deals with the prompt fission neutron multiplicity in the thermal neutron induced fission of 235U(n,f). The second, on the fission fragment properties in the thermal fission of 234U(n,f). The prompt fission neutron multiplicity has been measured at the JRC-IRMM using two liquid scintillators in coincidence with an ionization chamber. The first experimental campaign focused on 235U(nth,f) whereas a second experimental campaign is foreseen later for the same reaction at 5.5 MeV. The goal is to investigate how the so-called sawtooth shape changes as a function of fragment mass and excitation energy. Some harsh experimental conditions were experienced due to the large radiation background. The solution to this will be discussed along with preliminary results. In addition, the analysis of thermal neutron induced fission of 234U(n,f) will be discussed. Currently analysis of data is ongoing, originally taken at the ILL reactor. The experiment is of particular interest since no measurement exist of the mass and energy distributions for this system at thermal energies. One main problem encountered during analysis was the huge background of 235U(nth,f). Despite the negligible isotopic traces in the sample, the cross section difference is enormous. Solution to this parasitic background will be highlighted.

  16. Fission gas measuring technology

    International Nuclear Information System (INIS)

    Lee, Hyung Kwon; Kim, Eun Ka; Hwang, Yong Hwa; Lee, Eun Pyo; Chun, Yong Bum; Seo, Ki Seog; Park, Dea Gyu; Chu, Yong Sun; Ahn, Sang Bok.

    1998-02-01

    Safety and economy of nuclear plant are greatly affected by the integrity of nuclear fuels during irradiation reactor core. A series of post-irradiation examination (PIE) including non-destructive and destructive test is to be conducted to evaluate and characterize the nuclear performance. In this report, a principle of the examination equipment to measure and analyse fission gases existing nuclear fuels were described and features of the component and device consisting the fission gas measuring equipment are investigated. (author). 4 refs., 2 tabs., 6 figs

  17. Fission gas measuring technology

    Energy Technology Data Exchange (ETDEWEB)

    Lee, Hyung Kwon; Kim, Eun Ka; Hwang, Yong Hwa; Lee, Eun Pyo; Chun, Yong Bum; Seo, Ki Seog; Park, Dea Gyu; Chu, Yong Sun; Ahn, Sang Bok

    1998-02-01

    Safety and economy of nuclear plant are greatly affected by the integrity of nuclear fuels during irradiation reactor core. A series of post-irradiation examination (PIE) including non-destructive and destructive test is to be conducted to evaluate and characterize the nuclear performance. In this report, a principle of the examination equipment to measure and analyse fission gases existing nuclear fuels were described and features of the component and device consisting the fission gas measuring equipment are investigated. (author). 4 refs., 2 tabs., 6 figs.

  18. Fission modelling with FIFRELIN

    Energy Technology Data Exchange (ETDEWEB)

    Litaize, Olivier; Serot, Olivier; Berge, Leonie [CEA, DEN, DER, SPRC, Saint Paul Lez Durance (France)

    2015-12-15

    The nuclear fission process gives rise to the formation of fission fragments and emission of particles (n,γ, e{sup -}). The particle emission from fragments can be prompt and delayed. We present here the methods used in the FIFRELIN code, which simulates the prompt component of the de-excitation process. The methods are based on phenomenological models associated with macroscopic and/or microscopic ingredients. Input data can be provided by experiment as well as by theory. The fission fragment de-excitation can be performed within Weisskopf (uncoupled neutron and gamma emission) or a Hauser-Feshbach (coupled neutron/gamma emission) statistical theory. We usually consider five free parameters that cannot be provided by theory or experiments in order to describe the initial distributions required by the code. In a first step this set of parameters is chosen to reproduce a very limited set of target observables. In a second step we can increase the statistics to predict all other fission observables such as prompt neutron, gamma and conversion electron spectra but also their distributions as a function of any kind of parameters such as, for instance, the neutron, gamma and electron number distributions, the average prompt neutron multiplicity as a function of fission fragment mass, charge or kinetic energy, and so on. Several results related to different fissioning systems are presented in this work. The goal in the next decade will be i) to replace some macroscopic ingredients or phenomenological models by microscopic calculations when available and reliable, ii) to be a support for experimentalists in the design of detection systems or in the prediction of necessary beam time or count rates with associated statistics when measuring fragments and emitted particle in coincidence iii) extend the model to be able to run a calculation when no experimental input data are available, iv) account for multiple chance fission and gamma emission before fission, v) account for

  19. Hemi-fused structure mediates and controls fusion and fission in live cells.

    Science.gov (United States)

    Zhao, Wei-Dong; Hamid, Edaeni; Shin, Wonchul; Wen, Peter J; Krystofiak, Evan S; Villarreal, Seth A; Chiang, Hsueh-Cheng; Kachar, Bechara; Wu, Ling-Gang

    2016-06-23

    Membrane fusion and fission are vital for eukaryotic life. For three decades, it has been proposed that fusion is mediated by fusion between the proximal leaflets of two bilayers (hemi-fusion) to produce a hemi-fused structure, followed by fusion between the distal leaflets, whereas fission is via hemi-fission, which also produces a hemi-fused structure, followed by full fission. This hypothesis remained unsupported owing to the lack of observation of hemi-fusion or hemi-fission in live cells. A competing fusion hypothesis involving protein-lined pore formation has also been proposed. Here we report the observation of a hemi-fused Ω-shaped structure in live neuroendocrine chromaffin cells and pancreatic β-cells, visualized using confocal and super-resolution stimulated emission depletion microscopy. This structure is generated from fusion pore opening or closure (fission) at the plasma membrane. Unexpectedly, the transition to full fusion or fission is determined by competition between fusion and calcium/dynamin-dependent fission mechanisms, and is notably slow (seconds to tens of seconds) in a substantial fraction of the events. These results provide key missing evidence in support of the hemi-fusion and hemi-fission hypothesis in live cells, and reveal the hemi-fused intermediate as a key structure controlling fusion and fission, as fusion and fission mechanisms compete to determine the transition to fusion or fission.

  20. Spectroscopy of fission fragments using prompt-delayed ...

    Indian Academy of Sciences (India)

    2015-08-02

    Aug 2, 2015 ... A variety of high-spin phenomena related with the rotation of triaxial shapes [1,2], magnetic/antimagnetic rotations [3,4], shell model excitation [5,6], high-K isomers [7], octupole collectivity in heavy nuclei ..... and LINAC staff for providing excellent beam during the experiment. References. [1] N Rather et al, ...

  1. Role of Multichance Fission in the Description of Fission-Fragment Mass Distributions at High Energies

    Science.gov (United States)

    Hirose, K.; Nishio, K.; Tanaka, S.; Léguillon, R.; Makii, H.; Nishinaka, I.; Orlandi, R.; Tsukada, K.; Smallcombe, J.; Vermeulen, M. J.; Chiba, S.; Aritomo, Y.; Ohtsuki, T.; Nakano, K.; Araki, S.; Watanabe, Y.; Tatsuzawa, R.; Takaki, N.; Tamura, N.; Goto, S.; Tsekhanovich, I.; Andreyev, A. N.

    2017-12-01

    Fission-fragment mass distributions were measured for U 237 - 240 , Np 239 - 242 , and Pu 241 - 244 populated in the excitation-energy range from 10 to 60 MeV by multinucleon transfer channels in the reaction O 18 +U 238 at the Japan Atomic Energy Agency tandem facility. Among them, the data for U 240 and Np 240 ,241 ,242 were observed for the first time. It was found that the mass distributions for all the studied nuclides maintain a double-humped shape up to the highest measured energy in contrast to expectations of predominantly symmetric fission due to the washing out of nuclear shell effects. From a comparison with the dynamical calculation based on the fluctuation-dissipation model, this behavior of the mass distributions was unambiguously attributed to the effect of multichance fission.

  2. Fission fragment mass and total kinetic energy distributions of spontaneously fissioning plutonium isotopes

    Science.gov (United States)

    Pomorski, K.; Nerlo-Pomorska, B.; Bartel, J.; Schmitt, C.

    2018-03-01

    The fission-fragment mass and total kinetic energy (TKE) distributions are evaluated in a quantum mechanical framework using elongation, mass asymmetry, neck degree of freedom as the relevant collective parameters in the Fourier shape parametrization recently developed by us. The potential energy surfaces (PES) are calculated within the macroscopic-microscopic model based on the Lublin-Strasbourg Drop (LSD), the Yukawa-folded (YF) single-particle potential and a monopole pairing force. The PES are presented and analysed in detail for even-even Plutonium isotopes with A = 236-246. They reveal deep asymmetric valleys. The fission-fragment mass and TKE distributions are obtained from the ground state of a collective Hamiltonian computed within the Born-Oppenheimer approximation, in the WKB approach by introducing a neck-dependent fission probability. The calculated mass and total kinetic energy distributions are found in good agreement with the data.

  3. Discoveries of isotopes by fission

    Indian Academy of Sciences (India)

    2015-08-28

    Aug 28, 2015 ... Of the about 3000 isotopes presently known, about 20% have been discovered in fission. The history of fission as it relates to the discovery of isotopes as well as the various reaction mechanisms leading to isotope discoveries involving fission are presented.

  4. 50 years of nuclear fission

    International Nuclear Information System (INIS)

    Hilscher, D.

    1989-01-01

    The article tells the story of the discovery of nuclear fission in Berlin 50 years ago by Otto Hahn and Fritz Strassmann in cooperation with Lise Meitner. 50 years later nuclear fission is still a subject of research. Some question remain unanswered. Selected new research results are used to discuss the dynamics of the collective movement of the elementary nuclear fission process. (orig.) [de

  5. Story of Fission

    Indian Academy of Sciences (India)

    Home; Journals; Resonance – Journal of Science Education; Volume 21; Issue 3. Story of Fission: Unlocking Power of the Nucleus. Amit Roy. General Article Volume 21 Issue 3 March 2016 pp 247-258. Fulltext. Click here to view fulltext PDF. Permanent link: http://www.ias.ac.in/article/fulltext/reso/021/03/0247-0258 ...

  6. Story of Fission

    Indian Academy of Sciences (India)

    IAS Admin

    and contributes very little to global warming. The discovery of fission of uranium in 1939 changed forever the way society at large supported scientific research. Till that time, individual researchers or small groups would pursue their sub- jects of interest with whatever resources they could muster either from government or ...

  7. The discovery of fission

    International Nuclear Information System (INIS)

    McKay, H.A.C.

    1978-01-01

    In this article by the retired head of the Separation Processes Group of the Chemistry Division, Atomic Energy Research Establishment, Harwell, U.K., the author recalls what he terms 'an exciting drama, the unravelling of the nature of the atomic nucleus' in the years before the Second World War, including the discovery of fission. 12 references. (author)

  8. Prompt- and delayed-fission probabilities in actinides within a doorway state model

    International Nuclear Information System (INIS)

    Bellia, G.; Del Zoppo, A.; Migneco, E.; Russo, G.

    1984-01-01

    The formalism of the doorway state model for fission is extended to excitation energy as low as the pairing gap region in the intermediate well of the potential barrier. Expressions for the wave function amplitudes which describe the various possible admixtures of the vibrational modes into the compound-state sets are generalized and can be used to calculate prompt- and delayed-fission probabilities in the energy range between the isomer level and the top of the barrier. The occurrence of different coupling situations for the 238 U 1 - 0 channel is discussed

  9. Prompt- and delayed-fission probabilities in actinides within a doorway state model

    Energy Technology Data Exchange (ETDEWEB)

    Bellia, G.; Del Zoppo, A.; Migneco, E.; Russo, G. (Istituto Nazionale di Fisica Nucleare, Catania (Italy); Catania Univ. (Italy). Ist. di Fisica)

    1984-01-21

    The formalism of the doorway state model for fission is extended to excitation energy as low as the pairing gap region in the intermediate well of the potential barrier. Expressions for the wave function amplitudes which describe the various possible admixtures of the vibrational modes into the compound-state sets are generalized and can be used to calculate prompt- and delayed-fission probabilities in the energy range between the isomer level and the top of the barrier. The occurrence of different coupling situations for the /sup 238/U 1/sup -/0 channel is discussed.

  10. Membrane fission by protein crowding.

    Science.gov (United States)

    Snead, Wilton T; Hayden, Carl C; Gadok, Avinash K; Zhao, Chi; Lafer, Eileen M; Rangamani, Padmini; Stachowiak, Jeanne C

    2017-04-18

    Membrane fission, which facilitates compartmentalization of biological processes into discrete, membrane-bound volumes, is essential for cellular life. Proteins with specific structural features including constricting rings, helical scaffolds, and hydrophobic membrane insertions are thought to be the primary drivers of fission. In contrast, here we report a mechanism of fission that is independent of protein structure-steric pressure among membrane-bound proteins. In particular, random collisions among crowded proteins generate substantial pressure, which if unbalanced on the opposite membrane surface can dramatically increase membrane curvature, leading to fission. Using the endocytic protein epsin1 N-terminal homology domain (ENTH), previously thought to drive fission by hydrophobic insertion, our results show that membrane coverage correlates equally with fission regardless of the hydrophobicity of insertions. Specifically, combining FRET-based measurements of membrane coverage with multiple, independent measurements of membrane vesiculation revealed that fission became spontaneous as steric pressure increased. Further, fission efficiency remained equally potent when helices were replaced by synthetic membrane-binding motifs. These data challenge the view that hydrophobic insertions drive membrane fission, suggesting instead that the role of insertions is to anchor proteins strongly to membrane surfaces, amplifying steric pressure. In line with these conclusions, even green fluorescent protein (GFP) was able to drive fission efficiently when bound to the membrane at high coverage. Our conclusions are further strengthened by the finding that intrinsically disordered proteins, which have large hydrodynamic radii yet lack a defined structure, drove fission with substantially greater potency than smaller, structured proteins.

  11. K isomers as probes of nuclear structure

    Science.gov (United States)

    Tandel, S. K.

    2014-08-01

    K isomers are studied in Pu and Cm isotopes, and also in Hf and W nuclei. Many high-K states, several of which are isomeric, are identified. Lifetime measurements spanning the ns-s range have been performed, and decay paths of isomers established. Rotational bands built on high-K states are also identified in many cases. Isomer decays are considerably hindered in many instances, both in the A≈180 and 250 regions indicating that K is an approximately conserved quantum number. High-K states become the favored excitation mode at high spins in the A≈180 region. The energies of the 2-quasiparticle high-K states in Cm isotopes suggest the presence of a deformed subshell gap at N=152.

  12. K isomers as probes of nuclear structure

    Energy Technology Data Exchange (ETDEWEB)

    Tandel, S. K., E-mail: sujit.tandel@cbs.ac.in [UM-DAE Centre for Excellence in Basic Sciences, Mumbai 400098 (India)

    2014-08-14

    K isomers are studied in Pu and Cm isotopes, and also in Hf and W nuclei. Many high-K states, several of which are isomeric, are identified. Lifetime measurements spanning the ns-s range have been performed, and decay paths of isomers established. Rotational bands built on high-K states are also identified in many cases. Isomer decays are considerably hindered in many instances, both in the A≈180 and 250 regions indicating that K is an approximately conserved quantum number. High-K states become the favored excitation mode at high spins in the A≈180 region. The energies of the 2-quasiparticle high-K states in Cm isotopes suggest the presence of a deformed subshell gap at N=152.

  13. Theoretical prediction of the linear isomers for rare gas-carbon disulfide complexes: He-CS₂, Ne-CS₂, and Ar-CS₂.

    Science.gov (United States)

    Zang, Limin; Dai, Wei; Zheng, Limin; Duan, Chuanxi; Lu, Yunpeng; Yang, Minghui

    2014-03-21

    Theoretical studies of the potential energy surfaces (PESs) and bound states are performed for rare gas-carbon disulfide complexes, He-CS2, Ne-CS2, and Ar-CS2. Three two-dimensional intermolecular PESs are constructed from ab initio data points which are calculated at the CCSD(T) level with aug-cc-pVTZ basis set supplemented with bond functions. We find that the three PESs have very similar features and each PES can be characterized by a global T-shaped minimum, two equivalent local linear minima, and the saddle points between them. The T-shaped isomer is energetically more stable than the linear isomer for each complex. The linear isomers, which have not been observed in experiment so far, are predicted from our PESs and further identified by bound state calculations. Moreover, we assign several intermolecular vibrational states for both the T-shaped and linear isomers of the three complexes via the analysis of wavefunctions. The corresponding vibrational frequencies are calculated from the bound state energies for these assigned states. These frequencies could be helpful for further experimental studies, especially for the linear isomers. We also calculate the rovibrational transition frequencies for the three T-shaped isomers and the pure rotational transition frequencies for the linear isomers, respectively. The accuracy of the PESs is validated by the good agreement between theoretical and experimental results for the rovibrational transition frequencies and spectroscopic parameters.

  14. The fission track method

    International Nuclear Information System (INIS)

    Hansen, K.

    1990-01-01

    During the last decade fission track (FT) analysis has evolved as an important tool in exploration for hydrocarbon resources. Most important is this method's ability to yield information about temperatures at different times (history), and thus relate oil generation and time independently of other maturity parameters. The purpose of this paper is to introduce the basics of the method and give an example from the author's studies. (AB) (14 refs.)

  15. [Fission product yields of 60 fissioning reactions]. Final report

    International Nuclear Information System (INIS)

    Rider, B.F.

    1995-01-01

    In keeping with the statement of work, I have examined the fission product yields of 60 fissioning reactions. In co-authorship with the UTR (University Technical Representative) Talmadge R. England ''Evaluation and Compilation of Fission Product Yields 1993,'' LA-UR-94-3106(ENDF-349) October, (1994) was published. This is an evaluated set of fission product Yields for use in calculation of decay heat curves with improved accuracy has been prepared. These evaluated yields are based on all known experimental data through 1992. Unmeasured fission product yields are calculated from charge distribution, pairing effects, and isomeric state models developed at Los Alamos National Laboratory. The current evaluation has been distributed as the ENDF/B-VI fission product yield data set

  16. Measurement of fission yields far from the center of isotopic distributions in the thermal neutron fission of 235U

    International Nuclear Information System (INIS)

    Shmid, M.

    1979-08-01

    The main purpose of this work was to measure independent yields, in the thermal neutron fission of 235 U, of fission products which lie far from the centers of the isotopic and isobaric yield distributions. These measurements were used to test the predictions of semi-empirical systematics of fission yields and theoretical fission models. Delay times were measured as a function of temperature in the range 1200-2000degC. The very low delay times achieved in the present work permitted expanding the measurable region to the isotopes 147 , 148 Cs and 99 Rb which are of special interest in the present work. The delay times of Sr and Ba isotopes achieved were more than two orders of magnitude lower than values reported in the literature and thus short-lived isotopes of these elements could be separated for the first time by mass spectrometry. The half-lives of 147 Ba, 148 Ba, 149 La and 149 Ce were measured for the first time. The isotopic distributions of fission yields were measured for the elements Rb, Sr, Cs and Ba in the thermal neutron fission of 235 U, those of 99 Rb, 147 Cs and 148 Cs having been measured for the first time. A comparison of the experimental yields with the predictions of the currently accepted semi-empirical systematics of fission yields, which is the odd-even effect systematics, shows that the systematics succeeds in accounting for the strong odd-even proton effect and the weaker odd-even neutron effect and also in predicting the shape of the distributions in the central region. It is shown that prompt neutron emission broadens the distribution only slightly in the wing of heavy isotopes and more significantly in the wing of light isotopes. But the effect of prompt neutron emission cannot explain the large discrepancies existing between the predictions of fission models and the experimentally measured fission yield in the wings of the isotopic distributions. (B.G.)

  17. Crystal field contribution to Moessbauer isomer shift

    International Nuclear Information System (INIS)

    Singh, Avtar; Shrivastava, K.N.

    1975-01-01

    A new temperature dependent contribution to isomer shift in Fe 3+ (ed 5 ) is proposed. The static crystal field gives rise to a new second-order correction to Mossbauer resonance line and crystal field hamiltonian Hc=B 2 0 Y 2 0 +B 2 2 (Y 22 ) usually used in the study of electronspin resonance is employed. The electron charge density at the nuclear site, responsible for the isomer shift is affected by the crystal field through excitation of an electron from 3d to 4s subshell. Further, temperature dependence is analysed by the variation of crystal field parameters with temperature which occurs as a square in the final result. The importance of the sign of the field parameter (KD) is also realised in the isomer shift studies. Although the proposed new second-order contribution to Moessbauer isomer shift is static in nature, yet it is expected to have important implications in the study of temperature depedence of centre shift of a Moessbauer line. Numerical estimates of the shift are also presented. (author)

  18. Neutron emission anisotropy in fission

    OpenAIRE

    CHIETERA A.; STUTTGE L.; GOENNENWEIN F.; KOPATCH Y.; MUTTERER M.; GUSEVA I.; GAGARSKI A.; CHERNYSHEVA E; DORVAUX O; HAMBSCH Franz-Josef; HANAPPE F.; MEZENTSEVAH Z.; TELEZHNIKOVCH S.

    2015-01-01

    Experimental neutron angular distributions are investigated in the spontaneous fission process of 252Cf. The CORA experiment, presented in this paper, has the aim to study neutron angular correlations in order to elucidate the neutron emission mechanisms in the fission process. The experimental setup is composed by the CODIS fission chamber and the DEMON neutron multidetector. The development of a simulation toolkit based on GEANT4 and ROOT adopted as strategy to investigate the emission of t...

  19. General Description of Fission Observables: GEF Model Code

    Science.gov (United States)

    Schmidt, K.-H.; Jurado, B.; Amouroux, C.; Schmitt, C.

    2016-01-01

    The GEF ("GEneral description of Fission observables") model code is documented. It describes the observables for spontaneous fission, neutron-induced fission and, more generally, for fission of a compound nucleus from any other entrance channel, with given excitation energy and angular momentum. The GEF model is applicable for a wide range of isotopes from Z = 80 to Z = 112 and beyond, up to excitation energies of about 100 MeV. The results of the GEF model are compared with fission barriers, fission probabilities, fission-fragment mass- and nuclide distributions, isomeric ratios, total kinetic energies, and prompt-neutron and prompt-gamma yields and energy spectra from neutron-induced and spontaneous fission. Derived properties of delayed neutrons and decay heat are also considered. The GEF model is based on a general approach to nuclear fission that explains a great part of the complex appearance of fission observables on the basis of fundamental laws of physics and general properties of microscopic systems and mathematical objects. The topographic theorem is used to estimate the fission-barrier heights from theoretical macroscopic saddle-point and ground-state masses and experimental ground-state masses. Motivated by the theoretically predicted early localisation of nucleonic wave functions in a necked-in shape, the properties of the relevant fragment shells are extracted. These are used to determine the depths and the widths of the fission valleys corresponding to the different fission channels and to describe the fission-fragment distributions and deformations at scission by a statistical approach. A modified composite nuclear-level-density formula is proposed. It respects some features in the superfluid regime that are in accordance with new experimental findings and with theoretical expectations. These are a constant-temperature behaviour that is consistent with a considerably increased heat capacity and an increased pairing condensation energy that is

  20. Nuclear Forensics and Radiochemistry: Fission

    Energy Technology Data Exchange (ETDEWEB)

    Rundberg, Robert S. [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

    2017-11-07

    Radiochemistry has been used to study fission since it’ discovery. Radiochemical methods are used to determine cumulative mass yields. These measurements have led to the two-mode fission hypothesis to model the neutron energy dependence of fission product yields. Fission product yields can be used for the nuclear forensics of nuclear explosions. The mass yield curve depends on both the fuel and the neutron spectrum of a device. Recent studies have shown that the nuclear structure of the compound nucleus can affect the mass yield distribution.

  1. Micro plate fission chamber development

    International Nuclear Information System (INIS)

    Wang Mei; Wen Zhongwei; Lin Jufang; Jiang Li; Liu Rong; Wang Dalun

    2014-01-01

    To conduct the measurement of neutron flux and the fission rate distribution at several position in assemblies, the micro plate fission chamber was designed and fabricated. Since the requirement of smaller volume and less structure material was taken into consideration, it is convinient, commercial and practical to use fission chamber to measure neutron flux in specific condition. In this paper, the structure of fission chamber and process of fabrication were introduced and performance test result was presented. The detection efficiency is 91.7%. (authors)

  2. New K isomers in the neutron-rich N =100 isotones 162Sm, 163Eu, and 164Gd

    Science.gov (United States)

    Yokoyama, R.; Go, S.; Kameda, D.; Kubo, T.; Inabe, N.; Fukuda, N.; Takeda, H.; Suzuki, H.; Yoshida, K.; Kusaka, K.; Tanaka, K.; Yanagisawa, Y.; Ohtake, M.; Sato, H.; Shimizu, Y.; Baba, H.; Kurokawa, M.; Nishimura, D.; Ohnishi, T.; Iwasa, N.; Chiba, A.; Yamada, T.; Ideguchi, E.; Fujii, T.; Nishibata, H.; Ieki, K.; Murai, D.; Momota, S.; Sato, Y.; Hwang, J. W.; Kim, S.; Tarasov, O. B.; Morrissey, D. J.; Sherrill, B. M.; Simpson, G.; Praharaj, C. R.

    2017-03-01

    Very neutron-rich Z ˜60 isotopes produced by in-flight fission of a 345 MeV/nucleon 238U beam at the RI Beam Factory, RIKEN Nishina Center, have been studied by delayed γ -ray spectroscopy. New isomers were discovered in the neutron-rich N =100 isotones 162Sm, 163Eu, and 164Gd. Half-lives, γ -ray energies, and relative intensities of these isomers were obtained. Level schemes were proposed for these nuclei and the first 2+ and 4+ states were assigned for the even-even nuclei. The first 2+ and 4+ state energies decrease as the proton numbers get smaller. The energies and the half-lives of the new isomers are very similar to those of 4- isomers known in less neutron-rich N =100 isotones 168Er and 170Yb. A deformed Hartree-Fock with angular momentum projection model suggests Kπ=4- two-quasiparticle states with ν 7 /2 [633 ]⊗ν 1 /2 [521 ] configurations with similar excitation energy. The results suggest that neutron-rich N =100 nuclei are well deformed and the deformation gets larger as Z decreases to 62. The onset of K isomers with the same configuration at almost the same energy in N =100 isotones indicates that the neutron single-particle structures of neutron-rich isotones down to Z =62 do not change significantly from those of the Z =70 stable nuclei. Systematics of the excitation energies of new isomers can be explained without the predicted N =100 shell gap.

  3. phthalocyanine Positional Isomers for Non-linear O

    African Journals Online (AJOL)

    not observed for all isomers as the localization of these chemical shifts are also highly influenced by aggregation. 3.2. Electronic Absorption Spectroscopy, Magnetic Circular. Dichroism ... oxygen atom for the four regio isomers. When comparing the optimized energies of the isomers, no significant difference was observed.

  4. A New Measurement of Neutron Induced Fission Cross Sections

    Science.gov (United States)

    Magee, Joshua; Niffte Collaboration

    2017-09-01

    Neutron induced fission cross sections of actinides are of great interest in nuclear energy and stockpile stewardship. Traditionally, measurements of these cross sections have been made with fission chambers, which provide limited information on the actual fragments, and ultimately result in uncertainties on the order of several percent. The Neutron Induced Fission ragment Tracking Experiment (NIFFTE) collaboration designed and built a fission Time Projection Chamber (fissionTPC), which provides additional information on these processes, through 3-dimensional tracking, improved particle identification, and in-situ profiles of target and beam non-uniformities. Ultimately, this should provide sub-percent measurements of (n,f) cross-sections. During the 2016 run cycle, measurements of the 238U(n,f)/235U(n,f) cross section shape was performed at the Los Alamos Neutron Science Center (LANSCE) Weapons Neutron Research (WNR) facility. An overview of the fission TPC will be given, as well as these recently reported results. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

  5. Neutron angular distribution in plutonium-240 spontaneous fission

    Science.gov (United States)

    Marcath, Matthew J.; Shin, Tony H.; Clarke, Shaun D.; Peerani, Paolo; Pozzi, Sara A.

    2016-09-01

    Nuclear safeguards applications require accurate fission models that exhibit prompt neutron anisotropy. In the laboratory reference frame, an anisotropic neutron angular distribution is observed because prompt fission neutrons carry momentum from fully accelerated fission fragments. A liquid organic scintillation detector array was used with pulse shape discrimination techniques to produce neutron-neutron cross-correlation time distributions and angular distributions from spontaneous fission in a 252Cf, a 0.84 g 240Pueff metal, and a 1.63 g 240Pueff metal sample. The effect of cross-talk, estimated with MCNPX-PoliMi simulations, is removed from neutron-neutron coincidences as a function of the angle between detector pairs. Fewer coincidences were observed at detector angles near 90°, relative to higher and lower detector angles. As light output threshold increases, the observed anisotropy increases due to spectral effects arising from fission fragment momentum transfer to emitted neutrons. Stronger anisotropy was observed in Cf-252 spontaneous fission prompt neutrons than in Pu-240 neutrons.

  6. Tip model of cold fission

    International Nuclear Information System (INIS)

    Goennenwein, F.; Boersig, B.

    1991-01-01

    Cold fission is defined to be the limiting case of nuclear fission where virtually all of the available energy is converted into the total kinetic energy of the fragments. The fragments have, therefore, to be born in or at least close to their respective ground states. Starting from the viewpoint that cold fission corresponds to most compact scission configurations, energy constraints have been exploited to calculate minimum tip distances between the two nascent fragments in binary fission. Crucial input parameters to this tip model of cold fission are the ground-state deformations of fragment nuclei. It is shown that the minimum tip distances being compatible with energy conservation vary strongly with both the mass and charge fragmentation of the fission prone nucleus. The tip distances refer to nuclei with equivalent sharp surfaces. In keeping with the size of the surface width of leptodermous nuclei, only configurations where the tip distances are smaller than a few fm may be considered as valid scission configurations. From a comparison with experimental data on cold fission this critical tip distance appears to be 3.0 fm for the model parameters chosen. Whenever the model calculation yields tip distances being smaller than the critical value, a necessary condition for attaining cold fission is considered to be fulfilled. It is shown that this criterion allows to understand in fair agreement with experiment which mass fragmentations are susceptible to lead to cold fission and which fragment-charge divisions are the most favored in each isobaric mass chain. Being based merely on energy arguments, the model cannot aim at predicting fragment yields in cold fission. However, the tip model proposed appears well suited to delineate the phase space where cold fission phenomena may come into sight. (orig.)

  7. Post-scission fission theory: Neutron emission in fission

    International Nuclear Information System (INIS)

    Madland, D.G.

    1997-01-01

    A survey of theoretical representations of two of the observables in neutron emission in fission is given, namely, the prompt fission neutron spectrum N (E) and the average prompt neutron multiplicity bar ν p . Early representations of the two observables are presented and their deficiencies are discussed. This is followed by summaries and examples of recent theoretical models for the calculation of these quantities. Emphasis is placed upon the predictability and accuracy of the recent models. In particular, the dependencies of N (E) and bar ν p upon the fissioning nucleus and its excitation energy are treated. Recent work in the calculation of the prompt fission neutron spectrum matrix N (E, E n ), where E n is the energy of the neutron inducing fission, is then discussed. Concluding remarks address the current status of our ability to calculate these observables with confidence, the direction of future theoretical efforts, and limitations to current (and future) approaches

  8. Mass distribution of fission fragments within the Born-Oppenheimer approximation

    Science.gov (United States)

    Pomorski, K.; Ivanyuk, F. A.; Nerlo-Pomorska, B.

    2017-03-01

    The fission fragments mass-yield of 236 U is obtained by an approximate solution of the eigenvalue problem of the collective Hamiltonian that describes the dynamics of the fission process whose degrees of freedom are: the fission (elongation), the neck and mass-asymmetry modes. The macroscopic-microscopic method is used to evaluate the potential energy surface. The macroscopic energy part is calculated using the liquid drop model and the microscopic corrections are obtained using a Woods-Saxon single-particle levels. The four-dimensional modified Cassini ovals shape parametrization is used to describe the shape of the fissioning nucleus. The mass tensor is taken within a cranking-type approximation. The final fragment mass distribution is obtained by weighting the adiabatic density distribution in the collective space with the neck-dependent fission probability. The neck degree of freedom is found to play a significant role in determining the final fragment mass distribution.

  9. Fission hindrance and nuclear viscosity

    Indian Academy of Sciences (India)

    viscosity in slowing down the diffusion rate in comparison to the decay rate without vis- cosity predicted by Bohr and ... revived Kramers' dynamical approach to understand nuclear fission at finite temperature and angular momentum. ... tor and (2) a compact seven-element array of BaF2 detectors. The fission fragments were.

  10. Discoveries of isotopes by fission

    Indian Academy of Sciences (India)

    also contributed to the discovery of new isotopes. More recently, most of the very neutron- rich isotopes have been discovered by projectile fission. After a brief summary of the discovery of fission process itself, these production mechanisms will be discussed. The paper concludes with an outlook on future discoveries of ...

  11. Fission throughout the periodic table

    International Nuclear Information System (INIS)

    Moretto, L.G.; Wozniak, G.J.

    1989-04-01

    The dualistic view of fission and evaporation as two distinct compound nucleus processes is substituted with a unified view in which fission, complex fragment emission, and light particle evaporation are seen as different aspects of a single process. 47 refs., 22 figs

  12. Progress in fission product nuclear data

    International Nuclear Information System (INIS)

    Lammer, M.

    1984-09-01

    This is the tenth issue of a report series on Fission Product Data, which informs us about all the activities in this field, which are planned, ongoing, or have recently been completed. The types of activities included are measurements, compilations and evaluations of: fission product yields (neutron induced and spontaneous fission), neutron reaction cross sections of fission products, data related to the radioactive decay of fission products, delayed neutron data of fission products, lumped fission product data (decay heat, absorption, etc.). There is also a section with recent references relative to fission product nuclear data

  13. Industrial use of fission products

    International Nuclear Information System (INIS)

    Silverman, J.

    1989-01-01

    Perhaps the most disappointing and surprising development in the fifty year history of nuclear fission is the small role fission products play in modern technology. As a large and potentially inexpensive source of ionizing radiation, fission products were expected to offer major practical benefits. The attractive opportunities stimulated imaginative efforts to realize their fulfillment, but their direct impact has been minor. Fission products have not fared well, not only in somewhat indirect competition with nonradioactive alternatives, but also in direct competition with other radiation sources, especially electron accelerators and 60 Co. There is one major triumph for fission product technology: the application of 99 Mo and its daughter 99m Tc as an almost universal tracer system in nuclear medicine

  14. Mechanisms of fission neutron emission

    International Nuclear Information System (INIS)

    Maerten, H.

    1991-01-01

    The time evolution in fission is the starting point for discussing not only the main mechanism of fission neutron emission, the evaporation from fully accelerated fragments, but also possible secondary ones connected with dynamical features of nuclear fission. ''Asymptotic'' conditions as relevant for describing the particle release from highly excited, rapidly moving fragments are defined. Corresponding statistical model approaches to fission neutron emission, based on the adequate consideration of the intricate fragment occurrence probability, reproduce most of the experimental data. The remarkable influence of fission modes on neutron observables is analyzed in the framework of a macroscopic-microscopic scission point model consistent with energy conservation. Finally, chances and deficiencies for solving the mechanism puzzle are summarized. (author). 87 refs, 21 figs

  15. Ternary fission and cluster radioactivities

    CERN Document Server

    Poenaru, D N; Greiner, W; Gherghescu, R A; Hamilton, J H; Ramayya, A V

    2002-01-01

    Ternary fission yield for different kinds of light particle accompanied fission processes is compared to the Q-values for the corresponding cold phenomena, showing a striking correlation. The experimental evidence for the existence of a quasimolecular state in sup 1 sup 0 Be accompanied fission of sup 2 sup 5 sup 2 Cf may be explained using a three-center phenomenological model which generates a third minimum in the deformation energy at a separation distance very close to the touching point. This model is a natural extension of the unified approach to three groups of binary decay modes (cold fission, cluster radioactivities and alpha decay), illustrated by sup 2 sup 3 sup 4 U decay modes, and the alpha valley on the potential energy surfaces of sup 1 sup 0 sup 6 Te. New measurements of cluster decay modes, confirming earlier predictions within analytical superasymmetric fission model, are included in a comprehensive half-life systematics. (authors)

  16. Fission dynamics with microscopic level densities

    Science.gov (United States)

    Randrup, Jørgen; Ward, Daniel; Carlsson, Gillis; Døssing, Thomas; Möller, Peter; Åberg, Sven

    2018-03-01

    Working within the Langevin framework of nuclear shape dynamics, we study the dependence of the evolution on the degree of excitation. As the excitation energy of the fissioning system is increased, the pairing correlations and the shell effects diminish and the effective potential-energy surface becomes ever more liquid-drop like. This feature can be included in the treatment in a formally well-founded manner by using the local level densities as a basis for the shape evolution. This is particularly easy to understand and implement in the Metropolis treatment where the evolution is simulated by means of a random walk on the five-dimensional lattice of shapes for which the potential energy has been tabulated. Because the individual steps between two neighboring lattice sites are decided on the basis of the ratio of the statistical weights, what is needed is the ratio of the local level densities for those shapes, evaluated at the associated local excitation energies. For this purpose, we adapt a recently developed combinatorial method for calculating level densities which employs the same single-particle levels as those that were used for the calculation of the pairing and shell contributions to the macroscopic-microscopic deformation-energy surface. For each nucleus under consideration, the level density (for a fixed total angular momentum) is calculated microscopically for each of the over five million shapes given in the three-quadratic-surface parametrization. This novel treatment, which introduces no new parameters, is illustrated for the fission fragment mass distributions for selected uranium and plutonium cases.

  17. Systematics of fission cross sections at the intermediate energy region

    Energy Technology Data Exchange (ETDEWEB)

    Fukahori, Tokio; Chiba, Satoshi [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment

    1997-03-01

    The systematics was obtained with fitting experimental data for proton induced fission cross sections of Ag, {sup 181}Ta, {sup 197}Au, {sup 206,207,208}Pb, {sup 209}Bi, {sup 232}Th, {sup 233,235,238}U, {sup 237}Np and {sup 239}Pu above 20 MeV. The low energy cross section of actinoid nuclei is omitted from systematics study, since the cross section has a complicated shape and strongly depends on characteristic of nucleus. The fission cross sections calculated by the systematics are in good agreement with experimental data. (author)

  18. Fission fragment angular distribution in heavy ion induced fission

    Directory of Open Access Journals (Sweden)

    S. Soheyli

    2006-06-01

    Full Text Available   We have calculated the fission fragment angular anisotropy for 16O + 232Th,12C + 236U , 11B + 237 Np , 14 N + 232 Th , 11B + 235U , 12C + 232Th systems with the saddle point statistical model and compared the fission fragment angular anisotropy for these systems. This comparison was done with two methods a without neutron correction and b with neutron correction. Also we studied normal and anomalous behavior of the fission fragment angular anisotropy. Finally, we have predicted the average emitted neutron from compound nuclei considering the best fit for each system.

  19. Fission fragment angular distribution in heavy ion induced fission

    OpenAIRE

    S. Soheyli; I. Ziaeian

    2006-01-01

      We have calculated the fission fragment angular anisotropy for 16O + 232Th,12C + 236U , 11B + 237 Np , 14 N + 232 Th , 11B + 235U , 12C + 232Th systems with the saddle point statistical model and compared the fission fragment angular anisotropy for these systems. This comparison was done with two methods a) without neutron correction and b) with neutron correction. Also we studied normal and anomalous behavior of the fission fragment angular anisotropy. Finally, we have predicted the averag...

  20. Dynamical excitation in fission

    International Nuclear Information System (INIS)

    Ledergerber, T.; Paltiel, Z.; Fraenkel, Z.; Pauli, H.C.

    1976-01-01

    The excitation mechanism of the fission process is studied in terms of a model of particles moving in a deformed time-dependent potential. A residual interaction of the pairing type is incoporated by means of the BCS approximation. Only 2-quasi-particle excitations up to some cutoff energy are included. The separation of the total excitation energy into intrinsic and translational parts is made at the scission point. The present calculations for 240 Pu show that, in the framework of this model, most of the available energy at scission is transformed into intrinsic excitation energy. However the convergence of the calculated value for the cutoff energy is unsatisfactory and hence a description in terms of a better model space is needed. The fact that very many channels are involved suggests that a statistical treatment may be useful. (author)

  1. The spectroscopy of fission fragments

    International Nuclear Information System (INIS)

    Phillips, W.R.

    1998-01-01

    High-resolution measurements on γ rays from fission fragments have provided a rich source of information, unobtainable at the moment in any other way, on the spectroscopy of neutron-rich nuclei. In recent years important data have been obtained on the yrast- and near yrast-structure of neutron-rich fission fragments. We discuss the scope of measurements which can be made on prompt gamma rays from secondary fission fragments, the techniques used in the experiments and some results recently obtained. (author)

  2. The spectroscopy of fission fragments

    Energy Technology Data Exchange (ETDEWEB)

    Phillips, W.R. [Department of Physics and Astronomy, University of Manchester, Manchester, M13 9PL (United Kingdom); Collaboration: La Direction des Sciences de la Matiere du CEA (FR); Le Fonds National de la Recherche Scientifique de Belgique (BE)

    1998-12-31

    High-resolution measurements on {gamma} rays from fission fragments have provided a rich source of information, unobtainable at the moment in any other way, on the spectroscopy of neutron-rich nuclei. In recent years important data have been obtained on the yrast- and near yrast-structure of neutron-rich fission fragments. We discuss the scope of measurements which can be made on prompt gamma rays from secondary fission fragments, the techniques used in the experiments and some results recently obtained. (author) 24 refs., 8 figs., 1 tab.

  3. The ever-growing complexity of the mitochondrial fission machinery.

    Science.gov (United States)

    Pagliuso, Alessandro; Cossart, Pascale; Stavru, Fabrizia

    2018-02-01

    The mitochondrial network constantly changes and remodels its shape to face the cellular energy demand. In human cells, mitochondrial fusion is regulated by the large, evolutionarily conserved GTPases Mfn1 and Mfn2, which are embedded in the mitochondrial outer membrane, and by OPA1, embedded in the mitochondrial inner membrane. In contrast, the soluble dynamin-related GTPase Drp1 is recruited from the cytosol to mitochondria and is key to mitochondrial fission. A number of new players have been recently involved in Drp1-dependent mitochondrial fission, ranging from large cellular structures such as the ER and the cytoskeleton to the surprising involvement of the endocytic dynamin 2 in the terminal abscission step. Here we review the recent findings that have expanded the mechanistic model for the mitochondrial fission process in human cells and highlight open questions.

  4. Toroidal high-spin isomers in the nucleus 304120

    Science.gov (United States)

    Staszczak, A.; Wong, Cheuk-Yin; Kosior, A.

    2017-05-01

    Background: Strongly deformed oblate superheavy nuclei form an intriguing region where the toroidal nuclear structures may bifurcate from the oblate spheroidal shape. The bifurcation may be facilitated when the nucleus is endowed with a large angular moment about the symmetry axis with I =Iz . The toroidal high-K isomeric states at their local energy minima can be theoretically predicted using the cranked self-consistent Skyrme-Hartree-Fock method. Purpose: We use the cranked Skyrme-Hartree-Fock method to predict the properties of the toroidal high-spin isomers in the superheavy nucleus 120304184. Method: Our method consists of three steps: First, we use the deformation-constrained Skyrme-Hartree-Fock-Bogoliubov approach to search for the nuclear density distributions with toroidal shapes. Next, using these toroidal distributions as starting configurations, we apply an additional cranking constraint of a large angular momentum I =Iz about the symmetry z axis and search for the energy minima of the system as a function of the deformation. In the last step, if a local energy minimum with I =Iz is found, we perform at this point the cranked symmetry- and deformation-unconstrained Skyrme-Hartree-Fock calculations to locate a stable toroidal high-spin isomeric state in free convergence. Results: We have theoretically located two toroidal high-spin isomeric states of 120304184 with an angular momentum I =Iz=81 ℏ (proton 2p-2h, neutron 4p-4h excitation) and I =Iz=208 ℏ (proton 5p-5h, neutron 8p-8h) at the quadrupole moment deformations Q20=-297.7 b and Q20=-300.8 b with energies 79.2 and 101.6 MeV above the spherical ground state, respectively. The nuclear density distributions of the toroidal high-spin isomers 120304184(Iz=81 ℏ and 208 ℏ ) have the maximum density close to the nuclear matter density, 0.16 fm-3, and a torus major to minor radius aspect ratio R /d =3.25 . Conclusions: We demonstrate that aligned angular momenta of Iz=81 ℏ and 208 ℏ arising from

  5. A new approach to barrier-top fission dynamics

    Directory of Open Access Journals (Sweden)

    Bertsch G.F.

    2016-01-01

    Full Text Available We proposed a calculational framework for describing induced fission that avoids the Bohr-Wheeler assumption of well-defined fission channels. The building blocks of our approach are configurations that form a discrete, orthogonal basis and can be characterized by both energy and shape. The dynamics is to be determined by interaction matrix elements between the states rather than by a Hill-Wheeler construction of a collective coordinate. Within our approach, several simple limits can be seen: diffusion; quantized conductance; and ordinary decay through channels. The specific proposal for the discrete basis is to use the Kπ quantum numbers of the axially symmetric Hartree-Fock approximation to generate the configurations. Fission paths would be determined by hopping from configuration to configuration via the residual interaction. We show as an example the configurations needed to describe a fictitious fission decay 32S → 16 O + 16 O. We also examine the geometry of the path for fission of 236U, measuring distances by the number of jumps needed to go to a new Kπ partition.

  6. Isomer Energy Source for Space Propulsion Systems

    Science.gov (United States)

    2004-03-01

    absorbed during formation is reradiated, but in rare situations, such as with this hafnium isomer, “large differences between the spins of the isomeric...The ROVER & NERVA program generated a proven reactor design that was actually slated for a mission to Mars after the U.S. successfully landed on the...1.380 Sm Lanthanide 7.353 1,345 0.133 Hf Transition Metal 13.31 2,506 0.230 HfC Ceramic 12.2 4,173 ? Ta Transition Metal 16.65 3,290 0.575 TaC

  7. Multicomponent adsorption of hexane isomers in MOFs

    OpenAIRE

    Bárcia, Patrick da Silva; Silva, José A.C.; Rodrigues, A.E.

    2010-01-01

    We have performed a set of screening studies for quaternary mixtures of hexane isomers n-hexane (nHEX), 3-methylpentane (3MP), 2,3-dimethylbutane (23DMB) and 2,2-dimethylbutane (22DMB) in two porous rigid MOFs (figure 1). First, the chromium trimesate MIL-100(Cr),1 which possesses mesoporous cages accessible through 5-9 Å microporous windows, and secondly the zirconium terephthalate UiO-66,2 which exhibits a 3D microporous (5-10 Å) pore system. The temperature range 323-423 K and partial pres...

