WorldWideScience

Sample records for ferromagnetic spin ordering

  1. Defect and adsorbate induced ferromagnetic spin-order in magnesium oxide nanocrystallites

    Science.gov (United States)

    Kumar, Ashok; Kumar, Jitendra; Priya, Shashank

    2012-05-01

    We report the correlation between d0 ferromagnetism, photoluminescence (PL), and adsorbed hydrogen (H-) species in magnesium oxide (MgO) nanocrystallites. Our study suggests that the oxygen vacancies, namely singly ionized anionic vacancies (F+) and dimers (F22+) induce characteristic photoluminescence and the room-temperature ferromagnetic spin-order. Nanocrystallites with low population of oxygen vacancies have revealed diamagnetic behavior. Intriguingly, on adsorption of hydrogen (H-) species in the MgO nanocrystallites, ferromagnetic behavior was either enhanced (in the case of highly oxygen deficient nanocrystallites) or begun to percolate (in the case of nanocrystallite with low population density of oxygen vacancies).

  2. Spin-lattice dynamics simulation of external field effect on magnetic order of ferromagnetic iron

    International Nuclear Information System (INIS)

    Chui, C. P.; Zhou, Yan

    2014-01-01

    Modeling of field-induced magnetization in ferromagnetic materials has been an active topic in the last dozen years, yet a dynamic treatment of distance-dependent exchange integral has been lacking. In view of that, we employ spin-lattice dynamics (SLD) simulations to study the external field effect on magnetic order of ferromagnetic iron. Our results show that an external field can increase the inflection point of the temperature. Also the model provides a better description of the effect of spin correlation in response to an external field than the mean-field theory. An external field has a more prominent effect on the long range magnetic order than on the short range counterpart. Furthermore, an external field allows the magnon dispersion curves and the uniform precession modes to exhibit magnetic order variation from their temperature dependence

  3. First-order transition on the frustrated spin-1/2 Heisenberg ferromagnet on an anisotropic square lattice

    Energy Technology Data Exchange (ETDEWEB)

    Lapa, Rodrigo S.; Mendonça, Griffith [Departamento de Fi' sica, Universidade Federal de Minas Gerais, CP 702, 30161-970 Belo Horizonte, MG (Brazil); Universidade Federal do Amazonas, Departamento de Fi' sica, 3000, Japiim, 69077-000 Manaus, AM (Brazil); Roberto Viana, J. [Universidade Federal do Amazonas, Departamento de Fi' sica, 3000, Japiim, 69077-000 Manaus, AM (Brazil); Ricardo de Sousa, J., E-mail: jsousa@ufam.edu.br [Universidade Federal do Amazonas, Departamento de Fi' sica, 3000, Japiim, 69077-000 Manaus, AM (Brazil); National Institute of Science and Technology for Complex Systems, Universidade Federal do Amazonas, Departamento de Fisica, 3000, Japiim, 69077-000 Manaus, AM (Brazil)

    2014-11-15

    We have studied the quantum spin-1/2 frustrated Heisenberg model with two ferromagnetic interactions: nearest-neighbor (NN) with different coupling strengths J{sub 1} and J{sub 1}{sup ′} along x and y directions, respectively, competing with a next-nearest-neighbor (NNN) with coupling J{sub 2}. Using the effective-field theory we obtain the ground-state phase diagram in the (λ,α) space, where λ=J{sub 1}{sup ′}/J{sub 1} and α=J{sub 2}/J{sub 1}. Depending on the values of λ and α we observe three different states: ferromagnetic (F), collinear ferromagnetic (CF) and quantum paramagnetic (QP). We observe a QP state between the ordered F and CF phases in the region λ{sub 1}<λ<1 (λ{sub 1}≃0.62). - Highlights: • We study the ferromagnetic J{sub 1}−J{sub 1}{sup ′}−J{sub 2} model on an anisotropic square lattice by using effective-field theory. • We obtain the ground phase diagram in the λ−α plane (λ=J{sub 1}{sup ′}/J{sub 1} and α=J{sub 2}/J{sub 1}). • A comparison with the results of the antiferromagnetic J{sub 1}−J{sub 1}{sup ′}−J{sub 2} model. • We propose a functional for the free energy.

  4. Spin Currents and Spin Orbit Torques in Ferromagnets and Antiferromagnets

    Science.gov (United States)

    Hung, Yu-Ming

    This thesis focuses on the interactions of spin currents and materials with magnetic order, e.g., ferromagnetic and antiferromagnetic thin films. The spin current is generated in two ways. First by spin-polarized conduction-electrons associated with the spin Hall effect in heavy metals (HMs) and, second, by exciting spin-waves in ferrimagnetic insulators using a microwave frequency magnetic field. A conduction-electron spin current can be generated by spin-orbit coupling in a heavy non-magnetic metal and transfer its spin angular momentum to a ferromagnet, providing a means of reversing the magnetization of perpendicularly magnetized ultrathin films with currents that flow in the plane of the layers. The torques on the magnetization are known as spin-orbit torques (SOT). In the first part of my thesis project I investigated and contrasted the quasistatic (slowly swept current) and pulsed current-induced switching characteristics of micrometer scale Hall crosses consisting of very thin (thesis project studies and considers applications of SOT-driven domain wall (DW) motion in a perpendicularly magnetized ultrathin ferromagnet sandwiched between a heavy metal and an oxide. My experiment results demonstrate that the DW motion can be explained by a combination of the spin Hall effect, which generates a SOT, and Dzyaloshinskii-Moriya interaction, which stabilizes chiral Neel-type DW. Based on SOT-driven DW motion and magnetic coupling between electrically isolated ferromagnetic elements, I proposed a new type of spin logic devices. I then demonstrate the device operation by using micromagnetic modeling which involves studying the magnetic coupling induced by fringe fields from chiral DWs in perpendicularly magnetized nanowires. The last part of my thesis project reports spin transport and spin-Hall magnetoresistance (SMR) in yttrium iron garnet Y3Fe5O 12 (YIG)/NiO/Pt trilayers with varied NiO thickness. To characterize the spin transport through NiO we excite

  5. Spin Orbit Torque in Ferromagnetic Semiconductors

    KAUST Repository

    Li, Hang

    2016-06-21

    Electrons not only have charges but also have spin. By utilizing the electron spin, the energy consumption of electronic devices can be reduced, their size can be scaled down and the efficiency of `read\\' and `write\\' in memory devices can be significantly improved. Hence, the manipulation of electron spin in electronic devices becomes more and more appealing for the advancement of microelectronics. In spin-based devices, the manipulation of ferromagnetic order parameter using electrical currents is a very useful means for current-driven operation. Nowadays, most of magnetic memory devices are based on the so-called spin transfer torque, which stems from the spin angular momentum transfer between a spin-polarized current and the magnetic order parameter. Recently, a novel spin torque effect, exploiting spin-orbit coupling in non-centrosymmetric magnets, has attracted a massive amount of attention. This thesis addresses the nature of spin-orbit coupled transport and torques in non-centrosymmetric magnetic semiconductors. We start with the theoretical study of spin orbit torque in three dimensional ferromagnetic GaMnAs. Using the Kubo formula, we calculate both the current-driven field-like torque and anti-damping-like torque. We compare the numerical results with the analytical expressions in the model case of a magnetic Rashba two-dimensional electron gas. Parametric dependencies of the different torque components and similarities to the analytical results of the Rashba two-dimensional electron gas in the weak disorder limit are described. Subsequently we study spin-orbit torques in two dimensional hexagonal crystals such as graphene, silicene, germanene and stanene. In the presence of staggered potential and exchange field, the valley degeneracy can be lifted and we obtain a valley-dependent Berry curvature, leading to a tunable antidamping torque by controlling the valley degree of freedom. This thesis then addresses the influence of the quantum spin Hall

  6. Spin Hall and spin swapping torques in diffusive ferromagnets

    KAUST Repository

    Pauyac, C. O.

    2017-12-08

    A complete set of the generalized drift-diffusion equations for a coupled charge and spin dynamics in ferromagnets in the presence of extrinsic spin-orbit coupling is derived from the quantum kinetic approach, covering major transport phenomena, such as the spin and anomalous Hall effects, spin swapping, spin precession and relaxation processes. We argue that the spin swapping effect in ferromagnets is enhanced due to spin polarization, while the overall spin texture induced by the interplay of spin-orbital and spin precessional effects displays a complex spatial dependence that can be exploited to generate torques and nucleate/propagate domain walls in centrosymmetric geometries without use of external polarizers, as opposed to the conventional understanding of spin-orbit mediated torques.

  7. Spin dynamics with inertia in metallic ferromagnets

    Science.gov (United States)

    Kikuchi, Toru; Tatara, Gen

    2015-11-01

    The nonadiabatic contribution of environmental degrees of freedom yields an effective inertia of spin in the effective spin dynamics. In this paper, we study several aspects of the inertia of spin in metallic ferromagnets: (i) a concrete expression of the spin inertia ms: ms=ℏ Sc/(2 gsd) , where Sc is the spin polarization of conduction electrons and gsd is the s d coupling constant; (ii) a dynamical behavior of spin with inertia, discussed from the viewpoints of a spinning top and of a particle on a sphere; (iii) the behavior of spin waves and domain walls in the presence of inertia and the behavior of spin with inertia under a time-dependent magnetic field.

  8. Model for ballistic spin-transport in ferromagnet/two-dimensional electron gas/ferromagnet structures

    NARCIS (Netherlands)

    Schapers, T; Nitta, J; Heersche, HB; Takayanagi, H

    The spin dependent conductance of a ferromagnet/two-dimensional electron gas ferromagnet structure is theoretically examined in the ballistic transport regime. It is shown that the spin signal can be improved considerably by making use of the spin filtering effect of a barrier at the ferromagnet

  9. Integrability and soliton solutions for an inhomogeneous generalized fourth-order nonlinear Schrödinger equation describing the inhomogeneous alpha helical proteins and Heisenberg ferromagnetic spin chains

    International Nuclear Information System (INIS)

    Wang, Pan; Tian, Bo; Jiang, Yan; Wang, Yu-Feng

    2013-01-01

    For describing the dynamics of alpha helical proteins with internal molecular excitations, nonlinear couplings between lattice vibrations and molecular excitations, and spin excitations in one-dimensional isotropic biquadratic Heisenberg ferromagnetic spin with the octupole–dipole interactions, we consider an inhomogeneous generalized fourth-order nonlinear Schrödinger equation. Based on the Ablowitz–Kaup–Newell–Segur system, infinitely many conservation laws for the equation are derived. Through the auxiliary function, bilinear forms and N-soliton solutions for the equation are obtained. Interactions of solitons are discussed by means of the asymptotic analysis. Effects of linear inhomogeneity on the interactions of solitons are also investigated graphically and analytically. Since the inhomogeneous coefficient of the equation h=α x+β, the soliton takes on the parabolic profile during the evolution. Soliton velocity is related to the parameter α, distance scale coefficient and biquadratic exchange coefficient, but has no relation with the parameter β. Soliton amplitude and width are only related to α. Soliton position is related to β

  10. Ferromagnetic ordered phase of quantum spin ice system Yb{sub 2}Ti{sub 2}O{sub 7} under [001] magnetic field

    Energy Technology Data Exchange (ETDEWEB)

    Hamachi, Noriaki, E-mail: ce46414@meiji.ac.jp; Yasui, Yukio [Department of Physics, School of Science and Technology, Meiji University, Kawasaki, 214-8571 (Japan); Araki, Koji [Institute for Solid State Physics, The University of Tokyo, Kashiwa, 277-8581 (Japan); Department of Applied Physics, National Defense Academy, Yokosuka, 239-8686 (Japan); Kittaka, Shunichiro; Sakakibara, Toshiro [Institute for Solid State Physics, The University of Tokyo, Kashiwa, 277-8581 (Japan)

    2016-05-15

    Measurements of magnetization (M) and specific heat (C) under a [001] magnetic field were carried out on a single crystal of a quantum spin ice system Yb{sub 2}Ti{sub 2}O{sub 7} in order to investigate a feature of the transition occurred at T{sub C} ∼ 0.2 K. As a result of applying the magnetic field μ{sub 0}H < 0.1 T, the C/T − T curve structure and transition temperature barely changed. On the other hand, applying the more than 0.1 T magnetic field, the C/T − T curve structure drastically change from sharp peak structure to broad peak one, and the broad peak temperature of C/T − T curves linearly increases with increasing magnetic field (H). In the magnetic field μ{sub 0}H < 0.1 T, the magnetization drastically increases around T{sub C} ∼ 0.2 K with decreasing T, and a thermal hysteresis loop of the M − T curve is observed. With increasing H, the thermal hysteresis loop of the M − T curves disappears above μ{sub 0}H{sub C} = 0.1 T. We can understand these results, where Yb{sub 2}Ti{sub 2}O{sub 7} exhibits a first-order ferromagnetic transition associated with the latent heat corresponding to the energy of μ{sub 0}H{sub C} = 0.1 T. Basis of the H − T phase diagram along [001] magnetic field, the feature of the transition occurred at T{sub C} ∼ 0.2 K in quantum spin ice system Yb{sub 2}Ti{sub 2}O{sub 7} is discussed.

  11. Spin Transport in Ferromagnetic and Antiferromagnetic Textures

    KAUST Repository

    Akosa, Collins A.

    2016-12-07

    In this dissertation, we provide an accurate description of spin transport in magnetic textures and in particular, we investigate in detail, the nature of spin torque and magnetic damping in such systems. Indeed, as will be further discussed in this thesis, the current-driven velocity of magnetic textures is related to the ratio between the so-called non-adiabatic torque and magnetic damping. Uncovering the physics underlying these phenomena can lead to the optimal design of magnetic systems with improved efficiency. We identified three interesting classes of systems which have attracted enormous research interest (i) Magnetic textures in systems with broken inversion symmetry: We investigate the nature of magnetic damping in non-centrosymmetric ferromagnets. Based on phenomenological and microscopic derivations, we show that the magnetic damping becomes chiral, i.e. depends on the chirality of the magnetic texture. (ii) Ferromagnetic domain walls, skyrmions and vortices: We address the physics of spin transport in sharp disordered magnetic domain walls and vortex cores. We demonstrate that upon spin-independent scattering, the non-adiabatic torque can be significantly enhanced. Such an enhancement is large for vortex cores compared to transverse domain walls. We also show that the topological spin currents owing in these structures dramatically enhances the non-adiabaticity, an effect unique to non-trivial topological textures (iii) Antiferromagnetic skyrmions: We extend this study to antiferromagnetic skyrmions and show that such an enhanced topological torque also exist in these systems. Even more interestingly, while such a non-adiabatic torque inuences the undesirable transverse velocity of ferromagnetic skyrmions, in antiferromagnetic skyrmions, the topological non-adiabatic torque directly determines the longitudinal velocity. As a consequence, scaling down the antiferromagnetic skyrmion results in a much more efficient spin torque.

  12. The ferromagnetic-spin glass transition in PdMn alloys: symmetry breaking of ferromagnetism and spin glass studied by a multicanonical method.

    Science.gov (United States)

    Kato, Tomohiko; Saita, Takahiro

    2011-03-16

    The magnetism of Pd(1-x)Mn(x) is investigated theoretically. A localized spin model for Mn spins that interact with short-range antiferromagnetic interactions and long-range ferromagnetic interactions via itinerant d electrons is set up, with no adjustable parameters. A multicanonical Monte Carlo simulation, combined with a procedure of symmetry breaking, is employed to discriminate between the ferromagnetic and spin glass orders. The transition temperature and the low-temperature phase are determined from the temperature variation of the specific heat and the probability distributions of the ferromagnetic order parameter and the spin glass order parameter at different concentrations. The calculation results reveal that only the ferromagnetic phase exists at x glass phase exists at x > 0.04, and that the two phases coexist at intermediate concentrations. This result agrees semi-quantitatively with experimental results.

  13. Spin-flip scattering effect on the current-induced spin torque in ferromagnet-insulator-ferromagnet tunnel junctions

    International Nuclear Information System (INIS)

    Zhu Zhengang; Su Gang; Jin Biao; Zheng Qingrong

    2003-01-01

    We have investigated the current-induced spin transfer torque of a ferromagnet-insulator-ferromagnet tunnel junction by taking the spin-flip scatterings into account. It is found that the spin-flip scattering can induce an additional spin torque, enhancing the maximum of the spin torque and giving rise to an angular shift compared to the case when the spin-flip scatterings are neglected. The effects of the molecular fields of the left and right ferromagnets on the spin torque are also studied. It is found that τ Rx /I e (τ Rx is the spin-transfer torque acting on the right ferromagnet and I e is the tunneling electrical current) does vary with the molecular fields. At two certain angles, τ Rx /I e is independent of the molecular field of the right ferromagnet, resulting in two crossing points in the curve of τ Rx /I e versus the relevant orientation for different molecular fields

  14. Spin Heat Accumulation Induced by Tunneling from a Ferromagnet

    NARCIS (Netherlands)

    Vera-Marun, I.J.; Wees, B.J. van; Jansen, R.

    2014-01-01

    An electric current from a ferromagnet into a nonmagnetic material can induce a spin-dependent electron temperature. Here, it is shown that this spin heat accumulation, when created by tunneling from a ferromagnet, produces a non-negligible voltage signal that is comparable to that due to the

  15. Spin heat accumulation induced by tunneling from a ferromagnet.

    Science.gov (United States)

    Vera-Marun, I J; van Wees, B J; Jansen, R

    2014-02-07

    An electric current from a ferromagnet into a nonmagnetic material can induce a spin-dependent electron temperature. Here, it is shown that this spin heat accumulation, when created by tunneling from a ferromagnet, produces a non-negligible voltage signal that is comparable to that due to the coexisting electrical spin accumulation and can give a different Hanle spin precession signature. The effect is governed by the spin polarization of the Peltier coefficient of the tunnel contact, its Seebeck coefficient, and the spin heat resistance of the nonmagnetic material, which is related to the electrical spin resistance by a spin-Wiedemann-Franz law. Moreover, spin heat injection is subject to a heat conductivity mismatch that is overcome if the tunnel interface has a sufficiently large resistance.

  16. Ballistic spin filtering across the ferromagnetic-semiconductor interface

    Directory of Open Access Journals (Sweden)

    Y.H. Li

    2012-03-01

    Full Text Available The ballistic spin-filter effect from a ferromagnetic metal into a semiconductor has theoretically been studied with an intention of detecting the spin polarizability of density of states in FM layer at a higher energy level. The physical model for the ballistic spin filtering across the interface between ferromagnetic metals and semiconductor superlattice is developed by exciting the spin polarized electrons into n-type AlAs/GaAs superlattice layer at a much higher energy level and then ballistically tunneling through the barrier into the ferromagnetic film. Since both the helicity-modulated and static photocurrent responses are experimentally measurable quantities, the physical quantity of interest, the relative asymmetry of spin-polarized tunneling conductance, could be extracted experimentally in a more straightforward way, as compared with previous models. The present physical model serves guidance for studying spin detection with advanced performance in the future.

  17. On the temperature dependence of spin pumping in ferromagnet–topological insulator–ferromagnet spin valves

    Directory of Open Access Journals (Sweden)

    A.A. Baker

    Full Text Available Topological insulators (TIs have a large potential for spintronic devices owing to their spin-polarized, counter-propagating surface states. Recently, we have investigated spin pumping in a ferromagnet–TI–ferromagnet structure at room temperature. Here, we present the temperature-dependent measurement of spin pumping down to 10 K, which shows no variation with temperature. Keywords: Topological insulator, Spin pumping, Spintronics, Ferromagnetic resonance

  18. Spin-polarized tunneling through a ferromagnetic insulator

    NARCIS (Netherlands)

    Kok, M.; Kok, M.; Beukers, J.N.; Brinkman, Alexander

    2009-01-01

    The polarization of the tunnel conductance of spin-selective ferromagnetic insulators is modeled, providing a generalized concept of polarization including both the effects of electrode and barrier polarization. The polarization model is extended to take additional non-spin-polarizing insulating

  19. Diffusive Spin Dynamics in Ferromagnetic Thin Films with a Rashba Interaction

    KAUST Repository

    Wang, Xuhui

    2012-03-13

    In a ferromagnetic metal layer, the coupled charge and spin diffusion equations are obtained in the presence of both Rashba spin-orbit interaction and magnetism. The misalignment between the magnetization and the nonequilibrium spin density induced by the Rashba field gives rise to Rashba spin torque acting on the ferromagnetic order parameter. In a general form, we find that the Rashba torque consists of both in-plane and out-of-plane components, i.e., T=T Sy×m+T Sm×(y×m). Numerical simulations on a two-dimensional nanowire consider the impact of diffusion on the Rashba torque and reveal a large enhancement to the ratio T/T S for thin wires. Our theory provides an explanation for the mechanism driving the magnetization switching in a single ferromagnet as observed in the recent experiments. © 2012 American Physical Society.

  20. Dynamic detection of spin accumulation in ferromagnet-semiconductor devices by ferromagnetic resonance (Conference Presentation)

    Science.gov (United States)

    Crowell, Paul A.; Liu, Changjiang; Patel, Sahil; Peterson, Tim; Geppert, Chad C.; Christie, Kevin; Stecklein, Gordon; Palmstrøm, Chris J.

    2016-10-01

    A distinguishing feature of spin accumulation in ferromagnet-semiconductor devices is its precession in a magnetic field. This is the basis for detection techniques such as the Hanle effect, but these approaches become ineffective as the spin lifetime in the semiconductor decreases. For this reason, no electrical Hanle measurement has been demonstrated in GaAs at room temperature. We show here that by forcing the magnetization in the ferromagnet to precess at resonance instead of relying only on the Larmor precession of the spin accumulation in the semiconductor, an electrically generated spin accumulation can be detected up to 300 K. The injection bias and temperature dependence of the measured spin signal agree with those obtained using traditional methods. We further show that this new approach enables a measurement of short spin lifetimes (C. Liu, S. J. Patel, T. A. Peterson, C. C. Geppert, K. D. Christie, C. J. Palmstrøm, and P. A. Crowell, "Dynamic detection of electron spin accumulation in ferromagnet-semiconductor devices by ferromagnetic resonance," Nature Communications 7, 10296 (2016). http://dx.doi.org/10.1038/ncomms10296

  1. Spin excitation in granular structures with ferromagnetic nanoparticles

    CERN Document Server

    Lutsev, L V

    2002-01-01

    In terms of s-d-exchange model one studied spin excitations and relaxation in granular structures with metallic ferromagnetic nanoparticles in an insulating amorphous matrix. One studies spins of granule as a d-system; s-system represents a multitude of localized electrons of amorphous matrix. In terms of single-ring approximation on the basis of s-d-exchange interaction for the Green spin function expansion one determined spectrum of spin excitations composed of spin-wave excitations of granules and spin-polarization excitations. One studied spin-polarization relaxation occurring by way of spin-polarization excitations. Spin-polarization relaxation was determined to be efficient one within wide range of frequencies. Evaluations made for structures containing cobalt granules show that one should observe it in the centimeter, the millimeter and the submillimeter ranges of wavelength

  2. Quantitative study of the spin Hall magnetoresistance in ferromagnetic insulator/normal metal hybrids

    NARCIS (Netherlands)

    Althammer, M.; Meyer, S.; Nakayama, H.; Schreier, M.; Altmannshofer, S.; Weiler, M.; Huebl, H.; Gesprägs, S.; Opel, M.; Gross, R.; Meier, D.; Klewe, C.; Kuschel, T.; Schmalhorst, J.M.; Reiss, G.; Shen, L.; Gupta, A.; Chen, Y.T.; Bauer, G.E.W.; Saitoh, E.; Goennenwein, S.T.B.

    2013-01-01

    We experimentally investigate and quantitatively analyze the spin Hall magnetoresistance effect in ferromagnetic insulator/platinum and ferromagnetic insulator/nonferromagnetic metal/platinum hybrid structures. For the ferromagnetic insulator, we use either yttrium iron garnet, nickel ferrite, or

  3. Spin-orbit-coupled transport and spin torque in a ferromagnetic heterostructure

    KAUST Repository

    Wang, Xuhui

    2014-02-07

    Ferromagnetic heterostructures provide an ideal platform to explore the nature of spin-orbit torques arising from the interplay mediated by itinerant electrons between a Rashba-type spin-orbit coupling and a ferromagnetic exchange interaction. For such a prototypic system, we develop a set of coupled diffusion equations to describe the diffusive spin dynamics and spin-orbit torques. We characterize the spin torque and its two prominent—out-of-plane and in-plane—components for a wide range of relative strength between the Rashba coupling and ferromagnetic exchange. The symmetry and angular dependence of the spin torque emerging from our simple Rashba model is in an agreement with experiments. The spin diffusion equation can be generalized to incorporate dynamic effects such as spin pumping and magnetic damping.

  4. Spin Transport in Mesoscopic Superconducting-Ferromagnetic Hybrid Conductor

    Directory of Open Access Journals (Sweden)

    Zein W. A.

    2008-01-01

    Full Text Available The spin polarization and the corresponding tunneling magnetoresistance (TMR for a hybrid ferromagnetic/superconductor junction are calculated. The results show that these parameters are strongly depends on the exchange field energy and the bias voltage. The dependence of the polarization on the angle of precession is due to the spin flip through tunneling process. Our results could be interpreted as due to spin imbalance of carriers resulting in suppression of gap energy of the superconductor. The present investigation is valuable for manufacturing magnetic recording devices and nonvolatile memories which imply a very high spin coherent transport for such junction.

  5. Spin Transport in Mesoscopic Superconducting-Ferromagnetic Hybrid Conductor

    Directory of Open Access Journals (Sweden)

    Zein W. A.

    2008-01-01

    Full Text Available The spin polarization and the corresponding tunneling magnetoresistance (TMR for a hybrid ferromagnetic / superconductor junction are calculated. The results show that these parameters are strongly depends on the exchange field energy and the bias voltage. The dependence of the polarization on the angle of precession is due to the spin flip through tunneling process. Our results could be interpreted as due to spin imbalance of carriers resulting in suppression of gap energy of the superconductor. The present investigation is valuable for manufacturing magnetic recording devices and nonvolatile memories which imply a very high spin coherent transport for such junction.

  6. Tunneling Conductance in Ferromagnetic Metal/Normal Metal/Spin-Singlet -Wave Ferromagnetic Superconductor Junctions

    Directory of Open Access Journals (Sweden)

    Hamidreza Emamipour

    2013-01-01

    Full Text Available In the framework of scattering theory, we study the tunneling conductance in a system including two junctions, ferromagnetic metal/normal metal/ferromagnetic superconductor, where ferromagnetic superconductor is in spin-singlet -wave pairing state. The non-magnetic normal metal is placed in the intermediate layer with the thickness ( which varies from 1 nm to 10000 nm. The interesting result which we have found is the existence of oscillations in conductance curves. The period of oscillations is independent of FS and FN exchange field while it depends on . The obtained results can serve as a useful tool to determine the kind of pairing symmetry in ferromagnetic superconductors.

  7. Collective spin wave and phonon excitations in ferromagnetic organic polymers

    International Nuclear Information System (INIS)

    Leong, Jit-Liang; Sun, Shih-Jye

    2013-01-01

    We proposed a model to investigate the properties of a conductive and ferromagnetic organic-polymer (OCP), which contains two collective excitations—spin wave and phonon—competing with each other; namely, the spin wave excitation accompanies the electron–phonon (e–ph) interactions in the conductive and ferromagnetic OCP. The ferromagnetism of the OCP is induced from the conductive carriers which couple with the phonon to become polarons. Due to the competition between both excitations, the Curie temperature (T C ) is sensitively suppressed by the e–ph interaction. In addition, an optimal T C with a small e–ph interaction exists in a specific density of conduction carrier, yet is contrary to the large e–ph interaction case. Furthermore, the dimerization, i.e. the atomic displacement induced from the e–ph interactions, increases with the strength of the e–ph interaction and decreases upon reaching the maximum dimerization. (paper)

  8. Nonlocal spin-transport measurement of superconductor-ferromagnet nanostructures

    Energy Technology Data Exchange (ETDEWEB)

    Kolenda, Stefan; Wolf, Michael J.; Huebler, Florian; Beckmann, Detlef [Institut fuer Nanotechnologie, Karlsruher Institut fuer Technologie (Germany)

    2015-07-01

    We present measurements of the nonlocal conductance of nanostructures with several ferromagnetic electrodes lying perpendicular on a superconducting wire. In these structures nonlocal conductance is mostly given by diffusion of quasiparticles, which are injected by one of the electrodes and detected by an other one. Applying a magnetic field induces a Zeeman splitting in the quasiparticles density of states, which suppresses the relaxation of injected spin imbalance, thus spin transport over distances of several micrometers is found. While in the previous experiments the magnetic field was aligned parallel to the ferromagnetic electrodes, we also show measurements applying the magnetic field noncollinear with the magnetization of the ferromagnetic electrodes. We compare our results to the previous case.

  9. Spin exchange between ion probes and localized moments in ferromagnets as the origin of transient fields

    International Nuclear Information System (INIS)

    Hagelberg, F.; Das, T.P.; Speidel, K.

    1993-01-01

    The transient field phenomenon has been ascribed to a polarization transfer between the electrons of the ionic projectiles and the surplus of majority spin electrons of the ferromagnetic host over the minority spin electrons. Earlier attempts to explain this crucial process failed to account for the order of magnitude of the experimentally observed transient field strengths. A recent model which proposes spin exchange scattering between bound projectile electrons and quasifree host electrons as the mechanism of polarization transfer arrives at the correct orders of magnitude but is in conflict with the weak velocity dependence of the experimental polarization, exhibiting a strongly decreasing behavior with increasing velocity. The new model presented here proposes spin exchange between the ionic shell and localized electrons of the ferromagnet as a more adequate approach to the problem. It is shown that calculations involving hydrogenlike ions explain the size of the experimentally observed polarization effects as well as their velocity dependence for various ion probes traversing thin iron foils

  10. Biaxial-stress-driven full spin polarization in ferromagnetic hexagonal chromium telluride

    Energy Technology Data Exchange (ETDEWEB)

    Xiao, Xiang-Bo; Li, Jun [Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190 (China); Liu, Bang-Gui, E-mail: bgliu@iphy.ac.cn [Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190 (China); School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100190 (China)

    2017-03-15

    It is important to spintronics to achieve fully-spin-polarized magnetic materials that are stable and can be easily fabricated. Here, through systematical density-functional-theory investigations, we achieve high and even full spin polarization for carriers in the ground-state phase of CrTe by applying tensile biaxial stress. The resulting strain is tensile in the xy plane and compressive in the z axis. With the in-plane tensile strain increasing, the ferromagnetic order is stable against antiferromagnetic fluctuations, and a half-metallic ferromagnetism is achieved at an in-plane strain of 4.8%. With the spin-orbit coupling taken into account, the spin polarization is equivalent to 97% at the electronic transition point, and then becomes 100.0% at the in-plane strain of 6.0%. These make us believe that the full-spin-polarized ferromagnetism in this stable and easily-realizable hexagonal phase could be realized soon, and applied in spintronics. - Highlights: • Full spin polarization in the hexagonal ground-state phase of CrTe by biaxial stress. • The stress produces in-plane tensile strain and perpendicular compressive strain. • Reliable electronic structure is calculated with improved exchange functional. • Spin polarization is calculated with spin-orbit coupling taken into account.

  11. Coherence and stiffness of spin waves in diluted ferromagnets

    Czech Academy of Sciences Publication Activity Database

    Turek, Ilja; Kudrnovský, Josef; Drchal, Václav

    2016-01-01

    Roč. 94, č. 17 (2016), č. článku 174447. ISSN 2469-9950 R&D Projects: GA ČR GA15-13436S Institutional support: RVO:68081723 ; RVO:68378271 Keywords : spin waves * diluted ferromagnets * disordered systems Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.836, year: 2016

  12. Conductance of Rashba spin-split systems with ferromagnetic contacts

    DEFF Research Database (Denmark)

    Larsen, M. Høgsbro; Lunde, A.M.; Flensberg, Karsten

    2002-01-01

    We study theoretically the conductance of heterostructures with ferromagnetic (F) conductors and a two-dimensional electron gas with Rashba (R) spin-orbit interaction using a two-channel Landauer formula. Assuming a one-dimensional model, we first find the S matrix for the FR interface. This result...

  13. A cluster-bethe-lattice approach to spin-waves in dilute ferromagnets

    International Nuclear Information System (INIS)

    Salzberg, J.B.; Silva, C.E.T.G. da; Falicov, L.M.

    1975-01-01

    The spin-wave spectra of a dilute ferromagnet within the cluster-bethe-lattice approximation is studied. Short range order effects for the alloy are included. A study of finite size clusters connected at their edges to Bethe lattices of the same coordination number allows one to determine:(i) the stability condition for the magnetic system; (ii) the continuum spin-wave local density of states and (iii) the existence of localized states below and above the continuum states

  14. Long-Distance Entanglement of Spin Qubits via Ferromagnet

    Directory of Open Access Journals (Sweden)

    Luka Trifunovic

    2013-12-01

    Full Text Available We propose a mechanism of coherent coupling between distant spin qubits interacting dipolarly with a ferromagnet. We derive an effective two-spin interaction Hamiltonian and find a regime where the dynamics is coherent. Finally, we present a sequence for the implementation of the entangling controlled-not gate and estimate the corresponding operation time to be a few tens of nanoseconds. A particularly promising application of our proposal is to atomistic spin qubits such as silicon-based qubits and nitrogen-vacancy centers in diamond to which existing coupling schemes do not apply.

  15. Proximity effects and Josephson currents in ferromagnet. Spin-triplet superconductors junctions

    International Nuclear Information System (INIS)

    Terrade, Damien

    2015-01-01

    Spin-triplet superconductivity, first attached to the description of 3 He, is now generally considered to also occur in heavy-fermions compounds and in perovskite ruthenium oxide Sr 2 RuO 4 . The latter material is especially interesting since many experiments show strong evidences for a unitary chiral spin-triplet state. Moreover, the recent fabrication of thin heterostructures made of ferromagnetic SrRuO 3 on the top of Sr 2 RuO 4 strongly encourages new theoretical studies on the interplay between spin-triplet superconductor and ferromagnet in similar fashion to spin-singlet superconductors. Using an extended tight-binding Hamiltonian to model the superconductor, we discuss in this thesis the specific proximity effects of such interface by solving self-consistently the Bogoliubov-De Gennes equations on two- and three-dimensional lattices in the ballistic limit. We obtain the spatial profile of the superconducting order parameters at the interface as well as the spin-polarisation and the current across the Josephson junctions. In contrast to heterostructures made of spin-singlet superconductor, we show that the physical properties at the interface are not only controlled by the strength of the magnetization inside the ferromagnet but also by its orientation due to the existence of a finite pair spin projection of the spin-triplet Cooper pairs. We analyse in the first part the spin-polarisation and the Gibbs free energy at the three-dimensional ferromagnet-chiral spin-triplet superconductor interface. Then, the second part of the thesis is dedicated to the study of the Josephson junctions made of a chiral spin-triplet superconductor and a ferromagnetic barrier. More precisely, we analyse the existence of 0-π state transitions in two- and three-dimensional junctions with respect to the strength and the orientation of the magnetization. Finally, we study the proximity effects at the interface of helical spin-triplet superconductors. They differ from the chiral

  16. Induced spin polarization effect in graphene by ferromagnetic nanocontact

    Energy Technology Data Exchange (ETDEWEB)

    Mandal, Sumit; Saha, Shyamal K., E-mail: cnssks@iacs.res.in [Department of Materials Science, Indian Association for the Cultivation of Science, Jadavpur, Kolkata 700032 (India)

    2015-03-07

    Chemically synthesized graphene contains large number of defects which act as localized spin moments at the defect sites. Cobalt nanosheets of variable thickness are grown on graphene surface to investigate spin/magnetotransport through graphene sheets containing large number of localized spins. Negative magnetoresistance (MR) is observed over the entire temperature range (5–300 K) for thin cobalt sheets, while a cross-over from negative to positive MR with increasing temperature is noticed for thicker cobalt sheets. The observed MR results are explained on the basis of recently reported spin polarization effect in graphene due to the presence of ferromagnetic atoms on the surface considering a spin valve like Co/graphene/Co nanostructures.

  17. Effects of Rashba and Dresselhaus spin-orbit couplings on itinerant ferromagnetism

    Science.gov (United States)

    Liu, Mengnan; Xu, Liping; Wan, Yong; Yan, Xu

    2018-02-01

    Based on Stoner model for itinerant ferromagnet, effects of spin-orbit coupling (SOC) on ferromagnetism were investigated at zero temperature. It was found that SOC will enhance the critical ferromagnetic exchange interaction for spontaneous magnetization, and then suppress ferromagnetism. In case of the coexistence of Rashba and Dresselhaus SOCs, the mixture of the two spin-orbit couplings showed stronger suppressed effect on ferromagnetism than only one kind of SOC alone. When the two SOCs mixed with equal magnitude, ferromagnetism in itinerant ferromagnet was suppressed to minimum.

  18. Spin Tunneling in Junctions with Disordered Ferromagnets

    NARCIS (Netherlands)

    Paluskar, P.V.; Attema, J.J.; de Wijs, G.A.; Fiddy, S.; Snoeck, E.; Kohlhepp, J.T.; Swagten, H.J.M.; de Groot, R. A.; Koopmans, H.

    2008-01-01

    We provide compelling evidence to establish that, contrary to one’s elementary guess, the tunneling spin polarization (TSP) of amorphous CoFeB is larger than that of fcc CoFeB. First-principles atomic and electronic structure calculations reveal striking agreement between the measured TSP and the

  19. Dynamical spin injection at a quasi-one-dimensional ferromagnet-graphene interface

    International Nuclear Information System (INIS)

    Singh, S.; Ahmadi, A.; Mucciolo, E. R.; Barco, E. del; Cherian, C. T.; Özyilmaz, B.

    2015-01-01

    We present a study of dynamical spin injection from a three-dimensional ferromagnet into two-dimensional single-layer graphene. Comparative ferromagnetic resonance (FMR) studies of ferromagnet/graphene strips buried underneath the central line of a coplanar waveguide show that the FMR linewidth broadening is the largest when the graphene layer protrudes laterally away from the ferromagnetic strip, indicating that the spin current is injected into the graphene areas away from the area directly underneath the ferromagnet being excited. Our results confirm that the observed damping is indeed a signature of dynamical spin injection, wherein a pure spin current is pumped into the single-layer graphene from the precessing magnetization of the ferromagnet. The observed spin pumping efficiency is difficult to reconcile with the expected backflow of spins according to the standard spin pumping theory and the characteristics of graphene, and constitutes an enigma for spin pumping in two-dimensional structures

  20. Spin-wave-induced spin torque in Rashba ferromagnets

    Science.gov (United States)

    Umetsu, Nobuyuki; Miura, Daisuke; Sakuma, Akimasa

    2015-05-01

    We study the effects of Rashba spin-orbit coupling on the spin torque induced by spin waves, which are the plane-wave dynamics of magnetization. The spin torque is derived from linear-response theory, and we calculate the dynamic spin torque by considering the impurity-ladder-sum vertex corrections. This dynamic spin torque is divided into three terms: a damping term, a distortion term, and a correction term for the equation of motion. The distorting torque describes a phenomenon unique to the Rashba spin-orbit coupling system, where the distorted motion of magnetization precession is subjected to the anisotropic force from the Rashba coupling. The oscillation mode of the precession exhibits an elliptical trajectory, and the ellipticity depends on the strength of the nesting effects, which could be reduced by decreasing the electron lifetime.

  1. Tunable spin-tunnel contacts to silicon using low-work-function ferromagnets

    Science.gov (United States)

    Min, Byoung-Chul; Motohashi, Kazunari; Lodder, Cock; Jansen, Ron

    2006-10-01

    Magnetic tunnel junctions have become ubiquitous components appearing in magnetic random-access memory, read heads of magnetic disk drives and semiconductor-based spin devices. Inserting a tunnel barrier has been key to achieving spin injection from ferromagnetic (FM) metals into GaAs, but spin injection into Si has remained elusive. We show that Schottky barrier formation leads to a huge conductivity mismatch of the FM tunnel contact and Si, which cannot be solved by the well-known method of adjusting the tunnel barrier thickness. We present a radically different approach for spin-tunnelling resistance control using low-work-function ferromagnets, inserted at the FM/tunnel barrier interface. We demonstrate that in this way the resistance-area (RA) product of FM/Al2O3/Si contacts can be tuned over eight orders of magnitude, while simultaneously maintaining a reasonable tunnel spin polarization. This raises prospects for Si-based spintronics and presents a new category of ferromagnetic materials for spin-tunnel contacts in low-RA-product applications.

  2. Spin accumulation and magnetoresistance of ferromagnetic domain walls

    Science.gov (United States)

    Dzero, Maxim; Gor'kov, Lev; Zvezdin, Anatolii; Zvezdin, Konstantin

    2003-03-01

    Taking into account the difference in the density of states between the spin's majority and minority bands in a ferromagnet, we obtain a spatial behavior of the electrostatic potential at the domain wall boundaries. The value of discontinuity oscillates with the number of domains and contains information about system as a whole, such as the positions of the domain walls or collapse of the domain walls when an external magnetic field is applied. We explain experimentally observed values of magnetoresistance in terms of spin accumulation effects. For the latter we suggest that in nanowires made of itinerant ferromagnets a new type of domain walls is realized, in which system prefers to reduce the value of magnetization rather then rotating it going from one domain to another. We also discuss the questions related to conditions of stability of linear domain walls.

  3. Muon spin relaxation in ferromagnetic PdMn

    International Nuclear Information System (INIS)

    Dodds, S.A.; Gist, G.A.; Heffner, R.H.; Leon, M.; MacLaughlin, D.E.; Mydosh, J.A.; Nieuwenhuys, G.J.; Schillaci, M.E.

    1983-01-01

    Positive-muon (μ + ) spin relaxation experiments have been carried out in the dilute ferromagnetic alloy Pd + 2 at % Mn (T/sub c/ = 5.8 0 K). In the paramagnetic state the inhomogeneous μ + linewidth is proportional to the bulk magnetization. Below T/sub c/ the μ + linewidth and the width of the μ + local field distribution in zero applied field are both in qualitative accord with the Sherrington-Kirkpatrick theory of disordered magnets

  4. Ferromagnetic domain structures and spin configurations measured in doped manganite

    DEFF Research Database (Denmark)

    He, J.Q.; Volkov, V.V.; Beleggia, Marco

    2010-01-01

    We report on measurements of the spin configuration across ferromagnetic domains in La0.325Pr0.3Ca0.375MnO3 films obtained by means of low-temperature Lorentz electron microscopy with in situ magnetizing capabilities. Due to the particular crystal symmetry of the material, we observe two sets of ...... and the crystal symmetry might affect the magnetoresistivity under an applied magnetic field in a strongly correlated electron system....

  5. Inductive detection of fieldlike and dampinglike ac inverse spin-orbit torques in ferromagnet/normal-metal bilayers

    Science.gov (United States)

    Berger, Andrew J.; Edwards, Eric R. J.; Nembach, Hans T.; Karenowska, Alexy D.; Weiler, Mathias; Silva, Thomas J.

    2018-03-01

    Functional spintronic devices rely on spin-charge interconversion effects, such as the reciprocal processes of electric field-driven spin torque and magnetization dynamics-driven spin and charge flow. Both dampinglike and fieldlike spin-orbit torques have been observed in the forward process of current-driven spin torque and dampinglike inverse spin-orbit torque has been well studied via spin pumping into heavy metal layers. Here, we demonstrate that established microwave transmission spectroscopy of ferromagnet/normal metal bilayers under ferromagnetic resonance can be used to inductively detect the ac charge currents driven by the inverse spin-charge conversion processes. This technique relies on vector network analyzer ferromagnetic resonance (VNA-FMR) measurements. We show that in addition to the commonly extracted spectroscopic information, VNA-FMR measurements can be used to quantify the magnitude and phase of all ac charge currents in the sample, including those due to spin pumping and spin-charge conversion. Our findings reveal that Ni80Fe20/Pt bilayers exhibit both dampinglike and fieldlike inverse spin-orbit torques. While the magnitudes of both the dampinglike and fieldlike inverse spin-orbit torque are of comparable scale to prior reported values for similar material systems, we observed a significant dependence of the dampinglike magnitude on the order of deposition. This suggests interface quality plays an important role in the overall strength of the dampinglike spin-to-charge conversion.

  6. Vortex Flipping in Superconductor-Ferromagnet Spin Valve Structures

    Science.gov (United States)

    Patino, Edgar J.; Aprili, Marco; Blamire, Mark; Maeno, Yoshiteru

    2014-03-01

    We report in plane magnetization measurements on Ni/Nb/Ni/CoO and Co/Nb/Co/CoO spin valve structures with one of the ferromagnetic layers pinned by an antiferromagnetic layer. In samples with Ni, below the superconducting transition Tc, our results show strong evidence of vortex flipping driven by the ferromagnets magnetization. This is a direct consequence of proximity effect that leads to vortex supercurrents leakage into the ferromagnets. Here the polarized electron spins are subject to vortices magnetic field occasioning vortex flipping. Such novel mechanism has been made possible for the first time by fabrication of the F/S/F/AF multilayered spin valves with a thin-enough S layer to barely confine vortices inside as well as thin-enough F layers to align and control the magnetization within the plane. When Co is used there is no observation of vortex flipping effect. This is attributed to Co shorter coherence length. Interestingly instead a reduction in pinning field of about 400 Oe is observed when the Nb layer is in superconducting state. This effect cannot be explained in terms of vortex fields. In view of these facts any explanation must be directly related to proximity effect and thus a remarkable phenomenon that deserves further investigation. Programa Nacional de Ciencias Basicas COLCIENCIAS (No. 120452128168).

  7. Percolative transport in the vicinity of charge-order ferromagnetic ...

    Indian Academy of Sciences (India)

    The electric field driven charge transport in the system is modelled on the basis of an inhomogeneous medium consisting of ferromagnetic metallic clusters dispersed in a CO background. Keywords. Hole-doped manganite; percolative transport; charge-order; ferromagnetic transition. PACS Nos 75.30.Vn; 75.50.Dd. 1.

  8. Imaging and controlling spins in semiconductors and ferromagnets

    Science.gov (United States)

    Nowakowski, Mark Edward

    Spins possess robust coherent and exchange-driven properties in semiconductors and ferromagnets. In this work, we investigate three experiments that incorporate and exploit these spin properties to demonstrate innovated quantum information processing, magnetic detection and control techniques. In the first experiment we spatially confine an effective magnetic field to control the coherent state of moving electron spins. Optically-injected electron spin ensembles are transported through a gate-controlled, spatially-isolated region with a large effective magnetic field created by locally polarized nuclear spins within a GaAs channel at T = 8 K. By tuning the localized effective field strength and drift velocity we detect, using time-resolved Kerr rotation (TRKR), induced spin rotations of up to 5pi radians in 6 ns over a 30 mum distance. In the second experiment, we develop a sensitive electrical technique derived from the anomalous Hall effect (AHE) to measure domain wall (DW) motion with nanometer precision. We then use this system to study the elastic properties of single ferromagnetic DWs in (Ga,Mn)As. Full understanding of the electrical signal is only possible after accurately determining the DW location with respect to the electrical contacts. Therefore, we image the DWs using a custom-built, diffraction-limited video magneto-optical Kerr effect (MOKE) microscopy system while simultaneously measuring the AHE. By combining these detection schemes we are able to precisely measure temperature-dependent elastic DW dynamics and kinetics below TC. Finally, the third experiment relates our progress toward understanding the coupling between the multiferroic oxide BiFeO3 (BFO) and a CoFe magnetic layer. The exchange-bias mediated coupling between ferroelectric domains of the BFO and ferromagnetic domains in the CoFe layer suggest a pathway to realize electrical control of the magnetization properties. We investigate and model the ferroelectric influence on

  9. Spin-orbit torques in locally and globally noncentrosymmetric crystals: Antiferromagnets and ferromagnets

    KAUST Repository

    Železný, J.

    2017-01-10

    One of the main obstacles that prevents practical applications of antiferromagnets is the difficulty of manipulating the magnetic order parameter. Recently, following the theoretical prediction [J. Železný, Phys. Rev. Lett. 113, 157201 (2014)]PRLTAO0031-900710.1103/PhysRevLett.113.157201, the electrical switching of magnetic moments in an antiferromagnet was demonstrated [P. Wadley, Science 351, 587 (2016)]SCIEAS0036-807510.1126/science.aab1031. The switching is due to the so-called spin-orbit torque, which has been extensively studied in ferromagnets. In this phenomena a nonequilibrium spin-polarization exchange coupled to the ordered local moments is induced by current, hence exerting a torque on the order parameter. Here we give a general systematic analysis of the symmetry of the spin-orbit torque in locally and globally noncentrosymmetric crystals. We study when the symmetry allows for a nonzero torque, when is the torque effective, and its dependence on the applied current direction and orientation of magnetic moments. For comparison, we consider both antiferromagnetic and ferromagnetic orders. In two representative model crystals we perform microscopic calculations of the spin-orbit torque to illustrate its symmetry properties and to highlight conditions under which the spin-orbit torque can be efficient for manipulating antiferromagnetic moments.

  10. Spin-dependent transport and functional design in organic ferromagnetic devices

    Directory of Open Access Journals (Sweden)

    Guichao Hu

    2017-09-01

    Full Text Available Organic ferromagnets are intriguing materials in that they combine ferromagnetic and organic properties. Although challenges in their synthesis still remain, the development of organic spintronics has triggered strong interest in high-performance organic ferromagnetic devices. This review first introduces our theory for spin-dependent electron transport through organic ferromagnetic devices, which combines an extended Su–Schrieffer–Heeger model with the Green’s function method. The effects of the intrinsic interactions in the organic ferromagnets, including strong electron–lattice interaction and spin–spin correlation between π-electrons and radicals, are highlighted. Several interesting functional designs of organic ferromagnetic devices are discussed, specifically the concepts of a spin filter, multi-state magnetoresistance, and spin-current rectification. The mechanism of each phenomenon is explained by transmission and orbital analysis. These works show that organic ferromagnets are promising components for spintronic devices that deserve to be designed and examined in future experiments.

  11. Spin-independent transparency of pure spin current at normal/ferromagnetic metal interface

    Science.gov (United States)

    Hao, Runrun; Zhong, Hai; Kang, Yun; Tian, Yufei; Yan, Shishen; Liu, Guolei; Han, Guangbing; Yu, Shuyun; Mei, Liangmo; Kang, Shishou

    2018-03-01

    The spin transparency at the normal/ferromagnetic metal (NM/FM) interface was studied in Pt/YIG/Cu/FM multilayers. The spin current generated by the spin Hall effect (SHE) in Pt flows into Cu/FM due to magnetic insulator YIG blocking charge current and transmitting spin current via the magnon current. Therefore, the nonlocal voltage induced by an inverse spin Hall effect (ISHE) in FM can be detected. With the magnetization of FM parallel or antiparallel to the spin polarization of pure spin currents ({{\\boldsymbol{σ }}}sc}), the spin-independent nonlocal voltage is induced. This indicates that the spin transparency at the Cu/FM interface is spin-independent, which demonstrates that the influence of spin-dependent electrochemical potential due to spin accumulation on the interfacial spin transparency is negligible. Furthermore, a larger spin Hall angle of Fe20Ni80 (Py) than that of Ni is obtained from the nonlocal voltage measurements. Project supported by the National Basic Research Program of China (Grant No. 2015CB921502), the National Natural Science Foundation of China (Grant Nos. 11474184 and 11627805), the 111 Project, China (Grant No. B13029), and the Fundamental Research Funds of Shandong University, China.

  12. Valley and spin resonant tunneling current in ferromagnetic/nonmagnetic/ferromagnetic silicene junction

    Directory of Open Access Journals (Sweden)

    Yaser Hajati

    2016-02-01

    Full Text Available We study the transport properties in a ferromagnetic/nonmagnetic/ferromagnetic (FNF silicene junction in which an electrostatic gate potential, U, is attached to the nonmagnetic region. We show that the electrostatic gate potential U is a useful probe to control the band structure, quasi-bound states in the nonmagnetic barrier as well as the transport properties of the FNF silicene junction. In particular, by introducing the electrostatic gate potential, both the spin and valley conductances of the junction show an oscillatory behavior. The amplitude and frequency of such oscillations can be controlled by U. As an important result, we found that by increasing U, the second characteristic of the Klein tunneling is satisfied as a result of the quasiparticles chirality which can penetrate through a potential barrier. Moreover, it is found that for special values of U, the junction shows a gap in the spin and valley-resolve conductance and the amplitude of this gap is only controlled by the on-site potential difference, Δz. Our findings of high controllability of the spin and valley transport in such a FNF silicene junction may improve the performance of nano-electronics and spintronics devices.

  13. Anomalous Tunneling of Spin Wave in Heisenberg Ferromagnet

    Science.gov (United States)

    Kato, Yusuke; Watabe, Shohei; Ohashi, Yoji

    2012-12-01

    The ferromagnetic spin wave (FSW) in classical Heisenberg chain exhibits the perfect transmission in the long-wavelength limit in the transmission-reflection problem with an inhomogeneity of exchange integral. In the presence of local magnetic field, on the other hand, FSW undergoes the perfect reflection in the long-wavelength limit. This difference in the long-wavelength limit is attributed to the symmetry property of the scatterers; it is crucial whether the potential preserves or breaks the spin rotation symmetry. Our result implies that the anomalous tunneling (i.e., perfect transmission in the low-energy limit) found both in scalar and spinor BECs is not specific to gapless modes in superfluids but is a common property shared with generic Nambu-Goldstone modes in the presence of a symmetry-preserving potential scatterer.

  14. Anomalous Tunneling of Spin Wave in Heisenberg Ferromagnet

    International Nuclear Information System (INIS)

    Kato, Yusuke; Watabe, Shohei; Ohashi, Yoji

    2012-01-01

    The ferromagnetic spin wave (FSW) in classical Heisenberg chain exhibits the perfect transmission in the long-wavelength limit in the transmission-reflection problem with an inhomogeneity of exchange integral. In the presence of local magnetic field, on the other hand, FSW undergoes the perfect reflection in the long-wavelength limit. This difference in the long-wavelength limit is attributed to the symmetry property of the scatterers; it is crucial whether the potential preserves or breaks the spin rotation symmetry. Our result implies that the anomalous tunneling (i.e., perfect transmission in the low-energy limit) found both in scalar and spinor BECs is not specific to gapless modes in superfluids but is a common property shared with generic Nambu-Goldstone modes in the presence of a symmetry-preserving potential scatterer.

  15. Current-induced spin-orbit torques in ferromagnetic and antiferromagnetic systems

    KAUST Repository

    Manchon, Aurelien

    2018-01-29

    Spin-orbit coupling in inversion-asymmetric magnetic crystals and structures has emerged as a powerful tool to generate complex magnetic textures, interconvert charge and spin under applied current, and control magnetization dynamics. Current-induced spin-orbit torques mediate the transfer of angular momentum from the lattice to the spin system, leading to sustained magnetic oscillations or switching of ferromagnetic as well as antiferromagnetic structures. The manipulation of magnetic order, domain walls and skyrmions by spin-orbit torques provides evidence of the microscopic interactions between charge and spin in a variety of materials and opens novel strategies to design spintronic devices with potentially high impact in data storage, nonvolatile logic, and magnonic applications. This paper reviews recent progress in the field of spin-orbitronics, focusing on theoretical models, material properties, and experimental results obtained on bulk noncentrosymmetric conductors and multilayer heterostructures, including metals, semiconductors, and topological insulator systems. Relevant aspects for improving the understanding and optimizing the efficiency of nonequilibrium spin-orbit phenomena in future nanoscale devices are also discussed.

  16. Suhl instabilities for spin waves in ferromagnetic nanostripes and ultrathin films

    Energy Technology Data Exchange (ETDEWEB)

    Haghshenasfard, Zahra, E-mail: zhaghshe@uwo.ca; Nguyen, Hoa T.; Cottam, Michael G., E-mail: cottam@uwo.ca

    2017-03-15

    A microscopic (or Hamiltonian-based) theory is employed for the spin-wave instability thresholds of nonlinear processes in ultrathin ferromagnetic stripes and films under perpendicular pumping with an intense microwave field. The spatially-quantized linear spin waves in these nanostructures may participate in parametric processes through the three-magnon interactions (the first-order Suhl process) and the four-magnon interactions (the second-order Suhl process) when pumped. By contrast with most previous studies of spin-wave instabilities made for larger samples, where macroscopic (or continuum) theories involving Maxwell's equations for magnetic dipolar effects are used, a discrete lattice of effective spins is employed. Then a dipole-exchange spin Hamiltonian is employed to investigate the behavior of the quantized spin waves under perpendicular pumping, when modifications due to the more extensive spatial confinement and edges effects in these nanostructures become pronounced. The instability thresholds versus applied magnetic field are calculated, with emphasis on the size effects and geometries of the nanostructures and on the different relative strengths of the magnetic dipole-dipole and exchange interactions in materials. Numerical results are presented using parameters for Permalloy, YIG, and EuS. - Highlights: • Suhl instabilities for spin waves in magnetic stripes and films are investigated. • Three- and four-magnon processes in perpendicular pumping are taken into account. • Numerical applications are made to Permalloy, YIG, and EuS.

  17. The semi-infinite anisotropic spin-1/2 Heisenberg ferromagnet

    International Nuclear Information System (INIS)

    Benyoussef, A.; Boubekri, A.; Ez-Zahraouy, H.; Saber, M.

    1998-08-01

    Using the effective field theory with a probability distribution technique that accounts for the self-spin correlation functions, the phase transitions in the semi-infinite anisotropic spin-1/2 Heisenberg ferromagnet on a simple cubic lattice are examined. For fixed values of the reduced exchange anisotropic parameter, the critical temperature of the system is studied as a function of the ratio R of the surface exchange couplings to the bulk ones. It was found that if R ≤ R c , the system orders at the bulk critical temperature T B c /J and if R ≥ R c , the system exhibits two successive transitions. The surface orders at the surface critical temperature T S c /J which is higher than T B c /J and as the temperature is lowered, in the presence of ordered surface, the bulk orders at T B c /J. (author)

  18. Spin-dependent thermoelectric effects in superconductor-ferromagnet tunnel junctions

    Energy Technology Data Exchange (ETDEWEB)

    Kolenda, Stefan; Beckmann, Detlef [Institut fuer Nanotechnologie, Karlsruher Institut fuer Technologie (Germany); Suergers, Christoph [Physikalisches Institut, Karlsruher Institut fuer Technologie (Germany)

    2016-07-01

    Recently, large thermoelectric effects were predicted to occur in superconductor-ferromagnet tunnel junctions with a spin-splitting of the density of states. We have reported on the observation of these effects in samples where the spin splitting was induced by an applied magnetic field. Here, we show results on samples where the spin splitting is enhanced by exchange coupling to the ferromagnetic insulator europium sulfide.

  19. A novel magnetoresistance induced by charge ordering in ferromagnetic/charge-ordered/ferromagnetic trilayers

    Science.gov (United States)

    Wang, Haiou; Li, Jinwei; Su, Kunpeng; Huo, Dexuan; Tan, Weishi

    2015-10-01

    Microstructure, magnetoresistance (MR) and magnetic properties of Pr0.7Sr0.3MnO3/La0.5Ca0.5MnO3/Pr0.7Sr0.3MnO3 trilayers, which are shown to be tunable with different La0.5Ca0.5MnO3 spacer thickness, are investigated. The trilayer with 6 nm thick La0.5Ca0.5MnO3 spacer show \\text{MR}∼37{%} at 195 K in 1 T and \\text{MR}∼80{%} at 220 K in 9 T, which is realized through the double-exchange mechanism. In contrast, trilayers with the thicker La0.5Ca0.5MnO3 spacer show enhanced MR at a wide low-temperature range. The obtained \\text{MR}∼52{%} at 50 K in 1 T in the trilayer with 18 nm thick La0.5Ca0.5MnO3 spacer is superior to that of other magnetic nanoscales. We surmise that this MR originates in the ferromagnetic/antiferromagnetic competition accompanied with the formation of a charge-ordered antiferromagnetic state and the collapse of the charge-ordered state at the applied magnetic field, rather than in the double-exchange mechanism. Large and tunable MR can be realized by controlling the strain state (the thickness of the La0.5Ca0.5MnO3 spacer), which can be applied in the used devices.

  20. Coupling nitrogen-vacancy centers to a dynamic ferromagnetic vortex for fast, nanoscale spin addressability and control

    Science.gov (United States)

    Berezovsky, Jesse

    As we begin to look at how spin qubits might be integrated into a scalable platform, a promising strategy is to engineer the magnetic environment of the spins using micron- or nanometer-scale ferromagnetic (FM) elements, for functionalities such as nanoscale addressability, spin-wave mediated coupling, or enhanced sensing. The promise of these FM/spin interactions brings with it the question of how the coherence properties of the spin will be affected by coupling to these complex mesoscopic systems. To explore the physics of individual spins coupled to a proximal, dynamic ferromagnetic structure, we have studied interactions between individual nitrogen-vacancy (NV) spins and a model FM system - a vortex magnetization state. The complex, yet controllable, spin texture of a FM vortex, formed in a thin disk or nanowire, allows one to study different regimes of interaction with a nearby confined spin. The vortex core produces a large static dipole-like fringe field. The vortex state also displays discrete dynamic modes ranging from several 100 MHz to GHz. By applying an in-plane magnetic field, the position of the vortex core relative to the NV spin can be controlled with nanometer-scale resolution, and time resolution of 10s of nanoseconds. As the vortex core is translated into proximity with an NV spin, the fringe field from the core generates a large position-dependent spin splitting, permitting nanoscale spin addressability. We also find that the dynamic interaction of the vortex, NV spin, and applied microwave field results in amplification of the Rabi transition rate by more than an order of magnitude. Finally, we explore how spin decoherence and relaxation mechanisms are enhanced as the vortex core approaches the NVs, with implications for proposed technology incorporating coherent spins and proximal FM elements. We acknowledge support from DOE, Award No. DE-SC008148.

  1. Spin-orbit-torque and magnetic damping in tailored ferromagnetic bilayers

    OpenAIRE

    Lee, DongJoon; Kim, JongHyuk; Park, HeeGyum; Lee, Kyung-Jin; Ju, Byeong-Kwon; Koo, Hyun Cheol; Min, Byoung-Chul; Lee, OukJae

    2018-01-01

    We study spin-orbit-torque-driven ferromagnetic resonance (FMR) in ferromagnetic (FM) bilayers, consisting of Co and permalloy (Py), sandwiched between Pt and MgO layers. We find that the FM layer in contact with the Pt layers dominantly determines that spin Hall angle, which is consistent with the spin-transparency model. By contrast, the FMR linewidths are considerably influenced not only by the spin-pumping effect across the Pt|FM in terface but also by the spin relaxation such as two-magn...

  2. Critical phenomena in ferromagnetic spin systems on lattices

    International Nuclear Information System (INIS)

    Zinn-Justin, J.

    1974-01-01

    A perturbation expansion of the partition function, for a spin system on a lattice, is used in order to justify the renormalization group equations satisfied by the correlation functions in the critical domain of a second-order phase transition. These renormalization group equations correspond to a field theoretical formulation of Wilson's theory of critical phenomena [fr

  3. Spin-torque ferromagnetic resonance in arbitrarily magnetized thin films

    Science.gov (United States)

    Sklenar, Joseph

    The spin Hall effect (SHE) in non-magnetic metals can be used to generate spin-transfer-torque (STT), subsequently inducing ferromagnetic resonance (FMR) in magnetic thin films; this experimental method is termed spin-torque ferromagnetic resonance (ST-FMR). Most ST-FMR experiments that are reported have an applied magnetic field in the plane of the sample and the research focuses on material combinations that have large and efficient STT. The most common way ST-FMR signals are detected is through an anisotropic magnetoresistance (AMR) rectification process. In this work we will present ST-FMR results in thin films where the magnetization has both an in-plane and out-of-plane component. The arbitrary magnetization direction is achieved by tipping the applied magnetic field out of the sample plane. We find that when the material system is a permalloy/Pt bilayer, ST-FMR signals are not mirror-symmetric upon magnetic field reversal . This is because the combination of both a STT from the bulk SHE and the Oersted field-like torque from the device do not drive the dynamics in the same manner when the field is reversed. We interpret our results in the Py/Pt experiment by extending an already established ST-FMR lineshape model to describe the general case of arbitrarily magnetized films. We compare and contrast our Py/Pt experiment with another system we measured, a Py/MoS2 bilayer. For the Py/MoS2 system, in-plane experiments suggest that a large STT is present and are comparable to what is observed for the more traditional Py/Pt system . On the other hand, the out-of-plane experiment for the Py/MoS2 system is qualitatively very different from Py/Pt. Our results suggest that ST-FMR experiments for arbitrarily magnetized magnetic films are useful in characterizing STT generated from interface rather than bulk effects. Work at Northwestern was supported by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Science and Engineering Division under grant

  4. Multiterminal semiconductor/ferromagnet probes for spin-filter scanning tunneling microscopy

    NARCIS (Netherlands)

    Vera Marun, I.J.; Jansen, R.

    2009-01-01

    We describe the fabrication of multiterminal semiconductor/ferromagnet probes for a new technique to study magnetic nanostructures: spin-filter scanning tunneling microscopy. We describe the principle of the technique, which is based on spin-polarized tunneling and subsequent analysis of the spin

  5. Thickness dependence of the triplet spin-valve effect in superconductor-ferromagnet-ferromagnet heterostructures.

    Science.gov (United States)

    Lenk, Daniel; Zdravkov, Vladimir I; Kehrle, Jan-Michael; Obermeier, Günter; Ullrich, Aladin; Morari, Roman; Krug von Nidda, Hans-Albrecht; Müller, Claus; Kupriyanov, Mikhail Yu; Sidorenko, Anatolie S; Horn, Siegfried; Deminov, Rafael G; Tagirov, Lenar R; Tidecks, Reinhard

    2016-01-01

    In nanoscale layered S/F1/N/F2/AF heterostructures, the generation of a long-range, odd-in-frequency spin-projection one triplet component of superconductivity, arising at non-collinear alignment of the magnetizations of F1 and F2, exhausts the singlet state. This yields the possibility of a global minimum of the superconducting transition temperature T c, i.e., a superconducting triplet spin-valve effect, around mutually perpendicular alignment. The superconducting triplet spin valve is realized with S = Nb a singlet superconductor, F1 = Cu41Ni59 and F2 = Co ferromagnetic metals, AF = CoO x an antiferromagnetic oxide, and N = nc-Nb a normal conducting (nc) non-magnetic metal, which serves to decouple F1 and F2. The non-collinear alignment of the magnetizations is obtained by applying an external magnetic field parallel to the layers of the heterostructure and exploiting the intrinsic perpendicular easy-axis of the magnetization of the Cu41Ni59 thin film in conjunction with the exchange bias between CoO x and Co. The magnetic configurations are confirmed by superconducting quantum interference device (SQUID) magnetic moment measurements. The triplet spin-valve effect has been investigated for different layer thicknesses, d F1, of F1 and was found to decay with increasing d F1. The data is described by an empirical model and, moreover, by calculations using the microscopic theory. The long-range triplet component of superconducting pairing is generated from the singlet component mainly at the N/F2 interface, where the amplitude of the singlet component is suppressed exponentially with increasing distance d F1. The decay length of the empirical model is found to be comparable to twice the electron mean free path of F1 and, thus, to the decay length of the singlet component in F1. Moreover, the obtained data is in qualitative agreement with the microscopic theory, which, however, predicts a (not investigated) breakdown of the triplet spin-valve effect for d F1 smaller

  6. Observation of transverse spin Nernst magnetoresistance induced by thermal spin current in ferromagnet/non-magnet bilayers.

    Science.gov (United States)

    Kim, Dong-Jun; Jeon, Chul-Yeon; Choi, Jong-Guk; Lee, Jae Wook; Surabhi, Srivathsava; Jeong, Jong-Ryul; Lee, Kyung-Jin; Park, Byong-Guk

    2017-11-09

    Electric generation of spin current via spin Hall effect is of great interest as it allows an efficient manipulation of magnetization in spintronic devices. Theoretically, pure spin current can be also created by a temperature gradient, which is known as spin Nernst effect. Here, we report spin Nernst effect-induced transverse magnetoresistance in ferromagnet/non-magnetic heavy metal bilayers. We observe that the magnitude of transverse magnetoresistance in the bilayers is significantly modified by heavy metal and its thickness. This strong dependence of transverse magnetoresistance on heavy metal evidences the generation of thermally induced pure spin current in heavy metal. Our analysis shows that spin Nernst angles of W and Pt have the opposite sign to their spin Hall angles. Moreover, our estimate implies that the magnitude of spin Nernst angle would be comparable to that of spin Hall angle, suggesting an efficient generation of spin current by the spin Nernst effect.

  7. Search for Spin Filtering By Electron Tunneling Through Ferromagnetic EuS Barriers in Pbs

    Science.gov (United States)

    Figielski, T.; Morawski, A.; Wosinski, T.; Wrotek, S.; Makosa, A.; Lusakowska, E.; Story, T.; Sipatov, A. Yu.; Szczerbakow, A.; Grasza, K.; hide

    2002-01-01

    Perpendicular transport through single- and double-barrier heterostructures consisting of ferromagnetic EuS layers embedded into PbS matrix was investigated. Manifestations of both resonant tunneling and spin filtering through EuS barrier have been observed.

  8. Experimental study of the feasibility of a spin valve based on superconductor/ferromagnet proximity effect

    International Nuclear Information System (INIS)

    Garifullin, I. A.; Garif'yanov, N. N.; Salikhov, R. I.; Westerholt, K.; Sprungmann, D.; Zabel, H.; Brucas, R.; Hjoervarsson, B.

