WorldWideScience

Sample records for few-electron highly charged

  1. Charge-transfer collisions involving few-electron systems

    International Nuclear Information System (INIS)

    Kirchner, T.

    2016-01-01

    Ion-atom collision systems that involve more than one electron constitute nonseparable few-body problems, whose full solution is difficult to say the least. At impact energies well below 1 keV/amu an expansion of the stationary scattering wave function in terms of a limited number of products of nuclear and molecular state wave functions (amended to satisfy scattering boundary conditions) is feasible and usually sufficient to obtain accurate charge-transfer cross sections provided the electronic wave functions include configuration interaction. At energies above 1 keV/amu this approach becomes inefficient and close-coupling methods within the semi classical approximation are better suited to treat the problem. For bare-ion collisions from helium target atoms explicit solutions of the two-electron time-dependent Schrödinger equation can be achieved, but are computationally costly and cannot be extended to problems which involve more than two electrons.

  2. Electron scattering and few nucleon systems

    International Nuclear Information System (INIS)

    Frois, B.

    1983-08-01

    Recent result obtained by electron scattering in the few-nucleon systems (A 3 He charge and magnetic form factors are discussed. New theoretical results indicate that three body forces improve considerably the saturation properties of 3 He, 4 He and nuclear matter, but are not able to reconcile experiment and theory for the charge form factors of 3 He and 4 He. Calculations of meson exchange effects with different theoretical approaches bring the theory into reasonable agreement with the experimental charge and magnetic form factor fo 3 He. Recent results of the measurements of the two and three body break-up of 3 He are discussed

  3. High efficiency charge recuperation for electron beams of MeV energies

    International Nuclear Information System (INIS)

    MacLachlan, J.A.

    1996-05-01

    Electron cooling of ion beams with energies of some GeV per nucleon requires high-quality electron beams of MeV energies and currents as high as several amperes. The enormous beam power dictates that the beam current be returned to the high voltage terminal which provides the accelerating potential. The beam is returned to a carefully designed collector within the terminal and biased a few kV positive with respect to it. Thus the load on the HV supply is only the accelerating potential times the sum of the beam current loss and the current used to maintain a graded potential on the accelerating structure. If one employs an electrostatic HV supply like a Van de Graaff with maximum charging current of a few hundred microA, the permissible fractional loss is ∼ 10 -4 . During the 15 years or so the concept of medium energy electron cooling has been evolving, the need to demonstrate the practicability of such high efficiency beam recovery has been recognized. This paper will review some experimental tests and further experiments which have been proposed. The design and status are presented for a new re-circulation experiment at 2 MV being carried out by Fermilab at National Electrostatics Corp

  4. Atomic structure of highly-charged ions. Final report

    International Nuclear Information System (INIS)

    Livingston, A. Eugene

    2002-01-01

    Atomic properties of multiply charged ions have been investigated using excitation of energetic heavy ion beams. Spectroscopy of excited atomic transitions has been applied from the visible to the extreme ultraviolet wavelength regions to provide accurate atomic structure and transition rate data in selected highly ionized atoms. High-resolution position-sensitive photon detection has been introduced for measurements in the ultraviolet region. The detailed structures of Rydberg states in highly charged beryllium-like ions have been measured as a test of long-range electron-ion interactions. The measurements are supported by multiconfiguration Dirac-Fock calculations and by many-body perturbation theory. The high-angular-momentum Rydberg transitions may be used to establish reference wavelengths and improve the accuracy of ionization energies in highly charged systems. Precision wavelength measurements in highly charged few-electron ions have been performed to test the most accurate relativistic atomic structure calculations for prominent low-lying excited states. Lifetime measurements for allowed and forbidden transitions in highly charged few-electron ions have been made to test theoretical transition matrix elements for simple atomic systems. Precision lifetime measurements in laser-excited alkali atoms have been initiated to establish the accuracy of relativistic atomic many-body theory in many-electron systems

  5. Measurement of few-electron uranium ions on a high-energy electron beam ion trap

    International Nuclear Information System (INIS)

    Beiersdorfer, P.

    1994-01-01

    The high-energy electron beam ion trap, dubbed Super-EBIT, was used to produce, trap, and excite uranium ions as highly charged as fully stripped U 92+ . The production of such highly charged ions was indicated by the x-ray emission observed with high-purity Ge detectors. Moreover, high-resolution Bragg crystal spectromters were used to analyze the x-ray emission, including a detailed measurement of both the 2s 1/2 -2p 3/2 electric dipole and 2p 1/2 -2p 3/2 magnetic dipole transitions. Unlike in ion accelerators, where the uranium ions move at relativistic speeds, the ions in this trap are stationary. Thus very precise measurements of the transition energies could be made, and the QED contribution to the transition energies could be measured within less than 1 %. Details of the production of these highly charged ions and their measurement is given

  6. Electron capture by highly charged ions from surfaces and gases

    International Nuclear Information System (INIS)

    Allen, F.

    2008-01-01

    In this study highly charged ions produced in Electron Beam Ion Traps are used to investigate electron capture from surfaces and gases. The experiments with gas targets focus on spectroscopic measurements of the K-shell x-rays emitted at the end of radiative cascades following electron capture into Rydberg states of Ar 17+ and Ar 18+ ions as a function of collision energy. The ions are extracted from an Electron Beam Ion Trap at an energy of 2 keVu -1 , charge-selected and then decelerated down to 5 eVu -1 for interaction with an argon gas target. For decreasing collision energies a shift to electron capture into low orbital angular momentum capture states is observed. Comparative measurements of the K-shell x-ray emission following electron capture by Ar 17+ and Ar 18+ ions from background gas in the trap are made and a discrepancy in the results compared with those from the extraction experiments is found. Possible explanations are discussed. For the investigation of electron capture from surfaces, highly charged ions are extracted from an Electron Beam Ion Trap at energies of 2 to 3 keVu -1 , charge-selected and directed onto targets comprising arrays of nanoscale apertures in silicon nitride membranes. The highly charged ions implemented are Ar 16+ and Xe 44+ and the aperture targets are formed by focused ion beam drilling in combination with ion beam assisted thin film deposition, achieving hole diameters of 50 to 300 nm and aspect ratios of 1:5 to 3:2. After transport through the nanoscale apertures the ions pass through an electrostatic charge state analyzer and are detected. The percentage of electron capture from the aperture walls is found to be much lower than model predictions and the results are discussed in terms of a capillary guiding mechanism. (orig.)

  7. Few electron quantum dot coupling to donor implanted electron spins

    Science.gov (United States)

    Rudolph, Martin; Harvey-Collard, Patrick; Neilson, Erik; Gamble, John; Muller, Richard; Jacobson, Toby; Ten-Eyck, Greg; Wendt, Joel; Pluym, Tammy; Lilly, Michael; Carroll, Malcolm

    2015-03-01

    Donor-based Si qubits are receiving increased interest because of recent demonstrations of high fidelity electron or nuclear spin qubits and their coupling. Quantum dot (QD) mediated interactions between donors are of interest for future coupling of two donors. We present experiment and modeling of a polysilicon/Si MOS QD, charge-sensed by a neighboring many electron QD, capable of coupling to one or two donor implanted electron spins (D) while tuned to the few electron regime. The unique design employs two neighboring gated wire FETs and self-aligned implants, which supports many configurations of implanted donors. We can access the (0,1) ⇔(1,0) transition between the D and QD, as well as the resonance condition between the few electron QD and two donors ((0,N,1) ⇔(0,N +1,0) ⇔(1,N,0)). We characterize capacitances and tunnel rate behavior combined with semi-classical and full configuration interaction simulations to study the energy landscape and kinetics of D-QD transitions. This work was performed, in part, at the Center for Integrated Nanotechnologies, a U.S. DOE, Office of Basic Energy Sciences user facility. The work was supported by the Sandia National Laboratories Directed Research and Development Program. Sandia National Laboratories is a multi-program laboratory operated by Sandia Corporation, a Lockheed-Martin Company, for the U. S. Department of Energy under Contract No. DE-AC04-94AL85000.

  8. HITRAP: A Facility for Experiments with Trapped Highly Charged Ions

    International Nuclear Information System (INIS)

    Quint, W.; Dilling, J.; Djekic, S.; Haeffner, H.; Hermanspahn, N.; Kluge, H.-J.; Marx, G.; Moore, R.; Rodriguez, D.; Schoenfelder, J.; Sikler, G.; Valenzuela, T.; Verdu, J.; Weber, C.; Werth, G.

    2001-01-01

    HITRAP is a planned ion trap facility for capturing and cooling of highly charged ions produced at GSI in the heavy-ion complex of the UNILAC-SIS accelerators and the ESR storage ring. In this facility heavy highly charged ions up to uranium will be available as bare nuclei, hydrogen-like ions or few-electron systems at low temperatures. The trap for receiving and studying these ions is designed for operation at extremely high vacuum by cooling to cryogenic temperatures. The stored highly charged ions can be investigated in the trap itself or can be extracted from the trap at energies up to about 10 keV/q. The proposed physics experiments are collision studies with highly charged ions at well-defined low energies (eV/u), high-accuracy measurements to determine the g-factor of the electron bound in a hydrogen-like heavy ion and the atomic binding energies of few-electron systems, laser spectroscopy of HFS transitions and X-ray spectroscopy

  9. Electron capture by highly charged low-velocity ions

    International Nuclear Information System (INIS)

    Cocke, C.L.; Dubois, R.; Justiniano, E.; Gray, T.J.; Can, C.

    1982-01-01

    This paper describes the use of a fast heavy ion beam to produce, by bombardment of gaseous targets, highly-charged low-velocity recoil ions, and the use of these secondary ions in turn as projectiles in studies of electron capture and ionization in low-energy collision systems. The interest in collisions involving low-energy highly-charged projectiles comes both from the somewhat simplifying aspects of the physics which attend the long-range capture and from applications to fusion plasmas, astrophysics and more speculative technology such as the production of X-ray lasers. The ions of interest in such applications should have both electronic excitation and center-of-mass energies in the keV range and cannot be produced by simply stripping fast heavy ion beams. Several novel types of ion source have been developed to produce low-energy highly-charged ions, of which the secondary ion recoil source discussed in this paper is one. (Auth.)

  10. Evolution of electronic structure in highly charge doped MoS2 compounds

    Science.gov (United States)

    Bin Subhan, Mohammed; Watson, Matthew; Liu, Zhongkai; Walters, Andrew; Hoesch, Moritz; Howard, Chris; Diamond I05 beamline Collaboration

    Transition-metal dichalcogenides (TMDCs) are a group of layered materials that exhibit a rich array of electronic ground states including semiconductivity, metallicity, superconductivity and charge density waves. In recent years, 2D TMDCs have attracted considerable attention due to their unique properties and potential applications in optoelectronics. It has been shown that the charge carrier density in few layer MoS2 can be tunably increased via electrostatic gating. At high levels of doping, MoS2 exhibits superconductivity with a dome-like dependence of Tc on doping analogous to that found in the cuprate superconductors. High doping can also be achieved via intercalation of alkali metals in bulk MoS2. The origin of this superconductivity is not yet fully understood with predictions ranging from exotic pairing mechanisms in bulk systems to Ising superconductivity in single layers. Despite these interesting properties, there has been limited research to date on the electronic structure of these doped compounds. Here we present our work on alkali metal intercalated MoS2 using the low temperature metal ammonia solution method. Using X-ray diffraction, Raman spectroscopy and ARPES measurements we will discuss the physical and electronic structure of these materials. EPSRC, Diamond Light Source.

  11. Electron capture by highly charged ions from surfaces and gases

    Energy Technology Data Exchange (ETDEWEB)

    Allen, F.

    2008-01-11

    In this study highly charged ions produced in Electron Beam Ion Traps are used to investigate electron capture from surfaces and gases. The experiments with gas targets focus on spectroscopic measurements of the K-shell x-rays emitted at the end of radiative cascades following electron capture into Rydberg states of Ar{sup 17+} and Ar{sup 18+} ions as a function of collision energy. The ions are extracted from an Electron Beam Ion Trap at an energy of 2 keVu{sup -1}, charge-selected and then decelerated down to 5 eVu{sup -1} for interaction with an argon gas target. For decreasing collision energies a shift to electron capture into low orbital angular momentum capture states is observed. Comparative measurements of the K-shell x-ray emission following electron capture by Ar{sup 17+} and Ar{sup 18+} ions from background gas in the trap are made and a discrepancy in the results compared with those from the extraction experiments is found. Possible explanations are discussed. For the investigation of electron capture from surfaces, highly charged ions are extracted from an Electron Beam Ion Trap at energies of 2 to 3 keVu{sup -1}, charge-selected and directed onto targets comprising arrays of nanoscale apertures in silicon nitride membranes. The highly charged ions implemented are Ar{sup 16+} and Xe{sup 44+} and the aperture targets are formed by focused ion beam drilling in combination with ion beam assisted thin film deposition, achieving hole diameters of 50 to 300 nm and aspect ratios of 1:5 to 3:2. After transport through the nanoscale apertures the ions pass through an electrostatic charge state analyzer and are detected. The percentage of electron capture from the aperture walls is found to be much lower than model predictions and the results are discussed in terms of a capillary guiding mechanism. (orig.)

  12. Relativistic, QED and nuclear effects in highly charged ions revealed by resonant electron-ion recombination in storage rings

    OpenAIRE

    Schippers, Stefan

    2008-01-01

    Dielectronic recombination (DR) of few-electron ions has evolved into a sensitive spectroscopic tool for highly charged ions. This is due to technological advances in electron-beam preparation and ion-beam cooling techniques at heavy-ion storage rings. Recent experiments prove unambiguously that DR collision spectroscopy has become sensitive to 2nd order QED and to nuclear effects. This review discusses the most recent developments in high-resolution spectroscopy of low-energy DR resonances, ...

  13. Electron impact ionization of highly charged lithiumlike ions

    International Nuclear Information System (INIS)

    Wong, K.L.

    1992-10-01

    Electron impact ionization cross sections can provide valuable information about the charge-state and power balance of highly charged ions in laboratory and astrophysical plasmas. In the present work, a novel technique based on x-ray measurements has been used to infer the ionization cross section of highly charged lithiumlike ions on the Livermore electron beam ion trap. In particular, a correspondence is established between an observed x ray and an ionization event. The measurements are made at one energy corresponding to approximately 2.3 times the threshold energy for ionization of lithiumlike ions. The technique is applied to the transition metals between Z=22 (titanium, Ti 19+ ) and Z=26 (iron, Fe 23+ ) and to Z=56 (barium, Ba 53+ ). The results for the transition metals, which have an estimated 17-33% uncertainty, are in good overall agreement with a relativistic distorted-wave calculation. However, less good agreement is found for barium, which has a larger uncertainty. Methods for properly accounting for the polarization in the x-ray intensities and for inferring the charge-state abundances from x-ray observations, which were developed for the ionization measurements, as well as an x-ray model that assists in the proper interpretation of the data are also presented

  14. Charge sensing of a few-donor double quantum dot in silicon

    Energy Technology Data Exchange (ETDEWEB)

    Watson, T. F., E-mail: tfwatson15@gmail.com; Weber, B.; Büch, H.; Fuechsle, M.; Simmons, M. Y., E-mail: michelle.simmons@unsw.edu.au [Australian Research Council Centre of Excellence for Quantum Computation and Communication Technology, University of New South Wales, Sydney, New South Wales 2052 (Australia)

    2015-12-07

    We demonstrate the charge sensing of a few-donor double quantum dot precision placed with atomic resolution scanning tunnelling microscope lithography. We show that a tunnel-coupled single electron transistor (SET) can be used to detect electron transitions on both dots as well as inter-dot transitions. We demonstrate that we can control the tunnel times of the second dot to the SET island by ∼4 orders of magnitude by detuning its energy with respect to the first dot.

  15. Theoretical progress in studying the characteristic x-ray emission from heavy few-electron ions

    International Nuclear Information System (INIS)

    Surzhykov, Andrey; Stohlker, Thomas; Fritzsche, Stephan; Kabachnik, Nikolai M

    2009-01-01

    Recent theoretical progress in the study of the x-ray characteristic emission from highly-charged, few-electron ions is reviewed. These investigations show that the bound-state radiative transitions in high-Z ions provide a unique tool for better understanding the interplay between the structural and dynamical properties of heavy ions. In order to illustrate such an interplay, detailed calculations are presented for the K α1 decay of the helium-like uranium ions U 90+ following radiative electron capture, Coulomb excitation and dielectronic recombination processes.

  16. Abnormal Multiple Charge Memory States in Exfoliated Few-Layer WSe2 Transistors.

    Science.gov (United States)

    Chen, Mikai; Wang, Yifan; Shepherd, Nathan; Huard, Chad; Zhou, Jiantao; Guo, L J; Lu, Wei; Liang, Xiaogan

    2017-01-24

    To construct reliable nanoelectronic devices based on emerging 2D layered semiconductors, we need to understand the charge-trapping processes in such devices. Additionally, the identified charge-trapping schemes in such layered materials could be further exploited to make multibit (or highly desirable analog-tunable) memory devices. Here, we present a study on the abnormal charge-trapping or memory characteristics of few-layer WSe 2 transistors. This work shows that multiple charge-trapping states with large extrema spacing, long retention time, and analog tunability can be excited in the transistors made from mechanically exfoliated few-layer WSe 2 flakes, whereas they cannot be generated in widely studied few-layer MoS 2 transistors. Such charge-trapping characteristics of WSe 2 transistors are attributed to the exfoliation-induced interlayer deformation on the cleaved surfaces of few-layer WSe 2 flakes, which can spontaneously form ambipolar charge-trapping sites. Our additional results from surface characterization, charge-retention characterization at different temperatures, and density functional theory computation strongly support this explanation. Furthermore, our research also demonstrates that the charge-trapping states excited in multiple transistors can be calibrated into consistent multibit data storage levels. This work advances the understanding of the charge memory mechanisms in layered semiconductors, and the observed charge-trapping states could be further studied for enabling ultralow-cost multibit analog memory devices.

  17. Attosecond-controlled photoemission from metal nanowire tips in the few-electron regime

    KAUST Repository

    Ahn, B.

    2017-02-07

    Metal nanotip photoemitters have proven to be versatile in fundamental nanoplasmonics research and applications, including, e.g., the generation of ultrafast electron pulses, the adiabatic focusing of plasmons, and as light-triggered electron sources for microscopy. Here, we report the generation of high energy photoelectrons (up to 160 eV) in photoemission from single-crystalline nanowire tips in few-cycle, 750-nm laser fields at peak intensities of (2-7.3) × 1012 W/cm2. Recording the carrier-envelope phase (CEP)-dependent photoemission from the nanowire tips allows us to identify rescattering contributions and also permits us to determine the high-energy cutoff of the electron spectra as a function of laser intensity. So far these types of experiments from metal nanotips have been limited to an emission regime with less than one electron per pulse. We detect up to 13 e/shot and given the limited detection efficiency, we expect up to a few ten times more electrons being emitted from the nanowire. Within the investigated intensity range, we find linear scaling of cutoff energies. The nonlinear scaling of electron count rates is consistent with tunneling photoemission occurring in the absence of significant charge interaction. The high electron energy gain is attributed to field-induced rescattering in the enhanced nanolocalized fields at the wires apex, where a strong CEP-modulation is indicative of the attosecond control of photoemission.

  18. Acceleration of high charge density electron beams in the SLAC linac

    International Nuclear Information System (INIS)

    Sheppard, J.C.; Clendenin, J.E.; Jobe, R.K.; Lueth, V.G.; Millich, A.; Ross, M.C.; Seeman, J.T.; Stiening, R.F.

    1984-01-01

    The SLAC Linear Collider (SLC) will require both electron and positron beams of very high charge density and low emittance to be accelerated to about 50 GeV in the SLAC 3-km linac. The linac is in the process of being improved to meet this requirement. The program to accelerate an electron beam of high charge density through the first third of the SLC linac is described and the experimental results are discussed. 7 references, 5 figures

  19. Operation mode switchable charge-trap memory based on few-layer MoS2

    Science.gov (United States)

    Hou, Xiang; Yan, Xiao; Liu, Chunsen; Ding, Shijin; Zhang, David Wei; Zhou, Peng

    2018-03-01

    Ultrathin layered two-dimensional (2D) semiconductors like MoS2 and WSe2 have received a lot of attention because of their excellent electrical properties and potential applications in electronic devices. We demonstrate a charge-trap memory with two different tunable operation modes based on a few-layer MoS2 channel and an Al2O3/HfO2/Al2O3 charge storage stack. Our device shows excellent memory properties under the traditional three-terminal operation mode. More importantly, unlike conventional charge-trap devices, this device can also realize the memory performance with just two terminals (drain and source) because of the unique atomic crystal electrical characteristics. Under the two-terminal operation mode, the erase/program current ratio can reach up to 104 with a stable retention property. Our study indicates that the conventional charge-trap memory cell can also realize the memory performance without the gate terminal based on novel two dimensional materials, which is meaningful for low power consumption and high integration density applications.

  20. Highly charged ion trapping and cooling

    International Nuclear Information System (INIS)

    Beck, B. R.; Church, D. A.; Gruber, L.; Holder, J. P.; Schneider, D.; Steiger, J.

    1998-01-01

    In the past few years a cryogenic Penning trap (RETRAP) has been operational at the Electron Beam Ion Trap (EBIT) facility at Lawrence Livermore National Laboratory. The combination of RETRAP and EBIT provides a unique possibility of producing and re-trapping highly charged ions and cooling them to very low temperatures. Due to the high Coulomb potentials in such an ensemble of cold highly charged ions the Coulomb coupling parameter (the ratio of Coulomb potential to the thermal energy) can easily reach values of 172 and more. To study such systems is not only of interest in astrophysics to simulate White Dwarf star interiors but opens up new possibilities in a variety of areas (e.g. laser spectroscopy), cold highly charged ion beams

  1. Mechanism of Runaway Electron Generation at Gas Pressures from a Few Atmospheres to Several Tens of Atmospheres

    Science.gov (United States)

    Zubarev, N. M.; Ivanov, S. N.

    2018-04-01

    The mechanism of runaway electron generation at gas pressures from a few atmospheres to several tens of atmospheres is proposed. According to this mechanism, the electrons pass into the runaway mode in the enhanced field zone that arises between a cathode micropoint—a source of field-emission electrons—and the region of the positive ion space charge accumulated near the cathode in the tails of the developing electron avalanches. As a result, volume gas ionization by runaway electrons begins with a time delay required for the formation of the enhanced field zone. This process determines the delay time of breakdown. The influence of the gas pressure on the formation dynamics of the space charge region is analyzed. At gas pressures of a few atmospheres, the space charge arises due to the avalanche multiplication of the very first field-emission electron, whereas at pressures of several tens of atmospheres, the space charge forms as a result of superposition of many electron avalanches with a relatively small number of charge carriers in each.

  2. Atomic physics of highly charged ions in an electron beam ion trap

    International Nuclear Information System (INIS)

    Marrs, R.E.

    1990-07-01

    Two electron beam ion traps are in use at LLNL for the purpose of studying the properties of very highly charged ions and their interactions with electrons. This paper reviews the operation of the traps and discusses recent experiments in three areas: precision transition energy measurements in the limit of very high ion charge, dielectronic recombination measurements for the He-like isoelectronic sequence, and measurements of x-ray polarization. 22 refs., 11 figs., 1 tab

  3. Effects of magnetic configuration on hot electrons in highly charged ECR plasma

    International Nuclear Information System (INIS)

    Zhao, H Y; Zhao, H W; Sun, L T; Wang, H; Ma, B H; Zhang, X Zh; Li, X X; Ma, X W; Zhu, Y H; Lu, W; Shang, Y; Xie, D Z

    2009-01-01

    To investigate the hot electrons in highly charged electron cyclotron resonance (ECR) plasma, Bremsstrahlung radiations were measured on two ECR ion sources at the Institute of Modern Physics. Used as a comparative index of the mean energy of the hot electrons, a spectral temperature, T spe , is derived through a linear fitting of the spectra in a semi-logarithmic representation. The influences of the external source parameters, especially the magnetic configuration, on the hot electrons are studied systematically. This study has experimentally demonstrated the importance of high microwave frequency and high magnetic field in the electron resonance heating to produce a high density of hot electrons, which is consistent with the empirical ECR scaling laws. The experimental results have again shown that a good compromise is needed between the ion extraction and the plasma confinement for an efficient production of highly charged ion beams. In addition, this investigation has shown that the correlation between the mean energy of the hot electrons and the magnetic field gradient at the ECR is well in agreement with the theoretical models.

  4. Atomic physics with highly charged ions. Progress report

    Energy Technology Data Exchange (ETDEWEB)

    Richard, P.

    1994-08-01

    The study of inelastic collision phenomena with highly charged projectile ions and the interpretation of spectral features resulting from these collisions remain as the major focal points in the atomic physics research at the J.R. Macdonald Laboratory, Kansas State University, Manhattan, Kansas. The title of the research project, ``Atomic Physics with Highly Charged Ions,`` speaks to these points. The experimental work in the past few years has divided into collisions at high velocity using the primary beams from the tandem and LINAC accelerators and collisions at low velocity using the CRYEBIS facility. Theoretical calculations have been performed to accurately describe inelastic scattering processes of the one-electron and many-electron type, and to accurately predict atomic transition energies and intensities for x rays and Auger electrons. Brief research summaries are given for the following: (1) electron production in ion-atom collisions; (2) role of electron-electron interactions in two-electron processes; (3) multi-electron processes; (4) collisions with excited, aligned, Rydberg targets; (5) ion-ion collisions; (6) ion-molecule collisions; (7) ion-atom collision theory; and (8) ion-surface interactions.

  5. Laser wakefield electron acceleration. A novel approach employing supersonic microjets and few-cycle laser pulses

    International Nuclear Information System (INIS)

    Schmid, Karl

    2011-01-01

    This thesis covers the few-cycle laser-driven acceleration of electrons in a laser-generated plasma. This process, known as laser wakefield acceleration (LWFA), relies on strongly driven plasma waves for the generation of accelerating gradients in the vicinity of several 100 GV/m, a value four orders of magnitude larger than that attainable by conventional accelerators. This thesis demonstrates that laser pulses with an ultrashort duration of 8 fs and a peak power of 6 TW allow the production of electron energies up to 50 MeV via LWFA. The special properties of laser accelerated electron pulses, namely the ultrashort pulse duration, the high brilliance, and the high charge density, open up new possibilities in many applications of these electron beams. (orig.)

  6. Thermal spike analysis of highly charged ion tracks

    International Nuclear Information System (INIS)

    Karlušić, M.; Jakšić, M.

    2012-01-01

    The irradiation of material using swift heavy ion or highly charged ion causes excitation of the electron subsystem at nanometer scale along the ion trajectory. According to the thermal spike model, energy deposited into the electron subsystem leads to temperature increase due to electron–phonon coupling. If ion-induced excitation is sufficiently intensive, then melting of the material can occur, and permanent damage (i.e., ion track) can be formed upon rapid cooling. We present an extension of the analytical thermal spike model of Szenes for the analysis of surface ion track produced after the impact of highly charged ion. By applying the model to existing experimental data, more than 60% of the potential energy of the highly charged ion was shown to be retained in the material during the impact and transformed into the energy of the thermal spike. This value is much higher than 20–40% of the transferred energy into the thermal spike by swift heavy ion. Thresholds for formation of highly charged ion track in different materials show uniform behavior depending only on few material parameters.

  7. High-resolution x-ray scattering studies of charge ordering in highly correlated electron systems

    International Nuclear Information System (INIS)

    Ghazi, M.E.

    2002-01-01

    Many important properties of transition metal oxides such as, copper oxide high-temperature superconductivity and colossal magnetoresistance (CMR) in manganites are due to strong electron-electron interactions, and hence these systems are called highly correlated systems. These materials are characterised by the coexistence of different kinds of order, including charge, orbital, and magnetic moment. This thesis contains high-resolution X-ray scattering studies of charge ordering in such systems namely the high-T C copper oxides isostructural system, La 2-x Sr x NiO 4 with various Sr concentrations (x = 0.33 - 0.2), and the CMR manganite system, Nd 1/2 Sr 1/2 MnO 3 . It also includes a review of charge ordering in a large variety of transition metal oxides, such as ferrates, vanadates, cobaltates, nickelates, manganites, and cuprates systems, which have been reported to date in the scientific literature. Using high-resolution synchrotron X-ray scattering, it has been demonstrated that the charge stripes exist in a series of single crystals of La 2-x Sr x NiO 4 with Sr concentrations (x = 0.33 - 0.2) at low temperatures. Satellite reflections due to the charge ordering were found with the wavevector (2ε, 0, 1) below the charge ordering transition temperature, T CO , where 2ε is the amount of separation from the corresponding Bragg peak. The charge stripes are shown to be two-dimensional in nature both by measurements of their correlation lengths and by measurement of the critical exponents of the charge stripe melting transition with an anomaly at x = 0.25. The results show by decreasing the hole concentration from the x = 0.33 to 0.2, the well-correlated charge stripes change to a glassy state at x = 0.25. The electronic transition into the charge stripe phase is second-order without any corresponding structural transition. Above the second-order transition critical scattering was observed due to fluctuations into the charge stripe phase. In a single-crystal of Nd

  8. Practical Approaches to Mitigation of Specimen Charging in High-Resolution Transmission Electron Microscopy

    Directory of Open Access Journals (Sweden)

    Young-Min Kim

    2010-09-01

    Full Text Available Specimen charging that is associated with the electron bombardment on the sample is a practical hindrance to high-resolution transmission electron microscopy (HRTEM analysis because it causes a severe loss of resolution in either diffraction or image data. Conductive thin film deposition on an insulating specimen has been proposed as an effective approach to the mitigation of the specimen charging; however, this method is generally not useful in HRTEM imaging of materials because the deposited film induces another artifact in the HRTEM image contrast. In this study, we propose practical methods to mitigate the specimen charging that takes place during the HRTEM of materials. For bulk-type specimens prepared by either an ion-thinning or focused-ion beam (FIB process, a plasma cleaning treatment is significantly effective in eliminating the charging phenomenon. In the case of low-dimensional nanomaterials such as nanowires and nanoparticles, the plasma cleaning is not feasible; however, the charging effect can be effectively eliminated by adjusting the electron illumination condition. The proposed methods facilitate a decrease in the buildup of specimen charging, thereby enhancing the quality of high-resolution images significantly.

  9. A high-energy electron beam ion trap for production of high-charge high-Z ions

    International Nuclear Information System (INIS)

    Knapp, D.A.; Marrs, R.E.; Elliott, S.R.; Magee, E.W.; Zasadzinski, R.

    1993-01-01

    We have developed a new high-energy electron beam ion trap, the first laboratory source of low-energy, few-electron, high-Z ions. We describe the device and report measurements of its performance, including the electron beam diameter, current density and energy, and measurements of the ionization balance for several high-Z elements in the trap. This device opens up a wide range of possible experiments in atomic physics, plasma physics, and nuclear physics. (orig.)

  10. Measurements of the Properties of Highly-charged high-Z ions

    International Nuclear Information System (INIS)

    Augustine J. Smith, Ph.D.

    2007-01-01

    We had proposed carrying out a systematic experimental investigation of the atomic physics of highly charged, high-Z ions, produced in the Lawrence Livermore National Laboratory LLNL electron beam ion trap (EBIT-I) in its high energy mode, superEBIT. In particular we were going to accurately measure line positions for Δn=0 transitions in few electron high-Z ions; this was meant to enable us to investigate relativistic and quantum electrodynamics QED contributions to the energy levels as well as the nuclear properties of heavy ions. We were also going to measure cross sections for various electron-ion interactions, the degree of polarization of emitted x-rays, and radiation cooling rates of various ionization stages of highly charged, high-Z ions. This would enable us to study fundamental atomic physics of high-Z ions at relativistic electron impact energies and in the intense nuclear fields of highly ionized, high-Z ions. This would extend previous measurements we have carried out to a regime where there is a paucity of good data. These measurements were expected to generate increased theoretical interest and activity in this area. The project will extend a very successful collaboration between Morehouse College (MC) and a national laboratory LLNL, Minority student training and development are major components of the proposal

  11. Spectroscopy of highly charged tungsten ions with Electron Beam Ion Traps

    International Nuclear Information System (INIS)

    Sakaue, Hiroyuki A.; Kato, Daiji; Morita, Shigeru; Murakami, Izumi; Yamamoto, Norimasa; Ohashi, Hayato; Yatsurugi, Junji; Nakamura, Nobuyuki

    2013-01-01

    We present spectra of highly charged tungsten ions in the extreme ultra-violet (EUV) by using electron beam ion traps. The electron energy dependence of spectra is investigated of electron energies from 490 to 1440 eV. Previously unreported lines are presented in the EUV range, and some of them are identified by comparing the wavelengths with theoretical calculations. (author)

  12. Charge exchange processes of high energy heavy ions channeled in crystals

    International Nuclear Information System (INIS)

    Andriamonje, S.; Dural, J.; Toulemonde, M.; Groeneveld, K.O.; Maier, R.; Quere, Y.

    1990-01-01

    The interaction of moving ions with single crystals is very sensitive to the orientation of the incident beam with respect to the crystalline directions of the target. The experiments show that high energy heavy ion channeling deeply modifies the slowing down and charge exchange processes. In this review, we describe the opportunity offered by channeling conditions to study the charge exchange processes. Some aspects of the charge exchange processes with high energy channeled heavy ions are selected from the extensive literature published over the past few years on this subject. Special attention is given to the work performed at the GANIL facility on the study of Radiative Electron Capture (REG), Electron Impact Ionisation (EII), and convoy electron emission. Finally we emphasize the interest of studying resonant charge exchange processes such as Resonant Coherent Excitation (RCE), Resonant Transfer and Excitation (RTE) or Dielectronic Recombination (DR) and the recently proposed Nuclear Excitation by Electron Capture (NEEC)

  13. Correlated double electron capture in slow, highly charged ion-atom collisions

    International Nuclear Information System (INIS)

    Stolterfoht, N.; Havener, C.C.; Phaneuf, R.A.; Swenson, J.K.; Shafroth, S.M.; Meyer, F.W.

    1986-01-01

    Recent measurements of autoionization electrons produced in slow, highly charged ion-atom collisions are reviewed. Mechanisms for double electron capture into equivalent and nonequivalent configurations are analyzed by comparing the probabilities for the creation of L 1 L 23 X Coster Kronig electrons and L-Auger electrons. It is shown that the production of the Coster-Kronig electrons is due to electron correlation effects whose analysis leads beyond the independent-particle model. The importance of correlation effects on different capture mechanisms is discussed. 28 refs., 6 figs

  14. Spectroscopy of heavy few-electron ions

    International Nuclear Information System (INIS)

    Mokler, P.H.

    1986-07-01

    In this paper we ask first, why is it interesting to investigate heavy-few electron ions. Then the various accelerator-based methods to produce heavy few-electron ions are discussed. In the main part an overview on available heavy few-electron ion data and current experiments is given. The summary will end up with future aspects in this field. (orig.)

  15. Correlated double electron capture in slow, highly charged ion-atom collisions

    Energy Technology Data Exchange (ETDEWEB)

    Stolterfoht, N.; Havener, C.C.; Phaneuf, R.A.; Swenson, J.K.; Shafroth, S.M.; Meyer, F.W.

    1986-01-01

    Recent measurements of autoionization electrons produced in slow, highly charged ion-atom collisions are reviewed. Mechanisms for double electron capture into equivalent and nonequivalent configurations are analyzed by comparing the probabilities for the creation of L/sub 1/L/sub 23/X Coster Kronig electrons and L-Auger electrons. It is shown that the production of the Coster-Kronig electrons is due to electron correlation effects whose analysis leads beyond the independent-particle model. The importance of correlation effects on different capture mechanisms is discussed. 28 refs., 6 figs.

  16. Hearing shapes of few electrons quantum drums: A configuration–interaction study

    International Nuclear Information System (INIS)

    Ţolea, F.; Ţolea, M.

    2015-01-01

    The – highly remarkable – existence of non-congruent yet vibrationally isospectral shapes has been first proved theoretically and then also tested experimentally – by using electromagnetic waves in cavities, vibrating smectic films or electrons in nanostructures. In this context, we address the question whether isospectrality holds if two or more electrons interact electrostatically, using the accurate configuration–interaction method, in a discrete representation of the Bilby and Hawk shapes. Isospectral pairs offer an unique possibility to test how identical sets of single-particle energies may combine differently in the few-electrons eigenmodes, due to different wave functions spatial distributions. Our results point towards the break down of isospectrality in the presence of interactions. Thus one should be able to ”hear” the shapes of few electrons quantum drums. Interestingly however, for the analyzed two and three electrons cases, there exists an interaction strength (which can be tuned by changing the size of the shapes), for which the ground states energies of Bilby and Hawk coincide, but not the excited states as well. Wigner localization is studied and shown to occur at about the same size for both Bilby and Hawk shapes. Next, an exercise is proposed to use the two-electrons charge density of the Bilby and Hawk ground states in the phase extraction scheme as proposed by Moon et al. (2008). Results show that out-of-phase regions appear if the linear size of the shapes exceeds the Bohr radius as occupation of higher Slater determinants becomes significant

  17. Hearing shapes of few electrons quantum drums: A configuration–interaction study

    Energy Technology Data Exchange (ETDEWEB)

    Ţolea, F.; Ţolea, M., E-mail: tzolea@infim.ro

    2015-02-01

    The – highly remarkable – existence of non-congruent yet vibrationally isospectral shapes has been first proved theoretically and then also tested experimentally – by using electromagnetic waves in cavities, vibrating smectic films or electrons in nanostructures. In this context, we address the question whether isospectrality holds if two or more electrons interact electrostatically, using the accurate configuration–interaction method, in a discrete representation of the Bilby and Hawk shapes. Isospectral pairs offer an unique possibility to test how identical sets of single-particle energies may combine differently in the few-electrons eigenmodes, due to different wave functions spatial distributions. Our results point towards the break down of isospectrality in the presence of interactions. Thus one should be able to ”hear” the shapes of few electrons quantum drums. Interestingly however, for the analyzed two and three electrons cases, there exists an interaction strength (which can be tuned by changing the size of the shapes), for which the ground states energies of Bilby and Hawk coincide, but not the excited states as well. Wigner localization is studied and shown to occur at about the same size for both Bilby and Hawk shapes. Next, an exercise is proposed to use the two-electrons charge density of the Bilby and Hawk ground states in the phase extraction scheme as proposed by Moon et al. (2008). Results show that out-of-phase regions appear if the linear size of the shapes exceeds the Bohr radius as occupation of higher Slater determinants becomes significant.

  18. EUV spectrum of highly charged tungsten ions in electron beam ion trap

    International Nuclear Information System (INIS)

    Sakaue, H.A.; Kato, D.; Murakami, I.; Nakamura, N.

    2016-01-01

    We present spectra of highly charged tungsten ions in the extreme ultra-violet (EUV) by using electron beam ion traps. The electron energy dependence of spectra was investigated for electron energy from 540 to 1370 eV. Previously unreported lines were presented in the EUV range, and comparing the wavelengths with theoretical calculations identified them. (author)

  19. Space-charge effect in electron time-of-flight analyzer for high-energy photoemission spectroscopy

    International Nuclear Information System (INIS)

    Greco, G.; Verna, A.; Offi, F.; Stefani, G.

    2016-01-01

    Highlights: • Two methods for the simulation of space-charge effect in time-resolved PES. • Reliability and advantages in the use of the SIMION"® software. • Simulation of the space-charge effect in an electron TOF analyzer. • Feasibility of a TOF analyzer in time-resolved high-energy PES experiments at FEL. - Abstract: The space-charge effect, due to the instantaneous emission of many electrons after the absorption of a single photons pulse, causes distortion in the photoelectron energy spectrum. Two calculation methods have been applied to simulate the expansion during a free flight of clouds of mono- and bi-energetic electrons generated by a high energy pulse of light and their results have been compared. The accuracy of a widely used tool, such as SIMION"®, in predicting the energy distortion caused by the space-charge has been tested and the reliability of its results is verified. Finally we used SIMION"® to take into account the space-charge effects in the simulation of simple photoemission experiments with a time-of-flight analyzer.

  20. Electron ejection from solids induced by fast highly-charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Schiwietz, G. [Hahn-Meitner-Inst. GmbH, Berlin (Germany). Abt. FD; Xiao, G. [Hahn-Meitner-Inst. GmbH, Berlin (Germany). Abt. FD

    1996-02-01

    Total electron-ejection yields and Auger-electron spectra for highly-charged ions interacting with different foil targets have been investigated in this work. New experimental and theoretical data for normal incident 5 MeV/u heavy ions on graphite and polypropylene foils are presented and discussed. These two materials have been selected as model systems representing conductors and insulator targets. Our measured projectile nuclear-charge dependence of the total electron yield from carbon foils clearly deviates from results of some transport models that predict a proportionality with respect to the electronic stopping power of the projectiles. Possible reasons for this deviation are discussed. We have also extended our measurements on cascade-induced C-KLL Auger-electron production. The corresponding results for 5 MeV/u S ions on carbon were obtained with a new method and agree fairly well with previous data. Furthermore, we have performed an experimental and theoretical investigation on the nuclear-track potential in insulators. Comparison of experimental data with theoretical results for N{sup 7+}, Ne{sup 9+}, Ar{sup 16+} and Ni{sup 23+} ions allow for an estimate of the electron/hole pair recombination time at the center of the track in polypropylene. (orig.).

  1. Correlation effects on double electron capture in highly-charged, low-energy ion-atom collisions

    International Nuclear Information System (INIS)

    Meyer, F.W.; Griffin, D.C.; Havener, C.C.; Huq, M.S.; Phaneuf, R.A.; Swenson, J.K.; Stolterfoht, N.

    1987-01-01

    The method of zero-degree Auger electron spectroscopy has been used to study two-electron excited states populated in slow double capture collisions of highly charged ions with He and H 2 . The focus of this study is on production of autoionization electrons originating from the non-equivalent 1s 2 2pnl electron configurations in comparison with electron production resulting from the Auger decay of (near) equivalent 1s 2 nln'l' (with n∼n') configurations. It is shown that production of non-equivalent electron configurations is significant and involves electron-electron correlation effects whose analysis leads beyond the independent-particle model. Recent results that include a measurement at non-zero angles are presented to illustrate the angular dependence of electron emission from non-equivalent electron configurations, as well as the dependence on projectile charge state and target species. Comparison of high resolution scans over two lines of the 1s 2 2pnl sequence for the O 6+ + He system with accurate transition energy calculations shows preferential population of high angular momentum substation

  2. New experimental initiatives using very highly charged ions from an 'electron beam ion trap'

    International Nuclear Information System (INIS)

    Schneider, D.

    1996-01-01

    A short review of the experimental program in highly-charged heavy ion physics conducted at the Lawrence Livermore National Laboratory Electron Beam Ion Trap (EBIT) facility is presented. The heavy-ion research, involving ions up to fully stripped U 92+ , includes precision x-ray spectroscopy and lifetime studies, electron impact ionization and excitation cross section measurements. The investigations of ion-surface interactions following the impact of high-Z highly charged ions on surfaces are aimed to study the neutralization dynamics effecting the ion and the response of the surface as well. (author)

  3. Femtosecond few- to single-electron point-projection microscopy for nanoscale dynamic imaging

    Directory of Open Access Journals (Sweden)

    A. R. Bainbridge

    2016-03-01

    Full Text Available Femtosecond electron microscopy produces real-space images of matter in a series of ultrafast snapshots. Pulses of electrons self-disperse under space-charge broadening, so without compression, the ideal operation mode is a single electron per pulse. Here, we demonstrate femtosecond single-electron point projection microscopy (fs-ePPM in a laser-pump fs-e-probe configuration. The electrons have an energy of only 150 eV and take tens of picoseconds to propagate to the object under study. Nonetheless, we achieve a temporal resolution with a standard deviation of 114 fs (equivalent to a full-width at half-maximum of 269 ± 40 fs combined with a spatial resolution of 100 nm, applied to a localized region of charge at the apex of a nanoscale metal tip induced by 30 fs 800 nm laser pulses at 50 kHz. These observations demonstrate real-space imaging of reversible processes, such as tracking charge distributions, is feasible whilst maintaining femtosecond resolution. Our findings could find application as a characterization method, which, depending on geometry, could resolve tens of femtoseconds and tens of nanometres. Dynamically imaging electric and magnetic fields and charge distributions on sub-micron length scales opens new avenues of ultrafast dynamics. Furthermore, through the use of active compression, such pulses are an ideal seed for few-femtosecond to attosecond imaging applications which will access sub-optical cycle processes in nanoplasmonics.

  4. Electronic sputtering by swift highly charged ions of nitrogen on amorphous carbon

    International Nuclear Information System (INIS)

    Caron, M.; Haranger, F.; Rothard, H.; Ban d'Etat, B.; Boduch, P.; Clouvas, A.; Potiriadis, C.; Neugebauer, R.; Jalowy, T.

    2001-01-01

    Electronic sputtering with heavy ions as a function of both electronic energy loss dE/dx and projectile charge state q was studied at the French heavy ion accelerator GANIL. Amorphous carbon (untreated, and sputter-cleaned and subsequently exposed to nitrogen) was irradiated with swift highly charged ions (Z=6-73, q=6-54, energy 6-13 MeV/u) in an ultrahigh vacuum scattering chamber. The fluence dependence of ion-induced electron yields allows to deduce a desorption cross-section σ which varies approximately as σ∼(dE/dx) 1.65 or σ∼q 3.3 for sputter-cleaned amorphous carbon exposed to nitrogen. This q dependence is close to the cubic charge dependence observed for the emission of H + secondary ions which are believed to be emitted from the very surface. However, the power law σ∼(dE/dx) 1.65 , related to the electronic energy loss gives the best empirical description. The dependence on dE/dx is close to a quadratic one thus rather pointing towards a thermal evaporation-like effect

  5. ELECTRON-CAPTURE IN HIGHLY-CHARGED ION-ATOM COLLISIONS

    NARCIS (Netherlands)

    MORGENSTERN, R

    1993-01-01

    An attempt is made to identify the most important mechanisms responsible for the rearrangement of electrons during collisions between multiply charged ions and atoms at keV energies. It is discussed to which extent the influence of binding energy, angular momentum of heavy particles and electrons,

  6. Production of highly charged ion beams from electron cyclotron resonance ion sources (invited)

    International Nuclear Information System (INIS)

    Xie, Z.Q.

    1998-01-01

    Electron cyclotron resonance ion source (ECRIS) development has progressed with multiple-frequency plasma heating, higher mirror magnetic fields, and better technique to provide extra cold electrons. Such techniques greatly enhance the production of highly charged ions from ECRISs. So far at continuous wave (CW) mode operation, up to 300 eμA of O 7+ and 1.15 emA of O 6+ , more than 100 eμA of intermediate heavy ions for charge states up to Ar 13+ , Ca 13+ , Fe 13+ , Co 14+ , and Kr 18+ , and tens of eμA of heavy ions with charge states to Kr 26+ , Xe 28+ , Au 35+ , Bi 34+ , and U 34+ were produced from ECRISs. At an intensity of at least 1 eμA, the maximum charge state available for the heavy ions are Xe 36+ , Au 46+ , Bi 47+ , and U 48+ . An order of magnitude enhancement for fully stripped argon ions (I≥60enA) were also achieved. This article will review the ECR ion source progress and discuss key requirement for ECRISs to produce the highly charged ion beams. copyright 1998 American Institute of Physics

  7. Classical behavior of few-electron parabolic quantum dots

    International Nuclear Information System (INIS)

    Ciftja, O.

    2009-01-01

    Quantum dots are intricate and fascinating systems to study novel phenomena of great theoretical and practical interest because low dimensionality coupled with the interplay between strong correlations, quantum confinement and magnetic field creates unique conditions for emergence of fundamentally new physics. In this work we consider two-dimensional semiconductor quantum dot systems consisting of few interacting electrons confined in an isotropic parabolic potential. We study the many-electron quantum ground state properties of such systems in presence of a perpendicular magnetic field as the number of electrons is varied using exact numerical diagonalizations and other approaches. The results derived from the calculations of the quantum model are then compared to corresponding results for a classical model of parabolically confined point charges who interact with a Coulomb potential. We find that, for a wide range of parameters and magnetic fields considered in this work, the quantum ground state energy is very close to the classical energy of the most stable classical configuration under the condition that the classical energy is properly adjusted to incorporate the quantum zero point motion.

  8. Initial observations of high-charge, low-emittance electron beams at HIBAF (High Brightness Accelerator FEL)

    Energy Technology Data Exchange (ETDEWEB)

    Lumpkin, A.H.; Feldman, R.B.; Carsten, B.E.; Feldman, D.W.; Sheffield, R.L.; Stein, W.E.; Johnson, W.J.; Thode, L.E.; Bender, S.C.; Busch, G.E.

    1990-01-01

    We report our initial measurements of bright (high-charge, low-emittance) electron beams generated at the Los Alamos High Brightness Accelerator FEL (HIBAF) Facility. Normalized emittance values of less than 50 {pi} mm-mrad for charges ranging from 0.7 to 8.7 nC were obtained for single micropulses at a y-waist and at an energy of 14.7 MeV. These measurements were part of the commissioning campaign on the HIBAF photoelectric injector. Macropulse measurements have also been performed and are compared with PARMELA simulations. 5 refs., 8 figs., 3 tabs.

  9. ANISOTROPY EFFECTS IN SINGLE-ELECTRON TRANSFER BETWEEN LASER-EXCITED ATOMS AND HIGHLY-CHARGED IONS

    NARCIS (Netherlands)

    Recent collision experiments are reviewed in which one-electron transfer between laser excited target atoms and (highly charged) keV-ions has been studied. Especially results showing a dependence of the charge exchange on the initial target orbital alignment are discussed. The question to what

  10. Ultrafast electron microscopy: Instrument response from the single-electron to high bunch-charge regimes

    Science.gov (United States)

    Plemmons, Dayne A.; Flannigan, David J.

    2017-09-01

    We determine the instrument response of an ultrafast electron microscope equipped with a conventional thermionic electron gun and absent modifications beyond the optical ports. Using flat, graphite-encircled LaB6 cathodes, we image space-charge effects as a function of photoelectron-packet population and find that an applied Wehnelt bias has a negligible effect on the threshold levels (>103 electrons per pulse) but does appear to suppress blurring at the upper limits (∼105 electrons). Using plasma lensing, we determine the instrument-response time for 700-fs laser pulses and find that single-electron packets are laser limited (1 ps), while broadening occurs well below the space-charge limit.

  11. Spacecraft charging: incoming and outgoing electrons

    CERN Document Server

    Lai, Shu T.

    2013-04-22

    This paper presents an overview of the roles played by incoming and outgoing electrons in spacecraft surface and stresses the importance of surface conditions for spacecraft charging. The balance between the incoming electron current from the ambient plasma and the outgoing currents of secondary electrons, backscattered electrons, and photoelectrons from the surfaces determines the surface potential. Since surface conditions significantly affect the outgoing currents, the critical temperature and the surface potential are also significantly affected. As a corollary, high level differential charging of adjacent surfaces with very different surface conditions is a space hazard.

  12. Few electron transitions in atomic collisions. Final report, September 1, 1992--December 31, 1995

    Energy Technology Data Exchange (ETDEWEB)

    McGuire, J.

    1997-04-01

    During the past three years we have evaluated probabilities and cross sections for few and multiple electron transitions in atomic collisions. Our studies included interactions of atoms and molecules with incident protons, bare ions, electrons, positrons, anti-protons, ions carrying electrons and photons. We also: studied the inter-relation between collisions with charged particles and collisions involving various processes with photons. This work has complemented various studies of collisions of atoms with charged particles and with photons as well as more general efforts to understand the nature of multi-electron systems. Our aim has been to begin with relatively simple two electron systems and to focus on fast processes in which there is too little time for complicated processes to occur. We have used a variety of computational techniques, but we emphasize those appropriate for fast collisions in which we hope to obtain insight into the physical nature of the process itself. We generally considered systems in which experimental data was available.

  13. Generation of annular, high-charge electron beams at the Argonne wakefield accelerator

    Science.gov (United States)

    Wisniewski, E. E.; Li, C.; Gai, W.; Power, J.

    2013-01-01

    We present and discuss the results from the experimental generation of high-charge annular(ring-shaped)electron beams at the Argonne Wakefield Accelerator (AWA). These beams were produced by using laser masks to project annular laser profiles of various inner and outer diameters onto the photocathode of an RF gun. The ring beam is accelerated to 15 MeV, then it is imaged by means of solenoid lenses. Transverse profiles are compared for different solenoid settings. Discussion includes a comparison with Parmela simulations, some applications of high-charge ring beams,and an outline of a planned extension of this study.

  14. Generation of annular, high-charge electron beams at the Argonne wakefield accelerator

    Science.gov (United States)

    Wisniewski, E. E.; Li, C.; Gai, W.; Power, J.

    2012-12-01

    We present and discuss the results from the experimental generation of high-charge annular(ring-shaped)electron beams at the Argonne Wakefield Accelerator (AWA). These beams were produced by using laser masks to project annular laser profiles of various inner and outer diameters onto the photocathode of an RF gun. The ring beam is accelerated to 15 MeV, then it is imaged by means of solenoid lenses. Transverse profiles are compared for different solenoid settings. Discussion includes a comparison with Parmela simulations, some applications of high-charge ring beams,and an outline of a planned extension of this study.

  15. Testing partonic charge symmetry at a high-energy electron collider

    International Nuclear Information System (INIS)

    Hobbs, T.J.; Londergan, J.T.; Murdock, D.P.; Thomas, A.W.

    2011-01-01

    We examine the possibility that one could measure partonic charge symmetry violation (CSV) by comparing neutrino or antineutrino production through charged-current reactions induced by electrons or positrons at a possible electron collider at the LHC. We calculate the magnitude of CSV that might be expected at such a facility. We show that this is likely to be a several percent effect, substantially larger than the typical CSV effects expected for partonic reactions.

  16. Secondary-electron yield from Au induced by highly charged Ta ions

    Czech Academy of Sciences Publication Activity Database

    Krása, Josef; Láska, Leoš; Stöckli, M. P.; Fry, D.

    2001-01-01

    Roč. 173, - (2001), s. 281-286 ISSN 0168-583X R&D Projects: GA AV ČR IAA1010819 Institutional research plan: CEZ:AV0Z1010914 Keywords : highly charged ion-surface interaction * ion-induced electron emission * angle impact effect Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.041, year: 2001

  17. Modelling and design of high compression electron guns for EBIS/T charge breeders

    CERN Document Server

    AUTHOR|(CDS)2087190; Zschornack, G.; Lettry, J.; Wenander, F.

    In this thesis the optimization of the REXEBIS charge breeder at the ISOLDE facility is presented. REXEBIS in its current state provides a current density of 200A/cm² inside the trapping region at 2 T and will be optimized to the physical limit of its design. To overcome this limit a new electron gun, the HEC² gun, was designed in collaboration with the BNL and is in commission at TestEBIS. This electron gun promises a current density of >10 kA/cm², which decreases the charge breeding time significantly. This thesis presents novel simulation techniques supporting the commissioning phase by explaining the sources of occurring loss current and, in addition, evaluate the currently installed collector for compatibility with the HEC2 gun operating at its design limit. The experience gained from the commission of the HEC² gun and the established numerical techniques lead to the development of a smaller high-compression electron gun for medical purposes, the MEDeGUN. This electron gun should provide a high-quali...

  18. Electron Charged Graphite-based Hydrogen Storage Material

    Energy Technology Data Exchange (ETDEWEB)

    Dr. Chinbay Q. Fan; D Manager

    2012-03-14

    The electron-charge effects have been demonstrated to enhance hydrogen storage capacity using materials which have inherent hydrogen storage capacities. A charge control agent (CCA) or a charge transfer agent (CTA) was applied to the hydrogen storage material to reduce internal discharge between particles in a Sievert volumetric test device. GTI has tested the device under (1) electrostatic charge mode; (2) ultra-capacitor mode; and (3) metal-hydride mode. GTI has also analyzed the charge distribution on storage materials. The charge control agent and charge transfer agent are needed to prevent internal charge leaks so that the hydrogen atoms can stay on the storage material. GTI has analyzed the hydrogen fueling tank structure, which contains an air or liquid heat exchange framework. The cooling structure is needed for hydrogen fueling/releasing. We found that the cooling structure could be used as electron-charged electrodes, which will exhibit a very uniform charge distribution (because the cooling system needs to remove heat uniformly). Therefore, the electron-charge concept does not have any burden of cost and weight for the hydrogen storage tank system. The energy consumption for the electron-charge enhancement method is quite low or omitted for electrostatic mode and ultra-capacitor mode in comparison of other hydrogen storage methods; however, it could be high for the battery mode.

  19. New improvements on the Kansas State University cryogenic electron beam ion source, a user facility for low energy, highly charged ions

    International Nuclear Information System (INIS)

    Stockli, M. P.; Carnes, K.; Cocke, C. L.; DePaola, B. D.; Ehrenreich, T.; Fehrenbach, C.; Fry, D.; Gibson, P. E.; Kelly, S.; Lehnert, U.

    2000-01-01

    The Kansas State University cryogenic electron beam ion source supplies low energy ion beams to users of the Department of Energy user facility for highly charged ions. The ions escape the source with an initial energy between 1.6 and 5 kV per charge and are analyzed in a 90 degree sign dipole magnet located on the high voltage platform. When leaving the platform the ions can be accelerated by up to 160 kV per charge or can be decelerated to about 20% of their initial energy, covering 2.5 orders of magnitude. We are in the process of adding another order of magnitude to the range of available ion energies as a newly installed lens allows for deceleration down to a very few percent of the initial energy. In addition we present the current microbunching and chopping system which has been substantially improved over the past 2 yr. (c) 2000 American Institute of Physics

  20. Space-charge compensation of highly charged ion beam from laser ion source

    International Nuclear Information System (INIS)

    Kondrashev, S.A.; Collier, J.; Sherwood, T.R.

    1996-01-01

    The problem of matching an ion beam delivered by a high-intensity ion source with an accelerator is considered. The experimental results of highly charged ion beam transport with space-charge compensation by electrons are presented. A tungsten thermionic cathode is used as a source of electrons for beam compensation. An increase of ion beam current density by a factor of 25 is obtained as a result of space-charge compensation at a distance of 3 m from the extraction system. The process of ion beam space-charge compensation, requirements for a source of electrons, and the influence of recombination losses in a space-charge-compensated ion beam are discussed. (author)

  1. Production of highly charged ion beams with SECRAL

    International Nuclear Information System (INIS)

    Sun, L. T.; Zhao, H. W.; Zhang, X. Z.; Feng, Y. C.; Li, J. Y.; Guo, X. H.; Ma, H. Y.; Zhao, H. Y.; Ma, B. H.; Wang, H.; Li, X. X.; Jin, T.; Xie, D. Z.; Lu, W.; Cao, Y.; Shang, Y.

    2010-01-01

    Superconducting electron cyclotron resonance ion source with advanced design in Lanzhou (SECRAL) is an all-superconducting-magnet electron cyclotron resonance ion source (ECRIS) for the production of intense highly charged ion beams to meet the requirements of the Heavy Ion Research Facility in Lanzhou (HIRFL). To further enhance the performance of SECRAL, an aluminum chamber has been installed inside a 1.5 mm thick Ta liner used for the reduction of x-ray irradiation at the high voltage insulator. With double-frequency (18+14.5 GHz) heating and at maximum total microwave power of 2.0 kW, SECRAL has successfully produced quite a few very highly charged Xe ion beams, such as 10 e μA of Xe 37+ , 1 e μA of Xe 43+ , and 0.16 e μA of Ne-like Xe 44+ . To further explore the capability of the SECRAL in the production of highly charged heavy metal ion beams, a first test run on bismuth has been carried out recently. The main goal is to produce an intense Bi 31+ beam for HIRFL accelerator and to have a feel how well the SECRAL can do in the production of very highly charged Bi beams. During the test, though at microwave power less than 3 kW, more than 150 e μA of Bi 31+ , 22 e μA of Bi 41+ , and 1.5 e μA of Bi 50+ have been produced. All of these results have again demonstrated the great capability of the SECRAL source. This article will present the detailed results and brief discussions to the production of highly charged ion beams with SECRAL.

  2. Electron Impact Excitation and Dielectronic Recombination of Highly Charged Tungsten Ions

    Directory of Open Access Journals (Sweden)

    Zhongwen Wu

    2015-11-01

    Full Text Available Electron impact excitation (EIE and dielectronic recombination (DR of tungsten ions are basic atomic processes in nuclear fusion plasmas of the International Thermonuclear Experimental Reactor (ITER tokamak. Detailed investigation of such processes is essential for modeling and diagnosing future fusion experiments performed on the ITER. In the present work, we studied total and partial electron-impact excitation (EIE and DR cross-sections of highly charged tungsten ions by using the multiconfiguration Dirac–Fock method. The degrees of linear polarization of the subsequent X-ray emissions from unequally-populated magnetic sub-levels of these ions were estimated. It is found that the degrees of linear polarization of the same transition lines, but populated respectively by the EIE and DR processes, are very different, which makes diagnosis of the formation mechanism of X-ray emissions possible. In addition, with the help of the flexible atomic code on the basis of the relativistic configuration interaction method, DR rate coefficients of highly charged W37+ to W46+ ions are also studied, because of the importance in the ionization equilibrium of tungsten plasmas under running conditions of the ITER.

  3. Extraction of highly charged ions from the Berlin Electron Beam Ion Trap for interactions with a gas target

    International Nuclear Information System (INIS)

    Allen, F.I.; Biedermann, C.; Radtke, R.; Fussmann, G.

    2006-01-01

    Highly charged ions are extracted from the Berlin Electron Beam Ion Trap for investigations of charge exchange with a gas target. The classical over-the-barrier model for slow highly charged ions describes this process, whereby one or more electrons are captured from the target into Rydberg states of the ion. The excited state relaxes via a radiative cascade of the electron to ground energy. The cascade spectra are characteristic of the capture state. We investigate x-ray photons emitted as a result of interactions between Ar 17+ ions at energies ≤5q keV with Ar atoms. Of particular interest is the velocity dependence of the angular momentum capture state l c

  4. Review of highly charged heavy ion production with electron cyclotron resonance ion source (invited)

    International Nuclear Information System (INIS)

    Nakagawa, T.

    2014-01-01

    The electron cyclotron resonance ion source (ECRIS) plays an important role in the advancement of heavy ion accelerators and other ion beam applications worldwide, thanks to its remarkable ability to produce a great variety of intense highly charged heavy ion beams. Great efforts over the past decade have led to significant ECRIS performance improvements in both the beam intensity and quality. A number of high-performance ECRISs have been built and are in daily operation or are under construction to meet the continuously increasing demand. In addition, comprehension of the detailed and complex physical processes in high-charge-state ECR plasmas has been enhanced experimentally and theoretically. This review covers and discusses the key components, leading-edge developments, and enhanced ECRIS performance in the production of highly charged heavy ion beams

  5. Surface charge compensation for a highly charged ion emission microscope

    International Nuclear Information System (INIS)

    McDonald, J.W.; Hamza, A.V.; Newman, M.W.; Holder, J.P.; Schneider, D.H.G.; Schenkel, T.

    2003-01-01

    A surface charge compensation electron flood gun has been added to the Lawrence Livermore National Laboratory (LLNL) highly charged ion (HCI) emission microscope. HCI surface interaction results in a significant charge residue being left on the surface of insulators and semiconductors. This residual charge causes undesirable aberrations in the microscope images and a reduction of the Time-Of-Flight (TOF) mass resolution when studying the surfaces of insulators and semiconductors. The benefits and problems associated with HCI microscopy and recent results of the electron flood gun enhanced HCI microscope are discussed

  6. Electron-beam-charged dielectrics: Internal charge distribution

    Science.gov (United States)

    Beers, B. L.; Pine, V. W.

    1981-01-01

    Theoretical calculations of an electron transport model of the charging of dielectrics due to electron bombardment are compared to measurements of internal charge distributions. The emphasis is on the distribution of Teflon. The position of the charge centroid as a function of time is not monotonic. It first moves deeper into the material and then moves back near to the surface. In most time regimes of interest, the charge distribution is not unimodal, but instead has two peaks. The location of the centroid near saturation is a function of the incident current density. While the qualitative comparison of theory and experiment are reasonable, quantitative comparison shows discrepancies of as much as a factor of two.

  7. Electron yield from Be-Cu induced by highly charged Xe q+ ions

    Czech Academy of Sciences Publication Activity Database

    Krása, Josef; Láska, Leoš; Stöckli, M. P.; Fehrenbach, C. W.

    2002-01-01

    Roč. 196, - (2002), s. 61-67 ISSN 0168-583X R&D Projects: GA AV ČR IAA1010105; GA MŠk LN00A100 Institutional research plan: CEZ:AV0Z1010921 Keywords : highly charged ion-induced electron emission * angle impact effect * Be-Cu Subject RIV: BH - Optics, Masers, Lasers Impact factor: 1.158, year: 2002

  8. Fractional conductance oscillations in quantum rings: wave packet picture of transport in a few-electron system.

    Science.gov (United States)

    Chwiej, T; Szafran, B

    2013-04-17

    We study electron transfer across a two-terminal quantum ring using a time-dependent description of the scattering process. For the considered scattering event the quantum ring is initially charged with one or two electrons, with another electron incident to the ring from the input channel. We study the electron transfer probability (T) as a function of the external magnetic field. We determine the periodicity of T for a varied number of electrons confined within the ring. For that purpose we develop a method to describe the wave packet dynamics for a few electrons participating in the scattering process, taking into full account the electron-electron correlations. We find that electron transfer across the quantum ring initially charged by a single electron acquires a distinct periodicity of half of the magnetic flux quantum (Φ0/2), corresponding to the formation of a transient two-electron state inside the ring. In the case of a three-electron scattering problem with two electrons initially occupying the ring, a period of Φ0/3 for T is formed in the limit of thin channels. The effect of disorder present in the confinement potential of the ring is also discussed.

  9. Fractional conductance oscillations in quantum rings: wave packet picture of transport in a few-electron system

    International Nuclear Information System (INIS)

    Chwiej, T; Szafran, B

    2013-01-01

    We study electron transfer across a two-terminal quantum ring using a time-dependent description of the scattering process. For the considered scattering event the quantum ring is initially charged with one or two electrons, with another electron incident to the ring from the input channel. We study the electron transfer probability (T) as a function of the external magnetic field. We determine the periodicity of T for a varied number of electrons confined within the ring. For that purpose we develop a method to describe the wave packet dynamics for a few electrons participating in the scattering process, taking into full account the electron–electron correlations. We find that electron transfer across the quantum ring initially charged by a single electron acquires a distinct periodicity of half of the magnetic flux quantum (Φ 0 /2), corresponding to the formation of a transient two-electron state inside the ring. In the case of a three-electron scattering problem with two electrons initially occupying the ring, a period of Φ 0 /3 for T is formed in the limit of thin channels. The effect of disorder present in the confinement potential of the ring is also discussed. (paper)

  10. One- and two-electron processes in collisions between hydrogen molecules and slow highly charged ions

    International Nuclear Information System (INIS)

    Wells, E.; Carnes, K.D.; Tawara, H.; Ali, R.; Sidky, Emil Y.; Illescas, Clara; Ben-Itzhak, I.