  8. Shape coexistence in the lightest Tl isotopes studied by laser spectroscopy

    CERN Multimedia

    Herfurth, F; Antalic, S; Darby, I G; Venhart, M; Flanagan, K; Veselsky, M; Blaum, K; Radulov, D P; Beck, D; Kowalska, M; Schwarz, S; Chapman, R; Diriken, J V J; Lane, J; Rosenbusch, M

    This proposal aims at atomic spectroscopy studies of the very neutron-deficient isotopes $^{178-187}$Tl, at and far beyond the region of the neutron mid-shell at N=104, in which shape coexistence phenomena were investigated so far by particle and $\\gamma$-ray spectroscopy methods only. Our motivation for this proposal is as follows : \\\\\\\\ -These studies will provide direct data on magnetic dipole moment, spin, charge radii and deformations of these isotopes. The results will form a stringent test for our current understanding of the shape coexistence phenomena in the vicinity of the neutron mid-shell at N=104, where the relevant effects are expected to be the strongest (cf.shape staggering in the isotopes $^{181,183,185}$Hg). \\\\-The knowledge of the structure (configuration, spin, deformation) and whether one or two $\\beta$-decaying isomers are present in the parent isotopes $^{178,180,182}$Tl are crucial for understanding of the results of our recent studies of $\\beta$-delayed fission in the lightest thalli...

  9. Physics and chemistry of fission

    International Nuclear Information System (INIS)

    1979-01-01

    Full text: In the pleasant and hospitable atmosphere of the Kernforschungsanlage Juelich in the Federal Republic of Germany, the IAEA symposium on the Physics and Chemistry of Fission took place. Almost 200 scientists attended, 154 abstracts were submitted, and 57 papers presented, but more important than the numbers was the quality of the contributions and the progress reported at the symposium. The neutron was discovered almost 50 years ago; 40 years ago the idea of nuclear fission was born. Since then, a number of laboratories have worked hard to explain the phenomenon of fission One would expect that by now scientists would know exactly what happens in a nucleus before and during the process of fission, particularly as there are hundreds of power and research reactors in operation, and fission of uranium isotopes is the basis of their functioning. At first glance, fission seems a simple process: a neutron hits and penetrates the uranium nucleus which becomes excited, i.e. has a surplus of energy. One way to get rid of this energy is for the nucleus to split into two parts; additional products of this process are energy and more neutrons. Nature, however, seems to dislike such straightforward explanations. In the case of fission, scientists have observed a number of phenomena which disagree with a simple model. Sometimes, a nucleus will split into two parts without being 'attacked' by a neutron; this spontaneous fission opens up a new line of fission research and several contributions at the symposium reported on sophisticated experiments designed to unravel some of its specific details. Sometimes, a fissioning nucleus will emit another particle: ternary fission has become a powerful tool for studying the properties of nuclei during the fission process. For the scientist, it is fascinating to observe how the nucleus behaves during fission. They invent models which are supposed to reproduce the most probable course of events leading to fission. In one of these

  10. International handling of fissionable material

    International Nuclear Information System (INIS)

    1975-01-01

    The opinion of the ministry for foreign affairs on international handling of fissionable materials is given. As an introduction a survey is given of the possibilities to produce nuclear weapons from materials used in or produced by power reactors. Principles for international control of fissionable materials are given. International agreements against proliferation of nuclear weapons are surveyed and methods to improve them are proposed. (K.K.)

  11. The interstellar chemistry of H2C3O isomers.

    Science.gov (United States)

    Loison, Jean-Christophe; Agúndez, Marcelino; Marcelino, Núria; Wakelam, Valentine; Hickson, Kevin M; Cernicharo, José; Gerin, Maryvonne; Roueff, Evelyne; Guélin, Michel

    2016-03-11

    We present the detection of two H 2 C 3 O isomers, propynal and cyclopropenone, toward various starless cores and molecular clouds, together with upper limits for the third isomer propadienone. We review the processes controlling the abundances of H 2 C 3 O isomers in interstellar media showing that the reactions involved are gas-phase ones. We show that the abundances of these species are controlled by kinetic rather than thermodynamic effects.

  12. Isomer-specific degradation of branched and linear 4-nonylphenol isomers in an oxic soil.

    Science.gov (United States)

    Shan, Jun; Jiang, Bingqi; Yu, Bin; Li, Chengliang; Sun, Yuanyuan; Guo, Hongyan; Wu, Jichun; Klumpp, Erwin; Schäffer, Andreas; Ji, Rong

    2011-10-01

    Using (14)C- and (13)C-ring-labeling, degradation of five p-nonylphenol (4-NP) isomers including four branched (4-NP(38), 4-NP(65), 4-NP(111), and 4-NP(112)) and one linear (4-NP(1)) isomers in a rice paddy soil was studied under oxic conditions. Degradation followed an availability-adjusted first-order kinetics with the decreasing order of half-life 4-NP(111) (10.3 days) > 4-NP(112) (8.4 days) > 4-NP(65) (5.8 days) > 4-NP(38) (2.1 days) > 4-NP(1) (1.4 days), which is in agreement with the order of their reported estrogenicities. One metabolite of 4-NP(111) with less polarity than the parent compound occurred rapidly and remained stable in the soil. At the end of incubation (58 days), bound residues of 4-NP(111) amounted to 54% of the initially applied radioactivity and resided almost exclusively in the humin fraction of soil organic matter, in which chemically humin-bound residues increased over incubation. Our results indicate an increase of specific estrogenicity of the remaining 4-NPs in soil as a result of the isomer-specific degradation and therefore underline the importance of understanding the individual fate (including degradation, metabolism, and bound-residue formation) of isomers for risk assessment of 4-NPs in soil. 4-NP(1) should not be used as a representative of 4-NPs for studies on their environmental behavior.

  13. Radiochemistry and the Study of Fission

    Energy Technology Data Exchange (ETDEWEB)

    Rundberg, Robert S. [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

    2016-11-14

    These are slides from a lecture given at UC Berkeley. Radiochemistry has been used to study fission since its discovery. Radiochemical methods are used to determine cumulative mass yields. These measurements have led to the two-mode fission hypothesis to model the neutron energy dependence of fission product yields. Fission product yields can be used for the nuclear forensics of nuclear explosions. The mass yield curve depends on both the fuel and the neutron spectrum of a device. Recent studies have shown that the nuclear structure of the compound nucleus can affect the mass yield distribution. The following topics are covered: In the beginning: the discovery of fission; forensics using fission products: what can be learned from fission products, definitions of R-values and Q-values, fission bases, K-factors and fission chambers, limitations; the neutron energy dependence of the mass yield distribution (the two mode fission hypothesis); the influence of nuclear structure on the mass yield distribution. In summary: Radiochemistry has been used to study fission since its discovery. Radiochemical measurement of fission product yields have provided the highest precision data for developing fission models and for nuclear forensics. The two-mode fission hypothesis provides a description of the neutron energy dependence of the mass yield curve. However, data is still rather sparse and more work is needed near second and third chance fission. Radiochemical measurements have provided evidence for the importance of nuclear states in the compound nucleus in predicting the mass yield curve in the resonance region.

  14. Radiochemistry and the Study of Fission

    International Nuclear Information System (INIS)

    Rundberg, Robert S.

    2016-01-01

    These are slides from a lecture given at UC Berkeley. Radiochemistry has been used to study fission since its discovery. Radiochemical methods are used to determine cumulative mass yields. These measurements have led to the two-mode fission hypothesis to model the neutron energy dependence of fission product yields. Fission product yields can be used for the nuclear forensics of nuclear explosions. The mass yield curve depends on both the fuel and the neutron spectrum of a device. Recent studies have shown that the nuclear structure of the compound nucleus can affect the mass yield distribution. The following topics are covered: In the beginning: the discovery of fission; forensics using fission products: what can be learned from fission products, definitions of R-values and Q-values, fission bases, K-factors and fission chambers, limitations; the neutron energy dependence of the mass yield distribution (the two mode fission hypothesis); the influence of nuclear structure on the mass yield distribution. In summary: Radiochemistry has been used to study fission since its discovery. Radiochemical measurement of fission product yields have provided the highest precision data for developing fission models and for nuclear forensics. The two-mode fission hypothesis provides a description of the neutron energy dependence of the mass yield curve. However, data is still rather sparse and more work is needed near second and third chance fission. Radiochemical measurements have provided evidence for the importance of nuclear states in the compound nucleus in predicting the mass yield curve in the resonance region.

  15. New information on the T1/2=47 s isomer in the 136I nucleus

    International Nuclear Information System (INIS)

    Urban, W.; Rzaca-Urban, T.; Saha Sarkar, M.; Sarkar, S.; Durell, J.L.; Smith, A.G.; Genevey, J.A.; Pinston, J.A.; Simpson, G.S.; Ahmad, I.

    2006-01-01

    The 136 I nucleus, populated in the spontaneous fission of 248 Cm, was studied by means of prompt γ-ray spectroscopy using the EUROGAM2 array. The observation in this work of the 42.6 keV prompt-γ, M1+E2 transition de-exciting the 7 - level in 136 I indicates that this level, interpreted as the (πg 7/2 3 νf 7/2 ) 7- configuration, does not correspond to the T=47 s, β-decaying isomer in 136 I. The isomer is placed 42.6 keV below the 7 - level. It has spin 6 - and is interpreted as the (πg 7/2 2 d 5/2 νf 7/2 ) 6- configuration. This and other members of both multiplets can be reproduced properly only if one assumes that the πd 5/2 orbital in 136 I is located 400keV lower than in 133 Sb. Possible mechanisms causing this effect are discussed. (orig.)

  16. Fission fragment angular distributions and fission cross section validation

    International Nuclear Information System (INIS)

    Leong, Lou Sai

    2013-01-01

    The present knowledge of angular distributions of neutron-induced fission is limited to a maximal energy of 15 MeV, with large discrepancies around 14 MeV. Only 238 U and 232 Th have been investigated up to 100 MeV in a single experiment. The n-TOF Collaboration performed the fission cross section measurement of several actinides ( 232 Th, 235 U, 238 U, 234 U, 237 Np) at the n-TOF facility using an experimental set-up made of Parallel Plate Avalanche Counters (PPAC), extending the energy domain of the incident neutron above hundreds of MeV. The method based on the detection of the 2 fragments in coincidence allowed to clearly disentangle the fission reactions among other types of reactions occurring in the spallation domain. I will show the methods we used to reconstruct the full angular resolution by the tracking of fission fragments. Below 10 MeV our results are consistent with existing data. For example in the case of 232 Th, below 10 MeV the results show clearly the variation occurring at the first (1 MeV) and second (7 MeV) chance fission, corresponding to transition states of given J and K (total spin and its projection on the fission axis), and a much more accurate energy dependence at the 3. chance threshold (14 MeV) has been obtained. In the spallation domain, above 30 MeV we confirm the high anisotropy revealed in 232 Th by the single existing data set. I'll discuss the implications of this finding, related to the low anisotropy exhibited in proton-induced fission. I also explore the critical experiments which is valuable checks of nuclear data. The 237 Np neutron-induced fission cross section has recently been measured in a large energy range (from eV to GeV) at the n-TOF facility at CERN. When compared to previous measurements, the n-TOF fission cross section appears to be higher by 5-7 % beyond the fission threshold. To check the relevance of n-TOF data, we simulate a criticality experiment performed at Los Alamos with a 6 kg sphere of 237 Np. This

  17. Simultaneous measurement of neutron-induced fission and capture cross sections for 241Am at neutron energies below fission threshold

    Science.gov (United States)

    Hirose, K.; Nishio, K.; Makii, H.; Nishinaka, I.; Ota, S.; Nagayama, T.; Tamura, N.; Goto, S.; Andreyev, A. N.; Vermeulen, M. J.; Gillespie, S.; Barton, C.; Kimura, A.; Harada, H.; Meigo, S.; Chiba, S.; Ohtsuki, T.

    2017-06-01

    Fission and capture reactions were simultaneously measured in the neutron-induced reactions of 241Am at the spallation neutron facility of the Japan Proton Accelerator Research Complex (J-PARC). Data for the neutron energy range of En=0.1-20 eV were taken with the TOF method. The fission events were observed by detecting prompt neutrons accompanied by fission using liquid organic scintillators. The capture reaction was measured by detecting γ rays emitted in the deexcitation of the compound nuclei using the same detectors, where the prompt fission neutrons and capture γ rays were separated by a pulse shape analysis. The cross sections were obtained by normalizing the relative yields at the first resonance to evaluations or other experimental data. The ratio of the fission to capture cross sections at each resonance is compared with those from an evaluated nuclear data library and other experimental data. Some differences were found between the present values and the library/literature values at several resonances.

  18. Status of fission power

    International Nuclear Information System (INIS)

    Levenson, M.

    1977-01-01

    Fission energy is reviewed from the viewpoints of technology, economics, politics, manufacturers, consumers, and foreign countries. Technically, the reactor program is operating and the light water reactor industry shows signs of maturing, although recent business has been disappointing. Marketing of gas-cooled reactors depends, not on technical, but economic and political issues. Liquid metal fast breeder reactors have been demonstrated worldwide, while the gas-cooled fast breeder remains an undemonstrated option. Nuclear plants, currently costing the same as coal plants with scrubbers, are the cheapest option for utilities because most of the cost is imbedded. The defeat of nuclear initiatives in seven states indicates that public feeling is not as anti-nuclear as opponents to nuclear power claim. The harshness of last winter demonstrated the advantages of a power source that is not so sensitive to the weather for reliable operation and transport, as well as low cost energy. Other nations are proceeding to build a nuclear capability, which the U.S. may jeopardize because of concerns about the fuel cycle, nuclear waste disposal, uranium reserves, and nuclear proliferation

  19. Theoretical approaches to the emission of α particles during nuclear fission

    International Nuclear Information System (INIS)

    Carjan, N.

    1986-05-01

    Recent models as well as new trajectory calculations used to interpret the experimental data on α-accompanied fission are presented and experimental hints towards the emission mechanism are pointed out. The important question of the distribution of the emission points and moments is brought up: are these particles coming only from the region between the fragments (the neck) or, are they coming with comparable probability, from any point of the surface of the fissioning system and: are they emitted just at scission or at any sufficiently deformed stage of the fission process. The simultaneous division of the nucleus into three fragments (the true ternary fission) is discussed in terms of the dynamical liquid-drop model. It is suggested that this process occurs in the tail (corresponding to overelongated shapes) of the distribution of the fission probability in the multidimensional space of the collective coordinates

  20. Fragment Angular Distributions in Neutron-Induced Fission of w235U and 239Pu using a Time Projection Chamber

    Science.gov (United States)

    Kleinrath, Verena

    2014-09-01

    Fission fragment angular distributions can lend insights into fission barrier shapes and level densities at the scission point, both important for fission theory development. Fragment emission anisotropies are also valuable for precision cross section ratio measurements, if the distributions are different for the two isotopes used in the ratio. Available angular data is sparse for 235U and even more so for 239Pu, especially at neutron energies above 5 MeV. The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) time projection chamber, which enables precise tracking of charged particles, can be used to study angular distributions and emission anisotropies of fission fragments in neutron-induced fission. Analysis of in-beam data collected at the Los Alamos Neutron Science Center with a 239Pu/235U target will provide angular distributions as a function of incident neutron energy for these isotopes. Preliminary angular distributions for 235U and 239Pu using the NIFFTE time projection chamber will be presented. Fission fragment angular distributions can lend insights into fission barrier shapes and level densities at the scission point, both important for fission theory development. Fragment emission anisotropies are also valuable for precision cross section ratio measurements, if the distributions are different for the two isotopes used in the ratio. Available angular data is sparse for 235U and even more so for 239Pu, especially at neutron energies above 5 MeV. The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) time projection chamber, which enables precise tracking of charged particles, can be used to study angular distributions and emission anisotropies of fission fragments in neutron-induced fission. Analysis of in-beam data collected at the Los Alamos Neutron Science Center with a 239Pu/235U target will provide angular distributions as a function of incident neutron energy for these isotopes. Preliminary angular distributions for 235U and

  1. Patchouli alkohol isomers pogostemon herba predicted virtually

    Directory of Open Access Journals (Sweden)

    Sentot Joko Raharjo

    2014-02-01

    Full Text Available The aim of our research is predicting the alpha-patchouli alcohol isomer Pogostemon Herba as inhibitors cyclooxygenase (COX-1 and COX-2 isoenzymes. The data for the alpha-patchouli alcohol isomer (CD521903, CD442384, and/or CD6432585 Pogostemon Herba were explored from the pubchem database. Molecular interaction studies with COX-1 and COX-2 from mouse were done using the molecular docking tools Hex 6.12 and LeadIT2 Bisolve. The analysis of the alpha-patchouli alcohol compounds of patchouli oil showed that alpha-Patchouli alcohol (CD521903 binds to COX-1 at active sites including: LEU223B, ASP228B, LEU237B, ARG 332B, TRP 138A, GLU 139A, SER 142A, ASN 143A, and the interaction to COX-2 at active site including: GLN 289B, GLU 290B, ARG 222B, LYS 211B, THR 212B, HIS 214B, ASN 382B, HEM682B, GLN 454B, HIS 386B, TRP 387B, HIS 388B, VAL 274B, GLN 203B, VAL 291B, VAL 295B. The interaction hydrogen bond energy between alpha-patchouli alcohol: (CD521903-COX-1 complexes (-4 kJ/mol and CD521903-COX-2 complexes (-8 kJ/ mol by LeadIT2 Biosolve. This suggests alpha-patchouli alcohol CD521903 as candidate for a selective COX-2 inhibitor. These in silico data need further analyses of biological function activity

  2. Advances on fission chamber modelling

    International Nuclear Information System (INIS)

    Filliatre, Philippe; Jammes, Christian; Geslot, Benoit; Veenhof, Rob

    2013-06-01

    In-vessel, online neutron flux measurements are routinely performed in mock-up and material testing reactors by fission chambers. Those measurements have a wide range of applications, including characterization of experimental conditions, reactor monitoring and safety. Depending on the application, detectors may experience a wide range of constraints, of several magnitudes, in term of neutron flux, gamma-ray flux, temperature. Hence, designing a specific fission chamber and measuring chain for a given application is a demanding task. It can be achieved by a combination of experimental feedback and simulating tools, the latter being based on a comprehensive understanding of the underlying physics. A computation route that simulates fission chambers, named CHESTER, is presented. The retrieved quantities of interest are the neutron-induced charge spectrum, the electronic and ionic pulses, the mean current and variance, the power spectrum. It relies on the GARFIELD suite, originally developed for drift chambers, and makes use of the MAGBOLTZ code to assess the drift parameters of electrons within the filling gas, and the SRIM code to evaluate the stopping range of fission products. The effect of the gamma flux is also estimated. Computations made with several fission chambers exemplify the possibilities of the route. A good qualitative agreement is obtained when comparing the results with the experimental data available to date. In a near future, a comprehensive experimental programme will be undertaken to qualify the route using the known neutron sources, mock-up reactors and wide choice of fission chambers, with a stress on the predictiveness of the Campbelling mode. Depending on the results, a refinement of the modelling and an effort on the accuracy of input data are also to be considered. CHESTER will then make it possible to predict the overall sensitivity of a chamber, and to optimize the design for a given application. Another benefit will be to increase the

  3. The measurement of prompt neutron spectrum in spontaneous fission of {sup 244}Cm

    Energy Technology Data Exchange (ETDEWEB)

    Batenkov, O.I.; Boykov, G.S.; Drapchinsky, L.V.; Majorov, M.Ju.; Trenkin, V.A. [V.G. Khlopin Radium Inst., Saint Petersburg (Russian Federation)

    1997-03-01

    Under the Program of Measurements of Prompt Fission Neutron Spectra of Minor Actinides for Transmutation Purposes the integral neutron spectrum in spontaneous fission of {sup 244}Cm has been measured by the time-of-flight method in the energy range of 0.1-15 MeV relative to the standard neutron spectrum in {sup 252}Cf spontaneous fission. Essential attention was paid to revealing of possible systematic errors. It is shown, that the {sup 244}Cm spectrum shape may be well described by using Mannhart evaluation with appropriate parameter of Maxwell temperature T{sub M} = 1.37 MeV. (author)

  4. Contribution to the study of nuclear fission

    International Nuclear Information System (INIS)

    Serot, O.

    2009-09-01

    The author proposes an overview of his research activity during the past fifteen years and more particularly that dealing with nuclear fission. The first part reports works on nucleus physics at the scission via the investigation of ternary fission (experimental procedure, influence of fission modes, influence of resonance spin, influence of excitation energy of the fissioning nucleus, emission probabilities, energy spectra of ternary alphas and tritons, emission mechanism). The second part reports measurements and assessments of neutron-induced fission cross sections. The third part reports the investigation of some properties of fission products (efficiencies, branching ratios of the main delayed neutron precursors)

  5. The latest progress of fission track analysis

    International Nuclear Information System (INIS)

    Wang Shicheng

    1996-01-01

    Fission track analysis as a new nuclear track technique is based on fission track annealing in mineral and is used for oil and gas exploration successfully. The west part of China is the main exploration for oil and gas. The oil and gas basins there experienced much more complicated thermal history and higher paleotemperature. In order to apply fission track analysis to these basins, following work was be carried out: 1. The decomposition of grain age distribution of zircon fission tracks. 2. Study on thermal history of Ordos basin using zircon fission track analysis. 3. The fission track study on the Qiang Tang basin in tibet

  6. Search for isomers in nuclei near N = 50

    International Nuclear Information System (INIS)

    Taras, P.; Haas, B.; Merdinger, J.C.; Styczen, J.

    1979-01-01

    Targets of sup (58, 60, 61, 62, 64) Ni, Co, and Cu have been bombarded with 42 MeV 16 O beams. Several isomers were produced but no new isomer was found, in particular in 74 Kr which is expected to be a good candidate for yrast traps in the N = 50 region. (author)

  7. Stereospecific Synthesis of the Geometrical Isomers of a Natural Product

    Science.gov (United States)

    Grove, T.; DiLella, D.; Volker, E.

    2006-01-01

    Stereospecific synthesis of a geometrical isomer is not a common topic for the introductory organic chemistry laboratory. We have developed and tested an experiment for the synthesis of (Z) and (E) isomers that has been performed successfully by undergraduate students. The experiment is presented to the students as a puzzle in which they must…

  8. Simultaneous Determination of Two Isomers of Asarone in Piper ...

    African Journals Online (AJOL)

    Purpose: To develop a rapid and reliable reverse phase high performance liquid chromatography (RP-. HPLC) method to quantify the two isomers of asarones in P. sarmentosum extracts using two different columns under similar analytical conditions. Methods: Two isomers, α- and β-asarone, were analyzed using two types ...

  9. Anaerobic Degradation of Lindane and Other HCH Isomers

    NARCIS (Netherlands)

    Mehboob, F.; Langenhoff, A.A.M.; Schraa, G.; Stams, A.J.M.

    2013-01-01

    Lindane (¿-HCH) is a pesticide that has mainly been used in agriculture. Lindane and the other HCH isomers are highly chlorinated hydrocarbons. The presence of a large number of electron withdrawing chlorine groups makes some of the HCH isomers rather recalcitrant in oxic environments. Especially

  10. Thorium-uranium fission radiography

    Science.gov (United States)

    Haines, E. L.; Weiss, J. R.; Burnett, D. S.; Woolum, D. S.

    1976-01-01

    Results are described for studies designed to develop routine methods for in-situ measurement of the abundance of Th and U on a microscale in heterogeneous samples, especially rocks, using the secondary high-energy neutron flux developed when the 650 MeV proton beam of an accelerator is stopped in a 42 x 42 cm diam Cu cylinder. Irradiations were performed at three different locations in a rabbit tube in the beam stop area, and thick metal foils of Bi, Th, and natural U as well as polished silicate glasses of known U and Th contents were used as targets and were placed in contact with mica which served as a fission track detector. In many cases both bare and Cd-covered detectors were exposed. The exposed mica samples were etched in 48% HF and the fission tracks counted by conventional transmitted light microscopy. Relative fission cross sections are examined, along with absolute Th track production rates, interaction tracks, and a comparison of measured and calculated fission rates. The practicality of fast neutron radiography revealed by experiments to data is discussed primarily for Th/U measurements, and mixtures of other fissionable nuclei are briefly considered.

  11. Dynamical description of the fission process using the TD-BCS theory

    Energy Technology Data Exchange (ETDEWEB)

    Scamps, Guillaume, E-mail: scamps@nucl.phys.tohoku.ac.jp [Department of Physics, Tohoku University, Sendai 980-8578 (Japan); Simenel, Cédric [Department of Nuclear Physics, Research School of Physics and Engineering Australian National University, Canberra, Australian Capital Territory 2601 (Australia); Lacroix, Denis [Institut de Physique Nucléaire, IN2P3-CNRS, Université Paris-Sud, F-91406 Orsay Cedex (France)

    2015-10-15

    The description of fission remains a challenge for nuclear microscopic theories. The time-dependent Hartree-Fock approach with BCS pairing is applied to study the last stage of the fission process. A good agreement is found for the one-body observables: the total kinetic energy and the average mass asymmetry. The non-physical dependence of two-body observables with the initial shape is discussed.

  12. Change over from compound nuclear fission to quasi-fission

    International Nuclear Information System (INIS)

    Ghosh, T. K.; Banerjee, K.; Bhattacharya, C.; Bhattacharya, S.; Kundu, S.; Meena, J. K.; Mukherjee, G.; Mukhopadhyay, S.; Rana, T. K.; Golda, K. S.; Bhattacharya, P.

    2010-01-01

    Fission fragment mass distribution has been measured from the decay of 246 Bk nucleus populating via two entrance channels with slight difference in mass asymmetries but belonging on either side of the Businaro Gallone mass asymmetry parameter. Both the target nuclei were deformed. Near the Coulomb barrier, at similar excitation energies the width of the fission fragment mass distribution was found to be drastically different for the 14 N+ 232 Th reaction compared to the 11 B+ 235 U reaction. The entrance channel mass asymmetry was found to affect the fusion process sharply. (authors)

  13. Change over from compound nuclear fission to quasi-fission

    Directory of Open Access Journals (Sweden)

    Bhattacharya P.

    2010-03-01

    Full Text Available Fission fragment mass distribution has been measured in two reactions to populate compound nucleus 246Bk. Both the target nuclei were deformed. However, entrance channel mass asymmetry of the two systems was on the either side of the Businaro Gallone mass asymmetry parameter. Near the Coulomb barrier, at similar excitation energies, the width of the fission fragment mass distribution was found to be significantly different for the 14N+232Th reaction compared to the 11B+235U reaction. The entrance channel mass asymmetry was found to play a significant role in deciding the fusion process.

  14. Nuclear fission and neutron-induced fission cross-sections

    CERN Document Server

    James, G D; Michaudon, A; Michaudon, A; Cierjacks, S W; Chrien, R E

    2013-01-01

    Nuclear Fission and Neutron-Induced Fission Cross-Sections is the first volume in a series on Neutron Physics and Nuclear Data in Science and Technology. This volume serves the purpose of providing a thorough description of the many facets of neutron physics in different fields of nuclear applications. This book also attempts to bridge the communication gap between experts involved in the experimental and theoretical studies of nuclear properties and those involved in the technological applications of nuclear data. This publication will be invaluable to those interested in studying nuclear fis

  15. Complete Hexose Isomer Identification with Mass Spectrometry

    Science.gov (United States)

    Nagy, Gabe; Pohl, Nicola L. B.

    2015-04-01

    The first analytical method is presented for the identification and absolute configuration determination of all 24 aldohexose and 2-ketohexose isomers, including the D and L enantiomers for allose, altrose, galactose, glucose, gulose, idose, mannose, talose, fructose, psicose, sorbose, and tagatose. Two unique fixed ligand kinetic method combinations were discovered to create significant enough energetic differences to achieve chiral discrimination among all 24 hexoses. Each of these 24 hexoses yields unique ratios of a specific pair of fragment ions that allows for simultaneous determination of identification and absolute configuration. This mass spectrometric-based methodology can be readily employed for accurate identification of any isolated monosaccharide from an unknown biological source. This work provides a key step towards the goal of complete de novo carbohydrate analysis.

  16. Nuclear structure in cold rearrangement processes in fission and fusion

    Energy Technology Data Exchange (ETDEWEB)

    Armbruster, P.

    1998-11-01

    In fission and fusion of heavy nuclei large numbers of nucleons are rearranged at a scale of excitation energy very small compared to the binding energy of the nuclei. The energies involved are less than 40 MeV at nuclear temperatures below 1.5 MeV. The shapes of the configurations in the rearrangement of a binary system into a monosystem in fusion, or vice versa in fission, change their elongations by as much as 8 fm, the radius of the monosystem. The dynamics of the reactions macroscopically described by a potential energy surface, inertia parameters, dissipation, and a collision energy is strongly modified by the nuclear structure of the participating nuclei. Experiments showing nuclear structure effects in fusion and fission of the heaviest nuclei are reviewed. The reaction kinematics and the multitude of isotopes involved are investigated by detector techniques and by recoil spectrometers. The advancement of the latter allows to find very small reaction branches in the range of 10{sup -5} to 10{sup -10}. The experiments reveal nuclear structure effects in all stages of the rearrangement processes. These are discussed pointing to analogies in fusion and fission on the microscopic scale, notwithstanding that both processes macroscopically are irreversible. Heavy clusters, as 132Sn, 208Pb, nuclei with closed shell configurations N=82,126, Z=50,82 survive in large parts of the nuclear rearrangement. They determine the asymmetry in the mass distribution of low energy fission, and they allow to synthesise superheavy elements, until now up to element 112. Experiments on the cold rearrangement in fission and fusion are presented. Here, in the range of excitation energies below 12 MeV the phenomena are observed most convincingly. (orig.)

  17. Identification of isomers of organometallic compounds

    International Nuclear Information System (INIS)

    Mbue, Sona Peter; Cho, Kwang Hwi

    2015-01-01

    The yaChI is a newly suggested chemical naming system. However, yaChI is a derivative of the IUPAC InChI with a modified algorithm that includes additional layers of chemical structure information. Consequently, yaChI string contains more structure details while preserving the original structure file information and can distinctively identify very closely related compounds reducing the chances of ambiguity in chemical compound databases as opposed to the general SMILES, InChI, and InChIKey. This study examines the relative performances of yaChI, SMILES, InChI, and InChIKey in duplication check for isomers. For simplicity, a small data set of 28 organometallic compounds (structural isomers of Rh-containing compounds) subdivided into three major groups (A, B, and C) based on the number and the type of ligands attached to the center atom was used to study the performances of each encoding scheme in describing chemical structures. SMILES, InChI, and InChIKey were generated using Openbabel and RDkit, whereas yaChI strings were generated with in-house program. Strings generated from SMILES, InChI, and InChIKey though different, resulted to only three unique chemical identifiers, with each belonging to one group indicating the presence of only three unique compounds in the study data. However, yaChI results depicted that all structures in each group are indeed unique and differ among themselves as well as those from other groups, mapping each structure with a unique identifier given a total number of 28 unique structures in the study data. This high perception of yaChI probe justifies its accuracy and reliability in duplication check among closely related compounds especially structures exhibiting stereo properties

  18. Control system for a small fission reactor

    Science.gov (United States)

    Burelbach, J.P.; Kann, W.J.; Saiveau, J.G.

    1985-02-08

    A system for controlling the reactivity of a small fission reactor includes an elongated, flexible hollow tube in the general form of a helical coiled spring axially positioned around and outside of the reactor vessel in an annular space between the reactor vessel and a surrounding cylindrical-shaped neutron reflector. A neutron absorbing material is provided within the hollow tube with the rate of the reaction controlled by the extension and compression of the hollow tube, e.g., extension of the tube increases reactivity while its compression reduces reactivity, in varying the amount of neutron absorbing material disposed between the reactor vessel and the neutron reflector. Conventional mechanical displacement means may be employed to control the coil density of the hollow tube as desired.

  19. Shape coexistence in 153Ho

    Science.gov (United States)

    Pramanik, Dibyadyuti; Sarkar, S.; Saha Sarkar, M.; Bisoi, Abhijit; Ray, Sudatta; Dasgupta, Shinjinee; Chakraborty, A.; Krishichayan, Kshetri, Ritesh; Ray, Indrani; Ganguly, S.; Pradhan, M. K.; Ray Basu, M.; Raut, R.; Ganguly, G.; Ghugre, S. S.; Sinha, A. K.; Basu, S. K.; Bhattacharya, S.; Mukherjee, A.; Banerjee, P.; Goswami, A.

    2016-08-01

    The high-spin states in 153Ho have been studied by the La57(20Ne139,6 n ) reaction at a projectile energy of 139 MeV at the Variable Energy Cyclotron Centre (VECC), Kolkata, India, utilizing an earlier campaign of the Indian National Gamma Array (INGA) setup. Data from γ -γ coincidence, directional correlation, and polarization measurements have been analyzed to assign and confirm the spins and parities of the levels. We have suggested a few additions and revisions of the reported level scheme of 153Ho. The RF-γ time difference spectra have been useful to confirm the half-life of an isomer in this nucleus. From the comparison of experimental and theoretical results, it is found that there are definite indications of shape coexistence in this nucleus. The experimental and calculated lifetimes of several isomers have been compared to follow the coexistence and evolution of shape with increasing spin.

  20. Fission barriers from multidimensionally-constrained covariant density functional theories

    Directory of Open Access Journals (Sweden)

    Lu Bing-Nan

    2017-01-01

    Full Text Available In recent years, we have developed the multidimensionally-constrained covariant density functional theories (MDC-CDFTs in which both axial and spatial reflection symmetries are broken and all shape degrees of freedom described by βλμ with even μ, such as β20, β22, β30, β32, β40, etc., are included self-consistently. The MDC-CDFTs have been applied to the investigation of potential energy surfaces and fission barriers of actinide nuclei, third minima in potential energy surfaces of light actinides, shapes and potential energy surfaces of superheavy nuclei, octupole correlations between multiple chiral doublet bands in 78Br, octupole correlations in Ba isotopes, the Y32 correlations in N = 150 isotones and Zr isotopes, the spontaneous fission of Fm isotopes, and shapes of hypernuclei. In this contribution we present the formalism of MDC-CDFTs and the application of these theories to the study of fission barriers and potential energy surfaces of actinide nuclei.

  1. NEACRP thermal fission product benchmark

    International Nuclear Information System (INIS)

    Halsall, M.J.; Taubman, C.J.

    1989-09-01

    The objective of the thermal fission product benchmark was to compare the range of fission product data in use at the present time. A simple homogeneous problem was set with 200 atoms H/1 atom U235, to be burnt up to 1000 days and then decay for 1000 days. The problem was repeated with 200 atoms H/1 atom Pu239, 20 atoms H/1 atom U235 and 20 atoms H/1 atom Pu239. There were ten participants and the submissions received are detailed in this report. (author)

  2. Search for Singlet Fission Chromophores

    Energy Technology Data Exchange (ETDEWEB)

    Havlas, Z.; Akdag, A.; Smith, M. B.; Dron, P.; Johnson, J. C.; Nozik, A. J.; Michl, J.

    2012-01-01

    Singlet fission, in which a singlet excited chromophore shares its energy with a ground-state neighbor and both end up in their triplet states, is of potential interest for solar cells. Only a handful of compounds, mostly alternant hydrocarbons, are known to perform efficiently. In view of the large number of conditions that a successful candidate for a practical cell has to meet, it appears desirable to extend the present list of high performers to additional classes of compounds. We have (i) identified design rules for new singlet fission chromophores and for their coupling to covalent dimers, (ii) synthesized them, and (iii) evaluated their performance as neat solids or covalent dimers.

  3. Collective spectra along the fission barrier

    OpenAIRE

    Pigni M. T.; Andreev A. V.; Shneidman T. M.; Massimi C.; Vannini G.; Ventura A.

    2012-01-01

    Discrete and continuous spectra of fissioning nuclei at the humps of fission barriers (Bohr transition states) and in the intermediate wells (superdeformed and hyperdeformed states) play a key role in the calculation of fission cross sections. A theoretical evaluation of the collective parts of the spectra is possible within the framework of the dinuclear system model, which treats the wave function of the fissioning nucleus as a superposition of a mononucleus configuration and two–cluster co...

  4. Infrared Spectroscopy of Two Isomers of the OCS-CS_{2} Complex

    Science.gov (United States)

    Oliaee, J. N.; Dehghany, M.; Afshari, Mahin; Moazzen-Ahmadi, N.; McKellar, A. R. W.

    2009-06-01

    A second isomer of OCS-CS_{2} complex, with a nonplanar cross-shaped structure, has been studied for the first time by analysing an infrared band in the region of the OCS stretching vibration (2062 cm^{-1}). This isomer has C_{s} symmetry and the observed band consists of purely c-type rotational transitions. The ground state rotational parameters are found to be A=0.07306 cm^{-1}, B=0.03325 cm^{-1} and C=0.02879 cm^{-1}, in good agreement with a previous semi-empirical calculation. In addition, a hybrid band with a- and b-type rotational transitions has been assigned to be due to the known planar form of OCS-CS_{2}, as previously studied by microwave spectroscopy. The spectra were recorded using a rapid-scan tunable diode laser spectrometer to probe a pulsed supersonic jet expansion. Calculations indicate that the planar isomer of OCS-CS_{2} is the lowest in energy, in contrast to CO_{2}-CS_{2} where the crossed form is believed to be the lowest. J. J. Newby, M. M. Serafin, R. A. Peebles and S. A. Peebles, Phys. Chem. Chem. Phys. 7, 487 (2005). C. C. Dutton, D. A. Dows, R. Eikey, S. Evans and R. A. Beaudet, J. Phys. Chem. A 102, 6904 (1998).

  5. Selectivity of Brij-35 in Micellar Liquid Chromatographic Separation of Positional Isomers

    Directory of Open Access Journals (Sweden)

    Najma Memon

    2012-01-01

    Full Text Available Implementation of Brij-35, a nonionic surfactant, as a mobile phase for separation of positional isomers is investigated. Chromolith C-18 SpeedROD is used as a stationary phase. The effect of surfactant and organic modifier (propanol concentration on the separation of some selected isomers is studied and evaluated in terms of linear solvation energy relationship (LSER. Shape selectivity is assessed by α value of sorbic and benzoic acid, which is found to be 1.339 by using mobile phase composed of 0.5% aqueous solutions of Brij-35 and propanol in 9 : 1. Isomers of parabens, nitroanilines, nitrophenols, and quinolinols are successfully separated using mobile phases composed of various percentages of surfactant and propanol. System constants for nonionic MLC using LSER analysis show that hydrogen bond basicity and dipolarity may be major contributors to selectivity, while excess molar refraction helps fine-tuning the separation which also imparts unique selectivity to nonionic surfactants as compared to ionic ones.

  6. Charged particle-induced nuclear fission reactions – Progress and ...

    Indian Academy of Sciences (India)

    progress made in recent years and the prospects in the area of nuclear fission research will be the focus of this review. Keywords. Nuclear fission; charged particle-induced fission; heavy ions; fission angular distribu- tions; mass distributions; fission barrier; moment of inertia; shell effect in fission. PACS Nos 25.70.Jj; 25.85.

  7. Measurement of fission anisotropy for Ta

    Indian Academy of Sciences (India)

    F on many actinide targets with large deformations exhibit dramatic increase with decreasing energy [5]. In order to understand the data, an admixture of non compound reaction processes, like the fast fission, the quasifission with orientation dependence and the preequilibrium fission, is introduced as a source of fission like ...

  8. Fission fragment mass and angular distributions

    Indian Academy of Sciences (India)

    2015-07-22

    Jul 22, 2015 ... Synthesis of heavy and superheavy elements is severely hindered by fission and fission-like processes. The probability of these fission-like, non-equilibrium processes strongly depends on the entrance channel parameters. This article attempts to summarize the recent experimental findings and classify the ...

  9. Fission yield data evaluation system FYDES

    International Nuclear Information System (INIS)

    Liu Tingjin

    1998-01-01

    Taking account of some features of fission yield data, to do the fission yield data evaluation conveniently, a fission yield data evaluation system FYDES has been developed for last two years. Outline of the system, data retrieval and data table standardization, data correction codes, data averaging code, simultaneous evaluation code and data fit programs were introduced

  10. Charged particle-induced nuclear fission reactions

    Indian Academy of Sciences (India)

    The nuclear fission phenomenon continues to be an enigma, even after nearly 75 years of its discovery. Considerable progress has been made towards understanding the fission process. Both light projectiles and heavy ions have been employed to investigate nuclear fission. An extensive database of the properties of ...

  11. Proton induced fission of {sup 232}Th at intermediate energies

    Energy Technology Data Exchange (ETDEWEB)

    Gikal, K. B., E-mail: kgikal@mail.ru; Kozulin, E. M.; Bogachev, A. A. [JINR, Flerov Laboratory of Nuclear Reactions (Russian Federation); Burtebaev, N. T.; Edomskiy, A. V. [Institute of Nuclear Physics of Ministry of Energy of the Republic of Kazakhstan (Kazakhstan); Itkis, I. M.; Itkis, M. G.; Knyazhev, G. N. [JINR, Flerov Laboratory of Nuclear Reactions (Russian Federation); Kovalchuk, K. V.; Kvochkina, T. N. [Institute of Nuclear Physics of Ministry of Energy of the Republic of Kazakhstan (Kazakhstan); Piasecki, E. [Heavy Ion Laboratory of Warsaw University (Poland); Rubchenya, V. A. [University of Jyväskylä, Department of Physics (Finland); Sahiev, S. K. [Institute of Nuclear Physics of Ministry of Energy of the Republic of Kazakhstan (Kazakhstan); Trzaska, W. H. [University of Jyväskylä, Department of Physics (Finland); Vardaci, E. [INFN Napoli, Dipartimento di Scienze Fisiche dell’Università di Napoli (Italy)

    2016-12-15

    The mass-energy distributions and cross sections of proton-induced fission of {sup 232}Th have been measured at the proton energies of 7, 10, 13, 20, 40, and 55 MeV. Experiments were carried out at the proton beam of the K-130 cyclotron of the JYFL Accelerator Laboratory of the University of Jyväskylä and U-150m cyclotron of the Institute of Nuclear Physics, Ministry of Energy of the Republic of Kazakhstan. The yields of fission fragments in the mass range A = 60–170 a.m.u. have been measured up to the level of 10−4%. The three humped shape of the mass distribution up has been observed at higher proton energies. The contribution of the symmetric component grows up with increasing proton incident energy; although even at 55 MeV of proton energy the shoulders in the mass energy distribution clearly indicate the asymmetric fission peaks. Evolution of shell structure was observed in the fission fragment mass distributions even at high excitation energy.

  12. Fission of pancreatic islets during postnatal growth of the mouse.

    Science.gov (United States)

    Seymour, Philip A; Bennett, William R; Slack, Jonathan M W

    2004-02-01

    A cell composition analysis was made of the pancreatic islets in postnatal H253 mice. This line has a lacZ insertion on the X chromosome so that in female hemizygotes 50% of cells should be positive for beta-galactosidase and 50% negative. Immediately after birth, the islets were of a heterogeneous cell composition. However, by 4 weeks some islets have become homogeneous. This suggests that islets progress towards monoclonality in a similar way to the intestinal crypts and stomach gastric glands. Pancreatic islets may therefore represent 'structural proliferative units' in the overall histological organization of the pancreas. Reduction of genetic heterogeneity might arise from cell turnover, fission of islets or both. Analysis of the cell composition of the X-inactivation mosaic mice also provides the first clear evidence for islet fission in pancreatic development. Irregularly shaped islets resembling dumb-bells, with a characteristic neck of alpha-cells, were observed with decreasing frequency with increasing age. Three-dimensional reconstruction confirmed their resemblance to conjoined islets. The cell composition analysis showed: (1) the relatedness of the two sides of a dumb-bell islet is significantly higher than between two non-dumb-bell islets and (2) the relatedness of two randomly selected islets decreases as the distance between them increases. This suggests that dumb-bell islets are in a state of fission rather than fusion, and that islet fission is a mode of islet production in the postnatal pancreas.

  13. Revealing hidden regularities with a general approach to fission

    Energy Technology Data Exchange (ETDEWEB)

    Schmidt, Karl-Heinz; Jurado, Beatriz [Chemin du Solarium, CENBG, CNRS/IN2P3, B. P. 120, Gradignan (France)

    2015-12-15

    Selected aspects of a general approach to nuclear fission are described with the focus on the possible benefit of meeting the increasing need of nuclear data for the existing and future emerging nuclear applications. The most prominent features of this approach are the evolution of quantum-mechanical wave functions in systems with complex shape, memory effects in the dynamics of stochastic processes, the influence of the Second Law of thermodynamics on the evolution of open systems in terms of statistical mechanics, and the topological properties of a continuous function in multi-dimensional space. It is demonstrated that this approach allows reproducing the measured fission barriers and the observed properties of the fission fragments and prompt neutrons. Our approach is based on sound physical concepts, as demonstrated by the fact that practically all the parameters have a physical meaning, and reveals a high degree of regularity in the fission observables. Therefore, we expect a good predictive power within the region extending from Po isotopes to Sg isotopes where the model parameters have been adjusted. Our approach can be extended to other regions provided that there is enough empirical information available that allows determining appropriate values of the model parameters. Possibilities for combining this general approach with microscopic models are suggested. These are supposed to enhance the predictive power of the general approach and to help improving or adjusting the microscopic models. This could be a way to overcome the present difficulties for producing evaluations with the required accuracy. (orig.)

  14. Yield of Radionuclides and Isomers Measured in Fragmentation of the ^{nat}W and ^{186}W (97%) Targets with Protons at 630, 420 and 270 MeV

    CERN Document Server

    Karamian, S A; Chaloun, P; Filossofov, D V; Henzl, V; Henzlova, D; Kalinnikov, V G; Korolev, N A; Lebedev, N A; Novgorodov, A F; Collins, C B; Popescu, I I; Ur, C A

    2004-01-01

    Yields and cross sections of the radioactive nuclide formation have been measured via induced activity gamma-spectra after irradiation of the natural composition W and enriched ^{186)W targets at Dubna synchrocyclotron. Spallation and fission products have been represented among the detected nuclides. The high-spin isomers of Hf and Lu were produced and the isomer-to-ground state ratios could be estimated. The nuclide yields have also been calculated using the LAHET code at 6 values of proton energy in the range from 100 to 800 MeV both for ^{nat)W and for enriched ^{186)W targets. Measured isotope yields are generally in agreement with the calculations, however, the code is incapable to predict the isomer-to-ground state ratios. In experiment, it has been shown that the ^{177m}Lu, ^{178m2}Hf and ^{179m2}Hf high-spin isomers are produced with 2.5 times higher yield in the 97% enriched ^{186)W target as compared to the ^{nat)W target at identical irradiations. This makes significance for the creation of high-a...

  15. Spontaneous fission of superheavy nuclei

    Indian Academy of Sciences (India)

    collaborators [1,2]. The importance of deformed valleys in the potential energy surfaces. (PES) is that they provide the most favoured fission channels for the decay of superheavy nuclei. For the dynamics study, one has to introduce the influence of mass tensor. We use the results from pairing calculations for the occupation ...

  16. Fission hindrance and nuclear viscosity

    Indian Academy of Sciences (India)

    of fission in terms of the ratio of transition states at the saddle point to the level density ... It was also intended to probe any turning over or reduction of γ .... 4. Summary and discussion. In this contribution we have reviewed our measurements which were carried out to inves- tigate the dependence of nuclear viscosity ...

  17. Spontaneous fission of superheavy nuclei

    Indian Academy of Sciences (India)

    2015-08-02

    Aug 2, 2015 ... The macroscopic–microscopic method is extended to calculate the deformation energy and penetrability for binary nuclear configurations typical for fission processes. The deformed two-centre shell model is used to obtain single-particle energy levels for the transition region of two partially overlapped ...

  18. Spontaneous fission of superheavy nuclei

    Indian Academy of Sciences (India)

    the Yukawa-plus-exponential potential. The microscopic shell and pairing corrections are obtained using the Strutinsky and BCS approaches and the cranking formulae yield the inertia tensor. Finally, the WKB method is used to calculate penetrabilities and spontaneous fission half-lives. Calculations are performed for the ...