    2007-01-01

    The feasibility of a superconducting spin valve based on superconductor/ferromagnet proximity effect is discussed. Experimental results obtained by the authors to date in studies of this problem are presented

  9. Superconducting spin switch based on superconductor-ferromagnet nanostructures for spintronics

    International Nuclear Information System (INIS)

    Kehrle, Jan; Mueller, Claus; Obermeier, Guenter; Schreck, Matthias; Gsell, Stefan; Horn, Siegfried; Tidecks, Reinhard; Zdravkov, Vladimir; Morari, Roman; Sidorencko, Anatoli; Prepelitsa, Andrei; Antropov, Evgenii; Socrovisciiuc, Alexei; Nold, Eberhard; Tagirov, Lenar

    2011-01-01

    Very rapid developing area, spintronics, needs new devices, based on new physical principles. One of such devices - a superconducting spin-switch, consists of ferromagnetic and superconducting layers, and is based on a new phenomenon - reentrant superconductivity. The tuning of the superconducting and ferromagnetic layers thickness is investigated to optimize superconducting spin-switch effect for Nb/Cu 41 Ni 59 based nanoscale layered systems.

  10. Spin injection into a two-dimensional electron gas using inter-digital-ferromagnetic contacts

    DEFF Research Database (Denmark)

    Hu, C.M.; Nitta, J.; Jensen, Ane

    2002-01-01

    We present a model that describes the spin injection across a single interface with two electrodes. The spin-injection rate across a typical hybrid junction made of ferromagnet (FM) and a two-dimensional electron gas (2DEG) is found at the percentage level. We perforin spin-injection-detection ex......-injection-detection experiment on devices with two ferromagnetic contacts on a 2DEG confined in an InAs quantum well. A spin-injection rate of 4.5% is estimated from the measured magnetoresistance....

  11. Quantum spin and charge pumping through double quantum dots with ferromagnetic leads

    Energy Technology Data Exchange (ETDEWEB)

    Pan, Hui, E-mail: hpan@buaa.edu.cn [Department of Physics, Beijing University of Aeronautics and Astronautics, Beijing 100191 (China); Key Laboratory of Micro-Nano Measurement-Manipulation and Physics (Ministry of Education), Beihang University, Beijing 100191 (China); Chen, Ziyu; Zhao, Sufen [Department of Physics, Beijing University of Aeronautics and Astronautics, Beijing 100191 (China); Lue, Rong [Department of Physics, Tsinghua University, Beijing 100084 (China)

    2011-06-06

    The pumping of electrons through double quantum dots (DQDs) attached to ferromagnetic leads have been theoretically investigated by using the nonequilibrium Green's function method. It is found that an oscillating electric field applied to the quantum dot may give rise to the pumped charge and spin currents. In the case that both leads are ferromagnet, a pure spin current can be generated in the antiparallel magnetization configuration, where no net charge current exists. The possibility of manipulating the pumped spin current is explored by tuning the dot level and the ac field. By making use of various tunings, the magnitude and direction of the pumped spin current can be well controlled. For the case that only one lead is ferromagnetic, both of the charge and spin currents can be pumped and flow in opposite directions on the average. The control of the magnitude and direction of the pumped charge and spin currents is also discussed by means of the magnetic flux threading through the DQD ring. -- Highlights: → We theoretically investigate the pumping of electrons through double quantum dots attached to ferromagnetic leads. → An oscillating electric field applied to the quantum dot may give rise to the pumped charge and spin currents. → When both leads are ferromagnet, a pure spin current can be generated in the antiparallel magnetization configuration. → By making use of various tunings, the magnitude and direction of the pumped spin current can be well controlled. → When only one lead is ferromagnetic, both of the charge and spin currents can be pumped and flow in opposite directions.

  12. Spin pumping through a topological insulator probed by x-ray detected ferromagnetic resonance

    Energy Technology Data Exchange (ETDEWEB)

    Figueroa, A.I., E-mail: aifigueg@gmail.com [Magnetic Spectroscopy Group, Diamond Light Source, Didcot OX11 0DE (United Kingdom); Baker, A.A. [Magnetic Spectroscopy Group, Diamond Light Source, Didcot OX11 0DE (United Kingdom); Department of Physics, Clarendon Laboratory, University of Oxford, Oxford OX1 3PU (United Kingdom); Collins-McIntyre, L.J.; Hesjedal, T. [Department of Physics, Clarendon Laboratory, University of Oxford, Oxford OX1 3PU (United Kingdom); Laan, G. van der [Magnetic Spectroscopy Group, Diamond Light Source, Didcot OX11 0DE (United Kingdom)

    2016-02-15

    In the field of spintronics, the generation of a pure spin current (without macroscopic charge flow) through spin pumping of a ferromagnetic (FM) layer opens up the perspective of a new generation of dissipation-less devices. Microwave driven ferromagnetic resonance (FMR) can generate a pure spin current that enters adjacent layers, allowing for both magnetization reversal (through spin-transfer torque) and to probe spin coherence in non-magnetic materials. However, standard FMR is unable to probe multilayer dynamics directly, since the measurement averages over the contributions from the whole system. The synchrotron radiation-based technique of x-ray detected FMR (XFMR) offers an elegant solution to this drawback, giving access to element-, site-, and layer-specific dynamical measurements in heterostructures. In this work, we show how XFMR has provided unique information to understand spin pumping and spin transfer torque effects through a topological insulator (TI) layer in a pseudo-spin valve heterostructure. We demonstrate that TIs function as efficient spin sinks, while also allowing a limited dynamic coupling between ferromagnetic layers. These results shed new light on the spin dynamics of this novel class of materials, and suggest future directions for the development of room temperature TI-based spintronics. - Highlights: • X-ray detected ferromagnetic resonance is used to study the spin pumping phenomenon. • We show a powerful way to get information of spin transfer between magnetic layers. • We observe spin pumping through a topological insulators at room temperature. • Topological insulators function as efficient spin sinks.

  13. Spin pumping through a topological insulator probed by x-ray detected ferromagnetic resonance

    International Nuclear Information System (INIS)

    Figueroa, A.I.; Baker, A.A.; Collins-McIntyre, L.J.; Hesjedal, T.; Laan, G. van der

    2016-01-01

    In the field of spintronics, the generation of a pure spin current (without macroscopic charge flow) through spin pumping of a ferromagnetic (FM) layer opens up the perspective of a new generation of dissipation-less devices. Microwave driven ferromagnetic resonance (FMR) can generate a pure spin current that enters adjacent layers, allowing for both magnetization reversal (through spin-transfer torque) and to probe spin coherence in non-magnetic materials. However, standard FMR is unable to probe multilayer dynamics directly, since the measurement averages over the contributions from the whole system. The synchrotron radiation-based technique of x-ray detected FMR (XFMR) offers an elegant solution to this drawback, giving access to element-, site-, and layer-specific dynamical measurements in heterostructures. In this work, we show how XFMR has provided unique information to understand spin pumping and spin transfer torque effects through a topological insulator (TI) layer in a pseudo-spin valve heterostructure. We demonstrate that TIs function as efficient spin sinks, while also allowing a limited dynamic coupling between ferromagnetic layers. These results shed new light on the spin dynamics of this novel class of materials, and suggest future directions for the development of room temperature TI-based spintronics. - Highlights: • X-ray detected ferromagnetic resonance is used to study the spin pumping phenomenon. • We show a powerful way to get information of spin transfer between magnetic layers. • We observe spin pumping through a topological insulators at room temperature. • Topological insulators function as efficient spin sinks.

  14. Symmetry-selected spin-split hybrid states in C-60/ferromagnetic interfaces

    DEFF Research Database (Denmark)

    Li, Dongzhe; Barreteau, Cyrille; Kawahara, Seiji Leo

    2016-01-01

    The understanding of orbital hybridization and spin polarization at the organic-ferromagnetic interface is essential in the search for efficient hybrid spintronic devices. Here, using first-principles calculations, we report a systematic study of spin-split hybrid states of C60 deposited on various...

  15. Spin current generation by ultrafast laser pulses in ferromagnetic nickel films

    Science.gov (United States)

    Hurst, Jérôme; Hervieux, Paul-Antoine; Manfredi, Giovanni

    2018-01-01

    A semiclassical phase-space model is used to study the ultrafast charge and spin dynamics in thin ferromagnetic films. Both itinerant and localized magnetism are taken into account. It is shown that an oscillating spin current can be generated in the film via the application of a femtosecond laser pulse in the visible range.

  16. Spin-polarized transport in a two-dimensional electron gas with interdigital-ferromagnetic contacts

    DEFF Research Database (Denmark)

    Hu, C.-M.; Nitta, Junsaku; Jensen, Ane

    2001-01-01

    Ferromagnetic contacts on a high-mobility, two-dimensional electron gas (2DEG) in a narrow gap semiconductor with strong spin-orbit interaction are used to investigate spin-polarized electron transport. We demonstrate the use of magnetized contacts to preferentially inject and detect specific spi...

  17. Spin-filtering effect and proximity effect in normal metal/ferromagnetic insulator/normal metal/superconductor junctions

    International Nuclear Information System (INIS)

    Li Hong; Yang Wei; Yang Xinjian; Qin Minghui; Xu Yihong

    2007-01-01

    Taking into account the thickness of the ferromagnetic insulator (FI), the spin-filtering effect and proximity effect in normal metal/ferromagnetic insulator/normal metal/superconductor (NM/FI/NM/SC) junctions are studied based on an extended Blonder-Tinkham-Klapwijk (BTK) theory. It is shown that a spin-dependent energy shift during the tunneling process induces splitting of the sub-energy gap conductance peaks and the spin polarization in the ferromagnetic insulator causes an imbalance of the peak heights. Different from the ferromagnet the spin-filtering effect of the FI cannot cause the reversion of the normalized conductance in NM/FI/NM/SC junctions

  18. Spin pumping through a topological insulator probed by x-ray detected ferromagnetic resonance

    Science.gov (United States)

    Figueroa, A. I.; Baker, A. A.; Collins-McIntyre, L. J.; Hesjedal, T.; van der Laan, G.

    2016-02-01

    In the field of spintronics, the generation of a pure spin current (without macroscopic charge flow) through spin pumping of a ferromagnetic (FM) layer opens up the perspective of a new generation of dissipation-less devices. Microwave driven ferromagnetic resonance (FMR) can generate a pure spin current that enters adjacent layers, allowing for both magnetization reversal (through spin-transfer torque) and to probe spin coherence in non-magnetic materials. However, standard FMR is unable to probe multilayer dynamics directly, since the measurement averages over the contributions from the whole system. The synchrotron radiation-based technique of x-ray detected FMR (XFMR) offers an elegant solution to this drawback, giving access to element-, site-, and layer-specific dynamical measurements in heterostructures. In this work, we show how XFMR has provided unique information to understand spin pumping and spin transfer torque effects through a topological insulator (TI) layer in a pseudo-spin valve heterostructure. We demonstrate that TIs function as efficient spin sinks, while also allowing a limited dynamic coupling between ferromagnetic layers. These results shed new light on the spin dynamics of this novel class of materials, and suggest future directions for the development of room temperature TI-based spintronics.

  19. Fast nanoscale addressability of nitrogen-vacancy spins via coupling to a dynamic ferromagnetic vortex

    Science.gov (United States)

    Wolf, M. S.; Badea, R.; Berezovsky, J.

    2016-01-01

    The core of a ferromagnetic vortex domain creates a strong, localized magnetic field, which can be manipulated on nanosecond timescales, providing a platform for addressing and controlling individual nitrogen-vacancy centre spins in diamond at room temperature, with nanometre-scale resolution. Here, we show that the ferromagnetic vortex can be driven into proximity with a nitrogen-vacancy defect using small applied magnetic fields, inducing significant nitrogen-vacancy spin splitting. We also find that the magnetic field gradient produced by the vortex is sufficient to address spins separated by nanometre-length scales. By applying a microwave-frequency magnetic field, we drive both the vortex and the nitrogen-vacancy spins, resulting in enhanced coherent rotation of the spin state. Finally, we demonstrate that by driving the vortex on fast timescales, sequential addressing and coherent manipulation of spins is possible on ∼100 ns timescales. PMID:27296550

  20. Disentanglement of bulk and interfacial spin Hall effect in ferromagnet/normal metal interface

    Science.gov (United States)

    Zhou, X.; Tang, M.; Fan, X. L.; Qiu, X. P.; Zhou, S. M.

    2016-10-01

    Spin Hall effect in PdPt alloys in contact with ferromagnetic Ni80Fe20 alloys has been studied by spin torque ferromagnetic resonance technique. The spin torque spin Hall angle (ST-SHA) proves to be contributed by the interfacial and bulk SHAs. The bulk SHA is dominated by the skew scattering and reaches a maximal value for the largest randomization of Pt and Pd atoms at the intermediate alloy composition. In particular, the interfacial SHA becomes prominent for Pt-rich alloys. This phenomenon indicates the enhanced Rashba spin-orbit coupling at the interface, as Pt has a stronger spin-orbit coupling and larger z -potential gradient compared to Pd. The present work highlights the interfacial SHA and provides a pathway to improve the functionality and performance of the next generation spintronic devices.

  1. Coexistence of two vector order parameters: a holographic model for ferromagnetic superconductivity

    Energy Technology Data Exchange (ETDEWEB)

    Amoretti, Andrea [Dipartimento di Fisica, Università di Genova, and I.N.F.N. - Sezione di Genova, via Dodecaneso 33, 16146, Genova (Italy); Braggio, Alessandro [CNR-SPIN, via Dodecaneso 33, 16146, Genova (Italy); Maggiore, Nicola; Magnoli, Nicodemo [Dipartimento di Fisica, Università di Genova, and I.N.F.N. - Sezione di Genova, via Dodecaneso 33, 16146, Genova (Italy); Musso, Daniele [Physique Théorique et Mathématique, Université Libre de Bruxelles, C.P. 231, 1050 Bruxelles (Belgium)

    2014-01-13

    We study a generalization of the standard holographic p-wave superconductor featuring two interacting vector order parameters. Basing our argument on the symmetry and linear response properties of the model, we propose it as a holographic effective theory describing a strongly coupled ferromagnetic superconductor. We show that the two order parameters undergo concomitant condensations as a manifestation of an intrinsically interlaced charge/spin dynamics. Such intertwined dynamics is confirmed by the study of the transport properties. We characterize thoroughly the equilibrium and the linear response (i.e. optical conductivity and spin susceptibility) of the model at hand by means of a probe approximation analysis. Some insight about the effects of backreaction in the normal phase can be gained by analogy with the s-wave unbalanced holographic superconductor.

  2. Ferromagnetic Spin Coupling as the Origin of 0.7 Anomaly in Quantum Point Contacts

    OpenAIRE

    Aryanpour, K.; Han, J. E.

    2008-01-01

    We study one-dimensional itinerant electron models with ferromagnetic coupling to investigate the origin of 0.7 anomaly in quantum point contacts. Linear conductance calculations from the quantum Monte Carlo technique for spin interactions of different spatial range suggest that $0.7(2e^{2}/h)$ anomaly results from a strong interaction of low-density conduction electrons to ferromagnetic fluctuations formed across the potential barrier. The conductance plateau appears due to the strong incohe...

  3. Oxide Ferromagnetic Semiconductors for Spin-Electronic Transprt

    International Nuclear Information System (INIS)

    Pandey, R.K.

    2008-01-01

    The objective of this research was to investigate the viability of oxide magnetic semiconductors as potential materials for spintronics. We identified some members of the solid solution series of ilmenite (FeTiO3) and hematite (Fe2O3), abbreviated as (IH) for simplicity, for our investigations based on their ferromagnetic and semiconducting properties. With this objective in focus we limited our investigations to the following members of the modified Fe-titanates: IH33 (ilmenitehematite with 33 atomic percent hematite), IH45 (ilmenite-hematite with 45 atomic percent hematite), Mn-substituted ilmenite (Mn-FeTiO3), and Mn-substituted pseudobrookite (Mn- Fe2TiO5). All of them are: (1) wide bandgap semiconductors with band gaps ranging in values between 2.5 to 3.5 eV; (2) n-type semiconductors; (3) they exhibit well defined magnetic hysteresis loops and (4) their magnetic Curie points are greater than 400K. Ceramic, film and single crystal samples were studied and based on their properties we produced varistors (also known as voltage dependent resistors) for microelectronic circuit protection from power surges, three-terminal microelectronic devices capable of generating bipolar currents, and an integrated structured device with controlled magnetic switching of spins. Eleven refereed journal papers, three refereed conference papers and three invention disclosures resulted from our investigations. We also presented invited papers in three international conferences and one national conference. Furthermore two students graduated with Ph.D. degrees, three with M.S. degrees and one with B.S. degree. Also two post-doctoral fellows were actively involved in this research. We established the radiation hardness of our devices in collaboration with a colleague in an HBCU institution, at the Cyclotron Center at Texas A and M University, and at DOE National Labs (Los Alamos and Brookhaven). It is to be appreciated that we met most of our goals and expanded vastly the scope of

  4. Ferromagnetic spin coupling as the origin of 0.7 anomaly in quantum point contacts.

    Science.gov (United States)

    Aryanpour, K; Han, J E

    2009-02-06

    We study one-dimensional itinerant electron models with ferromagnetic coupling to investigate the origin of the 0.7 anomaly in quantum point contacts. Linear conductance calculations from the quantum Monte Carlo technique for spin interactions of different spatial range suggest that 0.7(2e;{2}/h) anomaly results from a strong interaction of low-density conduction electrons to ferromagnetic fluctuations formed across the potential barrier. The conductance plateau appears due to the strong incoherent scattering at high temperature when the electron traversal time matches the time scale of dynamic ferromagnetic excitations.

  5. Spin-filter effect in normal metal/ferromagnetic insulator/normal metal/superconductor structures

    International Nuclear Information System (INIS)

    Li, Hong; Yang, Wei; Yang, Xinjian; Qin, Minghui; Guo, Jianqin

    2007-01-01

    Taking into account the thickness of the ferromagnetic insulator, the spin-filter effect in normal metal/ferromagnetic insulator/normal metal/superconductor (NM/FI/NM/SC) junctions is studied based on the Blonder-Tinkham-Klapwijk (BTK) theory. It is shown that a spin-dependent energy shift during the tunneling process induces splitting of the subgap resonance peaks. The spin polarization due to the spin-filter effect of the FI causes an imbalance of the peaks heights and can enhance the Zeeman splitting of the gap peaks caused by an applied magnetic field. The spin-filter effect has no contribution to the proximity-effect-induced superconductivity in NM interlayer

  6. Dependence of the Efficiency of Spin Hall Torque on the Transparency of Pt-Ferromagnetic Layer Interfaces

    OpenAIRE

    Pai, Chi-Feng; Ou, Yongxi; Ralph, D. C.; Buhrman, R. A.

    2014-01-01

    We report that spin current transport across Pt-ferromagnet (FM) interfaces is strongly dependent on the type and the thickness of the FM layer and on post-deposition processing protocols. By employing both harmonic voltage measurements and spin-torque ferromagnetic resonance measurements, we find that the efficiency of the Pt spin Hall effect in exerting a damping-like spin torque on the FM ranges from 0.10 under different interfacial conditions. We also show that the temperature...

  7. Characterization of perpendicular STT-MRAM by spin torque ferromagnetic resonance

    Science.gov (United States)

    Sha, Chengcen; Yang, Liu; Lee, Han Kyu; Barsukov, Igor; Zhang, Jieyi; Krivorotov, Ilya

    We describe a method for simple quantitative measurement of magnetic anisotropy and Gilbert damping of the MTJ free layer in individual perpendicular STT-MRAM devices by spin torque ferromagnetic resonance (ST-FMR) with magnetic field modulation. We first show the dependence of ST-FMR spectra of an STT-MRAM element on out-of-plane magnetic field. In these spectra, resonances arising from excitation of the quasi-uniform and higher order spin wave eigenmodes of the free layer as well as acoustic mode of the synthetic antiferromagnet (SAF) are clearly seen. The quasi-uniform mode frequency at zero field gives magnetic anisotropy field of the free layer. Then we show dependence of the quasi-uniform mode linewidth on frequency is linear over a range of frequencies but deviatesfrom linearity in the low and high frequency regimes. Comparison to ST-FMR spectrareveals that the high frequency line broadening is linked to the SAF mode softening near the SAF spin flop transition at 5 kG. In the low field regime, the SAF mode frequency approaches that of the quasi-uniform mode, and resonant coupling of the modes leads to the line broadening. A linear fit to the linewidth data outside of the high and low field regimes gives the Gilbert damping parameter of the free layer. This work was supported by the Samsung Global MRAM Innovation Program.

  8. Electric-field-controlled spin reversal in a quantum dot with ferromagnetic contacts

    Science.gov (United States)

    Hauptmann, J. R.; Paaske, J.; Lindelof, P. E.

    2008-05-01

    Manipulation of the spin states of a quantum dot by purely electrical means is a highly desirable property of fundamental importance for the development of spintronic devices such as spin filters, spin transistors and single spin memories as well as for solid-state qubits. An electrically gated quantum dot in the Coulomb blockade regime can be tuned to hold a single unpaired spin-1/2, which is routinely spin polarized by an applied magnetic field. Using ferromagnetic electrodes, however, the quantum dot becomes spin polarized by the local exchange field. Here, we report on the experimental realization of this tunnelling-induced spin splitting in a carbon-nanotube quantum dot coupled to ferromagnetic nickel electrodes with a strong tunnel coupling ensuring a sizeable exchange field. As charge transport in this regime is dominated by the Kondo effect, we can use this sharp many-body resonance to read off the local spin polarization from the measured bias spectroscopy. We demonstrate that the exchange field can be compensated by an external magnetic field, thus restoring a zero-bias Kondo resonance, and we demonstrate that the exchange field itself, and hence the local spin polarization, can be tuned and reversed merely by tuning the gate voltage.

  9. Phase transitions in continuum ferromagnets with unbounded spins

    Energy Technology Data Exchange (ETDEWEB)

    Daletskii, Alexei, E-mail: alex.daletskii@york.ac.uk [Department of Mathematics, University of York, York YO10 DD (United Kingdom); Kondratiev, Yuri, E-mail: kondrat@math.uni-bielefeld.de [Fakultät für Mathematik, Universität Bielefeld, Bielefeld D-33615 (Germany); Kozitsky, Yuri, E-mail: jkozi@hektor.umcs.lublin.pl [Instytut Matematyki, Uniwersytet Marii Curie-Skłodowskiej, 20-031 Lublin (Poland)

    2015-11-15

    States of thermal equilibrium of an infinite system of interacting particles in ℝ{sup d} are studied. The particles bear “unbounded” spins with a given symmetric a priori distribution. The interaction between the particles is pairwise and splits into position-position and spin-spin parts. The position-position part is described by a superstable potential, and the spin-spin part is attractive and of finite range. Thermodynamic states of the system are defined as tempered Gibbs measures on the space of marked configurations. It is proved that the set of such measures contains at least two elements if the activity is big enough.

  10. Modulation of pure spin currents with a ferromagnetic insulator

    Science.gov (United States)

    Villamor, Estitxu; Isasa, Miren; Vélez, Saül; Bedoya-Pinto, Amilcar; Vavassori, Paolo; Hueso, Luis E.; Bergeret, F. Sebastián; Casanova, Fèlix

    2015-01-01

    We propose and demonstrate spin manipulation by magnetically controlled modulation of pure spin currents in cobalt/copper lateral spin valves, fabricated on top of the magnetic insulator Y3F e5O12 (YIG). The direction of the YIG magnetization can be controlled by a small magnetic field. We observe a clear modulation of the nonlocal resistance as a function of the orientation of the YIG magnetization with respect to the polarization of the spin current. Such a modulation can only be explained by assuming a finite spin-mixing conductance at the Cu/YIG interface, as it follows from the solution of the spin-diffusion equation. These results open a path towards the development of spin logics.

  11. Spin-Dependent Transparency of Ferromagnet/Superconductor Interfaces

    Czech Academy of Sciences Publication Activity Database

    Xia, K.; Kelly, P. J.; Bauer, G. E. W.; Turek, Ilja

    2002-01-01

    Roč. 89, č. 16 (2002), s. 166603 ISSN 0031-9007 R&D Projects: GA ČR GA202/00/0122 Institutional research plan: CEZ:AV0Z2041904 Keywords : interface * ferromagnet * superconductor Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 7.323, year: 2002

  12. Anomalous spin distribution in the superconducting ferromagnet UCoGe studied by polarized neutron diffraction

    NARCIS (Netherlands)

    Prokeš, K.; de Visser, A.; Huang, Y.K.; Fåk, B.; Ressouche, E.

    2010-01-01

    We report a polarized neutron-diffraction study conducted to reveal the nature of the weak ferromagnetic moment in the superconducting ferromagnet UCoGe. We find that the ordered moment in the normal phase in low magnetic fields (B∥c) is predominantly located at the U atom and has a magnitude of

  13. Ferromagnetic resonance study of the half-Heusler alloy NiMnSb. The benefit of using NiMnSb as a ferromagnetic layer in pseudo-spin-valve based spin-torque oscillators

    Energy Technology Data Exchange (ETDEWEB)

    Riegler, Andreas

    2011-11-25

    -beam lithography and measured by ferromagnetic resonance. The damping remains in the low 10{sup -3} range as determined directly by extracting the Gilbert damping from the line width. Additionally magnetostatic modes are observed in arrays of elements, which is further evidence of high material quality of the samples. By sputtering various metals on top of the NiMnSb, spin pumping from the ferromagnet into the non-magnetic layer is investigated. After these material investigations, pseudo-spin-valves using NiMnSb as one of the ferromagnet, in combination with Permalloy were fabricating using a self-aligned lithography process. These samples show a GMR ratio of 3.4% at room temperature and almost double at low temperature, comparing favourably to the best single stack GMR structures reported to date. Moreover, current induced switching measurements show promisingly low current densities are necessary to change the magnetic orientation of the free layer. These current densities compete with state-of-the-art GMR devices for metal based structures and almost with tunnel junction devices. The true potential of these devices however comes to light when they are operated as spin torque oscillators to emit high frequency, tunable, narrow spectrum electromagnetic waves. These Heusler based STOs show an outstanding q-factor of 4180, even when operating in the absence of an external field, a value which bests the highest value in the literature by more than an order of magnitude. While these devices currently still suffer from the same limited output power as all STO reported to date, their sub-micron lateral dimensions make the fabrication of an on-chip array of coupled oscillators, which is a promising path forward towards industrially relevant output power.

  14. Itinerant ferromagnetism in actinide 5 f -electron systems: Phenomenological analysis with spin fluctuation theory

    Science.gov (United States)

    Tateiwa, Naoyuki; Pospíšil, Jiří; Haga, Yoshinori; Sakai, Hironori; Matsuda, Tatsuma D.; Yamamoto, Etsuji

    2017-07-01

    We have carried out an analysis of magnetic data in 69 uranium, 7 neptunium, and 4 plutonium ferromagnets with the spin fluctuation theory developed by Takahashi [Y. Takahashi, J. Phys. Soc. Jpn. 55, 3553 (1986), 10.1143/JPSJ.55.3553]. The basic and spin fluctuation parameters of the actinide ferromagnets are determined and the applicability of the spin fluctuation theory to actinide 5 f system has been discussed. Itinerant ferromagnets of the 3 d transition metals and their intermetallics follow a generalized Rhodes-Wohlfarth relation between peff/ps and TC/T0 , viz., peff/ps∝(TC/T0) -3 /2 . Here, ps, peff, TC, and T0 are the spontaneous and effective magnetic moments, the Curie temperature, and the width of spin fluctuation spectrum in energy space, respectively. The same relation is satisfied for TC/T0uranium and neptunium ferromagnets below (TC/T0)kink=0.32 ±0.02 , where a kink structure appears in relation between the two quantities. ps increases more weakly above (TC/T0)kink. A possible interpretation with the TC/T0 dependence of ps is given.

  15. Effect of ferromagnetic exchange field on band gap and spin ...

    Indian Academy of Sciences (India)

    Partha Goswami

    2018-02-19

    Feb 19, 2018 ... these systems as a function of magnetisation strength. We also discuss the ..... require the discriminant of the quadratic in the variableε to be zero. This yields .... system for graphene in WSe2 at the Dirac point K. The band identification is as follows: spin-up valence band: '− *', spin-up conduction band: '−' ...

  16. Effect of ferromagnetic exchange field on band gap and spin ...

    Indian Academy of Sciences (India)

    The polarisation is found to be electric field tunable as well. Finally, there is anticrossing of non-parabolic bands with opposite spins, the gap closing with same spins, etc. around the Dirac points. A direct electric field control of magnetism at the nanoscale is needed here. The magnetic multiferroics, like B i F e O 3 (BFO), are ...

  17. Angular dependence and symmetry of Rashba spin torque in ferromagnetic heterostructures

    KAUST Repository

    Ortiz Pauyac, Christian

    2013-06-26

    In a ferromagnetic heterostructure, the interplay between Rashba spin-orbit coupling and exchange splitting gives rise to a current-driven spin torque. In a realistic device setup, we investigate the Rashba spin torque in the diffusive regime and report two major findings: (i) a nonvanishing torque exists at the edges of the device even when the magnetization and effective Rashba field are aligned; (ii) anisotropic spin relaxation rates driven by the Rashba spin-orbit coupling assign the spin torque a general expression T = T y (θ) m × (y × m) + T y (θ) y × m + T z (θ) m × (z × m) + T z (θ) z × m, where the coefficients T, y, z depend on the magnetization direction. Our results agree with recent experiments. © 2013 AIP Publishing LLC.

  18. Femtosecond Single-Shot Imaging of Nanoscale Ferromagnetic Order in Co/Pd Multilayers using Resonant X-ray Holography

    Energy Technology Data Exchange (ETDEWEB)

    Wang, Tianhan; Zhu, Diling; Benny Wu,; Graves, Catherine; Schaffert, Stefan; Rander, Torbjorn; Muller, leonard; Vodungbo, Boris; Baumier, Cedric; Bernstein, David P.; Brauer, Bjorn; Cros, Vincent; Jong, Sanne de; Delaunay, Renaud; Fognini, Andreas; Kukreja, Roopali; Lee, Sooheyong; Lopez-Flores, Victor; Mohanty, Jyoti; Pfau, Bastian; Popescu, 5 Horia

    2012-05-15

    We present the first single-shot images of ferromagnetic, nanoscale spin order taken with femtosecond x-ray pulses. X-ray-induced electron and spin dynamics can be outrun with pulses shorter than 80 fs in the investigated fluence regime, and no permanent aftereffects in the samples are observed below a fluence of 25 mJ/cm{sup 2}. Employing resonant spatially-muliplexed x-ray holography results in a low imaging threshold of 5 mJ/cm{sup 2}. Our results open new ways to combine ultrafast laser spectroscopy with sequential snapshot imaging on a single sample, generating a movie of excited state dynamics.

  19. Direct observation of spin-resolved full and empty electron states in ferromagnetic surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Berti, G., E-mail: giulia.berti@polimi.it; Calloni, A.; Brambilla, A.; Bussetti, G.; Duò, L.; Ciccacci, F. [Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, I-20133, Milano (Italy)

    2014-07-15

    We present a versatile apparatus for the study of ferromagnetic surfaces, which combines spin-polarized photoemission and inverse photoemission spectroscopies. Samples can be grown by molecular beam epitaxy and analyzed in situ. Spin-resolved photoemission spectroscopy analysis is done with a hemispherical electron analyzer coupled to a 25 kV-Mott detector. Inverse photoemission spectroscopy experiments are performed with GaAs crystals as spin-polarized electron sources and a UV bandpass photon detector. As an example, measurements on the oxygen passivated Fe(100)-p(1×1)O surface are presented.

  20. Local electron-electron interaction strength in ferromagnetic nickel determined by spin-polarized positron annihilation.

    Science.gov (United States)

    Ceeh, Hubert; Weber, Josef Andreas; Weber, Josef Andreass; Böni, Peter; Leitner, Michael; Benea, Diana; Chioncel, Liviu; Ebert, Hubert; Minár, Jan; Vollhardt, Dieter; Hugenschmidt, Christoph

    2016-02-16

    We employ a positron annihilation technique, the spin-polarized two-dimensional angular correlation of annihilation radiation (2D-ACAR), to measure the spin-difference spectra of ferromagnetic nickel. The experimental data are compared with the theoretical results obtained within a combination of the local spin density approximation (LSDA) and the many-body dynamical mean-field theory (DMFT). We find that the self-energy defining the electronic correlations in Ni leads to anisotropic contributions to the momentum distribution. By direct comparison of the theoretical and experimental results we determine the strength of the local electronic interaction U in ferromagnetic Ni as 2.0 ± 0.1 eV.

  1. Electron-spin polarization in tunnel junctions with ferromagnetic EuS barriers

    International Nuclear Information System (INIS)

    Hao, X.; Moodera, J.S.; Meservey, R.

    1989-01-01

    The authors report here spin-polarized tunneling experiments using non-ferromagnetic electrodes and ferromagnetic EuS barriers. Because of the conduction band in EuS splits into spin-up and spin-down subbands when the temperature is below 16.7 K, the Curie temperature of EuS, the tunnel barrier for electrons with different spin directions is different, therefore giving rise to tunnel current polarization. The spin-filter effect, as it may be called, was observed earlier, directly or indirectly, by several groups: Esaki et al. made a tunneling study on junctions having EuS and EuSe barriers; Thompson et al. studied Schottky barrier tunneling between In and doped EuS; Muller et al. and Kisker et al. performed electron field emission experiments on EuS-coated tungsten tips. The field emission experiments gave a maximum polarization of (89 + 7)% for the emitted electrons. Although the previous tunneling studies did not directly show electron polarization, their results were explained by the same spin- filter effect. This work uses the spin-polarized tunneling technique to show directly that tunnel current is indeed polarized and polarization can be as high as 85%

  2. Large spin-valve effect in a lateral spin-valve device based on ferromagnetic semiconductor GaMnAs

    Science.gov (United States)

    Asahara, Hirokatsu; Kanaki, Toshiki; Ohya, Shinobu; Tanaka, Masaaki

    2018-03-01

    We investigate the spin-dependent transport properties of a lateral spin-valve device based on the ferromagnetic semiconductor GaMnAs. This device is composed of a GaMnAs channel layer grown on GaAs with a narrow trench across the channel. Its current-voltage characteristics show tunneling behavior. Large magnetoresistance (MR) ratios of more than ˜10% are obtained. These values are much larger than those (˜0.1%) reported for lateral-type spin metal-oxide-semiconductor field-effect transistors. The magnetic field direction dependence of the MR curve differs from that of the anisotropic magnetoresistance of GaMnAs, which confirms that the MR signal originates from the spin-valve effect between the GaMnAs electrodes.

  3. Magnetoresistance in ferromagnetic multilayer with strong interfacial spin-orbit coupling (Conference Presentation)

    Science.gov (United States)

    Kim, Junyeon; Karube, Shutaro; Chen, Yan-Ting; Kondou, Kouta; Tatara, Gen; Otani, YoshiChika

    2016-10-01

    Spin-charge conversion induced by spin-orbit coupling (SOC) is attractive topic for alternative magnetization manipulation and involved various novel phenomena. Particularly Bi-based structure draws interest due to its large Rashba-Edelstein effect (REE) at interface between non-magnetic metal and Bi [1]. A recent report showed that spin-to-charge current conversion becomes more efficient when Bi2O3 is employed on behalf of the Bi [2]. Here we report novel type of magnetoresistance (MR) in Co25Fe75/Cu/Bi2O3 multilayer. This novel MR comes from conversion between spin and charge current at Cu/Bi2O3 interface, and distinctive spin transfer torque dependent on magnetization of the ferromagnetic Co25Fe75 layer. A Co25Fe75 (5)/Cu (0-30)/Bi2O3 (20) (unit:nm) multilayer was deposited with electron beam evaporation on shadow masked Si substrate. Hall bar shaped shadow mask was patterned with photo-lithography method. The MR measurement was performed via 4-point probe method with changing magnitude or angle of external field. Note that external field for angle dependent measurement was 6 T to make sure complete saturation of ferromagnetic layer. We found characteristic resistance drop when the magnetization of ferromagnetic layer is parallel to magnetic direction of spin accumulation, which is similar to spin Hall magnetoresistance (SMR) [3,4]. Further discussion will be given. [1] J. C. Rojas Sanchez et al. Nature Comm. 4, 2944 (2013). [2] S. Karube et al. Appl. Phys. Express. 9, 03301 (2016). [3] H. Nakayama et al. Phys. Rev. Lett. 110, 206601 (2013). [4] J. Kim et al. Phys. Rev. Lett. (in press).

  4. Unexpected ferromagnetic ordering enhancement with crystallite size growth observed in La{sub 0.5}Ca{sub 0.5}MnO₃ nanoparticles

    Energy Technology Data Exchange (ETDEWEB)

    Iniama, G.; Ita, B. I. [Department of Pure and Applied Chemistry, University of Calabar, Calabar (Nigeria); Presa, P. de la, E-mail: pmpresa@ucm.es; Hernando, A. [Instituto de Magnetismo Aplicado, UCM-ADIF-CSIC, 28230 Las Rozas (Spain); Fac. CC Físicas, Dpto. Física de Materiales, Univ. Complutense de Madrid, 28040 Madrid (Spain); Alonso, J. M. [Instituto de Magnetismo Aplicado, UCM-ADIF-CSIC, 28230 Las Rozas (Spain); Instituto de Ciencia de Materiales, CSIC, 28049-Madrid (Spain); Multigner, M. [Instituto de Magnetismo Aplicado, UCM-ADIF-CSIC, 28230 Las Rozas (Spain); Cortés-Gil, R.; Ruiz-González, M. L. [Fac. CC Químicas, Dpto. Química Inorgánica, Univ. Complutense de Madrid, 28040 Madrid (Spain); Gonzalez-Calbet, J. M. [Instituto de Magnetismo Aplicado, UCM-ADIF-CSIC, 28230 Las Rozas (Spain); Fac. CC Químicas, Dpto. Química Inorgánica, Univ. Complutense de Madrid, 28040 Madrid (Spain)

    2014-09-21

    In this paper, the physical properties of half-doped manganite La{sub 0.5}Ca{sub 0.5}MnO₃ with crystallite sizes ranging from 15 to 40 nm are investigated. As expected, ferromagnetic order strengthens at expense of antiferromagnetic one as crystallite size is reduced to 15 nm. However, contrary to previously reported works, an enhancement of saturation magnetization is observed as crystallite size increases from 15 to 22 nm. This unexpected behavior is accompanied by an unusual cell volume variation that seems to induce ferromagnetic-like behavior at expense of antiferromagnetic one. Besides, field cooled hysteresis loops show exchange bias field and coercivity enhancement for increasing cooling fields, which suggest a kind of core-shell structure with AFM-FM coupling for crystallite sizes as small as 15 nm. It is expected that inner core orders antiferromagnetically, whereas uncompensated surface spins behave as spin glass with ferromagnetic-like ordering.

  5. Pseudo spin-valve behavior in oxide ferromagnet/superconductor/ferromagnet trilayers

    Energy Technology Data Exchange (ETDEWEB)

    Pang, B.S.H. [Device Materials Group, Department of Materials Science and Metallurgy, University of Cambridge, New Museum Site, Pembroke Street, Cambridge CB2 3QZ (United Kingdom)]. E-mail: brianpang@cantab.net; Bell, C. [Device Materials Group, Department of Materials Science and Metallurgy, University of Cambridge, New Museum Site, Pembroke Street, Cambridge CB2 3QZ (United Kingdom); Tomov, R.I. [Device Materials Group, Department of Materials Science and Metallurgy, University of Cambridge, New Museum Site, Pembroke Street, Cambridge CB2 3QZ (United Kingdom); Durrell, J.H. [Device Materials Group, Department of Materials Science and Metallurgy, University of Cambridge, New Museum Site, Pembroke Street, Cambridge CB2 3QZ (United Kingdom); Blamire, M.G. [Device Materials Group, Department of Materials Science and Metallurgy, University of Cambridge, New Museum Site, Pembroke Street, Cambridge CB2 3QZ (United Kingdom)

    2005-06-20

    La{sub 0.7}Ca{sub 0.3}MnO{sub 3}/YBa{sub 2}Cu{sub 3}O{sub 7-{delta}}/La{sub 0.67}Sr{sub 0.33}MnO{sub 3} heterostructural devices with double coercivity have been fabricated. The superconducting critical current (I{sub c}) and critical temperature in both parallel (P) and antiparallel (AP) magnetic configurations remained unchanged within our measurement limits. This observation is contrary to results obtained elsewhere using similar metallic systems. A pseudo spin-valve magnetoresistive (MR) characteristic was observed at bias current (I{sub bias}){approx}I{sub c} at temperatures below the onset of superconductivity. The effect increased with decreasing temperature and I{sub bias} and can be explained using the assumption of the electron spin-charge separation.

  6. Intraband and interband spin-orbit torques in noncentrosymmetric ferromagnets

    KAUST Repository

    Li, Hang

    2015-04-01

    Intraband and interband contributions to the current-driven spin-orbit torque in magnetic materials lacking inversion symmetry are theoretically studied using the Kubo formula. In addition to the current-driven fieldlike torque TFL=τFLm×uso (uso being a unit vector determined by the symmetry of the spin-orbit coupling), we explore the intrinsic contribution arising from impurity-independent interband transitions and producing an anti-damping-like torque of the form TDL=τDLm×(uso×m). Analytical expressions are obtained in the model case of a magnetic Rashba two-dimensional electron gas, while numerical calculations have been performed on a dilute magnetic semiconductor (Ga,Mn)As modeled by the Kohn-Luttinger Hamiltonian exchange coupled to the Mn moments. Parametric dependencies of the different torque components and similarities to the analytical results of the Rashba two-dimensional electron gas in the weak disorder limit are described.

  7. Ferromagnetic and Antiferromagnetic Coupling of Spin Molecular Interfaces with High Thermal Stability.

    Science.gov (United States)

    Avvisati, Giulia; Cardoso, Claudia; Varsano, Daniele; Ferretti, Andrea; Gargiani, Pierluigi; Betti, Maria Grazia

    2018-03-26

    We report an advanced organic spin-interface architecture with magnetic remanence at room temperature, constituted by metal phthalocyanine molecules magnetically coupled with Co layer(s), mediated by graphene. Fe- and Cu-phthalocyanines assembled on graphene/Co have identical structural configurations, but FePc couples antiferromagnetically with Co up to room temperature, while CuPc couples ferromagnetically with weaker coupling and thermal stability, as deduced by element-selective X-ray magnetic circular dichroic signals. The robust antiferromagnetic coupling is stabilized by a superexchange interaction, driven by the out-of-plane molecular orbitals responsible of the magnetic ground state and electronically decoupled from the underlying metal via the graphene layer, as confirmed by ab initio theoretical predictions. These archetypal spin interfaces can be prototypes to demonstrate how antiferromagnetic and/or ferromagnetic coupling can be optimized by selecting the molecular orbital symmetry.

  8. Ferromagnetic transitions of a spin-one Ising film in a surface and bulk transverse fields

    International Nuclear Information System (INIS)

    Saber, A.; Lo Russo, S.; Mattei, G.; Mattoni, A.

    2002-01-01

    Using the effective field theory method, we have calculated the Curie temperature of a spin-one Ising ferromagnetic film in a surface and bulk transverse fields. Numerical calculations give phase diagrams under various parameters. Surface exchange enhancement is considered. The dependence of the critical transverse field on film thickness, and phase diagrams in the fields, critical surface transverse field versus the bulk one are presented

  9. Understanding lattice defects to influence ferromagnetic order of ZnO nanoparticles by Ni, Cu, Ce ions

    Energy Technology Data Exchange (ETDEWEB)

    Verma, Kuldeep Chand, E-mail: dkuldeep.physics@gmail.com [Department of Physics, Panjab University, Chandigarh 160014 (India); Kotnala, R.K., E-mail: rkkotnala@gmail.com [CSIR-National Physical Laboratory, New Delhi 110012 (India)

    2017-02-15

    Future spintronics technologies based on diluted magnetic semiconductors (DMS) will rely heavily on a sound understanding of the microscopic origins of ferromagnetism in such materials. It remains unclear, however, whether the ferromagnetism in DMS is intrinsic - a precondition for spintronics - or due to dopant clustering. For this, we include a simultaneous doping from transition metal (Ni, Cu) and rare earth (Ce) ions in ZnO nanoparticles that increase the antiferromagnetic ordering to achieve high-T{sub c} ferromagnetism. Rietveld refinement of XRD patterns indicate that the dopant ions in ZnO had a wurtzite structure and the dopants, Ni{sup 2+}, Cu{sup 2+}, Ce{sup 3+} ions, are highly influenced the lattice constants to induce lattice defects. The Ni, Cu, Ce ions in ZnO have nanoparticles formation than nanorods was observed in pure sample. FTIR involve some organic groups to induce lattice defects and the metal-oxygen bonding of Zn, Ni, Cu, Ce and O atoms to confirm wurtzite structure. Raman analysis evaluates the crystalline quality, structural disorder and defects in ZnO lattice with doping. Photoluminescence spectra have strong near-band-edge emission and visible emission bands responsible for defects due to oxygen vacancies. The energy band gap is calculated using Tauc relation. Room temperature ferromagnetism has been described due to bound magnetic polarons formation with Ni{sup 2+}, Cu{sup 2+}, Ce{sup 3+} ions in ZnO via oxygen vacancies. The zero field and field cooling SQUID measurement confirm the strength of antiferromagnetism in ZnO. The field cooling magnetization is studied by Curie-Weiss law that include antiferromagnetic interactions up to low temperature. The XPS spectra have involve +3/+4 oxidation states of Ce ions to influence the observed ferromagnetism. - Graphical abstract: The lattice defects/vacancies attributed by Ni and Ce ions in the wurtzite ZnO structure are responsible in high T{sub c} -ferromagnetism due to long-range magnetic

  10. The ferromagnet spin-1/2 Ising superlattice in a transverse field

    International Nuclear Information System (INIS)

    Bouziane, T.; Saber, M.; Belaaraj, A.; Ainane, A.

    1998-09-01

    The phase transitions of a ferromagnet spin-1/2 Ising superlattice consisting of two different materials in a transverse field is examined with the use of effective field theory that accounts for the self-spin function correlation. The critical temperature of the system is studied as a function of the thickness of the constituents in a unit cell and of exchange interactions in each material. A critical interface exchange interaction above which the interface magnetism appears is found. The effects of a uniform transverse field and the interface exchange interaction on the parameters of the system are also investigated. (author)

  11. Spin Seebeck effect in a simple ferromagnet near T c: a Ginzburg–Landau approach

    Science.gov (United States)

    Adachi, Hiroto; Yamamoto, Yutaka; Ichioka, Masanori

    2018-04-01

    A time-dependent Ginzburg–Landau theory is used to examine the longitudinal spin Seebeck effect in a simple ferromagnet in the vicinity of the Curie temperature T c. It is shown analytically that the spin Seebeck effect is proportional to the magnetization near T c, whose result is in line with the previous numerical finding. It is argued that the present result can be tested experimentally using a simple magnetic system such as EuO/Pt or EuS/Pt.

  12. Spin glass behaviour in ferromagnetic La2CoMnO6 perovskite manganite

    Science.gov (United States)

    Wang, X. L.; James, M.; Horvat, J.; Dou, S. X.

    2002-03-01

    La2CoMnO6 perovskite manganite was synthesized by solid-state reaction. Rietveld refinement of powder x-ray diffraction data indicated that this compound crystallized with an orthorhombic structure containing distorted (Co/Mn)O6 octahedra (Pnma; a = 5.5 Å b = 7.2 Å c = 5.4 Å. The dc magnetization and real part (x') of the ac susceptibility were measured at dc fields up to 1 T and an ac field of 0.1 Oe at frequencies of 21, 217, 600 and 2000 Hz over a wide range of temperatures from 300 K down to 4.2 K. A ferromagnetic transition was observed at Tc = 220 K. A spin glass ground state was also determined from the shift of a peak at 220 K in the real part of the ac susceptibility with frequency and slow spin relaxation for T < Tc as indicated by the time dependence of the remanent magnetization. The spin glass state arises from a ferromagnetic state and might be caused by competition between the ferromagnetic and antiferromagnetic interaction.

  13. Unidirectional spin-Hall and Rashba-Edelstein magnetoresistance in topological insulator-ferromagnet layer heterostructures.

    Science.gov (United States)

    Lv, Yang; Kally, James; Zhang, Delin; Lee, Joon Sue; Jamali, Mahdi; Samarth, Nitin; Wang, Jian-Ping

    2018-01-09

    The large spin-orbit coupling in topological insulators results in helical spin-textured Dirac surface states that are attractive for topological spintronics. These states generate an efficient spin-orbit torque on proximal magnetic moments. However, memory or logic spin devices based upon such switching require a non-optimal three-terminal geometry, with two terminals for the writing current and one for reading the state of the device. An alternative two-terminal device geometry is now possible by exploiting the recent discovery of the unidirectional spin Hall magnetoresistance in heavy metal/ferromagnet bilayers and unidirectional magnetoresistance in magnetic topological insulators. Here, we report the observation of such unidirectional magnetoresistance in a technologically relevant device geometry that combines a topological insulator with a conventional ferromagnetic metal. Our devices show a figure of merit (magnetoresistance per current density per total resistance) that is more than twice as large as the highest reported values in all-metal Ta/Co bilayers.

  14. β -detected NMR spin relaxation in a thin film heterostructure of ferromagnetic EuO

    Science.gov (United States)

    MacFarlane, W. A.; Song, Q.; Ingle, N. J. C.; Chow, K. H.; Egilmez, M.; Fan, I.; Hossain, M. D.; Kiefl, R. F.; Levy, C. D. P.; Morris, G. D.; Parolin, T. J.; Pearson, M. R.; Saadaoui, H.; Salman, Z.; Wang, D.

    2015-08-01

    We present β -detected NMR measurements of the spin-lattice relaxation of +8Li implanted into an epitaxial heterostructure based on a 100 nm thick film of ferromagnetic (FM) EuO as a function of temperature through its FM transition. In the FM state, the spin-lattice relaxation rate follows the same temperature dependence, determined by magnon scattering mechanisms, observed in the bulk by 153Eu NMR, but above 40 K, the signal is wiped out. We also find that +8Li stopped in material adjacent to the magnetic layer exhibits spin relaxation related to the critical slowing of the Eu spins. A particularly strong relaxation in the Au overlayer suggests an unusual strong nonlocal coupling mechanism to 8Li in the metal.

  15. Spin polarization and magnetic dichroism in core-level photoemission from ferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Menchero, Jose Gabriel [Univ. of California, Berkeley, CA (United States). Dept. of Physics

    1997-05-01

    In this thesis we present a theoretical investigation of angle- and spin-resolved core-level photoemission from ferromagnetic Fe and Ni. We also consider magneto-dichroic effects due to reversal of the photon helicity or reversal of the sample magnetization direction. In chapter 1, we provide a brief outline of the history of photoemission, and show how it has played an important role in the development of modern physics. We then review the basic elements of the theory of core-level photoemission, and discuss the validity of the some of the commonly-used approximations. In chapter 2, we present a one-electron theory to calculate spin- and angle-resolved photoemission spectra for an arbitrary photon polarization. The Hamiltonian includes both spin-orbit and exchange interactions. As test cases for the theory, we calculate the spin polarization and magnetic dichroism for the Fe 2p core level, and find that agreement with experiment is very good.

  16. Radiation damping in ferromagnetic resonance induced by a conducting spin sink

    Science.gov (United States)

    Qaid, Mohammad M.; Richter, Tim; Müller, Alexander; Hauser, Christoph; Ballani, Camillo; Schmidt, Georg

    2017-11-01

    We have investigated the damping in the ferromagnetic resonance (FMR) of yttrium iron garnet (YIG) caused by spin pumping into adjacent conducting materials, namely, Pt and the conducting polymer poly(3,4-ethylenedioxythiophene):poly(4-styrenesulfonate) (PEDOT:PSS). By a systematic study which also includes multilayers in which the conducting layer is separated from YIG by an insulator, we can show that a considerable part of the damping can be attributed to the so-called radiation damping which originates from the interaction of the magnetic fields caused by the precessing magnetization with the conducting layer. Especially, when PEDOT:PSS is used as a spin sink, the observed damping must be attributed completely to radiation damping, and no contribution from spin pumping can be identified. These results demonstrate that the Gilbert damping as a measure of spin pumping can only be used when careful control experiments accompany the investigation.

  17. A Phenomenological Model For The Spin Stiffness Of A Half-metallic Ferromagnet

    Science.gov (United States)

    Chura, Raul; Bedell, Kevin

    By using the Fermi Liquid Theory for Spin Polarized Systems, more specifically, by using the linearized form of Landau Silin Kinetic Equation, and after considering an appropriate approximation, we have obtained the dispersion relationships describing the collective modes for the spin waves in a Half Metallic Ferromagnetic (HMF) material. Our results predict the existence of a gapless mode for the spin dynamics of a HMF, in agreement with experiment. In addition, our calculations allowed us to get a phenomenological formula for the spin stiffness of HMF materials, which being entirely in terms of band theory and Landau interaction parameters, allowed us to test that formula for those HMF materials for which we were able to find, in the available literature, the required data. For these materials our model is consistent with experiment. Work supported by Grant Number CANON-CU-005-2013 at UNSAAC, Cusco, Peru.

  18. Orbital driven impurity spin effect on the magnetic order of quasi-3D cupric oxide

    Science.gov (United States)

    Ganga, B. G.; Santhosh, P. N.; Nanda, B. R. K.

    2017-04-01

    Density functional calculations are performed to study the magnetic order of the severely distorted square planar cupric oxide (CuO) and local spin disorder in it in the presence of the transition metal impurities M (=Cr, Mn, Fe, Co and Ni). The distortion in the crystal structure, arisen to reduce the band energy by minimizing the covalent interaction, creates two crisscrossing zigzag spin-1/2 chains. From the spin dimer analysis we find that while the spin chain along ≤ft[1 0 \\bar{1}\\right] has strong Heisenberg type antiferromagnetic coupling (J ~ 127 meV), along ≤ft[1 0 1\\right] it exhibits weak, but robust, ferromagnetic coupling (J ~ 9 meV) mediated by reminiscent p-d covalent interactions. The impurity effect on the magnetic ordering is independent of M and purely orbital driven. If the given spin-state of M is such that the {{d}{{x2}-{{y}2}}} orbital is spin-polarized, then the original long-range ordering is maintained. However, if {{d}{{x2}-{{y}2}}} orbital is unoccupied, the absence of corresponding covalent interaction breaks the weak ferromagnetic coupling and a spin-flip takes place at the impurity site leading to breakdown of the long range magnetic ordering.

  19. Phase-resolved detection of the spin Hall angle by optical ferromagnetic resonance in perpendicularly magnetized thin films

    Science.gov (United States)

    Capua, Amir; Wang, Tianyu; Yang, See-Hun; Rettner, Charles; Phung, Timothy; Parkin, Stuart S. P.

    2017-02-01

    The conversion of charge current to spin current by the spin Hall effect is of considerable current interest from both fundamental and technological perspectives. Measurement of the spin Hall angle, especially for atomically thin systems with large magnetic anisotropies, is not straightforward. Here we demonstrate a hybrid phase-resolved optical-electrical ferromagnetic resonance method that we show can robustly determine the spin Hall angle in heavy-metal/ferromagnet bilayer systems with large perpendicular magnetic anisotropy. We present an analytical model of the ferromagnetic resonance spectrum in the presence of the spin Hall effect, in which the spin Hall angle can be directly determined from the changes in the amplitude response as a function of the spin current that is generated from a dc charge current passing through the heavy-metal layer. Increased sensitivity to the spin current is achieved by operation under conditions for which the magnetic potential is shallowest at the "Smit point." Study of the phase response reveals that the spin Hall angle can be reliably extracted from a simplified measurement that does not require scanning over time or magnetic field but rather only on the dc current. The method is applied to the Pt-Co/Ni/Co system whose spin Hall angle was to date characterized only indirectly and that is especially relevant for spin-orbit torque devices.

  20. Spin-wave resonance frequency in ferromagnetic thin film with interlayer exchange coupling and surface anisotropy

    Science.gov (United States)

    Zhang, Shuhui; Rong, Jianhong; Wang, Huan; Wang, Dong; Zhang, Lei

    2018-01-01

    We have investigated the dependence of spin-wave resonance(SWR) frequency on the surface anisotropy, the interlayer exchange coupling, the ferromagnetic layer thickness, the mode number and the external magnetic field in a ferromagnetic superlattice film by means of the linear spin-wave approximation and Green's function technique. The SWR frequency of the ferromagnetic thin film is shifted to higher values corresponding to those of above factors, respectively. It is found that the linear behavior of SWR frequency curves of all modes in the system is observed as the external magnetic field is increasing, however, SWR frequency curves are nonlinear with the lower and the higher modes for different surface anisotropy and interlayer exchange coupling in the system. In addition, the SWR frequency of the lowest (highest) mode is shifted to higher (lower) values when the film thickness is thinner. The interlayer exchange coupling is more important for the energetically higher modes than for the energetically lower modes. The surface anisotropy has a little effect on the SWR frequency of the highest mode, when the surface anisotropy field is further increased.

  1. Modeling of thermal spin transport and spin-orbit effects in ferromagnetic/nonmagnetic mesoscopic devices

    NARCIS (Netherlands)

    Slachter, Abraham; Bakker, Frank Lennart; van Wees, Bart Jan

    2011-01-01

    In this article we extend the currently established diffusion theory of spin-dependent electrical conduction by including spin-dependent thermoelectricity and thermal transport. Using this theory, we propose experiments aimed at demonstrating novel effects such as the spin-Peltier effect, the

  2. Ferromagnetic Order from p-Electrons in Rubidium Oxide

    NARCIS (Netherlands)

    Riyadi, Syarif; Giriyapura, Shivakumara; de Groot, Robert A.; Caretta, Antonio; van Loosdrecht, Paul H. M.; Palstra, Thomas T. M.; Blake, Graeme R.

    2011-01-01

    Magnetic dioxygen molecules can be used as building blocks of model systems to investigate spin-polarization that arises from unpaired p-electrons, the scientific potential of which is evidenced by phenomena such as spin-polarized transport in graphene. In solid elemental oxygen and all of the known

  3. An effective correlated mean-field theory applied in the spin-1/2 Ising ferromagnetic model

    Energy Technology Data Exchange (ETDEWEB)

    Roberto Viana, J.; Salmon, Octávio R. [Universidade Federal do Amazonas – UFAM, Manaus 69077-000, AM (Brazil); Ricardo de Sousa, J. [Universidade Federal do Amazonas – UFAM, Manaus 69077-000, AM (Brazil); National Institute of Science and Technology for Complex Systems, Universidade Federal do Amazonas, 3000, Japiim, 69077-000 Manaus, AM (Brazil); Neto, Minos A.; Padilha, Igor T. [Universidade Federal do Amazonas – UFAM, Manaus 69077-000, AM (Brazil)

    2014-11-15

    We developed a new treatment for mean-field theory applied in spins systems, denominated effective correlated mean-field (ECMF). We apply this theory to study the spin-1/2 Ising ferromagnetic model with nearest-neighbor interactions on a square lattice. We use clusters of finite sizes and study the criticality of the ferromagnetic system, where we obtain a convergence of critical temperature for the value k{sub B}T{sub c}/J≃2.27905±0.00141. Also the behavior of magnetic and thermodynamic properties, using the condition of minimum energy of the physical system is obtained. - Highlights: • We developed spin models to study real magnetic systems. • We study the thermodynamic and magnetic properties of the ferromagnetism. • We enhanced a mean-field theory applied in spins models.

  4. Spin-injection efficiency and magnetoresistance in a hybrid ferromagnetic-semiconductor trilayer with interfacial barriers

    International Nuclear Information System (INIS)

    Agrawal, S.; Jalil, M.B.A.; Tan, S.G.; Teo, K.L.; Liew, T.

    2006-01-01

    We present a self-consistent model of spin transport in a ferromagnetic (FM)-semiconductor (SC)-FM trilayer structure with interfacial barriers at the FM-SC boundaries. The SC layer consists of a highly doped n 2+ AlGaAs-GaAs 2DEG while the interfacial resistance is modeled as delta potential (δ) barriers. The self-consistent scheme combines a ballistic model of spin-dependent transmission across the δ-barriers, and a drift-diffusion model within the bulk of the trilayer. The interfacial resistance (R I ) values of the two junctions were found to be asymmetric despite the symmetry of the trilayer structure. Transport characteristics such as the asymmetry in R I , spin-injection efficiency and magnetoresistance (MR) are calculated as a function of bulk conductivity σ s and spin-diffusion length (SDL) within the SC layer. In general a large σ s tends to improve all three characteristics, while a long SDL improves the MR ratio but reduces the spin-injection efficiency. These trends may be explained in terms of conductivity mismatch and spin accumulation either at the interfacial zones or within the bulk of the SC layer

  5. Graphitic silicon nitride: a metal-free ferromagnet with charge and spin current rectification.

    Science.gov (United States)

    Sen, Sabyasachi; Chakrabarti, Swapan

    2014-09-15

    As a first example, herein we show that g-Si(4)N(3) is expected to act as a metal-free ferromagnet featuring both charge and spin current rectification simultaneously. Such rectification is crucial for envisioning devices that contain both logic and memory functionality on a single chip. The spin coherent quantum-transport calculations on g-Si(4)N(3) reveal that the chosen system is a unique molecular spin filter, the current-voltage characteristics of which is asymmetric in nature, which can create a perfect background for synchronous charge and spin current rectification. To shed light on this highly unusual in-silico observation, we have meticulously inspected the bias-dependent modulation of the spin-polarized eigenstates. The results indicate that, whereas only the localized 2p orbitals of the outer-ring (OR) Si atoms participate in the transmission process in the positive bias, both OR Si and N atoms contribute in the reverse bias. Furthermore, we have evaluated the spin-polarized electron-transfer rate in the tunneling regime, and the results demonstrate that the transfer rates are unequal in the positive and negative bias range, leading to the possible realization of a simultaneous logic-memory device. © 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  6. Topological Hall effect in diffusive ferromagnetic thin films with spin-flip scattering

    Science.gov (United States)

    Zhang, Steven S.-L.; Heinonen, Olle

    2018-04-01

    We study the topological Hall (TH) effect in a diffusive ferromagnetic metal thin film by solving a Boltzmann transport equation in the presence of spin-flip scattering. A generalized spin-diffusion equation is derived which contains an additional source term associated with the gradient of the emergent magnetic field that arises from skyrmions. Because of the source term, spin accumulation may build up in the vicinity of the skyrmions. This gives rise to a spin-polarized diffusion current that in general suppresses the bulk TH current. Only when the spin-diffusion length is much smaller than the skyrmion size does the TH resistivity approach the value derived by Bruno et al. [Phys. Rev. Lett. 93, 096806 (2004), 10.1103/PhysRevLett.93.096806]. We derive a general expression of the TH resistivity that applies to thin-film geometries with spin-flip scattering, and show that the corrections to the TH resistivity become large when the size of room temperature skyrmions is further reduced to tens of nanometers.

  7. Real-space imaging of non-collinear antiferromagnetic order with a single-spin magnetometer

    Science.gov (United States)

    Gross, I.; Akhtar, W.; Garcia, V.; Martínez, L. J.; Chouaieb, S.; Garcia, K.; Carrétéro, C.; Barthélémy, A.; Appel, P.; Maletinsky, P.; Kim, J.-V.; Chauleau, J. Y.; Jaouen, N.; Viret, M.; Bibes, M.; Fusil, S.; Jacques, V.

    2017-09-01

    Although ferromagnets have many applications, their large magnetization and the resulting energy cost for switching magnetic moments bring into question their suitability for reliable low-power spintronic devices. Non-collinear antiferromagnetic systems do not suffer from this problem, and often have extra functionalities: non-collinear spin order may break space-inversion symmetry and thus allow electric-field control of magnetism, or may produce emergent spin-orbit effects that enable efficient spin-charge interconversion. To harness these traits for next-generation spintronics, the nanoscale control and imaging capabilities that are now routine for ferromagnets must be developed for antiferromagnetic systems. Here, using a non-invasive, scanning single-spin magnetometer based on a nitrogen-vacancy defect in diamond, we demonstrate real-space visualization of non-collinear antiferromagnetic order in a magnetic thin film at room temperature. We image the spin cycloid of a multiferroic bismuth ferrite (BiFeO3) thin film and extract a period of about 70 nanometres, consistent with values determined by macroscopic diffraction. In addition, we take advantage of the magnetoelectric coupling present in BiFeO3 to manipulate the cycloid propagation direction by an electric field. Besides highlighting the potential of nitrogen-vacancy magnetometry for imaging complex antiferromagnetic orders at the nanoscale, these results demonstrate how BiFeO3 can be used in the design of reconfigurable nanoscale spin textures.

  8. Anomalous spin distribution in the superconducting ferromagnet UCoGe studied by polarized neutron diffraction

    OpenAIRE

    Prokes, K.; de Visser, A.; Huang, Y. K.; Fak, B.; Ressouche, E.

    2010-01-01

    We report a polarized neutron diffraction study conducted to reveal the nature of the weak ferromagnetic moment in the superconducting ferromagnet UCoGe. We find that the ordered moment in the normal phase in low magnetic fields (B // c) is predominantly located at the U atom and has a magnitude of about 0.1 muB at 3 T, in agreement with bulk magnetization data. By increasing the magnetic field the U moment grows to about 0.3 muB in 12 T and most remarkably, induces a substantial moment (abou...

  9. Spin dependent tunneling through a quantum dot attached to ferromagnetic electrodes with non-collinear magnetizations

    International Nuclear Information System (INIS)

    Wawrzyniak, M.; Gmitra, M.; Barnas, J.

    2006-01-01

    Resonant tunneling through an interacting single-level quantum dot, coupled to ferromagnetic electrodes with non-collinear magnetizations has been analyzed theoretically. The dot is additionally subject to an external magnetic field. The non-equilibrium Green function technique and the equation of motion method have been applied to calculate electric current, tunnel magnetoresistance, and the average spin components in the dot. The relevant Green functions have been calculated in the Hartree-Fock approximation, and the calculations are restricted to the weak coupling regime. Numerical results are presented for a dot which is empty at equilibrium, but can be singly or doubly occupied when a bias voltage is applied

  10. Antenna design for propagating spin wave spectroscopy in ferromagnetic thin films

    Science.gov (United States)

    Zhang, Yan; Yu, Ting; Chen, Ji-lei; Zhang, You-guang; Feng, Jian; Tu, Sa; Yu, Haiming

    2018-03-01

    In this paper, we investigate the characteristics of antenna for propagating-spin-wave-spectroscopy (PSWS) experiment in ferromagnetic thin films. Firstly, we simulate the amplitude and phase distribution of the high-frequency magnetic field around antenna by high frequency structure simulator (HFSS). And then k distribution of the antenna is obtained by fast Fourier transformation (FFT). Furthermore, three kinds of antenna designs, i.e. micro-strip line, coplanar waveguide (CPW), loop, are studied and compared. How the dimension parameter of antenna influence the corresponding high-frequency magnetic field amplitude and k distribution are investigated in details.

  11. Dimensionality effects on spin-polarized quantum beats in ferromagnetic hosts with a pair of side-coupled impurities

    Energy Technology Data Exchange (ETDEWEB)

    Guessi, L.H.; Leandro, S.C.; Seridonio, A.C.; Siqueira, E.C. [Universidade Estadual Paulista Julio de Mesquita Filho (UNESP), Ilha Solteira, SP (Brazil). Dept. de Fisico Quimica; Souza, F.M.; Vernek, E. [Universidade Federal de Uberlandia (UFU), MG (Brazil). Inst. de Fisica; Yoshida, M. [Universidade Estadual Paulista Julio de Mesquita Filho (UNESP), Rio Claro, SP (Brazil); Figueira, M.S. [Universidade Federal Fluminense (UFF), Niteroi, RJ (Brazil). Inst. de Fisica

    2012-07-01

    Full text: In this work, we report a theoretical description of the differential conductance in the low bias regime, for a normal scanning tunneling microscope (STM) probe in the presence of ferromagnetic (FM) hosts with impurities. The hosts are treated as a spin-polarized electron gas hybridized to a pair of side-coupled impurities. Two setups of different dimensionalities are considered, a quantum wire (QW) and a metallic surface (MS). In order to deal with the non-interacting and the Coulomb blockade regimes of these systems, the analysis is done in the framework of the two-impurity Anderson model (TIAM) in combination with the equation of motion (EOM) approach for the Hamiltonian Green functions (GFs). The Fano effect appears in such setups, due to the quantum interference between the transport channels composed by the spin-polarized conduction bands and the electron tunneling into (or out of) the impurities. Thus the conductance of the STM reveals as a function of the probe position, a Fano interference strong dependent on the host dimensionality. It leads to the emergence of spin-polarized quantum beats in the Friedel oscillations for the conductance signal, which are uniform in the QW system in opposite to those found in the MS case, characterized by a long-range damped behavior. We remark that, the energy levels of the impurities and the Coulomb repulsion, modulate these beats. As a result, they establish a scenario where the interplay between the Coulomb blockade and the ferromagnetism of a metallic environment, can be useful for future quantum computation devices. (author)

  12. Perfect switching of the spin polarization in a ferromagnetic gapless graphene/superconducting gapped graphene junction

    International Nuclear Information System (INIS)

    Soodchomshom, Bumned; Tang, I-Ming; Hoonsawat, Rassmidara

    2010-01-01

    With the fabrication of gapped graphene, interest in the tunneling spectroscopy in graphene-based FG/SG junctions in which one side consists of a gapless ferro-magnetic graphene (FG) and the other side, of a gapped superconducting graphene (SG) has arisen. The carriers in the gapless (gapped) graphene are 2D relativistic particles having an energy spectrum given by E=√(h 2 v F 2 k 2 +(mv F 2 ) 2 ) (where mv F 2 is the gap and v F is the Fermi velocity). The spin currents in this FG/SG junction are obtained within the framework of the extended Blonder-Tinkham-Klapwijk (BTK) formalism. The effects of the superconducting energy gap in SG, of the gap mv F 2 which opened in the superconducting graphene, of the exchange field in FG, of the spin-dependent specular Andreev reflection, of the effective Fermi energy (E FF ) of FG and of the bias voltage across the junction (V) are simulated. It is seen that by adjusting E FF or V, the spin polarization (defined as SP(%) = 100% x (G ↑ - G ↓ )/(G ↑ + G ↓ )) can be switched from a pure spin up (SP = +100%) state to pure spin down (SP = -100%) state.