    2005-01-01

    A coincidence time-of-flight technique coupled with projectile charge state analysis was used to study electron capture in collisions between slow highly charged ions and hydrogen molecules. We found single electron capture with no target excitation to be the dominant process for both C 6+ projectiles at a velocity of 0.8 atomic units and Ar 11+ projectiles at v 0.63 a.u. Double electron capture and transfer excitation, however, were found to be comparable and occur about 30% of the time relative to single capture. Most projectiles (96%) auto-ionize quickly following double capture into doubly excited states. The data are compared to classical and quantum mechanical model calculations

  11. QED in highly-charged high Z ions - experiments at the storage ring ESR

    International Nuclear Information System (INIS)

    Mokler, P.H.

    1996-01-01

    A survey on the fundamental structure aspects of very heavy few -electron ions, in particular H-like systems, is presented. Special emphasis is given to contribution from quantum-electro-dynamics at strong central potentials. The technical possibilities to produce highly-charged heavy ions are reviewed and the ground-state Lamb-shift experiments performed at the heavy ion storage ring ESR are summarized. A short outlook on further developments in this field is added. (author). 23 refs, 9 figs

  12. Particle emission induced by the interaction of highly charged slow Xe-ions with a SiO2 surface

    International Nuclear Information System (INIS)

    Schiwietz, G.; Skogvall, B.; Schneider, D.; Clark, M.; DeWitt, D.; McDonald, J.

    1991-01-01

    Sputtering of surface atoms by low energy (a few keV) heavy ions is a commonly used technique in material science and applied physics. In general, sputtering occurs via nuclear energy transfer processes and is determined mainly by the atom-atom interaction potentials. In the energy range of interest these potentials depend only slightly on the charge state of one collision partner if the other is neutral. The development of new ion-sources, however, allows for the use of ions with charged states of q > 50. For these highly charged ions it is conceivable that electronic processes come into play as well. If, for example, the density of charged surface atoms exceeds a certain limit, then particle emission can occur via the electrostatic repulsion of target atoms, the so-called Coulomb explosion. Indications for such electronic effects have been found in a few investigations of ion-induced sputtering Si (q q+ ). However, the order of magnitude of this effect is not clear until now. In this work we present preliminary data on sputtering, ion backscattering, electron and photon emission from SiO 2 surface induced by incident Xe ions of very high charge states (q=30--50). The experiment was performed at the electron beam ion trap (EBIT) of the Lawrence Livermore National Laboratory using a time-of-flight (TOF) ion analyzer-system from the Hahn-Meitner-Institute, Berlin

  13. Production of High-Intensity, Highly Charged Ions

    CERN Document Server

    Gammino, S.

    2013-12-16

    In the past three decades, the development of nuclear physics facilities for fundamental and applied science purposes has required an increasing current of multicharged ion beams. Multiple ionization implies the formation of dense and energetic plasmas, which, in turn, requires specific plasma trapping configurations. Two types of ion source have been able to produce very high charge states in a reliable and reproducible way: electron beam ion sources (EBIS) and electron cyclotron resonance ion sources (ECRIS). Multiple ionization is also obtained in laser-generated plasmas (laser ion sources (LIS)), where the high-energy electrons and the extremely high electron density allow step-by-step ionization, but the reproducibility is poor. This chapter discusses the atomic physics background at the basis of the production of highly charged ions and describes the scientific and technological features of the most advanced ion sources. Particular attention is paid to ECRIS and the latest developments, since they now r...

  14. Techniques and mechanisms applied in electron cyclotron resonance sources for highly charged ions

    NARCIS (Netherlands)

    Drentje, AG

    Electron cyclotron resonance ion sources are delivering beams of highly charged ions for a wide range of applications in many laboratories. For more than two decades, the development of these ion sources has been to a large extent an intuitive and experimental enterprise. Much effort has been spent

  15. Between atomic and nuclear physics: radioactive decays of highly-charged ions

    International Nuclear Information System (INIS)

    Atanasov, Dinko; Bosch, Fritz; Brandau, Carsten; Chen, Xiangcheng; Dillmann, Iris; Gao, Bingshui; Geissel, Hans; Hagmann, Siegbert; Hillenbrand, Pierre-Michel; Kozhuharov, Christophor; Litvinov, Sergey A; Litvinov, Yuri A; Münzenberg, Gottfried; Blaum, Klaus; Bühler, Paul; Faestermann, Thomas; Gernhäuser, Roman; Izumikawa, Takuji; Kurcewicz, Jan; Ma, Xinwen

    2015-01-01

    Highly charged radioactive ions can be stored for extended periods of time in storage rings which allows for precision measurements of their decay modes. The straightforward motivation for performing such studies is that fully ionised nuclei or few-electron ions can be viewed as clean quantum-mechanical systems, in which the interactions of the many electrons can be either excluded or treated precisely. Thus, the influence of the electron shell on the decay probability can be investigated. Another important motivation is stellar nucleosynthesis, which proceeds at high temperatures and the involved atoms are therefore highly ionised. Presented here is a compact review of the relevant experiments conducted at heavy-ion storage rings. Furthermore, we outline the perspectives for future experiments at new-generation storage-ring facilities. (paper)

  16. Electron stereodynamics in coulomb explosion of molecules by slow highly charged ions

    International Nuclear Information System (INIS)

    Ichimura, Atsushi; Ohyama-Yamaguchi, Tomoko

    2008-01-01

    The three-center Coulombic over-the-barrier model is developed for Coulomb explosion of a homonuclear diatomic molecule in collisions with a slow (∼10 eV/amu) highly charged ion. A conventional two-step picture of multiple electron transfer followed by Coulomb explosion is far from appropriate because the molecule sets out to dissociate before the incident ion approaches the closest distance. We treat the formation of a quasi-molecule and its decay into the three moving atomic ions. Charge-asymmetric population between fragment ions observed in a triple-coincidence measurement is suggested to reflect the bond elongation during a collision. Collisions of Kr 8+ + N 2 are analyzed. (author)

  17. ECRIS sources for highly charged ions

    International Nuclear Information System (INIS)

    Geller, R.

    1991-01-01

    The so-called Philips ionization gauge ion sources (PIGIS) were used until quite recently in heavy ion accelerators so multiply charged ions could only be obtained by incorporating a stripper to remove electrons. Electron cyclotron resonance ion sources (ECRIS) now dominate as they produce more highly charged ions. (orig.)

  18. Electron-emission processes in highly charged Ar and Xe ions impinging on highly ordered pyrolytic graphite at energies just above the kinetic threshold

    NARCIS (Netherlands)

    Bodewits, E.; Hoekstra, R.; Dobes, K.; Aumayr, F.

    2014-01-01

    At keV energies, many electronic processes contribute to the emission of secondary electrons in the interaction of highly charged ions on surfaces. To unravel contributions resulting from isolated hollow atoms in front of the surface or embedded in the electron gas of the target, heavy highly

  19. Evaporative cooling of highly charged ions in EBIT [Electron Beam Ion Trap]: An experimental realization

    International Nuclear Information System (INIS)

    Schneider, M.B.; Levine, M.A.; Bennett, C.L.; Henderson, J.R.; Knapp, D.A.; Marrs, R.E.

    1988-01-01

    Both the total number and trapping lifetime of near-neon-like gold ions held in an electron beam ion trap have been greatly increased by a process of 'evaporative cooling'. A continuous flow of low-charge-state ions into the trap cools the high-charge-state ions in the trap. Preliminary experimental results using titanium ions as a coolant are presented. 8 refs., 6 figs., 2 tabs

  20. Extreme ultra-violet emission spectroscopy of highly charged gadolinium ions with an electron beam ion trap

    International Nuclear Information System (INIS)

    Ohashi, Hayato; Nakamura, Nobuyuki; Sakaue, Hiroyuki A

    2013-01-01

    We present extreme ultra-violet emission spectra of highly charged gadolinium ions obtained with an electron beam ion trap at electron energies of 0.53–1.51 keV. The electron energy dependence of the spectra in the 5.7–11.3 nm range is compared with calculation with the flexible atomic code. (paper)

  1. Charged vortices in high-Tc superconductors

    International Nuclear Information System (INIS)

    Matsuda, Y.; Kumagai, K.

    2002-01-01

    It is well known that a vortex in type II superconductors traps a magnetic flux. Recently the possibility that a vortex can accumulate a finite electric charge as well has come to be realized. The sign and magnitude of the vortex charge not only is closely related to the microscopic electronic structure of the vortex, but also strongly affects the dynamical properties of the vortex. In this chapter we demonstrate that a vortex in high-T c superconductors (HTSC) indeed traps a finite electronic charge, using the high resolution measurements of the nuclear quadrupole frequencies. We then discuss the vortex Hall anomaly whose relation with the vortex charging effect has recently received considerable attention. We show that the sign of the trapped charge is opposite to the sign predicted by the conventional BCS theory and deviation of the magnitude of the charge from the theory is also significant. We also show that the electronic structure of underlying system is responsible for the Hall sign in the vortex state and again the Hall sign is opposite to the sign predicted by the BCS theory. It appears that these unexpected features observed in both electrostatics and dynamics of the vortex may be attributed to the novel electronic structure of the vortex in HTSC. (orig.)

  2. Paraxial charge compensator for electron cryomicroscopy

    International Nuclear Information System (INIS)

    Berriman, John A.; Rosenthal, Peter B.

    2012-01-01

    We describe a multi-hole condenser aperture for the production of several electron beams in the transmission electron microscope (TEM) making it possible to simultaneously image and irradiate spatially separated regions of a specimen. When the specimen is a thin film of vitreous ice suspended over a holey carbon film, simultaneous irradiation of the adjacent carbon support with the off-axis beam compensates for some of the effects of charging in the image formed by a beam irradiating only the ice. Because the intervening region is not irradiated, charge-neutralization of frozen-hydrated specimens can occur by a through-space mechanism such as the emission of secondary electrons from a grounded carbon support film. We use paraxial charge compensation (PCC) to control the amount of charge build-up on the specimen and observe the effects of charge on images. The multi-hole aperture thus provides a tool for investigating the mechanism of charging and charge mitigation during the imaging of radiation sensitive biological specimens by cryomicroscopy. -- Highlights: ► A multi-hole condenser aperture produces multiple (paraxial) beams in TEM. ► Paraxial charge compensation is used to study electron-optical effects of charging. ► Emission of secondary electrons controls charging by a through space mechanism. ► Paraxial beams compensate for charging effects in frozen-hydrated specimens.

  3. Paraxial charge compensator for electron cryomicroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Berriman, John A. [Division of Physical Biochemistry, MRC National Institute for Medical Research, The Ridgeway, Mill Hill, London, NW7 1AA (United Kingdom); Rosenthal, Peter B., E-mail: peter.rosenthal@nimr.mrc.ac.uk [Division of Physical Biochemistry, MRC National Institute for Medical Research, The Ridgeway, Mill Hill, London, NW7 1AA (United Kingdom)

    2012-05-15

    We describe a multi-hole condenser aperture for the production of several electron beams in the transmission electron microscope (TEM) making it possible to simultaneously image and irradiate spatially separated regions of a specimen. When the specimen is a thin film of vitreous ice suspended over a holey carbon film, simultaneous irradiation of the adjacent carbon support with the off-axis beam compensates for some of the effects of charging in the image formed by a beam irradiating only the ice. Because the intervening region is not irradiated, charge-neutralization of frozen-hydrated specimens can occur by a through-space mechanism such as the emission of secondary electrons from a grounded carbon support film. We use paraxial charge compensation (PCC) to control the amount of charge build-up on the specimen and observe the effects of charge on images. The multi-hole aperture thus provides a tool for investigating the mechanism of charging and charge mitigation during the imaging of radiation sensitive biological specimens by cryomicroscopy. -- Highlights: Black-Right-Pointing-Pointer A multi-hole condenser aperture produces multiple (paraxial) beams in TEM. Black-Right-Pointing-Pointer Paraxial charge compensation is used to study electron-optical effects of charging. Black-Right-Pointing-Pointer Emission of secondary electrons controls charging by a through space mechanism. Black-Right-Pointing-Pointer Paraxial beams compensate for charging effects in frozen-hydrated specimens.

  4. Impact of measuring electron tracks in high-resolution scientific charge-coupled devices within Compton imaging systems

    International Nuclear Information System (INIS)

    Chivers, D.H.; Coffer, A.; Plimley, B.; Vetter, K.

    2011-01-01

    We have implemented benchmarked models to determine the gain in sensitivity of electron-tracking based Compton imaging relative to conventional Compton imaging by the use of high-resolution scientific charge-coupled devices (CCD). These models are based on the recently demonstrated ability of electron-tracking based Compton imaging by using fully depleted scientific CCDs. Here we evaluate the gain in sensitivity by employing Monte Carlo simulations in combination with advanced charge transport models to calculate two-dimensional charge distributions corresponding to experimentally obtained tracks. In order to reconstruct the angle of the incident γ-ray, a trajectory determination algorithm was used on each track and integrated into a back-projection routine utilizing a geodesic-vertex ray tracing technique. Analysis was performed for incident γ-ray energies of 662 keV and results show an increase in sensitivity consistent with tracking of the Compton electron to approximately ±30 o .

  5. Polarization effects in radiative recombination of an electron with a highly charged ion

    International Nuclear Information System (INIS)

    Klasnikov, A.E.; Shabaev, V.M.; Artemyev, A.N.; Kovtun, A.V.; Stoehlker, T.

    2005-01-01

    The radiative recombination of an unpolarized electron with a polarized highly charged H-like ion in its ground state is studied. The absolute and relative values of the electron spin-flip contribution to the cross section of the process for various scattering angles and photon polarizations are calculated. It is shown that, in addition to the forward and backward directions, there are some other scattering angles of the emitted photon, where, at a fixed linear photon polarization, the spin-flip transition gives a dominant contribution to the differential cross section

  6. Inherent Electrochemistry and Charge Transfer Properties of Few-Layer Two Dimensional Ti3C2Tx MXene

    KAUST Repository

    Nayak, Pranati

    2018-05-25

    We report the effect of Ti3C2Tx MXene flake thickness on its inherent electrochemistry and heterogeneous charge transfer characteristics. It is shown that the Ti3C2Tx undergoes irreversible oxidation in the positive potential window, which strongly depends on the flake thickness and pH of the electrolyte. Few-layer Ti3C2Tx exhibits faster electron transfer kinetics (k0=0.09533 cm/s) with Fe(CN)64−/3− redox mediator compared to multi-layer Ti3C2Tx (k0= 0.00503 cm/s). In addition, few-layer free standing Ti3C2Tx film electrode remains intact after enduring irreversible oxidation.

  7. Inherent Electrochemistry and Charge Transfer Properties of Few-Layer Two Dimensional Ti3C2Tx MXene

    KAUST Repository

    Nayak, Pranati; Jiang, Qiu; Mohanraman, Rajeshkumar; Anjum, Dalaver H.; Hedhili, Mohamed N.; Alshareef, Husam N.

    2018-01-01

    We report the effect of Ti3C2Tx MXene flake thickness on its inherent electrochemistry and heterogeneous charge transfer characteristics. It is shown that the Ti3C2Tx undergoes irreversible oxidation in the positive potential window, which strongly depends on the flake thickness and pH of the electrolyte. Few-layer Ti3C2Tx exhibits faster electron transfer kinetics (k0=0.09533 cm/s) with Fe(CN)64−/3− redox mediator compared to multi-layer Ti3C2Tx (k0= 0.00503 cm/s). In addition, few-layer free standing Ti3C2Tx film electrode remains intact after enduring irreversible oxidation.

  8. Relativistic quantum dynamics in strong fields: Photon emission from heavy, few-electron ions

    International Nuclear Information System (INIS)

    Fritzsche, S.; Stoehlker, T.

    2005-03-01

    Recent progress in the study of the photon emission from highly-charged heavy ions is reviewed. These investigations show that high-Z ions provide a unique tool for improving the understanding of the electron-electron and electron-photon interaction in the presence of strong fields. Apart from the bound-state transitions, which are accurately described in the framework of quantum electrodynamics, much information has been obtained also from the radiative capture of (quasi-) free electrons by high-Z ions. Many features in the observed spectra hereby confirm the inherently relativistic behavior of even the simplest compound quantum systems in nature. (orig.)

  9. Space Charge Effect in the Sheet and Solid Electron Beam

    Science.gov (United States)

    Song, Ho Young; Kim, Hyoung Suk; Ahn, Saeyoung

    1998-11-01

    We analyze the space charge effect of two different types of electron beam ; sheet and solid electron beam. Electron gun simulations are carried out using shadow and control grids for high and low perveance. Rectangular and cylindrical geometries are used for sheet and solid electron beam in planar and disk type cathode. The E-gun code is used to study the limiting current and space charge loading in each geometries.

  10. Measurements of Lunar Dust Charging Properties by Electron Impact

    Science.gov (United States)

    Abbas, Mian M.; Tankosic, Dragana; Craven, Paul D.; Schneider, Todd A.; Vaughn, Jason A.; LeClair, Andre; Spann, James F.; Norwood, Joseph K.

    2009-01-01

    Dust grains in the lunar environment are believed to be electrostatically charged predominantly by photoelectric emissions resulting from solar UV radiation on the dayside, and on the nightside by interaction with electrons in the solar wind plasma. In the high vacuum environment on the lunar surface with virtually no atmosphere, the positive and negative charge states of micron/submicron dust grains lead to some unusual physical and dynamical dust phenomena. Knowledge of the electrostatic charging properties of dust grains in the lunar environment is required for addressing their hazardous effect on the humans and mechanical systems. It is well recognized that the charging properties of individual small micron size dust grains are substantially different from the measurements on bulk materials. In this paper we present the results of measurements on charging of individual Apollo 11 and Apollo 17 dust grains by exposing them to mono-energetic electron beams in the 10-100 eV energy range. The charging/discharging rates of positively and negatively charged particles of approx. 0.1 to 5 micron radii are discussed in terms of the sticking efficiencies and secondary electron yields. The secondary electron emission process is found to be a complex and effective charging/discharging mechanism for incident electron energies as low as 10-25 eV, with a strong dependence on particle size. Implications of the laboratory measurements on the nature of dust grain charging in the lunar environment are discussed.

  11. Supersonic micro-jets and their application to few-cycle laser-driven electron acceleration

    International Nuclear Information System (INIS)

    Schmid, Karl

    2009-01-01

    This thesis covers the few-cycle laser-driven acceleration of electrons in a laser-generated plasma. The laser system employed in this work is a new development based on optical parametric chirped pulse amplification and is the only multi-TW few-cycle laser in the world. In the experiment, the laser beam is focused onto a supersonic helium gas jet which leads to the formation of a plasma channel. The laser pulse, having an intensity of 10 19 W/cm 2 propagates through the plasma with an electron density of 2 x 10 19 cm -3 and forms via a highly nonlinear interaction a strongly anharmonic plasma wave. The amplitude of the wave is so large that the wave breaks, thereby injecting electrons from the background plasma into the accelerating phase. The energy transfer from the laser pulse to the plasma is so strong that the maximum propagation distance is limited to the 100 m range. Therefore, gas jets specifically tuned to these requirements have to be employed. The properties of microscopic supersonic gas jets are thoroughly analyzed in this work. Based on numeric flow simulation, this study encompasses several extensive parameter studies that illuminate all relevant features of supersonic flows in microscopic gas nozzles. This allowed the optimized design of de Laval nozzles with exit diameters ranging from 150 μm to 3 mm. The employment of these nozzles in the experiment greatly improved the electron beam quality. After these optimizations, the laser-driven electron accelerator now yields monoenergetic electron pulses with energies up to 50 MeV and charges between one and ten pC. The electron beam has a typical divergence of 5 mrad and comprises an energy spectrum that is virtually free from low energetic background. The electron pulse duration could not yet be determined experimentally but simulations point towards values in the range of 1 fs. The acceleration gradient is estimated from simulation and experiment to be approximately 0.5 TV/m. The electron accelerator

  12. Supersonic micro-jets and their application to few-cycle laser-driven electron acceleration

    Energy Technology Data Exchange (ETDEWEB)

    Schmid, Karl

    2009-07-23

    This thesis covers the few-cycle laser-driven acceleration of electrons in a laser-generated plasma. The laser system employed in this work is a new development based on optical parametric chirped pulse amplification and is the only multi-TW few-cycle laser in the world. In the experiment, the laser beam is focused onto a supersonic helium gas jet which leads to the formation of a plasma channel. The laser pulse, having an intensity of 10{sup 19} W/cm{sup 2} propagates through the plasma with an electron density of 2 x 10{sup 19} cm{sup -3} and forms via a highly nonlinear interaction a strongly anharmonic plasma wave. The amplitude of the wave is so large that the wave breaks, thereby injecting electrons from the background plasma into the accelerating phase. The energy transfer from the laser pulse to the plasma is so strong that the maximum propagation distance is limited to the 100 m range. Therefore, gas jets specifically tuned to these requirements have to be employed. The properties of microscopic supersonic gas jets are thoroughly analyzed in this work. Based on numeric flow simulation, this study encompasses several extensive parameter studies that illuminate all relevant features of supersonic flows in microscopic gas nozzles. This allowed the optimized design of de Laval nozzles with exit diameters ranging from 150 {mu}m to 3 mm. The employment of these nozzles in the experiment greatly improved the electron beam quality. After these optimizations, the laser-driven electron accelerator now yields monoenergetic electron pulses with energies up to 50 MeV and charges between one and ten pC. The electron beam has a typical divergence of 5 mrad and comprises an energy spectrum that is virtually free from low energetic background. The electron pulse duration could not yet be determined experimentally but simulations point towards values in the range of 1 fs. The acceleration gradient is estimated from simulation and experiment to be approximately 0.5 TV/m. The

  13. Techniques for enhancing the performance of high charge state ECR ion sources

    International Nuclear Information System (INIS)

    Xie, Z.Q.

    1999-01-01

    Electron Cyclotron Resonance ion source (ECRIS), which produces singly to highly charged ions, is widely used in heavy ion accelerators and is finding applications in industry. It has progressed significantly in recent years thanks to a few techniques, such as multiple-frequency plasma heating, higher mirror magnetic fields and a better cold electron donor. These techniques greatly enhance the production of highly charged ions. More than 1 emA of He 2+ and O 6+ , hundreds of eμA of O 7+ , Ne 8+ , Ar 12+ , more than 100 eμA of intermediate heavy ions with charge states up to Ne 9+ , Ar 13+ , Ca 13+ , Fe 13+ , Co 14+ and Kr 18+ , tens of eμA of heavy ions with charge states up to Xe 28+ , Au 35+ , Bi 34+ and U 34+ were produced at cw mode operation. At an intensity of about 1 eμA, the charge states for the heavy ions increased up to Xe 36+ , Au 46+ , Bi 47+ and U 48+ . More than an order of magnitude enhancement of fully stripped argon ions was achieved (I≥0.1 and h;eμA). Higher charge state ions up to Kr 35+ , Xe 46+ and U 64+ at low intensities were produced for the first time from an ECRIS. copyright 1999 American Institute of Physics

  14. Production of microbunched beams of very highly charged ions with an electron beam ion source

    International Nuclear Information System (INIS)

    Stoeckli, M.P.

    1998-01-01

    Electron beam ion sources produce very highly charged ions most efficiently in a batch mode as the confinement time can be directly optimized for the production of the desired charge state. If, after confinement, the voltage of the ion-confining downstream dam is lowered rapidly, all ions escape and form an ion beam pulse with a length of a few tens of μs. Raising the main trap voltage while maintaining a constant dam voltage in a open-quotes spill-over expulsionclose quotes reduces the energy spread of the expelled ions. The longer time periods of open-quotes slow-,close quotes open-quotes leaky batch mode-,close quotes and open-quotes direct current (dc) batch mode-close quotes expulsions allow for increasing the ion beam duty cycle. Combining the rapid expulsion with one of the latter methods allows for the expulsion of the ions of a single batch in many small microbunches with variable intervals, maintaining the low energy spread and the increased duty cycle of slow expulsions. Combining the open-quotes microbunchingclose quotes with open-quotes dc batch mode productionclose quotes and a multitrap operation will eventually allow for the production of equally intense ion bunches over a wide range of frequencies without any deadtime, and with minimal compromise on the most efficient production parameters. copyright 1998 American Institute of Physics

  15. Determination of the charge radii of several light nuclei from precision, high-energy electron elastic scattering

    Energy Technology Data Exchange (ETDEWEB)

    Kabir, Al Amin [Kent State Univ., Kent, OH (United States)

    2015-12-01

    Analysis of high-energy electron scattering has been used to determine the charge radii of nuclei for several decades. Recent analysis of the Lamb shift in muonic hydrogen found an r.m.s. radius significantly different than the electron scattering result. To understand this puzzle we have analyzed the "LEDEX" data for the (e, e'p) reaction. This experiment includes measurements on several light nuclei, hydrogen, deuterium, lithium, boron, and carbon. To test our ability to measure absolute cross sections, as well as our ability to extract the charge radius, we tested our technique against the extremely well-measured carbon case and found excellent agreement using the Fourier-Bessel parametrization. We then extended the procedure to boron and lithium, which show nice agreement with the latest theoretical calculations. For hydrogen, we see clearly the limits of this technique and therefore, the charge radius is determined from the traditional extrapolation to q2 = 0. We will show that there is a model dependence in extracting the charge radius of hydrogen and its unambiguous determination is very difficult with available electron-scattering measurements.

  16. Precision laser spectroscopy of highly charged ions

    International Nuclear Information System (INIS)

    Kuehl, T.; Borneis, S.; Becker, S.; Dax, A.; Engel, T.; Grieser, R.; Huber, G.; Klaft, I.; Klepper, O.; Kohl, A.; Marx, D.; Meier, K.; Neumann, R.; Schmitt, F.; Seelig, P.; Voelker, L.

    1996-01-01

    Recently, intense beams of highly charged ions have become available at heavy ion cooler rings. The obstacle for producing these highly interesting candidates is the large binding energy of K-shell electrons in heavy systems in excess of 100 keV. One way to remove these electrons is to strip them off by passing the ion through material. In the cooler ring, the ions are cooled to a well defined velocity. At the SIS/ESR complex it is possible to produce, store, and cool highly charged ions up to bare uranium with intensities exceeding 10 8 atoms in the ring. This opens the door for precision laser spectroscopy of hydrogenlike-heavy ions, e.g. 209 Bi 82+ , and allows to examine the interaction of the single electron with the large fields of the heavy nucleus, exceeding any artificially produced electric and magnetic fields by orders of magnitude. In the electron cooler the interaction of electrons and highly charged ions otherwise only present in the hottest plasmas can be studied. (orig.)

  17. Doping dependence of charge order in electron-doped cuprate superconductors

    Science.gov (United States)

    Mou, Yingping; Feng, Shiping

    2017-12-01

    In the recent studies of the unconventional physics in cuprate superconductors, one of the central issues is the interplay between charge order and superconductivity. Here the mechanism of the charge-order formation in the electron-doped cuprate superconductors is investigated based on the t-J model. The experimentally observed momentum dependence of the electron quasiparticle scattering rate is qualitatively reproduced, where the scattering rate is highly anisotropic in momentum space, and is intriguingly related to the charge-order gap. Although the scattering strength appears to be weakest at the hot spots, the scattering in the antinodal region is stronger than that in the nodal region, which leads to the original electron Fermi surface is broken up into the Fermi pockets and their coexistence with the Fermi arcs located around the nodal region. In particular, this electron Fermi surface instability drives the charge-order correlation, with the charge-order wave vector that matches well with the wave vector connecting the hot spots, as the charge-order correlation in the hole-doped counterparts. However, in a striking contrast to the hole-doped case, the charge-order wave vector in the electron-doped side increases in magnitude with the electron doping. The theory also shows the existence of a quantitative link between the single-electron fermiology and the collective response of the electron density.

  18. Charge spill-out and work function of few-layer graphene on SiC(0 0 0 1)

    International Nuclear Information System (INIS)

    Renault, O; Rotella, H; Kaja, K; Blaise, P; Poiroux, T; Pascon, A M; Fonseca, L R C; Mathieu, C; Rault, J E; Barrett, N

    2014-01-01

    We report on the charge spill-out and work function of epitaxial few-layer graphene on 6 H-SiC(0 0 0 1). Experiments from high-resolution, energy-filtered x-ray photoelectron emission microscopy (XPEEM) are combined with ab initio density functional theory calculations using a relaxed interface model. The work function values obtained from theory and experiments are in qualitative agreement, reproducing the previously observed trend of increasing work function with each additional graphene plane. Electron transfer at the SiC/graphene interface through a buffer layer (BL) causes an interface dipole moment which is at the origin of the graphene work function modulation. The total charge transfer is independent of the number of graphene layers, and is consistent with the constant binding energy of the SiC component of the C 1s core-level, measured by XPEEM. Charge leakage into a vacuum depends on the number of graphene layers, explaining why the experimental, layer-dependent C 1s graphene core-level binding energy shift does not rigidly follow that of the work function. Thus, a combination of charge transfer at the SiC/graphene interface and charge spill-out into the vacuum resolves the apparent discrepancy between the experimental work function and C 1s binding energy. (paper)

  19. Production processes of multiply charged ions by electron impact

    International Nuclear Information System (INIS)

    Oda, Nobuo

    1980-02-01

    First, are compared the foil or gas stripper and the ion sources utilizing electron-atom ionizing collisions, which are practically used or are under development to produce multiply charged ions. A review is made of the fundamental physical parameters such as successive ionization potentials and various ionization cross sections by electron impact, as well as the primary processes in multiply charged ion production. Multiply charged ion production processes are described for the different existing ion sources such as high temperature plasma type, ion-trapping type and discharge type. (author)

  20. Beamline for low-energy transport of highly charged ions at HITRAP

    International Nuclear Information System (INIS)

    Andelkovic, Z.; Herfurth, F.; Kotovskiy, N.; König, K.; Maaß, B.; Murböck, T.; Neidherr, D.; Schmidt, S.; Steinmann, J.; Vogel, M.; Vorobjev, G.

    2015-01-01

    A beamline for transport of highly charged ions with energies as low as a few keV/charge has been constructed and commissioned at GSI. Complementary to the existing infrastructure of the HITRAP facility for deceleration of highly charged ions from the GSI accelerator, the new beamline connects the HITRAP ion decelerator and an EBIT with the associated experimental setups. Therefore, the facility can now transport the decelerated heavy highly charged ions to the experiments or supply them offline with medium-heavy highly charged ions from the EBIT, both at energies as low as a few keV/charge. Here we present the design of the 20 m long beamline with the corresponding beam instrumentation, as well as its performance in terms of energy and transport efficiency

  1. Experiments on ion space-charge neutralization with pulsed electron beams

    Energy Technology Data Exchange (ETDEWEB)

    Herleb, U; Riege, H [CERN LHC-Division, Geneva (Switzerland)

    1997-12-31

    The method of space-charge neutralization of heavy ion beams with electron beam pulses generated with electron guns incorporating ferroelectric cathodes was investigated experimentally. Several experiments are described, the results of which prove that the intensity of selected ion beam parts with defined charge states generated in a laser ion source can be increased by an order of magnitude. For elevated charge states the intensity amplification is more significant and may reach a factor of 4 for highly charged ions from an Al target. (author). 7 figs., 3 -refs.

  2. Intense highly charged ion beam production and operation with a superconducting electron cyclotron resonance ion source

    Science.gov (United States)

    Zhao, H. W.; Sun, L. T.; Guo, J. W.; Lu, W.; Xie, D. Z.; Hitz, D.; Zhang, X. Z.; Yang, Y.

    2017-09-01

    The superconducting electron cyclotron resonance ion source with advanced design in Lanzhou (SECRAL) is a superconducting-magnet-based electron cyclotron resonance ion source (ECRIS) for the production of intense highly charged heavy ion beams. It is one of the best performing ECRISs worldwide and the first superconducting ECRIS built with an innovative magnet to generate a high strength minimum-B field for operation with heating microwaves up to 24-28 GHz. Since its commissioning in 2005, SECRAL has so far produced a good number of continuous wave intensity records of highly charged ion beams, in which recently the beam intensities of 40Ar+ and 129Xe26+ have, for the first time, exceeded 1 emA produced by an ion source. Routine operations commenced in 2007 with the Heavy Ion accelerator Research Facility in Lanzhou (HIRFL), China. Up to June 2017, SECRAL has been providing more than 28,000 hours of highly charged heavy ion beams to the accelerator demonstrating its great capability and reliability. The great achievement of SECRAL is accumulation of numerous technical advancements, such as an innovative magnetic system and an efficient double-frequency (24 +18 GHz ) heating with improved plasma stability. This article reviews the development of SECRAL and production of intense highly charged ion beams by SECRAL focusing on its unique magnet design, source commissioning, performance studies and enhancements, beam quality and long-term operation. SECRAL development and its performance studies representatively reflect the achievements and status of the present ECR ion source, as well as the ECRIS impacts on HIRFL.

  3. Electron loss from hydrogen-like highly charged ions in collisions with electrons, protons and light atoms

    Science.gov (United States)

    Lyashchenko, K. N.; Andreev, O. Yu; Voitkiv, A. B.

    2018-03-01

    We consider electron loss from a hydrogen-like highly charged ion (HCI) in relativistic collisions with hydrogen and helium in the range of impact velocities v min ≤ v ≤ v max (v min and v max correspond to the threshold energy ε th for electron loss in collisions with a free electron and to ≈5 ε th, respectively) where any reliable data for loss cross sections are absent. In this range, where the loss process is characterized by large momentum transfers, we express it in terms of electron loss in collisions with equivelocity protons and electrons and explore by performing a detailed comparative study of these subprocesses. Our results, in particular, show that: (i) compared to equivelocity electrons protons are more effective in inducing electron loss, (ii) the relative effectiveness of electron projectiles grows with increase in the atomic number of a HCI, (iii) collisions with protons and electrons lead to a qualitatively different population of the final-state-electron momentum space and even when the total loss cross sections in these collisions become already equal the spectra of the outgoing electrons still remain quite different in almost the entire volume of the final-state-electron momentum space, (iv) in collisions with hydrogen and helium the contributions to the loss process from the interactions with the nucleus and the electron(s) of the atom could be rather well separated in a substantial part of the final-state-electron momentum space.

  4. Production, transport and charge capture measurements of highly charged recoil ions

    International Nuclear Information System (INIS)

    Trebus, U.E.

    1989-01-01

    An experiment is described to study highly charged recoil ions on-line to the heavy accelerator UNILAC at GSI. The highly charged recoil ions are produced by heavy-ion bombardment of a gas target. Subsequently the slow highly charged recoil ions are extracted from the ionization volume, and guided through a beam transport line to a Wien filter for charge state selection and to a collision region to study charge transfer processes. Several experiments were carried out to show the efficient charge state separation. Charge states up to q = 15 were observed. When using a retarding field analyzer cross sections for single electron capture were determined for different charge states of Xe q+ for q = 4 to 11 and He gas. The experiments demonstrated increasing charge transfer cross sections with increasing charge state q and indicated the effect of near resonant charge capture for q = 6. The flexible data acquisition system used, is described and other future experiments, such as for instance in flight ion-trapping are indicated in the appendix

  5. Production, transport and charge capture measurements of highly charged recoil ions

    International Nuclear Information System (INIS)

    Trebus, U.E.

    1989-05-01

    An experiment is described to study highly charged recoil ions on-line to the heavy ion accelerator UNILAC at GSI. The highly charged recoil ions are produced by heavy ion bombardment of a gas target. Subsequently the slow highly charged recoil ions are extracted from the ionization volume, and guided through a beam transport line to a Wien filter for charge state selection and to a collision region to study charge transfer processes. Several experiments were carried out to show the efficient charge state separation. Charge states up to q=15 were observed. When using a retarding field analyzer cross sections for single electron capture were determined for different charge states of Xe q+ for q=4 to 11 and He gas. The experiments demonstrated increasing charge transfer cross sections with increasing charge state q and indicated the effect of near resonant charge capture for q=6. The flexible data acquisition system used, is described and other future experiments, such as for instance in flight ion-trapping are indicated in the appendix. (orig.)

  6. Highly charged atomic physics at HIRFL-CSR

    International Nuclear Information System (INIS)

    Ma Xinwen; Wang Youde; Hou Mingdong; Jin Gengmin

    1996-01-01

    HIRFL-CSR is a proposed electron cooling storage ring optimized to accelerate and store beams of highly charged heavy ions. Several possibilities for advanced atomic physics studies are discussed, such as studies of electron-ion, ion-atoms, photon-ion-electron interactions and high resolution spectroscopy

  7. Highly charged ions trapping for lifetime measurements; Piegeage d'ions tres charges pour la mesure de duree de vie d'etats metastables

    Energy Technology Data Exchange (ETDEWEB)

    Attia, D

    2007-10-15

    A new experimental setup dedicated to highly charged ion trapping is presented in this work. The final goal is to perform lifetime measurement of metastable states produced by our ECR (Electron Cyclotron Resonance) ion source. Lifetimes to be measured are in the range of a few ms and more. We have measured the lifetimes of the M1 transitions of the metastable states of Ar{sup 9+}, Ar{sup 13+} and Ar{sup 14+}. These measurements are useful to test the N-body problem in the relativistic range. The trap we have built, was designed a few years ago at the Weizman Institute in Israel, it allows ions with an energy of several keV to be trapped for lifetimes of about 1 second. This trap was originally designed to study the dynamics of excited molecules. We have shown for the first time how the trap operates and that it can operate with highly charged ions. We have studied the beam dynamics of highly charged ions and the trap has been tested with various species of ions and different charge states: from O{sup +} to O{sup 6+}, from Ar{sup 8+} to Ar{sup 13+}, and from Kr{sup 13+} to Kr{sup 20+}.

  8. Charged particle measurements from a rocket-borne electron accelerator experiment

    International Nuclear Information System (INIS)

    Duprat, G.R.J.; McNamara, A.G.; Whalen, B.A.

    1982-01-01

    This chapter presents charged particle observations which relate to the spatial distribution of energetic (keV) charged particles surrounding the accelerator during gun firings, the energy distribution of energetic electrons produced in the plasma by the electron beam, and the dependence of these characteristics on the beam energy, current, and injection angle. The primary objective of the flight of the Nike Black Brant rocket (NUB-06) was to use an electron beam to probe the auroral field lines for electric fields parallel to the magnetic field. The secondary objectives were to study electron beam interactions in the ionosphere and spacecraft charging effects. It is demonstrated that during high current (greater than or equal to 10ma electron beam firings, an intense suprathermal as well as energetic electron population is created on flux tubes near the beam. Certain similarities exist between these measurements and corresponding ones made in the Houston vacuum tank suggesting that the same instability observed in the laboratory is occurring at high altitudes in the ionosphere

  9. Beta decay of highly charged ions

    International Nuclear Information System (INIS)

    Litvinov, Yuri A; Bosch, Fritz

    2011-01-01

    Beta decay of highly charged ions has attracted much attention in recent years. An obvious motivation for this research is that stellar nucleosynthesis proceeds at high temperatures where the involved atoms are highly ionized. Another important reason is addressing decays of well-defined quantum-mechanical systems, such as one-electron ions where all interactions with other electrons are excluded. The largest modifications of nuclear half-lives with respect to neutral atoms have been observed in beta decay of highly charged ions. These studies can be performed solely at ion storage rings and ion traps, because there high atomic charge states can be preserved for extended periods of time (up to several hours). Currently, all experimental results available in this field originate from experiments at the heavy-ion complex GSI in Darmstadt. There, the fragment separator facility FRS allows the production and separation of exotic, highly charged nuclides, which can then be stored and investigated in the storage ring facility ESR. In this review, we present and discuss in particular two-body beta decays, namely bound-state beta decay and orbital electron capture. Although we focus on experiments conducted at GSI, we will also attempt to provide general requirements common to any other experiment in this context. Finally, we address challenging but not yet performed experiments and we give prospects for the new radioactive beam facilities, such as FAIR in Darmstadt, IMP in Lanzhou and RIKEN in Wako.

  10. Electron beam charge state amplifier (EBQA)--a conceptual evaluation

    International Nuclear Information System (INIS)

    Dooling, J. C.

    1998-01-01

    A concept is presented for stripping low-energy, radioactive ions from 1+ to higher charge states. Referred to as an Electron Beam Charge State Amplifier (EBQA), this device accepts a continuous beam of singly-charged, radioactive ions and passes them through a high-density electron beam confined by a solenoidal magnetic field. Singly-charged ions may be extracted from standard Isotope-Separator-Online (ISOL) sources. An EBQA is potentially useful for increasing the charge state of ions prior to injection into post-acceleration stages at ISOL radioactive beam facilities. The stripping efficiency from q=1+ to 2+ (η 12 ) is evaluated as a function of electron beam radius at constant current with solenoid field, injected ion energy, and ion beam emittance used as parameters. Assuming a 5 keV, 1 A electron beam, η 12 = 0.38 for 0.1 keV, 132 Xe ions passing through an 8 Tesla solenoid, 1 m in length. Multi-pass configurations to achieve 3+ or 4+ charge states are also conceivable. The calculated efficiencies depend inversely on the initial ion beam emittances. The use of a helium-buffer-gas, ion-guide stage to improve the brightness of the 1+ beams [1] may enhance the performance of an EBQA

  11. Untangling the contributions of image charge and laser profile for optimal photoemission of high-brightness electron beams

    International Nuclear Information System (INIS)

    Portman, J.; Zhang, H.; Makino, K.; Ruan, C. Y.; Berz, M.; Duxbury, P. M.

    2014-01-01

    Using our model for the simulation of photoemission of high brightness electron beams, we investigate the virtual cathode physics and the limits to spatio-temporal and spectroscopic resolution originating from the image charge on the surface and from the profile of the exciting laser pulse. By contrasting the effect of varying surface properties (leading to expanding or pinned image charge), laser profiles (Gaussian, uniform, and elliptical), and aspect ratios (pancake- and cigar-like) under different extraction field strengths and numbers of generated electrons, we quantify the effect of these experimental parameters on macroscopic pulse properties such as emittance, brightness (4D and 6D), coherence length, and energy spread. Based on our results, we outline optimal conditions of pulse generation for ultrafast electron microscope systems that take into account constraints on the number of generated electrons and on the required time resolution.

  12. Multipartite electronic entanglement purification with charge detection

    Energy Technology Data Exchange (ETDEWEB)

    Sheng Yubo [Department of Physics, Tsinghua University, Beijing 100084 (China); Deng, Fu-Guo [Department of Physics, Beijing Normal University, Beijing 100875 (China); Long Guilu, E-mail: gllong@tsinghua.edu.c [Department of Physics, Tsinghua University, Beijing 100084 (China); Key Laboratory for Atomic and Molecular NanoSciences, Tsinghua University, Beijing 100084 (China); Tsinghua National Laboratory for Information Science and Technology, Beijing 100084 (China)

    2011-01-17

    We present a multipartite entanglement purification scheme in a Greenberger-Horne-Zeilinger state for electrons based on their spins and their charges. This scheme works for purification with two steps, i.e., bit-flip error correction and phase-flip error correction. By repeating these two steps, the parties in quantum communication can get some high-fidelity multipartite entangled electronic systems.

  13. Electron cooling of highly charged ions in penning traps; Elektronenkuehlung hochgeladener Ionen in Penningfallen

    Energy Technology Data Exchange (ETDEWEB)

    Moellers, B.

    2007-02-08

    For many high precision experiments with highly charged ions in ion traps it is necessary to work with low energy ions. One possibility to slow ions down to a very low energy in a trap is electron cooling, a method, which is already successfully used in storage rings to produce ion beams with high phase space density. Fast ions and a cold electron plasma are inserted into a Penning trap. The ions lose their energy due to Coulomb interaction with the electrons while they cross the plasma, the electrons are heated. The cooling time is the time, which is needed to cool an ion from a given initial energy to a low final energy. To calculate cooling times it is necessary to solve coupled differential equations for the ion energy and electron temperature. In a Penning trap the strong external magnetic field constitutes a theoretical challenge, as it influences the energy loss of the ions in an electron plasma, which can no longer be calculated analytically. In former estimates of cooling times this influence is neglected. But simulations show a dramatic decrease of the energy loss in the presence of a strong magnetic field, so it is necessary to investigate the effect of the magnetic field on the cooling times. This work presents a model to calculate cooling times, which includes both the magnetic field and the trap geometry. In a first step a simplified model without the external trap potential is developed. The energy loss of the ions in the magnetized electron plasma is calculated by an analytic approximation, which requires a numerical solution of integrals. With this model the dependence of the cooling time on different parameters like electron and ion density, magnetic field and the angle between ion velocity and magnetic field is studied for fully ionized uranium. In addition the influence of the electron heating is discussed. Another important topic in this context is the recombination between ions and electrons. The simplified model for cooling times allows to

  14. LUNAR DUST GRAIN CHARGING BY ELECTRON IMPACT: COMPLEX ROLE OF SECONDARY ELECTRON EMISSIONS IN SPACE ENVIRONMENTS

    International Nuclear Information System (INIS)

    Abbas, M. M.; Craven, P. D.; LeClair, A. C.; Spann, J. F.; Tankosic, D.

    2010-01-01

    Dust grains in various astrophysical environments are generally charged electrostatically by photoelectric emissions with radiation from nearby sources, or by electron/ion collisions by sticking or secondary electron emissions (SEEs). The high vacuum environment on the lunar surface leads to some unusual physical and dynamical phenomena involving dust grains with high adhesive characteristics, and levitation and transportation over long distances. Knowledge of the dust grain charges and equilibrium potentials is important for understanding a variety of physical and dynamical processes in the interstellar medium, and heliospheric, interplanetary/planetary, and lunar environments. It has been well recognized that the charging properties of individual micron-/submicron-size dust grains are expected to be substantially different from the corresponding values for bulk materials. In this paper, we present experimental results on the charging of individual 0.2-13 μm size dust grains selected from Apollo 11 and 17 dust samples, and spherical silica particles by exposing them to mono-energetic electron beams in the 10-200 eV energy range. The dust charging process by electron impact involving the SEEs discussed is found to be a complex charging phenomenon with strong particle size dependence. The measurements indicate substantial differences between the polarity and magnitude of the dust charging rates of individual small-size dust grains, and the measurements and model properties of corresponding bulk materials. A more comprehensive plan of measurements of the charging properties of individual dust grains for developing a database for realistic models of dust charging in astrophysical and lunar environments is in progress.

  15. Lunary Dust Grain Charging by Electron Impact: Complex Role of Secondary Electron Emissions in Space Environments

    Science.gov (United States)

    Abbas, M. M.; Tankosic, D.; Crave, P. D.; LeClair, A.; Spann, J. F.

    2010-01-01

    Dust grains in various astrophysical environments are generally charged electrostatically by photoelectric emissions with radiation from nearby sources, or by electron/ion collisions by sticking or secondary electron emissions (SEES). The high vacuum environment on the lunar surface leads to some unusual physical and dynamical phenomena involving dust grains with high adhesive characteristics, and levitation and transportation over long distances. Knowledge of the dust grain charges and equilibrium potentials is important for understanding a variety of physical and dynamical processes in the interstellar medium, and heliospheric, interplanetary/ planetary, and lunar environments. It has been well recognized that the charging properties of individual micron-/submicron-size dust grains are expected to be substantially different from the corresponding values for bulk materials. In this paper, we present experimental results on the charging of individual 0.2-13 m size dust grains selected from Apollo 11 and 17 dust samples, and spherical silica particles by exposing them to mono-energetic electron beams in the 10-200 eV energy range. The dust charging process by electron impact involving the SEES discussed is found to be a complex charging phenomenon with strong particle size dependence. The measurements indicate substantial differences between the polarity and magnitude of the dust charging rates of individual small-size dust grains, and the measurements and model properties of corresponding bulk materials. A more comprehensive plan of measurements of the charging properties of individual dust grains for developing a database for realistic models of dust charging in astrophysical and lunar environments is in progress.

  16. Charge deep-level transient spectroscopy study of high-energy-electron-beam-irradiated hydrogenated amorphous silicon

    NARCIS (Netherlands)

    Klaver, A.; Nádaždy, V.; Zeman, M.; Swaaiij, R.A.C.M.M.

    2006-01-01

    We present a study of changes in the defect density of states in hydrogenated amorphous silicon (a-Si:H) due to high-energy electron irradiation using charged deep-level transient spectroscopy. It was found that defect states near the conduction band were removed, while in other band gap regions the

  17. Direct electron-pair production by high energy heavy charged particles

    Science.gov (United States)

    Takahashi, Y.; Gregory, J. C.; Hayashi, T.; Dong, B. L.

    1989-01-01

    Direct electron pain production via virtual photons by moving charged particles is a unique electro-magnetic process having a substantial dependence on energy. Most electro-magnetic processes, including transition radiation, cease to be sensitive to the incident energy above 10 TeV/AMU. Thus, it is expected, that upon establishment of cross section and detection efficiency of this process, it may provide a new energy measuring technique above 10 TeV/AMU. Three accelerator exposures of emulsion chambers designed for measurements of direct electron-pains were performed. The objectives of the investigation were to provide the fundamental cross-section data in emulsion stacks to find the best-fit theoretical model, and to provide a calibration of measurements of direct electron-pairs in emulsion chamber configurations. This paper reports the design of the emulsion chambers, accelerator experiments, microscope measurements, and related considerations for future improvements of the measurements, and for possible applications to high energy cosmic ray experiments. Also discussed are the results from scanning 56m of emulsion tracks at 1200x magnification so that scanning efficiency is optimized. Measurements of the delta-ray range spectrum were also performed for much shorter track lengths, but with sufficiently large statistics in the number of measured delta-rays.

  18. Intense highly charged ion beam production and operation with a superconducting electron cyclotron resonance ion source

    Directory of Open Access Journals (Sweden)

    H. W. Zhao

    2017-09-01

    Full Text Available The superconducting electron cyclotron resonance ion source with advanced design in Lanzhou (SECRAL is a superconducting-magnet-based electron cyclotron resonance ion source (ECRIS for the production of intense highly charged heavy ion beams. It is one of the best performing ECRISs worldwide and the first superconducting ECRIS built with an innovative magnet to generate a high strength minimum-B field for operation with heating microwaves up to 24–28 GHz. Since its commissioning in 2005, SECRAL has so far produced a good number of continuous wave intensity records of highly charged ion beams, in which recently the beam intensities of ^{40}Ar^{12+} and ^{129}Xe^{26+} have, for the first time, exceeded 1 emA produced by an ion source. Routine operations commenced in 2007 with the Heavy Ion accelerator Research Facility in Lanzhou (HIRFL, China. Up to June 2017, SECRAL has been providing more than 28,000 hours of highly charged heavy ion beams to the accelerator demonstrating its great capability and reliability. The great achievement of SECRAL is accumulation of numerous technical advancements, such as an innovative magnetic system and an efficient double-frequency (24+18  GHz heating with improved plasma stability. This article reviews the development of SECRAL and production of intense highly charged ion beams by SECRAL focusing on its unique magnet design, source commissioning, performance studies and enhancements, beam quality and long-term operation. SECRAL development and its performance studies representatively reflect the achievements and status of the present ECR ion source, as well as the ECRIS impacts on HIRFL.

  19. Charge fluctuations in high-electron-mobility transistors: a review

    International Nuclear Information System (INIS)

    Green, F.

    1993-01-01

    The quasi-two-dimensional carrier population, free to move within a near-perfect crystalline matrix, is the key to remarkable improvements in signal gain, current density and quiet operation. Current-fluctuation effects are central to all of these properties. Some of these are easily understood within linear-response theory, but other fluctuation phenomena are less tractable. In particular, nonequilibrium noise poses significant theoretical challenges, both descriptive and predictive. This paper examines a few of the basic physical issues which motivate device-noise theory. The structure and operation of high-electron-mobility transistor are first reviewed. The recent nonlinear fluctuation theory of Stanton and Wilkins (1987) help to identify at least some of the complicated noise physics which can arise when carriers in GaAs-like conduction bands are subjected to high fields. Simple examples of fluctuation-dominated behaviour are discussed, with numerical illustrations. 20 refs., 9 figs

  20. A Study of Charged Current Single Charged Pion Productions on Carbon in a Few-GeV Neutrino Beam

    Energy Technology Data Exchange (ETDEWEB)

    Hiraide, Katsuki [Kyoto Univ. (Japan)

    2009-01-01

    Understanding single charged pion production via neutrino-nucleus charged current interaction in the neutrino energy region of a few GeV is essential for future neutrino oscillation experiments since this process is a dominant background for vμ → vx oscillation measurements. There are two contributions to this process: single pion production via baryonic resonance (vμN → μ-+) and coherent pion production interacting with the entire nucleus (vμA → μ-+), where N is nucleon in the nucleus and A is the nucleus. The purpose of the study presented in this thesis is a precise measurement of charged current single charged pion productions, resonant and coherent pion productions, with a good final state separation in the neutrino energy region of a few GeV. In this thesis, we focus on the study of charged current coherent pion production from muon neutrinos scattering on carbon, vμ 12C → μ-12+, in the SciBooNE experiment. This is motivated by the fact that without measuring this component first, the precise determination of resonant pion production cross section can not be achieved since the contribution of coherent pion production in the region of small muon scattering angle is not small. Furthermore, the coherent process is particularly interesting because it is deeply rooted in fundamental physics via Adler's partially conserved axial-vector current theorem. We took data from June 2007 until August 2008, in both the neutrino and antineutrino beam. In total, 2.52 x 1020 protons on target were collected. We have performed a search for charged current coherent pion production by using SciBooNE's full neutrino data set, corresponding to 0.99 x 1020 protons on target. No evidence for coherent pion production is observed. We set 90% confidence level upper limits on the cross section ratio

  1. Plasmon-enhanced scattering and charge transfer in few-layer graphene interacting with buried printed 2D-pattern of silver nanoparticles

    Science.gov (United States)

    Carles, R.; Bayle, M.; Bonafos, C.

    2018-04-01

    Hybrid structures combing silver nanoparticles and few-layer graphene have been synthetized by combining low-energy ion beam synthesis and stencil techniques. A single plane of metallic nanoparticles plays the role of an embedded plasmonic enhancer located in dedicated areas at a controlled nanometer distance from deposited graphene layers. Optical imaging, reflectance and Raman scattering mapping are used to measure the enhancement of electronic and vibrational properties of these layers. In particular electronic Raman scattering is shown as notably efficient to analyze the optical transfer of charge carriers between the systems and the presence of intrinsic and extrinsic defects.

  2. Structure and dynamics of highly charged heavy ions studied with the electron beam ion trap in Tokyo

    International Nuclear Information System (INIS)

    Nakamura, Nobuyuki; Hu, Zhimin; Watanabe, Hirofumi; Li, Yueming; Kato, Daiji; Currell, Fred J.; Tong Xiaomin; Watanabe, Tsutomu; Ohtani, Shunsuke

    2011-01-01

    In this paper, we present the structure and the dynamics of highly charged heavy ions studied through dielectronic recombination (DR) observations performed with the Tokyo electron beam ion trap. By measuring the energy dependence of the ion abundance ratio in the trap at equilibrium, we have observed DR processes for open shell systems very clearly. Remarkable relativistic effects due to the generalized Breit interaction have been clearly shown in DR for highly charged heavy ions. We also present the first result for the coincidence measurement of two photons emitted from a single DR event.

  3. The impact of irradiation induced specimen charging on microanalysis in a scanning electron microscope

    International Nuclear Information System (INIS)

    Stevens-Kalceff, M.A.

    2003-01-01

    Full text: It is necessary to assess and characterize the perturbing influences of experimental probes on the specimens under investigation. The significant influence of electron beam irradiation on poorly conducting materials has been assessed by a combination of specialized analytical scanning electron and scanning probe microscopy techniques including Cathodoluminescence Microanalysis and Kelvin Probe Microscopy. These techniques enable the defect structure and the residual charging of materials to be characterized at high spatial resolution. Cathodoluminescence is the non-incandescent emission of light resulting from the electron irradiation. CL microscopy and spectroscopy in a Scanning Electron Microscope (SEM) enables high spatial resolution and high sensitivity detection of defects in poorly conducting materials. Local variations in the distribution of defects can be non-destructively characterized with high spatial (lateral and depth) resolution by adjusting electron beam parameters to select the specimen micro-volume of interest. Kelvin Probe Microscopy (KPM) is a Scanning Probe Microscopy technique in which long-range Coulomb forces between a conductive atomic force probe and the specimen enable the surface potential to be characterized with high spatial resolution. A combination of Kelvin Probe Microscopy (KPM) and Cathodoluminescence (CL) microanalysis has been used to characterize ultra pure silicon dioxide exposed to electron irradiation in a Scanning Electron Microscope. Silicon dioxide is an excellent model specimen with which to investigate charging induced effects. It is a very poor electrical conductor, homogeneous and electron irradiation produces easily identifiable surface modification which enables irradiated regions to be easily and unambiguously located. A conductive grounded coating is typically applied to poorly conducting specimens prior to investigation in an SEM to prevent deflection of the electron beam and surface charging, however

  4. Atomic collision experiments utilizing low-velocity, highly-charged ion beams

    International Nuclear Information System (INIS)

    Johnson, B.M.; Jones, K.W.; Meron, M.

    1983-01-01

    Intense beams of highly-stripped ions are now routinely produced at low velocities using the Brookhaven dual MP-tandems in a unique four-stage accel/decel mode. This mode of operation combines three stages of acceleration, stripping at high energy, and one stage of deceleration to near-zero velocity. To date, experiments have used 10-100 nA beams of bare and few-electron heavy ions at energies as low as 0.2 MeV/amu, and upgrades of the facility should push the lower limit below 0.1 MeV/amu. Recent experiments, such as measurements of charge transfer and x-ray production for S 6 - 16 + on He and Ar at 6-20 MeV and P(b) measurements for MO x-rays produced in Cl 16 + + Ar collisions at 20, 10 and 5 MeV have demonstrated the usefulness of highly-stripped, low-velocity projectiles. These experiments and a few possibilities for future experiments are discussed

  5. Atomic collision experiments utilizing low-velocity, highly-charged ion beams

    International Nuclear Information System (INIS)

    Johnson, B.M.; Jones, K.W.; Meron, M.

    1982-01-01

    Intense beams of highly-stripped ions are now routinely produced at low velocities using the Brookhaven dual MP-tandens in a unique four-stage accel/decel mode. This mode of operation combines three stages of acceleration, stripping at high energy, and one stage of deceleration to near-zero velocity. To date, experiments have used 10-100 nA beams of bare and few-electron heavy ions at energies as low as 0.2 MeV/amu, and upgrades of the facility should push the lower limit below 0.1 MeV/amu. Recent experiments, such as measurements of charge transfer and x-ray production for S/sup 6-16+/ on He and Ar at 6 to 20 MeV and P(b) measurements for MO x-rays produced in Cl 16 + + Ar collisions at 20, 10, and 5 MeV have demonstrated the usefulness of highly-stripped, low-velocity projectiles. These experiments and a few possibilities for future experiments are discussed

  6. Excitation and ionization of highly charged ions by electron impact

    International Nuclear Information System (INIS)

    Sampson, D.H.

    1989-01-01

    Two approaches for very rapid calculation of atomic data for high temperature plasma modeling have been developed. The first uses hydrogenic basis states and has been developed and applied in many papers discussed in previous progress reports. Hence, it is only briefly discussed here. The second is a very rapid, yet accurate, fully relativistic approach that has been developed over the past two or three years. It is described in more detail. Recently it has been applied to large scale production of atomic data. Specifically, it has been used to calculate relativistic distorted wave collision strengths and oscillator strengths for the following: all transitions from the ground level to the n=3 and 4 excited levels in the 71 Neon-like ions with nuclear charge number Z in the range 22 ≤ Z ≤ 92; all transitions among the 2s 1/2 , 2p 1/2 and 2p 3/2 levels and from them to all nlj levels with n=3,4 and 5 in the 85 Li-like ions with 8 ≤ Z ≤ 92; all transitions among the 3s 1/2 , 3p 3/2 , 3d 3/2 and 3d 5/2 levels and from them to all nlj levels with n=4 and 5 in the 71 Na-like ions with 22 ≤ Z ≤ 92; and all transitions among 4s 1/2 , 4p 1/2 , 4p 3/2 , 4d 3/2 , 4d 5/2 , 4f 5/2 and 4f 7/2 levels and from them to all nlj levels with n=5 in the 33 Cu-like ions with 60 ≤ Z ≤ 92. Also the program has been extended to give cross-sections for excitation to specific magnetic sublevels of the target ion by an electron beam and very recently it has been extended to give relativistic distorted wave cross sections for ionization of highly charged ions by electron impact

  7. Specification of electron radiation environment at GEO and MEO for surface charging estimates

    Science.gov (United States)

    Ganushkina, N.; Dubyagin, S.; Mateo Velez, J. C.; Liemohn, M. W.

    2017-12-01

    A series of anomalies at GEO have been attributed to electrons of energy below 100 keV, responsible for surface charging. The process at play is charge deposition on covering insulating surfaces and is directly linked to the space environment at a time scale of a few tens of seconds. Even though modern satellites benefited from the analysis of past flight anomalies and losses, it appears that surface charging remains a source of problems. Accurate specification of the space environment at different orbits is of a key importance. We present the operational model for low energy (model (IMPTAM). This model has been operating online since March 2013 (http://fp7-spacecast.eu and imptam.fmi.fi) and it is driven by the real time solar wind and IMF parameters and by the real time Dst index. The presented model provides the low energy electron flux at all L-shells and at all satellite orbits, when necessary. IMPTAM is used to simulate the fluxes of low energy electrons inside the Earth's magnetosphere at the time of severe events measured on LANL satellites at GEO. There is no easy way to say what will be the flux of keV electrons at MEO when surface charging events are detected at GEO than to use a model. The maximal electron fluxes obtained at MEO (L = 4.6) within a few tens of minutes hours following the LANL events at GEO have been extracted to feed a database of theoretical/numerical worst-case environments for surface charging at MEO. All IMPTAM results are instantaneous, data have not been average. In order to validate the IMPTAM output at MEO, we conduct the statistical analysis of measured electron fluxes onboard Van Allen Probes (ECT HOPE (20 eV-45 keV) and ECT MagEIS (30 - 300 keV) at distances of 4.6 Re. IMPTAM e- flux at MEO is used as input to SPIS, the Spacecraft Plasma Interaction System Software toolkit for spacecraft-plasma interactions and spacecraft charging modelling (http://dev.spis.org/projects/spine/home/spis). The research leading to these results

  8. Beam extraction dynamics at the space-charge-limit of the high brightness E-XFEL electron source at DESY-PITZ

    Energy Technology Data Exchange (ETDEWEB)

    Chen, Ye; Gjonaj, Erion; Weiland, Thomas [TEMF, Technische Universitaet Darmstadt, Schlossgartenstrasse 8, 64289 Darmstadt (Germany)

    2015-07-01

    The physics of the photoemission, as one of the key issues for successful operation of linac based free-electron lasers like the European X-ray Free Electron Laser (E-XFEL) and the Free-electron Laser in Hamburg (FLASH), is playing an increasingly important role in the high brightness DESY-PITZ electron source. We study photoemission physics and discuss full three-dimensional numerical modeling of the electron bunch emission. The beam extraction dynamics at the photocathode has been investigated through the 3D fully electromagnetic (EM) Particle-in-Cell (PIC) solver of CST Particle Studio under the assumption of the photoemission source operating at or close to its space charge limit. PIC simulation results have shown good agreements with measurements on total emitted bunch charge for distinct experimental parameters. Further comparisons showed a general failure for the conventional Poisson solver based tracking algorithm to correctly predict the beam dynamics at the space charge limit. It is furthermore found, that fully EM PIC simulations are also consistent with a simple emission model based on the multidimensional Child-Langmuir law.

  9. Experimental investigations of single-electron detachment processes from H- ions colliding with MeV/u, highly charged ions

    International Nuclear Information System (INIS)

    Tawara, H.; Tonuma, T.; Kumagai, H.; Imai, T.; Uskov, D.B.; Presnyakov, L.P.

    1999-01-01

    Single electron detachment processes from negative hydrogen ions under collisions with MeV/u highly charged ions have been investigated using the so-called crossed-beams technique. The preliminary results of the single-electron detachment cross sections obtained is found to be in crude agreement with some empirical and theoretical estimations. (orig.)

  10. Spectroscopy with trapped highly charged ions

    International Nuclear Information System (INIS)

    Beiersdorfer, Peter

    2009-01-01

    We give an overview of atomic spectroscopy performed on electron beam ion traps at various locations throughout the world. Spectroscopy at these facilities contributes to various areas of science and engineering, including but not limited to basic atomic physics, astrophysics, extreme ultraviolet lithography, and the development of density and temperature diagnostics of fusion plasmas. These contributions are accomplished by generating, for example, spectral surveys, making precise radiative lifetime measurements, accounting for radiative power emitted in a given wavelength band, illucidating isotopic effects, and testing collisional-radiative models. While spectroscopy with electron beam ion traps had originally focused on the x-ray emission from highly charged ions interacting with the electron beam, the operating modes of such devices have expanded to study radiation in almost all wavelength bands from the visible to the hard x-ray region; and at several facilities the ions can be studied even in the absence of an electron beam. Photon emission after charge exchange or laser excitation has been observed; and the work is no longer restricted to highly charged ions. Much of the experimental capabilities are unique to electron beam ion traps, and the work performed with these devices cannot be undertaken elsewhere. However, in other areas the work on electron beam ion traps rivals the spectroscopy performed with conventional ion traps or heavy-ion storage rings. The examples we present highlight many of the capabilities of the existing electron beam ion traps and their contributions to physics.

  11. Laboratory X-ray Studies with Trapped Highly Charged Ions Using Synchrotrons and Free-electron Lasers

    Science.gov (United States)

    Crespo López-Urrutia, José R.

    2018-06-01

    Laboratory studies on highly charged ions (HCI) using electron beam ion traps (EBITs) can cover all charge states and chemical elements found in astrophysical sources. Since their introduction in 1986, a wealth of emission measurements from the optical to the x-ray range has been carried out by different groups. In most of the work, electron-impact excitation was the driving mechanism, and high resolution spectrometers were used for the diagnostic of the emitted radiation. Other recent studies included x-ray emission following charge exchange, a mechanism which is present in many astrophysical environments and can help explain some of the unknown spectral features at 3.55 keV.In the last decade, excitation and photoionization have also been investigated by exposing HCI trapped in an EBIT to intense, monochromatic radiation from free-electron lasers and synchrotron sources. Here, advanced monochromators in powerful undulator beamlines allowed us to work at photon energies from 50 eV to 15 keV while resolving the natural linewidths of x-ray transitions like the Kα complex of Fe up to the highest charge states, and to measure the oscillator strengths of, e. g., the neonlike Fe16+ spectrum. Photoionization studies have been performed for those species as well. Very recently, our novel compact EBIT with an off-axis electron gun allows for simultaneously using the photon beam downstream, enabling exact wavelength determinations referenced to HCI with accurately calculable transitions. We have performed a recalibration of the molecular and atomic oxygen soft x-ray absorption lines in the 500 eV range with an uncertainty estimate of 30 meV. This revealed a 600 meV calibration error that propagated through the literature for decades with the consequence of a 200 km/s misfit of the velocity in interstellar oxygen absorbers. Other possibilities for the compact EBIT are investigations of resonant photorecombination processes with excellent energy resolution. With the

  12. Electron capture to autoionizing states of multiply charged ions

    International Nuclear Information System (INIS)

    Mack, E.M.