  19. Spontaneous fission of superheavy nuclei

    Indian Academy of Sciences (India)

    2015-08-02

    Aug 2, 2015 ... ... nuclear configurations typical for fission processes. The deformed two-centre shell model is used to obtain single-particle energy levels for the transition region of two partially overlapped daughter and emitted fragment nuclei. The macroscopic part is obtained using the Yukawa-plus-exponential potential.

  20. Spin determination of fission resonances

    International Nuclear Information System (INIS)

    Keyworth, G.A.

    1976-01-01

    The present status of available information on the channel quantum numbers for resonance fission and the most urgently needed additional experiments are examined. The role of spin in the 235 U + n system is emphasized. The discussion relies heavily on recent alignment measurements and polarization results

  1. Fission approach to cluster radioactivity

    Indian Academy of Sciences (India)

    2015-08-04

    Aug 4, 2015 ... Also, the analytical superasymmetric fission (ASAF) model is successfully employed to make a systematic search and to predict, with other models, cluster ... those of the staff, the journals, various programmes, and Current Science, has changed from 'ias.ernet.in' (or 'academy.ias.ernet.in') to 'ias.ac.in'. Thus ...

  2. Nuclear fission with inertial confinement

    CERN Document Server

    Koshkarev, D G

    2002-01-01

    The possibility of initiating the explosive fission reaction in a small quantity of fissile material through the heavy ions beam from the powerful accelerator-driver, developed for realization of the thermonuclear synthesis in the deuterium-tritium cylindrical targets with the direct ignition, is considered. The consequences of applying this method in the nuclear engineering are discussed

  3. Proton radioactivity: the case for 53m Co proton-emitter isomer

    International Nuclear Information System (INIS)

    Tavares, O.A.P.; Medeiros, E.L.

    2010-01-01

    The partial proton emission half-life for 53m Co unstable isomer is re-examined in the framework of a semiempirical model based on tunneling through a Coulomb-plus centrifugal- plus-overlapping potential barrier within the spherical nucleus approximation. It is shown that the known measured half-life value of 17 s is compatible with a large prolate shape for 53m Co proton emitter and a high angular momentum ι = 11 assigned to the proton transition to the ground-state of 52 Fe. (author)

  4. Properties of neutron-rich hafnium high-spin isomers

    CERN Multimedia

    Tungate, G; Walker, P M; Neyens, G; Billowes, J; Flanagan, K; Koester, U H; Litvinov, Y

    It is proposed to study highly-excited multi-quasiparticle isomers in neutron-rich hafnium (Z=72) isotopes. Long half-lives have already been measured for such isomers in the storage ring at GSI, ensuring their accessibility with ISOL production. The present proposal focuses on:\\\\ (i) an on-line experiment to measure isomer properties in $^{183}$Hf and $^{184}$Hf, and\\\\ (ii) an off-line molecular breakup test using REXTRAP, to provide Hf$^{+}$ beams for future laser spectroscopy and greater sensitivity for the future study of more neutron-rich isotopes.

  5. Increasing Diversity of Biological Membrane Fission Mechanisms.

    Science.gov (United States)

    Renard, Henri-François; Johannes, Ludger; Morsomme, Pierre

    2018-01-04

    Membrane fission is essential to life. It is required for many fundamental cellular processes, as diverse as cyto- and karyokinesis, organelle division, membrane repair, and membrane trafficking and endocytosis. While membrane fission was originally seen as resulting from the action of mechanoenzymes such as dynamin, it is clear that the reality is more complex. In this review, we propose an updated overview of fission mechanisms, and try to extract essential requirements for each. We also present examples of cellular processes that involve these fission mechanisms. Finally, we list pending questions, whether they are specific to a peculiar fission mechanism or more general to the field. Copyright © 2017 Elsevier Ltd. All rights reserved.

  6. Heavy-ion induced fission reactions

    International Nuclear Information System (INIS)

    Britt, H.C.; Fowler, M.M.; Fraenkel, Z.; Gavron, A.; Plicht, J.; Wilhelmy, J.B.; Plasil, F.; Awes, T.; Young, G.

    1983-01-01

    Heavy-ion induced fission reactions are investigated. The problem of obtaining a representative set of fission-cross section data, so that it would be possible to test both the mass and angular momentum dependence of fission barriers in the mass region 150 9 Be through 64 Ni. The experimental data clearly show the qualitative effects of angular momentum, excitation energy and fissility on the fission cross section. They provide an ideal testing ground for theoretical models of fission in this mass region

  7. Analysis of fission product behavior in the Saclay Spitfire Loop Test SSL-1. [HTGR

    Energy Technology Data Exchange (ETDEWEB)

    Jensen, D.D.; Haire, M.J.; Ballagny, A.

    1978-02-01

    The behavior of the fission metal cesium and the fission gases krypton and xenon in the Saclay Spitfire Loop SSL-1 test has been compared to that predicted using General Atomic reference data and computer code models. This is the first in a series of analyses planned in order to provide quantitative validation of HTGR fission product design methods. In this analysis, the first attempt to rigorously verify fission product design methods, the FIPERQ code was used to model the diffusion of cesium graphite and release to the coolant stream. The comparisons showed that the cesium profile shape in the graphite web and the partition coefficient between fuel rod matrix material and fuel element graphite were correctly modeled, although the overall release was significantly underpredicted. Uncertainties in the source term (fissile particle failure fraction) and total release to the coolant precluded an accurate appraisal of the validity of FIPERQ. However, several recommendations are presented to improve the applicability of future in-pile test data for the validation of fission metal release codes. The half-life dependence of fission gas release during irradiation was found to be in good agreement with the model used in the reference design materials, providing assurance that this aspect of the fission gas release predictions is properly modeled.

  8. New signatures on dissipation from fission induced by relativistic heavy-ion collisions

    International Nuclear Information System (INIS)

    Jurado, B.; Schmitt, C.; Schmidt, K.H.; Enqvist, T.; Kelic, A.; Rejmund, F.; Benlliure, J.; Junghans, A.R.

    2004-03-01

    Fissile nuclei with small shape distortion relative to the ground-state deformation and with low angular momentum were produced in peripheral heavy-ion collisions. Under the conditions of small shape distortions and low angular momentum, the theoretical description of the fission process can be considerably simplified, and the relevant information on dissipation can be better extracted than in conventional experiments based on fusion-fission reactions. In addition, this experimental approach induces very high excitation energies, a condition necessary to observe transient effects. The experimental data were taken at GSI using a set-up especially conceived for fission studies in inverse kinematics. This set-up allowed determining three observables whose sensitivity to dissipation was investigated for the first time: the total fission cross sections of 238 U at 1 A GeV as a function of the target mass, and, for the reaction of 238 U at 1 A GeV on a (CH 2 ) n target, the partial fission cross sections and the partial charge distributions of the fission fragments. The comparison of the new experimental data with a reaction code adapted to the conditions of the reactions investigated leads to clear conclusions on the strength of dissipation at small deformation where the existing results are rather contradictory. (orig.)

  9. Carotenoids and Their Isomers: Color Pigments in Fruits and Vegetables

    Directory of Open Access Journals (Sweden)

    Yueming Jiang

    2011-02-01

    Full Text Available Fruits and vegetables are colorful pigment-containing food sources. Owing to their nutritional benefits and phytochemicals, they are considered as ‘functional food ingredients’. Carotenoids are some of the most vital colored phytochemicals, occurring as all-trans and cis-isomers, and accounting for the brilliant colors of a variety of fruits and vegetables. Carotenoids extensively studied in this regard include β-carotene, lycopene, lutein and zeaxanthin. Coloration of fruits and vegetables depends on their growth maturity, concentration of carotenoid isomers, and food processing methods. This article focuses more on several carotenoids and their isomers present in different fruits and vegetables along with their concentrations. Carotenoids and their geometric isomers also play an important role in protecting cells from oxidation and cellular damages.

  10. Simultaneous Determination of Two Isomers of Asarone in Piper ...

    African Journals Online (AJOL)

    Simultaneous Determination of Two Isomers of Asarone in Piper sarmentosum Roxburgh (Piperaceae) Extracts using Different Chromatographic Columns. Mohd Shahrul Ridzuan Hamil, Abdul Hakeem Memon, Amin Malik Shah Abdul Majid, Zhari Ismail ...

  11. A fission fragment detector for correlated fission output studies

    Energy Technology Data Exchange (ETDEWEB)

    Mosby, S., E-mail: smosby@lanl.gov [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States); Tovesson, F.; Couture, A. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States); Duke, D.L. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States); Colorado School of Mines, Golden, CO 80401 (United States); Kleinrath, V. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States); Idaho State University, Pocatello, ID 83201 (United States); Meharchand, R.; Meierbachtol, K.; O' Donnell, J.M.; Perdue, B.; Richman, D. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States); Shields, D. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States); Colorado School of Mines, Golden, CO 80401 (United States)

    2014-09-01

    A digital data acquisition system has been combined with a double Frisch gridded ionization chamber for use at both moderated and unmoderated neutron sources at the Los Alamos Neutron Science (LANSCE) facility. The high efficiency of the instrument combined with intense LANSCE beams and new acquisition system permits fission output measurements across 11 orders of magnitude incident neutron energy. The acquisition and analysis system is presented along with the first in-beam performance tests of the setup.

  12. Material synergism fusion-fission

    International Nuclear Information System (INIS)

    Sankara Rao, K.B.; Raj, B.; Cook, I.; Kohyama, A.; Dudarev, S.

    2007-01-01

    In fission and fusion reactors the common features such as operating temperatures and neutron exposures will have the greatest impact on materials performance and component lifetimes. Developing fast neutron irradiation resisting materials is a common issue for both fission and fusion reactors. The high neutron flux levels in both these systems lead to unique materials problems like void swelling, irradiation creep and helium embitterment. Both fission and fusion rely on ferritic-martensitic steels based on 9%Cr compositions for achieving the highest swelling resistance but their creep strength sharply decreases above ∝ 823K. The use of oxide dispersion strengthened (ODS) alloys is envisaged to increase the operating temperature of blanket systems in the fusion reactors and fuel clad tubes in fast breeder reactors. In view of high operating temperatures, cyclic and steady load conditions and the long service life, properties like creep, low cycle fatigue,fracture toughness and creepfatigue interaction are major considerations in the selection of structural materials and design of components for fission and fusion reactors. Currently, materials selection for fusion systems has to be based upon incomplete experimental database on mechanical properties. The usage of fairly well developed databases, in fission programmes on similar materials, is of great help in the initial design of fusion reactor components. Significant opportunities exist for sharing information on technology of irradiation testing, specimen miniaturization, advanced methods of property measurement, safe windows for metal forming, and development of common materials property data base system. Both fusion and fission programs are being directed to development of clean steels with very low trace and tramp elements, characterization of microstructure and phase stability under irradiation, assessment of irradiation creep and swelling behaviour, studies on compatibility with helium and developing

  13. Measurements of angular and energy distributions of prompt neutrons from thermal neutron-induced fission

    Science.gov (United States)

    Vorobyev, A. S.; Shcherbakov, O. A.; Pleva, Yu. S.; Gagarski, A. M.; Val'ski, G. V.; Petrov, G. A.; Petrova, V. I.; Zavarukhina, T. A.

    2009-01-01

    The experimental setup and methodology used to measure prompt neutron angular and energy distributions from thermal neutron-induced fission are described. The neutrons are detected using two scintillation detectors, while the fission fragments are detected by multi-wire proportional detectors in conjunction with the TOF technique. To separate events corresponding to neutrons and γ-quanta, a double discrimination by the pulse shape and the time-of-flight is applied. Some preliminary results of an experiment performed with the 235U target are presented and briefly discussed. The yield of "scission" neutrons has been estimated in the framework of a simple evaporation model and was found not to exceed 5% of the total neutron yield. Including an assumed of anisotropy of the fission neutron angular distribution in the center-of-mass system of fission fragments into the model calculation leads to an increase in the "scission" neutron yields inferred from the data.

  14. Inmersiones isométricas en variedades riemannianas

    Directory of Open Access Journals (Sweden)

    Carlos Alberto Marín Arango

    2011-01-01

    Full Text Available Este trabajo recapitula la teoría básica de conexiones en fibrados principales y fibrados vectoriales con el fin de aplicar tales teorías al estudio de inmersiones isométricas en variedades riemannianas; por medio de una versión apropiada del teorema de Frobenius mostramos un resultado que generaliza el teorema fundamental de las inmersiones isométricas.

  15. g-factor of the Kπ = 14+ isomer in 176 W

    International Nuclear Information System (INIS)

    Ionescu-Bujor, M.; Iordachescu, A.; Marginean, N.; Brandolini, F.; Pavan, P.; Lenzi, S.M.; De Poli, M.; Gadea, A.; Martinez, T.; Medina, N.H.; Ribas, R.V.; Podolyak, Zs.

    2000-01-01

    to the beam direction, respectively, were used. The target was placed in an external magnetic field of 27.2(6) kG whose direction was periodically reversed. The time spectra of the 240, 351, 440 and 558 keV transitions in the ground-state band of 176 W, which collects most of the isomer decay were analysed according to the TDPAD procedures. The modulation ratio corresponding to the total accumulated statistics is presented together with the least-squares fit. For the g-factor of the 14 + isomeric state in 176 W the value g = +0.475(15) has been determined. The sensitivity of the magnetic moment to the nature of the involved quasiparticles allowed a definite configuration assignment for the 14 + isomer. We estimated the g-factors for all four-quasiparticle configurations with J π = K π = 14 + by using g Ω values deduced from experimental g-factors of the deformed single-particle states in odd-mass neighbouring nuclei. The π7/2 + [404] x π 9/2 - [514] x ν7/2 + [633] x ν5/2 - [512] pure configuration has been assigned to the 14 + isomeric state based on the excellent agreement between the calculated g-factor g cal = +0.47 and the measured value. We note that this assignment is in accordance with Woods-Saxon calculations for multi-quasiparticle states in 176 W. Information concerning the isomer shape will be obtained from a static quadrupole moment measurement which is in progress. (authors)

  16. Fission-neutrons source with fast neutron-emission timing

    Energy Technology Data Exchange (ETDEWEB)

    Rusev, G., E-mail: rusev@lanl.gov; Baramsai, B.; Bond, E.M.; Jandel, M.

    2016-05-01

    A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of {sup 252}Cf. The time is provided by registering the fission fragments in a layer of a thin scintillation film with a signal rise time of 1 ns. The scintillation light output is measured by two silicon photomultipliers with rise time of 0.5 ns. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements using it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.

  17. Isomerization of vaccenic acid to cis and trans C18:1 isomers during biohydrogenation by rumen microbes.

    Science.gov (United States)

    Laverroux, S; Glasser, F; Gillet, M; Joly, C; Doreau, M

    2011-09-01

    In ruminants, cis and trans C18:1 isomers are intermediates of fatty acid transformations in the rumen and their relative amounts shape the nutritional quality of ruminant products. However, their exact synthetic pathways are unclear and their proportions change with the forage:concentrate ratio in ruminant diets. This study traced the metabolism of vaccenic acid, the main trans C18:1 isomer found in the rumen, through the incubation of labeled vaccenic acid with mixed ruminal microbes adapted to different diets. [1-(13)C]trans-11 C18:1 was added to in vitro cultures with ruminal fluids of sheep fed either a forage or a concentrate diet. (13)C enrichment in fatty acids was analyzed by gas-chromatography-mass spectrometry after 0, 5 and 24 h of incubation. (13)C enrichment was found in stearic acid and in all cis and trans C18:1 isomers. Amounts of (13)C found in fatty acids showed that 95% of vaccenic acid was saturated to stearic acid after 5 h of incubation with the concentrate diet, against 78% with the forage diet. We conclude that most vaccenic acid is saturated to stearic acid, but some is isomerized to all cis and trans C18:1 isomers, with probably more isomerization in sheep fed a forage diet.

  18. Microscopic description of fission in nobelium isotopes with the Gogny-D1M energy density functional

    Energy Technology Data Exchange (ETDEWEB)

    Rodriguez-Guzman, R. [Kuwait University, Physics Department, Kuwait (Kuwait); Robledo, L.M. [Universidad Autonoma de Madrid, Departamento de Fisica Teorica, Madrid (Spain)

    2016-11-15

    Constrained mean-field calculations, based on the Gogny-D1M energy density functional, have been carried out to describe fission in the isotopes {sup 250-260}No. The even-even isotopes have been considered within the standard Hartree-Fock-Bogoliobov (HFB) framework while for the odd-mass ones the Equal Filling Approximation (HFB-EFA) has been employed. Ground state quantum numbers and deformations, pairing energies, one-neutron separation energies, inner and outer barrier heights as well as fission isomer excitation energies are given. Fission paths, collective masses and zero-point quantum vibrational and rotational corrections are used to compute the systematic of the spontaneous fission half-lives t{sub SF} both for even-even and odd-mass nuclei. Though there exists a strong variance of the predicted fission rates with respect to the details involved in their computation, it is shown that both the specialization energy and the pairing quenching effects, taken into account within the self-consistent HFB-EFA blocking procedure, lead to larger t{sub SF} values in odd-mass nuclei as compared with their even-even neighbors. Alpha decay lifetimes have also been computed using a parametrization of the Viola-Seaborg formula. The high quality of the Gogny-D1M functional regarding nuclear masses leads to a very good reproduction of Q{sub α} values and consequently of lifetimes. (orig.)

  19. Nuclear Dissipation from Fission Time

    International Nuclear Information System (INIS)

    Gontchar, I.; Morjean, M.; Basnary, S.

    2000-01-01

    Fission times, pre-scission neutron multiplicities and GDR pre-scission γ-ray multiplicities measured for uranium or thorium nuclei formed with temperatures T ∼ 1.8 MeV have been compared with calculations performed with CDSM2, a two-dimensional dynamical model combined with a statistical one. Among the three experimental approaches considered, fission times give access to the most precise pieces of information on nuclear dissipation at high excitation energy. For the temperature range under consideration, an agreement between the model and data is achieved if one-body dissipation is used with a strength factor k red ∼ 0.45 ± 0.10 applied to the wall term for the mononuclear configuration. (authors)

  20. Sexual differentiation in fission yeast

    DEFF Research Database (Denmark)

    Egel, R; Nielsen, O; Weilguny, D

    1990-01-01

    The regulation of sexual reproduction in yeast constitutes the highest level of differentiation observed in these unicellular organisms. The various ramifications of this system involve DNA rearrangement, transcriptional control, post-translational modification (such as protein phosphorylation......) and receptor/signal processing. A few basic similarities are common to both fission and budding yeasts. The wiring of the regulatory circuitry, however, varies considerably between these divergent yeast groups....

  1. Recycling of used fission material

    International Nuclear Information System (INIS)

    Abrahams, K.

    1991-01-01

    One of the most important social obstructions for the final disposal of nuclear waste is the long lifetime of some radioactive nuclides. However there are new possibilities for recycling high-level radioactive wastes. By nuclear transformation the troublesome components in the waste, the actinides and the long-living fission products can be transformed into products with a shorter decay time. (author). 9 refs.; 2 figs.; 3 tabs

  2. The VERDI fission fragment spectrometer

    International Nuclear Information System (INIS)

    Fregeau, M. O.; Brys, T.; Gamboni, T.; Geerts, W.; Oberstedt, S.; Oberstedt, A.; Borcea, R.

    2013-01-01

    The VERDI time-of-flight spectrometer is dedicated to measurements of fission product yields and of prompt neutron emission data. Pre-neutron fission-fragment masses will be determined by the double time-of-flight (TOF) technique. For this purpose an excellent time resolution is required. The time of flight of the fragments will be measured by electrostatic mirrors located near the target and the time signal coming from silicon detectors located at 50 cm on both sides of the target. This configuration, where the stop detector will provide us simultaneously with the kinetic energy of the fragment and timing information, significantly limits energy straggling in comparison to legacy experimental setup where a thin foil was usually used as a stop detector. In order to improve timing resolution, neutron transmutation doped silicon will be used. The high resistivity homogeneity of this material should significantly improve resolution in comparison to standard silicon detectors. Post-neutron fission fragment masses are obtained form the time-of-flight and the energy signal in the silicon detector. As an intermediary step a diamond detector will also be used as start detector located very close to the target. Previous tests have shown that poly-crystalline chemical vapour deposition (pCVD) diamonds provides a coincidence time resolution of 150 ps not allowing complete separation between very low-energy fission fragments, alpha particles and noise. New results from using artificial single-crystal diamonds (sCVD) show similar time resolution as from pCVD diamonds but also sufficiently good energy resolution. (authors)

  3. Physics and Chemistry of Fission. Proceedings of the Second IAEA Symposium on the Physics and Chemistry of Fission

    International Nuclear Information System (INIS)

    1969-01-01

    Fission studies have developed rapidly and significantly since the first IAEA Symposium on the Physics and Chemistry of Fission, held in 1965 in Salzburg. Several surprising discoveries and some excellent experimental results have given rise to many new theoretical investigations. From the individual theoretical models, laboriously improved and carefully fitted to the experimental data, a more general theoretical picture has begun to take shape and this has provided fresh ideas for experimental work. The Second Symposium on the Physics and Chemistry of Fission, held at the IAEA Headquarters in Vienna from 28 July to 1 August 1969, was a short pause in the rapid flow of developing theoretical concepts and new experimental investigations; it was devoted to the discussion, comparison and analysis of the recent achievements, and to a glance at the way fission studies are likely to develop in the near future. Two facts, the emphasis on theory and the important interplay of theory and experiment, left a strong mark on the contributions and discussions. The number of papers dealing with theoretical aspects is substantially larger than at the earlier symposium; this points to the fact that with increased efforts the theoreticians have succeeded in narrowing the wide gap between the large amount of empirical data and the theoretical understanding of it. The titles of individual sessions indicate the new trends in fission research. Theories of fragment distribution, shell structure effects in fissioning nuclei, intermediate structure, and isomeric fission are topics which were discussed with a great deal of uncertainty at the Salzburg symposium. At the present meeting, they were far more prominent and they were argued with great confidence and with the intensity and enthusiasm that only such exciting ideas can arouse. From the extensiveness of the discussion records the vivid interest of the participants is clearly seen; the pertinent problems still to be solved are also

  4. Measurement of mass and isotopic fission yields for heavy fission products with the LOHENGRIN mass spectrometer; Mesures de rendements isobariques et isotopiques des produits de fission lourds sur le spectrometre de masse LOHENGRIN

    Energy Technology Data Exchange (ETDEWEB)

    Bail, A.

    2009-05-15

    In spite of the huge amount of fission yield data available in different libraries, more accurate values are still needed for nuclear energy applications and to improve our understanding of the fission process. Thus measurements of fission yields were performed at the mass spectrometer Lohengrin at the Institut Laue-Langevin in Grenoble, France. The mass separator Lohengrin is situated at the research reactor of the institute and permits the placement of an actinide layer in a high thermal neutron flux. It separates fragments according to their atomic mass, kinetic energy and ionic charge state by the action of magnetic and electric fields. Coupled to a high resolution ionization chamber the experiment was used to investigate the mass and isotopic yields of the light mass region. Almost all fission yields of isotopes from Th to Cf have been measured at Lohengrin with this method. To complete and improve the nuclear data libraries, these measurements have been extended in this work to the heavy mass region for the reactions {sup 235}U(n{sub th},f), {sup 239}Pu(n{sub th},f) and {sup 241}Pu(n{sub th},f). For these higher masses an isotopic separation is no longer possible. So, a new method was undertaken with the reaction {sup 239}Pu(n{sub th},f) to determine the isotopic yields by spectrometry. These experiments have allowed to reduce considerably the uncertainties. Moreover the ionic charge state and kinetic energy distributions were specifically studied and have shown, among others, nanosecond isomers for some masses. (author)

  5. The resonance neutron fission on heavy nuclei

    CERN Document Server

    Kopach, Yu N; Furman, V I; Alfimenkov, V P; Lason', L; Pikelner, L B; Gonin, N N; Kozlovskij, L K; Tambovtsev, D I; Gagarskij, A M; Petrov, G A; Sokolov, V E

    2001-01-01

    A new approach to the description of the fission, similar to the well-known reaction theory and based on the helicity representation for the exit fission channels, is briefly summarized. This approach allows one to connect the multimodal fission representation with A. Bohr's concept of the fission transition states and to obtain formulae for the partial and differential fission cross sections. The formulae are used for analysis of the angular anisotropy of fragments in the neutron resonance induced fission of aligned sup 2 sup 3 sup 5 U nuclei and of the P-even angular forward-backward and right-left correlations of fragments oe the P-odd correlations caused by the interference of s- and p-wave neutron resonances

  6. Collective spectra along the fission barrier

    Directory of Open Access Journals (Sweden)

    Pigni M. T.

    2012-12-01

    Full Text Available Discrete and continuous spectra of fissioning nuclei at the humps of fission barriers (Bohr transition states and in the intermediate wells (superdeformed and hyperdeformed states play a key role in the calculation of fission cross sections. A theoretical evaluation of the collective parts of the spectra is possible within the framework of the dinuclear system model, which treats the wave function of the fissioning nucleus as a superposition of a mononucleus configuration and two–cluster configurations in a dynamical way, permitting exchange of upper–shell nucleons between clusters. The impact of theoretical spectra on neutron–induced fission cross sections and, in combination with an improved version of the scission–point model, on angular distribution of fission fragments is evaluated for plutonium isotopes of interest to nuclear energy applications.

  7. Collective spectra along the fission barrier

    Science.gov (United States)

    Shneidman, T. M.; Andreev, A. V.; Pigni, M. T.; Massimi, C.; Vannini, G.; Ventura, A.

    2012-12-01

    Discrete and continuous spectra of fissioning nuclei at the humps of fission barriers (Bohr transition states) and in the intermediate wells (superdeformed and hyperdeformed states) play a key role in the calculation of fission cross sections. A theoretical evaluation of the collective parts of the spectra is possible within the framework of the dinuclear system model, which treats the wave function of the fissioning nucleus as a superposition of a mononucleus configuration and two-cluster configurations in a dynamical way, permitting exchange of upper-shell nucleons between clusters. The impact of theoretical spectra on neutron-induced fission cross sections and, in combination with an improved version of the scission-point model, on angular distribution of fission fragments is evaluated for plutonium isotopes of interest to nuclear energy applications.

  8. The resonance neutron fission on heavy nuclei

    International Nuclear Information System (INIS)

    Kopach, Yu.N.; Popov, A.B.; Furman, V.I.; Alfimenkov, V.P.; Lason', L.; Pikel'ner, L.B.; ); Gonin, N.N.; Kozlovskij, L.K.; Tambovtsev, D.I.; Gagarskij, A.M.; Petrov, G.A.; Sokolov, V.E.

    2001-01-01

    A new approach to the description of the fission, similar to the well-known reaction theory and based on the helicity representation for the exit fission channels, is briefly summarized. This approach allows one to connect the multimodal fission representation with A. Bohr's concept of the fission transition states and to obtain formulae for the partial and differential fission cross sections. The formulae are used for analysis of the angular anisotropy of fragments in the neutron resonance induced fission of aligned 235 U nuclei and of the P-even angular forward-backward and right-left correlations of fragments oe the P-odd correlations caused by the interference of s- and p-wave neutron resonances [ru

  9. International conference on fifty years research in nuclear fission

    International Nuclear Information System (INIS)

    1989-02-01

    These proceedings contain extended abstracts of the papers presented at the named conference. They deal with static properties of fission, instrumentation for fission studies, fission in compound-nucleus reactions, fission dynamics, fission-like heavy ion reactions, and fusion reactions. See hints under the relevant topics. (HSI)

  10. Comparative evaluation of solar, fission, fusion, and fossil energy resources. Part 2: Power from nuclear fission

    Science.gov (United States)

    Clement, J. D.

    1973-01-01

    Different types of nuclear fission reactors and fissionable materials are compared. Special emphasis is placed upon the environmental impact of such reactors. Graphs and charts comparing reactor facilities in the U. S. are presented.

  11. Fission of nuclei far from stability

    International Nuclear Information System (INIS)

    Schmidt, K.H.; Benlliure, J.; Junghans, A.R.

    2000-11-01

    The secondary-beam facility of GSI provided the technical equipment for a new kind of fission experiment. Fission properties of short-lived neutron-deficient nuclei have been investigated in inverse kinematics. The measured element distributions reveal new kinds of systematics on shell structure and even-odd effects and lead to an improved understanding of structure effects in nuclear fission. Prospects for further experimental studies are discussed. (orig.)

  12. Monte carlo sampling of fission multiplicity.

    Energy Technology Data Exchange (ETDEWEB)

    Hendricks, J. S. (John S.)

    2004-01-01

    Two new methods have been developed for fission multiplicity modeling in Monte Carlo calculations. The traditional method of sampling neutron multiplicity from fission is to sample the number of neutrons above or below the average. For example, if there are 2.7 neutrons per fission, three would be chosen 70% of the time and two would be chosen 30% of the time. For many applications, particularly {sup 3}He coincidence counting, a better estimate of the true number of neutrons per fission is required. Generally, this number is estimated by sampling a Gaussian distribution about the average. However, because the tail of the Gaussian distribution is negative and negative neutrons cannot be produced, a slight positive bias can be found in the average value. For criticality calculations, the result of rejecting the negative neutrons is an increase in k{sub eff} of 0.1% in some cases. For spontaneous fission, where the average number of neutrons emitted from fission is low, the error also can be unacceptably large. If the Gaussian width approaches the average number of fissions, 10% too many fission neutrons are produced by not treating the negative Gaussian tail adequately. The first method to treat the Gaussian tail is to determine a correction offset, which then is subtracted from all sampled values of the number of neutrons produced. This offset depends on the average value for any given fission at any energy and must be computed efficiently at each fission from the non-integrable error function. The second method is to determine a corrected zero point so that all neutrons sampled between zero and the corrected zero point are killed to compensate for the negative Gaussian tail bias. Again, the zero point must be computed efficiently at each fission. Both methods give excellent results with a negligible computing time penalty. It is now possible to include the full effects of fission multiplicity without the negative Gaussian tail bias.

  13. Measurements of Fission Cross Sections of Actinides

    CERN Multimedia

    Wiescher, M; Cox, J; Dahlfors, M

    2002-01-01

    A measurement of the neutron induced fission cross sections of $^{237}$Np, $^{241},{243}$Am and of $^{245}$Cm is proposed for the n_TOF neutron beam. Two sets of fission detectors will be used: one based on PPAC counters and another based on a fast ionization chamber (FIC). A total of 5x10$^{18}$ protons are requested for the entire fission measurement campaign.

  14. From ground state to fission fragments: A complex, multi-dimensional multi-path problem

    Energy Technology Data Exchange (ETDEWEB)

    Moeller, P. [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan); Nix, J.R. [Los Alamos National Lab., NM (United States); Swiatecki, W.J. [Lawrence Berkeley Lab., CA (United States)

    1992-03-01

    Experimental results on the fission properties of nuclei close to {sup 264}Fm show sudden and large changes with a change of only one or two neutrons or protons. The nucleus {sup 258}Fm, for instance, undergoes symmetric fission with a half-life of about 0.4 ms and a kinetic-energy distribution peaked at about 235 MeV whereas {sup 256}Fm undergoes asymmetric fission with a half-life of about 3 h and a kinetic-energy distribution peaked at about 200 MeV. Qualitatively, these sudden changes have been postulated to be due to the emergence of fragment shells in symmetric-fission products close to {sup 132}Sn. Here we present a quantitative calculation that shows where high-kinetic-energy symmetric fusion occurs and why it is associated with a sudden and large decrease in fission half-lives. We base our study on calculations of potential-energy surfaces in the macroscopic-microscopic model and a semi-empirical model for the nuclear inertia. We use the three-quadratic-surface parameterization to generate the shapes for which the potential-energy surfaces are calculated. The use of this parameterization and the use of the finite-range macroscopic model allows for the study of two touching spheres and similar shapes. Since these shapes are thought to correspond to the scission shapes for the high-kinetic-energy events it is of crucial importance that a continuous sequence of shapes leading from the nuclear ground state to these configurations can be studied within the framework of the model. We present the results of the calculations in terms of potential-energy surfaces and fission half-lives for heavy even nuclei. The surfaces are displayed in the form of contour diagrams as functions of two moments of the shape. They clearly show the appearance of a second fission valley, which leads to scission configurations close to tow touching spheres, for fissioning systems in the vicinity of {sup 264}Fm.

  15. Status of fission product yield data

    International Nuclear Information System (INIS)

    Cuninghame, J.G.

    1978-01-01

    The topics covered in this paper are: (a) cumulative yields in thermal neutron fission and in fast fission up to 14 MeV incident neutron energy, (b) dependence of the yields on incident neutron energy and spectrum, (c) independent yields, (d) charge dispersion and distribution, and (e) yields of light particles from ternary fission. The paper reviews information on these subjects for fission of actinides from 232 Th upwards with special emphasis on data published since the 1973 Bologna FPND Panel, compares data sets, and discusses the gaps still to be found in them. (author)

  16. Theoretical Description of the Fission Process

    Energy Technology Data Exchange (ETDEWEB)

    Witold Nazarewicz

    2003-07-01

    The main goals of the project can be summarized as follows: Development of effective energy functionals that are appropriate for the description of heavy nuclei. Our goal is to improve the existing energy density (Skyrme) functionals to develop a force that will be used in calculations of fission dynamics. Systematic self-consistent calculations of binding energies and fission barriers of actinide and trans-actinide nuclei using modern density functionals. This will be followed by calculations of spontaneous fission lifetimes and mass and charge divisions using dynamic adiabatic approaches based on the WKB approximation. Investigate novel microscopic (non-adiabatic) methods to study the fission process.

  17. Attachment of gaseous fission products to aerosols

    International Nuclear Information System (INIS)

    Skyrme, G.

    1985-01-01

    Accidents may occur in which the integrity of fuel cladding is breached and volatile fission products are released to the containment atmosphere. In order to assess the magnitude of the subsequent radiological hazard it is necessary to know the transport behaviour of such fission products. It is frequently assumed that the fission products remain in the gaseous phase. There is a possibility, however, that they may attach themselves to particles and hence substantially modify their transport properties. This paper provides a theoretical assessment of the conditions under which gaseous fission products may be attached to aerosol particles. Specific topics discussed are: the mass transfer of a gaseous fission product to an isolated aerosol particle in an infinite medium; the rate at which the concentration of fission products in the gas phase diminishes within a container as a result of deposition on a population of particles; and the distribution of deposited fission product between different particle sizes in a log-normal distribution. It is shown that, for a given mass, small particles are more efficient for fission product attachment, and that only small concentrations of such particles may be necessary to achieve rapid attachment. Conditions under which gaseous fission products are not attached to particles are also considered, viz, the competing processes of deposition onto the containment walls and onto aerosol particles, and the possibility of the removal of aerosols from the containment by various deposition processes, or agglomeration, before attachment takes place. (author)

  18. True ternary fission in 310126X

    International Nuclear Information System (INIS)

    Banupriya, B.; Vijayaraghavan, K.R.; Balasubramaniam, M.

    2015-01-01

    All possible combinations are minimized by the two dimensional minimization process and minimized with respect to neutron numbers and proton numbers of the fragments. Potential energy is low and Q - value is high at true ternary fission region. It shows that true ternary mode is the dominant mode in the ternary fission of superheavy nuclei. Also, the results show that the fragments with neutron magic numbers are the dominant one in the ternary fission of superheavy nuclei whereas the fragments with proton magic numbers are the dominant one in the ternary fission of heavy nuclei

  19. Nuclear fission studies: from LOHENGRIN to FIPPS

    International Nuclear Information System (INIS)

    Chebboubi, Abdelaziz

    2015-01-01

    Nuclear fission consists in splitting a nucleus, in general an actinide, into smaller nuclei. Despite nuclear fission was discovered in 1939 by Hahn and Strassman, fission models cannot predict the fission observables with an acceptable accuracy for nuclear fuel cycle studies for instance. Improvement of fission models is an important issue for the knowledge of the process itself and for the applications. To reduce uncertainties of the nuclear data used in a nuclear reactor simulation, a validation of the models hypothesis is mandatory. In this work, two features of the nuclear fission were investigated in order to test the resistance of the theories. One aspect is the study of the symmetric fission fragments through the measurement of their yield and kinetic energy distribution. The other aspect is the study of the fission fragment angular momentum.Two techniques are available to assess the angular momentum of a fission fragment. The first one is to look at the properties of the prompt gamma. The new spectrometer FIPPS (Fission Product Prompt gamma-ray Spectrometer), is currently under development at the ILL and will combine a fission filter with a large array of gamma and neutron detectors in order to respond to these issues. The first part of this work is dedicated to the study of the properties of a Gas Filled Magnet (GFM) which is the type of fission filter considered for the FIPPS project.The second part of this work deals with the measurement of isomeric yields and evaluations of the angular momentum distribution of fission fragments. The study of the spherical nucleus 132 Sn shed the light on the current limits of fission models. Finally, the last part of this work is about the measurement of the yields and kinetic energy distributions of symmetric fission fragments. Since models predict the existence of fission modes, the symmetry region is a suitable choice to investigate this kind of prediction. In parallel with all these studies, an emphasis on the

  20. Theoretical Description of the Fission Process

    International Nuclear Information System (INIS)

    Witold Nazarewicz

    2003-01-01

    The main goals of the project can be summarized as follows: Development of effective energy functionals that are appropriate for the description of heavy nuclei. Our goal is to improve the existing energy density (Skyrme) functionals to develop a force that will be used in calculations of fission dynamics. Systematic self-consistent calculations of binding energies and fission barriers of actinide and trans-actinide nuclei using modern density functionals. This will be followed by calculations of spontaneous fission lifetimes and mass and charge divisions using dynamic adiabatic approaches based on the WKB approximation. Investigate novel microscopic (non-adiabatic) methods to study the fission process

  1. Comments on the stochastic characteristics of fission chamber signals

    International Nuclear Information System (INIS)

    Pál, L.; Pázsit, I.; Elter, Zs.

    2014-01-01

    This paper reports on theoretical investigations of the stochastic properties of the signal series of ionisation chambers, in particular fission chambers. First, a simple and transparent derivation is given of the higher order moments of the random detector signal for incoming pulses with a non-homogeneous Poisson distribution and random pulse heights and arbitrary shape. Exact relationships are derived for the higher order moments of the detector signal, which constitute a generalisation of the so-called higher order Campbelling techniques. The probability distribution of the number of time points when the signal exceeds a certain level is also derived. Then, a few simple pulse shapes and amplitude distributions are selected as idealised models of the detector signals. Assuming that the incoming particles form a homogeneous Poisson process, explicit expressions are given for the higher order moments of the signal and the number of level crossings in a given time interval for the selected pulse shapes

  2. Fission - track age of the Marjalahti Pallasite

    International Nuclear Information System (INIS)

    Bondar, Yu.V.; Perelygin, V.P.

    2006-01-01

    Full text: Investigation of fossil charged-particle tracks in various mineral phases of extraterrestrial samples is a powerful method for research the early stages of the solar system. Over geological time, meteorites crystals have accumulated a record of tracks produced by heavily charged energetic particles from both internal (spontaneous fission of 238U and some other extinct isotopes) and external sources (galactic cosmic rays with Z>20). The fortunate fact that meteorite grains can accumulate latent and very long-lived tracks since soon after the end of nucleosynthesis in the solar nebula enables one to decode their radiation history and to detect any thermal events in the meteorite cosmic history by revealing these tracks through suitable etching procedures. Only a few minerals in meteorites (mainly phosphates) contain small amount of uranium; the fact that 238 U undergoes fission with fission-decay constant λ f ∼ 8.2x10 -17 yr -1 allows one to use this isotope as a chronometer. By measuring the U concentration in the crystals (by reactor irradiation) and the density of the spontaneous-fission tracks it is relatively easy to calculate the 'fission-track age' if 238 U is the main source of fission tracks. However the fission-track dating of extraterrestrial samples compared with the terrestrial ones has some peculiar features due to presence of a number of other potential track sources except the spontaneous fission of 238 U, such as the spontaneous fission of presently extinct 244 Pu, heavy nuclei of cosmic rays and induced fission by cosmic ray primaries. Only tracks from the spontaneous fission of U and Pu are suitable for fission-track dating. The competing effects of these fissioning elements, whose half-lives differ by a factor of ∼50, form a basis for a fission-track chronology for samples older than ∼ 4.0 Gyr. Over small intervals in time (∼ few x10 8 yr ) the track density from spontaneous fission of 238 U is nearly constant. However, the

  3. Substitution effects on the absorption spectra of nitrophenolate isomers.

    Science.gov (United States)

    Wanko, Marius; Houmøller, Jørgen; Støchkel, Kristian; Suhr Kirketerp, Maj-Britt; Petersen, Michael Åxman; Nielsen, Mogens Brøndsted; Nielsen, Steen Brøndsted; Rubio, Angel

    2012-10-05

    Charge-transfer excitations highly depend on the electronic coupling between the donor and acceptor groups. Nitrophenolates are simple examples of charge-transfer systems where the degree of coupling differs between ortho, meta and para isomers. Here we report the absorption spectra of the isolated anions in vacuo to avoid the complications of solvent effects. Gas-phase action spectroscopy was done with two different setups, an electrostatic ion storage ring and an accelerator mass spectrometer. The results are interpreted on the basis of CC2 quantum chemical calculations. We identified absorption maxima at 393, 532, and 399 nm for the para, meta, and ortho isomer, respectively, with the charge-transfer transition into the lowest excited singlet state. In the meta isomer, this π-π* transition is strongly redshifted and its oscillator strength reduced, which is related to the pronounced charge-transfer character, as a consequence of the topology of the conjugated π-system. Each isomer's different charge distribution in the ground state leads to a very different solvent shift, which in acetonitrile is bathochromic for the para and ortho, but hypsochromic for the meta isomer.

  4. Fragment Angular Distributions in Neutron-Induced Fission of {sup 235}U and {sup 239}Pu using a Time Projection Chamber

    Energy Technology Data Exchange (ETDEWEB)

    Kleinrath, Verena [NIFFTE collaboration, Los Alamos National Laboratory, Los Alamos, NM 87545 (United States)

    2015-07-01

    Fission fragment angular distributions can lend insights into fission barrier shapes and level densities at the scission point, both important for fission theory development. Fragment emission anisotropies are also valuable for precision cross section ratio measurements, if the distributions are different for the two isotopes used in the ratio. Available angular data is sparse for {sup 235}U and even more so for {sup 239}Pu, especially at neutron energies above 5 MeV. The Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) time projection chamber, which enables precise tracking of charged particles, can be used to study angular distributions and emission anisotropies of fission fragments in neutron-induced fission. In-beam data collected at the Los Alamos Neutron Science Center with a {sup 235}U/{sup 239}Pu target during the 2014 run-cycle will provide angular distributions as a function of incident neutron energy for these isotopes. (LA-UR-1426972). (authors)

  5. Development of a thin scintillation films fission-fragment detector and a novel neutron source

    Science.gov (United States)

    Rusev, G.; Jandel, M.; Baramsai, B.; Bond, E. M.; Bredeweg, T. A.; Couture, A.; Daum, J. K.; Favalli, A.; Ianakiev, K. D.; Iliev, M. L.; Mosby, S.; Roman, A. R.; Springs, R. K.; Ullmann, J. L.; Walker, C. L.

    2015-08-01

    Investigation of prompt fission and neutron-capture Υ rays from fissile actinide samples at the Detector for Advanced Neutron Capture Experiments (DANCE) requires use of a fission-fragment detector to provide a trigger or a veto signal. A fission-fragment detector based on thin scintillating films and silicon photomultipliers has been built to serve as a trigger/veto detector in neutron-induced fission measurements at DANCE. The fissile material is surrounded by scintillating films providing a 4π detection of the fission fragments. The scintillations were registered with silicon photomultipliers. A measurement of the 235U(n,f) reaction with this detector at DANCE revealed a correct time-of-flight spectrum and provided an estimate for the efficiency of the prototype detector of 11.6(7)%. Design and test measurements with the detector are described. A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of 252Cf and the same type of scintillating films and silicon photomultipliers. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements with it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.

  6. Evolution of uranium fission-fragment charge yields with neutron number. Strong effect of multi-chance fission on yield asymmetries

    Energy Technology Data Exchange (ETDEWEB)

    Moeller, Peter [Los Alamos National Laboratory, Theoretical Division, Los Alamos, NM (United States); Schmitt, Christelle [CEA/DSM-CNRS/IN2P3, Grand Accelerateur National d' Ions Lourds, Caen (France)

    2017-01-15

    We use the Brownian shape-motion model, with its recent extensions, which allow modeling of odd-even staggering, to calculate the evolution of fission-fragment charge distributions with neutron number for the compound-system sequence {sup 234}U, {sup 236}U, {sup 238}U, and {sup 240}U. We compare to experimental data where available, for neutron- and electromagnetic-induced fission over a compound-nucleus excitation energy range from about 6 to 20 MeV. A notable result of the study is that the evolution of the location of the peak charge yield from Z = 54 in {sup 234}U towards Z = 52 in heavier isotopes, seen in the experimental data, is present also in the calculated yields. We further show that to describe yields at higher compound-nucleus excitation energies, then, already at 20 MeV, it is necessary to take multi-chance fission into account. (orig.)

  7. Preferential polymerization and adsorption of L-optical isomers of amino acids relative to D-optical isomers on kaolinite templates.

    Science.gov (United States)

    Jackson, T. A.

    1971-01-01

    Experiments on the polymerization of the L- and D-optical isomers of aspartic acid and serine using kaolinite as a catalyst showed that the L-optical isomers were polymerized at a much higher rate than the D-optical isomers; racemic (DL-) mixtures were polymerized at an intermediate rate. The peptides formed from the L-monomers were preferentially adsorbed by the clay. In the absence of kaolinite, no significant or consistent difference in the behavior of the L- and D-optical isomers was observed. In experiments on the adsorption of L- and D-phenylalanine by kaolinite, the L-optical isomer was preferentially adsorbed.

  8. Identification of isomers and control of ionization and dissociation processes using dual-mass-spectrometer scheme and genetic algorithm optimization

    International Nuclear Information System (INIS)

    Chen Zhou; Qiu-Nan Tong; Zhang Cong-Cong; Hu Zhan

    2015-01-01

    Identification of acetone and its two isomers, and the control of their ionization and dissociation processes are performed using a dual-mass-spectrometer scheme. The scheme employs two sets of time of flight mass spectrometers to simultaneously acquire the mass spectra of two different molecules under the irradiation of identically shaped femtosecond laser pulses. The optimal laser pulses are found using closed-loop learning method based on a genetic algorithm. Compared with the mass spectra of the two isomers that are obtained with the transform limited pulse, those obtained under the irradiation of the optimal laser pulse show large differences and the various reaction pathways of the two molecules are selectively controlled. The experimental results demonstrate that the scheme is quite effective and useful in studies of two molecules having common mass peaks, which makes a traditional single mass spectrometer unfeasible. (paper)

  9. Anisotropy in the ternary cold fission

    CERN Document Server

    Delion, D S; Greiner, W

    2003-01-01

    We describe the spontaneous ternary cold fission of sup 2 sup 5 sup 2 Cf, accompanied by sup 4 He, sup 1 sup 0 Be and sup 1 sup 4 C within a stationary scattering formalism. We show that the light cluster should be born in the neck region. It decays from the first resonant eigenstate in the Coulomb plus harmonic oscillator potential, centred in this region and eccentric with respect to the symmetry axis. This description gives a simple answer to the question why the averaged values in the energy spectra of emitted clusters are close to each other, in spite of different Coulomb barriers. We have shown that the angular distribution of the emitted light particle is strongly connected with its deformation and the equatorial distance. Experimental angular distributions can be explained by the spherical shapes of emitted clusters, except for a deformed sup 1 sup 0 Be. We also predicted some dependences of half-lives for such tri-nuclear systems upon potential parameters.