  13. Spin and Isospin: Exotic Order in Quantum Hall Ferromagnets

    Science.gov (United States)

    Girvin, Steven M.

    Quantum mechanics is a strange business, and the quantum physics of strongly correlated many-electron systems can be stranger still. Good examples are the various quantum Hall effects. They are among the most remarkable many-body quantum phenomena discovered in the second half of the 20th century, comparable in intellectual import to superconductivity and superfluidity. The quantum Hall effects are an extremely rich set of phenomena with deep and truly fundamental theoretical implications...

  14. Ferromagnetic HfO2/Si/GaAs interface for spin-polarimetry applications

    Science.gov (United States)

    Tereshchenko, O. E.; Golyashov, V. A.; Eremeev, S. V.; Maurin, I.; Bakulin, A. V.; Kulkova, S. E.; Aksenov, M. S.; Preobrazhenskii, V. V.; Putyato, M. A.; Semyagin, B. R.; Dmitriev, D. V.; Toropov, A. I.; Gutakovskii, A. K.; Khandarkhaeva, S. E.; Prosvirin, I. P.; Kalinkin, A. V.; Bukhtiyarov, V. I.; Latyshev, A. V.

    2015-09-01

    In this letter, we present electrical and magnetic characteristics of HfO2-based metal-oxide-semiconductor capacitors (MOSCAPs), along with the effect of pseudomorphic Si as a passivating interlayer on GaAs(001) grown by molecular beam epitaxy. Ultrathin HfO2 high-k gate dielectric films (3-15 nm) have been grown on Si/GaAs(001) structures through evaporation of a Hf/HfO2 target in NO2 gas. The lowest interface states density Dit at Au/HfO2/Si/GaAs(001) MOS-structures were obtained in the range of (6 -13 )×1011 eV-1 cm-2 after annealing in the 400-500 °C temperature range as a result of HfO2 crystallization and the Si layer preservation in non-oxidized state on GaAs. HfO2-based MOSCAPs demonstrated the ferromagnetic properties which were attributed to the presence of both cation and anion vacancies according to the first-principle calculations. Room-temperature ferromagnetism in HfO2 films allowed us to propose a structure for the ferromagnetic MOS spin-detector.

  15. Spin-orbit driven ferromagnetic resonance: a nanoscale magnetic characterisation technique

    Czech Academy of Sciences Publication Activity Database

    Fang, D.; Kurebayashi, H.; Wunderlich, Joerg; Výborný, Karel; Zarbo, Liviu; Campion, R. P.; Casiraghi, A.; Gallagher, B. L.; Jungwirth, Tomáš; Ferguson, A.J.

    2011-01-01

    Roč. 6, č. 7 (2011), s. 413-417 ISSN 1748-3387 R&D Projects: GA AV ČR KAN400100652; GA MŠk LC510; GA AV ČR KJB100100802; GA MŠk(CZ) 7E08087 EU Projects: European Commission(XE) 214499 - NAMASTE; European Commission(XE) 215368 - SemiSpinNet Grant - others:AV ČR(CZ) AP0801 Program:Akademická prémie - Praemium Academiae Institutional research plan: CEZ:AV0Z10100521 Keywords : ferromagnetic resonance * spin-orbit coupling * nanomagnets Subject RIV: BM - Solid Matter Physics ; Magnet ism Impact factor: 27.270, year: 2011

  16. High-Density Physical Random Number Generator Using Spin Signals in Multidomain Ferromagnetic Layer

    Directory of Open Access Journals (Sweden)

    Sungwoo Chun

    2015-01-01

    Full Text Available A high-density random number generator (RNG based on spin signals in a multidomain ferromagnetic layer in a magnetic tunnel junction (MTJ is proposed and fabricated. Unlike conventional spin-based RNGs, the proposed method does not require one to control an applied current, leading to a time delay in the system. RNG demonstrations are performed at room temperature. The randomness of the bit sequences generated by the proposed RNG is verified using the FIPS 140-2 statistical test suite provided by the NIST. The test results validate the effectiveness of the proposed RNGs. Our results suggest that we can obtain high-density, ultrafast RNGs if we can achieve high integration on the chip.

  17. Soliton instabilities in the easy plane ferromagnet Heisenberg chain with out-of-plane spin deviation

    Energy Technology Data Exchange (ETDEWEB)

    Pozo, J.; Leon, A. [Instituto de Ciencias Basicas, Facultad de Ingenieria, Universidad Diego Portales, Casilla 298-V, Santiago (Chile)]. e-mail: julio.pozo@udp.cl

    2006-07-01

    In this paper we investigate the presence of out-of-plane spin deviation {rho}({xi}) in the easy-plane ferromagnetic Heisenberg chain by using the coupled-boson operators together with the Schwinger transformation for the spin operator; this method allows us to conclude that the critical behaviour of the instability is due to the velocity of the nonlinear excitations (solitons) only for an appropriate range of the magnetic field. In this case, when the velocity becomes lower, the stable soliton corresponding to {rho}({xi}) is distorted by magnons and loses stability. If we increase the velocity of {rho}({xi}), it then decays into high frequency-oscillations. Nevertheless, we find an opposite competence effect produced by the velocity and the magnetic field on {rho}({xi}). (Author)

  18. Spin-wave mode profiles versus surface/interface conditions in ferromagnetic Fe/Ni layered composites

    CERN Document Server

    Krawczyk, M; Levy, J C S; Mercier, D

    2003-01-01

    Spin-wave excitations in ferromagnetic layered composite (AB centre dot centre dot centre dot BA; A and B being different homogeneous ferromagnetic materials) are analysed theoretically, by means of the transfer matrix approach. The properties of multilayer spin-wave mode profiles are discussed in relation to multilayer characteristics, such as the filling fraction and the exchange or magnetization contrast; also, surface spin pinning conditions and dipolar interactions are taken into account. The interface conditions are satisfied by introducing an effective exchange field expressed by interface gradients of the exchange constant and the magnetization. This approach provides an easy way to find frequencies and amplitudes of standing spin waves in the multilayer. The developed theory is applied to interpretation of spin wave resonance (SWR) spectra obtained experimentally by Chambers et al in two systems: a bilayer Fe/Ni and a trilayer Ni/Fe/Ni, in perpendicular (to the multilayer surface) configuration of th...

  19. Spin-exchange interaction between transition metals and metalloids in soft-ferromagnetic metallic glasses

    Science.gov (United States)

    Das, Santanu; Choudhary, Kamal; Chernatynskiy, Aleksandr; Choi Yim, Haein; Bandyopadhyay, Asis K.; Mukherjee, Sundeep

    2016-06-01

    High-performance magnetic materials have immense industrial and scientific importance in wide-ranging electronic, electromechanical, and medical device technologies. Metallic glasses with a fully amorphous structure are particularly suited for advanced soft-magnetic applications. However, fundamental scientific understanding is lacking for the spin-exchange interaction between metal and metalloid atoms, which typically constitute a metallic glass. Using an integrated experimental and molecular dynamics approach, we demonstrate the mechanism of electron interaction between transition metals and metalloids. Spin-exchange interactions were investigated for a Fe-Co metallic glass system of composition [(Co1-x Fe x )0.75B0.2Si0.05]96Cr4. The saturation magnetization increased with higher Fe concentration, but the trend significantly deviated from simple rule of mixtures. Ab initio molecular dynamics simulation was used to identify the ferromagnetic/anti-ferromagnetic interaction between the transition metals and metalloids. The overlapping band-structure and density of states represent ‘Stoner type’ magnetization for the amorphous alloys in contrast to ‘Heisenberg type’ in crystalline iron. The enhancement of magnetization by increasing iron was attributed to the interaction between Fe 3d and B 2p bands, which was further validated by valence-band study.

  20. Two-dimensional ferromagnet/semiconductor transition metal dichalcogenide contacts: p-type Schottky barrier and spin-injection control

    KAUST Repository

    Gan, Liyong

    2013-09-26

    We study the ferromagnet/semiconductor contacts formed by transition metal dichalcogenide monolayers, focusing on semiconducting MoS2 and WS2 and ferromagnetic VS2. We investigate the degree of p-type doping and demonstrate tuning of the Schottky barrier height by vertical compressive pressure. An analytical model is presented for the barrier heights that accurately describes the numerical findings and is expected to be of general validity for all transition metal dichalcogenide metal/semiconductor contacts. Furthermore, magnetic proximity effects induce a 100% spin polarization at the Fermi level in the semiconductor where the spin splitting increases up to 0.70 eV for increasing pressure.

  1. Evidence for the ferromagnetic frustration in a classical spin- 1 / 2 system with multisite interaction in external magnetic field: Exact results

    Science.gov (United States)

    Jurčišinová, E.; Jurčišin, M.

    2017-11-01

    We investigate the influence of the multisite interaction among sites within elementary triangles of the kagome-like recursive lattice on the properties of the classical spin- 1 / 2 ferromagnetic Ising model in the external magnetic field. The exact solution of the model is found and it is shown that the model exhibits a nontrivial structure of the first order as well as second order phase transitions in nonzero external magnetic fields related to the multisite interaction. The equation for the exact determination of the positions of the critical points of the second order phase transitions is derived. The thermodynamic properties of the model are investigated in detail and it is shown that the competition between the ferromagnetic interaction and the multisite interaction leads to the appearance of strong ferromagnetic frustration effects represented by the formation of a nontrivial system of macroscopically degenerated plateau-like and single-point-like ground states. The residual entropies of all ground states are found and the kagome spin-ice-like highly macroscopically degenerated plateau state with nonzero magnetization is identified with the exact residual entropy per site s /kB = ln(4 / 3) / 3 ≈ 0 . 095894. The properties of the specific heat are investigated, its Schottky-type behavior near the single-point ground state values of the magnetic field is identified, the existence of large magnetocaloric effect is discussed, and the existence of the first order phase transitions without the specific heat capacity change is demonstrated.

  2. Complex magnetic order in the kagome ferromagnet Pr3Ru4Al12

    Science.gov (United States)

    Henriques, M. S.; Gorbunov, D. I.; Andreev, A. V.; Fabrèges, X.; Gukasov, A.; Uhlarz, M.; Petříček, V.; Ouladdiaf, B.; Wosnitza, J.

    2018-01-01

    In the hexagonal crystal structure of Pr3Ru4Al12 , the Pr atoms form a distorted kagome lattice, and their magnetic moments, are subject to competing exchange and anisotropy interactions. We performed magnetization, magnetic-susceptibility, specific-heat, electrical-resistivity, and neutron-scattering measurements. Pr3Ru4Al12 is a uniaxial ferromagnet with TC=39 K that displays a collinear magnetic structure (in the high-temperature range of the magnetically ordered state) for which the only crystallographic position of Pr is split into two sites carrying different magnetic moments. A spin-reorientation phase transition is found at 7 K. Below this temperature, part of the Pr moments rotate towards the basal plane, resulting in a noncollinear magnetic state with a lower magnetic symmetry. We argue that unequal RKKY exchange interactions competing with the crystal electric field lead to a moment instability and qualitatively explain the observed magnetic phases in Pr3Ru4Al12 .

  3. Effect of ferromagnetic exchange field on band gap and spin polarisation of graphene on a TMD substrate

    Science.gov (United States)

    Goswami, Partha

    2018-03-01

    We calculate the electronic band dispersion of graphene monolayer on a two-dimensional transition metal dichalcogenide substrate (GrTMD) around K and K^' } points by taking into account the interplay of the ferromagnetic impurities and the substrate-induced interactions. The latter are (strongly enhanced) intrinsic spin-orbit interaction (SOI), the extrinsic Rashba spin-orbit interaction (RSOI) and the one related to the transfer of the electronic charge from graphene to substrate. We introduce exchange field ( M) in the Hamiltonian to take into account the deposition of magnetic impurities on the graphene surface. The cavalcade of the perturbations yield particle-hole symmetric band dispersion with an effective Zeeman field due to the interplay of the substrate-induced interactions with RSOI as the prime player. Our graphical analysis with extremely low-lying states strongly suggests the following: The GrTMDs, such as graphene on WY2, exhibit (direct) band-gap narrowing / widening (Moss-Burstein (MB) gap shift) including the increase in spin polarisation ( P) at low temperature due to the increase in the exchange field ( M) at the Dirac points. The polarisation is found to be electric field tunable as well. Finally, there is anticrossing of non-parabolic bands with opposite spins, the gap closing with same spins, etc. around the Dirac points. A direct electric field control of magnetism at the nanoscale is needed here. The magnetic multiferroics, like BiFeO3 (BFO), are useful for this purpose due to the coupling between the magnetic and electric order parameters.

  4. Short-range order above the Curie temperature in the dynamic spin-fluctuation theory

    International Nuclear Information System (INIS)

    Melnikov, N.B.; Reser, B.I.

    2016-01-01

    Based on the dynamic spin-fluctuation theory, we study the spin-density correlations in the ferromagnetic metals. We obtain computational formulae for the correlation function and correlation radius in different approximations of the theory. Using these formulae, we calculate the magnetic short-range order above the Curie temperature in bcc Fe. Results of the calculation confirm our theoretical prediction that the inverse correlation radius increases linearly with temperature for T sufficiently large. The calculated short-range order is small but sufficient to correctly describe neutron scattering experiments. A considerable amount of the short-range order is shown to persist up to temperatures much higher than the Curie temperature. - Highlights: • We study the spin correlations in ferromagnetic metals above the Curie temperature. • We derive computational formulae for the spin correlator and correlation radius. • The correlation radius decreases inversely with temperature over a wide interval. • The calculated short-range order in Fe is small, in agreement with experiment. • A considerable amount of short-range order in Fe persists up to high temperatures.

  5. Dissipative environment may improve the quantum annealing performances of the ferromagnetic p -spin model

    Science.gov (United States)

    Passarelli, G.; De Filippis, G.; Cataudella, V.; Lucignano, P.

    2018-02-01

    We investigate the quantum annealing of the ferromagnetic p -spin model in a dissipative environment (p =5 and p =7 ). This model, in the large-p limit, codifies Grover's algorithm for searching in an unsorted database [L. K. Grover, Proceedings of the 28th Annual ACM Symposium on Theory of Computing (ACM, New York, 1996), pp. 212-219]. The dissipative environment is described by a phonon bath in thermal equilibrium at finite temperature. The dynamics is studied in the framework of a Lindblad master equation for the reduced density matrix describing only the spins. Exploiting the symmetries of our model Hamiltonian, we can describe many spins and extrapolate expected trends for large N and p . While at weak system-bath coupling the dissipative environment has detrimental effects on the annealing results, we show that in the intermediate-coupling regime, the phonon bath seems to speed up the annealing at low temperatures. This improvement in the performance is likely not due to thermal fluctuation but rather arises from a correlated spin-bath state and persists even at zero temperature. This result may pave the way to a new scenario in which, by appropriately engineering the system-bath coupling, one may optimize quantum annealing performances below either the purely quantum or the classical limit.

  6. Simulation study of ballistic spin-MOSFET devices with ferromagnetic channels based on some Heusler and oxide compounds

    Science.gov (United States)

    Graziosi, Patrizio; Neophytou, Neophytos

    2018-02-01

    Newly emerged materials from the family of Heuslers and complex oxides exhibit finite bandgaps and ferromagnetic behavior with Curie temperatures much higher than even room temperature. In this work, using the semiclassical top-of-the-barrier FET model, we explore the operation of a spin-MOSFET that utilizes such ferromagnetic semiconductors as channel materials, in addition to ferromagnetic source/drain contacts. Such a device could retain the spin polarization of injected electrons in the channel, the loss of which limits the operation of traditional spin transistors with non-ferromagnetic channels. We examine the operation of four material systems that are currently considered some of the most prominent known ferromagnetic semiconductors: three Heusler-type alloys (Mn2CoAl, CrVZrAl, and CoVZrAl) and one from the oxide family (NiFe2O4). We describe their band structures by using data from DFT (Density Functional Theory) calculations. We investigate under which conditions high spin polarization and significant ION/IOFF ratio, two essential requirements for the spin-MOSFET operation, are both achieved. We show that these particular Heusler channels, in their bulk form, do not have adequate bandgap to provide high ION/IOFF ratios and have small magnetoconductance compared to state-of-the-art devices. However, with confinement into ultra-narrow sizes down to a few nanometers, and by engineering their spin dependent contact resistances, they could prove promising channel materials for the realization of spin-MOSFET transistor devices that offer combined logic and memory functionalities. Although the main compounds of interest in this paper are Mn2CoAl, CrVZrAl, CoVZrAl, and NiFe2O4 alone, we expect that the insight we provide is relevant to other classes of such materials as well.

  7. High-field magnetic circular dichroism in ferromagnetic InMnSb and InMnAs: Spin-orbit-split hole bands and g factors

    Science.gov (United States)

    Meeker, M. A.; Magill, B. A.; Khodaparast, G. A.; Saha, D.; Stanton, C. J.; McGill, S.; Wessels, B. W.

    2015-09-01

    Carrier-induced ferromagnetism in magnetic III-V semiconductors has opened up several opportunities for spintronic device applications as well as for fundamental studies of a material system in which itinerant carriers interact with the localized spins of magnetic impurities. In order to understand the hole mediated ferromagnetism, probing the band structure in these material systems is crucial. Here we present magnetic circular dichroism (MCD) studies on MOVPE grown InMnSb and InMnAs, both with the Curie temperatures above 300 K. The measurements were performed on samples with different Mn contents with the excitation energy tuned from 0.92-1.42 eV and external magnetic fields up to 31 T. The large g factors in these systems allow us to measure the MCD at relatively high temperatures (190 K). These measurements are compared with MCD calculations based on an eight-band Pidgeon-Brown model, which is generalized to include the coupling between the electron/hole and the Mn spin in a ferromagnetic state. Comparison of the observed MCD with the theoretical calculations provides a direct method to probe the band structure including the temperature dependence of the spin-orbit split-off gap and g factors, and to estimate the s p -d coupling constants.

  8. Competing Spin Liquids and Hidden Spin-Nematic Order in Spin Ice with Frustrated Transverse Exchange

    Directory of Open Access Journals (Sweden)

    Mathieu Taillefumier

    2017-12-01

    Full Text Available Frustration in magnetic interactions can give rise to disordered ground states with subtle and beautiful properties. The spin ices Ho_{2}Ti_{2}O_{7} and Dy_{2}Ti_{2}O_{7} exemplify this phenomenon, displaying a classical spin-liquid state, with fractionalized magnetic-monopole excitations. Recently, there has been great interest in closely related “quantum spin-ice” materials, following the realization that anisotropic exchange interactions could convert spin ice into a massively entangled, quantum spin liquid, where magnetic monopoles become the charges of an emergent quantum electrodynamics. Here we show that even the simplest model of a quantum spin ice, the XXZ model on the pyrochlore lattice, can realize a still-richer scenario. Using a combination of classical Monte Carlo simulation, semiclassical molecular-dynamics simulation, and analytic field theory, we explore the properties of this model for frustrated transverse exchange. We find not one, but three competing forms of spin liquid, as well as a phase with hidden, spin-nematic order. We explore the experimental signatures of each of these different states, making explicit predictions for inelastic neutron scattering. These results show an intriguing similarity to experiments on a range of pyrochlore oxides.

  9. Competing Spin Liquids and Hidden Spin-Nematic Order in Spin Ice with Frustrated Transverse Exchange

    Science.gov (United States)

    Taillefumier, Mathieu; Benton, Owen; Yan, Han; Jaubert, L. D. C.; Shannon, Nic

    2017-10-01

    Frustration in magnetic interactions can give rise to disordered ground states with subtle and beautiful properties. The spin ices Ho2 Ti2 O7 and Dy2 Ti2 O7 exemplify this phenomenon, displaying a classical spin-liquid state, with fractionalized magnetic-monopole excitations. Recently, there has been great interest in closely related "quantum spin-ice" materials, following the realization that anisotropic exchange interactions could convert spin ice into a massively entangled, quantum spin liquid, where magnetic monopoles become the charges of an emergent quantum electrodynamics. Here we show that even the simplest model of a quantum spin ice, the XXZ model on the pyrochlore lattice, can realize a still-richer scenario. Using a combination of classical Monte Carlo simulation, semiclassical molecular-dynamics simulation, and analytic field theory, we explore the properties of this model for frustrated transverse exchange. We find not one, but three competing forms of spin liquid, as well as a phase with hidden, spin-nematic order. We explore the experimental signatures of each of these different states, making explicit predictions for inelastic neutron scattering. These results show an intriguing similarity to experiments on a range of pyrochlore oxides.

  10. Polar-core spin vortex of quasi-2D ferromagnetic spin-1 condensate in a flat-bottomed optical trap with a weak magnetic field

    Science.gov (United States)

    Zheng, Gong-Ping; Li, Pin; Li, Ting; Xue, Ya-Jie

    2018-02-01

    Motivated by the recent experiments realized in a flat-bottomed optical trap (Navon et al., 2015; Chomaz et al., 2015), we study the ground state of polar-core spin vortex of quasi-2D ferromagnetic spin-1 condensate in a finite-size homogeneous trap with a weak magnetic field. The exact spatial distribution of local spin is obtained with a variational method. Unlike the fully-magnetized planar spin texture with a zero-spin core, which was schematically demonstrated in previous studies for the ideal polar-core spin vortex in a homogeneous trap with infinitely large boundary, some plateaus and two-cores structure emerge in the distribution curves of spin magnitude in the polar-core spin vortex we obtained for the larger effective spin-dependent interaction. More importantly, the spin values of the plateaus are not 1 as expected in the fully-magnetized spin texture, except for the sufficiently large spin-dependent interaction and the weak-magnetic-field limit. We attribute the decrease of spin value to the effect of finite size of the system. The spin values of the plateaus can be controlled by the quadratic Zeeman energy q of the weak magnetic field, which decreases with the increase of q.

  11. Thermoelectric properties of a ferromagnet-superconductor hybrid junction: Role of interfacial Rashba spin-orbit interaction

    Science.gov (United States)

    Dutta, Paramita; Saha, Arijit; Jayannavar, A. M.

    2017-09-01

    We investigate thermoelectric properties of a ferromagnet-superconductor hybrid structure with Rashba spin-orbit interaction and delta function potential barrier at the interfacial layer. The exponential rise of thermal conductance with temperature manifests a crossover temperature scale separating two opposite behaviors of it with the change of polarization in the ferromagnet whereas the inclusion of an interfacial Rashba spin-orbit field results in a nonmonotonic behavior of it with the strength of the Rashba field. We employ scattering matrix approach to determine the amplitudes of all the scattering processes possible at the interface to explain the thermoelectric properties of the device. We examine Seebeck effect and show that higher thermopower can be achieved when the polarization of the ferromagnet tends towards the half-metallic limit. It can be enhanced even for lower polarization in the presence of the finite potential barrier. In the presence of interfacial Rashba spin-orbit interaction, the Seebeck coefficient rises with the increase of barrier strength and polarization at weak or moderate interfacial Rashba field. From the application perspective, we compute the figure of merit and show that z T ˜4 -5 with higher polarization of the ferromagnet both in absence and presence of weak or moderate Rashba spin-orbit interaction along with the scalar potential barrier.

  12. Renormalization of Long Wavelength Spin Waves in the 2d Ferromagnet Rb2CrCl4

    DEFF Research Database (Denmark)

    Lindgård, Per-Anker; Als-Nielsen, Jens Aage; Hutchings, M. T.

    1980-01-01

    Rb2CrCl4 is a nearly 2d-ferromagnetic, optically transparent insulator isomorphous with K2CuF4. High resolution neutron scattering data for temperatures below Tc = 52.4 K of the low energy long wavelength spin waves are presented and a Hartree-Fock analysis yields Hamiltonian parameters...

  13. Spin-memory loss due to spin-orbit coupling at ferromagnet/heavy-metal interfaces: Ab initio spin-density matrix approach

    Science.gov (United States)

    Dolui, Kapildeb; Nikolić, Branislav K.

    2017-12-01

    Spin-memory loss (SML) of electrons traversing ferromagnetic-metal/heavy-metal (FM/HM), FM/normal-metal (FM/NM), and HM/NM interfaces is a fundamental phenomenon that must be invoked to explain consistently large numbers of spintronic experiments. However, its strength extracted by fitting experimental data to phenomenological semiclassical theory, which replaces each interface by a fictitious bulk diffusive layer, is poorly understood from a microscopic quantum framework and/or materials properties. Here we describe an ensemble of flowing spin quantum states using spin-density matrix, so that SML is measured like any decoherence process by the decay of its off-diagonal elements or, equivalently, by the reduction of the magnitude of polarization vector. By combining this framework with density functional theory, we examine how all three components of the polarization vector change at Co/Ta, Co/Pt, Co/Cu, Pt/Cu, and Pt/Au interfaces embedded within Cu/FM/HM/Cu vertical heterostructures. In addition, we use ab initio Green's functions to compute spectral functions and spin textures over FM, HM, and NM monolayers around these interfaces which quantify interfacial spin-orbit coupling and explain the microscopic origin of SML in long-standing puzzles, such as why it is nonzero at the Co/Cu interface; why it is very large at the Pt/Cu interface; and why it occurs even in the absence of disorder, intermixing and magnons at the interface.

  14. Nonlinear spin fluctuations in the Fermi liquid of itinerant electron ferromagnets

    International Nuclear Information System (INIS)

    Solontsov, A.; Lacroix, C.

    2003-01-01

    A microscopic derivation of nonlinear equations of magnetic dynamics for itinerant ferromagnets is presented within the electron Fermi liquid model accounting for both long-range Coulomb and short-range interactions of quasiparticles, which founds the basis for the phenomenological description of nonlinear spin fluctuations (SF) using the Ginsburg-Landau formalism. Crystal lattice is shown to play a significant role screening the long-range Coulomb interaction and affecting magnetic dynamics. The spectrum of longitudinal SF with account of nonlinear mode-mode coupling is shown to result from an interplay of quasielastic SF and inelastic excitations near the magnon frequencies, both having mainly the nonlinear nature and arising due to their emission (absorption) by magnons

  15. Transport Through a Precessing Spin Coupled to Noncollinearly Polarized Ferromagnetic Leads

    International Nuclear Information System (INIS)

    Wang Xianchao; Xin Zihua; Feng Liya

    2010-01-01

    The quantum electronic transport through a precessing magnetic spin coupled to noncollinearly polarized ferromagnetic leads (F-MS-F) has been studied in this paper. The nonequilibrium Green function approach is used to calculate local density of states (LDOS) and current in the presence of external bias. The characters of LDOS and the electronic current are obtained. The tunneling current is investigated for different precessing angle and different configurations of the magnetization of the leads. The investigation reveals that when the precessing angle takes θ < π/2 and negative bias is applied, the resonant tunneling current appears, otherwise, it appears when positive bias is applied. When the leads are totally polarized and the precessing angel takes 0, the tunneling current changes with the configuration of two leads; and it becomes zero when the two leads are antiparallel. (condensed matter: electronic structure, electrical, magnetic, and optical properties)

  16. Monte Carlo simulations of core/shell nanoparticles containing interfacial defects: Role of disordered ferromagnetic spins

    International Nuclear Information System (INIS)

    Ho, Le Bin; Lan, Tran Nguyen; Hai, Tran Hoang

    2013-01-01

    In this work, we have used the Monte Carlo simulation to investigate the magnetic properties of an isolated composite magnetic nanoparticle with ferromagnetic (FM) core and antiferromagnetic (AFM) shell morphology. The defects were assumed to be randomly located at the AFM interface. The Néel anisotropy was used for the FM interface spins at where there are the lacks of crystal symmetry due to the vacancies at AFM interface. With a moderate defect concentration, the coercive field non-monotonously depends on the Néel anisotropy. We have examined the dependence of coercivity, exchange bias field, and vertical shift on defect concentration. We found that in addition to AFM shell, the disordered FM interface is another pining-source for exchange bias phenomenon. We discuss our simulated results in the relation to recent experimental findings

  17. Beyond Gaussian approximation in the spin-fluctuation theory of metallic ferromagnetism

    Energy Technology Data Exchange (ETDEWEB)

    Reser, B I; Grebennikov, V I [Institute of Metal Physics, Russian Academy of Sciences, Ekaterinburg (Russian Federation); Melnikov, N B, E-mail: reser@imp.uran.r [Lomonosov Moscow State University, Moscow (Russian Federation)

    2010-01-15

    A characteristic feature of the Gaussian spin-fluctuation theory is the jump transition into the paramagnetic state. We eliminate the jump and obtain a continuous second-order phase transition by taking into account the high-order terms of the free energy of electrons in the fluctuating exchange field. The third-order term of the free energy yields a renormalization of the mean field, and fourth-order term, responsible for the interaction of the fluctuations, gives a renormalization of the spin susceptibility. The extended theory is applied to the calculation of magnetic properties of Fe-Ni Invar.

  18. Systematic study of the spin stiffness dependence on phosphorus alloying in the ferromagnetic semiconductor (Ga,Mn)As

    International Nuclear Information System (INIS)

    Shihab, S.; Thevenard, L.; Bardeleben, H. J. von; Gourdon, C.; Riahi, H.; Lemaître, A.

    2015-01-01

    We study the dependence of the spin stiffness constant on the phosphorus concentration in the ferromagnetic semiconductor (Ga,Mn)(As,P) with the aim of determining whether alloying with phosphorus is detrimental, neutral, or advantageous to the spin stiffness. Time-resolved magneto-optical experiments are carried out in thin epilayers. Laser pulses excite two perpendicular standing spin wave modes, which are exchange related. We show that the first mode is spatially uniform across the layer corresponding to a k≈0 wavevector. From the two frequencies and k-vector spacings we obtain the spin stiffness constant for different phosphorus concentrations using weak surface pinning conditions. The mode assessment is checked by comparison to the spin stiffness obtained from domain pattern analysis for samples with out-of-plane magnetization. The spin stiffness is found to exhibit little variation with phosphorus concentration in contradiction with ab-initio predictions

  19. Spin correlations and magnetic order in Co-Ga alloys: A comprehensive study

    Energy Technology Data Exchange (ETDEWEB)

    Yasin, Sk Mohammad [Department of Physics, Indian Institute of Technology Madras, Chennai 600 036 (India); Saha, Ritwik [Department of Condensed Matter Physics and Materials Science, TIFR, Colaba, Mumbai 400 005 (India); Srinivas, V., E-mail: veeturi@iitm.ac.in [Department of Physics, Indian Institute of Technology Madras, Chennai 600 036 (India); Kasiviswanathan, S. [Department of Physics, Indian Institute of Technology Madras, Chennai 600 036 (India); Nigam, A.K. [Department of Condensed Matter Physics and Materials Science, TIFR, Colaba, Mumbai 400 005 (India)

    2015-11-15

    Low temperature magnetic properties of binary Co{sub x}Ga{sub 100−x} alloy with Co concentration in the range 54 ≤ x ≤ 61.5 at% have been investigated. From the temperature and magnetic field dependent magnetization measurements magnetic phase diagram has been identified. Cluster spin glass like features are noticed in x = 54, 55 compositions, while the compositions x > 57 exhibit double magnetic transition i.e., at higher temperatures paramagnetic (PM) – ferromagnetic (FM) and at lower temperatures FM-SG like transition. The critical concentration is identified to be near x = 57 composition where discernible spontaneous magnetization emerges and the long range ferromagnetic order develops above this composition in addition to the spin glass transition (or mixed magnetic phase). Analysis of temperature dependence magnetization data in the different temperature ranges for the compositions x = 60 and 61.5 indicate that the mean field models are not suitable to understand the phase transition. Magnetic isotherms in the critical region were analyzed using non-mean-field approach and the critical exponents (γ = 1.31 and β = 0.337) found to be close to 3D Heisenberg model suggesting the importance of short range magnetic order. The data satisfies magnetic equation of state characteristic of a second order phase transition. The results obtained from the present study corroborate well with the phenomenological interacting spin cluster model. - Graphical abstract: Low temperature magnetic properties of binary Co{sub x}Ga{sub 1−x} alloy with Co concentration in the range 54 ≤ x ≤ 61.5 at% have been investigated. From the temperature and magnetic field dependent magnetization measurements magnetic phase diagram has been identified. Cluster spin glass (SG) like features are noticed in x = 54, 55.5 compositions, while the compositions x > 57 exhibit double magnetic transition i.e., at higher temperatures paramagnetic (PM) – ferromagnetic (FM) and at lower

  20. Gate-Tunable Spin Exchange Interactions and Inversion of Magnetoresistance in Single Ferromagnetic ZnO Nanowires.

    Science.gov (United States)

    Modepalli, Vijayakumar; Jin, Mi-Jin; Park, Jungmin; Jo, Junhyeon; Kim, Ji-Hyun; Baik, Jeong Min; Seo, Changwon; Kim, Jeongyong; Yoo, Jung-Woo

    2016-04-26

    Electrical control of ferromagnetism in semiconductor nanostructures offers the promise of nonvolatile functionality in future semiconductor spintronics. Here, we demonstrate a dramatic gate-induced change of ferromagnetism in ZnO nanowire (NW) field-effect transistors (FETs). Ferromagnetism in our ZnO NWs arose from oxygen vacancies, which constitute deep levels hosting unpaired electron spins. The magnetic transition temperature of the studied ZnO NWs was estimated to be well above room temperature. The in situ UV confocal photoluminescence (PL) study confirmed oxygen vacancy mediated ferromagnetism in the studied ZnO NW FET devices. Both the estimated carrier concentration and temperature-dependent conductivity reveal the studied ZnO NWs are at the crossover of the metal-insulator transition. In particular, gate-induced modulation of the carrier concentration in the ZnO NW FET significantly alters carrier-mediated exchange interactions, which causes even inversion of magnetoresistance (MR) from negative to positive values. Upon sweeping the gate bias from -40 to +50 V, the MRs estimated at 2 K and 2 T were changed from -11.3% to +4.1%. Detailed analysis on the gate-dependent MR behavior clearly showed enhanced spin splitting energy with increasing carrier concentration. Gate-voltage-dependent PL spectra of an individual NW device confirmed the localization of oxygen vacancy-induced spins, indicating that gate-tunable indirect exchange coupling between localized magnetic moments played an important role in the remarkable change of the MR.

  1. Heisenberg spin glass experiments and the chiral ordering scenario

    International Nuclear Information System (INIS)

    Campbell, Ian A.; Petit, Dorothee C.M.C.

    2010-01-01

    An overview is given of experimental data on Heisenberg spin glass materials so as to make detailed comparisons with numerical results on model Heisenberg spin glasses, with particular reference to the chiral driven ordering transition scenario due to Kawamura and collaborators. On weak anisotropy systems, experiments show critical exponents which are very similar to those estimated numerically for the model Heisenberg chiral ordering transition but which are quite different from those at Ising spin glass transitions. Again on weak anisotropy Heisenberg spin glasses, experimental torque data show well defined in-field transverse ordering transitions up to strong applied fields, in contrast to Ising spin glasses where fields destroy ordering. When samples with stronger anisotropies are studied, critical and in-field behavior tend progressively towards the Ising limit. It can be concluded that the essential physics of laboratory Heisenberg spin glasses mirrors that of model Heisenberg spin glasses, where chiral ordering has been demonstrated numerically. (author)

  2. Spin-orbit torque in 3D topological insulator-ferromagnet heterostructure: crossover between bulk and surface transport

    KAUST Repository

    Ghosh, Sumit

    2017-11-29

    Current-driven spin-orbit torques are investigated in a heterostructure composed of a ferromagnet deposited on top of a three dimensional topological insulator using the linear response formalism. We develop a tight-binding model of the heterostructure adopting a minimal interfacial hybridization scheme that promotes induced magnetic exchange on the topological surface states, as well as induced Rashba-like spin-orbit coupling in the ferromagnet. Therefore, our model accounts for spin Hall effect from bulk states together with inverse spin galvanic and magnetoelectric effects at the interface on equal footing. By varying the transport energy across the band structure, we uncover a crossover from surface-dominated to bulk-dominated transport regimes. We show that the spin density profile and the nature of the spin-orbit torques differ substantially in both regimes. Our results, which compare favorably with experimental observations, demonstrate that the large damping torque reported recently is more likely attributed to interfacial magnetoelectric effect, while spin Hall torque remains small even in the bulk-dominated regime.

  3. Spin-orbit torque in a three-dimensional topological insulator–ferromagnet heterostructure: Crossover between bulk and surface transport

    KAUST Repository

    Ghosh, Sumit

    2018-04-02

    Current-driven spin-orbit torques are investigated in a heterostructure composed of a ferromagnet deposited on top of a three-dimensional topological insulator using the linear response formalism. We develop a tight-binding model of the heterostructure adopting a minimal interfacial hybridization scheme that promotes induced magnetic exchange on the topological surface states, as well as induced Rashba-like spin-orbit coupling in the ferromagnet. Therefore our model accounts for the spin Hall effect from bulk states together with inverse spin galvanic and magnetoelectric effects at the interface on equal footing. By varying the transport energy across the band structure, we uncover a crossover from surface-dominated to bulk-dominated transport regimes. We show that the spin density profile and the nature of the spin-orbit torques differ substantially in both regimes. Our results, which compare favorably with experimental observations, demonstrate that the large dampinglike torque reported recently is more likely attributed to the Berry curvature of interfacial states, while spin Hall torque remains small even in the bulk-dominated regime.

  4. Ground state study of the thin ferromagnetic nano-islands for artificial spin ice arrays

    Energy Technology Data Exchange (ETDEWEB)

    Vieira Júnior, D. S., E-mail: damiao.vieira@ifsudestemg.edu.br [Departamento Acadêmico de Matemática, Física e Estatística, Instituto Federal de Educação, Ciência e Tecnologia do Sudeste de Minas Gerais - Câmpus Rio Pomba, Rio Pomba, Minas Gerais 36180-000 (Brazil); Departamento de Física, Laboratório de Simulação Computacional, Universidade Federal de Juiz de Fora, Juiz de Fora, Minas Gerais 36036-330 (Brazil); Leonel, S. A., E-mail: sidiney@fisica.ufjf.br; Dias, R. A., E-mail: radias@fisica.ufjf.br; Toscano, D., E-mail: danilotoscano@fisica.ufjf.br; Coura, P. Z., E-mail: pablo@fisica.ufjf.br; Sato, F., E-mail: sjfsato@fisica.ufjf.br [Departamento de Física, Laboratório de Simulação Computacional, Universidade Federal de Juiz de Fora, Juiz de Fora, Minas Gerais 36036-330 (Brazil)

    2014-09-07

    In this work, we used numerical simulations to study the magnetic ground state of the thin elongated (elliptical) ferromagnetic nano-islands made of Permalloy. In these systems, the effects of demagnetization of dipolar source generate a strong magnetic anisotropy due to particle shape, defining two fundamental magnetic ground state configurations—vortex or type C. To describe the system, we considered a model Hamiltonian in which the magnetic moments interact through exchange and dipolar potentials. We studied the competition between the vortex states and aligned states—type C—as a function of the shape of each elliptical nano-islands and constructed a phase diagram vortex—type C state. Our results show that it is possible to obtain the elongated nano-islands in the C-state with aspect ratios less than 2, which is interesting from the technological point of view because it will be possible to use smaller islands in spin ice arrays. Generally, the experimental spin ice arrangements are made with quite elongated particles with aspect ratio approximately 3 to ensure the C-state.

  5. High-temperature spin dynamics of a cubic ferromagnet Pd2MnSn

    International Nuclear Information System (INIS)

    Kohgi, M.; Endoh, Y.; Ishikawa, Y.; Yoshizawa, H.; Shirane, G.

    1986-01-01

    The paramagnetic scattering function S(q,ω) of the metallic ferromagnet Pd 2 MnSn has been investigated up to 4T/sub C/ over a wide q range along the [100], [011], and [111] directions by means of both polarized and unpolarized neutron scattering techniques. The temperature and q dependence of the static response, k/sub B/Tchi(q), is explained rather well by the Heisenberg model with long-range interactions, although there are nontrivial deviations from the theory. The features of the dynamical response are summarized as follows: (i) The scattering function has a simple one-peak form centered at hω = 0 in the whole q range at 1.5T/sub C/ and 4T/sub C/. (ii) The linewidths of the function near zone boundaries agree well with the calculations based on the three-pole approximation of the Heisenberg model. (iii) The linewidths near q = 0 show the anomalously large temperature dependence, and have no q 2 dependence at 4T/sub C/. These facts point to the importance of the nonadiabatic effects of the conduction electrons at high temperatures, even though the Heisenberg-type interactions between localized spins play the major role on the spin dynamics in this system

  6. Unexpected ferromagnetic ordering enhancement with crystallite size growth observed in La0.5Ca0.5MnO3 nanoparticles

    International Nuclear Information System (INIS)

    Iniama, G.; Ita, B. I.; Presa, P. de la; Hernando, A.; Alonso, J. M.; Multigner, M.; Cortés-Gil, R.; Ruiz-González, M. L.; Gonzalez-Calbet, J. M.

    2014-01-01

    In this paper, the physical properties of half-doped manganite La 0.5 Ca 0.5 MnO 3 with crystallite sizes ranging from 15 to 40 nm are investigated. As expected, ferromagnetic order strengthens at expense of antiferromagnetic one as crystallite size is reduced to 15 nm. However, contrary to previously reported works, an enhancement of saturation magnetization is observed as crystallite size increases from 15 to 22 nm. This unexpected behavior is accompanied by an unusual cell volume variation that seems to induce ferromagnetic-like behavior at expense of antiferromagnetic one. Besides, field cooled hysteresis loops show exchange bias field and coercivity enhancement for increasing cooling fields, which suggest a kind of core-shell structure with AFM-FM coupling for crystallite sizes as small as 15 nm. It is expected that inner core orders antiferromagnetically, whereas uncompensated surface spins behave as spin glass with ferromagnetic-like ordering.

  7. Thickness dependence of the triplet spin-valve effect in superconductor–ferromagnet–ferromagnet heterostructures

    Directory of Open Access Journals (Sweden)

    Daniel Lenk

    2016-07-01

    Full Text Available Background: In nanoscale layered S/F1/N/F2/AF heterostructures, the generation of a long-range, odd-in-frequency spin-projection one triplet component of superconductivity, arising at non-collinear alignment of the magnetizations of F1 and F2, exhausts the singlet state. This yields the possibility of a global minimum of the superconducting transition temperature Tc, i.e., a superconducting triplet spin-valve effect, around mutually perpendicular alignment.Results: The superconducting triplet spin valve is realized with S = Nb a singlet superconductor, F1 = Cu41Ni59 and F2 = Co ferromagnetic metals, AF = CoOx an antiferromagnetic oxide, and N = nc-Nb a normal conducting (nc non-magnetic metal, which serves to decouple F1 and F2. The non-collinear alignment of the magnetizations is obtained by applying an external magnetic field parallel to the layers of the heterostructure and exploiting the intrinsic perpendicular easy-axis of the magnetization of the Cu41Ni59 thin film in conjunction with the exchange bias between CoOx and Co. The magnetic configurations are confirmed by superconducting quantum interference device (SQUID magnetic moment measurements. The triplet spin-valve effect has been investigated for different layer thicknesses, dF1, of F1 and was found to decay with increasing dF1. The data is described by an empirical model and, moreover, by calculations using the microscopic theory.Conclusion: The long-range triplet component of superconducting pairing is generated from the singlet component mainly at the N/F2 interface, where the amplitude of the singlet component is suppressed exponentially with increasing distance dF1. The decay length of the empirical model is found to be comparable to twice the electron mean free path of F1 and, thus, to the decay length of the singlet component in F1. Moreover, the obtained data is in qualitative agreement with the microscopic theory, which, however, predicts a (not investigated breakdown of the

  8. Nanostructures based on superconducting Nb and ferromagnetic CuNi alloy for elaboration of spin-valve core

    International Nuclear Information System (INIS)

    Morari, Roman

    2013-01-01

    The main goal of our research group is the elaboration of superconducting spin-switch (valve) based on Ferromagnetic/Superconductor/Ferromagnetic core. We could realize all building blocks necessary for the fabrication of the core structure of the superconducting spin valve, consisting of two mirror symmetric bilayers. In other words, the spin valve consists of a F/S * /F trilayer, which can be regarded as a package of a F/S and S/F bilayer so that S * =2S in the trilayer. For such a trilayer, the theory predicts that the critical temperature depends on the relative orientation of the magnetization of the ferromagnetic layers. To enable a reversal of one of the magnetizations of the layers with respect to the other by an external magnetic field, the coercive forces of the F layers have to be different due to either intrinsic properties or to an antiferromagnetic pinning layer delivering an exchange bias. The main points of our study are presented here. (author)

  9. A ferromagnetic ground state for Mn-Co surface ordered alloy on Co(001) substrate

    International Nuclear Information System (INIS)

    M'Passi-Mabiala, B.; Meza-Aguilar, S.; Demangeat, C.

    2001-07-01

    Recent Low-energy electron diffraction experiments concerning submonolayer Mn coverage on Co/Cu(001) substrates displayed a well-defined Mn 0.5 Co 0.5 surface ordered alloy. Through the Magneto-optic Kerr effect and X-ray magnetic circular dichroism a ferromagnetic coupling between Mn and Co was obtained. Ab initio density functional theory within generalized gradient approximation is able to explain these results. (author)

  10. Spin-wave mode profiles versus surface/interface conditions in ferromagnetic Fe/Ni layered composites

    International Nuclear Information System (INIS)

    Krawczyk, M; Puszkarski, H; Levy, J-C S; Mercier, D

    2003-01-01

    Spin-wave excitations in ferromagnetic layered composite (AB · · · BA; A and B being different homogeneous ferromagnetic materials) are analysed theoretically, by means of the transfer matrix approach. The properties of multilayer spin-wave mode profiles are discussed in relation to multilayer characteristics, such as the filling fraction and the exchange or magnetization contrast; also, surface spin pinning conditions and dipolar interactions are taken into account. The interface conditions are satisfied by introducing an effective exchange field expressed by interface gradients of the exchange constant and the magnetization. This approach provides an easy way to find frequencies and amplitudes of standing spin waves in the multilayer. The developed theory is applied to interpretation of spin wave resonance (SWR) spectra obtained experimentally by Chambers et al in two systems: a bilayer Fe/Ni and a trilayer Ni/Fe/Ni, in perpendicular (to the multilayer surface) configuration of the applied magnetic field. By fitting the SWR spectra obtained experimentally and those found numerically, the surface anisotropies are estimated on multilayer surfaces; then, the observed resonance lines are identified as associated with bulk, surface or interface modes. The theory can be extended to a general case of any multi-component layered system

  11. Thickness dependence of the triplet spin-valve effect in superconductor-ferromagnet heterostructures

    Energy Technology Data Exchange (ETDEWEB)

    Lenk, Daniel; Zdravkov, Vladimir I.; Kehrle, Jan; Obermeier, Guenther; Krug von Nidda, Hans-Albrecht; Mueller, Claus; Horn, Siegfried; Tidecks, Reinhard [Institut fuer Physik, Universitaet Augsburg (Germany); Morari, Roman [Institut fuer Physik, Universitaet Augsburg (Germany); D. Ghitsu Institute of Electronic Engineering and Nanotechnologies ASM, Kishinev (Moldova, Republic of); Sidorenko, Anatolie S. [D. Ghitsu Institute of Electronic Engineering and Nanotechnologies ASM, Kishinev (Moldova, Republic of); Tagirov, Lenar [Solid State Physics Department, Kazan Federal University (Russian Federation)

    2015-07-01

    We investigated the triplet spin-valve effect in nanoscale layered S/F{sub 1}/N/F{sub 2}/AF heterostructures with varying F{sub 1}-layer thickness (where S=Nb is a singlet superconducting, F{sub 1}=Cu{sub 41}Ni{sub 59} and F{sub 2}=Co a ferromagnetic, and N a normal-conducting, non-magnetic layer). The theory predicts a long-range, odd-in-frequency triplet component of superconductivity at non-collinear alignment of the magnetizations of F{sub 1} and F{sub 2}. This triplet component exhausts the singlet state and, thus, lowers the superconducting transition temperature, T{sub c}, yielding a global minimum of T{sub c} close to the perpendicular mutual orientations of the magnetizations. We found an oscillating decay of T{sub c} suppression, due to the generation of the triplet component, with increasing F{sub 1} layer thickness, which we discuss in the framework of recent theories.

  12. Optimized spin-injection efficiency and spin MOSFET operation based on low-barrier ferromagnet/insulator/n-Si tunnel contact

    Science.gov (United States)

    Yang, Yang; Wu, Zhenhua; Yang, Wen; Li, Jun; Chen, Songyan; Li, Cheng

    2017-06-01

    We theoretically investigate the spin injection in different ferromagnet/insulator/n-Si tunnel contacts by using the lattice non-equilibrium Green’s function method. We find that the tunnel contacts with low-barrier materials such as TiO2 and Ta2O5 have far lower resistances than the conventional-barrier materials, resulting in a wider and attainable optimum parameters window for improving the spin-injection efficiency and magnetoresistance ratio of a vertical-spin metal-oxide-semiconductor field-effect transistor. Additionally, we find that the spin-asymmetry coefficient of the TiO2 tunnel contact has a negative value, while that of the Ta2O5 contact can be tuned between positive and negative values by changing the parameters.

  13. Muon spin relaxation study on itinerant ferromagnet CeCrGe₃ and the effect of Ti substitution on magnetism of CeCrGe₃.

    Science.gov (United States)

    Das, Debarchan; Bhattacharyya, A; Anand, V K; Hillier, A D; Taylor, J W; Gruner, T; Geibel, C; Adroja, D T; Hossain, Z

    2015-01-14

    A Muon spin relaxation (µSR) study has been performed on the Kondo lattice heavy fermion itinerant ferromagnet CeCrGe3. Recent investigations of bulk properties have revealed a long-range ordering of Cr moments at Tc = 70 K in this compound. Our µSR investigation between 1.2 K and 125 K confirm the bulk magnetic order which is marked by a loss in initial asymmetry below 70 K accompanied with a sharp increase in the muon depolarization rate. Field dependent µSR spectra show that the internal field at the muon site is higher than 0.25 T apparently due to the ferromagnetic nature of ordering. The effect of Ti substitution on the magnetism in CeCrGe3 is presented. A systematic study has been made on polycrystalline CeCr(1-x)Ti(x)Ge3 (0 ⩽ x ⩽ 1) using magnetic susceptibility χ(T), isothermal magnetization M(H), specific heat C(T) and electrical resistivity ρ(T) measurements which clearly reveal that the substitution of Ti for Cr in CeCrGe3 strongly influences the exchange interaction and ferromagnetic ordering of Cr moments. The Cr moment ordering temperature is suppressed gradually with increasing Ti concentration up to x = 0.50 showing Tc = 7 K beyond which Ce moment ordering starts to dominate and a crossover between Cr and Ce moment ordering is observed with a Ce moment ordering Tc = 14 K for x = 1.0. The Kondo lattice behavior is evident from temperature dependence of ρ(T) in all CeCr(1-x)Ti(x)Ge3 samples.

  14. Ferromagnetism in metallocene-doped fullerenes

    CERN Document Server

    Mihailovic, D

    2003-01-01

    Ferromagnetism in fullerene-based systems doped with metallocenes is reviewed. These compounds form a ferromagnetic state by spin-coupling between pi electrons on fullerene units, while the metallocene molecules do not contribute to the spin ordering. One of these compounds has the highest critical temperature (19 K) for this class of compound. The magnetic properties of these materials are very strongly dependent on the crystallization conditions. Refs. 19 (author)

  15. Ferromagnetism in metallocene-doped fullerenes

    International Nuclear Information System (INIS)

    Mihailovic, D.

    2003-01-01

    Ferromagnetism in fullerene-based systems doped with metallocenes is reviewed. These compounds form a ferromagnetic state by spin-coupling between π electrons on fullerene units, while the metallocene molecules do not contribute to the spin ordering. One of these compounds has the highest critical temperature (19 K) for this class of compound. The magnetic properties of these materials are very strongly dependent on the crystallization conditions. Refs. 19 (author)

  16. Evidence for 3D isotropic long range spin-spin interaction near the ferromagnetic transition in bulk and thin film SrRuO3

    Science.gov (United States)

    Sow, Chanchal; Pramanik, A. K.; Kumar, P. S. Anil

    2015-05-01

    In the case of metallic ferromagnets there has always been a controversy, i.e. whether the magnetic interaction is itinerant or localized. For example SrRuO3 is known to be an itinerant ferromagnet where the spin-spin interaction is expected to be mean field in nature. However, it is reported to behave like Ising, Heisenberg or mean field by different groups. Despite several theoretical and experimental studies and the importance of strongly correlated systems, the experimental conclusion regarding the type of spin-spin interaction in SrRuO3 is lacking. To resolve this issue, we have investigated the critical behaviour in the vicinity of the paramagnetic-ferromagnetic phase transition using various techniques on polycrystalline as well as (001) oriented SrRuO3 films. Our analysis reveals that the application of a scaling law in the field-cooled magnetization data extracts the value of the critical exponent only when it is measured at H → 0. To substantiate the actual nature without any ambiguity, the critical behavior is studied across the phase transition using the modified Arrott plot, Kouvel-Fisher plot and M-H isotherms. The critical analysis yields self-consistent β, γ and δ values and the spin interaction follows the long-range mean field model. Further the directional dependence of the critical exponent is studied in thin films and it reveals the isotropic nature. It is elucidated that the different experimental protocols followed by different groups are the reason for the ambiguity in determining the critical exponents in SrRuO3.

  17. Pressure-tuned spin state and ferromagnetism in La1-xMxCoO3 (M=Ca,Sr)

    Science.gov (United States)

    Fita, I.; Szymczak, R.; Puzniak, R.; Troyanchuk, I. O.; Fink-Finowicki, J.; Mukovskii, Ya. M.; Varyukhin, V. N.; Szymczak, H.

    2005-06-01

    Pressure effect on magnetic order and anisotropy of low-doped La1-xCaxCoO3 (0.1⩽x⩽0.2) and La1-xSrxCoO3 (0.1⩽x⩽0.3) single crystals and ceramics was studied by magnetization measurements. It was found that applied hydrostatic pressure leads to a quite different effect on ferromagnetic (FM) interactions in materials doped with ions of different size. For La1-xCaxCoO3 , a remarkable suppression of FM interactions leading to a contraction of FM phase fraction was observed under pressure, in good agreement with reduction of effective paramagnetic moment μeff and already reported pressure-induced increase of electrical resistivity. The behavior may be explained by recently proposed mechanism of pressure-induced suppression of double exchange FM interactions in cobaltites, due to an increase of the energy of the crystal-field splitting (t2g-eg) , leading to a suppression of eg -electron hopping. In strong contrast, an opposite pressure effect on ferromagnetism was found in La1-xSrxCoO3 . It appears that pressure enhances visibly the FM interactions in the spin- or cluster-glass state as well as in the long-range FM state for x=0.3 but surprisingly the pressure coefficient dTC/dP changes sign at the percolation threshold. The intricate behavior indicates on a competition of at least two different mechanisms on overall pressure effect in La1-xSrxCoO3 with an expanded unit cell caused by doping with a large size ion. In addition, in Sr-doped single crystals with developed long-range FM order, a drastic changes in magnetic anisotropy with pressure were observed at around 9kbar , leading in the case of La0.7Sr0.3CoO3 to nearly isotropic magnetization within the ac plane at P>9kbar . The radical changes in the magnetic anisotropy suggest some kind of pressure-induced phase transition.

  18. Orbital and spin moments in the ferromagnetic superconductor URhGe by x-ray magnetic circular dichroism

    Science.gov (United States)

    Wilhelm, F.; Sanchez, J. P.; Brison, J.-P.; Aoki, D.; Shick, A. B.; Rogalev, A.

    2017-06-01

    The ferromagnetic superconductor URhGe has been investigated by high field magnetic circular dichroism (XMCD) at the U M4 ,5, Rh L2 ,3, and Ge K edges at 2.1 K and at applied fields up to 17 T. The XMCD performed at the M4 ,5 absorption edges allows us to determine the spectroscopic branching ratio and the 5 f electron contribution to the valence spin-orbit interaction. Combination with polarized neutron diffraction results allows us to derive the individual U orbital and spin moments and the magnetic-dipole contribution . There is no evidence for any change of the orbital-to-spin moment ratios across the spin reorientation transition at HR=12 T , when the field is applied along the initial hard b axis. We also confirm that the magnetism of URhGe is dominated by U , with the contribution of Rh representing only about 10 % of the macroscopic moment. The orbital and spin moments at the Rh site are found to be parallel to each other and parallel to the macroscopic magnetization, but an unexpectedly large orbital-to-spin moment ratio is observed. The XMCD at the Ge K edge reveals the presence of a small induced Ge 4 p orbital moment, parallel to the macroscopic magnetization. The results are discussed against predictions of the electronic band structure calculations by the density functional theory plus Coulomb U , including spin-orbit coupling (DFT +U +SOC ) .

  19. Tunneling conductance and twofold spin-singlet Andreev reflections in ferromagnet/ferromagnet/iron pnictide superconductor hybrid structures with collinear magnetizations

    Science.gov (United States)

    Tao, Y. C.; Tao, Ze; Yu, Qingyun; Yang, X.; Xu, H. Y.

    2017-11-01

    Iron-based superconductors, as some other high-temperature superconducting materials such as the cuprates, are confronted with uncovering the unconventional pairing symmetry, although most researchers favor the so-called s±-wave pairing state. Herein, we theoretically investigate the tunneling conductance of clean ferromagnet (FM)/FM/iron pnictide superconductor (SC) hybrid structures with the SC having s±(two energy gaps have phase difference) pairing symmetry. Novel twofold spin-singlet pairing states near the FM/SC interface in collinear magnetizations emerge due to the presence of two bands in the SC. Conversions of the differential conductance in the ferromagnetic alignment of the two FMs between the peak and valley are shown to be much different from those in the antiferromagnetic alignment. More importantly, two rather different properties in contrast with tunneling into a conventional s-wave SC and an s++-wave SC (two energy gaps have the same sign) are also exhibited, which can be experimentally used to probe and identify the s±pairing symmetry in the iron pnictide SC.

  20. Bias induced up to 100% spin-injection and detection polarizations in ferromagnet/bilayer-hBN/graphene/hBN heterostructures

    NARCIS (Netherlands)

    Gurram, Mallikarjuna; Omar, Siddharta; van Wees, Bart

    2017-01-01

    We study spin transport in a fully hBN encapsulated monolayer-graphene van der Waals heterostructure at room temperature. A top-layer of bilayer-hBN is used as a tunnel barrier for spin-injection and detection in graphene with ferromagnetic cobalt electrodes. We report surprisingly large and

  1. Spin, charge, and orbital orderings in iron-based superconductors

    International Nuclear Information System (INIS)

    Jiang Qing; Kang Yao-Tai; Yao Dao-Xin

    2013-01-01

    In this article, we briefly review spin, charge, and orbital orderings in iron-based superconductors, as well as the multi-orbital models. The interplay of spin, charge, and orbital orderings is a key to understand the high temperature superconductivity. As an illustration, we use the two-orbital model to show the spin and charge orderings in iron-based superconductors based on the mean-field approximation in real space. The typical spin and charge orderings are shown by choosing appropriate parameters, which are in good agreement with experiments. We also show the effect of Fe vacancies, which can introduce the nematic phase and interesting magnetic ground states. The orbital ordering is also discussed in iron-based superconductors. It is found that disorder may play a role to produce the superconductivity. (topical review - iron-based high temperature superconductors)

  2. Spin configuration in a frustrated ferromagnetic/antiferromagnetic thin-film system

    Energy Technology Data Exchange (ETDEWEB)

    Yamada, T K [Faculty of Science, Gakushuin University, 171-8588 Mejiro, Tokyo (Japan); MartInez, E [Fachbereich Physik, Universitaet Osnabrueck, D-49069 Osnabrueck (Germany); Vega, A [Departamento de Fisica Teorica, Atomica y Optica, Universidad de Valladolid, 47011 Valladolid (Spain); Robles, R [Department of Physics, Uppsala University, SE-75121 (Sweden); Stoeffler, D [Institut de Physique et Chimie des Materiaux de Strasbourg (UMR C7504 CNRS-ULP), Strasbourg (France); Parga, A L Vazquez de [Departamento de Fisica de la Materia Condensada, Universidad Autonoma de Madrid, Cantoblanco 28049, Madrid (Spain); Mizoguchi, T [Faculty of Science, Gakushuin University, 171-8588 Mejiro, Tokyo (Japan); Kempen, H van [Institute for Molecules and Materials, Radboud University, Toernooiveld 1, 6525 ED Nijmegen (Netherlands)

    2007-06-13

    We have studied the magnetic configuration in ultrathin antiferromagnetic Mn films grown around monoatomic steps on an Fe(001) surface by spin-polarized scanning tunnelling microscopy/spectroscopy and ab initio-parameterized self-consistent real-space tight-binding calculations in which the spin quantization axis is independent for each site, thus allowing noncollinear magnetism. Mn grown on Fe(001) presents a layered antiferromagnetic structure. In the regions where the Mn films overgrows Fe steps the magnetization of the surface layer is reversed across the steps. Around these defects a frustration of the antiferromagnetic order occurs. Due to the weakened magnetic coupling at the central Mn layers, the amount of frustration is smaller than in Cr, and the width of the wall induced by the step does not change with the thickness, at least for coverages up to seven monolayers.

  3. Effect of asymmetric interface on charge and spin transport across two dimensional electron gas with Dresselhaus spin-orbit coupling/ferromagnet junction

    Science.gov (United States)

    Srisongmuang, B.; Pasanai, K.

    2018-04-01

    We theoretically studied the effect of interfacial scattering on the transport of charge and spin across the junction of a two-dimensional electron gas with Dresselhaus spin-orbit coupling and ferromagnetic material junction, via the conductance (G) and the spin-polarization of the conductance spectra (P) using the scattering method. At the interface, not only were the effects of spin-conserving (Z0) and spin-flip scattering (Zf) considered, but also the interfacial Rashba spin-orbit coupling scattering (ZRSOC) , which was caused by the asymmetry of the interface, was taken into account, and all of them were modeled by the delta potential. It was found that G was suppressed with increasing Z0 , as expected. Interestingly, a particular value of Zf can cause G and P to reach a maximum value. In particular, ZRSOC plays a crucial role to reduce G and P in the metallic limit, but its influence on the tunneling limit was quite weak. On the other hand, the effect of ZRSOC was diminished in the tunneling limit of the magnetic junction.

  4. Ultrathin Epitaxial Ferromagneticγ-Fe2O3Layer as High Efficiency Spin Filtering Materials for Spintronics Device Based on Semiconductors

    KAUST Repository

    Li, Peng

    2016-06-01

    In spintronics, identifying an effective technique for generating spin-polarized current has fundamental importance. The spin-filtering effect across a ferromagnetic insulating layer originates from unequal tunneling barrier heights for spin-up and spin-down electrons, which has shown great promise for use in different ferromagnetic materials. However, the low spin-filtering efficiency in some materials can be ascribed partially to the difficulty in fabricating high-quality thin film with high Curie temperature and/or partially to the improper model used to extract the spin-filtering efficiency. In this work, a new technique is successfully developed to fabricate high quality, ferrimagnetic insulating γ-Fe2O3 films as spin filter. To extract the spin-filtering effect of γ-Fe2O3 films more accurately, a new model is proposed based on Fowler–Nordheim tunneling and Zeeman effect to obtain the spin polarization of the tunneling currents. Spin polarization of the tunneled current can be as high as −94.3% at 2 K in γ-Fe2O3 layer with 6.5 nm thick, and the spin polarization decays monotonically with temperature. Although the spin-filter effect is not very high at room temperature, this work demonstrates that spinel ferrites are very promising materials for spin injection into semiconductors at low temperature, which is important for development of novel spintronics devices. © 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim

  5. Ferromagnetic Ni decorated ordered mesoporous carbons as magnetically separable adsorbents for methyl orange

    International Nuclear Information System (INIS)

    Liu Ningning; Yin Longwei; Zhang Luyuan; Wang Changbin; Lun Ning; Qi Yongxin; Wang Chengxiang

    2011-01-01

    Highlights: ► Magnetically separable Ni-decorated ordered mesoporous carbon (OMC) was successfully synthesized. ► The adsorption capacities for MO dyes on ordered mesoporous carbons, Ni-OMC and activated carbon powder were comparatively investigated. ► The effects of surface area, pore structure, and Ni deposition on the absorption capacities for MO were investigated. ► The ferromagnetic Ni decorated OMC can be easily dispersed in aqueous solution and removed by an external magnetic field. - Abstract: Magnetic ordered mesoporous carbons (OMCs) with Ni nanoparticle (average size: 10 nm) homogeneously modified on surfaces of OMCs were successfully fabricated via a facile casting route. The microstructure, pore size distribution, pore structure, and surface area of the synthesized OMCs and Ni decorated OMCs (Ni-OMCs) were characterized by X-ray diffraction, field emission scanning electron microscopy, high-resolution transmission electron microscopy and N 2 sorption. The characterization by magnetic hysteresis loops suggests a ferromagnetic behavior for the Ni-OMCs samples with a magnetization saturation of 2.34 emu g −1 at 300 K, high enough for magnetic separation. The ferromagnetic Ni-OMCs were used as magnetically separable high-performance adsorbents for methyl orange (MO). The adsorption capacities for MO on the Ni-OMCs as magnetically separable adsorbents were investigated comparatively with pristine OMCs and activated carbon powder (ACP). The results show that the adsorption capacities for MO on the OMCs and Ni-OMCs adsorbents could be well described according to Langmuir isotherm with MO molecule preferentially adsorbed in the structured mesopores, suggesting the adsorption type of monolayer coverage of MO dye onto the mesoporous samples. The effects of surface area, pore structure, and the Ni deposition on the adsorption capacities for MO were systematically investigated. The effects of several important parameters such as contact time, temperature

  6. Temperature dependences of rhombohedral lattice distortion and of ferromagnetic uranium ordering in the uranium monochalcogenides

    International Nuclear Information System (INIS)

    Herrmannsdoerfer, T.; Fischer, P.; Mattenberger, K.; Vogt, O.

    2006-01-01

    By means of high-resolution neutron diffraction, high-quality powder samples of UX (X = S, Se, Te) were investigated in the temperature range from 8 to 299 K in order to establish the relation between ferromagnetic U ordering and rhombohedral lattice distortion as a function of temperature. For US, USe and UTe the rhombohedral angle α of the pseudocubic unit cell is at 10 K approximately 0.4 deg., 0.5 deg. and 0.3 deg. smaller than 90 deg., respectively. Within error limits, the determined ordered magnetic moment values of US and UTe in zero external magnetic field agree with previous neutron single crystal studies, but the larger value derived in the present study for USe, suggest that a higher degree of localisation than previously assumed should be considered for this compound

  7. Manipulation of incoherent and coherent spin ensembles in diluted magnetic semiconductors via ferromagnetic fringe fields; Manipulation inkohaerenter und kohaerenter Spinensembles in verduennt-magnetischen Halbleitern mittels ferromagnetischer Streufelder

    Energy Technology Data Exchange (ETDEWEB)

    Halm, Simon

    2009-05-19

    In this thesis it is demonstrated that fringe fields of nanostructured ferromagnets provide the opportunity to manipulate both incoherent and coherent spin ensembles in a dilute magnetic semiconductor (DMS). Fringe fields of Fe/Tb ferromagnets with a remanent out-of-plane magnetization induce a local magnetization in a (Zn,Cd,Mn)Se DMS. Due to the sp-d exchange interaction, optically generated electron-hole pairs align their spin along the DMS magnetization. One obtains a local, remanent spin polarization which was probed by spatially resolved, polarization sensitive photoluminescence spectroscopy. Fringe fields from in-plane magnetized Co ferromagnets allow to locally modify the precession frequency of the Manganese magnetic moments of the DMS in an external magnetic field. This was probed by time-resolved Kerr rotation technique. The inhomogeneity of the fringe field leads to a shortening of the ensemble decoherence time and to the effect of a time-dependent ensemble precession frequency. (orig.)

  8. Spin beam splitter based on Goos-Haenchen shifts in two-dimensional electron gas modulated by ferromagnetic and Schottky metal stripes

    Energy Technology Data Exchange (ETDEWEB)

    Lu, Mao-Wang; Huang, Xin-Hong; Zhang, Gui-Lin; Chen, Sai-Yan [College of Science, Guilin University of Technology, Guilin 541004 (China)

    2012-11-15

    We present a theoretical study on the spin-dependent Goos-Haenchen (GH) effect in a two-dimensional electron gas modulated by ferromagnetic and Schottky metal (SM) stripes. The GH shifts for spin electron beams across this device are calculated with the help of the stationary phase method. It is shown that the GH shift of spin-up beam is significantly different from that of spin-down beam, i.e., this device shows up a considerable spin polarization effect in GH shifts of electron beams. It also is shown that both magnitude and sign of spin polarization of GH shifts are closely related to the stripe width, the magnetic strength and the gated voltage under SM stripe. These interesting properties not only provide an effective method of spin injection for spintronics application, but also give rise to a tunable spin beam splitter. (Copyright copyright 2012 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  9. Spin ordering in dense matter and magnetic fields of neutron stars

    International Nuclear Information System (INIS)

    Kutschera, M.; Wojcik, W.