    1987-01-01

    The present thesis investigates electron capture reactions resulting from slow collisions (V q+ ) and neutral gas targets (B). The energy spectra of the emitted electrons are measured; detection angle is 50 0 . Mainly, autoionizing double capture resulting from collisions with two-electron targets (He, H 2 ) is studied; then, the emitted electrons stem from doubly excited projectile states. The projectiles used are bare C 6+ , the H-like and He-like ions of C, N and O, He-like Ne 8+ and Ne-like Ar 8+ . Excited metastable projectiles used are C 5+ (2s), He-like projectiles A q+ (1s2s 3 S) and Ar 8+ (...2p 5 3s). Comparison is made with the predictions of a recently proposed extended classical barrier model, that was developed in connection with the work. This model assumes sequential capture of the electrons ('two-step' process); it predicts the realized binding enegies of the captured electrons - which may be directly determined from the autoionization spectra using only the projectile charge, the ionization potentials of the target and the collision velocity as parameters. No adjustable parameter enters into the calculations. The term energies and decay modes of the highly excited product ions themselves are studied. Generally, the autoionizing decay of these states is found to proceed preferentially to the directly adjacent lower singly excited state. Experimental evidence is presented, that triply excited states decay by successive emission of two electrons, whenever this is energetically possible. Finally, the L-MM decay in few-electron systems is considered. 314 refs.; 96 figs.; 29 tabs

  13. Nonextensive electron and ion dust charging currents

    International Nuclear Information System (INIS)

    Amour, Rabia; Tribeche, Mouloud

    2011-01-01

    The correct nonextensive electron and ion charging currents are presented for the first time based on the orbit motion limited approach. For -1< q<1, where q measures the amount of plasma nonextensivity, the nonextensive electron charging current is expressed in terms of the hypergeometric function. The variable dust charge is expressed in terms of the Lambert function and we take advantage of this transcendental function to investigate succinctly the effects of nonextensive charge carriers. The obtained formulas bring a possibility to build theories on nonlinear collective process in variable charge nonextensive dusty plasmas.

  14. Few-cycle surface plasmon enhanced electron acceleration

    International Nuclear Information System (INIS)

    Racz, P.; Lenner, M.; Kroo, N.; Farkas, Gy.; Dombi, P.; Takao Fuji; Krausz, F.; Irvine, S.E.; Elezzabi, A.Y.

    2010-01-01

    Complete text of publication follows. It is possible to generate high-quality ultrafast electron beams with keV energy based on surface plasmon-enhanced electron acceleration. The beam generated this way can be also used to investigate ultrafast phenomena in the plasmon field. For the better understanding of the temporal behavior of these ultrafast surface processes we carried out time-resolved experiments with 5.5 fs laser pulses for the first time. In this experiment, we executed an autocorrelation measurement with an ultra-broadband interferometer. By generating surface plasmons at the output of the interferometer, we measured the plasmonic photocurrent as a function of the delay between the interferometer arms. Figure (a) shows a typical measured result, and figure (b) shows the fourth order calculated autocorrelation function of the 5.5 fs long laser pulse, corresponding to the fourth order nonlinearity of the electron emission process. According to the correspondence of these two curves, we can also state that the length of the generated surface plasmon pulse is only 2-3 optical cycles. As a further experiment, we executed spectrally resolved measurements of the electron beam at higher intensities. According to these results, it is possible to reach electron beams with keV energy in the few-cycle regime too. It was found that the field strength of the surface plasmons is x 7 to x 30 higher than that of the focused laser pulse.

  15. Dose errors due to charge storage in electron irradiated plastic phantoms

    International Nuclear Information System (INIS)

    Galbraith, D.M.; Rawlinson, J.A.; Munro, P.

    1984-01-01

    Commercial plastics used for radiation dosimetry are good electrical insulators. Used in electron beams, these insulators store charge and produce internal electric fields large enough to measurably alter the electron dose distribution in the plastic. The reading per monitor unit from a cylindrical ion chamber imbedded in a polymethylmethacrylate (PMMA) or polystyrene phantom will increase with accumulated electron dose, the increase being detectable after about 20 Gy of 6-MeV electrons. The magnitude of the effect also depends on the type of the plastic, the thickness of the plastic, the wall thickness of the detector, the diameter and depth of the hole in the plastic, the energy of the electron beam, and the dose rate used. Effects of charge buildup have been documented elsewhere for very low energy electrons at extremely high doses and dose rates. Here we draw attention to the charging effects in plastics at the dose levels encountered in therapy dosimetry where ion chamber or other dosimeter readings may easily increase by 5% to 10% and where a phantom, once charged, will also affect subsequent readings taken in 60 Co beams and high-energy electron and x-ray beams for periods of several days to many months. It is recommended that conducting plastic phantoms replace PMMA and polystyrene phantoms in radiation dosimetry

  16. Laser-pump/X-ray-probe experiments with electrons ejected from a Cu(111) target: space-charge acceleration.

    Science.gov (United States)

    Schiwietz, G; Kühn, D; Föhlisch, A; Holldack, K; Kachel, T; Pontius, N

    2016-09-01

    A comprehensive investigation of the emission characteristics for electrons induced by X-rays of a few hundred eV at grazing-incidence angles on an atomically clean Cu(111) sample during laser excitation is presented. Electron energy spectra due to intense infrared laser irradiation are investigated at the BESSY II slicing facility. Furthermore, the influence of the corresponding high degree of target excitation (high peak current of photoemission) on the properties of Auger and photoelectrons liberated by a probe X-ray beam is investigated in time-resolved pump and probe measurements. Strong electron energy shifts have been found and assigned to space-charge acceleration. The variation of the shift with laser power and electron energy is investigated and discussed on the basis of experimental as well as new theoretical results.

  17. Direct Observation of Individual Charges and Their Dynamics on Graphene by Low-Energy Electron Holography.

    Science.gov (United States)

    Latychevskaia, Tatiana; Wicki, Flavio; Longchamp, Jean-Nicolas; Escher, Conrad; Fink, Hans-Werner

    2016-09-14

    Visualizing individual charges confined to molecules and observing their dynamics with high spatial resolution is a challenge for advancing various fields in science, ranging from mesoscopic physics to electron transfer events in biological molecules. We show here that the high sensitivity of low-energy electrons to local electric fields can be employed to directly visualize individual charged adsorbates and to study their behavior in a quantitative way. This makes electron holography a unique probing tool for directly visualizing charge distributions with a sensitivity of a fraction of an elementary charge. Moreover, spatial resolution in the nanometer range and fast data acquisition inherent to lens-less low-energy electron holography allows for direct visual inspection of charge transfer processes.

  18. Transmutation prospect of long-lived nuclear waste induced by high-charge electron beam from laser plasma accelerator

    Science.gov (United States)

    Wang, X. L.; Xu, Z. Y.; Luo, W.; Lu, H. Y.; Zhu, Z. C.; Yan, X. Q.

    2017-09-01

    Photo-transmutation of long-lived nuclear waste induced by a high-charge relativistic electron beam (e-beam) from a laser plasma accelerator is demonstrated. A collimated relativistic e-beam with a high charge of approximately 100 nC is produced from high-intensity laser interaction with near-critical-density (NCD) plasma. Such e-beam impinges on a high-Z convertor and then radiates energetic bremsstrahlung photons with flux approaching 1011 per laser shot. Taking a long-lived radionuclide 126Sn as an example, the resulting transmutation reaction yield is the order of 109 per laser shot, which is two orders of magnitude higher than obtained from previous studies. It is found that at lower densities, a tightly focused laser irradiating relatively longer NCD plasmas can effectively enhance the transmutation efficiency. Furthermore, the photo-transmutation is generalized by considering mixed-nuclide waste samples, which suggests that the laser-accelerated high-charge e-beam could be an efficient tool to transmute long-lived nuclear waste.

  19. Charge density of 58Ni, by scattering of electrons at high moment transfer

    International Nuclear Information System (INIS)

    Turck, Sylvaine

    1976-01-01

    Due to the unique electromagnetic interaction involved, electron elastic scattering allows a nuclear structure to be tested through nucleus magnetisation and charge distribution. In a first part, this research thesis reports experiments performed on the Saclay Linear Accelerator (ALS) with the 58 Ni nucleus, a well closed magic nucleus which allows a qualitative comparison between experiments and Hartree-Fock calculations to be performed. The author presents the experimental set-up, describes data acquisition, data reduction and corrections. The second part proposes a theoretical introduction to electron scattering, discusses the analysis without model, and theoretical predictions of charge density

  20. Powder bed charging during electron-beam additive manufacturing

    International Nuclear Information System (INIS)

    Cordero, Zachary C.; Meyer, Harry M.; Nandwana, Peeyush; Dehoff, Ryan R.

    2017-01-01

    Electrons injected into the build envelope during powder bed electron-beam additive manufacturing can accumulate on the irradiated particles and cause them to repel each other. Under certain conditions, these electrostatic forces can grow so large that they drive the particles out of the build envelope in a process known as “smoking”. In the present work, we investigate the causes of powder bed charging and smoking during electron-beam additive manufacturing. In the first part of the paper, we characterize the surface chemistry of a common feedstock material—gas-atomized Ti-6Al-4V powder—and find that a thick, electrically insulating oxide overlayer encapsulates the particles. Based on these experimental results, we then formulate an analytical model of powder bed charging in which each particle is approximated as a capacitor, where the particle and its substrate are the electrodes and the oxide overlayer is the dielectric. Using this model, we estimate the charge distribution in the powder bed, the electrostatic forces acting on the particles, and the conditions under which the powder bed will smoke. It is found that the electrical resistivity of the oxide overlayer strongly influences the charging behavior of the powder bed and that a high resistivity promotes charge accumulation and consequent smoking. This analysis suggests new quality control and process design measures that can help suppress smoking.

  1. Collisionally excited few-electron systems: theoretical introduction and survey

    International Nuclear Information System (INIS)

    Ford, A.L.; Reading, J.F.; Becker, R.L.

    1982-01-01

    We consider excitation, ionization, and charge transfer in collisions of protons (and antiprotons) with the single-electron targets H, He + , and Li 2+ . These collisions are first compared to other types of ion-atom collisions. A brief review of our own theoretical method is given; in particular we describe how we allow for both large charge transfer and ionization probabilities while retaining the computational efficiency that allows us to consider a variety of collision partners and collision energies. We comment on the comparison of our results to other theoretical work and to experiment. The qualitative features of the various inelastic cross sections are discussed, in particular how they scale with collision energy, target nuclear charge, and the sign of the projectile charge. 15 references, 6 figures

  2. Highly charged ions at rest: The HITRAP project at GSI

    International Nuclear Information System (INIS)

    Herfurth, F.; Beier, T.; Dahl, L.; Eliseev, S.; Heinz, S.; Kester, O.; Kluge, H.-J.; Kozhuharov, C.; Maero, G.; Quint, W.

    2005-01-01

    A decelerator will be installed at GSI in order to provide and study bare heavy nuclei or heavy nuclei with only few electrons at very low energies or even at rest. Highly-charged ions will be produced by stripping at relativistic energies. After electron cooling and deceleration in the Experimental Storage Ring the ions are ejected out of the storage ring at 4 MeV/u and further decelerated in a combination of an IH and RFQ structure. Finally, they are injected into a Penning trap where the ions are cooled to 4 K. From here, the ions can be transferred in a quasi dc or in a pulsed mode to different experimental setups. This article describes the technical concepts of this project as well as planned key experiments

  3. Photoelectric effect in the relativistic domain revealed by the time-reversed process for highly charged uranium ions

    International Nuclear Information System (INIS)

    Stoehlker, T.; Mokler, P.H.; Kozhuharov, C.; Warczak, A.

    1996-10-01

    The photoelectric effect in the near relativistic energy regime of 80 to 350 keV is studied by the time-reversed process in ion-atom collisions, i.e. by the radiative capture of a quasi-free target electron. We review shell and subshell differential photon-angular distribution studies of radiative capture into highly-charged uranium ions. The experimental data are compared with exact relativistic calculations and give detailed insight into both the atomic structure of high-Z few-electron ions and into the fundamental electron-photon interaction process involved. In particular it is shown that the angular-differential measurements provide a unique method to study the magnetic interaction in relativistic electron-photon encoun- (orig.)

  4. Ionization and single electron capture in collision of highly charged Ar16+ ions with helium

    International Nuclear Information System (INIS)

    Wang Fei; Gou Bingcong

    2008-01-01

    This paper uses the two-centre atomic orbital close-coupling method to study the ionization and the single electron capture in collision of highly charged Ar 16+ ions with He atoms in the velocity range of 1.2–1.9 a.u. The relative importance of single ionization (SI) to single capture (SC) is explored. The comparison between the calculation and experimental data shows that the SI/SC cross section ratios from this work are in good agreement with experimental data. The total single electron ionization cross sections and the total single electron capture cross sections are also given for this collision. The investigation of the partial electron capture cross section shows a general tendency of capture to larger n and l with increasing velocity from 1.2 to 1.9 a.u

  5. Bond charges and electronic charge transfer in ternary semiconductors

    International Nuclear Information System (INIS)

    Pietsch, U.

    1986-01-01

    By means of a simple molecule-theoretic model of 'linear superposition of two-electron molecules' the bond charges between nearest neighbours and the effective charges of ions are calculated for ternary zinc-blende structure alloys as well as chalcopyrite semiconductors. Taking into account both, the charge transfer among the ions caused by the differences of electronegativities of atoms used and between the bonds created by the internal stress of the lattice a nearly unvaried averaged bond charge amount of the alloy is found, but rather dramatically changed local bond charge parameters in comparison with the respective values of binary compounds used. This fact should influence the noncentral force interaction in such semiconductors. (author)

  6. Quantum electrodynamic theory of recombination of an electron with a highly charged ion

    International Nuclear Information System (INIS)

    Shabaev, V.M.

    1994-01-01

    The consequent quantum electrodynamic theory of the process of the recombination of an electron with a multicharged ion is considered. The reduction technique for the calculation of this process by perturbation theory is formulated. The process of the recombination of an electron with a very highly charged one-electron ion for the case of resonance with the doubly excited (2s,2s) 0 , (2p 1/2 ,2p 1/2 ) 0 , (2s,2p 1/2 ) 0,1 states is studied. The formulas for the cross section of the process are derived for two possible versions of the experiment. The interference between the radiative-recombination process and the dielectronic-recombination (DR) process, and the interference between the DR amplitudes for the levels with the identical quantum numbers [(2s,2s) 0 , (2p 1/2 ) 0 ] are taken into account. The deviation of the shape of the resonances from the Lorentz one, due to the interference terms, is discussed

  7. A method to restrain the charging effect on an insulating substrate in high energy electron beam lithography

    Science.gov (United States)

    Mingyan, Yu; Shirui, Zhao; Yupeng, Jing; Yunbo, Shi; Baoqin, Chen

    2014-12-01

    Pattern distortions caused by the charging effect should be reduced while using the electron beam lithography process on an insulating substrate. We have developed a novel process by using the SX AR-PC 5000/90.1 solution as a spin-coated conductive layer, to help to fabricate nanoscale patterns of poly-methyl-methacrylate polymer resist on glass for phased array device application. This method can restrain the influence of the charging effect on the insulating substrate effectively. Experimental results show that the novel process can solve the problems of the distortion of resist patterns and electron beam main field stitching error, thus ensuring the accuracy of the stitching and overlay of the electron beam lithography system. The main characteristic of the novel process is that it is compatible to the multi-layer semiconductor process inside a clean room, and is a green process, quite simple, fast, and low cost. It can also provide a broad scope in the device development on insulating the substrate, such as high density biochips, flexible electronics and liquid crystal display screens.

  8. Charging of Individual Micron-Size Interstellar/Planetary Dust Grains by Secondary Electron Emissions

    Science.gov (United States)

    Tankosic, D.; Abbas, M. M.

    2012-01-01

    Dust grains in various astrophysical environments are generally charged electrostatically by photoelectric emissions with UV/X-ray radiation, as well as by electron/ion impact. Knowledge of physical and optical properties of individual dust grains is required for understanding of the physical and dynamical processes in space environments and the role of dust in formation of stellar and planetary systems. In this paper, we discuss experimental results on dust charging by electron impact, where low energy electrons are scattered or stick to the dust grains, thereby charging the dust grains negatively, and at sufficiently high energies the incident electrons penetrate the grain leading to excitation and emission of electrons referred to as secondary electron emission (SEE). Currently, very limited experimental data are available for charging of individual micron-size dust grains, particularly by low energy electron impact. Available theoretical models based on the Sternglass equation (Sternglass, 1954) are applicable for neutral, planar, and bulk surfaces only. However, charging properties of individual micron-size dust grains are expected to be different from the values measured on bulk materials. Our recent experimental results on individual, positively charged, micron-size lunar dust grains levitated in an electrodynamic balance facility (at NASA-MSFC) indicate that the SEE by electron impact is a complex process. The electron impact may lead to charging or discharging of dust grains depending upon the grain size, surface potential, electron energy, electron flux, grain composition, and configuration (e.g. Abbas et al, 2010). Here we discuss the complex nature of SEE charging properties of individual micron-size lunar dust grains and silica microspheres.

  9. Electronic energy loss spectra from mono-layer to few layers of phosphorene

    International Nuclear Information System (INIS)

    Mohan, Brij; Thakur, Rajesh; Ahluwalia, P. K.

    2016-01-01

    Using first principles calculations, electronic and optical properties of few-layers phosphorene has been investigated. Electronic band structure show a moderate band gap of 0.9 eV in monolayer phosphorene which decreases with increasing number of layers. Optical properties of few-layers of phosphorene in infrared and visible region shows tunability with number of layers. Electron energy loss function has been plotted and huge red shift in plasmonic behaviours is found. These tunable electronic and optical properties of few-layers of phosphorene can be useful for the applications of optoelectronic devices.

  10. Electronic energy loss spectra from mono-layer to few layers of phosphorene

    Energy Technology Data Exchange (ETDEWEB)

    Mohan, Brij, E-mail: brijmohanhpu@yahoo.com; Thakur, Rajesh; Ahluwalia, P. K. [Department of Physics, Himachal Pradesh University, Shimla (HP) India 171005 (India)

    2016-05-23

    Using first principles calculations, electronic and optical properties of few-layers phosphorene has been investigated. Electronic band structure show a moderate band gap of 0.9 eV in monolayer phosphorene which decreases with increasing number of layers. Optical properties of few-layers of phosphorene in infrared and visible region shows tunability with number of layers. Electron energy loss function has been plotted and huge red shift in plasmonic behaviours is found. These tunable electronic and optical properties of few-layers of phosphorene can be useful for the applications of optoelectronic devices.

  11. Two and three electron Auger transitions in collisions of highly-charged ions with surfaces

    International Nuclear Information System (INIS)

    Moretto-Capelle, P.; Bordenave-Montesquieu, A.; Benoit-Cattin, P.; Andriamonje, S.; Andrae, H.J.

    1991-01-01

    The Auger electron spectra from Ar 9+ approaching at 265 eV a Si or metal surface in vacua of 10 -5 Pa or UHV are identical. Experiments on atomic physics in front of surfaces are thus possible in standard vacuum. N 7+ approaching a surface at 1000 eV penetrates with great probability into the bulk and gives rise to K 2 L 2 L double Auger lines, observed for the first time with low energy highly charged ions. (orig.)

  12. Electron holography studies of the charge on dislocations in GaN

    Energy Technology Data Exchange (ETDEWEB)

    Cherns, D.; Jiao, C.G.; Mokhtari, H. [H.H. Wills Physics Laboratory, University of Bristol, Tyndall Avenue, Bristol BS8 1TL (United Kingdom); Cai, J.; Ponce, F.A. [Department of Physics and Astronomy, Arizona State University, Tempe, AZ85287 (United States)

    2002-12-01

    The measurement of charge on dislocations in GaN by electron holography is described. Recent results are presented showing that edge dislocations in n-doped GaN are highly negatively charged, whereas those in p-doped GaN are positively charged. It is shown that the results are consistent with a model which assumes Fermi level pinning at dislocation states about 2.5 V below the conduction band edge. The application of electron holography to screw dislocations, and the dependence of the observations on the dislocation core structure, are also discussed. (Abstract Copyright [2002], Wiley Periodicals, Inc.)

  13. High electron mobility InN

    International Nuclear Information System (INIS)

    Jones, R. E.; Li, S. X.; Haller, E. E.; van Genuchten, H. C. M.; Yu, K. M.; Ager, J. W. III; Liliental-Weber, Z.; Walukiewicz, W.; Lu, H.; Schaff, W. J.

    2007-01-01

    Irradiation of InN films with 2 MeV He + ions followed by thermal annealing below 500 deg. C creates films with high electron concentrations and mobilities, as well as strong photoluminescence. Calculations show that electron mobility in irradiated samples is limited by triply charged donor defects. Subsequent thermal annealing removes a fraction of the defects, decreasing the electron concentration. There is a large increase in electron mobility upon annealing; the mobilities approach those of the as-grown films, which have 10 to 100 times smaller electron concentrations. Spatial ordering of the triply charged defects is suggested to cause the unusual increase in electron mobility

  14. Dual structure in the charge excitation spectrum of electron-doped cuprates

    Science.gov (United States)

    Bejas, Matías; Yamase, Hiroyuki; Greco, Andrés

    2017-12-01

    Motivated by the recent resonant x-ray scattering (RXS) and resonant inelastic x-ray scattering (RIXS) experiments for electron-doped cuprates, we study the charge excitation spectrum in a layered t -J model with the long-range Coulomb interaction. We show that the spectrum is not dominated by a specific type of charge excitations, but by different kinds of charge fluctuations, and is characterized by a dual structure in the energy space. Low-energy charge excitations correspond to various types of bond-charge fluctuations driven by the exchange term (J term), whereas high-energy charge excitations are due to usual on-site charge fluctuations and correspond to plasmon excitations above the particle-hole continuum. The interlayer coupling, which is frequently neglected in many theoretical studies, is particularly important to the high-energy charge excitations.

  15. Space-charge-limit instabilities in electron beams

    International Nuclear Information System (INIS)

    Coutsias, E.A.; Sullivan, D.J.

    1983-01-01

    The method of characteristics and multiple-scaling perturbation techniques are used to study the space-charge instability of electron beams. It is found that the stable oscillating state (virtual cathode) created when the space-charge limit is exceeded is similar to a collisionless shock wave. The oscillatory solution originates at the bifurcation point of two unstable steady states. Complementary behavior (virtual anode) results when an ion beam exceeds its space-charge limit. The virtual cathode can also exist in the presence of a neutralizing heavy-ion background. The Pierce instability, where the electron and ion charge densities are equal, is a special case of this broader class. Estimates of the nonlinear growth rate of the instability at the space-charge limit are given

  16. Atomic and electronic structure of trilayer graphene/SiC(0001): Evidence of Strong Dependence on Stacking Sequence and charge transfer.

    Science.gov (United States)

    Pierucci, Debora; Brumme, Thomas; Girard, Jean-Christophe; Calandra, Matteo; Silly, Mathieu G; Sirotti, Fausto; Barbier, Antoine; Mauri, Francesco; Ouerghi, Abdelkarim

    2016-09-15

    The transport properties of few-layer graphene are the directly result of a peculiar band structure near the Dirac point. Here, for epitaxial graphene grown on SiC, we determine the effect of charge transfer from the SiC substrate on the local density of states (LDOS) of trilayer graphene using scaning tunneling microscopy/spectroscopy and angle resolved photoemission spectroscopy (ARPES). Different spectra are observed and are attributed to the existence of two stable polytypes of trilayer: Bernal (ABA) and rhomboedreal (ABC) staking. Their electronic properties strongly depend on the charge transfer from the substrate. We show that the LDOS of ABC stacking shows an additional peak located above the Dirac point in comparison with the LDOS of ABA stacking. The observed LDOS features, reflecting the underlying symmetry of the two polytypes, were reproduced by explicit calculations within density functional theory (DFT) including the charge transfer from the substrate. These findings demonstrate the pronounced effect of stacking order and charge transfer on the electronic structure of trilayer or few layer graphene. Our approach represents a significant step toward understand the electronic properties of graphene layer under electrical field.

  17. Electron-capture cross sections for low-energy highly charged neon and argon ions from molecular and atomic hydrogen

    International Nuclear Information System (INIS)

    Can, C.; Gray, T.J.; Varghese, S.L.; Hall, J.M.; Tunnell, L.N.

    1985-01-01

    Electron-capture cross sections for low-velocity (10 6 --10 7 cm/s) highly charged Ne/sup q/+ (2< or =q< or =7) and Ar/sup q/+ (2< or =q< or =10)= projectiles incident on molecular- and atomic-hydrogen targets have been measured. A recoil-ion source that used the collisions of fast heavy ions (1 MeV/amu) with target gas atoms was utilized to produce slow highly charged ions. Atomic hydrogen was produced by dissociating hydrogen molecules in a high-temperature oven. Measurements and analysis of the data for molecular- and atomic-hydrogen targets are discussed in detail. The measured absolute cross sections are compared with published data and predictions of theoretical models

  18. A data driven method to measure electron charge mis-identification rate

    CERN Document Server

    Bakhshiansohi, Hamed

    2009-01-01

    Electron charge mis-measurement is an important challenge in analyses which depend on the charge of electron. To estimate the probability of {\\it electron charge mis-measurement} a data driven method is introduced and a good agreement with MC based methods is achieved.\\\\ The third moment of $\\phi$ distribution of hits in electron SuperCluster is studied. The correlation between this variable and the electron charge is also investigated. Using this `new' variable and some other variables the electron charge measurement is improved by two different approaches.

  19. Mechanically delaminated few layered MoS2 nanosheets based high performance wire type solid-state symmetric supercapacitors

    Science.gov (United States)

    Krishnamoorthy, Karthikeyan; Pazhamalai, Parthiban; Veerasubramani, Ganesh Kumar; Kim, Sang Jae

    2016-07-01

    Two dimensional nanostructures are increasingly used as electrode materials in flexible supercapacitors for portable electronic applications. Herein, we demonstrated a ball milling approach for achieving few layered molybdenum disulfide (MoS2) via exfoliation from their bulk. Physico-chemical characterizations such as X-ray diffraction, field emission scanning electron microscope, and laser Raman analyses confirmed the occurrence of exfoliated MoS2 sheets with few layers from their bulk via ball milling process. MoS2 based wire type solid state supercapacitors (WSCs) are fabricated and examined using cyclic voltammetry (CV), electrochemical impedance spectroscopy, and galvanostatic charge discharge (CD) measurements. The presence of rectangular shaped CV curves and symmetric triangular shaped CD profiles suggested the mechanism of charge storage in MoS2 WSC is due to the formation of electrochemical double layer capacitance. The MoS2 WSC device delivered a specific capacitance of 119 μF cm-1, and energy density of 8.1 nW h cm-1 with better capacitance retention of about 89.36% over 2500 cycles, which ensures the use of the ball milled MoS2 for electrochemical energy storage devices.

  20. Injection and propagation of a nonrelativistic electron beam and spacecraft charging

    International Nuclear Information System (INIS)

    Okuda, H.; Berchem, J.

    1987-05-01

    Two-dimensional numerical simulations have been carried out in order to study the injection and propagation of a nonrelativistic electron beam from a spacecraft into a fully ionized plasma in a magnetic field. Contrary to the earlier results in one-dimension, a high density electron beam whose density is comparable to the ambient density can propagate into a plasma. A strong radial electric field resulting from the net charges in the beam causes the beam electrons to spread radially reducing the beam density. When the injection current exceeds the return current, significant charging of the spacecraft is observed along with the reflection of the injected electrons back to the spacecraft. Recent data on the electron beam injection from the Spacelab 1 (SEPAC) are discussed

  1. Radiative recombination of highly charged ions: Enhanced rates at low energies

    International Nuclear Information System (INIS)

    Frank, A.; Mueller, A.; Haselbauer, J.; Schennach, S.; Spies, W.; Uwira, O.; Wagner, M.

    1992-01-01

    In a single-pass merged-beams experiment employing a dense cold electron target recombination of highly charged ions is studied. Unexpected high recombination rates are observed at low energies E cm in the electron-ion center-of-mass frame. In particular, theoretical estimates for radiative recombination are dramatically exceeded by the experimental recombination rates at E cm =0 eV for U 28+ and for Au 25+ ions. Considerable rate enhancement is also observed for Ar 15+ . This points to a general phenomenon which has to be interpreted as a consequence of high electron densities, low electron beam temperatures, high ion charge states and presence of strong magnetic fields. (orig.)

  2. Interaction of slow, highly charged ions with the surface of ionic crystals

    International Nuclear Information System (INIS)

    Heller, Rene

    2009-01-01

    In this thesis the creation of permanent nanostructures induced by the impact of very slow (v≤5 x 10 5 m/s) highly charged (q≤40) ions on the ionic crystal surfaces of CaF 2 and KBr is investigated. The systematic analysis of the samples surfaces by means of atomic force microscopy supplies information on the influence of the potential as well as the kinetic projectile energy on the process of structure creation. The individual impact of highly charged ions on the KBr(001) surface can initiate the creation of mono-atomic deep pit-like structures -nanopits- with a lateral size of a few 10 nm. The volume of these pits and the corresponding number of sputtered secondary particles show a linear dependence on the projectiles potential energy. For the onset of pit formation a kinetic energy dependent threshold in the potential energy E grenz pot (E kin ) could be identified. Based on the defect-mediated desorption by electrons and by including effects of defect agglomeration a consistent model for the process of pit formation was drawn. In this work the recently discovered creation of hillock-like structures by impact of highly charged ions on CaF 2 (111) surfaces could be verified for lowest kinetic energies (E kin ≤150 eV x q). For the first time the potential energy of impinging projectiles could be identified to be exclusively responsible for the creation of nanostructures. Furthermore, a shift of potential energy threshold for hillock formation was observed for very small projectile velocities. Within the framework of cooperation with the Vienna University of Technology simulations based on the inelastic thermal spike model were performed, which allowed to interlink the individual hillock formation with a local melting of the ionic lattice. The essential influence of electron emission during the interaction of the highly charged ions with the surface on the process of nanostructuring was taken into consideration by complementary investigations of the secondary

  3. Charge Dissipating Transparent Conformal Coatings for Spacecraft Electronics, Phase I

    Data.gov (United States)

    National Aeronautics and Space Administration — The space environment poses significant challenges to spacecraft electronics in the form of electrostatic discharge (ESD) as a result of exposure to highly charged...

  4. Charge-transfer properties in the gas electron multiplier

    International Nuclear Information System (INIS)

    Han, Sanghyo; Kim, Yongkyun; Cho, Hyosung

    2004-01-01

    The charge transfer properties of a gas electron multiplier (GEM) were systematically investigated over a broad range of electric field configurations. The electron collection efficiency and the charge sharing were found to depend on the external fields, as well as on the GEM voltage. The electron collection efficiency increased with the collection field up to 90%, but was essentially independent of the drift field strength. A double conical GEM has a 10% gain increase with time due to surface charging by avalanche ions whereas this effect was eliminated with the cylindrical GEM. The positive-ion feedback is also estimated. (author)

  5. Electron Neutrino Charged-Current Quasielastic Scattering in the MINERvA Experiment

    Energy Technology Data Exchange (ETDEWEB)

    Wolcott, Jeremy [Rochester U.

    2015-10-28

    The electron-neutrino charged-current quasielastic (CCQE) cross section on nuclei is an important input parameter to appearance-type neutrino oscillation experiments. Current experiments typically work from the muon neutrino cross section and apply corrections from theoretical arguments to obtain a prediction for the electron neutrino cross section, but to date there has been no experimental verification of the estimates for this channel at an energy scale appropriate to such experiments. We present the first measurement of an exclusive reaction in few-GeV electron neutrino interactions, namely, the cross section for a CCQE-like process, made using the MINERvA detector. The result is given as differential cross-sections vs. the electron energy, electron angle, and square of the four-momentum transferred to the nucleus, $Q^2$. We also compute the ratio to a muon neutrino cross-section in $Q^2$ from MINERvA. We find satisfactory agreement between this measurement and the predictions of the GENIE generator.

  6. The status of the Electron Beam Ion Sources

    Energy Technology Data Exchange (ETDEWEB)

    Stockli, M.P.

    1990-01-01

    More than twenty years after its invention, 13 examples of the Electron Beam Ion Sources (EBIS) are in operation worldwide. The substantial progress in operation and insight, achieved over the last few years, made the EBISes become reliable tools for the production of beams of very highly charged, low-energy ions. For example, 8 EBISes produce bare argon on a standard basis. The successful production of hydrogen-like xenon presents the ions with the highest ionization energy, whereas the production of Th80+ presents the highest achieved charge state. Several synchrotrons are fed by EBIS injectors, taking advantage of the EBIS batch mode production, which yields the highest charge states. A few EBISes are used for ion source development. However, most of the EBISes' efforts are directed to research the physics of highly charged ions. Some of those are used to study the electron--ion interaction inside the source. But normally, most EBISes deliver the ions for external experiments, which so far concentrate on the recombination of the highly charged ions with atoms, molecules and surfaces. The ions are typically produced at a potential of 1 to a few kilovolts per charge; but in most cases, the EBIS is mounted on a high voltage platform or is followed by an RFQ, and therefore can generate ion energies from a few hundred volts up to a few hundred kilovolts per charge. The delivered beams have a low emittance and a low energy spread, which is an advantage for high-resolution experiments. This paper presents briefly all operational EBISes, their capabilities, their achievements, and their contribution to physics research. 5 figs., 1 tab., 59 refs.

  7. The status of the Electron Beam Ion Sources

    International Nuclear Information System (INIS)

    Stockli, M.P.

    1990-01-01

    More than twenty years after its invention, 13 examples of the Electron Beam Ion Sources (EBIS) are in operation worldwide. The substantial progress in operation and insight, achieved over the last few years, made the EBISes become reliable tools for the production of beams of very highly charged, low-energy ions. For example, 8 EBISes produce bare argon on a standard basis. The successful production of hydrogen-like xenon presents the ions with the highest ionization energy, whereas the production of Th80+ presents the highest achieved charge state. Several synchrotrons are fed by EBIS injectors, taking advantage of the EBIS batch mode production, which yields the highest charge states. A few EBISes are used for ion source development. However, most of the EBISes' efforts are directed to research the physics of highly charged ions. Some of those are used to study the electron--ion interaction inside the source. But normally, most EBISes deliver the ions for external experiments, which so far concentrate on the recombination of the highly charged ions with atoms, molecules and surfaces. The ions are typically produced at a potential of 1 to a few kilovolts per charge; but in most cases, the EBIS is mounted on a high voltage platform or is followed by an RFQ, and therefore can generate ion energies from a few hundred volts up to a few hundred kilovolts per charge. The delivered beams have a low emittance and a low energy spread, which is an advantage for high-resolution experiments. This paper presents briefly all operational EBISes, their capabilities, their achievements, and their contribution to physics research. 5 figs., 1 tab., 59 refs

  8. The status of the Electron Beam Ion Sources

    Energy Technology Data Exchange (ETDEWEB)

    Stockli, M.P.

    1990-12-31

    More than twenty years after its invention, 13 examples of the Electron Beam Ion Sources (EBIS) are in operation worldwide. The substantial progress in operation and insight, achieved over the last few years, made the EBISes become reliable tools for the production of beams of very highly charged, low-energy ions. For example, 8 EBISes produce bare argon on a standard basis. The successful production of hydrogen-like xenon presents the ions with the highest ionization energy, whereas the production of Th80+ presents the highest achieved charge state. Several synchrotrons are fed by EBIS injectors, taking advantage of the EBIS batch mode production, which yields the highest charge states. A few EBISes are used for ion source development. However, most of the EBISes` efforts are directed to research the physics of highly charged ions. Some of those are used to study the electron--ion interaction inside the source. But normally, most EBISes deliver the ions for external experiments, which so far concentrate on the recombination of the highly charged ions with atoms, molecules and surfaces. The ions are typically produced at a potential of 1 to a few kilovolts per charge; but in most cases, the EBIS is mounted on a high voltage platform or is followed by an RFQ, and therefore can generate ion energies from a few hundred volts up to a few hundred kilovolts per charge. The delivered beams have a low emittance and a low energy spread, which is an advantage for high-resolution experiments. This paper presents briefly all operational EBISes, their capabilities, their achievements, and their contribution to physics research. 5 figs., 1 tab., 59 refs.

  9. Measurements of Charging of Apollo 17 Lunar Dust Grains by Electron Impact

    Science.gov (United States)

    Abbas, Mian M.; Tankosic, Dragana; Spann, James F.; Dube, Michael J.

    2008-01-01

    It is well known since the Apollo missions that the lunar surface is covered with a thick layer of micron size dust grains with unusually high adhesive characteristics. The dust grains observed to be levitated and transported on the lunar surface are believed to have a hazardous impact on the robotic and human missions to the Moon. The observed dust phenomena are attributed to the lunar dust being charged positively during the day by UV photoelectric emissions, and negatively during the night by the solar wind electrons. The current dust charging and the levitation models, however, do not fully explain the observed phenomena, with the uncertainty of dust charging processes and the equilibrium potentials of the individual dust grains. It is well recognized that the charging properties of individual dust grains are substantially different from those determined from measurements made on bulk materials that are currently available. An experimental facility has been developed in the Dusty Plasma Laboratory at MSFC for investigating the charging and optical properties of individual micron/sub-micron size positively or negatively charged dust grains by levitating them in an electrodynamic balance in simulated space environments. In this paper, we present the laboratory measurements on charging of Apollo 17 individual lunar dust grains by a low energy electron beam. The charging rates and the equilibrium potentials produced by direct electron impact and by secondary electron emission process are discussed.

  10. Local charge measurement using off-axis electron holography

    DEFF Research Database (Denmark)

    Beleggia, Marco; Gontard, L.C.; Dunin-Borkowski, R.0E.

    2016-01-01

    A model-independent approach based on Gauss’ theorem for measuring the local charge in a specimen from an electron-optical phase image recorded using off-axis electron holography was recently proposed. Here, we show that such a charge measurement is reliable when it is applied to determine the to...

  11. Lead Halide Perovskites as Charge Generation Layers for Electron Mobility Measurement in Organic Semiconductors.

    Science.gov (United States)

    Love, John A; Feuerstein, Markus; Wolff, Christian M; Facchetti, Antonio; Neher, Dieter

    2017-12-06

    Hybrid lead halide perovskites are introduced as charge generation layers (CGLs) for the accurate determination of electron mobilities in thin organic semiconductors. Such hybrid perovskites have become a widely studied photovoltaic material in their own right, for their high efficiencies, ease of processing from solution, strong absorption, and efficient photogeneration of charge. Time-of-flight (ToF) measurements on bilayer samples consisting of the perovskite CGL and an organic semiconductor layer of different thickness are shown to be determined by the carrier motion through the organic material, consistent with the much higher charge carrier mobility in the perovskite. Together with the efficient photon-to-electron conversion in the perovskite, this high mobility imbalance enables electron-only mobility measurement on relatively thin application-relevant organic films, which would not be possible with traditional ToF measurements. This architecture enables electron-selective mobility measurements in single components as well as bulk-heterojunction films as demonstrated in the prototypical polymer/fullerene blends. To further demonstrate the potential of this approach, electron mobilities were measured as a function of electric field and temperature in an only 127 nm thick layer of a prototypical electron-transporting perylene diimide-based polymer, and found to be consistent with an exponential trap distribution of ca. 60 meV. Our study furthermore highlights the importance of high mobility charge transporting layers when designing perovskite solar cells.

  12. Self-sputtering runaway in high power impulse magnetron sputtering: The role of secondary electrons and multiply charged metal ions

    International Nuclear Information System (INIS)

    Anders, Andre

    2008-01-01

    Self-sputtering runaway in high power impulse magnetron sputtering is closely related to the appearance of multiply charged ions. This conclusion is based on the properties of potential emission of secondary electrons and energy balance considerations. The effect is especially strong for materials whose sputtering yield is marginally greater than unity. The absolute deposition rate increases ∼Q 1/2 , whereas the rate normalized to the average power decreases ∼Q -1/2 , with Q being the mean ion charge state number

  13. Experimental Investigation of Charging Properties of Interstellar Type Silica Dust Grains by Secondary Electron Emissions

    Science.gov (United States)

    Tankosic, D.; Abbas, M. M.

    2013-01-01

    The dust charging by electron impact is an important dust charging processes in astrophysical and planetary environments. Incident low energy electrons are reflected or stick to the grains charging the dust grains negatively. At sufficiently high energies electrons penetrate the grains, leading to excitation and emission of electrons referred to as secondary electron emission (SEE). Available classical theoretical models for calculations of SEE yields are generally applicable for neutral, planar, or bulk surfaces. These models, however, are not valid for calculations of the electron impact charging properties of electrostatically charged micron/submicron-size dust grains in astrophysical environments. Rigorous quantum mechanical models are not yet available, and the SEE yields have to be determined experimentally for development of more accurate models for charging of individual dust grains. At the present time, very limited experimental data are available for charging of individual micron-size dust grains, particularly for low energy electron impact. The experimental results on individual, positively charged, micron-size lunar dust grains levitated carried out by us in a unique facility at NASA-MSFC, based on an electrodynamic balance, indicate that the SEE by electron impact is a complex process. The electron impact may lead to charging or discharging of dust grains depending upon the grain size, surface potential, electron energy, electron flux, grain composition, and configuration (Abbas et al, 2010, 2012). In this paper, we discuss SEE charging properties of individual micron-size silica microspheres that are believed to be analogs of a class of interstellar dust grains. The measurements indicate charging of the 0.2m silica particles when exposed to 25 eV electron beams and discharging when exposed to higher energy electron beams. Relatively large size silica particles (5.2-6.82m) generally discharge to lower equilibrium potentials at both electron energies

  14. Efficient temporal shaping of electron distributions for high-brightness photoemission electron guns

    Directory of Open Access Journals (Sweden)

    Ivan V. Bazarov

    2008-04-01

    Full Text Available To achieve the lowest emittance electron bunches from photoemission electron guns, it is essential to limit the uncorrelated emittance growth due to space charge forces acting on the bunch in the vicinity of the photocathode through appropriate temporal shaping of the optical pulses illuminating the photocathode. We present measurements of the temporal profile of electron bunches from a bulk crystal GaAs photocathode illuminated with 520 nm wavelength pulses from a frequency-doubled Yb-fiber laser. A transverse deflecting rf cavity was used to make these measurements. The measured laser pulse temporal profile and the corresponding electron beam temporal profile have about 30 ps FWHM duration, with rise and fall times of a few ps. GaAs illuminated by 520 nm optical pulses is a prompt emitter within our measurement uncertainty of ∼1  ps rms. Combined with the low thermal emittance of negative electron affinity photocathodes, GaAs is a very suitable photocathode for high-brightness photoinjectors. We also report measurements of the photoemission response time for GaAsP, which show a strong dependence on the quantum efficiency of the photocathode.

  15. Charge collection efficiency in ionization chambers exposed to electron beams with high dose per pulse

    Energy Technology Data Exchange (ETDEWEB)

    Laitano, R F [Istituto Nazionale di Metrologia delle Radiazioni Ionizzanti, ENEA Centro Ricerche Casaccia, c.p. 2400 Rome (Italy); Guerra, A S [Istituto Nazionale di Metrologia delle Radiazioni Ionizzanti, ENEA Centro Ricerche Casaccia, c.p. 2400 Rome (Italy); Pimpinella, M [Istituto Nazionale di Metrologia delle Radiazioni Ionizzanti, ENEA Centro Ricerche Casaccia, c.p. 2400 Rome (Italy); Caporali, C [Istituto Nazionale di Metrologia delle Radiazioni Ionizzanti, ENEA Centro Ricerche Casaccia, c.p. 2400 Rome (Italy); Petrucci, A [A.C.O. S. Filippo Neri, U.O. Fisica Sanitaria, Rome (Italy)

    2006-12-21

    The correction for charge recombination was determined for different plane-parallel ionization chambers exposed to clinical electron beams with low and high dose per pulse, respectively. The electron energy was nearly the same (about 7 and 9 MeV) for any of the beams used. Boag's two-voltage analysis (TVA) was used to determine the correction for ion losses, k{sub s}, relevant to each chamber considered. The presence of free electrons in the air of the chamber cavity was accounted for in determining k{sub s} by TVA. The determination of k{sub s} was made on the basis of the models for ion recombination proposed in past years by Boag, Hochhaeuser and Balk to account for the presence of free electrons. The absorbed dose measurements in both low-dose-per-pulse (less than 0.3 mGy per pulse) and high-dose-per-pulse (20-120 mGy per pulse range) electron beams were compared with ferrous sulphate chemical dosimetry, a method independent of the dose per pulse. The results of the comparison support the conclusion that one of the models is more adequate to correct for ion recombination, even in high-dose-per-pulse conditions, provided that the fraction of free electrons is properly assessed. In this respect the drift velocity and the time constant for attachment of electrons in the air of the chamber cavity are rather critical parameters because of their dependence on chamber dimensions and operational conditions. Finally, a determination of the factor k{sub s} was also made by zero extrapolation of the 1/Q versus 1/V saturation curves, leading to the conclusion that this method does not provide consistent results in high-dose-per-pulse beams.

  16. Magneto-transport properties of a random distribution of few-layer graphene patches

    International Nuclear Information System (INIS)

    Iacovella, Fabrice; Mitioglu, Anatolie; Pierre, Mathieu; Raquet, Bertrand; Goiran, Michel; Plochocka, Paulina; Escoffier, Walter; Trinsoutrot, Pierre; Vergnes, Hugues; Caussat, Brigitte; Conédéra, Véronique

    2014-01-01

    In this study, we address the electronic properties of conducting films constituted of an array of randomly distributed few layer graphene patches and investigate on their most salient galvanometric features in the moderate and extreme disordered limit. We demonstrate that, in annealed devices, the ambipolar behaviour and the onset of Landau level quantization in high magnetic field constitute robust hallmarks of few-layer graphene films. In the strong disorder limit, however, the magneto-transport properties are best described by a variable-range hopping behaviour. A large negative magneto-conductance is observed at the charge neutrality point, in consistency with localized transport regime

  17. Charge transfer and excitation in high-energy ion-atom collisions

    International Nuclear Information System (INIS)

    Schlachter, A.S.; Berkner, K.H.; McDonald, R.J.

    1986-11-01

    Coincidence measurements of charge transfer and simultaneous projectile electron excitation provide insight into correlated two-electron processes in energetic ion-atom collisions. Projectile excitation and electron capture can occur simultaneously in a collision of a highly charged ion with a target atom; this process is called resonant transfer and excitation (RTE). The intermediate excited state which is thus formed can subsequently decay by photon emission or by Auger-electron emission. Results are shown for RTE in both the K shell of Ca ions and the L shell of Nb ions, for simultaneous projectile electron loss and excitation, and for the effect of RTE on electron capture

  18. Electronic excitation effects on secondary ion emission in highly charged ion-solid interaction

    International Nuclear Information System (INIS)

    Sekioka, T.; Terasawa, M.; Mitamura, T.; Stoeckli, M.P.; Lehnert, U.; Fehrenbach, C.

    2001-01-01

    In order to investigate the secondary ion emission from the surface of conductive materials bombarded by highly charged heavy ions, we have done two types of experiments. First, we have measured the yield of the sputtered ions from the surface of solid targets of conductive materials (Al, Si, Ni, Cu) bombarded by Xe q+ (q=15-44) at 300 keV (v p =0.30 a.u) and at 1.0 MeV (v p =0.54 a.u). In view of the secondary ion yields as a function of the potential energy of the projectile, the increase rates below q=35, where the potential energy amounts to 25.5 keV, were rather moderate and showed a prominent increase above q=35. These phenomena were rather strong in the case of the metal targets. Second, we have measured the energy dependence of the yield of the sputtered ions from the surface of solid targets of conductive materials (C, Al) bombarded by Xe q+ (q=30,36,44) between 76 keV (v p =0.15 a.u) and 6.0 MeV (v p =1.3 a.u). A broad enhancement of the secondary ion yield has been found for Al target bombarded by Xe 44+ . From these experimental results, the electronic excitation effects in conductive materials for impact of slow highly charged heavy ions bearing high potential energy is discussed

  19. Study of K, L vacancies production mechanisms by X spectrometry in the interaction induced by a few MeV/A charged particles

    International Nuclear Information System (INIS)

    Andriamonje, S.

    1982-01-01

    The analysis of different mechanisms producing electronic inner shell vacancies in ion atom collisions at a few MeV/A charged is presented. The mutual influence of nuclear and atomic excitation in the ionization probability has been discussed. The 106 Cd(p,p') 106 Cd reaction (Ep=10 MeV) has been particularly investigated from this point. The investigation is followed up by the description of the theoretical and experimental methods which permit the determination of the total and/or differential X rays production cross section for different interaction. The gold sub-shell L 1 , L 2 , L 3 ionization probability has been studied in the Au(H + ,H + )Au reaction at Ep=1 MeV. In the second part of the manuscript we investigate in detail the influence of the charge exchange process on inner shell vacancy production. The N 2 , Ar, Kr targets have been produced by a system jet gas and bombarded by 0.8 28 Si 14+ ions at E=125 MeV. The cross section for the capture of an electron in K shell, L shell and total charge exchange have been measured and compared to the CDW theory (Continuum Distorted Wave). In the CDW validity domain the experimental and theoretical results are a good agreement. In the collisions induced by H + , ionization is found to be the main excitation process. On the contrary, in collisions induced by 28 Si 14+ charge exchange is dominant compared to ionization [fr

  20. Exciton-dopant and exciton-charge interactions in electronically doped OLEDs

    International Nuclear Information System (INIS)

    Williams, Christopher; Lee, Sergey; Ferraris, John; Zakhidov, A. Anvar

    2004-01-01

    The electronic dopants, like tetrafluorocyanoquinodimethane (F 4 -TCNQ) molecules, used for p-doping of hole transport layers in organic light-emitting diodes (OLEDs) are found to quench the electroluminescence (EL) if they diffuse into the emissive layer. We observed EL quenching in OLED with F 4 -TCNQ doped N,N'-diphenyl-N'N'-bis(1-naphthyl)-1,1'-biphenyl-4,4'-diamine hole transport layer at large dopant concentrations, >5%. To separate the effects of exciton-dopant quenching, from exciton-polaron quenching we have intentionally doped the emissive layer of (8-tris-hydroxyquinoline) with three acceptors (A) of different electron affinities: F 4 -TCNQ, TCNQ, and C 60 , and found that C 60 is the strongest EL-quencher, while F 4 -TCNQ is the weakest, contrary to intuitive expectations. The new effects of charge transfer and usually considered energy transfer from exciton to neutral (A) and charged acceptors (A - ) are compared as channels for non-radiative Ex-A decay. At high current loads the EL quenching is observed, which is due to decay of Ex on free charge carriers, hole polarons P + . We consider contributions to Ex-P + interaction by short-range charge transfer and describe the structure of microscopic charge transfer (CT)-processes responsible for it. The formation of metastable states of 'charged excitons' (predicted and studied by Agranovich et al. Chem. Phys. 272 (2001) 159) by electron transfer from a P to an Ex is pointed out, and ways to suppress non-radiative Ex-P decay are suggested

  1. Electronic couplings for molecular charge transfer: Benchmarking CDFT, FODFT, and FODFTB against high-level ab initio calculations

    Energy Technology Data Exchange (ETDEWEB)

    Kubas, Adam; Blumberger, Jochen, E-mail: j.blumberger@ucl.ac.uk [Department of Physics and Astronomy, University College London, Gower Street, London WC1E 6BT (United Kingdom); Hoffmann, Felix [Department of Physics and Astronomy, University College London, Gower Street, London WC1E 6BT (United Kingdom); Lehrstuhl für Theoretische Chemie, Ruhr-Universität Bochum, Universitätsstr. 150, 44801 Bochum (Germany); Heck, Alexander; Elstner, Marcus [Institute of Physical Chemistry, Karlsruhe Institute of Technology, Fritz-Haber-Weg 6, 76131 Karlsruhe (Germany); Oberhofer, Harald [Department of Chemistry, Technical University of Munich, Lichtenbergstr. 4, 85747 Garching (Germany)

    2014-03-14

    We introduce a database (HAB11) of electronic coupling matrix elements (H{sub ab}) for electron transfer in 11 π-conjugated organic homo-dimer cations. High-level ab inito calculations at the multireference configuration interaction MRCI+Q level of theory, n-electron valence state perturbation theory NEVPT2, and (spin-component scaled) approximate coupled cluster model (SCS)-CC2 are reported for this database to assess the performance of three DFT methods of decreasing computational cost, including constrained density functional theory (CDFT), fragment-orbital DFT (FODFT), and self-consistent charge density functional tight-binding (FODFTB). We find that the CDFT approach in combination with a modified PBE functional containing 50% Hartree-Fock exchange gives best results for absolute H{sub ab} values (mean relative unsigned error = 5.3%) and exponential distance decay constants β (4.3%). CDFT in combination with pure PBE overestimates couplings by 38.7% due to a too diffuse excess charge distribution, whereas the economic FODFT and highly cost-effective FODFTB methods underestimate couplings by 37.6% and 42.4%, respectively, due to neglect of interaction between donor and acceptor. The errors are systematic, however, and can be significantly reduced by applying a uniform scaling factor for each method. Applications to dimers outside the database, specifically rotated thiophene dimers and larger acenes up to pentacene, suggests that the same scaling procedure significantly improves the FODFT and FODFTB results for larger π-conjugated systems relevant to organic semiconductors and DNA.

  2. Nanometer-size surface modification produced by single, low energy, highly charged ions

    International Nuclear Information System (INIS)

    Stockli, M.P.

    1994-01-01

    Atomically flat surfaces of insulators have been bombarded with low energy, highly charged ions to search for nanometer-size surface modifications. It is expected that the high electron deficiency of highly charged ions will capture and/or remove many of the insulator's localized electrons when impacting on an insulating surface. The resulting local electron deficiency is expected to locally disintegrate the insulator through a open-quotes Coulomb explosionclose quotes forming nanometer-size craters. Xe ions with charge states between 10+ and 45+ and kinetic energies between 0 and 10 keV/q were obtained from the KSU-CRYEBIS, a CRYogenic Electron Beam Ion Source and directed onto various insulating materials. Mica was favored as target material as atomically flat surfaces can be obtained reliably through cleaving. However, the authors observations with an atomic force microscope have shown that mica tends to defoliate locally rather than disintegrate, most likely due to the small binding forces between adjacent layers. So far the authors measurements indicate that each ion produces one blister if the charge state is sufficiently high. The blistering does not seem to depend very much on the kinetic energy of the ions

  3. Secondary Electron Emission from Dust and Its Effect on Charging

    Science.gov (United States)

    Saikia, B. K.; Kakati, B.; Kausik, S. S.; Bandyopadhyay, M.

    2011-11-01

    Hydrogen plasma is produced in a plasma chamber by striking discharge between incandescent tungsten filaments and the permanent magnetic cage [1], which is grounded. The magnetic cage has a full line cusped magnetic field geometry used to confine the plasma elements. A cylindrical Langmuir probe is used to study the plasma parameters in various discharge conditions. The charge accumulated on the dust particles is calculated using the capacitance model and the dust current is measured by the combination of a Faraday cup and an electrometer at different discharge conditions. It is found Secondary electron emission from dust having low emission yield effects the charging of dust particles in presence of high energetic electrons.

  4. Secondary Electron Emission from Dust and Its Effect on Charging

    International Nuclear Information System (INIS)

    Saikia, B. K.; Kakati, B.; Kausik, S. S.; Bandyopadhyay, M.

    2011-01-01

    Hydrogen plasma is produced in a plasma chamber by striking discharge between incandescent tungsten filaments and the permanent magnetic cage [1], which is grounded. The magnetic cage has a full line cusped magnetic field geometry used to confine the plasma elements. A cylindrical Langmuir probe is used to study the plasma parameters in various discharge conditions. The charge accumulated on the dust particles is calculated using the capacitance model and the dust current is measured by the combination of a Faraday cup and an electrometer at different discharge conditions. It is found Secondary electron emission from dust having low emission yield effects the charging of dust particles in presence of high energetic electrons.

  5. Nonlinear dust acoustic waves in a charge varying dusty plasma with suprathermal electrons

    International Nuclear Information System (INIS)

    Tribeche, Mouloud; Bacha, Mustapha

    2010-01-01

    Arbitrary amplitude dust acoustic waves in a dusty plasma with a high-energy-tail electron distribution are investigated. The effects of charge variation and electron deviation from the Boltzmann distribution on the dust acoustic soliton are then considered. The dust charge variation makes the dust acoustic soliton more spiky. The dust grain surface collects less electrons as the latter evolves far away from their thermodynamic equilibrium. The dust accumulation caused by a balance of the electrostatic forces acting on the dust grains is more effective for lower values of the electron spectral index. Under certain conditions, the dust charge fluctuation may provide an alternate physical mechanism causing anomalous dissipation, the strength of which becomes important and may prevail over that of dispersion as the suprathermal character of the plasma becomes important. Our results may explain the strong spiky waveforms observed in auroral plasmas.

  6. Electron beam charging of insulators: A self-consistent flight-drift model

    International Nuclear Information System (INIS)

    Touzin, M.; Goeuriot, D.; Guerret-Piecourt, C.; Juve, D.; Treheux, D.; Fitting, H.-J.

    2006-01-01

    Electron beam irradiation and the self-consistent charge transport in bulk insulating samples are described by means of a new flight-drift model and an iterative computer simulation. Ballistic secondary electron and hole transport is followed by electron and hole drifts, their possible recombination and/or trapping in shallow and deep traps. The trap capture cross sections are the Poole-Frenkel-type temperature and field dependent. As a main result the spatial distributions of currents j(x,t), charges ρ(x,t), the field F(x,t), and the potential slope V(x,t) are obtained in a self-consistent procedure as well as the time-dependent secondary electron emission rate σ(t) and the surface potential V 0 (t). For bulk insulating samples the time-dependent distributions approach the final stationary state with j(x,t)=const=0 and σ=1. Especially for low electron beam energies E 0 G of a vacuum grid in front of the target surface. For high beam energies E 0 =10, 20, and 30 keV high negative surface potentials V 0 =-4, -14, and -24 kV are obtained, respectively. Besides open nonconductive samples also positive ion-covered samples and targets with a conducting and grounded layer (metal or carbon) on the surface have been considered as used in environmental scanning electron microscopy and common SEM in order to prevent charging. Indeed, the potential distributions V(x) are considerably small in magnitude and do not affect the incident electron beam neither by retarding field effects in front of the surface nor within the bulk insulating sample. Thus the spatial scattering and excitation distributions are almost not affected

  7. Space shuttle charging or beam-plasma discharge: What can electron spectrometer observations contribute to solving the question?

    International Nuclear Information System (INIS)

    Watermann, J.; Wilhelm, K.; Torkar, K.M.; Riedler, W.

    1988-01-01

    Several cooperative plasma experiments were carried out on board Spacelab-1, the ninth payload of the Space Transportation System (STS-9). Among them, the electron spectrometer 1ES019A was designed to observe 01.-12.5 keV electron fluxes with high temporal and spatial resolution, while the SEPAC electron beam accelerator emitted electron beams with currents up to 280 mA and maximum energies of 5 keV. Since the question of orbiter charging to high voltages has controversially been discussed in several publications on STS-3 and STS-9 electron beam experiments, an attempt is made to relate information from the return electron flux observed during the SEPAC operations to the vehicle charging interpretation. A close examination reveals that most of our observations can be understood if the occurrence of a beam-plasma discharge is assumed at least for electron beam intensities above 100 mA. This would provide a substantial return current capability. High orbiter charging effects during electron beam accelerator electron emissions are consequently not supported by the observations

  8. Attraction of likely charged nano-sized grains in dust-electron plasmas

    Energy Technology Data Exchange (ETDEWEB)

    Vishnyakov, Vladimir I., E-mail: eksvar@ukr.net [Physical-Chemical Institute for Environmental and Human Protection, Odessa 65082 (Ukraine)

    2016-01-15

    Dust-electron plasma, which contains only the dust grains and electrons, emitted by them, is studied. Assumption of almost uniform spatial electrons distribution, which deviates from the uniformity only near the dust grains, leads to the grain charge division into two parts: first part is the individual for each grain “visible” charge and the second part is the common charge of the neutralized background. The visible grain charge can be both negative and positive, while the total grain charge is only positive. The attraction of likely charged grains is possible, because the grain interaction is determined by the visible charges. The equilibrium state between attraction and repulsion of grains is demonstrated.

  9. Space-charge dynamics of polymethylmethacrylate under electron beam irradiation

    CERN Document Server

    Gong, H; Ong, C K

    1997-01-01

    Space-charge dynamics of polymethylmethacrylate (PMMA) under electron beam irradiation has been investigated employing a scanning electron microscope. Assuming a Gaussian space-charge distribution, the distribution range (sigma) has been determined using a time-resolved current method in conjunction with a mirror image method. sigma is found to increase with irradiation time and eventually attain a stationary value. These observations have been discussed by taking into account radiation-induced conductivity and charge mobility. (author)

  10. Charging effects of PET under electron beam irradiation in a SEM

    International Nuclear Information System (INIS)

    Jbara, O; Rondot, S; Hadjadj, A; Patat, J M; Fakhfakh, S; Belhaj, M

    2008-01-01

    This paper deals with charge trapping and charge transport of polyethylene terephthalate (PET) polymer subjected to electron irradiation in a scanning electron microscope (SEM). Measurement of displacement current and leakage current using an arrangement adapted to the SEM allows the amount of trapped charge during and after electron irradiation to be determined and the charge mechanisms regulation to be studied. These mechanisms involve several parameters related to the electronic injection, the characteristics of insulator and the effects of the trapped charge itself. The dynamic trapping properties of PET samples are investigated and the time constants of charging are evaluated for various conditions of irradiation. The determination of the trapping cross section for electrons is possible by using the trapping rate at the onset of irradiation. Many physical processes are involved in the charging and discharging mechanisms; among them surface conduction is outlined. Through the control of irradiation conditions, various types of surface discharging (flashover phenomenon) behaviour are also observed. The strength of the electric field initiating surface discharge is estimated.

  11. Few-layered MoSe2 nanosheets as an advanced electrode material for supercapacitors.

    Science.gov (United States)

    Balasingam, Suresh Kannan; Lee, Jae Sung; Jun, Yongseok

    2015-09-21

    We report the synthesis of few-layered MoSe2 nanosheets using a facile hydrothermal method and their electrochemical charge storage behavior. A systematic study of the structure and morphology of the as-synthesized MoSe2 nanosheets was performed. The downward peak shift in the Raman spectrum and the high-resolution transmission electron microscopy images confirmed the formation of few-layered nanosheets. The electrochemical energy-storage behavior of MoSe2 nanosheets was also investigated for supercapacitor applications in a symmetric cell configuration. The MoSe2 nanosheet electrode exhibited a maximum specific capacitance of 198.9 F g(-1) and the symmetric device showed 49.7 F g(-1) at a scan rate of 2 mV s(-1). A capacitance retention of approximately 75% was observed even after 10 000 cycles at a high charge-discharge current density of 5 A g(-1). The two-dimensional MoSe2 nanosheets exhibited a high specific capacitance and good cyclic stability, which makes it a promising electrode material for supercapacitor applications.

  12. Electron Beam Charge Diagnostics for Laser Plasma Accelerators

    International Nuclear Information System (INIS)

    Nakamura, Kei; Gonsalves, Anthony; Lin, Chen; Smith, Alan; Rodgers, David; Donahue, Rich; Byrne, Warren; Leemans, Wim

    2011-01-01

    A comprehensive study of charge diagnostics is conducted to verify their validity for measuring electron beams produced by laser plasma accelerators (LPAs). First, a scintillating screen (Lanex) was extensively studied using subnanosecond electron beams from the Advanced Light Source booster synchrotron, at the Lawrence Berkeley National Laboratory. The Lanex was cross calibrated with an integrating current transformer (ICT) for up to the electron energy of 1.5 GeV, and the linear response of the screen was confirmed for charge density and intensity up to 160 pC/mm 2 and 0.4 pC/(ps mm 2 ), respectively. After the radio-frequency accelerator based cross calibration, a series of measurements was conducted using electron beams from an LPA. Cross calibrations were carried out using an activation-based measurement that is immune to electromagnetic pulse noise, ICT, and Lanex. The diagnostics agreed within ±8%, showing that they all can provide accurate charge measurements for LPAs.

  13. Electron beam charge diagnostics for laser plasma accelerators

    Directory of Open Access Journals (Sweden)

    K. Nakamura

    2011-06-01

    Full Text Available A comprehensive study of charge diagnostics is conducted to verify their validity for measuring electron beams produced by laser plasma accelerators (LPAs. First, a scintillating screen (Lanex was extensively studied using subnanosecond electron beams from the Advanced Light Source booster synchrotron, at the Lawrence Berkeley National Laboratory. The Lanex was cross calibrated with an integrating current transformer (ICT for up to the electron energy of 1.5 GeV, and the linear response of the screen was confirmed for charge density and intensity up to 160  pC/mm^{2} and 0.4  pC/(ps  mm^{2}, respectively. After the radio-frequency accelerator based cross calibration, a series of measurements was conducted using electron beams from an LPA. Cross calibrations were carried out using an activation-based measurement that is immune to electromagnetic pulse noise, ICT, and Lanex. The diagnostics agreed within ±8%, showing that they all can provide accurate charge measurements for LPAs.

  14. Determination of the Electronics Charge--Electrolysis of Water Method.

    Science.gov (United States)

    Venkatachar, Arun C.

    1985-01-01

    Presents an alternative method for measuring the electronic charge using data from the electrolysis of acidified distilled water. The process (carried out in a commercially available electrolytic cell) has the advantage of short completion time so that students can determine electron charge and mass in one laboratory period. (DH)

  15. Highly mobile charge-transfer excitons in two-dimensional WS2/tetracene heterostructures

    Science.gov (United States)

    Zhu, Tong; Yuan, Long; Zhao, Yan; Zhou, Mingwei; Wan, Yan; Mei, Jianguo; Huang, Libai

    2018-01-01

    Charge-transfer (CT) excitons at heterointerfaces play a critical role in light to electricity conversion using organic and nanostructured materials. However, how CT excitons migrate at these interfaces is poorly understood. We investigate the formation and transport of CT excitons in two-dimensional WS2/tetracene van der Waals heterostructures. Electron and hole transfer occurs on the time scale of a few picoseconds, and emission of interlayer CT excitons with a binding energy of ~0.3 eV has been observed. Transport of the CT excitons is directly measured by transient absorption microscopy, revealing coexistence of delocalized and localized states. Trapping-detrapping dynamics between the delocalized and localized states leads to stretched-exponential photoluminescence decay with an average lifetime of ~2 ns. The delocalized CT excitons are remarkably mobile with a diffusion constant of ~1 cm2 s−1. These highly mobile CT excitons could have important implications in achieving efficient charge separation. PMID:29340303

  16. Contribution of charge-transfer processes to ion-induced electron emission

    International Nuclear Information System (INIS)

    Roesler, M.; Garcia de Abajo, F.J.

    1996-01-01

    Charge changing events of ions moving inside metals are shown to contribute significantly to electron emission in the intermediate velocity regime via electrons coming from projectile ionization. Inclusion of equilibrium charge state fractions, together with two-electron Auger processes and resonant-coherent electron loss from the projectile, results in reasonable agreement with previous calculations for frozen protons, though a significant part of the emission is now interpreted in terms of charge exchange. The quantal character of the surface barrier transmission is shown to play an important role. The theory compares well with experimental observations for H projectiles. copyright 1996 The American Physical Society

  17. Three-dimensional space charge distribution measurement in electron beam irradiated PMMA

    International Nuclear Information System (INIS)

    Imaizumi, Yoichi; Suzuki, Ken; Tanaka, Yasuhiro; Takada, Tatsuo

    1996-01-01

    The localized space charge distribution in electron beam irradiated PMMA was investigated using pulsed electroacoustic method. Using a conventional space charge measurement system, the distribution only in the depth direction (Z) can be measured assuming the charges distributed uniformly in the horizontal (X-Y) plane. However, it is difficult to measure the distribution of space charge accumulated in small area. Therefore, we have developed the new system to measure the three-dimensional space charge distribution using pulsed electroacoustic method. The system has a small electrode with a diameter of 1mm and a motor-drive X-Y stage to move the sample. Using the data measured at many points, the three-dimensional distribution were obtained. To estimate the system performance, the electron beam irradiated PMMA was used. The electron beam was irradiated from transmission electron microscope (TEM). The depth of injected electron was controlled using the various metal masks. The measurement results were compared with theoretically calculated values of electron range. (author)

  18. Electronic structure of fractionally nuclear charged atoms

    International Nuclear Information System (INIS)

    Pavao, Antonio C.; Bastos, Cristiano C.; Ferreira, Joacy V.