  10. Shape coexistence in the odd-odd nucleus Y98 : The role of the g9/2 neutron extruder

    Energy Technology Data Exchange (ETDEWEB)

    Urban, W.; Czerwiński, M.; Kurpeta, J.; Rząca-Urban, T.; Wiśniewski, J.; Materna, T.; Iskra, Ł. W.; Smith, A. G.; Ahmad, I.; Blanc, A.; Faust, H.; Köster, U.; Jentschel, M.; Mutti, P.; Soldner, T.; Simpson, G. S.; Pinston, J. A.; de France, G.; Ur, C. A.; Elomaa, V. -V.; Eronen, T.; Hakala, J.; Jokinen, A.; Kankainen, A.; Moore, I. D.; Rissanen, J.; Saastamoinen, A.; Szerypo, J.; Weber, C.; Äystö, J.

    2017-10-01

    Excited states in Y-98, populated in neutron-induced fission of U-235 and in spontaneous fission of Cm-248 and Cf-252, have been studied by means of gamma spectroscopy using the Lohengrin fission-fragment separator at ILL Grenoble and the EXILL, Eurogam2, and Gammasphere Ge arrays. Two new isomers have been found in Y-98: a deformed one with T-1/2 = 180(7) ns and a rotational band on top of it, and a spherical one with T-1/2 = 0.45(15) mu s, analogous to the 8(+) isomer in Y-96, corresponding to the (nu g(7/2), pi g(9/2))(8+) spherical configuration. Using the JYFLTRAP Penning trap, an accurate excitation energy of 465.7(7) keV has been determined for the 2.36-s isomer in Y-98. This result and the studies of excited levels in Zr-98, populated in beta-decay of the isomer, indicate a new spin-parity, I-pi = (7)(+) for the isomer. The high spin and the decay properties of this isomer suggest the presence of the 9/2(+)[ 404] neutron extruder orbital in its structure. This is consistent with the large deformation of the isomer, reported recently. The present work does not provide arguments to support the special role of the nu g(7/2)-pi g(9/2) interaction (the spin-orbit-partner, or SOP, mechanism).

  11. Laser isotope and isomer separations: History and trends

    International Nuclear Information System (INIS)

    Paper will review history and principles of laser isotope and nuclear isomer separation: laser multistep photoionization of isotopic and isomeric atoms, laser IR-UV two-step photodissociation of molecules, laser IR multiphoton photodissociation of polyatomic molecules. The comparison and areas of applications of these methods will be considered. Paper will discuss a present state of art of technology of these methods in practical scale in various countries. In conclusion the trends of research in this field including applications of laser-separated isotopes and isomers will be considered

  12. Theoretical Study of the Diastereofacial Isomers of Aldrin and Dieldrin

    Directory of Open Access Journals (Sweden)

    Zoran Zdravkovski

    2006-02-01

    Full Text Available The Diels-Alder reaction of hexachlorocyclopentadiene with norbornadiene givesaldrin but theoretically three other diastereofacial isomers are possible. On oxidation theseisomers can generate eight adducts one of which is known as dieldrin. All these, as well asthe corresponding reactions with hexafluorocyclopenadiene were studied by semiempirical(AM1 and PM3 and hybrid density functional (B3LYP methods. Besides the energy levels,the transition states were calculated for the reactions leading to the diastereofacial isomers ofaldrin, which indicate that aldrin is the favored product of the reaction both fromthermodynamic and kinetic point of view.

  13. Nuclear Power from Fission Reactors. An Introduction.

    Science.gov (United States)

    Department of Energy, Washington, DC. Technical Information Center.

    The purpose of this booklet is to provide a basic understanding of nuclear fission energy and different fission reaction concepts. Topics discussed are: energy use and production, current uses of fuels, oil and gas consumption, alternative energy sources, fossil fuel plants, nuclear plants, boiling water and pressurized water reactors, the light…

  14. Progress in fission product nuclear data

    International Nuclear Information System (INIS)

    Lammer, M.

    1982-07-01

    This is the eighth issue of a report series on Fission Product Nuclear Data (FPND) which is published by the Nuclear Data Section (NDS) of the International Atomic Energy Agency (IAEA). The purpose of this series is to inform scientists working on FPND, or using such data, about all activities in this field which are planned, ongoing, or have recently been completed. The main part of this report consists of unaltered original contributions which the authors have sent to IAEA/NDS. Therefore, the IAEA cannot be held responsible for the information contained nor for any consequences resulting from the use of this information. The present issue contains also a section with some recent references relative to fission product nuclear data, which were not covered by the contributions submitted. The types of activities being included in this report are measurements, compilations and evaluations of: Fission product yields (neutron induced and spontaneous fission); Neutron reaction cross sections of fission products; Data related to the radioactive decay of fission products; Delayed neutron data of fission products; and lumped fission product data (decay heat, absorption etc.). The seventh issue of this series has been published in July 1981 as INDC(NDS)-116. The present issue includes contributions which were received by NDS between 1 August 1981 and 15 June 1982

  15. Progress in fission product nuclear data

    International Nuclear Information System (INIS)

    Lammer, M.

    1983-08-01

    This is the ninth issue of a report series on Fission Product Nuclear Data (FPND) which is published by the Nuclear Data Section (NDS) of the International Atomic Energy Agency (IAEA). The purpose of this series is to inform scientists working on FPND, or using such data, about all activities in this field which are planned, ongoing, or have recently been completed. The main part of this report consists of unaltered original contributions which the authors have sent to IAEA/NDS. The present issue contains also a section with some recent references relative to fission product nuclear data, which were not covered by the contributions submitted. The types of activities being included in this report are measurements, compilations and evaluations of: Fission product yields (neutron induced and spontaneous fission); Neutron reaction cross sections of fission products; Data related to the radioactive decay of fission products; Delayed neutron data of fission products; and lumped fission product data (decay heat, absorption etc.). The eighth issue of this series has been published in July 1982 as INDC(NDS)-130. The present issue includes contributions which were received by NDS between 1 August 1982 and 25 June 1983

  16. Progress in fission product nuclear data

    International Nuclear Information System (INIS)

    Lammer, M.

    1981-06-01

    This is the seventh issue of a report series on Fission Product Nuclear Data (FPND) which is published by the Nuclear Data Section (NDS) of the International Atomic Energy Agency (IAEA). The purpose of this series is to inform scientists working on FPND, or using such data, about all activities in this field which are planned, ongoing, or have recently been completed. The present issue contains also a section with some recent references relative to fission product nuclear data, which were not covered by the contributions submitted. The types of activities being included in this report are measurements, compilations and evaluations of: fission product yields (neutron induced and spontaneous fission); neutron reaction cross sections of fission products; data related to the radioactive decay of fission products; delayed neutron data of fission products; and lumped fission product data (decay heat, absorption etc.). The sixth issue of this series has been published in June 1980 as INDC(NDS)-113/G+P. The present issue includes contributions which were received by NDS between 1 August 1980 and 25 May 1981

  17. Seventy-five years of nuclear fission

    Indian Academy of Sciences (India)

    the angular distribution of the fragments with the direction of the incident projectile caus- ing fission will depend on .... But in harnessing nuclear energy through the critical fission reactors, disposal of nuclear waste ... experimental technique based on a gridded ion chamber, emission spectra and angular distributions of the ...

  18. Induced-Fission Imaging of Nuclear Material

    International Nuclear Information System (INIS)

    This paper presents initial results from development of the induced-fission imaging technique, which can be used for the purpose of measuring or verifying the distribution of fissionable material in an unopened container. The technique is based on stimulating fissions in nuclear material with 14 MeV neutrons from an associated-particle deuterium-tritium (D-T) generator and counting the subsequent induced fast fission neutrons with an array of fast organic scintillation detectors. For each source neutron incident on the container, the neutron creation time and initial trajectory are known from detection of the associated alpha particle of the d + t → α + n reaction. Many induced fissions will lie along (or near) the interrogating neutron path, allowing an image of the spatial distribution of prompt induced fissions, and thereby fissionable material, to be constructed. A variety of induced-fission imaging measurements have been performed at Oak Ridge National Laboratory with a portable, low-dose D-T generator, including single-view radiographic measurements and three-dimensional tomographic measurements. Results from these measurements will be presented along with the neutron transmission images that have been performed simultaneously. This new capability may have applications to a number of areas in which there may be a need to confirm the presence or configuration of nuclear materials, such as nuclear material control and accountability, quality assurance, treaty confirmation, or homeland security applications.

  19. Some aspects of fission and quasifission processes

    Indian Academy of Sciences (India)

    2015-07-22

    Jul 22, 2015 ... The discovery of nuclear fission in 1938–1939 had a profound influence on the field of nuclear physics and it brought this branch of physics into the forefront as it was recognized for having the potential for its seminal influence on modern society. Although many of the basic features of actinide fission were ...

  20. Cumulative fission yield of Ce-148 produced by thermal-neutron fission of U-235

    International Nuclear Information System (INIS)

    Hasan, A.A.

    1984-12-01

    Cumulative fission yield of 148 cesium isotopes and some other fission products produced by thermal-neutron fission of 235 uranium is determined by Germanium/Lithium spectroscopic methods. The measuremets were done at Tsing-Hua open pool reactor using 3 to 4 mg of 93.15% enriched 235 uranium samples. Gamma rays are assigned to the responsible fission products by matching gamma rays energies and half lives. Fission rate is calculated by fission track method. Cumulative fission yields of 148 cesium, 90 krypton, 130 iodine, 144 lanthanum, 89 krypton, 136 xenon, 137 xenon and 140 cesium are calculated. This values are compared with previously predicted values and showed good agreement. 21 Ref

  1. Fission Surface Power Technology Development Status

    Science.gov (United States)

    Palac, Donald T.; Mason, Lee S.; Houts, Michael G.; Harlow, Scott

    2010-01-01

    Power is a critical consideration in planning exploration of the surfaces of the Moon, Mars, and beyond. Nuclear power is an important option, especially for locations in the solar system where sunlight is limited in availability or intensity. NASA is maintaining the option for fission surface power for the Moon and Mars by developing and demonstrating technology for an affordable fission surface power system. Because affordability drove the determination of the system concept that this technology will make possible, low development and recurring costs result, while required safety standards are maintained. However, an affordable approach to fission surface power also provides the benefits of simplicity, robustness, and conservatism in design. This paper will illuminate the multiplicity of benefits to an affordable approach to fission surface power, and will describe how the foundation for these benefits is being developed and demonstrated in the Exploration Technology Development Program s Fission Surface Power Project.

  2. Physics of neutron emission in fission

    International Nuclear Information System (INIS)

    Lemmel, H.D.

    1989-06-01

    The document contains the proceedings of the IAEA Consultants' Meeting on the Physics of Neutron Emission in Fission, Mito City (Japan), 24-27 May 1988. Included are the conclusions and recommendations reached at the meeting and the papers presented by the meeting participants. These papers cover the following topics: Energy dependence of the number of fission neutrons ν-bar (3 papers), multiplicity distribution of fission neutrons (3 papers), competition between neutron and γ-ray emission (4 papers), the fission neutron yield in resonances (2 papers) and the energy spectrum of fission neutrons in experiment (9 papers), theory (4 papers) and evaluation (1 paper). A separate abstract was prepared for each of these papers. Refs, figs and tabs

  3. Progress in fission product nuclear data

    International Nuclear Information System (INIS)

    Lammer, G.

    1975-01-01

    This is the first issue of a report series on Fission Product Nuclear Data (FPND), published every six months by the Nuclear Data Section (NDS) of the International Atomic Energy Agency (IAEA). Its purpose is to inform scientists working on FPND, or using such data, about all activities in this field which are planned, ongoing, or have recently been completed. The types of activities being included in this report are measurements, compilations and evaluations of: fission product yields; neutron cross-section data of fission products; data related to β-, γ-decay of fission products; delayed neutron data; and fission product decay-heat. The present issue includes contributions which were received by NDS before 1 November 1975

  4. Fission gas behaviour in water reactor fuels

    International Nuclear Information System (INIS)

    2002-01-01

    During irradiation, nuclear fuel changes volume, primarily through swelling. This swelling is caused by the fission products and in particular by the volatile ones such as krypton and xenon, called fission gas. Fission gas behaviour needs to be reliably predicted in order to make better use of nuclear fuel, a factor which can help to achieve the economic competitiveness required by today's markets. These proceedings communicate the results of an international seminar which reviewed recent progress in the field of fission gas behaviour in light water reactor fuel and sought to improve the models used in computer codes predicting fission gas release. State-of-the-art knowledge is presented for both uranium-oxide and mixed-oxide fuels loaded in water reactors. (author)

  5. Contained fissionly vaporized imploded fission explosive breeder reactor

    International Nuclear Information System (INIS)

    Marwick, E.F.

    1978-01-01

    Disclosed is a nuclear reactor system which produces useful thermal power and breeds fissile isotopes wherein large spherical complex slugs containing fissile and fertile isotopes as well as vaporizing and tamping materials are exploded seriatim in a large containing chamber having walls protected from the effects of the explosion by about two thousand tons of slurry of fissile and fertile isotopes in molten alkali metal. The slug which is slightly sub-critical prior to its entry into the centroid portion of the chamber, then becomes slightly more than prompt-critical because of the near proximity of neutron-reflecting atoms and of fissioning atoms within the slurry. The slurry is heated by explosion of the slugs and serves as a working fluid for extraction of heat energy from the reactor. Explosive debris is precipitated from the slurry and used for the fabrication of new slugs

  6. Influence of pre-saddle neutrons on the fission fragment angular distribution

    Science.gov (United States)

    Fröbrich, P.; Rossner, H.

    1994-06-01

    In the present note it is shown that distinguishing between pre-saddle and saddle-to-scission neutrons removes a discrepancy previously found [2 4] between data for the fission fragment anisotropy and an analysis in the framework of the transition state theory in which it has been assumed that all pre-scission neutrons influence the temperature at the saddle point. The analysis of the present paper requires a fairly weak (β=2 * 1021 s -1) friction at compact shapes, in agreement with a previous [9,10] analysis of prescission neutron multiplicities and fission probabilities.

  7. Generalized seniority states and isomers in tin isotopes

    Science.gov (United States)

    Jain, Ashok Kumar; Maheshwari, Bhoomika

    2017-07-01

    Isomeric studies in neutron-rich nuclei are a powerful tool for exploring structure at the nuclear extremes. In this paper we discuss the systematic features of the excitation energies and transition probabilities of Sn isotopes in the region N = 50-82 and present their basic understanding in terms of generalized seniority. We further use generalized seniority as a probe to explore the neutron-rich {6}+ seniority isomers in 134-138Sn, and to validate the neutron single-particle energies beyond N = 82. We show that these isomers behave as generalized seniority isomers, where the so-called anomalous {{B}}(E2) behavior of the {6}+ isomer in 136Sn may be naturally explained. We support these results by shell model calculations, where the latest neutron single-particle energies of the N = 82-126 region have been used, and the i13/2 neutron single-particle energy has been suitably modified in the renormalized charge-dependent Bonn interaction. This entails a possible new subshell closure at N = 112 due to the suggested higher location of the i13/2 neutron orbital, also consistent with the choice of orbitals in the generalized seniority scheme. However, a small reduction in the f7/2 two-body matrix elements is still required in the shell model calculations to consistently reproduce the experimental level energies as well as the transition probabilities in 134-138Sn isotopes.

  8. The molecular properties of nitrobenzanthrone isomers and their mutagenic activities.

    Science.gov (United States)

    Ostojić, Bojana D; Stanković, Branislav; Ðorđević, Dragana S

    2014-06-01

    The mutagenic activity of five mono-substituted nitrobenzanthrones (NBA) has been determined in the Ames assay (Takamura-Enya et al., 2006). In the present study, a theoretical investigation of the electronic properties of all mono-substituted NBA isomers and their relation to mutagenic activity are presented. Equilibrium geometries, vertical ionization potentials (VIP), vertical electron affinities (VEA), relative energies, dipole moments and electronic dipole polarizabilities, and the IR and Raman spectra of NBA isomers calculated by Density Functional Theory (DFT) methods are presented. The position of the nitro group affects the spectral features of the IR and Raman spectra of the NBA isomers. The results show that a good linear relationship exists between the summation of Raman activities (∑ARaman) over all the 3N-6 vibrational modes and the mutagenic activity of the NBA isomers in Salmonella typhimurium strains. The spectroscopic results suggest that the unknown mutagenic activities of 4-NBA, 5-NBA, 6-NBA, 8-NBA and 10-NBA are predicted to follow the order 4-NBA>10-NBA>5-NBA>8-NBA>6-NBA. Copyright © 2013 Elsevier Ltd. All rights reserved.

  9. Determination of the excitation energy of high spin isomers

    International Nuclear Information System (INIS)

    Bjoernholm, S.; Borggreen, J.; Christensen, O.; Del Zoppo, A.; Herskind, B.; Pedersen, J.; Sletten, G.

    1979-01-01

    The sum spectrometer technique to study delayed radiation is discussed. Results on half-lives and isomer excitation energies are presented for 144 Gd, 147 Gd, 148 Tb, 151 Dy, 152 Dy, 149-153 Ho, 151 Er, 152 Er, 153 Er, and 154 Er. 2 figures, 1 table

  10. Heme isomers substantially affect heme's electronic structure and function

    DEFF Research Database (Denmark)

    Kepp, Kasper Planeta

    2017-01-01

    Inspection of heme protein structures in the protein data bank reveals four isomers of heme characterized by different relative orientations of the vinyl side chains; remarkably, all these have been reported in multiple protein structures. Density functional theory computations explain this as due...

  11. Pregnanolone isomers, pregnenolone and their polar conjugates around parturition

    Czech Academy of Sciences Publication Activity Database

    Klak, J.; Hill, M.; Pařízek, A.; Havlíková, H.; Bičíková, M.; Hampl, R.; Fait, T.; Šulcová, J.; Pouzar, Vladimír; Kancheva, R.; Stárka, L.

    2003-01-01

    Roč. 52, - (2003), s. 211-221 ISSN 0862-8408 R&D Projects: GA ČR GA303/00/1559 Institutional research plan: CEZ:AV0Z4055905 Keywords : pregnanolone isomers * pregnanolone * maternal plasma Subject RIV: CC - Organic Chemistry Impact factor: 0.939, year: 2003

  12. Fuel properties of heptadecene isomers prepared via tandem isomerization-decarboxylation of oleic acid

    Science.gov (United States)

    Heptadecene isomers were prepared via tandem isomerization-decarboxylation of oleic acid using catalytic triruthenium dodecacarbonyl [Ru3(CO)12]. Chromatographic and spectroscopic characterization of the isolated heptadecene mixture indicated that it consisted of 96% internal isomers and 4% aromatic...

  13. Aerosols and fission product transport

    International Nuclear Information System (INIS)

    Megaw, W.J.

    1987-12-01

    A survey is presented of current knowledge of the possible role of aerosols in the consequences of in- and out-of-core LOCAs and of end fitting failures in CANDU reactors. An extensive literature search has been made of research on the behaviour of aerosols in possible accidents in water moderated and cooled reactors and the results of various studies compared. It is recommended that further work should be undertaken on the formation of aerosols during these possible accidents and to study their subsequent behaviour. It is also recommended that the fission products behaviour computer code FISSCON II should be re-examined to determine whether it reflects the advances incorporated in other codes developed for light water reactors which have been extensively compared. 47 refs

  14. Geology behind nuclear fission technology

    International Nuclear Information System (INIS)

    Dhana Raju, R.

    2005-01-01

    Geology appears to have played an important role of a precursor to Nuclear Fission Technology (NFT), in the latter's both birth from the nucleus of an atom of and most important application as nuclear power extracted from Uranium (U), present in its minerals. NFT critically depends upon the availability of its basic raw material, viz., nuclear fuel as U and/ or Th, extracted from U-Th minerals of specific rock types in the earth's crust. Research and Development of the Nuclear Fuel Cycle (NFC) depends heavily on 'Geology'. In this paper, a brief review of the major branches of geology and their contributions during different stages of NFC, in the Indian scenario, is presented so as to demonstrate the important role played by 'Geology' behind the development of NFT, in general, and NFC, in particular. (author)

  15. Laser driven fusion fission hybrids

    International Nuclear Information System (INIS)

    Hansen, L.F.; Maniscalco, J.A.

    1977-11-01

    The role of the fusion-fission hybrid reactor (FFHR) as a fissile fuel and/or power producer is discussed. As long range options to supply the world energy needs, hybrid-fueled thermal-burner reactors are compared to liquid metal fast breeder reactors (LMFBR). A discussion of different fuel cycles (thorium, depleted uranium, and spent fuel) is presented in order to compare the energy multiplication, the production of fissile fuel, the laser efficiency and pellet gain requirements of the hybrid reactor. Lawrence Livermore Laboratory (LLL) has collaborated with Bechtel Corporation and with Westinghouse in two engineering design studies of laser fusion driven hybrid power plants. The hybrid designs which have resulted from these two studies are briefly described and analyzed by considering operational parameters, such as energy multiplication, power density, burn-up and plutonium production as a function time

  16. More detailed study of fission dynamics in fusion-fission reactions within a stochastic approach

    Science.gov (United States)

    Nadtochy, P. N.; Adeev, G. D.; Karpov, A. V.

    2002-06-01

    A stochastic approach based on three-dimensional Langevin equations was applied to a more detailed study of fission dynamics in fusion-fission reactions. The dynamical model has been developed and extended to investigate fission characteristics of light fissioning nuclei at low excitation energies. The energy dependences of an anisotropy of the fission fragment angular distribution, an evaporation residue cross section, a fission cross section, mean prescission neutron, and giant dipole γ multiplicities have been analyzed for the 16O+208Pb-induced fission of 224Th. Also, dependence of the prescission neutron multiplicity on the fragment mass asymmetry and total kinetic energy have been calculated. Analysis of the results shows that not only characteristics of the mass-energy distribution of fission fragments, but also the mass and kinetic-energy dependence of the prescission neutron multiplicity, the angular anisotropy, and fission probability can be reproduced using a modified one-body mechanism for nuclear dissipation with a reduction coefficient of the contribution from a wall formula ks=0.25 0.5 for compound nuclei 172Yb, 205Fr, 215Fr, and 224Th. Decrease of the prescission neutron multiplicities with fragment mass asymmetry is due to a decrease of the fission time. The results obtained show that prescission neutrons are evaporated predominantly from the nearly spherical compound nucleus at an early stage of fission process before the saddle point is reached. From performed analysis one can conclude that coordinate-independent reduction coefficient ks is not compatible with simultaneous description of the main fission characteristics for heavy fissioning systems 256Fm and 252Fm.

  17. Determination of the fission barrier height in fission of heavy radioactive beams induced by the (d,p)-transfer

    CERN Multimedia

    A theoretical framework is described, allowing to determine the fission barrier height using the observed cross sections of fission induced by the (d,p)-transfer with accuracy, which is not achievable in another type of low-energy fission of neutron-deficient nuclei, the $\\beta$-delayed fission. The primary goal is to directly determine the fission barrier height of proton-rich fissile nuclei, preferably using the radio-active beams of isotopes of odd elements, and thus confirm or exclude the low values of fission barrier heights, typically extracted using statistical calculations in the compound nucleus reactions at higher excitation energies. Calculated fission cross sections in transfer reactions of the radioactive beams show sufficient sensitivity to fission barrier height. In the probable case that fission rates will be high enough, mass asymmetry of fission fragments can be determined. Results will be relevant for nuclear astrophysics and for production of super-heavy nuclei. Transfer induced fission of...

  18. On the mechanism of fission neutron emission

    International Nuclear Information System (INIS)

    Maerten, H.; Richter, D.; Seeliger, D.

    1986-01-01

    This review represents the present knowledge of the mechanism of prompt fission neutron emission. Starting with a brief fission process characterization related with neutron emission, possible emission mechanisms are discussed. It is emphasized that the experimental study of special mechanisms, i.e. scission neutron emission processes, requires a sufficiently correct description of emission probabilities on the base of the main mechanism, i.e. the evaporation from fully accelerated fragments. Adequate statistical-model approaches have to account for the complexity of nuclear fission reflected by an intricate fragment distribution. The present picture of scission neutron emission is not clarified neither experimentally nor theoretically. Deduced data are contradictory and depend on the used analysis procedures often involving rough discriptions of evaporated-neutron distributions. The contribution of two secondary mechanisms of fission neutron emission, i.e. the neutron evaporation during fragment acceleration and neutron emission due to the decay of 5 He after ternary fission, is estimated. We summarize the recent progress of the theoretical description of fission neutron spectra in the framework of statistical models considering the standard spectrum of 252 Cf(sf) neutrons especially. The main experimental basis for the study of fission neutron emission is the accurate measurement of emission probabilities as a function of emission energy and angle (at least) as well as fragment parameters (mass number ratio and kinetic energy). The present status is evaluated. (author)

  19. Static quadrupole moment of the Kπ = 14+ isomer in 176W

    International Nuclear Information System (INIS)

    Ionescu-Bujor, M.; Iordachescu, A.; Bucurescu, D.; Brandolini, F.; Lenzi, S. M.; Pavan, P.; Rossi Alvarez, C.; Marginean, N.; Medina, N.H.; Ribas, R.V.; De Poli, M.; Napoli, D. R.; Podolyak, Zs.; Ur, C. A.

    2001-01-01

    The investigation of high-K isomeric states in the deformed nuclei of the A∼180 region has found renewed interest in recent years. Much experimental and theoretical work was devoted to understand the mechanisms which govern their decay to lower-lying states, particularly the anomalous strong decays to low-K states. Other questions of great importance are the quenching of the pairing correlations and the shape polarization effects in the high-seniority multi-quasiparticle excitations. Our interest focused on the 41 ns K π =14 + 3746 keV isomeric state with anomalous decay in 176 W. On the basis of a precise g-factor measurement we assigned to this isomer a pure four-quasiparticle configuration, composed by two protons in the 7/2 + [404] and 9/2 - [514] orbitals and two neutrons in the 7/2 + [633] and 5/2 - [512] orbitals. In the present work the measurement of its static quadrupole moment has been performed. Prior to our experiment, static quadrupole moments have been measured only for three high-K isomeric states of seniority ≥ 4 in the A∼180 region: 16 + in 178 Hf, 35/2 - in 179 W and 25 + in 182 Os. A deformation very similar to that of the ground state has been deduced for the 16 + isomer in 178 Hf, while for the high-K isomers in 179 W and 182 Os significantly smaller deformations were reported. The quadrupole interaction of the 14 + isomeric state in 176 W has been investigated in the electric field gradient (EFG) of the polycrystalline lattice of metallic Tl by applying the time-differential perturbed angular distribution method. For W impurities in Tl host the EFG strength and its temperature dependence have been recently reported. The isomer was populated in the 164 Dy( 16 O,4n) 176 W reaction using a 83 MeV 16 O pulsed beam (pulse width 1.5 ns, repetition period 800 ns) delivered by the XTU-Tandem of Laboratori Nazionali di Legnaro. The target consisted of 0.5 mg/cm 2 metallic 164 Dy on thick Tl backing in which both the recoiling 176 W nuclei and

  20. Isomers and oblate collectivity at high spin in neutron-rich Pt isotopes

    Directory of Open Access Journals (Sweden)

    Tandel S.K.

    2016-01-01

    Full Text Available Isomers and high-spin structures with rotation-aligned oblate configurations have been studied in several Pt isotopes. The 12+ states in the even Pt isotopes from 192–198Pt are found to be metastable, and have (i13/22 neutron character. The progression of E2 transition probabilities from the 12+ to 10+ states across the Pt isotopic chain implies reduction in collectivity, followed by an abrupt decrease at N=120 (198Pt. This behavior is quite distinct from the gradual decrease of B(E2 values near the respective ground states. A large contribution from aligned angular momentum, to the rotational sequences built on the 12+ states, is visible. This is due to the relatively small crossing frequencies for nucleons in low-Ω orbitals at oblate deformation in comparison to higher values for prolate shapes. As a result, oblate rotation is found to be increasingly favored for higher neutron numbers.

  1. Identifying isomers of C-78 by means of x-ray spectroscopy

    DEFF Research Database (Denmark)

    Bassan, Arianna; Nyberg, Mats; Luo, Yi

    2002-01-01

    X-ray photoelectron and absorption spectra of C-78 isomers have been generated using density functional theory with inclusion of the full core-hole potentials. Strong isomer dependence has been found in absorption, but not in the photoelectron spectra. C-78 isomers can be thought to be formed...

  2. Fission cross section measurements for minor actinides

    Energy Technology Data Exchange (ETDEWEB)

    Fursov, B. [IPPE, Obninsk (Russian Federation)

    1997-03-01

    The main task of this work is the measurement of fast neutron induced fission cross section for minor actinides of {sup 238}Pu, {sup 242m}Am, {sup 243,244,245,246,247,248}Cm. The task of the work is to increase the accuracy of data in MeV energy region. Basic experimental method, fissile samples, fission detectors and electronics, track detectors, alpha counting, neutron generation, fission rate measurement, corrections to the data and error analysis are presented in this paper. (author)

  3. Nuclear fission induced by high energy protons

    International Nuclear Information System (INIS)

    Barashenkov, V.S.; Shmakov, S.Yu.

    1979-01-01

    The fission of 203 Pb, 232 Th, 238 U, 239 Pu, 209 Br nuclei in the energy region T approximately equal to 0.1-2 GeV is considered on the basis of intranuclear cascade model. The competition between fission and evaporation of excited nuclei remaining after the cascade phase of the interaction is taken into account. Fong's model is used to calculate the fission process. The multiplicity of produced particles (d, t, 3 He, α), the energy spectra of neutrons, the distributions of residual nuclei are discussed. The calculated results are compared with the experiment and with the known theoretical data

  4. Fusion barrier distributions and fission anisotropies

    International Nuclear Information System (INIS)

    Hinde, D.J.; Morton, C.R.; Dasgupta, M.; Leigh, J.R.; Lestone, J.P.; Lemmon, R.C.; Mein, J.C.; Newton, J.O.; Timmers, H.; Rowley, N.; Kruppa, A.T.

    1995-01-01

    Fusion excitation functions for 16,17 O+ 144 Sm have been measured to high precision. The extracted fusion barrier distributions show a double-peaked structure interpreted in terms of coupling to inelastic collective excitations of the target. The effect of the positive Q-value neutron stripping channel is evident in the reaction with 17 O. Fission and evaporation residue cross-sections and excitation functions have been measured for the reaction of 16 O+ 208 Pb and the fusion barrier distribution and fission anisotropies determined. It is found that the moments of the fusion l-distribution determined from the fusion and fission measurements are in good agreement. ((orig.))

  5. Prompt fission neutron investigation in 235U(nth,f) reaction

    Science.gov (United States)

    Zeynalov, Shakir; Sedyshev, Pavel; Shvetsov, Valery; Sidorova, Olga

    2017-09-01

    The prompt neutron emission in thermal neutron induced fission of 235U has been investigated applying digital signal electronics. The goal was to compare the results of this digital data acquisition and digital signal processing analysis to the results of the pioneering work of Apalin et al. Using a twin Frisch grid ionization chamber for the fission fragment detection and a NE213 equivalent neutron detector in total about 106 neutron coincidences have been registered. The fission fragment kinetic energy, mass and angular distribution has been investigated along with prompt neutron time of flight and pulse shape using a six channel synchronous waveform digitizer with sampling frequency of 250 MHz and 12 bit resolution. The signals have been analyzed using digital pulse processing algorithms, developed by authors. The thermal neutron beam was transported from the IBR-2 reactor to the target with bent mirror neutron guide.

  6. Prompt fission neutron investigation in 235U(nth,f reaction

    Directory of Open Access Journals (Sweden)

    Zeynalov Shakir

    2017-01-01

    Full Text Available The prompt neutron emission in thermal neutron induced fission of 235U has been investigated applying digital signal electronics. The goal was to compare the results of this digital data acquisition and digital signal processing analysis to the results of the pioneering work of Apalin et al. Using a twin Frisch grid ionization chamber for the fission fragment detection and a NE213 equivalent neutron detector in total about 106 neutron coincidences have been registered. The fission fragment kinetic energy, mass and angular distribution has been investigated along with prompt neutron time of flight and pulse shape using a six channel synchronous waveform digitizer with sampling frequency of 250 MHz and 12 bit resolution. The signals have been analyzed using digital pulse processing algorithms, developed by authors. The thermal neutron beam was transported from the IBR-2 reactor to the target with bent mirror neutron guide.

  7. Charge distributions of fission fragments of low- and high-energy fission of Fm, No, and Rf isotopes

    Science.gov (United States)

    Paşca, H.; Andreev, A. V.; Adamian, G. G.; Antonenko, N. V.

    2018-03-01

    The charge (mass) distributions of fission fragments resulting from low- and high-energy fission of the even-even nuclei 254 -260 ,264Fm , 258 -264No , and 262 -266Rf are studied with the statistical scission-point model. The calculated results are compared with the available experimental data. In contrast to the experimental data, the calculated mass distribution for 258Fm (s.f.) is strikingly similar to the experimental one for 257Fm (s.f.). The transformation of the shape of charge distribution with increasing isospin and excitation energy occurs gradually and in a similar fashion like that of the mass distribution, but slower. For 254Fm(i.f.), 257Fm(nt h,f), and 260Fm (s.f.), the unexpected difference (symmetric or asymmetric) between the shapes of charge and mass distributions is predicted for the first time. At some critical excitation energy, the saturation of the symmetric component of charge (mass) yields is demonstrated.

  8. Recovery and use of fission product noble metals

    Energy Technology Data Exchange (ETDEWEB)

    Jensen, G.A.; Rohmann, C.A.; Perrigo, L.D.

    1980-06-01

    Noble metals in fission products are of strategic value. Market prices for noble metals are rising more rapidly than recovery costs. A promising concept has been developed for recovery of noble metals from fission product waste. Although the assessment was made only for the three noble metal fission products (Rh, Pd, Ru), there are other fission products and actinides which have potential value. (DLC)

  9. Recovery and use of fission product noble metals

    International Nuclear Information System (INIS)

    Jensen, G.A.; Rohmann, C.A.; Perrigo, L.D.

    1980-06-01

    Noble metals in fission products are of strategic value. Market prices for noble metals are rising more rapidly than recovery costs. A promising concept has been developed for recovery of noble metals from fission product waste. Although the assessment was made only for the three noble metal fission products (Rh, Pd, Ru), there are other fission products and actinides which have potential value

  10. Fission fragment anisotropy of 235U measured with the fissionTPC

    Science.gov (United States)

    Hensle, David; Greife, Uwe; Niffte Collaboration

    2017-09-01

    The fissionTPC, built for the purpose of making neutron-induced fission cross section measurements with unprecedented precision, is a two-chamber MICROMEGAS time projection chamber that allows for three-dimensional tracking of charged particles. This three-dimensional tracking capability also provides a direct measurement of fission fragment angular distributions for neutron-induced fission. Fragment angular anisotropy is an important experimental observable for understanding the quantum mechanical state of the fissioning nucleus and a parameter required to determine detection efficiency for cross section measurements. Preliminary results for 235U fission fragment anisotropy as a function of neutron energies in the range 130 keV - 100 MeV will be presented.

  11. Neutron emission as a probe of fusion-fission and quasi-fission dynamics

    International Nuclear Information System (INIS)

    Hinde, D.J.

    1991-01-01

    Pre- and post scission neutron yeilds have been measured as a function of projectile mass, compound nucleus fissility, and fission mass-split and total kinetic energy (TKE) for 27 fusion-fission and quasi-fission reactions induced by beams of 16,18 O, 40 Ar and 64 Ni. A new method of interpretation of experimental pre-scission neutron multiplicities ν-pre and mean kinetic energies ε ν allows the extraction of fission time scales with much less uncertainty than previously, all fusion-fission results being consistent with a dynamical time scale of (35±15) x 10 -21 s for symmetric fission. All reactions show that ν-pre falls quite rapidly with increasing mass-asymmetry; evidence is presented that for fusion-fission reactions this is partly due to a reduction of the dynamical fission time scale with mass-asymmetry. For quasi-fission, the data indicate that the pre-scission multiplicity and mean neutron kinetic energy are very sensitive to the final mass-asymmetry, but that the time scale is virtually independent of mass-asymmetry. It is concluded that for fusion-fission there is no dependence of ν-pre on TKE, whilst for 64 Ni-induced quasi-fission reactions, a strong increase of ν-pre with decreasing TKE is observed, probably largely caused by neutron emission during the acceleration time of the fission fragments in these fast reactions. Interpretation of post-scission multiplicities in terms of fragment excitation energies leads to deduced time scales consistent with those determined from the pre-scission data. 54 refs., 17 tabs., 25 figs

  12. Determination of the fission products yields, lanthanide and yttrium, in the fission of 238U with neutrons of fission spectra

    International Nuclear Information System (INIS)

    Nicoli, I.G.

    1981-06-01

    A radiochemical investigation is performed to measure the cumulative fission product yields of several lantanides and yttrium nuclides in the 238 U by fission neutron spectra. Natural and depleted uranium are irradiated under the same experimental conditions in order to find a way to subtract the contribution of the 235 U fission. 235 U percentage in the natural uranium was 3.5 times higher than in the depleted uranium. Uranium oxides samples are irradiated inside the core of the Argonaut Reactor, at the Instituto de Engenharia Nuclear, and the lantanides and yttrium are chemically separated. The fission products gamma activities were detected, counted and analysed in a system constituted by a high resolution Ge(Li) detector, 4096 multichannel analyser and a PDP-11 computer. Cumulative yields for fission products with half-lives between 1 to 33 hours are measured: 93 Y, 141 La, 142 La, 143 Ce and 149 Nd. The chain total yields are calculated. The cumulative fission yields measured for 93 Y, 141 La, 142 La, 143 Ce and 149 Nd are 4,49%, 4,54%, 4,95%, 4,16% and 1,37% respectively and they are in good agreement with the values found in the literature. (Author) [pt

  13. (d,p)-transfer induced fission of heavy radioactive beams

    CERN Document Server

    Veselsky, Martin

    2012-01-01

    (d,p)-transfer induced fission is proposed as a tool to study low energy fission of exotic heavy nuclei. Primary goal is to directly determine the fission barrier height of proton-rich fissile nuclei, preferably using the radio-active beams of isotopes of odd elements, and thus confirm or exclude the low values of fission barrier heights, typically extracted using statistical calculations in the compound nucleus reactions at higher excitation energies. Calculated fission cross sections in transfer reactions of the radioactive beams show sufficient sensitivity to fission barrier height. In the probable case that fission rates will be high enough, mass asymmetry of fission fragments can be determined. Results will be relevant for nuclear astrophysics and for production of super-heavy nuclei. Transfer induced fission offers a possibility for systematic study the low energy fission of heavy exotic nuclei at the ISOLDE.

  14. Independent fission yields of Rb and Cs from thermal-neutron-induced fission of 239Pu

    International Nuclear Information System (INIS)

    Balestrini, S.J.; Forman, L.

    1975-01-01

    The relative independent fission yields of Rb and Cs from thermal-neutron-induced fission of 239 Pu have been measured on line using a mass spectrograph and thermalized neutrons from a burst reactor. Independent yields were derived by normalizing the measurements to products of chain yields and fractional independent yields, estimating the latter from measured cumulative yields of Kr and Xe. Comparing the independent yields with those from 238 U fission, the 239 Pu results show shifts in isotopic yield distribution toward lower mass for both Rb and Cs and also toward the production of more Cs and less Rb when 239 Pu is fissioned

  15. Angular momenta of fission fragments in the {alpha}-accompanied fission of {sup 252}Cf

    Energy Technology Data Exchange (ETDEWEB)

    Jandel, M.; Kliman, J.; Krupa, L.; Morhac, M. [Slovak Academy of Sciences, Department of Nuclear Physics, Bratislava (Slovakia); Joint Institute for Nuclear Research, Flerov Laboratory for Nuclear Reactions, Dubna (Russian Federation); Hamilton, J.H.; Kormicki, J.; Ramayya, A.V.; Hwang, J.K.; Luo, Y.X.; Fong, D.; Gore, P. [Vanderbilt University, Department of Physics, Nashville, TN (United States); Ter-Akopian, G.M.; Oganessian, Yu.Ts.; Rodin, A.M.; Fomichev, A.S.; Popeko, G.S. [Joint Institute for Nuclear Research, Flerov Laboratory for Nuclear Reactions, Dubna (Russian Federation); Daniel, A.V. [Lawrence Berkeley National Laboratory, Berkeley, CA (United States); Rasmussen, J.O.; Macchiavelli, A.O.; Stoyer, M.A. [Lawrence Livermore National Laboratory, Livermore, CA (United States); Donangelo, R.; Cole, J.D.

    2005-06-01

    For the first time, average angular momenta of the ternary fission fragments {sup 100,102}Zr, {sup 106}Mo, {sup 144,146}Ba and {sup 138,140,142}Xe from the {alpha}-accompanied fission of {sup 252}Cf were obtained from relative intensities of prompt {gamma}-ray transitions with the use of the statistical model calculation. Average values of the angular momenta were compared with the corresponding values for the same fission fragments from the binary fission of {sup 252}Cf. Results indicate the presence of a decreasing trend in the average values of angular momenta induced in ternary fission fragments compared to the same binary fission fragments. On the average, the total angular momentum extracted for ternary fission fragments is {proportional_to}1.4{Dirac_h} lower than in binary fission. Consequently, results indicate that the mechanism of the ternary {alpha}-particles emission may directly effect an induction of angular momenta of fission fragments, and possible scenarios of such mechanisms are discussed. Further, the dependence of the angular momenta of {sup 106}Mo and {sup 140}Xe on the number of emitted neutrons from correlated pairs of primary fragments was obtained also showing a decreasing dependence of average angular momenta with increasing number of emitted neutrons. Consequences are briefly discussed. (orig.)

  16. The LANL/LLNL Prompt Fission Neutron Spectrum Program at LANSCE and Approach to Uncertainties

    Energy Technology Data Exchange (ETDEWEB)

    Haight, R.C., E-mail: haight@lanl.gov [Los Alamos National Laboratory, Los Alamos, NM 87545,USA (United States); Wu, C.Y. [Lawrence Livermore National Laboratory, Livermore, CA 94551 (United States); Lee, H.Y.; Taddeucci, T.N.; Perdue, B.A.; O' Donnell, J.M.; Fotiades, N.; Devlin, M.; Ullmann, J.L.; Bredeweg, T.A.; Jandel, M.; Nelson, R.O.; Wender, S.A.; Neudecker, D.; Rising, M.E.; Mosby, S.; Sjue, S.; White, M.C. [Los Alamos National Laboratory, Los Alamos, NM 87545,USA (United States); Bucher, B.; Henderson, R. [Lawrence Livermore National Laboratory, Livermore, CA 94551 (United States)

    2015-01-15

    New data on the prompt fission neutron spectra (PFNS) from neutron-induced fission with higher accuracies are needed to resolve discrepancies in the literature and to address gaps in the experimental data. The Chi-Nu project, conducted jointly by LANL and LLNL, aims to measure the shape of the PFNS for fission of {sup 239}Pu induced by neutrons from 0.5 to 20 MeV with accuracies of 3–5% in the outgoing energy from 0.1 to 9 MeV and 15% from 9 to 12 MeV and to provide detailed experimental uncertainties. Neutrons from the WNR/LANSCE neutron source are being used to induce fission in a Parallel-Plate Avalanche Counter (PPAC). Two arrays of neutron detectors are used to cover the energy range of neutrons emitted promptly in the fission process. Challenges for the present experiment include background reduction, use of {sup 239}Pu in a PPAC, and understanding neutron detector response. Achieving the target accuracies requires the understanding of many systematic uncertainties. The status and plans for the future will be presented.

  17. The LANL/LLNL Prompt Fission Neutron Spectrum Program at LANSCE and Approach to Uncertainties

    Science.gov (United States)

    Haight, R. C.; Wu, C. Y.; Lee, H. Y.; Taddeucci, T. N.; Perdue, B. A.; O'Donnell, J. M.; Fotiades, N.; Devlin, M.; Ullmann, J. L.; Bredeweg, T. A.; Jandel, M.; Nelson, R. O.; Wender, S. A.; Neudecker, D.; Rising, M. E.; Mosby, S.; Sjue, S.; White, M. C.; Bucher, B.; Henderson, R.

    2015-01-01

    New data on the prompt fission neutron spectra (PFNS) from neutron-induced fission with higher accuracies are needed to resolve discrepancies in the literature and to address gaps in the experimental data. The Chi-Nu project, conducted jointly by LANL and LLNL, aims to measure the shape of the PFNS for fission of 239Pu induced by neutrons from 0.5 to 20 MeV with accuracies of 3-5% in the outgoing energy from 0.1 to 9 MeV and 15% from 9 to 12 MeV and to provide detailed experimental uncertainties. Neutrons from the WNR/LANSCE neutron source are being used to induce fission in a Parallel-Plate Avalanche Counter (PPAC). Two arrays of neutron detectors are used to cover the energy range of neutrons emitted promptly in the fission process. Challenges for the present experiment include background reduction, use of 239Pu in a PPAC, and understanding neutron detector response. Achieving the target accuracies requires the understanding of many systematic uncertainties. The status and plans for the future will be presented.

  18. Even-odd effects in the prompt fission emission of even Z actinides

    Directory of Open Access Journals (Sweden)

    Tudora Anabella

    2016-01-01

    Full Text Available The investigation of even-odd effects in the prompt emission of even Z actinides showed a sawtooth shape of ν(Z with staggering in the asymmetric fission region. Average prompt emission quantities as a function of A, e.g. ν(A, of even Z fragmentations are higher than those of odd Z fragmentations and they exhibit oscillations with a periodicity of about 5 mass units in the asymmetric fission region. This periodicity is not due to the Z even-odd effect in fragment distributions. The even-odd effect in (TKE is increasing with increasing TKE and it decreases with increasing mass of the fissioning nucleus. The global even-odd effect in total average prompt emission quantities is decreasing with increasing mass of the fissioning nucleus. In the case of an even-odd fissioning nucleus, 234U(n,f, the global even-odd effect in prompt emission quantities exhibits a very slow variation with the incident neutron energy.

  19. Development of fission Mo-99 production technology

    International Nuclear Information System (INIS)

    Park, Jin Ho; Choung, W. M.; Lee, K. I. and others

    2000-05-01

    Fission Mo-99 is the only parent nuclide of Tc-99m, an extremely useful tool for mdeical diagnosis, with an estimated usage of greater than 80% of nuclear medicine applicatons. HEU and LEU targets to optimize in HANARO irradiation condition suggested and designed for domestic production of fission Mo-99. The optimum process conditions are established in each unit process to meet quality requirements of fission Mo-99 products, and the results of performance test in combined process show Mo separation and purification yield of the above 97%. The concept of Tc generator production process is established, and the result of performance test show Tc production yield of 98.4% in Tc generator procuction process. The drafts is prepared for cooperation of technical cooperation and business investment with foreign country. Evaluation on economic feasibility is accompanied for fission Mo-99 and Tc-99m generator production

  20. Energy from nuclear fission an introduction

    CERN Document Server

    De Sanctis, Enzo; Ripani, Marco

    2016-01-01

    This book provides an overview on nuclear physics and energy production from nuclear fission. It serves as a readable and reliable source of information for anyone who wants to have a well-balanced opinion about exploitation of nuclear fission in power plants. The text is divided into two parts; the first covers the basics of nuclear forces and properties of nuclei, nuclear collisions, nuclear stability, radioactivity, and provides a detailed discussion of nuclear fission and relevant topics in its application to energy production. The second part covers the basic technical aspects of nuclear fission reactors, nuclear fuel cycle and resources, safety, safeguards, and radioactive waste management. The book also contains a discussion of the biological effects of nuclear radiation and of radiation protection, and a summary of the ten most relevant nuclear accidents. The book is suitable for undergraduates in physics, nuclear engineering and other science subjects. However, the mathematics is kept at a level that...