    1990-08-01

    The spin properties of the ground-state dense baryon matter are discussed in the nucleon as well as in the quark phase. Predictions for magnetic properties of neutron stars possessing a ferromagnetic core are given. Astrophysical measurements of the magnetic fields of neutron stars are reviewed. An attempt is made to reproduce the data with the ferromagnetic core model. 29 refs., 8 figs. (author)

  10. Intradot spin-flip Andreev reflection tunneling through a ferromagnet-quantum dot-superconductor system with ac field

    International Nuclear Information System (INIS)

    Song Hongyan; Zhou Shiping

    2008-01-01

    We investigate Andreev reflection (AR) tunneling through a ferromagnet-quantum dot-superconductor (F-QD-S) system in the presence of an external ac field. The intradot spin-flip scattering in the QD is involved. Using the nonequilibrium Green function and BCS quasiparticle spectrum for superconductor, time-averaged AR conductance is formulated. The competition between the intradot spin-flip scattering and photon-assisted tunneling dominates the resonant behaviors of the time-averaged AR conductance. For weak intradot spin-flip scattering strengths, the AR conductance shows a series of equal interval resonant levels. However, the single-peak at main resonant level develops into a well-resolved double-peak resonance at a strong intradot spin-flip scattering strength. Remarkable, multiple-photon-assisted tunneling that generates photonic sideband peaks with a variable interval has been found. In addition, the AR conductance-bias voltage characteristic shows a transition between the single-peak to double-peak resonance as the ratio of the two tunneling strengths varies

  11. Spectral properties of an extended Hubbard ladder with long range anti-ferromagnetic order

    Science.gov (United States)

    Yang, Chun; Feiguin, Adrian

    We study the spectral properties of a Hubbard ladder with anti-ferromagnetic long range order by introducing a staggered Heisenberg interaction that decays algebraically. Unlike an alternating field or the t -Jz model, our problem preserves both SU (2) and translational invariance. We solve the problem with the time-dependent density matrix renormalization group and analyze the binding between holons and spinons and the structure of the elementary excitations. We discuss the implications in the context of the 2D Hubbard model at, and away from half-filling by using cluster perturbation theory (CPT). AF acknowledges the U.S. Department of Energy, Office of Basic Energy Sciences, for support under Grant DE-SC0014407.

  12. Magnetocaloric effect in ferromagnetic and ferrimagnetic systems under first and second order phase transition

    Energy Technology Data Exchange (ETDEWEB)

    Ranke, P.J. von, E-mail: von.ranke@uol.com.b [Instituto de Fisica ' Armando Dias Tavares' , Universidade do Estado do Rio de Janeiro-UERJ, Rua Sao Francisco Xavier, 524, 20550-013 RJ (Brazil); Oliveira, N.A. de; Alho, B.P.; Sousa, V.S.R. de; Plaza, E.J.R. [Instituto de Fisica ' Armando Dias Tavares' , Universidade do Estado do Rio de Janeiro-UERJ, Rua Sao Francisco Xavier, 524, 20550-013 RJ (Brazil); Carvalho, A. Magnus G. [Divisao de Metrologia de Materiais, Instituto Nacional de Metrologia, Normalizacao e Qualidade Industrial, Duque de Caxias, RJ (Brazil)

    2010-01-15

    In this work we present a model to describe the magnetocaloric effect (MCE) in ferrimagnetic arrangements. Our model takes into account the magnetoelastic interactions in the two coupled magnetic sublattices, which can lead to the onset of the first order magnetic phase transition and the giant-MCE. Several profiles of the MCE, such as: the inverse- and giant-MCE were systematically studied. Application of the model to the ferromagnetic compounds GdAl{sub 2}, Gd{sub 5}(Ge{sub 1.72}Si{sub 2.28}), Gd{sub 5}(Ge{sub 2}Si{sub 2}), and to the ferrimagnetic compound Y{sub 3}Fe{sub 5}O{sub 12} was performed, showing a good agreement with the experimental data.

  13. Effect of random field disorder on the first order transition in p-spin interaction model

    Science.gov (United States)

    Sumedha; Singh, Sushant K.

    2016-01-01

    We study the random field p-spin model with Ising spins on a fully connected graph using the theory of large deviations in this paper. This is a good model to study the effect of quenched random field on systems which have a sharp first order transition in the pure state. For p = 2, the phase-diagram of the model, for bimodal distribution of the random field, has been well studied and is known to undergo a continuous transition for lower values of the random field (h) and a first order transition beyond a threshold, htp(≈ 0.439) . We find the phase diagram of the model, for all p ≥ 2, with bimodal random field distribution, using large deviation techniques. We also look at the fluctuations in the system by calculating the magnetic susceptibility. For p = 2, beyond the tricritical point in the regime of first order transition, we find that for htp ho = 1 / p!), the system does not show ferromagnetic order even at zero temperature. We find that the magnetic susceptibility for p ≥ 3 is discontinuous at the transition point for h

  14. Controlled tunnel-coupled ferromagnetic electrodes for spin injection in organic single-crystal transistors

    NARCIS (Netherlands)

    Naber, W.J.M.; Craciun, M.F.; Lemmens, J.H.J.; Arkenbout, A.H.; Palstra, T.T.M.; Morpurgo, A.F.; van der Wiel, Wilfred Gerard

    2010-01-01

    We report on single-crystal rubrene field-effect transistors (FETs) with ferromagnetic Co electrodes, tunnel-coupled to the conduction channel via an Al2O3 tunnel barrier. Magnetic and electronic characterization shows that the Al2O3 film not only protects the Co from undesired oxidation, but also

  15. Controlled tunnel-coupled ferromagnetic electrodes for spin injection in organic single-crystal transistors

    NARCIS (Netherlands)

    Naber, W. J. M.; Craciun, M. F.; Lemmens, J. H. J.; Arkenbout, A. H.; Palstra, T. T. M.; Morpurgo, A. F.; van der Wiel, W. G.

    We report on single-crystal rubrene. eld-effect transistors (FETs) with ferromagnetic Co electrodes, tunnel-coupled to the conduction channel via an Al(2)O(3) tunnel barrier. Magnetic and electronic characterization shows that the Al(2)O(3) film not only protects the Co from undesired oxidation, but

  16. k-asymmetric spin splitting at the interface between transition metal ferromagnets and heavy metals

    KAUST Repository

    Grytsiuk, Sergii

    2016-05-23

    We systematically investigate the spin-orbit coupling-induced band splitting originating from inversion symmetry breaking at the interface between a Co monolayer and 4d (Tc, Ru, Rh, Pd, and Ag) or 5d (Re, Os, Ir, Pt, and Au) transition metals. In spite of the complex band structure of these systems, the odd-in-k spin splitting of the bands displays striking similarities with the much simpler Rashba spin-orbit coupling picture. We establish a clear connection between the overall strength of the odd-in-k spin splitting of the bands and the charge transfer between the d orbitals at the interface. Furthermore, we show that the spin splitting of the Fermi surface scales with the induced orbital moment, weighted by the spin-orbit coupling.

  17. The role of mesoscopic structuring on the intermixing of spin-polarised conduction channels in thin-film ferromagnets for spintronics

    Science.gov (United States)

    Alcer, D.; Atkinson, D.

    2017-09-01

    The separation of spin-up and spin-down conduction channels is fundamental to electronic transport in ferromagnets and essential for spintronic functionality. The spin states available for conduction are defined by the ferromagnetic material, but additional physical factors can affect scattering and modify the spin-dependence of conduction. Here the effect of mesoscopic structuring, arising during the growth of ferromagnetic thin films, on the electronic transport was investigated. Resistivity and anisotropic magnetoresistance were measured in a series of Ni80Fe20 thin films as a function of nominal film thickness from 3 {nm} up to 20 {nm}. The observed thickness dependence of the resisivity and magnetic anisotropy of resistivity are interpreted using a model that accounts for the macroscopic structuring from the growth of the films and incorporates a structural dependence of the spin-flip scattering. The model shows good agreement for both the thickness dependence of the resistivity and the reduction of the anisotropic magnetoresistivity. The latter indicating that increasing mixing of the conducting spin channels occurs in ultra-thin films, mainly a consequence of macroscopic structuring of the films.

  18. Neutron Scattering Investigation of the Temperature Dependence of Long-Wavelength Spin Waves in Ferromagnetic Rb2CrCI4

    DEFF Research Database (Denmark)

    Hutchings, M T; Als-Nielsen, Jens Aage; Lindgård, Per-Anker

    1981-01-01

    The long-wavelength spin waves in Rb2CrCl4, a nearly two-dimensional ferromagnet, have been investigated at several temperatures below Tc=52.4K using neutron inelastic scattering techniques. The data have been analysed in terms of a Hartree-Fock theory using matching-matrix elements to give...

  19. Effect of Second-Order Spin-Orbit Coupling on the Interaction between Spin States in Spin-Crossover Systems.

    Science.gov (United States)

    Sousa, Carmen; Domingo, Alex; de Graaf, Coen

    2017-11-16

    The second-order spin-orbit coupling is evaluated in two transition-metal complexes to establish the effect on the deactivation mechanism of the excited low-spin state in systems that undergo spin transitions under the influence of light. We compare the standard perturbational approach to calculate the second-order interaction with a variational strategy based on the effective Hamiltonian theory and show that the former one can only be applied in some special cases and even then gives results that largely overestimate the interaction. The combined effect of geometry distortions and second-order spin-orbit coupling leads to sizeable interactions for states that are nearly uncoupled in the symmetric (average) structure of the complex. This opens the possibility of a direct deactivation from the singlet and triplet states of the metal-to-ligand charge-transfer manifold to the final high-spin state as suggested from the interpretation of experimental data but so far not supported by theoretical descriptions of the light-induced spin crossover. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

  20. Field-induced transition of the magnetic ground state from A-type antiferromagnetic to ferromagnetic order in CsCo2Se2

    Science.gov (United States)

    von Rohr, Fabian; Krzton-Maziopa, Anna; Pomjakushin, Vladimir; Grundmann, Henrik; Guguchia, Zurab; Schnick, Wolfgang; Schilling, Andreas

    2016-07-01

    We report on the magnetic properties of CsCo2Se2 with ThCr2Si2 structure, which we have characterized through a series of magnetization and neutron diffraction measurements. We find that CsCo2Se2 undergoes a phase transition to an antiferromagnetically ordered state with a Néel temperature of {{T}\\text{N}}≈ 66 K. The nearest neighbour interactions are ferromagnetic as observed by the positive Curie-Weiss temperature of \\Theta≈ 51.0 K. We find that the magnetic structure of CsCo2Se2 consists of ferromagnetic sheets, which are stacked antiferromagnetically along the tetragonal c-axis, generally referred to as A-type antiferromagnetic order. The observed magnitude of the ordered magnetic moment at T  =  1.5 K is found to be only 0.20(1){μ\\text{Bohr}}  / Co. Already in comparably small magnetic fields of {μ0}H{{}\\text{MM}}(5~K)≈ 0.3 T, we observe a metamagnetic transition that can be attributed to spin-rearrangements of CsCo2Se2, with the moments fully ferromagnetically saturated in a magnetic field of {μ0}{{H}\\text{FM}}(5~K)≈ 6.4 T. We discuss the entire experimentally deduced magnetic phase diagram for CsCo2Se2 with respect to its unconventionally weak magnetic coupling. Our study characterizes CsCo2Se2, which is chemically and electronically posed closely to the A x Fe2-y Se2 superconductors, as a host of versatile magnetic interactions.

  1. Third-order-harmonic generation in coherently spinning molecules

    Science.gov (United States)

    Prost, E.; Zhang, H.; Hertz, E.; Billard, F.; Lavorel, B.; Bejot, P.; Zyss, Joseph; Averbukh, Ilya Sh.; Faucher, O.

    2017-10-01

    The rotational Doppler effect occurs when circularly polarized light interacts with a rotating anisotropic material. It is manifested by the appearance of a spectral shift ensuing from the transfer of angular momentum and energy between radiation and matter. Recently, we reported terahertz-range rotational Doppler shifts produced in third-order nonlinear optical conversion [O. Faucher et al., Phys. Rev. A 94, 051402(R) (2016), 10.1103/PhysRevA.94.051402]. The experiment was performed in an ensemble of coherently spinning molecules prepared by a short laser pulse exhibiting a twisted linear polarization. The present work provides an extensive analysis of the rotational Doppler effect in third-order-harmonic generation from spinning linear molecules. The underlying physics is investigated both experimentally and theoretically. The implication of the rotational Doppler effect in higher-order processes like high-order-harmonic generation is discussed.

  2. Role of spin diffusion in current-induced domain wall motion for disordered ferromagnets

    KAUST Repository

    Akosa, Collins Ashu

    2015-03-12

    Current-induced spin transfer torque and magnetization dynamics in the presence of spin diffusion in disordered magnetic textures is studied theoretically. We demonstrate using tight-binding calculations that weak, spin-conserving impurity scattering dramatically enhances the nonadiabaticity. To further explore this mechanism, a phenomenological drift-diffusion model for incoherent spin transport is investigated. We show that incoherent spin diffusion indeed produces an additional spatially dependent torque of the form ∼∇2[m×(u⋅∇)m]+ξ∇2[(u⋅∇)m], where m is the local magnetization direction, u is the direction of injected current, and ξ is a parameter characterizing the spin dynamics (precession, dephasing, and spin-flip). This torque, which scales as the inverse square of the domain wall width, only weakly enhances the longitudinal velocity of a transverse domain wall but significantly enhances the transverse velocity of vortex walls. The spatial-dependent spin transfer torque uncovered in this study is expected to have significant impact on the current-driven motion of abrupt two-dimensional textures such as vortices, skyrmions, and merons.

  3. Spin dynamics in ferromagnets: Gilbert dymping and two-magnon scattering

    Czech Academy of Sciences Publication Activity Database

    Zakeri, Kh.; Lindner, J.; Barsukov, I.; Meckenstock, R.; Farle, M.; von Horsten, U.; Wende, H.; Keune, W.; Rocker, J.; Kalarickal, S.S.; Lenz, K.; Kuch, W.; Baberschke, K.; Frait, Zdeněk

    2007-01-01

    Roč. 76, č. 10 (2007), 104416/1-104416/8 ISSN 1098-0121 Grant - others:Deutsche Forschunggemeinschaft(DE) Sfb 491; EC Marie Curie Research Training Network(XE) MRTN-CT-2004-005567, 2004-2008 Institutional research plan: CEZ:AV0Z10100520 Keywords : ferromagnetic resonance * Gilbert damping * two-magnon scattering * Fe 3 Si films Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.172, year: 2007

  4. Charge-spin excitations of the Ising-type fractional quantum Hall ferromagnets

    Czech Academy of Sciences Publication Activity Database

    Výborný, Karel; Dethlefsen, A.F.; Haug, R.J.; Wójs, A.

    2009-01-01

    Roč. 80, č. 4 (2009), 045407/1-045407/13 ISSN 1098-0121 R&D Projects: GA MŠk LC510; GA AV ČR KJB100100802; GA AV ČR KAN400100652 Institutional research plan: CEZ:AV0Z10100521 Keywords : fractional quantum Hall effect * quantum Hall ferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.475, year: 2009

  5. Visualization of anomalous Ettingshausen effect in a ferromagnetic film: Direct evidence of different symmetry from spin Peltier effect

    Science.gov (United States)

    Seki, T.; Iguchi, R.; Takanashi, K.; Uchida, K.

    2018-04-01

    Spatial distribution of temperature modulation due to the anomalous Ettingshausen effect (AEE) is visualized in a ferromagnetic FePt thin film with in-plane and out-of-plane magnetizations using the lock-in thermography technique. Comparing the AEE of FePt with the spin Peltier effect (SPE) of a Pt/yttrium iron garnet junction provides direct evidence of different symmetries of AEE and SPE. Our experiments and numerical calculations reveal that the distribution of heat sources induced by AEE strongly depends on the direction of magnetization, leading to the remarkable different temperature profiles in the FePt thin film between the in-plane and perpendicularly magnetized configurations.

  6. First-principles study of high spin-polarization and thermoelectric efficiency of ferromagnetic CoFeCrAs quaternary Heusler alloy

    Science.gov (United States)

    Bhat, Tahir Mohiuddin; Gupta, Dinesh C.

    2018-03-01

    The ground state properties along with thermodynamic and thermoelectric properties of quaternary CoFeCrAs alloy within the ordered LiMgPdSn-type structure have been investigated by employing first-principles calculations. The alloy offers half-metallic ferromagnet character with an indirect band gap of 1.12 eV in the minority spin state with total spin magnetic moment of 4μB and follows Slater-Pauling relation. Effects on various properties of the material has been studied by the variation of the pressure and temperature. CoFeCrAs tenders large value of the Grüneisen parameter and small value for the thermal expansion coefficient. The materials present high Seebeck coefficient and huge power factor with the room temperature value of ∼-40 μV/K and 18 (1014 μWcm-1 K-2 s-1) respectively, which make CoFeCrAs promising candidate for efficient thermoelectric material.

  7. Superconductivity and spin excitations in orbitally ordered FeSe

    Science.gov (United States)

    Kreisel, Andreas; Mukherjee, Shantanu; Hirschfeld, P. J.; Andersen, B. M.

    We provide a band-structure with low-energy properties consistent with recent photoemission and quantum oscillations measurements on the Fe-based superconductor FeSe, including a mean-field like orbital ordering in the dxz /dyz channel, and show that this model also accounts for the temperature dependence of the measured Knight shift and the spin-relaxation rate. An RPA calculation of the dynamical spin susceptibility yields spin excitations which are peaked at wave vector (π , 0) in the 1-Fe Brillouin zone, with a broad maximum at energies of order a few meV. Furthermore, the superconducting gap structure obtained from spin fluctuation theory exhibits nodes on the electron pockets, consistent with the 'V'-shaped density of states measured by tunneling spectroscopy on this material. The redistribution of spectral weight in the superconducting state creates a (π , 0) ''neutron resonance'' as seen in recent experiments. Comparing to various experimental results, we give predictions for further studies A.K. and B.M.A. acknowledge financial support from a Lundbeckfond fellowship (Grant No. A9318). P.J.H. was partially supported by the Department of Energy under Grant No. DE-FG02-05ER46236.

  8. Superconductivity and spin excitations in orbitally ordered FeSe

    Energy Technology Data Exchange (ETDEWEB)

    Kreisel, Andreas; Andersen, Brian M. [Niels Bohr Institute, University of Copenhagen (Denmark); Mukherjee, Shantanu [Niels Bohr Institute, University of Copenhagen (Denmark); Dept. of Physics, State University of New York at Binghamton, Binghamton, NY (United States); Hirschfeld, Peter J. [University of Florida, Gainesville, FL (United States)

    2016-07-01

    We provide a band-structure with low-energy properties consistent with recent photoemission and quantum oscillations measurements on the Fe-based superconductor FeSe, including a mean-field like orbital ordering in the d{sub xz}/d{sub yz} channel, and show that this model also accounts for the temperature dependence of the measured Knight shift and the spin-relaxation rate. An RPA calculation of the dynamical spin susceptibility yields spin excitations which are peaked at wave vector (π,0) in the 1-Fe Brillouin zone, with a broad maximum at energies of order a few meV. Furthermore, the superconducting gap structure obtained from spin fluctuation theory exhibits nodes on the electron pockets, consistent with the 'V'-shaped density of states measured by tunneling spectroscopy on this material. The redistribution of spectral weight in the superconducting state creates a (π,0) ''neutron resonance'' as seen in recent experiments. Comparing to various experimental results, we give predictions for further studies.

  9. Room temperature p-type conductivity and coexistence of ferroelectric order in ferromagnetic Li doped ZnO nanoparticles

    KAUST Repository

    Awan, Saif Ullah

    2014-10-28

    Memory and switching devices acquired new materials which exhibit ferroelectric and ferromagnetic order simultaneously. We reported multiferroic behavior in Zn1-yLiyO(0.00≤y≤0.10) nanoparticles. The analysis of transmission electron micrographs confirmed the hexagonal morphology and wurtzite crystalline structure. We investigated p-type conductivity in doped samples and measured hole carriers in range 2.4×1017/cc to 7.3×1017/cc for different Li contents. We found that hole carriers are responsible for long range order ferromagnetic coupling in Li doped samples. Room temperature ferroelectric hysteresis loops were observed in 8% and 10% Li doped samples. We demonstrated ferroelectric coercivity (remnant polarization) 2.5kV/cm (0.11 μC/cm2) and 2.8kV/cm (0.15 μC/cm2) for y=0.08 and y=0.10 samples. We propose that the mechanism of Li induced ferroelectricity in ZnO is due to indirect dipole interaction via hole carriers. We investigated that if the sample has hole carriers ≥5.3×1017/cc, they can mediate the ferroelectricity. Ferroelectric and ferromagnetic measurements showed that higher electric polarization and larger magnetic moment is attained when the hole concentration is larger and vice versa. Our results confirmed the hole dependent coexistence of ferromagnetic and ferroelectric behavior at room temperature, which provide potential applications for switchable and memory devices.

  10. Spin-cycloid instability as the origin of weak ferromagnetism in the disordered perovskite Bi0.8La0.2Fe0.5Mn0.5O3

    Science.gov (United States)

    Bertinshaw, J.; Cortie, D. L.; Cheng, Z. X.; Avdeev, M.; Studer, A. J.; Klose, F.; Ulrich, C.; Wang, X. L.

    2014-04-01

    Powder neutron diffraction and magnetometry studies have been conducted to investigate the crystallographic and magnetic structure of Bi0.8La0.2Fe0.5Mn0.5O3. The compound stabilizes in the Imma orthorhombic crystal symmetry in the measured temperature range of 5 to 380 K, with a transition to antiferromagnetic order at TN≈240 K. The spin cycloid present for BiFeO3 is found to be absent with 50% Mn3+ cation substitution, leading to G-type antiferromagnetic order with an enhanced out-of-plane canted ferromagnetic component, evident from measurable weak-ferromagnetic hysteresis. Structural modifications do not solely explain this behavior, indicating that modified electron exchange interactions must be taken into account. A classical spin simulation was developed to investigate the effect of random substitution in a disordered pseudocubic perovskite. The calculations took into account the nearest-neighbor, next-nearest-neighbor, and Dzyaloshinskii-Moriya interactions, along with the local spin anisotropy. Using this framework to extend the established Hamiltonian model for BiFeO3, we show that only certain types of perturbations at a magnetic defect and the surrounding molecular fields trigger a simultaneous collapse of cycloidal order and the emergence of the long-range weak-ferromagnetic component. By adopting values for the Mn molecular fields appropriate for REMnO3 (RE = rare earth), simulations of BiMn0.5Fe0.5O3 exhibit the key magnetic properties of our experimental observations.

  11. Energy landscape of 3D spin Hamiltonians with topological order.

    Science.gov (United States)

    Bravyi, Sergey; Haah, Jeongwan

    2011-10-07

    We explore the feasibility of a quantum self-correcting memory based on 3D spin Hamiltonians with topological quantum order in which thermal diffusion of topological defects is suppressed by macroscopic energy barriers. To this end we characterize the energy landscape of stabilizer code Hamiltonians with local bounded-strength interactions which have a topologically ordered ground state but do not have stringlike logical operators. We prove that any sequence of local errors mapping a ground state of such a Hamiltonian to an orthogonal ground state must cross an energy barrier growing at least as a logarithm of the lattice size. Our bound on the energy barrier is tight up to a constant factor for one particular 3D spin Hamiltonian.

  12. Ensemble-averaged Rabi oscillations in a ferromagnetic CoFeB film.

    Science.gov (United States)

    Capua, Amir; Rettner, Charles; Yang, See-Hun; Phung, Timothy; Parkin, Stuart S P

    2017-06-28

    Rabi oscillations describe the process whereby electromagnetic radiation interacts coherently with spin states in a non-equilibrium interaction. To date, Rabi oscillations have not been studied in one of the most common spin ensembles in nature: spins in ferromagnets. Here, using a combination of femtosecond laser pulses and microwave excitations, we report the classical analogue of Rabi oscillations in ensemble-averaged spins of a ferromagnet. The microwave stimuli are shown to extend the coherence-time resulting in resonant spin amplification. The results we present in a dense magnetic system are qualitatively similar to those reported previously in semiconductors which have five orders of magnitude fewer spins and which require resonant optical excitations to spin-polarize the ensemble. Our study is a step towards connecting concepts used in quantum processing with spin-transport effects in ferromagnets. For example, coherent control may become possible without the complications of driving an electromagnetic field but rather by using spin-polarized currents.

  13. Ensemble-averaged Rabi oscillations in a ferromagnetic CoFeB film

    Science.gov (United States)

    Capua, Amir; Rettner, Charles; Yang, See-Hun; Phung, Timothy; Parkin, Stuart S. P.

    2017-06-01

    Rabi oscillations describe the process whereby electromagnetic radiation interacts coherently with spin states in a non-equilibrium interaction. To date, Rabi oscillations have not been studied in one of the most common spin ensembles in nature: spins in ferromagnets. Here, using a combination of femtosecond laser pulses and microwave excitations, we report the classical analogue of Rabi oscillations in ensemble-averaged spins of a ferromagnet. The microwave stimuli are shown to extend the coherence-time resulting in resonant spin amplification. The results we present in a dense magnetic system are qualitatively similar to those reported previously in semiconductors which have five orders of magnitude fewer spins and which require resonant optical excitations to spin-polarize the ensemble. Our study is a step towards connecting concepts used in quantum processing with spin-transport effects in ferromagnets. For example, coherent control may become possible without the complications of driving an electromagnetic field but rather by using spin-polarized currents.

  14. Zero-field Spin Depolarization of Low-Energy Muons in Ferromagnetic Nickel and Silver Metal

    Science.gov (United States)

    Saadaoui, H.; Salman, Z.; Prokscha, T.; Suter, A.; Wojek, B. M.; Morenzoni, E.

    We present zero-field muon-spin depolarization measurements in nickel and silver performed using low-energy muon-spin relaxation technique.Ni or Ag are usually used in this depth-resolved technique as a backing material to enable background subtraction when studying small crystals or materials with weak magnetism. The depolarization rate of the asymmetry in silver and that of the slow relaxing part of the asymmetry in nickel are small(≤ 0.05 μs-1), and weakly temperature and energy-dependent.

  15. Evidence for triplet superconductivity in a superconductor-ferromagnet spin valve.

    Science.gov (United States)

    Leksin, P V; Garif'yanov, N N; Garifullin, I A; Fominov, Ya V; Schumann, J; Krupskaya, Y; Kataev, V; Schmidt, O G; Büchner, B

    2012-08-03

    We have studied the dependence of the superconducting (SC) transition temperature on the mutual orientation of magnetizations of Fe1 and Fe2 layers in the spin valve system CoO(x)/Fe1/Cu/Fe2/Pb. We find that this dependence is nonmonotonic when passing from the parallel to the antiparallel case and reveals a distinct minimum near the orthogonal configuration. The analysis of the data in the framework of the SC triplet spin valve theory gives direct evidence for the long-range triplet superconductivity arising due to noncollinearity of the two magnetizations.

  16. Metal-free ferromagnetic metal and intrinsic spin semiconductor: two different kinds of SWCNT functionalized BN nanoribbons.

    Science.gov (United States)

    Lou, Ping

    2015-03-28

    Two different kinds of SWCNT functionalized zigzag edge BN nanoribbons with n chains (n-ZBNNRs), namely, (a) B-edge functionalized by (m,m)SWCNT and N-edge modified with H (nZBNNR-B-(m,m)SWCNTs); and (b) the B-edge modified with H and the N-edge functionalized by (m,m)SWCNT (nZBNNR-N-(m,m)SWCNTs), have been predicted. Amazingly, we find that unlike the semiconducting and nonmagnetic H-modified n-ZBNNRs, the nZBNNR-B-(m,m)SWCNTs are intrinsic ferromagnetic metals, regardless of ribbon widths n and tube diameters (m,m). At a given (m,m), their local magnetic moments, at first, exhibit oscillation with increasing n, whereas when n is larger than 5, they are independent of n. In contrast, unlike the metallic and nonmagnetic (m,m)SWCNTs, the nZBNNR-N-(m,m)SWCNTs are ferromagnetic intrinsic spin-semiconductors with direct band gaps, regardless of n and (m,m). Their local magnetic moments and band gaps are independent of n and (m,m). The DFT calculations reveal that the process of SWCNT functionalization of the n-ZBNNRs does not need any activation energy. Moreover, the formation energies of the SWCNT functionalized n-ZBNNRs are always less than zero. Therefore, the SWCNT functionalized n-ZBNNRs are not only stable, but can also be spontaneously formed. Furthermore, compared with n-ZBNNRs, the SWCNT functionalized n-ZBNNRs show significant improvements in their thermal and mechanical stabilities. Thus, (m,m)SWCNT functionalization of n-ZBNNRs may open new routes toward practical nanoelectronic and optoelectronic as well as spintronic devices based on BNC-based materials.

  17. Superconducting Ferromagnetic Nanodiamond.

    Science.gov (United States)

    Zhang, Gufei; Samuely, Tomas; Xu, Zheng; Jochum, Johanna K; Volodin, Alexander; Zhou, Shengqiang; May, Paul W; Onufriienko, Oleksandr; Kačmarčík, Jozef; Steele, Julian A; Li, Jun; Vanacken, Johan; Vacík, Jiri; Szabó, Pavol; Yuan, Haifeng; Roeffaers, Maarten B J; Cerbu, Dorin; Samuely, Peter; Hofkens, Johan; Moshchalkov, Victor V

    2017-06-27

    Superconductivity and ferromagnetism are two mutually antagonistic states in condensed matter. Research on the interplay between these two competing orderings sheds light not only on the cause of various quantum phenomena in strongly correlated systems but also on the general mechanism of superconductivity. Here we report on the observation of the electronic entanglement between superconducting and ferromagnetic states in hydrogenated boron-doped nanodiamond films, which have a superconducting transition temperature T c ∼ 3 K and a Curie temperature T Curie > 400 K. In spite of the high T Curie , our nanodiamond films demonstrate a decrease in the temperature dependence of magnetization below 100 K, in correspondence to an increase in the temperature dependence of resistivity. These anomalous magnetic and electrical transport properties reveal the presence of an intriguing precursor phase, in which spin fluctuations intervene as a result of the interplay between the two antagonistic states. Furthermore, the observations of high-temperature ferromagnetism, giant positive magnetoresistance, and anomalous Hall effect bring attention to the potential applications of our superconducting ferromagnetic nanodiamond films in magnetoelectronics, spintronics, and magnetic field sensing.

  18. Spin lattice relaxation of 8Li in a ferromagnetic EuO epitaxial thin film

    Science.gov (United States)

    Song, Q.; Chow, K. H.; Egilmez, M.; Fan, I.; Hossain, M. D.; Kiefl, R. F.; Kreitzman, S. R.; Levy, C. D. P.; Morris, G. D.; Parolin, T. J.; Pearson, M. R.; Salman, Z.; Saadaoui, H.; Smadella, M.; Wang, D.; Ingle, N. J. C.; MacFarlane, W. A.

    2009-04-01

    We inject a low energy spin polarized Li+8 beam into an epitaxially grown multilayer film consisting of Au(20 nm)/EuO(100 nm)/ LaAlO3, and investigate the nuclear spin relaxation at 3.33 T. The relaxation varies with implantation energy below 28 keV as the fraction of the probe Li8 stopping in each layer changes. We attribute the fast relaxating component to the EuO, while the much slower relaxation has contributions from both the Au and the substrate. However, fast relaxation is still observed at the lowest implantation energy where all the Li8 stops in the Au capping layer. This may be due to a proximity effect from the EuO.

  19. Spin lattice relaxation of {sup 8}Li in a ferromagnetic EuO epitaxial thin film

    Energy Technology Data Exchange (ETDEWEB)

    Song, Q., E-mail: susan@phas.ubc.c [Department of Physics, University of British Columbia, Vancouver, BC, V6T 1Z1 (Canada); Chow, K.H.; Egilmez, M.; Fan, I. [Department of Physics, University of Alberta, Edmonton, AB, T6G 2G7 (Canada); Hossain, M.D. [Department of Physics, University of British Columbia, Vancouver, BC, V6T 1Z1 (Canada); Kiefl, R.F. [Department of Physics, University of British Columbia, Vancouver, BC, V6T 1Z1 (Canada); Canadian Institute of Advanced Research (Canada); Kreitzman, S.R.; Levy, C.D.P.; Morris, G.D. [TRIMF, 4004 Wesbrook Mall, Vancouver, BC, V6T 2A3 (Canada); Parolin, T.J. [Chemistry Department, University of British Columbia, Vancouver, BC, V6T 1Z1 (Canada); Pearson, M.R. [TRIMF, 4004 Wesbrook Mall, Vancouver, BC, V6T 2A3 (Canada); Salman, Z. [TRIMF, 4004 Wesbrook Mall, Vancouver, BC, V6T 2A3 (Canada); Physics Department, Oxford University, Parks Road, Oxford, OX1 3PU (United Kingdom); Saadaoui, H.; Smadella, M.; Wang, D. [Department of Physics, University of British Columbia, Vancouver, BC, V6T 1Z1 (Canada); Ingle, N.J.C. [AMPEL, University of British Columbia, Vancouver (Canada); MacFarlane, W.A. [Chemistry Department, University of British Columbia, Vancouver, BC, V6T 1Z1 (Canada)

    2009-04-15

    We inject a low energy spin polarized {sup 8}Li{sup +} beam into an epitaxially grown multilayer film consisting of Au(20 nm)/EuO(100 nm)/LaAlO{sub 3}, and investigate the nuclear spin relaxation at 3.33 T. The relaxation varies with implantation energy below 28 keV as the fraction of the probe {sup 8}Li stopping in each layer changes. We attribute the fast relaxating component to the EuO, while the much slower relaxation has contributions from both the Au and the substrate. However, fast relaxation is still observed at the lowest implantation energy where all the {sup 8}Li stops in the Au capping layer. This may be due to a proximity effect from the EuO.

  20. Spin-transfer induced ultrafast precessional switching enhanced by interface anisotropy in a ferromagnetic nanopillar

    International Nuclear Information System (INIS)

    Daniel, M.; Sabareesan, P.

    2009-07-01

    Spin-transfer induced ultrafast precessional switching of magnetization in the Co/Cu/Co nanopillar device is studied. Micromagnetic calculations show that, precessional magnetization switching occurs above a threshold current. The presence of interface uniaxial anisotropy in the Co-thin film free layer, influences heavily the current and energy required to initiate the switching in the device, and the speed of the precessional switching. The threshold current and the precessional switching time are significantly reduced by this effect. (author)

  1. Electron spin resonance study of the demagnetization fields of the ferromagnetic and paramagnetic films

    Directory of Open Access Journals (Sweden)

    I.I. Gimazov, Yu.I. Talanov

    2015-12-01

    Full Text Available The results of the electron spin resonance study of the La1-xCaxMnO3 manganite and the diphenyl-picrylhydrazyl thin films for the magnetic field parallel and perpendicular to plane of the films are presented. The temperature dependence of the demagnetizing field is obtained. The parameters of the Curie-Weiss law are estimated for the paramagnetic thin film.

  2. Local structural distortions, orbital ordering, and ferromagnetism in underdoped La1 -xSrxMnO3

    Science.gov (United States)

    Zhou, J.-S.; Goodenough, J. B.

    2015-02-01

    In order to elucidate the origin of the ferromagnetism found in underdoped L a1 -xS rxMn O3 , we have grown a series of single crystals with a fine step of doping and characterized them with a structural study and measurements of magnetization, resistivity, thermoelectric power, and thermal conductivity. The paramagnetic phase of the underdoped L a1 -xS rxMn O3 is a small-polaron conductor. However, the Weiss constant extracted from the paramagnetic susceptibility shows a ferromagnetic coupling and tracks the Curie temperature. Given that the double exchange interaction cannot be delivered by the hopping motion of small polarons, we have made a systematic analysis of the structural changes with x and studied whether the superexchange interaction can account for the ferromagnetic coupling found in the paramagnetic phase. Intrinsic local site distortions in LaMn O3 change as x increases in L a1 -xS rxMn O3 . The influence of the local structural distortion and the cooperative orbital ordering on lattice parameters have been demonstrated by a comparison between the measured change of lattice parameters versus hole doping and a simulation with the software SPuDs, in which rigid octahedra are assumed. Changes with x of the bond length splitting in Mn O6 octahedra induces an orbital mixing of (3 x2-r2) +(y2-z2) or (3 y2-r2) +(z2-x2) , which progressively converts two-dimensional ferromagnetism in the parent perovskite LaMn O3 into three-dimensional ferromagnetism. The correlation between the particular lattice distortions and the cooperative orbital ordering and orbital mixing can in turn be used to test the superexchange model by measuring the change of transition temperatures under uniaxial stress. Nearly identical uniaxial stress effects found in crystals of the mixed-valent L a0.875S r.125Mn O3 and single-valent LaM n0.5G a0.5O3 confirm unambiguously that superexchange interactions play the dominant role in the ferromagnetic coupling of underdoped L a1 -xS rxMn O3 .

  3. Reply to Comment on 'Commented review: UCu2Ge2 and UCu2Si2-compounds with only ferromagnetic ordering'

    International Nuclear Information System (INIS)

    Kuznietz, Moshe

    2005-01-01

    In a reply to the preceding Comment by Roy et al (2005 J. Phys.: Condens. Matter 17 3113) on 'Commented review: UCu 2 Ge 2 and UCu 2 Si 2 -compounds with only ferromagnetic ordering', published recently by the present author (Kuznietz 2003 J. Phys.: Condens. Matter 15 8957), the assertion that only ferromagnetic ordering occurs in UCu 2 Ge 2 , as observed by means of neutron diffraction and other methods, is stated and documented. None of the variety of experimental results on UCu 2 Ge 2 produced by Roy et al and summarized briefly, but without any new neutron diffraction data, can contradict or serve as a basis for disputing that there is only ferromagnetic ordering in UCu 2 Ge 2 in zero and low applied magnetic fields, as observed by means of neutron diffraction and ac susceptibility, respectively. The comparison between UCu 2 Ge 2 and some Ce(Fe,M) 2 solid solutions made by Roy et al, and the similarities of some of their magnetic properties, are claimed to be coincidental, and not to lead to conclusions regarding UCu 2 Ge 2 magnetism. Only new neutron diffraction data could truly justify such a Comment on the 'Commented review'. (reply)

  4. Evaluation of Schottky and MgO-based tunnelling diodes with different ferromagnets for spin injection in n-Si

    International Nuclear Information System (INIS)

    Uhrmann, T; Dimopoulos, T; Brueckl, H; Kovacs, A; Kohn, A; Weyers, S; Paschen, U; Smoliner, J

    2009-01-01

    In this work we present the electrical properties of sputter-deposited ferromagnetic (FM) Schottky diodes and MgO-based tunnelling diodes to n-doped (0 0 1) silicon. The effective Schottky barrier height (SBH) has been evaluated as a function of the FM electrode (Co 70 Fe 30 , Co 40 Fe 40 B 20 and Ni 80 Fe 20 ), the silicon doping density (10 15 to 10 18 cm -3 ), the MgO tunnelling barrier thickness (0, 1.5 and 2.5 nm) and post-deposition annealing up to 400 0 C. The ideality factors of the Schottky diodes are close to unity, indicating transport by thermionic emission and the absence of an interfacial oxide layer, which is confirmed by transmission electron microscopy. The effective SBH is found to be approximately 0.65 eV, independent of the FM material and decreasing with increasing doping density. The changes induced by high temperature annealing at the current-voltage characteristic of the Schottky diodes depend strongly on the FM electrode. The effective SBH for the tunnelling diodes is as low as 0.3 eV, which suggests a high density of oxide and interface traps. It is again independent of the FM electrode, decreasing with increasing doping density and annealing temperature. The inclusion of MgO leads to higher thermal stability of the tunnelling diodes. The measured contact resistance values are discussed with respect to the conductivity mismatch for spin injection and detection.

  5. Proximity Band Structure and Spin Textures on Both Sides of Topological-Insulator/Ferromagnetic-Metal Interface and Their Charge Transport Probes.

    Science.gov (United States)

    Marmolejo-Tejada, Juan Manuel; Dolui, Kapildeb; Lazić, Predrag; Chang, Po-Hao; Smidstrup, Søren; Stradi, Daniele; Stokbro, Kurt; Nikolić, Branislav K

    2017-09-13

    The control of recently observed spintronic effects in topological-insulator/ferromagnetic-metal (TI/FM) heterostructures is thwarted by the lack of understanding of band structure and spin textures around their interfaces. Here we combine density functional theory with Green's function techniques to obtain the spectral function at any plane passing through atoms of Bi 2 Se 3 and Co or Cu layers comprising the interface. Instead of naively assumed Dirac cone gapped by the proximity exchange field spectral function, we find that the Rashba ferromagnetic model describes the spectral function on the surface of Bi 2 Se 3 in contact with Co near the Fermi level E F 0 , where circular and snowflake-like constant energy contours coexist around which spin locks to momentum. The remnant of the Dirac cone is hybridized with evanescent wave functions from metallic layers and pushed, due to charge transfer from Co or Cu layers, a few tenths of an electron-volt below E F 0 for both Bi 2 Se 3 /Co and Bi 2 Se 3 /Cu interfaces while hosting distorted helical spin texture wounding around a single circle. These features explain recent observation of sensitivity of spin-to-charge conversion signal at TI/Cu interface to tuning of E F 0 . Crucially for spin-orbit torque in TI/FM heterostructures, few monolayers of Co adjacent to Bi 2 Se 3 host spectral functions very different from the bulk metal, as well as in-plane spin textures (despite Co magnetization being out-of-plane) due to proximity spin-orbit coupling in Co induced by Bi 2 Se 3 . We predict that out-of-plane tunneling anisotropic magnetoresistance in Cu/Bi 2 Se 3 /Co vertical heterostructure can serve as a sensitive probe of the type of spin texture residing at E F 0 .

  6. Spin-label Order Parameter Calibrations for Slow Motion

    DEFF Research Database (Denmark)

    Marsh, Derek

    2018-01-01

    Calibrations are given to extract orientation order parameters from pseudo-powder electron paramagnetic resonance line shapes of 14N-nitroxide spin labels undergoing slow rotational diffusion. The nitroxide z-axis is assumed parallel to the long molecular axis. Stochastic-Liouville simulations...... (Formula presented.) which characterizes fluctuations of the long molecular axis. This results in empirical expressions for order parameter and isotropic hyperfine coupling: (Formula presented.) and (Formula presented.), respectively. Values of the calibration constants (Formula presented.), (Formula...... presented.), (Formula presented.), (Formula presented.) and (Formula presented.) are given for different values of (Formula presented.) in fast and slow motional regimes. The calibrations are relatively insensitive to anisotropy of rotational diffusion (Formula presented.), and corrections are less...

  7. Static critical exponents of the ferromagnetic transition in spin glass re-entrant systems.

    Science.gov (United States)

    Haetinger, Cláudia M; Ghivelder, Luis; Schaf, Jacob; Pureur, Paulo

    2009-12-16

    The static critical phenomenology near the Curie temperature of the re-entrant metallic alloys Au(0.81)Fe(0.19), Ni(0.78)Mn(0.22), Ni(0.79)Mn(0.21) and amorphous a-Fe(0.98)Zr(0.08) is studied using a variety of experimental techniques and methods of analysis. We have generally found that the values for the exponents α, β, γ and δ depart significantly from the predictions for the 3D Heisenberg model and are intermediate between these expectations and the values characterizing a typical spin glass transition. Comparing the exponents obtained in our work with indices for other re-entrant systems reported in the literature, a weak universality class may be defined where the exponents are distributed within a certain range around average values.

  8. Quantum spin-glass transition in the two-dimensional electron gas

    Indian Academy of Sciences (India)

    An average ferromagnetic moment may also be present, and the spin-glass order then resides in the plane orthogonal to the ferromagnetic moment. We argue that a quantum transition involving the destruction of the spin-glass order in an applied in-plane magnetic field offers a natural explanation of some features of recent ...

  9. Mutual influence between macrospin reversal order and spin-wave dynamics in isolated artificial spin-ice vertices

    Science.gov (United States)

    Montoncello, F.; Giovannini, L.; Bang, Wonbae; Ketterson, J. B.; Jungfleisch, M. B.; Hoffmann, A.; Farmer, B. W.; De Long, L. E.

    2018-01-01

    We theoretically and experimentally investigate magnetization reversal and associated spin-wave dynamics of isolated threefold vertices that constitute a Kagome lattice. The three permalloy macrospins making up the vertex have an elliptical cross section and a uniform thickness. We study the dc magnetization curve and the frequency versus field curves (dispersions) of those spin-wave modes that produce the largest response. We also investigate each macrospin reversal from a dynamic perspective, by performing micromagnetic simulations of the reversal processes, and revealing their relationships to the soft-mode profile calculated at the equilibrium state immediately before reversal. The theoretical results are compared with the measured magnetization curves and ferromagnetic resonance spectra. The agreement achieved suggests that a much deeper understanding of magnetization reversal and accompanying hysteresis can be achieved by combining theoretical calculations with static and dynamic magnetization experiments.

  10. Topological order in an exactly solvable 3D spin model

    International Nuclear Information System (INIS)

    Bravyi, Sergey; Leemhuis, Bernhard; Terhal, Barbara M.

    2011-01-01

    Research highlights: RHtriangle We study exactly solvable spin model with six-qubit nearest neighbor interactions on a 3D face centered cubic lattice. RHtriangle The ground space of the model exhibits topological quantum order. RHtriangle Elementary excitations can be geometrically described as the corners of rectangular-shaped membranes. RHtriangle The ground space can encode 4g qubits where g is the greatest common divisor of the lattice dimensions. RHtriangle Logical operators acting on the encoded qubits are described in terms of closed strings and closed membranes. - Abstract: We study a 3D generalization of the toric code model introduced recently by Chamon. This is an exactly solvable spin model with six-qubit nearest-neighbor interactions on an FCC lattice whose ground space exhibits topological quantum order. The elementary excitations of this model which we call monopoles can be geometrically described as the corners of rectangular-shaped membranes. We prove that the creation of an isolated monopole separated from other monopoles by a distance R requires an operator acting on Ω(R 2 ) qubits. Composite particles that consist of two monopoles (dipoles) and four monopoles (quadrupoles) can be described as end-points of strings. The peculiar feature of the model is that dipole-type strings are rigid, that is, such strings must be aligned with face-diagonals of the lattice. For periodic boundary conditions the ground space can encode 4g qubits where g is the greatest common divisor of the lattice dimensions. We describe a complete set of logical operators acting on the encoded qubits in terms of closed strings and closed membranes.

  11. Coexistence of ferromagnetic and antiferromagnetic orders in Ba-doped cobalt perovskites studied by neutron scattering

    Science.gov (United States)

    Cao, Huibo; Wang, Fangwei; Garlea, Vasile; Gukasov, Arsen; Cheng, Zhaohua

    2011-03-01

    Cobalt-containing oxide compounds have attracted a great deal of interest in recent years due to the variety of magnetic and electrical properties. We performed single crystal neutron diffraction on 6T2 at~the~LLB in France and~the~HB3A four-circle diffractometor at~the~HFIR of ORNL. The Ba-doped cobalt perovskite (La 0.8 Ba 0.2 Co O3) crystal was measured in the temperature range of 2-250 K. At temperature T < 200 K, a set of ferromagnetic peaks (k1 = 0) onsets and then antiferromagnetic peaks with k2 * = (1 / 2 0 1 / 2) and (0 0 3 / 2) join in at T < 100 K . Both ferromagnetic and antiferromagnetic peaks saturate at T ~ 40 K . By refining the peaks collected for k1 and k2 sets, magnetic structures were determined. This research is supported by UT Battelle, LLC, Contract DE-AC05-00OR22725 for U.S. D.O.E., and the National Basic Research Program of China (973 Program, 2010CB833102).

  12. Intrinsic quantum spin Hall and anomalous Hall effects in h-Sb/Bi epitaxial growth on a ferromagnetic MnO2 thin film.

    Science.gov (United States)

    Zhou, Jian; Sun, Qiang; Wang, Qian; Kawazoe, Yoshiyuki; Jena, Puru

    2016-06-07

    Exploring a two-dimensional intrinsic quantum spin Hall state with a large band gap as well as an anomalous Hall state in realizable materials is one of the most fundamental and important goals for future applications in spintronics, valleytronics, and quantum computing. Here, by combining first-principles calculations with a tight-binding model, we predict that Sb or Bi can epitaxially grow on a stable and ferromagnetic MnO2 thin film substrate, forming a flat honeycomb sheet. The flatness of Sb or Bi provides an opportunity for the existence of Dirac points in the Brillouin zone, with its position effectively tuned by surface hydrogenation. The Dirac points in spin up and spin down channels split due to the proximity effects induced by MnO2. In the presence of both intrinsic and Rashba spin-orbit coupling, we find two band gaps exhibiting a large band gap quantum spin Hall state and a nearly quantized anomalous Hall state which can be tuned by adjusting the Fermi level. Our findings provide an efficient way to realize both quantized intrinsic spin Hall conductivity and anomalous Hall conductivity in a single material.

  13. The influence of the spin-dependent phases of tunneling electrons on the conductance of a point ferromagnet/isolator/d-wave superconductor contact.

    Science.gov (United States)

    Vodopyanov, B P

    2010-05-12

    The influence of the spin-dependent phase shifts (SDPSs) associated with the electronic reflection and transmission amplitudes acquired by electrons upon scattering at the potential barrier on the Andreev reflection probability of electron and hole excitations for a ferromagnet/isolator/d-wave superconductor (FIS) contact and on the charge conductance of the FIS contact is studied. Various superconductor orientations are considered. It has been found that for strong ferromagnets and ultrathin interface potential for the {110} oriented d-wave superconductor the presence of the SDPS can lead to the appearance of finite-voltage peaks in the charge conductance of the F/I/d-wave superconductor contact. On the contrary, for the {100} orientation of the d-wave superconductor the presence of the SDPS can lead to restoration of the zero-voltage peak and suppression of finite-voltage peaks. The spin-dependent amplitudes of the Andreev reflection probability and energy levels of the spin-dependent Andreev bound states are found.

  14. Soft mode and energy gap in spin wave spectrum for a second order orientation phase transition. AFMR in YFe3

    International Nuclear Information System (INIS)

    Balbashov, A.M.; Berezin, A.G.; Gufan, Yu.M.; Kolyadko, G.S.; Marchukov, P.Yu.; Rudashevskij, E.G.

    1987-01-01

    A pronounced energy gap of a nonmagnetoelastic origin is observed experimentally in the spectrum of the low-frequency (quasiferromagnetic) antiferromagnetic resonance branch during a second order spin-flip phase transition in an external magnetic field directed along the a axis of the rhombic weak ferromagnetic YFeO 3 . From the theory developed which takes into account the susceptibility along the antiferromagnetism axis and dissipation processes, it follows that beside the usual AFMR oscillatory branches there should also be a relaxation mode which is ''soft'' fo the given transition. The magnitude of the energy gaps, the values of the kinetic coefficients, Dzyaloshinsky field strengths and ratio of the longitudinal susceptibility to the transverse susceptibility are determined by analyzing the experimental data obtained in fields up to 130 kOe in the frequency range from 60 to 400 GHz at room temperature

  15. Novel room temperature ferromagnetic semiconductors

    Energy Technology Data Exchange (ETDEWEB)

    Gupta, Amita [KTH Royal Inst. of Technology, Stockholm (Sweden)

    2004-06-01

    Today's information world, bits of data are processed by semiconductor chips, and stored in the magnetic disk drives. But tomorrow's information technology may see magnetism (spin) and semiconductivity (charge) combined in one 'spintronic' device that exploits both charge and 'spin' to carry data (the best of two worlds). Spintronic devices such as spin valve transistors, spin light emitting diodes, non-volatile memory, logic devices, optical isolators and ultra-fast optical switches are some of the areas of interest for introducing the ferromagnetic properties at room temperature in a semiconductor to make it multifunctional. The potential advantages of such spintronic devices will be higher speed, greater efficiency, and better stability at a reduced power consumption. This Thesis contains two main topics: In-depth understanding of magnetism in Mn doped ZnO, and our search and identification of at least six new above room temperature ferromagnetic semiconductors. Both complex doped ZnO based new materials, as well as a number of nonoxides like phosphides, and sulfides suitably doped with Mn or Cu are shown to give rise to ferromagnetism above room temperature. Some of the highlights of this work are discovery of room temperature ferromagnetism in: (1) ZnO:Mn (paper in Nature Materials, Oct issue, 2003); (2) ZnO doped with Cu (containing no magnetic elements in it); (3) GaP doped with Cu (again containing no magnetic elements in it); (4) Enhancement of Magnetization by Cu co-doping in ZnO:Mn; (5) CdS doped with Mn, and a few others not reported in this thesis. We discuss in detail the first observation of ferromagnetism above room temperature in the form of powder, bulk pellets, in 2-3 mu-m thick transparent pulsed laser deposited films of the Mn (<4 at. percent) doped ZnO. High-resolution transmission electron microscopy (HRTEM) and electron energy loss spectroscopy (EELS) spectra recorded from 2 to 200nm areas showed homogeneous

  16. Long-range spin-singlet proximity effect for a Josephson system with a single-crystal ferromagnet due to its band-structure features

    Science.gov (United States)

    Avdeev, M. V.; Proshin, Yu. N.

    2018-03-01

    A possible explanation for the long-range proximity effect observed in single-crystalline cobalt nanowires sandwiched between two tungsten superconducting electrodes [Nat. Phys. 6, 389 (2010), 10.1038/nphys1621] is proposed. The theoretical model uses properties of a ferromagnet band structure. Specifically, to connect the exchange field with the momentum of quasiparticles the distinction between the effective masses in majority and minority spin subbands and the Fermi-surface anisotropy are considered. The derived Eilenberger-like equations allowed us to obtain a renormalized exchange interaction that is completely compensated for some crystallographic directions under certain conditions. The proposed theoretical model is compared with previous approaches.

  17. Proton spin in leading order of the covariant approach

    Czech Academy of Sciences Publication Activity Database

    Závada, Petr

    2014-01-01

    Roč. 88, č. 1 (2014), "014012-1"-"014012-16" ISSN 1550-7998 R&D Projects: GA MŠk(CZ) LG13031 Institutional support: RVO:68378271 Keywords : proton spin * spin structure functions * covariant quark-parton model Subject RIV: BF - Elementary Particles and High Energy Physics Impact factor: 4.643, year: 2014

  18. Spin waves and the order-disorder transition in chromium

    DEFF Research Database (Denmark)

    Als-Nielsen, Jens Aage; Dietrich, O.W.

    1969-01-01

    The inelastic magnetic scattering of neutrons has been studied in Cr and Cr0.95-Mn0.05 both below and above the Neel temperature. The temperature dependence of the spin-wave velocity in the alloy has been measured below TN. The scattering above TN may also be interpreted in terms of spin-wavelike...

  19. Topological order in an exactly solvable 3D spin model

    Science.gov (United States)

    Bravyi, Sergey; Leemhuis, Bernhard; Terhal, Barbara M.

    2011-04-01

    We study a 3D generalization of the toric code model introduced recently by Chamon. This is an exactly solvable spin model with six-qubit nearest-neighbor interactions on an FCC lattice whose ground space exhibits topological quantum order. The elementary excitations of this model which we call monopoles can be geometrically described as the corners of rectangular-shaped membranes. We prove that the creation of an isolated monopole separated from other monopoles by a distance R requires an operator acting on Ω( R2) qubits. Composite particles that consist of two monopoles (dipoles) and four monopoles (quadrupoles) can be described as end-points of strings. The peculiar feature of the model is that dipole-type strings are rigid, that is, such strings must be aligned with face-diagonals of the lattice. For periodic boundary conditions the ground space can encode 4 g qubits where g is the greatest common divisor of the lattice dimensions. We describe a complete set of logical operators acting on the encoded qubits in terms of closed strings and closed membranes.

  20. Relativistic spin-polarized KKR theory for superconducting heterostructures: Oscillating order parameter in the Au layer of Nb/Au/Fe trilayers

    Science.gov (United States)

    Csire, Gábor; Deák, András; Nyári, Bendegúz; Ebert, Hubert; Annett, James F.; Újfalussy, Balázs

    2018-01-01

    The fully relativistic spin-polarized multiple-scattering theory is developed for inhomogeneous superconductors, including superconducting/normal-metal/ferromagnet heterostructures. The method allows the solution of the first-principles Dirac-Bogoliubov-de Gennes equations combined with a semiphenomenological parametrization of the exchange-correlation functional. Simple conditions are derived for the case when the right-hand-side and left-hand-side solutions must be treated separately when setting up the corresponding Green's function. As an application of the theory, we calculate the order parameters of Nb/Fe and Nb/Au/Fe systems. We find Fulde-Ferrell-Larkin-Ovchinnikov-like oscillations in the iron layers, but more interestingly an oscillatory behavior is observed in the gold layers as well. The band-structure calculations suggest that this is the consequence of an interplay between the quantum-well states and ferromagnetism.

  1. Coexistence of ferromagnetism and superconductivity in iron based pnictides: a time resolved magnetooptical study.

    Science.gov (United States)

    Pogrebna, A; Mertelj, T; Vujičić, N; Cao, G; Xu, Z A; Mihailovic, D

    2015-01-13

    Ferromagnetism and superconductivity are antagonistic phenomena. Their coexistence implies either a modulated ferromagnetic order parameter on a lengthscale shorter than the superconducting coherence length or a weak exchange coupling between the itinerant superconducting electrons and the localized ordered spins. In some iron based pnictide superconductors the coexistence of ferromagnetism and superconductivity has been clearly demonstrated. The nature of the coexistence, however, remains elusive since no clear understanding of the spin structure in the superconducting state has been reached and the reports on the coupling strength are controversial. We show, by a direct optical pump-probe experiment, that the coupling is weak, since the transfer of the excess energy from the itinerant electrons to ordered localized spins is much slower than the electron-phonon relaxation, implying the coexistence without the short-lengthscale ferromagnetic order parameter modulation. Remarkably, the polarization analysis of the coherently excited spin wave response points towards a simple ferromagnetic ordering of spins with two distinct types of ferromagnetic domains.

  2. Leading order finite size effects with spins for inspiralling compact binaries

    International Nuclear Information System (INIS)

    Levi, Michele; Steinhoff, Jan

    2015-01-01

    The leading order finite size effects due to spin, namely that of the cubic and quartic in spin interactions, are derived for the first time for generic compact binaries via the effective field theory for gravitating spinning objects. These corrections enter at the third and a half and fourth post-Newtonian orders, respectively, for rapidly rotating compact objects. Hence, we complete the leading order finite size effects with spin up to the fourth post-Newtonian accuracy. We arrive at this by augmenting the point particle effective action with new higher dimensional nonminimal coupling worldline operators, involving higher-order derivatives of the gravitational field, and introducing new Wilson coefficients, corresponding to constants, which describe the octupole and hexadecapole deformations of the object due to spin. These Wilson coefficients are fixed to unity in the black hole case. The nonminimal coupling worldline operators enter the action with the electric and magnetic components of the Weyl tensor of even and odd parity, coupled to even and odd worldline spin tensors, respectively. Moreover, the non relativistic gravitational field decomposition, which we employ, demonstrates a coupling hierarchy of the gravito-magnetic vector and the Newtonian scalar, to the odd and even in spin operators, respectively, which extends that of minimal coupling. This observation is useful for the construction of the Feynman diagrams, and provides an instructive analogy between the leading order spin-orbit and cubic in spin interactions, and between the leading order quadratic and quartic in spin interactions.

  3. Singlet-Triplet Conversion and the Long-Range Proximity Effect in Superconductor-Ferromagnet Structures with Generic Spin Dependent Fields

    Science.gov (United States)

    Bergeret, F. S.; Tokatly, I. V.

    2013-03-01

    The long-range proximity effect in superconductor-ferromagnet (S/F) hybrid nanostructures is observed if singlet Cooper pairs from the superconductor are converted into triplet pairs which can diffuse into the ferromagnet over large distances. It is commonly believed that this happens only in the presence of magnetic inhomogeneities. We show that there are other sources of the long-range triplet component (LRTC) of the condensate and establish general conditions for their occurrence. As a prototypical example, we consider first a system where the exchange field and spin-orbit coupling can be treated as time and space components of an effective SU(2) potential. We derive a SU(2) covariant diffusive equation for the condensate and demonstrate that an effective SU(2) electric field is responsible for the long-range proximity effect. Finally, we extend our analysis to a generic ferromagnet and establish a universal condition for the LRTC. Our results open a new avenue in the search for such correlations in S/F structures and make a hitherto unknown connection between the LRTC and Yang-Mills electrostatics.

  4. Proximity effects in ferromagnet/superconductor structures

    International Nuclear Information System (INIS)

    Yu, H.L.; Sun, G.Y.; Yang, L.Y.; Xing, D.Y.

    2004-01-01

    The Nambu spinor Green's function approach is applied to study proximity effects in ferromagnet/superconductor (FM/SC) structures. They include the induced superconducting order parameter and density of states (DOS) with superconducting feature on the FM side, and spin-dependent DOS within the energy gap on the SC side. The latter indicates an appearance of gapless superconductivity and a coexistence of ferromagnetism and superconductivity in a small regime near the interface. The influence of exchange energy in FM and barrier strength at interface on the proximity effects is discussed

  5. Atom and Amine Adsorption on Flat and Stepped Gold Surfaces & Structure, Stability and Spin Ordering in Manganese Sulfide Clusters

    Science.gov (United States)

    Lewoczko, April D.

    In part I, we investigate gold catalysis in the chemistry of organonitrogen compounds. We examine the adsorption of oxygen, nitrogen and sulfur atoms on the gold (111), (100) and (211) surfaces using density functional theory (DFT). Sulfur atoms bind most strongly, followed by oxygen and nitrogen atoms with stronger adsorption for greater coordination to the surface. We see a trend of stronger adsorption to undercoordinated gold, but find it is non-universal with the adsorption strength trend: (111) > (211) > (100). We consider the diffusion of oxygen, nitrogen and sulfur adatoms and find facile long-range diffusion of oxygen atoms on the (100) surface. Lastly, we compare the adsorption of methylamine on gold to that of a selection of alkylamines, methanol and methanethiol. In each case, the ontop site is preferred with stronger adsorption at low coordinated gold. At oxygen atom coverages of 0.125 -- 0.25 ML on Au (111), we find cooperative adsorption of methylamine and oxygen atoms. Energetic costs for adsorbate tilt from the surface normal and rotation about the gold-nitrogen bond are calculated. While methylamine rotation is barrierless on the (111) and (211) surfaces, it has a low energetic barrier for the 0.125 ML and 0.25 ML O atom pre-covered Au (111) surfaces. In part II, we interpret the experimental mass spectrum of small gas phase manganese sulfide clusters using DFT and elucidate the role of ionicity and spin ordering in sizes with special stability, i.e. magic clusters. We first consider nine low lying minima (MnS)6 structures and reveal antiferromagnetic (AFM) spin ordering with a ˜0.1 eV/pair AFM energy benefit and a ˜0.1 A shrinkage of average Mn-Mn distances over clusters with ferromagnetic (FM) spin ordering. We calculate energetic barriers for interconversion between the two lowest lying (MnS)6 isomers and predict an elevated cluster melting temperature due to increased configurational entropy in a pre-melted state. Second, we demonstrate the

  6. Theory for spin and orbital orderings in high temperature phase in $YVO_3$

    OpenAIRE

    De Silva, Theja N.; Joshi, Anuvrat; Ma, Michael; Zhang, Fu Chun

    2003-01-01

    Motivated by the recent neutron diffraction experiment on $YVO_3$, we consider a microscopic model where each $V^{3+}$ ion is occupied by two 3d electrons of parallel spins with two fold degenerate orbital configurations. The mean field classical solutions of the spin-orbital superexchange model predicts an antiferro-orbital ordering at a higher temperature followed by a C-type antiferromagnetic spin ordering at a lower temperature. Our results are qualitatively consistent with the observed o...

  7. Pressure and field induced magnetic order in the spin liquid Tb2Ti2O7 as studied by single crystal neutron diffraction.

    Science.gov (United States)

    Mirebeau, I; Goncharenko, I N; Dhalenne, G; Revcolevschi, A

    2004-10-29

    We have studied the spin liquid Tb2Ti2O7 by single crystal neutron diffraction under high pressure up to 2.8 GPa, together with uniaxial stress, down to 0.1 K, in zero and high magnetic fields up to 7 T. In zero magnetic field, a long-range ordered antiferromagnetic structure is induced by pressure. The Néel temperature and ordered magnetic moment can be tuned by the anisotropic pressure component. Under magnetic field, the antiferromagnetic structure transforms into a canted ferromagnetic one at 0.6 T. Spin canting persists even at 7 T. The magnetic phase diagram under pressure shows a strong increase of the Néel temperature with the field.

  8. Pressure and field induced magnetic order in the spin liquid Tb2Ti2O7 as studied by single crystal neutron diffraction

    International Nuclear Information System (INIS)

    Mirebeau, I.; Goncharenko, I. N.; Dhalenne, G.; Revcolevschi, A.

    2004-01-01

    We have studied the spin liquid Tb 2 Ti 2 O 7 by single crystal neutron diffraction under high pressure up to 2.8 GPa, together with uniaxial stress, down to 0.1 K, in zero and high magnetic fields up to 7 T. In zero magnetic field, a long-range ordered antiferromagnetic structure is induced by pressure. The Neel temperature and ordered magnetic moment can be tuned by the anisotropic pressure component. Under magnetic field, the antiferromagnetic structure transforms into a canted ferromagnetic one at 0.6 T. Spin canting persists even at 7 T. The magnetic phase diagram under pressure shows a strong increase of the Neel temperature with the field

  9. Josephson tunnel junctions with ferromagnetic interlayer

    Energy Technology Data Exchange (ETDEWEB)

    Weides, M.P.

    2006-07-01

    Superconductivity and ferromagnetism are well-known physical properties of solid states that have been widely studied and long thought about as antagonistic phenomena due to difference in spin ordering. It turns out that the combination of both superconductor and ferromagnet leads to a very rich and interesting physics. One particular example, the phase oscillations of the superconducting order parameter inside the ferromagnet, will play a major role for the devices discussed in this work. In this thesis, I present Josephson junctions with a thin Al{sub 2}O{sub 3} tunnel barrier and a ferromagnetic interlayer, i.e. superconductor-insulator-ferromagnet-superconductor (SIFS) stacks. The fabrication of junctions was optimized regarding the insulation of electrodes and the homogeneity of the current transport. The junctions were either in the 0 or {pi} coupled ground state, depending on the thickness of the ferromagnetic layer and on temperature. The influence of ferromagnetic layer thickness on the transport properties and the coupling (0, {pi}) of SIFS tunnel junctions was studied. Furthermore, using a stepped ferromagnetic layer with well-chosen thicknesses, I obtained the so-called 0-{pi} Josephson junction. At a certain temperature this 0-{pi} junction can be made perfectly symmetric. In this case the ground state corresponds to a vortex of supercurrent creating a magnetic flux which is a fraction of the magnetic flux quantum {phi}{sub 0}. Such structures allow to study the physics of fractional vortices and to build various electronic circuits based on them. The SIFS junctions presented here have an exponentially vanishing damping at T {yields} 0. The SIFS technology developed within the framework of this work may be used to construct classical and quantum devices such as oscillators, memory cells and qubits. (orig.)

  10. Emergence of chiral spin liquids via quantum melting of noncoplanar magnetic orders

    Science.gov (United States)

    Hickey, Ciarán; Cincio, Lukasz; Papić, Zlatko; Paramekanti, Arun

    2017-09-01

    Quantum spin liquids (QSLs) are highly entangled states of quantum magnets which lie beyond the Landau paradigm of classifying phases of matter via broken symmetries. A physical route to arriving at QSLs is via frustration-induced quantum melting of ordered states such as valence bond crystals or magnetic orders. Here we show, using extensive exact diagonalization (ED) and density-matrix renormalization group (DMRG) studies of concrete S U (2 ) invariant spin models on honeycomb, triangular, and square lattices, that chiral spin liquids (CSLs) emerge as descendants of triple-Q spin crystals with tetrahedral magnetic order and a large scalar spin chirality. Such ordered-to-CSL melting transitions may yield lattice realizations of effective Chern-Simons-Higgs field theories. Our work provides a distinct unifying perspective on the emergence of CSLs and suggests that materials with certain noncoplanar magnetic orders might provide a good starting point to search for CSLs.

  11. Complementary Response of Static Spin-Stripe Order and Superconductivity to Nonmagnetic Impurities in Cuprates

    Science.gov (United States)

    Guguchia, Z.; Roessli, B.; Khasanov, R.; Amato, A.; Pomjakushina, E.; Conder, K.; Uemura, Y. J.; Tranquada, J. M.; Keller, H.; Shengelaya, A.