    2008-01-01

    Different properties of quark chemistry are studied by performing accurate ab initio Hartree- Fock calculations on fractionally nuclear charged atoms. Ground and first excited states of sodium atoms with quarks attached to the nucleus are obtained using CI calculations. It is suggested that the sodium 2 P -> 2 S electronic transition can be used as a guide in searching for unconfined quarks. Also, the variation of the binding electronic energy with nuclear charge in the isoelectronic series of fractionally nuclear charged atoms A ±2/3 and A ±1/3 (A = H, Li, Na, P and Ca) is analyzed. The present calculations suggest that unconfined colored particles have large appetite for heavy nuclei and that quark-antiquark pairs could be stabilized in presence of the atomic matter. (author)

  19. Investigation of electron-beam charging for inertial-confinement-fusion targets. Charged Particle Research Laboratory report No. 3-82

    International Nuclear Information System (INIS)

    Kim, K.; Elsayed-Ali, H.E.

    1982-04-01

    Techniques for charging inertial confinement fusion targets using electron beam are investigated. A brief review of the various possible charging techniques is presented, along with a discussion of the advantages and disadvantages of each. The reasons for selecting the electron beam charging and a physical picture of the charging mechanism are described. Experimental results are presented and compared with the theoretical predictions

  20. Charging of insulators by multiply-charged-ion impact probed by slowing down of fast binary-encounter electrons

    Science.gov (United States)

    de Filippo, E.; Lanzanó, G.; Amorini, F.; Cardella, G.; Geraci, E.; Grassi, L.; La Guidara, E.; Lombardo, I.; Politi, G.; Rizzo, F.; Russotto, P.; Volant, C.; Hagmann, S.; Rothard, H.

    2010-12-01

    The interaction of ion beams with insulators leads to charging-up phenomena, which at present are under investigation in connection with guiding phenomena in nanocapillaries with possible application in nanofocused beams. We studied the charging dynamics of insulating foil targets [Mylar, polypropylene (PP)] irradiated with swift ion beams (C, O, Ag, and Xe at 40, 23, 40, and 30 MeV/u, respectively) via the measurement of the slowing down of fast binary-encounter electrons. Also, sandwich targets (Mylar covered with a thin Au layer on both surfaces) and Mylar with Au on only one surface were used. Fast-electron spectra were measured by the time-of-flight method at the superconducting cyclotron of Laboratori Nazionali del Sud (LNS) Catania. The charge buildup leads to target-material-dependent potentials of the order of 6.0 kV for Mylar and 2.8 kV for PP. The sandwich targets, surprisingly, show the same behavior as the insulating targets, whereas a single Au layer on the electron and ion exit side strongly suppresses the charging phenomenon. The accumulated number of projectiles needed for charging up is inversely proportional to electronic energy loss. Thus, the charging up is directly related to emission of secondary electrons.

  1. Charging of insulators by multiply-charged-ion impact probed by slowing down of fast binary-encounter electrons

    International Nuclear Information System (INIS)

    De Filippo, E.; Lanzano, G.; Cardella, G.; Amorini, F.; Geraci, E.; Grassi, L.; Politi, G.; La Guidara, E.; Lombardo, I.; Rizzo, F.; Russotto, P.; Volant, C.; Hagmann, S.; Rothard, H.

    2010-01-01

    The interaction of ion beams with insulators leads to charging-up phenomena, which at present are under investigation in connection with guiding phenomena in nanocapillaries with possible application in nanofocused beams. We studied the charging dynamics of insulating foil targets [Mylar, polypropylene (PP)] irradiated with swift ion beams (C, O, Ag, and Xe at 40, 23, 40, and 30 MeV/u, respectively) via the measurement of the slowing down of fast binary-encounter electrons. Also, sandwich targets (Mylar covered with a thin Au layer on both surfaces) and Mylar with Au on only one surface were used. Fast-electron spectra were measured by the time-of-flight method at the superconducting cyclotron of Laboratori Nazionali del Sud (LNS) Catania. The charge buildup leads to target-material-dependent potentials of the order of 6.0 kV for Mylar and 2.8 kV for PP. The sandwich targets, surprisingly, show the same behavior as the insulating targets, whereas a single Au layer on the electron and ion exit side strongly suppresses the charging phenomenon. The accumulated number of projectiles needed for charging up is inversely proportional to electronic energy loss. Thus, the charging up is directly related to emission of secondary electrons.

  2. Space Charge Saturated Sheath Regime and Electron Temperature Saturation in Hall Thrusters

    International Nuclear Information System (INIS)

    Raitses, Y.; Staack, D.; Smirnov, A.; Fisch, N.J.

    2005-01-01

    Secondary electron emission in Hall thrusters is predicted to lead to space charge saturated wall sheaths resulting in enhanced power losses in the thruster channel. Analysis of experimentally obtained electron-wall collision frequency suggests that the electron temperature saturation, which occurs at high discharge voltages, appears to be caused by a decrease of the Joule heating rather than by the enhancement of the electron energy loss at the walls due to a strong secondary electron emission

  3. Laser wakefield acceleration with high-power, few-cycle mid-IR lasers

    OpenAIRE

    Papp, Daniel; Wood, Jonathan C.; Gruson, Vincent; Bionta, Mina; Gruse, Jan-Niclas; Cormier, Eric; Najmudin, Zulfikar; Légaré, François; Kamperidis, Christos

    2018-01-01

    The study of laser wakefield electron acceleration (LWFA) using mid-IR laser drivers is a promising path for future laser driven electronaccelerators, when compared to traditional near-IR laser drivers uperating at 0.8-1 {\\mu}m central wavelength ({\\lambda}laser), as the necessary vector potential a_0 for electron injection can be achieved with smaller laser powers due to the linear dependence on {\\lambda}laser. In this work, we perform 2D PIC simulations on LWFA using few-cycle high power (5...

  4. Electron cyclotron resonance (E.C.R.) multiply charged ion sources

    International Nuclear Information System (INIS)

    Geller, R.

    1978-01-01

    High charge state ions can be produced by electron bombardment inside targets when the target electron density n (cm -3 ) multiplied by the ion transit time through the target tau (sec) is: n tau > 5.10 9 cm -3 sec. The relative velocity between electrons and ions determines the balance between stripping and capture i.e. the final ion charge state. (In a stripper foil fast ions interact with slow electrons involving typically n approximately 10 24 cm -3 , tau approximately 10 -14 sec). In the E.C.R. source a cold ion plasma created in a first stage diffuses slowly through a second stage containing a hot E.C.R. plasma with n > 3.10 11 cm -3 and tau > 10 -2 sec. Continuous beams of several μA of C 6+ N 7+ Ne 9+ A 11+ are extracted from the second stage with normalized emittances of approximately 0.5 π mm mrad. The absence of cathodes and plasma arcs makes the source very robust, reliable and well-fitted for cyclotron injection. A super conducting source is under development

  5. The Eindhoven High-Brightness Electron Programme

    NARCIS (Netherlands)

    Brussaard, G.J.H.; Wiel, van der M.J.

    2004-01-01

    The Eindhoven High-Brightness programme is aimed at producing ultra-short intense electron bunches from compact accelerators. The RF electron gun is capable of producing 100 fs electron bunches at 7.5 MeV and 10 pC bunch charge. The DC/RF hybrid gun under development will produce bunches <75 fs at

  6. Carrier mobility and scattering lifetime in electric double-layer gated few-layer graphene

    Energy Technology Data Exchange (ETDEWEB)

    Piatti, E.; Galasso, S.; Tortello, M.; Nair, J.R.; Gerbaldi, C. [Dipartimento di Scienza Applicata e Tecnologia, Politecnico di Torino, 10129 Torino (Italy); Bruna, M.; Borini, S. [Istituto Nazionale di Ricerca Metrologica (INRIM), 10135 Torino (Italy); Daghero, D. [Dipartimento di Scienza Applicata e Tecnologia, Politecnico di Torino, 10129 Torino (Italy); Gonnelli, R.S., E-mail: renato.gonnelli@polito.it [Dipartimento di Scienza Applicata e Tecnologia, Politecnico di Torino, 10129 Torino (Italy)

    2017-02-15

    Highlights: • We fabricated few-layer graphene FETs by mechanical exfoliation and standard microfabrication techniques. • We employed a Li-TFSI based ion gel to induce carrier densities as high as ≈6e14 e{sup −}/cm{sup 2} in the devices' channel. • We found a strong asymmetry in the sheet conductance and mobility doping dependences between electron and hole doping. • We combined the experimental results with ab initio DFT calculations to obtain the average scattering lifetime of the charge carriers. • We found that the increase in the carrier density and an unexpected increase in the density of charged scattering centers compete in determining the scattering lifetime. - Abstract: We fabricate electric double-layer field-effect transistor (EDL-FET) devices on mechanically exfoliated few-layer graphene. We exploit the large capacitance of a polymeric electrolyte to study the transport properties of three, four and five-layer samples under a large induced surface charge density both above and below the glass transition temperature of the polymer. We find that the carrier mobility shows a strong asymmetry between the hole and electron doping regime. We then employ ab initio density functional theory (DFT) calculations to determine the average scattering lifetime from the experimental data. We explain its peculiar dependence on the carrier density in terms of the specific properties of the electrolyte we used in our experiments.

  7. Effect of collective response on electron capture and excitation in collisions of highly charged ions with fullerenes.

    Science.gov (United States)

    Kadhane, U; Misra, D; Singh, Y P; Tribedi, Lokesh C

    2003-03-07

    Projectile deexcitation Lyman x-ray emission following electron capture and K excitation has been studied in collisions of bare and Li-like sulphur ions (of energy 110 MeV) with fullerenes (C(60)/C(70)) and different gaseous targets. The intensity ratios of different Lyman x-ray lines in collisions with fullerenes are found to be substantially lower than those for the gas targets, both for capture and excitation. This has been explained in terms of a model based on "solidlike" effect, namely, wakefield induced stark mixing of the excited states populated via electron capture or K excitation: a collective phenomenon of plasmon excitation in the fullerenes under the influence of heavy, highly charged ions.

  8. Computer simulations analysis for determining the polarity of charge generated by high energy electron irradiation of a thin film

    DEFF Research Database (Denmark)

    Malac, Marek; Hettler, Simon; Hayashida, Misa

    2017-01-01

    Detailed simulations are necessary to correctly interpret the charge polarity of electron beam irradiated thin film patch. Relying on systematic simulations we provide guidelines and movies to interpret experimentally the polarity of the charged area, to be understood as the sign of the electrost......Detailed simulations are necessary to correctly interpret the charge polarity of electron beam irradiated thin film patch. Relying on systematic simulations we provide guidelines and movies to interpret experimentally the polarity of the charged area, to be understood as the sign...... of the electrostatic potential developed under the beam with reference to a ground electrode. We discuss the two methods most frequently used to assess charge polarity: Fresnel imaging of the irradiated area and Thon rings analysis. We also briefly discuss parameter optimization for hole free phase plate (HFPP...

  9. Optical pumping of electron and nuclear spin in a negatively-charged quantum dot

    Science.gov (United States)

    Bracker, Allan; Gershoni, David; Korenev, Vladimir

    2005-03-01

    We report optical pumping of electron and nuclear spins in an individual negatively-charged quantum dot. With a bias-controlled heterostructure, we inject one electron into the quantum dot. Intense laser excitation produces negative photoluminescence polarization, which is easily erased by the Hanle effect, demonstrating optical pumping of a long-lived resident electron. The electron spin lifetime is consistent with the influence of nuclear spin fluctuations. Measuring the Overhauser effect in high magnetic fields, we observe a high degree of nuclear spin polarization, which is closely correlated to electron spin pumping.

  10. A high charge state heavy ion beam source for HIF

    International Nuclear Information System (INIS)

    Eylon, S.; Henestroza, E.

    1995-04-01

    A high current low emittance high charge state heavy ion beam source is being developed. This is designed to deliver HIF (heavy ion fusion) driver accelerator scale beam. Using high-charge-state beam in a driver accelerator for HIF may increase the acceleration efficiency, leading to a reduction in the driver accelerator size and cost. The proposed source system which consists of the gas beam electron stripper followed by a high charge state beam separator, can be added to existing single charge state, low emittance, high brightness ion sources and injectors. We shall report on the source physics design using 2D beam envelope simulations and experimental feasibility studies' results using a neutral gas stripper and a beam separator at the exit of the LBL 2 MV injector

  11. To the theory of spin-charge separation in one-dimensional correlated electron systems

    International Nuclear Information System (INIS)

    Zvyagin, A.A.

    2004-01-01

    Spin-charge separation is considered to be one of the key properties that distinguish low-dimensional electron systems from others. Three-dimensional correlated electron systems are described by the Fermi liquid theory. There, low-energy excitations (quasiparticles) are reminiscent of noninteracting electrons: They carry charges -e and spins 1/2 . It is believed that for any one-dimensional correlated electron system, low-lying electron excitations carry either only spin and no charge, or only charge without spin. That is why recent experiments looked for such low-lying collective electron excitations, one of which carries only spin, and the other carries only charge. Here we show that despite the fact that for exactly solvable one-dimensional correlated electron models there exist excitations which carry only spin and only charge, in all these models with short-range interactions the low-energy physics is described by low-lying collective excitations, one of which carries both spin and charge

  12. High Pressure Optical Studies of the Thallous Halides and of Charge-Transfer Complexes

    Science.gov (United States)

    Jurgensen, Charles Willard

    High pressure was used to study the insulator -to-metal transition in sulfur and the thallous halides and to study the intermolecular interactions in charge -transfer complexes. The approach to the band overlap insulator -to-metal transition was studied in three thallous halides and sulfur by optical absorption measurements of the band gap as a function of pressure. The band gap of sulfur continuously decreases with pressure up to the insulator -to-metal transition which occurs between 450 and 485 kbars. The results on the thallous halides indicate that the indirect gap decreases more rapidly than the direct gap; the closing of the indirect gap is responsible for the observed insulator -to-metal transitions. High pressure electronic and vibrational spectroscopic measurements on the solid-state complexes of HMB-TCNE were used to study the intermolecular interactions of charge -transfer complexes. The vibrational frequency shifts indicate that the degree of charge transfer increases with pressure which is independently confirmed by an increase in the molar absorptivity of the electronic charge-transfer peak. Induction and dispersion forces contribute towards a red shift of the charge-transfer peak; however, charge-transfer resonance contributes toward a blue shift and this effect is dominant for the HMB-TCNE complexes. High pressure electronic spectra were used to study the effect of intermolecular interactions on the electronic states of TCNQ and its complexes. The red shifts with pressure of the electronic spectra of TCNQ and (TCNQ)(' -) in polymer media and of crystalline TCNQ can be understood in terms of Van der Waals interactions. None of the calculations which considered intradimer distance obtained the proper behavior for either the charge-transfer of the locally excited states of the complexes. The qualitative behavior of both states can be interpreted as the effect of increased mixing of the locally excited and charge transfer states.

  13. Highly solvatochromic emission of electron donor-acceptor compounds containing propanedioato boron electron acceptors

    NARCIS (Netherlands)

    Brouwer, A.M.; Bakker, N.A.C.; Wiering, P.G.; Verhoeven, J.W.

    1991-01-01

    Light-induced electron transfer occurs in bifunctional compounds consisting of 1,3-diphenylpropanedioato boron oxalate or fluoride electron acceptors and simple aromatic electron-donor groups, linked by a methylene bridge; fluorescence from the highly polar charge-transfer excited state is

  14. Charge-state correlated cross sections for the production of low-velocity highly charged Ne ions by heavy-ion bombardment

    International Nuclear Information System (INIS)

    Gray, T.J.; Cocke, C.L.; Justiniano, E.

    1980-01-01

    We report measured cross sections for the collisional production of highly charged low-velocity Ne recoil ions resulting from the bombardment of a thin Ne gas target by highly charged 1-MeV/amu C, N, O, and F projectiles. The measurements were made using time-of-flight techniques which allowed the simultaneous identification of the final charge state of both the low-velocity recoil ion and the high-velocity projectile for each collision event. For a given incident-projectile charge state, the recoil charge-state distribution is very dependent upon the final charge state of the projectile. Single- and double-electron capture events by incident bare nuclei and projectile K-shell ionization during the collision cause large shifts in the recoil charge-state distributions toward higher charge states. A previously proposed energy-deposition model is modified to include the effects of projectile charge-changing collisions during the collision for bare and hydrogenlike projectiles and is used to discuss the present experimental results

  15. Mechanisms for production of highly charged ions

    International Nuclear Information System (INIS)

    McGuire, J.H.

    1987-01-01

    Various experimental data at high collision velocity are interpreted in terms of direct (D) and rearrangement (R) mechanisms for production of multiply charged ions. We consider double ionization in helium by protons, electrons, heavy ions, antiprotons, positrons and photons. Qualitative differences are discussed in the context of the R and D mechanisms. Multiple ionization in many electron atoms is considered as is simultaneous capture and ionization and fragmentation of methane molecules. Some other theoretical methods are briefly discussed. (orig.)

  16. Stochastic Coulomb interactions in space charge limited electron emission

    International Nuclear Information System (INIS)

    Nijkerk, M.D.; Kruit, P.

    2004-01-01

    Emission models that form the basis of self-consistent field computations make use of the approximation that emitted electrons form a smooth space charge jelly. In reality, electrons are discrete particles that are subject to statistical Coulomb interactions. A Monte Carlo simulation tool is used to evaluate the influence of discrete space charge effects on self-consistent calculations of cathode-ray tube optics. We find that interactions in the space charge cloud affect the electron trajectories such that the velocity distribution is Maxwellian, regardless of the current density. Interactions near the emitter effectively conserve the Maxwellian distribution. The surprising result is that the width of the distribution of transversal velocities does not change. The distribution of longitudinal velocities does broaden, as expected from existing theories

  17. Secondary electron/reflected particle coincidence studies during slow highly charged ion-surface interactions

    Energy Technology Data Exchange (ETDEWEB)

    McGrath, C.T.; Szilagyi, Z.; Shah, M.B.; McCullough, R.W. [Queen' s Univ., Belfast, Northern Ireland (United Kingdom); Woolsey, J.M. [Stirling Univ. (United Kingdom). DBMS; Trassl, R.; Salzborn, E. [Giessen Univ. (Germany). Inst. fuer Kernphysik

    2001-07-01

    We have measured the secondary electron emission statistics (ES) for 5 keV N{sup q+} (q = 1-4) ions incident at 10 on polycrystalline aluminium, in coincidence with specularly reflected N{sup 0}. In this arrangement the kinetic contribution to secondary electron emission is minimised. The experimental data shows that the coincident electron yield, {gamma}, increases linearly with incident ion charge state. The kinetic emission contribution has also been determined from this data. The ES due to 2 and 4 keV He{sup 2+} impact on polycrystalline aluminium in coincidence with specularly reflected He{sup +} and He{sup 0} have also been determined. The process He{sup 2+} {yields} He{sup 0} yields a larger {gamma} value than the process He{sup 2+} {yields} He{sup +}. (orig.)

  18. Control of single-electron charging of metallic nanoparticles onto amorphous silicon surface.

    Science.gov (United States)

    Weis, Martin; Gmucová, Katarína; Nádazdy, Vojtech; Capek, Ignác; Satka, Alexander; Kopáni, Martin; Cirák, Július; Majková, Eva

    2008-11-01

    Sequential single-electron charging of iron oxide nanoparticles encapsulated in oleic acid/oleyl amine envelope and deposited by the Langmuir-Blodgett technique onto Pt electrode covered with undoped hydrogenated amorphous silicon film is reported. Single-electron charging (so-called quantized double-layer charging) of nanoparticles is detected by cyclic voltammetry as current peaks and the charging effect can be switched on/off by the electric field in the surface region induced by the excess of negative/positive charged defect states in the amorphous silicon layer. The particular charge states in amorphous silicon are created by the simultaneous application of a suitable bias voltage and illumination before the measurement. The influence of charged states on the electric field in the surface region is evaluated by the finite element method. The single-electron charging is analyzed by the standard quantized double layer model as well as two weak-link junctions model. Both approaches are in accordance with experiment and confirm single-electron charging by tunnelling process at room temperature. This experiment illustrates the possibility of the creation of a voltage-controlled capacitor for nanotechnology.

  19. Macroscopic charge quantization in single-electron devices

    NARCIS (Netherlands)

    Burmistrov, I.S.; Pruisken, A.M.M.

    2010-01-01

    In a recent paper by the authors [I. S. Burmistrov and A. M. M. Pruisken, Phys. Rev. Lett. 101, 056801 (2008)] it was shown that single-electron devices (single-electron transistor or SET) display "macroscopic charge quantization" which is completely analogous to the quantum Hall effect observed on

  20. Transverse Space-Charge Field-Induced Plasma Dynamics for Ultraintense Electron-Beam Characterization

    Directory of Open Access Journals (Sweden)

    R. Tarkeshian

    2018-05-01

    Full Text Available Similarly to laser or x-ray beams, the interaction of sufficiently intense particle beams with neutral gases will result in the creation of plasma. In contrast to photon-based ionization, the strong unipolar field of a particle beam can generate a plasma where the electron population receives a large initial momentum kick and escapes, leaving behind unshielded ions. Measuring the properties of the ensuing Coulomb exploding ions—such as their kinetic energy distribution, yield, and spatial distribution—can provide information about the peak electric fields that are achieved in the electron beams. Particle-in-cell simulations and analytical models are presented for high-brightness electron beams of a few femtoseconds or even hundreds of attoseconds, and transverse beam sizes on the micron scale, as generated by today’s free electron lasers. Different density regimes for the utilization as a potential diagnostics are explored, and the fundamental differences in plasma dynamical behavior for e-beam or photon-based ionization are highlighted. By measuring the dynamics of field-induced ions for different gas and beam densities, a lower bound on the beam charge density can be obtained in a single shot and in a noninvasive way. The exponential dependency of the ionization yield on the beam properties can provide unprecedented spatial and temporal resolution, at the submicrometer and subfemtosecond scales, respectively, offering a practical and powerful approach to characterizing beams from accelerators at the frontiers of performance.

  1. Few-layer molybdenum disulfide transistors and circuits for high-speed flexible electronics.

    Science.gov (United States)

    Cheng, Rui; Jiang, Shan; Chen, Yu; Liu, Yuan; Weiss, Nathan; Cheng, Hung-Chieh; Wu, Hao; Huang, Yu; Duan, Xiangfeng

    2014-10-08

    Two-dimensional layered materials, such as molybdenum disulfide, are emerging as an exciting material system for future electronics due to their unique electronic properties and atomically thin geometry. Here we report a systematic investigation of MoS2 transistors with optimized contact and device geometry, to achieve self-aligned devices with performance including an intrinsic gain over 30, an intrinsic cut-off frequency fT up to 42 GHz and a maximum oscillation frequency fMAX up to 50 GHz, exceeding the reported values for MoS2 transistors to date (fT~0.9 GHz, fMAX~1 GHz). Our results show that logic inverters or radio frequency amplifiers can be formed by integrating multiple MoS2 transistors on quartz or flexible substrates with voltage gain in the gigahertz regime. This study demonstrates the potential of two-dimensional layered semiconductors for high-speed flexible electronics.

  2. Few-layer molybdenum disulfide transistors and circuits for high-speed flexible electronics

    Science.gov (United States)

    Cheng, Rui; Jiang, Shan; Chen, Yu; Liu, Yuan; Weiss, Nathan; Cheng, Hung-Chieh; Wu, Hao; Huang, Yu; Duan, Xiangfeng

    2014-01-01

    Two-dimensional layered materials, such as molybdenum disulfide, are emerging as an exciting material system for future electronics due to their unique electronic properties and atomically thin geometry. Here we report a systematic investigation of MoS2 transistors with optimized contact and device geometry, to achieve self-aligned devices with performance including an intrinsic gain over 30, an intrinsic cut-off frequency fT up to 42 GHz and a maximum oscillation frequency fMAX up to 50 GHz, exceeding the reported values for MoS2 transistors to date (fT ~ 0.9 GHz, fMAX ~ 1 GHz). Our results show that logic inverters or radio frequency amplifiers can be formed by integrating multiple MoS2 transistors on quartz or flexible substrates with voltage gain in the gigahertz regime. This study demonstrates the potential of two-dimensional layered semiconductors for high-speed flexible electronics. PMID:25295573

  3. Production of highly charged ion beams from ECR ion sources

    International Nuclear Information System (INIS)

    Xie, Z.Q.

    1997-09-01

    Electron Cyclotron Resonance (ECR) ion source development has progressed with multiple-frequency plasma heating, higher mirror magnetic fields and better technique to provide extra cold electrons. Such techniques greatly enhance the production of highly charged ions from ECR ion sources. So far at cw mode operation, up to 300 eμA of O 7+ and 1.15 emA of O 6+ , more than 100 eμA of intermediate heavy ions for charge states up to Ar 13+ , Ca 13+ , Fe 13+ , Co 14+ and Kr 18+ , and tens of eμA of heavy ions with charge states to Kr 26+ , Xe 28+ , Au 35+ , Bi 34+ and U 34+ have been produced from ECR ion sources. At an intensity of at least 1 eμA, the maximum charge state available for the heavy ions are Xe 36+ , Au 46+ , Bi 47+ and U 48+ . An order of magnitude enhancement for fully stripped argon ions (I ≥ 60 enA) also has been achieved. This article will review the ECR ion source progress and discuss key requirement for ECR ion sources to produce the highly charged ion beams

  4. HIGH-CURRENT ERL-BASED ELECTRON COOLING FOR RHIC

    International Nuclear Information System (INIS)

    BEN-ZVI, I.

    2005-01-01

    The design of an electron cooler must take into account both electron beam dynamics issues as well as the electron cooling physics. Research towards high-energy electron cooling of RHIC is in its 3rd year at Brookhaven National Laboratory. The luminosity upgrade of RHIC calls for electron cooling of various stored ion beams, such as 100 GeV/A gold ions at collision energies. The necessary electron energy of 54 MeV is clearly out of reach for DC accelerator system of any kind. The high energy also necessitates a bunched beam, with a high electron bunch charge, low emittance and small energy spread. The Collider-Accelerator Department adopted the Energy Recovery Linac (ERL) for generating the high-current, high-energy and high-quality electron beam. The RHIC electron cooler ERL will use four Superconducting RF (SRF) 5-cell cavities, designed to operate at ampere-class average currents with high bunch charges. The electron source will be a superconducting, 705.75 MHz laser-photocathode RF gun, followed up by a superconducting Energy Recovery Linac (ERL). An R and D ERL is under construction to demonstrate the ERL at the unprecedented average current of 0.5 amperes. Beam dynamics performance and luminosity enhancement are described for the case of magnetized and non-magnetized electron cooling of RHIC

  5. Fast electron beam charge injection and switching in dielectrics

    Energy Technology Data Exchange (ETDEWEB)

    Fitting, Hans-Joachim; Schreiber, Erik [Institute of Physics, University of Rostock, Universitaetsplatz 3, 18051 Rostock (Germany); Touzin, Matthieu [Laboratoire de Structure et Proprietes de l' Etat Solide, UMR CNRS 8008, Universite de Lille 1, 59655 Villeneuve d' Ascq (France)

    2011-04-15

    Basic investigations of secondary electrons (SE) relaxation and attenuation are made by means of Monte Carlo simulations using ballistic electron scattering and interactions with optical and acoustic phonons as well as impact ionization of valence band electrons. Then the electron beam induced selfconsistent charge transport and secondary electron emission in insulators are described by means of an electron-hole flight-drift model (FDM). Ballistic secondary electrons and holes, their attenuation and drift, as well as their recombination, trapping, and field- and temperature-dependent Poole-Frenkel detrapping are included. Whereas the initial switching-on of the secondary electron emission proceeds over milli-seconds due to long-lasting selfconsistent charging, the switching-off process occurs much faster, even over femto-seconds. Thus a rapid electron beam switching becomes possible with formation of ultra-short electron beam pulses offering an application in stroboscopic electron microscopy and spectroscopy. (copyright 2011 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

  6. Competition between deformability and charge transport in semiconducting polymers for flexible and stretchable electronics

    International Nuclear Information System (INIS)

    Printz, Adam D.; Lipomi, Darren J.

    2016-01-01

    The primary goal of the field concerned with organic semiconductors is to produce devices with performance approaching that of silicon electronics, but with the deformability—flexibility and stretchability—of conventional plastics. However, an inherent competition between deformability and charge transport has long been observed in these materials, and achieving the extreme (or even moderate) deformability implied by the word “plastic” concurrently with high charge transport may be elusive. This competition arises because the properties needed for high carrier mobilities—e.g., rigid chains in π-conjugated polymers and high degrees of crystallinity in the solid state—are antithetical to deformability. On the device scale, this competition can lead to low-performance yet mechanically robust devices, or high-performance devices that fail catastrophically (e.g., cracking, cohesive failure, and delamination) under strain. There are, however, some observations that contradict the notion of the mutual exclusivity of electronic and mechanical performances. These observations suggest that this problem may not be a fundamental trade-off, but rather an inconvenience that may be negotiated by a logical selection of materials and processing conditions. For example, the selection of the poly(3-alkylthiophene) with a critical side-chain length—poly(3-heptylthiophene) (n = 7)—marries the high deformability of poly(3-octylthiophene) (n = 8) with the high electronic performance (as manifested in photovoltaic efficiency) of poly(3-hexylthiophene) (n = 6). This review explores the relationship between deformability and charge transport in organic semiconductors. The principal conclusions are that reducing the competition between these two parameters is in fact possible, with two demonstrated routes being: (1) incorporation of softer, insulating material into a stiffer, semiconducting material and (2) increasing disorder in a highly ordered film, but not

  7. Competition between deformability and charge transport in semiconducting polymers for flexible and stretchable electronics

    Energy Technology Data Exchange (ETDEWEB)

    Printz, Adam D.; Lipomi, Darren J., E-mail: dlipomi@ucsd.edu [Department of NanoEngineering, University of California, San Diego, 9500 Gilman Drive, Mail Code 0448, La Jolla, California 92093-0448 (United States)

    2016-06-15

    The primary goal of the field concerned with organic semiconductors is to produce devices with performance approaching that of silicon electronics, but with the deformability—flexibility and stretchability—of conventional plastics. However, an inherent competition between deformability and charge transport has long been observed in these materials, and achieving the extreme (or even moderate) deformability implied by the word “plastic” concurrently with high charge transport may be elusive. This competition arises because the properties needed for high carrier mobilities—e.g., rigid chains in π-conjugated polymers and high degrees of crystallinity in the solid state—are antithetical to deformability. On the device scale, this competition can lead to low-performance yet mechanically robust devices, or high-performance devices that fail catastrophically (e.g., cracking, cohesive failure, and delamination) under strain. There are, however, some observations that contradict the notion of the mutual exclusivity of electronic and mechanical performances. These observations suggest that this problem may not be a fundamental trade-off, but rather an inconvenience that may be negotiated by a logical selection of materials and processing conditions. For example, the selection of the poly(3-alkylthiophene) with a critical side-chain length—poly(3-heptylthiophene) (n = 7)—marries the high deformability of poly(3-octylthiophene) (n = 8) with the high electronic performance (as manifested in photovoltaic efficiency) of poly(3-hexylthiophene) (n = 6). This review explores the relationship between deformability and charge transport in organic semiconductors. The principal conclusions are that reducing the competition between these two parameters is in fact possible, with two demonstrated routes being: (1) incorporation of softer, insulating material into a stiffer, semiconducting material and (2) increasing disorder in a highly ordered film, but not

  8. Comparison of the target-thickness dependence of the convoy electron yield and the Rydberg electron yield measured in coincidence with exit charge states in fast ion-solid collisions

    International Nuclear Information System (INIS)

    Gaither, C.C. III; Breinig, M.; Freyou, J.; Underwood, T.A.

    1988-01-01

    We have simultaneously measured the yield of convoy electrons and the yield of electrons in high Rydberg states of the projectile (n /approx gt/ 70), produced by 2MeV/u C projectiles passing through C foils, whose thicknesses range from 4--10 ug/cm 2 , for incident charge states q/sub i/ = 4--6 and exit charge states q/sub e/ = 4--6. We have found that these yields exhibit similar trends as a function of foil thickness, but that, nevertheless, the ratio of the number of convoy electrons detected in coincidence with ions of exit charge state q/sub e/ to the number of electrons detected in high Rydberg states of ions with the same exit charge state is a function of foil thickness. This may be due to a broadening of the convoy electron energy spectrum with increasing foil thickness. 6 refs., 3 figs

  9. Maximum entropy theory of recoil charge distributions in electron-capture collisions

    International Nuclear Information System (INIS)

    Aberg, T.; Blomberg, A.; Tulkki, J.; Goscinski, O.

    1984-01-01

    A generalized Fermi-Dirac distribution is derived and applied to charge-state distributions in single collisions between multiply charged ions and rare-gas atoms. It relates multiple electron loss in single-electron capture to multiple ionization in multiphoton absorption and discloses inner-shell vacancy formation in double- and triple-electron capture

  10. Compact femtosecond electron diffractometer with 100 keV electron bunches approaching the single-electron pulse duration limit

    International Nuclear Information System (INIS)

    Waldecker, Lutz; Bertoni, Roman; Ernstorfer, Ralph

    2015-01-01

    We present the design and implementation of a highly compact femtosecond electron diffractometer working at electron energies up to 100 keV. We use a multi-body particle tracing code to simulate electron bunch propagation through the setup and to calculate pulse durations at the sample position. Our simulations show that electron bunches containing few thousands of electrons per bunch are only weakly broadened by space-charge effects and their pulse duration is thus close to the one of a single-electron wavepacket. With our compact setup, we can create electron bunches containing up to 5000 electrons with a pulse duration below 100 fs on the sample. We use the diffractometer to track the energy transfer from photoexcited electrons to the lattice in a thin film of titanium. This process takes place on the timescale of few-hundred femtoseconds and a fully equilibrated state is reached within 1 ps

  11. X-ray spectroscopy of highly-charged ions in a storage ring. Invited lecture

    International Nuclear Information System (INIS)

    Beyer, H.F.

    1994-11-01

    The purpose of the present lectures is to carry through the methods and procedures necessary for a meaningful spectroscopy of the heaviest few-electron ions in relation to present theories. Results achieved so far in accelerator-based X-ray experiments are highlighted with emphasis on recent developments on heavy-ion storage rings. Starting with a brief account of the basics of one-electron ions, the motivation for doing X-ray spectroscopy of the simplest atomic systems with a high nuclear charge is given. In section 2 X-ray instrumentation and techniques are discussed including the precautions necessary when dealing with fast-beam sources. Peculiarities of heavy-ion storage rings are investigated in section 3 with regard to their use for spectroscopy. In section 4 are discussed results obtained so far on the measurement of the Lamb shift in very heavy ions. Section 5 gives some perspectives for the near future. (orig.)

  12. Ion accumulation and space charge neutralization in intensive electron beams for ion sources and electron cooling

    International Nuclear Information System (INIS)

    Shirkov, G.D.

    1996-01-01

    The Electron Beam Ion Sources (EBIS), Electron Beam Ion Traps (EBIT) and electron beams for electron cooling application have the beam parameters in the same ranges of magnitudes. EBIS and EBIT produce and accumulate ions in the beam due to electron impact ionization. The cooling electron beam accumulates positive ions from the residual gas in the accelerator chamber during the cooling cycle. The space charge neutralization of cooling beam is also used to reduce the electron energy spread and enhance the cooling ability. The advanced results of experimental investigations and theoretical models of the EBIS electron beams are applied to analyze the problem of beam neutralization in the electron cooling techniques. The report presents the analysis of the most important processes connected with ion production, accumulation and losses in the intensive electron beams of ion sources and electron cooling systems for proton and ion colliders. The inelastic and elastic collision processes of charged particles in the electron beams are considered. The inelastic processes such as ionization, charge exchange and recombination change the charge states of ions and neutral atoms in the beam. The elastic Coulomb collisions change the energy of particles and cause the energy redistribution among components in the electron-ion beams. The characteristic times and specific features of ionization, beam neutralization, ion heating and loss in the ion sources and electron cooling beams are determined. The dependence of negative potential in the beam cross section on neutralization factor is studied. 17 refs., 5 figs., 1 tab

  13. High-resolution X-ray spectra from low-temperature, highly charged ions

    International Nuclear Information System (INIS)

    Beiersdorfer, P.

    1996-09-01

    The electron beam ion traps (EBIT) at Livermore were designed for studying the x-ray emission of highly charged ions produced and excited by a monoenergetic electron beam. The precision with which the x-ray emission can be analyzed has recently been increased markedly when it became possible to decouple the temperature of the ions from the energy of the electron beam by several orders of magnitude. By adjusting the trap parameters, ion temperatures as low as 15.8±4.4 eV for Ti 20+ and 59.4±9.9 eV for Cs 45+ were achieved. These temperatures were more than two orders of magnitude lower than the energy of the multi-keV electron beam used for the production and excitation of the ions. A discussion of the techniques used to produce and study low-temperature highly charged ions is presented in this progress report. The low ion temperatures enabled measurements heretofore impossible. As an example, a direct observation of the natural line width of fast electric dipole allowed x-ray transitions is described. From the observed natural line width and b making use of the time-energy relations of the uncertainty principle we were able to determine a radiative transition rate of 1.65 fs for the 2p-3d resonance transition in neonlike Cs 45+ . A brief discussion of other high-precision measurements enabled by our new technique is also given

  14. Charge transport in highly efficient iridium cored electrophosphorescent dendrimers

    Science.gov (United States)

    Markham, Jonathan P. J.; Samuel, Ifor D. W.; Lo, Shih-Chun; Burn, Paul L.; Weiter, Martin; Bässler, Heinz

    2004-01-01

    Electrophosphorescent dendrimers are promising materials for highly efficient light-emitting diodes. They consist of a phosphorescent core onto which dendritic groups are attached. Here, we present an investigation into the optical and electronic properties of highly efficient phosphorescent dendrimers. The effect of dendrimer structure on charge transport and optical properties is studied using temperature-dependent charge-generation-layer time-of-flight measurements and current voltage (I-V) analysis. A model is used to explain trends seen in the I-V characteristics. We demonstrate that fine tuning the mobility by chemical structure is possible in these dendrimers and show that this can lead to highly efficient bilayer dendrimer light-emitting diodes with neat emissive layers. Power efficiencies of 20 lm/W were measured for devices containing a second-generation (G2) Ir(ppy)3 dendrimer with a 1,3,5-tris(2-N-phenylbenzimidazolyl)benzene electron transport layer.

  15. Charging of Dust Grains in a Nuclear-Induced Plasma at High Pressures

    International Nuclear Information System (INIS)

    Pal’, A. F.; Starostin, A. N.; Filippov, A. V.

    2001-01-01

    The process of dust-grain charging in plasmas produced by radioactive decay products or spontaneous fission fragments in air and xenon at high pressures is studied numerically in the hydrodynamic approximation. It is shown that, at sufficiently high rates of gas ionization, the dust grains in air are charged by electrons rather than ions, so that the grain charge in air is comparable to that in electropositive gases. The results of numerical calculations based on a complete model agree well with the experimental data. The time evolution of the grain charge is investigated, and the characteristic time scales on which the grains acquire an electric charge are established. The validity of approximate theories of dust-grain charging in electropositive and electronegative gases at high pressures is examined

  16. Effective tuning of electron charge and spin distribution in a dot-ring nanostructure at the ZnO interface

    Science.gov (United States)

    Chakraborty, Tapash; Manaselyan, Aram; Barseghyan, Manuk

    2018-05-01

    Electronic states and the Aharonov-Bohm effect in ZnO quantum dot-ring nanostructures containing few interacting electrons reveal several unique features. We have shown here that in contrast to the dot-rings made of conventional semiconductors, such as InAs or GaAs, the dot-rings in ZnO heterojunctions demonstrate several unique characteristics due to the unusual properties of quantum dots and rings in ZnO. In particular the energy spectra of the ZnO dot-ring and the Aharnov-Bohm oscillations are strongly dependant on the electron number in the dot or in the ring. Therefore even small changes of the confinement potential, sizes of the dot-ring or the magnetic field can drastically change the energy spectra and the behavior of Aharonov-Bohm oscillations in the system. Due to this interesting phenomena it is possible to effectively control with high accuracy the electron charge and spin distribution inside the dot-ring structure. This controlling can be achieved either by changing the magnetic field or the confinement potentials.

  17. Facile synthesis of 3D few-layered MoS2 coated TiO2 nanosheet core-shell nanostructures for stable and high-performance lithium-ion batteries

    Science.gov (United States)

    Chen, Biao; Zhao, Naiqin; Guo, Lichao; He, Fang; Shi, Chunsheng; He, Chunnian; Li, Jiajun; Liu, Enzuo

    2015-07-01

    Uniform transition metal sulfide deposition on a smooth TiO2 surface to form a coating structure is a well-known challenge, caused mainly due to their poor affinities. Herein, we report a facile strategy for fabricating mesoporous 3D few-layered (glucose as a binder. The core-shell structure has been systematically examined and corroborated by transmission electron microscopy, scanning transmission electron microscopy, and X-ray photoelectron spectroscopy analyses. It is found that the resultant 3D FL-MoS2@TiO2 as a lithium-ion battery anode delivers an outstanding high-rate capability with an excellent cycling performance, relating to the unique structure of 3D FL-MoS2@TiO2. The 3D uniform coverage of few-layered (glucose as a binder. The core-shell structure has been systematically examined and corroborated by transmission electron microscopy, scanning transmission electron microscopy, and X-ray photoelectron spectroscopy analyses. It is found that the resultant 3D FL-MoS2@TiO2 as a lithium-ion battery anode delivers an outstanding high-rate capability with an excellent cycling performance, relating to the unique structure of 3D FL-MoS2@TiO2. The 3D uniform coverage of few-layered (<4 layers) MoS2 onto the TiO2 can remarkably enhance the structure stability and effectively shortens the transfer paths of both lithium ions and electrons, while the strong synergistic effect between MoS2 and TiO2 can significantly facilitate the transport of ions and electrons across the interfaces, especially in the high-rate charge-discharge process. Moreover, the facile fabrication strategy can be easily extended to design other oxide/carbon-sulfide/oxide core-shell materials for extensive applications. Electronic supplementary information (ESI) available: Supplementary SEM, TEM, XPS and EIS analyses. See DOI: 10.1039/c5nr03334a

  18. Electronically shielded solid state charged particle detector

    International Nuclear Information System (INIS)

    Balmer, D.K.; Haverty, T.W.; Nordin, C.W.; Tyree, W.H.

    1996-01-01

    An electronically shielded solid state charged particle detector system having enhanced radio frequency interference immunity includes a detector housing with a detector entrance opening for receiving the charged particles. A charged particle detector having an active surface is disposed within the housing. The active surface faces toward the detector entrance opening for providing electrical signals representative of the received charged particles when the received charged particles are applied to the active surface. A conductive layer is disposed upon the active surface. In a preferred embodiment, a nonconductive layer is disposed between the conductive layer and the active surface. The conductive layer is electrically coupled to the detector housing to provide a substantially continuous conductive electrical shield surrounding the active surface. The inner surface of the detector housing is supplemented with a radio frequency absorbing material such as ferrite. 1 fig

  19. Charge dynamics in aluminum oxide thin film studied by ultrafast scanning electron microscopy.

    Science.gov (United States)

    Zani, Maurizio; Sala, Vittorio; Irde, Gabriele; Pietralunga, Silvia Maria; Manzoni, Cristian; Cerullo, Giulio; Lanzani, Guglielmo; Tagliaferri, Alberto

    2018-04-01

    The excitation dynamics of defects in insulators plays a central role in a variety of fields from Electronics and Photonics to Quantum computing. We report here a time-resolved measurement of electron dynamics in 100 nm film of aluminum oxide on silicon by Ultrafast Scanning Electron Microscopy (USEM). In our pump-probe setup, an UV femtosecond laser excitation pulse and a delayed picosecond electron probe pulse are spatially overlapped on the sample, triggering Secondary Electrons (SE) emission to the detector. The zero of the pump-probe delay and the time resolution were determined by measuring the dynamics of laser-induced SE contrast on silicon. We observed fast dynamics with components ranging from tens of picoseconds to few nanoseconds, that fits within the timescales typical of the UV color center evolution. The surface sensitivity of SE detection gives to the USEM the potential of applying pump-probe investigations to charge dynamics at surfaces and interfaces of current nano-devices. The present work demonstrates this approach on large gap insulator surfaces. Copyright © 2018 Elsevier B.V. All rights reserved.

  20. Atomic physics and synchrotron radiation: The production and accumulation of highly charged ions

    International Nuclear Information System (INIS)

    Johnson, B.M.; Meron, M.; Agagu, A.; Jones, K.W.

    1986-01-01

    Synchrotron radiation can be used to produce highly-charged ions, and to study photoexcitation and photoionization for ions of virtually any element in the periodic table. To date, with few exceptions, atomic physics studies have been limited to rare gases and a few metal vapors, and to photoexcitation energies in the VUV region of the electromagnetic spectrum. These limitations can now be overcome using photons produced by high-brightness synchrotron storage rings, such as the x-ray ring at the National Synchrotron Light Source (NSLS) at Brookhaven. Furthermore, calculations indicate that irradiation of an ion trap with an intense energetic photon beam will result in a viable source of highly-charged ions that can be given the name PHOBIS: the PHOton Beam Ion Source. Promising results, which encourage the wider systematic use of synchrotron radiation in atomic physics research, have been obtained in recent experiments on VUV photoemission and the production and storage of multiply-charged ions. 26 refs., 4 figs., 1 tab

  1. High-k shallow traps observed by charge pumping with varying discharging times

    International Nuclear Information System (INIS)

    Ho, Szu-Han; Chen, Ching-En; Tseng, Tseung-Yuen; Chang, Ting-Chang; Lu, Ying-Hsin; Lo, Wen-Hung; Tsai, Jyun-Yu; Liu, Kuan-Ju; Wang, Bin-Wei; Cao, Xi-Xin; Chen, Hua-Mao; Cheng, Osbert; Huang, Cheng-Tung; Chen, Tsai-Fu

    2013-01-01

    In this paper, we investigate the influence of falling time and base level time on high-k bulk shallow traps measured by charge pumping technique in n-channel metal-oxide-semiconductor field-effect transistors with HfO 2 /metal gate stacks. N T -V high level characteristic curves with different duty ratios indicate that the electron detrapping time dominates the value of N T for extra contribution of I cp traps. N T is the number of traps, and I cp is charge pumping current. By fitting discharge formula at different temperatures, the results show that extra contribution of I cp traps at high voltage are in fact high-k bulk shallow traps. This is also verified through a comparison of different interlayer thicknesses and different Ti x N 1−x metal gate concentrations. Next, N T -V high level characteristic curves with different falling times (t falling time ) and base level times (t base level ) show that extra contribution of I cp traps decrease with an increase in t falling time . By fitting discharge formula for different t falling time , the results show that electrons trapped in high-k bulk shallow traps first discharge to the channel and then to source and drain during t falling time . This current cannot be measured by the charge pumping technique. Subsequent measurements of N T by charge pumping technique at t base level reveal a remainder of electrons trapped in high-k bulk shallow traps

  2. Physics of high intensity nanosecond electron source

    International Nuclear Information System (INIS)

    Herrera-Gomez, A.; Spicer, W.E.

    1993-08-01

    A new high-intensity, short-time electron source is now being used at the Stanford Linear Accelerator Center (SLAC). Using a GaAs negative affinity semiconductor in the construction of the cathode, it is possible to fulfill operation requirements such as peak currents of tens of amperes, peak widths of the order of nanoseconds, hundreds of hours of operation stability, and electron spin polarization. The cathode is illuminated with high intensity laser pulses, and photoemitted electrons constitute the yield. Because of the high currents, some nonlinear effects are present. Very noticeable is the so-called Charge Limit (CL) effect, which consists of a limit on the total charge in each pulse-that is, the total bunch charge stops increasing as the light pulse total energy increases. In this paper, we explain the mechanism of the CL and how it is caused by the photovoltaic effect. Our treatment is based on the Three-Step model of photoemission. We relate the CL to the characteristics of the surface and bulk of the semiconductor, such as doping, band bending, surface vacuum level, and density of surface states. We also discuss possible ways to prevent the Char's Level effect

  3. Characterization of Charge-Carrier Transport in Semicrystalline Polymers: Electronic Couplings, Site Energies, and Charge-Carrier Dynamics in Poly(bithiophene- alt -thienothiophene) [PBTTT

    KAUST Repository

    Poelking, Carl; Cho, Eunkyung; Malafeev, Alexander; Ivanov, Viktor; Kremer, Kurt; Risko, Chad; Bré das, Jean-Luc; Andrienko, Denis

    2013-01-01

    We establish a link between the microscopic ordering and the charge-transport parameters for a highly crystalline polymeric organic semiconductor, poly(2,5-bis(3-tetradecylthiophen-2-yl)thieno[3,2-b]thiophene) (PBTTT). We find that the nematic and dynamic order parameters of the conjugated backbones, as well as their separation, evolve linearly with temperature, while the side-chain dynamic order parameter and backbone paracrystallinity change abruptly upon the (also experimentally observed) melting of the side chains around 400 K. The distribution of site energies follows the behavior of the backbone paracrystallinity and can be treated as static on the time scale of a single-charge transfer reaction. On the contrary, the electronic couplings between adjacent backbones are insensitive to side-chain melting and vary on a much faster time scale. The hole mobility, calculated after time-averaging of the electronic couplings, reproduces well the value measured in a short-channel thin-film transistor. The results underline that to secure efficient charge transport in lamellar arrangements of conjugated polymers: (i) the electronic couplings should present high average values and fast dynamics, and (ii) the energetic disorder (paracrystallinity) should be small. © 2013 American Chemical Society.

  4. Characterization of Charge-Carrier Transport in Semicrystalline Polymers: Electronic Couplings, Site Energies, and Charge-Carrier Dynamics in Poly(bithiophene- alt -thienothiophene) [PBTTT

    KAUST Repository

    Poelking, Carl

    2013-01-31

    We establish a link between the microscopic ordering and the charge-transport parameters for a highly crystalline polymeric organic semiconductor, poly(2,5-bis(3-tetradecylthiophen-2-yl)thieno[3,2-b]thiophene) (PBTTT). We find that the nematic and dynamic order parameters of the conjugated backbones, as well as their separation, evolve linearly with temperature, while the side-chain dynamic order parameter and backbone paracrystallinity change abruptly upon the (also experimentally observed) melting of the side chains around 400 K. The distribution of site energies follows the behavior of the backbone paracrystallinity and can be treated as static on the time scale of a single-charge transfer reaction. On the contrary, the electronic couplings between adjacent backbones are insensitive to side-chain melting and vary on a much faster time scale. The hole mobility, calculated after time-averaging of the electronic couplings, reproduces well the value measured in a short-channel thin-film transistor. The results underline that to secure efficient charge transport in lamellar arrangements of conjugated polymers: (i) the electronic couplings should present high average values and fast dynamics, and (ii) the energetic disorder (paracrystallinity) should be small. © 2013 American Chemical Society.

  5. Experimental design of high energy electron gun by means of scaling rules

    International Nuclear Information System (INIS)

    Wojcicki, S.

    1996-01-01

    The possibility of the design of a new family of electron guns by means of scaling theory of electron-optical devices (EOD) is presented. According to the theory, EOD with a relatively big space charge, as in high energy Pierce type electron guns used in technological equipment, generally cannot be scaled, because of their nonlinear space charge nature. Therefore, the scaling rules are applied here only to the anode zone of the gun, where the electron beam perveance is small, and the cathode lens of gun with considerable space charge remains unchanged. The procedure for scaling a 25 kV and 150 mA gun with cylindrical electron beam into a high voltage 75 kV and 150 mA electron system is given. An experimental investigation proved the high technological quality of a high voltage gun constructed according to the above conception. (author)

  6. Doping Phosphorene with Holes and Electrons through Molecular Charge Transfer.

    Science.gov (United States)

    Vishnoi, Pratap; Rajesh, S; Manjunatha, S; Bandyopadhyay, Arkamita; Barua, Manaswee; Pati, Swapan K; Rao, C N R

    2017-11-03

    An important aspect of phosphorene, the novel two-dimensional semiconductor, is whether holes and electrons can both be doped in this material. Some reports found that only electrons can be preferentially doped into phosphorene. There are some theoretical calculations showing charge-transfer interaction with both tetrathiafulvalene (TTF) and tetracyanoethylene (TCNE). We have carried out an investigation of chemical doping of phosphorene by a variety of electron donor and acceptor molecules, employing both experiment and theory, Raman scattering being a crucial aspect of the study. We find that both electron acceptors and donors interact with phosphorene by charge-transfer, with the acceptors having more marked effects. All the three Raman bands of phosphorene soften and exhibit band broadening on interaction with both donor and acceptor molecules. First-principles calculations establish the occurrence of charge-transfer between phosphorene with donors as well as acceptors. The absence of electron-hole asymmetry is noteworthy. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

  7. Production of highly charged ion beams Kr32+, Xe44+, Au54+ with Electron String Ion Source (ESIS) Krion-2 and corresponding basic and applied studies

    Science.gov (United States)

    Donets, D. E.; Donets, E. D.; Donets, E. E.; Salnikov, V. V.; Shutov, V. B.

    2010-09-01

    Electron String Ion Source (ESIS) Krion-2 (JINR, Dubna) was used for basic and applied research in various aspects of multiply charged heavy ions production. Energy recuperation mode in ESIS has been proofed first and used for production of highly charged ions 84Kr28+÷84Kr32+, 124Xe40÷124Xe44 and Au51+÷ Au54+. Krion-2 ESIS was mounted on high voltage (HV) platform of LU-20 Linac and used as an injector of highly charged ions during Nuclotron run N° 41. Krion-2 ESIS has produced 3.0.107 124Xe42+ ions per pulse of 7 μs duration. This ion beam was injected into LU-20 and Nuclotron, accelerated up to energy of 186 GeV and the extracted Xe beam was used for physics experiments. Electron String Ion Source Krion-2 demonstrated the high reliability and stability running during 30 days on HV platform. We believe that it is due to an extremely low electron beam power, provided by using the electron string mode of operation: 50 W pulse power and about 10 W average power. Other possible application of ESIS could be its use in injection complexes of synchrotrons and cyclotrons for cancer therapy. Slow and fast extraction of C4+ and C6+ beams from Krion-2 ESIS were preliminary studied towards ESIS optimization for medical accelerators requirements.

  8. Few-layer SnSe{sub 2} transistors with high on/off ratios

    Energy Technology Data Exchange (ETDEWEB)

    Pei, Tengfei; Bao, Lihong, E-mail: lhbao@iphy.ac.cn; Wang, Guocai; Ma, Ruisong; Yang, Haifang; Li, Junjie; Gu, Changzhi; Du, Shixuan; Gao, Hong-jun [Institute of Physics, Chinese Academy of Sciences, P. O. Box 603, Beijing 100190 (China); Pantelides, Sokrates [Department of Physics and Astronomy, Vanderbilt University, Nashville, Tennessee 37235 (United States); Material Science and Technology Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37381 (United States)

    2016-02-01

    We report few-layer SnSe{sub 2} field effect transistors (FETs) with high current on/off ratios. By trying different gate configurations, 300 nm SiO{sub 2} and 70 nm HfO{sub 2} as back gate only and 70 nm HfO{sub 2} as back gate combined with a top capping layer of polymer electrolyte, few-layer SnSe{sub 2} FET with a current on/off ratio of 10{sup 4} can be obtained. This provides a reliable solution for electrically modulating quasi-two-dimensional materials with high electron density (over 10{sup 13} cm{sup −2}) for field-effect transistor applications.

  9. Physical mechanisms leading to high currents of highly charged ions in laser-driven ion sources

    International Nuclear Information System (INIS)

    Haseroth, Helmut; Hora, Heinrich; Regensburg Inst. of Tech.

    1996-01-01

    Heavy ion sources for the big accelerators, for example, the LHC, require considerably more ions per pulse during a short time than the best developed classical ion source, the electron cyclotron resonance (ECR) provides; thus an alternative ion source is needed. This can be expected from laser-produced plasmas, where dramatically new types of ion generation have been observed. Experiments with rather modest lasers have confirmed operation with one million pulses of 1 Hz, and 10 11 C 4+ ions per pulse reached 2 GeV/u in the Dubna synchrotron. We review here the complexities of laser-plasma interactions to underline the unique and extraordinary possibilities that the laser ion source offers. The complexities are elaborated with respect to keV and MeV ion generation, nonlinear (ponderomotive) forces, self-focusing, resonances and ''hot'' electrons, parametric instabilities, double-layer effects, and the few ps stochastic pulsation (stuttering). Recent experiments with the laser ion source have been analyzed to distinguish between the ps and ns interaction, and it was discovered that one mechanism of highly charged ion generation is the electron impact ionization (EII) mechanism, similar to the ECR, but with so much higher plasma densities that the required very large number of ions per pulse are produced. (author)

  10. Physical mechanisms leading to high currents of highly charged ions in laser-driven ion sources

    Energy Technology Data Exchange (ETDEWEB)

    Haseroth, Helmut [European Organization for Nuclear Research, Geneva (Switzerland); Hora, Heinrich [New South Wales Univ., Kensington, NSW (Australia)]|[Regensburg Inst. of Tech. (Germany). Anwenderzentrum

    1996-12-31

    Heavy ion sources for the big accelerators, for example, the LHC, require considerably more ions per pulse during a short time than the best developed classical ion source, the electron cyclotron resonance (ECR) provides; thus an alternative ion source is needed. This can be expected from laser-produced plasmas, where dramatically new types of ion generation have been observed. Experiments with rather modest lasers have confirmed operation with one million pulses of 1 Hz, and 10{sup 11} C{sup 4+} ions per pulse reached 2 GeV/u in the Dubna synchrotron. We review here the complexities of laser-plasma interactions to underline the unique and extraordinary possibilities that the laser ion source offers. The complexities are elaborated with respect to keV and MeV ion generation, nonlinear (ponderomotive) forces, self-focusing, resonances and ``hot`` electrons, parametric instabilities, double-layer effects, and the few ps stochastic pulsation (stuttering). Recent experiments with the laser ion source have been analyzed to distinguish between the ps and ns interaction, and it was discovered that one mechanism of highly charged ion generation is the electron impact ionization (EII) mechanism, similar to the ECR, but with so much higher plasma densities that the required very large number of ions per pulse are produced. (author).

  11. Possibility of resonant capture of antiprotons by highly charged hydrogenlike ions

    International Nuclear Information System (INIS)

    Genkin, M.; Lindroth, E.

    2009-01-01

    Recently, an experimental setup was proposed by Lapierre et al. which would allow antiprotons and highly charged ions to collide repeatedly in an electron beam ion trap (EBIT) due to a nested trap configuration. As mentioned by the authors, such a setup may open the possibility to study antiproton capture into well-defined states through a resonant process which involves simultaneous electron excitation. In the present work, we give some theoretical estimations of the feasibility of that process. It appears that the exotic dielectronic-like process of resonant anti-proton capture in highly charged ions does not seem to be completely out of reach

  12. Application of CTOF method to detect secondly charged particle from 2 GeV electron

    International Nuclear Information System (INIS)

    Takahashi, Kazutoshi; Sanami, Toshiya; Ban, Syuichi; Lee, Hee-Seok; Sato, Tatsuhiko

    2002-01-01

    To design a shield and evaluate leakage radiation at high energy electron accelerators, the energy and angular data of secondary particle from the reaction of electrons with structural materials are required. Secondly neutron spectrum from structural materials has been measured by using electron accelerator in PAL (Pohang Accelerator Laboratory). In the neutron measurement, the electronics with Multi-hit TDC (MHTDC) was adopted to measure Time of Flight of every particles (TOFs) emitted from the reactions by each single electron bunch. The measurements are extended to secondly charged particles. For the charged particles measurement, the pulse height data for every particles are indispensable to distinguish charged particles by Δ E-E method. A new system which can measure pulse height for every particle is required instead of the MHTDC system. For this requirement, the method which can take output current from detectors was developed by using digital storage oscilloscope system is named ''Current Time of Flight method'' (CTOF). The CTOF method is able to measure pulse height and TOF for every particles produced by single electron bunch. Electrons are accelerated to 2.04 GeV and the repetition rate is 10 Hz. These electrons bombard thin disk samples of Cu 1mm, Al 4 mm and W 0.5 mm. Secondly charged particles, proton and deuteron, are produced in the samples by photonuclear reaction. Two dimensional of Δ E-E spectrum for each the samples measured by CTOF shows separation between proton and deuteron perfectly. Thus, proton and deuteron spectrum are obtained from this data. (M. Suetake)

  13. Charged dust in planetary magnetospheres: Hamiltonian dynamics and numerical simulations for highly charged grains

    Science.gov (United States)

    Schaffer, L.; Burns, J. A.

    1994-01-01

    We use a combination of analytical and numerical methods to investigate the dynamics of charged dust grains in planetary magnetospheres. Our emphasis is on obtaining results valid for particles that are not necessarily dominated either by gravitational or electromagnetic forces. A Hamiltonian formulation of the problem yields exact results, for all values of charge-to-mass ratio, when we introduce two constraints: particles remain in the equatorial plane and the magnetic field is taken as axially symmetric. In particular, we obtain locations of equilibrium points, the frequencies of stable periodic orbits, the topology of separatrices in phase space, and the rate of longitudinal drift. These results are significant for specific applications: motion in the nearly aligned dipolar field of Saturn, and the trajectories of arbitrarily charged particles in complex magnetic fields for limited periods of time after ejection from parent bodies. Since the model is restrictive, we also use numerical integrations of the full three-dimensional equations of motion and illustrate under what conditions the constrained problem yields reasonable results. We show that a large fraction of the intermediately charged and highly charged (gyrating) particles will always be lost to a planet's atmosphere within a few hundred hours, for motion through tilted-dipole magnetic fields. We find that grains must have a very high charge-to-mass ratio in order to be mirrored back to the ring plane. Thus, except perhaps at Saturn where the dipole tilt is very small, the likely inhabitants of the dusty ring systems are those particles that are either nearly Keplerian (weakly charged) grains or grains whose charges place them in the lower end of the intermediate charge zone. Fianlly, we demonstrate the effect of plasma drag on the orbits of gyrating particles to be a rapid decrease in gyroradius followed by a slow radial evolution of the guiding center.

  14. Charge transport through DNA based electronic barriers

    Science.gov (United States)

    Patil, Sunil R.; Chawda, Vivek; Qi, Jianqing; Anantram, M. P.; Sinha, Niraj

    2018-05-01

    We report charge transport in electronic 'barriers' constructed by sequence engineering in DNA. Considering the ionization potentials of Thymine-Adenine (AT) and Guanine-Cytosine (GC) base pairs, we treat AT as 'barriers'. The effect of DNA conformation (A and B form) on charge transport is also investigated. Particularly, the effect of width of 'barriers' on hole transport is investigated. Density functional theory (DFT) calculations are performed on energy minimized DNA structures to obtain the electronic Hamiltonian. The quantum transport calculations are performed using the Landauer-Buttiker framework. Our main findings are contrary to previous studies. We find that a longer A-DNA with more AT base pairs can conduct better than shorter A-DNA with a smaller number of AT base pairs. We also find that some sequences of A-DNA can conduct better than a corresponding B-DNA with the same sequence. The counterions mediated charge transport and long range interactions are speculated to be responsible for counter-intuitive length and AT content dependence of conductance of A-DNA.

  15. Large-Area Synthesis of High-Quality Uniform Few-Layer MoTe2.

    Science.gov (United States)

    Zhou, Lin; Xu, Kai; Zubair, Ahmad; Liao, Albert D; Fang, Wenjing; Ouyang, Fangping; Lee, Yi-Hsien; Ueno, Keiji; Saito, Riichiro; Palacios, Tomás; Kong, Jing; Dresselhaus, Mildred S

    2015-09-23

    The controlled synthesis of large-area, atomically thin molybdenum ditelluride (MoTe2) crystals is crucial for its various applications based on the attractive properties of this emerging material. In this work, we developed a chemical vapor deposition synthesis to produce large-area, uniform, and highly crystalline few-layer 2H and 1T' MoTe2 films. It was found that these two different phases of MoTe2 can be grown depending on the choice of Mo precursor. Because of the highly crystalline structure, the as-grown few-layer 2H MoTe2 films display electronic properties that are comparable to those of mechanically exfoliated MoTe2 flakes. Our growth method paves the way for the large-scale application of MoTe2 in high-performance nanoelectronics and optoelectronics.

  16. Near-field enhanced electron acceleration from dielectric nanospheres in intense few-cycle laser fields

    International Nuclear Information System (INIS)

    Zherebtsov, S.; Znakovskaya, I.; Wirth, A.; Herrwerth, O.; Suessmann, F.; Ahmad, I.; Trushin, S.; Fennel, Th.; Plenge, J.; Antonsson, E.

    2010-01-01

    Complete text of publication follows. The interaction of nanostructured materials with few-cycle laser light has attracted significant attention lately. This interest is driven by both the quest for fundamental insight into the real-time dynamics of many-electron systems and a wide range of far-reaching applications, such as, e.g. ultrafast computation and information storage on the nanoscale and the generation of XUV frequency combs. We investigated the above-threshold electron emission from isolated SiO 2 nanoparticles in waveform controlled few-cycle laser fields at intensities close to the tunneling regime. The enhancement of the electron acceleration from the silica nanoparticles was explored as a function of the particle size (ranging from 50 to 147 nm) and the laser peak intensity (1 - 4x10 13 W/cm 2 ). Obtained cut-off values in the kinetic energy spectra are displayed in Fig. 1. The cut-off values show a linear dependence with intensity within the studied intensity range, with the average cut-off energy being 53 U P , indicated by the black line. Quasi-classical simulations of the emission process reveal that electron rescattering in the locally enhanced near-field of the particle is responsible for the large energy gain. The observed near-field enhancement offers promising new routes for pushing the limits of strong-field phenomena relying on electron rescattering, such as, high-harmonic generation and molecular imaging.

  17. Charge amplification and transfer processes in the gas electron multiplier

    International Nuclear Information System (INIS)

    Bachmann, S.; Bressan, A.; Ropelewski, L.; Sauli, F.; Sharma, A.; Moermann, D.