  1. Is channeling of fission tracks taking place?

    CERN Document Server

    Yada, K

    1999-01-01

    A single crystal of natural zircon which is sliced to have (010) basal plane and thinned by ion thinning is electron microscopically observed after slow neutron irradiation to ascertain whether channeling of the nuclear fission fragments is taking place or not. A fairly large number of the induced fission tracks are recognized at low magnification images where a considerable number of them are parallel to low-index lattice planes such as 100, 001, 101, 301, 103 though their directions changed some time up to several degrees. High resolution images of fission tracks often show a variety of zigzag passing of the tracks along low-index lattice planes in atomistic level. The rate of the tracks which are parallel to these low-index lattice planes is fairly high as about 45%, which strongly suggests that channeling of the fission tracks is taking place.

  2. Development of fission Mo-99 production technology

    Energy Technology Data Exchange (ETDEWEB)

    Park, Jin Ho; Choung, W. M.; Lee, K. I. and others

    2000-05-01

    Fission Mo-99 is the only parent nuclide of Tc-99m, an extremely useful tool for mdeical diagnosis, with an estimated usage of greater than 80% of nuclear medicine applicatons. HEU and LEU targets to optimize in HANARO irradiation condition suggested and designed for domestic production of fission Mo-99. The optimum process conditions are established in each unit process to meet quality requirements of fission Mo-99 products, and the results of performance test in combined process show Mo separation and purification yield of the above 97%. The concept of Tc generator production process is established, and the result of performance test show Tc production yield of 98.4% in Tc generator procuction process. The drafts is prepared for cooperation of technical cooperation and business investment with foreign country. Evaluation on economic feasibility is accompanied for fission Mo-99 and Tc-99m generator production.

  3. Fission cross section measurements at intermediate energies

    International Nuclear Information System (INIS)

    Laptev, Alexander

    2005-01-01

    The activity in intermediate energy particle induced fission cross-section measurements of Pu, U isotopes, minor actinides and sub-actinides in PNPI of Russia is reviewed. The neutron-induced fission cross-section measurements are under way in the wide energy range of incident neutrons from 0.5 MeV to 200 MeV at the GNEIS facility. In number of experiments at the GNEIS facility, the neutron-induced fission cross sections were obtained for many nuclei. In another group of experiments the proton-induced fission cross-section have been measured for proton energies ranging from 200 to 1000 MeV at 100 MeV intervals using the proton beam of PNPI synchrocyclotron. (author)

  4. Uranium deposits obtention for fission chambers

    International Nuclear Information System (INIS)

    Artacho Saviron, E.

    1972-01-01

    The obtention of uranium deposits of the required quality for small cylindrical fission chambers presents some difficulties. With the method of electroplating here described the uniformity, reproducibility and adherence of the obtained deposits were satisfactory. (Author) 6 refs

  5. Decay and fission of the oriented nuclei

    CERN Document Server

    Kadmenskij, S G

    2002-01-01

    The fragment angular distributions for binary decay of oriented spherical and deformed nuclei with taking into account the correct transformational properties of wave functions under time inversion have been investigated. It has been shown that for description of fragment angular distributions the adiabatic approximation for collective rotational nuclear degrees of freedom is not correct. It has been demonstrated that this approximation is valid for description of spontaneous and induced low-energy nuclear fission. The dependence of partial fission widths on the orientation of the internal axes spins, projections of spins, and relative angular moments of fission fragments has been analyzed. It has been shown that the adiabatic approximation results in coherent interference of wave functions of fragments relative movement. This interference forms fragments the universal angular distributions of fission fragments for oriented nuclei. For these distributions the deviations from A. Bohr's formula have been invest...

  6. Mass and Charge Distribution in Low-Energy Fission

    International Nuclear Information System (INIS)

    Wahl, A.C.

    1965-01-01

    The mass and charge distributions for thermal-neutron fission of U 235 are discussed in considerable detail and compared with the corresponding distributions in other low-energy fission processes. Points discussed in connection with the mass distributions for binary fission include the positions of the peaks, valley and fine structure in a mass yield curve with respect to filled nuclear shells and the changes in the positions that occur with changing fissioning nucleus and excitation energy. The mass distribution from ternary fission is discussed also. For both binary and ternary fission comments are made concerning the mass distributions of primary fragments (before neutron evaporation) and of fission products (after neutron evaporation). Charge distribution is discussed in terms of charge dispersion among fission products with the same mass number and the variation with mass number of Zp, the ''most probable charge'' (non-integral) for a given mass number. Although direct information about charge distribution is limited to fission products, estimates are presented of charge distribution for primary fission fragments. Knowledge and estimates of mass and charge distribution for a fission process allow estimation of primary yields of all fission products or fragments. Although many estimated primary yields are quite uncertain mainly because of lack of knowledge of charge distribution, especially for fission products formed in low yield; some estimates of primary yields are presented to illustrate the need for and possible practicality of further experimentation. Fission processes other than thermal-neutron fission of U 235 that are discussed include thermal-neutron fission of U 233 and Pu 239 , spontaneous fission of Pu 240 and Cf 252 , 14-MeV neutron fission of U 235 and U 238 , 11-MeV proton fission of Ra 226 and 22-MeV deuteron fission of Bi 209 . (author) [fr

  7. The Search for High Spin State Isomers in the Atomic Mass Region 178-192

    International Nuclear Information System (INIS)

    Ellahrah, M.S.; Arfa, N.S.

    2007-01-01

    Isomers for elements far a way from line of stability are a new field for research to produce artificial isomers that can store considerable amount of energy in small amount of mass without the dangerous hazards on life and environment. These isomers could have very short life time or very long one 10th and 100th of years. It will be possible to get the stored energy by stimulated emission . The purpose of this work to use a theorical model based on Bcs method to find out the possible isomers in the mass reg on 178-192 even -even isotopes so that experimentalists can concentrate their research on these predicted isomers.

  8. A revised calculational model for fission

    International Nuclear Information System (INIS)

    Atchison, F.

    1998-09-01

    A semi-empirical parametrization has been developed to calculate the fission contribution to evaporative de-excitation of nuclei with a very wide range of charge, mass and excitation-energy and also the nuclear states of the scission products. The calculational model reproduces measured values (cross-sections, mass distributions, etc.) for a wide range of fissioning systems: Nuclei from Ta to Cf, interactions involving nucleons up to medium energy and light ions. (author)

  9. Hyperfission - a new mode of nuclear fission

    International Nuclear Information System (INIS)

    Ion, D.B.; Ivascu, M.; Ion-Mihai, R.

    1988-02-01

    In this paper the nuclear hyperfission as a new mode of fission, possible for heavy elements with Z > 92, is investigated. The Q-systematics, hyperfissibility parameters, hyperfission barrier as well as the essential hindrance factors are presented. The hyperfission hindrance factor relative to that of fission is found to be in the interval 1.0x10 -17 - 3.4x10 -16 for the parent nuclei with Z = 92-108. (orig.)

  10. Live Cell Imaging in Fission Yeast.

    Science.gov (United States)

    Mulvihill, Daniel P

    2017-10-03

    Live cell imaging complements the array of biochemical and molecular genetic approaches to provide a comprehensive insight into functional dependencies and molecular interactions in fission yeast. Fluorescent proteins and vital dyes reveal dynamic changes in the spatial distribution of organelles and the proteome and how each alters in response to changes in environmental and genetic composition. This introduction discusses key issues and basic image analysis for live cell imaging of fission yeast. © 2017 Cold Spring Harbor Laboratory Press.

  11. Transport properties of fission product vapors

    International Nuclear Information System (INIS)

    Im, K.H.; Ahluwalia, R.K.

    1983-07-01

    Kinetic theory of gases is used to calculate the transport properties of fission product vapors in a steam and hydrogen environment. Provided in tabular form is diffusivity of steam and hydrogen, viscosity and thermal conductivity of the gaseous mixture, and diffusivity of cesium iodide, cesium hydroxide, diatomic tellurium and tellurium dioxide. These transport properties are required in determining the thermal-hydraulics of and fission product transport in light water reactors

  12. Modeling Fission Product Sorption in Graphite Structures

    International Nuclear Information System (INIS)

    Szlufarska, Izabela; Morgan, Dane; Allen, Todd

    2013-01-01

    The goal of this project is to determine changes in adsorption and desorption of fission products to/from nuclear-grade graphite in response to a changing chemical environment. First, the project team will employ principle calculations and thermodynamic analysis to predict stability of fission products on graphite in the presence of structural defects commonly observed in very high-temperature reactor (VHTR) graphites. Desorption rates will be determined as a function of partial pressure of oxygen and iodine, relative humidity, and temperature. They will then carry out experimental characterization to determine the statistical distribution of structural features. This structural information will yield distributions of binding sites to be used as an input for a sorption model. Sorption isotherms calculated under this project will contribute to understanding of the physical bases of the source terms that are used in higher-level codes that model fission product transport and retention in graphite. The project will include the following tasks: Perform structural characterization of the VHTR graphite to determine crystallographic phases, defect structures and their distribution, volume fraction of coke, and amount of sp2 versus sp3 bonding. This information will be used as guidance for ab initio modeling and as input for sorptivity models; Perform ab initio calculations of binding energies to determine stability of fission products on the different sorption sites present in nuclear graphite microstructures. The project will use density functional theory (DFT) methods to calculate binding energies in vacuum and in oxidizing environments. The team will also calculate stability of iodine complexes with fission products on graphite sorption sites; Model graphite sorption isotherms to quantify concentration of fission products in graphite. The binding energies will be combined with a Langmuir isotherm statistical model to predict the sorbed concentration of fission products

  13. Modeling Fission Product Sorption in Graphite Structures

    Energy Technology Data Exchange (ETDEWEB)

    Szlufarska, Izabela [University of Wisconsin, Madison, WI (United States); Morgan, Dane [University of Wisconsin, Madison, WI (United States); Allen, Todd [University of Wisconsin, Madison, WI (United States)

    2013-04-08

    The goal of this project is to determine changes in adsorption and desorption of fission products to/from nuclear-grade graphite in response to a changing chemical environment. First, the project team will employ principle calculations and thermodynamic analysis to predict stability of fission products on graphite in the presence of structural defects commonly observed in very high- temperature reactor (VHTR) graphites. Desorption rates will be determined as a function of partial pressure of oxygen and iodine, relative humidity, and temperature. They will then carry out experimental characterization to determine the statistical distribution of structural features. This structural information will yield distributions of binding sites to be used as an input for a sorption model. Sorption isotherms calculated under this project will contribute to understanding of the physical bases of the source terms that are used in higher-level codes that model fission product transport and retention in graphite. The project will include the following tasks: Perform structural characterization of the VHTR graphite to determine crystallographic phases, defect structures and their distribution, volume fraction of coke, and amount of sp2 versus sp3 bonding. This information will be used as guidance for ab initio modeling and as input for sorptivity models; Perform ab initio calculations of binding energies to determine stability of fission products on the different sorption sites present in nuclear graphite microstructures. The project will use density functional theory (DFT) methods to calculate binding energies in vacuum and in oxidizing environments. The team will also calculate stability of iodine complexes with fission products on graphite sorption sites; Model graphite sorption isotherms to quantify concentration of fission products in graphite. The binding energies will be combined with a Langmuir isotherm statistical model to predict the sorbed concentration of fission

  14. Overview of tritium fast-fission yields

    International Nuclear Information System (INIS)

    Tanner, J.E.

    1981-03-01

    Tritium production rates are very important to the development of fast reactors because tritium may be produced at a greater rate in fast reactors than in light water reactors. This report focuses on tritium production and does not evaluate the transport and eventual release of the tritium in a fast reactor system. However, if an order-of-magnitude increase in fast fission yields for tritium is confirmed, fission will become the dominant production source of tritium in fast reactors

  15. Experimental Studies of quasi-fission reactions

    International Nuclear Information System (INIS)

    Back, B.B.

    1989-01-01

    A large number of recent experimental studies have shown that a substantial fraction of the total reaction cross section in heavy-ion reactions is found in fission-like processes, which do not result from the fission decay of a completely fused system. Following the suggestion of Swiatecki such processes, which represents a complete relaxation of the relative kinetic energy and a substantial amount of net mass transfer between the two fragments, are denoted quasi-fission reactions. They are distinct from compound fission reactions by bypassing the stage of a completely fused system. This typically means that they are associated with short reaction times, which results in several measurable characteristics such as broken forward-backward symmetries, large anisotropies of the angular distributions and increased widths of the fragment mass distributions. The distinction between quasi-fission and deep inelastic reactions is less stringent and has the character of a gradual evolution from one reaction type to the other, as found also as quasi-elastic reaction evolves into deeply inelastic processes as a function of the total kinetic energy loss. In the present paper some of the experimental data characterizing quasi-fission reactions are reviewed and discussed. (author)

  16. Spontaneous fission of the heaviest elements

    Energy Technology Data Exchange (ETDEWEB)

    Hoffman, D.C.

    1989-04-01

    Although spontaneous fission was discovered in /sup 238/U in 1940, detailed studies of the process were first made possible in the 1960's with the availability of milligram quantities of /sup 252/Cf. The advent of solid-state detectors made it possible to perform measurements of coincident fission fragments from even very short-lived spontaneous fission activities or those available in only very small quantities. Until 1971 it was believed that the main features of the mass and kinetic-energy distributions were essentially the same as those for thermal neutron-induced fission and that all low-energy fission proceeded via asymmetric mass division with total kinetic energies which could be derived by linear extrapolation from those of lighter elements. In 1971, measurements of /sup 257/Fm showed an increase in symmetric mass division with anomalously high TKE's. Subsequent experiments showed that in /sup 258/Fm and /sup 259/Fm, the most probable mass split was symmetric with very high total kinetic energy. Measurements for the heavier elements have shown symmetric mass distributions with both high and low total kinetic energies. Recent results for spontaneous fission properties of the heaviest elements are reviewed and compared with theory. 31 refs., 8 figs., 1 tab.

  17. Isomer-specific consumption of galactooligosaccharides by bifidobacterial species

    Science.gov (United States)

    Tsui, Man Ki; Mills, David A.; Lebrilla, Carlito B.

    2014-01-01

    Prebiotics are non-digestible substrates that stimulate the growth of beneficial microbes in the human intestine. Galactooligosaccharides (GOS) are food ingredients that possess prebiotic properties, in particular, promoting the growth of bifidobacteria in situ. However precise mechanistic details of GOS consumption by bifidobacteria remains poorly understood. Because GOS are mixtures of polymers of different lengths and linkages, there is interest to determine which specific structures provide prebiotic effects in order to potentially create better supplements. We here present a method comprising porous graphitic carbon separation, isotopic labeling and mass spectrometry analysis for the structure specific analysis of GOS isomers and their bacterial consumption rate. Using this strategy, the differential bacterial consumption of GOS by the bifidobacteria species B. longum subsp. infantis, B. animalis subsp. lactis and B. adolescentis was determined, indicating that the use of specific GOS isomers in infant formula may provide enrichment of distinct species. PMID:24313277

  18. Inmersiones isométricas en variedades riemannianas

    Directory of Open Access Journals (Sweden)

    Carlos Alberto Marín Arango

    2011-06-01

    Full Text Available Este trabajo recapitula la teoría básica de conexiones en fibrados principales y fibrados vectoriales con el fin de aplicar tales teorías al estudio de inmersiones isométricas en variedades riemannianas; por medio de una versión apropiada del teorema de Frobenius mostramos un resultado que generaliza el teorema fundamental de las inmersiones isométricas. Abstract. This paper summarizes the basic theory of connections in principal bundles and vector bundles in order to apply these theories to the study of isometric immersions in Riemannian manifolds; by an appropriate version of the Frobenius theorem we show a result that generalizes the Fundamental Theorem of isometric immersions.

  19. The Gamma Resonance Problem of Long-Lived Nuclear Isomers

    Science.gov (United States)

    Davydov, Andrey V.

    2001-07-01

    A review is given of the studies relating to the problem of γ-resonant (Mössbauer) excitation of long-lived nuclear isomers. The theoretical estimates of possible γ-line broadening are presented. Earlier experiments are described with 107mAg and 109mAg isomers using polycrystalline samples of pure Ag and Ag-Pd alloys. The results of these experiments did not contradict the theoretical predictions. The series of papers using Ag single-crystal γ-sources is reviewed. Their results were interpreted as indications of a rather small 109mAg γ-line broadening, which cannot be explained by modern theory. The results of the last experiments by ITEP group with 109mAg are also presented. These data may be coordinated with results of other research, if one takes into account the Zeeman splitting of the γ-spectra by Earth's magnetic field.

  20. Biological effectiveness of fission neutrons

    International Nuclear Information System (INIS)

    Sasaki, M.S.; Saigusa, S.; Kimura, I.

    1992-01-01

    Human peripheral blood lymphocytes were exposed to the uranium fission neutrons with different energy spectra, and the effects of changing pattern of energy spectrum on the relative biological effectiveness (RBE) were studied by analyzing dose-response relationship of chromosome aberrations. When the contribution of contaminated gamma-rays was subtracted, the efficiency of chromosomal response to the neutron dose was found to be refractory to the difference in the energy spectrum while the mean energy ranged from 2 MeV to 27 keV. This chromosomal refractoriness to energy spectrum may be explained by the similarity of energy spectrum for kerma contribution; most of the doses being given by neutrons with energy above 50 keV. Small doses given by short tracks may be less efficient. A comparison of these observations with chromosome aberration frequencies in lymphocytes of A-bomb survivors leads to somewhat higher estimate of neutron dose in Hiroshima than the estimate by the recently revised dosimetry system, DS86. (author)

  1. Fission of Polyanionic Metal Clusters

    Science.gov (United States)

    König, S.; Jankowski, A.; Marx, G.; Schweikhard, L.; Wolfram, M.

    2018-04-01

    Size-selected dianionic lead clusters Pbn2 -, n =34 - 56 , are stored in a Penning trap and studied with respect to their decay products upon photoexcitation. Contrary to the decay of other dianionic metal clusters, these lead clusters show a variety of decay channels. The mass spectra of the fragments are compared to the corresponding spectra of the monoanionic precursors. This comparison leads to the conclusion that, in the cluster size region below about n =48 , the fission reaction Pbn2 -→Pbn-10 -+Pb10- is the major decay process. Its disappearance at larger cluster sizes may be an indication of a nonmetal to metal transition. Recently, the pair of Pb10- and Pbn-10 - were observed as pronounced fragments in electron-attachment studies [S. König et al., Int. J. Mass Spectrom. 421, 129 (2017), 10.1016/j.ijms.2017.06.009]. The present findings suggest that this combination is the fingerprint of the decay of doubly charged lead clusters. With this assumption, the dianion clusters have been traced down to Pb212 -, whereas the smallest size for the direct observation was as high as n =28 .

  2. Fission-fusion neutron source

    Science.gov (United States)

    Yu, Jinnan; Yu, Gang

    2009-04-01

    In order to meet the requirements of fusion power reactors and nuclear waste treatment, a concept of fission-fusion neutron source is proposed, which consists of a LiD assembly located in the heavy water region of the China Advanced Research Reactor. This assembly of LiD fuel rods will be irradiated with slow neutrons and will produce fusion neutrons in the central hole via the reaction 6Li(n, α). More precisely, tritium ions with a high energy of 2.739 MeV will be produced in LiD by the impinging slow neutrons. The tritium ions will in turn bombard the deuterium ions present in the LiD assembly, which will induce fusion reaction and then the production of 14 MeV neutrons. The fusion reaction rate will increase with the accumulation of tritium in LiD by the reaction between tritium and deuteron recoils produced by the 14 MeV neutrons. When the concentration of tritium reaches 0.5 · 10 22 and the fraction of fusion reactions between tritium and deuteron recoils approaches 1, the 14 MeV neutron flux is doubled and redoubled, an so forth, approaching saturation in which the tritium produced at a time t is exhausted by the fusion reactions to keep constant the tritium concentration in LiD.

  3. High spin states and Yrast isomers in 211Rn

    International Nuclear Information System (INIS)

    Poletti, A.R.; Dracoulis, G.D.; Fahlander, C.; Morrison, I.

    1981-01-01

    Excited states in 211 Rn with spins up to 53/2 have been identified using (HI,xn) reactions and γ-ray techniques. A shell model calculation can reproduce the ordering of the yrast sequence up to spin 41/2 - . Several yrast isomers have been identified. Enhanced E3 transitions are observed and their systematic occurrence in this region discussed. The influence of the neutron hole, and possible core excitations on the effective moment of inertia are also pointed out

  4. Island of high-spin isomers near N = 82

    International Nuclear Information System (INIS)

    Pedersen, J.; Back, B.B.; Bernthal, F.M.; Bjornholm, S.; Borggreen, J.; Christensen, O.; Folkmann, F.; Herskind, B.; Khoo, T.L.; Neiman, M.; Puehlhofer, F.; Sletten, G.

    1977-01-01

    Experiments aimed at testing for the existence of yrast traps are reported. A search for delayed γ radiation of lifetimes longer than approx. 10 ns and of high multiplicity has been performed by producing more than 100 compound nuclei between Ba and Pb in bombardments with 40 Ar, 50 Ti, and 65 Cu projectiles. An island of high-spin isomers is found to exist in the region 64 or approx. = 71 and N < or approx. = 82

  5. High spin states and yrast isomers in 211Rn

    International Nuclear Information System (INIS)

    Poletti, A.R.; Dracoulis, G.D.; Fahlander, C.; Morrison, I.

    1980-12-01

    Excited states in 211 Rn with spins up to 53/2 have been identified using (HI,xn) reactions and γ-ray techniques. A shell model calculation can reproduce the ordering of the yrast sequence up to spin 41/2. Several yrast isomers have been identified. Enhanced E3 transitions are observed and their systematic occurrence in this region discussed. The influence of the neutron hole, and possible core excitations on the effective moment of inertia are also pointed out

  6. Observation of the new isomer 32mAl

    International Nuclear Information System (INIS)

    Robinson, M.; Halse, P.; Lewitowicz, M.; Saint-Laurent, M.G.

    1995-01-01

    A new isomer in the neutron-rich isotope 32 Al has been identified among the fragmentation products of a 40 Ar 16+ beam using the LISE spectrometer at GANIL. The population of the isomeric state was inferred from the detection of γ-radiation following its decay in coincidence with its respective heavy-ion implantation signal. The half-life of 32m Al was determined to be 240 ± 30 ns. (author)

  7. Butane isomer separation with composite zeolite MFI mebranes

    Czech Academy of Sciences Publication Activity Database

    Hrabánek, Pavel; Zikánová, Arlette; Bernauer, B.; Fíla, V.; Kočiřík, Milan

    2009-01-01

    Roč. 245, 1-3 (2009), s. 437-443 ISSN 0011-9164 R&D Projects: GA ČR GA203/07/1443; GA AV ČR KAN400720701; GA AV ČR(CZ) 1QS401250509 Institutional research plan: CEZ:AV0Z40400503 Keywords : zeolite MFI * membranes * separation * butane isomers Subject RIV: CF - Physical ; Theoretical Chemistry Impact factor: 2.034, year: 2009

  8. Characteristics of Butanol Isomers Oxidation in a Micro Flow Reactor

    KAUST Repository

    Bin Hamzah, Muhamad Firdaus

    2017-05-01

    Ignition and combustion characteristics of n-butanol/air, 2-butanol.air and isobutanol/air mixtures at stoichiometric (ϕ = 1) and lean (ϕ = 0.5) conditions were investigated in a micro flow reactor with a controlled temperature profile from 323 K to 1313 K, under atmospheric pressure. Sole distinctive weak flame was observed for each mixture, with inlet fuel/air mixture velocity set low at 2 cm/s. One-dimensional computation with comprehensive chemistry and transport was conducted. At low mixture velocities, one-stage oxidation was confirmed from heat release rate profiles, which was broadly in agreement with the experimental results. The weak flame positions were congruent with literature describing reactivity of the butanol isomers. These weak flame responses were also found to mirror the trend in Anti-Knock Indexes of the butanol isomers. Flux and sensitivity analyses were performed to investigate the fuel oxidation pathways at low and high temperatures. Further computational investigations on oxidation of butanol isomers at higher pressure of 5 atm indicated two-stage oxidation through the heat release rate profiles. Low temperature chemistry is accentuated in the region near the first weak cool flame for oxidation under higher pressure, and its impact on key species – such as hydroxyl radical, hydrogen peroxide and carbon monoxide – were considered. Both experimental and computational findings demonstrate the advantage of employing the micro flow reactor in investigating oxidation processes in the temperature region of interest along the reactor channel. By varying physical conditions such as pressure, the micro flow reactor system is proven to be highly beneficial in elucidating oxidation behavior of butanol isomers in conditions in engines such as those that mirror HCCI operations.

  9. Comparison of the Weisskopf estimates in spin and K-isomers

    International Nuclear Information System (INIS)

    Garg, Swati; Maheshwari, B.; Rajput, Rohit; Srivastava, P.C.; Jain, A.K.

    2014-01-01

    Nuclear isomers are the excited metastable states, which exist due to the hindrance on their decay. Study of isomers has recently become very popular due to advances in the experimental techniques and also the arrival of radioactive beams. Large amount of new experimental data is becoming available. The very first 'Atlas of nuclear isomers' lists more than 2460 nuclear isomers with the half-life cut off at 10 ns. Spin isomers mostly exist due to the difficulty in meeting the spin selection rules and cluster around the semi-magic regions. The isomers far from the magic-numbers, which lie in the well-deformed region, mostly exist due to the goodness of the K-quantum number and large K-difference between the decaying states. They are known as K-isomers

  10. Isomer probes of nuclear structure following deep inelastic collisions

    CERN Document Server

    Al-Garni, S A; Walker, P

    2002-01-01

    Deep-inelastic collisions of sup 1 sup 3 sup 6 Xe ions with tantalum, tungsten and rhenium targets have been used to study beta-decays and high-spin isomers in neutron-rich A approx 180 nuclei at the GSI on-line mass separator. In particular, gamma rays -associated with the decay of the previously identified K suppi = 37/2 sup - , T sub 1 sub / sub 2 = 51 min isomer in sup 1 sup 7 sup 7 Hf have been observed, but with an unexpectedly high yield considering the release efficiency for short-lived hafnium isotopes from a thermal ion source. These results may be interpreted as possible evidence for a hitherto unrecognised, high-spin beta-decaying isomer in sup 1 sup 7 sup 7 Lu. A two-component half-life analysis of the sup 1 sup 7 sup 7 Hf gamma-ray intensities gives an upper-lying component of 6 + 3 - 2 min, when the lower-lying component half-life is fixed at 51 min. Nilsson multi-quasiparticle calculations with BCS pairing predict a favoured K suppi = 39/2 sup - state in sup 1 sup 7 sup 7 Lu, which is a candid...

  11. Correlated prompt fission data in transport simulations

    Science.gov (United States)

    Talou, P.; Vogt, R.; Randrup, J.; Rising, M. E.; Pozzi, S. A.; Verbeke, J.; Andrews, M. T.; Clarke, S. D.; Jaffke, P.; Jandel, M.; Kawano, T.; Marcath, M. J.; Meierbachtol, K.; Nakae, L.; Rusev, G.; Sood, A.; Stetcu, I.; Walker, C.

    2018-01-01

    Detailed information on the fission process can be inferred from the observation, modeling and theoretical understanding of prompt fission neutron and γ-ray observables. Beyond simple average quantities, the study of distributions and correlations in prompt data, e.g., multiplicity-dependent neutron and γ-ray spectra, angular distributions of the emitted particles, n - n, n - γ, and γ - γ correlations, can place stringent constraints on fission models and parameters that would otherwise be free to be tuned separately to represent individual fission observables. The FREYA and CGMF codes have been developed to follow the sequential emissions of prompt neutrons and γ rays from the initial excited fission fragments produced right after scission. Both codes implement Monte Carlo techniques to sample initial fission fragment configurations in mass, charge and kinetic energy and sample probabilities of neutron and γ emission at each stage of the decay. This approach naturally leads to using simple but powerful statistical techniques to infer distributions and correlations among many observables and model parameters. The comparison of model calculations with experimental data provides a rich arena for testing various nuclear physics models such as those related to the nuclear structure and level densities of neutron-rich nuclei, the γ-ray strength functions of dipole and quadrupole transitions, the mechanism for dividing the excitation energy between the two nascent fragments near scission, and the mechanisms behind the production of angular momentum in the fragments, etc. Beyond the obvious interest from a fundamental physics point of view, such studies are also important for addressing data needs in various nuclear applications. The inclusion of the FREYA and CGMF codes into the MCNP6.2 and MCNPX - PoliMi transport codes, for instance, provides a new and powerful tool to simulate correlated fission events in neutron transport calculations important in

  12. Asymmetry in ternary fission induced by polarized neutrons and fission mechanism

    International Nuclear Information System (INIS)

    Bunakov, V.E.; Gennenvajn, F.; Dzhessinger, P.; Mutterer, M.; Petrov, G.A.

    2003-01-01

    The results of measuring the P-odd, P-even (right-left) and T-odd asymmetries of the charged particles emission in the double and ternary fission, induced by the polarized neutrons, are considered. It is shown, what kind of information on the mechanism of the ternary nuclear fission may be obtained from the theoretical analysis of these data [ru

  13. Nuclear spectroscopy by radioactivity. Study of nuclei adjacent to the 82 neutron closed shell and application to fission

    International Nuclear Information System (INIS)

    Carraz, L.-C.

    1974-01-01

    Chemical separation techniques have been developed which make it possible to obtain a certain number of isotopes presenting anomalies in the fission efficiencies (near the magic shell N=82). A short description is given of the fission phenomenon by analysing the selection of isotopes investigated; it is shown how it was possible to explain the results by means of computers and the various chemical separations perfected are described. Thus a study was made of the 144 La direct γ spectrum. It was shown that the anomalies in the fission efficiencies of certain nuclei are apparent only. Hence, it is the presence of isomers and the distribution of the corresponding efficiency between two isomers which are the cause of the apparent weakness of the efficiency of 134 I, 136 I and 136 Cs, and of certain isotopes of Nb(Z=41). The nuclear spectrometry of nuclei of the area N=82 has made it possible to extend the existence of a metastable state to 136 Xe and 138 Ba. The value of the energies of the first 2 + , 4 + , 6 + levels and the half life duration of the 6 + metastable state are given. The discussion of the results and of the models show that the interpretation of the 0 + , 2 + , 4 + of the 82 neutron nuclei by means of a two quasi-particle (protons) model gives a fairly satisfactory description of the various experimental events: elastic scattering, gamma spectrometry and proton transfer reactions; on the other hand the interpretation of higher energy levels, requires the use of more complicated configurations [fr

  14. Actinide nuclide deposit preparation for fission chambers; Elaboration de depots de radionucleides d'actinides pour chambres a fissions

    Energy Technology Data Exchange (ETDEWEB)

    Maillard, Ch.; Adnet, J.M. [CEA Valrho, (DCC/DRRV/SPHA), 30 - Marcoule (France); Blandin, Ch. [CEA Cadarache, Direction des Reacteurs Nucleaires (DRN/DER/SSAE), 13 - Saint-Paul-lez-Durance (France)

    2000-07-01

    Fission chambers are basically gas ionization detectors where one electrode is coated with fissile material. For many years, the Fuel Cycle Division has been contributing to the manufacture of fission chambers (traditional domain of the Nuclear Research Division) by providing the fissile material deposits. In 9999, a transfer of knowledge about the manufacture of deposits on cylindrical electrodes (i.e. imposed current electrolysis) took place between the two Division. This transfer resulted in the installation of a new generation of experimental rigs for electrolysis, the development of procedures designed to obtain very high accuracy on the fissile mass deposited, and the performance of several electro-depositions of actinide radionuclides. Thanks to the use of machined parts and the study of the shape of certain parts, the new electrolysis rig offers easy installation and disassembly of the various parts, maintenance of a constant distance between the electrodes, and minimized trapping of hydrogen bubbles formed at the cathode during electrolysis. The latter two qualities are necessary to obtain a homogeneous deposit. The knowledge of the mass deposited and its uncertainty are essential data for the users of the fission ionization chambers. In the procedure selected, isotopic dilution is combined with ICP-MS analysis to measure the radioelement content of the electrolyte before and after electrodeposition, and to weigh the electrolyte. These measurement techniques help determine the fissile mass deposited with a low uncertainty (approximately 2 %) (see Tables I and II). To validate the procedures, ten electrolytic deposits of plutonium and uranium with deposition mass ranging from 100 {mu}g to 5 mg were carried out on cylindrical metallic electrodes 0.7 mm, 2.5 mm and 6.5 mm in diameter (Table I). The deposits were uniform and displayed good adherence. However, the electrolysis yields varied (20 to 99 %) with electrodeposition yields ranging from 80 % to 100

  15. Fission-product yields for thermal-neutron fission of curium-243

    International Nuclear Information System (INIS)

    Breederland, D.G.

    1982-01-01

    Cumulative fission yields for 25 gamma rays emitted during the decay of 23 fission products produced by thermal-neutron fission of 243 Cm have been determined. Using Ge(Li) spectroscopy, 33 successive pulse-height spectra of gamma rays emitted from a 77-ng sample of 243 Cm over a period of approximately two and one-half months were analyzed. Reduction of these spectra resulted in the identification and matching of gamma-ray energies and half-lives to specific radionuclides. Using these results, 23 cumulative fission-product yields were calculated. Only those radionuclides having half-lives between 6 hours and 65 days were observed. Prior to this experiment, no fission-product yields had been recorded for 243 Cm

  16. Mechanism of cytokinetic contractile ring constriction in fission yeast.

    Science.gov (United States)

    Stachowiak, Matthew R; Laplante, Caroline; Chin, Harvey F; Guirao, Boris; Karatekin, Erdem; Pollard, Thomas D; O'Shaughnessy, Ben

    2014-06-09

    Cytokinesis involves constriction of a contractile actomyosin ring. The mechanisms generating ring tension and setting the constriction rate remain unknown because the organization of the ring is poorly characterized, its tension was rarely measured, and constriction is coupled to other processes. To isolate ring mechanisms, we studied fission yeast protoplasts, in which constriction occurs without the cell wall. Exploiting the absence of cell wall and actin cortex, we measured ring tension and imaged ring organization, which was dynamic and disordered. Computer simulations based on the amounts and biochemical properties of the key proteins showed that they spontaneously self-organize into a tension-generating bundle. Together with rapid component turnover, the self-organization mechanism continuously reassembles and remodels the constricting ring. Ring constriction depended on cell shape, revealing that the ring operates close to conditions of isometric tension. Thus, the fission yeast ring sets its own tension, but other processes set the constriction rate. Copyright © 2014 Elsevier Inc. All rights reserved.

  17. Theoretical study of different features of the fission process of excited nuclei in the framework of the modified statistical model and four-dimensional dynamical model

    Science.gov (United States)

    Eslamizadeh, H.

    2017-02-01

    Evaporation residue cross section, fission probability, anisotropy of fission fragment angular distribution, mass and energy distributions of fission fragments and the pre-scission neutron multiplicity for the excited compound nuclei {}168{{Y}}{{b}}, {}172{{Y}}{{b}}, {}178{{W}} and {}227{{P}}{{a}} produced in fusion reactions have been calculated in the framework of the modified statistical model and multidimensional dynamical model. In the dynamical calculations, the dynamics of fission of excited nuclei has been studied by solving three- and four-dimensional Langevin equations with dissipation generated through the chaos-weighted wall and window friction formula. Three collective shape coordinates plus the projection of total spin of the compound nucleus to the symmetry axis, K, were considered in the four-dimensional dynamical model. A non-constant dissipation coefficient of K, {γ }k, was applied in the four-dimensional dynamical calculations. A comparison of the results of the three- and four-dimensional dynamical models with the experimental data showed that the results of the four-dimensional dynamical model for the evaporation residue cross section, fission probability, anisotropy of fission fragment angular distribution, mass and energy distributions of fission fragments and the pre-scission neutron multiplicity are in better agreement with the experimental data. It was also shown that the modified statistical model can reproduce the above-mentioned experimental data by choosing appropriate values of the temperature coefficient of the effective potential, λ , and the scaling factor of the fission-barrier height, {r}s.

  18. Fission Surface Power Technology Development Update

    Science.gov (United States)

    Palac, Donald T.; Mason, Lee S.; Houts, Michael G.; Harlow, Scott

    2011-01-01

    Power is a critical consideration in planning exploration of the surfaces of the Moon, Mars, and places beyond. Nuclear power is an important option, especially for locations in the solar system where sunlight is limited or environmental conditions are challenging (e.g., extreme cold, dust storms). NASA and the Department of Energy are maintaining the option for fission surface power for the Moon and Mars by developing and demonstrating technology for a fission surface power system. The Fission Surface Power Systems project has focused on subscale component and subsystem demonstrations to address the feasibility of a low-risk, low-cost approach to space nuclear power for surface missions. Laboratory demonstrations of the liquid metal pump, reactor control drum drive, power conversion, heat rejection, and power management and distribution technologies have validated that the fundamental characteristics and performance of these components and subsystems are consistent with a Fission Surface Power preliminary reference concept. In addition, subscale versions of a non-nuclear reactor simulator, using electric resistance heating in place of the reactor fuel, have been built and operated with liquid metal sodium-potassium and helium/xenon gas heat transfer loops, demonstrating the viability of establishing system-level performance and characteristics of fission surface power technologies without requiring a nuclear reactor. While some component and subsystem testing will continue through 2011 and beyond, the results to date provide sufficient confidence to proceed with system level technology readiness demonstration. To demonstrate the system level readiness of fission surface power in an operationally relevant environment (the primary goal of the Fission Surface Power Systems project), a full scale, 1/4 power Technology Demonstration Unit (TDU) is under development. The TDU will consist of a non-nuclear reactor simulator, a sodium-potassium heat transfer loop, a power

  19. Four-quasiparticle isomers and K-forbidden transitions in 176Lu

    International Nuclear Information System (INIS)

    McGoram, T.R.; Dracoulis, G.D.; Kibedi, T.; Mullins, M.; Byrne, A.P.; Baxter, A.M.

    2000-01-01

    Full text: The odd-odd nucleus 176 Lu has been the subject of extensive experimental and theoretical investigation over the last forty years. Much of this interest has stemmed from the role of 176 Lu in the s-process in nucleosynthesis. From a nuclear structure perspective, 176 Lu resides in a region of the nuclear chart where collective rotation and high-K, multi-quasiparticle states compete to form the yrast line (the locus of state with the lowest energy at a given angular momentum). The electromagnetic decay of intermediate and high-K states is often hindered due to the K-selection rule, while apparent violations of this selection rule have been ascribed to Coriolis mixing, shape changes in the gamma-degree of freedom, and so-called 'statistical' mixing. The relative importance of these mechanisms remains an open question. We present here the results of gamma-ray and conversion-electron spectroscopic measurements, performed at the Heavy Ion Facility at the Australian National University in Canberra, using the reaction 176 Yb( 7 Li, α3n) at a beam energy of 45 MeV. Two new four-quasiparticle isomers have been established, with mean lives of 400(100)ns and 58(5)μs, and spin projections and parities of 12 + and (14 + ) respectively. The shorter--lived isomer displays both normal and anomalous K-forbidden decays, which we show is the result of two-state mixing between the isomeric state and a member of a two-quasiparticle rotational band. The implied mixing matrix element of only 5 eV shows explicitly that very small mixing matrix elements may be responsible for anomalous K-hindered decays

  20. An improved technique for fission track dating

    International Nuclear Information System (INIS)

    Zhao Yunlong; Wu Zhaohui; Xia Yuliang

    1996-01-01

    The necessity of improving the fission track dating (FTD) technique both at home and abroad is illustrated. The ways of making such improvement are also proposed. It is suggested to calibrate the constant b value of the uranium standard glass by using the method of fission products activity. The 3 kinds of uranium standard glass which have been calibrated are NBS SRM962a, UB 1 and UB 2 . An established new method σ·Φ ρ d /b, to measure neutron fluence, avoids the influence of the varying neutron spectrum on measuring neutron fluence. The improved etching technique for fission tracks in zircon adopted a two-step method which includes the molten alkali system etching using NaOH + KOH and the mixed acid system etching using HNO 3 + HF; this technique results in adequate track etching, increased track clarity and less interference. In this way the intensity of tracks is authentically reflected. Dividing angular zone in accordance with the angular distribution of spontaneous fission track on the crystal surface of minerals to count the tracks and using the improved etching technique to remove the non-uniform angular distribution of spontaneous fission tracks in zircon, ensure the accuracy of tracks count. The improved FTD techniques were used to finish Laboratory Standardized Calibration. The tests using international FTD age standards samples have proved that above mentioned techniques are reliable and practical in obtaining the accurate FTD data. (8 tabs.; 3 figs.)

  1. Theoretical models of neutron emission in fission

    International Nuclear Information System (INIS)

    Madland, D.G.

    1992-01-01

    A brief survey of theoretical representations of two of the observables in neutron emission in fission is given, namely, the prompt fission neutron spectrum N(E) and the average prompt neutron multiplicity bar v p . Early representations of the two observables are presented and their deficiencies are discussed. This is followed by summaries and examples of recent theoretical models for the calculation of these quantities. Emphasis is placed upon the predictability and accuracy of the new models. In particular, the dependencies of N(E) and bar v p upon the fissioning nucleus and its excitation energy are treated. Recent work in the calculation of the prompt fission neutron spectrum matrix N(E,E n ), where E n is the energy of the neutron inducing fission, is then discussed. Concluding remarks address the current status of our ability to calculate these observables with confidence, the direction of future theoretical efforts, and limititations to current and future calculations. Finally, recommendations are presented as to which model should be used currently and which model should be pursued in future efforts

  2. Theory of neutron emission in fission

    International Nuclear Information System (INIS)

    Madland, D.G.

    1998-01-01

    A survey of theoretical representations of two of the observables in neutron emission in fission is given, namely, the prompt fission neutron spectrum N(E) and the average prompt neutron multiplicity bar ν p . Early representations of the two observables are presented and their deficiencies are discussed. This is followed by summaries and some examples of recent theoretical models for the calculation of these quantities. Emphasis is placed upon the predictability and accuracy of the recent models. In particular, the dependencies of N(E) and bar ν p upon the fissioning nucleus and its excitation energy are treated in detail for the Los Alamos model. Recent work in the calculation of the prompt fission neutron spectrum matrix N(E, E n ), where E n is the energy of the neutron inducing fission, is then discussed. Concluding remarks address the current status of the ability to calculate these observables with confidence, the direction of future theoretical efforts, and limitations to current (and future) approaches. This paper is an extension of a similar paper presented at the International Centre for Theoretical Physics in 1996

  3. Fission characteristics of the excited compound nucleus 210Rn in the framework of the four-dimensional dynamical model

    Science.gov (United States)

    Eslamizadeh, H.; Ahadi, E.

    2017-09-01

    The evaporation residue cross section, the anisotropy of the fission fragments angular distribution, the fission probability, the mass-energy distribution of the fission fragments, and the average prescission neutron multiplicity have been calculated for the compound nucleus 210Rn by using four-dimensional Langevin equations with dissipation generated through the chaos-weighted wall and window friction formula. Three collective shape coordinates plus the projection of the total spin of the compound nucleus to the symmetry axis K were considered in the four-dimensional dynamical model. In the dynamical calculations dissipation coefficient of K ,γk was considered as a free parameter, and its magnitude was inferred by fitting measured data on the evaporation residue cross section and the anisotropy of the fission fragments angular distribution for the compound nucleus 210Rn. It was shown that the results of the calculations are in good agreement with the experimental data by using values of the dissipation coefficient of K , equal to γk=(0 .185 -0 .200 ) (MeVzs) -1 /1 22 . It also was shown that the influence of the dissipation coefficient of K on the results of the calculations of the fission probability, the mass-energy distribution of the fission fragments, and the average prescission neutron multiplicity for the compound nucleus 210Rn is small.

  4. Electron microscopic investigations of tracks of Cf252 fission fragments in quartz glass

    International Nuclear Information System (INIS)

    Werba, T.; Granzer, F.

    1977-01-01

    Using a single stage carbon replication technique, track pits of Cf 252 -fission products in quartz glass could be revealed by transmission electron microscopy with a high degree of resolution. From the shape of the track pits the angles of incidence of the nuclear particles were determined down to extremely small angles. In addition track pits on the fracture surface of irradiated quartz glass samples have been investigated by scanning electron microscopy. (author)

  5. Complementing ultrafast shape recognition with an optical isomerism descriptor.

    Science.gov (United States)

    Zhou, Ting; Lafleur, Karine; Caflisch, Amedeo

    2010-11-01

    We introduce the mixed product of three vectors spanning four molecular locations as a descriptor of optical isomerism. This descriptor is very efficient as it does not require molecular superposition, and is very robust in discriminating between a given isomer and its mirror image. In particular, conformational isomers that are mirror images of each other, as well as optical isomers have opposite sign of the descriptor value. For efficient database searches, the optical isomerism descriptor can be used to complement an available ultrafast shape recognition (USR) method based solely on distances, which is not able to distinguish enantiomers. By an extensive comparison of the USR-based similarity score with an approach based on Gaussian molecular volume overlap, the accuracy and completeness of the former are discussed. Copyright © 2010 Elsevier Inc. All rights reserved.

  6. Dynamical simulation of the fission process and anisotropy of the fission fragment angular distributions of excited nuclei produced in fusion reactions

    Science.gov (United States)

    Eslamizadeh, H.

    2016-10-01

    Abstract. A stochastic approach based on four-dimensional Langevin equations was applied to calculate the anisotropy of fission fragment angular distributions, average prescission neutron multiplicity, and the fission probability in a wide range of fissile parameters for the compound nuclei 197Tl,225Pa,248Cf , and 264Rf produced in fusion reactions. Three collective shape coordinates plus the projection of total spin of the compound nucleus to the symmetry axis K were considered in the four-dimensional dynamical model. In the dynamical calculations, nuclear dissipation was generated through the chaos-weighted wall and window friction formula. Furthermore, in the dynamical calculations the dissipation coefficient of K ,γk was considered as a free parameter, and its magnitude inferred by fitting measured data on the anisotropy of fission fragment angular distributions for the compound nuclei 197Tl,225Pa,248Cf , and 264Rf. Comparison of the calculated results for the anisotropy of fission fragment angular distributions with the experimental data showed that the results of the calculations are in good agreement with the experimental data by using values of the dissipation coefficient of K equal to (0.185-0.205), (0.175-0.192), (0.077-0.090), and (0.075-0.085) (MeVzs ) -1 /2 for the compound nuclei 197Tl,225Pa,248Cf , and 264Rf, respectively. It was also shown that the influence of the dissipation coefficient of K on the results of the calculations of the prescission neutron multiplicity and fission probability is small.