    2017-08-01

    We report muon-spin rotation and neutron-scattering experiments on nonmagnetic Zn impurity effects on the static spin-stripe order and superconductivity of the La214 cuprates. Remarkably, it was found that, for samples with hole doping x ≈1 /8 , the spin-stripe ordering temperature Tso decreases linearly with Zn doping y and disappears at y ≈4 %, demonstrating a high sensitivity of static spin-stripe order to impurities within a CuO2 plane. Moreover, Tso is suppressed by Zn in the same manner as the superconducting transition temperature Tc for samples near optimal hole doping. This surprisingly similar sensitivity suggests that the spin-stripe order is dependent on intertwining with superconducting correlations.

  12. Recoil velocity at second post-Newtonian order for spinning black hole binaries

    International Nuclear Information System (INIS)

    Racine, Etienne; Buonanno, Alessandra; Kidder, Larry

    2009-01-01

    We compute the flux of linear momentum carried by gravitational waves emitted from spinning binary black holes at second post-Newtonian (2PN) order for generic orbits. In particular we provide explicit expressions of three new types of terms, namely, next-to-leading order spin-orbit terms at 1.5 post-Newtonian (1.5PN) order, spin-orbit tail terms at 2PN order, and spin-spin terms at 2PN order. Restricting ourselves to quasicircular orbits, we integrate the linear-momentum flux over time to obtain the recoil velocity as function of orbital frequency. We find that in the so-called superkick configuration the higher-order spin corrections can increase the recoil velocity up to a factor ∼3 with respect to the leading-order PN prediction. Whereas the recoil velocity computed in PN theory within the adiabatic approximation can accurately describe the early inspiral phase, we find that its fast increase during the late inspiral and plunge, and the arbitrariness in determining until when it should be trusted, makes the PN predictions for the total recoil not very accurate and robust. Nevertheless, the linear-momentum flux at higher PN orders can be employed to build more reliable resummed expressions aimed at capturing the nonperturbative effects until merger. Furthermore, we provide expressions valid for generic orbits, and accurate at 2PN order, for the energy and angular momentum carried by gravitational waves emitted from spinning binary black holes. Specializing to quasicircular orbits we compute the spin-spin terms at 2PN order in the expression for the evolution of the orbital frequency and found agreement with Mikoczi, Vasuth, and Gergely. We also verified that in the limit of extreme mass ratio our expressions for the energy and angular momentum fluxes match the ones of Tagoshi, Shibata, Tanaka, and Sasaki obtained in the context of black hole perturbation theory.

  13. Sign of inverse spin Hall voltages generated by ferromagnetic resonance and temperature gradients in yttrium iron garnet platinum bilayers

    International Nuclear Information System (INIS)

    Schreier, Michael; Lotze, Johannes; Gross, Rudolf; Goennenwein, Sebastian T B; Bauer, Gerrit E W; Uchida, Ken-ichi; Daimon, Shunsuke; Kikkawa, Takashi; Saitoh, Eiji; Vasyuchka, Vitaliy I; Lauer, Viktor; Chumak, Andrii V; Serga, Alexander A; Hillebrands, Burkard; Flipse, Joost; Van Wees, Bart J

    2015-01-01

    We carried out a concerted effort to determine the absolute sign of the inverse spin Hall effect voltage generated by spin currents injected into a normal metal. We focus on yttrium iron garnet (YIG)∣platinum bilayers at room temperature, generating spin currents by microwaves and temperature gradients. We find consistent results for different samples and measurement setups that agree with theory. We suggest a right-hand-rule to define a positive spin Hall angle corresponding to the voltage expected for the simple case of scattering of free electrons from repulsive Coulomb charges. (paper)

  14. Electrical tuning of the band alignment and magnetoconductance in an n-type ferromagnetic semiconductor (In,Fe)As-based spin-Esaki diode

    Science.gov (United States)

    Anh, Le Duc; Hai, Pham Nam; Tanaka, Masaaki

    2018-03-01

    We report a strong bias dependence of the magnetoconductance (MC) of a spin-Esaki diode composed of n+-type ferromagnetic semiconductor (FMS) (In,Fe)As and p+-type Be doped InAs grown on a p+-InAs (001) substrate by molecular beam epitaxy. When the bias voltage V is increased above 450 mV in the forward bias, we found that the MC, measured at 3.5 K under a magnetic field H of 1 T in the in-plane [110] direction, changes its sign from positive to negative and its magnitude rises rapidly from 0.5% at V fluid model, we explain both the magnitude and the anisotropy of the MC based on the evolution of the spin-Esaki diode's band profile with V. This analysis provides insights into the density of states and spin-polarization of the conduction band and the Fe-related impurity band in n-type FMS (In,Fe)As.

  15. Spin injection from a normal metal into a mesoscopic superconductor

    Energy Technology Data Exchange (ETDEWEB)

    Wolf, Michael J.; Kolenda, Stefan [Institut fuer Nanotechnologie, KIT, 76021 Karlsruhe (Germany); Huebler, Florian [Institut fuer Nanotechnologie, KIT, 76021 Karlsruhe (Germany); Center for Functional Nanostructures, KIT, 76131 Karlsruhe (Germany); Institut fuer Festkoerperphysik, KIT, 76021 Karlsruhe (Germany); Loehneysen, Hilbert v. [Center for Functional Nanostructures, KIT, 76131 Karlsruhe (Germany); Institut fuer Festkoerperphysik, KIT, 76021 Karlsruhe (Germany); Physikalisches Institut, KIT, 76128 Karlsruhe (Germany); Beckmann, Detlef [Institut fuer Nanotechnologie, KIT, 76021 Karlsruhe (Germany); Center for Functional Nanostructures, KIT, 76131 Karlsruhe (Germany)

    2013-07-01

    We report on nonlocal transport in superconductor hybrid structures, with ferromagnetic as well as normal-metal tunnel junctions attached to the superconductor. In the presence of a strong Zeeman splitting of the density of states, both charge and spin imbalance is injected into the superconductor. While previous experiments demonstrated spin injection from ferromagnetic electrodes, we show that spin imbalance is also created for normal-metal injector contacts. Using the combination of ferromagnetic and normal-metal detectors allows us to directly discriminate between charge and spin injection, and demonstrate a complete separation of charge and spin imbalance. The relaxation length of the spin imbalance is of the order of several μm and is found to increase with a magnetic field, but is independent of temperature. We further discuss possible relaxation mechanisms for the explanation of the spin relaxation length.

  16. Spin reorientation and magnetoelastic properties of ferromagnetic T b1 -xN dxC o2 systems with a morphotropic phase boundary

    Science.gov (United States)

    Murtaza, Adil; Yang, Sen; Chang, Tieyan; Ghani, Awais; Khan, Muhammad Tahir; Zhang, Rui; Zhou, Chao; Song, Xiaoping; Suchomel, Matthew; Ren, Yang

    2018-03-01

    The spin reorientation (SR) and magnetoelastic properties of pseudobinary ferromagnetic T b1 -xN dxC o2 (0 ≤x ≤1.0 ) systems involving a morphotropic phase boundary (MPB) were studied by high-resolution synchrotron x-ray diffraction (XRD), magnetization, and magnetostriction measurements. The easy magnetization direction of the Laves phase lies along the 〈111 〉 axis with x 0.65 below Curie temperature (TC). The temperature-dependent magnetization curves showed SR; this can be explained by a two-sublattice model. Based on the synchrotron (XRD) and magnetization measurements, the SR phase diagram for a MPB composition of T b0.35N d0.65C o2 was obtained. Contrary to previously reported ferromagnetic systems involving MPB, the MPB composition of T b0.35N d0.65C o2 exhibits a low saturation magnetization (MS), indicating a compensation of the Tb and Nd magnetic moments at MPB. The anisotropic magnetostriction (λS) first decreased until x =0.8 and then continuously increased in the negative direction with further increase of Nd concentration. The decrease in magnetostriction can be attributed to the decrease of spontaneous magnetostriction λ111 and increase of λ100 with opposite sign to λ111. This paper indicates an anomalous type of MPB in the ferromagnetic T b1 -xN dxC o2 system and provides an active way to design novel functional materials with exotic properties.

  17. Observation of exchange bias and spin-glass-like ordering in ε-Fe2 ...

    Indian Academy of Sciences (India)

    glass-like ordering, that arises from the freezing of localized frustrated spins. Keywords. Nanoparticles; nitride; exchange bias; spin glass. PACS Nos 75.50.Lk; 75.50.Tt; 75.50.Bb. 1. Introduction. The 3d transition metal nitrides are not extensively studied since they are relatively less stable as compared to oxides due to their ...

  18. Orbital and spin moments in the ferromagnetic superconductor URhGe by x-ray magnetic circular dichroism

    Czech Academy of Sciences Publication Activity Database

    Wilhelm, F.; Sanchez, J.P.; Brison, J.P.; Aoki, D.; Shick, Alexander; Rogalev, A.

    2017-01-01

    Roč. 95, č. 23 (2017), s. 1-10, č. článku 235147. ISSN 2469-9950 R&D Projects: GA ČR GA15-07172S Institutional support: RVO:68378271 Keywords : ferromagnetic superconductors * density functional theory Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 3.836, year: 2016

  19. 89Y NMR observation of ferromagnetic and antiferromagnetic spin fluctuations in the collapsed tetragonal phase of YFe2(Ge,Si)2

    Science.gov (United States)

    Srpčič, J.; Jeglič, P.; Felner, I.; Lv, Bing; Chu, C. W.; Arčon, D.

    2017-11-01

    The surprising discovery of tripling the superconducting critical temperature of KFe2As2 at high pressures has led to an intriguing question of how the superconductivity in the collapsed tetragonal phase differs from that in the noncollapsed phases of Fe-based superconductors. Here we report a 89Y nuclear magnetic resonance study of YFe2GexSi2 -x compounds whose electronic structure is similar to that of iron-pnictide collapsed tetragonal phases already at ambient pressure. We find that Fe(Ge,Si) layers show ferromagnetic spin fluctuations, whereas the layers are coupled antiferromagnetically. Furthermore, localized moments attributed either to Fe interstitial or antisite defects may account for magnetic impurity pair-breaking effects, thus explaining the substantial variation of superconductivity among different YFe2Ge2 samples.

  20. Higher-order spin and charge dynamics in a quantum dot-lead hybrid system.

    Science.gov (United States)

    Otsuka, Tomohiro; Nakajima, Takashi; Delbecq, Matthieu R; Amaha, Shinichi; Yoneda, Jun; Takeda, Kenta; Allison, Giles; Stano, Peter; Noiri, Akito; Ito, Takumi; Loss, Daniel; Ludwig, Arne; Wieck, Andreas D; Tarucha, Seigo

    2017-09-22

    Understanding the dynamics of open quantum systems is important and challenging in basic physics and applications for quantum devices and quantum computing. Semiconductor quantum dots offer a good platform to explore the physics of open quantum systems because we can tune parameters including the coupling to the environment or leads. Here, we apply the fast single-shot measurement techniques from spin qubit experiments to explore the spin and charge dynamics due to tunnel coupling to a lead in a quantum dot-lead hybrid system. We experimentally observe both spin and charge time evolution via first- and second-order tunneling processes, and reveal the dynamics of the spin-flip through the intermediate state. These results enable and stimulate the exploration of spin dynamics in dot-lead hybrid systems, and may offer useful resources for spin manipulation and simulation of open quantum systems.

  1. A graphene solution to conductivity mismatch: spin injection from ferromagnetic metal/graphene tunnel contacts into silicon

    Science.gov (United States)

    van't Erve, Olaf

    2014-03-01

    New paradigms for spin-based devices, such as spin-FETs and reconfigurable logic, have been proposed and modeled. These devices rely on electron spin being injected, transported, manipulated and detected in a semiconductor channel. This work is the first demonstration on how a single layer of graphene can be used as a low resistance tunnel barrier solution for electrical spin injection into Silicon at room temperature. We will show that a FM metal / monolayer graphene contact serves as a spin-polarized tunnel barrier which successfully circumvents the classic metal / semiconductor conductivity mismatch issue for electrical spin injection. We demonstrate electrical injection and detection of spin accumulation in Si above room temperature, and show that the corresponding spin lifetimes correlate with the Si carrier concentration, confirming that the spin accumulation measured occurs in the Si and not in interface trap states. An ideal tunnel barrier should exhibit several key material characteristics: a uniform and planar habit with well-controlled thickness, minimal defect / trapped charge density, a low resistance-area product for minimal power consumption, and compatibility with both the FM metal and semiconductor, insuring minimal diffusion to/from the surrounding materials at temperatures required for device processing. Graphene, offers all of the above, while preserving spin injection properties, making it a compelling solution to the conductivity mismatch for spin injection into Si. Although Graphene is very conductive in plane, it exhibits poor conductivity perpendicular to the plane. Its sp2 bonding results in a highly uniform, defect free layer, which is chemically inert, thermally robust, and essentially impervious to diffusion. The use of a single monolayer of graphene at the Si interface provides a much lower RA product than any film of an oxide thick enough to prevent pinholes (1 nm). Our results identify a new route to low resistance-area product spin

  2. Phase transitions in spin systems with modulated order

    International Nuclear Information System (INIS)

    Coutinho Filho, M.D.

    1984-01-01

    Spin systems which may display modulated structures are treated. A layered Ising model with competing interactions between nearest and next-nearest layers in the presence of a magnetic field is studied. In the context of a mean-field approximation, the high-temperature region of the phase diagram is studied analytically. The Λ surface, separating the paramagnetic and the modulated phases, is bounded by two lines of tricritical points which join smoothly at the Lifshitz point and terminate at multicritical points, beyond which lines of critical and double critical end points are expected to appear. The low-temperature region is studied numerically. T-H phase diagrams, which exhibit a variety of modulated phases, for various values of the ratio of the strength of the competing interactions are constructed. A theoretical interpretation for the occurrence of a Lifshitz point in the field-temperature phase diagram of MnP is presented. These results, which are based on a X-Y localized spin Hamiltonian, are in qualitative agreement with recently reported experiments. In particular, asymptotic expressions are obtained for the phase boundaries, which meet tangentially at the Lifshitz point, and for some other thermodynamic quantities of interest, such as the longitudinal and transverse susceptibilities. (Author) [pt

  3. Spin Electronics

    Science.gov (United States)

    2003-08-01

    applications, a ferromagnetic metal may be used as a source of spin-polarized electronics to be injected into a semiconductor, a superconductor or a...physical phenomena in II-VI and III-V semiconductors. In II-VI systems, the Mn2+ ions act to boost the electron spin precession up to terahertz ...conductors, proximity effect between ferromagnets and superconductors , and the effects of spin injection on the physical properties of the

  4. Period-doubling bifurcation cascade observed in a ferromagnetic nanoparticle under the action of a spin-polarized current

    Energy Technology Data Exchange (ETDEWEB)

    Horley, Paul P., E-mail: paul.horley@cimav.edu.mx [Centro de Investigación en Materiales Avanzados, S.C. (CIMAV), Chihuahua/Monterrey, 120 Avenida Miguel de Cervantes, 31109 Chihuahua (Mexico); Kushnir, Mykola Ya. [Yuri Fedkovych Chernivtsi National University, 2 Kotsyubynsky str., 58012 Chernivtsi (Ukraine); Morales-Meza, Mishel [Centro de Investigación en Materiales Avanzados, S.C. (CIMAV), Chihuahua/Monterrey, 120 Avenida Miguel de Cervantes, 31109 Chihuahua (Mexico); Sukhov, Alexander [Institut für Physik, Martin-Luther Universität Halle-Wittenberg, 06120 Halle (Saale) (Germany); Rusyn, Volodymyr [Yuri Fedkovych Chernivtsi National University, 2 Kotsyubynsky str., 58012 Chernivtsi (Ukraine)

    2016-04-01

    We report on complex magnetization dynamics in a forced spin valve oscillator subjected to a varying magnetic field and a constant spin-polarized current. The transition from periodic to chaotic magnetic motion was illustrated with bifurcation diagrams and Hausdorff dimension – the methods developed for dissipative self-organizing systems. It was shown that bifurcation cascades can be obtained either by tuning the injected spin-polarized current or by changing the magnitude of applied magnetic field. The order–chaos transition in magnetization dynamics can be also directly observed from the hysteresis curves. The resulting complex oscillations are useful for development of spin-valve devices operating in harmonic and chaotic modes.

  5. First-principles study of spin-polarized electronic band structures in ferromagnetic Zn1-xTMxS (TM = Fe, Co and Ni)

    KAUST Repository

    Saeed, Yasir

    2010-10-01

    We report a first-principles study of structural, electronic and magnetic properties of crystalline alloys Zn1-xTMxS (TM = Fe, Co and Ni) at x = 0.25. Structural properties are computed from the total ground state energy convergence and it is found that the cohesive energies of Zn 1-xTMxS are greater than that of zincblende ZnS. We also study the spin-polarized electronic band structures, total and partial density of states and the effect of TM 3d states. Our results exhibit that Zn 0.75Fe0.25S, Zn0.75Co0.25S and Zn0.75Ni0.25S are half-metallic ferromagnetic with a magnetic moment of 4μB, 3μB and 2μB, respectively. Furthermore, we calculate the TM 3d spin-exchange-splitting energies Δx (d), Δx (x-d), exchange constants N0α and N0β, crystal field splitting (ΔEcrystEt2g-Eeg), and find that p-d hybridization reduces the local magnetic moment of TM from its free space charge value. Moreover, robustness of Zn1-xTMxS with respect to the variation of lattice constants is also discussed. © 2010 Elsevier B.V. All rights reserved.

  6. Multicritical phase diagrams of the ferromagnetic spin-3/2 Blume-Emery-Griffiths model with repulsive biquadratic coupling including metastable phases: The cluster variation method and the path probability method with the point distribution

    Energy Technology Data Exchange (ETDEWEB)

    Keskin, Mustafa [Department of Physics, Erciyes University, 38039 Kayseri (Turkey)], E-mail: keskin@erciyes.edu.tr; Canko, Osman [Department of Physics, Erciyes University, 38039 Kayseri (Turkey)

    2008-01-15

    We study the thermal variations of the ferromagnetic spin-3/2 Blume-Emery-Griffiths (BEG) model with repulsive biquadratic coupling by using the lowest approximation of the cluster variation method (LACVM) in the absence and presence of the external magnetic field. We obtain metastable and unstable branches of the order parameters besides the stable branches and phase transitions of these branches are investigated extensively. The classification of the stable, metastable and unstable states is made by comparing the free energy values of these states. We also study the dynamics of the model by using the path probability method (PPM) with the point distribution in order to make sure that we find and define the metastable and unstable branches of the order parameters completely and correctly. We present the metastable phase diagrams in addition to the equilibrium phase diagrams in the (kT/J, K/J) and (kT/J, D/J) planes. It is found that the metastable phase diagrams always exist at the low temperatures, which are consistent with experimental and theoretical works.

  7. Multicritical phase diagrams of the ferromagnetic spin-3/2 Blume-Emery-Griffiths model with repulsive biquadratic coupling including metastable phases: The cluster variation method and the path probability method with the point distribution

    International Nuclear Information System (INIS)

    Keskin, Mustafa; Canko, Osman

    2008-01-01

    We study the thermal variations of the ferromagnetic spin-3/2 Blume-Emery-Griffiths (BEG) model with repulsive biquadratic coupling by using the lowest approximation of the cluster variation method (LACVM) in the absence and presence of the external magnetic field. We obtain metastable and unstable branches of the order parameters besides the stable branches and phase transitions of these branches are investigated extensively. The classification of the stable, metastable and unstable states is made by comparing the free energy values of these states. We also study the dynamics of the model by using the path probability method (PPM) with the point distribution in order to make sure that we find and define the metastable and unstable branches of the order parameters completely and correctly. We present the metastable phase diagrams in addition to the equilibrium phase diagrams in the (kT/J, K/J) and (kT/J, D/J) planes. It is found that the metastable phase diagrams always exist at the low temperatures, which are consistent with experimental and theoretical works

  8. Spin-polarized charge transport in HgTe/CdTe quantum well topological insulator under a ferromagnetic metal strip

    Science.gov (United States)

    Wu, Zhenhua; Luo, Kun; Yu, Jiahan; Wu, Xiaobo; Lin, Liangzhong

    2018-02-01

    Electron tunneling through a single magnetic barrier in a HgTe topological insulator has been theoretically investigated. We find that the perpendicular magnetic field would not lead to spin-flip of the edge states due to the conservation of the angular moment. By tuning the magnetic field and the Fermi energy, the edge channels can be transited from switch-on states to switch-off states and the current from unpolarized states can be filtered to fully spin polarized states. These features offer us an efficient way to control charge/spin transport in a HgTe/CdTe quantum well, and pave a way to construct the nanoelectronic devices utilizing the topological edge states.

  9. Destabilization of Magnetic Order in a Dilute Kitaev Spin Liquid Candidate

    Science.gov (United States)

    Lampen-Kelley, P.; Banerjee, A.; Aczel, A. A.; Cao, H. B.; Stone, M. B.; Bridges, C. A.; Yan, J.-Q.; Nagler, S. E.; Mandrus, D.

    2017-12-01

    The insulating honeycomb magnet α -RuCl3 exhibits fractionalized excitations that signal its proximity to a Kitaev quantum spin liquid state; however, at T =0 , fragile long-range magnetic order arises from non-Kitaev terms in the Hamiltonian. Spin vacancies in the form of Ir3 + substituted for Ru are found to destabilize this long-range order. Neutron diffraction and bulk characterization of Ru1 -xIrxCl3 show that the magnetic ordering temperature is suppressed with increasing x , and evidence of zizag magnetic order is absent for x >0.3 . Inelastic neutron scattering demonstrates that the signature of fractionalized excitations is maintained over the full range of x investigated. The depleted lattice without magnetic order thus hosts a spin-liquid-like ground state that may indicate the relevance of Kitaev physics in the magnetically dilute limit of RuCl3 .

  10. Fracton topological order from nearest-neighbor two-spin interactions and dualities

    Science.gov (United States)

    Slagle, Kevin; Kim, Yong Baek

    2017-10-01

    Fracton topological order describes a remarkable phase of matter, which can be characterized by fracton excitations with constrained dynamics and a ground-state degeneracy that increases exponentially with the length of the system on a three-dimensional torus. However, previous models exhibiting this order require many-spin interactions, which may be very difficult to realize in a real material or cold atom system. In this work, we present a more physically realistic model which has the so-called X-cube fracton topological order [Vijay, Haah, and Fu, Phys. Rev. B 94, 235157 (2016), 10.1103/PhysRevB.94.235157] but only requires nearest-neighbor two-spin interactions. The model lives on a three-dimensional honeycomb-based lattice with one to two spin-1/2 degrees of freedom on each site and a unit cell of six sites. The model is constructed from two orthogonal stacks of Z2 topologically ordered Kitaev honeycomb layers [Kitaev, Ann. Phys. 321, 2 (2006), 10.1016/j.aop.2005.10.005], which are coupled together by a two-spin interaction. It is also shown that a four-spin interaction can be included to instead stabilize 3+1D Z2 topological order. We also find dual descriptions of four quantum phase transitions in our model, all of which appear to be discontinuous first-order transitions.

  11. A next-to-leading order QCD analysis of the spin structure function $g_1$

    CERN Document Server

    Adeva, B; Arik, E; Badelek, B; Bardin, G; Baum, G; Berglund, P; Betev, L; Birsa, R; De Botton, N R; Bradamante, Franco; Bravar, A; Bressan, A; Bültmann, S; Burtin, E; Crabb, D; Cranshaw, J; Çuhadar-Dönszelmann, T; Dalla Torre, S; Van Dantzig, R; Derro, B R; Deshpande, A A; Dhawan, S K; Dulya, C M; Eichblatt, S; Fasching, D; Feinstein, F; Fernández, C; Forthmann, S; Frois, Bernard; Gallas, A; Garzón, J A; Gilly, H; Giorgi, M A; von Goeler, E; Görtz, S; Gracia, G; De Groot, N; Grosse-Perdekamp, M; Haft, K; Von Harrach, D; Hasegawa, T; Hautle, P; Hayashi, N; Heusch, C A; Horikawa, N; Hughes, V W; Igo, G; Ishimoto, S; Iwata, T; Kabuss, E M; Kageya, T; Karev, A G; Kessler, H J; Ketel, T; Kiryluk, J; Kiselev, Yu F; Krämer, Dietrich; Krivokhizhin, V G; Kröger, W; Kukhtin, V V; Kurek, K; Kyynäräinen, J; Lamanna, M; Landgraf, U; Le Goff, J M; Lehár, F; de Lesquen, A; Lichtenstadt, J; Litmaath, M; Magnon, A; Mallot, G K; Marie, F; Martin, A; Martino, J; Matsuda, T; Mayes, B W; McCarthy, J S; Medved, K S; Meyer, W T; Van Middelkoop, G; Miller, D; Miyachi, Y; Mori, K; Moromisato, J H; Nassalski, J P; Naumann, Lutz; Niinikoski, T O; Oberski, J; Ogawa, A; Ozben, C; Pereira, H; Perrot-Kunne, F; Peshekhonov, V D; Piegia, R; Pinsky, L; Platchkov, S K; Pló, M; Pose, D; Postma, H; Pretz, J; Puntaferro, R; Rädel, G; Rijllart, A; Reicherz, G; Roberts, J; Rodríguez, M; Rondio, Ewa; Sabo, I; Saborido, J; Sandacz, A; Savin, I A; Schiavon, R P; Schiller, A; Sichtermann, E P; Simeoni, F; Smirnov, G I; Staude, A; Steinmetz, A; Stiegler, U; Stuhrmann, H B; Szleper, M; Tessarotto, F; Thers, D; Tlaczala, W; Tripet, A; Ünel, G; Velasco, M; Vogt, J; Voss, Rüdiger; Whitten, C; Windmolders, R; Willumeit, R; Wislicki, W; Witzmann, A; Ylöstalo, J; Zanetti, A M; Zaremba, K; Zhao, J

    1998-01-01

    We present a next-to-leading order QCD analysis of the presently available data on the spin structure function $g_1$ including the final data from the Spin Muon Collaboration (SMC). We present resu lts for the first moments of the proton, deuteron and neutron structure functions, and determine singlet and non-singlet parton distributions in two factorization schemes. We also test the Bjor ken sum rule and find agreement with the theoretical prediction at the level of 10\\%.

  12. Equivalence of two formalisms for calculating higher order synchrotron sideband spin resonances

    International Nuclear Information System (INIS)

    Mane, S.R.

    1988-01-01

    Synchrotron sideband resonances of a first order spin resonance are generally regarded as the most important higher order spin resonances in a high-energy storage ring. Yokoya's formula for these resonances is rederived, including some extra terms, which he neglected, but which turn out to be of comparable magnitude to the terms retained. Including these terms, Yokoya's formalism and the SMILE algorithm are shown to be equivalent to leading order in the resonance strengths. The theoretical calculations are shown to agree with certain measurements from SPEAR

  13. 76 FR 68167 - Spin Master, Inc. and Spin Master, Ltd., Provisional Acceptance of a Settlement Agreement and Order

    Science.gov (United States)

    2011-11-03

    ... hydroxybutyrate (GHB), a Schedule I controlled substance. On October 19, 2007, Spin Master received information... CONSUMER PRODUCT SAFETY COMMISSION [CPSC Docket No. 12-C0003] Spin Master, Inc. and Spin Master... Agreement with Spin Master, Inc. and Spin Master, Ltd., containing a civil penalty of $1,300,000.00. DATES...

  14. Spin- and valley-dependent electrical conductivity of ferromagnetic group-IV 2D sheets in the topological insulator phase

    Science.gov (United States)

    Hoi, Bui Dinh; Yarmohammadi, Mohsen; Mirabbaszadeh, Kavoos; Habibiyan, Hamidreza

    2018-03-01

    In this work, based on the Kubo-Greenwood formalism and the k . p Hamiltonian model, the impact of Rashba spin-orbit coupling on electronic band structure and electrical conductivity of spin-up and spin-down subbands in counterparts of graphene, including silicene, stanene, and germanene nanosheets has been studied. When Rashba coupling is considered, the effective mass of Dirac fermions decreases significantly and no significant change is caused by this coupling for the subband gaps. All these nanosheets are found to be in topological insulator quantum phase at low staggered on-site potentials due to the applied perpendicular external electric field. We point out that the electrical conductivity of germanene increases gradually with Rashab coupling, while silicene and stanene have some fluctuations due to their smaller Fermi velocity. Furthermore, some critical temperatures with the same electrical conductivity values for jumping to the higher energy levels are observed at various Rashba coupling strengths. For all structures, a broad peak appears at low temperatures in electrical conductivity curves corresponding to the large entropy of systems when the thermal energy reaches to the difference between the energy states. Finally, we have reported that silicene has the larger has the larger electrical conductivity than two others.

  15. Equivalence of ADM Hamiltonian and Effective Field Theory approaches at next-to-next-to-leading order spin1-spin2 coupling of binary inspirals

    International Nuclear Information System (INIS)

    Levi, Michele; Steinhoff, Jan

    2014-01-01

    The next-to-next-to-leading order spin1-spin2 potential for an inspiralling binary, that is essential for accuracy to fourth post-Newtonian order, if both components in the binary are spinning rapidly, has been recently derived independently via the ADM Hamiltonian and the Effective Field Theory approaches, using different gauges and variables. Here we show the complete physical equivalence of the two results, thereby we first prove the equivalence of the ADM Hamiltonian and the Effective Field Theory approaches at next-to-next-to-leading order with the inclusion of spins. The main difficulty in the spinning sectors, which also prescribes the manner in which the comparison of the two results is tackled here, is the existence of redundant unphysical spin degrees of freedom, associated with the spin gauge choice of a point within the extended spinning object for its representative worldline. After gauge fixing and eliminating the unphysical degrees of freedom of the spin and its conjugate at the level of the action, we arrive at curved spacetime generalizations of the Newton-Wigner variables in closed form, which can also be used to obtain further Hamiltonians, based on an Effective Field Theory formulation and computation. Finally, we make use of our validated result to provide gauge invariant relations among the binding energy, angular momentum, and orbital frequency of an inspiralling binary with generic compact spinning components to fourth post-Newtonian order, including all known sectors up to date

  16. Correlated calculations of indirect nuclear spin-spin coupling constants using second-order polarization propagator approximations: SOPPA and SOPPA(CCSD)

    DEFF Research Database (Denmark)

    Enevoldsen, Thomas; Oddershede, Jens; Sauer, Stephan P. A.

    1998-01-01

    We present correlated calculations of the indirect nuclear spin-spin coupling constants of HD, HF, H2O, CH4, C2H2, BH, AlH, CO and N2 at the level of the second-order polarization propagator approximation (SOPPA) and the second-order polarization propagator approximation with coupled-cluster sing...

  17. Spin-polarized structural, elastic, electronic and magnetic properties of half-metallic ferromagnetism in V-doped ZnSe

    Energy Technology Data Exchange (ETDEWEB)

    Monir, M. El Amine.; Baltache, H. [Laboratoire de Physique Quantique de la Matière et de la Modélisation Mathématique (LPQ3M), Faculté des Sciences, Université de Mascara, Mascara 29000 (Algeria); Murtaza, G., E-mail: murtaza@icp.edu.pk [Materials Modeling Lab, Department of Physics, Islamia College University, Peshawar (Pakistan); Khenata, R., E-mail: khenata_rabah@yahoo.fr [Laboratoire de Physique Quantique de la Matière et de la Modélisation Mathématique (LPQ3M), Faculté des Sciences, Université de Mascara, Mascara 29000 (Algeria); Ahmed, Waleed K. [ERU, Faculty of Engineering, United Arab Emirates University, Al Ain (United Arab Emirates); Bouhemadou, A. [Laboratory for Developing New Materials and their Characterization, Department of Physics, Faculty of Science, University of Setif, 19000 Setif (Algeria); Omran, S. Bin [Department of Physics and Astronomy, College of Science, King Saud University, P.O. Box 2455, Riyadh 11451 (Saudi Arabia); Seddik, T. [Laboratoire de Physique Quantique de la Matière et de la Modélisation Mathématique (LPQ3M), Faculté des Sciences, Université de Mascara, Mascara 29000 (Algeria)

    2015-01-15

    Based on first principles spin-polarized density functional theory, the structural, elastic electronic and magnetic properties of Zn{sub 1−x}V{sub x}Se (for x=0.25, 0.50, 0.75) in zinc blende structure have been studied. The investigation was done using the full-potential augmented plane wave method as implemented in WIEN2k code. The exchange-correlation potential was treated with the generalized gradient approximation PBE-GGA for the structural and elastic properties. Moreover, the PBE-GGA+U approximation (where U is the Hubbard correlation terms) is employed to treat the “d” electrons properly. A comparative study between the band structures, electronic structures, total and partial densities of states and local moments calculated within both GGA and GGA+U schemes is presented. The analysis of spin-polarized band structure and density of states shows the half-metallic ferromagnetic character and are also used to determine s(p)-d exchange constants N{sub 0}α (conduction band ) and N{sub 0}β (valence band) due to Se(4p)–V(3d) hybridization. It has been clearly evidence that the magnetic moment of V is reduced from its free space change value of 3 µ{sub B} and the minor atomic magnetic moment on Zn and Se are generated. - Highlights: • Half metallicity origins by doping V in ZnSe. • PBE-GGA+U approximation is employed to treat the “d” electrons properly. • s(p)-d Exchange constants N{sub 0}α (conduction band ) and N{sub 0}β (valence band) are due to Se(4p)-V(3d) hybridization.

  18. Inverse spin Hall effect in Pt/(Ga,Mn)As

    Science.gov (United States)

    Nakayama, H.; Chen, L.; Chang, H. W.; Ohno, H.; Matsukura, F.

    2015-06-01

    We investigate dc voltages under ferromagnetic resonance in a Pt/(Ga,Mn)As bilayer structure. A part of the observed dc voltage is shown to originate from the inverse spin Hall effect. The sign of the inverse spin Hall voltage is the same as that in Py/Pt bilayer structure, even though the stacking order of ferromagnetic and nonmagnetic layers is opposite to each other. The spin mixing conductance at the Pt/(Ga,Mn)As interface is determined to be of the order of 1019 m-2, which is about ten times greater than that of (Ga,Mn)As/p-GaAs.

  19. Itinerant ferromagnetism in the narrow band limit

    CERN Document Server

    Liu, S H

    2000-01-01

    It is shown that in the narrow band, strong interaction limit the paramagnetic state of an itinerant ferromagnet is described by the disordered local moment state. As a result, the Curie temperature is orders of magnitude lower than what is expected from the large exchange splitting of the spin bands. An approximate analysis has also been carried out for the partially ordered state, and the result explains the temperature evolvement of the magnetic contributions to the resistivity and low-energy optical conductivity of CrO sub 2.

  20. Reentrant behaviors in the phase diagram of spin-1 planar ferromagnets with easy-axis single-ion anisotropy via the Devlin two-time Green function framework

    Science.gov (United States)

    Mercaldo, M. T.; Rabuffo, I.; De Cesare, L.; Caramico D'Auria, A.

    2017-10-01

    The Devlin two-time Green function framework is used to investigate the role played by the easy-axis single-ion anisotropy on the phase diagram of (d > 2) -dimensional spin-1 planar ferromagnets which exhibit a magnetic-field-induced quantum phase transition (QPT). In this scheme, the exchange anisotropy terms in the equations of motion are treated at the Tyablikov decoupling level while the crystal field anisotropy contribution is handled exactly. The emerging key result is a reentrant structure of the phase diagram close to the quantum critical point for a well defined window of values of the single-ion anisotropy parameter. This experimentally interesting feature was recently recovered by employing the Anderson-Callen decoupling (ACD) which is considered to provide meaningful results only for small values of the single-ion anisotropy parameter. In this context, our findings suggest that the simplest ACD treatment offers the possibility to have, at least qualitatively, a correct physical scenario of quantum criticality close to a field-induced QPT avoiding the limiting mathematical difficulties involved in the Devlin scheme.

  1. Magnetic ordering and spin excitations in Mn(dca) sub 2 (pyz) [dca=N(CN) sub 2 sup - , pyz=pyrazine

    CERN Document Server

    Manson, J L; Argyriou, D N; Bordallo, H N; Lynn, J W; Huang, Q; Feyerherm, R; Loose, A

    2002-01-01

    We have studied the T- and H-dependent magnetism in Mn(dca) sub 2 (pyz) [dca=N(CN) sub 2 sup - , pyz=pyrazine] using neutron-scattering methods. The crystal structure can be viewed as a molecular analog of ReO sub 3 , where 1D Mn-pyz-Mn chains connect 2D Mn(dca) sub 2 square sheets to form a 3D network. In zero field, the Mn sup 2 sup + moments order antiferromagnetically below 2.53(2) K along the ac diagonal with a magnitude of 4.15(6) mu B at 1.35 K. The field-dependent response of the [111] magnetic reflection is consistent with spin-flop and induced ferromagnetic phase transitions as previously observed in magnetization measurements. Diffuse-scattering studies indicated no evidence for low-dimensional spin correlations. Using quasielastic neutron scattering, a low-energy spin-wave excitation was observed at propor to 0.23 meV, which is propor to 1/6 the momentum transfer observed in Mn(dca) sub 2 owing to a reduced number of magnetic nearest neighbors. (orig.)

  2. Infinitely robust order and local order-parameter tulips in Apollonian networks with quenched disorder

    Science.gov (United States)

    Kaplan, C. Nadir; Hinczewski, Michael; Berker, A. Nihat

    2009-06-01

    For a variety of quenched random spin systems on an Apollonian network, including ferromagnetic and antiferromagnetic bond percolation and the Ising spin glass, we find the persistence of ordered phases up to infinite temperature over the entire range of disorder. We develop a renormalization-group technique that yields highly detailed information, including the exact distributions of local magnetizations and local spin-glass order parameters, which turn out to exhibit, as function of temperature, complex and distinctive tulip patterns.

  3. Ferromagnetism versus charge ordering in the Pr0.5Ca0.5MnO3 and La0.5Ca0.5MnO3 nanocrystals

    Science.gov (United States)

    Jirák, Z.; Hadová, E.; Kaman, O.; Knížek, K.; Maryško, M.; Pollert, E.; Dlouhá, M.; Vratislav, S.

    2010-01-01

    The half-doped perovskite manganites Pr0.5Ca0.5MnO3 and La0.5Ca0.5MnO3 in bulk and nanocrystalline form were structurally studied by x-ray and neutron-diffraction methods. The magnetic properties were probed by dc and ac susceptibilities and by isothermal magnetization measurements. The study shows that the room-temperature Pbnm perovskite structure, as concerns the lattice distortion, Mn-O distances, and octahedral tilts, is practically unaffected by the particle size. Nonetheless, the low-temperature structural distortion, characteristic for (long- or short-range) charge and orbital ordering in bulk samples, is not observed for 25 nm particles. The absence of the charge-ordering transition is confirmed also by magnetic data. The different behavior compared to bulk is explained by effects of the particle surface. In the nanocrystalline Pr0.5Ca0.5MnO3 , an onset of ferromagnetic (FM) arrangement is observed at ˜100K . At the lowest temperature, the magnetic state of the sample can be characterized as a mixture of particles in the metallic FM state with those in the insulating charge and orbitally disordered phase with frozen spins. There is a possibility to induce a global FM state by external field. The La0.5Ca0.5MnO3 nanocrystals develop FM ordering spontaneously below TC=260K .

  4. Electrical manipulation of ferromagnetic NiFe by antiferromagnetic IrMn

    Science.gov (United States)

    Tshitoyan, V.; Ciccarelli, C.; Mihai, A. P.; Ali, M.; Irvine, A. C.; Moore, T. A.; Jungwirth, T.; Ferguson, A. J.

    2015-12-01

    We demonstrate that an antiferromagnet can be employed for a highly efficient electrical manipulation of a ferromagnet. In our study, we use an electrical detection technique of the ferromagnetic resonance driven by an in-plane ac current in a NiFe/IrMn bilayer. At room temperature, we observe antidampinglike spin torque acting on the NiFe ferromagnet, generated by an in-plane current driven through the IrMn antiferromagnet. A large enhancement of the torque, characterized by an effective spin-Hall angle exceeding most heavy transition metals, correlates with the presence of the exchange-bias field at the NiFe/IrMn interface. It highlights that, in addition to the strong spin-orbit coupling, the antiferromagnetic order in IrMn governs the observed phenomenon.

  5. Aperiodic spin state ordering of bistable molecules and its photoinducede erasing

    Czech Academy of Sciences Publication Activity Database

    Collet, E.; Watanabe, H.; Bréfuel, N.; Palatinus, Lukáš; Roudaut, L.; Toupet, L.; Tanaka, K.; Tuchagues, J.-P.; Fertey, P.; Ravy, S.; Toudic, B.; Cailleau, H.

    2012-01-01

    Roč. 109, č. 25 (2012), "257206-1"-"257206-5" ISSN 0031-9007 Institutional research plan: CEZ:AV0Z10100521 Keywords : photocrystallography * aperiodic structure * spin-state ordering Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 7.943, year: 2012

  6. Spin-glass-like ordering of the magnetic moments of interacting nanosized maghemite particles

    DEFF Research Database (Denmark)

    Mørup, Steen; Bødker, Franz; Hendriksen, Peter Vang

    1995-01-01

    measurements of the decay of remanence are much lower. These results are not in accordance with the Néel model for superparamagnetic relaxation, but can be explained by the formation of an ordered spin-glass-like state at low temperatures. At a critical temperature a transition to a superparamagnetic state...

  7. Superconducting Ferromagnetic Nanodiamond

    Czech Academy of Sciences Publication Activity Database

    Zhang, G.; Samuely, T.; Xu, Z.; Jochum, J. K.; Volodin, A.; Zhou, S. Q.; May, P. W.; Onufriienko, O.; Kacmarik, J.; Steele, J. A.; Li, J.; Vanacken, J.; Vacík, Jiří; Szabo, P.; Yuan, H. F.; Roeffaers, M. B. J.; Cerbu, D.; Samuely, P.; Hofkens, J.; Moshchalkov, V.V.

    2017-01-01

    Roč. 11, č. 6 (2017), s. 5358-5366 ISSN 1936-0851 R&D Projects: GA ČR(CZ) GBP108/12/G108; GA MŠk LM2015056 Institutional support: RVO:61389005 Keywords : nanodiamond * superconductivity and ferromagnetism * spin fluctuations * giant positive magnetoresistance * anamalous Hall effect Subject RIV: BG - Nuclear, Atomic and Molecular Physics, Colliders OBOR OECD: Nano-materials (production and properties) Impact factor: 13.942, year: 2016

  8. Low Spin-Casting Solution Temperatures Enhance the Molecular Ordering in Polythiophene Films

    International Nuclear Information System (INIS)

    Lee, Wi Hyoung; Lee, Hwa Sung; Park, Yeong Don

    2014-01-01

    High-crystallinity poly(3-hexylthiophene) (P3HT) thin films were prepared by aging the precursor solutions, prepared using a good solvent, chloroform, at low temperatures prior to spin-casting. Lower solution temperatures significantly improved the molecular ordering in the spin-cast P3HT films and, therefore, the electrical properties of field-effect transistors prepared using these films. Solution cooling enhanced the electrical properties by shifting the P3HT configuration equilibrium away from random coils and toward more ordered aggregates. At room temperature, the P3HT molecules were completely solvated in chloroform and adopted a random coil conformation. Upon cooling, however, the chloroform poorly solvated the P3HT molecules, favoring the formation of ordered P3HT aggregates, which then yielded more highly crystalline molecular ordering in the P3HT thin films produced from the solution

  9. Coupling between Spin and Charge Order Driven by Magnetic Field in Triangular Ising System LuFe2O4+δ

    Directory of Open Access Journals (Sweden)

    Lei Ding

    2018-02-01

    Full Text Available We present a study of the magnetic-field effect on spin correlations in the charge ordered triangular Ising system LuFe2O4+δ through single crystal neutron diffraction. In the absence of a magnetic field, the strong diffuse neutron scattering observed below the Neel temperature (TN = 240 K indicates that LuFe2O4+δ shows short-range, two-dimensional (2D correlations in the FeO5 triangular layers, characterized by the development of a magnetic scattering rod along the 1/3 1/3 L direction, persisting down to 5 K. We also found that on top of the 2D correlations, a long range ferromagnetic component associated with the propagation vector k1 = 0 sets in at around 240 K. On the other hand, an external magnetic field applied along the c-axis effectively favours a three-dimensional (3D spin correlation between the FeO5 bilayers evidenced by the increase of the intensity of satellite reflections with propagation vector k2 = (1/3, 1/3, 3/2. This magnetic modulation is identical to the charge ordered superstructure, highlighting the field-promoted coupling between the spin and charge degrees of freedom. Formation of the 3D spin correlations suppresses both the rod-type diffuse scattering and the k1 component. Simple symmetry-based arguments provide a natural explanation of the observed phenomenon and put forward a possible charge redistribution in the applied magnetic field.

  10. Spin amplification by controlled symmetry breaking for spin-based logic

    Science.gov (United States)

    Kawakami, Roland K.

    2015-09-01

    Spin amplification is one of the most critical challenges for spintronics and spin-based logic in order to achieve spintronic circuits with fan-out. We propose a new concept for spin amplification that will allow a small spin current in a non-magnetic spin channel to control the magnetization of an attached ferromagnet. The key step is to bring the ferromagnet into an unstable symmetric state (USS), so that a small spin transfer torque from a small spin current can provide a magnetic bias to control the spontaneous symmetry breaking and select the final magnetization direction of the ferromagnet. Two proposed methods for achieving the USS configuration are voltage-controlled Curie temperature (VC-TC) and voltage-controlled magnetic anisotropy (VC-MA). We believe the development of new 2D magnetic materials with greater tunability of VC-TC and VC-MA will be needed for practical applications. A successful realization of spin amplification by controlled symmetry breaking will be important for the implementation of existing spin-logic proposals (e.g. ‘all spin logic’) and could inspire alternative ideas for spintronic circuits and devices.

  11. Spin amplification by controlled symmetry breaking for spin-based logic

    International Nuclear Information System (INIS)

    Kawakami, Roland K

    2015-01-01

    Spin amplification is one of the most critical challenges for spintronics and spin-based logic in order to achieve spintronic circuits with fan-out. We propose a new concept for spin amplification that will allow a small spin current in a non-magnetic spin channel to control the magnetization of an attached ferromagnet. The key step is to bring the ferromagnet into an unstable symmetric state (USS), so that a small spin transfer torque from a small spin current can provide a magnetic bias to control the spontaneous symmetry breaking and select the final magnetization direction of the ferromagnet. Two proposed methods for achieving the USS configuration are voltage-controlled Curie temperature (VC-T C ) and voltage-controlled magnetic anisotropy (VC-MA). We believe the development of new 2D magnetic materials with greater tunability of VC-T C and VC-MA will be needed for practical applications. A successful realization of spin amplification by controlled symmetry breaking will be important for the implementation of existing spin-logic proposals (e.g. ‘all spin logic’) and could inspire alternative ideas for spintronic circuits and devices. (paper)

  12. Molecular ferromagnetism

    International Nuclear Information System (INIS)

    Epstein, A.J.

    1990-01-01

    This past year has been one of substantial advancement in both the physics and chemistry of molecular and polymeric ferromagnets. The specific heat studies of (DMeFc)(TCNE) have revealed a cusp at the three-dimensional ferromagnetic transition temperature with a crossover to primarily 1-D behavior at higher temperatures. This paper discusses these studies

  13. Mean fields and self consistent normal ordering of lattice spin and gauge field theories

    International Nuclear Information System (INIS)

    Ruehl, W.

    1986-01-01

    Classical Heisenberg spin models on lattices possess mean field theories that are well defined real field theories on finite lattices. These mean field theories can be self consistently normal ordered. This leads to a considerable improvement over standard mean field theory. This concept is carried over to lattice gauge theories. We construct first an appropriate real mean field theory. The equations determining the Gaussian kernel necessary for self-consistent normal ordering of this mean field theory are derived. (orig.)

  14. Towards spin injection into silicon

    Energy Technology Data Exchange (ETDEWEB)

    Dash, S.P.

    2007-08-15

    Si has been studied for the purpose of spin injection extensively in this thesis. Three different concepts for spin injection into Si have been addressed: (1) spin injection through a ferromagnet-Si Schottky contact, (2) spin injection using MgO tunnel barriers in between the ferromagnet and Si, and (3) spin injection from Mn-doped Si (DMS) as spin aligner. (1) FM-Si Schottky contact for spin injection: To be able to improve the interface qualities one needs to understand the atomic processes involved in the formation of silicide phases. In order to obtain more detailed insight into the formation of such phases the initial stages of growth of Co and Fe were studied in situ by HRBS with monolayer depth resolution.(2) MgO tunnel barrier for spin injection into Si: The fabrication and characterization of ultra-thin crystalline MgO tunnel barriers on Si (100) was presented. (3) Mn doped Si for spin injection: Si-based diluted magnetic semiconductor samples were prepared by doping Si with Mn by two different methods i) by Mn ion implantation and ii) by in-diffusion of Mn atoms (solid state growth). (orig.)

  15. Graphene based superconducting junctions as spin sources for spintronics

    Science.gov (United States)

    Emamipour, Hamidreza

    2018-02-01

    We investigate spin-polarized transport in graphene-based ferromagnet-superconductor junctions within the Blonder-Tinkham-Klapwijk formalism by using spin-polarized Dirac-Bogoliubov-de-Gennes equations. We consider superconductor in spin-singlet s-wave pairing state and ferromagnet is modeled by an exchange field with energy of Ex. We have found that graphene-based junctions can be used to produce highly spin-polarized current in different situations. For example, if we design a junction with high Ex and EF compared to order parameter of superconductor, then one can have a large spin-polarized current which is tunable in magnitude and sign by bias voltage and Ex. Therefore graphene-based superconducting junction can be used in spintronic devices in alternative to conventional junctions or half-metallic ferromagnets. Also, we have found that the calculated spin polarization can be used as a tool to distinguish specular Andreev reflection (SAR) from the conventional Andreev reflection (CAR) such that in the case of CAR, spin polarization in sub-gap region is completely negative which means that spin-down current is greater than spin-up current. When the SAR is dominated, the spin polarization is positive at all bias-voltages, which itself shows that spin-up current is greater than spin-down current.

  16. Electrical manipulation of a ferromagnet by an antiferromagnet

    Science.gov (United States)

    Tshitoyan, V.; Ciccarelli, C.; Mihai, A. P.; Ali, M.; Irvine, A. C.; Moore, T. A.; Jungwirth, T.; Ferguson, A. J.

    Several recent studies of antiferromagnetic (AFM) spintronics have focused on transmission and detection of spin-currents in AFMs. Efficient spin transmission through AFMs was inferred from experiments in FM/AFM/NM (normal metal) structures. Measurements in FM/AFM bilayers have demonstrated that a metallic AFM can also act as an efficient ISHE detector of the spin-current, with spin-Hall angles comparable to heavy NMs. Here we demonstrate that an antiferromagnet can be employed for a highly efficient electrical manipulation of a ferromagnet. We use an all-electrical excitation and detection technique of ferromagnetic resonance in a NiFe/IrMn bilayer. We observe antidamping-like spin torque acting on the NiFe generated by the in-plane current driven through the IrMn antiferromagnet. A large enhancement of the torque, characterized by an effective spin-Hall angle exceeding most heavy transition metals, correlates with the presence of the exchange-bias field at the NiFe/IrMn interface. It highlights that, in addition to strong spin-orbit coupling, the AFM order in IrMn governs the observed phenomenon.

  17. Two-dimensional spin diffusion in multiterminal lateral spin valves

    Science.gov (United States)

    Saha, D.; Basu, D.; Holub, M.; Bhattacharya, P.

    2008-01-01

    The effects of two-dimensional spin diffusion on spin extraction in lateral semiconductor spin valves have been investigated experimentally and theoretically. A ferromagnetic collector terminal of variable size is placed between the ferromagnetic electron spin injector and detector of a conventional lateral spin valve for spin extraction. It is observed that transverse spin diffusion beneath the collector terminal plays an important role along with the conventional longitudinal spin diffusion in describing the overall transport of spin carriers. Two-dimensional spin diffusion reduces the perturbation of the channel electrochemical potentials and improves spin extraction.

  18. Proposal for an All-Spin Artificial Neural Network: Emulating Neural and Synaptic Functionalities Through Domain Wall Motion in Ferromagnets.

    Science.gov (United States)

    Sengupta, Abhronil; Shim, Yong; Roy, Kaushik

    2016-12-01

    Non-Boolean computing based on emerging post-CMOS technologies can potentially pave the way for low-power neural computing platforms. However, existing work on such emerging neuromorphic architectures have either focused on solely mimicking the neuron, or the synapse functionality. While memristive devices have been proposed to emulate biological synapses, spintronic devices have proved to be efficient at performing the thresholding operation of the neuron at ultra-low currents. In this work, we propose an All-Spin Artificial Neural Network where a single spintronic device acts as the basic building block of the system. The device offers a direct mapping to synapse and neuron functionalities in the brain while inter-layer network communication is accomplished via CMOS transistors. To the best of our knowledge, this is the first demonstration of a neural architecture where a single nanoelectronic device is able to mimic both neurons and synapses. The ultra-low voltage operation of low resistance magneto-metallic neurons enables the low-voltage operation of the array of spintronic synapses, thereby leading to ultra-low power neural architectures. Device-level simulations, calibrated to experimental results, was used to drive the circuit and system level simulations of the neural network for a standard pattern recognition problem. Simulation studies indicate energy savings by  ∼  100× in comparison to a corresponding digital/analog CMOS neuron implementation.

  19. Coexisting static magnetic ordering and superconductivity in CeCu2.1Si2 found by muon spin relaxation

    Science.gov (United States)

    Uemura, Y. J.; Kossler, W. J.; Yu, X. H.; Schone, H. E.; Kempton, J. R.; Stronach, C. E.; Barth, S.; Gygax, F. N.; Hitti, B.; Schenck, A.

    1988-01-01

    Zero- and longitudinal-field muon spin relaxation measurements on a heavy fermion system CeCu2.1 Si2 have revealed an onset of static magnetic ordering below T(M) approximately 0.8 K, which coexists with superconductivity below T(c) = 0.7 K. The line shapes of the observed muon spin depolarization functions suggest an ordering in either spin glass or incommensurate spin-density-wave state, with a small averaged static moment of the order of 0.1 micro-B per formula unit at T approaches 0.

  20. Gd doping induced weak ferromagnetic ordering in ZnS nanoparticles synthesized by low temperature co-precipitation technique

    Energy Technology Data Exchange (ETDEWEB)

    Kaur, Palvinder [Department of Physics, Punjabi University, Patiala, Punjab, 147002 (India); Kumar, Sanjeev, E-mail: sanjeev04101977@gmail.com [Applied Science Department, PEC University of Technology, Chandigarh, 160012 (India); Chen, Chi-Liang, E-mail: chen.cl@nsrrc.org.tw [National Synchrotron Radiation Research Center (NSRRC), Hsinchu, 30076, Taiwan (China); Yang, Kai-Siang [National Synchrotron Radiation Research Center (NSRRC), Hsinchu, 30076, Taiwan (China); Department of Mechanical Engineering, National Taipei University of Technology, Taipei, Taiwan (China); Wei, Da-Hua [Department of Mechanical Engineering, National Taipei University of Technology, Taipei, Taiwan (China); Dong, Chung-Li [Department of Physics, Tamkang University, Tamsui, Taiwan (China); Srivastava, C. [Materials Engineering Department, Indian Institute of Science, Bangalore, 560012 (India); Rao, S.M. [Department of Physics, Punjabi University, Patiala, Punjab, 147002 (India); Institute of Physics, Academia Sinica, Taipei, 11529, Taiwan (China)

    2017-01-15

    Zn{sub 1−x}Gd{sub x}S nanoparticles with Gd concentration x = 0.00, 0.02 and 0.04 were synthesized by the chemical co-precipitation technique using thioglycerol as capping agent. X-ray diffraction (XRD), transmission electron microscopy (TEM), photoluminescence (PL) spectroscopy, X-ray absorption near-edge structure (XANES) and vibrating sample magnetometer (VSM) were employed to characterize the as synthesized Gd doped ZnS nanoparticles. XRD and TEM studies show the formation of cubic ZnS nanoparticles with an average size in the range 5–10 nm. The doping did not alter the phase of the ZnS. The PL spectra of doped ZnS nanoparticles showed the presence of sulphur vacancies in the lattice. XANES of Gd doped ZnS nanoparticles depicts spectral changes may arise from charge transfer between host Zn and dopant Gd ions. A VSM study shows that the weak ferromagnetic behaviour increases with increase in Gd doping ZnS nanoparticles. - Highlights: • Gd doped ZnS nanoparticles synthesized using co-precipitation technique. • PL studies depict sulphur and zinc vacancies in Gd doped ZnS nanoparticles. • XANES studies depict the charge transfer between host Zn and dopant Gd ions. • Room temperature weak ferromagnetism is observed in Gd doped ZnS nanoparticles.

  1. Spin model for nontrivial types of magnetic order in inverse-perovskite antiferromagnets

    Science.gov (United States)

    Mochizuki, Masahito; Kobayashi, Masaya; Okabe, Reoya; Yamamoto, Daisuke

    2018-02-01

    Nontrivial magnetic orders in the inverse-perovskite manganese nitrides are theoretically studied by constructing a classical spin model describing the magnetic anisotropy and frustrated exchange interactions inherent in specific crystal and electronic structures of these materials. With a replica-exchange Monte Carlo technique, a theoretical analysis of this model reproduces the experimentally observed triangular Γ5 g and Γ4 g spin-ordered patterns and the systematic evolution of magnetic orders. Our Rapid Communication solves a 40-year-old problem of nontrivial magnetism for the inverse-perovskite manganese nitrides and provides a firm basis for clarifying the magnetism-driven negative thermal expansion phenomenon discovered in this class of materials.

  2. Scattering of two spinning black holes in post-Minkowskian gravity, to all orders in spin, and effective-one-body mappings

    Science.gov (United States)

    Vines, Justin

    2018-04-01

    We demonstrate equivalences, under simple mappings, between the dynamics of three distinct systems—(i) an arbitrary-mass-ratio two-spinning-black-hole system, (ii) a spinning test black hole in a background Kerr spacetime, and (iii) geodesic motion in Kerr—when each is considered in the first post-Minkowskian (1PM) approximation to general relativity, i.e. to linear order G but to all orders in 1/c, and to all orders in the black holes’ spins, with all orders in the multipole expansions of their linearized gravitational fields. This is accomplished via computations of the net results of weak gravitational scattering encounters between two spinning black holes, namely the net O(G) changes in the holes’ momenta and spins as functions of the incoming state. The results are given in remarkably simple closed forms, found by solving effective Mathisson–Papapetrou–Dixon-type equations of motion for a spinning black hole in conjunction with the linearized Einstein equation, with appropriate matching to the Kerr solution. The scattering results fully encode the gauge-invariant content of a canonical Hamiltonian governing binary-black-hole dynamics at 1PM order, for generic (unbound and bound) orbits and spin orientations. We deduce one such Hamiltonian, which reproduces and resums the 1PM parts of all such previous post-Newtonian results, and which directly manifests the equivalences with the test-body limits via simple effective-one-body mappings.

  3. Block renormalization for quantum Ising models in dimension d = 2: applications to the pure and random ferromagnet, and to the spin-glass

    International Nuclear Information System (INIS)

    Monthus, Cécile

    2015-01-01

    For the quantum Ising chain, the self-dual block renormalization procedure of Fernandez-Pacheco (1979 Phys. Rev. D 19 3173) is known to reproduce exactly the location of the zero-temperature critical point and the correlation length exponent ν = 1. Recently, Miyazaki and Nishimori (2013 Phys. Rev. E 87 032154) have proposed to study the disordered quantum Ising model in dimensions d > 1 by applying the Fernandez-Pacheco procedure successively in each direction. To avoid the inequivalence of directions of their approach, we propose here an alternative procedure where the d directions are treated on the same footing. For the pure model, this leads to the correlation length exponents ν ≃ 0.625 in d = 2 (to be compared with the 3D classical Ising model exponent ν ≃ 0.63) and ν ≃ 0.5018 (to be compared with the 4D classical Ising model mean-field exponent ν = 1/2). For the disordered model in dimension d = 2, either ferromagnetic or spin-glass, the numerical application of the renormalization rules to samples of linear size L = 4096 yields that the transition is governed by an Infinite Disorder Fixed Point, with the activated exponent ψ ≃ 0.65, the typical correlation exponent ν typ  ≃ 0.44 and the finite-size correlation exponent ν FS  ≃ 1.25. We discuss the similarities and differences with the Strong Disorder Renormalization results. (paper)

  4. Spin current through quantum-dot spin valves

    International Nuclear Information System (INIS)

    Wang, J; Xing, D Y

    2006-01-01

    We report a theoretical study of the influence of the Coulomb interaction on the equilibrium spin current in a quantum-dot spin valve, in which the quantum dot described by the Anderson impurity model is coupled to two ferromagnetic leads with noncollinear magnetizations. In the Kondo regime, electrons transmit through the quantum dot via higher-order virtual processes, in which the spin of either lead electrons or a localized electron on the quantum dot may reverse. It is found that the magnitude of the spin current decreases with increasing Coulomb interactions due to spin flip effects on the dot. However, the spatial direction of the spin current remains unchanged; it is determined only by the exchange coupling between two noncollinear magnetizations

  5. Spin Orbit Interaction Engineering for beyond Spin Transfer Torque memory

    Science.gov (United States)

    Wang, Kang L.

    Spin transfer torque memory uses electron current to transfer the spin torque of electrons to switch a magnetic free layer. This talk will address an alternative approach to energy efficient non-volatile spintronics through engineering of spin orbit interaction (SOC) and the use of spin orbit torque (SOT) by the use of electric field to improve further the energy efficiency of switching. I will first discuss the engineering of interface SOC, which results in the electric field control of magnetic moment or magneto-electric (ME) effect. Magnetic memory bits based on this ME effect, referred to as magnetoelectric RAM (MeRAM), is shown to have orders of magnitude lower energy dissipation compared with spin transfer torque memory (STTRAM). Likewise, interests in spin Hall as a result of SOC have led to many advances. Recent demonstrations of magnetization switching induced by in-plane current in heavy metal/ferromagnetic heterostructures have been shown to arise from the large SOC. The large SOC is also shown to give rise to the large SOT. Due to the presence of an intrinsic extraordinarily strong SOC and spin-momentum lock, topological insulators (TIs) are expected to be promising candidates for exploring spin-orbit torque (SOT)-related physics. In particular, we will show the magnetization switching in a chromium-doped magnetic TI bilayer heterostructure by charge current. A giant SOT of more than three orders of magnitude larger than those reported in heavy metals is also obtained. This large SOT is shown to come from the spin-momentum locked surface states of TI, which may further lead to innovative low power applications. I will also describe other related physics of SOC at the interface of anti-ferromagnetism/ferromagnetic structure and show the control exchange bias by electric field for high speed memory switching. The work was in part supported by ERFC-SHINES, NSF, ARO, TANMS, and FAME.

  6. Spin and orbital orderings behind multiferroicity in delafossite and related compounds

    Science.gov (United States)

    Terada, Noriki

    2014-11-01

    Coupling between noncollinear magnetic ordering and ferroelectricicty in magnetoelectric multiferroics has been extensively studied in the last decade. Delafossite family compounds with triangular lattice structure provide a great opportunity to study the coupling between spin and electric dipole in multiferroics due to the variety of magnetic phases with different symmetry. This review introduces the magnetic and ferroelectric phase transitions in delafossite ferrites, CuFe1-xXxO2 (X = Al, Ga), AgFeO2 and the related compound α-NaFeO2. In CuFeO2, the ferroelectric phase appears under a magnetic field or chemical substitution. The proper screw magnetic ordering with the magnetic point group 21‧, which has been determined by detailed analysis in neutron diffraction experiments, induces the ferroelectric polarization along the monoclinic b axis in CuFeO2. The cycloidal magnetic orderings are realized in AgFeO2 and α-NaFeO2, which are of the point group m1‧ allowing polarization in the ac plane. The emergence of ferroelectric polarization can be explained by both the extended inverse Dzyaloshinsky-Moriya effect and the d - p hybridization mechanism. These mechanisms are supported by experimental evidence in CuFe1-xGaxO2. The polarized neutron diffraction experiment demonstrated one-to-one correspondence between ferroelectric polarization and spin helicity, Si × Sj . The incommensurate orbital ordering with 2{Q} wave vector, observed by the soft x-ray resonant diffraction experiment, proved that the spin-orbit interaction ties spin and orbital orders to each other, playing a crucial role for the emergence of ferroelectricity in CuFe1-xGaxO2.

  7. Spin diffusion and torques in disordered antiferromagnets

    KAUST Repository

    Manchon, Aurelien

    2017-02-01

    We have developed a drift-diffusion equation of spin transport in collinear bipartite metallic antiferromagnets. Starting from a model tight-binding Hamiltonian, we obtain the quantum kinetic equation within Keldysh formalism and expand it to the lowest order in spatial gradient using Wigner expansion method. In the diffusive limit, these equations track the spatio-temporal evolution of the spin accumulations and spin currents on each sublattice of the antiferromagnet. We use these equations to address the nature of the spin transfer torque in (i) a spin-valve composed of a ferromagnet and an antiferromagnet, (ii) a metallic bilayer consisting of an antiferromagnet adjacent to a heavy metal possessing spin Hall effect, and in (iii) a single antiferromagnet possessing spin Hall effect. We show that the latter can experience a self-torque thanks to the non-vanishing spin Hall effect in the antiferromagnet.

  8. Ferroquadrupolar Order in the Spin-1 Bilinear-Biquadratic Model up to the Second Nearest Neighbor

    Science.gov (United States)

    Pires, A. S. T.

    2017-10-01

    We have studied some ferroquadrupolar phases of the S = 1 Heisenberg model with bilinear and biquadratic exchange interactions on the square lattice up to the second nearest neighbor, using the SU(3) Schwinger bosons formalism in a mean field approximation. This technique is very convenient to treat nematic order. This technique has the advantage of using the fundamental representation of the SU(N) group instead of SU(2), designed to capture spin-quadrupolar order in addition to the dipolar magnetic order. We also present quadrupole structure factors that can be measured in future experiments. Our calculations can have implications in the study of iron-based superconductors.

  9. Study of spin-temperature effects using energy-ordered continuum gamma-ray spectroscopy technique

    Energy Technology Data Exchange (ETDEWEB)

    Baktash, C.; Halbert, M.L.; Hensley, D.C.; Johnson, N.R.; Lee, I.Y.; McConnell, J.W.; McGowan, F.K.

    1990-01-01

    We have investigated a new continuum {gamma}-ray spectroscopy technique which is based on the detection of all emitted {gamma} rays in a 4{pi} detector system, and ordering them according to their energies on an event-by-event basis. The technique allows determination of gamma strength functions, and rotational damping width as a function of spin and temperature. Thus, it opens up the possibility of studying the onset of motional narrowing, order-to-chaos transition, and the mapping of the evolution of nuclear collectivity with a spin and temperature. Application of the technique for preferential entry-state population, exit-channel selection, and feeding of the discrete states via selective pathways will be discussed. 20 refs., 4 figs.

  10. Spin-current noise from fluctuation relations

    Energy Technology Data Exchange (ETDEWEB)

    Lim, Jong Soo [Institut de Fisica Interdisciplinària i Sistemes Complexos IFISC (UIB-CSIC), E-07122 Palma de Mallorca (Spain); Sánchez, David; López, Rosa [Institut de Fisica Interdisciplinària i Sistemes Complexos IFISC (UIB-CSIC), E-07122 Palma de Mallorca, Spain and Departement de Fisica, Universitat de les Illes Balears, E-07122 Palma de Mallorca (Spain)

    2013-12-04

    We present fluctuation relations that connect spin-polarized current and noise in mesoscopic conductors. In linear response, these relations are equivalent to the fluctuation-dissipation theorem that relates equilibrium current-current correlations to the linear conductance. More interestingly, in the weakly nonlinear regime of transport, these relations establish a connection between the leading-order rectification spin conductance, the spin noise susceptibility and the third cumulant of spin current fluctuations at equilibrium. Our results are valid even for systems in the presence of magnetic fields and coupled to ferromagnetic electrodes.

  11. First-order transition and tricritical behavior of the transverse crystal field spin-1 Ising model

    Science.gov (United States)

    Costabile, Emanuel; Viana, J. Roberto; de Sousa, J. Ricardo; de Arruda, Alberto S.

    2015-06-01

    The phase diagram of the spin-1 Ising model in the presence of a transverse crystal-field anisotropy (Dx) is studied within the framework of an effective-field theory with correlation. The effect of the coordination number (z) on the phase diagram in the T -Dx plane is investigated. We observe only second-order transitions for coordination number z Ricardo de Sousa and Branco, Phys. Rev. E 77 (2008) 012104] with a single tricritical point in the phase diagram.

  12. Spin excitations and quantum criticality in the quasi-one-dimensional Ising-like ferromagnet CoCl2·2D2O in a transverse field

    DEFF Research Database (Denmark)

    Larsen, J.; Schäffer, T. K.; Hansen, U. B.

    2017-01-01

    We present experimental evidence for a quantum phase transition in the easy-axis S = 3/2 anisotropic quasione-dimensional ferromagnet CoCl2 · 2D2O in a transverse field. Elastic neutron scattering shows that the magnetic order parameter vanishes at a transverse critical field μ0Hc = 16.05(4) T...... that the quantum phase transition in CoCl2 · 2D2O differs significantly from the textbook version of a S = 1/2 Ising chain in a transverse field. We attribute the difference to weak but finite three-dimensionality of the magnetic interactions......., while inelastic neutron scattering shows that the gap in the magnetic excitation spectrum vanishes at the same field value, and reopens for H>Hc. The field dependence of the order parameter and the gap are well described by critical exponents β = 0.45 ± 0.09 and zν close to 1/2, implying...