    1999-01-01

    We report the results of systematic investigations on the operating properties of detectors based on the gas electron multiplier (GEM). The dependence of gain and charge collection efficiency on the external fields has been studied in a range of values for the hole diameter and pitch. The collection efficiency of ionization electrons into the multiplier, after an initial increase, reaches a plateau extending to higher values of drift field the larger the GEM voltage and its optical transparency. The effective gain, fraction of electrons collected by an electrode following the multiplier, increases almost linearly with the collection field, until entering a steeper parallel plate multiplication regime. The maximum effective gain attainable increases with the reduction in the hole diameter, stabilizing to a constant value at a diameter approximately corresponding to the foil thickness. Charge transfer properties appear to depend only on ratios of fields outside and within the channels, with no interaction between the external fields. With proper design, GEM detectors can be optimized to satisfy a wide range of experimental requirements: tracking of minimum ionizing particles, good electron collection with small distortions in high magnetic fields, improved multi-track resolution and strong ion feedback suppression in large volume and time-projection chambers

  18. Intense beam production of highly charged heavy ions by the superconducting electron cyclotron resonance ion source SECRAL.

    Science.gov (United States)

    Zhao, H W; Sun, L T; Zhang, X Z; Guo, X H; Cao, Y; Lu, W; Zhang, Z M; Yuan, P; Song, M T; Zhao, H Y; Jin, T; Shang, Y; Zhan, W L; Wei, B W; Xie, D Z

    2008-02-01

    There has been increasing demand to provide higher beam intensity and high enough beam energy for heavy ion accelerator and some other applications, which has driven electron cyclotron resonance (ECR) ion source to produce higher charge state ions with higher beam intensity. One of development trends for highly charged ECR ion source is to build new generation ECR sources by utilization of superconducting magnet technology. SECRAL (superconducting ECR ion source with advanced design in Lanzhou) was successfully built to produce intense beams of highly charged ion for Heavy Ion Research Facility in Lanzhou (HIRFL). The ion source has been optimized to be operated at 28 GHz for its maximum performance. The superconducting magnet confinement configuration of the ion source consists of three axial solenoid coils and six sextupole coils with a cold iron structure as field booster and clamping. An innovative design of SECRAL is that the three axial solenoid coils are located inside of the sextupole bore in order to reduce the interaction forces between the sextupole coils and the solenoid coils. For 28 GHz operation, the magnet assembly can produce peak mirror fields on axis of 3.6 T at injection, 2.2 T at extraction, and a radial sextupole field of 2.0 T at plasma chamber wall. During the commissioning phase at 18 GHz with a stainless steel chamber, tests with various gases and some metals have been conducted with microwave power less than 3.5 kW by two 18 GHz rf generators. It demonstrates the performance is very promising. Some record ion beam intensities have been produced, for instance, 810 e microA of O(7+), 505 e microA of Xe(20+), 306 e microA of Xe(27+), and so on. The effect of the magnetic field configuration on the ion source performance has been studied experimentally. SECRAL has been put into operation to provide highly charged ion beams for HIRFL facility since May 2007.

  19. Electronic structure and correlated wave functions of a few electron quantum dots

    Energy Technology Data Exchange (ETDEWEB)

    Sako, Tokuei [Laboratory of Physics, College of Science and Technology, Nihon University, 7-24-1 Narashinodai, Funabashi, Chiba 274-8501 (Japan); Ishida, Hiroshi [College of Humanities and Sciences, Nihon University, Tokyo 156-8550 (Japan); Fujikawa, Kazuo [Institute of Quantum Science, College of Science and Technology, Nihon University, Chiyoda-ku, Tokyo 101-8308 (Japan)

    2015-01-22

    The energy spectra and wave functions of a few electrons confined by a quasi-one-dimensional harmonic and anharmonic potentials have been studied by using a full configuration interaction method employing a Cartesian anisotropic Gaussian basis set. The energy spectra are classified into three regimes of the strength of confinement, namely, large, medium and small. The polyad quantum number defined by a total number of nodes in the wave functions is shown to be a key ingredient to interpret the energy spectra for the whole range of the confinement strength. The nodal pattern of the wave functions exhibits normal modes for the harmonic confining potential, indicating collective motions of electrons. These normal modes are shown to undergo a transition to local modes for an anharmonic potential with large anharmonicity.

  20. Secondary electron emission and self-consistent charge transport in semi-insulating samples

    Energy Technology Data Exchange (ETDEWEB)

    Fitting, H.-J. [Institute of Physics, University of Rostock, Universitaetsplatz 3, D-18051 Rostock (Germany); Touzin, M. [Unite Materiaux et Transformations, UMR CNRS 8207, Universite de Lille 1, F-59655 Villeneuve d' Ascq (France)

    2011-08-15

    Electron beam induced self-consistent charge transport and secondary electron emission (SEE) in insulators are described by means of an electron-hole flight-drift model (FDM) now extended by a certain intrinsic conductivity (c) and are implemented by an iterative computer simulation. Ballistic secondary electrons (SE) and holes, their attenuation to drifting charge carriers, and their recombination, trapping, and field- and temperature-dependent detrapping are included. As a main result the time dependent ''true'' secondary electron emission rate {delta}(t) released from the target material and based on ballistic electrons and the spatial distributions of currents j(x,t), charges {rho}(x,t), field F(x,t), and potential V(x,t) are obtained where V{sub 0} = V(0,t) presents the surface potential. The intrinsic electronic conductivity limits the charging process and leads to a conduction sample current to the support. In that case the steady-state total SE yield will be fixed below the unit: i.e., {sigma} {eta} + {delta} < 1.

  1. Charged particle emission effects on the characteristics of glow discharges with oscillating electrons

    CERN Document Server

    Nikulin, S P

    2001-01-01

    One discusses the effect of selection of charged particles on conditions to maintain and the characteristics of a glow discharge with oscillating electrons. It is shown that there is a pressure dependent optimal level of ion selection when the energy efficiency of ion source reaches its maximum value. It is determined that departure of fast ionizing electrons affects negatively the discharge maintenance wile emission of slow plasma electrons may promote maintenance of a discharge high current shape. It is shown that high efficient electron emission without violation of a discharge stability may take place in a magnetic field due to different nature of spatial distributions of fast and slow particles in discharges with electron oscillation

  2. Highly charged ions: a miniature laboratory for new fundamental science

    International Nuclear Information System (INIS)

    Gillaspy, J.D.

    2002-01-01

    Full text: Highly charged ions are 10-100 times smaller than ordinary atoms, yet they present within themselves a remarkably rich arena for testing fundamental aspects of physics. These tests are based on a precise analysis of the energy distribution of the photons that are emitted as electrons hop between energy levels within the highly charged ions. With sufficiently precise analysis, it may be possible to obtain new information about the structure of the vacuum, the effect of special relativity on many-body correlation, physics beyond the Standard Model, and the fundamental nature of quantum measurements. This talk will review the current state-of-the-art in the spectroscopy of highly charged ions, and give a look towards the future

  3. Charge state distributions from highly charged ions channeled at a metal surface

    International Nuclear Information System (INIS)

    Folkerts, L.; Meyer, F.W.; Schippers, S.

    1994-01-01

    The vast majority of the experimental work in the field of multicharged ion-surface interactions, to date, has focused on x-ray and particularly on electron emission. These experiments include measurements of the total electron yield, the emission statistics of the electrons, and, most of all, the electron energy distributions. So far, little attention has been paid to the fate of the multicharged projectile ions after the scattering. To our knowledge, the only measurement of the charge state distribution of the scattered ions is the pioneering experiment of de Zwart et al., who measured the total yield of scattered 1+, 2+, and 3+ ions as a function of the primary charge state q (q = 1--11) for 20 key Ne, Ar, and Kr ions after reflection from a polycrystalline tungsten target. Their main finding is the sudden onset of scattered 3+ ions when inner-shell vacancies are present in the primary particles. This suggests that a certain fraction of the inner-shell vacancies survives the entire collision event, and decays via autoionization on the outgoing path. Since the projectiles scattered in the neutral charge state could not be detected in the experiment of de Zwart et al., they were not able to provide absolute charge state fractions. In our present experiment, we focus on the scattered projectiles, measuring both the final charge state and the total scattering angle with a single 2D position sensitive detector (PSD). This method gives us the number of positive, as well as neutral and negative, scattered ions, thus allowing us to extract absolute charge state fractions. Using a well-prepared single Au(110) crystal and a grazing incidence geometry, we were able to observe surface channeling along the [001] channels

  4. Electron cyclotron resonance multiply charged ion sources

    International Nuclear Information System (INIS)

    Geller, R.

    1975-01-01

    Three ion sources, that deliver multiply charged ion beams are described. All of them are E.C.R. ion sources and are characterized by the fact that the electrons are emitted by the plasma itself and are accelerated to the adequate energy through electron cyclotron resonance (E.C.R.). They can work without interruption during several months in a quasi-continuous regime. (Duty cycle: [fr

  5. Electron mobility in few-layer MoxW1-xS2

    International Nuclear Information System (INIS)

    Chandrasekar, Hareesh; Nath, Digbijoy N

    2015-01-01

    Heterostructures of two-dimensional (2D) layered materials are increasingly being explored for electronics in order to potentially extend conventional transistor scaling and to exploit new device designs and architectures. Alloys form a key underpinning of any heterostructure device technology and therefore an understanding of their electronic properties is essential. In this paper, we study the intrinsic electron mobility in few-layer Mo x W 1−x S 2 as limited by various scattering mechanisms. The room temperature, energy-dependent scattering times corresponding to polar longitudinal optical (LO) phonon, alloy and background impurity scattering mechanisms are estimated based on the Born approximation to Fermi’s golden rule. The contribution of individual scattering rates is analyzed as a function of 2D electron density as well as of alloy composition in Mo x W 1−x S 2 . While impurity scattering limits the mobility for low carrier densities (<2–4×10 12 cm −2 ), LO polar phonon scattering is the dominant mechanism for high electron densities. Alloy scattering is found to play a non-negligible role for 0.5 < x < 0.7 in Mo x W 1−x S 2 . The LO phonon-limited and impurity-limited mobilities show opposing trends with respect to alloy mole fractions. The understanding of electron mobility in Mo x W 1−x S 2 presented here is expected to enable the design and realization of heterostructures and devices based on alloys of MoS 2 and WS 2 . (paper)

  6. Slowly moving test charge in two-electron component non-Maxwellian plasma

    International Nuclear Information System (INIS)

    Ali, S.; Eliasson, B.

    2015-01-01

    Potential distributions around a slowly moving test charge are calculated by taking into account the electron-acoustic waves in an unmagnetized plasma. Considering a neutralizing background of static positive ions, the supra-thermal hot and cold electrons are described by the Vlasov equations to account for the Kappa (power-law in velocity space) and Maxwell equilibrium distributions. Fourier analysis further leads to the derivation of electrostatic potential showing the impact of supra-thermal hot electrons. The test charge moves slowly in comparison with the hot and cold electron thermal speeds and is therefore shielded by the electrons. This gives rise to a short-range Debye-Hückel potential decaying exponentially with distance and to a far field potential decaying as inverse third power of the distance from the test charge. The results are relevant for both laboratory and space plasmas, where supra-thermal hot electrons with power-law distributions have been observed

  7. Electronic shell structure in multiply charged silver clusters

    International Nuclear Information System (INIS)

    Kandler, O.; Athanassenas, K.; Echt, O.; Kreisle, D.; Leisner, T.; Recknagel, E.

    1991-01-01

    Silver clusters are generated by standard laser vaporization technique and ionized via multiphoton ionization. Time-of-flight mass spectrometry reveals singly, doubly and triply charged clusters, Ag n z+ (z=1, 2, 3). The spectra show, for all charge states, intensity variations, indicating enhanced stabilities for cluster sizes with closed electronic configurations in accord with the spherical jellium model. (orig.)

  8. Density-dependent electron transport and precise modeling of GaN high electron mobility transistors

    Energy Technology Data Exchange (ETDEWEB)

    Bajaj, Sanyam, E-mail: bajaj.10@osu.edu; Shoron, Omor F.; Park, Pil Sung; Krishnamoorthy, Sriram; Akyol, Fatih; Hung, Ting-Hsiang [Department of Electrical and Computer Engineering, The Ohio State University, Columbus, Ohio 43210 (United States); Reza, Shahed; Chumbes, Eduardo M. [Raytheon Integrated Defense Systems, Andover, Massachusetts 01810 (United States); Khurgin, Jacob [Department of Electrical and Computer Engineering, Johns Hopkins University, Baltimore, Maryland 21218 (United States); Rajan, Siddharth [Department of Electrical and Computer Engineering, The Ohio State University, Columbus, Ohio 43210 (United States); Department of Material Science and Engineering, The Ohio State University, Columbus, Ohio 43210 (United States)

    2015-10-12

    We report on the direct measurement of two-dimensional sheet charge density dependence of electron transport in AlGaN/GaN high electron mobility transistors (HEMTs). Pulsed IV measurements established increasing electron velocities with decreasing sheet charge densities, resulting in saturation velocity of 1.9 × 10{sup 7 }cm/s at a low sheet charge density of 7.8 × 10{sup 11 }cm{sup −2}. An optical phonon emission-based electron velocity model for GaN is also presented. It accommodates stimulated longitudinal optical (LO) phonon emission which clamps the electron velocity with strong electron-phonon interaction and long LO phonon lifetime in GaN. A comparison with the measured density-dependent saturation velocity shows that it captures the dependence rather well. Finally, the experimental result is applied in TCAD-based device simulator to predict DC and small signal characteristics of a reported GaN HEMT. Good agreement between the simulated and reported experimental results validated the measurement presented in this report and established accurate modeling of GaN HEMTs.

  9. Density-dependent electron transport and precise modeling of GaN high electron mobility transistors

    International Nuclear Information System (INIS)

    Bajaj, Sanyam; Shoron, Omor F.; Park, Pil Sung; Krishnamoorthy, Sriram; Akyol, Fatih; Hung, Ting-Hsiang; Reza, Shahed; Chumbes, Eduardo M.; Khurgin, Jacob; Rajan, Siddharth

    2015-01-01

    We report on the direct measurement of two-dimensional sheet charge density dependence of electron transport in AlGaN/GaN high electron mobility transistors (HEMTs). Pulsed IV measurements established increasing electron velocities with decreasing sheet charge densities, resulting in saturation velocity of 1.9 × 10 7  cm/s at a low sheet charge density of 7.8 × 10 11  cm −2 . An optical phonon emission-based electron velocity model for GaN is also presented. It accommodates stimulated longitudinal optical (LO) phonon emission which clamps the electron velocity with strong electron-phonon interaction and long LO phonon lifetime in GaN. A comparison with the measured density-dependent saturation velocity shows that it captures the dependence rather well. Finally, the experimental result is applied in TCAD-based device simulator to predict DC and small signal characteristics of a reported GaN HEMT. Good agreement between the simulated and reported experimental results validated the measurement presented in this report and established accurate modeling of GaN HEMTs

  10. Zero-degree binary encounter electrons in fast collisions of highly charged F and O ions with H2 targets

    International Nuclear Information System (INIS)

    Lee, D.H.; Zouros, T.J.M.; Sanders, J.M.; Hidmi, H.; Richard, P.

    1993-01-01

    Doubly differential cross sections (DDCS) for binary encounter electrons (BEe) produced by 0.5-2 MeV/u highly-charged F and O ions in collisions with H 2 gas targets have been studied at 0 with respect to the ion beam direction. The measured DDCS of the broad binary encounter peak was well described by a simple impulse approximation (IA) treatment for bare ions, and was demonstrated to provide in situ detection efficiency of the electron spectrometer. The projectile energy dependence of the BEe production for nonbare (clothed) projectiles is found to follow a scaled IA prediction, in which a BEe enhancement is consistently exhibited for the collision energy range studied. (orig.)

  11. Electron acceleration via high contrast laser interacting with submicron clusters

    International Nuclear Information System (INIS)

    Zhang Lu; Chen Liming; Wang Weiming; Yan Wenchao; Yuan Dawei; Mao Jingyi; Wang Zhaohua; Liu Cheng; Shen Zhongwei; Li Yutong; Dong Quanli; Lu Xin; Ma Jinglong; Wei Zhiyi; Faenov, Anatoly; Pikuz, Tatiana; Li Dazhang; Sheng Zhengming; Zhang Jie

    2012-01-01

    We experimentally investigated electron acceleration from submicron size argon clusters-gas target irradiated by a 100 fs, 10 TW laser pulses having a high-contrast. Electron beams are observed in the longitudinal and transverse directions to the laser propagation. The measured energy of the longitudinal electron reaches 600 MeV and the charge of the electron beam in the transverse direction is more than 3 nC. A two-dimensional particle-in-cell simulation of the interaction has been performed and it shows an enhancement of electron charge by using the cluster-gas target.

  12. Dissociative electron attachment and charge transfer in condensed matter

    International Nuclear Information System (INIS)

    Bass, A.D.; Sanche, L.

    2003-01-01

    Experiments using energy-selected beams of electrons incident from vacuum upon thin vapour deposited solids show that, as in the gas-phase, scattering cross sections at low energies are dominated by the formation of temporary negative ions (or resonances) and that molecular damage may be effected via dissociative electron attachment (DEA). Recent results also show that charge transfer between anionic states of target molecules and their environment is often crucial in determining cross sections for electron driven processes. Here, we review recent work from our laboratory, in which charge transfer is observed. For rare gas solids, electron exchange between the electron-exciton complex and either a metal substrate or co-adsorbed molecule enhances the desorption of metastable atoms and/or molecular dissociation. We discuss how transient electron capture by surface electron states of a substrate and subsequent electron transfer to a molecular adsorbate enhances the effective cross sections for DEA. We also consider the case of DEA to CF 2 Cl 2 condensed on water and ammonia ices, where electron exchange between pre-solvated electron states of ice and transient molecular anions can also increase DEA cross sections. Electron transfer from molecular resonances into pre-solvated electron states of ice is also discussed

  13. Absolute beam-charge measurement for single-bunch electron beams

    International Nuclear Information System (INIS)

    Suwada, Tsuyoshi; Ohsawa, Satoshi; Furukawa, Kazuro; Akasaka, Nobumasa

    2000-01-01

    The absolute beam charge of a single-bunch electron beam with a pulse width of 10 ps and that of a short-pulsed electron beam with a pulse width of 1 ns were measured with a Faraday cup in a beam test for the KEK B-Factory (KEKB) injector linac. It is strongly desired to obtain a precise beam-injection rate to the KEKB rings, and to estimate the amount of beam loss. A wall-current monitor was also recalibrated within an error of ±2%. This report describes the new results for an absolute beam-charge measurement for single-bunch and short-pulsed electron beams, and recalibration of the wall-current monitors in detail. (author)

  14. Space-charge effects in high-energy photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Verna, Adriano, E-mail: adriano.verna@uniroma3.it [Dipartimento di Scienze, Università degli Studi Roma Tre, Via della Vasca Navale 84, I-00146 Roma (Italy); CNISM Unità di Roma Tre, Via della Vasca Navale 84, I-00146 Roma (Italy); Greco, Giorgia [Dipartimento di Scienze, Università degli Studi Roma Tre, Via della Vasca Navale 84, I-00146 Roma (Italy); Lollobrigida, Valerio [Dipartimento di Scienze, Università degli Studi Roma Tre, Via della Vasca Navale 84, I-00146 Roma (Italy); Scuola Dottorale in Matematica e Fisica, Università Roma Tre, Via della Vasca Navale 84, I-00146 Roma (Italy); Offi, Francesco; Stefani, Giovanni [Dipartimento di Scienze, Università degli Studi Roma Tre, Via della Vasca Navale 84, I-00146 Roma (Italy); CNISM Unità di Roma Tre, Via della Vasca Navale 84, I-00146 Roma (Italy)

    2016-05-15

    Highlights: • N-body simulations of interacting photoelectrons in hard X-ray experiments. • Secondary electrons have a pivotal role in determining the energy broadening. • Space charge has negligible effects on the photoelectron momentum distribution. • A simple model provides the characteristic time for energy-broadening mechanism. • The feasibility of time-resolved high-energy experiments with FELs is discussed. - Abstract: Pump-and-probe photoelectron spectroscopy (PES) with femtosecond pulsed sources opens new perspectives in the investigation of the ultrafast dynamics of physical and chemical processes at the surfaces and interfaces of solids. Nevertheless, for very intense photon pulses a large number of photoelectrons are simultaneously emitted and their mutual Coulomb repulsion is sufficiently strong to significantly modify their trajectory and kinetic energy. This phenomenon, referred as space-charge effect, determines a broadening and shift in energy for the typical PES structures and a dramatic loss of energy resolution. In this article we examine the effects of space charge in PES with a particular focus on time-resolved hard X-ray (∼10 keV) experiments. The trajectory of the electrons photoemitted from pure Cu in a hard X-ray PES experiment has been reproduced through N-body simulations and the broadening of the photoemission core-level peaks has been monitored as a function of various parameters (photons per pulse, linear dimension of the photon spot, photon energy). The energy broadening results directly proportional to the number N of electrons emitted per pulse (mainly represented by secondary electrons) and inversely proportional to the linear dimension a of the photon spot on the sample surface, in agreement with the literature data about ultraviolet and soft X-ray experiments. The evolution in time of the energy broadening during the flight of the photoelectrons is also studied. Despite its detrimental consequences on the energy

  15. Stochastic Coulomb interactions in space charge limited electron emission

    NARCIS (Netherlands)

    Nijkerk, M.D.; Kruit, P.

    2004-01-01

    A Monte Carlo simulation tool, which was used to evaluate the influence of discrete space charge effects on self-consistent calculations of cathode-ray tube optics, was discussed. It was found that interactions in the space charge cloud affect the electron trajectories such that the velocity

  16. Hydration of excess electrons trapped in charge pockets on molecular surfaces

    Science.gov (United States)

    Jalbout, Abraham F.; Del Castillo, R.; Adamowicz, Ludwik

    2007-01-01

    In this work we strive to design a novel electron trap located on a molecular surface. The process of electron trapping involves hydration of the trapped electron. Previous calculations on surface electron trapping revealed that clusters of OH groups can form stable hydrogen-bonded networks on one side of a hydrocarbon surface (i.e. cyclohexane sheets), while the hydrogen atoms on the opposite side of the surface form pockets of positive charge that can attract extra negative charge. The excess electron density on such surfaces can be further stabilized by interactions with water molecules. Our calculations show that these anionic systems are stable with respect to vertical electron detachment (VDE).

  17. A high charge state heavy ion beam source for heavy ion fusion

    International Nuclear Information System (INIS)

    Eylon, S.; Henestroza, E.

    1996-01-01

    A high current, low emittance, high charge state heavy ion beam source is being developed. This is designed to deliver a heavy ion fusion (HIF) driver accelerator scale beam. Using a high charge state beam in a driver accelerator for HIF may increase the acceleration efficiency, leading to a reduction in the driver accelerator size and cost. The proposed source system, which consists of a gas beam electron stripper followed by a high charge state beam separator, can be added to existing single charge state, low emittance, high brightness ion sources and injectors. We shall report on the source physics design using 3D beam simulations and experimental feasibility study results using a neutral gas stripper and a beam separator at the exit of the LBL 2 MV injector. (orig.)

  18. Phonon-electron coupling and tunneling effect on charge transport in organic semi-conductor crystals of Cn-BTBT

    Science.gov (United States)

    Zhou, Yecheng; Deng, Wei-Qiao; Zhang, Hao-Li

    2016-09-01

    Cn-[1]benzothieno[3,2-b][1]-benzothiophene (BTBT) crystals show very high hole mobilities in experiments. These high mobilities are beyond existing theory prediction. Here, we employed different quantum chemistry methods to investigate charge transfer in Cn-BTBT crystals and tried to find out the reasons for the underestimation in the theory. It was found that the hopping rate estimated by the Fermi Golden Rule is higher than that of the Marcus theory due to the high temperature approximation and failure at the classic limit. More importantly, molecular dynamics simulations revealed that the phonon induced fluctuation of electronic transfer integral is much larger than the average of the electronic transfer integral itself. Mobilities become higher if simulations implement the phonon-electron coupling. This conclusion indicates that the phonon-electron coupling promotes charge transfer in organic semi-conductors at room temperature.

  19. Van der Waals stacks of few-layer h-AlN with graphene: an ab initio study of structural, interaction and electronic properties

    International Nuclear Information System (INIS)

    Dos Santos, Renato B; Mota, F de Brito; Rivelino, R; Kakanakova-Georgieva, A; Gueorguiev, G K

    2016-01-01

    Graphite-like hexagonal AlN (h-AlN) multilayers have been experimentally manifested and theoretically modeled. The development of any functional electronics applications of h-AlN would most certainly require its integration with other layered materials, particularly graphene. Here, by employing vdW-corrected density functional theory calculations, we investigate structure, interaction energy, and electronic properties of van der Waals stacking sequences of few-layer h-AlN with graphene. We find that the presence of a template such as graphene induces enough interlayer charge separation in h-AlN, favoring a graphite-like stacking formation. We also find that the interface dipole, calculated per unit cell of the stacks, tends to increase with the number of stacked layers of h-AlN and graphene. (paper)

  20. Electron scattering by nuclei and transition charge densities

    International Nuclear Information System (INIS)

    Gul'karov, I.S.

    1988-01-01

    Transition charge densities for states of electric type, for nuclei with A≤40--50 as obtained from data on inelastic electron scattering, are studied. The formalism of electroexcitation of nuclei is considered, together with various models (macroscopic and microscopic) used to calculate form factors, transition charge densities, and the moments of these densities: B(Eλ) and R/sub λ/ . The macroscopic models are derived microscopically, and it is shown that the model-independent sum rules lead to the same transition densities as calculations based on various hydrodynamic models. The sum rules with and without allowance for the Skyrme exchange interaction are discussed. The results of the calculations are compared with the experimental form factors of electron scattering by nuclei from 12 C to 48 Ca with excitation in them of normal-parity states with I/sup π/ = 0 + , 1 - , 2 + , 3 - , 4 + , 5 - and T = 0. The model-independent transition charge densities for the weakly collectivized excitations differ strongly from the model-dependent densities. The influence of neutrons on the transition charge densities of the nuclear isotopes 16 /sup ,/ 18 O, 32 /sup ,/ 34 S, and 40 /sup ,/ 48 Ca is considered

  1. High-sensitivity visualization of localized electric fields using low-energy electron beam deflection

    Science.gov (United States)

    Jeong, Samuel; Ito, Yoshikazu; Edwards, Gary; Fujita, Jun-ichi

    2018-06-01

    The visualization of localized electronic charges on nanocatalysts is expected to yield fundamental information about catalytic reaction mechanisms. We have developed a high-sensitivity detection technique for the visualization of localized charges on a catalyst and their corresponding electric field distribution, using a low-energy beam of 1 to 5 keV electrons and a high-sensitivity scanning transmission electron microscope (STEM) detector. The highest sensitivity for visualizing a localized electric field was ∼0.08 V/µm at a distance of ∼17 µm from a localized charge at 1 keV of the primary electron energy, and a weak local electric field produced by 200 electrons accumulated on the carbon nanotube (CNT) apex can be visualized. We also observed that Au nanoparticles distributed on a CNT forest tended to accumulate a certain amount of charges, about 150 electrons, at a ‑2 V bias.

  2. Effect of minimum strength of mirror magnetic field (Bmin) on production of highly charged heavy ions from RIKEN liquid-He-free super conducting electron-cyclotron resonance ion source (RAMSES)

    International Nuclear Information System (INIS)

    Arai, Hideyuki; Imanaka, Masashi; Lee, S.-M.Sang-Moo; Higurashi, Yoshihide; Nakagawa, Takahide; Kidera, Masanori; Kageyama, Tadashi; Kase, Masayuki; Yano, Yasushige; Aihara, Toshimitsu

    2002-01-01

    We measured the beam intensity of highly charged heavy ions (O, Ar and Kr ions) as a function of the minimum strength of mirror magnetic field (B min ) of the RIKEN liquid-He-free super conducting electron-cyclotron resonance ion source. In this experiment, we found that the optimum value of B min exists to maximize the beam intensity of highly charged heavy ions and the value was almost the same (∼0.49 T) for various charge state heavy ions

  3. Electron collection enhancement arising from neutral gas jets on a charged vehicle in the ionosphere

    International Nuclear Information System (INIS)

    Gilchrist, B.E.; Banks, P.M.; Neubert, T.; Williamson, P.R.; Myers, N.B.; Raitt, W.J.; Sasaki, Susumu

    1990-01-01

    Observations of current collection enhancements due to cold nitrogen gas control jet emissions from a highly charged, isolated rocket payload in the ionosphere have been made during the cooperative high altitude rocket gun experiment (CHARGE) 2 using an electrically tethered mother/daughter payload system. The current collection enhancement was observed on a platform (daughter payload) located 100 to 400 m away from the main payload firing an energetic electron beam (mother payload). The authors interpret these results in terms of an electrical discharge forming in close proximity to the daughter vehicle during the short periods of gas emission. The results indicate that it is possible to enhance the electron current collection capability of positively charged vehicles by means of deliberate neutral gas releases into an otherwise undisturbed space plasma. The results are also compared with recent laboratory observations of hollow cathode plasma contactors operating in the ignited mode

  4. Spectroscopic Investigations of Highly Charged Ions using X-Ray Calorimeter Spectrometers

    Energy Technology Data Exchange (ETDEWEB)

    Thorn, Daniel Bristol [Univ. of California, Davis, CA (United States)

    2008-11-19

    Spectroscopy of K-shell transitions in highly charged heavy ions, like hydrogen-like uranium, has the potential to yield information about quantum electrodynamics (QED) in extremely strong nuclear fields as well as tests of the standard model, specifically parity violation in atomic systems. These measurements would represent the 'holy grail' in high-Z atomic spectroscopy. However, the current state-of-the-art detection schemes used for recording the K-shell spectra from highly charged heavy ions does not yet have the resolving power to be able to attain this goal. As such, to push the field of high-Z spectroscopy forward, new detectors must be found. Recently, x-ray calorimeter spectrometers have been developed that promise to make such measurements. In an effort to make the first steps towards attaining the 'holy grail', measurements have been performed with two x-ray calorimeter spectrometers (the XRS/EBIT and the ECS) designed and built at Goddard Space Flight Center in Greenbelt, MD. The calorimeter spectrometers have been used to record the K-shell spectra of highly charged ions produced in the SuperEBIT electron beam ion trap at Lawrence Livermore National Laboratory in Livermore, CA. Measurements performed with the XRS/EBIT calorimeter array found that the theoretical description of well-above threshold electron-impact excitation cross sections for hydrogen-like iron and nickel ions are correct. Furthermore, the first high-resolution spectrum of hydrogen-like through carbon-like praseodymium ions was recorded with a calorimeter. In addition, the new high-energy array on the EBIT Calorimeter Spectrometer (ECS) was used to resolve the K-shell x-ray emission spectrum of highly charged xenon ions, where a 40 ppm measurement of the energy of the K-shell resonance transition in helium-like xenon was achieved. This is the highest precision result, ever, for an element with such high atomic number. In addition, a first-of-its-kind measurement of

  5. Spectroscopic Investigations of Highly Charged Ions using X-Ray Calorimeter Spectrometers

    International Nuclear Information System (INIS)

    Thorn, D. B.

    2008-01-01

    Spectroscopy of K-shell transitions in highly charged heavy ions, like hydrogen-like uranium, has the potential to yield information about quantum electrodynamics (QED) in extremely strong nuclear fields as well as tests of the standard model, specifically parity violation in atomic systems. These measurements would represent the 'holy grail' in high-Z atomic spectroscopy. However, the current state-of-the-art detection schemes used for recording the K-shell spectra from highly charged heavy ions does not yet have the resolving power to be able to attain this goal. As such, to push the field of high-Z spectroscopy forward, new detectors must be found. Recently, x-ray calorimeter spectrometers have been developed that promise to make such measurements. In an effort to make the first steps towards attaining the 'holy grail', measurements have been performed with two x-ray calorimeter spectrometers (the XRS/EBIT and the ECS) designed and built at Goddard Space Flight Center in Greenbelt, MD. The calorimeter spectrometers have been used to record the K-shell spectra of highly charged ions produced in the SuperEBIT electron beam ion trap at Lawrence Livermore National Laboratory in Livermore, CA. Measurements performed with the XRS/EBIT calorimeter array found that the theoretical description of well-above threshold electron-impact excitation cross sections for hydrogen-like iron and nickel ions are correct. Furthermore, the first high-resolution spectrum of hydrogen-like through carbon-like praseodymium ions was recorded with a calorimeter. In addition, the new high-energy array on the EBIT Calorimeter Spectrometer (ECS) was used to resolve the K-shell x-ray emission spectrum of highly charged xenon ions, where a 40 ppm measurement of the energy of the K-shell resonance transition in helium-like xenon was achieved. This is the highest precision result, ever, for an element with such high atomic number. In addition, a first-of-its-kind measurement of the effect of the

  6. Tuning the Electron Gas at an Oxide Heterointerface via Free Surface Charges

    Energy Technology Data Exchange (ETDEWEB)

    Bell, Christopher

    2011-08-11

    Oxide heterointerfaces are emerging as one of the most exciting materials systems in condensed matter science. One remarkable example is the LaAlO{sub 3}/SrTiO{sub 3} (LAO/STO) interface, a model system in which a highly mobile electron gas forms between two band insulators, exhibiting two dimensional superconductivity and unusual magnetotransport properties. An ideal tool to tune such an electron gas is the electrostatic field effect. In principle, the electrostatic field can be generated by bound charges due to polarization (as in the normal and ferroelectric field effects) or by adding excess free charge. In previous studies, a large modulation of the carrier density and mobility of the LAO/STO interface has been achieved using the normal field effect. However, little attention has been paid to the field effect generated by free charges. This issue is scarcely addressed, even in conventional semiconductor devices, since the free charges are typically not stable. Here, we demonstrate an unambiguous tuning of the LAO/STO interface conductivity via free surface charges written using conducting atomic force microscopy (AFM). The modulation of the carrier density was found to be reversible, nonvolatile and surprisingly large, {approx}3 x 10{sup 13} cm{sup -2}, comparable to the maximum modulation by the normal field effect. Our finding reveal the efficiency of free charges in controlling the conductivity of this oxide interface, and suggest that this technique may be extended more generally to other oxide systems.

  7. Bond charge approximation for valence electron density in elemental semiconductors

    International Nuclear Information System (INIS)

    Bashenov, V.K.; Gorbachov, V.E.; Marvakov, D.I.

    1985-07-01

    The spatial valence electron distribution in silicon and diamond is calculated in adiabatic bond charge approximation at zero temperature when bond charges have the Gaussian shape and their tensor character is taken into account. An agreement between theory and experiment has been achieved. For this purpose Xia's ionic pseudopotentials and Schulze-Unger's dielectric function are used. By two additional parameters Asub(B) and Zsub(B)sup(') we describe the spatial extent of the bond charge and local-field corrections, respectively. The parameter Zsub(B)sup(') accounts for the ratio between the Coulomb and exchange correlation interactions of the valence electrons and its silicon and diamond values have different signs. (author)

  8. Design and dosimetry of a few leaf electron collimator for energy modulated electron therapy

    International Nuclear Information System (INIS)

    Al-Yahya, Khalid; Verhaegen, Frank; Seuntjens, Jan

    2007-01-01

    Despite the capability of energy modulated electron therapy (EMET) to achieve highly conformal dose distributions in superficial targets it has not been widely implemented due to problems inherent in electron beam radiotherapy such as planning dosimetry accuracy, and verification as well as a lack of systems for automated delivery. In previous work we proposed a novel technique to deliver EMET using an automated 'few leaf electron collimator' (FLEC) that consists of four motor-driven leaves fit in a standard clinical electron beam applicator. Integrated with a Monte Carlo based optimization algorithm that utilizes patient-specific dose kernels, a treatment delivery was incorporated within the linear accelerator operation. The FLEC was envisioned to work as an accessory tool added to the clinical accelerator. In this article the design and construction of the FLEC prototype that match our compact design goals are presented. It is controlled using an in-house developed EMET controller. The structure of the software and the hardware characteristics of the EMET controller are demonstrated. Using a parallel plate ionization chamber, output measurements were obtained to validate the Monte Carlo calculations for a range of fields with different energies and sizes. Further verifications were also performed for comparing 1-D and 2-D dose distributions using energy independent radiochromic films. Comparisons between Monte Carlo calculations and measurements of complex intensity map deliveries show an overall agreement to within ±3%. This work confirms our design objectives of the FLEC that allow for automated delivery of EMET. Furthermore, the Monte Carlo dose calculation engine required for EMET planning was validated. The result supports the potential of the prototype FLEC for the planning and delivery of EMET

  9. High-k shallow traps observed by charge pumping with varying discharging times

    Energy Technology Data Exchange (ETDEWEB)

    Ho, Szu-Han; Chen, Ching-En; Tseng, Tseung-Yuen [Department of Electronics Engineering, National Chiao Tung University, Hsinchu 300, Taiwan (China); Chang, Ting-Chang, E-mail: tcchang@mail.phys.nsysu.edu.tw [Department of Physics, National Sun Yat-Sen University, Kaohsiung 804, Taiwan (China); Advanced Optoelectronics Technology Center, National Cheng Kung University, Tainan, Taiwan (China); Lu, Ying-Hsin; Lo, Wen-Hung; Tsai, Jyun-Yu; Liu, Kuan-Ju [Department of Physics, National Sun Yat-Sen University, Kaohsiung 804, Taiwan (China); Wang, Bin-Wei; Cao, Xi-Xin [Department of Embedded System Engineering, Peking University, Beijing, P.R.China (China); Chen, Hua-Mao [Department of Photonics and Institute of Electro-Optical Engineering, National Chiao Tung University, Hsinchu, Taiwan (China); Cheng, Osbert; Huang, Cheng-Tung; Chen, Tsai-Fu [Device Department, United Microelectronics Corporation, Tainan Science Park, Taiwan (China)

    2013-11-07

    In this paper, we investigate the influence of falling time and base level time on high-k bulk shallow traps measured by charge pumping technique in n-channel metal-oxide-semiconductor field-effect transistors with HfO{sub 2}/metal gate stacks. N{sub T}-V{sub high} {sub level} characteristic curves with different duty ratios indicate that the electron detrapping time dominates the value of N{sub T} for extra contribution of I{sub cp} traps. N{sub T} is the number of traps, and I{sub cp} is charge pumping current. By fitting discharge formula at different temperatures, the results show that extra contribution of I{sub cp} traps at high voltage are in fact high-k bulk shallow traps. This is also verified through a comparison of different interlayer thicknesses and different Ti{sub x}N{sub 1−x} metal gate concentrations. Next, N{sub T}-V{sub high} {sub level} characteristic curves with different falling times (t{sub falling} {sub time}) and base level times (t{sub base} {sub level}) show that extra contribution of I{sub cp} traps decrease with an increase in t{sub falling} {sub time}. By fitting discharge formula for different t{sub falling} {sub time}, the results show that electrons trapped in high-k bulk shallow traps first discharge to the channel and then to source and drain during t{sub falling} {sub time}. This current cannot be measured by the charge pumping technique. Subsequent measurements of N{sub T} by charge pumping technique at t{sub base} {sub level} reveal a remainder of electrons trapped in high-k bulk shallow traps.

  10. On a possibility of creation of positive space charge cloud in a system with magnetic insulation of electrons

    International Nuclear Information System (INIS)

    Goncharov, A.A.; Dobrovol'skii, A.M.; Dunets, S.P.; Evsyukov, A.N.; Protsenko, I.M.

    2009-01-01

    We describe a new approach for creation an effective, low-cost, low-maintenance axially symmetric plasma optical tools for focusing and manipulating high-current beams of negatively charged particles, electrons and negative ions. This approach is based on fundamental plasma optical concept of magnetic insulation of electrons and non-magnetized positive ions providing creation of controlled uncompensated cloud of the space charge. The axially symmetric electrostatic plasma optical lens is well-known and well developed tool where this concept is used successfully. This provides control and focusing high-current positive ion beams in wide range of parameters. Here for the first time we present optimistic experimental results describing the application of an idea of magnetic insulation of electrons for generation of the stable cloud of positive space charge by focusing onto axis the converging stream of heavy ions produced by circular accelerator with closed electron drift. The estimations of a maximal concentration of uncompensated cloud of positive ions are also made

  11. Spectral measurements of few-electron uranium ions produced and trapped in a high-energy electron beam ion trap

    International Nuclear Information System (INIS)

    Beiersdorfer, P.

    1994-01-01

    Measurements of 2s l/2 -2p 3/2 electric dipole and 2p 1/2 -2p 3/2 magnetic dipole and electric quadrupole transitions in U 82+ through U 89+ have been made with a high-resolution crystal spectrometer that recorded the line radiation from stationary ions produced and trapped in a high-energy electron beam ion trap. From the measurements we infer -39.21 ± 0.23 eV for the QED contribution to the 2s 1/2 -2p 3/2 transition energy of lithiumlike U 89+ . A comparison between our measurements and various computations illustrates the need for continued improvements in theoretical approaches for calculating the atomic structure of ions with two or more electrons in the L shell

  12. Injection of an electron beam into a plasma and spacecraft charging

    International Nuclear Information System (INIS)

    Okuda, H.; Kan, J.R.

    1987-01-01

    Injection of a nonrelativistic electron beam into a fully ionized plasma from a spacecraft including the effect of charging has been studied using a one-dimensional particle simulation model. It is found that the spacecraft charging remains negligible and the beam can propagate into a plasma, if the beam density is much smaller than the ambient density. When the injection current is increased by increasing the beam density, significant spacecraft charging takes place and the reflection of beam electrons back to the spacecraft reduces the beam current significantly. On the other hand, if the injection current is increased by increasing the beam energy, spacecraft charging remains negligible and a beam current much larger than the thermal return current can be injected. It is shown that the electric field caused by the beam--plasma instability accelerates the ambient electrons toward the spacecraft thereby enhancing the return current

  13. Simulation of the interaction of positively charged beams and electron clouds

    International Nuclear Information System (INIS)

    Markovik, Aleksandar

    2013-01-01

    The incoherent (head-tail) effect on the bunch due to the interaction with electron clouds (e-clouds) leads to a blow up of the transverse beam size in storage rings operating with positively charged beams. Even more the e-cloud effects are considered to be the main limiting factor for high current, high-brightness or high-luminosity operation of future machines. Therefore the simulation of e-cloud phenomena is a highly active field of research. The main focus in this work was set to a development of a tool for simulation of the interaction of relativistic bunches with non-relativistic parasitic charged particles. The result is the Particle-In-Cell Program MOEVE PIC Tracking which can track a 3D bunch under the influence of its own and external electromagnetic fields but first and foremost it simulates the interaction of relativistic positively charged bunches and initially static electrons. In MOEVE PIC Tracking the conducting beam pipe can be modeled with an arbitrary elliptical cross-section to achieve more accurate space charge field computations for both the bunch and the e-cloud. The simulation of the interaction between positron bunches and electron clouds in this work gave a detailed insight of the behavior of both particle species during and after the interaction. Further and ultimate goal of this work was a fast estimation of the beam stability under the influence of e-clouds in the storage ring. The standard approach to simulate the stability of a single bunch is to track the bunch particles through the linear optics of the machine by multiplying the 6D vector of each particle with the transformation matrices describing the lattice. Thereby the action of the e-cloud on the bunch is approximated by a pre-computed wake kick which is applied on one or more points in the lattice. Following the idea of K.Ohmi the wake kick was pre-computed as a two variable function of the bunch part exiting the e-cloud and the subsequent parts of a bunch which receive a

  14. Understanding charge transport in molecular electronics.

    Science.gov (United States)

    Kushmerick, J J; Pollack, S K; Yang, J C; Naciri, J; Holt, D B; Ratner, M A; Shashidhar, R

    2003-12-01

    For molecular electronics to become a viable technology the factors that control charge transport across a metal-molecule-metal junction need to be elucidated. We use an experimentally simple crossed-wire tunnel junction to interrogate how factors such as metal-molecule coupling, molecular structure, and the choice of metal electrode influence the current-voltage characteristics of a molecular junction.

  15. Charge exchange as a recombination mechanism in high-temperature plasmas

    International Nuclear Information System (INIS)

    Hulse, R.A.; Post, D.E.; Mikkelsen, D.R.

    1980-03-01

    Charge exchange with neutral hydrogen is examined as a recombination mechanism for multi-charged impurity ions present in high-temperature fusion plasmas. At sufficiently low electron densities, fluxes of atomic hydrogen produced by either the injection of neutral heating beams or the background of thermal neutrals can yield an important or even dominant recombination process for such ions. Equilibrium results are given for selected impurity elements showing the altered ionization balance and radiative cooling rate produced by the presence of various neutral populations. A notable result is that the stripping of impurities to relatively non-radiative ionization states with increasing electron temperature can be postponed or entirely prevented by the application of intense neutral beam heating power. A time dependent calculation modelling the behavior of iron in recent PLT tokamak high power neutral beam heating experiments is also presented

  16. Optical Pumping of the Electronic and Nuclear Spin of Single Charge-Tunable Quantum Dots

    Science.gov (United States)

    Bracker, A. S.; Stinaff, E. A.; Gammon, D.; Ware, M. E.; Tischler, J. G.; Shabaev, A.; Efros, Al. L.; Park, D.; Gershoni, D.; Korenev, V. L.; Merkulov, I. A.

    2005-02-01

    We present a comprehensive examination of optical pumping of spins in individual GaAs quantum dots as we change the net charge from positive to neutral to negative with a charge-tunable heterostructure. Negative photoluminescence polarization memory is enhanced by optical pumping of ground state electron spins, which we prove with the first measurements of the Hanle effect on an individual quantum dot. We use the Overhauser effect in a high longitudinal magnetic field to demonstrate efficient optical pumping of nuclear spins for all three charge states of the quantum dot.

  17. Possible Diamond-Like Nanoscale Structures Induced by Slow Highly-Charged Ions on Graphite (HOPG)

    Energy Technology Data Exchange (ETDEWEB)

    Sideras-Haddad, E.; Schenkel, T.; Shrivastava, S.; Makgato, T.; Batra, A.; Weis, C. D.; Persaud, A.; Erasmus, R.; Mwakikunga, B.

    2009-01-06

    The interaction between slow highly-charged ions (SHCI) of different charge states from an electron-beam ion trap and highly oriented pyrolytic graphite (HOPG) surfaces is studied in terms of modification of electronic states at single-ion impact nanosizeareas. Results are presented from AFM/STM analysis of the induced-surface topological features combined with Raman spectroscopy. I-V characteristics for a number of different impact regions were measured with STM and the results argue for possible formation of diamond-like nanoscale structures at the impact sites.

  18. Highly charged ion impact induced nanodefects in diamond

    Energy Technology Data Exchange (ETDEWEB)

    Makgato, T.N., E-mail: thuto.makgato@wits.ac.za [School of Physics, University of the Witwatersrand, Johannesburg 2050 (South Africa); Microscopy and Microanalysis Unit, University of the Witwatersrand, Johannesburg 2050 (South Africa); Sideras-Haddad, E. [School of Physics, University of the Witwatersrand, Johannesburg 2050 (South Africa); Centre of Excellence in Strong Materials, Physics Building, University of the Witwatersrand, Johannesburg 2050 (South Africa); Shrivastava, S. [School of Physics, University of the Witwatersrand, Johannesburg 2050 (South Africa); Schenkel, T. [E.O. Lawrence Berkeley National Laboratory, Berkeley, CA 94720 (United States); Ritter, R.; Kowarik, G.; Aumayr, F. [Institute of Applied Physics, TU Wien-Vienna University of Technology, 1040 Vienna (Austria); Crespo Lopez-Urrutia, J.; Bernitt, S.; Beilmann, C.; Ginzel, R. [Max-Planck Institute for Nuclear Physics, Saupfercheckweg 1, 69117 Heidelberg (Germany)

    2013-11-01

    We investigate the interaction of slow highly charged ion (SHCI) beams with insulating type Ib diamond (1 1 1) surfaces. Bismuth and Xenon SHCI beams produced using an Electron Beam Ion Trap (EBIT) and an Electron Cyclotron Resonance source (ECR) respectively, are accelerated onto type Ib diamond (1 1 1) surfaces with impact velocities up to ≈0.4 υ{sub Bohr}. SHCIs with charge states corresponding to potential energies between 4.5 keV and 110 keV are produced for this purpose. Atomic Force Microscopy analysis (AFM) of the diamond surfaces following SHCI impact reveals surface morphological modifications characterized as nanoscale craters (nano-craters). To interpret the results from Tapping Mode AFM analysis of the irradiated diamond surfaces we discuss the interplay between kinetic and potential energy in nano-crater formation using empirical data together with Stopping and Range of Ions in Matter (SRIM) Monte Carlo Simulations.

  19. Electron transfer and decay processes of highly charged iodine ions

    International Nuclear Information System (INIS)

    Sakaue, Hiroyuki A.; Danjo, Atsunori; Hosaka, Kazumoto

    2005-01-01

    In the present experimental work we have investigated multi-electron transfer processes in I q+ (q=10, 15, 20 and 25) + Ne, Ar, Kr and Xe collisions at 1.5q keV energy. The branching ratios between Auger and radiative decay channels have been measured in decay processes of multiply excited states formed by multi-electron transfer collisions. It has been shown that, in all the multi-electron transfer processes investigated, the Auger decays are far dominant over the radiative decay processes and the branching ratios are clearly characterized by the average principal quantum number of the initial excited states of projectile ions. We could express the branching ratios in high Rydberg states formed in multi-electron transfer processes by using the decay probability of one Auger electron emission. (author)

  20. Kapton charging characteristics: Effects of material thickness and electron-energy distribution

    Science.gov (United States)

    Williamson, W. S.; Dulgeroff, C. R.; Hymann, J.; Viswanathan, R.

    1985-01-01

    Charging characteristics of polyimide (Kapton) of varying thicknesses under irradiation by a very-low-curent-density electron beam, with the back surface of the sample grounded are reported. These charging characteristics are in good agreement with a simple analytical model which predicts that in thin samples at low current density, sample surface potential is limited by conduction leakage through the bulk material. The charging of Kapton in a low-current-density electron beam in which the beam energy was modulated to simulate Maxwellian and biMaxwellian distribution functions is measured.

  1. Guiding effect of bent macroscopic quartz tube for high current electron beam

    International Nuclear Information System (INIS)

    Zhang Mingwu; Chen Jing; Wu Yehong; Yang Bian; Wang Wei; Xue Yingli; Yu Deyang; Cai Xiaohong

    2012-01-01

    By using an incident electron beam with the high current and high energy, the guiding effect of the bent macroscopic quartz tube for the electron beam has been investigated. The angular distributions of outgoing electrons depending on the current and energy of incident electrons were measured. The dependences of electron transmitted fraction on energy and current of incident electrons are also shown. As the incident electron energy increasing, the electron transmitted fraction increases, but it decreases while the incident electron current increasing. The results have been compared with the present data. This work presents, the process of guiding electrons is essentially different from that of guiding highly charged ions, the guiding electron beam was caused by both elastic and inelastic collisions between electrons and inner walls of quartz tube, rather than self-organized charging effect on the surface of inner wall of quartz tube. (authors)

  2. Strong-field relativistic processes in highly charged ions

    Energy Technology Data Exchange (ETDEWEB)

    Postavaru, Octavian

    2010-12-08

    In this thesis we investigate strong-field relativistic processes in highly charged ions. In the first part, we study resonance fluorescence of laser-driven highly charged ions in the relativistic regime by solving the time-dependent master equation in a multi-level model. Our ab initio approach based on the Dirac equation allows for investigating highly relativistic ions, and, consequently, provides a sensitive means to test correlated relativistic dynamics, bound-state quantum electrodynamic phenomena and nuclear effects by applying coherent light with x-ray frequencies. Atomic dipole or multipole moments may be determined to unprecedented accuracy by measuring the interference-narrowed fluorescence spectrum. Furthermore, we investigate the level structure of heavy hydrogenlike ions in laser beams. Interaction with the light field leads to dynamic shifts of the electronic energy levels, which is relevant for spectroscopic experiments. We apply a fully relativistic description of the electronic states by means of the Dirac equation. Our formalism goes beyond the dipole approximation and takes into account non-dipole effects of retardation and interaction with the magnetic field components of the laser beam. We predicted cross sections for the inter-shell trielectronic recombination (TR) and quadruelectronic recombination processes which have been experimentally confirmed in electron beam ion trap measurements, mainly for C-like ions, of Ar, Fe and Kr. For Kr{sup 30}+, inter-shell TR contributions of nearly 6% to the total resonant photorecombination rate were found. (orig.)

  3. Nonlinear charge transport in bipolar semiconductors due to electron heating

    International Nuclear Information System (INIS)

    Molina-Valdovinos, S.; Gurevich, Yu.G.

    2016-01-01

    It is known that when strong electric field is applied to a semiconductor sample, the current voltage characteristic deviates from the linear response. In this letter, we propose a new point of view of nonlinearity in semiconductors which is associated with the electron temperature dependence on the recombination rate. The heating of the charge carriers breaks the balance between generation and recombination, giving rise to nonequilibrium charge carriers concentration and nonlinearity. - Highlights: • A new mechanism of nonlinearity of current-voltage characteristic (CVC) is proposed. • The hot electron temperature violates the equilibrium between electrons and holes. • This violation gives rise to nonequilibrium concentration of electrons and holes. • This leads to nonlinear CVC (along with the heating nonlinearity).

  4. Nonlinear charge transport in bipolar semiconductors due to electron heating

    Energy Technology Data Exchange (ETDEWEB)

    Molina-Valdovinos, S., E-mail: sergiom@fisica.uaz.edu.mx [Universidad Autónoma de Zacatecas, Unidad Académica de Física, Calzada Solidaridad esq. Paseo, La Bufa s/n, CP 98060, Zacatecas, Zac, México (Mexico); Gurevich, Yu.G. [Centro de Investigación y de Estudios Avanzados del IPN, Departamento de Física, Av. IPN 2508, México D.F., CP 07360, México (Mexico)

    2016-05-27

    It is known that when strong electric field is applied to a semiconductor sample, the current voltage characteristic deviates from the linear response. In this letter, we propose a new point of view of nonlinearity in semiconductors which is associated with the electron temperature dependence on the recombination rate. The heating of the charge carriers breaks the balance between generation and recombination, giving rise to nonequilibrium charge carriers concentration and nonlinearity. - Highlights: • A new mechanism of nonlinearity of current-voltage characteristic (CVC) is proposed. • The hot electron temperature violates the equilibrium between electrons and holes. • This violation gives rise to nonequilibrium concentration of electrons and holes. • This leads to nonlinear CVC (along with the heating nonlinearity).

  5. Complex Role of Secondary Electron Emissions in Dust Grain Charging in Space Environments: Measurements on Apollo 11 and 17 Dust Grains

    Science.gov (United States)

    Abbas, M. M.; Tankosic, D.; Spann, J. F.; LeClair, A. C.

    2010-01-01

    Dust grains in various astrophysical environments are generally charged electrostatically by photoelectric emissions with radiation from nearby sources, or by electron/ion collisions by sticking or secondary electron emissions. Knowledge of the dust grain charges and equilibrium potentials is important for understanding of a variety of physical and dynamical processes in the interstellar medium (ISM), and heliospheric, interplanetary, planetary, and lunar environments. The high vacuum environment on the lunar surface leads to some unusual physical and dynamical phenomena involving dust grains with high adhesive characteristics, and levitation and transportation over long distances. It has been well recognized that the charging properties of individual micron/submicron size dust grains are expected to be substantially different from the corresponding values for bulk materials and theoretical models. In this paper we present experimental results on charging of individual dust grains selected from Apollo 11 and Apollo 17 dust samples by exposing them to mono-energetic electron beams in the 10- 400 eV energy range. The charging rates of positively and negatively charged particles of approximately 0.2 to 13 microns diameters are discussed in terms of the secondary electron emission (SEE) process, which is found to be a complex charging process at electron energies as low as 10-25 eV, with strong particle size dependence. The measurements indicate substantial differences between dust charging properties of individual small size dust grains and of bulk materials.

  6. Electron capture rates in stars studied with heavy ion charge exchange reactions

    Science.gov (United States)

    Bertulani, C. A.

    2018-01-01

    Indirect methods using nucleus-nucleus reactions at high energies (here, high energies mean ~ 50 MeV/nucleon and higher) are now routinely used to extract information of interest for nuclear astrophysics. This is of extreme relevance as many of the nuclei involved in stellar evolution are short-lived. Therefore, indirect methods became the focus of recent studies carried out in major nuclear physics facilities. Among such methods, heavy ion charge exchange is thought to be a useful tool to infer Gamow-Teller matrix elements needed to describe electron capture rates in stars and also double beta-decay experiments. In this short review, I provide a theoretical guidance based on a simple reaction model for charge exchange reactions.

  7. X-ray radiography with highly charged ions

    Science.gov (United States)

    Marrs, Roscoe E.

    2000-01-01

    An extremely small (1-250 micron FWHM) beam of slow highly charged ions deexciting on an x-ray production target generates x-ray monochromatic radiation that is passed through a specimen and detected for imaging. The resolution of the x-ray radiograms is improved and such detection is achieved with relatively low dosages of radiation passing through the specimen. An apparatus containing an electron beam ion trap (and modifications thereof) equipped with a focusing column serves as a source of ions that generate radiation projected onto an image detector. Electronic and other detectors are able to detect an increased amount of radiation per pixel than achieved by previous methods and apparati.

  8. Experiments with highly charged ions up to bare U92+ on the electron beam ion trap

    International Nuclear Information System (INIS)

    Beiersdorfer, P.

    1994-07-01

    An overview is given of the current experimental effort to investigate the level structure of highly charged ions with the Livermore electron beam ion trap (EBIT) facility. The facility allows the production and study of virtually any ionization state of any element up to bare U 92+ . Precision spectroscopic measurements have been performed for a range of Δn = 0 and Δn = 1 transitions. Examples involving 3-4 and 2-3 as well as 3-3 and 2-2 transitions in uranium ions are discussed that illustrated some of the measurement and analysis techniques employed. The measurements have allowed tests of calculations of the the quantum electrodynamical contributions to the transitions energies at the 0.4% level in a regime where (Zα) ∼ 1

  9. Decay characteristics of electronic charged states of Si quantum dots as evaluated by an AFM/Kelvin probe technique

    International Nuclear Information System (INIS)

    Nishitani, Junichiro; Makihara, Katsunori; Ikeda, Mitsuhisa; Murakami, Hideki; Higashi, Seiichiro; Miyazaki, Seiichi

    2006-01-01

    Si quantum dots (Si-QDs) with an areal dot density of 8 x 10 11 cm -2 on SiO 2 have been prepared by the thermal decomposition of monosilane to characterize charged states of Si-QDs using AFM/Kelvin probe force microscopy (KFM). The temporal changes in the surface potential induced by electron charging and discharging at Si-QDs covered with a ∼ 2-nm-thick oxide layer have been measured. In electron charging and discharging at Si-QDs, a Rh-coated AFM tip was electrically biased in the range of - 5 to 5 V and scanned on the sample surface in a tapping mode. The surface potential changes on Si-QDs by electron injection and extraction were observable, while no potential change was detected elsewhere. The surface potential of charged Si-QDs decays with time at rates depending on charge injection conditions. The observed decay characteristics can be interpreted in terms of discharging of stored electrons in Si-QDs due to electron tunneling through the bottom oxide to the substrate and neutralization of stored holes due to recombination with electrons tunneling from the substrates. The defect generation in oxide is likely to be responsible for a fairly slow decay as observed in the case of electron extraction by the tip bias as high as + 4.8 V with respect to p-Si(100)

  10. A Combined Model of Charging of the Surface and Bulk of a Dielectric Target by Electrons with the Energies 10-30 keV

    Science.gov (United States)

    Zykov, V. M.; Neiman, D. A.

    2018-04-01

    A physico-mathematical model of the processes of radiation-induced charging of dielectric materials with open surfaces, irradiated with monoenergetic electrons in the energy range 10-30 keV, is described. The model takes into account the relationship between the processes of surface and bulk charging for the given conditions of the experimental design, which accounts for the effect of anomalously long charging of dielectrics after the incident energy of primary electrons during charging is reduced to below the second critical energy for the secondary electronic emission coefficient. The initial fast phase of charging a high-resistivity dielectric material (Al2O3) is investigated. It is shown that as the incident electron energy is approaching the second critical energy during charging, the secondary electronic emission is partially suppressed due to negative charging of the open surface of the dielectric and formation of a near-surface inversion electrical field retarding the electronic emission yield.

  11. Few-layered Ni(OH)2 nanosheets for high-performance supercapacitors

    Science.gov (United States)

    Sun, Wenping; Rui, Xianhong; Ulaganathan, Mani; Madhavi, Srinivasan; Yan, Qingyu

    2015-11-01

    Few-layered Ni(OH)2 nanosheets (4-5 nm in thickness) are synthesized towards high-performance supercapacitors. The ultrathin Ni(OH)2 nanosheets show high specific capacitance and good rate capability in both three-electrode and asymmetric devices. In the three-electrode device, the Ni(OH)2 nanosheets deliver a high capacitance of 2064 F g-1 at 2 A g-1, and the capacitance still has a retention of 1837 F g-1 at a high current density of 20 A g-1. Such excellent performance is by far one of the best for Ni(OH)2 electrodes. In the two-electrode asymmetric device, the specific capacitance is 248 F g-1 at 1 A g-1, and reaches 113 F g-1 at 20 A g-1. The capacitance of the asymmetric device maintains to be 166 F g-1 during the 4000th cycle at 2 A g-1, suggesting good cycling stability of the device. Besides, the asymmetric device exhibits gravimetric energy density of 22 Wh kg-1 at a power density of 0.8 kW kg-1. The present results demonstrate that the ultrathin Ni(OH)2 nanosheets are highly attractive electrode materials for achieving fast charging/discharging and high-capacity supercapacitors.

  12. The physics of highly charged heavy ions revealed by storage/cooler rings

    International Nuclear Information System (INIS)

    Mokler, P.H.; Stoehlker, T.

    1996-01-01

    With the successful commissioning of storage and cooler rings for bright beams of very heavy ions near the threshold of the last decade of this century, not only did a prosperous development in heavy ion accelerator technology come to its present summit, but also fundamental fields in heavy ion physics were opened widely for exciting explorations. Now, essential aspects in this area are accessible, aspects one only dared to dream of another decade ago. In the meantime, great progress already has been made in the fundamental physics in this field. This is particularly true for achievements in the atomic physics of highly charged heavy ions. In this chapter, we present a review of the current advances in this rapidly developing field. There are two general domains to be considered in the atomic physics of highly charged heavy ions: the fields of collisions and of atomic structure. Both aspects have to be explored equally, as they are strongly interconnected. One has to investigate the interaction processes to know, for instance, the population of excited states to help answer questions on the atomic structure; and conversely, one has to know the structure to understand the interactions. In both the fields, fundamental principles can be studied uniquely. This is in particular true for the heaviest ion species with only a few- or even zero-electrons left. 140 refs., 39 figs

  13. Production of highly charged heavy ions by 18 GHz superconducting electron cyclotron resonance at Research Center for Nuclear Physics.

    Science.gov (United States)

    Yorita, Tetsuhiko; Hatanaka, Kichiji; Fukuda, Mitsuhiro; Kibayashi, Mitsuru; Morinobu, Shunpei; Okamura, Hiroyuki; Tamii, Atsushi

    2010-02-01

    An 18 GHz superconducting electron cyclotron resonance ion source has been installed as a subject of the azimuthally varying field cyclotron upgrade project (K. Hatanaka et al., in Proceedings of the 17th International Conference on Cyclotrons and Their Applications, Tokyo, Japan, 18-22 October 2004, pp. 115-117), in order to increase beam currents and to extend the variety of ions. The production development of several ions has been performed since 2006 and some of them have already been used for user experiments [T. Yorita et al., Rev. Sci. Instrum. 79, 02A311 (2008)]. Further optimizations for each component such as the material of plasma electrode, material, and shape of bias probe and mirror field have been continued and more intense ion beams have been obtained for O, N, and Ar. For the purpose of obtaining highly charged Xe with several microamperes, the optimization of position and shape of plasma electrode and bias disk has also been done and highly charged Xe(32+) beam has been obtained successfully.

  14. Charge Modulation in Graphitic Carbon Nitride as a Switchable Approach to High-Capacity Hydrogen Storage.

    Science.gov (United States)

    Tan, Xin; Kou, Liangzhi; Tahini, Hassan A; Smith, Sean C

    2015-11-01

    Electrical charging of graphitic carbon nitride nanosheets (g-C4 N3 and g-C3 N4 ) is proposed as a strategy for high-capacity and electrocatalytically switchable hydrogen storage. Using first-principle calculations, we found that the adsorption energy of H2 molecules on graphitic carbon nitride nanosheets is dramatically enhanced by injecting extra electrons into the adsorbent. At full hydrogen coverage, the negatively charged graphitic carbon nitride achieves storage capacities up to 6-7 wt %. In contrast to other hydrogen storage approaches, the storage/release occurs spontaneously once extra electrons are introduced or removed, and these processes can be simply controlled by switching on/off the charging voltage. Therefore, this approach promises both facile reversibility and tunable kinetics without the need of specific catalysts. Importantly, g-C4 N3 has good electrical conductivity and high electron mobility, which can be a very good candidate for electron injection/release. These predictions may prove to be instrumental in searching for a new class of high-capacity hydrogen storage materials. © 2015 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  15. Improvement of highly charged ion production in the ECR source of heavy ions

    International Nuclear Information System (INIS)

    Shirkov, G.D.

    1996-01-01

    Some physical limitations of the highly charged ion production in the ECR source are analyzed in this report. A few possible ways to improve the output of highly charged ions from the ECR source for heavy ions are proposed. A new library of computer codes for the numerical simulation of heavy ion production in the ECR ion source is used to examine these ways to improve the ECR source operation according to the CERN program of heavy ion acceleration. copyright 1996 American Institute of Physics

  16. The interactions of high-energy, highly-charged ions with fullerenes

    International Nuclear Information System (INIS)

    Ali, R.; Berry, H.G.; Cheng, S.

    1996-01-01

    In 1985, Robert Curl and Richard Smalley discovered a new form of carbon, the fullerene, C 60 , which consists of 60 carbon atoms in a closed cage resembling a soccer ball. In 1990, Kritschmer et al. were able to make macroscopic quantities of fullerenes. This has generated intense activity to study the properties of fullerenes. One area of research involves collisions between fullerenes and atoms, ions or electrons. In this paper we describe experiments involving interactions between fullerenes and highly charged ions in which the center-of-mass energies exceed those used in other work by several orders of magnitude. The high values of projectile velocity and charge state result in excitation and decay processes differing significantly from those seen in studies 3 at lower energies. Our results are discussed in terms of theoretical models analogous to those used in nuclear physics and this provides an interesting demonstration of the unity of physics

  17. EBIT spectroscopy of highly charged heavy ions relevant to hot plasmas

    Science.gov (United States)

    Nakamura, Nobuyuki

    2013-05-01

    An electron beam ion trap (EBIT) is a versatile device for studying highly charged ions. We have been using two types of EBITs for the spectroscopic studies of highly charged ions. One is a high-energy device called the Tokyo-EBIT, and another is a compact low-energy device called CoBIT. Complementary use of them enables us to obtain spectroscopic data for ions over a wide charge-state range interacting with electrons over a wide energy range. In this talk, we present EBIT spectra of highly charged ions for tungsten, iron, bismuth, etc., which are relevant to hot plasmas. Tungsten is considered to be the main impurity in the ITER (the next generation nuclear fusion reactor) plasma, and thus its emission lines are important for diagnosing and controlling the ITER plasma. We have observed many previously unreported lines to supply the lack of spectroscopic data of tungsten ions. Iron is one of the main components of the solar corona, and its spectra are used to diagnose temperature, density, etc. The diagnostics is usually done by comparing observed spectra with model calculations. An EBIT can provide spectra under a well-defined condition; they are thus useful to test the model calculations. Laser-produced bismuth plasma is one of the candidates for a soft x-ray source in the water window region. An EBIT has a narrow charge state distribution; it is thus useful to disentangle the spectra of laser-produced plasma containing ions with a wide charge-state range. Performed with the support and under the auspices of the NIFS Collaboration Research program (NIFS09KOAJ003) and JSPS KAKENHI Number 23246165, and partly supported by the JSPS-NRF-NSFC A3 Foresight Program in the field of Plasma Physics.