  7. Fusion-fission study at IUAC: Recent results

    Science.gov (United States)

    Pullanhiotan, Sugathan

    2016-10-01

    Several properties observed in heavy ion induced fission led to the conclusion that fission is not always originated from fully equilibrated compound nucleus. Soon after the collision of two nuclei, it forms a di-nuclear system than can fission before a compound nucleus is formed. This process termed quasi-fission is a major hurdle to the formation of heavier elements by fusion. Fission originated before complete equilibration showed anomalously large angular anisotropy and mass distribution wider than what is expected from compound nucleus fission. The standard statistical model fails to predict the outcome of quasi-fission and currently no dynamical model is fully developed to predict all the features of quasi-fission. Though much progress has been made in recent times, a full understanding of the fission dynamics is still missing. Experiments identifying the influence of entrance channel parameters on dynamics of fusion-fission showed contrasting results. At IUAC accelerator facility many experiments have been performed to make a systematic study of fission dynamics using mass distribution, angular distribution and neutron multiplicity measurements in mass region around A ∼ 200. Recent measurement on mass distribution of fission fragment from reaction 19 F +206,208 Pb around fusion barrier energy showed the influence of multi-mode fission in enhancing the mass variance at low excitation energy. In this talk I will present some of these results.

  8. Accurate isotopic fission yields of electromagnetically induced fission of 238U measured in inverse kinematics at relativistic energies

    Science.gov (United States)

    Pellereau, E.; Taïeb, J.; Chatillon, A.; Alvarez-Pol, H.; Audouin, L.; Ayyad, Y.; Bélier, G.; Benlliure, J.; Boutoux, G.; Caamaño, M.; Casarejos, E.; Cortina-Gil, D.; Ebran, A.; Farget, F.; Fernández-Domínguez, B.; Gorbinet, T.; Grente, L.; Heinz, A.; Johansson, H.; Jurado, B.; Kelić-Heil, A.; Kurz, N.; Laurent, B.; Martin, J.-F.; Nociforo, C.; Paradela, C.; Pietri, S.; Rodríguez-Sánchez, J. L.; Schmidt, K.-H.; Simon, H.; Tassan-Got, L.; Vargas, J.; Voss, B.; Weick, H.

    2017-05-01

    SOFIA (Studies On Fission with Aladin) is a novel experimental program, dedicated to accurate measurements of fission-fragment isotopic yields. The setup allows us to fully identify, in nuclear charge and mass, both fission fragments in coincidence for the whole fission-fragment range. It was installed at the GSI facility (Darmstadt), to benefit from the relativistic heavy-ion beams available there, and thus to use inverse kinematics. This paper reports on fission yields obtained in electromagnetically induced fission of 238U.

  9. Fission products in glasses. Pt. 2

    International Nuclear Information System (INIS)

    De, A.K.; Luckscheiter, B.; Malow, G.; Schiewer, E.

    1977-09-01

    Glass ceramics of different composition with high leach and impact resistance can be produced for fission product solidification. In contrast to commercial glass products, they consist of a number of crystalline phases and a residual glass phase. The major crystalline phase allows a classification into celsian, diopside, encryptite, and perovskite ceramics. They all are of special importance as host phases for long-lived fission products. The paper reports on relations between product composition and melting properties, viscosity, crystallization properties, and fixation capability for fission products. Further investigations deal with dimensional stability, impact resistance, thermal expansion, and thermal conductivity. The properties of the ceramics are compared with those of the basic products. The problems still to be solved with regard to further improvement and application of these products are discussed. (RB) [de

  10. Tight connection between fission gas discharge channels

    International Nuclear Information System (INIS)

    Jung, W.; Peehs, M.; Rau, P.; Krug, W.; Stechemesser, H.

    1978-01-01

    The invention is concerned with the tight connection between the fission gas discharge channel, leading away from the support plate of a gas-cooled reactor, and the top of the fuel element suspended from this support plate. The closure is designed to be gas-tight for the suspended as well as for the released fuel element. The tight connection has got an annular body resting on the core support plate in the mouth region of the fission gas discharge channel. This body is connected with the fission gas discharge channel in the fuel element top fitting via a gas-tight part and supported by a compression spring. Care is taken for sealing if the fuel element is removal. (RW) [de

  11. Dynamical Model of Fission Fragment Angular Distribution

    Science.gov (United States)

    Drozdov, V. A.; Eremenko, D. O.; Fotina, O. V.; Platonov, S. Yu.; Yuminov, O. A.; Giardina, G.; Taccone, A.

    2002-01-01

    A dynamical model of fission fragment angular distributions is suggested. The model allows one to calculate fission fragment angular distributions, prescission light particle multyplicities, evaporation residue cross sections etc. for the cases of decay of hot and rotating heavy nuclei. The experimental data on angular anisotropies of fission fragments and prescission neutron multiplicities are analyzed for the 16O + 208Pb, 232Th, 248Cm and 238U reactions at the energies of the incident 16O ions ranging from 90 to 160 MeV. This analysis allows us to extract both the nuclear friction coefficient value and the relaxation time for the tilting mode. It is also demonstrated that the angular distributions are sensitive to the deformation dependence of the nuclear friction.

  12. Antiproton Induced Fission and Fragmentation of Nuclei

    CERN Multimedia

    2002-01-01

    The annihilation of slow antiprotons with nuclei results in a large highly localized energy deposition primarily on the nuclear surface. \\\\ \\\\ The study of antiproton induced fission and fragmentation processes is expected to yield new information on special nuclear matter states, unexplored fission modes, multifragmentation of nuclei, and intranuclear cascades.\\\\ \\\\ In order to investigate the antiproton-nucleus interaction and the processes following the antiproton annihilation at the nucleus, we propose the following experiments: \\item A)~Measurement of several fragments from fission and from multifragmentation in coincidence with particle spectra, especially neutrons and kaons. \\item B)~Precise spectra of $\\pi$, K, n, p, d and t with time-of-flight techniques. \\item C)~Installation of the Berlin 4$\\pi$ neutron detector with a 4$\\pi$ Si detector placed inside for fragments and charged particles. This yields neutron multiplicity distributions and consequently distributions of thermal excitation energies and...

  13. Lunar surface fission power supplies: Radiation issues

    International Nuclear Information System (INIS)

    Houts, M.G.; Lee, S.K.

    1994-01-01

    A lunar space fission power supply shield that uses a combination of lunar regolith and materials brought from earth may be optimal for early lunar outposts and bases. This type of shield can be designed such that the fission power supply does not have to be moved from its landing configuration, minimizing handling and required equipment on the lunar surface. Mechanisms for removing heat from the lunar regolith are built into the shield, and can be tested on earth. Regolith activation is greatly reduced compared with a shield that uses only regolith, and it is possible to keep the thermal conditions of the fission power supply close to those seen in free space. For a well designed shield, the additional mass required to be brought from earth should be less than 1,000 kg. Detailed radiation transport calculations confirm the feasibility of such a shield

  14. Solar vs. Fission Surface Power for Mars

    Science.gov (United States)

    Rucker, Michelle A.; Oleson, Steve; George, Pat; Landis, Geoffrey A.; Fincannon, James; Bogner, Amee; Jones, Robert E.; Turnbull, Elizabeth; Martini, Michael C.; Gyekenyesi, John Z.; hide

    2016-01-01

    A multi-discipline team of experts from the National Aeronautics and Space Administration (NASA) developed Mars surface power system point design solutions for two conceptual missions. The primary goal of this study was to compare the relative merits of solar- versus fission-powered versions of each surface mission. First, the team compared three different solar power options against a fission power system concept for a sub-scale, uncrewed demonstration mission. The 4.5 meter (m) diameter pathfinder lander's primary mission would be to demonstrate Mars entry, descent, and landing techniques. Once on the Martian surface, the lander's In Situ Resource Utilization (ISRU) payload would demonstrate liquid oxygen propellant production using atmospheric resources. For the purpose of this exercise, location was assumed to be at the Martian equator. The three solar concepts considered included a system that only operated during daylight hours (at roughly half the daily propellant production rate of a round-the-clock fission design), a battery-augmented system that operated through the night (matching the fission concept's propellant production rate), and a system that operated only during daylight, but at a higher rate (again, matching the fission concept's propellant production rate). Including 30% mass growth allowance, total payload masses for the three solar concepts ranged from 1,116 to 2,396 kg, versus the 2,686 kg fission power scheme. However, solar power masses are expected to approach or exceed the fission payload mass at landing sites further from the equator, making landing site selection a key driver in the final power system decision. The team also noted that detailed reliability analysis should be performed on daytime-only solar power schemes to assess potential issues with frequent ISRU system on/off cycling. Next, the team developed a solar-powered point design solution for a conceptual four-crew, 500-day surface mission consisting of up to four landers per

  15. Asymmetric Fission in the 78Kr+40Ca reactions at 5.5 MeV/nucleon

    Directory of Open Access Journals (Sweden)

    Roy R.

    2012-02-01

    Full Text Available The cross section, kinetic energy distribution and angular distribution of fragments with atomic number 3 ≤ Z ≤ 28 emitted in the reaction 78Kr + 40Ca at the bombarding energy of 5.5 MeV/nucleon and coincidence between light charged particles and fragments were measured by means of the 4π-INDRA array to study the decay mechanism of medium mass excited nucleus. Global features indicate a high degree of relaxation and are compatible with a binary fission from compound nucleus. The mean value of the kinetic energy distributions of fragments indicates dominance of Coulomb interaction, while the width of the distribution signals large fluctuations. Inclusive cross-section distributions of fragments with charge 3 ≤ Z ≤ 28 are bell-shaped and a strong even-odd-staggering (o-es is observed for 3 ≤ Z ≤ 12. Coincidence measurements suggest that the light partners in very asymmetric fission are emitted at excitation energies below the particle emission thresholds. Data were confronted to the predictions of statistical model describing the decay of compound nuclei by emission of light particles and fragments. Calculations assuming spherical fission fragments and finite-range liquid drop fission barriers are not able to explain the experimental features. Attempts have been made to improve the agreement with experimental data. The analysis indicates the strong influence of the shape parameterization of the potential energy surface in describing the fission process of intermediate mass compound nuclei.

  16. Decay of Plutonium isotopes via spontaneous and heavy-ion induced fission paths

    Science.gov (United States)

    Sharma, Kanishka; Sawhney, Gudveen; Sharma, Manoj K.; Gupta, Raj K.

    2018-04-01

    Based on the collective clusterization approach, we have extended our earlier study on α-decay, exotic cluster-decay, and heavy particle radioactivity, to the phenomenon of spontaneous fission (SF) in the ground-state (g.s.) decays of even mass 234-246Pu parents. The calculations for the SF half-lives of these Pu-isotopes have been made within the framework of preformed cluster model (PCM), both for spherical as well as β2-deformed choices of shapes, and a comparison is made with the relevant available experimental data, which prefer spherical shapes. The importance of the orientation degree of freedom (hot compact or cold elongated configurations) is also explored. Next, in order to look for the exclusive role of heavy-ion induced fission, the dynamics of 6He + 238U reaction forming 244Pu* is studied over the center of mass energy range of E c . m . = 15.0- 28.8MeV, using the dynamical cluster-decay model (DCM), an extension of the PCM with temperature T- and angular momentum ℓ-effects included. The β2-deformed fragments of 244Pu* in the mass range A2 = 106- 113 (plus their complementary heavy fragments), corresponding to asymmetric fission peaks, are found contributing towards the fission cross-section. Finally, the potential energy surfaces and barrier modification effects are presented for the relative comparison of spontaneous and the heavy-ion induced fission processes. Both are found to behave similar with respect to the probable emission of fragments and hence point out to the shell closure property of the decay fragments.

  17. Modeling the Fission Fragment Detection Efficiency of the NIFFTE fissionTPC

    Science.gov (United States)

    Bowden, Nathaniel; Niffte Collaboration

    2017-09-01

    The goal of the Neutron Induced Fission Fragment Tracking Experiment (NIFFTE) is to measure neutron-induced fission cross section ratios with unprecedented precision. The NIFFTE Collaboration has designed and built a Time Projection Chamber, the fissionTPC, for this purpose. The detector enables charged particle tracking with full three-dimensional charge cloud reconstruction, allowing for the characterization of fission fragments originating from a thin central target. Quantifying the fission fragment detection efficiency is a central element of these cross section ratio measurements. Here we describe how the wealth of data captured for every fission event allows us to build and validate a detailed Monte Carlo efficiency model. Effects such as anisotropy, fission fragment energy degradation, and target thickness, composition, and roughness must all be taken into account. LLNL-ABS-733618. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

  18. Study on fission blanket fuel cycling of a fusion-fission hybrid energy generation system

    International Nuclear Information System (INIS)

    Zhou, Z.; Yang, Y.; Xu, H.

    2011-01-01

    This paper presents a preliminary study on neutron physics characteristics of a light water cooled fission blanket for a new type subcritical fusion-fission hybrid reactor aiming at electric power generation with low technical limits of fission fuel. The major objective is to study the fission fuel cycling performance in the blanket, which may possess significant impacts on the feasibility of the new concept of fusion-fission hybrid reactor with a high energy gain (M) and tritium breeding ratio (TBR). The COUPLE2 code developed by the Institute of Nuclear and New Energy Technology of Tsinghua University is employed to simulate the neutronic behaviour in the blanket. COUPLE2 combines the particle transport code MCNPX with the fuel depletion code ORIGEN2. The code calculation results show that soft neutron spectrum can yield M > 20 while maintaining TBR >1.15 and the conversion ratio of fissile materials CR > 1 in a reasonably long refuelling cycle (>five years). The preliminary results also indicate that it is rather promising to design a high-performance light water cooled fission blanket of fusion-fission hybrid reactor for electric power generation by directly loading natural or depleted uranium if an ITER-scale tokamak fusion neutron source is achievable.

  19. Coincident measurements of prompt fission γ rays and fission fragments at DANCE

    Science.gov (United States)

    Walker, C. L.; Baramsai, B.; Jandel, M.; Rusev, G.; Couture, A.; Mosby, S.; Ullmann, J.; Kawano, T.; Stetcu, I.; Talou, P.

    2015-10-01

    Modern statistical approaches to modeling fission involve the calculation of not only average quantities but also fully correlated distributions of all fission products. Applications such as those involving the detection of special nuclear materials also rely on fully correlated data of fission products. Experimental measurements of correlated data are thus critical to the validation of theory and the development of important applications. The goal of this experiment was to measure properties of prompt fission gamma-ray emission as a function of fission fragments' total kinetic energy in the spontaneous fission of 252Cf. The measurement was carried out at the Detector for Advanced Neutron Capture Experiments (DANCE), a 4 π γ-ray calorimeter. A prototype design consisting of two silicon detectors was installed in the center of DANCE, allowing simultaneous measurement of fission fragments and γ rays. Effort has been taken to simulate fragment kinetic energy losses as well as γ-ray attenuation in DANCE using such tools as GEANT4 and SRIM. Theoretical predictions generated by the code CGMF were also incorporated as input for these simulations. Results from the experiment and simulations will be presented, along with plans for future measurements.

  20. Solar Versus Fission Surface Power for Mars

    Science.gov (United States)

    Rucker, Michelle A.; Oleson, Steve; George, Pat; Landis, Geoffrey A.; Fincannon, James; Bogner, Amee; Jones, Robert E.; Turnbull, Elizabeth; McNatt, Jeremiah; Martini, Michael C.; hide

    2016-01-01

    A multi-discipline team of experts from the National Aeronautics and Space Administration (NASA) developed Mars surface power system point design solutions for two conceptual missions to Mars using In-situ resource utilization (ISRU). The primary goal of this study was to compare the relative merits of solar- versus fission-powered versions of each surface mission. First, the team compared three different solar-power options against a fission power system concept for a sub-scale, uncrewed demonstration mission. This “pathfinder” design utilized a 4.5 meter diameter lander. Its primary mission would be to demonstrate Mars entry, descent, and landing techniques. Once on the Martian surface, the lander’s ISRU payload would demonstrate liquid oxygen propellant production from atmospheric resources. For the purpose of this exercise, location was assumed to be at the Martian equator. The three solar concepts considered included a system that only operated during daylight hours (at roughly half the daily propellant production rate of a round-the-clock fission design), a battery-augmented system that operated through the night (matching the fission concept’s propellant production rate), and a system that operated only during daylight, but at a higher rate (again, matching the fission concept’s propellant production rate). Including 30% mass growth allowance, total payload masses for the three solar concepts ranged from 1,128 to 2,425 kg, versus the 2,751 kg fission power scheme. However, solar power masses increase as landing sites are selected further from the equator, making landing site selection a key driver in the final power system decision. The team also noted that detailed reliability analysis should be performed on daytime-only solar power schemes to assess potential issues with frequent ISRU system on/off cycling.

  1. Three minor valepotriate isomers from Valeriana jatamansi and their cytotoxicity.

    Science.gov (United States)

    Lin, Sheng; Fu, Peng; Chen, Tao; Ye, Ji; Yang, Xian-Wen; Zhang, Wei-Dong

    2017-01-01

    Three new minor valepotriate isomers, jatamanvaltrates Z1 (1), Z2 (2), and Z3 (3), have been isolated from the whole plants of Valeriana jatamansi (syn. Valeriana wallichii.). Their structures were elucidated by extensive spectroscopic analysis, especially 2D NMR and ESI-MS/MS n . All isolated compounds displayed moderate cytotoxicity against the lung adenocarcinoma (A549), metastatic prostate cancer (PC-3 M), colon cancer (HCT-8), and hepatoma (Bel7402) cell lines with IC 50 values of 2.8-8.3 μM.

  2. Spins, Electromagnetic Moments, and Isomers of 107-129Cd

    CERN Document Server

    Yordanov, D T; Bieron, J; Bissell, M L; Blaum, K; Budincevic, I; Fritzsche, S; Frommgen, N; Georgiev, G; Geppert, Ch; Hammen, M; Kowalska, M; Kreim, K; Krieger, A; Neugart, R; Nortershauser, W; Papuga, J; Schmidt, S

    2013-01-01

    The neutron-rich isotopes of cadmium up to the N=82 shell closure have been investigated by high-resolution laser spectroscopy. Deep-UV excitation at 214.5 nm and radioactive-beam bunching provided the required experimental sensitivity. Long-lived isomers are observed in 127Cd and 129Cd for the first time. One essential feature of the spherical shell model is unambiguously confirmed by a linear increase of the 11/2- quadrupole moments. Remarkably, this mechanism is found to act well beyond the h11/2 shell.

  3. Decays of 116Sb isomers to levels in 116Sn

    International Nuclear Information System (INIS)

    Gacsi, Z.; Raman, S.

    1994-01-01

    The excited states of 116 Sn were studied by means of the decays of the 15.8-min, 3 + 116 Sb ground state, and the 60.3-min, 8 - 116 Sb isomer. Over 50 γ rays were observed; these were incorporated into a level scheme consisting of 32 excited states. Except for one new level proposed at 3.986 MeV, the current study fully supports an exhaustive study of levels in 116 Sn reported earlier. The previous study was an attempt to develop a nearly ''complete'' level scheme of 116 Sn up to an excitation energy of 4.3 MeV

  4. Chemistry of fission products for accident analysis

    International Nuclear Information System (INIS)

    Potter, P.E.

    1985-01-01

    Current knowledge concerning the chemical state of the fission product elements during the development of accidents in water reactor systems is reviewed in this paper. The fission product elements which have been considered are Cs, I, Te, Sr and Ba but aspects of the behavior of Mo, Ru and the lanthanides are also discussed. Some features of the reactions of the various species of these elements with other components of the reactor systems are described. The importance of having an adequate knowledge of thermodynamic data and phase equilibria of relatively simple systems in order to interpret experimental observations on complex multi-component systems is stressed

  5. Obsidian dating by fission track method

    International Nuclear Information System (INIS)

    Araya, A.M.O.

    1990-12-01

    The fission track method was employed to obtain the age of twelve obsidian sample from Ecuador. By using the plateau-age correction method, we obtained the true age of each sample and were able to identify four groups of ages in the studied area. Thereafter we studied the fading of fission tracks in two obsidian samples with different origins: Yanaurcu, Ecuador and Monte Arci, Italy. We constructed Arrhenius plots and calculated activation energies for both samples. The results from thermal annealing experiments were compared with theoretical curves obtained by integrating an equation proposed by Shukolyukov et al (1965). (author). 43 refs, 20 figs, 10 tabs

  6. Fission product release mechanisms and groupings

    International Nuclear Information System (INIS)

    Iglesia, F.C.; Brito, A.C.; Liu, Y.

    1995-01-01

    During CANDU postulated accidents the reactor fuel is estimated to be exposed to a variety of conditions. These conditions are dynamic and, during the course of an accident, the fuel may experience a wide range of temperatures and conditions from highly oxidizing to mildly reducing environments. The exposure of the reactor fuel to these environments and temperatures may affect its stoichiometry and release performance. In this paper a review of the important fission product release mechanisms is presented, the results of three out-of-pile experimental programs are summarized, and fission product release groups, for both oxidizing and reducing conditions are proposed. (author)

  7. True ternary fission of 252Cf

    International Nuclear Information System (INIS)

    Vijayaraghavan, K.R.; Balasubramaniam, M.; Oertzen, W. von

    2014-01-01

    Splitting of heavy radioactive nucleus into three fragments is known as ternary fission. If the size of the fragments are almost equal it is referred to as true ternary fission. Recently, Yu. V. Pyatkov et al observed/reported the experimental observation of true ternary fission in 252 Cf. In this work, the possibilities of different true ternary fission modes of 252 Cf through potential energy surface (PES) calculations based on three cluster model (TCM) are discussed. In TCM a condition on the mass numbers of the fission fragments is implied as A 1 ≥ A 2 ≥ A 3 in order to avoid repetition of combinations. Due to this condition, the values of Z 3 vary from 0 to 36 and Z 2 vary from 16 to 51. Of the different pairs having similar (Z 2 , Z 3 ) with different potential energy, a pair possessing minimum potential energy is chosen. Thus identified favourable combinations are plotted. For the PES calculations the arrangement of the fragments is considered in the order of A 1 +A 2 +A 3 . i.e. the heavy and the lightest fragments are kept at the ends. It is seen that the deepest minimum in the PES occurs for Z 3 =2 labelled as (Z 2 ; 2) indicating He accompanied breakup as the most favourable one. Of which, the breakup with Z 2 around 46 to 48 is the least (shown by dashed (Z 1 = 50) and dotted (Z 1 = 52) lines indicating a constant Z 1 value). The other notable minima in the PES are labelled and they correspond to the (Z 2 , Z 3 ) pairs viz., (20, 20), (28, 20), (28, 28) and (32, 32). Of these four minima, the first three are associated with the magic numbers 20 and 28. For Z 3 =20, there are two minimums at (20,20) and (28,20) among them (28,20) is the lowest minimum through which the minimum-path passes, and it is the ternary decay observed by Yu. V. Pyatkov et al. The fourth minima is the most interesting due to the fact that it corresponds to true ternary fission mode with Z 2 =32, Z 3 =32 and Z 1 =34. The minimum potential energy path also goes through this true

  8. Systematics of neutron-induced fission yields

    International Nuclear Information System (INIS)

    Blachot, J.; Brissot, R.

    1983-10-01

    The main characteristics of the mass and charge distributions for thermal neutron induced fission of actinides are reviewed. We show that these distributions can be reasonably reproduced with only 24 data as input. We use a representation where the element yields together with the most probable mass Ap(Z) play the dominant role. The ability of this model to calculate mass yields for the fission of not yet measured actinides is also shown. The influence of the excitation energy of the fissile system on charge and mass distribution is also discussed

  9. Analytical evaluation of fission product sensitivities

    International Nuclear Information System (INIS)

    Sola, A.

    1977-01-01

    Evaluating the concentration of a fission product produced in a reactor requires the knowledge of a fairly large number of variables. Sensitivity studies were made to ascertain the important variables. Analytical formulae were developed sufficiently simple to allow numerical computations. Some simplified formulas are also given and they are applied to the following isotopes: 80 Se, 82 Se, 81 Br, 82 Br, 82 Kr, 83 Kr, 84 Kr, 85 Kr, 86 Kr. Their sensitivities to capture cross sections, fission yields, ratios of activation cross sections, half-lives (during and after irradiation), branching ratios, as well as to the neutron flux and to the time are considered

  10. Chemistry of actinides and fission products

    International Nuclear Information System (INIS)

    Pruett, D.J.; Sherrow, S.A.; Toth, L.M.

    1988-01-01

    This task is concerned primarily with the fundamental chemistry of the actinide and fission product elements. Special efforts are made to develop research programs in collaboration with researchers at universities and in industry who have need of national laboratory facilities. Specific areas currently under investigation include: (1) spectroscopy and photochemistry of actinides in low-temperature matrices; (2) small-angle scattering studies of hydrous actinide and fission product polymers in aqueous and nonaqueous solvents; (3) kinetic and thermodynamic studies of complexation reactions in aqueous and nonaqueous solutions; and (4) the development of inorganic ion exchange materials for actinide and lanthanide separations. Recent results from work in these areas are summarized here

  11. Actinide and fission product separation and transmutation

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1993-07-01

    The second international information exchange meeting on actinide and fission product separation and transmutation, took place in Argonne National Laboratory in Illinois United States, on 11-13 November 1992. The proceedings are presented in four sessions: Current strategic system of actinide and fission product separation and transmutation, progress in R and D on partitioning processes wet and dry, progress in R and D on transmutation and refinements of neutronic and other data, development of the fuel cycle processes fuel types and targets. (A.L.B.)

  12. Analysis of RNA metabolism in fission yeast

    DEFF Research Database (Denmark)

    Wise, Jo Ann; Nielsen, Olaf

    2017-01-01

    Here we focus on the biogenesis and function of messenger RNA (mRNA) in fission yeast cells. Following a general introduction that also briefly touches on other classes of RNA, we provide an overview of methods used to analyze mRNAs throughout their life cycles.......Here we focus on the biogenesis and function of messenger RNA (mRNA) in fission yeast cells. Following a general introduction that also briefly touches on other classes of RNA, we provide an overview of methods used to analyze mRNAs throughout their life cycles....

  13. Thermal and epithermal data assessment for fission reactors

    International Nuclear Information System (INIS)

    Tellier, H.

    1991-01-01

    Sensitivity calculations indicated that the wrong computation of the reactivity temperature coefficient of a multiplying medium could be explained by a change of the neutron cross section shapes for the major actinides in the thermal energy range. Consequently, new measurements of these shapes were recently performed in several laboratories. Nu-bar, the fission and total cross sections, the eta parameter and some resonance widths were measured again. The isotopes of interest are uranium 238, uranium 235, plutonium 239 and plutonium 240. Now the results of these new measurements are almost all available. The purpose of the present paper is the review of the new results and a proposal, if it is necessary, of a modification of some cross sections shapes which were previously used in the evaluated files. The new cross section values are validated against a wide set of integral experiments which includes buckling and temperature coefficient of reactivity measurements. It seems that we observe a satisfactory agreement between the new microcospic data and the values which are deduced from the integral experiments

  14. New fission-neutron-spectrum representation for ENDF

    International Nuclear Information System (INIS)

    Madland, D.G.

    1982-04-01

    A new representation of the prompt fission neutron spectrum is proposed for use in the Evaluated Nuclear Data File (ENDF). The proposal is made because a new theory exists by which the spectrum can be accurately predicted as a function of the fissioning nucleus and its excitation energy. Thus, prompt fission neutron spectra can be calculated for cases where no measurements exist or where measurements are not possible. The mathematical formalism necessary for application of the new theory within ENDF is presented and discussed for neutron-induced fission and spontaneous fission. In the case of neutron-induced fission, expressions are given for the first-chance, second-chance, third-chance, and fourth-chance fission components of the spectrum together with that for the total spectrum. An ENDF format is proposed for the new fission spectrum representation, and an example of the use of the format is given

  15. Reexamination of fission fragment angular distributions and the fission process: Formalism

    International Nuclear Information System (INIS)

    Bond, P.D.

    1985-01-01

    The theory of fission fragment angular distributions is examined and the universally used expression is found to be valid only under restrictive assumptions. A more general angular distribution formula is derived and applied to recent data of high spin systems. At the same time it is shown that the strong anisotropies observed from such systems can be understood without changing the essential basis of standard fission theory. The effects of reaction mechanisms other than complete fusion on fission fragment angular distributions are discussed and possible angular distribution signatures of noncompound nucleus formation are mentioned

  16. A fission-fragment-sensitive target for X-ray spectroscopy in neutron-induced fission

    CERN Document Server

    Ethvignot, T; Giot, L; Casoli, P; Nelson, R O

    2002-01-01

    A fission-fragment-sensitive detector built for low-energy photon spectroscopy applications at the WNR 'white' neutron source at Los Alamos is described. The detector consists of eight layers of thin photovoltaic cells, onto which 1 mg/cm sup 2 of pure sup 2 sup 3 sup 8 U is deposited. The detector serves as an active target to select fission events from background and other reaction channels. The fairly small thickness of the detector with respect to transmission of 20-50 keV photons permits the measurement of prompt fission-fragment X-rays. Results with the GEANIE photon spectrometer are presented.

  17. Dynamic effect analysis in 240Pu fission at low energy

    International Nuclear Information System (INIS)

    Patin, Y.; Lachkar, J.; Sigaud, J.

    1975-01-01

    The variations of kinetic and excitation energies and fragment masses have been analyzed as a function of the fissioning nucleus excitation energy. Most interest has been taken in the fission of 240 Pu where many experimental data have been reported. The results tend, in the whole, to illustrate the existence of two modes of fission; the first one is superfluid, the other is strongly damped in the last stage of the fission process [fr

  18. Delayed β ray spectrum of 235U fission fragments

    International Nuclear Information System (INIS)

    Pascholati, P.R.

    1973-01-01

    The time-dependent electron spectra of fission fragments from the thermal-neutron-induced fission of 235 U are calculated. The Gross theory of nuclear beta decay is used to obtain the decay constant and individual electron spectra. The mean energy per fission carried by the electrons and the number of electrons per fission are also calculated. Comparison of these calculated spectra to experimental ones shows good agreements. (Author) [pt

  19. Mass dependence of positive pion-induced fission

    International Nuclear Information System (INIS)

    Khan, H.A.; Khan, N.A.; Peterson, R.J.

    1991-01-01

    Fission cross sections for a range of targets have been measured by solid-state track detectors following 80 and 100 MeV π + bombardment. Fission probabilities have been inferred by comparison to computed reaction cross sections. Fission probabilities for heavy targets agree with those for other probes of comparable energy and with statistical calculations. Probabilities for lighter targets are much above those previously observed or computed. Ternary fission cross sections and multiplicities of light fragments have also been determined

  20. Delayed Neutrons and Photoneutrons from Fission Products

    International Nuclear Information System (INIS)

    Amiel, S.

    1965-01-01

    Delayed neutrons: Most studies of the delayed neutrons from fission have involved analysis of the kinetic behaviour of fusion chain- reacting systems, analysis of the gross neutron decay (resolved into six groups with approximate half-lives of 0.2, 0.5, 2, 6, 22 and 55 s) and some measurements of the neutron spectra (the energies extendfrom 0.1 to 1.2 MeV, peaking in the range 0.2 to 0.5 MeV). Rapid separations of fission-produced halogens have indicated seven isotopes (Br 87,88,89,90 and I 137,138,139 ). and rare gas analysis has indicated 1.5-s Kr and 6-s Rb as definite delayed neutron precursors. These identified precursors account for some 80% of the total delayed neutron yields. Theoretical predictions of possible precursors point to a few tens of such nuclides to be found mainly in regions just above closed neutron shells. Total neutron yields are observed to increase with mass number and decrease with atomic number of the fissioning nuclide. Yields are nearly independent of the energy of the incident fissioning neutron at energies up to several MeV. In this range observed group yields,-especially of the long-lived precursors, ate in fairly good agreement with fission mass and charge distributions, and calculated neutron emission probabilities. . Further detailed studies of delayed neutron precursors (particularly in the difficult short half-life region) require development of ultra-fast radiochemical separation procedures (or on-line isotope separation) and fast neutron spectroscopy of high resolution and efficiency. Photoneutrons; A knowledge of the intensities and gamma-ray spectra of fission products is of practical importance in reactor technology particularly with respect to gamma heating, shielding and radiation effects. Gamma-rays of energies greater than 2.23 and 1.67 MeV cause emission of photoneutrons from deuterium and beryllium respectively, and are important in the kinetics of heavy water and beryllium-moderated reactors. The rate of

  1. Constitutional Isomers of Pentahydroxy-Functionalized Pillar[5]arenes: Synthesis, Characterization, and Crystal Structures.

    Science.gov (United States)

    Al-Azemi, Talal F; Vinodh, Mickey; Alipour, Fatemeh H; Mohamod, Abdirahman A

    2017-10-20

    We herein report the preparation of constitutional isomers of pentahydroxy-functionalized pillar[5]arenes via the deprotection of their benzylated derivatives by catalytic hydrogenation. The structures of the obtained isomers were then established using single crystal X-ray diffraction. We also found that the yield distribution of the different constitutional isomers was dependent on the nature of the substitution, as revealed by HPLC analysis of the crude mixture. Finally, further characterization of the separated constitutional isomers indicated that they possess different melting points, NMR spectra, crystal structures, and stacking patterns in the solid state.

  2. Calculations of long-lived isomer production in neutron reactions

    International Nuclear Information System (INIS)

    Chadwick, M.B.; Young, P.G.

    1992-01-01

    We present theoretical calculations for the production of the long-lived isomers 93m Nb (1/2-, 16 yr), 121m Sn (11/2-, 55 yr), 166m Ho (7-, 1200 yr), 184m Re (8+, 165 d), 186m Re (8+, 2x10 5 yr), 178 Hf (16+, 31 yr), 179m Hf (25/2-, 25 d), and 192m Ir (9+, 241 yr), all of which pose potential radiation activation problems in nuclear fusion reactors if produced in 14-MeV neutron-induced reactions. We consider (n,2n), (n,n'), and (n,γ) production modes and compare our results both with experimental data (where available) and systematics. We also investigate the dependence of the isomeric cross section ratio on incident neutron energy for the isomers under consideration. The statistical Hauser-Feshbach plus preequilibrium code GNASH was used for the calculations. Where discrete state experimental information was lacking, rotational band members above the isomeric state, which can be justified theoretically but have not been experimentally resolved, were reconstructed. (author). 16 refs, 10 figs, 4 tabs

  3. CHEMICAL SIMULATIONS OF PREBIOTIC MOLECULES: INTERSTELLAR ETHANIMINE ISOMERS

    Energy Technology Data Exchange (ETDEWEB)

    Quan, Donghui; Durr, Allison [Department of Chemistry, Eastern Kentucky University, Richmond, KY 40475 (United States); Herbst, Eric [Departments of Chemistry and Astronomy, University of Virginia, Charlottesville, VA 22904 (United States); Corby, Joanna F. [Department of Astronomy, University of Virginia, Charlottesville, VA 22904 (United States); Hassel, George [Physics and Astronomy Department, Siena College, Loudonville, NY 12211 (United States)

    2016-06-20

    The E- and Z- isomers of ethanimine (CH{sub 3}CHNH) were recently detected toward the star-forming region Sagittarius (Sgr) B2(N) using the Green Bank Telescope PRIMOS cm-wave spectral data, and imaged by the Australia Telescope Compact Array. Ethanimine is not reported in the hot cores of Sgr B2, but only in gas that absorbs at +64 and +82 km s{sup −1} in the foreground of continuum emission generated by H ii regions. The ethanimine isomers can serve as precursors of the amino acid alanine and may play important roles in forming biological molecules in the interstellar medium. Here we present a study of the chemistry of ethanimine using a gas-grain simulation based on rate equations, with both isothermal and warm-up conditions. In addition, the density, kinetic temperature, and cosmic ray ionization rate have been varied. For a variety of physical conditions in the warm-up models for Sgr B2(N) and environs, the simulations show reasonable agreement with observationally obtained abundances. Isothermal models of translucent clouds along the same line of sight yield much lower abundances, so that ethanimine would be much more difficult to detect in these sources despite the fact that other complex molecules have been detected there.

  4. Degradation of a chiral nonylphenol isomer in two agricultural soils

    International Nuclear Information System (INIS)

    Zhang Haifeng; Spiteller, Michael; Guenther, Klaus; Boehmler, Gabriele; Zuehlke, Sebastian

    2009-01-01

    The degradation of a chiral nonylphenol isomer, 4-(1-ethyl-1,4-dimethylpentyl)phenol (NP 112 ), in two agricultural soils from Monheim and Dortmund, Germany has been studied. The degradation of NP 112 and the formation of a nitro-nonylphenol metabolite were determined by means of GC-MS analysis. The degradation followed bi-exponential order kinetics, with half-life of less than 5 days in both soils. The nitro-metabolite was found at different concentration levels in the two soils. The nitro-metabolite of NP 112 was more persistent than its parent compound. After 150 days about 13% of the initially applied NP 112 remained in the Monheim soil as its nitro-metabolite. Results of the E-screen assay revealed that the nitro-NP 112 has oestrogenic potency of 85% of that of NP 112 . Furthermore, the results of chiral GC-MS analysis revealed that no chiral degradation of NP 112 occurred in this study. - The degradation of a chiral nonylphenol isomer in agricultural soils followed bi-exponential order kinetics resulting in a more persistent nitro-metabolite.

  5. Fission probability of nucleus of sup(232)Th mesoatom

    International Nuclear Information System (INIS)

    Cojocaru, V.; Gavrilov, Yu.K.; Kim Si wan; Krogulski, T.; Kuznetsov, V.D.; Ortlepp, H.-G.; Polikanov, S.M.

    1975-01-01

    The fission probability of the nucleus of the sup(232)Th muonic atom has been measured. The fission yield was measured simultaneously with the intensity of 5g-4f transition in the muonic atom sup(232)Th. A good agreement with previous result obtained in measurements with the fission chamber and evident disagreement with the photoemulsion data have been obtained

  6. Factors affecting use of fission foils as dosimetry sensors

    International Nuclear Information System (INIS)

    Griffin, P.J.; Vehar, D.W.; Kelly, J.G.; Holm, C.V.

    1996-01-01

    Fission foils are commonly used as dosimetry sensors. They play a very important role in neutron spectrum determinations. This paper provides a combination of experimental measurements and calculations to quantify the importance and synergy of several factors that affect the fission response of a dosimeter. Only when these effects are properly treated can fission dosimeters be used with sufficient fidelity

  7. Fission barrier heights in the A ∼ 200 mass region

    Indian Academy of Sciences (India)

    Abstract. Statistical model analysis is carried out for p- and α-induced fission reactions using a consistent description for fission barrier and level density in A ∼ 200 mass region. A continuous damping of shell correction with excitation energy is considered. Extracted fission barriers agree well with the recent ...

  8. SYMMETRICAL AND ASYMMETRIC TERNARY FISSION OF HOT NUCLEI

    NARCIS (Netherlands)

    SIWEKWILCZYNSKA, K; WILCZYNSKI, J; LEEGTE, HKW; SIEMSSEN, RH; WILSCHUT, HW; GROTOWSKI, K; PANASIEWICZ, A; SOSIN, Z; WIELOCH, A

    Emission of a particles accompanying fusion-fission processes in the Ar-40 + Th-232 reaction at E(Ar-40) = 365 MeV was studied in a wide range of in-fission-plane and out-of-plane angles. The exact determination of the emission angles of both fission fragments combined with the time-of-flight

  9. Chemical immobilization of fission products reactive with nuclear reactor components

    International Nuclear Information System (INIS)

    Grossman, L.N.; Kaznoff, A.I.; Clukey, H.V.

    1975-01-01

    This invention teaches a method of immobilizing deleterious fission products produced in nuclear fuel materials during nuclear fission chain reactions through the use of additives. The additives are disposed with the nuclear fuel materials in controlled quantities to form new compositions preventing attack of reactor components, especially nuclear fuel cld, by the deleterious fission products. (Patent Office Record)

  10. Enabling the Use of Space Fission Propulsion Systems

    Energy Technology Data Exchange (ETDEWEB)

    Mike Houts; Melissa Van Dyke; Tom Godfroy; James Martin; Kevin Pedersen; Ricky Dickens; Ivana Hrbud; Leo Bitteker; Bruce Patton; Suman Chakrabarti; Joe Bonometti

    2000-06-04

    This paper gives brief descriptions of advantages of fission technology for reaching any point in the solar system and of earlier efforts to develop space fission propulsion systems, and gives a more detailed description of the safe, affordable fission engine (SAFE) concept being pursued at the National Aeronautics and Space Administration's Marshall Space Flight Center.

  11. Charged particle-induced nuclear fission reactions – Progress and ...

    Indian Academy of Sciences (India)

    of fission process for nuclei at moderately high excitation energies with large angular momentum values. ... model analysis of these data, the fission barrier can be determined for the fissioning com- pound nucleus. .... qualitative understanding of the various features of mass division are understood in terms of scission point ...

  12. Fission barrier heights in the A∼ 200 mass region

    Indian Academy of Sciences (India)

    2015-07-19

    Jul 19, 2015 ... Statistical model analysis is carried out for - and -induced fission reactions using a consistent description for fission barrier and level density in A ∼ 200 mass region. A continuous damping of shell correction with excitation energy is considered. Extracted fission barriers agree well with the recent ...

  13. A molecular heterojunction of zinc phthalocyanine and peanut-shaped fullerene polymer: A density functional study

    Science.gov (United States)

    Tanikawa, Kousei; Ohno, Kaoru; Noda, Yusuke; Ono, Shota; Kuwahara, Riichi; Takashima, Akito; Nakaya, Masato; Onoe, Jun

    2017-10-01

    We have performed first-principles density functional calculations of a molecular heterojunction of a zinc phthalocyanine (ZnPc) molecule and a peanut-shaped fullerene polymer (PSFP) made from several coalesced cross-linked C60 molecules. The PSFP has many isomers and all have both spatially localized (near ZnPc) and metallic conducting levels. Here we consider four typical isomers. From the resulting electronic structure, we discuss the applicability of these isomers to organic photovoltaics (OPV), electrodes, and light harvesting materials. If one of the isomers called T3, which has the largest energy gap, is used together with ZnPc for OPV, this system shows more than 20% energy conversion efficiency.

  14. Nuclear fission: a review of experimental advances and phenomenology

    Science.gov (United States)

    Andreyev, A. N.; Nishio, K.; Schmidt, K.-H.

    2018-01-01

    In the last two decades, through technological, experimental and theoretical advances, the situation in experimental fission studies has changed dramatically. With the use of advanced production and detection techniques both much more detailed and precise information can now be obtained for the traditional regions of fission research and, crucially, new regions of nuclei have become routinely accessible for fission studies. This work first of all reviews the recent developments in experimental fission techniques, in particular the resurgence of transfer-induced fission reactions with light and heavy ions, the emerging use of inverse-kinematic approaches, both at Coulomb and relativistic energies, and of fission studies with radioactive beams. The emphasis on the fission-fragment mass and charge distributions will be made in this work, though some of the other fission observables, such as prompt neutron and γ-ray emission will also be reviewed. A particular attention will be given to the low-energy fission in the so far scarcely explored nuclei in the very neutron-deficient lead region. They recently became the focus for several complementary experimental studies, such as β-delayed fission with radioactive beams at ISOLDE(CERN), Coulex-induced fission of relativistic secondary beams at FRS(GSI), and several prompt fusion–fission studies. The synergy of these approaches allows a unique insight in the new region of asymmetric fission around {\\hspace{0pt}}180 Hg, recently discovered at ISOLDE. Recent extensive theoretical efforts in this region will also be outlined. The unprecedented high-quality data for fission fragments, completely identified in Z and A, by means of reactions in inverse kinematics at FRS(GSI) and VAMOS(GANIL) will be also reviewed. These experiments explored an extended range of mercury-to-californium elements, spanning from the neutron-deficient to neutron-rich nuclides, and covering both asymmetric, symmetric and transitional fission regions

  15. Schapiro Shapes

    Science.gov (United States)

    O'Connell, Emily

    2009-01-01

    This article describes a lesson on Schapiro Shapes. Schapiro Shapes is based on the art of Miriam Schapiro, who created a number of works of figures in action. Using the basic concepts of this project, students learn to create their own figures and styles. (Contains 1 online resource.)

  16. Radiochemical studies on nuclear fission at Trombay

    Indian Academy of Sciences (India)

    2015-07-30

    Jul 30, 2015 ... Since the discovery of nuclear fission in the year 1939, both physical and radiochemical techniques have been adopted for the study of various aspects of the phenomenon. ... At Trombay, a small group of radiochemists initiated the work on radiochemical studies of mass distribution in the early sixties.

  17. Seventy-five years of nuclear fission

    Indian Academy of Sciences (India)

    2015-07-19

    Jul 19, 2015 ... ... fission related research has not only provided new insights in the physics of large scale motion, deformation and subsequent division of a heavy nucleus, but has also opened several new frontiers of research in nuclear physics. This article is a narrative giving an overview of the landmarks of the progress ...

  18. Angular distribution in ternary cold fission

    International Nuclear Information System (INIS)

    Delion, D.S.; J.W. Goethe Univ., Frankfurt; Sandulescu, A.; J.W. Goethe Univ., Frankfurt; Greiner, W.

    2003-01-01

    We describe the spontaneous ternary cold fission of 252 Cf, accompanied by 4 He, 10 Be and 14 C. The light cluster decays from the first resonant eigenstate in the Coulomb potential plus a harmonic oscillator potential. We have shown that the angular distribution of the emitted light particle is strongly connected with its deformation and the equatorial distance. (author)

  19. Liquid uranium alloy-helium fission reactor

    Science.gov (United States)

    Minkov, Vladimir

    1986-01-01

    This invention teaches a nuclear fission reactor having a core vessel and at least one tandem heat exchanger vessel coupled therewith across upper and lower passages to define a closed flow loop. Nuclear fuel such as a uranium alloy in its liquid phase fills these vessels and flow passages. Solid control elements in the reactor core vessel are adapted to be adjusted relative to one another to control fission reaction of the liquid fuel therein. Moderator elements in the other vessel and flow passages preclude fission reaction therein. An inert gas such as helium is bubbled upwardly through the heat exchanger vessel operable to move the liquid fuel upwardly therein and unidirectionally around the closed loop and downwardly through the core vessel. This helium gas is further directed to heat conversion means outside of the reactor vessels to utilize the heat from the fission reaction to generate useful output. The nuclear fuel operates in the 1200.degree.-1800.degree. C. range, and even higher to 2500.degree. C., limited only by the thermal effectiveness of the structural materials, increasing the efficiency of power generation from the normal 30-35% with 300.degree.-500.degree. C. upper limit temperature to 50-65%. Irradiation of the circulating liquid fuel, as contrasted to only localized irradiation of a solid fuel, provides improved fuel utilization.

  20. Angular distribution of oriented nucleus fission neutrons

    International Nuclear Information System (INIS)

    Barabanov, A.L.; Grechukhin, D.P.