  13. Adjustable third-order nonlinear optical properties of the spin coating phenoxazinium–PMMA films

    International Nuclear Information System (INIS)

    Miao, Jia-Tao; Sun, Ru; Yan, Bao-Long; Wu, Xing-Zhi; Song, Ying-Lin; Lu, Jian-Mei; Ge, Jian-Feng

    2014-01-01

    The third-order nonlinear optical properties of spin coating poly(methyl methacrylate) films doped with 3,7-bis(diethylamino)phenoxazin-5-ium chloride (1) are reported. The third-order nonlinear optical properties were tested by Z-scan technology with nanosecond laser beam at 532 nm. The third-order nonlinear absorptions change from reverse saturation absorption to saturation absorption with increasing percentage of the phenoxazinium dye in the poly(methyl methacrylate) film. The different forms of the spin coating films were obtained by atomic force microscopy and transmission electron microscope, and the different aggregation phenomenon of the phenoxazinium in the films can explain the adjustable third-order nonlinear absorption phenomena. Moreover, large third-order nonlinear optical susceptibilities (up to 10 −7  esu) and high second hyperpolarizabilities (up to 10 −28  esu) are found with these films. The results indicate that the phenoxazinium dye is the potential material for the third-order nonlinear optical application. - Highlights: • Third-order NLO properties of the phenoxazinium doped PMMA films were obtained. • Reverse saturated absorption changes to saturated absorption by the different percentage of phenoxazinium in the PMMA films. • Different states of films were obtained

  14. Antiferromagnetic ordering in spin-chain multiferroic Gd{sub 2}BaNiO{sub 5} studied by electronic spin resonance

    Energy Technology Data Exchange (ETDEWEB)

    Guo, Y. M.; Ruan, M. Y.; Cheng, J. J.; Sun, Y. C. [Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology, Wuhan 430074 (China); School of Physics, Huazhong University of Science and Technology, Wuhan 430074 (China); Ouyang, Z. W., E-mail: zwouyang@mail.hust.edu.cn; Xia, Z. C. [Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology, Wuhan 430074 (China); Rao, G. H. [School of Materials Science and Engineering, Guilin University of Electronic Technology, Guilin 541004 (China)

    2015-06-14

    High-field electron spin resonance (ESR) has been employed to study the antiferromagnetic (AFM) ordering state (T < T{sub N} = 55 K) of spin-chain multiferroic Gd{sub 2}BaNiO{sub 5}. The spin reorientation at T{sub SR} = 24 K is well characterized by the temperature-dependent ESR spectra. The magnetization data evidence a field-induced spin-flop transition at 2 K. The frequency-field relationship of the ESR data can be explained by conventional AFM resonance theory with uniaxial anisotropy, in good agreement with magnetization data. Related discussion on zero-field spin gap is presented.

  15. Ferromagnetism in Cr-doped passivated AlN nanowires

    KAUST Repository

    Kanoun, Mohammed

    2014-01-01

    We apply first principles calculations to predict the effect of Cr doping on the electronic and magnetic properties of passivated AlN nanowires. We compare the energetics of the possible dopant sites and demonstrate the favorable configuration ferromagnetic ordering. The charge density of the pristine passivated AlN nanowires is used to elucidate the bonding character. Spin density maps demonstrate an induced spin polarization for N atoms next to dopant atoms, though most of the magnetism is carried by the Cr atoms. Cr-doped AlN nanowires turn out to be interesting for spintronic devices. © 2014 the Partner Organisations.

  16. TOPICAL REVIEW: Spin current, spin accumulation and spin Hall effect

    Directory of Open Access Journals (Sweden)

    Saburo Takahashi and Sadamichi Maekawa

    2008-01-01

    Full Text Available Nonlocal spin transport in nanostructured devices with ferromagnetic injector (F1 and detector (F2 electrodes connected to a normal conductor (N is studied. We reveal how the spin transport depends on interface resistance, electrode resistance, spin polarization and spin diffusion length, and obtain the conditions for efficient spin injection, spin accumulation and spin current in the device. It is demonstrated that the spin Hall effect is caused by spin–orbit scattering in nonmagnetic conductors and gives rise to the conversion between spin and charge currents in a nonlocal device. A method of evaluating spin–orbit coupling in nonmagnetic metals is proposed.

  17. The influence of atomic order on the magnetic and structural properties of the ferromagnetic shape memory compound Ni sub 2 MnGa

    CERN Document Server

    Kreissl, M; Stephens, T; Ziebeck, K R A

    2003-01-01

    The effect of atomic order on the martensitic phase transition and magnetic properties of stoichiometric Ni sub 2 MnGa has been investigated in a sample quenched from 1000 deg C. Magnetization, resistivity and x-ray diffraction measurements indicate that the structural phase transition occurs at approx 103 K, substantially lower than the value reported for samples quenched from 800 deg C and ordered in the Heusler L2 sub 1 structure. A small reduction in the ferromagnetic moment was also observed, although the Curie temperature remained largely unaffected. The electronic Sommerfeld coefficient obtained from heat capacity measurements is enhanced but smaller than that observed for the 800 deg C quenched sample. The results are consistent with band structure calculations and the electronic changes brought about by atomic disorder.

  18. Magnetic and Structural Properties of A-Site Ordered Chromium Spinel Sulfides: Alternating Antiferromagnetic and Ferromagnetic Interactions in the Breathing Pyrochlore Lattice

    Science.gov (United States)

    Okamoto, Yoshihiko; Mori, Masaki; Katayama, Naoyuki; Miyake, Atsushi; Tokunaga, Masashi; Matsuo, Akira; Kindo, Koichi; Takenaka, Koshi

    2018-03-01

    We report a comprehensive study on the magnetic and structural properties of the spinel sulfides LiInCr4S8, LiGaCr4S8, and CuInCr4S8, where Li+/Cu+ and Ga3+/In3+ ions form a zinc-blende-type order. On the basis of synchrotron X-ray diffraction and magnetization data obtained using polycrystalline samples, these three sulfides are suggested to be breathing pyrochlore magnets with alternating antiferromagnetic and ferromagnetic interactions on the small and large tetrahedra, respectively. The measured magnetization processes of the three sulfides up to 72 T are significantly different. The magnetization curves of LiInCr4S8 and CuInCr4S8 have large hysteresis loops with different shapes, while there is no hysteresis in that of LiGaCr4S8. Geometrical frustration of the small tetrahedron is likely to give rise to a wide variety of ground states, indicating the rich physics in these antiferromagnetic-ferromagnetic breathing pyrochlore magnets.

  19. HfMnSb{sub 2}: a metal-ordered NiAs-type pnictide with a conical spin order

    Energy Technology Data Exchange (ETDEWEB)

    Murakami, Taito; Yamamoto, Takafumi; Tassel, Cedric; Takatsu, Hiroshi; Ajiro, Yoshitami; Kageyama, Hiroshi [Graduate School of Engineering, Kyoto University, Kyoto, 615-8510 (Japan); Ritter, Clemens [Institut Laue-Langevin, 6, rue Jules Horowitz, Grenoble, 38000 (France)

    2016-08-16

    The NiAs-type structure is one of the most common structures in solids, but metal order has been almost exclusively limited to chalcogenides. The synthesis of HfMnSb{sub 2} is reported with a novel metal-ordered NiAs-type structure. HfMnSb{sub 2} undergoes a conical spin order below 270 K, in marked contrast to conventional magnetic order observed in NiAs-type pnictides. We argue that the layered arrangement of Hf and Mn makes it a quasi 2D magnet, where the Mn layers with localized magnetic moments (Mn{sup 2+}; S=5/2) can interact only through RKKY interactions, instead of metal-metal bonding that is otherwise dominant for typical NiAs-type pnictides. This result suggests that controlling order-disorder in NiAs-type pnictides enables a study of 2D-to-3D crossover behavior in itinerant magnetic system. (copyright 2016 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  20. Next-to-next-to-leading order gravitational spin-squared potential via the effective field theory for spinning objects in the post-Newtonian scheme

    International Nuclear Information System (INIS)

    Levi, Michele; Steinhoff, Jan

    2016-01-01

    The next-to-next-to-leading order spin-squared interaction potential for generic compact binaries is derived for the first time via the effective field theory for gravitating spinning objects in the post-Newtonian scheme. The spin-squared sector is an intricate one, as it requires the consideration of the point particle action beyond minimal coupling, and mainly involves the spin-squared worldline couplings, which are quite complex, compared to the worldline couplings from the minimal coupling part of the action. This sector also involves the linear in spin couplings, as we go up in the nonlinearity of the interaction, and in the loop order. Hence, there is an excessive increase in the number of Feynman diagrams, of which more are higher loop ones. We provide all the Feynman diagrams and their values. The beneficial ''nonrelativistic gravitational'' fields are employed in the computation. This spin-squared correction, which enters at the fourth post-Newtonian order for rapidly rotating compact objects, completes the conservative sector up to the fourth post-Newtonian accuracy. The robustness of the effective field theory for gravitating spinning objects is shown here once again, as demonstrated in a recent series of papers by the authors, which obtained all spin dependent sectors, required up to the fourth post-Newtonian accuracy. The effective field theory of spinning objects allows to directly obtain the equations of motion, and the Hamiltonians, and these will be derived for the potential obtained here in a forthcoming paper

  1. Intrinsic and spatially nonuniform ferromagnetism in Co-doped ZnO films

    Science.gov (United States)

    Tseng, L. T.; Suter, A.; Wang, Y. R.; Xiang, F. X.; Bian, P.; Ding, X.; Tseng, A.; Hu, H. L.; Fan, H. M.; Zheng, R. K.; Wang, X. L.; Salman, Z.; Prokscha, T.; Suzuki, K.; Liu, R.; Li, S.; Morenzoni, E.; Yi, J. B.

    2017-09-01

    Co doped ZnO films have been deposited by a laser-molecular beam epitaxy system. X-ray diffraction and UV spectra analysis show that Co effectively substitutes the Zn site. Transmission electron microscopy (TEM) and secondary ion mass spectroscopy analysis indicate that there are no clusters. Co dopants are uniformly distributed in ZnO film. Ferromagnetic ordering is observed in all samples deposited under an oxygen partial pressure, PO2=10-3 , 10-5, and 10-7 torr, respectively. However, the magnetization of PO2=10-3 and 10-5 is very small at room temperature. At low temperature, the ferromagnetic ordering is enhanced. Muon spin relaxation (μ SR ) measurements confirm the ferromagnetism in all samples, and the results are consistent with magnetization measurements. From μ SR and TEM analysis, the film deposited under PO2=10-7 torr shows intrinsic ferromagnetism. However, the volume fraction of the ferromagnetism phase is approximately 70%, suggesting that the ferromagnetism is not carrier mediated. Resistivity versus temperature measurements indicate Efros variable range hopping dominates the conductivity. From the above results, we can confirm that a bound magnetic polaron is the origin of the ferromagnetism.

  2. Next-to-next-to-leading order gravitational spin-orbit coupling via the effective field theory for spinning objects in the post-Newtonian scheme

    International Nuclear Information System (INIS)

    Levi, Michele; Steinhoff, Jan

    2016-01-01

    We implement the effective field theory for gravitating spinning objects in the post-Newtonian scheme at the next-to-next-to-leading order level to derive the gravitational spin-orbit interaction potential at the third and a half post-Newtonian order for rapidly rotating compact objects. From the next-to-next-to-leading order interaction potential, which we obtain here in a Lagrangian form for the first time, we derive straightforwardly the corresponding Hamiltonian. The spin-orbit sector constitutes the most elaborate spin dependent sector at each order, and accordingly we encounter a proliferation of the relevant Feynman diagrams, and a significant increase of the computational complexity. We present in detail the evaluation of the interaction potential, going over all contributing Feynman diagrams. The computation is carried out in terms of the ''nonrelativistic gravitational'' fields, which are advantageous also in spin dependent sectors, together with the various gauge choices included in the effective field theory for gravitating spinning objects, which also optimize the calculation. In addition, we automatize the effective field theory computations, and carry out the automated computations in parallel. Such automated effective field theory computations would be most useful to obtain higher order post-Newtonian corrections. We compare our Hamiltonian to the ADM Hamiltonian, and arrive at a complete agreement between the ADM and effective field theory results. Finally, we provide Hamiltonians in the center of mass frame, and complete gauge invariant relations among the binding energy, angular momentum, and orbital frequency of an inspiralling binary with generic compact spinning components to third and a half post-Newtonian order. The derivation presented here is essential to obtain further higher order post-Newtonian corrections, and to reach the accuracy level required for the successful detection of gravitational radiation

  3. Silicon spintronics with ferromagnetic tunnel devices

    International Nuclear Information System (INIS)

    Jansen, R; Sharma, S; Dash, S P; Min, B C

    2012-01-01

    In silicon spintronics, the unique qualities of ferromagnetic materials are combined with those of silicon, aiming at creating an alternative, energy-efficient information technology in which digital data are represented by the orientation of the electron spin. Here we review the cornerstones of silicon spintronics, namely the creation, detection and manipulation of spin polarization in silicon. Ferromagnetic tunnel contacts are the key elements and provide a robust and viable approach to induce and probe spins in silicon, at room temperature. We describe the basic physics of spin tunneling into silicon, the spin-transport devices, the materials aspects and engineering of the magnetic tunnel contacts, and discuss important quantities such as the magnitude of the spin accumulation and the spin lifetime in the silicon. We highlight key experimental achievements and recent progress in the development of a spin-based information technology. (topical review)

  4. Spin thermoelectric effects in organic single-molecule devices

    Energy Technology Data Exchange (ETDEWEB)

    Wang, H.L.; Wang, M.X.; Qian, C.; Hong, X.K.; Zhang, D.B.; Liu, Y.S.; Yang, X.F., E-mail: xfyang@cslg.edu.cn

    2017-05-25

    Highlights: • A stronger spin thermoelectric performance in a polyacetylene device is observed. • For the antiferromagnetic (AFM) ordering, a transport gap is opened. Thus the thermoelectric effects are largely enhanced. - Abstract: The spin thermoelectric performance of a polyacetylene chain bridging two zigzag graphene nanoribbons (ZGNRs) is investigated based on first principles method. Two different edge spin arrangements in ZGNRs are considered. For ferromagnetic (FM) ordering, transmission eigenstates with different spin indices distributed below and above Fermi level are observed, leading directly to a strong spin thermoelectric effect in a wide temperature range. With the edge spins arranged in the antiferromagnetic (AFM) ordering, an obvious transport gap appears in the system, which greatly enhances the thermoelectric effects. The presence of a small spin splitting also induces a spin thermoelectric effect greater than the charge thermoelectric effect in certain temperature range. In general, the single-molecule junction exhibits the potential to be used for the design of perfect thermospin devices.

  5. Evidence of spin-glass like ordering and exchange bias effect in antisite-disordered nanometric La1.5Ca0.5CoMnO6 double perovskite

    Science.gov (United States)

    Sahoo, R. C.; Paladhi, D.; Nath, T. K.

    2017-08-01

    Single-phase polycrystalline La1.5Ca0.5CoMnO6 double perovskite nanoparticles (∼25 nm) have been synthesized by chemical sol-gel method. We report here the structural, magnetic and transport properties using X-ray diffraction, dc magnetization, ac susceptibility, exchange bias and dc resistivity measurements. The Rietveld refinement of X-ray diffraction pattern reveals that the La1.5Ca0.5CoMnO6 (LCCMO) system crystallizes in orthorhombic structure with pbnm space group. Mn and Co ions are not completely ordered on the B sites due to the presence of about 30% antisite-disorder in the system. The ordering of Co2+ and Mn4+ gives rise to the ferromagnetism below 145 K. A spin glass like ground state has also been observed near 37.6(4) K, arising mainly due to the presence of competing magnetic interactions and antisite-disorder in the LCCMO nanoparticles. The frequency dependence peak shift of the Ac-susceptibility peak in the glassy state follows the critical slowing down model. The observed memory effect in ac susceptibility data reveals the existence of interacting clusters in a competing magnetic interactions state. The presence of noticeable exchange bias effect can be best explained on the basis of uncompensated interface (ferromagnetic/spin-glass) spins of antisite-disordered LCCMO system. This anti-site disordered nanocompound exhibits semiconducting behavior with variable range hopping kind of electronic conduction mechanism in the temperature range of 200-300 K. We have also observed large negative magnetoresistance (-30% at 100 K and 60 kOe) mainly due to the spin-polarized transport across the grain boundaries.

  6. Quantum spin-glass transition in the two-dimensional electron gas

    Indian Academy of Sciences (India)

    Home; Journals; Pramana – Journal of Physics; Volume 58; Issue 2 ... Spin glasses; quantum phase transition; ferromagnetism; electron gas. ... We argue that a quantum transition involving the destruction of the spin-glass order in an applied in-plane magnetic field offers a natural explanation of some features of recent ...

  7. Ab initio study of charge, spin and orbital ordering in manganites

    CERN Document Server

    Tyer, R

    2001-01-01

    The subject of this thesis was the calculation of the electronic structure for the manganites LaMnO sub 3 and CaMnO sub 3. The implementation of the Self-Interaction Corrected Local Spin Density (SIC-LSD) formalism within the Tight Binding Linear Muffin-Tin Orbital method in conjunction with the Atomic Sphere Approximation was used for these calculations. The SIC-LSD total energy functional has been used to investigate the spin ordering and valency of CaMnO sub 3 and LaMnO sub 3. In order to assess the role of the structural distortion in LaMnO sub 3 , these calculations were performed for an idealised cubic structure as well as for the observed distorted orthorhombic structure. Orbital rotations of the localised (SIC corrected) states were implemented. These orbital rotations were then used to perform the first ab-initio investigation of orbital ordering in LaMnO sub 3. For the experimentally observed A-type antiferromagnetic ordering, the correct orbital structure of alternating manganese d sub 3 sub x sub ...

  8. Spin ice Thin Film: Surface Ordering, Emergent Square ice, and Strain Effects

    Science.gov (United States)

    Jaubert, L. D. C.; Lin, T.; Opel, T. S.; Holdsworth, P. C. W.; Gingras, M. J. P.

    2017-05-01

    Motivated by recent realizations of Dy2 Ti2 O7 and Ho2 Ti2 O7 spin ice thin films, and more generally by the physics of confined gauge fields, we study a model spin ice thin film with surfaces perpendicular to the [001] cubic axis. The resulting open boundaries make half of the bonds on the interfaces inequivalent. By tuning the strength of these inequivalent "orphan" bonds, dipolar interactions induce a surface ordering equivalent to a two-dimensional crystallization of magnetic surface charges. This surface ordering may also be expected on the surfaces of bulk crystals. For ultrathin films made of one cubic unit cell, once the surfaces have ordered, a square ice phase is stabilized over a finite temperature window. The square ice degeneracy is lifted at lower temperature and the system orders in analogy with the well-known F transition of the 6-vertex model. To conclude, we consider the addition of strain effects, a possible consequence of interface mismatches at the film-substrate interface. Our simulations qualitatively confirm that strain can lead to a smooth loss of Pauling entropy upon cooling, as observed in recent experiments on Dy2 Ti2 O7 films.

  9. Standing magnetic wave on Ising ferromagnet: Nonequilibrium phase transition

    Energy Technology Data Exchange (ETDEWEB)

    Halder, Ajay, E-mail: ajay.rs@presiuniv.ac.in; Acharyya, Muktish, E-mail: muktish.physics@presiuniv.ac.in

    2016-12-15

    The dynamical response of an Ising ferromagnet to a plane polarised standing magnetic field wave is modelled and studied here by Monte Carlo simulation in two dimensions. The amplitude of standing magnetic wave is modulated along the direction x. We have detected two main dynamical phases namely, pinned and oscillating spin clusters. Depending on the value of field amplitude the system is found to undergo a phase transition from oscillating spin cluster to pinned as the system is cooled down. The time averaged magnetisation over a full cycle of magnetic field oscillations is defined as the dynamic order parameter. The transition is detected by studying the temperature dependences of the variance of the dynamic order parameter, the derivative of the dynamic order parameter and the dynamic specific heat. The dependence of the transition temperature on the magnetic field amplitude and on the wavelength of the magnetic field wave is studied at a single frequency. A comprehensive phase boundary is drawn in the plane described by the temperature and field amplitude for two different wavelengths of the magnetic wave. The variation of instantaneous line magnetisation during a period of magnetic field oscillation for standing wave mode is compared to those for the propagating wave mode. Also the probability that a spin at any site, flips, is calculated. The above mentioned variations and the probability of spin flip clearly distinguish between the dynamical phases formed by propagating magnetic wave and by standing magnetic wave in an Ising ferromagnet. - Highlights: • The Ising ferromagnet. • The system is driven by standing magnetic wave. • The low temperature pinned phase is observed • The high temperature oscillating spin bands are observed • The nonequilibrium phase boundary is drawn.

  10. Magnetic ordering in pressure-induced phases with giant spin-driven ferroelectricity in multiferroic TbMnO3

    Science.gov (United States)

    Terada, Noriki; Khalyavin, Dmitry D.; Manuel, Pascal; Osakabe, Toyotaka; Kikkawa, Akiko; Kitazawa, Hideaki

    2016-02-01

    In order to clarify the mechanism associated with pressure/magnetic-field-induced giant ferroelectric polarization in TbMnO3, this work investigated changes in magnetic ordering brought about by variations in temperature, magnetic field, and pressure. This was accomplished by means of neutron diffraction analyses under high pressures and high magnetic fields, employing a single crystal. The incommensurate magnetic ordering of a cycloid structure was found to be stable below the reported critical pressure of 4.5 GPa. In contrast, a commensurate E -type spin ordering of Mn spins and a noncollinear configuration of Tb spins with k =(0 ,1/2 ,0 ) appeared above 4.5 GPa. The application of a magnetic field along the a axis (H∥a) under pressure induces a k =(0 ,0 ,0 ) antiferromagnetic structure in the case of Tb spins above H∥a, enhancing the ferroelectric polarization, while the E -type ordering of Mn spins is stable even above the critical field. From the present experimental findings, we conclude that the E -type ordering of Mn spins induces giant ferroelectric polarization through an exchange striction mechanism. The H∥a-induced polarization enhancement can be understood by considering that the polarization, reduced by the polar ordering of Tb moments in a zero field, can be recovered through a field-induced change to nonpolar k =(0 ,0 ,0 ) ordering at H∥a˜2 T.

  11. Self-assembly of linear [Mn II 2 Mn III ] units with end-on azido bridges: the construction of a ferromagnetic chain using S T = 7 high-spin trimers

    KAUST Repository

    Jiang, Yuan

    2015-01-01

    © The Royal Society of Chemistry 2015. The controlled organization of high-spin complexes into 1D coordination polymers is a challenge in molecular magnetism. In this work, we report a ferromagnetic Mn trimer Mn3(HL)2(CH3OH)6(Br)4·Br·(CH3OH)21 (H2L = 2-[(9H-fluoren-9-yl)amino]propane-1,3-diol) with the ground spin state of ST = 7 that can be assembled into a one-dimensional coordination chain [Mn3(HL)2(CH3OH)2(Br)4(N3)(H2O)·CH3OH]∞2 using azido bridging ligands. Interestingly, the ferromagnetic nature of 1 is well retained in 2. However, due to the negligible magnetic anisotropy in 1, both 1 and 2 do not show slow-relaxation of magnetization, which indicates that during the process of molecular assembly not only the intratrimer magnetic interaction but also the magnetic anisotropy of the trimer can be reserved.

  12. Self-assembly of linear [Mn(II)2Mn(III)] units with end-on azido bridges: the construction of a ferromagnetic chain using ST = 7 high-spin trimers.

    Science.gov (United States)

    Jiang, Yuan; Qin, Lei; Li, Guanghua; Abbas, Ghulam; Cao, Yaqun; Wu, Gang; Han, Tian; Zheng, Yan-Zhen; Qiu, Shilun

    2015-03-21

    The controlled organization of high-spin complexes into 1D coordination polymers is a challenge in molecular magnetism. In this work, we report a ferromagnetic Mn trimer Mn3(HL)2(CH3OH)6(Br)4·Br·(CH3OH)2 1 (H2L = 2-[(9H-fluoren-9-yl)amino]propane-1,3-diol) with the ground spin state of ST = 7 that can be assembled into a one-dimensional coordination chain [Mn3(HL)2(CH3OH)2(Br)4(N3)(H2O)·CH3OH]∞ 2 using azido bridging ligands. Interestingly, the ferromagnetic nature of 1 is well retained in 2. However, due to the negligible magnetic anisotropy in 1, both 1 and 2 do not show slow-relaxation of magnetization, which indicates that during the process of molecular assembly not only the intratrimer magnetic interaction but also the magnetic anisotropy of the trimer can be reserved.

  13. Microscopic studies of nonlocal spin dynamics and spin transport (invited)

    Energy Technology Data Exchange (ETDEWEB)

    Adur, Rohan; Du, Chunhui; Cardellino, Jeremy; Scozzaro, Nicolas; Wolfe, Christopher S.; Wang, Hailong; Herman, Michael; Bhallamudi, Vidya P.; Pelekhov, Denis V.; Yang, Fengyuan; Hammel, P. Chris, E-mail: hammel@physics.osu.edu [Department of Physics, The Ohio State University, Columbus, Ohio 43210 (United States)

    2015-05-07

    Understanding the behavior of spins coupling across interfaces in the study of spin current generation and transport is a fundamental challenge that is important for spintronics applications. The transfer of spin angular momentum from a ferromagnet into an adjacent normal material as a consequence of the precession of the magnetization of the ferromagnet is a process known as spin pumping. We find that, in certain circumstances, the insertion of an intervening normal metal can enhance spin pumping between an excited ferromagnetic magnetization and a normal metal layer as a consequence of improved spin conductance matching. We have studied this using inverse spin Hall effect and enhanced damping measurements. Scanned probe magnetic resonance techniques are a complementary tool in this context offering high resolution magnetic resonance imaging, localized spin excitation, and direct measurement of spin lifetimes or damping. Localized magnetic resonance studies of size-dependent spin dynamics in the absence of lithographic confinement in both ferromagnets and paramagnets reveal the close relationship between spin transport and spin lifetime at microscopic length scales. Finally, detection of ferromagnetic resonance of a ferromagnetic film using the photoluminescence of nitrogen vacancy spins in neighboring nanodiamonds demonstrates long-range spin transport between insulating materials, indicating the complexity and generality of spin transport in diverse, spatially separated, material systems.

  14. Evidence for Crossed Andreev Reflections in (100)YBa2Cu3O7+δ-SrRuO3 superconductor-ferromagnet bilayers

    International Nuclear Information System (INIS)

    Asulin, I.; Yuli, O.; Millo, O.; Koren, G.

    2005-01-01

    Full Text:Since the ferromagnetic side of a superconductor-ferromagnet junction is spin polarized, Andreev reflections are suppressed. Consequently, the proximity induced superconductor order parameter in the ferromagnet is expected to decay rapidly, on the order of a nm, the typical coherence length in a ferromagnet. Our scanning tunneling spectroscopy measurements on thin epitaxial (100)YBa 2 Cu 3 O 7+ δ-SrRuO 3 (YBaCuO-SrO) bilayers, where SrO is a ferromagnet, indeed show that on most of the junction area the superconductor order parameter vanishes in the SrO layers thicker than 8 nm. However, we find localized regions, arranged along narrow (< 10 nm) stripes, where the order parameter (superconductor-like gap structure) penetrates the ferromagnet over more than 20 nm. This is attributed to 'Crossed Andreev Reflections,' taking place at domain boundaries, where an electron from one magnetic domain is retro reflected as a hole with opposite spin in an adjacent domain. Our observation may account for the (not abundant) cases where a long-range proximity effect was found in superconductor-ferromagnet proximity systems

  15. Experimental Studies of Spin, Charge and Orbital Order at Extreme Conditions

    OpenAIRE

    Carlsson, Sandra J E

    2009-01-01

    Spin, charge and orbital ordering in various crystalline compounds have been studied under extreme conditions. The main techniques used were synchrotron X-ray and neutron powder diffraction. High-pressure conditions were obtained by using a diamond anvil cell and the Paris-Edinburgh cell. Changes in the valence state of BiNiO3 perovskite under pressure have been investigated by a neutron powder diffraction study and bond valence sum (BVS) calculations. At ambient pressure, BiNiO3 has the u...

  16. Transport through hybrid superconducting/ferromagnetic double-path junction

    Energy Technology Data Exchange (ETDEWEB)

    Facio, T.J.S. [Departamento de Física e Química, Universidade Estadual Paulista – UNESP, 15385-000, Ilha Solteira, SP (Brazil); Orellana, P.A. [Departamento de Física, Universidad Técnica Federico Santa Maria, Av. Vicuña Mackenna, 3939, Santiago (Chile); Jurelo, A.R. [Departamento de Física, Universidade Estadual de Ponta Grossa – UEPG, 84030-000, Ponta Grossa, PR (Brazil); Figueira, M.S. [Instituto de Física, Universidade Federal Fluminense, 24210-340, Niterói, RJ (Brazil); Cabrera, G.G. [Instituto de Física ‘Gleb Wataghin’, Universidade Estadual de Campinas – UNICAMP, 13083-859, Campinas, SP (Brazil); Siqueira, E.C., E-mail: ecosta@utfpr.edu.br [Departamento de Física, Universidade Tecnológica Federal do Paraná – UTFPR, 84016-210, Ponta Grossa, PR (Brazil)

    2017-02-05

    In this paper we study a double-path junction formed by a ferromagnetic and a superconductor lead. The first path connects the superconductor and ferromagnet directly while the second path connects these metals through a quantum dot. The whole system works as an Aharonov–Bohm interferometer allowing the study of the interference between these two paths under the presence of spin imbalance and Andreev bound states. We considered the effect of Fano interference on the electronic transmittance through the quantum dot and observed two regimes of conduction depending on the strength of the direct coupling. For the weak coupling regime, the transmittance presented the usual four resonances due to the Andreev bound states whereas for the strong coupling regime the profile was inverted and resonances became anti-resonances. However, even in the strong coupling regime it was possible to observe a central resonance due to the interference between the Andreev bound states. We have also studied the signatures of Fano interference on the average occupation within the quantum dot. The spin accumulation was analyzed and how it depends on the direct coupling and an external magnetic field applied to the system. The results obtained may be used in a possible experimental implementation of this system in order to probe spin related effects in ferromagnetic superconductor nanostructures. - Highlights: • An Aharonov–Bohm interferometer composed by a quantum-dot coupled to a superconductor and ferromagnetic lead is studied. • The transmittance through the QD is determined by the interplay between Andreev and Fano interference. • Spin accumulation within the quantum dot is studied as a function of bias/gate voltages and an external magnetic flux.

  17. Sound dispersion in a spin-1 Ising system near the second-order phase transition point

    International Nuclear Information System (INIS)

    Erdem, Ryza; Keskin, Mustafa

    2003-01-01

    Sound dispersion relation is derived for a spin-1 Ising system and its behaviour near the second-order phase transition point or the critical point is analyzed. The method used is a combination of molecular field approximation and Onsager theory of irreversible thermodynamics. If we assume a linear coupling of sound wave with the order parameter fluctuations in the system, we find that the dispersion which is the relative sound velocity change with frequency behaves as ω 0 ε 0 , where ω is the sound frequency and ε the temperature distance from the critical point. In the ordered region, one also observes a frequency-dependent velocity or dispersion minimum which is shifted from the corresponding attenuation maxima. These phenomena are in good agreement with the calculations of sound velocity in other magnetic systems such as magnetic metals, magnetic insulators, and magnetic semiconductors

  18. Photoemission and ferromagnetism

    International Nuclear Information System (INIS)

    Johnson, P.D.

    1994-01-01

    Photoemission is a well established technique for the study of the electronic structure of atoms and solids. In particular, angle-resolved photoemission has been used extensively to map the band structure of clean and adsorbate covered surfaces, both metal and semiconductor. Extending the technique by measuring the spin of the photoemitted electrons allows the possibility of examining the exchange split band structures characterizing ferromagnetic systems. Here the technique becomes particularly useful in the study of the magnetic properties of surfaces, thin films and associated interfaces

  19. Room temperature ferromagnetism in liquid-phase pulsed laser ablation synthesized nanoparticles of nonmagnetic oxides

    International Nuclear Information System (INIS)

    Singh, S. C.; Gopal, R.; Kotnala, R. K.

    2015-01-01

    Intrinsic Room Temperature Ferromagnetism (RTF) has been observed in undoped/uncapped zinc oxide and titanium dioxide spherical nanoparticles (NPs) obtained by a purely green approach of liquid phase pulsed laser ablation of corresponding metal targets in pure water. Saturation magnetization values observed for zinc oxide (average size, 9 ± 1.2 nm) and titanium dioxide (average size, 4.4 ± 0.3 nm) NPs are 62.37 and 42.17 memu/g, respectively, which are several orders of magnitude larger than those of previous reports. In contrast to the previous works, no postprocessing treatments or surface modification is required to induce ferromagnetism in the case of present communication. The most important result, related to the field of intrinsic ferromagnetism in nonmagnetic materials, is the observation of size dependent ferromagnetism. Degree of ferromagnetism in titanium dioxide increases with the increase in particle size, while it is reverse for zinc oxide. Surface and volume defects play significant roles for the origin of RTF in zinc oxide and titanium dioxide NPs, respectively. Single ionized oxygen and neutral zinc vacancies in zinc oxide and oxygen and neutral/ionized titanium vacancies in titanium dioxide are considered as predominant defect centres responsible for observed ferromagnetism. It is expected that origin of ferromagnetism is a consequence of exchange interactions between localized electron spin moments resulting from point defects

  20. Fourth-order wave equation in Bhabha-Madhavarao spin-3 2 theory

    Science.gov (United States)

    Markov, Yu. A.; Markova, M. A.; Bondarenko, A. I.

    2017-09-01

    Within the framework of the Bhabha-Madhavarao formalism, a consistent approach to the derivation of a system of the fourth-order wave equations for the description of a spin-3 2 particle is suggested. For this purpose an additional algebraic object, the so-called q-commutator (q is a primitive fourth root of unity) and a new set of matrices ημ, instead of the original matrices βμ of the Bhabha-Madhavarao algebra, are introduced. It is shown that in terms of the ημ matrices we have succeeded in reducing a procedure of the construction of fourth root of the fourth-order wave operator to a few simple algebraic transformations and to some operation of the passage to the limit z → q, where z is some (complex) deformation parameter entering into the definition of the η-matrices. In addition, a set of the matrices 𝒫1/2 and 𝒫3/2(±)(q) possessing the properties of projectors is introduced. These operators project the matrices ημ onto the spins 1/2- and 3/2-sectors in the theory under consideration. A corresponding generalization of the obtained results to the case of the interaction with an external electromagnetic field introduced through the minimal coupling scheme is carried out. The application to the problem of construction of the path integral representation in para-superspace for the propagator of a massive spin-3 2 particle in a background gauge field within the Bhabha-Madhavarao approach is discussed.

  1. Second order formalism for spin (1/2) fermions and Compton scattering

    International Nuclear Information System (INIS)

    Delgado-Acosta, E. G.; Napsuciale, Mauro; Rodriguez, Simon

    2011-01-01

    We develop a second order formalism for massive spin 1/2 fermions based on the projection over Poincare invariant subspaces in the ((1/2),0)+(0,(1/2)) representation of the homogeneous Lorentz group. Using the U(1) em gauge principle we obtain a second order description for the electromagnetic interactions of a spin 1/2 fermion with two free parameters, the gyromagnetic factor g and a parameter ξ related to odd-parity Lorentz structures. We calculate Compton scattering in this formalism. In the particular case g=2, ξ=0, and for states with well-defined parity, we recover Dirac results. In general, we find the correct classical limit and a finite value r c 2 for the forward differential cross section, independent of the photon energy and of the value of the parameters g and ξ. The differential cross section vanishes at high energies for all g, ξ except in the forward direction. The total cross section at high energies vanishes only for g=2, ξ=0. We argue that this formalism is more convenient than Dirac theory in the description of low energy electromagnetic properties of baryons and illustrate the point with the proton case.

  2. Proximity effect between a ferromagnetic insulator and a superconductor

    Energy Technology Data Exchange (ETDEWEB)

    Wolf, Michael J.; Beckmann, Detlef [Karlsruher Institut fuer Technologie (KIT), Karlsruhe (Germany). Inst. fuer Nanotechnologie; Huebler, Florian [Karlsruher Institut fuer Technologie (KIT), Karlsruhe (Germany). Inst. fuer Nanotechnologie; Karlsruher Institut fuer Technologie (KIT), Karlsruhe (Germany). Inst. fuer Festkoerperphysik; Suergers, Christoph [Karlsruher Institut fuer Technologie (KIT), Karlsruhe (Germany). Physikalisches Inst.; Loehneysen, Hilbert von [Karlsruher Institut fuer Technologie (KIT), Karlsruhe (Germany). Inst. fuer Festkoerperphysik; Karlsruher Institut fuer Technologie (KIT), Karlsruhe (Germany). Physikalisches Inst.

    2012-07-01

    Electron transfer through spin-active interfaces can be modeled by the transmission amplitudes and a relative phase shift between spin-up and spin-down wavefunctions, the spin-mixing angle. Recently, Andreev bound states have been observed in F/S tunnel contacts which imply a non-zero spin-mixing angle of the ultrathin F/S barrier. In order to separate the spin-active interface from the detector tunnel contact, we have fabricated normal metal/superconductor tunnel contacts on top of a ferromagnetic insulator. We prepared EuS thin films (d{approx}20 nm) on top of Si(111) substrates by means of e-beam evaporation and created Al/Al-Oxide/Cu tunnel contacts by means of shadow evaporation. In an applied magnetic field, the tunnel spectra show an enhanced Zeeman splitting which is due to the presence of the exchange field of the EuS layer. Furthermore, we observe small peaks in the subgap region of the tunnel spectra which may be attributed to Andreev bound states due to a non-zero spin-mixing angle at the EuS/Al interface. The results suggest the use of EuS thin films for generating equal-spin triplet superconductivity.

  3. PREFACE: Half Metallic Ferromagnets

    Science.gov (United States)

    Dowben, Peter

    2007-08-01

    Since its introduction by de Groot and colleagues in the early 1980s [1], the concept of half metallic ferromagnetism has attracted great interest. Idealized, half-metals have only one spin channel for conduction: the spin-polarized band structure exhibits metallic behavior for one spin channel, while the other spin band structure exhibits a gap at the Fermi level. Due to the gap for one spin direction, the density of states at the Fermi level has, theoretically, 100 & spin polarization. This gap in the density of states in one spin at the Fermi level, for example ↓ so N↓ (EF) = 0, also causes the resistance of that channel to go to infinity. At zero or low temperatures, the nonquasiparticle density of states (electron correlation effects), magnons and spin disorder reduce the polarization from the idealized 100 & polarization. At higher temperatures magnon-phonon coupling and irreversible compositional changes affect polarization further. Strategies for assessing and reducing the effects of finite temperatures on the polarization are now gaining attention. The controversies surrounding the polarization stability of half metallic ferromagnets are not, however, limited to the consideration of finite temperature effects alone. While many novel half metallic materials have been predicted, materials fabrication can be challenging. Defects, surface and interface segregation, and structural stability can lead to profound decreases in polarization, but can also suppress long period magnons. There is a 'delicate balance of energies required to obtain half metallic behaviour: to avoid spin flip scattering, tiny adjustments in atomic positions might occur so that a gap opens up in the other spin channel' [2]. When considering 'spintronics' devices, a common alibi for the study of half metallic systems, surfaces and interfaces become important. Free enthalpy differences between the surface and the bulk will lead to spin minority surface and interface states, as well as

  4. Charge, spin and orbital order in the candidate multiferroic material LuFe2O4

    International Nuclear Information System (INIS)

    Groot, Joost de

    2012-01-01

    This thesis is a detailed study of the magnetic, structural and orbital order parameters of the candidate multiferroic material LuFe 2 O 4 . Multiferroic oxides with a strong magnetoelectric coupling are of high interest for potential information technology applications, but they are rare because the traditional mechanism of ferroelectricity is incompatible with magnetism. Consequently, much attention is focused on various unconventional mechanisms of ferroelectricity. Of these, ferroelectricity originating from charge ordering (CO) is particularly intriguing because it potentially combines large electric polarizations with strong magneto-electric coupling. However, examples of oxides where this mechanism occurs are exceedingly rare and none is really well understood. LuFe 2 O 4 is often cited as the prototypical example of CO-based ferroelectricity. In this material, the order of Fe valences has been proposed to render the triangular Fe/O bilayers polar by making one of the two layers rich in Fe 2+ and the other rich in Fe 3+ , allowing for a possible ferroelectric stacking of the individual bilayers. Because of this new mechanism for ferroelectricity, and also because of the high transition temperatures of charge order (T CO ∝320K) and ferro magnetism (T N ∝240 K) LuFe 2 O 4 has recently attracted increasing attention. Although these polar bilayers are generally accepted in the literature for LuFe 2 O 4 , direct proof is lacking. An assumption-free experimental determination of whether or not the CO in the Fe/O bilayers is polar would be crucial, given the dependence of the proposed mechanism of ferroelectricity from CO in LuFe 2 O 4 on polar bilayers. This thesis starts with a detailed characterization of the macroscopic magnetic properties, where growing ferrimagnetic contributions observed in magnetization could be ascribed to increasing oxygen off-stoichiometry. The main focus is on samples exhibiting a sharp magnetic transition to long-range spin order

  5. Ferromagnetic insulating and spin glass properties of La{sub 0.7}Sr{sub 0.3}MnO{sub 3}-TiO{sub 2} composites

    Energy Technology Data Exchange (ETDEWEB)

    Phong, P.T., E-mail: ptphong.nh@khanhhoa.edu.vn [Department of Advanced Materials Chemistry, Dongguk University, 707 Suckjang-dong, Gyeongju-Si, Gyeonbuk 780-714 (Korea, Republic of); Nha Trang Pedagogic College, 01 Nguyen Chanh Street, Nha Trang City, Khanh Hoa Province (Viet Nam); Manh, D.H.; Phuc, N.X. [Institute of Materials Science, Vietnam Academy of Science and Technology, 18 Hoang Quoc Viet Road, Cau Giay District, Ha Noi (Viet Nam); Lee, I.-J. [Department of Advanced Materials Chemistry, Dongguk University, 707 Suckjang-dong, Gyeongju-Si, Gyeonbuk 780-714 (Korea, Republic of)

    2013-01-01

    In this study, the effect of TiO{sub 2} doping on the electro-magnetic properties of (1-x)La{sub 0.7}Sr{sub 0.3}MnO{sub 3}+xTiO{sub 2} (with 0%{<=}x{<=}6%, in wt%) composites has been investigated. X-ray diffraction observations show the evidence of reaction between the La{sub 0.7}Sr{sub 0.3}MnO{sub 3} and TiO{sub 2} grains. Also the results show that by increasing TiO{sub 2} doping levels, the metal insulator transition temperatures decrease and the system becomes an insulator. Furthermore, the paramagnetic-ferromagnetic transition temperature also decreases as TiO{sub 2} content increases. The spin glass state exists in the composites with x=5% and 6%. The dynamic properties of the magnetic properties are investigated by temperature dependence of dc magnetization and frequency dependence of ac susceptibilities. A dynamic scaling analysis of ac susceptibility data using conventional critical slowing down indicates that a finite spin-glass phase-transition temperature (T{sub g}) and a dynamic exponent (zv) change from 103 K and 9.30 correspondingly for 0.95La{sub 0.7}Sr{sub 0.3}MnO{sub 3}/0.05TiO{sub 2} to 133 K and 9.10, for 0.94La{sub 0.7}Sr{sub 0.3}MnO{sub 3}/0.06TiO{sub 2}. In addition, MR in low temperature of these samples decline simultaneously with occur spin-glass behavior. These results are interpreted as the dilution of Mn{sup 3+}/Mn{sup 4+} interactions by the random Ti substitution on the Mn site considerably reduces the ferromagnetic double exchange interaction within the manganese lattice.

  6. Spin gating electrical current

    Science.gov (United States)

    Ciccarelli, C.; Zârbo, L. P.; Irvine, A. C.; Campion, R. P.; Gallagher, B. L.; Wunderlich, J.; Jungwirth, T.; Ferguson, A. J.

    2012-09-01

    The level of the chemical potential is a fundamental parameter of the electronic structure of a physical system, which consequently plays an important role in defining the properties of active electrical devices. We directly measure the chemical potential shift in the relativistic band structure of the ferromagnetic semiconductor (Ga,Mn)As, controlled by changes in its magnetic order parameter. Our device comprises a non-magnetic aluminum single electron channel capacitively coupled to the (Ga,Mn)As gate electrode. The chemical potential shifts of the gate are directly read out from the shifts in the Coulomb blockade oscillations of the single electron transistor. The experiments introduce a concept of spin gating electrical current. In our spin transistor spin manipulation is completely removed from the electrical current carrying channel.

  7. High frequency spin torque oscillators with composite free layer spin valve

    International Nuclear Information System (INIS)

    Natarajan, Kanimozhi; Arumugam, Brinda; Rajamani, Amuda

    2016-01-01

    We report the oscillations of magnetic spin components in a composite free layer spin valve. The associated Landau–Lifshitz–Gilbert–Slonczewski (LLGS) equation is studied by stereographically projecting the spin on to a complex plane and the spin components were found. A fourth order Runge–Kutta numerical integration on LLGS equation also confirms the similar trajectories of the spin components. This study establishes the possibility of a Spin Torque Oscillator in a composite free layer spin valve, where the exchange coupling is ferromagnetic in nature. In-plane and out-of-plane precessional modes of magnetization oscillations were found in zero applied magnetic field and the frequencies of the oscillations were calculated from Fast Fourier Transform of the components of magnetization. Behavior of Power Spectral Density for a range of current density is studied. Finally our analysis shows the occurrence of highest frequency 150 GHz, which is in the second harmonics for the specific choice of system parameters.

  8. Spin Hall effects in metallic antiferromagnets – perspectives for future spin-orbitronics

    Directory of Open Access Journals (Sweden)

    Joseph Sklenar

    2016-05-01

    Full Text Available We investigate angular dependent spin-orbit torques from the spin Hall effect in a metallic antiferromagnet using the spin-torque ferromagnetic resonance technique. The large spin Hall effect exists in PtMn, a prototypical CuAu-I-type metallic antiferromagnet. By applying epitaxial growth, we previously reported an appreciable difference in spin-orbit torques for c- and a-axis orientated samples, implying anisotropic effects in magnetically ordered materials. In this work we demonstrate through bipolar-magnetic-field experiments a small but noticeable asymmetric behavior in the spin-transfer-torque that appears as a hysteresis effect. We also suggest that metallic antiferromagnets may be good candidates for the investigation of various unidirectional effects related to novel spin-orbitronics phenomena.

  9. Magnetic order, magnetic correlations, and spin dynamics in the pyrochlore antiferromagnet Er2Ti2O7

    Science.gov (United States)

    Dalmas de Réotier, P.; Yaouanc, A.; Chapuis, Y.; Curnoe, S. H.; Grenier, B.; Ressouche, E.; Marin, C.; Lago, J.; Baines, C.; Giblin, S. R.

    2012-09-01

    Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of the ground state, leading to an ordered state. Here we report detailed measurements of the low-temperature magnetic properties of Er2Ti2O7, which displays a second-order phase transition at TN≃1.2 K with coexisting short- and long-range orders. Magnetic susceptibility studies show that there is no spin-glass-like irreversible effect. Heat capacity measurements reveal that the paramagnetic critical exponent is typical of a 3-dimensional XY magnet while the low-temperature specific heat sets an upper limit on the possible spin-gap value and provides an estimate for the spin-wave velocity. Muon spin relaxation measurements show the presence of spin dynamics in the nanosecond time scale down to 21 mK. This time range is intermediate between the shorter time characterizing the spin dynamics in Tb2Sn2O7, which also displays long- and short-range magnetic order, and the time scale typical of conventional magnets. Hence the ground state is characterized by exotic spin dynamics. We determine the parameters of a symmetry-dictated Hamiltonian restricted to the spins in a tetrahedron, by fitting the paramagnetic diffuse neutron scattering intensity for two reciprocal lattice planes. These data are recorded in a temperature region where the assumption that the correlations are limited to nearest neighbors is fair.

  10. Coexistence of ferromagnetism and unconventional spin-glass freezing in the site-disordered kagome ferrite SrS n2F e4O11

    Science.gov (United States)

    Shlyk, L.; Strobel, S.; Farmer, B.; De Long, L. E.; Niewa, R.

    2018-02-01

    Single-crystal x-ray diffraction refinements indicate SrS n2F e4O11 crystallizes in the hexagonal R -type ferrite structure with noncentrosymmetric space group P 63m c and lattice parameters a =5.9541 (2 )Å , c =13.5761 (5 )Å , Z =2 (R (F )=0.034 ). Octahedrally coordinated 2 a [M (1) and M (1a)] and 6 c sites [M (2 )] have random, mixed occupation by Sn and Fe; whereas the tetrahedrally coordinated 2 b sites [Fe(3) and Fe(3a)] are exclusively occupied by Fe, whose displacement from the ideal position with trigonal-bipyramidal coordination causes the loss of inversion symmetry. Our dc and ac magnetization data indicate SrS n2F e4O11 single crystals undergo a ferro- or ferri-magnetic transition below a temperature TC=630 K with very low coercive fields μoHc ⊥=0.27 Oe and μoHc ∥=1.5 Oe at 300 K, for applied field perpendicular and parallel to the c axis, respectively. The value for TC is exceptionally high, and the coercive fields exceptionally low, among the known R-type ferrites. Time-dependent dc magnetization and frequency-dependent ac magnetization data indicate the onset of short-range, spin-glass freezing below Tf=35.8 K , which results from crystallographic disorder of magnetic F e3 + and nonmagnetic S n4 + ions on a frustrated Kagome sublattice. Anomalous ac susceptibility and thermomagnetic relaxation behavior in the short-range-ordered state differs from that of conventional spin glasses. Optical measurements in the ultraviolet to visible frequency range in a diffuse reflectance geometry indicate an overall optical band gap of 0.8 eV, consistent with observed semiconducting properties.

  11. Evidence of spin-glass like ordering and exchange bias effect in antisite-disordered nanometric La{sub 1.5}Ca{sub 0.5}CoMnO{sub 6} double perovskite

    Energy Technology Data Exchange (ETDEWEB)

    Sahoo, R.C.; Paladhi, D.; Nath, T.K., E-mail: tnath@phy.iitkgp.ernet.in

    2017-08-15

    Highlights: • SG has been observed due to antisite disorder and different magnetic interactions. • The observed EB can be best explained on the basis of uncompensated interface spins. • −30% MR has been observed due to the spin-polarized transport at grain boundaries. - Abstract: Single-phase polycrystalline La{sub 1.5}Ca{sub 0.5}CoMnO{sub 6} double perovskite nanoparticles (∼25 nm) have been synthesized by chemical sol-gel method. We report here the structural, magnetic and transport properties using X-ray diffraction, dc magnetization, ac susceptibility, exchange bias and dc resistivity measurements. The Rietveld refinement of X-ray diffraction pattern reveals that the La{sub 1.5}Ca{sub 0.5}CoMnO{sub 6} (LCCMO) system crystallizes in orthorhombic structure with pbnm space group. Mn and Co ions are not completely ordered on the B sites due to the presence of about 30% antisite-disorder in the system. The ordering of Co{sup 2+} and Mn{sup 4+} gives rise to the ferromagnetism below 145 K. A spin glass like ground state has also been observed near 37.6(4) K, arising mainly due to the presence of competing magnetic interactions and antisite-disorder in the LCCMO nanoparticles. The frequency dependence peak shift of the Ac-susceptibility peak in the glassy state follows the critical slowing down model. The observed memory effect in ac susceptibility data reveals the existence of interacting clusters in a competing magnetic interactions state. The presence of noticeable exchange bias effect can be best explained on the basis of uncompensated interface (ferromagnetic/spin-glass) spins of antisite-disordered LCCMO system. This anti-site disordered nanocompound exhibits semiconducting behavior with variable range hopping kind of electronic conduction mechanism in the temperature range of 200–300 K. We have also observed large negative magnetoresistance (−30% at 100 K and 60 kOe) mainly due to the spin-polarized transport across the grain boundaries.

  12. The effect of partial order on galvanomagnetic transport properties of ferromagnetic PdFe and PdCo alloys

    Czech Academy of Sciences Publication Activity Database

    Kudrnovský, Josef; Drchal, Václav; Turek, Ilja

    2015-01-01

    Roč. 92, č. 22 (2015), "224421-1"-"224421-8" ISSN 1098-0121 R&D Projects: GA ČR GA15-13436S Institutional support: RVO:68378271 ; RVO:68081723 Keywords : anomalous Hall effect * anisotropis magnetoresistance * first-principles * effect of ordering Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.736, year: 2014

  13. Evidence of spin transition and charge order in cobalt substituted La sub 0 sub . sub 7 Ca sub 0 sub . sub 3 MnO sub 3

    CERN Document Server

    Srivastava, C M; Gundurao, T K; Nigam, A K; Bahadur, D

    2003-01-01

    The transport and magnetic studies of a series of compounds having the general formula La sub 0 sub . sub 7 Ca sub 0 sub . sub 3 Mn sub 1 sub - sub x Co sub x O sub 3 (0.1 = 0.25 there is a clear spin transition at low temperature from the high to the low spin state of trivalent cobalt and this leads to change in ferromagnetic (FM) and antiferromagnetic (AFM) phases. For x >= 0.25 there are two transitions for each value of x: the upper one gives the FM and AFM spin arrangement depending upon whether the DE or the SE dominates; the lower one is obtained due to the transition from the high to the low spin state of the trivalent cobalt ion.

  14. Coexistence of ferromagnetism and spin glass freezing in the site-disordered kagome ferrite SrSn2Fe4O11

    Science.gov (United States)

    Shlyk, Larysa; Strobel, S.; Farmer, B.; De Long, L. E.; Niewa, R.

    2018-05-01

    Single-crystal x-ray diffraction refinements indicate SrSn2Fe4O11 crystallizes in the hexagonal R-type ferrite structure with non-centrosymmetric space group P63mc and lattice parameters a = 5.9541(2) Å, c = 13.5761(5) Å, Z = 2 (R(F) = 0.034). Octahedrally coordinated sites are randomly occupied by Sn and Fe; whereas tetrahedrally coordinated sites are exclusively occupied by Fe, whose displacement from ideal trigonal-bipyramidal coordination causes the loss of inversion symmetry. DC magnetization data indicate SrSn2Fe4O11 single crystals undergo ferro- or ferri-magnetic order below a transition temperature TC = 630 K with very low coercive fields Hc ⊥ = 0.27 Oe and Hc// = 1.5 Oe at 300 K, for applied fields perpendicular and parallel to the c-axis, respectively. The value for TC is exceptionally high, and the coercive fields exceptionally low, among the known R-type ferrites. Enhanced coercivity and thermomagnetic hysteresis suggest the onset of short-range, spin glass order occurs below Tf = 35 K. Optical measurements indicate a band gap of 0.8 eV, consistent with wide-gap semiconducting behavior and a previously established empirical correlation between the semiconducting gap and TC for R-type ferrites based upon Ru.

  15. Spin precession and spin Hall effect in monolayer graphene/Pt nanostructures

    Science.gov (United States)

    Savero Torres, W.; Sierra, J. F.; Benítez, L. A.; Bonell, F.; Costache, M. V.; Valenzuela, S. O.

    2017-12-01

    Spin Hall effects have surged as promising phenomena for spin logics operations without ferromagnets. However, the magnitude of the detected electric signals at room temperature in metallic systems has been so far underwhelming. Here, we demonstrate a two-order of magnitude enhancement of the signal in monolayer graphene/Pt devices when compared to their fully metallic counterparts. The enhancement stems in part from efficient spin injection and the large spin resistance of graphene but we also observe 100% spin absorption in Pt and find an unusually large effective spin Hall angle of up to 0.15. The large spin-to-charge conversion allows us to characterise spin precession in graphene under the presence of a magnetic field. Furthermore, by developing an analytical model based on the 1D diffusive spin-transport, we demonstrate that the effective spin-relaxation time in graphene can be accurately determined using the (inverse) spin Hall effect as a means of detection. This is a necessary step to gather full understanding of the consequences of spin absorption in spin Hall devices, which is known to suppress effective spin lifetimes in both metallic and graphene systems.

  16. Impact of temperature-dependent local and global spin order in RMnO3 compounds for spin-phonon coupling and electromagnon activity

    Science.gov (United States)

    Elsässer, S.; Schiebl, M.; Mukhin, A. A.; Balbashov, A. M.; Pimenov, A.; Geurts, J.

    2017-01-01

    The orthorhombic rare-earth manganite compounds RMnO3 show a global magnetic order for T {T}{{cycl}}, in contrast to the hitherto assumed incommensurate sinusoidal phase in the intermediate temperature range. The development of the magnetization pattern can be described in terms of an order-disorder transition at T cycl within a pseudospin model of localized spin cycloids with opposite chirality.

  17. Effect of quenched disorder on charge-orbital-spin ordering in single-layer manganites

    International Nuclear Information System (INIS)

    Uchida, Masaya; Mathieu, Roland; He, Jinping; Kaneko, Yoshio; Tokura, Yoshinori; Asamitsu, Atsushi; Kumai, Reiji; Tomioka, Yasuhide; Matsui, Yoshio

    2006-01-01

    Structural and magnetic properties have been investigated for half-doped single-layer manganites RE 0.5 Sr 1.5 MnO 4 [RE=La, (La, Pr), Pr, Nd, Sm, and Eu]. Analyses of electron diffraction and ac susceptibility measurements have revealed that the long-range charge-orbital ordering (CO-OO) state as observed in La 0.5 Sr 1.5 MnO 4 is suppressed for the other materials: the CO-OO transition temperature, as well as the correlation length decreases with a decrease in the cation size of RE. Such a short-range CO-OO state shows a spin-glass behavior at low temperatures. A new electronic phase diagram is established with quenched disorder as the control parameter. (author)

  18. Long Range Order and Spin-Fluctuations in Strongly Correlated Electron System with Valence Instability

    Science.gov (United States)

    Alekseev, P. A.; Menushenkov, A. P.; Mignot, J.-M.; Nemkovski, K. S.; Yaroslavtsev, A. A.; Kozlenko, D. P.

    Rare-earth based strongly correlated electron systems (SCES) exhibit a large variety of different ground states, ranging from the simple paramagnetism of crystal-field-split f-electron multiplets to highly unconventional Kondo-insulator states with a combination of charge gap, spin gap and valence instability, in which long-range magnetic order can eventually arise from an initially singlet state. The physical background for these properties of the electron subsystem may be clarified by performing detailed neutron scattering experiments, namely magnetic neutron scattering spectroscopy and diffraction. This report reviews the results of the previous and new experimental studies on a number of rare-earth intermetallic compounds, which shed light on peculiar features of those unusual ground states.

  19. Unifying Exchange Sensitivity in Transition-Metal Spin-State Ordering and Catalysis through Bond Valence Metrics.

    Science.gov (United States)

    Gani, Terry Z H; Kulik, Heather J

    2017-11-14

    Accurate predictions of spin-state ordering, reaction energetics, and barrier heights are critical for the computational discovery of open-shell transition-metal (TM) catalysts. Semilocal approximations in density functional theory, such as the generalized gradient approximation (GGA), suffer from delocalization error that causes them to overstabilize strongly bonded states. Descriptions of energetics and bonding are often improved by introducing a fraction of exact exchange (e.g., erroneous low-spin GGA ground states are instead correctly predicted as high-spin with a hybrid functional). The degree of spin-splitting sensitivity to exchange can be understood based on the chemical composition of the complex, but the effect of exchange on reaction energetics within a single spin state is less well-established. Across a number of model iron complexes, we observe strong exchange sensitivities of reaction barriers and energies that are of the same magnitude as those for spin splitting energies. We rationalize trends in both reaction and spin energetics by introducing a measure of delocalization, the bond valence of the metal-ligand bonds in each complex. The bond valence thus represents a simple-to-compute property that unifies understanding of exchange sensitivity for catalytic properties and spin-state ordering in TM complexes. Close agreement of the resulting per-metal-organic-bond sensitivity estimates, together with failure of alternative descriptors demonstrates the utility of the bond valence as a robust descriptor of how differences in metal-ligand delocalization produce differing relative energetics with exchange tuning. Our unified description explains the overall effect of exact exchange tuning on the paradigmatic two-state FeO + /CH 4 reaction that combines challenges of spin-state and reactivity predictions. This new descriptor-sensitivity relationship provides a path to quantifying how predictions in transition-metal complex screening are sensitive to the

  20. Symmetry-broken dissipative exchange flows in thin-film ferromagnets with in-plane anisotropy

    Science.gov (United States)

    Iacocca, Ezio; Silva, T. J.; Hoefer, Mark A.

    2017-10-01

    Planar ferromagnetic channels have been shown to theoretically support a long-range ordered and coherently precessing state where the balance between local spin injection at one edge and damping along the channel establishes a dissipative exchange flow, sometimes referred to as a spin superfluid. However, realistic materials exhibit in-plane anisotropy, which breaks the axial symmetry assumed in current theoretical models. Here, we study dissipative exchange flows in a ferromagnet with in-plane anisotropy from a dispersive hydrodynamic perspective. Through the analysis of a boundary value problem for a damped sine-Gordon equation, dissipative exchange flows in a ferromagnetic channel can be excited above a spin current threshold that depends on material parameters and the length of the channel. Symmetry-broken dissipative exchange flows display harmonic overtones that redshift the fundamental precessional frequency and lead to a reduced spin pumping efficiency when compared to their symmetric counterpart. Micromagnetic simulations are used to verify that the analytical results are qualitatively accurate, even in the presence of nonlocal dipole fields. Simulations also confirm that dissipative exchange flows can be driven by spin transfer torque in a finite-sized region. These results delineate the important material parameters that must be optimized for the excitation of dissipative exchange flows in realistic systems.

  1. Spin Hall magnetoresistance in antiferromagnet/normal metal bilayers

    KAUST Repository

    Manchon, Aurelien

    2017-01-01

    We investigate the emergence of spin Hall magnetoresistance in a magnetic bilayer composed of a normal metal adjacent to an antiferromagnet. Based on a recently derived drift diffusion equation, we show that the resistance of the bilayer depends on the relative angle between the direction transverse to the current flow and the Néel order parameter. While this effect presents striking similarities with the spin Hall magnetoresistance recently reported in ferromagnetic bilayers, its physical origin is attributed to the anisotropic spin relaxation of itinerant spins in the antiferromagnet.

  2. Unusual Room Temperature Ferromagnetism in Bulk Sintered GaP Doped with Copper

    Energy Technology Data Exchange (ETDEWEB)

    Owens, F. J.; Gupta, A.; Rao, K. V.; Iqbal, Z.; Osorio Guillen, J. M.; Ahuja, R.; Guo, J.-H.

    2007-06-01

    Robust room temperature ferromagnetism is obtained in single phase Gallium Phosphide doped with Cu{sup 2+} prepared by simple solid state reaction route. The saturation magnetization at 300 K is 1.5 times 10{sup -2} emu/g and the coercivity was found to be 125 Oe. A strong ferromagnetic resonance signal confirms the long range magnetic order which persists to temperatures as high as 739 K. X-ray absorption spectroscopy (XAS) indicate that Cu is in a +2 state. Ab initio calculations also show that the ferromagnetic ordering is energetically favorable in Cu doped GaP. When the spin-orbit coupling is included we get an enhanced total magnetic moment of 0.31 muB with a local moment on Cu 0.082 and on P 0.204 mu{sub B}. per atom.

  3. Structural, optical and vibrational properties of Cr2O3 with ferromagnetic and antiferromagnetic order: A combined experimental and density functional theory study

    Science.gov (United States)

    Larbi, T.; Ouni, B.; Gantassi, A.; Doll, K.; Amlouk, M.; Manoubi, T.

    2017-12-01

    Chromium oxide (Cr2O3) thin films have been synthesized on glass substrates by the spray pyrolysis technique. The structural, morphological and optical properties of the sample have been studied by X-ray diffraction (XRD), Raman spectroscopy, FTIR spectroscopy, scanning probe microscopy and UV-vis spectroscopy respectively. X-ray diffraction results reveal that as deposited film is polycrystalline with a rhombohedral corundum structure and a preferential orientation of the crystallites along the (1 0 4) direction. IR and Raman spectra were recorded in the 100-900 cm-1 range and the observed modes were analysed and assigned to different normal modes of vibration. The direct optical band gap energy value calculated from the transmittance spectra of as-deposited thin film is about 3.38 eV. We employ first principles calculations based on density functional theory (DFT) with the B3LYP hybrid functional and a coupled perturbed Hartree-Fock/Kohn-Sham approach (CPHF/KS). We study the electronic structure, optimum geometry, and IR and Raman spectra of ferromagnetically and antiferromagnetically ordered Cr2O3. The computed results are consistent with the experimental measurements, and provide complete vibrational assignment, for the characterization of Cr2O3 thin film materials which can be used in photocatalysis and gas sensors.

  4. Low temperature properties of spin filter NbN/GdN/NbN Josephson junctions

    Energy Technology Data Exchange (ETDEWEB)

    Massarotti, D., E-mail: dmassarotti@na.infn.it [Dipartimento di Ingegneria Industriale e dell’Informazione, Seconda Università di Napoli, via Roma 29, 81031 Aversa (CE) (Italy); CNR-SPIN UOS Napoli, Complesso Universitario di Monte Sant’Angelo, via Cinthia, 80126 Napoli (Italy); Caruso, R. [Dipartimento di Fisica, Università degli Studi di Napoli Federico II, Via Cinthia, 80126 Napoli (Italy); CNR-SPIN UOS Napoli, Complesso Universitario di Monte Sant’Angelo, via Cinthia, 80126 Napoli (Italy); Pal, A. [Department of Materials Science and Metallurgy, University of Cambridge, Cambridge CB3 0FS (United Kingdom); Rotoli, G. [Dipartimento di Ingegneria Industriale e dell’Informazione, Seconda Università di Napoli, via Roma 29, 81031 Aversa (CE) (Italy); Longobardi, L. [Dipartimento di Ingegneria Industriale e dell’Informazione, Seconda Università di Napoli, via Roma 29, 81031 Aversa (CE) (Italy); American Physical Society, 1 Research Road, Ridge, New York 11961 (United States); Pepe, G.P. [Dipartimento di Fisica, Università degli Studi di Napoli Federico II, Via Cinthia, 80126 Napoli (Italy); CNR-SPIN UOS Napoli, Complesso Universitario di Monte Sant’Angelo, via Cinthia, 80126 Napoli (Italy); Blamire, M.G. [Department of Materials Science and Metallurgy, University of Cambridge, Cambridge CB3 0FS (United Kingdom); Tafuri, F. [Dipartimento di Ingegneria Industriale e dell’Informazione, Seconda Università di Napoli, via Roma 29, 81031 Aversa (CE) (Italy); CNR-SPIN UOS Napoli, Complesso Universitario di Monte Sant’Angelo, via Cinthia, 80126 Napoli (Italy)

    2017-02-15

    Highlights: • We study the phase dynamics of ferromagnetic NbN/GdN/NbN Josephson junctions. • The ferromagnetic insulator GdN barrier generates spin-filtering properties. • Spin filter junctions fall in the underdamped regime. • MQT occurs with the same phenomenology as in conventional Josephson junctions. • Dissipation is studied in a wide range of critical current density values. - Abstract: A ferromagnetic Josephson junction (JJ) represents a special class of hybrid system where different ordered phases meet and generate novel physics. In this work we report on the transport measurements of underdamped ferromagnetic NbN/GdN/NbN JJs at low temperatures. In these junctions the ferromagnetic insulator gadolinium nitride barrier generates spin-filtering properties and a dominant second harmonic component in the current-phase relation. These features make spin filter junctions quite interesting also in terms of fundamental studies on phase dynamics and dissipation. We discuss the fingerprints of spin filter JJs, through complementary transport measurements, and their implications on the phase dynamics, through standard measurements of switching current distributions. NbN/GdN/NbN JJs, where spin filter properties can be controllably tuned along with the critical current density (J{sub c}), turn to be a very relevant term of reference to understand phase dynamics and dissipation in an enlarged class of JJs, not necessarily falling in the standard tunnel limit characterized by low J{sub c} values.

  5. Static magnetic ordering of CeCu2.1Si2 found by muon spin relaxation

    Science.gov (United States)

    Uemura, Y. J.; Kossler, W. J.; Yu, X. H.; Schone, H. E.; Kempton, J. R.; Stronach, C. E.; Barth, S.; Gygax, F. N.; Hitti, B.; Schenck, A.

    1988-01-01

    Zero- and longitudinal-field muon spin relaxation measurements on a polycrystal sample of a heavy fermion superconductor CeCu2.1 Si2 (T(c) = 0.7 K) have revealed an onset of static magnetic ordering below T approximately 0.8 K. The line shapes of the observed spectra in zero field indicate a wide distribution of static random local fields at muon sites, suggesting that the ordering is either spin glass or incommensurate spin-density-wave state. The observed width of the random local field at T = 0.05 K corresponds to a small averaged static moment of the order of 0.1 micro-B per formula unit.

  6. Superconductivity-induced magnetization depletion in a ferromagnet through an insulator in a ferromagnet-insulator-superconductor hybrid oxide heterostructure.