  18. Aspects of space charge theory applied to dielectric under electron beam irradiation

    International Nuclear Information System (INIS)

    Oliveira, L.N. de.

    1975-01-01

    Irradiation of solid dielectric with electron beams has been used as a power full tool in investigations of charge storage and transport in such materials. Some of the results that have been obtained in this area are reviewed and the formulation of a transport equation for excess charge in irradiated insulators is dicussed. This equation is subsequently applied to various experimental set-ups. It is found that space charge effects play an essential role in the establishment of stationary currents in samples subject to quasi-penetrating electron beams. Such effects may, however, be neglected for low electron ranges. Theoretical results are in good agreement with experimental findings by Spear (1955)

  19. Fragment-orbital tunneling currents and electronic couplings for analysis of molecular charge-transfer systems.

    Science.gov (United States)

    Hwang, Sang-Yeon; Kim, Jaewook; Kim, Woo Youn

    2018-04-04

    In theoretical charge-transfer research, calculation of the electronic coupling element is crucial for examining the degree of the electronic donor-acceptor interaction. The tunneling current (TC), representing the magnitudes and directions of electron flow, provides a way of evaluating electronic couplings, along with the ability of visualizing how electrons flow in systems. Here, we applied the TC theory to π-conjugated organic dimer systems, in the form of our fragment-orbital tunneling current (FOTC) method, which uses the frontier molecular-orbitals of system fragments as diabatic states. For a comprehensive test of FOTC, we assessed how reasonable the computed electronic couplings and the corresponding TC densities are for the hole- and electron-transfer databases HAB11 and HAB7. FOTC gave 12.5% mean relative unsigned error with regard to the high-level ab initio reference. The shown performance is comparable with that of fragment-orbital density functional theory, which gave the same error by 20.6% or 13.9% depending on the formulation. In the test of a set of nucleobase π stacks, we showed that the original TC expression is also applicable to nondegenerate cases under the condition that the overlap between the charge distributions of diabatic states is small enough to offset the energy difference. Lastly, we carried out visual analysis on the FOTC densities of thiophene dimers with different intermolecular alignments. The result depicts an intimate topological connection between the system geometry and electron flow. Our work provides quantitative and qualitative grounds for FOTC, showing it to be a versatile tool in characterization of molecular charge-transfer systems.

  20. Resonance charge exchange mechanism at high and moderate energies

    International Nuclear Information System (INIS)

    Bogdanov, A.V.; Gevorkyan, A.S.

    1984-01-01

    Charge exchange mechanisms at high and medium energies are investigated, ta king the resonance charge exchange of a proton by an hydrogen atom as an example . It is established that there are two classical charge exchange mechanisms rel ated to direct proton knockout from the bound state and one quantum-mechanical mechanism corresponding to the electron tunnelling from one bound state to anoth er. The classical cross-section diverges for two of these mechanisms, and the quasiclassical scattering amplitude must be calculated on the base of a complex classical trajectory. Physical grounds for the choice of such trajectories are discussed and calculations of the Van Vleck determinant for these mechanisms a re presented. Contributions from different mechanisms to the total charge excha nge cross-section are analyzed. A comparison with experimental data and results of other authors is made

  1. On the nature of high field charge transport in reinforced silicone dielectrics: Experiment and simulation

    Energy Technology Data Exchange (ETDEWEB)

    Huang, Yanhui, E-mail: huangy12@rpi.edu; Schadler, Linda S. [Department of Material Science and Engineering, Rensselaer Polytechnic Institute, 110 8th street, Troy, New York 12180 (United States)

    2016-08-07

    The high field charge injection and transport properties in reinforced silicone dielectrics were investigated by measuring the time-dependent space charge distribution and the current under dc conditions up to the breakdown field and were compared with the properties of other dielectric polymers. It is argued that the energy and spatial distribution of localized electronic states are crucial in determining these properties for polymer dielectrics. Tunneling to localized states likely dominates the charge injection process. A transient transport regime arises due to the relaxation of charge carriers into deep traps at the energy band tails and is successfully verified by a Monte Carlo simulation using the multiple-hopping model. The charge carrier mobility is found to be highly heterogeneous due to the non-uniform trapping. The slow moving electron packet exhibits a negative field dependent drift velocity possibly due to the spatial disorder of traps.

  2. Proposed LLNL electron beam ion trap

    International Nuclear Information System (INIS)

    Marrs, R.E.; Egan, P.O.; Proctor, I.; Levine, M.A.; Hansen, L.; Kajiyama, Y.; Wolgast, R.

    1985-01-01

    The interaction of energetic electrons with highly charged ions is of great importance to several research fields such as astrophysics, laser fusion and magnetic fusion. In spite of this importance there are almost no measurements of electron interaction cross sections for ions more than a few times ionized. To address this problem an electron beam ion trap (EBIT) is being developed at LLNL. The device is essentially an EBIS except that it is not intended as a source of extracted ions. Instead the (variable energy) electron beam interacting with the confined ions will be used to obtain measurements of ionization cross sections, dielectronic recombination cross sections, radiative recombination cross sections, energy levels and oscillator strengths. Charge-exchange recombinaion cross sections with neutral gasses could also be measured. The goal is to produce and study elements in many different charge states up to He-like xenon and Ne-like uranium. 5 refs., 2 figs

  3. Generation of Low-Energy High-Current Electron Beams in Plasma-Anode Electron Guns

    Science.gov (United States)

    Ozur, G. E.; Proskurovsky, D. I.

    2018-01-01

    This paper is a review of studies on the generation of low-energy high-current electron beams in electron guns with a plasma anode and an explosive-emission cathode. The problems related to the initiation of explosive electron emission under plasma and the formation and transport of high-current electron beams in plasma-filled systems are discussed consecutively. Considerable attention is given to the nonstationary effects that occur in the space charge layers of plasma. Emphasis is also placed on the problem of providing a uniform energy density distribution over the beam cross section, which is of critical importance in using electron beams of this type for surface treatment of materials. Examples of facilities based on low-energy high-current electron beam sources are presented and their applications in materials science and practice are discussed.

  4. Performance of the PHIN High Charge Photo Injector

    CERN Document Server

    Petrarca, M; Doebert, S; Dabrowski, A; Divall, M; Fedoseev, V; Lebas, N; Lefevre, T; Losito, R; Egger, D; Mete, O

    2010-01-01

    The high charge PHIN photo injector is studied at CERN as an electron source for the CLIC Test Facility (CTF3) drive beam as an alternative to the present thermionic gun. The objective of PHIN is to demonstrate the feasibility of a laser-based electron source for CLIC. The photo injector operates with a 2.5 cell, 3 GHz RF gun using a Cs2Te photocathode illuminated by UV laser pulses generated by amplifying and frequency quadrupling the signal from a Nd:YLF oscillator running at 1.5GHz. The challenge is to generate a beam structure of 1908 micro bunches with 2.33nC per micro bunch at 1.5GHz leading to a high integrated train charge of 4446nC and nominal beam energy of 5.5MeV with current stability below 1%. In this paper we report and discuss the time resolved transverse and longitudinal beam parameters measurements. The performance of the photo cathodes made at CERN with a peak quantum efficiency of 18 % is shown as well. Laser pointing and amplitude stability results are discussed taking into account correla...

  5. Few femtosecond, few kilo-ampere electron bunch produced by a laser-plasma accelerator

    International Nuclear Information System (INIS)

    Lundh, O.; Lim, J.; Rechatin, C.; Ammoura, L.; Goddet, J.P.; Malka, V.; Faure, J.; Ben-Ismail, A.; Davoine, X.; Lefebvre, E.; Gallot, G.

    2011-01-01

    Particle accelerators driven by the interaction of ultra-intense and ultrashort laser pulses with a plasma can generate accelerating electric fields of several hundred giga-volts per meter and deliver high-quality electron beams with low energy spread, low emittance and up to 1 GeV peak energy. Moreover, it is expected they may soon be able to produce bursts of electrons shorter than those produced by conventional particle accelerators, down to femtosecond durations and less. Here we present wide-band spectral measurements of coherent transition radiation which we use for temporal characterization. Our analysis shows that the electron beam, produced using controlled optical injection, contains a temporal feature that can be identified as a 15 pC, 1.4-1.8 fs electron bunch (root mean square) leading to a peak current of 3-4 kA depending on the bunch shape. We anticipate that these results will have a strong impact on emerging applications such as short-pulse and short-wavelength radiation sources, and will benefit the realization of laboratory-scale free-electron lasers. (authors)

  6. Electron emission following collisions between multi-charged ions and D2 molecules

    International Nuclear Information System (INIS)

    Laurent, G.

    2004-05-01

    Dissociative ionisation mechanisms induced in collisions involving a highly charged ion (S 15+ , 13.6 MeV/u) and a molecular deuterium target, have been studied through momentum vector correlations of both the D + fragments and the electrons produced. An experimental apparatus has been developed in order to detect in coincidence all the charged particles produced during the collision. The measurement of their momentum vectors, which allows one to determine both their kinetic energy and direction of emission with respect to the projectile one, combines Time of Flight, Position Sensitive Detection, and multi-coincidence techniques. The correlation of the fragment and electron kinetic energies enables not only to determine branching ratios between the dissociative ionisation pathways, but also to separate unambiguously kinetic energy distributions of fragments associated to each process. Finally, the angular distributions of ejected electrons, as a function of the orientation of the molecular axis with respect to the projectile direction, are deduced from the spatial correlation. Measurements are compared to theoretical angular distributions obtained using the CDW-EIS (Continuum Distorted Wave-Eikonal Initial State) method. (author)

  7. Development of Discrete Power Supply with Charge Pump Method for High Powered Sonar System

    Directory of Open Access Journals (Sweden)

    Kristian Ismail

    2012-07-01

    Full Text Available Power supply is one of the electronic devices that can provide electric energy for electronic systems or other systems. There are several types of power supplies that can be applied depend on the requirement and functions. One example is the use of power supply for sonar systems. Sonar system is a device which can be used to detect a target under water. The sonar system is an electronic circuit that requires a power supply with specific characteristics when the sonar functions as a transmitter and a receiver in the specific span time (when on and the specific lag time (when off. This paper discusses the design of power supply for high-powered sonar systems with discrete methods in which high power supply is only applied when the acoustic waves radiated under water. Charge pump was used to get the appropriate output voltage from lower input voltage. Charge pump utilized a combination of series and parallel connections of capacitors. The working mode of this power supply used the lag time as the calculation of time to charge charge pump capacitors in parallel while the span time was used for the calculation of discharging the charge pump capacitors in series.

  8. Positronium Inhibition and Quenching by Organic Electron Acceptors and Charge Transfer Complexes

    DEFF Research Database (Denmark)

    Jansen, P.; Eldrup, Morten Mostgaard; Jensen, Bror Skytte

    1975-01-01

    Positron lifetime measurements were performed on a series of organic electron acceptors and charge-transfer complexes in solution. The acceptors cause both positronium (Ps) inhibition (with maybe one exception) and quenching, but when an acceptor takes part in a charge-transfer complex...... in terms of the spur reaction model of Ps formation. Correlation was also made to gas phase reaction between electron acceptors and free electron, as well as to pulse radiolysis data....

  9. Charging suppression in focused-ion beam fabrication of visible subwavelength dielectric grating reflector using electron conducting polymer

    KAUST Repository

    Alias, Mohd Sharizal; Liao, Hsien-Yu; Ng, Tien Khee; Ooi, Boon S.

    2015-01-01

    Nanoscale periodic patterning on insulating materials using focused-ion beam (FIB) is challenging because of charging effect, which causes pattern distortion and resolution degradation. In this paper, the authors used a charging suppression scheme using electron conducting polymer for the implementation of FIB patterned dielectric subwavelength grating (SWG) reflector. Prior to the FIB patterning, the authors numerically designed the optimal structure and the fabrication tolerance for all grating parameters (period, grating thickness, fill-factor, and low refractive index layer thickness) using the rigorous-coupled wave analysis computation. Then, the authors performed the FIB patterning on the dielectric SWG reflector spin-coated with electron conducting polymer for the anticharging purpose. They also performed similar patterning using thin conductive film anticharging scheme (30 nm Cr coating) for comparison. Their results show that the electron conducting polymer anticharging scheme effectively suppressing the charging effect during the FIB patterning of dielectric SWG reflector. The fabricated grating exhibited nanoscale precision, high uniformity and contrast, constant patterning, and complied with fabrication tolerance for all grating parameters across the entire patterned area. Utilization of electron conducting polymer leads to a simpler anticharging scheme with high precision and uniformity for FIB patterning on insulator materials.

  10. Charging suppression in focused-ion beam fabrication of visible subwavelength dielectric grating reflector using electron conducting polymer

    KAUST Repository

    Alias, Mohd Sharizal

    2015-08-19

    Nanoscale periodic patterning on insulating materials using focused-ion beam (FIB) is challenging because of charging effect, which causes pattern distortion and resolution degradation. In this paper, the authors used a charging suppression scheme using electron conducting polymer for the implementation of FIB patterned dielectric subwavelength grating (SWG) reflector. Prior to the FIB patterning, the authors numerically designed the optimal structure and the fabrication tolerance for all grating parameters (period, grating thickness, fill-factor, and low refractive index layer thickness) using the rigorous-coupled wave analysis computation. Then, the authors performed the FIB patterning on the dielectric SWG reflector spin-coated with electron conducting polymer for the anticharging purpose. They also performed similar patterning using thin conductive film anticharging scheme (30 nm Cr coating) for comparison. Their results show that the electron conducting polymer anticharging scheme effectively suppressing the charging effect during the FIB patterning of dielectric SWG reflector. The fabricated grating exhibited nanoscale precision, high uniformity and contrast, constant patterning, and complied with fabrication tolerance for all grating parameters across the entire patterned area. Utilization of electron conducting polymer leads to a simpler anticharging scheme with high precision and uniformity for FIB patterning on insulator materials.

  11. Internal Charging

    Science.gov (United States)

    Minow, Joseph I.

    2014-01-01

    (1) High energy (>100keV) electrons penetrate spacecraft walls and accumulate in dielectrics or isolated conductors; (2) Threat environment is energetic electrons with sufficient flux to charge circuit boards, cable insulation, and ungrounded metal faster than charge can dissipate; (3) Accumulating charge density generates electric fields in excess of material breakdown strenght resulting in electrostatic discharge; and (4) System impact is material damage, discharge currents inside of spacecraft Faraday cage on or near critical circuitry, and RF noise.

  12. Study of the Effects of the Electric Field on Charging Measurements on Individual Micron-size Dust Grains by Secondary Electron Emissions

    Science.gov (United States)

    Tankosic, D.; Abbas, M. M.

    2013-01-01

    The dust charging by electron impact is an important dust charging process in Astrophysical, Planetary, and the Lunar environments. Low energy electrons are reflected or stick to the grains charging the dust grains negatively. At sufficiently high energies electrons penetrate the grain leading to excitation and emission of electrons referred to as secondary electron emission (SEE). Available theoretical models for the calculation of SEE yield applicable for neutral, planar or bulk surfaces are generally based on Sternglass Equation. However, viable models for charging of individual dust grains do not exist at the present time. Therefore, the SEE yields have to be obtained by some experimental methods at the present time. We have conducted experimental studies on charging of individual micron size dust grains in simulated space environments using an electrodynamic balance (EDB) facility at NASA-MSFC. The results of our extensive laboratory study of charging of individual micron-size dust grains by low energy electron impact indicate that the SEE by electron impact is a very complex process expected to be substantially different from the bulk materials. It was found that the incident electrons may lead to positive or negative charging of dust grains depending upon the grain size, surface potential, electron energy, electron flux, grain composition, and configuration. In this paper we give a more elaborate discussion about the possible effects of the AC field in the EDB on dust charging measurements by comparing the secondary electron emission time-period (tau (sub em) (s/e)) with the time-period (tau (sub ac) (ms)) of the AC field cycle in the EDB that we have briefly addressed in our previous publication.

  13. Colliding beam studies of electron detachement from H- by multiply-charged ions

    International Nuclear Information System (INIS)

    Melchert, F.; Benner, M.; Kruedener, S.; Schulze, R.; Meuser, S.; Pfaff, S.; Petri, S.; Huber, K.; Salzborn, E.; Presnyakov, L.P.; Uskov, D.B.

    1993-01-01

    Employing the crossed-beams technique, we have investigated electron-detachment processes from H - in collisions with multiply-charged noble gas ions A q+ . Absolute cross sections for single- and double-electron removal have been measured at center-of-mass energies from 50 keV to 200 keV and charge states q up to 8

  14. Electron spectroscopy with fast heavy ions

    International Nuclear Information System (INIS)

    Schneider, D.

    1983-01-01

    Since about 1970 the spectroscopy of Auger-electrons and characteristic x-rays following energetic ion-atom collisions has received a great deal of attention. An increasing number of accelerators, capable of providing a large number of projectile ion species over a wide range of projectile energies, became available for studying ion-atom collision phenomena. Many charged particles from protons up to heavy ions like uranium can be accelerated to energies ranging over six orders of magnitude. This allows us to study systematically a great variety of effects accompanied by dynamic excitation processes of the atomic shells in either the projectile- or target-atoms. The studies yield fundamental information regarding the excitation mechanism (e.g., Coulomb and quasi-molecular excitation) and allow sensitive tests of atomic structure theories. This information in turn is valuable to other fields in physics like plasma-, astro-, or solid-state (surface) physics. It is a characteristic feature of fast heavy-ion accelerators that they can produce highly stripped ion species which have in turn the capability to highly ionize neutral target atoms or molecules in a single collision. The ionization process, mainly due to the strong electrical fields that are involved, allows us to study few-electron atoms with high atomic numbers Z. High resolution spectroscopy performed with these atoms allows a particularly good test of relativistic and QED effects. The probability of producing these few electron systems is determined by the charge state and the velocity of the projectile ions. In this contribution the possibilities of using electron spectroscopy as a tool to investigate fast ion-atom collisions is discussed and demonstrated with a few examples. 30 references

  15. High Intensity High Charge State ECR Ion Sources

    CERN Document Server

    Leitner, Daniela

    2005-01-01

    The next-generation heavy ion beam accelerators such as the proposed Rare Isotope Accelerator (RIA), the Radioactive Ion Beam Factory at RIKEN, the GSI upgrade project, the LHC-upgrade, and IMP in Lanzhou require a great variety of high charge state ion beams with a magnitude higher beam intensity than currently achievable. High performance Electron Cyclotron Resonance (ECR) ion sources can provide the flexibility since they can routinely produce beams from hydrogen to uranium. Over the last three decades, ECR ion sources have continued improving the available ion beam intensities by increasing the magnetic fields and ECR heating frequencies to enhance the confinement and the plasma density. With advances in superconducting magnet technology, a new generation of high field superconducting sources is now emerging, designed to meet the requirements of these next generation accelerator projects. The talk will briefly review the field of high performance ECR ion sources and the latest developments for high intens...

  16. Photonics at the frontiers. Generation of few-cycle light pulses via NOPCPA and real-time probing of charge transfer in hybrid photovoltaics

    Energy Technology Data Exchange (ETDEWEB)

    Herrmann, Daniel

    2011-11-11

    In the first part of this thesis the methodics of the non-collinear, optically parametric amplification of chirped light pulses (NOPCPA) for the generation of few-cycle light pulses in the visible (Vis) and near infrared (NIR) with of 5-8 fs half-width are essential further developed. Fundamental parametric influences, like the existence of a parametrically induced phase and the generation of optically parametric fluorescence (OPF), are studied both by theoretical analyses and numerical simulations and by concrete experiments. Experimentally in the framework of this thesis fwe-cycle light pulses with a pulse width of 7.9 fs, 130 mJ energy, at 805 nm central wavelength and a very high seed-pulse-limited prepulse contrast of 11 and 8 orders of magnitude are reached at 30 ps and approximately 3 ps. One the one hand it has been succeeded to accelerate with the broad-band pulse amplifier quasi-monoenergetic electrons with energies of up to 50 MeV. For this the light pulse is focussed to relativistic intensities of several W/cm{sup 2} in a helium gas jet. On the other hand XUV light was produced up to the 20th harmonic of the generated light pulse from the broad-band pulse amplifier by its sub-cycle interaction with solid surfaces. In the framework of this thesis furthermore new, extended concepts for still broader-band NOPCPA over one octave were developed and characterized, which contain the application of two pump pulses in one NOPCPA stage and the application of two different pump wavelength in two subsequent NOPCPA stages. In the second part of this thesis broad-band white-light spectra and by means of NOPCPA spectrally tunable light pulses are applied in order to realize a transient absorption spectrometer with multichannel detection. This new excitation-query construction combines a very broad-band UV-Vis-NIR query with a high time resolution of 40 fs and high sensitivity for the transient change of the optical density of less than 10{sup -4}. By this it has in

  17. Calculating method for confinement time and charge distribution of ions in electron cyclotron resonance sources

    International Nuclear Information System (INIS)

    Dougar-Jabon, V.D.; Umnov, A.M.; Kutner, V.B.

    1996-01-01

    It is common knowledge that the electrostatic pit in a core plasma of electron cyclotron resonance sources exerts strict control over generation of ions in high charge states. This work is aimed at finding a dependence of the lifetime of ions on their charge states in the core region and to elaborate a numerical model of ion charge dispersion not only for the core plasmas but for extracted beams as well. The calculated data are in good agreement with the experimental results on charge distributions and magnitudes for currents of beams extracted from the 14 GHz DECRIS source. copyright 1996 American Institute of Physics

  18. Charge-coupled device area detector for low energy electrons

    Czech Academy of Sciences Publication Activity Database

    Horáček, Miroslav

    2003-01-01

    Roč. 74, č. 7 (2003), s. 3379 - 3384 ISSN 0034-6748 R&D Projects: GA ČR GA102/00/P001 Institutional research plan: CEZ:AV0Z2065902 Keywords : low energy electrons * charged-coupled device * detector Subject RIV: JA - Electronics ; Optoelectronics, Electrical Engineering Impact factor: 1.343, year: 2003

  19. Electron correlation in highly-charged-ion collisions

    International Nuclear Information System (INIS)

    Hansen, J.P.; Taulbjerg, K.

    1992-01-01

    We have used the coupled-channel method to study the significance of electron correlation in the reaction mechanism for two-electron capture in C 5+ -He collisions. Two different sets of calculations were performed. While the static correlation energy was generally included in the calculations, further correlation effects were ignored in the first set of calculations. In the second set of calculations the so-called doubly excited symmetry basis (DESB) states were used to model the spatial electron correlation. The difference between the two sets of results is so profound that we can conclude that electron correlation plays an essential role in the reaction mechanism. The results of the DESB-based calculations are in good agreement with experimental data [Holt et al., Phys. Rev. A 43, 607 (1991)

  20. Long-Lived Charge Separation at Heterojunctions between Semiconducting Single-Walled Carbon Nanotubes and Perylene Diimide Electron Acceptors

    Energy Technology Data Exchange (ETDEWEB)

    Kang, Hyun Suk [National Renewable Energy Laboratory (NREL), Golden, CO (United States); Arias, Dylan H [National Renewable Energy Laboratory (NREL), Golden, CO (United States); Blackburn, Jeffrey L [National Renewable Energy Laboratory (NREL), Golden, CO (United States); Sisto, Thomas J. [Columbia University; Peurifoy, Samuel [Columbia University; Zhang, Boyuan [Columbia University; Nuckolls, Colin [Columbia University

    2018-04-13

    Nonfullerene electron acceptors have facilitated a recent surge in the efficiencies of organic solar cells, although fundamental studies of the nature of exciton dissociation at interfaces with nonfullerene electron acceptors are still relatively sparse. Semiconducting single-walled carbon nanotubes (s-SWCNTs), unique one-dimensional electron donors with molecule-like absorption and highly mobile charges, provide a model system for studying interfacial exciton dissociation. Here, we investigate excited-state photodynamics at the heterojunction between (6,5) s-SWCNTs and two perylene diimide (PDI)-based electron acceptors. Each of the PDI-based acceptors, hPDI2-pyr-hPDI2 and Trip-hPDI2, is deposited onto (6,5) s-SWCNT films to form a heterojunction bilayer. Transient absorption measurements demonstrate that photoinduced hole/electron transfer occurs at the photoexcited bilayer interfaces, producing long-lived separated charges with lifetimes exceeding 1.0 us. Both exciton dissociation and charge recombination occur more slowly for the hPDI2-pyr-hPDI2 bilayer than for the Trip-hPDI2 bilayer. To explain such differences, we discuss the potential roles of the thermodynamic charge transfer driving force available at each interface and the different molecular structure and intermolecular interactions of PDI-based acceptors. Detailed photophysical analysis of these model systems can develop the fundamental understanding of exciton dissociation between organic electron donors and nonfullerene acceptors, which has not been systematically studied.

  1. Solvation of excess electrons trapped in charge pockets on molecular surfaces

    Science.gov (United States)

    Jalbout, Abraham F.

    This work considers the ability of hydrogen fluoride (HF) to solvate excess electrons located on cyclic hydrocarbon surfaces. The principle applied involves the formation of systems in which excess electrons can be stabilized not only on concentrated molecular surface charge pockets but also by HF. Recent studies have shown that OH groups can form stable hydrogen-bonded networks on one side of a hydrocarbon surface (i.e. cyclohexane sheets), at the same time, the hydrogen atoms on the opposite side of this surface form a pocket of positive charge can attract the excess electron. This density can be further stabilized by the addition of an HF molecule that can form an 'anion with an internally solvated electron' (AISE) state. These systems are shown to be stable with respect to vertical electron detachment (VDE).

  2. Development of high-current-density LAB6 thermionic emitters for a space-charge-limited electron gun

    International Nuclear Information System (INIS)

    Herniter, M.E.; Getty, W.D.

    1987-01-01

    An electron gun has been developed for investigation of high current density, space charge limited operation of a lenthanum hexaboride (LaB 6 ) thermionic cathode. The 2.8 cm 2 cathode disk is heated by electron bombardment from a tungsten filament. For LaB 6 cathode temperatures greater than 1600 0 C it has been found that evaporation from the LaB 6 causes an increase in the tungsten filament emission, leading to an instability in the bombardment heating system. This instability has been investigated and eliminated by using a graphite disk in place of the LaB 6 cathode or by shielding the filament from the LaB 6 cathode by placing the LaB 6 in a graphite cup and bombarding the cup. The graphite disk has been heated to 1755 0 C with 755 W of heating power, and the shielded LaB 6 cathode has been heated to 1695 0 C. This temperature range is required for emission current densities in the 30 Acm 2 range. It is believed that the evaporation of lanthanum lowers the tungsten work function. In electron-gun use, the LaB 6 cathode has been operated up to 6.7 Acm 2 at 36 kV. A 120 kV Marx generator has been built to allow operation up to 40 Acm 2

  3. Polarization of electron-beam irradiated LDPE films: contribution to charge generation and transport

    Science.gov (United States)

    Banda, M. E.; Griseri, V.; Teyssèdre, G.; Le Roy, S.

    2018-04-01

    Electron-beam irradiation is an alternative way to generate charges in insulating materials, at controlled position and quantity, in order to monitor their behaviour in regard to transport phenomena under the space charge induced electric field or external field applied. In this study, low density polyethylene (LDPE) films were irradiated by a 80 keV electron-beam with a flux of 1 nA cm‑2 during 10 min in an irradiation chamber under vacuum conditions, and were then characterized outside the chamber using three experimental methods. The electrical behaviour of the irradiated material was assessed by space charge measurements using the pulsed electro-acoustic (PEA) method under dc stress. The influence of the applied electric field polarity and amplitude has been tested in order to better understand the charge behaviour after electron-beam irradiation. Fourier transform infra-red spectroscopy (FTIR) and photoluminescence (PL) measurements were performed to evaluate the impact of the electron beam irradiation, i.e. deposited charges and energy, on the chemical structure of the irradiated samples. The present results show that the electrical behaviour in LDPE after irradiation is mostly driven by charges, i.e. by physical process functions of the electric field, and that changes in the chemical structure seems to be mild.

  4. Quantum electrodynamical effects in heavy highly-charged ions

    International Nuclear Information System (INIS)

    Yerokhin, V.A.; Artemyev, A.N.; Indelicato, P.; Shabaev, V.M.

    2003-01-01

    The present status of theoretical calculations of QED effects in highly charged ions is reviewed for several important cases: the Lamb shift in heavy H-like ions, the 2p 1/2 -2s transition energy in heavy Li-like ions, and the bound-electron g factor in H-like ions. Theoretical predictions are compared with experimental results. Special attention is paid to the discussion of uncertainties of theoretical predictions

  5. Space-charge effects on bunching of electrons in the CEBAF injector

    International Nuclear Information System (INIS)

    Liu, H.

    1997-01-01

    The main injector for the 4 GeV CEBAF accelerator at Thomas Jefferson national accelerator facility was designed to deliver simultaneously three CW electron beams for nuclear physics research. The maximum design current for a single beam from the injector is 100 μA, or 0.2 pC per microbunch at a repetition rate of 499 MHz. It was found through computer simulation that space charge even at a subpicocoulomb level can spoil the bunching of electrons significantly, and some unexpected phenomena observed experimentally could be explained accordingly. This problem arises because of the low-momentum tilt allowed for bunching to preserve low-momentum spread. In this paper, we analyze in detail the space-charge effects on bunching of electrons with the CEBAF injector as an example. Conditions for effective matching of longitudinal phase space in the presence of space charge are discussed. (orig.)

  6. Electron capture into excited states of multi-charged ions

    International Nuclear Information System (INIS)

    Dijkkamp, D.

    1985-01-01

    This thesis deals with charge exchange reactions in slow collisions of multi-charged ions with neutral atoms or molecules. These reactions proceed very efficiently via a curve crossing mechanism, which leads to preferential population of excited states of the ion. The subsequent decay of these states leads to the emission of characteristic radiation. From wavelength resolved measurements of the absolute intensity of this radiation, cross sections for selective population of the excited (n,l-) states of the ion were determined. In addition, for some systems the total capture cross section was measured directly by means of charge state analysis of the secondary projectile ions. The role of charge exchange processes in fusion plasmas and in astrophysical plasmas is indicated. An experimental set-up is described with emphasis on the Electron Cyclotron Resonance Ion Source that was used in the experiments. Results for collisions of C 6+ , N 6+ , O 6+ and Ne 6+ with He, H 2 and Ar are presented as well as for electron capture from Li atoms by C 4+ and He 2+ . The interaction of the iso-electronic sequence C 4+ , N 5+ , O 6+ with atomic hydrogen, molecular hydrogen and helium is studied. First results for partial and total cross sections in collisions of fully stripped carbon, nitrogen and oxygen ions with atomic hydrogen are presented. These data are of particular importance for applications in fusion diagnostics. The data indicate that calculations of both molecular and atomic orbital type yield correct results, if an extended basis set is used. (Auth.)

  7. Correction of the deterministic part of space–charge interaction in momentum microscopy of charged particles

    Energy Technology Data Exchange (ETDEWEB)

    Schönhense, G., E-mail: schoenhense@uni-mainz.de [Institut für Physik, Johannes Gutenberg-Universität, 55128 Mainz (Germany); Medjanik, K. [Institut für Physik, Johannes Gutenberg-Universität, 55128 Mainz (Germany); Tusche, C. [Max-Planck-Institut für Mikrostrukturphysik, 06120 Halle (Germany); Loos, M. de; Geer, B. van der [Pulsar Physics, Burghstraat 47, 5614 BC Eindhoven (Netherlands); Scholz, M.; Hieke, F.; Gerken, N. [Physics Department and Center for Free-Electron Laser Science, Univ. Hamburg, 22761 Hamburg (Germany); Kirschner, J. [Max-Planck-Institut für Mikrostrukturphysik, 06120 Halle (Germany); Wurth, W. [Physics Department and Center for Free-Electron Laser Science, Univ. Hamburg, 22761 Hamburg (Germany); DESY Photon Science, 22607 Hamburg (Germany)

    2015-12-15

    Ultrahigh spectral brightness femtosecond XUV and X-ray sources like free electron lasers (FEL) and table-top high harmonics sources (HHG) offer fascinating experimental possibilities for analysis of transient states and ultrafast electron dynamics. For electron spectroscopy experiments using illumination from such sources, the ultrashort high-charge electron bunches experience strong space–charge interactions. The Coulomb interactions between emitted electrons results in large energy shifts and severe broadening of photoemission signals. We propose a method for a substantial reduction of the effect by exploiting the deterministic nature of space–charge interaction. The interaction of a given electron with the average charge density of all surrounding electrons leads to a rotation of the electron distribution in 6D phase space. Momentum microscopy gives direct access to the three momentum coordinates, opening a path for a correction of an essential part of space–charge interaction. In a first experiment with a time-of-flight momentum microscope using synchrotron radiation at BESSY, the rotation in phase space became directly visible. In a separate experiment conducted at FLASH (DESY), the energy shift and broadening of the photoemission signals were quantified. Finally, simulations of a realistic photoemission experiment including space–charge interaction reveals that a gain of an order of magnitude in resolution is possible using the correction technique presented here. - Highlights: • Photoemission spectromicroscopy with high-brightness pulsed sources is examined. • Deterministic interaction of an electron with the average charge density can be corrected. • Requires a cathode-lens type microscope optimized for best k-resolution in reciprocal plane. • Extractor field effectively separates pencil beam of secondary electrons from true signal. • Simulations reveal one order of magnitude gain in resolution.

  8. Emittance simulation for a different electron bunch charges with upgraded PITZ setup

    Energy Technology Data Exchange (ETDEWEB)

    Vashchenko, Grygorii [DESY, Platanenallee 6, 15738 Zeuthen (Germany)

    2013-07-01

    The photo injector test facility at DESY, Zeuthen site (PITZ) was invented with an aim to develop, characterize and optimize the electron sources for linac driven free electron lasers like FLASH and European XFEL. As a prerequisite for a successful experimental emittance optimization, emittance dependencies on the majority of linac parameters have to be studied in simulations. Despite that the nominal electron bunch charge for the operation of FLASH and XFEL is 1nC, there is an interest of the community to operate with other bunch charges. Emittance dependencies on such machine parameters like laser spot size on the photo cathode, laser pulse length, gun launching phase, focusing solenoid current and first accelerating structure gradient are simulated for different electron bunch charges. Based on the simulations data the systematic errors caused by detuning of the different machine parameters from their optimum values are estimated.

  9. Efficient scattering of electrons below few keV by Time Domain Structures around injection fronts

    Science.gov (United States)

    Vasko, I.; Agapitov, O. V.; Mozer, F.; Artemyev, A.; Krasnoselskikh, V.

    2016-12-01

    Van Allen Probes observations show an abundance of non-linear large-amplitude electrostatic spikes around injection fronts in the outer radiation belt. These spikes referred to as Time Domain Structures (TDS) include electron holes, double layers and more complicated solitary waves. The electron scattering driven by TDS may not be evaluated via the standard quasi-linear theory, since TDS are in principle non-linear plasma modes. In this paper we analyze the scattering of electrons by three-dimensional TDS (with non-negligible perpendicular electric field) around injection fronts. We derive the analytical formulas describing the local scattering by single TDS and show that the most efficiently scattered electrons are those in the first cyclotron resonance (electrons crossing TDS on a time scale comparable with their gyroperiod). The analytical formulas are verified via the test-particle simulation. We compute the bounce-averaged diffusion coefficients and demonstrate their dependence on the TDS spatial distribution, individual TDS parameters and L shell. We show that TDS are able to provide the pitch-angle scattering of <5 keV electrons at rate 10-2-10-4 s-1 and, thus, can be responsible for driving loss of electrons out of injections fronts on a time scale from few minutes to few hours. TDS can be, thus, responsible for driving diffuse aurora precipitations conjugated to injection fronts. We show that the pitch-angle scattering rates driven by TDS are comparable with those due to chorus waves and exceed those due to electron cyclotron harmonics. For injections fronts with no significant wave activity in the frequency range corresponding to chorus waves, TDS can be even dominant mechanism for losses of below few keV electrons.

  10. Structure of very heavy few-electron ions - new results from the heavy ion storage ring, ESR

    International Nuclear Information System (INIS)

    Mokler, P.H.; Stoehlker, T.; Kozhuharov, C.; Moshammer, R.; Rymuza, P.; Bosch, F.; Kandler, T.

    1993-08-01

    The heavy ion synchrotron/storage ring facility at GSI, SIS/ESR, provides intense beams of cooled, highly-charged ions up to naked uranium (U 92+ ). By electron capture during ion-atom collisions in the gas target of the ESR or by recombination at ion-electron encounters in the ''electron cooler'' excited states are populated. The detailed structure of very heavy one-, two- and three-electron ions is studied. The different mechanisms leading to the excited states are described, as well as the new experimental tools now available for a detailed spectroscopy of these interesting systems. Special emphasis is given to X-ray transitions to the groundstates in H- and He-like systems. For the heaviest species the groundstate Lambshift can now be probed on an accuracy level of better than 10% using solid-state X-ray detectors. Applying dispersive X-ray analyzing techniques, this accuracy will certainly be improved in future. However, utilizing the dielectronic resonances for a spectroscopy, the structure in Li-like heavy ions can already be probed now on the sub eV level. (orig.)

  11. Charge symmetry of electron wave functions in a quantized electromagnetic wave field

    Energy Technology Data Exchange (ETDEWEB)

    Fedorov, M V [AN SSSR, Moscow. Fizicheskij Inst.

    1975-01-01

    An attempt to clear up the reasons of the electron charge symmetry violation in the quantum wave field was made in this article. For this purpose the connection between the Dirac equation and the electron wave functions in the external field with the exact equation of quantum electrodynamics is established. Attention is paid to the fact that a number of equations for single-electron wave functions can be used in the framework of the same assumptions. It permits the construction of the charge-symmetric solutions in particular.

  12. Single ion induced surface nanostructures: a comparison between slow highly charged and swift heavy ions.

    Science.gov (United States)

    Aumayr, Friedrich; Facsko, Stefan; El-Said, Ayman S; Trautmann, Christina; Schleberger, Marika

    2011-10-05

    This topical review focuses on recent advances in the understanding of the formation of surface nanostructures, an intriguing phenomenon in ion-surface interaction due to the impact of individual ions. In many solid targets, swift heavy ions produce narrow cylindrical tracks accompanied by the formation of a surface nanostructure. More recently, a similar nanometric surface effect has been revealed for the impact of individual, very slow but highly charged ions. While swift ions transfer their large kinetic energy to the target via ionization and electronic excitation processes (electronic stopping), slow highly charged ions produce surface structures due to potential energy deposited at the top surface layers. Despite the differences in primary excitation, the similarity between the nanostructures is striking and strongly points to a common mechanism related to the energy transfer from the electronic to the lattice system of the target. A comparison of surface structures induced by swift heavy ions and slow highly charged ions provides a valuable insight to better understand the formation mechanisms. © 2011 IOP Publishing Ltd

  13. Laboratory Measurements of Charging of Apollo 17 Lunar Dust Grains by Low Energy Electrons

    Science.gov (United States)

    Abbas, Mian M.; Tankosic, Dragana; Spann, James F.; Dube, Michael J.; Gaskin, Jessica

    2007-01-01

    It is well recognized that the charging properties of individual micron/sub-micron size dust grains by various processes are expected to be substantially different from the currently available measurements made on bulk materials. Solar UV radiation and the solar wind plasma charge micron size dust grains on the lunar surface with virtually no atmosphere. The electrostatically charged dust grains are believed to be levitated and transported long distances over the lunar terminator from the day to the night side. The current models do not fully explain the lunar dust phenomena and laboratory measurements are needed to experimentally determine the charging properties of lunar dust grains. An experimental facility has been developed in the Dusty Plasma Laboratory at NASA Marshall Space Flight Center MSFC for investigating the charging properties of individual micron/sub-micron size positively or negatively charged dust grains by levitating them in an electrodynamic balance in simulated space environments. In this paper, we present laboratory measurements on charging of Apollo 17 individual lunar dust grains by low energy electron beams in the 5-100 eV energy range. The measurements are made by levitating Apollo 17 dust grains of 0.2 to 10 micrometer diameters, in an electrodynamic balance and exposing them to mono-energetic electron beams. The charging rates and the equilibrium potentials produced by direct electron impact and by secondary electron emission processes are discussed.

  14. Contrast and Raman spectroscopy study of single- and few-layered charge density wave material: 2H-TaSe2

    Science.gov (United States)

    Hajiyev, Parviz; Cong, Chunxiao; Qiu, Caiyu; Yu, Ting

    2013-01-01

    In this article, we report the first successful preparation of single- and few-layers of tantalum diselenide (2H-TaSe2) by mechanical exfoliation technique. Number of layers is confirmed by white light contrast spectroscopy and atomic force microscopy (AFM). Vibrational properties of the atomically thin layers of 2H-TaSe2 are characterized by micro-Raman spectroscopy. Room temperature Raman measurements demonstrate MoS2-like spectral features, which are reliable for thickness determination. E1g mode, usually forbidden in backscattering Raman configuration is observed in the supported TaSe2 layers while disappears in the suspended layers, suggesting that this mode may be enabled because of the symmetry breaking induced by the interaction with the substrate. A systematic in-situ low temperature Raman study, for the first time, reveals the existence of incommensurate charge density wave phase transition in single and double-layered 2H-TaSe2 as reflected by a sudden softening of the second-order broad Raman mode resulted from the strong electron-phonon coupling (Kohn anomaly). PMID:24005335

  15. Experiments with highly-charged heavy-ions performed at the storage ring ESR

    International Nuclear Information System (INIS)

    Mokler, P.H.

    1992-01-01

    The new heavy ion accelerator facility SIS/ESR was inaugurated in April 1990. During 1991 the experimental storage ring, ESR, has been commissioned. Highly-charged heavy ions from O 8+ up to Bi 82+ were successfully accumulated, cooled, and stored in the ring. Now all highly-charged, heavy ions can be provided for experiments at comfortable storage times and at energies roughly between 100 and 500 MeV/u. A report on the achievements and on the first experimental results will be given. For the experiments, special emphasis is put on capture processes in the electron cooler, i.e. on radiative and dielectronic recombination processes as well as on capture events of bound target electrons from a gas jet. In this case, the capture leads either directly (REC) or by cascading to X-ray emission, which is also exploited for a precision spectroscopy of the structure of the heaviest ions. Another exciting topic is the radioactive decay of highly charged ions: For instance the β-decay into bound atomic states, which is not possible for neutral atoms, was studied for stored naked Dy ions. (orig.)

  16. Electron-molecule chemistry and charging processes on organic ices and Titan's icy aerosol surrogates

    Science.gov (United States)

    Pirim, C.; Gann, R. D.; McLain, J. L.; Orlando, T. M.

    2015-09-01

    Electron-induced polymerization processes and charging events that can occur within Titan's atmosphere or on its surface were simulated using electron irradiation and dissociative electron attachment (DEA) studies of nitrogen-containing organic condensates. The DEA studies probe the desorption of H- from hydrogen cyanide (HCN), acetonitrile (CH3CN), and aminoacetonitrile (NH2CH2CN) ices, as well as from synthesized tholin materials condensed or deposited onto a graphite substrate maintained at low temperature (90-130 K). The peak cross sections for H- desorption during low-energy (3-15 eV) electron irradiation were measured and range from 3 × 10-21 to 2 × 10-18 cm2. Chemical and structural transformations of HCN ice upon 2 keV electron irradiation were investigated using X-ray photoelectron and Fourier-transform infrared spectroscopy techniques. The electron-beam processed materials displayed optical properties very similar to tholins produced by conventional discharge methods. Electron and negative ion trapping lead to 1011 charges cm-2 on a flat surface which, assuming a radius of 0.05 μm for Titan aerosols, is ∼628 charges/radius (in μm). The facile charge trapping indicates that electron interactions with nitriles and complex tholin-like molecules could affect the conductivity of Titan's atmosphere due to the formation of large negative ion complexes. These negatively charged complexes can also precipitate onto Titan's surface and possibly contribute to surface reactions and the formation of dunes.

  17. Commissioning results of the ReA EBIT charge breeder at the NSCL: First reacceleration of stable-isotope beams

    Energy Technology Data Exchange (ETDEWEB)

    Lapierre, A., E-mail: lapierre@nscl.msu.edu; Schwarz, S.; Kittimanapun, K.; Rodriguez, J.A.; Sumithrarachchi, C.; Barquest, B.; Berryman, E.; Cooper, K.; Fogleman, J.; Krause, S.; Kwarsick, J.; Nash, S.; Perdikakis, G.; Portillo, M.; Rencsok, R.; Skutt, D.; Steiner, M.; Tobos, L.; Wittmer, W.; Bollen, G.; and others

    2013-12-15

    Highlights: • Latest results with the electron-beam ion trap of the ReA post-accelerator at the NSCL. • First reacceleration of stable-isotope beams. • First injection of stable-isotope beams from the NSCL’s beam stopping vault. -- Abstract: ReA is a reaccelerator of rare-isotope beams at the National Superconducting Cyclotron Laboratory (NSCL). The rare isotopes are produced by fast projectile fragmentation. After production, they are separated in-flight and thermalized in a He gas “catcher” cell before being sent to ReA for reacceleration to a few MeV/u. One of its main components is an electron-beam ion trap (EBIT) employed to convert injected singly charged ions to highly charged ions prior to injection into linear-accelerator structures. The ReA EBIT features a high-current electron gun, a long trap structure, and a two-field superconducting magnet to provide both the high electron-beam current density needed for fast charge breeding and high capture probability of injected beams. This paper presents recent commissioning results. In particular, {sup 39}K{sup +} ions have been injected, charge bred to {sup 39}K{sup 16+} and extracted for reacceleration up to 60 MeV. First charge-breeding results of beams injected from a commissioning Rb ion source in the NSCL’s beam “stopping” vault are also presented.

  18. Polarized electrons, trions, and nuclei in charged quantum dots

    Science.gov (United States)

    Bracker, A. S.; Tischler, J. G.; Korenev, V. L.; Gammon, D.

    2003-07-01

    We have investigated spin polarization in GaAs quantum dots. Excitons and trions are polarized directly by optical excitation and studied through polarization of photoluminescence. Electrons and nuclei are polarized indirectly through subsequent relaxation processes. Polarized electrons are identified by the Hanle effect for exciton and trion photoluminescence, while polarized nuclei are identified through the Overhauser effect in individual charged quantum dots.

  19. Electron holography study of the charging effect in microfibrils of sciatic nerve tissues.

    Science.gov (United States)

    Kim, Ki Hyun; Akase, Zentaro; Shindo, Daisuke; Ohno, Nobuhiko; Fujii, Yasuhisa; Terada, Nobuo; Ohno, Shinichi

    2013-08-01

    The charging effects of microfibrils of sciatic nerve tissues due to electron irradiation are investigated using electron holography. The phenomenon that the charging effects are enhanced with an increase of electron intensity is visualized through direct observations of the electric potential distribution around the specimen. The electric potential at the surface of the specimen could be quantitatively evaluated by simulation, which takes into account the reference wave modulation due to the long-range electric field.

  20. Prospects for parity-nonconservation experiments with highly charged heavy ions

    OpenAIRE

    Maul, Martin; Schäfer, Andreas; Greiner, Walter; Indelicato, Paul

    2006-01-01

    We discuss the prospects for parity-nonconservation experiments with highly charged heavy ions. Energy levels and parity mixing for heavy ions with 2–5 electrons are calculated. We investigate two-photon transitions and the possibility of observing interference effects between weak-matrix elements and Stark matrix elements for periodic electric field configurations.

  1. Super TOF secondary ion mass spectroscopy using very highly charged primary ions up to Th70+

    International Nuclear Information System (INIS)

    Briere, M.A.; Schenkel, T.; Schneider, D.

    1995-01-01

    The LLNL Electron Beam Ion Trap (EBIT) has made low emittance beams of slow highly charged ions available for ion-solid interaction studies. Such interactions feature the dominance of electronic over collisional effects, and the shock waves generated by the ionized target atoms can desorb large numbers of large molecular species from the surface. This paper presents the first systematic study of the sputtering process due to the incidence of slow very highly charged ions; Th 70+ ions are extracted from EBIT at 7 keV * q and directed onto thin SiO 2 films on Si. Results suggest secondary ion yields of up to 25 per incident ion for Th 70+ (secondary ion yield is increased over that for singly or moderately charged ions). Correlations of the negative, positive, and negative cluster ion yields show promise for application of highly charged ion induced sputtering for enhanced sensitivity and quantitative (absolute) SIMS analysis of deep submicron scale surface layers and polymeric and biomolecular material analysis

  2. Interaction of slow, highly charged ions with the surface of ionic crystals; Wechselwirkung langsamer hochgeladener Ionen mit der Oberflaeche von Ionenkristallen

    Energy Technology Data Exchange (ETDEWEB)

    Heller, Rene

    2009-08-15

    In this thesis the creation of permanent nanostructures induced by the impact of very slow (v{<=}5 x 10{sup 5} m/s) highly charged (q{<=}40) ions on the ionic crystal surfaces of CaF{sub 2} and KBr is investigated. The systematic analysis of the samples surfaces by means of atomic force microscopy supplies information on the influence of the potential as well as the kinetic projectile energy on the process of structure creation. The individual impact of highly charged ions on the KBr(001) surface can initiate the creation of mono-atomic deep pit-like structures -nanopits- with a lateral size of a few 10 nm. The volume of these pits and the corresponding number of sputtered secondary particles show a linear dependence on the projectiles potential energy. For the onset of pit formation a kinetic energy dependent threshold in the potential energy E{sup grenz}{sub pot}(E{sub kin}) could be identified. Based on the defect-mediated desorption by electrons and by including effects of defect agglomeration a consistent model for the process of pit formation was drawn. In this work the recently discovered creation of hillock-like structures by impact of highly charged ions on CaF{sub 2}(111) surfaces could be verified for lowest kinetic energies (E{sub kin}{<=}150 eV x q). For the first time the potential energy of impinging projectiles could be identified to be exclusively responsible for the creation of nanostructures. Furthermore, a shift of potential energy threshold for hillock formation was observed for very small projectile velocities. Within the framework of cooperation with the Vienna University of Technology simulations based on the inelastic thermal spike model were performed, which allowed to interlink the individual hillock formation with a local melting of the ionic lattice. The essential influence of electron emission during the interaction of the highly charged ions with the surface on the process of nanostructuring was taken into consideration by

  3. Few layer graphene wrapped mixed phase TiO2 nanofiber as a potential electrode material for high performance supercapacitor applications

    Science.gov (United States)

    Thirugnanam, Lavanya; Sundara, Ramaprabhu

    2018-06-01

    A combination of favorable composition and optimized anatase/rutile mixed-phase TiO2 (MPTNF)/Hydrogen exfoliated graphene (HEG) composite nanofibers (MPTNF/HEG) and anatase/rutile mixed-phase TiO2/reduced graphene oxide (rGO) composite nanofibers (MPTNF/rGO) have been reported to enhance the electrochemical properties for supercapacitor applications. These composite nanofibers have been synthesized by an efficient route of electrospinning together with the help of easy chemical methods. Both the composites exhibit good charge storage capability with enhanced pseudocapacitance and electric double-layer capacitance (EDLC) as confirmed by cyclic voltammetry studies. MPTNF/HEG composite showed maximum specific capacitance of 210.5 F/g at the current density of 1 A/g, which was mainly due to its availability of the more active sites for ions adsorption on a few layers of graphene wrapped TiO2 nanofiber surface. The synergistic effect of anatase/rutile mixed phase with one dimensional nanostructure and the electronic interaction between TiO2 and few layer graphene provided the subsequent improvement of ion adsorption capacity. Also exhibit excellent electrochemical performance to improve the capacitive properties of TiO2 electrode materials which is required for the development of flexible electrodes in energy storage devices and open up new opportunities for high performance supercapacitors.

  4. Nonlinear energy loss of highly charged heavy ions

    International Nuclear Information System (INIS)

    Zwicknagel, G.Guenter.

    2000-01-01

    For slow, highly charged heavy ions strong coupling effects in the energy transfer from the projectile-ion to an electron target plasma become important. A theoretical description of this nonlinear ion stopping has to go beyond the standard approaches like the dielectric linear response or the binary collision model which are strictly valid only at weak ion-target coupling. Here we outline an improved treatment which is based on a suitable combination of binary collision and linear response contributions. As has been verified for isotropic, nonmagnetized electron plasmas by comparison with simulations, this approach well reproduces the essential features of nonlinear stopping up to moderate coupling strength. Its extension to anisotropic, magnetized electron plasmas basically involves the fully numerical determination of the momentum and energy transfer in binary ion-electron collisions in the presence of a magnetic field. First results of such calculations are presented and discussed

  5. Electron energy distribution function, effective electron temperature, and dust charge in the temporal afterglow of a plasma

    International Nuclear Information System (INIS)

    Denysenko, I. B.; Azarenkov, N. A.; Kersten, H.

    2016-01-01

    Analytical expressions describing the variation of electron energy distribution function (EEDF) in an afterglow of a plasma are obtained. Especially, the case when the electron energy loss is mainly due to momentum-transfer electron-neutral collisions is considered. The study is carried out for different EEDFs in the steady state, including Maxwellian and Druyvesteyn distributions. The analytical results are not only obtained for the case when the rate for momentum-transfer electron-neutral collisions is independent on electron energy but also for the case when the collisions are a power function of electron energy. Using analytical expressions for the EEDF, the effective electron temperature and charge of the dust particles, which are assumed to be present in plasma, are calculated for different afterglow durations. An analytical expression for the rate describing collection of electrons by dust particles for the case when the rate for momentum-transfer electron-neutral collisions is independent on electron energy is also derived. The EEDF profile and, as a result, the effective electron temperature and dust charge are sufficiently different in the cases when the rate for momentum-transfer electron-neutral collisions is independent on electron energy and when the rate is a power function of electron energy.

  6. Consideration of Relativistic Dynamics in High-Energy Electron Coolers

    CERN Document Server

    Bruhwiler, David L

    2005-01-01

    A proposed electron cooler for RHIC would use ~55 MeV electrons to cool fully-ionized 100 GeV/nucleon gold ions.* At two locations in the collider ring, the electrons and ions will co-propagate for ~13 m, with velocities close to c and gamma>100. To lowest-order, one can Lorentz transform all physical quantities into the beam frame and calculate the dynamical friction forces assuming a nonrelativisitc, electrostatic plasma. However, we show that nonlinear space charge forces of the bunched electron beam on the ions must be calculated relativistically, because an electrostatic beam-frame calculation is not valid for such short interaction times. The validity of nonrelativistic friction force calculations must also be considered. Further, the transverse thermal velocities of the high-charge (~20 nC) electron bunch are large enough that some electrons have marginally relativistic velocities, even in the beam frame. Hence, we consider relativistic binary collisions – treating the model problem of ...

  7. Space charge effects and aberrations on electron pulse compression in a spherical electrostatic capacitor.

    Science.gov (United States)

    Yu, Lei; Li, Haibo; Wan, Weishi; Wei, Zheng; Grzelakowski, Krzysztof P; Tromp, Rudolf M; Tang, Wen-Xin

    2017-12-01

    The effects of space charge, aberrations and relativity on temporal compression are investigated for a compact spherical electrostatic capacitor (α-SDA). By employing the three-dimensional (3D) field simulation and the 3D space charge model based on numerical General Particle Tracer and SIMION, we map the compression efficiency for a wide range of initial beam size and single-pulse electron number and determine the optimum conditions of electron pulses for the most effective compression. The results demonstrate that both space charge effects and aberrations prevent the compression of electron pulses into the sub-ps region if the electron number and the beam size are not properly optimized. Our results suggest that α-SDA is an effective compression approach for electron pulses under the optimum conditions. It may serve as a potential key component in designing future time-resolved electron sources for electron diffraction and spectroscopy experiments. Copyright © 2017 Elsevier B.V. All rights reserved.

  8. Production of high intensity electron bunches for the SLAC Linear Collider

    International Nuclear Information System (INIS)

    James, M.B.

    1987-08-01

    This thesis describes the design and performance of a high intensity electron injecfor for the SLAC Linear Collider. Motivation for the collider and the specifications for the injector are discussed. An analytic theory of the bunching and capture of electrons by rf fields is discussed in the limit of low space charge and small signal. The design and performance of SLAC's main injector are described to illustrate a successful application of this theory. The bunching and capture of electrons by rf fields are then discussed in the limit of high space charge and large signal, and a description of the design of the collider injector follows. In the limit of high space charge forces and large rf signals, the beam dynamics are considerably more complex and numerical simulations are required to predict particle motion. A computer code which models the longitudinal dynamics of electrons in the presence of space charge and rf fields is described. The results of the simulations, the resulting collider injector design and the various components which make up the collider injector are described. These include the gun, subharmonic bunchers, traveling-wave buncher and velocity-of-light accelerator section. Finally, the performance of the injector is described including the beam intensity, bunch length, transverse emittance and energy spectrum. While the final operating conditions differ somewaht from the design, the performance of the collider injector is in good agreement with the numerical simulations and meets all of the collider specifications. 28 refs

  9. Experimental study of interactions of highly charged ions with atoms at keV energies: Progress report for period May 15, 1985-February 15, 1987

    International Nuclear Information System (INIS)

    Kostroun, V.O.

    1987-01-01

    Interest in interactions of low energy highly charged ions with electrons, atoms or ions is due to their importance to controlled thermonuclear fusion research and the interesting nature of the fundamental processes involved. Studies of such interactions have long been hampered by a lack of suitable ions sources. A superconducting solenoid, cryogenic Electron Beam Ion Source, CEBIS, has been constructed at Cornell University to produce low energy very highly charged ions. At present, using a pulsed 0.5A,8.5 keV electron beam, the source is capable of producing highly charged ions of C,N,O, including bare nuclei, and ions of Ar up to charge state 11 + in 1 millisecond of confinement time. The source is being used in experiments to investigate charge transfer and accompanying processes in low energy, highly charged ion-atom collisions

  10. Calculation of electromagnetic observables in few-body systems

    International Nuclear Information System (INIS)

    Gibson, B.F.

    1986-10-01

    An introduction to the calculation of electromagnetic observables in few-body systems is given by studying two examples in the trinucleon system: (1) the elastic electron scattering charge form factor in configuration space and momentum space and (2) the two-body photodisintegration of 3 H leading to a neutron-deuteron final state in a separable potential formalism. In the discussion of charge form factor calculations, a number of related topics are touched upon: the relation of structure in Psi to the properties of simple NN forces, the Faddeev and Schroedinger solution to the harmonic oscillator problem, the Rosenbluth formula for electron scattering from a spin-1/2 nuclear target (e.g., the proton or 3 H), and the charge density operator. Formulae for 3 He and 3 H charge form factors in a central force approximation are given in configuration and momentum space. The physics of these form factors is discussed in light of results from realistic nucleon-nucleon potential model calculations, including the effects of two-pion-exchange three-body force models. Topics covered are the rms charge densities, and the Coulomb energy of 3 He. In the discussion of the 3 H photodisintegration, the Siegert form of the electric dipole operator (in the long wave length limit) is derived as are the separable potential equations which describe the off-shell transition amplitudes which connect nucleon-plus-corrected-pair states. Expressions for the Born amplitudes required to complete the two-body photodisintegration amplitude calculation are given. Numerical results for a model central force problem are discussed and compared with an approximate calculation. Comparisons with 3 H(γ,n)d and 3 He(γ,p)d data are made, and the significant features of the exact theoretical calculation are outlined. 61 refs., 26 figs

  11. Electron-ion recombination in merged beams

    International Nuclear Information System (INIS)

    Wolf, A.; Habs, D.; Lampert, A.; Neumann, R.; Schramm, U.; Schuessler, T.; Schwalm, D.

    1993-01-01

    Detailed studies of recombination processes between electrons and highly charged ions have become possible by recent improvements of merged-beams experiments. We discuss in particular measurements with stored cooled ion beams at the Test Storage Ring (TSR) in Heidelberg. The cross section of dielectronic recombination was measured with high energy resolution for few-electron systems up to the nuclear charge of Cu at a relative energy up to 2.6 keV. At low energy (∼0.1 eV) total recombination rates of several ions were measured and compared with calculated radiative recombination rates. Laser-stimulated recombination of protons and of C 6+ ions was investigated as a function of the photon energy using visible radiation. Both the total recombination rates and the stimulated recombination spectra indicate that in spite of the short interaction time in merged beams, also collisional capture of electrons into weakly bound levels (related to three-body recombination) could be important

  12. Few-electron Qubits in Silicon Quantum Electronic Devices

    Science.gov (United States)

    2014-09-01

    Calculation of the charge relaxation time T1 . . . . . . . . . . . . . . 63 5.1 The absence of spin blockade in dual-gated DQD devices . . . . . . . 70...2013. 98 115 [102] M. Pioro-Ladrière, T. Obata, Y. Tokura, Y.-S. Shin, T. Kubo , K. Yoshida, T. Taniyama, and S. Tarucha. Nat. Phys., 4:776–779

  13. Comparison between the 30- to 80-keV electron channels at ATS 6 and 1976-059A during conjunction and application to spacecraft charging prediction

    International Nuclear Information System (INIS)

    Garrett, H.B.; Schwank, D.C.; Higbie, P.R.; Baker, D.N.

    1980-01-01

    The ATS 6 satellite, during an orbital maneuver in September 1976, passed within a few hundred kilometers of the geosynchronous satellite 1976-059A. Analysis of the 30- to 80-keV electron data from the University of California at San Diego (UCSD) electrostatic analyzers on ATS 6 and the 30- to 300-keV electron data from the Los Alamos Scientific Laboratory instrument on 1976-059A during this period reveals good agreement between the two instruments even when the separation is +- 7 0 . The low-energy UCSD ion data from ATS 6 allow a simultaneous determination of the potential difference between ATS 6 and th ambient medium. Use of the 1976-059A electron data to approximate the ambient plasma electron density and temperature during these charging periods indicates sufficient information exists in order to estimate the maximum potentials to which ATS 6 charges in sunlight an eclipse. As data from 1976-059A and similar satellites are potentially available in real time, the information therefore exists to create a satellite charging index for the geosynchronous regime that would be valid within at least +- 7 0 longitude of the position of each measurement

  14. Novel simulation method of space charge effects in electron optical systems including emission of electrons

    Czech Academy of Sciences Publication Activity Database

    Zelinka, Jiří; Oral, Martin; Radlička, Tomáš

    2018-01-01

    Roč. 184, JAN (2018), s. 66-76 ISSN 0304-3991 R&D Projects: GA MŠk(CZ) LO1212; GA MŠk ED0017/01/01 Institutional support: RVO:68081731 Keywords : space charge * self-consistent simulation * aberration polynomial * electron emission Subject RIV: JA - Electronics ; Optoelectronics, Electrical Engineering Impact factor: 2.843, year: 2016

  15. 2D scattering of unpolarized beams of electrons by charged nanomagnets

    Energy Technology Data Exchange (ETDEWEB)

    Senbeta, Teshome, E-mail: teshearada@yahoo.com [Department of Physics, Addis Ababa University, P.O. Box 1176, Addis Ababa (Ethiopia); Mal' nev, V.N., E-mail: vnmalnev@aau.edu.et [Department of Physics, Addis Ababa University, P.O. Box 1176, Addis Ababa (Ethiopia)

    2012-07-15

    2D spin-dependent scattering of slow unpolarized beams of electrons by charged nanomagnets is analyzed in the Born approximation. The obtained scattering lengths are larger than those from the neutral nanomagnets approximately by one order. It is shown that for particular parameters of the system it is possible to polarize completely the scattered electrons in a narrow range of scattering angles. The most suitable system for realization of these effects is 2D Si electron gas with immersed nanomagnets. - Highlights: Black-Right-Pointing-Pointer We study 2D spin dependent electron scattering by charged nanomagnets. Black-Right-Pointing-Pointer The applicability of the Born approximation to the problem is discussed. Black-Right-Pointing-Pointer Unpolarized incident beams used to obtain completely polarized scattered electrons. Black-Right-Pointing-Pointer The study shows peculiarities of 2D spin dependent scattering enhanced by Coulomb potential. Black-Right-Pointing-Pointer The result obtained can be used as one method of controlling spin currents.

  16. Modal description of longitudinal space-charge fields in pulse-driven free-electron devices

    Directory of Open Access Journals (Sweden)

    Yu. Lurie

    2010-05-01

    Full Text Available In pulsed-beam free-electron devices, longitudinal space-charge fields result in collective effects leading to an expansion of short electron bunches along their trajectory. This effect restricts an application of intense ultrashort electron pulses in free-electron radiation sources. A careful theoretical treatment is required in order to achieve an accurate description of the self-fields and the resulted electron beam dynamics. In this paper, longitudinal space-charge fields are considered in the framework of a three-dimensional, space-frequency approach. The model is based on the expansion of the total electromagnetic field (including self-fields in terms of transverse eigenmodes of the (cold cavity, in which the field is excited and propagates. The electromagnetic field, originally obtained in the model as a solution of the wave equation, is shown to satisfy also Gauss’s law. We applied the theory to derive an analytical expression for the longitudinal electric field of a pointlike charge, moving along a waveguide at a constant velocity. This enables consideration and study of the role played by different terms of the resulted expressions, such as components arising from forward and backward waves, propagating waves, and under cutoff frequencies, and so on. Possible simplifications in evaluation of longitudinal space-charge fields are discussed.

  17. Operation of Lanzhou all permanent electron cyclotron resonance ion source No. 2 on 320 kV platform with highly charged ions.

    Science.gov (United States)

    Lu, W; Li, J Y; Kang, L; Liu, H P; Li, H; Li, J D; Sun, L T; Ma, X W

    2014-02-01

    The 320 kV platform for multi-discipline research with highly charged ions is a heavy ion beam acceleration instrument developed by Institute of Modern Physics, which is dedicated to basic scientific researches such as plasma, atom, material physics, and astrophysics, etc. The platform has delivered ion beams of 400 species for 36,000 h. The average operation time is around 5000 h/year. With the beams provided by the platform, lots of outstanding progresses were made in various research fields. The ion source of the platform is an all-permanent magnet electron cyclotron resonance ion source, LAPECR2 (Lanzhou All Permanent ECR ion source No. 2). The maximum axial magnetic fields are 1.28 T at injection and 1.07 T at extraction, and the radial magnetic field is up to 1.21 T at the inner wall of the plasma chamber. The ion source is capable to produce low, medium, and high charge state gaseous and metallic ion beams, such as H(+), (40)Ar(8+), (129)Xe(30+), (209)Bi(33+), etc. This paper will present the latest result of LAPECR2 and the routine operation status for the high voltage platform.

  18. High temperature electron beam ion source for the production of single charge ions of most elements of the Periodic Table

    CERN Document Server

    Panteleev, V N; Barzakh, A E; Fedorov, D V; Ivanov, V S; Moroz, F V; Orlov, S Y; Seliverstov, D M; Stroe, L; Tecchio, L B; Volkov, Y M

    2003-01-01

    A new type of a high temperature electron beam ion source (HTEBIS) with a working temperature up to 2500 deg. C was developed for production of single charge ions of practically all elements. Off-line tests and on-line experiments making use of the developed ion source coupled with uranium carbide targets of different density, have been carried out. The ionization efficiency measured for stable atoms of many elements varied in the interval of 1-6%. Using the HTEBIS, the yields and on-line production efficiency of neutron rich isotopes of Mn, Fe, Co, Cu, Rh, Pd, Ag, Cd, In, Sn and isotopes of heavy elements Pb, Bi, Po and some others have been determined. The revealed confinement effect of the ions produced in the narrow electron beam inside a hot ion source cavity has been discussed.