    1982-01-01

    Calculations of anisotropy of angular distribution of oriented 235 U nuclei thermal fission neutrons have been carried out. the neutrons were assumed to evaporate isotropically by completely accelerated fragements in the fragment system with only its small part, i. e. fission-producing neutrons, emitted at the moment of neck break. It has been found out that at low energies of neutrons Esub(n)=1-2 MeV the sensitivity of the angular distribution anisotropy to variations of spectrum of neutron evaporation from fragments and the magnitude of a share of fission-producing neutrons reaches approximately 100%, which at high energies, Esub(n) > 5 MeV it does not exceed approximately 20%. Therefore the angular distribution of fast neutrons to a greater degree of confidence may be used for restoring the angular distribution anisotropy of fragments while the angular distribution of low energy neutrons may be used for deriving information on the fission process, but only in case 6f the experiment accuracy is better than approximately 3%

  1. Fission Detection Using the Associated Particle Technique

    International Nuclear Information System (INIS)

    R.P. Keegan; J.P. Hurley; J.R. Tinsley; R. Trainham; S.C. Wilde

    2008-01-01

    A beam of tagged 14 MeV neutrons from the deuterium-tritium (DT) reaction is used to induce fission in a target composed of depleted uranium. The generator yield is 10 7 neutrons/second radiated into a 4 x 4 in. NaI detectors are used for gamma-ray detection. The fission process is known to produce multiple gamma-rays and neutrons. Triple coincidences (α-γ-γ) are measured as a function of neutron flight time up to 90 ns after fission, where the α-particle arises from the DT reaction. A sudden increase in the triple coincidence rate at the location of the material is used to localize and detect fission in the interrogated target. Comparisons are made with experiment runs where lead, tungsten, and iron were used as target materials. The triple coincidence response profile from depleted uranium is noted to be different to those observed from the other target materials. The response from interrogation targets composed of fissile material is anticipated to be even more unique than that observed from depleted uranium

  2. Fission--fusion systems: classification and critique

    International Nuclear Information System (INIS)

    Lidsky, L.M.

    1974-01-01

    A useful classification scheme for hybrid systems is described and some common features that the scheme makes apparent are pointed out. The early history of fusion-fission systems is reviewed. Some designs are described along with advantages and disadvantages of each. The extension to low and moderate Q devices is noted. (U.S.)

  3. Some aspects of fission and quasifission processes

    Indian Academy of Sciences (India)

    The events leading up to the discovery of the nuclear fission process took place at the end of 1938. The chemistry studies .... in the assembly of the first two atomic bombs in Los Alamos. In the following sections, .... tion from his research in Cambridge, but with the start of World War II that year, he decided to stay in India and ...

  4. Radiochemical studies on nuclear fission at Trombay

    Indian Academy of Sciences (India)

    Due to the ability to separate individual elements from a complex reaction mixture with a high degree of sensitivity and ... Trombay, a small group of radiochemists initiated the work on radiochemical studies of mass dis- tribution in the ..... angular anisotropies vs. mass number of different fission products in the two systems. It.

  5. Development of fission Mo-99 production technology

    International Nuclear Information System (INIS)

    Park, Jin Ho; Choung, W. M.; Lee, K. I. and others

    2001-05-01

    This R and D project is planed to supply domestic demands of Mo-99 through fission route, and consequently this project will be expected to rise up utilization of HANARO and KAERI's capability for marketing extension into domestic and oversea radiopharmaceutical market. HEU and LEU target types are decided and designed for fission Mo-99 production in domestic. Experimental study of target fabrication technology was performed and developed processing equipments. And conceptual design of target loading/unloading in/from HANARO device are performed. Tracer test of Mo-99 separation and purification process was performed, test results reach to Mo-99 recovery yield above 80% and decontamination factor above 1600. Combined Mo-99 separation and purification process was decided for hot test scheduled from next year, and performance test was performed. Conceptual design for modification of existing hot cell for fission Mo-99 production facility was performed and will be used for detail design. Assumption for the comparison of LEU and HEU target in fission Mo-99 production process were suggested and compared of merits and demerits in view of fabrication technology and economy feasibility

  6. Actinide and fission product partitioning and transmutation

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1995-07-01

    The third international information exchange meeting on actinide and fission product partitioning and transmutation, took place in Cadarache France, on 12-14 December 1994. The proceedings are presented in six sessions : an introduction session, the major programmes and international cooperation, the systems studies, the reactors fuels and targets, the chemistry and a last discussions session. (A.L.B.)

  7. Otto Hahn (1944). Discovery of nuclear fission

    CERN Document Server

    Hahn, Otto

    2003-01-01

    Otto Hahn (Frankfurt-on-Main, 1879-Gotinga, 1968) is the discoverer of nuclear fission, which awarded him the Nobel Prize for Chemistry in 1944. After leaving Germany during the Second World War to settle in the United Kingdom, he returned to this country as a renown figure.

  8. Development of fission Mo-99 production technology

    Energy Technology Data Exchange (ETDEWEB)

    Park, Jin Ho; Choung, W. M.; Lee, K. I. and others

    2001-05-01

    This R and D project is planed to supply domestic demands of Mo-99 through fission route, and consequently this project will be expected to rise up utilization of HANARO and KAERI's capability for marketing extension into domestic and oversea radiopharmaceutical market. HEU and LEU target types are decided and designed for fission Mo-99 production in domestic. Experimental study of target fabrication technology was performed and developed processing equipments. And conceptual design of target loading/unloading in/from HANARO device are performed. Tracer test of Mo-99 separation and purification process was performed, test results reach to Mo-99 recovery yield above 80% and decontamination factor above 1600. Combined Mo-99 separation and purification process was decided for hot test scheduled from next year, and performance test was performed. Conceptual design for modification of existing hot cell for fission Mo-99 production facility was performed and will be used for detail design. Assumption for the comparison of LEU and HEU target in fission Mo-99 production process were suggested and compared of merits and demerits in view of fabrication technology and economy feasibility.

  9. Angular-momentum-bearing modes in fission

    International Nuclear Information System (INIS)

    Moretto, L.G.; Peaslee, G.F.; Wozniak, G.J.

    1989-03-01

    The angular-momentum-bearing degrees of freedom involved in the fission process are identified and their influence on experimental observables is discussed. The excitation of these modes is treated in the ''thermal'' limit, and the resulting distributions of observables are calculated. Experiments demonstrating the role of these modes are presented and discussed. 61 refs., 12 figs

  10. Actinide and fission product partitioning and transmutation

    International Nuclear Information System (INIS)

    1995-01-01

    The third international information exchange meeting on actinide and fission product partitioning and transmutation, took place in Cadarache France, on 12-14 December 1994. The proceedings are presented in six sessions : an introduction session, the major programmes and international cooperation, the systems studies, the reactors fuels and targets, the chemistry and a last discussions session. (A.L.B.)

  11. Seventy-five years of nuclear fission

    Indian Academy of Sciences (India)

    Under his leadership, India's first reactor APSARA became operational as early as. 1956 and India became the first country in Asia to have indigenous capability in designing and building a nuclear reactor. In India, nuclear fission research started quite early in the mid-1950s under the inspiring leadership of Raja Ramanna ...

  12. UBA domain containing proteins in fission yeast

    DEFF Research Database (Denmark)

    Hartmann-Petersen, Rasmus; Semple, Colin A M; Ponting, Chris P

    2003-01-01

    characterised on both the functional and structural levels. One example of a widespread ubiquitin binding module is the ubiquitin associated (UBA) domain. Here, we discuss the approximately 15 UBA domain containing proteins encoded in the relatively small genome of the fission yeast Schizosaccharomyces pombe...

  13. Probing the time scale of asymmetric fission

    International Nuclear Information System (INIS)

    Kamanin, D.

    1999-12-01

    The author describes the measurement of the mass-energy distributions of fission fragments in the reactions 197 Au( 14 N,X) at 34 A.MeV and 232 Th( 7 Li,X) at 43 A.MeV. He presents results on the mass-asymmetry and excitation energy sharing. (HSI)

  14. Neutron induced fission of 234U

    Directory of Open Access Journals (Sweden)

    Pomp S.

    2012-02-01

    Full Text Available The fission fragment properties of 234U(n,f were investigated as a function of incident neutron energy from 0.2 MeV up to 5 MeV. The fission fragment mass, angular distribution and kinetic energy were measured with a double Frisch-grid ionization chamber using both analogue and digital data acquisition techniques. The reaction 234U(n,f is relevant, since it involves the same compound nucleus as formed after neutron evaporation from highly excited 236U*, the so-called second-chance fission of 235U. Experimental data on fission fragment properties like fission fragment mass and total kinetic energy (TKE as a function of incident neutron energy are rather scarce for this reaction. For the theoretical modelling of the reaction cross sections for Uranium isotopes this information is a crucial input parameter. In addition, 234U is also an important isotope in the Thorium-based fuel cycle. The strong anisotropy of the angular distribution around the vibrational resonance at En = 0.77 MeV could be confirmed using the full angular range. Fluctuations in the fragment TKE have been observed in the threshold region around the strong vibrational resonance at En = 0.77 MeV. The present results are in contradiction with corresponding literature values. Changes in the mass yield around the vibrational resonance and at En = 5 MeV relative to En = 2 MeV show a different signature. The drop in mean TKE around 2.5 to 3 MeV points to pair breaking as also observed in 235,238U(n,f. The measured two-dimensional mass yield and TKE distribution have been described in terms of fission modes. The yield of the standard 1 (S1 mode shows fluctuations in the threshold of the fission cross section due to the influence of the resonance and levels off at about 20% yield for higher incident neutron energies. The S2 mode shows the respective opposite behaviour. The mean TKE of both modes decreases with En. The decrease in mean TKE overrules the increase in S1 yield, so the mean

  15. Neutron induced fission of 234U

    Science.gov (United States)

    Hambsch, F.-J.; Al-Adili, A.; Oberstedt, S.; Pomp, S.

    2012-02-01

    The fission fragment properties of 234U(n,f) were investigated as a function of incident neutron energy from 0.2 MeV up to 5 MeV. The fission fragment mass, angular distribution and kinetic energy were measured with a double Frisch-grid ionization chamber using both analogue and digital data acquisition techniques. The reaction 234U(n,f) is relevant, since it involves the same compound nucleus as formed after neutron evaporation from highly excited 236U*, the so-called second-chance fission of 235U. Experimental data on fission fragment properties like fission fragment mass and total kinetic energy (TKE) as a function of incident neutron energy are rather scarce for this reaction. For the theoretical modelling of the reaction cross sections for Uranium isotopes this information is a crucial input parameter. In addition, 234U is also an important isotope in the Thorium-based fuel cycle. The strong anisotropy of the angular distribution around the vibrational resonance at En = 0.77 MeV could be confirmed using the full angular range. Fluctuations in the fragment TKE have been observed in the threshold region around the strong vibrational resonance at En = 0.77 MeV. The present results are in contradiction with corresponding literature values. Changes in the mass yield around the vibrational resonance and at En = 5 MeV relative to En = 2 MeV show a different signature. The drop in mean TKE around 2.5 to 3 MeV points to pair breaking as also observed in 235,238U(n,f). The measured two-dimensional mass yield and TKE distribution have been described in terms of fission modes. The yield of the standard 1 (S1) mode shows fluctuations in the threshold of the fission cross section due to the influence of the resonance and levels off at about 20% yield for higher incident neutron energies. The S2 mode shows the respective opposite behaviour. The mean TKE of both modes decreases with En. The decrease in mean TKE overrules the increase in S1 yield, so the mean TKE is dropping

  16. Langevin model of low-energy fission

    Science.gov (United States)

    Sierk, Arnold J.

    2017-09-01

    Background: Since the earliest days of fission, stochastic models have been used to describe and model the process. For a quarter century, numerical solutions of Langevin equations have been used to model fission of highly excited nuclei, where microscopic potential-energy effects have been neglected. Purpose: In this paper I present a Langevin model for the fission of nuclei with low to medium excitation energies, for which microscopic effects in the potential energy cannot be ignored. Method: I solve Langevin equations in a five-dimensional space of nuclear deformations. The macroscopic-microscopic potential energy from a global nuclear structure model well benchmarked to nuclear masses is tabulated on a mesh of approximately 107 points in this deformation space. The potential is defined continuously inside the mesh boundaries by use of a moving five-dimensional cubic spline approximation. Because of reflection symmetry, the effective mesh is nearly twice this size. For the inertia, I use a (possibly scaled) approximation to the inertia tensor defined by irrotational flow. A phenomenological dissipation tensor related to one-body dissipation is used. A normal-mode analysis of the dynamical system at the saddle point and the assumption of quasiequilibrium provide distributions of initial conditions appropriate to low excitation energies, and are extended to model spontaneous fission. A dynamical model of postscission fragment motion including dynamical deformations and separation allows the calculation of final mass and kinetic-energy distributions, along with other interesting quantities. Results: The model makes quantitative predictions for fragment mass and kinetic-energy yields, some of which are very close to measured ones. Varying the energy of the incident neutron for induced fission allows the prediction of energy dependencies of fragment yields and average kinetic energies. With a simple approximation for spontaneous fission starting conditions

  17. New isomers in the neutron-rich A∼190 mass region

    International Nuclear Information System (INIS)

    Caamano, M.

    2002-02-01

    Previously unobserved isomeric states in 188 Ta, 190 W, 192 Re, 193 Re, 195 Os, 197 Ir, 198 Ir, 200 Pt, 201 Pt, 202 Pt and 203 Au, with half-lives ranging from 10 ns to 290 μs have been populated and studied using a fragmentation reaction in conjunction with a forward focussing spectrometer. In most cases, this provided the first ever spectroscopic data made available for the nucleus, and 200 Pt presented the first new seniority 4 state, on the basis of γ-γ coincidences, following a fragmentation reaction. Half-lives have been measured and tentative level schemes have been drawn for each isomer, spins and parities being consistent with blocked BCS calculations, hindrance factors, systematics and the relative intensities of γ-rays and X-rays (where possible). Isomeric ratios have been measured, values ranging from 1 % to 64 %. Potential Energy Surface calculations were performed in parallel to the blocked BCS calculations, in order to provide deformation parameters, excitation energies and quasiparticle configurations. Ground state (or lowest level) shape calculations reveal a change from axially symmetric, through triaxial, to spherical shapes across the data set, from 188 Ta to 203 Au, as 208 Pb is approached. Weisskopf hindrance factors provide evidence for the erosion of the goodness of the K-quantum number, compatible with soft or axially symmetric shapes. The prolate-oblate phase transition region, with respect to tungsten, osmium and platinum, shows 195 Os to be the pivotal nucleus in the osmium isotopic chain, with a calculated triaxial ground state. On comparison with the systematics of the region, results obtained for 190 W show evidence for a Z ≤ 74 sub-shell closure, analogous to that at Z = 64. Finally, new isotopes, 167 Tb, 170 Dy and 199 Ir were discovered. (author)

  18. Insights into nuclear structure and the fission process from spontaneous fission

    Energy Technology Data Exchange (ETDEWEB)

    Hamilton, J.H.; Butler-Moore, K.; Ramayya, A.V. [Vanderbilt Univ., Nashville, TN (United States)] [and others

    1993-12-31

    The {gamma}-rays emitted following spontaneous and induced fission are rich sources of information about the structure of neutron-rich nuclei and about the fission process itself. The study of spontaneous fissioning isotopes with large Ge detector arrays are providing a wealth of such information as seen, for example, in recent reports. In this paper we present some of our most recent results on nuclear structure studies and conclusions on the fission process itself. In our work, we have employed in spontaneous fission, a triple gamma coincidence study for the first time and a high resolution, X-ray detector-{gamma}-coincidence study. These data provide powerful ways of separating the gamma rays which belong to a particular nucleus. The triple coincidence technique was used to uniquely identify the levels in {sup 136}Te and higher spin states in its N=84 isotones, {sup 138}Xe and {sup 140}Ba{sup 171}. Some other examples of the level structures observed in the low and high mass partners are presented, including a detailed analysis of the backbending of the moment of inertia in {sup 112,114,116}Pd. Finally, we present the first examples of how our analysis allows one to extract a detailed picture of the dependence of the angular momentum on the mass and atomic numbers of the fission fragments and of the long-sought neutron multiplicity distribution from zero-n to ten-n as a function of the charge and mass asymmetry.

  19. Quadrupole moment of the 7/21- isomer state in 43S. Shell model study of sulfur isotopes around N=28

    International Nuclear Information System (INIS)

    Chevrier, Raphael

    2013-01-01

    The goal of this work consists in providing new insights in the shape coexistence expected in neutron-rich nuclei around the N=28 shell closure. In 43 S, recent experimental data as well as their interpretation in the shell model framework were used to predict the coexistence between a J π =3/2 1 - prolate deformed ground state and a 7/2 1 - rather spherical isomer state. We report on the quadrupole moment measurement Q s of the 7/2 1 - isomer state [E*=320.5(5) keV, T 1/2 =415(3) ns] in 43 S. The TDPAD method was applied on 43 S nuclei produced by the fragmentation of a 48 Ca primary beam at 345 A.MeV, and selected in-flight through the BigRIPS spectrometer at RIKEN (Japan). The measured value, |Q s |=23(3) efm 2 , is in remarkable agreement with that calculated in the shell model framework, although it is significantly larger than that expected for a single-particle state. In order to understand the nature of the correlations responsible for the departure of the isomer state from a pure spherical shape, we report on the results of a shell model study using the modern SDPF-U interaction of the neighbors sulfur isotopes 42,44,46 S. Those calculations allowed to identify a slight triaxial degree of freedom in the structure of these nuclei, although the latter happens to be highly hindered at N=28 in 44 S. Spectroscopic factor calculations show that this slight triaxial degree of freedom also impacts the low-lying structure in 43 S. It allows to better understand the deviation of the spectroscopic quadrupole moment value of the isomer state from the limit case of a pure spherical state. (author) [fr

  20. Application of the dinuclear system model to fission process

    Science.gov (United States)

    Andreev, A. V.; Shneidman, T. M.; Ventura, A.

    2016-01-01

    A theoretical evaluation of the collective excitation spectra of nucleus at large deformations is possible within the framework of the dinuclear system model, which treats the wave function of the fissioning nucleus as a superposition of a mononucleus configuration and two-cluster configurations in a dynamical way, permitting exchange of nucleons between clusters. In this work the method of calculation of the potential energy and the collective spectrum of fissioning nucleus at scission point is presented. Combining the DNS model calculations and the statistical model of fission we calculate the mass, total kinetic energy, and angular distribution of fission fragments for the neutron-induced fission of 239Pu.

  1. Application of the dinuclear system model to fission process

    Directory of Open Access Journals (Sweden)

    Andreev A. V.

    2016-01-01

    Full Text Available A theoretical evaluation of the collective excitation spectra of nucleus at large deformations is possible within the framework of the dinuclear system model, which treats the wave function of the fissioning nucleus as a superposition of a mononucleus configuration and two-cluster configurations in a dynamical way, permitting exchange of nucleons between clusters. In this work the method of calculation of the potential energy and the collective spectrum of fissioning nucleus at scission point is presented. Combining the DNS model calculations and the statistical model of fission we calculate the mass, total kinetic energy, and angular distribution of fission fragments for the neutron–induced fission of 239Pu.

  2. 14. International workshop on nuclear fission physics. Proceedings

    International Nuclear Information System (INIS)

    2000-01-01

    The meetings on nuclear fission took place 12-15 October 1998 and was organized by Institute of Physics and Power Engineering. The aim of the workshop was to present and discuss main new both theoretical and experimental results obtained in the area of nuclear fission, dynamical feature, properties of fission fragments and complementary radiation. As usual the program of the workshop was designed to cover a wide range of physical phenomena - from low energy and spontaneous fission to fission of hot rotating nuclei and multifragmentation at intermediate and high energies. Reaction induced by slow and fast neutron, light and heavy ions were discussed [ru

  3. Developing of CIAE2170 pulse shape discriminator

    International Nuclear Information System (INIS)

    Shen Guanren; Wuru Gongsang; Zhou Zuying; Guo Li; Gao Weixiang; Ni Hefeng; Sun Gong

    1995-01-01

    The pulse shape discriminator is very important electronics for reducing γ rays background. The CIAE2170 pulse shape discriminator is developed and is applied to the experiments on neutron and fission physics and measurements of nuclear data for more than 1500 h. It's very stable and reliable, and continually worked for more than 200 h. The main performance is carefully tested and is in the lead in china and arrived at international advanced level. Specially, the temperature stability is less than 0.10 ns/degree C in 5-45 degree C range

  4. Progress in fission product nuclear data. No. 14

    International Nuclear Information System (INIS)

    Lammer, M.

    1994-06-01

    This is the 14th issue of a report series on Fission Product Nuclear Data published by the Nuclear Data Section of the IAEA. The types of activities included are measurements, compilations and evaluations of fission product yields, neutron reaction cross sections of fission products, data related to the radioactive decay of fission products, delayed neutron data from neutron induced and spontaneous fission, lumped fission product data. The first part of the report consists of unaltered original contributions which the authors have sent to IAEA/NDS. The second part contains some recent references relative to fission product nuclear data, which were not covered by the contributions submitted, and selected papers from conferences. The third part contains requirements for further measurements

  5. Progress in fission product nuclear data. No. 13

    International Nuclear Information System (INIS)

    Lammer, M.

    1990-11-01

    This is the 13th issue of a report series published by the Nuclear Data Section of the IAEA. The types of activities included are measurements, compilations and evaluations of: Fission product yields (neutron induced and spontaneous fission), neutron reaction cross-sections of fission products, data related to the radioactive decay of fission products, delayed neutron data of fission products and bumped fission product data (decay heat, absorption, etc.). The first part of the report consists of unaltered original data which the authors have sent to IAEA/NDS. The second part contains some recent references relative to fission product nuclear data, which were not covered by the contributions submitted, and selected papers from conferences. Part 3 contains requirements for further measurements

  6. Bimodal nature in low-energy fission of light actinides

    International Nuclear Information System (INIS)

    Nagame, Yuichiro; Nishinaka, Ichiro; Tsukada, Kazuaki; Ikezoe, Hiroshi; Otsuki, Tsutomu; Sueki, Keisuke; Nakahara, Hiromichi; Kudo, Hisaaki.

    1995-01-01

    To solve various problems in the mass division process of light actinoids, some experiments on the basis of bimodal fission were carried. Mass and kinetic energy distribution of Th-232 and U-238 were determined. Pa-225 (N= 134) and Pa-227 (N=136), fission nuclei, were produced by Bi-209 + 0-16 and Bi-209 + 0-18 heavy ion nucleus reactions, and the mass yield distribution were determined by the time-of-flight method and the radiochemical procedure. From the results, two independent deforming processes were proved in the fission process of light actinoid nuclei. On the deforming process through the low fission barrier, nucleus fissioned after small deformation under the influence of stabilization of the shell structure of fission product. In the case of process through the high barrier, however, the nucleus fissioned after large deformation. The unsymmetrical mass division was derived from the former and the symmetrical one from the latter. (S.Y.)

  7. Calculated apparent yields of rare gas fission products

    International Nuclear Information System (INIS)

    Delucchi, A.A.

    1975-01-01

    The apparent fission yield of the rare gas fission products from four mass chains is calculated as a function of separation time for six different fissioning systems. A plot of the calculated fission yield along with a one standard deviation error band is given for each rare gas fission product and for each fissioning system. Those parameters in the calculation that were major contributors to the calculated standard deviation at each separation time were identified and the results presented on a separate plot. To extend the usefulness of these calculations as new and better values for the input parameters become available, a third plot was generated for each system which shows how sensitive the derived fission yield is to a change in any given parameter used in the calculation. (U.S.)

  8. Nano-Second Isomers in Neutron-Rich Ni Region Produced by Deep-Inelastic Collisions

    International Nuclear Information System (INIS)

    Ishii, T.; Asai, M.; Matsuda, M.; Ichikawa, S.; Makishima, A.; Hossain, I.; Kleinheinz, P.; Ogawa, M.

    2001-01-01

    Nuclear structure of the doubly magic 68 Ni and its neighbors has been studied by spectroscopic techniques. Developing a new instrument isomer-scope, we have measured γ rays from nano-second isomers produced in heavy-ion deep-inelastic collisions with great sensitivity. (author)

  9. A new isomer in 195Bi identified at the focal plane of HYRA

    International Nuclear Information System (INIS)

    Roy, T.; Mukherjee, G.; Asgar, Md. A.

    2014-01-01

    Due to the presence of high-j (h 9/2 and i 13/2 ) orbitals near the proton and neutron Fermi levels, high spin isomers are expected to occur for neutron deficient Bismuth nuclei (Z = 83) in A = 190 region. A 750 ns isomer has been known for a long time in 195 Bi whose excitation energy and decay path have been reported recently. A rotational band has been reported in this nucleus based on 13/2 + isomer, originated from the deformation driving i 13/2 orbital. This band reported to have prompt feeding through a 457 keV γ-ray apart from a strong feeding from the 750 ns isomer. In 193 Bi, the 29/2 - state is a 3μs isomer, another isomer with half-life >10μs is also known in this nucleus but its excitation energy, spin and parity are not known. Similar isomer has not yet been observed in 195 Bi. The aim of the present work was to find isomers and their decays in 193,195 Bi

  10. The behaviour of EDDHA isomers in soils as influenced by soil properties.

    NARCIS (Netherlands)

    Schenkeveld, W.D.C.; Reichwein, A.M.; Temminghoff, E.J.M.; Riemsdijk, van W.H.

    2007-01-01

    FeEDDHA products are applied to correct iron chlorosis in plants and consist of a mixture of EDDHA isomers chelated to iron. In this study such mixtures have been divided into four (groups of) isomers: racemic o,o-EDDHA, meso o,o-EDDHA, o,p-EDDHA and rest-EDDHA. The physical and chemical properties

  11. Ion mobility studies of carbohydrates as group I adducts: isomer specific collisional cross section dependence on metal ion radius.

    Science.gov (United States)

    Huang, Yuting; Dodds, Eric D

    2013-10-15

    Carbohydrates play numerous critical roles in biological systems. Characterization of oligosaccharide structures is essential to a complete understanding of their functions in biological processes; nevertheless, their structural determination remains challenging in part due to isomerism. Ion mobility spectrometry provides the means to resolve gas phase ions on the basis of their shape-to-charge ratios, thus providing significant potential for separation and differentiation of carbohydrate isomers. Here, we report on the determination of collisional cross sections for four groups of isomeric carbohydrates (including five isomeric disaccharides, four isomeric trisaccharides, two isomeric pentasaccharides, and two isomeric hexasaccharides) as their group I metal ion adducts (i.e., [M + Li](+), [M + Na](+), [M + K](+), [M + Rb](+), and [M + Cs](+)). In all, 65 collisional cross sections were measured, the great majority of which have not been previously reported. As anticipated, the collisional cross sections of the carbohydrate metal ion adducts generally increase with increasing metal ion radius; however, the collisional cross sections were found to scale with the group I cation size in isomer specific manners. Such measurements are of substantial analytical value, as they illustrate how the selection of charge carrier influences carbohydrate ion mobility determinations. For example, certain pairs of isomeric carbohydrates assume unique collisional cross sections upon binding one metal ion, but not another. On the whole, these data suggest a role for the charge carrier as a probe of carbohydrate structure and thus have significant implications for the continued development and application of ion mobility spectrometry for the distinction and resolution of isomeric carbohydrates.

  12. Lutein and Zeaxanthin Isomers in Eye Health and Disease.

    Science.gov (United States)

    Mares, Julie

    2016-07-17

    Current evidence suggests lutein and its isomers play important roles in ocular development in utero and throughout the life span, in vision performance in young and later adulthood, and in lowering risk for the development of common age-related eye diseases in older age. These xanthophyll (oxygen-containing) carotenoids are found in a wide variety of vegetables and fruits, and they are present in especially high concentrations in leafy green vegetables. Additionally, egg yolks and human milk appear to be bioavailable sources. The prevalence of lutein, zeaxanthin, and meso-zeaxanthin in supplements is increasing. Setting optimal and safe ranges of intake requires additional research, particularly in pregnant and lactating women. Accumulating evidence about variable interindividual response to dietary intake of these carotenoids, based on genetic or metabolic influences, suggests that there may be subgroups that benefit from higher levels of intake and/or alternate strategies to improve lutein and zeaxanthin status.

  13. Statistical and dynamical modeling of heavy-ion fusion-fission reactions

    Science.gov (United States)

    Eslamizadeh, H.; Razazzadeh, H.

    2018-02-01

    A modified statistical model and a four dimensional dynamical model based on Langevin equations have been used to simulate the fission process of the excited compound nuclei 207At and 216Ra produced in the fusion 19F + 188Os and 19F + 197Au reactions. The evaporation residue cross section, the fission cross section, the pre-scission neutron, proton and alpha multiplicities and the anisotropy of fission fragments angular distribution have been calculated for the excited compound nuclei 207At and 216Ra. In the modified statistical model the effects of spin K about the symmetry axis and temperature have been considered in calculations of the fission widths and the potential energy surfaces. It was shown that the modified statistical model can reproduce the above mentioned experimental data by using appropriate values of the temperature coefficient of the effective potential equal to λ = 0.0180 ± 0.0055, 0.0080 ± 0.0030 MeV-2 and the scaling factor of the fission barrier height equal to rs = 1.0015 ± 0.0025, 1.0040 ± 0.0020 for the compound nuclei 207At and 216Ra, respectively. Three collective shape coordinates plus the projection of total spin of the compound nucleus on the symmetry axis, K, were considered in the four dimensional dynamical model. In the dynamical calculations, dissipation was generated through the chaos weighted wall and window friction formula. Comparison of the theoretical results with the experimental data showed that two models make it possible to reproduce satisfactorily the above mentioned experimental data for the excited compound nuclei 207At and 216Ra.

  14. Statistical and dynamical modeling of heavy-ion fusion–fission reactions

    Directory of Open Access Journals (Sweden)

    H. Eslamizadeh

    2018-02-01

    Full Text Available A modified statistical model and a four dimensional dynamical model based on Langevin equations have been used to simulate the fission process of the excited compound nuclei 207At and 216Ra produced in the fusion 19F + 188Os and 19F + 197Au reactions. The evaporation residue cross section, the fission cross section, the pre-scission neutron, proton and alpha multiplicities and the anisotropy of fission fragments angular distribution have been calculated for the excited compound nuclei 207At and 216Ra. In the modified statistical model the effects of spin K about the symmetry axis and temperature have been considered in calculations of the fission widths and the potential energy surfaces. It was shown that the modified statistical model can reproduce the above mentioned experimental data by using appropriate values of the temperature coefficient of the effective potential equal to λ=0.0180±0.0055, 0.0080±0.0030 MeV−2 and the scaling factor of the fission barrier height equal to rs=1.0015±0.0025, 1.0040±0.0020 for the compound nuclei 207At and 216Ra, respectively. Three collective shape coordinates plus the projection of total spin of the compound nucleus on the symmetry axis, K, were considered in the four dimensional dynamical model. In the dynamical calculations, dissipation was generated through the chaos weighted wall and window friction formula. Comparison of the theoretical results with the experimental data showed that two models make it possible to reproduce satisfactorily the above mentioned experimental data for the excited compound nuclei 207At and 216Ra.

  15. Axisymmetric Magnetic Mirror Fusion-Fission Hybrid

    Energy Technology Data Exchange (ETDEWEB)

    Moir, R. W. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Martovetsky, N. N. [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Molvik, A. W. [Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Ryutov, D. D. [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Simonen, T. C. [Univ. of California, Berkeley, CA (United States)

    2011-05-13

    The achieved performance of the gas dynamic trap version of magnetic mirrors and today’s technology we believe are sufficient with modest further efforts for a neutron source for material testing (Q=Pfusion/Pinput~0.1). The performance needed for commercial power production requires considerable further advances to achieve the necessary high Q>>10. An early application of the mirror, requiring intermediate performance and intermediate values of Q~1 are the hybrid applications. The Axisymmetric Mirror has a number of attractive features as a driver for a fusion-fission hybrid system: geometrical simplicity, inherently steady-state operation, and the presence of the natural divertors in the form of end tanks. This level of physics performance has the virtue of low risk and only modest R&D needed and its simplicity promises economy advantages. Operation at Q~1 allows for relatively low electron temperatures, in the range of 4 keV, for the DT injection energy ~ 80 keV. A simple mirror with the plasma diameter of 1 m and mirror-to-mirror length of 35 m is discussed. Simple circular superconducting coils are based on today’s technology. The positive ion neutral beams are similar to existing units but designed for steady state. A brief qualitative discussion of three groups of physics issues is presented: axial heat loss, MHD stability in the axisymmetric geometry, microstability of sloshing ions. Burning fission reactor wastes by fissioning actinides (transuranics: Pu, Np, Am, Cm, .. or just minor actinides: Np, Am, Cm, …) in the hybrid will multiply fusion’s energy by a factor of ~10 or more and diminish the Q needed to less than 1 to overcome the cost of recirculating power for good economics. The economic value of destroying actinides by fissioning is rather low based on either the cost of long-term storage or even deep geologic disposal so most of the revenues of hybrids will come from electrical power. Hybrids that obtain revenues from

  16. Comparative Autoignition Trends in Butanol Isomers at Elevated Pressure

    KAUST Repository

    Weber, Bryan W.

    2013-03-21

    Autoignition experiments of stoichiometric mixtures of s-, t-, and i-butanol in air have been performed using a heated rapid compression machine (RCM). At compressed pressures of 15 and 30 bar and for compressed temperatures in the range 715-910 K, no evidence of a negative temperature coefficient region in terms of ignition delay response is found. The present experimental results are also compared with previously reported RCM data of n-butanol in air. The order of reactivity of the butanols is n-butanol > s-butanol ≈ i-butanol > t-butanol at the lower pressure but changes to n-butanol > t-butanol > s-butanol > i-butanol at higher pressure. In addition, t-butanol shows preignition heat release behavior, which is especially evident at higher pressures. To help identify the controlling chemistry leading to this preignition heat release, off-stoichiometric experiments are further performed at 30 bar compressed pressure, for t-butanol at φ = 0.5 and φ = 2.0 in air. For these experiments, higher fuel loading (i.e., φ = 2.0) causes greater preignition heat release (as indicated by greater pressure rise) than the stoichiometric or φ = 0.5 cases. Comparison of the experimental ignition delays with the simulated results using two literature kinetic mechanisms shows generally good agreement, and one mechanism is further used to explore and compare the fuel decomposition pathways of butanol isomers. Using this mechanism, the importance of peroxy chemistry in the autoignition of the butanol isomers is highlighted and discussed. © 2013 American Chemical Society.

  17. K-Isomers as a Probe of Nuclear Structure and Advanced Applications

    Science.gov (United States)

    Kondev, F. G.

    2005-05-01

    Nuclear K-isomers play a pivotal role in understanding the structure of deformed, axially symmetric nuclei. Examples are presented of recent studies of exotic multi-quasiparticle isomers in the A˜180 rare-earth region at the extreme of angular momentum and neutron number. A specific band-mixing scenario is invoked to explain the unusual decay path of the Kπ=57/2- isomer (T1/2=22 ns) in 175Hf, the highest spin K-isomer known in nature. The discovery of a suite of high-K isomers, above the previously known Kπ=23/2- (T1/2=160 d) state in 177Lu, using deep-inelastic and multi-nucleon transfer reactions is discussed.

  18. K-Isomers as a Probe of Nuclear Structure and Advanced Applications

    International Nuclear Information System (INIS)

    Kondev, F.G.

    2005-01-01

    Nuclear K-isomers play a pivotal role in understanding the structure of deformed, axially symmetric nuclei. Examples are presented of recent studies of exotic multi-quasiparticle isomers in the A∼180 rare-earth region at the extreme of angular momentum and neutron number. A specific band-mixing scenario is invoked to explain the unusual decay path of the Kπ=57/2- isomer (T1/2=22 ns) in 175Hf, the highest spin K-isomer known in nature. The discovery of a suite of high-K isomers, above the previously known Kπ=23/2- (T1/2=160 d) state in 177Lu, using deep-inelastic and multi-nucleon transfer reactions is discussed

  19. Aqueous phase partitioning of hexachlorocyclohexane (HCH) isomers by biosurfactant produced by Pseudomonas aeruginosa WH-2

    International Nuclear Information System (INIS)

    Sharma, Suman; Singh, Partapbir; Raj, Mayil; Chadha, Bhupinder Singh; Saini, Harvinder Singh

    2009-01-01

    The different isomers of technical-grade hexachlorocyclohexane (t-HCH) including the insecticidal γ-isomer, commonly known as lindane, have been reported to be toxic, carcinogenic and endocrine disrupters. The spatial arrangements of the chlorine atoms on different isomers and low aqueous phase solubility contribute to their persistence in environment, β-HCH being the most resistance to transformation. The biosurfactant preparation of Pseudomonas aeruginosa isolate WH-2 was evaluated for its ability to improve the aqueous phase partitioning of different isomers of HCH-muck. Further, the ability of biosurfactant preparation to emulsify HCH and n-hexadecane was checked under different conditions, usually characteristic of sites contaminated with pollutants viz. wide range of pH, temperature, and salinity. The data obtained from this study will be helpful in designing suitable bioremediation strategies for huge stock piles of HCH-muck and sites polluted by reckless use/disposal of HCH-isomers.

  20. Investigation of the heavy nuclei fission with anomalously high values of the fission fragments total kinetic energy

    Science.gov (United States)

    Khryachkov, Vitaly; Goverdovskii, Andrei; Ketlerov, Vladimir; Mitrofanov, Vecheslav; Sergachev, Alexei

    2018-03-01

    Binary fission of 232Th and 238U induced by fast neutrons were under intent investigation in the IPPE during recent years. These measurements were performed with a twin ionization chamber with Frisch grids. Signals from the detector were digitized for further processing with a specially developed software. It results in information of kinetic energies, masses, directions and Bragg curves of registered fission fragments. Total statistics of a few million fission events were collected during each experiment. It was discovered that for several combinations of fission fragment masses their total kinetic energy was very close to total free energy of the fissioning system. The probability of such fission events for the fast neutron induced fission was found to be much higher than for spontaneous fission of 252Cf and thermal neutron induced fission of 235U. For experiments with 238U target the energy of incident neutrons were 5 MeV and 6.5 MeV. Close analysis of dependence of fission fragment distribution on compound nucleus excitation energy gave us some explanation of the phenomenon. It could be a process in highly excited compound nucleus which leads the fissioning system from the scission point into the fusion valley with high probability.

  1. Investigation of the heavy nuclei fission with anomalously high values of the fission fragments total kinetic energy

    Directory of Open Access Journals (Sweden)

    Khryachkov Vitaly

    2018-01-01

    Full Text Available Binary fission of 232Th and 238U induced by fast neutrons were under intent investigation in the IPPE during recent years. These measurements were performed with a twin ionization chamber with Frisch grids. Signals from the detector were digitized for further processing with a specially developed software. It results in information of kinetic energies, masses, directions and Bragg curves of registered fission fragments. Total statistics of a few million fission events were collected during each experiment. It was discovered that for several combinations of fission fragment masses their total kinetic energy was very close to total free energy of the fissioning system. The probability of such fission events for the fast neutron induced fission was found to be much higher than for spontaneous fission of 252Cf and thermal neutron induced fission of 235U. For experiments with 238U target the energy of incident neutrons were 5 MeV and 6.5 MeV. Close analysis of dependence of fission fragment distribution on compound nucleus excitation energy gave us some explanation of the phenomenon. It could be a process in highly excited compound nucleus which leads the fissioning system from the scission point into the fusion valley with high probability.

  2. Neutron emission as a clock and thermometer to probe the dynamics of fusion-fission and quasi-fission

    Science.gov (United States)

    Hinde, D. J.

    1993-03-01

    A compilation of currently available data on pre-scission neutron multiplicities shows clearly that the excitation energy in the fission fragments hardly increases with bombarding energy. This can be explained if fission is always a slow process, whilst evaporation becomes more and more rapid. The neutron clock-thermometer is introduced as a tool to deduce the dynamical timescale for fusion-fission, giving (35±15)×10-21 s. Quasi-fission is faster than fusion-fission because the equilibrium deformation is never reached (the mononucleus is thought to be always very deformed) thus fragment temperatures are higher, and the strong variation of vpre with TKE shows that a significant number of neutrons are emitted while the fragments are accelerating after scission. This appears not to be the case for fusion-fission. The fall in vpre for asymmetric mass-splits suggests that the dynamical time scale is shorter: this will influence fission mass-distributions.

  3. Progress in the investigation of fission fragment angular anisotropy in the resonance neutron induced fission of aligned 235U target

    Science.gov (United States)

    Furman, W. I.; Kopach, Yu. N.; Popov, A. B.; Gonin, N. N.; Kozlovsky, L. K.; Tambovtsev, D. I.; Kliman, J.; Postma, H.

    1998-10-01

    New results of the analysis of experimental data on angular anisotropy of fission fragments in the neutron induced fission of aligned 235U nuclei are reported. A new approach to the theoretical description of the fission process led to the modified formulate for the differential fission cross sections. An R-matrix formalism was applied for the data analysis using the modified code SAMMY and the original code on the basis of the FUMILI procedure. The obtained values of the angular anisotropy coefficients A2(E) were analyzed together with the total neutron, total fission and spin separated fission cross sections in dependence on neutron energy E. Three fission channels were taken into account for the spin J=3 (K=0,1,2) and two for the spin J=4 (K=1,2).

  4. Multiple-scattering Corrections to Measurements of the Prompt Fission Neutron Spectrum

    Science.gov (United States)

    Taddeucci, T. N.; Haight, R. C.; Lee, H. Y.; Neudecker, D.; O'Donnell, J. M.; White, M. C.; Perdue, B. A.; Devlin, M.; Fotiadis, N.; Ullmann, J. L.; Nelson, R. O.; Bredeweg, T. A.; Rising, M. E.; Sjue, S. K.; Wender, S. A.; Wu, C. Y.; Henderson, R.

    2015-01-01

    The Chi-Nu project, conducted jointly by LANL and LLNL, aims to measure the shape of the prompt fission neutron spectrum (PFNS) for fission of 239Pu induced by neutrons from 50 keV to 15 MeV with accuracies of 3-5% in the outgoing energy from 50 keV to 9 MeV and 15% from 9 to 15 MeV. In order to meet this goal, detailed Monte Carlo simulations are being used to assess the importance and effect of every component in the experimental configuration. As part of this effort, we have also simulated some past PFNS measurements to identify possible sources of systematic error. We find that multiple scattering plays an important role in the target geometry, collimators, and detector response and that past experiments probably underestimated the extent of this effect.

  5. Multiple-scattering Corrections to Measurements of the Prompt Fission Neutron Spectrum

    Energy Technology Data Exchange (ETDEWEB)

    Taddeucci, T.N., E-mail: taddeucci@lanl.gov [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States); Haight, R.C.; Lee, H.Y.; Neudecker, D.; O' Donnell, J.M.; White, M.C.; Perdue, B.A.; Devlin, M.; Fotiadis, N.; Ullmann, J.L.; Nelson, R.O.; Bredeweg, T.A.; Rising, M.E.; Sjue, S.K.; Wender, S.A. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States); Wu, C.Y.; Henderson, R. [Lawrence Livermore National Laboratory, Livermore, CA 94551 (United States)

    2015-01-15

    The Chi-Nu project, conducted jointly by LANL and LLNL, aims to measure the shape of the prompt fission neutron spectrum (PFNS) for fission of {sup 239}Pu induced by neutrons from 50 keV to 15 MeV with accuracies of 3–5% in the outgoing energy from 50 keV to 9 MeV and 15% from 9 to 15 MeV. In order to meet this goal, detailed Monte Carlo simulations are being used to assess the importance and effect of every component in the experimental configuration. As part of this effort, we have also simulated some past PFNS measurements to identify possible sources of systematic error. We find that multiple scattering plays an important role in the target geometry, collimators, and detector response and that past experiments probably underestimated the extent of this effect.

  6. Fission cross section measurement of Am-242m using lead slowing-down spectrometer

    Energy Technology Data Exchange (ETDEWEB)

    Kai, Tetsuya; Kobayashi, Katsuhei; Yamamoto, Shuji; Fujita, Yoshiaki [Kyoto Univ., Kumatori, Osaka (Japan). Research Reactor Inst.; Kimura, Itsuro; Ohkawachi, Yasushi; Wakabayashi, Toshio

    1998-03-01

    By making use of double fission chamber and lead slowing-down spectrometer coupled to an electron linear accelerator, fission cross section for the {sup 242m}Am(n,f) reaction has been measured relative to that for the {sup 235}U(n,f) reaction in the energy range from 0.1 eV to 10 keV. The measured result was compared with the evaluated nuclear data appeared in ENDF/B-VI and JENDL-3.2, of which evaluated data were broadened by the energy resolution function of the spectrometer. Although the JENDL-3.2 data seem to be a little smaller than the present measurement, good agreement can be seen in the general shape and the absolute values. The ENDF/B-VI data are larger more than 50 % than the present values above 3 eV. (author)

  7. Etching behavior of fission fragment tracks in synthetic quartz and its application to neutron detection

    International Nuclear Information System (INIS)

    Sawamura, Teruko; Baba, Satoshi; Narita, Masakuni; Yamazaki, Hatsuo

    1994-01-01

    The etching behavior of fission fragment tracks in synthetic quartz plates concerning to +x, y and z planes was studied using NaOH solution as an etchant. Systematic experiments gave an optimum etching condition of 65% NaOH at 150degC suitable for track detection. Under this etching condition, following several properties were studied; the bulk etching rate, the etched track opening shape and its growth rate, the critical angle of track etching, and the irradiation effect of low LET radiation. All of three different cuts were demonstrated to be useful for plates as fission track detectors. An application to neutron detection was studied for the +x-plane of an x-cut plate. The detection sensitivity of the plane in close contact with a Th-radiator was 2.7x10 -6 tracks/fluence for 14 MeV neutrons. (author)

  8. Physics and chemistry of fission. Proceedings of the second IAEA symposium

    International Nuclear Information System (INIS)

    1969-01-01

    Fission studies have developed rapidly and significantly since the first IAEA Symposium on the Physics and Chemistry of Fission, held in 1965 in Salzburg. Several surprising discoveries and some excellent experimental results have given rise to many new theoretical investigations. From the individual theoretical models, laboriously improved and carefully fitted to the experimental data, a more general theoretical picture has begun to take shape and this has provided fresh ideas for experimental work. The Second Symposium on the Physics and Chemistry of Fission, held at the IAEA Headquarters in Vienna from 28 July to 1 August 1969, was a short pause in the rapid flow of developing theoretical concepts and new experimental investigations; it was devoted to the discussion, comparison and analysis of the recent achievements, and to a glance at the way fission studies are likely to develop in the near future. Two facts, the emphasis on theory and the important interplay of theory and experiment, left a strong mark on the contributions and discussions. The number of papers dealing with theoretical aspects is substantially larger than at the earlier symposium; this points to the fact that with increased efforts the theoreticians have succeeded in narrowing the wide gap between the large amount of empirical data and the theoretical understanding of it. The titles of individual sessions indicate the new trends in fission research. Theories of fragment distribution, shell structure effects in fissioning nuclei, intermediate structure, and isomeric fission are topics which were discussed with a great deal of uncertainty at the Salzburg symposium. At the present meeting, they were far more prominent and they were argued with great confidence and with the intensity and enthusiasm that only such exciting ideas can arouse. From the extensiveness of the discussion records the vivid interest of the participants is clearly seen; the pertinent problems still to be solved are also

  9. Correlation of errors in the Monte Carlo fission source and the fission matrix fundamental-mode eigenvector

    International Nuclear Information System (INIS)

    Dufek, Jan; Holst, Gustaf

    2016-01-01

    Highlights: • Errors in the fission matrix eigenvector and fission source are correlated. • The error correlations depend on coarseness of the spatial mesh. • The error correlations are negligible when the mesh is very fine. - Abstract: Previous studies raised a question about the level of a possible correlation of errors in the cumulative Monte Carlo fission source and the fundamental-mode eigenvector of the fission matrix. A number of new methods tally the fission matrix during the actual Monte Carlo criticality calculation, and use its fundamental-mode eigenvector for various tasks. The methods assume the fission matrix eigenvector is a better representation of the fission source distribution than the actual Monte Carlo fission source, although the fission matrix and its eigenvectors do contain statistical and other errors. A recent study showed that the eigenvector could be used for an unbiased estimation of errors in the cumulative fission source if the errors in the eigenvector and the cumulative fission source were not correlated. Here we present new numerical study results that answer the question about the level of the possible error correlation. The results may be of importance to all methods that use the fission matrix. New numerical tests show that the error correlation is present at a level which strongly depends on properties of the spatial mesh used for tallying the fission matrix. The error correlation is relatively strong when the mesh is coarse, while the correlation weakens as the mesh gets finer. We suggest that the coarseness of the mesh is measured in terms of the value of the largest element in the tallied fission matrix as that way accounts for the mesh as well as system properties. In our test simulations, we observe only negligible error correlations when the value of the largest element in the fission matrix is about 0.1. Relatively strong error correlations appear when the value of the largest element in the fission matrix raises

  10. Preparative electrophoresis of industrial fission product solutions

    International Nuclear Information System (INIS)

    Tret, Joel

    1971-07-01

    The aim of this work is to contribute to the development of the continuous electrophoresis technique while studying its application in the preparative electrophoresis of industrial fission product solutions. The apparatus described is original. It was built for the purposes of the investigation and proved very reliable in operation. The experimental conditions necessary to maintain and supervise the apparatus in a state of equilibrium are examined in detail; their stability is an important factor, indispensable to the correct performance of an experiment. By subjecting an industrial solution of fission products to preparative electrophoresis it is possible, according to the experimental conditions, to prepare carrier-free radioelements of radiochemical purity (from 5 to 7 radioelements): 137 Cs, 90 Sr, 141+144 Ce, 91 Y, 95 Nb, 95 Zr, 103+106 Ru. (author) [fr

  11. Fission Surface Power Technology Development Status

    Science.gov (United States)

    Palac, Donald T.; Mason, Lee S.; Harlow, Scott

    2009-01-01

    With the potential future deployment of a lunar outpost there is expected to be a clear need for a high-power, lunar surface power source to support lunar surface operations independent of the day-night cycle, and Fission Surface Power (FSP) is a very effective solution for power levels above a couple 10 s of kWe. FSP is similarly enabling for the poorly illuminated surface of Mars. The power levels/requirements for a lunar outpost option are currently being studied, but it is known that cost is clearly a predominant concern to decision makers. This paper describes the plans of NASA and the DOE to execute an affordable fission surface power system technology development project to demonstrate sufficient technology readiness of an affordable FSP system so viable and cost-effective FSP system options will be available when high power lunar surface system choices are expected to be made in the early 2010s.