    Science.gov (United States)

    Prajapat, C L; Singh, Surendra; Paul, Amitesh; Bhattacharya, D; Singh, M R; Mattauch, S; Ravikumar, G; Basu, S

    2016-05-21

    Coupling between superconducting and ferromagnetic states in hybrid oxide heterostructures is presently a topic of intense research. Such a coupling is due to the leakage of the Cooper pairs into the ferromagnet. However, tunneling of the Cooper pairs though an insulator was never considered plausible. Using depth sensitive polarized neutron reflectivity we demonstrate the coupling between superconductor and magnetic layers in epitaxial La2/3Ca1/3MnO3 (LCMO)/SrTiO3/YBa2Cu3O7-δ (YBCO) hybrid heterostructures, with SrTiO3 as an intervening oxide insulator layer between the ferromagnet and the superconductor. Measurements above and below the superconducting transition temperature (TSC) of YBCO demonstrate a large modulation of magnetization in the ferromagnetic layer below the TSC of YBCO in these heterostructures. This work highlights a unique tunneling phenomenon between the epitaxial layers of an oxide superconductor (YBCO) and a magnetic layer (LCMO) through an insulating layer. Our work would inspire further investigations on the fundamental aspect of a long range order of the triplet spin-pairing in hybrid structures.

  7. Modified spin-wave theory with ordering vector optimization: frustrated bosons on the spatially anisotropic triangular lattice

    Energy Technology Data Exchange (ETDEWEB)

    Hauke, Philipp [ICFO-Institut de Ciencies Fotoniques, Meditarranean Technology Park, E-08860 Castelldefels, Barcelona (Spain); Roscilde, Tommaso [Laboratoire de Physique, Ecole Normale Superieure de Lyon, 46 Allee d' Italie, F-69007 Lyon (France); Murg, Valentin; Ignacio Cirac, J; Schmied, Roman, E-mail: Philipp.Hauke@icfo.e [Max-Planck-Institut fuer Quantenoptik, Hans-Kopfermann-Strasse 1, D-85748 Garching (Germany)

    2010-05-15

    We investigate a system of frustrated hardcore bosons, modeled by an XY antiferromagnet on the spatially anisotropic triangular lattice, using Takahashi's modified spin-wave (MSW) theory. In particular, we implement ordering vector optimization on the ordered reference state of MSW theory, which leads to significant improvement of the theory and accounts for quantum corrections to the classically ordered state. The MSW results at zero temperature compare favorably to exact diagonalization (ED) and projected entangled-pair state (PEPS) calculations. The resulting zero-temperature phase diagram includes a one-dimensional (1D) quasi-ordered phase, a 2D Neel ordered phase and a 2D spiraling ordered phase. Strong indications coming from the ED and PEPS calculations, as well as from the breakdown of MSW theory, suggest that the various ordered or quasi-ordered phases are separated by spin-liquid phases with short-range correlations, in analogy to what has been predicted for the Heisenberg model on the same lattice. Within MSW theory, we also explore the finite-temperature phase diagram. In agreement with the Berezinskii-Kosterlitz-Thouless (BKT) theory, we find that zero-temperature long-range-ordered phases turn into quasi-ordered phases (up to a BKT transition temperature), while zero-temperature quasi-ordered phases become short-range correlated at finite temperature. These results show that, despite its simplicity, MSW theory is very well suited to describing ordered and quasi-ordered phases of frustrated XY spins (or, equivalently, of frustrated lattice bosons) both at zero and finite temperatures. While MSW theory, just as other theoretical methods, cannot describe spin-liquid phases, its breakdown provides a fast and reliable method for singling out Hamiltonians that may feature these intriguing quantum phases. We thus suggest a tool for guiding our search for interesting systems whose properties are necessarily studied with a physical quantum simulator

  8. Modified spin-wave theory with ordering vector optimization: frustrated bosons on the spatially anisotropic triangular lattice

    Science.gov (United States)

    Hauke, Philipp; Roscilde, Tommaso; Murg, Valentin; Cirac, J. Ignacio; Schmied, Roman

    2010-05-01

    We investigate a system of frustrated hardcore bosons, modeled by an XY antiferromagnet on the spatially anisotropic triangular lattice, using Takahashi's modified spin-wave (MSW) theory. In particular, we implement ordering vector optimization on the ordered reference state of MSW theory, which leads to significant improvement of the theory and accounts for quantum corrections to the classically ordered state. The MSW results at zero temperature compare favorably to exact diagonalization (ED) and projected entangled-pair state (PEPS) calculations. The resulting zero-temperature phase diagram includes a one-dimensional (1D) quasi-ordered phase, a 2D Néel ordered phase and a 2D spiraling ordered phase. Strong indications coming from the ED and PEPS calculations, as well as from the breakdown of MSW theory, suggest that the various ordered or quasi-ordered phases are separated by spin-liquid phases with short-range correlations, in analogy to what has been predicted for the Heisenberg model on the same lattice. Within MSW theory, we also explore the finite-temperature phase diagram. In agreement with the Berezinskii-Kosterlitz-Thouless (BKT) theory, we find that zero-temperature long-range-ordered phases turn into quasi-ordered phases (up to a BKT transition temperature), while zero-temperature quasi-ordered phases become short-range correlated at finite temperature. These results show that, despite its simplicity, MSW theory is very well suited to describing ordered and quasi-ordered phases of frustrated XY spins (or, equivalently, of frustrated lattice bosons) both at zero and finite temperatures. While MSW theory, just as other theoretical methods, cannot describe spin-liquid phases, its breakdown provides a fast and reliable method for singling out Hamiltonians that may feature these intriguing quantum phases. We thus suggest a tool for guiding our search for interesting systems whose properties are necessarily studied with a physical quantum simulator instead

  9. Effects of electric field and magnetic induction on spin injection into organic semiconductors

    International Nuclear Information System (INIS)

    Wang, Y.M.; Ren, J.F.; Yuan, X.B.; Dou, Z.T.; Hu, G.C.

    2011-01-01

    Spin-polarized injection and transport into ferromagnetic/organic semiconductor structure are studied theoretically in the presence of the external electric field and magnetic induction. Based on the spin-drift-diffusion theory and Ohm's law, we obtain the charge current polarization, which takes into account the special carriers of organic semiconductors. From the calculation, it is found that the current spin polarization is enhanced by several orders of magnitude by tuning the magnetic induction and electric fields. To get an apparent current spin polarization, the effects of spin-depended interfacial resistances and the special carriers in the organic semiconductor, which are polarons and bipolarons, are also discussed. -- Research highlights: → Current polarization in ferromagnetic/organic semiconductor structure is obtained. → Calculations are based on spin-drift-diffusion theory and Ohm's law. → Current polarization is enhanced by tuning magnetic induction and electric fields. → Effects of interfacial resistances and the special carriers are also discussed.

  10. Field-controlled magnetic order in the quantum spin-ladder system (Hpip)2CuBr4

    DEFF Research Database (Denmark)

    Thielemann, B.; Rüegg, C.; Kiefer, K.

    2009-01-01

    Neutron diffraction is used to investigate the field-induced, antiferromagnetically ordered state in the two-leg spin-ladder material (Hpip)(2)CuBr4. This "classical" phase, a consequence of weak interladder coupling, is nevertheless highly unconventional: its properties are influenced strongly b...... the quantum fluctuation corrections to the mean-field interaction.......Neutron diffraction is used to investigate the field-induced, antiferromagnetically ordered state in the two-leg spin-ladder material (Hpip)(2)CuBr4. This "classical" phase, a consequence of weak interladder coupling, is nevertheless highly unconventional: its properties are influenced strongly...

  11. Influence of Ba substitution upon ferromagnetism in charge ordered Nd{sub 1-x}Ca{sub x}MnO{sub 3}: singular behaviour of x = 0.43

    Energy Technology Data Exchange (ETDEWEB)

    Yaicle, C; Raveau, B; Maignan, A; Hardy, V; Martin, C; Hervieu, M [Laboratoire CRISMAT, UMR 6508, CNRS ENSICAEN, 6 boulevard Marechal Juin, 14050 Caen Cedex, 4 (France)

    2005-02-16

    The study of the substitution of Ba for Ca in the orbital-charge ordered manganites Nd{sub 1-x}Ca{sub x}MnO{sub 3}, with 0.37 {<=} x {<=} 0.50, for low Ba levels (smaller than 6%) shows that, similarly to the Pr{sub 1-x}Ca{sub x}MnO{sub 3} system (Zhu et al 2004 J. Phys.: Condens. Matter 16 2861), a ferromagnetic ground state is obtained. The evolution of the ferromagnetic fraction in zero field is quite similar: it goes through a maximum at x = 0.43, which, for 4% Ba, is like for Pr a full ferromagnet at 2.5 K, with a ferromagnetic fraction of 90%. The higher Ba level necessary to reach the FM state in Nd phases compared to Pr is explained in terms of the antagonist effects of charge-orbital stability and local counter-distortion due to Ba. The different behaviour in a magnetic field, and especially the much larger magnetizations reached by Nd phases with respect to the Pr ones, 0.43 {<=} x {<=} 0.50, is explained in terms of Nd-Mn magnetic interactions, which destabilize the CE-type AFM structure.

  12. Tunnel barrier and noncollinear magnetization effects on shot noise in ferromagnetic/semiconductor/ferromagnetic heterojunctions

    International Nuclear Information System (INIS)

    An Xingtao; Liu Jianjun

    2008-01-01

    Based on the scattering approach, we investigate transport properties of electrons in a one-dimensional waveguide that contains a ferromagnetic/semiconductor/ferromagnetic heterojunction and tunnel barriers in the presence of Rashba and Dresselhaus spin-orbit interactions. We simultaneously consider significant quantum size effects, quantum coherence, Rashba and Dresselhaus spin-orbit interactions and noncollinear magnetizations. It is found that the tunnel barrier plays a decisive role in the transmission coefficient and shot noise of the ballistic spin electron transport through the heterojunction. When the small tunnel barriers are considered, the transport properties of electrons are quite different from those without tunnel barriers

  13. Neutron Scattering from the Heisenberg Ferromagnets EuO and EuS

    DEFF Research Database (Denmark)

    Dietrich, O. W.; Als-Nielsen, Jens Aage; Passell, L.

    1976-01-01

    Inelastic neutron scattering has been used to investigate the spin dynamics of the isotropic Heisenberg ferromagnet EuO over a wide range of wave vectors and over a temperature range extending from 0.14 to 1.9TC. Below the ordering temperature spin-wave renormalization is found to agree well...... with the predictions of Dyson-Maleev theory (including the dynamical but not the kinematical interaction) when both exchange and dipolar couplings between the Eu2+ ions are taken into account. At temperatures near TC broadening of the spin-wave lines was observed. For hydrodynamic spin waves, the wave......-vector dependence of the linewidths is found to be consistent with the expectations of microscopic spin-wave theory and the temperature dependence with predictions based on dynamical scaling. At TC, linewidths were found to deviate from the q5/2 wave-vector dependence expected on the basis of dynamical scaling...

  14. An order-by-disorder process in the cyclic phase of spin-2 condensate with a weak magnetic field

    International Nuclear Information System (INIS)

    Zheng, Gong-Ping; Xu, Lei-Kuan; Qin, Shuai-Feng; Jian, Wen-Tian; Liang, J.-Q.

    2013-01-01

    We present in this paper a model study on the “order-by-disorder” process in the cyclic phase of spin-2 condensate, which forms a family of incommensurable, spiral degenerate ground states. On the basis of the ordering mechanism of entropic splitting, it is demonstrated that the energy corrections resulting from quantum fluctuations of disorder lift the accidental degeneracy of the cyclic configurations and thus lead to an eventual spiral order called the cyclic order. The order-by-disorder phenomenon is then realized even if the magnetic field exists. Finally, we show that our theoretic observations can be verified experimentally by direct detection of the cyclic order in the 87 Rb condensate of a spin-2 manifold with a weak magnetic field. -- Highlights: •A model for the order-by-disorder process in the cyclic phase of spin-2 condensate is presented. •The second-order quantum fluctuations of the mean-field states are studied. •The energy corrections lift the accidental degeneracy of the cyclic configurations. •The order-by-disorder phenomenon is realized even if a magnetic field exists. •The theoretic observations can be verified experimentally for 87 Rb condensate

  15. Dirac Magnons in Honeycomb Ferromagnets

    Science.gov (United States)

    Pershoguba, Sergey S.; Banerjee, Saikat; Lashley, J. C.; Park, Jihwey; Ågren, Hans; Aeppli, Gabriel; Balatsky, Alexander V.

    2018-01-01

    The discovery of the Dirac electron dispersion in graphene [A. H. Castro Neto, et al., The Electronic Properties of Graphene, Rev. Mod. Phys. 81, 109 (2009), 10.1103/RevModPhys.81.109] led to the question of the Dirac cone stability with respect to interactions. Coulomb interactions between electrons were shown to induce a logarithmic renormalization of the Dirac dispersion. With a rapid expansion of the list of compounds and quasiparticle bands with linear band touching [T. O. Wehling, et al., Dirac Materials, Adv. Phys. 63, 1 (2014), 10.1080/00018732.2014.927109], the concept of bosonic Dirac materials has emerged. We consider a specific case of ferromagnets consisting of van der Waals-bonded stacks of honeycomb layers, e.g., chromium trihalides CrX3 (X =F , Cl, Br and I), that display two spin wave modes with energy dispersion similar to that for the electrons in graphene. At the single-particle level, these materials resemble their fermionic counterparts. However, how different particle statistics and interactions affect the stability of Dirac cones has yet to be determined. To address the role of interacting Dirac magnons, we expand the theory of ferromagnets beyond the standard Dyson theory [F. J. Dyson, General Theory of Spin-Wave Interactions, Phys. Rev. 102, 1217 (1956), 10.1103/PhysRev.102.1217, F. J. Dyson, Thermodynamic Behavior of an Ideal Ferromagnet, Phys. Rev. 102, 1230 (1956), 10.1103/PhysRev.102.1230] to the case of non-Bravais honeycomb layers. We demonstrate that magnon-magnon interactions lead to a significant momentum-dependent renormalization of the bare band structure in addition to strongly momentum-dependent magnon lifetimes. We show that our theory qualitatively accounts for hitherto unexplained anomalies in nearly half-century-old magnetic neutron-scattering data for CrBr3 [W. B. Yelon and R. Silberglitt, Renormalization of Large-Wave-Vector Magnons in Ferromagnetic CrBr3 Studied by Inelastic Neutron Scattering: Spin-Wave Correlation

  16. Dirac Magnons in Honeycomb Ferromagnets

    Directory of Open Access Journals (Sweden)

    Sergey S. Pershoguba

    2018-01-01

    Full Text Available The discovery of the Dirac electron dispersion in graphene [A. H. Castro Neto, et al., The Electronic Properties of Graphene, Rev. Mod. Phys. 81, 109 (2009RMPHAT0034-686110.1103/RevModPhys.81.109] led to the question of the Dirac cone stability with respect to interactions. Coulomb interactions between electrons were shown to induce a logarithmic renormalization of the Dirac dispersion. With a rapid expansion of the list of compounds and quasiparticle bands with linear band touching [T. O. Wehling, et al., Dirac Materials, Adv. Phys. 63, 1 (2014ADPHAH0001-873210.1080/00018732.2014.927109], the concept of bosonic Dirac materials has emerged. We consider a specific case of ferromagnets consisting of van der Waals-bonded stacks of honeycomb layers, e.g., chromium trihalides CrX_{3} (X=F, Cl, Br and I, that display two spin wave modes with energy dispersion similar to that for the electrons in graphene. At the single-particle level, these materials resemble their fermionic counterparts. However, how different particle statistics and interactions affect the stability of Dirac cones has yet to be determined. To address the role of interacting Dirac magnons, we expand the theory of ferromagnets beyond the standard Dyson theory [F. J. Dyson, General Theory of Spin-Wave Interactions, Phys. Rev. 102, 1217 (1956PHRVAO0031-899X10.1103/PhysRev.102.1217, F. J. Dyson, Thermodynamic Behavior of an Ideal Ferromagnet, Phys. Rev. 102, 1230 (1956PHRVAO0031-899X10.1103/PhysRev.102.1230] to the case of non-Bravais honeycomb layers. We demonstrate that magnon-magnon interactions lead to a significant momentum-dependent renormalization of the bare band structure in addition to strongly momentum-dependent magnon lifetimes. We show that our theory qualitatively accounts for hitherto unexplained anomalies in nearly half-century-old magnetic neutron-scattering data for CrBr_{3} [W. B. Yelon and R. Silberglitt, Renormalization of Large-Wave-Vector Magnons in

  17. Anisotropic spin motive force in multi-layered Dirac fermion system, α-(BEDT-TTF)2I3

    International Nuclear Information System (INIS)

    Kubo, K; Morinari, T

    2015-01-01

    We investigate the anisotropic spin motive force in α-(BEDT-TTF) 2 I 3 , which is a multi-layered massless Dirac fermion system under pressure. Assuming the interlayer antiferromagnetic interaction and the interlayer anisotropic ferromagnetic interaction, we numerically examine the spin ordered state of the ground state using the steepest descent method. The anisotropic interaction leads to the anisotropic spin ordered state. We calculate the spin motive force produced by the anisotropic spin texture. The result quantitatively agrees with the experiment. (paper)

  18. Quantum stability for the Heisenberg ferromagnet

    International Nuclear Information System (INIS)

    Bargheer, Till; Beisert, Niklas; Gromov, Nikolay

    2008-01-01

    Highly spinning classical strings on RxS 3 are described by the Landau-Lifshitz model or equivalently by the Heisenberg ferromagnet in the thermodynamic limit. The spectrum of this model can be given in terms of spectral curves. However, it is a priori not clear whether any given admissible spectral curve can actually be realized as a solution to the discrete Bethe equations, a property which can be referred to as stability. In order to study the issue of stability, we find and explore the general two-cut solution or elliptic curve. It turns out that the moduli space of this elliptic curve shows a surprisingly rich structure. We present the various cases with illustrations and thus gain some insight into the features of multi-cut solutions. It appears that all admissible spectral curves are indeed stable if the branch cuts are positioned in a suitable, non-trivial fashion.

  19. Inner Phases of Colloidal Hexagonal Spin Ice

    Science.gov (United States)

    Libál, A.; Nisoli, C.; Reichhardt, C. J. O.; Reichhardt, C.

    2018-01-01

    Using numerical simulations that mimic recent experiments on hexagonal colloidal ice, we show that colloidal hexagonal artificial spin ice exhibits an inner phase within its ice state that has not been observed previously. Under increasing colloid-colloid repulsion, the initially paramagnetic system crosses into a disordered ice regime, then forms a topologically charge ordered state with disordered colloids, and finally reaches a threefold degenerate, ordered ferromagnetic state. This is reminiscent of, yet distinct from, the inner phases of the magnetic kagome spin ice analog. The difference in the inner phases of the two systems is explained by their difference in energetics and frustration.

  20. Coupled magnetoelastic waves in ferromagnetic shape-memory alloys

    Science.gov (United States)

    Bar'Yakhtar, V. G.; Danilevich, A. G.; L'Vov, V. A.

    2011-10-01

    The theory of the spectra of coupled magnetoelastic waves in ferromagnetic shape-memory alloys (FSMA) is developed. The possibility of an abnormally strong coupling of spin waves with the soft elastic mode at approaching the martensitic transformation (MT) temperature is disclosed. In particular the magnetoelastic waves in Ni-Mn-Ga single crystals are considered. A considerable (by an order of magnitude) reduction of the shear elastic modulus and an appropriate lowering of the transversal velocity of sound in the applied magnetic field are predicted. Optimum conditions for the experimental observation of the predicted effects are specified.

  1. Spin correlations and spin-wave excitations in Dirac-Weyl semimetals

    Science.gov (United States)

    Araki, Yasufumi; Nomura, Kentaro

    We study correlations among magnetic dopants in three-dimensional Dirac and Weyl semimetals. Effective field theory for localized magnetic moments is derived by integrating out the itinerant electron degrees of freedom. We find that spin correlation in the spatial direction parallel to local magnetization is more rigid than that in the perpendicular direction, reflecting spin-momentum locking nature of the Dirac Hamiltonian. Such an anisotropy becomes stronger for Fermi level close to the Dirac points, due to Van Vleck paramagnetism triggered by spin-orbit coupling. One can expect topologically nontrivial spin textures under this anisotropy, such as a hedgehog around a single point, or a radial vortex around an axis, as well as a uniform ferromagnetic order. We further investigate the characteristics of spin waves in the ferromagnetic state. Spin-wave dispersion also shows a spatial anisotropy, which is less dispersed in the direction transverse to the magnetization than that in the longitudinal direction. The spin-wave dispersion anisotropy can be traced back to the rigidity and flexibility of spin correlations discussed above. This work was supported by Grant-in-Aid for Scientific Research (Grants No.15H05854, No.26107505, and No.26400308) from the Ministry of Education, Culture, Sports, Science and Technology (MEXT), Japan.

  2. Wireless power transfer exploring spin rectification and inverse spin Hall effects

    Science.gov (United States)

    Seeger, R. L.; Garcia, W. J. S.; Dugato, D. A.; da Silva, R. B.; Harres, A.

    2018-04-01

    Devices based on spin rectification effects are of great interest for broadband communication applications, since they allow the rectification of radio frequency signals by simple ferromagnetic materials. The phenomenon is enhanced at ferromagnetic resonance condition, which may be attained when an external magnetic field is applied. The necessity of such field, however, hinders technological applications. Exploring spin rectification and spin Hall effects in exchange-biased samples, we were able to rectify radio frequency signals without an external applied magnetic field. Direct voltages of the order of μV were obtained when Ta/NiFe/FeMn/Ta thin films were exposed to microwaves in a shorted microstrip line for a relatively broad frequency range. Connecting the films to a resistive load, we estimated the fraction of the incident radio frequency power converted into usable dc power.

  3. High efficiency spin-valve and spin-filter in a doped rhombic graphene quantum dot device

    Science.gov (United States)

    Silva, P. V.; Saraiva-Souza, A.; Maia, D. W.; Souza, F. M.; Filho, A. G. Souza; Meunier, V.; Girão, E. C.

    2018-04-01

    Spin-polarized transport through a rhombic graphene quantum dot (rGQD) attached to armchair graphene nanoribbon (AGNR) electrodes is investigated by means of the Green's function technique combined with single-band tight-binding (TB) approach including a Hubbard-like term. The Hubbard repulsion was included within the mean-field approximation. Compared to anti-ferromagnetic (AFM), we show that the ferromagnetic (FM) ordering of the rGQD corresponds to a smaller bandgap, thus resulting in an efficient spin injector. As a consequence, the electron transport spectrum reveals a spin valve effect, which is controlled by doping with B/N atoms creating a p-n-type junction. The calculations point out that such systems can be used as spin-filter devices with efficiency close to a 100 % .

  4. Honeycomb artificial spin ice at low temperatures

    Science.gov (United States)

    Zeissler, Katharina; Chadha, Megha; Cohen, Lesley; Branford, Will

    2015-03-01

    Artificial spin ice is a macroscopic playground for magnetically frustrated systems. It consists of a geometrically ordered but magnetically frustrated arrangement of ferromagnetic macros spins, e.g. an arrangement of single domain ferromagnetic nanowires on a honeycomb lattice. Permalloy and cobalt which have critical temperature scales far above 290 K, are commonly used in the construction of such systems. Previous measurements have shown unusual features in the magnetotransport signature of cobalt honeycomb artificial spin ice at temperatures below 50 K which are due to changes in the artificial spin ice's magnetic reversal. In that case, the artificial spin ice bars were 1 micron long, 100 nm wide and 20 nm thick. Here we explore the low temperature magnetic behavior of honeycomb artificial spin ice structures with a variety of bar dimensions, indirectly via electrical transport, as well as, directly using low temperature magnetic imaging techniques. We discuss the extent to which this change in the magnetic reversal at low temperatures is generic to the honeycomb artificial spin ice geometry and whether the bar dimensions have an influence on its onset temperature. The EPSRC (Grant No. EP/G004765/1; Grant No. EP/L504786/1) and the Leverhulme Trust (Grant No. RPG 2012-692) funded this scientific work.

  5. Spin order in the charge disproportionated phases of the A -site layer ordered triple perovskite LaC a2F e3O9

    Science.gov (United States)

    Arevalo-Lopez, Angel M.; Hosaka, Yoshiteru; Guo, Haichuan; Denis Romero, Fabio; Saito, Takashi; Attfield, J. Paul; Shimakawa, Yuichi

    2018-01-01

    The coupling between spins and charge disproportionation states has been investigated in the LaC a2F e3O9 oxide with neutron powder diffraction. This A -site layer ordered triple perovskite LaC a2F e3O9 undergoes charge disproportionation on cooling and shows two different charge ordering patterns. At 230 K, F e3.67 + disproportionates into a 2:1 ratio of F e3 +:F e5 + , which order in a layered manner along the 〈010 〉 direction of the pseudocubic unit cell. At lower temperatures (T Neutron powder diffraction data show that in the intermediate temperature range (170 K spins order into a cycloidal structure on the a c plane for the F e3 + cations while the F e5 + cations remain paramagnetic. For the lowest temperature range (2 K spin structure follows the charge ordering and evolves to a 〈111 〉 layered magnetic structure.

  6. Anomalous second ferromagnetic phase transition in Co{sub 0.08}Bi{sub 1.92}Se{sub 3} topological insulator

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, Min, E-mail: zmzmi1987@163.com; Liu, Ligang; Yang, Hui

    2016-09-05

    We report the observation of ferromagnetism in topological insulator Co{sub 0.08}Bi{sub 1.92}Se{sub 3} single crystal. The structural, magnetic, and microstructure properties of Co{sub 0.08}Bi{sub 1.92}Se{sub 3} are investigated. The existence of complicated ferromagnetic ordering, indicates the anomalous second ferromagnetic phase transition below 30 K. Well-defined ferromagnetic hysteresis in the magnetization was found in the sample. The origin of bulk ferromagnetism in Co{sub 0.08}Bi{sub 1.92}Se{sub 3} is concerned with three aspects: Co cluster, RKKY interactions, and the spin texture of Co impurities. - Highlights: • The bulk ferromagnetism have been found in the C{sub o0.08}Bi{sub 1.92}Se{sub 3} single crystal. • The anomalous second ferromagnetic phase transition is found below 30 K. • The origin of bulk ferromagnetism in Co{sub 0.08}Bi{sub 1.92}Se{sub 3} is concerned with three aspects.

  7. Spin transport and spin torque in antiferromagnetic devices

    Science.gov (United States)

    Železný, J.; Wadley, P.; Olejník, K.; Hoffmann, A.; Ohno, H.

    2018-03-01

    Ferromagnets are key materials for sensing and memory applications. In contrast, antiferromagnets, which represent the more common form of magnetically ordered materials, have found less practical application beyond their use for establishing reference magnetic orientations via exchange bias. This might change in the future due to the recent progress in materials research and discoveries of antiferromagnetic spintronic phenomena suitable for device applications. Experimental demonstration of the electrical switching and detection of the Néel order open a route towards memory devices based on antiferromagnets. Apart from the radiation and magnetic-field hardness, memory cells fabricated from antiferromagnets can be inherently multilevel, which could be used for neuromorphic computing. Switching speeds attainable in antiferromagnets far exceed those of ferromagnetic and semiconductor memory technologies. Here, we review the recent progress in electronic spin-transport and spin-torque phenomena in antiferromagnets that are dominantly of the relativistic quantum-mechanical origin. We discuss their utility in pure antiferromagnetic or hybrid ferromagnetic/antiferromagnetic memory devices.

  8. Coexistence of short- and long-range ferromagnetic order in nanocrystalline Fe2Mn1-xCuxAl (x=0.0, 0.1 and 0.3) synthesized by high-energy ball milling

    Science.gov (United States)

    Thanh, Tran Dang; Nanto, Dwi; Tuyen, Ngo Thi Uyen; Nan, Wen-Zhe; Yu, YiKyung; Tartakovsky, Daniel M.; Yu, S. C.

    2015-11-01

    In this work, we prepared nanocrystalline Fe2Mn1-xCuxAl (x=0.0, 0.1 and 0.3) powders by the high energy ball milling technique, and then studied their critical properties. Our analysis reveals that the increase of Cu-doping concentration (up to x=0.3) in these powders leads to a gradual increase of the ferromagnetic-paramagnetic transition temperature from 406 to 452 K. The Banerjee criterion suggests that all the samples considered undergo a second-order phase transition. A modified Arrott plot and scaling analysis indicate that the critical exponents (β=0.419 and 0.442, γ=1.082 and 1.116 for x=0.0 and 0.1, respectively) are located in between those expected for the 3D-Heisenberg and the mean-field models; the values of β=0.495 and γ=1.046 for x=0.3 sample are very close to those of the mean-field model. These features reveal the coexistence of the short- and long-range ferromagnetic order in the nanocrystalline Fe2Mn1-xCuxAl powders. Particularly, as the concentration of Cu increases, values of the critical exponent shift towards those of the mean-field model. Such results prove the Cu doping favors establishing a long-range ferromagnetic order.

  9. Magnetization switching in ferromagnets by adsorbed chiral molecules without current or external magnetic field

    Science.gov (United States)

    Ben Dor, Oren; Yochelis, Shira; Radko, Anna; Vankayala, Kiran; Capua, Eyal; Capua, Amir; Yang, See-Hun; Baczewski, Lech Tomasz; Parkin, Stuart Stephen Papworth; Naaman, Ron; Paltiel, Yossi

    2017-02-01

    Ferromagnets are commonly magnetized by either external magnetic fields or spin polarized currents. The manipulation of magnetization by spin-current occurs through the spin-transfer-torque effect, which is applied, for example, in modern magnetoresistive random access memory. However, the current density required for the spin-transfer torque is of the order of 1 × 106 A.cm-2, or about 1 × 1025 electrons s-1 cm-2. This relatively high current density significantly affects the devices' structure and performance. Here we demonstrate magnetization switching of ferromagnetic thin layers that is induced solely by adsorption of chiral molecules. In this case, about 1013 electrons per cm2 are sufficient to induce magnetization reversal. The direction of the magnetization depends on the handedness of the adsorbed chiral molecules. Local magnetization switching is achieved by adsorbing a chiral self-assembled molecular monolayer on a gold-coated ferromagnetic layer with perpendicular magnetic anisotropy. These results present a simple low-power magnetization mechanism when operating at ambient conditions.

  10. Heat and spin interconversion

    International Nuclear Information System (INIS)

    Ohnuma, Yuichi; Matsuo, Mamoru; Maekawa, Sadamichi; Saitoh, Eeiji

    2017-01-01

    Spin Seebeck and spin Peltier effects, which are mutual conversion phenomena of heat and spin, are discussed on the basis of the microscopic theory. First, the spin Seebeck effect, which is the spin-current generation due to heat current, is discussed. The recent progress in research on the spin Seebeck effect are introduced. We explain the origin of the observed sign changes of the spin Seebeck effect in compensated ferromagnets. Next, the spin Peltier effect, which is the heat-current generation due to spin current, is discussed. Finally, we show that the spin Seebeck and spin Peltier effects are summarized by Onsager's reciprocal relation and derive Kelvin's relation for the spin and heat transports. (author)

  11. Hydrostatic pressure effect on the spin reorientation transition of ferromagnetic Sm0.7-xLaxSr0.3MnO3 (x = 0, 0.1) polycrystals

    Science.gov (United States)

    Thiyagarajan, R.; Arumugam, S.; Sivaprakash, P.; Kannan, M.; Saravanan, C.; Yang, Wenge

    2017-06-01

    The hydrostatic pressure effect on the resistivity and magnetization of the narrow band gap manganite Sm0.7-xLaxSr0.3MnO3 (x = 0, 0.1) systems has been investigated. At ambient pressure measurements, the parent compound Sm0.7Sr0.3MnO3 showed a ferromagnetic-insulating nature, whereas the 10% La-doped compound Sm0.6La0.1Sr0.3MnO3 showed a ferromagnetic-metallic nature. Furthermore, both samples showed a spin-reorientation transition (TSR) below Curie temperature, which originated from the Mn sublattice and was supported by an antiferromagnetic Sm(4f)-Mn(3d) interaction. Both samples exhibited a normal and inverse magnetocaloric effect as a result of these two different magnetic transitions. Magnetization measurements on Sm0.7Sr0.3MnO3 under pressure did not show an appreciable change in the Curie temperature, but enhanced TSR, whereas an insulator-metallic transition was observed during resistivity measurements under pressure. On the other hand, for Sm0.6La0.1Sr0.3MnO3, TC increased and TSR reduced upon the application of pressure. The metallic nature which is observed at ambient pressure resistivity measurement was further enhanced with 97% of piezoresistance. The pressure did not change the normal magnetocaloric effect of Sm0.7Sr0.3MnO3, but increased it in Sm0.6La0.1Sr0.3MnO3. However, there was not much change in the inverse magnetocaloric effect of both compounds. These studies were analyzed based on the pressure effect on the activation energy and scattering interaction factors.

  12. Unconventional spin order in the triangular lattice system NaCrO2: A neutron scattering study

    International Nuclear Information System (INIS)

    Hsieh, D.; Qian, D.; Berger, R.F.; Cava, R.J.; Lynn, J.W.; Huang, Q.; Hasan, M.Z.

    2008-01-01

    We report high resolution neutron scattering measurements on the rhombohedrally stacked triangular antiferromagnet NaCrO 2 which has recently been shown to exhibit an unusually broad fluctuating cross-over regime extending far below the onset of spin freezing at T c . Our results show that at T c purely two-dimensional quasi-static spin correlations of the 120 o type exist. Below some cross-over temperature (T∼0.75T c ) a small incommensuration develops which helps resolve the inter-layer spin frustration and drives short-range three-dimensional magnetic order. This incommensuration assisted dimensional cross-over suggests that inter-layer frustration is responsible for stabilizing the rare 2D correlated phase above 0.75T c

  13. Phase transitions between different spin-glass phases and between different chaoses in quenched random chiral systems

    Science.gov (United States)

    Ćaǧlar, Tolga; Berker, A. Nihat

    2017-09-01

    The left-right chiral and ferromagnetic-antiferromagnetic double-spin-glass clock model, with the crucially even number of states q =4 and in three dimensions d =3 , has been studied by renormalization-group theory. We find, for the first time to our knowledge, four spin-glass phases, including conventional, chiral, and quadrupolar spin-glass phases, and phase transitions between spin-glass phases. The chaoses, in the different spin-glass phases and in the phase transitions of the spin-glass phases with the other spin-glass phases, with the non-spin-glass ordered phases, and with the disordered phase, are determined and quantified by Lyapunov exponents. It is seen that the chiral spin-glass phase is the most chaotic spin-glass phase. The calculated phase diagram is also otherwise very rich, including regular and temperature-inverted devil's staircases and reentrances.

  14. The order parameters of a spin-1 Ising film in a transverse field

    International Nuclear Information System (INIS)

    Saber, A.; Ainane, A.; Dujardin, F.; Saber, M.; Stebe, B.

    1998-08-01

    Using the effective field theory with a probability distribution technique that accounts for the self-spin correlation functions, the layer longitudinal magnetizations and quadrupolar moments of a spin-1 Ising film and their averages are examined. These quantities as functions of the temperature, the ratio of the surface exchange interactions to the bulk ones, the strength of the transverse field and the film thickness are calculated numerically and some interesting results are obtained. (author)

  15. High-temperature ferromagnetism in Si:Mn alloys

    Science.gov (United States)

    Men'Shov, V. N.; Tugushev, V. V.; Caprara, S.; Chulkov, E. V.

    2011-01-01

    A possible mechanism for high-temperature ferromagnetic order in Si:Mn alloys is proposed. These materials, which are semiconducting or metallic, depending on the Mn content, are suggested to undergo phase separation. In the phase-separated state, again depending on the Mn content, Mn atoms can be gathered within nanometer-sized particles or micrometer-sized islands composed of the MnSi2-z precipitate with z≈(0.25-0.30), which are embedded in the Mn-poor silicon matrix. We consider the MnSi2-z precipitate to be the MnSi1.7 silicide host containing a certain amount of magnetic defects associated with unbound Mn 3d orbitals. The MnSi1.7 silicide is considered to be a weak itinerant ferromagnet, where sizable spin fluctuations (paramagnons) exist far above its intrinsic Curie temperature, leading to a strong enhancement of the exchange coupling between the local moments of the defects. As a result, a significant enhancement of the temperature of onset of long-range order among the local moments may be achieved. We associate this temperature with the global Curie temperature of the precipitate. A phenomenological model is developed to determine the spatial structures and characteristics of ferromagnetic order for the cases of a bulk precipitate and of precipitate particles of various shapes. Moreover, allowing for the presence of strong quenched disorder in the precipitate, we describe short-range ferromagnetic order in the system. Experimental data on Si:Mn alloys are interpreted on the basis of our theoretical results.

  16. Cotunneling through a magnetic quantum dot coupled to ferromagnetic leads with noncollinear magnetizations

    International Nuclear Information System (INIS)

    Weymann, I.; Barnas, J.

    2006-01-01

    By means of the second-order perturbation theory, we analyze theoretically spin-dependent electronic transport through a singly occupied quantum dot in the cotunneling regime. The system is described by the impurity Anderson Hamiltonian with arbitrary Coulomb correlation parameter U. The dot is coupled to two ferromagnetic leads whose magnetic moments are noncollinear. It is also assumed that the dot level is intrinsically spin-split due to an effective molecular field. It is shown that the tunnel magnetoresistance strongly depends on the angle between the leads' magnetizations

  17. Double-Exchange Interaction in Optically Induced Nonequilibrium State: A Conversion from Ferromagnetic to Antiferromagnetic Structure

    Science.gov (United States)

    Ono, Atsushi; Ishihara, Sumio

    2017-11-01

    The double-exchange (DE) interaction, that is, a ferromagnetic (FM) interaction due to a combination of electron motion and the Hund coupling, is a well-known source of a wide class of FM orders. Here, we show that the DE interaction in highly photoexcited states is antiferromagnetic (AFM). Transient dynamics of quantum electrons coupled with classical spins are analyzed. An ac field applied to a metallic FM state results in an almost perfect Néel state. A time characterizing the FM-to-AFM conversion is scaled by light amplitude and frequency. This hidden AFM interaction is attributable to the electron-spin coupling under nonequilibrium electron distribution.

  18. Spin-dependent shot noise in semiconductor and graphene nanostructures

    Science.gov (United States)

    Dragomirova, Ralitsa L.

    on the shot noise and look for a relationship between the degree of quantum coherence of transported spins and the shot noise of charge currents. This allows us to propose electrical shot noise-based scheme to probe spin as a measurable degree of freedom. Injection of unpolarized charge current through the longitudinal leads of a four-terminal two-dimensional electron gas with the Rashba SO coupling and SO scattering off extrinsic impurities is responsible not only for the pure spin Hall current in the transverse leads, but also for nonequilibrium random time-dependent current fluctuations. We employ the spin-dependent scattering approach in Chapter 6 [3, 5] to analyze the shot noise of transverse pure spin Hall current and zero charge current, or transverse spin current and non-zero charge Hall current, driven by unpolarized or spin-polarized injected longitudinal charge current, respectively. Since any spin-flip acts as an additional source of noise, we argue that these shot noises provide a unique experimental tool to differentiate between intrinsic and extrinsic SO mechanisms underlying the spin Hall effect in paramagnetic devices. Recently graphene---a one-atom-thick crystal of carbon atoms arranged into a honeycomb lattice---has emerged as one of the most promising materials for future nanoelectronic devices. It combines exceptional sample quality and accessibility with the unique possibility to explore quantum electrodynamics phenomena in a condensed matter system since current is carried by massless Dirac fermions behaving as charged neutrinos. Furthermore, special nanostructures derived from graphene, the so called zigzag nanoribbons, favor ferromagnetic ordering along their edges. Recently shot noise measurements have been used to characterize ballistic transport through evanescent states introduced into clean undoped graphene strips by the attached metallic electrodes. We demonstrate in Chapter 7 [4] that this shot noise can be substantially modified in

  19. Suppression of the ferromagnetic state by disorder in the Kondo lattice

    International Nuclear Information System (INIS)

    Crisan, M.; Popoviciu, C.

    1992-01-01

    This paper reports that ferromagnetic ground state of a Kondo lattice with a low concentration of conduction electrons is ferromagnetic. Assuming the existence of disorder in the Fermi liquid of the conduction electrons the authors show that the ferromagnetic state can be suppressed by the effect of the spin fluctuations of the disordered Fermi liquid

  20. Approaching Pomeranchuk instabilities from ordered phase: A crossing-symmetric equation method

    International Nuclear Information System (INIS)

    Reidy, Kelly; Quader, Khandker; Bedell, Kevin

    2014-01-01

    We explore features of a 3D Fermi liquid near generalized Pomeranchuk instabilities using a tractable crossing-symmetric equation method. We approach the instabilities from the ordered ferromagnetic phase. We find “quantum multi-criticality” as approach to the ferromagnetic instability drives instability in other channel(s). It is found that a charge nematic instability precedes and is driven by Pomeranchuk instabilities in both the ℓ=0 spin and density channels

  1. Anisotropic magnetocapacitance in ferromagnetic-plate capacitors

    Science.gov (United States)

    Haigh, J. A.; Ciccarelli, C.; Betz, A. C.; Irvine, A.; Novák, V.; Jungwirth, T.; Wunderlich, J.

    2015-04-01

    The capacitance of a parallel-plate capacitor can depend on the applied magnetic field. Previous studies have identified capacitance changes induced via classical Lorentz force or spin-dependent Zeeman effects. Here we measure a magnetization direction-dependent capacitance in parallel-plate capacitors where one plate is a ferromagnetic semiconductor, gallium manganese arsenide. This anisotropic magnetocapacitance is due to the anisotropy in the density of states dependent on the magnetization through the strong spin-orbit interaction.

  2. Strain-induced extrinsic high-temperature ferromagnetism in the Fe-doped hexagonal barium titanate.

    Science.gov (United States)

    Zorko, A; Pregelj, M; Gomilšek, M; Jagličić, Z; Pajić, D; Telling, M; Arčon, I; Mikulska, I; Valant, M

    2015-01-09

    Diluted magnetic semiconductors possessing intrinsic static magnetism at high temperatures represent a promising class of multifunctional materials with high application potential in spintronics and magneto-optics. In the hexagonal Fe-doped diluted magnetic oxide, 6H-BaTiO3-δ, room-temperature ferromagnetism has been previously reported. Ferromagnetism is broadly accepted as an intrinsic property of this material, despite its unusual dependence on doping concentration and processing conditions. However, the here reported combination of bulk magnetization and complementary in-depth local-probe electron spin resonance and muon spin relaxation measurements, challenges this conjecture. While a ferromagnetic transition occurs around 700 K, it does so only in additionally annealed samples and is accompanied by an extremely small average value of the ordered magnetic moment. Furthermore, several additional magnetic instabilities are detected at lower temperatures. These coincide with electronic instabilities of the Fe-doped 3C-BaTiO3-δ pseudocubic polymorph. Moreover, the distribution of iron dopants with frozen magnetic moments is found to be non-uniform. Our results demonstrate that the intricate static magnetism of the hexagonal phase is not intrinsic, but rather stems from sparse strain-induced pseudocubic regions. We point out the vital role of internal strain in establishing defect ferromagnetism in systems with competing structural phases.

  3. Angular and linear momentum of excited ferromagnets

    NARCIS (Netherlands)

    Yan, P.; Kamra, A.; Cao, Y.; Bauer, G.E.W.

    2013-01-01

    The angular momentum vector of a Heisenberg ferromagnet with isotropic exchange interaction is conserved, while under uniaxial crystalline anisotropy the projection of the total spin along the easy axis is a constant of motion. Using Noether's theorem, we prove that these conservation laws persist

  4. Ferromagnetism in poly(N-perfluorophenylpyrrole)

    Energy Technology Data Exchange (ETDEWEB)

    Čík, G., E-mail: gabriel.cik@stuba.sk [Department of Environmental Engineering, Faculty of Chemical and Food Technology, Slovak University of Technology, 812 37 Bratislava (Slovakia); Šeršeň, F. [Institute of Chemistry, Faculty of Natural Sciences, Comenius University, 842 15 Bratislava (Slovakia); Dlháň, L. [Department of Inorganic Chemistry, Faculty of Chemical and Food Technology, Slovak University of Technology, 812 37 Bratislava (Slovakia); Zálupský, P. [Department of Organic Chemistry, Faculty of Chemical and Food Technology, Slovak University of Technology, 812 37 Bratislava (Slovakia); Rapta, P. [Department of Physical Chemistry, Faculty of Chemical and Food Technology, Slovak University of Technology, 812 37 Bratislava (Slovakia); Hrnčariková, K. [Department of Organic Chemistry, Faculty of Chemical and Food Technology, Slovak University of Technology, 812 37 Bratislava (Slovakia); Plecenik, T. [Department of Experimental Physics, Faculty of Mathematics, Physics and Informatics, Comenius University, 842 48 Bratislava (Slovakia)

    2015-10-01

    Magnetic properties of the synthesized poly(N-perfluorophenylpyrrole) were studied. The synthesized polymer dissolves in common organic solvents. By the zero-field cooling-field cooling method (ZFC–FC) we found that at low temperatures (T{sub b}<50 K) the synthetic polymer reaches a state with prevailing ferromagnetism. The synthesized polymer retained ferromagnetism even at 300 K. The anomalous magnetic behavior was explained in terms of spin–spin interaction of triplet polarons. As can be seen from the calculated spin density of SOMO and SOMO 1 such a state arise as a consequence of 1-D spin interactions of polarons. Based on the calculated and visualized spin density (SOMO) on the polymer chain such interactions can be explained by the theory of flat-band-ferromagnetism. - Highlights: • We synthesized a new conducting polymer poly(N-perfluorophenylpyrrole). • By the ZFC–FC and EPR methods we measured magnetic properties of the prepared polymer. • We discussed stability and interactions of the polarons in triplet states. • At low temperatures the synthesized polymer reached ferromagnetism.

  5. Correlation Effects and Hidden Spin-Orbit Entangled Electronic Order in Parent and Electron-Doped Iridates Sr_{2}IrO_{4}

    Directory of Open Access Journals (Sweden)

    Sen Zhou

    2017-10-01

    Full Text Available Analogs of the high-T_{c} cuprates have been long sought after in transition metal oxides. Because of the strong spin-orbit coupling, the 5d perovskite iridates Sr_{2}IrO_{4} exhibit a low-energy electronic structure remarkably similar to the cuprates. Whether a superconducting state exists as in the cuprates requires understanding the correlated spin-orbit entangled electronic states. Recent experiments discovered hidden order in the parent and electron-doped iridates, some with striking analogies to the cuprates, including Fermi surface pockets, Fermi arcs, and pseudogap. Here, we study the correlation and disorder effects in a five-orbital model derived from the band theory. We find that the experimental observations are consistent with a d-wave spin-orbit density wave order that breaks the symmetry of a joint twofold spin-orbital rotation followed by a lattice translation. There is a Berry phase and a plaquette spin flux due to spin procession as electrons hop between Ir atoms, akin to the intersite spin-orbit coupling in quantum spin Hall insulators. The associated staggered circulating J_{eff}=1/2 spin current can be probed by advanced techniques of spin-current detection in spintronics. This electronic order can emerge spontaneously from the intersite Coulomb interactions between the spatially extended iridium 5d orbitals, turning the metallic state into an electron-doped quasi-2D Dirac semimetal with important implications on the possible superconducting state suggested by recent experiments.

  6. Magnetic Hamiltonian and phase diagram of the quantum spin liquid Ca10Cr7O28

    Science.gov (United States)

    Balz, Christian; Lake, Bella; Nazmul Islam, A. T. M.; Singh, Yogesh; Rodriguez-Rivera, Jose A.; Guidi, Tatiana; Wheeler, Elisa M.; Simeoni, Giovanna G.; Ryll, Hanjo

    2017-05-01

    A spin liquid is a new state of matter with topological order where the spin moments continue to fluctuate coherently down to the lowest temperatures rather than develop static long-range magnetic order as found in conventional magnets. For spin liquid behavior to arise in a material the magnetic Hamiltonian must be "frustrated", where the combination of lattice geometry, interactions, and anisotropies gives rise to competing spin arrangements in the ground state. Theoretical Hamiltonians which produce spin liquids are spin ice, the Kitaev honeycomb model, and the kagome antiferromagnet. Spin liquid behavior, however, in real materials is rare because they can only approximate these Hamiltonians and often have weak higher-order terms that destroy the spin liquid state. Ca10Cr7O28 is a new quantum spin liquid candidate with magnetic Cr5 + ions that possess quantum spin number S =½ . The spins are entirely dynamic in the ground state and the excitation spectrum is broad and diffuse, as is typical of spinons which are the excitations of a spin liquid. In this paper we determine the Hamiltonian of Ca10Cr7O28 using inelastic neutron scattering under high magnetic field to induce a field-polarized paramagnetic ground state and spin-wave excitations that can be fitted to extract the interactions. We further explore the phase diagram by using inelastic neutron scattering and heat capacity measurements and establish the boundaries of the spin liquid phase as a function of magnetic field and temperature. Our results show that Ca10Cr7O28 consists of distorted kagome bilayers with several isotropic ferromagnetic and antiferromagnetic interactions where, unexpectedly, the ferromagnetic interactions are stronger than the antiferromagnetic ones. This complex Hamiltonian does not correspond to any known spin liquid model and points to new directions in the search for quantum spin liquid behavior.

  7. Temperature dependent dynamic susceptibility calculations for itinerant ferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Cooke, J. F.

    1980-10-01

    Inelastic neutron scattering experiments have revealed a variety of interesting and unusual phenomena associated with the spin dynamics of the 3-d transition metal ferromagnets nickel and iron. An extensive series of calculations based on the itinerant electron formalism has demonstrated that the itinerant model does provide an excellent quantitative as well as qualitative description of the measured spin dynamics of both nickel and iron at low temperatures. Recent angular photo emission experiments have indicated that there is a rather strong temperature dependence of the electronic spin-splitting which, from relatively crude arguments, appears to be inconsistent with neutron scattering results. In order to investigate this point and also the origin of spin-wave renormalization, a series of calculations of the dynamic susceptibility of nickel and iron has been undertaken. The results of these calculations indicate that a discrepancy exists between the interpretations of neutron and photoemission experimental results regarding the temperature dependence of the spin-splitting of the electronic energy bands.

  8. Ferroelectricity and lattice distortion associated with spin orderings in a multiferroic delafossite AgFeO2

    Science.gov (United States)

    Terada, Noriki; Khalyavin, Dmitry D.; Manuel, Pascal; Tsujimoto, Yoshihiro; Knight, Kevin; Radaelli, Paolo G.; Suzuki, Hiroyuki S.; Kitazawa, Hideaki

    2013-01-01

    Spin-lattice coupling and ferroelectric polarization associated with the magnetic ordering in a geometrically frustrated delafossite AgFeO2 have been studied by high resolution neutron powder diffraction and dielectric measurements. The cycloidal magnetic ground state found in this material and the character of the lattice distortions are unprecedented in the family of the delafossite compounds, implying a peculiar mechanism lifting the geometrical frustration.

  9. Ferroelectricity and lattice distortion associated with spin orderings in a multiferroic delafossite AgFeO2

    Directory of Open Access Journals (Sweden)

    Suzuki Hiroyuki S.

    2013-01-01

    Full Text Available Spin-lattice coupling and ferroelectric polarization associated with the magnetic ordering in a geometrically frustrated delafossite AgFeO2 have been studied by high resolution neutron powder diffraction and dielectric measurements. The cycloidal magnetic ground state found in this material and the character of the lattice distortions are unprecedented in the family of the delafossite compounds, implying a peculiar mechanism lifting the geometrical frustration.

  10. Rectifying full-counting statistics in a spin Seebeck engine

    Science.gov (United States)

    Tang, Gaomin; Chen, Xiaobin; Ren, Jie; Wang, Jian

    2018-02-01

    In terms of the nonequilibrium Green's function framework, we formulate the full-counting statistics of conjugate thermal spin transport in a spin Seebeck engine, which is made by a metal-ferromagnet insulator interface driven by a temperature bias. We obtain general expressions of scaled cumulant generating functions of both heat and spin currents that hold special fluctuation symmetry relations, and demonstrate intriguing properties, such as rectification and negative differential effects of high-order fluctuations of thermal excited spin current, maximum output spin power, and efficiency. The transport and noise depend on the strongly fluctuating electron density of states at the interface. The results are relevant for designing an efficient spin Seebeck engine and can broaden our view in nonequilibrium thermodynamics and the nonlinear phenomenon in quantum transport systems.

  11. Magnetic Spin-Wave Properties of Ferromagnetic Nanosystems of Various Shapes. Peculiarities of the Border Conditions Accounting in the Process of the Wavenumber Values Spectrum Finding

    Directory of Open Access Journals (Sweden)

    Volodymyr V. Kulish

    2017-09-01

    Conclusions. The obtained expressions for the spectrum of the values of the investigated spin waves’ wavenumbers can be used for a wider range of cases than the ones obtained in the previous papers dedicated to the investigated configurations of nanosystems. For a nanotube of the circular cross-section with small (compared to the inverse characteristic size of the nanotube cross-section values of the longitudinal wave number, the dependence of the latter on the transverse wave number is weak, as well as for the big longitudinal to transverse wavenumber component ratio. The obtained dependence is also represented graphically.

  12. Theory of relaxation phenomena in a spin-3/2 Ising system near the second-order phase transition temperature

    International Nuclear Information System (INIS)

    Keskin, Mustafa; Canko, Osman

    2005-01-01

    The relaxation behavior of the spin-3/2 Ising model Hamiltonian with bilinear and biquadratic interactions near the second-order phase transition temperature or critical temperature is studied by means of the Onsager's theory of irreversible thermodynamics or the Onsager reciprocity theorem (ORT). First, we give the equilibrium case briefly within the molecular-field approximation in order to study the relaxation behavior by using the ORT. Then, the ORT is applied to the model and the kinetic equations are obtained. By solving these equations, three relaxation times are calculated and examined for temperatures near the second-order phase transition temperature. It is found that one of the relaxation times goes to infinity near the critical temperature on either side, the second relaxation time makes a cusp at the critical temperature and third one behaves very differently in which it terminates at the critical temperature while approaching it, then showing a 'flatness' property and then decreases. We also study the influences of the Onsager rate coefficients on the relaxation times. The behavior of these relaxation times is discussed and compared with the spin-1/2 and spin-1 Ising systems

  13. Sign-Problem-Free Quantum Monte Carlo Study on Thermodynamic Properties and Magnetic Phase Transitions in Orbital-Active Itinerant Ferromagnets

    Directory of Open Access Journals (Sweden)

    Shenglong Xu

    2015-06-01

    Full Text Available The microscopic mechanism of itinerant ferromagnetism is a long-standing problem due to the lack of nonperturbative methods to handle strong magnetic fluctuations of itinerant electrons. We nonpertubatively study thermodynamic properties and magnetic phase transitions of a two-dimensional multiorbital Hubbard model exhibiting ferromagnetic ground states. Quantum Monte Carlo simulations are employed, which are proved in a wide density region free of the sign problem usually suffered by simulations for fermions. Both Hund’s coupling and electron itinerancy are essential for establishing the ferromagnetic coherence. No local magnetic moments exist in the system as a priori; nevertheless, the spin channel remains incoherent showing the Curie-Weiss-type spin magnetic susceptibility down to very low temperatures at which the charge channel is already coherent, exhibiting a weakly temperature-dependent compressibility. For the SU(2 invariant systems, the spin susceptibility further grows exponentially as approaching zero temperature in two dimensions. In the paramagnetic phase close to the Curie temperature, the momentum space Fermi distributions exhibit strong resemblance to those in the fully polarized state. The long-range ferromagnetic ordering appears when the symmetry is reduced to the Ising class, and the Curie temperature is accurately determined. These simulations provide helpful guidance to searching for novel ferromagnetic materials in both strongly correlated d-orbital transition-metal oxide layers and the p-orbital ultracold atom optical lattice systems.

  14. Singular ferromagnetic susceptibility of the transverse-field Ising antiferromagnet on the triangular lattice

    Science.gov (United States)

    Biswas, Sounak; Damle, Kedar

    2018-02-01

    A transverse magnetic field Γ is known to induce antiferromagnetic three-sublattice order of the Ising spins σz in the triangular lattice Ising antiferromagnet at low enough temperature. This low-temperature order is known to melt on heating in a two-step manner, with a power-law ordered intermediate temperature phase characterized by power-law correlations at the three-sublattice wave vector Q : ˜cos(Q .R ⃗) /|R⃗| η (T ) with the temperature-dependent power-law exponent η (T )∈(1 /9 ,1 /4 ) . Here, we use a quantum cluster algorithm to study the ferromagnetic easy-axis susceptibility χu(L ) of an L ×L sample in this power-law ordered phase. Our numerical results are consistent with a recent prediction of a singular L dependence χu(L ) ˜L2 -9 η when η (T ) is in the range (1 /9 ,2 /9 ) . This finite-size result implies, via standard scaling arguments, that the ferromagnetic susceptibility χu(B ) to a uniform field B along the easy axis is singular at intermediate temperatures in the small B limit, χu(B ) ˜|B| -4/-18 η 4 -9 η for η (T )∈(1 /9 ,2 /9 ) , although there is no ferromagnetic long-range order in the low temperature state. Additionally we establish similar two-step melting behavior (via a study of the order parameter susceptibility χQ) in the case of the ferrimagnetic three-sublattice ordered phase which is stabilized by ferromagnetic next-neighbor couplings (J2) and confirm that the ferromagnetic susceptibility obeys the predicted singular form in the associated power-law ordered phase.

  15. Spin excitations in the quasi-two-dimensional charge-ordered insulator α -(BEDT-TTF ) 2I3 probed via 13C NMR

    Science.gov (United States)

    Ishikawa, Kyohei; Hirata, Michihiro; Liu, Dong; Miyagawa, Kazuya; Tamura, Masafumi; Kanoda, Kazushi

    2016-08-01

    The spin excitations from the nonmagnetic charge-ordered insulating state of α -(BEDT-TTF ) 2I3 at ambient pressure have been investigated by probing the static and low-frequency dynamic spin susceptibilities via site-selective nuclear magnetic resonance at 13C sites. The site-dependent values of the shift and the spin-lattice relaxation rate 1 /T1 below the charge-ordering transition temperature (TCO≈135 K ) demonstrate a spin density imbalance in the unit cell, in accord with the charge-density ratio reported earlier. The shift and 1 /T1 show activated temperature dependence with a static (shift) gap ΔS≈47 -52 meV and a dynamic (1 /T1 ) gap ΔR≈40 meV . The sizes of the gaps are well described in terms of a localized spin model, where spin-1/2 antiferromagnetic dimer chains are weakly coupled with each other.

  16. Oscillating electromagnetic soliton in an anisotropic ferromagnetic medium

    Energy Technology Data Exchange (ETDEWEB)

    Sathishkumar, P., E-mail: perumal_sathish@yahoo.co.in [Department of Physics, K.S.R. College of Engineering (Autonomous), Tiruchengode 637215, Tamilnadu (India); Senjudarvannan, R. [Department of Physics, Jansons Institute of Technology, Karumathampatty, Coimbatore 641659 (India)

    2017-05-01

    We investigate theoretically the propagation of electromagnetic oscillating soliton in the form of breather in an anisotropic ferromagnetic medium. The interaction of magnetization with the magnetic field component of the electromagnetic (EM) wave has been studied by solving Maxwell's equations coupled with a Landau–Lifshitz equation for the magnetization of the medium. We made a small perturbation on the magnetization and magnetic field along the direction of propagation of EM wave in the framework of reductive perturbation method and the associated nonlinear magnetization dynamics is governed by a generalized derivative nonlinear Schrödinger (DNLS) equation. In order to understand the dynamics of the concerned system, we employ the Jacobi elliptic function method to solve the DNLS equation and deduce breatherlike soliton modes for the EM wave in the medium. - Highlights: • The propagation of electromagnetic oscillating soliton in an anisotropic ferromagnetic medium is investigated in the presence of varying external magnetic field. • The magnetization and electromagnetic wave modulates in the form of breathing like oscillating solitons. • The governing nonlinear spin dynamical equation is studied through a reductive perturbation method. • The magnetization components of the ferromagnetic medium are derived using Jacobi elliptic functions method with the aid of symbolic computation.

  17. Spin Torques in Systems with Spin Filtering and Spin Orbit Interaction

    KAUST Repository

    Ortiz Pauyac, Christian

    2016-06-19

    In the present thesis we introduce the reader to the field of spintronics and explore new phenomena, such as spin transfer torques, spin filtering, and three types of spin-orbit torques, Rashba, spin Hall, and spin swapping, which have emerged very recently and are promising candidates for a new generation of memory devices in computer technology. A general overview of these phenomena is presented in Chap. 1. In Chap. 2 we study spin transfer torques in tunnel junctions in the presence of spin filtering. In Chap. 3 we discuss the Rashba torque in ferromagnetic films, and in Chap. 4 we study spin Hall effect and spin swapping in ferromagnetic films, exploring the nature of spin-orbit torques based on these mechanisms. Conclusions and perspectives are summarized in Chap. 5.

  18. Orbital occupancy evolution across spin- and charge-ordering transitions in YBaFe2O5

    Science.gov (United States)

    Lindén, J.; Lindroos, F.; Karen, P.

    2017-08-01

    Thermal evolution of the Fe2+-Fe3+ valence mixing in YBaFe2O5 is investigated using Mössbauer spectroscopy. In this high-spin double-cell perovskite, the d6 and d5 Fe states differ by the single minority-spin electron which then controls all the spin- and charge-ordering transitions. Orbital occupancies can be extracted from the spectra in terms of the dxz , dz2 and either dx2-y2 (Main Article) or dxy (Supplement) populations of this electron upon conserving its angular momentum. At low temperatures, the minority-spin electrons fill up the ordered dxz orbitals of Fe2+, in agreement with the considerable orthorhombic distortion of the structure. Heating through the Verwey transition supplies 93% of the mixing entropy, at which point the predominantly mixing electron occupies mainly the dx2-y2 /dxy orbitals weakly bonding the two Fe atoms that face each other across the bases of their coordination pyramids. This might stabilize a weak coulombic checkerboard order suggested by McQueeney et alii in Phys. Rev. B 87(2013)045127. When the remaining 7% of entropy is supplied at a subsequent transition, the mixing electron couples the two Fe atoms predominantly via their dz2 orbitals. The valence mixing concerns more than 95% of the Fe atoms present in the crystalline solid; the rest is semi-quantitatively interpreted as domain walls and antiphase boundaries formed upon cooling through the Néel and Verwey-transition temperatures, respectively.

  19. Spin-orbit torque in two-dimensional antiferromagnetic topological insulators

    KAUST Repository

    Ghosh, Sumit

    2017-01-24

    We investigate spin transport in two-dimensional ferromagnetic (FTI) and antiferromagnetic (AFTI) topological insulators. In the presence of an in-plane magnetization AFTI supports zero energy modes, which enables topologically protected edge conduction at low energy. We address the nature of current-driven spin torque in these structures and study the impact of spin-independent disorder. Interestingly, upon strong disorder the spin torque develops an antidamping component (i.e., even upon magnetization reversal) along the edges, which could enable current-driven manipulation of the antiferromagnetic order parameter. This antidamping torque decreases when increasing the system size and when the system enters the trivial insulator regime.

  20. Observation of long-range ferromagnetic order in the heavy-fermion compuound URu/sub 1. 2/Re/sub 0. 8/Si/sub 2/ by neutron scattering

    Energy Technology Data Exchange (ETDEWEB)

    Torikachvili, M.S.; Rebelsky, L.; Motoya, K.; Shapiro, S.M.; Dalichaouch, Y.; Maple, M.B.

    1989-01-01

    We have performed a neutron scattering study of the heavy-fermion compound URu/sub 1.2/Re/sub 0.8/Si/sub 2/, in order to verify the occurrence of long-range ferromagnetic order. This study consisted of measurements of elastic, inelastic, and polarized neutron scattering, measurement of low-angle critical scattering, and the determination of the temperature dependence of the order parameter. We found a sharp peak in the critical scattering at /approx/ 30 K for the wavevector q = 0.08 /angstrom//sup /minus/1/; and an enhancement of the intensity at the position of the (101) nuclear Bragg reflection below the Curie temperature. These measurements suggest the occurrence of long-range magnetic order. The value of the ordered moment is estimated to be /approx/ 0.53 /mu//sub B/ at 10 K. 17 refs., 3 figs.

  1. Half-metallic superconducting triplet spin multivalves

    Science.gov (United States)

    Alidoust, Mohammad; Halterman, Klaus

    2018-02-01

    We study spin switching effects in finite-size superconducting multivalve structures. We examine F1F2SF3 and F1F2SF3F4 hybrids where a singlet superconductor (S) layer is sandwiched among ferromagnet (F) layers with differing thicknesses and magnetization orientations. Our results reveal a considerable number of experimentally viable spin-valve configurations that lead to on-off switching of the superconducting state. For S widths on the order of the superconducting coherence length ξ0, noncollinear magnetization orientations in adjacent F layers with multiple spin axes leads to a rich variety of triplet spin-valve effects. Motivated by recent experiments, we focus on samples where the magnetizations in the F1 and F4 layers exist in a fully spin-polarized half-metallic phase, and calculate the superconducting transition temperature, spatially and energy resolved density of states, and the spin-singlet and spin-triplet superconducting correlations. Our findings demonstrate that superconductivity in these devices can be completely switched on or off over a wide range of magnetization misalignment angles due to the generation of equal-spin and opposite-spin triplet pairings.

  2. The effect of disorder and fluctuations on the magnetotransport of a double-exchange ferromagnet (abstract)

    International Nuclear Information System (INIS)

    Byers, J.M.

    1996-01-01

    The discovery of colossal magnetoresistance (CMR) in the doped perovskite manganites has reawakened interest in the double-exchange mechanism proposed to Zener. To account for the close relation between ferromagnetism and metallic transport in lanthanum manganites doped with divalent cation (Ca, Sr, Ba) Zener claimed that an electron could delocalize on lattice of spins and still conform to Hund close-quote s Rule if a ferromagnetic coupling between spins were mediated by that same electron. Thus, the onset of metallic behavior (delocalization) is intimately linked to ferromagnetic ordering of the spin lattice. Clearly, the double-exchange mechanism provides some necessary physics but is not sufficient in explaining the key mystery of the CMR materials: What causes the large peak in the resistivity vs. temperature and why is it removed by an applied magnetic field. The effect of disorder and fluctuations on the double-exchange mechanism may provide the answers. Several sources of disorder in these materials act to form a mobility edge via Anderson localization: intrinsic divalent/trivalent cation disorder, off-diagonal disorder caused by the spin lattice and oxygen vacancy disorder. A mean-field calculation reveals that below the Curie temperature those carriers aligned opposite to the magnetization experience a narrowing band as the temperature is reduced. Fermi glass behavior is induced in this minority carrier band by the Fermi level falling below the mobility edge. However, the mean-field result does not contain a peak in resistivity since the majority carrier band does not behave as a Fermi glass and effectively open-quote open-quote shorts out close-quote close-quote the more resistive minority conduction channel. The formation of the resistivity peak requires the inclusion of ferromagnetic fluctuations above the Curie temperature that tend to open-quote open-quote mix close-quote close-quote the two conduction channels. (Abstract Truncated)

  3. Electrically detected ferromagnetic resonance

    NARCIS (Netherlands)

    Goennenwein, S.T.B.; Schink, S.W.; Brandlmaier, A.; Boger, A.; Opel, M.; Gross, R.; Keizer, R.S.; Klapwijk, T.M.; Gupta, A.; Huebl, H.; Bihler, C.; Brandt, M.S.

    2007-01-01

    We study the magnetoresistance properties of thin ferromagnetic CrO2 and Fe3O4 films under microwave irradiation. Both the sheet resistance ? and the Hall voltage VHall characteristically change when a ferromagnetic resonance (FMR) occurs in the film. The electrically detected ferromagnetic

  4. Communication: Orientational self-ordering of spin-labeled cholesterol analogs in lipid bilayers in diluted conditions

    Energy Technology Data Exchange (ETDEWEB)

    Kardash, Maria E.; Dzuba, Sergei A., E-mail: dzuba@kinetics.nsc.ru [Voevodsky Institute of Chemical Kinetics and Combustion, 630090 Novosibirsk, Russia, and Novosibirsk State University, 630090 Novosibirsk (Russian Federation)

    2014-12-07

    Lipid-cholesterol interactions are responsible for different properties of biological membranes including those determining formation in the membrane of spatial inhomogeneities (lipid rafts). To get new information on these interactions, electron spin echo (ESE) spectroscopy, which is a pulsed version of electron paramagnetic resonance (EPR), was applied to study 3β-doxyl-5α-cholestane (DCh), a spin-labeled analog of cholesterol, in phospholipid bilayer consisted of equimolecular mixture of 1,2-dipalmitoyl-sn-glycero-3-phosphocholine and 1,2-dioleoyl-sn-glycero-3-phosphocholine. DCh concentration in the bilayer was between 0.1 mol.% and 4 mol.%. For comparison, a reference system containing a spin-labeled 5-doxyl-stearic acid (5-DSA) instead of DCh was studied as well. The effects of “instantaneous diffusion” in ESE decay and in echo-detected (ED) EPR spectra were explored for both systems. The reference system showed good agreement with the theoretical prediction for the model of spin labels of randomly distributed orientations, but the DCh system demonstrated remarkably smaller effects. The results were explained by assuming that neighboring DCh molecules are oriented in a correlative way. However, this correlation does not imply the formation of clusters of cholesterol molecules, because conventional continuous wave EPR spectra did not show the typical broadening due to aggregation of spin labels and the observed ESE decay was not faster than in the reference system. So the obtained data evidence that cholesterol molecules at low concentrations in biological membranes can interact via large distances of several nanometers which results in their orientational self-ordering.