  19. Energy loss and charge exchange processes of high energy heavy ions channeled in crystals

    International Nuclear Information System (INIS)

    Poizat, J.C.; Andriamonje, S.; Anne, R.; Faria, N.V.d.C.; Chevallier, M.; Cohen, C.; Dural, J.; Farizon-Mazuy, B.; Gaillard, M.J.; Genre, R.; Hage-Ali, M.; Kirsch, R.; L'hoir, A.; Mory, J.; Moulin, J.; Quere, Y.; Remillieux, J.; Schmaus, D.; Toulemonde, M.

    1990-01-01

    The interaction of moving ions with single crystals is very sensitive to the orientation of the incident beam with respect to the crystalline directions of the target. Our experiments show that high energy heavy ion channeling deeply modifies their slowing down and charge exchange processes. This is due to the fact that channeled ions interact only with outershell target electrons, which means that the electron density they experience is very low and that the binding energy, and then the momentum distribution of these electrons, are quite different from the corresponding average values associated to random incidence. The two experimental studies presented here show the reduction of the energy loss rate for fast channeled heavy ions and illustrate the two aspects of channeling effects on charge exchange, the reduction of electron loss on one hand, and of electron capture on the other hand

  20. High current polarized electron source

    Science.gov (United States)

    Suleiman, R.; Adderley, P.; Grames, J.; Hansknecht, J.; Poelker, M.; Stutzman, M.

    2018-05-01

    Jefferson Lab operates two DC high voltage GaAs photoguns with compact inverted insulators. One photogun provides the polarized electron beam at the Continuous Electron Beam Accelerator Facility (CEBAF) up to 200 µA. The other gun is used for high average current photocathode lifetime studies at a dedicated test facility up to 4 mA of polarized beam and 10 mA of un-polarized beam. GaAs-based photoguns used at accelerators with extensive user programs must exhibit long photocathode operating lifetime. Achieving this goal represents a significant challenge for proposed facilities that must operate in excess of tens of mA of polarized average current. This contribution describes techniques to maintain good vacuum while delivering high beam currents, and techniques that minimize damage due to ion bombardment, the dominant mechanism that reduces photocathode yield. Advantages of higher DC voltage include reduced space-charge emittance growth and the potential for better photocathode lifetime. Highlights of R&D to improve the performance of polarized electron sources and prolong the lifetime of strained-superlattice GaAs are presented.

  1. Electron beam patterning for writing of positively charged gold colloidal nanoparticles

    Science.gov (United States)

    Zafri, Hadar; Azougi, Jonathan; Girshevitz, Olga; Zalevsky, Zeev; Zitoun, David

    2018-02-01

    Synthesis at the nanoscale has progressed at a very fast pace during the last decades. The main challenge today lies in precise localization to achieve efficient nanofabrication of devices. In the present work, we report on a novel method for the patterning of gold metallic nanoparticles into nanostructures on a silicon-on-insulator (SOI) wafer. The fabrication makes use of relatively accessible equipment, a scanning electron microscope (SEM), and wet chemical synthesis. The electron beam implants electrons into the insulating material, which further anchors the positively charged Au nanoparticles by electrostatic attraction. The novel fabrication method was applied to several substrates useful in microelectronics to add plasmonic particles. The resolution and surface density of the deposition were tuned, respectively, by the electron energy (acceleration voltage) and the dose of electronic irradiation. We easily achieved the smallest written feature of 68 ± 18 nm on SOI, and the technique can be extended to any positively charged nanoparticles, while the resolution is in principle limited by the particle size distribution and the scattering of the electrons in the substrate. [Figure not available: see fulltext.

  2. Achieving few-femtosecond time-sorting at hard X-ray free-electron lasers

    Science.gov (United States)

    Harmand, M.; Coffee, R.; Bionta, M. R.; Chollet, M.; French, D.; Zhu, D.; Fritz, D. M.; Lemke, H. T.; Medvedev, N.; Ziaja, B.; Toleikis, S.; Cammarata, M.

    2013-03-01

    Recently, few-femtosecond pulses have become available at hard X-ray free-electron lasers. Coupled with the available sub-10 fs optical pulses, investigations into few-femtosecond dynamics are not far off. However, achieving sufficient synchronization between optical lasers and X-ray pulses continues to be challenging. We report a `measure-and-sort' approach, which achieves sub-10 fs root-mean-squared (r.m.s.) error measurement at hard X-ray FELs, far beyond the 100-200 fs r.m.s. jitter limitations. This timing diagnostic, now routinely available at the Linac Coherent Light Source (LCLS), is based on ultrafast free-carrier generation in optically transparent materials. Correlation between two independent measurements enables unambiguous demonstration of ~6 fs r.m.s. error in reporting the optical/X-ray delay, with single shot error suggesting the possibility of reaching few-femtosecond resolution.

  3. Charge redistribution and properties of high-temperature superconductors

    International Nuclear Information System (INIS)

    Khomskii, D.I.; Kusmartsev, F.V.

    1992-01-01

    We show that in high-T c superconductors (HTSC) with two groups of electrons (e.g., holes in CuO 2 planes and in a ''reservoir'') there should exist a charge redistribution with the temperature: the hole concentration N h in ''active'' superconducting CuO 2 planes increases below T c . This effect may explain structural changes such as the shift of the apical oxygen atom, anomalous thermal expansion, the shift of nuclear quadrupole resonance lines, the change of the positron lifetime, and the modification of the ion channeling below T c . Some other possible consequences of the charge redistribution (the modification of the temperature dependence of a gap Δ and of the ratio 2Δ 0 /T c , the phenomena at a contact of HTSC with normal metals and semiconductors) are discussed

  4. Electron-hole collision limited transport in charge-neutral bilayer graphene

    Science.gov (United States)

    Nam, Youngwoo; Ki, Dong-Keun; Soler-Delgado, David; Morpurgo, Alberto F.

    2017-12-01

    Ballistic transport occurs whenever electrons propagate without collisions deflecting their trajectory. It is normally observed in conductors with a negligible concentration of impurities, at low temperature, to avoid electron-phonon scattering. Here, we use suspended bilayer graphene devices to reveal a new regime, in which ballistic transport is not limited by scattering with phonons or impurities, but by electron-hole collisions. The phenomenon manifests itself in a negative four-terminal resistance that becomes visible when the density of holes (electrons) is suppressed by gate-shifting the Fermi level in the conduction (valence) band, above the thermal energy. For smaller densities, transport is diffusive, and the measured conductivity is reproduced quantitatively, with no fitting parameters, by including electron-hole scattering as the only process causing velocity relaxation. Experiments on a trilayer device show that the phenomenon is robust and that transport at charge neutrality is governed by the same physics. Our results provide a textbook illustration of a transport regime that had not been observed previously and clarify the nature of conduction through charge-neutral graphene under conditions in which carrier density inhomogeneity is immaterial. They also demonstrate that transport can be limited by a fully electronic mechanism, originating from the same microscopic processes that govern the physics of Dirac-like plasmas.

  5. High-voltage pulse generator for electron gun power supply

    International Nuclear Information System (INIS)

    Korenev, S.A.; Enchevich, I.B.; Mikhov, M.K.

    1987-01-01

    High-voltage pulse generator with combined capacitive and inductive energy storages for electron gun power supply is described. Hydrogen thyratron set in a short magnetic lense is a current breaker. Times of current interruption in thyratrons are in the range from 100 to 300 ns. With 1 kV charging voltage of capacitive energy storage 25 kV voltage pulse is obtained in the load. The given high-voltage pulse generator was used for supply of an electron gun generating 10-30 keV low-energy electron beam

  6. Coherent transition radiation from a laser wakefield accelerator as an electron bunch diagnostic

    International Nuclear Information System (INIS)

    Tilborg, J. van; Geddes, C.G.R.; Toth, C.; Esarey, E.; Schroeder, C.B.; Martin, M.C.; Hao, Z.; Leemans, W.P.

    2004-01-01

    The observation and modeling of coherent transition radiation from femtosecond laser accelerated electron bunches is discussed. The coherent transition radiation, scaling quadratically with bunch charge, is generated as the electrons transit the plasma-vacuum boundary. Due to the limited transverse radius of the plasma boundary, diffraction effects will strongly modify the angular distribution and the total energy radiated is reduced compared to an infinite transverse boundary. The multi-nC electron bunches, concentrated in a length of a few plasma periods (several tens of microns), experience partial charge neutralization while propagating inside the plasma towards the boundary. This reduces the space-charge blowout of the beam, allowing for coherent radiation at relatively high frequencies (several THz). The charge distribution of the electron bunch at the plasma-vacuum boundary can be derived from Fourier analysis of the coherent part of the transition radiation spectrum. A Michelson interferometer was used to measure the coherent spectrum, and electron bunches with duration on the order of 50 fs (rms) were observed

  7. Space charge and wake field analysis for a high brightness electron source

    International Nuclear Information System (INIS)

    Parsa, Z.

    1991-01-01

    We present a brief overview of the formalism used, and some simulation results for transverse and longitudinal motion of a bunch of particles moving through a cavity (e.g., the Brookhaven National Laboratory high brightness photocathode gun), including effects of the accelerating field, space charge forces (e.g., arising from the interaction of the cavity surface and the self field of the bunch). 3 refs., 12 figs

  8. Stable electron beams from laser wakefield acceleration with few-terawatt driver using a supersonic air jet

    Science.gov (United States)

    Boháček, K.; Kozlová, M.; Nejdl, J.; Chaulagain, U.; Horný, V.; Krůs, M.; Ta Phuoc, K.

    2018-03-01

    The generation of stable electron beams produced by the laser wakefield acceleration mechanism with a few-terawatt laser system (600 mJ, 50 fs) in a supersonic synthetic air jet is reported and the requirements necessary to build such a stable electron source are experimentally investigated in conditions near the bubble regime threshold. The resulting electron beams have stable energies of (17.4 ± 1.1) MeV and an energy spread of (13.5 ± 1.5) MeV (FWHM), which has been achieved by optimizing the properties of the supersonic gas jet target for the given laser system. Due to the availability of few-terawatt laser systems in many laboratories around the world these stable electron beams open possibilities for applications of this type of particle source.

  9. Model of charge-state distributions for electron cyclotron resonance ion source plasmas

    Directory of Open Access Journals (Sweden)

    D. H. Edgell

    1999-12-01

    Full Text Available A computer model for the ion charge-state distribution (CSD in an electron cyclotron resonance ion source (ECRIS plasma is presented that incorporates non-Maxwellian distribution functions, multiple atomic species, and ion confinement due to the ambipolar potential well that arises from confinement of the electron cyclotron resonance (ECR heated electrons. Atomic processes incorporated into the model include multiple ionization and multiple charge exchange with rate coefficients calculated for non-Maxwellian electron distributions. The electron distribution function is calculated using a Fokker-Planck code with an ECR heating term. This eliminates the electron temperature as an arbitrary user input. The model produces results that are a good match to CSD data from the ANL-ECRII ECRIS. Extending the model to 1D axial will also allow the model to determine the plasma and electrostatic potential profiles, further eliminating arbitrary user input to the model.

  10. Charge transfer in gas electron multipliers

    Energy Technology Data Exchange (ETDEWEB)

    Ottnad, Jonathan; Ball, Markus; Ketzer, Bernhard; Ratza, Viktor; Razzaghi, Cina [HISKP, Bonn University, Nussallee 14-16, D-53115 Bonn (Germany)

    2015-07-01

    In order to efficiently employ a Time Projection Chamber (TPC) at interaction rates higher than ∝1 kHz, as foreseen e.g. in the ALICE experiment (CERN) and at CB-ELSA (Bonn), a continuous operation and readout mode is required. A necessary prerequisite is to minimize the space charge coming from the amplification system and to maintain an excellent spatial and energy resolution. Unfortunately these two goals can be in conflict to each other. Gas Electron Multipliers (GEM) are one candidate to fulfill these requirements. It is necessary to understand the processes within the amplification structure to find optimal operation conditions. To do so, we measure the charge transfer processes in and between GEM foils with different geometries and field configurations, and use an analytical model to describe the results. This model can then be used to predict and optimize the performance. The talk gives the present status of the measurements and describes the model.

  11. Surface structure modification of single crystal graphite after slow, highly charged ion irradiation

    Science.gov (United States)

    Alzaher, I.; Akcöltekin, S.; Ban-d'Etat, B.; Manil, B.; Dey, K. R.; Been, T.; Boduch, P.; Rothard, H.; Schleberger, M.; Lebius, H.

    2018-04-01

    Single crystal graphite was irradiated by slow, highly charged ions. The modification of the surface structure was studied by means of Low-Energy Electron Diffraction. The observed damage cross section increases with the potential energy, i.e. the charge state of the incident ion, at a constant kinetic energy. The potential energy is more efficient for the damage production than the kinetic energy by more than a factor of twenty. Comparison with earlier results hints to a strong link between early electron creation and later target atom rearrangement. With increasing ion fluence, the initially large-scale single crystal is first transformed into μ m-sized crystals, before complete amorphisation takes place.

  12. Charge-exchange-induced formation of hollow atoms in high-intensity laser-produced plasmas

    Energy Technology Data Exchange (ETDEWEB)

    Rosmej, F.B. [TU-Darmstadt, Institut fuer Kernphysik, Darmstadt (Germany); Faenov, A.Ya.; Pikuz, T.A.; Magunov, A.I.; Skobelev, I.Yu. [Multicharged Ions Spectra Data Center of VNIIFTRI, Mendeleevo (Russian Federation); Auguste, T.; D' Oliveira, P.; Hulin, S.; Monot, P. [Commissariat a lEnergie Atomique DSM/DRECAM/SPAM, Gif-Sur-Yvette Cedex (France); Andreev, N.E.; Chegotov, M.V.; Veisman, M.E. [High Energy Density Research Centre, Institute of High Temperatures of Russian Academy of Sciences, Moscow (Russian Federation)

    1999-03-14

    For the first time registration of high-resolution soft x-ray emission and atomic data calculations of hollow-atom dielectronic satellite spectra of highly charged nitrogen have been performed. Double-electron charge-exchange processes from excited states are proposed for the formation of autoionizing levels nln'l' in high-intensity laser-produced plasmas, when field-ionized ions penetrate into the residual gas. Good agreement is found between theory and experiment. Plasma spectroscopy with hollow ions is proposed and a temperature diagnostic for laser-produced plasmas in the long-lasting recombining regime is developed. (author). Letter-to-the-editor.

  13. Photoinduced High-Frequency Charge Oscillations in Dimerized Systems

    Science.gov (United States)

    Yonemitsu, Kenji

    2018-04-01

    Photoinduced charge dynamics in dimerized systems is studied on the basis of the exact diagonalization method and the time-dependent Schrödinger equation for a one-dimensional spinless-fermion model at half filling and a two-dimensional model for κ-(bis[ethylenedithio]tetrathiafulvalene)2X [κ-(BEDT-TTF)2X] at three-quarter filling. After the application of a one-cycle pulse of a specifically polarized electric field, the charge densities at half of the sites of the system oscillate in the same phase and those at the other half oscillate in the opposite phase. For weak fields, the Fourier transform of the time profile of the charge density at any site after photoexcitation has peaks for finite-sized systems that correspond to those of the steady-state optical conductivity spectrum. For strong fields, these peaks are suppressed and a new peak appears on the high-energy side, that is, the charge densities mainly oscillate with a single frequency, although the oscillation is eventually damped. In the two-dimensional case without intersite repulsion and in the one-dimensional case, this frequency corresponds to charge-transfer processes by which all the bonds connecting the two classes of sites are exploited. Thus, this oscillation behaves as an electronic breathing mode. The relevance of the new peak to a recently found reflectivity peak in κ-(BEDT-TTF)2X after photoexcitation is discussed.

  14. Guiding of low-energy electrons by highly ordered Al2 O3 nanocapillaries

    DEFF Research Database (Denmark)

    Milosavljević, A.R.; Víkor, G.; Pešić, Z.D.

    2007-01-01

    We report an experimental study of guided transmission of low-energy (200-350 eV) electrons through highly ordered Al2 O3 nanocapillaries with large aspect ratio (140 nm diameter and 15 μm length). The nanochannel array was prepared using self-ordering phenomena during a two-step anodization...... process of a high-purity aluminum foil. The experimental results clearly show the existence of the guiding effect, as found for highly charged ions. The guiding of the electron beam was observed for tilt angles up to 12°. As seen for highly charged ions, the guiding efficiency increases with decreasing...

  15. Controlling charge injection in organic electronic devices using self-assembled monolayers

    Science.gov (United States)

    Campbell, I. H.; Kress, J. D.; Martin, R. L.; Smith, D. L.; Barashkov, N. N.; Ferraris, J. P.

    1997-12-01

    We demonstrate control and improvement of charge injection in organic electronic devices by utilizing self-assembled monolayers (SAMs) to manipulate the Schottky energy barrier between a metal electrode and the organic electronic material. Hole injection from Cu electrodes into the electroluminescent conjugated polymer poly[2-methoxy,5-(2'-ethyl-hexyloxy)-1,4-phenylene vinylene] was varied by using two conjugated-thiol based SAMs. The chemically modified electrodes were incorporated in organic diode structures and changes in the metal/polymer Schottky energy barriers and current-voltage characteristics were measured. Decreasing (increasing) the Schottky energy barrier improves (degrades) charge injection into the polymer.

  16. Electronic structure and superconductivity of multi-layered organic charge transfer salts

    Energy Technology Data Exchange (ETDEWEB)

    Jeschke, Harald O.; Altmeyer, Michaela; Guterding, Daniel; Valenti, Roser [Institut fuer Theoretische Physik, Goethe-Universitaet Frankfurt, 60438 Frankfurt (Germany)

    2015-07-01

    We examine the electronic properties of polymorphs of (BEDT-TTF){sub 2}Ag(CF{sub 3}){sub 4}(TCE) (1,1,2-trichloroethane) within density functional theory (DFT). While a phase with low superconducting transition temperature T{sub c}=2.6 K exhibits a κ packing motif, two high T{sub c} phases are layered structures consisting of α{sup '} and κ packed layers. We determine the electronic structures and discuss the influence of the insulating α{sup '} layer on the conducting κ layer. In the κ-α{sub 1}{sup '} dual-layered compound, we find that the stripes of high and low charge in the α{sup '} layer correspond to a stripe pattern of hopping parameters in the κ layer. Based on the different underlying Hamiltonians, we study the superconducting properties and try to explain the differences in T{sub c}.

  17. Current feedback operational amplifiers as fast charge sensitive preamplifiers for photomultiplier read out

    Energy Technology Data Exchange (ETDEWEB)

    Giachero, A; Gotti, C; Maino, M; Pessina, G, E-mail: claudio.gotti@mib.infn.it [INFN - Sezione di Milano-Bicocca, I-20126, Milano (Italy)

    2011-05-01

    Fast charge sensitive preamplifiers were built using commercial current feedback operational amplifiers for fast read out of charge pulses from a photomultiplier tube. Current feedback opamps prove to be particularly well suited for this application where the charge from the detector is large, of the order of one million electrons, and high timing resolution is required. A proper circuit arrangement allows very fast signals, with rise times down to one nanosecond, while keeping the amplifier stable. After a review of current feedback circuit topology and stability constraints, we provide a 'recipe' to build stable and very fast charge sensitive preamplifiers from any current feedback opamp by adding just a few external components. The noise performance of the circuit topology has been evaluated and is reported in terms of equivalent noise charge.

  18. High-quality electron beam generation in a proton-driven hollow plasma wakefield accelerator

    Science.gov (United States)

    Li, Y.; Xia, G.; Lotov, K. V.; Sosedkin, A. P.; Hanahoe, K.; Mete-Apsimon, O.

    2017-10-01

    Simulations of proton-driven plasma wakefield accelerators have demonstrated substantially higher accelerating gradients compared to conventional accelerators and the viability of accelerating electrons to the energy frontier in a single plasma stage. However, due to the strong intrinsic transverse fields varying both radially and in time, the witness beam quality is still far from suitable for practical application in future colliders. Here we demonstrate the efficient acceleration of electrons in proton-driven wakefields in a hollow plasma channel. In this regime, the witness bunch is positioned in the region with a strong accelerating field, free from plasma electrons and ions. We show that the electron beam carrying the charge of about 10% of 1 TeV proton driver charge can be accelerated to 0.6 TeV with a preserved normalized emittance in a single channel of 700 m. This high-quality and high-charge beam may pave the way for the development of future plasma-based energy frontier colliders.

  19. Electron-photon and electron-electron interactions in the presence of strong electromagnetic fields

    International Nuclear Information System (INIS)

    Surzhykov, A.; Fritzsche, S.; Stoehlker, Th.

    2010-01-01

    During the last decade, photon emission from highly-charged, heavy ions has been in the focus of intense studies at the GSI accelerator and storage ring facility in Darmstadt. These studies have revealed unique information about the electron-electron and electron-photon interactions in the presence of extremely strong nuclear fields. Apart from the radiative electron capture processes, characteristic photon emission following collisional excitation of projectile ions has also attracted much interest. In this contribution, we summarize the recent theoretical studies on the production of excited ionic states and their subsequent radiative decay. We will pay special attention to the angular and polarization properties of Kα emission from helium-like ions produced by means of dielectronic recombination. The results obtained for this (resonant) capture process will be compared with the theoretical predictions for the characteristic X-rays following Coulomb excitation and radiative recombination of few-electron, heavy ions. Work is supported by Helmholtz Association and GSl under the project VH-NG--421. (author)

  20. Onset of turbulence induced by electron nonthermality in a complex plasma in presence of positively charged dust grains

    Directory of Open Access Journals (Sweden)

    Susmita Sarkar

    2018-03-01

    Full Text Available In this paper onset of turbulence has been detected from the study of non linear dust acoustic wave propagation in a complex plasma considering electrons nonthermal and equilibrium dust charge positive. Dust grains are charged by secondary electron emission process. Our analysis shows that increase in electron nonthermality makes the grain charging process faster by reducing the magnitude of the nonadiabaticity induced pseudo viscosity. Consequently nature of dust charge variation changes from nonadiabatic to adiabatic one. For further increase of electron nonthermality, this pseudo viscosity becomes negative and hence generates a turbulent grain charging behaviour. This turbulent grain charging phenomenon is exclusively the outcome of this nonlinear study which was not found in linear analysis.

  1. Preparation of cold Mg+ion clouds for sympathetic cooling of highly charged ions at SPECTRAP

    International Nuclear Information System (INIS)

    Cazan, Radu Mircea

    2012-02-01

    The bound electrons in hydrogen-like or lithium-like heavy ions experience extremely strong electric and magnetic fields in the surrounding of the nucleus. Laser spectroscopy of the ground-state hyperfine splitting in the lead region provides a sensitive tool to test strong-field quantum electro dynamics (QED), especially in the magnetic sector. Previous measurements on hydrogen-like systems performed in an electron-beam ion trap (EBIT) or at the experimental storage ring (ESR) were experimentally limited in accuracy due to statistics, the large Doppler broadening and the ion energy. The full potential of the QED test can only be exploited if measurements for hydrogen- and lithium-like ions are performed with accuracy improved by 2-3 orders of magnitude. Therefore, the new Penning trap setup SPECTRAP - dedicated for laser spectroscopy on trapped and cooled highly charged ions - is currently commissioned at GSI Darmstadt. Heavy highly charged ions will be delivered to this trap by the HITRAP facility in the future. SPECTRAP is a cylindrical Penning trap with axial access for external ion injection and radial optical access mounted inside a cold-bore superconducting Helmholtz-type split-coil magnet. To reach the targeted accuracy in laser spectroscopy, an efficient and fast cooling process for the highly charged ions must be employed. This can be realized by sympathetic cooling with a cloud of laser-cooled light ions. Within this thesis work, a laser system and an ion source for the production of such a 24 Mg + ion cloud was developed and commissioned at SPECTRAP. An all-solid-state laser system for the generation of 279.6 nm light was designed and built. It consists of a fiber laser at 1118.5 nm followed by frequency quadrupling using two successive second-harmonic generation stages with actively stabilized ring resonators and nonlinear crystals. The laser system can deliver more than 15 mW of UV laser power under optimal conditions and requires little maintenance

  2. Penning traps with unitary architecture for storage of highly charged ions.

    Science.gov (United States)

    Tan, Joseph N; Brewer, Samuel M; Guise, Nicholas D

    2012-02-01

    Penning traps are made extremely compact by embedding rare-earth permanent magnets in the electrode structure. Axially-oriented NdFeB magnets are used in unitary architectures that couple the electric and magnetic components into an integrated structure. We have constructed a two-magnet Penning trap with radial access to enable the use of laser or atomic beams, as well as the collection of light. An experimental apparatus equipped with ion optics is installed at the NIST electron beam ion trap (EBIT) facility, constrained to fit within 1 meter at the end of a horizontal beamline for transporting highly charged ions. Highly charged ions of neon and argon, extracted with initial energies up to 4000 eV per unit charge, are captured and stored to study the confinement properties of a one-magnet trap and a two-magnet trap. Design considerations and some test results are discussed.

  3. Penning traps with unitary architecture for storage of highly charged ions

    International Nuclear Information System (INIS)

    Tan, Joseph N.; Guise, Nicholas D.; Brewer, Samuel M.

    2012-01-01

    Penning traps are made extremely compact by embedding rare-earth permanent magnets in the electrode structure. Axially-oriented NdFeB magnets are used in unitary architectures that couple the electric and magnetic components into an integrated structure. We have constructed a two-magnet Penning trap with radial access to enable the use of laser or atomic beams, as well as the collection of light. An experimental apparatus equipped with ion optics is installed at the NIST electron beam ion trap (EBIT) facility, constrained to fit within 1 meter at the end of a horizontal beamline for transporting highly charged ions. Highly charged ions of neon and argon, extracted with initial energies up to 4000 eV per unit charge, are captured and stored to study the confinement properties of a one-magnet trap and a two-magnet trap. Design considerations and some test results are discussed.

  4. Charging dynamics and strong localization of a two-dimensional electron cloud

    International Nuclear Information System (INIS)

    Dianoux, R; Smilde, H J H; Marchi, F; Buffet, N; Mur, P; Comin, F; Chevrier, J

    2007-01-01

    The dynamics of charge injection in silicon nanocrystals embedded in a silicon dioxide matrix is studied using electrostatic force microscopy. We show that the presence of silicon nanocrystals with a density of 10 11 cm -2 is essential for strong localization of charges, and results in exceptional charge retention properties compared to nanocrystal-free SiO 2 samples. In both systems, a logarithmic dependence of the diameter of the charged area on the injection time is experimentally observed on a timescale between 0.1 and 10 s (voltage≤10 V). A field-emission injection, limited by Coulomb blockade and a lateral charge spreading due to a repulsive radial electric field are used to model the sample charging. Once the tip is retracted, the electron cloud is strongly confined in the nanocrystals and remains static

  5. Laser-driven strong magnetostatic fields with applications to charged beam transport and magnetized high energy-density physics

    Science.gov (United States)

    Santos, Joao

    2017-10-01

    Powerful laser-plasma processes are explored to generate discharge currents of a few 100 kA in coil targets, yielding magnetostatic fields (B-fields) in the kTesla range. The B-fields are measured by proton-deflectometry and high-frequency bandwidth B-dot probes. According to our modeling, the quasi-static currents are provided from hot electron ejection from the laser-irradiated surface, accounting for the space charge neutralization and the plasma magnetization. The major control parameter is the laser irradiance Iλ2 . The B-fields ns-scale is long enough to magnetize secondary targets through resistive diffusion. We applied it in experiments of laser-generated relativistic electron transport into solid dielectric targets, yielding an unprecedented enhancement of a factor 5 on the energy-density flux at 60 µm depth, compared to unmagnetized transport conditions. These studies pave the ground for magnetized high-energy density physics investigations, related to laser-generated secondary sources of radiation and/or high-energy particles and their transport, to high-gain fusion energy schemes and to laboratory astrophysics. We acknowledge funding from French National Agency for Research (ANR), Grant TERRE ANR-2011-BS04-014, and from EUROfusion Consortium, European Union's Horizon 2020 research and innovation programme, Grant 633053.

  6. Transverse acceptance calculation for continuous ion beam injection into the electron beam ion trap charge breeder of the ReA post-accelerator

    Energy Technology Data Exchange (ETDEWEB)

    Kittimanapun, K., E-mail: kritsadak@slri.or.th [National Superconducting Cyclotron Laboratory (NSCL), Michigan State University (MSU), 640 S. Shaw Lane, East Lansing, Michigan 48824 (United States); Synchrotron Light Research Institute (SLRI), 111 University Avenue, Muang District, Nakhon Ratchasima, 30000 (Thailand); Baumann, T.M.; Lapierre, A.; Schwarz, S. [National Superconducting Cyclotron Laboratory (NSCL), Michigan State University (MSU), 640 S. Shaw Lane, East Lansing, Michigan 48824 (United States); Bollen, G. [National Superconducting Cyclotron Laboratory (NSCL), Michigan State University (MSU), 640 S. Shaw Lane, East Lansing, Michigan 48824 (United States); Facility for Rare Isotope Beams (FRIB), Michigan State University, 640 S. Shaw Lane, East Lansing, Michigan 48824 (United States)

    2015-11-11

    The ReA post-accelerator at the National Superconducting Cyclotron Laboratory (NSCL) employs an electron beam ion trap (EBIT) as a charge breeder. A Monte-Carlo simulation code was developed to calculate the transverse acceptance phase space of the EBIT for continuously injected ion beams and to determine the capture efficiency in dependence of the transverse beam emittance. For this purpose, the code records the position and time of changes in charge state of injected ions, leading either to capture or loss of ions. To benchmark and validate the code, calculated capture efficiencies were compared with results from a geometrical model and measurements. The results of the code agree with the experimental findings within a few 10%. The code predicts a maximum total capture efficiency of 50% for EBIT parameters readily achievable and an efficiency of up to 80% for an electron beam current density of 1900 A/cm{sup 2}.

  7. Evidence for charge exchange effects in electronic excitations in Al by slow singly charged He ions

    Energy Technology Data Exchange (ETDEWEB)

    Riccardi, P., E-mail: Pierfrancesco.riccardi@fis.unical.it [Dipartimento di Fisica, Università della Calabria and INFN Gruppo collegato di Cosenza, Via P. Bucci cubo 31C, 87036 – Arcavacata di Rende, Cosenza (Italy); Sindona, A. [Dipartimento di Fisica, Università della Calabria and INFN Gruppo collegato di Cosenza, Via P. Bucci cubo 31C, 87036 – Arcavacata di Rende, Cosenza (Italy); Dukes, C.A. [Laboratory for Astrophysics and Surface Physics, Materials Science and Engineering, University of Virginia, Charlottesville, Virginia 22904 (United States)

    2016-09-01

    We report on experiments of secondary electron emission in the interaction of helium ions with aluminum surfaces. Comparison between the electron emission induced by the impact of {sup 3}He{sup +} and {sup 4}He{sup +} on Al illustrates similarities and differences between the two projectiles. The intensity of emission shows the same dependence on velocity for the two isotopes, showing that KEE yields for helium ions impact on Al are dominated by direct excitation of valence electrons and not by electron promotion. Electron promotion and charge transfer processes are unambiguously identified by the observation of Auger electron emission from Al, at energies below the excitation threshold of Al–Al collisions, indicating energy losses for the projectiles higher than those commonly considered.

  8. Electron Electric Dipole Moment from CP Violation in the Charged Higgs Sector

    International Nuclear Information System (INIS)

    Bowser-Chao, D.; Keung, W.; Chang, D.; Chang, D.

    1997-01-01

    The leading contributions to the electron (or muon) electric dipole moment due to CP violation in the charged Higgs sector are at the two level. A careful model-independent analysis of the heavy fermion contribution is provided. We also consider some specific scenarios to demonstrate how charged Higgs sector CP violation can naturally give rise to large electric dipole moments. Numerical results show that the electron electric dipole moment in such models can lie at the experimentally accessible level. copyright 1997 The American Physical Society

  9. Search for excited charged leptons in electron positron collisions

    CERN Document Server

    Vachon, Brigitte Marie Christine; Sobie, Randall

    2002-01-01

    A search for evidence that fundamental particles are made of smaller subconstituents is performed. The existence of excited states of fundamental particles would be an unambiguous indication of their composite nature. Experimental signatures compatible with the production of excited states of charged leptons in electron-positron collisions are studied. The data analysed were collected by the OPAL detector at the LEP collider. No evidence for the existence of excited states of charged leptons was found. Upper limits on the product of the cross-section and the electromagnetic branching fraction are inferred. Using results from the search for singly produced excited leptons, upper limits on the ratio of the excited lepton coupling constant to the compositeness scale are calculated. From pair production searches, 95% confidence level lower limits on the masses of excited electrons, muons and taus are determined to be 103.2 GeV.

  10. Few-body strange systems

    International Nuclear Information System (INIS)

    Gibson, B.F.

    1985-01-01

    Three fascinating aspects of few-body Λ-hypernuclei are discussed: 3-body forces, charge symmetry breaking, and ΛN-ΣN coupling. The need for improved data on hyperon-nucleon scattering is emphasized. 29 refs., 3 tabs

  11. Energy loss of a high charge bunched electron beam in plasma: Simulations, scaling, and accelerating wakefields

    Directory of Open Access Journals (Sweden)

    J. B. Rosenzweig

    2004-06-01

    Full Text Available The energy loss and gain of a beam in the nonlinear, “blowout” regime of the plasma wakefield accelerator, which features ultrahigh accelerating fields, linear transverse focusing forces, and nonlinear plasma motion, has been asserted, through previous observations in simulations, to scale linearly with beam charge. Additionally, from a recent analysis by Barov et al., it has been concluded that for an infinitesimally short beam, the energy loss is indeed predicted to scale linearly with beam charge for arbitrarily large beam charge. This scaling is predicted to hold despite the onset of a relativistic, nonlinear response by the plasma, when the number of beam particles occupying a cubic plasma skin depth exceeds that of plasma electrons within the same volume. This paper is intended to explore the deviations from linear energy loss using 2D particle-in-cell simulations that arise in the case of experimentally relevant finite length beams. The peak accelerating field in the plasma wave excited behind the finite-length beam is also examined, with the artifact of wave spiking adding to the apparent persistence of linear scaling of the peak field amplitude into the nonlinear regime. At large enough normalized charge, the linear scaling of both decelerating and accelerating fields collapses, with serious consequences for plasma wave excitation efficiency. Using the results of parametric particle-in-cell studies, the implications of these results for observing severe deviations from linear scaling in present and planned experiments are discussed.

  12. Characterization of Cs-Sb cathodes for high charge RF photoinjectors

    CERN Document Server

    AUTHOR|(CDS)2082505; Beghi, Marco

    Future accelerators such as CLIC (Compact LInear Collider), require high brightness electron beams that could be produced with a photoinjector (laser-driven electron source). Cs2Te photocathodes in combination with ultra-violet (UV) laser beams are currently used in many photoinjector facilities, but requirements to the electron sources for future accelerators like CLIC are more demanding. The main challenge for the CLIC drive beam photoinjector is to achieve high bunch charges (8.4 nC), high bunch repetition rates (500 MHz) within long trains (140 s) and with suciently long cathode lifetimes. In particular the laser pulse energy in UV, for such long pulse trains, is currently limited due to a degradation of the beam quality during the 4th harmonic frequency conversion process. Using the 2nd harmonic (green laser beam), provided it is matched with a low photoemission threshold photocathode material, would overcome this limitation. Cesium antimonide (Cs3Sb), being a photoemissive material in the visible range,...

  13. Measuring the Weak Charge of the Proton via Elastic Electron-Proton Scattering

    Energy Technology Data Exchange (ETDEWEB)

    Jones, Donald C. [Univ. of Virginia, Charlottesville, VA (United States)

    2015-10-01

    The Qweak experiment which ran in Hall C at Jefferson Lab in Newport News, VA, and completed data taking in May 2012, measured the weak charge of the proton QpW via elastic electron-proton scattering. Longitudinally polarized electrons were scattered from an unpolarized liquid hydrogen target. The helicity of the electron beam was flipped at approximately 1 kHz between left and right spin states. The Standard Model predicts a small parity-violating asymmetry of scattering rates between right and left helicity states due to the weak interaction. An initial result using 4% of the data was published in October 2013 [1] with a measured parity-violating asymmetry of -279 ± 35(stat) ± 31 (syst) ppb. This asymmetry, along with other data from parity-violating electron scattering experiments, provided the world's first determination of the weak charge of the proton. The weak charge of the proton was found to be pW = 0.064 ± 0.012, in good agreement with the Standard Model prediction of pW(SM) = 0.0708 ± 0.0003[2].

  14. Catastrophic processes in dielectrics in irradiation by high-current electron beams

    Energy Technology Data Exchange (ETDEWEB)

    Oleshko, V. [Tomsk Polytechnic University, 634050 Tomsk (Russian Federation); Lisitsyna, L., E-mail: lisitsyn@tpu.r [Tomsk State University of Architecture and Building, 634003 Tomsk (Russian Federation); Malys, D.; Damamme, G. [Commissariat a l' energie atomique, Paris 75015 (France); Lisitsyn, V. [Tomsk Polytechnic University, 634050 Tomsk (Russian Federation)

    2010-10-01

    The results of the research in explosive decomposition of heavy metal azides initiated by electric ('streamer') charges induced by high-current electron beam have been considered. A physical model for initiation of heavy metal azides explosive decomposition by electron beam has been suggested. The model suggests formation of strong electric field in the sample and its neutralization by ultrasound anode charges. The streamer front generates 'hot spots' which start the formation of explosive decomposition sites in a condensed reactive material.

  15. Highly charged ions generated with intense laser beams

    Czech Academy of Sciences Publication Activity Database

    Krása, Josef; Jungwirth, Karel; Králiková, Božena; Láska, Leoš; Pfeifer, Miroslav; Rohlena, Karel; Skála, Jiří; Ullschmied, Jiří; Hnatowicz, Vladimír; Peřina, Vratislav; Badziak, J.; Parys, P.; Wolowski, J.; Woryna, E.; Szydlowski, A.

    2003-01-01

    Roč. 205, - (2003), s. 355-359 ISSN 0168-583X. [International Symposium on Swift Heavy Ions in Matter /5./. Taormina-Giardini Naxos, 22.05.2002-25.05.2002] R&D Projects: GA MŠk LN00A100 Grant - others:HPRI(XE) CT-1999-00053; IAEA(XE) 11535/RO Institutional research plan: CEZ:AV0Z2043910; CEZ:AV0Z1010921 Keywords : laser-produced plasma * highly charged ions * ion implantation * windowless electron multiplier Subject RIV: BH - Optics, Masers, Lasers Impact factor: 1.041, year: 2003

  16. Revealing the ultrafast charge carrier dynamics in organo metal halide perovskite solar cell materials using time resolved THz spectroscopy

    Science.gov (United States)

    Ponseca, C. S., Jr.; Sundström, V.

    2016-03-01

    Ultrafast charge carrier dynamics in organo metal halide perovskite has been probed using time resolved terahertz (THz) spectroscopy (TRTS). Current literature on its early time characteristics is unanimous: sub-ps charge carrier generation, highly mobile charges and very slow recombination rationalizing the exceptionally high power conversion efficiency for a solution processed solar cell material. Electron injection from MAPbI3 to nanoparticles (NP) of TiO2 is found to be sub-ps while Al2O3 NPs do not alter charge dynamics. Charge transfer to organic electrodes, Spiro-OMeTAD and PCBM, is sub-ps and few hundreds of ps respectively, which is influenced by the alignment of energy bands. It is surmised that minimizing defects/trap states is key in optimizing charge carrier extraction from these materials.

  17. C library for topological study of the electronic charge density.

    Science.gov (United States)

    Vega, David; Aray, Yosslen; Rodríguez, Jesús

    2012-12-05

    The topological study of the electronic charge density is useful to obtain information about the kinds of bonds (ionic or covalent) and the atom charges on a molecule or crystal. For this study, it is necessary to calculate, at every space point, the electronic density and its electronic density derivatives values up to second order. In this work, a grid-based method for these calculations is described. The library, implemented for three dimensions, is based on a multidimensional Lagrange interpolation in a regular grid; by differentiating the resulting polynomial, the gradient vector, the Hessian matrix and the Laplacian formulas were obtained for every space point. More complex functions such as the Newton-Raphson method (to find the critical points, where the gradient is null) and the Cash-Karp Runge-Kutta method (used to make the gradient paths) were programmed. As in some crystals, the unit cell has angles different from 90°, the described library includes linear transformations to correct the gradient and Hessian when the grid is distorted (inclined). Functions were also developed to handle grid containing files (grd from DMol® program, CUBE from Gaussian® program and CHGCAR from VASP® program). Each one of these files contains the data for a molecular or crystal electronic property (such as charge density, spin density, electrostatic potential, and others) in a three-dimensional (3D) grid. The library can be adapted to make the topological study in any regular 3D grid by modifying the code of these functions. Copyright © 2012 Wiley Periodicals, Inc.

  18. Tuning charge balance in PHOLEDs with ambipolar host materials to achieve high efficiency

    International Nuclear Information System (INIS)

    Padmaperuma, Asanga B.; Koech, Phillip K.; Cosimbescu, Lelia; Polikarpov, Evgueni; Swensen, James S.; Chopra, Neetu; So, Franky; Sapochak, Linda S.; Gaspar, Daniel J.

    2009-01-01

    The efficiency and stability of blue organic light emitting devices (OLEDs) continue to be a primary roadblock to developing organic solid state white lighting. For OLEDs to meet the high power conversion efficiency goal, they will require both close to 100% internal quantum efficiency and low operating voltage in a white light emitting device. It is generally accepted that such high quantum efficiency, can only be achieved with the use of organometallic phosphor doped OLEDs. Blue OLEDs are particularly important for solid state lighting. The simplest (and therefore likely the lowest cost) method of generating white light is to down convert part of the emission from a blue light source with a system of external phosphors. A second method of generating white light requires the superposition of the light from red, green and blue OLEDs in the correct ratio. Either of these two methods (and indeed any method of generating white light with a high color rendering index) critically depends on a high efficiency blue light component. A simple OLED generally consists of a hole-injecting anode, a preferentially hole transporting organic layer (HTL), an emissive layer that contains the recombination zone and ideally transports both holes and electrons, a preferentially electron-transporting layer (ETL) and an electron-injecting cathode. Color in state-of-the-art OLEDs is generated by an organometallic phosphor incorporated by co-sublimation into the emissive layer (EML). New materials functioning as hosts, emitters, charge transporting, and charge blocking layers have been developed along with device architectures leading to electrophosphorescent based OLEDs with high quantum efficiencies near the theoretical limit. However, the layers added to the device architecture to enable high quantum efficiencies lead to higher operating voltages and correspondingly lower power efficiencies. Achievement of target luminance power efficiencies will require new strategies for lowering

  19. ERC sources for the production of highly charged ions (invited)

    International Nuclear Information System (INIS)

    Lyneis, C.M.; Antaya, T.A.

    1990-01-01

    Electron cyclotron resonance ion sources (ECRIS) using rf between 5 and 16 GHz have been developed into stable, reliable sources of highly charged ions produced from a wide range of elements. These devices are currently used as ion sources for cyclotrons, synchrotrons, and heavy-ion linacs for nuclear and relativistic heavy-ion physics. They also serve the atomic physics community as a source of low energy multiply charged ions. In order to improve their performance both with respect to maximum charge state and beam intensity, ECRIS builders are now designing and constructing sources which will operate at frequencies up to 30 GHz. In this article we review the present status of operating ECRIS, review recent experimental measurements on plasma parameters, and look at the technology and potential of sources operating at frequencies up to 30 GHz

  20. Prospects for Parity Non-conservation Experiments with Highly Charged Heavy Ions

    OpenAIRE

    Maul, M.; Schäfer, A.; Greiner, W.; Indelicato, P.

    1996-01-01

    We discuss the prospects for parity non-conservation experiments with highly charged heavy ions. Energy levels and parity mixing for heavy ions with two to five electrons are calculated. We investigate two-photon-transitions and the possibility to observe interference effects between weak-matrix elements and Stark matrix elements for periodic electric field configurations.

  1. Single-electron charging effects and implications for tunneling measurements of the high-T/sub c/ superconductors

    International Nuclear Information System (INIS)

    Barner, J.B.; Honkanen, M.J.; Ruggiero, S.T.; Mullen, K.; Ben-Jacob, E.; Pelton, A.R.; Michigan Univ., Ann Arbor, MI

    1989-01-01

    The authors present a theory for the dynamics of two voltage-biased, ultra-small-capacitance tunnel junctions connected in series when one or more electrodes are superconducting and experiments performed on parallel arrays of such junctions. Using the semiclassical model, they find that the I-V characteristics display steps and therefore multiple peaks in dI/dV, corresponding to the time-average occupation of the interjunction region by integral numbers of electrons. The voltage at which the first step is located depends on the superconducting gap, Δ(T), and the capacitances of the junctions. The spacing between subsequent steps depends solely on the capacitances. They discuss electron tunneling results performed on metal/Al/sub 2/O/sub 3//2-10 nm-diameter metal particles/Al/sub 2/O/sub 3//metal junctions where this multiple-peak structure is observed. They present preliminary tunneling results in junctions employing Pb-particles, where they observe a shift of the peaks when the sample is cooled below T/sub c/ of Pb consistent with theory. Taken together, these results indicate that the multiple-peak structure commonly observed in tunneling data of high-T/sub c/ oxide superconductors can be explained in terms of charging effects in a material with a single superconducting gap. Finally, they discuss possible applications in a new type of transistor element

  2. Controlling charge injection in organic electronic devices using self-assembled monolayers

    Energy Technology Data Exchange (ETDEWEB)

    Campbell, I.H.; Kress, J.D.; Martin, R.L.; Smith, D.L. [Los Alamos National Laboratory, Los Alamos, New Mexico 87545 (United States); Barashkov, N.N.; Ferraris, J.P. [The University of Texas at Dallas, Richardson, Texas 75083 (United States)

    1997-12-01

    We demonstrate control and improvement of charge injection in organic electronic devices by utilizing self-assembled monolayers (SAMs) to manipulate the Schottky energy barrier between a metal electrode and the organic electronic material. Hole injection from Cu electrodes into the electroluminescent conjugated polymer poly[2-methoxy,5-(2{sup {prime}}-ethyl-hexyloxy)-1,4-phenylene vinylene] was varied by using two conjugated-thiol based SAMs. The chemically modified electrodes were incorporated in organic diode structures and changes in the metal/polymer Schottky energy barriers and current{endash}voltage characteristics were measured. Decreasing (increasing) the Schottky energy barrier improves (degrades) charge injection into the polymer. {copyright} {ital 1997 American Institute of Physics.}

  3. KEKCB electron cyclotron resonance charge breeder at TRIAC

    International Nuclear Information System (INIS)

    Imai, N.; Jeong, S. C.; Oyaizu, M.; Arai, S.; Fuchi, Y.; Hirayama, Y.; Ishiyama, H.; Miyatake, H.; Tanaka, M. H.; Okada, M.; Watanabe, Y. X.; Ichikawa, S.; Kabumoto, H.; Osa, A.; Otokawa, Y.; Sato, T. K.

    2008-01-01

    The KEKCB is an electron cyclotron resonance (ECR) ion source for converting singly charged ions to multicharged ones at Tokai Radioactive Ion Accelerator Complex. By using the KEKCB, singly charged gaseous and nongaseous ions were converted to multicharged ones of A/q≅7 with efficiencies of 7% and 2%, respectively. The conversion efficiency was found to be independent of the lifetime of the radioactive nuclei having lifetimes of the order of one second. Three collimators located at the entrance and the exit of the KEKCB defined the beam axis and facilitated beam injection. Grinding and washing the surfaces of aluminum electrode and plasma chamber dramatically reduced impurities originating from the ECR plasma of the KEKCB

  4. Quantum–classical simulations of the electronic stopping force and charge on slow heavy channelling ions in metals

    International Nuclear Information System (INIS)

    Race, C P; Mason, D R; Foo, M H F; Foulkes, W M C; Sutton, A P; Horsfield, A P

    2013-01-01

    By simulating the passage of heavy ions along open channels in a model crystalline metal using semi-classical Ehrenfest dynamics we directly investigate the nature of non-adiabatic electronic effects. Our time-dependent tight-binding approach incorporates both an explicit quantum mechanical electronic system and an explicit representation of a set of classical ions. The coupled evolution of the ions and electrons allows us to explore phenomena that lie beyond the approximations made in classical molecular dynamics simulations and in theories of electronic stopping. We report a velocity-dependent charge-localization phenomenon not predicted by previous theoretical treatments of channelling. This charge localization can be attributed to the excitation of electrons into defect states highly localized on the channelling ion. These modes of excitation only become active when the frequency at which the channelling ion moves from interstitial point to equivalent interstitial point matches the frequency corresponding to excitations from the Fermi level into the localized states. Examining the stopping force exerted on the channelling ion by the electronic system, we find broad agreement with theories of slow ion stopping (a stopping force proportional to velocity) for a low velocity channelling ion (up to about 0.5 nm fs −1 from our calculations), and a reduction in stopping power attributable to the charge localization effect at higher velocities. By exploiting the simplicity of our electronic structure model we are able to illuminate the physics behind the excitation processes that we observe and present an intuitive picture of electronic stopping from a real-space, chemical perspective. (paper)

  5. Spectroscopic Investigations of Highly Charged Tungsten Ions - Atomic Spectroscopy and Fusion Plasma Diagnostics

    Energy Technology Data Exchange (ETDEWEB)

    Clementson, Joel [Lund Univ. (Sweden)

    2010-05-01

    The spectra of highly charged tungsten ions have been investigated using x-ray and extreme ultraviolet spectroscopy. These heavy ions are of interest in relativistic atomic structure theory, where high-precision wavelength measurements benchmark theoretical approaches, and in magnetic fusion research, where the ions may serve to diagnose high-temperature plasmas. The work details spectroscopic investigations of highly charged tungsten ions measured at the Livermore electron beam ion trap (EBIT) facility. Here, the EBIT-I and SuperEBIT electron beam ion traps have been employed to create, trap, and excite tungsten ions of M- and L-shell charge states. The emitted spectra have been studied in high resolution using crystal, grating, and x-ray calorimeter spectrometers. In particular, wavelengths of n = 0 M-shell transitions in K-like W55+ through Ne-like W64+, and intershell transitions in Zn-like W44+ through Co-like W47+ have been measured. Special attention is given to the Ni-like W46+ ion, which has two strong electric-dipole forbidden transitions that are of interest for plasma diagnostics. The EBIT measurements are complemented by spectral modeling using the Flexible Atomic Code (FAC), and predictions for tokamak spectra are presented. The L-shell tungsten ions have been studied at electron-beam energies of up to 122 keV and transition energies measured in Ne-like W64+ through Li-like W71+. These spectra constitute the physics basis in the design of the ion-temperature crystal spectrometer for the ITER tokamak. Tungsten particles have furthermore been introduced into the Sustained Spheromak Physics Experiment (SSPX) spheromak in Livermore in order to investigate diagnostic possibilities of extreme ultraviolet tungsten spectra for the ITER divertor. The spheromak measurement and spectral modeling using FAC suggest that tungsten ions in charge states around Er-like W6+ could be useful for

  6. Efficient charge generation by relaxed charge-transfer states at organic interfaces

    KAUST Repository

    Vandewal, Koen

    2013-11-17

    Interfaces between organic electron-donating (D) and electron-accepting (A) materials have the ability to generate charge carriers on illumination. Efficient organic solar cells require a high yield for this process, combined with a minimum of energy losses. Here, we investigate the role of the lowest energy emissive interfacial charge-transfer state (CT1) in the charge generation process. We measure the quantum yield and the electric field dependence of charge generation on excitation of the charge-transfer (CT) state manifold via weakly allowed, low-energy optical transitions. For a wide range of photovoltaic devices based on polymer:fullerene, small-molecule:C60 and polymer:polymer blends, our study reveals that the internal quantum efficiency (IQE) is essentially independent of whether or not D, A or CT states with an energy higher than that of CT1 are excited. The best materials systems show an IQE higher than 90% without the need for excess electronic or vibrational energy. © 2014 Macmillan Publishers Limited.

  7. Efficient charge generation by relaxed charge-transfer states at organic interfaces

    KAUST Repository

    Vandewal, Koen; Albrecht, Steve N.; Hoke, Eric T.; Graham, Kenneth; Widmer, Johannes; Douglas, Jessica D.; Schubert, Marcel; Mateker, William R.; Bloking, Jason T.; Burkhard, George F.; Sellinger, Alan; Frechet, Jean; Amassian, Aram; Riede, Moritz Kilian; McGehee, Michael D.; Neher, Dieter; Salleo, Alberto

    2013-01-01

    Interfaces between organic electron-donating (D) and electron-accepting (A) materials have the ability to generate charge carriers on illumination. Efficient organic solar cells require a high yield for this process, combined with a minimum of energy losses. Here, we investigate the role of the lowest energy emissive interfacial charge-transfer state (CT1) in the charge generation process. We measure the quantum yield and the electric field dependence of charge generation on excitation of the charge-transfer (CT) state manifold via weakly allowed, low-energy optical transitions. For a wide range of photovoltaic devices based on polymer:fullerene, small-molecule:C60 and polymer:polymer blends, our study reveals that the internal quantum efficiency (IQE) is essentially independent of whether or not D, A or CT states with an energy higher than that of CT1 are excited. The best materials systems show an IQE higher than 90% without the need for excess electronic or vibrational energy. © 2014 Macmillan Publishers Limited.

  8. Solar photovoltaic charging of high voltage nickel metal hydride batteries using DC power conversion

    Science.gov (United States)

    Kelly, Nelson A.; Gibson, Thomas L.

    There are an increasing number of vehicle choices available that utilize batteries and electric motors to reduce tailpipe emissions and increase fuel economy. The eventual production of electricity and hydrogen in a renewable fashion, such as using solar energy, can achieve the long-term vision of having no tailpipe environmental impact, as well as eliminating the dependence of the transportation sector on dwindling supplies of petroleum for its energy. In this report we will demonstrate the solar-powered charging of the high-voltage nickel-metal hydride (NiMH) battery used in the GM 2-mode hybrid system. In previous studies we have used low-voltage solar modules to produce hydrogen via the electrolysis of water and to directly charge lithium-ion battery modules. Our strategy in the present work was to boost low-voltage PV voltage to over 300 V using DC-DC converters in order to charge the high-voltage NiMH battery, and to regulate the battery charging using software to program the electronic control unit supplied with the battery pack. A protocol for high-voltage battery charging was developed, and the solar to battery charging efficiency was measured under a variety of conditions. We believe this is the first time such high-voltage batteries have been charged using solar energy in order to prove the concept of efficient, solar-powered charging for battery-electric vehicles.

  9. Few-layered MnO2/SWCNT hybrid in-plane supercapacitor with high energy density

    Science.gov (United States)

    Dutta, Shibsankar; Pal, Shreyasi; De, Sukanta

    2018-05-01

    In this present work we have synthesized few layered MnO2 nanosheets by mixed solvent exfoliation process for the application as electrode material of in-plane supercapacitor. The Structure and surface morphology of the as prepared samples are characterized by Raman, Transmission electron microscopy and Scanning electron microscopy. The patterns of the hybrids were directly fabricated by (50: 50 wt %) mixture of MnO2 and SWCNT dispersions with the help of a customized mask, and directly transferred onto a flexible PET substrate. Remarkably, the prepared in-plane supercapacitors deliver high energy density of 2.62mWh/cm2. Furthermore, our supercapacitors shows exceptional flexibility and stable performance under bending conditions

  10. Effect of electrode for producing the highly charged heavy ions from RIKEN 18 GHz electron cyclotron resonance ion source

    International Nuclear Information System (INIS)

    Kurita, Tetsuro; Nakagawa, Takahide; Kidera, Masanori

    1999-01-01

    We successfully produced the intense beam of highly charged Kr ions using an electrode. Under the pulsed mode operation, we found that the depth of the plasma potential dip strongly depends on the duration of the microwave and takes about 40 ms to reach the equilibrium state. Taking these results into account, we compared the beam intensities of highly charged Kr ions with and without the use of an electrode under the pulsed mode operation. We observed that the density of highly charged Kr ions and ion confinement time increase with increasing mirror magnetic field strength. The plasma potential dip becomes shallower with insertion of the electrode. Consequently, when we increase the mirror magnetic field strength and insert the electrode into the plasma, the beam intensities of highly charged ions increase. (author)

  11. On the possibility of gamma-laser pumping occurring at a charged particle counter motion and in density-modulated electron beams by a high frequency intensive radiation

    International Nuclear Information System (INIS)

    Maksyuta, N.V.

    1999-01-01

    The given report deals with the problem of motion and radiation of relativistic electron in a field of opposite plane density-modulated relativistic electron beam. Physical essence of high-frequency intensive radiation origin could be explained, first by the additional Lorentz reduction of the electron beam modulation period (modulation period Λ in a laboratory co-ordinate system reduces by a factor γ as compared with the modulation period in a beam co-ordinate system) and, secondly, a simultaneous γ-fold increase of transverse components of relativistic electrons of the beam electric and magnetic fields. Such a moving modulated electron beam can be regarded as a dynamic micro-ondulator. Unlike static micro-ondulators we can observe here one more positive moment along with a small period Λ = Λ'/γ, i.e. the electric and magnetic fields in a transverse direction are changed according to the law of exp(-2πx/Λ'). It means that charged particle interaction with a dynamic micro-ondulator will be effective in a wide range of transverse distances, i.e., to get an intensive short wave radiation one can use charged particle beams with rather large apertures which leads to an additional radiation intensity increase. A discussion is given showing that the proposed dynamic modulator possesses some essential merits. A detailed calculation is presented. (author)

  12. The character of resonant charge exchange involving highly excited atoms

    International Nuclear Information System (INIS)

    Kosarim, A. V.; Smirnov, B. M.; Capitelli, M.; Laricchiuta, A.

    2012-01-01

    We study the process of resonant charge exchange involving excited helium atoms with the principal quantum number n = 5 colliding with the helium ion in the ground state in the collision energy range from thermal up to 10 eV. This information may be important for the analysis of planet atmospheres containing helium, in particular, for Jupiter’s atmosphere, but our basic interest is the transition from the quantum to classical description of this process, where, due to large cross sections, evaluations of the cross sections are possible. For the chosen process, quantum theory allows determining the cross section as a result of a tunnel electron transition, while classical theory accounts for over-barrier electron transitions. The classical theory additionally requires effective transitions between states with close energies. The analysis of these transitions for helium with n = 5 shows that electron momenta and their projections are mixed for a part of the states, while for other states, the mixing is absent. A simple criterion to separate such states is given. In addition, the main contribution to the cross section of resonant charge exchange follows from tunnel electron transitions. As a result, the quantum theory is better for calculating the cross sections of resonant charge exchange than the classical one and also allows finding the partial cross sections of resonant charge exchange, while the classical approach gives the cross section of resonant charge exchange in a simple manner with the accuracy of 20%.

  13. Liouville master equation for multielectron dynamics: Neutralization of highly charged ions near a LiF surface

    International Nuclear Information System (INIS)

    Wirtz, Ludger; Reinhold, Carlos O.; Lemell, Christoph; Burgdoerfer, Joachim

    2003-01-01

    We present a simulation of the neutralization of highly charged ions in front of a lithium fluoride surface including the close-collision regime above the surface. The present approach employs a Monte Carlo solution of the Liouville master equation for the joint probability density of the ionic motion and the electronic population of the projectile and the target surface. It includes single as well as double particle-hole (de)excitation processes and incorporates electron correlation effects through the conditional dynamics of population strings. The input in terms of elementary one- and two-electron transfer rates is determined from classical trajectory Monte Carlo calculations as well as quantum-mechanical Auger calculations. For slow projectiles and normal incidence, the ionic motion depends sensitively on the interplay between image acceleration towards the surface and repulsion by an ensemble of positive hole charges in the surface ('trampoline effect'). For Ne 10+ we find that image acceleration is dominant and no collective backscattering high above the surface takes place. For grazing incidence, our simulation delineates the pathways to complete neutralization. In accordance with recent experimental observations, most ions are reflected as neutral or even as singly charged negative particles, irrespective of the charge state of the incoming ions

  14. Tuning of few-electron states and optical absorption anisotropy in GaAs quantum rings.

    Science.gov (United States)

    Wu, Zhenhua; Li, Jian; Li, Jun; Yin, Huaxiang; Liu, Yu

    2017-11-15

    The electronic and optical properties of a GaAs quantum ring (QR) with few electrons in the presence of the Rashba spin-orbit interaction (RSOI) and the Dresselhaus spin-orbit interaction (DSOI) have been investigated theoretically. The configuration interaction (CI) method is employed to calculate the eigenvalues and eigenstates of the multiple-electron QR accurately. Our numerical results demonstrate that the symmetry breaking induced by the RSOI and DSOI leads to an anisotropic distribution of multi-electron states. The Coulomb interaction offers additional modulation of the electron distribution and thus the optical absorption indices in the quantum rings. By tuning the magnetic/electric fields and/or electron numbers in a quantum ring, one can change its optical properties significantly. Our theory provides a new way to control the multi-electron states and optical properties of a QR by hybrid modulations or by electrical means only.

  15. Charge transport through image charged stabilized states in a single molecule single electron transistor device

    International Nuclear Information System (INIS)

    Hedegard, Per; Bjornholm, Thomas

    2005-01-01

    The present paper gives an elaborate theoretical description of a new molecular charge transport mechanism applying to a single molecule trapped between two macroscopic electrodes in a solid state device. It is shown by a Hubbard type model of the electronic and electrostatic interactions, that the close proximity of metal electrodes may allow electrons to tunnel from the electrode directly into very localized image charge stabilized states on the molecule. Due to this mechanism, an exceptionally large number of redox states may be visited within an energy scale which would normally not allow the molecular HOMO-LUMO gap to be transversed. With a reasonable set of parameters, a good fit to recent experimental values may be obtained. The theoretical model is furthermore used to search for the physical boundaries of this effect, and it is found that a rather narrow geometrical space is available for the new mechanism to work: in the specific case of oligophenylenevinylene molecules recently explored in such devices several atoms in the terminal benzene rings need to be at van der Waal's distance to the electrode in order for the mechanism to work. The model predicts, that chemisorption of the terminal benzene rings too gold electrodes will impede the image charge effect very significantly because the molecule is pushed away from the electrode by the covalent thiol-gold bond

  16. Secondary ions produced from condensed rare gas targets under highly charged MeV/amu heavy ion bombardment

    International Nuclear Information System (INIS)

    Tawara, H.; Tonuma, T.; Kumagai, H.; Matsuo, T.

    1994-01-01

    Secondary ions produced from condensed rare gas targets are observed under MeV/amu, highly charged, heavy ion impact. The intensities of the observed cluster ions decrease smoothly as the cluster sizes become large but show some discontinuities at particular sizes of cluster ions. This seems to be closely related to the stabilities of cluster ion structures. It is also noted that very few doubly charged or practically no triply/higher charged ions have been observed, in sharp contrast to that of some condensed molecular targets. (orig.)

  17. Development of a Sweetness Sensor for Aspartame, a Positively Charged High-Potency Sweetener

    Directory of Open Access Journals (Sweden)

    Masato Yasuura

    2014-04-01

    Full Text Available Taste evaluation technology has been developed by several methods, such as sensory tests, electronic tongues and a taste sensor based on lipid/polymer membranes. In particular, the taste sensor can individually quantify five basic tastes without multivariate analysis. However, it has proven difficult to develop a sweetness sensor, because sweeteners are classified into three types according to the electric charges in an aqueous solution; that is, no charge, negative charge and positive charge. Using membrane potential measurements, the taste-sensing system needs three types of sensor membrane for each electric charge type of sweetener. Since the commercially available sweetness sensor was only intended for uncharged sweeteners, a sweetness sensor for positively charged high-potency sweeteners such as aspartame was developed in this study. Using a lipid and plasticizers, we fabricated various lipid/polymer membranes for the sweetness sensor to identify the suitable components of the sensor membranes. As a result, one of the developed sensors showed responses of more than 20 mV to 10 mM aspartame and less than 5 mV to any other taste. The responses of the sensor depended on the concentration of aspartame. These results suggested that the developed sweetness sensor had high sensitivity to and high selectivity for aspartame.

  18. Development of a sweetness sensor for aspartame, a positively charged high-potency sweetener.

    Science.gov (United States)

    Yasuura, Masato; Tahara, Yusuke; Ikezaki, Hidekazu; Toko, Kiyoshi

    2014-04-23

    Taste evaluation technology has been developed by several methods, such as sensory tests, electronic tongues and a taste sensor based on lipid/polymer membranes. In particular, the taste sensor can individually quantify five basic tastes without multivariate analysis. However, it has proven difficult to develop a sweetness sensor, because sweeteners are classified into three types according to the electric charges in an aqueous solution; that is, no charge, negative charge and positive charge. Using membrane potential measurements, the taste-sensing system needs three types of sensor membrane for each electric charge type of sweetener. Since the commercially available sweetness sensor was only intended for uncharged sweeteners, a sweetness sensor for positively charged high-potency sweeteners such as aspartame was developed in this study. Using a lipid and plasticizers, we fabricated various lipid/polymer membranes for the sweetness sensor to identify the suitable components of the sensor membranes. As a result, one of the developed sensors showed responses of more than 20 mV to 10 mM aspartame and less than 5 mV to any other taste. The responses of the sensor depended on the concentration of aspartame. These results suggested that the developed sweetness sensor had high sensitivity to and high selectivity for aspartame.

  19. A universal self-charging system driven by random biomechanical energy for sustainable operation of mobile electronics

    Science.gov (United States)

    Niu, Simiao; Wang, Xiaofeng; Yi, Fang; Zhou, Yu Sheng; Wang, Zhong Lin

    2015-12-01

    Human biomechanical energy is characterized by fluctuating amplitudes and variable low frequency, and an effective utilization of such energy cannot be achieved by classical energy-harvesting technologies. Here we report a high-efficient self-charging power system for sustainable operation of mobile electronics exploiting exclusively human biomechanical energy, which consists of a high-output triboelectric nanogenerator, a power management circuit to convert the random a.c. energy to d.c. electricity at 60% efficiency, and an energy storage device. With palm tapping as the only energy source, this power unit provides a continuous d.c. electricity of 1.044 mW (7.34 W m-3) in a regulated and managed manner. This self-charging unit can be universally applied as a standard `infinite-lifetime' power source for continuously driving numerous conventional electronics, such as thermometers, electrocardiograph system, pedometers, wearable watches, scientific calculators and wireless radio-frequency communication system, which indicates the immediate and broad applications in personal sensor systems and internet of things.