  12. Fusion-fission energy systems evaluation

    International Nuclear Information System (INIS)

    Teofilo, V.L.; Aase, D.T.; Bickford, W.E.

    1980-01-01

    This report serves as the basis for comparing the fusion-fission (hybrid) energy system concept with other advanced technology fissile fuel breeding concepts evaluated in the Nonproliferation Alternative Systems Assessment Program (NASAP). As such, much of the information and data provided herein is in a form that meets the NASAP data requirements. Since the hybrid concept has not been studied as extensively as many of the other fission concepts being examined in NASAP, the provided data and information are sparse relative to these more developed concepts. Nevertheless, this report is intended to provide a perspective on hybrids and to summarize the findings of the rather limited analyses made to date on this concept

  13. 60 years controlled nuclear fission: CP-1

    International Nuclear Information System (INIS)

    Anon.

    2002-01-01

    On December 2, 1942, the Chicago Pile 1 (CP-1) went critical for the first time. In this way, the scientists and engineers involved in the project under the leadership of Enrico Fermi succeeded in demonstrating that a self-sustaining nuclear reaction with nuclear fission processes was technically feasible. Only four years after the discovery and proof of nuclear fission by Otto Hahn, Fritz Strassmann, and Lise Meitner, the experiment consisting of graphite blocks as the moderator and uranium dioxide pellets as the fuel, as well as instrumentation and control devices, had been set up in the former squash court of the field and track stadium of the University of Chicago. Precisely at 3.36 a.m. Chicago time, after control rods had been withdrawn, the instruments showed the chain reaction by the neutron flux they indicated. An important cornerstone in the use of nuclear power had thus been laid. (orig.)

  14. Anisotropic Neutron Evaporation from Spinning Fission Fragments

    Science.gov (United States)

    Stuttgé, L.; Dorvaux, O.; Gönnenwein, F.; Mutterer, M.; Kopatch, Yu.; Chernysheva, E.; Hanappe, F.; Hambsch, F.-J.

    2011-10-01

    Neutron evaporation anisotropy in the centre of mass of the rotating fission fragments in the spontaneous fission of 252Cf has been investigated within the CORA experiments. If it is well accepted that the bulk of emitted neutrons originate from an isotropic evaporation in the centre of mass of the moving fragments, discrepancies in experimental as well as in theoretical energy and angular distributions appear throughout many attempts performed by various authors. Scission neutrons most probably contribute but don't allow to explain totally the observed anisotropy. Due to its weak contribution to the total anisotropy, the centre of mass anisotropy is very difficult to be highlighted. A novel experimental approach has been developed to extract this effect and will be presented as well as some first results.

  15. Fusion-fission energy systems evaluation

    Energy Technology Data Exchange (ETDEWEB)

    Teofilo, V.L.; Aase, D.T.; Bickford, W.E.

    1980-01-01

    This report serves as the basis for comparing the fusion-fission (hybrid) energy system concept with other advanced technology fissile fuel breeding concepts evaluated in the Nonproliferation Alternative Systems Assessment Program (NASAP). As such, much of the information and data provided herein is in a form that meets the NASAP data requirements. Since the hybrid concept has not been studied as extensively as many of the other fission concepts being examined in NASAP, the provided data and information are sparse relative to these more developed concepts. Nevertheless, this report is intended to provide a perspective on hybrids and to summarize the findings of the rather limited analyses made to date on this concept.

  16. Polarization and alignment of nucleus fission fragments

    International Nuclear Information System (INIS)

    Barabanov, A.L.; Grechukhin, D.P.

    1987-01-01

    Correlation of fragment orientation with orientation axis of fissile nucleus and with n-vector f vector of fragment divergence is considered. Estimations of polarization and alignment of fission fragments of preliminarily oriented nuclei in correlation (with n-vector f recording) and integral (with n-vector f averaging) experiments were conducted. It is shown that high sensitivity of polarization and fragment alignment to the character of nucleus movement at the stage of descent from barrier to rupture point exists

  17. Opimization of fusion-driven fissioning systems

    International Nuclear Information System (INIS)

    Chapin, D.L.; Mills, R.G.

    1976-01-01

    Potential advantages of hybrid or fusion/fission systems can be exploited in different ways. With selection of the 238 U-- 239 Pu fuel cycle, we show that the system has greatest value as a power producer. Numerical examples of relative revenue from power production vs. 239 Pu production are discussed, and possible plant characteristics described. The analysis tends to show that the hybrid may be more economically attractive than pure fusion systems

  18. Actinide and fission product partitioning and transmutation

    International Nuclear Information System (INIS)

    1997-01-01

    The fourth international information exchange meeting on actinide and fission product partitioning and transmutation, took place in Mito City in Japan, on 111-13 September 1996. The proceedings are presented in six sessions: the major programmes and international cooperation, the partitioning and transmutation programs, feasibility studies, particular separation processes, the accelerator driven transmutation, and the chemistry of the fuel cycle. (A.L.B.)

  19. Actinide and fission product partitioning and transmutation

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1997-07-01

    The fourth international information exchange meeting on actinide and fission product partitioning and transmutation, took place in Mito City in Japan, on 111-13 September 1996. The proceedings are presented in six sessions: the major programmes and international cooperation, the partitioning and transmutation programs, feasibility studies, particular separation processes, the accelerator driven transmutation, and the chemistry of the fuel cycle. (A.L.B.)

  20. Release of fission products in transients

    International Nuclear Information System (INIS)

    Christensen, H.; Lundqwist, R.

    1979-07-01

    A station for automatic sampling of coolant has been put in operation at the Oskarshamn-1 reactor. The release of 131 J and other fission products in spikes in connection with reactor trips and scheduled shutdowns has been measured. A model developed at General Electric has been used to predict the spike release in Oskarshamn-1 and the predicted values have been compared with experimental values. Literature data of iodine spikes in BWR and PWR have been reviewed. (author)

  1. Fission, fusion and photonuclear physics. Chapter 2

    International Nuclear Information System (INIS)

    Berlanger, M.; Deleplanque, M.A.; Gerschel, C.; Hanappe, F.; Leblanc, M.; Mayault, J.F.; Ngo, C.; Paya, D.; Perrin, N.; Peter, J.; Tamain, B.; Valentin, L.

    The γ-ray multiplicity has been measured for the quasi-fission events in the Cu + Au reaction at 443MeV. Using the usual assumption on the γ-ray multipolarity and estimating the angular momentum carried away by the evaporated particles, a value of 57h is obtained for the angular momentum transferred to the fragments, in agreement with the sticking hypothesis [fr

  2. Fissionable material handlers certification training program

    International Nuclear Information System (INIS)

    Strangeland, J.V.

    1979-07-01

    A formal program for certification of fissionable material handlers is presented that cultivates safe working practices. This certification complies with the training requirements of the Department of Energy Directive 0530 (ERDA Manual Chapter 0530), Nuclear Criticality Safety. The program consists of a series of classroom lectures, on-the-job training, and examinations in criticality safety, radiation protection, industrial safety, emergency procedures, and the employee's specific work operations. The program for recertification is also discussed

  3. Measurement of fission fragments energy loss

    CERN Document Server

    Benetti, P; Calligarich, E; Cesana, A; Dolfini, R; Ioppolo, T; Raselli, G L; Terrani, M

    2002-01-01

    The mean energy of sup 2 sup 5 sup 2 Cf fission fragments emerging from an absorber and the determination of the capture rate in the absorber itself have been measured using two independent and complementary nuclear techniques. The results can be applied to the measurement of the energy self-absorption in a non-zero thickness source and can be used to validate simulation programs.

  4. Cumulative and Averaging Fission of Beliefs

    OpenAIRE

    Josang, Audun

    2007-01-01

    Belief fusion is the principle of combining separate beliefs or bodies of evidence originating from different sources. Depending on the situation to be modelled, different belief fusion methods can be applied. Cumulative and averaging belief fusion is defined for fusing opinions in subjective logic, and for fusing belief functions in general. The principle of fission is the opposite of fusion, namely to eliminate the contribution of a specific belief from an already fused belief, with the pur...

  5. Enhanced E3 transitions and mixed configurations for core excited isomers in 210At and 211At

    International Nuclear Information System (INIS)

    Dracoulis, G.D.; Steed, C.A.; Byrne, A.P.; Poletti, S.J.; Stuchbery, A.E.; Bark, R.A.

    1986-09-01

    The lifetime and branching ratio of the 19 + isomer in 210 At have been measured. Its enhanced E3 decay and g-factor, and those of the related 39/2 - isomer in 211 At are compared with the results of a semi-empirical shell model calculation which includes couplings to the 3 - octupole vibration, resulting in mixed configurations. Lifetimes were also obtained for the 15 - isomer in 210 At, and he 29/2 + isomer in 209 At

  6. Neutron-neutron angular correlations in spontaneous fission of 252Cf and 240Pu

    Science.gov (United States)

    Verbeke, J. M.; Nakae, L. F.; Vogt, R.

    2018-04-01

    Background: Angular anisotropy has been observed between prompt neutrons emitted during the fission process. Such an anisotropy arises because the emitted neutrons are boosted along the direction of the parent fragment. Purpose: To measure the neutron-neutron angular correlations from the spontaneous fission of 252Cf and 240Pu oxide samples using a liquid scintillator array capable of pulse-shape discrimination. To compare these correlations to simulations combining the Monte Carlo radiation transport code MCNPX with the fission event generator FREYA. Method: Two different analysis methods were used to study the neutron-neutron correlations with varying energy thresholds. The first is based on setting a light output threshold while the second imposes a time-of-flight cutoff. The second method has the advantage of being truly detector independent. Results: The neutron-neutron correlation modeled by FREYA depends strongly on the sharing of the excitation energy between the two fragments. The measured asymmetry enabled us to adjust the FREYA parameter x in 240Pu, which controls the energy partition between the fragments and is so far inaccessible in other measurements. The 240Pu data in this analysis was the first available to quantify the energy partition for this isotope. The agreement between data and simulation is overall very good for 252Cf(sf ) and 240Pu(sf ) . Conclusions: The asymmetry in the measured neutron-neutron angular distributions can be predicted by FREYA. The shape of the correlation function depends on how the excitation energy is partitioned between the two fission fragments. Experimental data suggest that the lighter fragment is disproportionately excited.

  7. Near Term Fission-Fusion Hybrids- Advantages for Fission and Fusion

    Science.gov (United States)

    Kotschenreuther, M.; Mahajan, S.; Valanju, P.

    2010-11-01

    Fission-fusion hybrids are described with unique advantages relative to fission only systems, for different missions. Innovative designs allow hybrids to incinerate waste, or produce fuel, with far fewer hybrids than would be possible with fission-only fast reactors. In addition, hybrids can perform these missions while addressing concerns regarding proliferation, by using unique fuel cycles, not accessible to fission alone, that use no reprocessing, or greatly reduced reprocessing. These goals can be achieved using fusion devices in the range considered for fusion Component Test Facilities (CTF). The fusion physics and fusion engineering performance necessary for these missions is far less stringent than for a pure fusion power reactor. Unique designs aspects substantially separate the fission and fusion aspects, allowing much more independent development of each. Hence, a suitable hybrid can provide a nearer term, lower risk, application for fusion, and be an additional incentive to implement a fusion CTF device. The fuel cycle possibilities above are verified using Monte-Carlo neutron calculations. Fusion neutron sources with high power densities and modest power levels are sufficient and necessary.

  8. Shell effects in fission and quasi-fission of heavy and superheavy nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Itkis, M.G. E-mail: itkis@flnr.jinr.ru; Aeystoe, J.; Beghini, S.; Bogachev, A.A.; Corradi, L.; Dorvaux, O.; Gadea, A.; Giardina, G.; Hanappe, F.; Itkis, I.M.; Jandel, M.; Kliman, J.; Khlebnikov, S.V.; Kniajeva, G.N.; Kondratiev, N.A.; Kozulin, E.M.; Krupa, L.; Latina, A.; Materna, T.; Montagnoli, G.; Oganessian, Yu.Ts.; Pokrovsky, I.V.; Prokhorova, E.V.; Rowley, N.; Rubchenya, V.A.; Rusanov, A.Ya.; Sagaidak, R.N.; Scarlassara, F.; Stefanini, A.M.; Stuttge, L.; Szilner, S.; Trotta, M.; Trzaska, W.H.; Vakhtin, D.N.; Vinodkumar, A.M.; Voskressenski, V.M.; Zagrebaev, V.I

    2004-04-05

    Results of the experiments aimed at the study of fission and quasi-fission processes in the reactions {sup 12}C+{sup 204}Pb, {sup 48}Ca+{sup 144,154}Sm, {sup 168}Er, {sup 208}Pb, {sup 244}Pu, {sup 248}Cm; {sup 58}Fe+{sup 208}Pb, {sup 244}Pu, {sup 248}Cm, and {sup 64}Ni+{sup 186}W, {sup 242}Pu are presented in the work. The choice of the above-mentioned reactions was inspired by recent experiments on the production of the isotopes {sup 283}112, {sup 289}114 and {sup 283}116 at Dubna [1],[2] using the same reactions. The {sup 58}Fe and {sup 64}Ni projectiles were chosen since the corresponding projectile-target combinations lead to the synthesis of even heavier elements. The experiments were carried out at the U-400 accelerator of the Flerov Laboratory of Nuclear Reactions (JINR, Russia), the XTU Tandem accelerator of the National Laboratory of Legnaro (LNL, Italy) and the Accelerator of the Laboratory of University of Jyvaskyla (JYFL, Finland) using the time-of-flight spectrometer of fission fragments CORSET[3] and the neutron multi-detector DEMON[4],[5]. The role of shell effects and the influence of the entrance channel on the mechanism of the compound nucleus fusion-fission and the competitive process of quasi-fission are discussed.

  9. Temperature dependence of nuclear fission time in heavy-ion fusion-fission reactions

    Science.gov (United States)

    Eccles, Chris; Roy, Sanil; Gray, Thomas H.; Zaccone, Alessio

    2017-11-01

    Accounting for viscous damping within Fokker-Planck equations led to various improvements in the understanding and analysis of nuclear fission of heavy nuclei. Analytical expressions for the fission time are typically provided by Kramers' theory, which improves on the Bohr-Wheeler estimate by including the time scale related to many-particle dissipative processes along the deformation coordinate. However, Kramers' formula breaks down for sufficiently high excitation energies where Kramers' assumption of a large barrier no longer holds. Focusing on the overdamped regime for energies T >1 MeV, Kramers' theory should be replaced by a new analytical theory derived from the Ornstein-Uhlenbeck first-passage time method that is proposed here. The theory is applied to fission time data from fusion-fission experiments on 16O+208Pb→224Th . The proposed model provides an internally consistent one-parameter fitting of fission data with a constant nuclear friction as the fitting parameter, whereas Kramers' fitting requires a value of friction which falls out of the allowed range. The theory provides also an analytical formula that in future work can be easily implemented in numerical codes such as cascade or joanne4.

  10. Increased Exploration Capacity Promotes Group Fission in Gregarious Foraging Herbivores.

    Directory of Open Access Journals (Sweden)

    Sophie Lardy

    Full Text Available Many gregarious species display rapid fission-fusion dynamics with individuals frequently leaving their groups to reunite or to form new ones soon after. The adaptive value of such ephemeral associations might reflect a frequent tilt in the balance between the costs and benefits of maintaining group cohesion. The lack of information on the short-term advantages of group fission, however, hampers our understanding of group dynamics. We investigated the effect of group fission on area-restricted search, a search tactic that is commonly used when food distribution is spatially autocorrelated. Specifically, we determine if roe deer (Capreolus capreolus improve key aspects of their extensive search mode immediately after fission. We found that groups indeed moved faster and farther over time immediately after than before fission. This gain was highest for the smallest group that resulted from fission, which was more likely to include the fission's initiator. Sex of group members further mediated the immediate gain in search capacity, as post-fission groups moved away at farthest rate when they were only comprised of males. Our study suggests that social conflicts during the extensive search mode can promote group fission and, as such, can be a key determinant of group fission-fusion dynamics that are commonly observed in gregarious herbivores.

  11. General Description of Fission Observables - JEFF Report 24. GEF Model

    International Nuclear Information System (INIS)

    Schmidt, Karl-Heinz; Jurado, Beatriz; Amouroux, Charlotte

    2014-06-01

    The Joint Evaluated Fission and Fusion (JEFF) Project is a collaborative effort among the member countries of the OECD Nuclear Energy Agency (NEA) Data Bank to develop a reference nuclear data library. The JEFF library contains sets of evaluated nuclear data, mainly for fission and fusion applications; it contains a number of different data types, including neutron and proton interaction data, radioactive decay data, fission yield data and thermal scattering law data. The General fission (GEF) model is based on novel theoretical concepts and ideas developed to model low energy nuclear fission. The GEF code calculates fission-fragment yields and associated quantities (e.g. prompt neutron and gamma) for a large range of nuclei and excitation energy. This opens up the possibility of a qualitative step forward to improve further the JEFF fission yields sub-library. This report describes the GEF model which explains the complex appearance of fission observables by universal principles of theoretical models and considerations on the basis of fundamental laws of physics and mathematics. The approach reveals a high degree of regularity and provides a considerable insight into the physics of the fission process. Fission observables can be calculated with a precision that comply with the needs for applications in nuclear technology. The relevance of the approach for examining the consistency of experimental results and for evaluating nuclear data is demonstrated. (authors)

  12. JENDL-3 fission product nuclear data library

    International Nuclear Information System (INIS)

    Kawai, Masayoshi; Iijima, Shungo; Nakagawa, Tsuneo; Nakajima, Yutaka; Sugi, Teruo; Watanabe, Takashi; Matsunobu, Hiroyuki; Sasaki, Makoto; Zukeran, Atsushi.

    1992-01-01

    Neutron nuclear data in the energy range between 10 -5 eV and 20 MeV have been evaluated for 172 nuclides from 75 As to 159 Tb in the fission product mass region to provide data for the JENDL-3 fission product nuclear data library. Evaluation was made on the basis of recent experimental data reported up to 1988 and the nuclear model calculations. Resonance parameters have been evaluated on the basis of measured data set and a REPSTOR system developed in JAERI. The spherical optical model and statistical theory were applied to calculation of the total, capture, elastic and inelastic scattering cross sections, and the multistep evaporation model and pre-equilibrium theory were used for threshold reaction cross section calculations. For the even-even nuclides around fission yield peaks, direct inelastic scattering cross sections were calculated with the distorted wave Born approximation. Nuclear model parameters, such as optical model parameters, level density parameters, γ-ray strength functions and Kalbach constant of the pre-equilibrium model were determined so as to give a good agreement between the calculated and measured cross sections. The parameter systematics were obtained as a function of nuclear mass or atomic number. For thermal capture cross sections, a simple relation between measured and calculated cross sections was found as a function of level spacing. The evaluated results were compiled in the ENDF-5 format. (author) 59 refs

  13. Hybrid fission-fusion nuclear reactors

    International Nuclear Information System (INIS)

    Zucchetti, Massimo

    2011-01-01

    A fusion-fission hybrid could contribute to all components of nuclear power - fuel supply, electricity production, and waste management. The idea of the fusion-fission hybrid is many decades old. Several ideas, both new and revisited, have been investigated by hybrid proponents. These ideas appear to have attractive features, but they require various levels of advances in plasma science and fusion and nuclear technology. As a first step towards the development of hybrid reactors, fusion neutron sources can be considered as an option. Compact high-field tokamaks can be a candidate for being the neutron source in a fission-fusion hybrid, essentially due to their design characteristics, such as compact dimensions, high magnetic field, flexibility of operation. This study presents the development of a tokamak neutron source for a material testing facility using an Ignitor-based concept. The computed values show the potential of this neutron-rich device for fusion materials testing. Some full-power months of operation are sufficient to obtain relevant radiation damage values in terms of dpa. (Author)

  14. Simulating an Exploding Fission-Bomb Core

    Science.gov (United States)

    Reed, Cameron

    2016-03-01

    A time-dependent desktop-computer simulation of the core of an exploding fission bomb (nuclear weapon) has been developed. The simulation models a core comprising a mixture of two isotopes: a fissile one (such as U-235) and an inert one (such as U-238) that captures neutrons and removes them from circulation. The user sets the enrichment percentage and scattering and fission cross-sections of the fissile isotope, the capture cross-section of the inert isotope, the number of neutrons liberated per fission, the number of ``initiator'' neutrons, the radius of the core, and the neutron-reflection efficiency of a surrounding tamper. The simulation, which is predicated on ordinary kinematics, follows the three-dimensional motions and fates of neutrons as they travel through the core. Limitations of time and computer memory render it impossible to model a real-life core, but results of numerous runs clearly demonstrate the existence of a critical mass for a given set of parameters and the dramatic effects of enrichment and tamper efficiency on the growth (or decay) of the neutron population. The logic of the simulation will be described and results of typical runs will be presented and discussed.

  15. Undergraduate Measurements For Fission Reactor Applications

    Science.gov (United States)

    Hicks, S. F.; Kersting, L. J.; Lueck, C. J.; McDonough, P.; Crider, B. P.; McEllistrem, M. T.; Peters, E. E.; Vanhoy, J. R.

    2011-06-01

    Undergraduate students at the University of Dallas (UD) have investigated elastic and inelastic neutron scattering cross sections on structural materials important for criticality considerations in nuclear fission processes. Neutrons scattered off of 23Na and NatFe were detected using neutron time-of-flight techniques at the University of Kentucky Low-Energy Nuclear Accelerator Facility. These measurements are part of an effort to increase the efficiency of power generation from existing fission reactors in the US and in the design of new fission systems. Students have learned the basics of how to operate the Model CN Van de Graaff generator at the laboratory, setup detectors and electronics, use data acquisition systems, and they are currently analyzing the angular dependence of the scattered neutrons for incident neutron energies of 3.57 and 3.80 MeV. Most students participating in the project will use the research experience as the material for their undergraduate research thesis required for all Bachelor of Science students at the University of Dallas. The first student projects on this topic were completed during the summer of 2010; an overview of student participation in this investigation and their preliminary results will be presented.

  16. Capture and fission with DANCE and NEUANCE

    Energy Technology Data Exchange (ETDEWEB)

    Jandel, M.; Baramsai, B.; Bond, E.; Rusev, G.; Walker, C.; Bredeweg, T.A.; Chadwick, M.B.; Couture, A.; Fowler, M.M.; Hayes, A.; Kawano, T.; Mosby, S.; Stetcu, I.; Taddeucci, T.N.; Talou, P.; Ullmann, J.L.; Vieira, D.J.; Wilhelmy, J.B. [Los Alamos National Laboratory, Los Alamos, New Mexico (United States)

    2015-12-15

    A summary of the current and future experimental program at DANCE is presented. Measurements of neutron capture cross sections are planned for many actinide isotopes with the goal to reduce the present uncertainties in nuclear data libraries. Detailed studies of capture gamma rays in the neutron resonance region will be performed in order to derive correlated data on the de-excitation of the compound nucleus. New approaches on how to remove the DANCE detector response from experimental data and retain the correlations between the cascade gamma rays are presented. Studies on {sup 235}U are focused on quantifying the population of short-lived isomeric states in {sup 236}U after neutron capture. For this purpose, a new neutron detector array NEUANCE is under construction. It will be installed in the central cavity of the DANCE array and enable the highly efficient tagging of fission and capture events. In addition, developments of fission fragment detectors are also underway to expand DANCE capabilities to measurements of fully correlated data on fission observables. (orig.)

  17. Capture and fission with DANCE and NEUANCE

    Science.gov (United States)

    Jandel, M.; Baramsai, B.; Bond, E.; Rusev, G.; Walker, C.; Bredeweg, T. A.; Chadwick, M. B.; Couture, A.; Fowler, M. M.; Hayes, A.; Kawano, T.; Mosby, S.; Stetcu, I.; Taddeucci, T. N.; Talou, P.; Ullmann, J. L.; Vieira, D. J.; Wilhelmy, J. B.

    2015-12-01

    A summary of the current and future experimental program at DANCE is presented. Measurements of neutron capture cross sections are planned for many actinide isotopes with the goal to reduce the present uncertainties in nuclear data libraries. Detailed studies of capture gamma rays in the neutron resonance region will be performed in order to derive correlated data on the de-excitation of the compound nucleus. New approaches on how to remove the DANCE detector response from experimental data and retain the correlations between the cascade gamma rays are presented. Studies on 235U are focused on quantifying the population of short-lived isomeric states in 236U after neutron capture. For this purpose, a new neutron detector array NEUANCE is under construction. It will be installed in the central cavity of the DANCE array and enable the highly efficient tagging of fission and capture events. In addition, developments of fission fragment detectors are also underway to expand DANCE capabilities to measurements of fully correlated data on fission observables.

  18. A theoretical study on the geometry and spectroscopic properties of ground-state and local minima isomers of (CuS)n=2-6 clusters

    Science.gov (United States)

    Luque-Ceballos, Jonathan C.; Posada-Borbón, Alvaro; Herrera-Urbina, Ronaldo; Aceves, R.; Juárez-Sánchez, J. Octavio; Posada-Amarillas, Alvaro

    2018-03-01

    Spectroscopic properties of gas-phase copper sulfide clusters (CuS)n (n = 2-6) are calculated using Density Functional Theory (DFT) and time-dependent (TD) DFT approaches. The energy landscape of the potential energy surface is explored through a basin-hopping DFT methodology. Ground-state and low-lying isomer structures are obtained. The global search was performed at the B3PW91/SDD level of theory. Normal modes are calculated to validate the existence of optimal cluster structures. Energetic properties are obtained for the ground-state and isomer clusters and their relative energies are evaluated for probing isomerization. This is a few tenths of an eV, except for (CuS)2 cluster, which presents energy differences of ∼1 eV. Notable differences in the infrared spectra exist between the ground-state and first isomer structures, even for the (CuS)5 cluster, which has in both configurations a core copper pyramid. TDDFT provides the simulated absorption spectrum, presenting a theoretical description of optical absorption bands in terms of electronic excitations in the UV and visible regions. Results exhibit a significant dependence of the calculated UV/vis spectra on clusters size and shape regarding the ground state structures. Optical absorption is strong in the UV region, and weak or forbidden in the visible region of the spectrum.

  19. Study of the stability of the ground states and K-isomeric states of 250Fm and 254102 against spontaneous fission

    International Nuclear Information System (INIS)

    Lazarev, Yu.A.; Lobanov, Yu.V.; Sagajdak, R.N.; Utenkov, V.K.; Kharitonov, Yu.P.; Shirokovskij, I.V.; Tret'yakova, S.P.; Oganessyan, Yu.Ts.

    1988-01-01

    By employing the 249 Cf( 4 He, 3n) and 208 Pb( 48 Ca,2n) reactions, experiments to study the stability against spontaneous fission of the nuclides 250 Fm and 254 102 as well as of the two-quasi-particle (2 q-p) K isomers 250 Fm (T 1/2 =1,8±0,1 s) and 254 102 (T 1/2 =0,28±0,04 s) have been performed. The groundstate spontaneous fission of the two nuclides has been discovered and the corresponding branching ratios b sf and partial half-lives T sf , respectively, have been determined to be: (6,9±1,0)x10 -5 , 0,83±0,15 yr for 250 Fm; (1,7±0,5)x10 -3 , (3,2±0,9)x10 4 s for 254 102. As a by-product of these studies, new data about cross sections of the 206,208 Pb( 48 Ca,xn) reactions have been obtained. Experiments designed to search for the spontaneous fission of the 2 q-p K-isometric states in 250 Fm and 254 102 have not revealed the effect in question. The lower limits of the ratios of the partial spontaneous fission half-lives for the 2 q-p K-isomeric states to those for the respective ground states, T * sf /T sf , have been established to be≥10 -1 for 250m Fm/ 250 Fm and ≥5x10 -3 for 254m 102/ 254 102. This means that the stability of the 2 q-p K-isomeric states in 250 Fm and 254 102 against spontaneous fission is practically not inferior to that of the ground states of these nuclei. In accord with the experimental findings, the theoretical estimates of T * sf /T sf made in the present paper show that, due to the influence of the specialization and blocking effects on the potential energy and the effective mass associated with fission, spontaneous fission from 2 q-p K-isomeric states cannot be facilitated but, on the contrary, should be essentially hindered compared with ground-state spontaneous fission

  20. Characterization of a facility for the measurement of fission fragment transport effects: experimental determination of the fission rates for fissile and fissionable isotopes

    International Nuclear Information System (INIS)

    Benetti, P.; Raselli, G.L.; Tigliole, A. Borio di; Cagnazzo, M.; Cesana, A.; Mongelli, S.; Terrani, M.

    2002-01-01

    The transfer facility of the LENA laboratory allows the direct neutron irradiation of fissionable material in the D channel of the TRIGA reactor. A test measurement carried out with a ionization chamber and a 239 Pu sample shows the possibility to use this tool for the study of the transport effects of the fission fragment emerging from thin layers of fissile materials. (author)

  1. Preliminary fission product energy release measurements for thermal neutron fission of 235U

    International Nuclear Information System (INIS)

    Dickens, J.K.; Love, T.A.; McConnell, J.W.; Emery, J.F.; Peelle, R.W.

    1976-03-01

    An experimental system to measure time-dependent spectra of β and γ rays from fission-product production by thermal neutron fission of 235 U is described, and for each component (β and γ) the system has been tested with a pilot data-accumulation run. Data reduction techniques are described and test results given. Gamma-ray spectra are compared with calculations using ENDF/B-IV data files. Both β- and γ-ray spectra were integrated to give total yields and total energy-release results for times after fission between 3 and 14400 sec. These preliminary integral data are compared with previous measurements and with integral calculations using ENDF/B-IV data files

  2. Prediction of fission barrier height for induced fission reactions with 16O at several energies

    Directory of Open Access Journals (Sweden)

    S Soheyli

    2009-09-01

    Full Text Available We have calculated the fission barrier height for 16O+208Pb, 16O+209Bi, 16O+232Th, 16O+238U and 16O+248Cm systems in energy range between 90 MeV to 215 MeV. This method is based on the experimental data for angular anisotropies of fission fragments. In present work, we have used the transition state model (STM for two different cases: the first case is without neutron emission correction and the second case is with neutron emission correction. In this paper, we have predicted the fission barrier for the two super heavy nuclei that were not reported previously with experimental methods.

  3. Investigation of the fission yields of the fast neutron-induced fission of 233U

    International Nuclear Information System (INIS)

    Galy, J.

    1999-09-01

    As a stars, a survey of the different methods of investigations of the fission product yields and the experimental data status have been studied, showing advantages and shortcomings for the different approaches. An overview of the existing models for the fission product distributions has been as well intended. The main part of this thesis was the measurement of the independent yields of the fast neutron-induced fission of 233 U, never investigated before this work. The experiment has been carried out using the mass separator OSIRIS (Isotope Separator On-Line). Its integrated ion-source and its specific properties required an analysis of the delay-parameter and ionisation efficiency for each chemical species. On the other hand, this technique allows measurement of independent yields and cumulative yields for elements from Cu to Ba, covering most of the fission yield distribution. Thus, we measured about 180 independent yields from Zn (Z=30) to Sr (Z=38) in the mass range A=74-99 and from Pd (Z=46) to Ba (Z=56) in the mass range A=113-147, including many isomeric states. An additional experiment using direct γ-spectroscopy of aggregates of fission products was used to determine more than 50 cumulative yields of element with half-life from 15 min to a several days. All experimental data have been compared to estimates from a semi-empirical model, to calculated values and to evaluated values from the European library JEF 2.2. Furthermore, a study of both thermal and fast neutron-induced fission of 233 U measured at Studsvik, the comparison of the OSIRIS and LOHENGRIN facilities and the trends in new data for the Reactors Physics have been discussed. (author)

  4. Frequent gene fissions associated with human pathogenic bacteria.

    Science.gov (United States)

    Karamichali, Ioanna; Koumandou, V Lila; Karagouni, Amalia D; Kossida, Sophia

    2014-01-01

    Gene fusion and fission events are important for evolutionary studies and for predicting protein-protein interactions. Previous studies have shown that fusion events always predominate over fission events and, in their majority, they represent singular events throughout evolution. In this project, the role of fusion and fission events in the genome evolution of 104 human bacterial pathogens was studied. 141 protein pairs were identified to be involved in gene fusion or fission events. Surprisingly, we find that, in the species analyzed, gene fissions prevail over fusions. Moreover, while most events appear to have occurred only once in evolution, 23% of the gene fusion and fission events identified are deduced to have occurred independently multiple times. Comparison of the analyzed bacteria with non-pathogenic close relatives indicates that this impressive result is associated with the recent evolutionary history of the human bacterial pathogens, and thus is probably caused by their pathogenic lifestyle. Copyright © 2014 Elsevier Inc. All rights reserved.

  5. Nuclear data for neutron emission in the fission process

    International Nuclear Information System (INIS)

    Ganesan, S.

    1991-11-01

    This document contains the proceedings of the IAEA Consultants' Meeting on Nuclear Data for Neutron Emission in the Fission Process, Vienna, 22 - 24 October 1990. Included are the conclusions and recommendations reached at the meeting and the papers presented by the meeting participants. These papers provide a review of the status of experimental and theoretical data on neutron emission in spontaneous and neutron induced fission with reference to the data needs for reactor applications oriented towards actinide burner studies. The specific topics covered are the following: experimental measurements and theoretical predictions and evaluations of fission neutron energy spectra, average prompt fission neutron multiplicity, correlation in neutron emission from complementary fragments, neutron emission during acceleration of fission fragments, statistical properties of neutron rich nuclei by study of emission spectra of neutrons from the excited fission fragments, integral qualification of nu-bar for the major fissile isotopes, nu-bar total of 239 Pu and 235 U, and related problems. Refs figs and tabs

  6. Fission Reaction Event Yield Algorithm FREYA 2.0.2

    Science.gov (United States)

    Verbeke, J. M.; Randrup, J.; Vogt, R.

    2018-01-01

    FREYA (Fission Reaction Event Yield Algorithm) is a fission event generator which models complete fission events. As such, it automatically includes fluctuations as well as correlations between observables, resulting from conservation of energy and momentum. The purpose of this paper is to present the main differences between FREYA versions 1.0 and 2.0.2 : additional fissionable isotopes, angular momentum conservation, Giant Dipole Resonance form factor for the statistical emission of photons, improved treatment of fission photon emission using RIPL database, and dependence on the incident neutron direction. FREYA 2.0.2 has been integrated into the LLNL Fission Library 2.0.2, which has itself been integrated into MCNP6.2, TRIPOLI-4.10, and can be called from Geant4.10.

  7. The wastes of nuclear fission; Les dechets de la fission nucleaire

    Energy Technology Data Exchange (ETDEWEB)

    Doubre, H. [Paris-11 Univ., Centre de Spectrometrie Nucleaire et de Spectrometrie de Masse, IN2P3/CNRS, 91 - Orsay (France)

    2005-07-01

    In this paper the author presents the problems of the radioactive wastes generated by the nuclear fission. The first part devoted to the fission phenomenon explains the incident neutron energy and the target nuclei role. The second part devoted to the nuclear wastes sources presents the production of wastes upstream of the reactors, in the reactors and why these wastes are dangerous. The third part discusses the radioactive wastes management in France (classification, laws). The last part details the associated research programs: the radionuclides separation, the disposal, the underground storage, the transmutation and the thorium cycle. (A.L.B.)

  8. Theoretical studies of possible toroidal high-spin isomers in the light-mass region

    Directory of Open Access Journals (Sweden)

    Staszczak Andrzej

    2016-01-01

    Full Text Available We review our theoretical knowledge of possible toroidal high-spin isomers in the light mass region in 28≤A≤52 obtained previously in cranked Skyrme-Hartree-Fock calculations. We report additional toroidal high-spin isomers in 56Ni with I=114ħ and 140ħ, which follow the same (multi-particle–(multi-hole systematics as other toroidal high-spin isomers. We examine the production of these exotic nuclei by fusion of various projectiles on 20Ne or 28Si as an active target in time-projection-chamber (TPC experiments.

  9. Solvation effect on isomer stability and electronic structures of protonated serotonin

    Science.gov (United States)

    Omidyan, Reza; Amanollahi, Zohreh; Azimi, Gholamhassan

    2017-07-01

    Microsolvation effect on geometry and transition energies of protonated serotonin has been investigated by MP2 and CC2 quantum chemical methods. Also, conductor-like screening model, implemented recently in the MP2 and ADC(2) methods, was examined to address the bulk water environment's effect on the isomer stability and electronic transition energies of protonated serotonin. It has been predicted that the dipole moment of gas phase isomers plays the main role on the isomer stabilization in water solution and electronic transition shifts. Also, both red- and blue-shift effects have been predicted to take place on electronic transition energies, upon hydration.

  10. Identification of a new isomer from a reversible isomerization of ceftriaxone in aqueous solution.

    Science.gov (United States)

    Tian, Ye; Lu, Li; Chang, Yan; Zhang, Dou-sheng; Li, Jin; Feng, Yan-Chun; Hu, Chang-Qin

    2015-01-01

    A reversible isomerization of ceftriaxone in aqueous solution was observed, and the structure of the isomer was determined by mass spectrometry and various 1D and 2D NMR techniques. The mechanism of isomerization was also discussed. Finally, molecular docking simulations were performed and the antimicrobial activities of the isomers were measured. This showed that the biological activity of ceftriaxone was stronger than that of its isomer. The results reported in this article may be important to quality control requirements and to the stability of ceftriaxone products. Copyright © 2014 Elsevier B.V. All rights reserved.

  11. Isomer-specific regulation of metabolism and PPARgamma signaling by CLA in human preadipocytes

    DEFF Research Database (Denmark)

    Brown, J Mark; Boysen, Maria Sandberg; Jensen, Søren Skov

    2003-01-01

    Trans-10,cis-12 conjugated linoleic acid (CLA) has previously been shown to be the CLA isomer responsible for CLA-induced reductions in body fat in animal models, and we have shown that this isomer, but not the cis-9,trans-11 CLA isomer, specifically decreased triglyceride (TG) accumulation...... transporter 4 gene expression. Furthermore, trans-10,cis-12 CLA reduced oleic acid uptake and oxidation when compared with all other treatments. In parallel to CLA's effects on metabolism, trans-10,cis-12 CLA decreased, whereas cis-9,trans-11 CLA increased, the expression of peroxisome proliferator...

  12. Impact of fuel chemistry on fission product behaviour

    International Nuclear Information System (INIS)

    Poortmans, C.; Van Uffelen, P.; Van den Berghe, S.

    1999-01-01

    The report contains a series of papers presented at SCK-CEN's workshop on the impact of fuel chemistry on fission product behaviour. Contributing authors discuss different processes affecting the behaviour of fission products in different types of spent nuclear fuel. In addition, a number of papers discusses the behaviour of actinides and fission products released from spent fuel and vitrified high-level waste in geological disposal conditions

  13. Separation of fission strontium from nuclear fuels by ammonium molybdatophosphate

    International Nuclear Information System (INIS)

    Hermann, A.

    1984-01-01

    The separation of fission strontium from solutions of prolonged cooled nuclear fuel has been performed using ammoniummolybdatophosphate (AMP) columns. The sorption mechanism of bivalent ions of AMP has been investigated by column and batch experiments. A pure ion exchange of Sr 2+ for two H + or NH 4 + ions has been established. Conditions for the sepasorption and elution of fission strontium and other fission products on AMP columns are described. (author)

  14. Neutron flux profile monitor for use in a fission reactor

    Science.gov (United States)

    Kopp, Manfred K.; Valentine, Kenneth H.

    1983-01-01

    A neutron flux monitor is provided which consists of a plurality of fission counters arranged as spaced-apart point detectors along a delay line. As a fission event occurs in any one of the counters, two delayed current pulses are generated at the output of the delay line. The time separation of the pulses identifies the counter in which the particular fission event occured. Neutron flux profiles of reactor cores can be more accurately measured as a result.

  15. Magnetic Materials Suitable for Fission Power Conversion in Space Missions

    Science.gov (United States)

    Bowman, Cheryl L.

    2012-01-01

    Terrestrial fission reactors use combinations of shielding and distance to protect power conversion components from elevated temperature and radiation. Space mission systems are necessarily compact and must minimize shielding and distance to enhance system level efficiencies. Technology development efforts to support fission power generation scenarios for future space missions include studying the radiation tolerance of component materials. The fundamental principles of material magnetism are reviewed and used to interpret existing material radiation effects data for expected fission power conversion components for target space missions. Suitable materials for the Fission Power System (FPS) Project are available and guidelines are presented for bounding the elevated temperature/radiation tolerance envelope for candidate magnetic materials.

  16. Generalized Energy-Dependent Q Values for Fission

    Energy Technology Data Exchange (ETDEWEB)

    Vogt, R

    2010-03-31

    We extend Madland's parameterization of the energy release in fission to obtain the dependence of the fission Q value for major and minor actinides on the incident neutron energies in the range 0 {le} E{sub n} {le} 20 MeV. Our parameterization is based on the actinide evaluations recommended for the ENDF/B-VII.1 release. This paper describes the calculation of energydependent fission Q values based on the calculation of the prompt energy release in fission by Madland. This calculation was adopted for use in the LLNL ENDL database and then generalized to obtain the prompt fission energy release for all actinides. Here the calculation is further generalized to the total energy release in fission. There are several stages in a fission event, depending on the time scale. Neutrons and gammas may be emitted at any time during the fission event.While our discussion here is focussed on compound nucleus creation by an incident neutron, similar parameterizations could be obtained for incident gammas or spontaneous fission.

  17. Fusion – fission dynamics: fragment mass distribution studies

    Directory of Open Access Journals (Sweden)

    Bhattacharya S.

    2015-01-01

    Full Text Available Using the major accelerator facilities available in India, detailed experimental studies have been made to understand the mechanism of quasi-fission and role of nuclear shell effect in heavy nuclei. Fission fragment mass distribution has been used as the probe to explore the role of entrance channel effects on fusion-fission and quasifission dynamics. Fission fragment mass distribution has also been demonstrated to be useful to identify the phenomenon of ‘washing out’ of nuclear shell effect with excitation energy.

  18. Simulation of Fission Product Liftoff Behavior During Depressurization Transients

    International Nuclear Information System (INIS)

    Tak, Nam-il; Yoon, Churl; Lee, Sung Nam

    2016-01-01

    As one of crucial technologies for the NHDD project, the development of the GAMMA-FP code is on-going. The GAMMA-FP code is targeted for fission product transport analysis under accident conditions. A well-known experiment named COMEDIE considered two important phenomena, i.e., fission product plateout and liftoff, for fission product transport within the primary circuit of a prismatic high temperature gas cooled reactor. The accumulated fission products on the structural material via the plateout can be liftoff during a blowdown phase after a pipe break accident. Since the fission product liftoff can increase a radioactivity risk, it is important to predict the amount of fission product liftoff during depressurization accidents. In this work, a model for fission product liftoff is implemented into the GAMMA-FP code and the GAMMA-FP code with the implemented model is validated using the COMEDIE blowdown test data. The results of GAMMA-FP show that the GAMMA-FP code can reliably simulate a pressure transient during blowdown phase after a pipe break accident. In addition, a reasonable amount of fission product liftoff was predicted by the GAMMA-FP code. The maximum difference between the measured and predicted liftoff fraction was less than a factor of 10. More in-depth study is required to increase the accuracy of prediction for a fission product liftoff

  19. Possible origin of transition from symmetric to asymmetric fission

    Directory of Open Access Journals (Sweden)

    H. Paşca

    2016-09-01

    Full Text Available The charged distributions of fragments produced in the electromagnetic-induced fission of the even–even isotopes of Rn, Ra, Th, and U are described within an improved scission-point model and compared with the available experimental data. The three-equal-peaked charge distributions are predicted for several fissioning nuclei with neutron number N=136. The possible explanation of the transition from a symmetric fission mode to an asymmetric one around N∼136 is presented. The excitation energy dependencies of the asymmetric and symmetric fission modes are anticipated.

  20. Fission cross sections in the intermediate energy region

    International Nuclear Information System (INIS)

    Lisowski, P.W.; Gavron, A.; Parker, W.E.; Ullmann, J.L.; Balestrini, S.J.; Carlson, A.D.; Wasson, O.A.; Hill, N.W.

    1991-01-01

    Until recently there has been very little cross section data for neutron-induced fission in the intermediate energy region, primarily because no suitable neutron source has existed. At Los Alamos, the WNR target-4 facility provides a high-intensity source of neutrons nearly ideal for fission measurements extending from a fraction of a MeV to several hundred MeV. This paper summarizes the status of fission cross section data in the intermediate energy range (En > 30 MeV) and presents our fission cross section data for 235 U and 238 U compared to intranuclear cascade and statistical model predictions