  20. Dynamical mechanism of charge separation by photoexcited generation of proton–electron pairs in organic molecular systems. A nonadiabatic electron wavepacket dynamics study

    Energy Technology Data Exchange (ETDEWEB)

    Yamamoto, Kentaro, E-mail: kyamamoto@fukui.kyoto-u.ac.jp; Takatsuka, Kazuo, E-mail: kaztak@fukui.kyoto-u.ac.jp

    2016-08-22

    Graphical abstract: Asymptotic biradical state produced by the excited-state coupled proton–electron transfer (CPET), resulting in charge separation (proton–electron pair creation) on a proton–electron acceptor A, in a series of photochemical systems generally denoted as X–Mn–OH{sub 2}⋯A, where X = (OH, Ca(OH){sub 3}) and A = (N-methylformamidine, guanidine, imidazole, or ammonia clusters). - Abstract: In this perspective article, we review, along with presenting new results, a series of our theoretical analyses on the excited-state mechanism of charge separation (proton–electron pair creation) relevant to the photoinduced water-splitting reaction (2H{sub 2}O → 4H{sup +} + 4e{sup −} + O{sub 2}) in organic and biological systems, which quite often includes Mn clusters in various molecular configurations. The present mechanism is conceived to be universal in the triggering process of the photoexcited water splitting dynamics. In other words, any Mn-based catalytic charge separation is quite likely to be initiated according to this mechanism. As computationally tractable yet realistic models, we examine a series of systems generally expressed as X–Mn–OH{sub 2}⋯A, where X = (OH, Ca(OH){sub 3}) and A = (N-methylformamidine, guanidine, imidazole or ammonia cluster) in terms of the theory of nonadiabatic electron wavepacket dynamics. We first find both an electron and a proton are simultaneously transferred to the acceptors through conical intersections upon photoexcitation. In this mechanism, the electron takes different pathways from that of the proton and reaches the densely lying Rydberg-like states of the acceptors in the end, thereby inducing charge separation. Therefore the presence of the Rydberg-like diffused unoccupied states as an electron acceptor is critical for this reaction to proceed. We also have found another crucial nonadiabatic process that deteriorates the efficiency of charge separation by rendering the created pair of proton

  1. Preparation of cold Mg{sup +}ion clouds for sympathetic cooling of highly charged ions at SPECTRAP

    Energy Technology Data Exchange (ETDEWEB)

    Cazan, Radu Mircea

    2012-02-15

    The bound electrons in hydrogen-like or lithium-like heavy ions experience extremely strong electric and magnetic fields in the surrounding of the nucleus. Laser spectroscopy of the ground-state hyperfine splitting in the lead region provides a sensitive tool to test strong-field quantum electro dynamics (QED), especially in the magnetic sector. Previous measurements on hydrogen-like systems performed in an electron-beam ion trap (EBIT) or at the experimental storage ring (ESR) were experimentally limited in accuracy due to statistics, the large Doppler broadening and the ion energy. The full potential of the QED test can only be exploited if measurements for hydrogen- and lithium-like ions are performed with accuracy improved by 2-3 orders of magnitude. Therefore, the new Penning trap setup SPECTRAP - dedicated for laser spectroscopy on trapped and cooled highly charged ions - is currently commissioned at GSI Darmstadt. Heavy highly charged ions will be delivered to this trap by the HITRAP facility in the future. SPECTRAP is a cylindrical Penning trap with axial access for external ion injection and radial optical access mounted inside a cold-bore superconducting Helmholtz-type split-coil magnet. To reach the targeted accuracy in laser spectroscopy, an efficient and fast cooling process for the highly charged ions must be employed. This can be realized by sympathetic cooling with a cloud of laser-cooled light ions. Within this thesis work, a laser system and an ion source for the production of such a {sup 24}Mg{sup +} ion cloud was developed and commissioned at SPECTRAP. An all-solid-state laser system for the generation of 279.6 nm light was designed and built. It consists of a fiber laser at 1118.5 nm followed by frequency quadrupling using two successive second-harmonic generation stages with actively stabilized ring resonators and nonlinear crystals. The laser system can deliver more than 15 mW of UV laser power under optimal conditions and requires little

  2. Large-area few-layer MoS 2 deposited by sputtering

    KAUST Repository

    Huang, Jyun-Hong

    2016-06-06

    Direct magnetron sputtering of transition metal dichalcogenide targets is proposed as a new approach for depositing large-area two-dimensional layered materials. Bilayer to few-layer MoS2 deposited by magnetron sputtering followed by post-deposition annealing shows superior area scalability over 20 cm(2) and layer-by-layer controllability. High crystallinity of layered MoS2 was confirmed by Raman, photo-luminescence, and transmission electron microscopy analysis. The sputtering temperature and annealing ambience were found to play an important role in the film quality. The top-gate field-effect transistor by using the layered MoS2 channel shows typical n-type characteristics with a current on/off ratio of approximately 10(4). The relatively low mobility is attributed to the small grain size of 0.1-1 mu m with a trap charge density in grain boundaries of the order of 10(13) cm(-2).

  3. Charge-coupled device area detector for low energy electrons

    International Nuclear Information System (INIS)

    Horacek, Miroslav

    2003-01-01

    A fast position-sensitive detector was designed for the angle- and energy-selective detection of signal electrons in the scanning low energy electron microscope (SLEEM), based on a thinned back-side directly electron-bombarded charged-coupled device (CCD) sensor (EBCCD). The principle of the SLEEM operation and the motivation for the development of the detector are explained. The electronics of the detector is described as well as the methods used for the measurement of the electron-bombarded gain and of the dark signal. The EBCCD gain of 565 for electron energy 5 keV and dynamic range 59 dB for short integration time up to 10 ms at room temperature were obtained. The energy dependence of EBCCD gain and the detection efficiency are presented for electron energy between 2 and 5 keV, and the integration time dependence of the output signals under dark conditions is given for integration time from 1 to 500 ms

  4. Application of relativistic distorted-wave method to electron-impact excitation of highly charged Fe XXIV ion embedded in weakly coupled plasmas

    Science.gov (United States)

    Chen, Zhanbin

    2018-05-01

    The process of excitation of highly charged Fe XXIV ion embedded in weakly coupled plasmas by electron impact is studied, together with the subsequent radiative decay. For the target structure, the calculation is performed using the multiconfiguration Dirac-Hartree-Fock method incorporating the Debye-Hückel potential for the electron-nucleus interaction. Fine-structure levels of the 1s22p and 1s2s2p configurations and the transition properties among these levels are presented over a wide range of screening parameters. For the collision dynamics, the distorted-wave method in the relativistic frame is adopted to include the effect of plasma background, in which the interparticle interactions in the system are described by screened interactions of the Debye-Hückel type. The continuum wave function of the projectile electron is obtained by solving the modified Dirac equations. The influence of plasma strength on the cross section, the linear polarization, and the angular distribution of x-ray photon emission are investigated in detail. Comparison of the present results with experimental data and other theoretical predictions, when available, is made.

  5. Observation of visible and uv magnetic dipole transitions in highly charged xenon and barium

    International Nuclear Information System (INIS)

    Morgan, C.A.; Serpa, F.G.; Takacs, E.; Meyer, E.S.; Gillaspy, J.D.; Sugar, J.; Roberts, J.R.; Brown, C.M.; Feldman, U.

    1995-01-01

    We have observed an unusual transition which is predicted to result in visible and near-uv emission from very highly charged titaniumlike ions spanning the entire upper half of the periodic table. Measurements of the wavelengths of the 3d 4 D 2 - 5 D 3 transitions in Ba +34 and Xe +32 are in surprisingly poor agreement with ab initio calculations. This work was carried out in an electron beam ion trap and demonstrates that such a device can be an important tool for visible spectroscopy of highly charged ions

  6. Proton-coupled electron transfer versus hydrogen atom transfer: generation of charge-localized diabatic states.

    Science.gov (United States)

    Sirjoosingh, Andrew; Hammes-Schiffer, Sharon

    2011-03-24

    The distinction between proton-coupled electron transfer (PCET) and hydrogen atom transfer (HAT) mechanisms is important for the characterization of many chemical and biological processes. PCET and HAT mechanisms can be differentiated in terms of electronically nonadiabatic and adiabatic proton transfer, respectively. In this paper, quantitative diagnostics to evaluate the degree of electron-proton nonadiabaticity are presented. Moreover, the connection between the degree of electron-proton nonadiabaticity and the physical characteristics distinguishing PCET from HAT, namely, the extent of electronic charge redistribution, is clarified. In addition, a rigorous diabatization scheme for transforming the adiabatic electronic states into charge-localized diabatic states for PCET reactions is presented. These diabatic states are constructed to ensure that the first-order nonadiabatic couplings with respect to the one-dimensional transferring hydrogen coordinate vanish exactly. Application of these approaches to the phenoxyl-phenol and benzyl-toluene systems characterizes the former as PCET and the latter as HAT. The diabatic states generated for the phenoxyl-phenol system possess physically meaningful, localized electronic charge distributions that are relatively invariant along the hydrogen coordinate. These diabatic electronic states can be combined with the associated proton vibrational states to generate the reactant and product electron-proton vibronic states that form the basis of nonadiabatic PCET theories. Furthermore, these vibronic states and the corresponding vibronic couplings may be used to calculate rate constants and kinetic isotope effects of PCET reactions.

  7. Space charge effects and electronic bistability

    International Nuclear Information System (INIS)

    Ruffini, A.; Strumia, F.; Tommasi, O.

    1996-01-01

    The excitation of metastable states in an atomic beam apparatus by means of electron collision is a widespread technique. The authors have observed a large bistable behaviour in apparatus designed to provide an intense and collimated beam of metastable helium by excitation with orthogonally impinging electrons. This bistable behaviour largely affects the efficiency of the apparatus and is therefore worth of being carefully investigated. The apparatus has an electrode configuration equivalent to that of a tetrode valve with large intergrid distances. The bistability consists in a hysteresis cycle in the curve of the anode current vs. grid voltage. Experimental measurements, supported by a simple theoretical model and by numerical simulation, stress out the crucial role played by space charge effects for the onset of bistability. A comparison with previous observations of this phenomenon is given. Spontaneous current oscillations with various shapes have been recorded in one of the two curves of the hysteresis cycle

  8. Materials Characterization at Utah State University: Facilities and Knowledge-base of Electronic Properties of Materials Applicable to Spacecraft Charging

    Science.gov (United States)

    Dennison, J. R.; Thomson, C. D.; Kite, J.; Zavyalov, V.; Corbridge, Jodie

    2004-01-01

    In an effort to improve the reliability and versatility of spacecraft charging models designed to assist spacecraft designers in accommodating and mitigating the harmful effects of charging on spacecraft, the NASA Space Environments and Effects (SEE) Program has funded development of facilities at Utah State University for the measurement of the electronic properties of both conducting and insulating spacecraft materials. We present here an overview of our instrumentation and capabilities, which are particularly well suited to study electron emission as related to spacecraft charging. These measurements include electron-induced secondary and backscattered yields, spectra, and angular resolved measurements as a function of incident energy, species and angle, plus investigations of ion-induced electron yields, photoelectron yields, sample charging and dielectric breakdown. Extensive surface science characterization capabilities are also available to fully characterize the samples in situ. Our measurements for a wide array of conducting and insulating spacecraft materials have been incorporated into the SEE Charge Collector Knowledge-base as a Database of Electronic Properties of Materials Applicable to Spacecraft Charging. This Database provides an extensive compilation of electronic properties, together with parameterization of these properties in a format that can be easily used with existing spacecraft charging engineering tools and with next generation plasma, charging, and radiation models. Tabulated properties in the Database include: electron-induced secondary electron yield, backscattered yield and emitted electron spectra; He, Ar and Xe ion-induced electron yields and emitted electron spectra; photoyield and solar emittance spectra; and materials characterization including reflectivity, dielectric constant, resistivity, arcing, optical microscopy images, scanning electron micrographs, scanning tunneling microscopy images, and Auger electron spectra. Further

  9. Simulations of space charge neutralization in a magnetized electron cooler

    Energy Technology Data Exchange (ETDEWEB)

    Gerity, James [Texas A-M; McIntyre, Peter M. [Texas A-M; Bruhwiler, David Leslie [RadiaSoft, Boulder; Hall, Christopher [RadiaSoft, Boulder; Moens, Vince Jan [Ecole Polytechnique, Lausanne; Park, Chong Shik [Fermilab; Stancari, Giulio [Fermilab

    2017-02-02

    Magnetized electron cooling at relativistic energies and Ampere scale current is essential to achieve the proposed ion luminosities in a future electron-ion collider (EIC). Neutralization of the space charge in such a cooler can significantly increase the magnetized dynamic friction and, hence, the cooling rate. The Warp framework is being used to simulate magnetized electron beam dynamics during and after the build-up of neutralizing ions, via ionization of residual gas in the cooler. The design follows previous experiments at Fermilab as a verification case. We also discuss the relevance to EIC designs.

  10. Nanoscale transformation of sp2 to sp3 of graphite by slow highly charged ion irradiation

    International Nuclear Information System (INIS)

    Meguro, T.; Hida, A.; Koguchi, Y.; Miyamoto, S.; Yamamoto, Y.; Takai, H.; Maeda, K.; Aoyagi, Y.

    2003-01-01

    Nanoscale transformation of electronic states by highly charged ion (HCI) impact on graphite surfaces is described. The high potential energy of slow HCI, which induces multiple emission of electrons from the surface, provides a strong modification of the electronic states of the local area upon graphite surfaces. The HCI impact and the subsequent surface treatment either by electron injection from a scanning tunneling microscopy tip or by He-Cd laser irradiation induce a localized transition from sp 2 to sp 3 hybridization in graphite, resulting in the formation of nanoscale diamond-like structures (nanodiamond) at the impact region. From Raman spectroscopic measurements on sp 2 related peaks, it is found that the HCI irradiation creates vacancy complexes in contrast to ions having a lower charge state, which generate single vacancies. It is of interest that a single impact of HCI creates one nanodiamond structure, suggesting potential applications of HCI in nanoscale material processing

  11. Accumulative charge separation for solar fuels production: coupling light-induced single electron transfer to multielectron catalysis.

    Science.gov (United States)

    Hammarström, Leif

    2015-03-17

    The conversion and storage of solar energy into a fuel holds promise to provide a significant part of the future renewable energy demand of our societies. Solar energy technologies today generate heat or electricity, while the large majority of our energy is used in the form of fuels. Direct conversion of solar energy to a fuel would satisfy our needs for storable energy on a large scale. Solar fuels can be generated by absorbing light and converting its energy to chemical energy by electron transfer leading to separation of electrons and holes. The electrons are used in the catalytic reduction of a cheap substrate with low energy content into a high-energy fuel. The holes are filled by oxidation of water, which is the only electron source available for large scale solar fuel production. Absorption of a single photon typically leads to separation of a single electron-hole pair. In contrast, fuel production and water oxidation are multielectron, multiproton reactions. Therefore, a system for direct solar fuel production must be able to accumulate the electrons and holes provided by the sequential absorption of several photons in order to complete the catalytic reactions. In this Account, the process is termed accumulative charge separation. This is considerably more complicated than charge separation on a single electron level and needs particular attention. Semiconductor materials and molecular dyes have for a long time been optimized for use in photovoltaic devices. Efforts are made to develop new systems for light harvesting and charge separation that are better optimized for solar fuel production than those used in the early devices presented so far. Significant progress has recently been made in the discovery and design of better homogeneous and heterogeneous catalysts for solar fuels and water oxidation. While the heterogeneous ones perform better today, molecular catalysts based on transition metal complexes offer much greater tunability of electronic and

  12. Charge migration and charge transfer in molecular systems

    Directory of Open Access Journals (Sweden)

    Hans Jakob Wörner

    2017-11-01

    Full Text Available The transfer of charge at the molecular level plays a fundamental role in many areas of chemistry, physics, biology and materials science. Today, more than 60 years after the seminal work of R. A. Marcus, charge transfer is still a very active field of research. An important recent impetus comes from the ability to resolve ever faster temporal events, down to the attosecond time scale. Such a high temporal resolution now offers the possibility to unravel the most elementary quantum dynamics of both electrons and nuclei that participate in the complex process of charge transfer. This review covers recent research that addresses the following questions. Can we reconstruct the migration of charge across a molecule on the atomic length and electronic time scales? Can we use strong laser fields to control charge migration? Can we temporally resolve and understand intramolecular charge transfer in dissociative ionization of small molecules, in transition-metal complexes and in conjugated polymers? Can we tailor molecular systems towards specific charge-transfer processes? What are the time scales of the elementary steps of charge transfer in liquids and nanoparticles? Important new insights into each of these topics, obtained from state-of-the-art ultrafast spectroscopy and/or theoretical methods, are summarized in this review.

  13. Projectile- and charge-state-dependent electron yields from ion penetration of solids as a probe of preequilibrium stopping power

    DEFF Research Database (Denmark)

    Rothard, H.; Schou, Jørgen; Groeneveld, K.-O.

    1992-01-01

    Kinetic electron-emission yields gamma from swift ion penetration of solids are proportional to the (electronic) stopping power gamma approximately Beta-S*, if the preequilibrium evolution of the charge and excitation states of the positively charged ions is taken into account. We show...... by investigating the "transport factor" beta, the energy spectrum of directly ejected recoil electrons and the evolution of ionic charge state inside solids. Estimates of the energy-loss fraction leading to electron emission and the effective charges of the ions near the surface allow a quantitative description...

  14. Generation of static magnetic fields by a test charge in a plasma with anisotropic electron temperature

    Energy Technology Data Exchange (ETDEWEB)

    Aliev, Yu.M.; Bychenkov, V.Yu.; Frolov, A.A. (AN SSSR, Moscow. Fizicheskij Inst.)

    Structure of electomagnetic field generated with a charge in a plasma with anisotropic electron temperature has been studied. Unlike a hydrodynamical approach to study on the magnetic field qeneration with a test charge a kinetic theory describing spatial distribution of both magnetic and electrostatic components of charge field was constructed. Such theory results permit to investigate the charge field structure both at distances larger than length of free electron path and not exceeding it. The developed theory can serve as the basis for development of new methods for anisotropic plasma diagnostics.

  15. A multislit transverse-emittance diagnostic for space-charge-dominated electron beams

    International Nuclear Information System (INIS)

    Piot, P.; Song, J.; Li, R.

    1997-01-01

    Jefferson Lab is developing a 10 MeV injector to provide an electron beam for a high-power free-electron laser (FEL). To characterize the transverse phase space of the space-charged-dominated beam produced by this injector, the authors designed an interceptive multislit emittance diagnostic. It incorporates an algorithm for phase-space reconstruction and subsequent calculation of the Twiss parameters and emittance for both transverse directions at an update rate exceeding 1 Hz, a speed that will facilitate the transverse-phase-space matching between the injector and the FEL's accelerator that is critical for proper operation. This paper describes issues pertaining to the diagnostic's design. It also discusses the acquisition system, as well as the software algorithm and its implementation in the FEL control system. First results obtained from testing this diagnostic in Jefferson Lab's Injector Test Stand are also included

  16. Ultralight Cut-Paper-Based Self-Charging Power Unit for Self-Powered Portable Electronic and Medical Systems.

    Science.gov (United States)

    Guo, Hengyu; Yeh, Min-Hsin; Zi, Yunlong; Wen, Zhen; Chen, Jie; Liu, Guanlin; Hu, Chenguo; Wang, Zhong Lin

    2017-05-23

    The development of lightweight, superportable, and sustainable power sources has become an urgent need for most modern personal electronics. Here, we report a cut-paper-based self-charging power unit (PC-SCPU) that is capable of simultaneously harvesting and storing energy from body movement by combining a paper-based triboelectric nanogenerator (TENG) and a supercapacitor (SC), respectively. Utilizing the paper as the substrate with an assembled cut-paper architecture, an ultralight rhombic-shaped TENG is achieved with highly specific mass/volume charge output (82 nC g -1 /75 nC cm -3 ) compared with the traditional acrylic-based TENG (5.7 nC g -1 /5.8 nC cm -3 ), which can effectively charge the SC (∼1 mF) to ∼1 V in minutes. This wallet-contained PC-SCPU is then demonstrated as a sustainable power source for driving wearable and portable electronic devices such as a wireless remote control, electric watch, or temperature sensor. This study presents a potential paper-based portable SCPU for practical and medical applications.

  17. Electron Heating and Quasiparticle Tunnelling in Superconducting Charge Qubits

    Science.gov (United States)

    Shaw, M. D.; Bueno, J.; Delsing, P.; Echternach, P. M.

    2008-01-01

    We have directly measured non-equilibrium quasiparticle tunnelling in the time domain as a function of temperature and RF carrier power for a pair of charge qubits based on the single Cooper-pair box, where the readout is performed with a multiplexed quantum capacitance technique. We have extracted an effective electron temperature for each applied RF power, using the data taken at the lowest power as a reference curve. This data has been fit to a standard T? electron heating model, with a reasonable correspondence with established material parameters.

  18. Fragile charge order in the nonsuperconducting ground state of the underdoped high-temperature superconductors.

    Science.gov (United States)

    Tan, B S; Harrison, N; Zhu, Z; Balakirev, F; Ramshaw, B J; Srivastava, A; Sabok-Sayr, S A; Sabok, S A; Dabrowski, B; Lonzarich, G G; Sebastian, Suchitra E

    2015-08-04

    The normal state in the hole underdoped copper oxide superconductors has proven to be a source of mystery for decades. The measurement of a small Fermi surface by quantum oscillations on suppression of superconductivity by high applied magnetic fields, together with complementary spectroscopic measurements in the hole underdoped copper oxide superconductors, point to a nodal electron pocket from charge order in YBa2Cu3(6+δ). Here, we report quantum oscillation measurements in the closely related stoichiometric material YBa2Cu4O8, which reveals similar Fermi surface properties to YBa2Cu3(6+δ), despite the nonobservation of charge order signatures in the same spectroscopic techniques, such as X-ray diffraction, that revealed signatures of charge order in YBa2Cu3(6+δ). Fermi surface reconstruction in YBa2Cu4O8 is suggested to occur from magnetic field enhancement of charge order that is rendered fragile in zero magnetic fields because of its potential unconventional nature and/or its occurrence as a subsidiary to more robust underlying electronic correlations.

  19. Bistable intrinsic charge fluctuations of a dust grain subject to secondary electron emission in a plasma.

    Science.gov (United States)

    Shotorban, B

    2015-10-01

    A master equation was formulated to study intrinsic charge fluctuations of a grain in a plasma as ions and primary electrons are attached to the grain through collisional collection, and secondary electrons are emitted from the grain. Two different plasmas with Maxwellian and non-Maxwellian distributions were considered. The fluctuations could be bistable in either plasma when the secondary electron emission is present, as two stable macrostates, associated with two stable roots of the charge net current, may exist. Metastablity of fluctuations, manifested by the passage of the grain charge between two macrostates, was shown to be possible.

  20. Mode-selective vibrational modulation of charge transport in organic electronic devices

    KAUST Repository

    Bakulin, Artem A.

    2015-08-06

    The soft character of organic materials leads to strong coupling between molecular, nuclear and electronic dynamics. This coupling opens the way to influence charge transport in organic electronic devices by exciting molecular vibrational motions. However, despite encouraging theoretical predictions, experimental realization of such approach has remained elusive. Here we demonstrate experimentally that photoconductivity in a model organic optoelectronic device can be modulated by the selective excitation of molecular vibrations. Using an ultrafast infrared laser source to create a coherent superposition of vibrational motions in a pentacene/C60 photoresistor, we observe that excitation of certain modes in the 1,500–1,700 cm−1 region leads to photocurrent enhancement. Excited vibrations affect predominantly trapped carriers. The effect depends on the nature of the vibration and its mode-specific character can be well described by the vibrational modulation of intermolecular electronic couplings. This presents a new tool for studying electron–phonon coupling and charge dynamics in (bio)molecular materials.

  1. Mode-selective vibrational modulation of charge transport in organic electronic devices

    KAUST Repository

    Bakulin, Artem A.; Lovrincic, Robert; Yu, Xi; Selig, Oleg; Bakker, Huib J.; Rezus, Yves L. A.; Nayak, Pabitra K.; Fonari, Alexandr; Coropceanu, Veaceslav; Bredas, Jean-Luc; Cahen, David

    2015-01-01

    The soft character of organic materials leads to strong coupling between molecular, nuclear and electronic dynamics. This coupling opens the way to influence charge transport in organic electronic devices by exciting molecular vibrational motions. However, despite encouraging theoretical predictions, experimental realization of such approach has remained elusive. Here we demonstrate experimentally that photoconductivity in a model organic optoelectronic device can be modulated by the selective excitation of molecular vibrations. Using an ultrafast infrared laser source to create a coherent superposition of vibrational motions in a pentacene/C60 photoresistor, we observe that excitation of certain modes in the 1,500–1,700 cm−1 region leads to photocurrent enhancement. Excited vibrations affect predominantly trapped carriers. The effect depends on the nature of the vibration and its mode-specific character can be well described by the vibrational modulation of intermolecular electronic couplings. This presents a new tool for studying electron–phonon coupling and charge dynamics in (bio)molecular materials.

  2. Spectroscopy of multi-charged ions: a short review

    International Nuclear Information System (INIS)

    Berry, H.G.

    1983-01-01

    Recent and future applications of multiply charged ions to spectroscopy and atomic structure are discussed. The experimental techniques use either very fast ions produced in heavy ion accelerators, or slow ions produced directly both in electron beam ion sources and from collisions of fast accelerated ions. For the accelerated fast ions, spectroscopic measurements on using gas target excitation, solid foil excitation and laser excitation. In gas target excitation, both X-ray and electron spectroscopy have been applied to analyse atomic structures and secondary collision effects. Highlycharged secondary ions have also been trapped electro-magnetically for further similar studies in controlled conditions. Spectroscopic detection following solid foil interaction has led to atomic lifetime measurements, principally of metastable level, analysis of complex highly-ionized heavy ion spectra, and investigations of relativistic and QED effects in few electron ions

  3. Instrumentation in high energy physics

    International Nuclear Information System (INIS)

    Serin, L.

    2007-01-01

    The instrumentation in high energy physics is a wide and advanced domain which cannot be covered in a single lesson. The main basic physics processes for charged and neutral particles are recalled with the definition of a few concepts needed to understand or design a detector. The application of these principles to charged particle measurement devices (momentum), light detection or energy measurement are presented mostly with examples from collider experiments. The particle identification which is often the combination of different techniques in a same experiment is also discussed. Finally in a very short section, a few considerations about electronics/processing with their impact on the detector performance are given

  4. Electron-cloud effects in high-luminosity colliders

    Energy Technology Data Exchange (ETDEWEB)

    Zimmermann, F.

    1998-01-01

    Electron-cloud instabilities are expected to be important in most high-luminosity double-ring colliders. In this report, the author describes a few parameter regimes and some critical parameter dependences of this type of instability, and illustrate these with simulation results for the PEP-II and KEK B factories, the LHC, the VLHC, and DAPHNE. In addition, the author studies the possibility and the potential impact of an electron cloud in the interaction region.

  5. The CMS Beam Halo Monitor Electronics

    CERN Document Server

    AUTHOR|(CDS)2080684; Fabbri, F.; Grassi, T.; Hughes, E.; Mans, J.; Montanari, A.; Orfanelli, S.; Rusack, R.; Torromeo, G.; Stickland, D.P.; Stifter, K.

    2016-01-01

    The CMS Beam Halo Monitor has been successfully installed in the CMS cavern in LHC Long Shutdown 1 for measuring the machine induced background for LHC Run II. The system is based on 40 detector units composed of synthetic quartz Cherenkov radiators coupled to fast photomultiplier tubes. The readout electronics chain uses many components developed for the Phase 1 upgrade to the CMS Hadronic Calorimeter electronics, with dedicated firmware and readout adapted to the beam monitoring requirements. The PMT signal is digitized by a charge integrating ASIC (QIE10), providing both the signal rise time, with few ns resolution, and the charge integrated over one bunch crossing. The backend electronics uses microTCA technology and receives data via a high-speed 5 Gbps asynchronous link. It records histograms with sub-bunch crossing timing resolution and is readout by IPbus using the newly designed CMS data acquisition for non-event based data. The data is processed in real time and published to CMS and the LHC, providi...

  6. Experimental study on the production of high density electron bunches from a GaAs photocathode

    International Nuclear Information System (INIS)

    Calabrese, R.; Masoli, F.; Gong, J.M.; Guidi, V.; Tecchio, L.

    1991-01-01

    In order to obtain a high charge, low emittance electron source, useful for FEL electron injector and for e + e - collider experiments, we performed a test experiment on a gallium arsenide photocathode, activated by negative electron affinity technique and illuminated with a 10 ns long laser pulse of 532 nm wavelength. We measured a maximum charge delivered, at relatively low potentials, of about 18 nC/bunch. The mean lifetime is greater than 60 h. (orig.)

  7. Laboratory Measurements on Charging of Individual Micron-Size Apollo-11 Dust Grains by Secondary Electron Emissions

    Science.gov (United States)

    Tankosic, D.; Abbas, M. M.

    2012-01-01

    Observations made during Apollo missions, as well as theoretical models indicate that the lunar surface and dust grains are electrostatically charged, levitated and transported. Lunar dust grains are charged by UV photoelectric emissions on the lunar dayside and by the impact of the solar wind electrons on the nightside. The knowledge of charging properties of individual lunar dust grains is important for developing appropriate theoretical models and mitigating strategies. Currently, very limited experimental data are available for charging of individual micron-size size lunar dust grains in particular by low energy electron impact. However, experimental results based on extensive laboratory measurements on the charging of individual 0.2-13 micron size lunar dust grains by the secondary electron emissions (SEE) have been presented in a recent publication. The SEE process of charging of micron-size dust grains, however, is found to be very complex phenomena with strong particle size dependence. In this paper we present some examples of the complex nature of the SEE properties of positively charged individual lunar dust grains levitated in an electrodynamic balance (EDB), and show that they remain unaffected by the variation of the AC field employed in the above mentioned measurements.

  8. How to emit a high-power electron beam from a magnetospheric spacecraft?

    Science.gov (United States)

    Delzanno, G. L.; Lucco Castello, F.; Borovsky, J.; Miars, G.; Leon, O.; Gilchrist, B. E.

    2017-12-01

    The idea of using a high-power electron beam to actively probe magnetic-field-line connectivity in space has been discussed since the 1970's. It could solve longstanding questions in magnetospheric/ionospheric physics by establishing causality between phenomena occurring in the magnetosphere and their image in the ionosphere. However, this idea has never been realized onboard a magnetospheric spacecraft because the tenuous magnetospheric plasma cannot provide the return current necessary to keep the charging of the spacecraft under control. Recently, Delzanno et al. [1] have proposed a spacecraft-charging mitigation scheme to enable the emission of a high-power electron beam from a magnetospheric spacecraft. It is based on the plasma contactor, i.e. a high-density neutral plasma emitted prior to and with the electron beam. The contactor acts as an ion emitter (not as an electron collector, as previously thought): a high ion current can be emitted off the quasi-spherical contactor surface, without the strong space-charge limitations typical of planar ion beams, and the electron-beam current can be successfully compensated. In this work, we will discuss our theoretical/simulation effort to improve the understanding of contactor-based ion emission. First, we will present a simple mathematical model useful for the interpretation of the results of [1]. The model is in spherical geometry and the contactor dynamics is described by only two surfaces (its quasi-neutral surface and the front of the outermost ions). It captures the results of self-consistent Particle-In-Cell (PIC) simulations with good accuracy and highlights the physics behind the charge-mitigation scheme clearly. PIC simulations connecting the 1D model to the actual geometry of the problem will be presented to obtain the scaling of the spacecraft potential varying contactor emission area. Finally, results for conditions relevant to an actual mission will also be discussed. [1] G. L. Delzanno, J. E. Borovsky

  9. Highly charged ion based time-of-flight emission microscope

    International Nuclear Information System (INIS)

    Hamza, Alex V.; Barnes, Alan V.; Magee, Ed; Newman, Mike; Schenkel, Thomas; McDonald, Joseph W.; Schneider, Dieter H.

    2000-01-01

    An emission microscope using highly charged ions as the excitation source has been designed, constructed, and operated. A novel ''acorn'' objective lens has been used to simultaneously image electron and secondary ion emission. A resistive anode-position sensitive detector is used to determine the x-y position and time of arrival of the secondary events at the microscope image plane. Contrast in the image can be based on the intensity of the electron emission and/or the presence of particular secondary ions. Spatial resolution of better than 1 μm and mass resolution m/Δm of better than 400 were demonstrated. Background rejection from uncorrelated events of greater than an order of magnitude is also achieved. (c) 2000 American Institute of Physics

  10. Shielding for high energy, high intensity electron accelerator installation

    International Nuclear Information System (INIS)

    Warawas, C.; Chongkum, S.

    1997-03-01

    The utilization of electron accelerators (eBA) is gradually increased in Thailand. For instance, a 30-40 MeV eBA are used for tumor and cancer therapy in the hospitals, and a high current eBA in for gemstone colonization. In the near future, an application of eBA in industries will be grown up in a few directions, e.g., flue gases treatment from the coal fire-power plants, plastic processing, rubber vulcanization and food preservation. It is the major roles of Office of Atomic Energy for Peace (OAEP) to promote the peaceful uses of nuclear energy and to regulate the public safety and protection of the environment. By taking into account of radiation safety aspect, high energy electrons are not only harmful to human bodies, but the radioactive nuclides can be occurred. This report presents a literature review by following the National Committee on Radiation Protection and Measurements (NCRP) report No.31. This reviews for parametric calculation and shielding design of the high energy (up to 100 MeV), high intensity electron accelerator installation

  11. Exploring charge density analysis in crystals at high pressure: data collection, data analysis and advanced modelling.

    Science.gov (United States)

    Casati, Nicola; Genoni, Alessandro; Meyer, Benjamin; Krawczuk, Anna; Macchi, Piero

    2017-08-01

    The possibility to determine electron-density distribution in crystals has been an enormous breakthrough, stimulated by a favourable combination of equipment for X-ray and neutron diffraction at low temperature, by the development of simplified, though accurate, electron-density models refined from the experimental data and by the progress in charge density analysis often in combination with theoretical work. Many years after the first successful charge density determination and analysis, scientists face new challenges, for example: (i) determination of the finer details of the electron-density distribution in the atomic cores, (ii) simultaneous refinement of electron charge and spin density or (iii) measuring crystals under perturbation. In this context, the possibility of obtaining experimental charge density at high pressure has recently been demonstrated [Casati et al. (2016). Nat. Commun. 7, 10901]. This paper reports on the necessities and pitfalls of this new challenge, focusing on the species syn-1,6:8,13-biscarbonyl[14]annulene. The experimental requirements, the expected data quality and data corrections are discussed in detail, including warnings about possible shortcomings. At the same time, new modelling techniques are proposed, which could enable specific information to be extracted, from the limited and less accurate observations, like the degree of localization of double bonds, which is fundamental to the scientific case under examination.

  12. Benchmark of Space Charge Simulations and Comparison with Experimental Results for High Intensity, Low Energy Accelerators

    CERN Document Server

    Cousineau, Sarah M

    2005-01-01

    Space charge effects are a major contributor to beam halo and emittance growth leading to beam loss in high intensity, low energy accelerators. As future accelerators strive towards unprecedented levels of beam intensity and beam loss control, a more comprehensive understanding of space charge effects is required. A wealth of simulation tools have been developed for modeling beams in linacs and rings, and with the growing availability of high-speed computing systems, computationally expensive problems that were inconceivable a decade ago are now being handled with relative ease. This has opened the field for realistic simulations of space charge effects, including detailed benchmarks with experimental data. A great deal of effort is being focused in this direction, and several recent benchmark studies have produced remarkably successful results. This paper reviews the achievements in space charge benchmarking in the last few years, and discusses the challenges that remain.

  13. Enhanced Electron-Phonon Coupling at Metal Surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Plummer, Ward E.

    2010-08-04

    The Born-Oppenheimer approximation (BOA) decouples electronic from nuclear motion, providing a focal point for most quantum mechanics textbooks. However, a multitude of important chemical, physical and biological phenomena are driven by violations of this approximation. Vibronic interactions are a necessary ingredient in any process that makes or breaks a covalent bond, for example, conventional catalysis or enzymatically delivered biological reactions. Metastable phenomena associated with defects and dopants in semiconductors, oxides, and glasses entail violation of the BOA. Charge exchange in inorganic polymers, organic slats and biological systems involves charge- induced distortions of the local structure. A classic example is conventional superconductivity, which is driven by the electron-lattice interaction. High-resolution angle-resolved photoemission experiments are yielding new insight into the microscopic origin of electron-phonon coupling (EPC) in anisotropic two-dimensional systems. Our recent surface phonon measurement on the surface of a high-Tc material clearly indicates an important momentum dependent EPC in these materials. In the last few years we have shifted our research focus from solely looking at electron phonon coupling to examining the structure/functionality relationship at the surface of complex transition metal compounds. The investigation on electron phonon coupling has allowed us to move to systems where there is coupling between the lattice, the electrons and the spin.

  14. Electronic structure of charge carriers in a polysilane quantum wire

    International Nuclear Information System (INIS)

    Kumagai, J.; Yoshida, H.; Ichikawa, T.

    1997-01-01

    The ESR, ESEEM and spectrophotometric studies on polysilane radical ions revealed that charge carriers, hole and conducting electrons, are not delocalized all over the Si-Si main chain but confined to a part of the chain composed of only six Si atoms, probably near the branch on the main chain. Comparison of the ESR spectra of the radical cations and anions revealed that the hole can migrate from the main chain to an adjacent polymer chain via the side chains, whereas the conducting electron can not migrate since the side chains act as good intermolecular insulators for the electron. (author)

  15. Mechanisms of dust grain charging in plasma with allowance for electron emission processes

    Energy Technology Data Exchange (ETDEWEB)

    Mol’kov, S. I.; Savin, V. N., E-mail: moped@onego.ru [Petrozavodsk State University (Russian Federation)

    2017-02-15

    The process of dust grain charging is described with allowance for secondary, ion-induced, photoelectric, and thermal electron emission from the grain surface. The roughness of the grain surface is taken into account. An intermediate charging regime involving ion–atom collisions and electron ionization in the perturbed plasma region is analyzed using the moment equations and Poisson’s equation. A calculation method is proposed that allows one to take into account the influence of all the above effects and determine the radius of the plasma region perturbed by the dust grain.

  16. Dynamic investigation of electron trapping and charge decay in electron-irradiated Al sub 2 O sub 3 in a scanning electron microscope: Methodology and mechanisms

    CERN Document Server

    Fakhfakh, S; Belhaj, M; Fakhfakh, Z; Kallel, A; Rau, E I

    2002-01-01

    The charging and discharging of polycrystalline Al sub 2 O sub 3 submitted to electron-irradiation in a scanning electron microscope (SEM) are investigated by means of the displacement current method. To circumvent experimental shortcomings inherent to the use of the basic sample holder, a redesign of the latter is proposed and tests are carried out to verify its operation. The effects of the primary beam accelerating voltage on charging, flashover and discharging phenomena during and after electron-irradiation are studied. The experimental results are then analyzed. In particular, the divergence between the experimental data and those predicted by the total electron emission yield approach (TEEYA) is discussed. A partial discharge was observed immediately after the end of the electron-irradiation exposure. The experimental data suggests, that the discharge is due to the evacuation to the ground, along the insulator surface, of released electrons from shallow traps at (or in the close vicinity of) the insulat...

  17. Designing Two-Dimensional Dirac Heterointerfaces of Few-Layer Graphene and Tetradymite-Type Sb2Te3 for Thermoelectric Applications.

    Science.gov (United States)

    Jang, Woosun; Lee, Jiwoo; In, Chihun; Choi, Hyunyong; Soon, Aloysius

    2017-12-06

    Despite the ubiquitous nature of the Peltier effect in low-dimensional thermoelectric devices, the influence of finite temperature on the electronic structure and transport in the Dirac heterointerfaces of the few-layer graphene and layered tetradymite, Sb 2 Te 3 (which coincidently have excellent thermoelectric properties) are not well understood. In this work, using the first-principles density-functional theory calculations, we investigate the detailed atomic and electronic structure of these Dirac heterointerfaces of graphene and Sb 2 Te 3 and further re-examine the effect of finite temperature on the electronic band structures using a phenomenological temperature-broadening model based on Fermi-Dirac statistics. We then proceed to understand the underlying charge redistribution process in this Dirac heterointerfaces and through solving the Boltzmann transport equation, we present the theoretical evidence of electron-hole asymmetry in its electrical conductivity as a consequence of this charge redistribution mechanism. We finally propose that the hexagonal-stacked Dirac heterointerfaces are useful as efficient p-n junction building blocks in the next-generation thermoelectric devices where the electron-hole asymmetry promotes the thermoelectric transport by "hot" excited charge carriers.

  18. The negatively charged nitrogen-vacancy centre in diamond: the electronic solution

    International Nuclear Information System (INIS)

    Doherty, M W; Hollenberg, L C L; Manson, N B; Delaney, P

    2011-01-01

    The negatively charged nitrogen-vacancy centre is a unique defect in diamond that possesses properties highly suited to many applications, including quantum information processing, quantum metrology and biolabelling. Although the unique properties of the centre have been extensively documented and utilized, a detailed understanding of the physics of the centre has not yet been achieved. Indeed, there persist a number of points of contention regarding the electronic structure of the centre, such as the ordering of the dark intermediate singlet states. Without a detailed model of the centre's electronic structure, the understanding of the system's unique dynamical properties cannot effectively progress. In this work, the molecular model of the defect centre is fully developed to provide a self-consistent model of the complete electronic structure of the centre. The application of the model to describe the effects of electric, magnetic and strain interactions, as well as the variation of the centre's fine structure with temperature, provides an invaluable tool to those studying the centre and a means of designing future empirical and ab initio studies of this important defect.

  19. Dynamic simulation of charging processes in polar dielectrics irradiated by the electron bunches of middle level energy

    International Nuclear Information System (INIS)

    Maslovskaya, A.G.

    2011-01-01

    Nowadays the scanning electron microscopy techniques are widely used practically in condenser matter physics to study properties and structure of solids. The electron probe of scanning electron microscope is not merely a passive indicator of the geometrical or potential profile of the sample surface, but also the source producing ionizing, electric and thermal action on the sample. The application of raster electron methods to polar materials, responding to electric and heat exposures of the electron bunches allows us to get a response and create new modes of image formation. Let assume, that a sample surface of dielectric is irradiated by thin focused electron bunches of middle level energy (with order 1÷50 keV). When electrons bombard the dielectric sample the accumulation of absorbed electrons occurs. As a result generated charged areas can irregular drift the initial bunches. Charging effect occurs at any magnifications and any actual probe current. This work considers the results of dynamic simulation of charging process in polar dielectrics under the investigation with the scanning electron microscope. The purpose of present study is design and model implementation of three-dimensional dynamic model of charge relaxation in polar materials irradiated by electron bunches of middle level energy. The mathematical problem definition is given by the system of the continuity equation and Poisson equation. Final system of equations was modified in terms of intrinsic radiation-induced conductivity in sample as well as cylindrical symmetry of the problem. The simulation is based on numerical method solving of boundary problem for partial derivative equation system. In addition the initial electron distribution is determined by Monte-Carlo method using the programming implementation. To solve this problem we used the computational methods of solution of nonstationary mathematical physics problem such as finite difference method and finite element method realized with

  20. Charge amplitude distribution of the Gossip gaseous pixel detector

    Energy Technology Data Exchange (ETDEWEB)

    Blanco Carballo, V.M. [Twente University, Enschede (Netherlands); Chefdeville, M. [NIKHEF, P.B. 41882, 1009DB Amsterdam (Netherlands); Colas, P.; Giomataris, Y. [Saclay, Gif-sur-Yvette (France); Graaf, H. van der; Gromov, V. [NIKHEF, P.B. 41882, 1009DB Amsterdam (Netherlands); Hartjes, F. [NIKHEF, P.B. 41882, 1009DB Amsterdam (Netherlands)], E-mail: F.Hartjes@nikhef.nl; Kluit, R.; Koffeman, E. [NIKHEF, P.B. 41882, 1009DB Amsterdam (Netherlands); Salm, C.; Schmitz, J.; Smits, S.M. [Twente University, Enschede (Netherlands); Timmermans, J.; Visschers, J.L. [NIKHEF, P.B. 41882, 1009DB Amsterdam (Netherlands)

    2007-12-11

    The Gossip gaseous pixel detector is being developed for the detection of charged particles in extreme high radiation environments as foreseen close to the interaction point of the proposed super LHC. The detecting medium is a thin layer of gas. Because of the low density of this medium, only a few primary electron/ion pairs are created by the traversing particle. To get a detectable signal, the electrons drift towards a perforated metal foil (Micromegas) whereafter they are multiplied in a gas avalanche to provide a detectable signal. The gas avalanche occurs in the high field between the Micromegas and the pixel readout chip (ROC). Compared to a silicon pixel detector, Gossip features a low material budget and a low cooling power. An experiment using X-rays has indicated a possible high radiation tolerance exceeding 10{sup 16} hadrons/cm{sup 2}. The amplified charge signal has a broad amplitude distribution due to the limited statistics of the primary ionization and the statistical variation of the gas amplification. Therefore, some degree of inefficiency is inevitable. This study presents experimental results on the charge amplitude distribution for CO{sub 2}/DME (dimethyl-ether) and Ar/iC{sub 4}H{sub 10} mixtures. The measured curves were fitted with the outcome of a theoretical model. In the model, the physical Landau distribution is approximated by a Poisson distribution that is convoluted with the variation of the gas gain and the electronic noise. The value for the fraction of pedestal events is used for a direct calculation of the cluster density. For some gases, the measured cluster density is considerably lower than given in literature.

  1. Charge amplitude distribution of the Gossip gaseous pixel detector

    Science.gov (United States)

    Blanco Carballo, V. M.; Chefdeville, M.; Colas, P.; Giomataris, Y.; van der Graaf, H.; Gromov, V.; Hartjes, F.; Kluit, R.; Koffeman, E.; Salm, C.; Schmitz, J.; Smits, S. M.; Timmermans, J.; Visschers, J. L.

    2007-12-01

    The Gossip gaseous pixel detector is being developed for the detection of charged particles in extreme high radiation environments as foreseen close to the interaction point of the proposed super LHC. The detecting medium is a thin layer of gas. Because of the low density of this medium, only a few primary electron/ion pairs are created by the traversing particle. To get a detectable signal, the electrons drift towards a perforated metal foil (Micromegas) whereafter they are multiplied in a gas avalanche to provide a detectable signal. The gas avalanche occurs in the high field between the Micromegas and the pixel readout chip (ROC). Compared to a silicon pixel detector, Gossip features a low material budget and a low cooling power. An experiment using X-rays has indicated a possible high radiation tolerance exceeding 10 16 hadrons/cm 2. The amplified charge signal has a broad amplitude distribution due to the limited statistics of the primary ionization and the statistical variation of the gas amplification. Therefore, some degree of inefficiency is inevitable. This study presents experimental results on the charge amplitude distribution for CO 2/DME (dimethyl-ether) and Ar/iC 4H 10 mixtures. The measured curves were fitted with the outcome of a theoretical model. In the model, the physical Landau distribution is approximated by a Poisson distribution that is convoluted with the variation of the gas gain and the electronic noise. The value for the fraction of pedestal events is used for a direct calculation of the cluster density. For some gases, the measured cluster density is considerably lower than given in literature.

  2. Charge amplitude distribution of the Gossip gaseous pixel detector

    International Nuclear Information System (INIS)

    Blanco Carballo, V.M.; Chefdeville, M.; Colas, P.; Giomataris, Y.; Graaf, H. van der; Gromov, V.; Hartjes, F.; Kluit, R.; Koffeman, E.; Salm, C.; Schmitz, J.; Smits, S.M.; Timmermans, J.; Visschers, J.L.

    2007-01-01

    The Gossip gaseous pixel detector is being developed for the detection of charged particles in extreme high radiation environments as foreseen close to the interaction point of the proposed super LHC. The detecting medium is a thin layer of gas. Because of the low density of this medium, only a few primary electron/ion pairs are created by the traversing particle. To get a detectable signal, the electrons drift towards a perforated metal foil (Micromegas) whereafter they are multiplied in a gas avalanche to provide a detectable signal. The gas avalanche occurs in the high field between the Micromegas and the pixel readout chip (ROC). Compared to a silicon pixel detector, Gossip features a low material budget and a low cooling power. An experiment using X-rays has indicated a possible high radiation tolerance exceeding 10 16 hadrons/cm 2 . The amplified charge signal has a broad amplitude distribution due to the limited statistics of the primary ionization and the statistical variation of the gas amplification. Therefore, some degree of inefficiency is inevitable. This study presents experimental results on the charge amplitude distribution for CO 2 /DME (dimethyl-ether) and Ar/iC 4 H 10 mixtures. The measured curves were fitted with the outcome of a theoretical model. In the model, the physical Landau distribution is approximated by a Poisson distribution that is convoluted with the variation of the gas gain and the electronic noise. The value for the fraction of pedestal events is used for a direct calculation of the cluster density. For some gases, the measured cluster density is considerably lower than given in literature

  3. Interplay of electronic and geometry shell effects in properties of neutral and charged Sr clusters

    DEFF Research Database (Denmark)

    Lyalin, Andrey; Solov'yov, Ilia; Solov'yov, Andrey V.

    2007-01-01

    that the size evolution of structural and electronic properties of strontium clusters is governed by an interplay of the electronic and geometry shell closures. Influence of the electronic shell effects on structural rearrangements can lead to violation of the icosahedral growth motif of strontium clusters......The optimized structure and electronic properties of neutral, singly, and doubly charged strontium clusters have been investigated using ab initio theoretical methods based on density-functional theory. We have systematically calculated the optimized geometries of neutral, singly, and doubly...... charged strontium clusters consisting of up to 14 atoms, average bonding distances, electronic shell closures, binding energies per atom, the gap between the highest occupied and the lowest unoccupied molecular orbitals, and spectra of the density of electronic states (DOS). It is demonstrated...

  4. Charge injection engineering of ambipolar field-effect transistors for high-performance organic complementary circuits.

    Science.gov (United States)

    Baeg, Kang-Jun; Kim, Juhwan; Khim, Dongyoon; Caironi, Mario; Kim, Dong-Yu; You, In-Kyu; Quinn, Jordan R; Facchetti, Antonio; Noh, Yong-Young

    2011-08-01

    Ambipolar π-conjugated polymers may provide inexpensive large-area manufacturing of complementary integrated circuits (CICs) without requiring micro-patterning of the individual p- and n-channel semiconductors. However, current-generation ambipolar semiconductor-based CICs suffer from higher static power consumption, low operation frequencies, and degraded noise margins compared to complementary logics based on unipolar p- and n-channel organic field-effect transistors (OFETs). Here, we demonstrate a simple methodology to control charge injection and transport in ambipolar OFETs via engineering of the electrical contacts. Solution-processed caesium (Cs) salts, as electron-injection and hole-blocking layers at the interface between semiconductors and charge injection electrodes, significantly decrease the gold (Au) work function (∼4.1 eV) compared to that of a pristine Au electrode (∼4.7 eV). By controlling the electrode surface chemistry, excellent p-channel (hole mobility ∼0.1-0.6 cm(2)/(Vs)) and n-channel (electron mobility ∼0.1-0.3 cm(2)/(Vs)) OFET characteristics with the same semiconductor are demonstrated. Most importantly, in these OFETs the counterpart charge carrier currents are highly suppressed for depletion mode operation (I(off) 0.1-0.2 mA). Thus, high-performance, truly complementary inverters (high gain >50 and high noise margin >75% of ideal value) and ring oscillators (oscillation frequency ∼12 kHz) based on a solution-processed ambipolar polymer are demonstrated.

  5. Electronic charge rearrangement at metal/organic interfaces induced by weak van der Waals interactions

    Science.gov (United States)

    Ferri, Nicola; Ambrosetti, Alberto; Tkatchenko, Alexandre

    2017-07-01

    Electronic charge rearrangements at interfaces between organic molecules and solid surfaces play a key role in a wide range of applications in catalysis, light-emitting diodes, single-molecule junctions, molecular sensors and switches, and photovoltaics. It is common to utilize electrostatics and Pauli pushback to control the interface electronic properties, while the ubiquitous van der Waals (vdW) interactions are often considered to have a negligible direct contribution (beyond the obvious structural relaxation). Here, we apply a fully self-consistent Tkatchenko-Scheffler vdW density functional to demonstrate that the weak vdW interactions can induce sizable charge rearrangements at hybrid metal/organic systems (HMOS). The complex vdW correlation potential smears out the interfacial electronic density, thereby reducing the charge transfer in HMOS, changes the interface work functions by up to 0.2 eV, and increases the interface dipole moment by up to 0.3 Debye. Our results suggest that vdW interactions should be considered as an additional control parameter in the design of hybrid interfaces with the desired electronic properties.

  6. Controlling nonlinear longitudinal space charge oscillations for high peak current bunch train generation

    Directory of Open Access Journals (Sweden)

    P. Musumeci

    2013-10-01

    Full Text Available The evolution of picosecond modulations of the longitudinal profile of an electron beam generated in an rf photoinjector is analyzed and optimized with the goal of obtaining high peak current electron bunch trains at very high frequencies (≥THz. Taking advantage of nonlinear longitudinal space charge forces, it is found that more than 500 A peak current 1 THz bunch trains can be generated using a standard 1.6 cell SLAC/UCLA/BNL rf gun. Postacceleration is used to freeze the longitudinal phase space dynamics after one half plasma oscillation. Applications range from tunable narrow bandwidth THz radiation generation to drivers for high frequency high gradient accelerators.

  7. Charge Screening in a Charged Condensate

    International Nuclear Information System (INIS)

    Gabadadze, Gregory; Rosen, Rachel A.

    2009-01-01

    We consider a highly dense system of helium-4 nuclei and electrons in which the helium-4 nuclei have condensed. We present the condensation mechanism in the framework of low energy effective field theory and discuss the screening of electric charge in the condensate.

  8. Electron bunch profile reconstruction in the few fs regime using coherent Smith-Purcell radiation

    International Nuclear Information System (INIS)

    Bartolini, R; Delerue, N; Doucas, G; Reichold, A; Clarke, C

    2012-01-01

    Advanced accelerators for fourth generation light sources based on high brightness linacs or laser-driven wakefield accelerators will operate with intense, highly relativistic electron bunches that are only a few fs long. Diagnostic techniques for the determination of temporal profile of such bunches are required to be non invasive, single shot, economic and with the required resolution in the fs regime. The use of a radiative process such as coherent Smith-Purcell radiation (SPR), is particularly promising with this respect. In this technique the beam is made to radiate a small amount of electromagnetic radiation and the temporal profile is reconstructed from the measured spectral distribution of the radiation. We summarise the advantages of SPR and present the design parameters and preliminary results of the experiments at the FACET facility at SLAC. We also discuss a new approach to the problem of the recovery of the 'missing phase', which is essential for the accurate reconstruction of the temporal bunch profile.

  9. Electron Bunch Profile Reconstruction in the Few fs Regime using Coherent Smith-Purcell Radiation

    International Nuclear Information System (INIS)

    Bartolini, R.; Clarke, C.; Delerue, N.; Doucasa, G.; Reicholda, A.

    2012-01-01

    Advanced accelerators for fourth generation light sources based on high brightness linacs or laser-driven wakefield accelerators will operate with intense, highly relativistic electron bunches that are only a few fs long. Diagnostic techniques for the determination of temporal profile of such bunches are required to be non invasive, single shot, economic and with the required resolution in the fs regime. The use of a radiative process such as coherent Smith-Purcell radiation (SPR), is particularly promising with this respect. In this technique the beam is made to radiate a small amount of electromagnetic radiation and the temporal profile is reconstructed from the measured spectral distribution of the radiation. We summarise the advantages of SPR and present the design parameters and preliminary results of the experiments at the FACET facility at SLAC. We also discuss a new approach to the problem of the recovery of the 'missing phase', which is essential for the accurate reconstruction of the temporal bunch profile.

  10. Understanding the effects of electronic polarization and delocalization on charge-transport levels in oligoacene systems

    KAUST Repository

    Sutton, Christopher; Tummala, Naga Rajesh; Kemper, Travis; Aziz, Saadullah G.; Sears, John; Coropceanu, Veaceslav; Bredas, Jean-Luc

    2017-01-01

    Electronic polarization and charge delocalization are important aspects that affect the charge-transport levels in organic materials. Here, using a quantum mechanical/ embedded-charge (QM/EC) approach based on a combination of the long-range corrected omega B97X-D exchange-correlation functional (QM) and charge model 5 (CM5) point-charge model (EC), we evaluate the vertical detachment energies and polarization energies of various sizes of crystalline and amorphous anionic oligoacene clusters. Our results indicate that QM/EC calculations yield vertical detachment energies and polarization energies that compare well with the experimental values obtained from ultraviolet photoemission spectroscopy measurements. In order to understand the effect of charge delocalization on the transport levels, we considered crystalline naphthalene systems with QM regions including one or five-molecules. The results for these systems show that the delocalization and polarization effects are additive; therefore, allowing for electron delocalization by increasing the size of the QM region leads to the additional stabilization of the transport levels. Published by AIP Publishing.

  11. Understanding the effects of electronic polarization and delocalization on charge-transport levels in oligoacene systems

    KAUST Repository

    Sutton, Christopher

    2017-06-13

    Electronic polarization and charge delocalization are important aspects that affect the charge-transport levels in organic materials. Here, using a quantum mechanical/ embedded-charge (QM/EC) approach based on a combination of the long-range corrected omega B97X-D exchange-correlation functional (QM) and charge model 5 (CM5) point-charge model (EC), we evaluate the vertical detachment energies and polarization energies of various sizes of crystalline and amorphous anionic oligoacene clusters. Our results indicate that QM/EC calculations yield vertical detachment energies and polarization energies that compare well with the experimental values obtained from ultraviolet photoemission spectroscopy measurements. In order to understand the effect of charge delocalization on the transport levels, we considered crystalline naphthalene systems with QM regions including one or five-molecules. The results for these systems show that the delocalization and polarization effects are additive; therefore, allowing for electron delocalization by increasing the size of the QM region leads to the additional stabilization of the transport levels. Published by AIP Publishing.

  12. Electronic structure, Born effective charges and spontaneous polarization in magnetoelectric gallium ferrite

    International Nuclear Information System (INIS)

    Roy, Amritendu; Garg, Ashish; Mukherjee, Somdutta; Gupta, Rajeev; Prasad, Rajendra; Auluck, Sushil

    2011-01-01

    We present a theoretical study of the structure-property correlation in gallium ferrite, based on first-principles calculations followed by a subsequent comparison with experiments. The local spin density approximation (LSDA + U) of the density functional theory has been used to calculate the ground state structure, electronic band structure, density of states and Born effective charges. The calculations reveal that the ground state structure is orthorhombic Pc 2 1 n having A-type antiferromagnetic spin configuration, with lattice parameters matching well with those obtained experimentally. Plots of the partial density of states of constituent ions exhibit noticeable hybridization of Fe 3d, Ga 4s, Ga 4p and O 2p states. However, the calculated charge density and electron localization function show a largely ionic character of the Ga/Fe-O bonds which is also supported by a lack of any significant anomaly in the calculated Born effective charges with respect to the corresponding nominal ionic charges. The calculations show a spontaneous polarization of ∼ 59 μC cm -2 along the b-axis which is largely due to asymmetrically placed Ga1, Fe1, O1, O2 and O6 ions.

  13. Few-Photon Multiple Ionization of Ne and Ar by Strong Free-Electron-Laser Pulses

    International Nuclear Information System (INIS)

    Moshammer, R.; Jiang, Y. H.; Rudenko, A.; Ergler, Th.; Schroeter, C. D.; Luedemann, S.; Zrost, K.; Dorn, A.; Ferger, T.; Kuehnel, K. U.; Ullrich, J.; Foucar, L.; Titze, J.; Jahnke, T.; Schoeffler, M.; Doerner, R.; Fischer, D.; Weber, T.; Zouros, T. J. M.; Duesterer, S.

    2007-01-01

    Few-photon multiple ionization of Ne and Ar atoms by strong vacuum ultraviolet laser pulses from the free-electron laser at Hamburg was investigated differentially with the Heidelberg reaction microscope. The light-intensity dependence of Ne 2+ production reveals the dominance of nonsequential two-photon double ionization at intensities of I 12 W/cm 2 and significant contributions of three-photon ionization as I increases. Ne 2+ recoil-ion-momentum distributions suggest that two electrons absorbing ''instantaneously'' two photons are ejected most likely into opposite hemispheres with similar energies

  14. Development of a high average current polarized electron source with long cathode operational lifetime

    Energy Technology Data Exchange (ETDEWEB)

    C. K. Sinclair; P. A. Adderley; B. M. Dunham; J. C. Hansknecht; P. Hartmann; M. Poelker; J. S. Price; P. M. Rutt; W. J. Schneider; M. Steigerwald

    2007-02-01

    Substantially more than half of the electromagnetic nuclear physics experiments conducted at the Continuous Electron Beam Accelerator Facility of the Thomas Jefferson National Accelerator Facility (Jefferson Laboratory) require highly polarized electron beams, often at high average current. Spin-polarized electrons are produced by photoemission from various GaAs-based semiconductor photocathodes, using circularly polarized laser light with photon energy slightly larger than the semiconductor band gap. The photocathodes are prepared by activation of the clean semiconductor surface to negative electron affinity using cesium and oxidation. Historically, in many laboratories worldwide, these photocathodes have had short operational lifetimes at high average current, and have often deteriorated fairly quickly in ultrahigh vacuum even without electron beam delivery. At Jefferson Lab, we have developed a polarized electron source in which the photocathodes degrade exceptionally slowly without electron emission, and in which ion back bombardment is the predominant mechanism limiting the operational lifetime of the cathodes during electron emission. We have reproducibly obtained cathode 1/e dark lifetimes over two years, and 1/e charge density and charge lifetimes during electron beam delivery of over 2?105???C/cm2 and 200 C, respectively. This source is able to support uninterrupted high average current polarized beam delivery to three experimental halls simultaneously for many months at a time. Many of the techniques we report here are directly applicable to the development of GaAs photoemission electron guns to deliver high average current, high brightness unpolarized beams.

  15. Space-charge-limited currents in electron-irradiated dielectrics

    International Nuclear Information System (INIS)

    Nunes de Oliveira, L.; Gross, B.

    1975-01-01

    This paper develops the theory of steady-state currents generated in a dielectric placed between positively or negatively biased electrodes and irradiated with a partially penetrating electron beam. The dielectric is divided into an irradiated region (IR), which extends from the electrode of incidence to the extrapolated range of the beam, and a nonirradiated region (NIR). In the IR the primary beam generates an electron-hole plasma. Its end plane acts as a virtual electrode embedded in the dielectric. Currents are space-charge limited in the NIR and Ohmic in the IR which is characterized by a uniform radiation-induced conductivity. Depending on the polarity of the electrode bias, electrons or holes are drawn from the IR into the NIR. The theory correctly predicts an apparent threshold effect for the inset of steady-state currents: the current amplitudes remain small as long as the electron range is smaller than half the sample thickness, and increase strongly only afterwards. Calculated current curves for different beam energies are in satisfactory agreement with experimental results. The role of the electron beam as a virtual electrode is discussed

  16. Single-crystal charge transfer interfaces for efficient photonic devices (Conference Presentation)

    Science.gov (United States)

    Alves, Helena; Pinto, Rui M.; Maçôas, Ermelinda M. S.; Baleizão, Carlos; Santos, Isabel C.

    2016-09-01

    Organic semiconductors have unique optical, mechanical and electronic properties that can be combined with customized chemical functionality. In the crystalline form, determinant features for electronic applications such as molecular purity, the charge mobility or the exciton diffusion length, reveal a superior performance when compared with materials in a more disordered form. Combining crystals of two different conjugated materials as even enable a new 2D electronic system. However, the use of organic single crystals in devices is still limited to a few applications, such as field-effect transistors. In 2013, we presented the first system composed of single-crystal charge transfer interfaces presenting photoconductivity behaviour. The system composed of rubrene and TCNQ has a responsivity reaching 1 A/W, corresponding to an external quantum efficiency of nearly 100%. A similar approach, with a hybrid structure of a PCBM film and rubrene single crystal also presents high responsivity and the possibility to extract excitons generated in acceptor materials. This strategy led to an extended action towards the near IR. By adequate material design and structural organisation of perylediimides, we demonstrate that is possible to improve exciton diffusion efficiency. More recently, we have successfully used the concept of charge transfer interfaces in phototransistors. These results open the possibility of using organic single-crystal interfaces in photonic applications.

  17. Study on discrete space charge effects in electron beams and guns

    International Nuclear Information System (INIS)

    Tang Tiantong

    1990-01-01

    The discrete space charge effects in electron beams are studied and a statistical dynamics equation of the ensemble of beam electrons is derived. An approximated analytical solution of this equation is given. This equation has been applied to beam crossover and field-emission and thermal-emission gun problems. The computer calculation results agree on the whole with those of Monte Carlo simulation and experimental data. (orig.)

  18. Channel mobility degradation and charge trapping in high-k/metal gate NMOSFETs

    International Nuclear Information System (INIS)

    Mathew, Shajan; Bera, L.K.; Balasubramanian, N.; Joo, M.S.; Cho, B.J.

    2004-01-01

    NMOSFETs with Metalo-Organic Chemical Vapor Deposited (MOCVD) HfAlO gate dielectric and TiN metal gate have been fabricated. Channel electron mobility was measured using the split-CV method and compared with SiO 2 devices. All high-k devices showed lower mobility compared with SiO 2 reference devices. High-k MOSFETs exhibited significant charge trapping and threshold instability. Threshold voltage recovery with time was studied on devices with oxide/nitride interfacial layer between high-k film and silicon substrate

  19. Tuning electronic properties of graphene nanoflake polyaromatic hydrocarbon through molecular charge-transfer interactions

    Science.gov (United States)

    Sharma, Vaishali; Dabhi, Shweta D.; Shinde, Satyam; Jha, Prafulla K.

    2018-05-01

    By means of first principles calculation we have tuned the electronic properties of graphene nanoflake polyaromatic hydrocarbon via molecular charge transfer. Acceptor/donor Tetracyanoquinodimethane (TCNQ) and Tetrathiafulvalene (TTF) organic molecules are adsorbed on polyaromatic hydrocarbons (PAH) in order to introduce the charge transfer. The substrate's n- or p- type nature depends on the accepting/donating behavior of dopant molecules. Two different classes of PAH (extended form of triangulene) namely Bow-tie graphene nanoflake (BTGNF) and triangular zigzag graphene nanoflake (TZGNF). It is revealed that all the TCNQ and TTF modified graphene nanoflakes exhibit significant changes in HOMO-LUMO gap in range from 0.58 eV to 0.64 eV and 0.01 eV to 0.05 eV respectively. The adsorption energies are in the range of -0.05 kcal/mol to -2.6 kcal/mol. The change in work function is also calculated and discussed, the maximum charge transfer is for TCNQ adsorbed BTGNF. These alluring findings in the tuning of electronic properties will be advantageous for promoting graphene nanoflake polyaromatic hydrocarbon for their applications in electronic devices.

  20. Modification of diode characteristics by electron back-scatter from high-atomic-number anodes

    International Nuclear Information System (INIS)

    Mosher, D.; Cooperstein, G.; Rose, D.V.; Swanekamp, S.B.

    1996-01-01

    In high-power vacuum diodes with high-atomic-number anodes, back-scattered electrons alter the vacuum space charge and resulting electron and ion currents. Electron multiple back-scattering was studied through equilibrium solutions of the Poisson equation for 1-dimensional, bipolar diodes in order to predict their early-time behavior. Before ion turn-on, back-scattered electrons from high-Z anodes suppress the diode current by about 10%. After ion turn-on in the same diodes, electron back-scatter leads to substantial enhancements of both the electron and ion currents above the Child-Langmuir values. Current enhancements with ion flow from low-Z anodes are small. (author). 5 figs., 7 refs