  5. Theory of Magnetic Ordering in the Heavy Rare Earths: Ab Initio Electronic Origin of Pair- and Four-Spin Interactions

    Science.gov (United States)

    Mendive-Tapia, Eduardo; Staunton, Julie B.

    2017-05-01

    We describe a disordered local moment theory for long-period magnetic phases and investigate the temperature and magnetic field dependence of the magnetic states in the heavy rare earth elements (HREs), namely, paramagnetic, conical and helical antiferromagnetic (HAFM), fan, and ferromagnetic (FM) states. We obtain a generic HRE magnetic phase diagram which is consequent on the response of the common HRE valence electronic structure to f -electron magnetic moment ordering. The theory directly links the first-order HAFM-FM transition to the loss of Fermi surface nesting, induced by this magnetic ordering, as well as provides a template for analyzing the other phases and exposing where f -electron correlation effects are particularly intricate. Gadolinium, for a range of hexagonal, close-packed lattice constants c and a , is the prototype, described ab initio, and applications to other HREs are made straightforwardly by scaling the effective pair and quartic local moment interactions that emerge naturally from the theory with de Gennes factors and choosing appropriate lanthanide-contracted c and a values.

  6. Scattering bottleneck for spin dynamics in metallic helical antiferromagnetic dysprosium

    Science.gov (United States)

    Langner, M. C.; Roy, S.; Kemper, A. F.; Chuang, Y.-D.; Mishra, S. K.; Versteeg, R. B.; Zhu, Y.; Hertlein, M. P.; Glover, T. E.; Dumesnil, K.; Schoenlein, R. W.

    2015-11-01

    Ultrafast studies of magnetization dynamics have revealed fundamental processes that govern spin dynamics, and the emergence of time-resolved x-ray techniques has extended these studies to long-range spin structures that result from interactions with competing symmetries. By combining time-resolved resonant x-ray scattering and ultrafast magneto-optical Kerr studies, we show that the dynamics of the core spins in the helical magnetic structure occur on much longer time scales than the excitation of conduction electrons in the lanthanide metal Dy. The observed spin behavior differs markedly from that observed in the ferromagnetic phase of other lanthanide metals or transition metals and is strongly dependent on temperature and excitation fluence. This unique behavior results from coupling of the real-space helical spin structure to the shape of the conduction electron Fermi surface in momentum space, which creates a bottleneck in spin scattering events that transfer the valence excitation to the core spins. The dependence of the dynamics on the intersite interactions renders the helical ordering much more robust to perturbations than simple ferromagnetic or antiferromagnetic ordering, where dynamics are driven primarily by on-site interactions.

  7. Comparison between muon spin rotation and neutron scattering studies on the 3-dimensional magnetic ordering of La2CuO(4-y)

    Science.gov (United States)

    Uemura, Y. J.; Kossler, W. J.; Kempton, J. R.; Yu, X. H.; Schone, H. E.; Opie, D.; Stronach, C. E.; Brewer, J. H.; Kiefl, R. F.; Kreitzman, S. R.

    1988-01-01

    Muon spin rotation and neutron scattering studies on powder and single-crystal specimens of La2CuO(4-y) are compared. The apparent difference between the muon and neutron results for the ordered moment in the antiferromagnetic state is interpreted as the signature of increasingly short-ranged spatial spin correlations with increasing oxygen content.

  8. Dynamics of antiferromagnetic skyrmion driven by the spin Hall effect

    Science.gov (United States)

    Jin, Chendong; Song, Chengkun; Wang, Jianbo; Liu, Qingfang

    2016-10-01

    Magnetic skyrmion moved by the spin-Hall effect is promising for the application of the generation racetrack memories. However, the Magnus force causes a deflected motion of skyrmion, which limits its application. Here, we create an antiferromagnetic skyrmion by injecting a spin-polarized pulse in the nanostripe and investigate the spin Hall effect-induced motion of antiferromagnetic skyrmion by micromagnetic simulations. In contrast to ferromagnetic skyrmion, we find that the antiferromagnetic skyrmion has three evident advantages: (i) the minimum driving current density of antiferromagnetic skyrmion is about two orders smaller than the ferromagnetic skyrmion; (ii) the velocity of the antiferromagnetic skyrmion is about 57 times larger than the ferromagnetic skyrmion driven by the same value of current density; (iii) antiferromagnetic skyrmion can be driven by the spin Hall effect without the influence of Magnus force. In addition, antiferromagnetic skyrmion can move around the pinning sites due to its property of topological protection. Our results present the understanding of antiferromagnetic skyrmion motion driven by the spin Hall effect and may also contribute to the development of antiferromagnetic skyrmion-based racetrack memories.

  9. Glass-like recovery of antiferromagnetic spin ordering in a photo-excited manganite Pr0.7Ca0.3MnO3

    Energy Technology Data Exchange (ETDEWEB)

    Zhou, S. Y.; Langner, M. C.; Zhu, Y.; Chuang, Y. -D.; Rini, M.; Glover, T. E.; Hertlein, M. P.; Gonzalez, A.G. Cruz; Tahir, N.; Tomioka, Y.; Tokura, Y.; Hussain, Z.; Schoenlein, R. W.

    2014-01-16

    Electronic orderings of charges, orbitals and spins are observed in many strongly correlated electron materials, and revealing their dynamics is a critical step toward understanding the underlying physics of important emergent phenomena. Here we use time-resolved resonant soft x-ray scattering spectroscopy to probe the dynamics of antiferromagnetic spin ordering in the manganite Pr0:7Ca0:3MnO3 following ultrafast photo-exitation. Our studies reveal a glass-like recovery of the spin ordering and a crossover in the dimensionality of the restoring interaction from quasi-1D at low pump fluence to 3D at high pump fluence. This behavior arises from the metastable state created by photo-excitation, a state characterized by spin disordered metallic droplets within the larger charge- and spin-ordered insulating domains. Comparison with time-resolved resistivity measurements suggests that the collapse of spin ordering is correlated with the insulator-to-metal transition, but the recovery of the insulating phase does not depend on the re-establishment of the spin ordering.

  10. Topological magnon bands in ferromagnetic star lattice

    Science.gov (United States)

    Owerre, S. A.

    2017-05-01

    The experimental observation of topological magnon bands and thermal Hall effect in a kagomé lattice ferromagnet Cu(1-3, bdc) has inspired the search for topological magnon effects in various insulating ferromagnets that lack an inversion center allowing a Dzyaloshinskii-Moriya (DM) spin-orbit interaction. The star lattice (also known as the decorated honeycomb lattice) ferromagnet is an ideal candidate for this purpose because it is a variant of the kagomé lattice with additional links that connect the up-pointing and down-pointing triangles. This gives rise to twice the unit cell of the kagomé lattice, and hence more interesting topological magnon effects. In particular, the triangular bridges on the star lattice can be coupled either ferromagnetically or antiferromagnetically which is not possible on the kagomé lattice ferromagnets. Here, we study DM-induced topological magnon bands, chiral edge modes, and thermal magnon Hall effect on the star lattice ferromagnet in different parameter regimes. The star lattice can also be visualized as the parent material from which topological magnon bands can be realized for the kagomé and honeycomb lattices in some limiting cases.

  11. Possible evidence for spin-transfer torque induced by spin-triplet supercurrent

    KAUST Repository

    Li, Lailai

    2017-10-04

    Cooper pairs in superconductors are normally spin singlet. Nevertheless, recent studies suggest that spin-triplet Cooper pairs can be created at carefully engineered superconductor-ferromagnet interfaces. If Cooper pairs are spin-polarized they would transport not only charge but also a net spin component, but without dissipation, and therefore minimize the heating effects associated with spintronic devices. Although it is now established that triplet supercurrents exist, their most interesting property - spin - is only inferred indirectly from transport measurements. In conventional spintronics, it is well known that spin currents generate spin-transfer torques that alter magnetization dynamics and switch magnetic moments. The observation of similar effects due to spin-triplet supercurrents would not only confirm the net spin of triplet pairs but also pave the way for applications of superconducting spintronics. Here, we present a possible evidence for spin-transfer torques induced by triplet supercurrents in superconductor/ferromagnet/superconductor (S/F/S) Josephson junctions. Below the superconducting transition temperature T_c, the ferromagnetic resonance (FMR) field at X-band (~ 9.0 GHz) shifts rapidly to a lower field with decreasing temperature due to the spin-transfer torques induced by triplet supercurrents. In contrast, this phenomenon is absent in ferromagnet/superconductor (F/S) bilayers and superconductor/insulator/ferromagnet/superconductor (S/I/F/S) multilayers where no supercurrents pass through the ferromagnetic layer. These experimental observations are discussed with theoretical predictions for ferromagnetic Josephson junctions with precessing magnetization.

  12. Final Report. Novel Behavior of Ferromagnet/Superconductor Hybrid Systems

    Energy Technology Data Exchange (ETDEWEB)

    Birge, Norman [Michigan State Univ., East Lansing, MI (United States)

    2016-09-26

    Final report for grant DE-FG02-06ER46341. This work has produced a most convincing experimental demonstration that spin-triplet supercurrent can appear in Josephson junctions containing ferromagnetic materials, even when the superconducting electrodes are conventional, spin-singlet superconductors.

  13. Magnetic excitations in CuMn spin-glass alloys

    International Nuclear Information System (INIS)

    Tsunoda, Y.; Kunitomi, N.; Cable, J.W.

    1985-01-01

    Recent neutron scattering measurements have helped to clarify two important features of CuMn spin glasses. Murani and co-workers have studied the dynamical behavior of spin-glass systems and have observed characteristic ferromagnetic spin correlations with a broad distribution of relaxation times and a dynamical freezing process. By means of the polarization analysis technique, Cable and co-workers have observed the coexistence of two types of magnetic short-range order (MSRO): one is a modulated-spin structure, and the other is a ferromagnetic cluster associated with the atomic short-range order (ASRO). These ordered regions produce diffraction maxima which are found at the (1 1/2 +/- delta 0) and the (1 1/2 0) reciprocal lattice points, respectively. Both of these observations seem to be essential for understanding the CuMn spin-glass system. However, the physical relationship of these properties is not yet understood. The authors have studied the inelastic scattering of neutrons around the magnetic diffuse peak positions of a Cu/sub 78.7/Mn/sub 21.3/ single crystal. The spin-glass freezing temperature of a CuMn alloy with this Mn concentration is estimated to be T/sub f/ approx. 90 K. Most of the data were taken by scanning along the [0 1 0] direction from the (1 0 0) to the (1 1 0) reciprocal lattice points

  14. Orbital-dependent second-order scaled-opposite-spin correlation functionals in the optimized effective potential method

    Energy Technology Data Exchange (ETDEWEB)

    Grabowski, Ireneusz, E-mail: ig@fizyka.umk.pl; Śmiga, Szymon; Buksztel, Adam [Institute of Physics, Faculty of Physics, Astronomy and Informatics, Nicolaus Copernicus University, Grudziadzka 5, 87-100 Torun (Poland); Fabiano, Eduardo [National Nanotechnology Laboratory, Istituto Nanoscienze–CNR, Via per Arnesano, I-73100 Lecce (Italy); Teale, Andrew M. [School of Chemistry, University of Nottingham, University Park, Nottingham NG7 2RD (United Kingdom); Centre for Theoretical and Computational Chemistry, Department of Chemistry, University of Oslo, P.O. Box 1033 Blindern, N-0315 Oslo (Norway); Sala, Fabio Della [National Nanotechnology Laboratory, Istituto Nanoscienze–CNR, Via per Arnesano, I-73100 Lecce (Italy); Center for Biomolecular Nanotechnologies @UNILE, Istituto Italiano di Tecnologia (IIT), Via Barsanti, 73010 Arnesano (LE) (Italy)

    2014-07-14

    The performance of correlated optimized effective potential (OEP) functionals based on the spin-resolved second-order correlation energy is analysed. The relative importance of singly- and doubly- excited contributions as well as the effect of scaling the same- and opposite- spin components is investigated in detail comparing OEP results with Kohn–Sham (KS) quantities determined via an inversion procedure using accurate ab initio electronic densities. Special attention is dedicated in particular to the recently proposed scaled-opposite–spin OEP functional [I. Grabowski, E. Fabiano, and F. Della Sala, Phys. Rev. B 87, 075103 (2013)] which is the most advantageous from a computational point of view. We find that for high accuracy, a careful, system dependent, selection of the scaling coefficient is required. We analyse several size-extensive approaches for this selection. Finally, we find that a composite approach, named OEP2-SOSh, based on a post-SCF rescaling of the correlation energy can yield high accuracy for many properties, being comparable with the most accurate OEP procedures previously reported in the literature but at substantially reduced computational effort.

  15. Mapping the Ultrafast Changes of Continuous Shape Measures in Photoexcited Spin Crossover Complexes without Long-Range Order

    Energy Technology Data Exchange (ETDEWEB)

    Canton, S. E. [Department; Zhang, X. [X-ray; Lawson Daku, M. L. [Département; Liu, Y. [Centre; Zhang, J. [School; Alvarez, S. [Departament

    2015-01-30

    Establishing a tractable yet complete reaction coordinate for the spin-state interconversion in d(4)-d(7) transition metal complexes is an integral aspect of controlling the dynamics that govern their functionality. For spin crossover phenomena, the limitations of a single-mode approximation that solely accounts for an isotropic increase in the metal-ligand bond length have long been recognized for all but the simple octahedral monodentate FeII compounds. However, identifying the coupled deformations that also impact on the unimolecular rate constants remains experimentally and theoretically challenging, especially for samples that do not display long-range order or when crystallization profoundly alters the dynamics. Owing to the rapid progress in ultrafast X-ray absorption spectroscopy (XAS), it is now possible to obtain transient structural information in any physical phase with unprecedented details. Using picosecond XAS and DFT modeling, the structure adopted by the photoinduced high-spin state of solvated [Fe(terpy)(2)](2+) (terpy: 2,2':6',2 ''-terpyridine) has been recently established. Based on these results, the methodology of the continuous shape measure is applied to classify and quantify the short-lived distortion of the first coordination shell. The reaction coordinate of the spin-state interconversion is clearly identified as a double axial bending. This finding sets a benchmark for gauging the influence of first-sphere and second-sphere interactions in the family of FeII complexes that incorporate terpy derivatives. Some implications for the optimization of related photoactive FeII complexes are also outlined.

  16. Absence of magnetic long range order in Ba3ZnRu2O9. A spin-liquid candidate in the S = 3/2 dimer lattice

    International Nuclear Information System (INIS)

    Terasaki, Ichiro; Igarashi, Taichi; Nagai, Takayuki

    2017-01-01

    We have discovered a novel candidate for a spin liquid state in a ruthenium oxide composed of dimers of S = 3/2 spins of Ru 5+ , Ba 3 ZnRu 2 O 9 . This compound lacks a long range order down to 37 mK, which is a temperature 5000-times lower than the magnetic interaction scale of around 200 K. Partial substitution for Zn can continuously vary the magnetic ground state from an antiferromagnetic order to a spin-gapped state through the liquid state. This indicates that the spin-liquid state emerges from a delicate balance of inter- and intra-dimer interactions, and the spin state of the dimer plays a vital role. This unique feature should realize a new type of quantum magnetism. (author)

  17. Polarized-neutron-scattering study of the spin-wave excitations in the 3-k ordered phase of uranium antimonide.

    Science.gov (United States)

    Magnani, N; Caciuffo, R; Lander, G H; Hiess, A; Regnault, L-P

    2010-03-24

    The anisotropy of magnetic fluctuations propagating along the [1 1 0] direction in the ordered phase of uranium antimonide has been studied using polarized inelastic neutron scattering. The observed polarization behavior of the spin waves is a natural consequence of the longitudinal 3-k magnetic structure; together with recent results on the 3-k-transverse uranium dioxide, these findings establish this technique as an important tool to study complex magnetic arrangements. Selected details of the magnon excitation spectra of USb have also been reinvestigated, indicating the need to revise the currently accepted theoretical picture for this material.

  18. Neutron diffraction study of the pressure-induced magnetic ordering in the spin gap system TlCuCl sub 3

    CERN Document Server

    Oosawa, A; Kakurai, K; Fujisawa, M; Tanaka, H

    2003-01-01

    Neutron elastic scattering measurements have been performed under a hydrostatic pressure in order to investigate the spin structure of the pressure-induced magnetic ordering in the spin gap system TlCuCl sub 3. Below the ordering temperature T sub N = 16.9 K for the hydrostatic pressure P = 1.48 GPa, magnetic Bragg reflections were observed at reciprocal lattice points Q = (h, 0, l) with integer h and odd l, which are equivalent to those points with the lowest magnetic excitation energy at ambient pressure. This indicates that the spin gap close due to the applied pressure. The spin structure of the pressure-induced magnetic ordered state for P = 1.48 GPa was determined. (author)

  19. Spin transport in spin filtering magnetic tunneling junctions.

    Science.gov (United States)

    Li, Yun; Lee, Eok Kyun

    2007-11-01

    Taking into account spin-orbit coupling and s-d interaction, we investigate spin transport properties of the magnetic tunneling junctions with spin filtering barrier using Landauer-Büttiker formalism implemented with the recursive algorithm to calculate the real-space Green function. We predict completely different bias dependence of negative tunnel magnetoresistance (TMR) between the systems composed of nonmagnetic electrode (NM)/ferromagnetic barrier (FB)/ferromagnet (FM) and NM/FB/FM/NM spin filtering tunnel junctions (SFTJs). Analyses of the results provide us possible ways of designing the systems which modulate the TMR in the negative magnetoresistance regime.

  20. Magnons coherent transmission and its heat transport at ultrathin insulating ferromagnetic nanojunctions

    Directory of Open Access Journals (Sweden)

    Ghantous M. Abou

    2012-06-01

    Full Text Available A model calculation is presented for the magnons coherent transmission and corresponding heat transport at magnetic insulating nanojunctions. The system consists of a ferromagnetically ordered ultrathin insulating junction between two semi-infinite ferromagnetically ordered leads. Spin dynamics are analyzed using the equations of motion for the spin precession displacements, valid for the range of temperatures of interest. Coherent scattering cross-sections at the junction boundary are calculated using the phase field matching theory, for all the incidence angles on the boundary from the lead bands, for arbitrary angles of incidence, at variable temperatures, and for different nano thicknesses of the ultrathin junction. The model is general; it is applied in particular to the Fe/Gd/Fe system with a sandwiched ferromagnetic Gd junction. It yields also the thermal conductivity due to the magnons coherent transmission between the two leads when these are maintained at slightly different temperatures. The calculation is carried out for state of the art values of the exchange constants, and elucidates the relation between the coherent scattering transmission of magnons and their thermal conductivity, for different thicknesses.

  1. Spin-torque generation in topological insulator based heterostructures

    KAUST Repository

    Fischer, Mark H.

    2016-03-11

    Heterostructures utilizing topological insulators exhibit a remarkable spin-torque efficiency. However, the exact origin of the strong torque, in particular whether it stems from the spin-momentum locking of the topological surface states or rather from spin-Hall physics of the topological-insulator bulk, remains unclear. Here, we explore a mechanism of spin-torque generation purely based on the topological surface states. We consider topological-insulator-based bilayers involving ferromagnetic metal (TI/FM) and magnetically doped topological insulators (TI/mdTI), respectively. By ascribing the key theoretical differences between the two setups to location and number of active surface states, we describe both setups within the same framework of spin diffusion of the nonequilibrium spin density of the topological surface states. For the TI/FM bilayer, we find large spin-torque efficiencies of roughly equal magnitude for both in-plane and out-of-plane spin torques. For the TI/mdTI bilayer, we elucidate the dominance of the spin-transfer-like torque. However, we cannot explain the orders of magnitude enhancement reported. Nevertheless, our model gives an intuitive picture of spin-torque generation in topological-insulator-based bilayers and provides theoretical constraints on spin-torque generation due to topological surface states.

  2. Spin-Mechanical Inertia in Antiferromagnet

    Science.gov (United States)

    Cheng, Ran; Wu, Xiaochuan; Xiao, Di

    Interplay between spin dynamics and mechanical motions is responsible for numerous striking phenomena, which has shaped a rapidly expanding field known as spin-mechanics. The guiding principle of this field has been the conservation of angular momentum that involves both quantum spins and classical mechanical rotations. However, in an antiferromagnet, the macroscopic magnetization vanishes while the order parameter (Néel order) does not carry an angular momentum. It is therefore not clear whether the order parameter dynamics has any mechanical consequence as its ferromagnetic counterparts. Here we demonstrate that the Néel order dynamics affects the mechanical motion of a rigid body by modifying its inertia tensor in the presence of strong magnetocrystalline anisotropy. This effect depends on temperature when magnon excitations are considered. Such a spin-mechanical inertia can produce measurable consequences at nanometer scales. Our discovery establishes spin-mechanical inertia as an essential ingredient to properly describe spin-mechanical effects in AFs, which supplements the known governing physics from angular momentum conservation. This work was supported by the DOE, Basic Energy Sciences, Grant No. DE-SC0012509. D.X. also acknowledges support from a Research Corporation for Science Advancement Cottrell Scholar Award.

  3. Magnetoanisotropic Andreev reflection in ferromagnet-superconductor junctions.

    Science.gov (United States)

    Högl, Petra; Matos-Abiague, Alex; Žutić, Igor; Fabian, Jaroslav

    2015-09-11

    Andreev reflection spectroscopy of ferromagnet-superconductor (FS) junctions [corrected] is an important probe of spin polarization. We theoretically investigate spin-polarized transport in FS junctions in the presence of Rashba and Dresselhaus interfacial spin-orbit fields and show that Andreev reflection can be controlled by changing the magnetization orientation. We predict a giant in- and out-of-plane magnetoanisotropy of the junction conductance. If the ferromagnet is highly spin polarized-in the half-metal limit-the magnetoanisotropic Andreev reflection depends universally on the spin-orbit fields only. Our results show that Andreev reflection spectroscopy can be used for sensitive probing of interfacial spin-orbit fields in a FS junction.

  4. Coexistence of short- and long-range ferromagnetic order in nanocrystalline Fe2Mn1−xCuxAl (x=0.0, 0.1 and 0.3) synthesized by high-energy ball milling

    International Nuclear Information System (INIS)

    Thanh, Tran Dang; Nanto, Dwi; Tuyen, Ngo Thi Uyen; Nan, Wen-Zhe; Yu, YiKyung; Tartakovsky, Daniel M.; Yu, S.C.

    2015-01-01

    In this work, we prepared nanocrystalline Fe 2 Mn 1−x Cu x Al (x=0.0, 0.1 and 0.3) powders by the high energy ball milling technique, and then studied their critical properties. Our analysis reveals that the increase of Cu-doping concentration (up to x=0.3) in these powders leads to a gradual increase of the ferromagnetic–paramagnetic transition temperature from 406 to 452 K. The Banerjee criterion suggests that all the samples considered undergo a second-order phase transition. A modified Arrott plot and scaling analysis indicate that the critical exponents (β=0.419 and 0.442, γ=1.082 and 1.116 for x=0.0 and 0.1, respectively) are located in between those expected for the 3D-Heisenberg and the mean-field models; the values of β=0.495 and γ=1.046 for x=0.3 sample are very close to those of the mean-field model. These features reveal the coexistence of the short- and long-range ferromagnetic order in the nanocrystalline Fe 2 Mn 1−x Cu x Al powders. Particularly, as the concentration of Cu increases, values of the critical exponent shift towards those of the mean-field model. Such results prove the Cu doping favors establishing a long-range ferromagnetic order. - Highlights: • Fe 2 Mn 1−x Cu x Al nanocrystals were prepared by a high energy ball milling method. • A coexistence of the short- and long-range FM order in the nanocrystals. • Cu doping favors establishing a long-range FM order in the nanocrystals. • All the ΔS m (T, H) data are followed a universal master curve

  5. High-performance molybdenum disulfide field-effect transistors with spin tunnel contacts.

    Science.gov (United States)

    Dankert, André; Langouche, Lennart; Kamalakar, Mutta Venkata; Dash, Saroj Prasad

    2014-01-28

    Molybdenum disulfide has recently emerged as a promising two-dimensional semiconducting material for nanoelectronic, optoelectronic, and spintronic applications. Here, we investigate the field-effect transistor behavior of MoS2 with ferromagnetic contacts to explore its potential for spintronics. In such devices, we elucidate that the presence of a large Schottky barrier resistance at the MoS2/ferromagnet interface is a major obstacle for the electrical spin injection and detection. We circumvent this problem by a reduction in the Schottky barrier height with the introduction of a thin TiO2 tunnel barrier between the ferromagnet and MoS2. This results in an enhancement of the transistor on-state current by 2 orders of magnitude and an increment in the field-effect mobility by a factor of 6. Our magnetoresistance calculation reveals that such integration of ferromagnetic tunnel contacts opens up the possibilities for MoS2-based spintronic devices.

  6. Carrier-induced ferromagnetism in half-metallic Co-doped ZnS-diluted magnetic semiconductor: a DFT study

    Science.gov (United States)

    Saikia, D.; Borah, J. P.

    2018-03-01

    Systematic experimental and theoretical calculations have been performed to investigate the origin of the carrier-induced ferromagnetism in the Co-doped ZnS-diluted magnetic semiconductors. The crystalline structure, morphology of the chemically synthesized Co-doped ZnS nanoparticles are evaluated using X-ray diffraction (XRD) and transmission electron microscopy (TEM) and obtained the average crystallite size in the range 5-8 nm. Fourier transform-infrared spectra reveal the characteristic Zn-S vibrations of cubic ZnS and also show the splitting of peaks with increasing Co concentration which indicates that the Co-doping level beyond 3% affects the structure of ZnS. The room temperature ferromagnetic behavior analyzed by M- H curve exhibited up to the doping level 5%, achieving due to the indirect ` p- d' exchange interactions between the localized ` d' spins of Co2+ ion and the free-delocalized carriers in the host lattice. The existence of the antiferromagnetic coupling is discernable beyond the 5% doping level, owing to the short-range super-exchange interactions between the characteristic ` d' spins of the Co2+ ions which minimize the ferromagnetic ordering. Band structure and density of states (DOS) calculations demonstrate the p- d hybridization mechanism in Co-doped ZnS system which is the main cause of realizing ferromagnetic ordering in the system and also shows the half-metallic characteristics with the combination of semiconducting and metallic nature in the spin-up and spin-down states, respectively.

  7. Fermi Surface Manipulation by External Magnetic Field Demonstrated for a Prototypical Ferromagnet

    Directory of Open Access Journals (Sweden)

    E. Młyńczak

    2016-12-01

    Full Text Available We consider the details of the near-surface electronic band structure of a prototypical ferromagnet, Fe(001. Using high-resolution angle-resolved photoemission spectroscopy, we demonstrate openings of the spin-orbit-induced electronic band gaps near the Fermi level. The band gaps, and thus the Fermi surface, can be manipulated by changing the remanent magnetization direction. The effect is of the order of ΔE=100  meV and Δk=0.1  Å^{−1}. We show that the observed dispersions are dominated by the bulk band structure. First-principles calculations and one-step photoemission calculations suggest that the effect is related to changes in the electronic ground state and not caused by the photoemission process itself. The symmetry of the effect indicates that the observed electronic bulk states are influenced by the presence of the surface, which might be understood as related to a Rashba-type effect. By pinpointing the regions in the electronic band structure where the switchable band gaps occur, we demonstrate the significance of spin-orbit interaction even for elements as light as 3d ferromagnets. These results set a new paradigm for the investigations of spin-orbit effects in the spintronic materials. The same methodology could be used in the bottom-up design of the devices based on the switching of spin-orbit gaps such as electric-field control of magnetic anisotropy or tunneling anisotropic magnetoresistance.

  8. Charge, spin and orbital order in the candidate multiferroic material LuFe{sub 2}O{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Groot, Joost de

    2012-06-28

    main focus is on samples exhibiting a sharp magnetic transition to long-range spin order at T{sub N}{proportional_to}240 K accompanied at T{sub LT} {proportional_to}170 K by a low temperature phase transition into a phase with glassy magnetic dynamics. It is proposed that this magnetic behavior best approximates the intrinsic defectfree behavior of LuFe{sub 2}O{sub 4}. The spin structures of the long-range ordered phases could be refined properly by neutron diffraction as antiferromagnetic (AFM) and ferrimagnetic (fM) spin alignments. The two solutions exhibit a simple geometrical relation, where all spins in half of the bilayers change their sign. Furthermore, it is demonstrated that at T{sub N} and H=0 competing AFM and fM spin structures, which correspond respectively to ferro and antiferro stacking of equivalently ordered bilayers, are nearly degenerate. The observation of diffuse magnetic scattering in neutron diffraction far above T{sub N} indicates the random stacking of still individually ferrimagnetic ordered bilayers. The first crystal structural refinement, taking into account the superstructure due to the CO in LuFe{sub 2}O{sub 4}, was performed on these stoichiometric samples with the help of a monoclinic unit-cell and the C2/m symmetry. By clearly identifying the positions of Fe{sup 2+} and Fe{sup 3+} valences in this structure with the Bond Valence Sum (BVS) analysis, a completely new and unexpected CO pattern with charged Fe/O bilayers emerges. This new CO arrangement with charged, and consequently non-polar, bilayers is in strong contrast to all previously suggested CO configurations with polar bilayers. The implications of this result on ''ferroelectricity from CO'' in LuFe{sub 2}O{sub 4} are discussed, addressing the possibility of polarizing the charged bilayers by an external electric or magnetic field, which could not be verified for our samples. In summary, a possible ferroelectric behavior of LuFe{sub 2}O{sub 4} from CO is

  9. Magnetic Correlations in the Quasi-2D Semiconducting Ferromagnet CrSiTe3

    Science.gov (United States)

    Williams, Travis; Aczel, Adam; Lumsden, Mark; Nagler, Steve; Stone, Matt; Yan, Jianqiang; Mandrus, David

    2015-03-01

    The quasi-two-dimensional, semiconducting ferromagnet CrSiTe3 is a particularly attractive candidate for spintronics applications due its relatively accessible transition temperature and large magnetic moment. In this study, we use neutron scattering to measure the static and dynamic magnetic properties. Neutron diffraction shows 3D ordering below TC=33K, but two dimensional static correlations persist up to at least 300K. The inelastic neutron scattering data shows two distinct spin wave bands, which are nearly dispersionless along the c-axis. The exchange constants extracted from the data suggest that the spins are very nearly Heisenberg, but only weakly coupled perpendicular to the 2D planes. Above the Curie temperature, the spin wave intensity decreases drastically but, like the static correlations, these dynamic magnetic correlations persist within the 2D planes up to room temperature.

  10. Effective bond orders from two-step spin-orbit coupling approaches: the I2, At2, IO(+), and AtO(+) case studies.

    Science.gov (United States)

    Maurice, Rémi; Réal, Florent; Gomes, André Severo Pereira; Vallet, Valérie; Montavon, Gilles; Galland, Nicolas

    2015-03-07

    The nature of chemical bonds in heavy main-group diatomics is discussed from the viewpoint of effective bond orders, which are computed from spin-orbit wave functions resulting from spin-orbit configuration interaction calculations. The reliability of the relativistic correlated wave functions obtained in such two-step spin-orbit coupling frameworks is assessed by benchmark studies of the spectroscopic constants with respect to either experimental data, or state-of-the-art fully relativistic correlated calculations. The I2, At2, IO(+), and AtO(+) species are considered, and differences and similarities between the astatine and iodine elements are highlighted. In particular, we demonstrate that spin-orbit coupling weakens the covalent character of the bond in At2 even more than electron correlation, making the consideration of spin-orbit coupling compulsory for discussing chemical bonding in heavy (6p) main group element systems.

  11. Tunneling time and Hartman effect in a ferromagnetic graphene superlattice

    Directory of Open Access Journals (Sweden)

    Farhad Sattari

    2012-03-01

    Full Text Available Using transfer-matrix and stationary phase methods, we study the tunneling time (group delay time in a ferromagnetic monolayer graphene superlattice. The system we peruse consists of a sequence of rectangular barriers and wells, which can be realized by putting a series of electronic gates on the top of ferromagnetic graphene. The magnetization in the two ferromagnetic layers is aligned parallel. We find out that the tunneling time for normal incident is independent of spin state of electron as well as the barrier height and electron Fermi energy while for the oblique incident angles the tunneling time depends on the spin state of electron and has an oscillatory behavior. Also the effect of barrier width on tunneling time is also investigated and shown that, for normal incident, the Hartman effect disappears in a ferromagnetic graphene superlattice but it appears for oblique incident angles when the x component of the electron wave vector in the barrier is imaginary.

  12. Partial magnetic order in the itinerant-electron magnet MnSi

    Indian Academy of Sciences (India)

    MnSi is an itinerant ferromagnet with a long-wavelength helical modulation of the spin structure. Macroscopic measurements suggest that the ordering temperature c is reduced with increasing pressure from c = 30 K at = 0 to zero at the critical pressure c = 14.6 kbar. Resistivity measurements show that MnSi enters a ...

  13. Polarization dependence of the magnetic fluctuations in the weak itinerant ferromagnet MnSi below T{sub c}

    Energy Technology Data Exchange (ETDEWEB)

    Boeni, P.; Tixier, S. [Paul Scherrer Inst. (PSI), Villigen (Switzerland); Endoh, Y. [Tohoku Univ., Sendai (Japan); Roessli, B. [Institut Max von Laue - Paul Langevin, 75 - Paris (France); Shirane, G. [Brookhaven (United States)

    1997-09-01

    The dispersion of the spin-flip and non-spin-flip excitations in the weak itinerant ferromagnet MnSi have been measured in the ferromagnetic phase using inelastic polarized neutron scattering. Spin wave excitations are well defined at energy transfers as large as 7 meV. The cross section of the non-spin-flip excitations is compatible with a quasielastic response function. (author) 2 figs., 3 refs.

  14. Conductance spectra of asymmetric ferromagnet/ferromagnet/ferromagnet junctions

    Energy Technology Data Exchange (ETDEWEB)

    Pasanai, K., E-mail: krisakronmsu@gmail.com

    2017-01-15

    A theory of tunneling spectroscopy of ferromagnet/ferromagnet/ferromagnet junctions was studied. We applied a delta-functional approximation for the interface scattering properties under a one-dimensional system of a free electron approach. The reflection and transmission probabilities were calculated in the ballistic regime, and the conductance spectra were then calculated using the Landauer formulation. The magnetization directions were set to be either parallel (P) or anti-parallel (AP) alignments, for comparison. We found that the conductance spectra was suppressed when increasing the interfacial scattering at the interfaces. Moreover, the electron could exhibit direct transmission when the thickness was rather thin. Thus, there was no oscillation in this case. However, in the case of a thick layer the conductance spectra oscillated, and this oscillation was most prominent when the middle layer thickness increased. In the case of direct transmission, the conductance spectra of P and AP systems were definitely suppressed with increased exchange energy of the middle ferromagnet. This also refers to an increase in the magnetoresistance of the junction. In the case of oscillatory behavior, the positions of the resonance peaks were changed as the exchange energy was changed. - Highlights: • The conductance spectra of a FM/FM/FM junction were calculated. • The conductance spectra were suppressed by the exchange energy. • The exchange energy and the potential strength play similar roles in the junctions.

  15. Room-temperature five-tesla coercivity of a rare-earth-free shell-ferromagnet

    Science.gov (United States)

    Scheibel, F.; Spoddig, D.; Meckenstock, R.; Gottschall, T.; ćakır, A.; Krenke, T.; Farle, M.; Gutfleisch, O.; Acet, M.

    2017-05-01

    Ni2MnX-based Heusler (X: main group element), when enriched with Mn, will decompose into ferromagnetic Ni2MnX and antiferromagnetic NiMn when temper-annealed around 650 K. When the starting material is chosen such that the X-composition is about 5 at. % and the annealing takes place in the presence of a magnetic field of about 1 T, the resulting material is a composite of nanoprecipitate strongly pinned shell-ferromagnets with a soft ferromagnetic core embedded in the antiferromagnetic matrix. We show that the shells of the precipitates are so strongly pinned that the estimated field required to fully reorient the spins is in the order of 20 T. We examine in a Ni50.0Mn45.1In4.9 sample the pinning and the magnetic interactions of the precipitate and the matrix with magnetization and ferromagnetic resonance studies carried out in fields ranging up to 14 and 12 T, respectively.

  16. Robust spin transfer torque in antiferromagnetic tunnel junctions

    KAUST Repository

    Saidaoui, Hamed Ben Mohamed

    2017-04-18

    We theoretically study the current-induced spin torque in antiferromagnetic tunnel junctions, composed of two semi-infinite antiferromagnetic layers separated by a tunnel barrier, in both clean and disordered regimes. We find that the torque enabling electrical manipulation of the Néel antiferromagnetic order parameter is out of plane, ∼n×p, while the torque competing with the antiferromagnetic exchange is in plane, ∼n×(p×n). Here, p and n are the Néel order parameter direction of the reference and free layers, respectively. Their bias dependence shows behavior similar to that in ferromagnetic tunnel junctions, the in-plane torque being mostly linear in bias, while the out-of-plane torque is quadratic. Most importantly, we find that the spin transfer torque in antiferromagnetic tunnel junctions is much more robust against disorder than that in antiferromagnetic metallic spin valves due to the tunneling nature of spin transport.

  17. Magnetic nesting and co-existence of ferromagnetism and superconductivity

    International Nuclear Information System (INIS)

    Elesin, V.F.; Kapaev, V.V.; Kopaev, Yu.V.

    2004-01-01

    In the case of providing for the magnetic nesting conditions of the electron spin dispersion law the co-existence of ferromagnetism and superconductivity is possible by any high magnetization. The co-existence of ferromagnetism and superconductivity in the layered cuprate compounds of the RuSr 2 GdCu 2 O 8 -type is explained on this basis, wherein due to the nonstrict provision of the magnetic nesting condition there exists the finite but sufficiently high critical magnetization [ru

  18. Spin-polarized light-emitting diodes based on organic bipolar spin valves

    Energy Technology Data Exchange (ETDEWEB)

    Vardeny, Zeev Valentine; Nguyen, Tho Duc; Ehrenfreund, Eitan Avraham

    2017-10-25

    Spin-polarized organic light-emitting diodes are provided. Such spin-polarized organic light-emitting diodes incorporate ferromagnetic electrodes and show considerable spin-valve magneto-electroluminescence and magneto-conductivity responses, with voltage and temperature dependencies that originate from the bipolar spin-polarized space charge limited current.

  19. Carrier concentration induced ferromagnetism in semiconductors

    International Nuclear Information System (INIS)

    Story, T.

    2007-01-01

    In semiconductor spintronics the key materials issue concerns ferromagnetic semiconductors that would, in particular, permit an integration (in a single multilayer heterostructure) of standard electronic functions of semiconductors with magnetic memory function. Although classical semiconductor materials, such as Si or GaAs, are nonmagnetic, upon substitutional incorporation of magnetic ions (typically of a few atomic percents of Mn 2+ ions) and very heavy doping with conducting carriers (at the level of 10 20 - 10 21 cm -3 ) a ferromagnetic transition can be induced in such diluted magnetic semiconductors (also known as semimagnetic semiconductors). In the lecture the spectacular experimental observations of carrier concentration induced ferromagnetism will be discussed for three model semiconductor crystals. p - Ga 1-x Mn x As currently the most actively studied and most perspective ferromagnetic semiconductor of III-V group, in which ferromagnetism appears due to Mn ions providing both local magnetic moments and acting as acceptor centers. p - Sn 1-x Mn x Te and p - Ge 1-x Mn x Te classical diluted magnetic semiconductors of IV-VI group, in which paramagnet-ferromagnet and ferromagnet-spin glass transitions are found for very high hole concentration. n - Eu 1-x Gd x Te mixed magnetic crystals, in which the substitution of Gd 3+ ions for Eu 2+ ions creates very high electron concentration and transforms antiferromagnetic EuTe (insulating compound) into ferromagnetic n-type semiconductor alloy. For each of these materials systems the key physical features will be discussed concerning: local magnetic moments formation, magnetic phase diagram as a function of magnetic ions and carrier concentration as well as Curie temperature and magnetic anisotropy engineering. Various theoretical models proposed to explain the effect of carrier concentration induced ferromagnetism in semiconductors will be briefly discussed involving mean field approaches based on Zener and RKKY

  20. Simulation of magnetic tunnel junction in ferromagnetic/insulator/semiconductor structure

    Science.gov (United States)

    Kostrov, Alexander I.; Stempitsky, Viktor R.; Kazimirchik, Vladimir N.

    2008-07-01

    In this work, we present a physical model and electrical macromodel for simulation of Magnetic Tunnel Junction (MTJ) effect based on Ferromagnetic/Insulator/Semiconductor (FIS) nanostructure. A modified Brinkman model has been proposed by including the voltage-dependent density of states of the ferromagnetic electrodes in order to explain the bias dependence magnitoresistance. The model takes into account injection of carriers in the semiconductor and Shottky barrier, electron tunneling through thin insulator and spin-transfer torque writing approach in memory cell. These very promising features should constitute the third generation of Magnetoresistive RAM (MRAM). Besides, the model can efficiently be used to design magnetic CMOS circuits. The behavioral macro-model has been developed by means of Verilog-AMS language and implemented on the Cadence Virtuoso platform with Spectre simulator.

  1. Searching Room Temperature Ferromagnetism in Wide Gap Semiconductors Fe-doped Strontium Titanate and Zinc Oxide

    CERN Document Server

    Pereira, LMC; Wahl, U

    Scientific findings in the very beginning of the millennium are taking us a step further in the new paradigm of technology: spintronics. Upgrading charge-based electronics with the additional degree of freedom of the carriers spin-state, spintronics opens a path to the birth of a new generation of devices with the potential advantages of non-volatility and higher processing speed, integration densities and power efficiency. A decisive step towards this new age lies on the attribution of magnetic properties to semiconductors, the building block of today's electronics, that is, the realization of ferromagnetic semiconductors (FS) with critical temperatures above room temperature. Unfruitful search for intrinsic RT FS lead to the concept of Dilute(d) Magnetic Semiconductors (DMS): ordinary semiconductor materials where 3 d transition metals randomly substitute a few percent of the matrix cations and, by some long-range mechanism, order ferromagnetically. The times are of intense research activity and the last fe...

  2. Unusual magnetic excitations in the weakly ordered spin- 12 chain antiferromagnet Sr2CuO3: Possible evidence for Goldstone magnon coupled with the amplitude mode

    International Nuclear Information System (INIS)

    Sergeicheva, E. G.; Sosin, S. S.; Prozorova, L. A.; Gu, G. D.; Zaliznyak, I. A.

    2017-01-01

    We report on an electron spin resonance (ESR) study of a nearly one-dimensional (1D) spin-1/2 chain antiferromagnet, Sr 2 CuO 3 , with extremely weak magnetic ordering. The ESR spectra at T > T N , in the disordered Luttinger-spin-liquid phase, reveal nearly ideal Heisenberg-chain behavior with only a very small, field-independent linewidth, ~1/T. In the ordered state, below T N , we identify field-dependent antiferromagnetic resonance modes, which are well described by pseudo-Goldstone magnons in the model of a collinear biaxial antiferromagnet. Additionally, we observe a major resonant mode with unusual and strongly anisotropic properties, which is not anticipated by the conventional theory of Goldstone spin waves. Lastly, we propose that this unexpected magnetic excitation can be attributed to a field-independent magnon mode renormalized due to its interaction with the high-energy amplitude (Higgs) mode in the regime of weak spontaneous symmetry breaking.

  3. Structure, magnetic ordering, and spin filtering efficiency of NiFe{sub 2}O{sub 4}(111) ultrathin films

    Energy Technology Data Exchange (ETDEWEB)

    Matzen, S.; Moussy, J.-B., E-mail: jean-baptiste.moussy@cea.fr [CEA, IRAMIS, SPCSI, F-91191 Gif-sur-Yvette (France); Wei, P. [Francis Bitter Magnet Laboratory, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139 (United States); Gatel, C. [CEMES-CNRS, F-31055 Toulouse (France); Cezar, J. C. [ESRF, F-38043 Grenoble (France); Arrio, M. A.; Sainctavit, Ph. [IMPMC, F-75015 Paris (France); Moodera, J. S. [Francis Bitter Magnet Laboratory, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139 (United States); Physics Department, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139 (United States)

    2014-05-05

    NiFe{sub 2}O{sub 4}(111) ultrathin films (3–5 nm) have been grown by oxygen-assisted molecular beam epitaxy and integrated as effective spin-filter barriers. Structural and magnetic characterizations have been performed in order to investigate the presence of defects that could limit the spin filtering efficiency. These analyses have revealed the full strain relaxation of the layers with a cationic order in agreement with the inverse spinel structure but also the presence of antiphase boundaries. A spin-polarization up to +25% has been directly measured by the Meservey-Tedrow technique in Pt(111)/NiFe{sub 2}O{sub 4}(111)/γ-Al{sub 2}O{sub 3}(111)/Al tunnel junctions. The unexpected positive sign and relatively small value of the spin-polarization are discussed, in comparison with predictions and previous indirect tunnelling magnetoresistance measurements.

  4. The Physics of Ferromagnetism

    CERN Document Server

    Miyazaki, Terunobu

    2012-01-01

    This book covers both basic physics of ferromagnetism such as magnetic moment, exchange coupling, magnetic anisotropy and recent progress in advanced ferromagnetic materials. Special interests are focused on NdFeB permanent magnets and the materials studied in the field of spintronics. In the latter, development of tunnel magnetoresistance effect through so called giant magnetoresistance effect is explained.

  5. Detection and quantification of inverse spin Hall effect from spin pumping in permalloy/normal metal bilayers

    NARCIS (Netherlands)

    Mosendz, O.; Vlaminck, V.; Pearson, J.E.; Fradin, F.Y.; Bauer, G.E.W.; Bader, S.D.; Hoffmann, A.

    2010-01-01

    Spin pumping is a mechanism that generates spin currents from ferromagnetic resonance over macroscopic interfacial areas, thereby enabling sensitive detection of the inverse spin Hall effect that transforms spin into charge currents in nonmagnetic conductors. Here we study the spin-pumping-induced

  6. 139La NMR investigation of the charge and spin order in a La1.885Sr0.115CuO4 single crystal

    Science.gov (United States)

    Arsenault, A.; Takahashi, S. K.; Imai, T.; He, W.; Lee, Y. S.; Fujita, M.

    2018-02-01

    139La NMR is suited for investigations into magnetic properties of La2CuO4 -based cuprates in the vicinity of their magnetic instabilities, owing to the modest hyperfine interactions between 139La nuclear spins and Cu electron spins. We report comprehensive 139La NMR measurements on a single-crystal sample of high-Tc superconductor La1.885Sr0.115CuO4 in a broad temperature range across the charge and spin order transitions (Tcharge≃80 K, Tspinneutron≃Tc=30 K). From the high-precision measurements of the linewidth for the nuclear spin Iz=+1 /2 to -1 /2 central transition, we show that paramagnetic line broadening sets in precisely at Tcharge due to enhanced spin correlations within the CuO2 planes. Additional paramagnetic line broadening ensues below ˜35 K, signaling that Cu spins in some segments of CuO2 planes are on the verge of three-dimensional magnetic order. A static hyperfine magnetic field arising from ordered Cu moments along the a b plane, however, begins to develop only below Tspinμ S R=15 -20 K, where earlier muon spin rotation measurements detected Larmor precession for a small volume fraction (˜20 % ) of the sample. Based on the measurement of 139La nuclear-spin-lattice relaxation rate 1 /T1 , we also show that charge order triggers enhancement of low-frequency Cu spin fluctuations inhomogeneously; a growing fraction of 139La sites is affected by enhanced low-frequency spin fluctuations toward the eventual magnetic order, whereas a diminishing fraction continues to exhibit a behavior analogous to the optimally superconducting phase even below Tcharge. These 139La NMR results corroborate our recent 63Cu NMR observation that a very broad, anomalous winglike signal gradually emerges below Tcharge, whereas the normally behaving, narrower main peak is gradually wiped out [T. Imai et al., Phys. Rev. B 96, 224508 (2017), 10.1103/PhysRevB.96.224508]. Furthermore, we show that the enhancement of low-energy spin excitations in the low-temperature regime

  7. Ordering of spin-1/2 excitations of the nucleon in lattice QCD

    International Nuclear Information System (INIS)

    Mahbub, M.S.; Kamleh, Waseem; Leinweber, Derek B.; O Cais, Alan; Williams, Anthony G.

    2010-01-01

    We present results for the negative parity low-lying state of the nucleon, N1/2 - (1535 MeV) S 11 , from a variational analysis method. The analysis is performed in quenched QCD with the FLIC fermion action. The principal focus of this Letter is to explore the level ordering between the Roper (P 11 ) and the negative parity ground (S 11 ) states of the nucleon. Evidence of the physical level ordering is observed at light quark masses. A wide variety of smeared-smeared correlation functions are used to construct correlation matrices. A comprehensive correlation matrix analysis is performed to ensure an accurate isolation of the N1/2 - state.

  8. Decoupling of the Leading Order DGLAP Evolution Equation with Spin Dependent Structure Functions

    Science.gov (United States)

    Azadbakht, F. Teimoury; Boroun, G. R.

    2018-02-01

    We propose an analytical solution for DGLAP evolution equations with polarized splitting functions at the Leading Order (LO) approximation based on the Laplace transform method. It is shown that the DGLAP evolution equations can be decoupled completely into two second order differential equations which then are solved analytically by using the initial conditions δ FS(x,Q2)=F[partial δ FS0(x), δ FS0(x)] and {δ G}(x,Q2)=G[partial δ G0(x), δ G0(x)]. We used this method to obtain the polarized structure function of the proton as well as the polarized gluon distribution function inside the proton and compared the numerical results with experimental data of COMPASS, HERMES, and AAC'08 Collaborations. It was found that there is a good agreement between our predictions and the experiments.

  9. Role of the antiferromagnetic bulk spins in exchange bias

    Energy Technology Data Exchange (ETDEWEB)

    Schuller, Ivan K. [Center for Advanced Nanoscience and Physics Department, University of California San Diego, La Jolla, CA 92093 (United States); Morales, Rafael, E-mail: rafael.morales@ehu.es [Department of Chemical-Physics & BCMaterials, University of the Basque Country UPV/EHU (Spain); IKERBASQUE, Basque Foundation for Science, 48011 Bilbao (Spain); Batlle, Xavier [Departament Física Fonamental and Institut de Nanociència i Nanotecnologia, Universitat de Barcelona, c/ Martí i Franqués s/n, 08028 Barcelona, Catalonia (Spain); Nowak, Ulrich [Department of Physics, University of Konstanz, 78464 Konstanz (Germany); Güntherodt, Gernot [Physics Institute (IIA), RWTH Aachen University, Campus RWTH-Melaten, 52074 Aachen (Germany)

    2016-10-15

    This “Critical Focused Issue” presents a brief review of experiments and models which describe the origin of exchange bias in epitaxial or textured ferromagnetic/antiferromagnetic bilayers. Evidence is presented which clearly indicates that inner, uncompensated, pinned moments in the bulk of the antiferromagnet (AFM) play a very important role in setting the magnitude of the exchange bias. A critical evaluation of the extensive literature in the field indicates that it is useful to think of this bulk, pinned uncompensated moments as a new type of a ferromagnet which has a low total moment, an ordering temperature given by the AFM Néel temperature, with parallel aligned moments randomly distributed on the regular AFM lattice. - Highlights: • We address the role of bulk antiferromagnetic spins in the exchange bias phenomenon. • Significant experiments on how bulk AFM spins determine exchange bias are highlighted. • We explain the model that accounts for experimental results.

  10. Ferromagnetism in the multiband Kondo lattice model

    Science.gov (United States)

    Sharma, A.; Nolting, W.

    2008-08-01

    The ferromagnetic spin-exchange interaction between the itinerant electrons and localized moments on a periodic lattice, studied within the so-called Kondo lattice model, is considered for multiband situation where the hopping integral is a matrix in general. The modified Ruderman-Kittel-Kasuya-Yosida theory, wherein one can map such a model onto an effective Heisenberg-type system, is extended to a multiband case with finite bandwidth and hybridization on a simple-cubic lattice. As an input for the evaluation of the effective exchange integrals, one requires the multiband electronic self-energy, which is taken from an earlier proposed ansatz. Using the above procedure, we determine the magnetic properties of the system such as Curie temperature while calculating the chemical potential and magnetization within a self-consistent scheme for various values of system parameters. The results are discussed in detail and the model is motivated in order to study the electronic, transport, and magnetic properties of real materials like GdN.

  11. The investigation of the magnetodielectric effect in ferroelectric-ferromagnets

    International Nuclear Information System (INIS)

    Gong, S.J.; Jiang, Q.

    2004-01-01

    In ferroelectromagnets, for the coupling interaction between the ferroelectric and magnetic order, the dielectric and magnetic properties are closely correlated. We define this kind of magnetoelectric correlation as magnetodielectric effect. In this Letter, temperature and magnetic field dependence of the magnetodielectric behavior are given thorough research in ferroelectric-ferromagnets. As a function of temperature, large magnetocapacitance and magnetodielectric response are observed around the magnetic phase transition temperature TN. As a function of the external magnetic field, the magnetocapacitance increases with the increasing magnetic field, while the magnetodielectric response decreases with the increasing magnetic field. When the magnetic field is high enough, the magnetocapacitance get saturated and the magnetodielectric response decreases to zero. We also analyze the origin of the magnetodielectric behavior and find that the fluctuation of the spin-pair correlation plays a critical role. Soft-mode theory based on DIFFOUR model and the mean-field theory are combined to deal with the ferroelectromagnetic system

  12. Density Functional Theory studies of spin, charge, and orbital ordering in YBaT.sub.2./sub.O .sub.5./sub. (T = Mn, Fe, Co)

    Czech Academy of Sciences Publication Activity Database

    Vidya, R.; Ravindran, P.; Knížek, Karel; Kjekshus, A.; Fjellvåg, H.

    2008-01-01

    Roč. 47, č. 15 (2008), 6608-6620 ISSN 0020-1669 Institutional research plan: CEZ:AV0Z10100521 Keywords : spin ordering * orbital ordering * transition metal oxides * DFT calculation Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 4.147, year: 2008

  13. Bifurcation analysis and phase diagram of a spin-string model with buckled states.

    Science.gov (United States)

    Ruiz-Garcia, M; Bonilla, L L; Prados, A

    2017-12-01

    We analyze a one-dimensional spin-string model, in which string oscillators are linearly coupled to their two nearest neighbors and to Ising spins representing internal degrees of freedom. String-spin coupling induces a long-range ferromagnetic interaction among spins that competes with a spin-spin antiferromagnetic coupling. As a consequence, the complex phase diagram of the system exhibits different flat rippled and buckled states, with first or second order transition lines between states. This complexity translates to the two-dimensional version of the model, whose numerical solution has been recently used to explain qualitatively the rippled to buckled transition observed in scanning tunneling microscopy experiments with suspended graphene sheets. Here we describe in detail the phase diagram of the simpler one-dimensional model and phase stability using bifurcation theory. This gives additional insight into the physical mechanisms underlying the different phases and the behavior observed in experiments.

  14. Ultrafast Enhancement of Ferromagnetism via Photoexcited Holes inGaMnAs

    Energy Technology Data Exchange (ETDEWEB)

    Wang, J.; Cotoros, I.; Dani, K.M.; Liu, X.; Furdyna, J.K.; Chemla, D.S.

    2007-02-17

    We report on the observation of ultrafast photo-enhanced ferromagnetism in GaMnAs. It is manifested as a transient magnetization increase on a 100-ps time scale, after an initial sub-ps demagnetization. The dynamic magnetization enhancement exhibits a maximum below the Curie temperature {Tc} and dominates the demagnetization component when approaching {Tc}. We attribute the observed ultrafast collective ordering to the p-d exchange interaction between photoexcited holes and Mn spins, leading to a correlation-induced peak around 20K and a transient increase in {Tc}.

  15. Superconductivity and non-Fermi liquid behavior on the border of itinerant ferromagnetism

    Energy Technology Data Exchange (ETDEWEB)

    Ritz, Robert

    2013-10-04

    When magnetic order is suppressed under pressure, a superconducting (SC) phase emerges in the ferromagnet UGe{sub 2} and an extended non-Fermi liquid (NFL) regime is observed in the helimagnet MnSi. We report thermal expansion measurements of UGe{sub 2} under pressure by means of neutron Larmor diffraction. We find a new, putatively non-magnetic transition at the temperature TL at pressures close to the SC phase. In MnSi we report Hall effect measurements under pressure. We find a topological Hall effect, as the signature of a topologically non-trivial spin texture, above the critical pressure in the NFL regime.

  16. Long-time predictability in disordered spin systems following a deep quench

    Science.gov (United States)

    Ye, J.; Gheissari, R.; Machta, J.; Newman, C. M.; Stein, D. L.

    2017-04-01

    We study the problem of predictability, or "nature vs nurture," in several disordered Ising spin systems evolving at zero temperature from a random initial state: How much does the final state depend on the information contained in the initial state, and how much depends on the detailed history of the system? Our numerical studies of the "dynamical order parameter" in Edwards-Anderson Ising spin glasses and random ferromagnets indicate that the influence of the initial state decays as dimension increases. Similarly, this same order parameter for the Sherrington-Kirkpatrick infinite-range spin glass indicates that this information decays as the number of spins increases. Based on these results, we conjecture that the influence of the initial state on the final state decays to zero in finite-dimensional random-bond spin systems as dimension goes to infinity, regardless of the presence of frustration. We also study the rate at which spins "freeze out" to a final state as a function of dimensionality and number of spins; here the results indicate that the number of "active" spins at long times increases with dimension (for short-range systems) or number of spins (for infinite-range systems). We provide theoretical arguments to support these conjectures, and also study analytically several mean-field models: the random energy model, the uniform Curie-Weiss ferromagnet, and the disordered Curie-Weiss ferromagnet. We find that for these models, the information contained in the initial state does not decay in the thermodynamic limit—in fact, it fully determines the final state. Unlike in short-range models, the presence of frustration in mean-field models dramatically alters the dynamical behavior with respect to the issue of predictability.

  17. Scattering of polarized low-energy electrons by ferromagnetic metals

    International Nuclear Information System (INIS)

    Helman, J.S.

    1981-01-01

    A source of spin polarized electrons with remarkable characteristics based on negative electron affinity (NEA) GaAs has recently been developed. It constitutes a unique tool to investigate spin dependent interactions in electron scattering processes. The characteristics and working principles of the source are briefly described. Some theoretical aspects of the scattering of polarized low-energy electrons by ferromagnetic metals are discussed. Finally, the results of the first polarized low-energy electron diffraction experiment using the NEA GaAs source are reviewed; they give information about the surface magnetization of ferromagnetic Ni (110). (Author) [pt

  18. Higher-order Zeeman and spin terms in the electron paramagnetic resonance spin Hamiltonian; their description in irreducible form using Cartesian, tesseral spherical tensor and Stevens' operator expressions

    International Nuclear Information System (INIS)

    McGavin, Dennis G; Tennant, W Craighead

    2009-01-01

    In setting up a spin Hamiltonian (SH) to study high-spin Zeeman and high-spin nuclear and/or electronic interactions in electron paramagnetic resonance (EPR) experiments, it is argued that a maximally reduced SH (MRSH) framed in tesseral combinations of spherical tensor operators is necessary. Then, the SH contains only those terms that are necessary and sufficient to describe the particular spin system. The paper proceeds then to obtain interrelationships between the parameters of the MRSH and those of alternative SHs expressed in Cartesian tensor and Stevens operator-equivalent forms. The examples taken, initially, are those of Cartesian and Stevens' expressions for high-spin Zeeman terms of dimension BS 3 and BS 5 . Starting from the well-known decomposition of the general Cartesian tensor of second rank to three irreducible tensors of ranks 0, 1 and 2, the decomposition of Cartesian tensors of ranks 4 and 6 are treated similarly. Next, following a generalization of the tesseral spherical tensor equations, the interrelationships amongst the parameters of the three kinds of expressions, as derived from equivalent SHs, are determined and detailed tables, including all redundancy equations, set out. In each of these cases the lowest symmetry, 1-bar Laue class, is assumed and then examples of relationships for specific higher symmetries derived therefrom. The validity of a spin Hamiltonian containing mixtures of terms from the three expressions is considered in some detail for several specific symmetries, including again the lowest symmetry. Finally, we address the application of some of the relationships derived here to seldom-observed low-symmetry effects in EPR spectra, when high-spin electronic and nuclear interactions are present.

  19. Micromechanical instruments for ferromagnetic measurements

    CERN Document Server

    Moreland, J

    2003-01-01

    I review some of the novel methods for measuring ferromagnetic properties of thin films based on micromechanical magnetometers and put them into context relative to current research on nanomagnetism. Measurements rely on the detection of mechanical forces or torques on thin films deposited onto microcantilevers. Displacements of the cantilever are detected by optical methods similar to those developed for atomic force microscopy. High sensitivities are achieved by integrating the sample with the detector, allowing magnetic measurements of samples with a total magnetic moment smaller than that detectable with conventional magnetometers. Cantilevers with low spring constants and high mechanical Q are essential for these measurements. Sensitivities better than 10 sup 5 mu sub B are possible at room temperature with the potential for single spin detection below 1 K, where the thermomechanical noise of micromechanical sensors is substantially reduced. (topical review)

  20. Charge and Spin Transport in Spin-orbit Coupled and Topological Systems

    KAUST Repository

    Ndiaye, Papa Birame

    2017-10-31

    In the search for low power operation of microelectronic devices, spin-based solutions have attracted undeniable increasing interest due to their intrinsic magnetic nonvolatility. The ability to electrically manipulate the magnetic order using spin-orbit interaction, associated with the recent emergence of topological spintronics with its promise of highly efficient charge-to-spin conversion in solid state, offer alluring opportunities in terms of system design. Although the related technology is still at its infancy, this thesis intends to contribute to this engaging field by investigating the nature of the charge and spin transport in spin-orbit coupled and topological systems using quantum transport methods. We identified three promising building blocks for next-generation technology, three classes of systems that possibly enhance the spin and charge transport efficiency: (i)- topological insulators, (ii)- spin-orbit coupled magnonic systems, (iii)- topological magnetic textures (skyrmions and 3Q magnetic state). Chapter 2 reviews the basics and essential concepts used throughout the thesis: the spin-orbit coupling, the mathematical notion of topology and its importance in condensed matter physics, then topological magnetism and a zest of magnonics. In Chapter 3, we study the spin-orbit torques at the magnetized interfaces of 3D topological insulators. We demonstrated that their peculiar form, compared to other spin-orbit torques, have important repercussions in terms of magnetization reversal, charge pumping and anisotropic damping. In Chapter 4, we showed that the interplay between magnon current jm and magnetization m in homogeneous ferromagnets with Dzyaloshinskii-Moriya (DM) interaction, produces a field-like torque as well as a damping-like torque. These DM torques mediated by spin wave can tilt the imeaveraged magnetization direction and are similar to Rashba torques for electronic systems. Moreover, the DM torque is more efficient when magnons are

  1. Amplification of spin-current polarization

    Science.gov (United States)

    Saha, D.; Holub, M.; Bhattacharya, P.

    2007-08-01

    A ferromagnet/semiconductor based electrically controlled spin-current amplifier using a dual-drain nonlocal lateral spin valve is demonstrated. The spin polarization injected by the source into the channel is amplified at the second drain contact. An amplified current spin polarization of 100% is measured. The controlled variation of amplifier gain with bias is also demonstrated. The observations are explained in the framework of the spin drift-diffusion model.

  2. Ferromagnetism and half metallicity induced by oxygen vacancies in the double perovskite BaSrNiWO{sub 6}: DFT study

    Energy Technology Data Exchange (ETDEWEB)

    Aharbil, Y. [Laboratoire de Chimie Physique des Matériaux LCPM, Faculté des Sciences Ben M' Sik, Casablanca (Morocco); Labrim, H. [Unité Science de la Matière/DERS/Centre National de l’Energie, des Sciences et des Techniques Nucléaires (CNESTEN), Rabat (Morocco); Benmokhtar, S.; Haddouch, M. Ait [Laboratoire de Chimie Physique des Matériaux LCPM, Faculté des Sciences Ben M' Sik, Casablanca (Morocco); Bahmad, L., E-mail: bahmad@fsr.ac.ma [Mohammed V University in Rabat, Laboratoire de Magnétisme et Physique des Hautes Energies L.M.P.H.E. URAC-12, B.P. 1014, Rabat (Morocco); Belhaj, A. [LIRST, Département de Physique, Faculté Poly-disciplinaire, Université Sultan Moulay Slimane, Béni Mellal (Morocco); Ez-Zahraouy, H.; Benyoussef, A. [Mohammed V University in Rabat, Laboratoire de Magnétisme et Physique des Hautes Energies L.M.P.H.E. URAC-12, B.P. 1014, Rabat (Morocco)

    2016-11-01

    Using the spin polarized density functional theory (DFT) and exploring the Plane-Wave Self-Consistent Field (PWscf) code implemented in Quantum-ESPRESSO package, we investigate the effect of the Oxygen vacancies (V{sub O}) and the Oxygen interstitial (O{sub i}) on the double perovskite BaSrNiWO{sub 6}. This deals with the magnetic ordering and the electronic structure in such a pure sample exhibiting the insulating anti-ferromagnetic (AFM) state. This study shows that the presence of oxygen deficient defects converts the insulating to half metal with ferromagnetic or anti-ferromagnetic states. The magnetic ordering in BaSrNiWO{sub 6−δ} depends on the position of the Oxygen vacancy in the unit cell. However, it has been shown that the Oxygen interstitial preserves the anti-ferromagnetic propriety. We have computed the formation energies of different positions of the Oxygen vacancy (V{sub O}) and the Oxygen interstitial (O{sub i}) in the BaSrNiWO{sub 6} compound. We showed that the formation of V{sub O} is easier and vice versa for the O{sub i} formation. The obtained results reveal(V{sub O}) and the Oxygen interstitial (O{sub i}) that the anti-ferromagnetic can be converted to ferromagnetic in the double perovskite BaSrNiWO{sub 6} induced by Oxygen vacancies V{sub O}. - Highlights: • We have studied the ferromagnetism and Half Metallicity in Double Perovskite BaSrNiWO{sub 6}. • We have applied the Ab-inito calculations using the DFT approach. • We showed the effects induced by Oxygen Vacancies and Oxygen interstitial. • We found that the magnetic ordering in BaSrNiWO{sub 6−δ} depends on the position of the Oxygen vacancy in the unit cell.

  3. Direct-current voltages in (Ga,Mn)As structures induced by ferromagnetic resonance

    Science.gov (United States)

    Chen, Lin; Matsukura, Fumihiro; Ohno, Hideo

    2013-06-01

    Spin pumping is the phenomenon that magnetization precession in a ferromagnetic layer under ferromagnetic resonance produces a pure spin current in an adjacent non-magnetic layer. The pure spin current is converted to a charge current by the spin-orbit interaction, and produces a d.c. voltage in the non-magnetic layer, which is called the inverse spin Hall effect. The combination of spin pumping and inverse spin Hall effect has been utilized to determine the spin Hall angle of the non-magnetic layer in various ferromagnetic/non-magnetic systems. Magnetization dynamics of ferromagnetic resonance also produces d.c. voltage in the ferromagnetic layer through galvanomagnetic effects. Here we show a method to separate voltages of different origins using (Ga,Mn)As/p-GaAs as a model system, where sizable galvanomagnetic effects are present. Neglecting the galvanomagnetic effects can lead to an overestimate of the spin Hall angle by factor of 8, indicating that separating the d.c. voltages of different origins is critical.

  4. Radiography of weakly ferromagnetic metals with polarized neutrons

    Energy Technology Data Exchange (ETDEWEB)

    Schulz, Michael; Calzada, Elbio; Muehlbauer, Martin; Schillinger, Burkhard [FRM II, Garching (Germany); E21, Physik Department TUM, Garching (Germany); Boeni, Peter; Neubauer, Andreas; Pfleiderer, Christian [E21, Physik Department TUM, Garching (Germany)

    2009-07-01

    The depolarization of a neutron beam passing through a ferromagnet crucially depends on the magnetic properties of the sample. Combining neutron depolarisation measurements with neutron radiography allows obtaining spatially resolved information about these properties. For measuring the depolarization, we have installed a longitudinal polarized beam setup at the ANTARES beamline consisting of {sup 3}He polarizers and flat coil spin flippers. With this setup we have performed radiography with polarized neutrons in the weak itinerant ferromagnets Pd{sub 1-x}Ni{sub x} in order to determine the spatial distribution of the Curie temperatures T{sub C} in the samples. The results show that the single crystals are rather inhomogeneous showing large variations in T{sub C}. The data allows firstly to cut out small crystals with improved homogeneity for neutron scattering experiments and secondly to provide feedback for improving the growth techniques for the crystals. In the future we hope to use the potential of this method to map out magnetic domains across large volume samples.

  5. Thermal expansion of two-dimensional itinerant nearly ferromagnetic metal

    International Nuclear Information System (INIS)

    Konno, R; Hatayama, N; Takahashi, Y; Nakano, H

    2009-01-01

    Thermal expansion of two-dimensional itinerant nearly ferromagnetic metal is investigated according to the recent theoretical development of magneto-volume effect for the three-dimensional weak ferromagnets. We particularly focus on the T 2 -linear thermal expansion of magnetic origin at low temperatures, so far disregarded by conventional theories. As the effect of thermal spin fluctuations we have found that the T-linear thermal expansion coefficient shows strong enhancement by assuming the double Lorentzian form of the non-interacting dynamical susceptibility justified in the small wave-number and low frequency region. It grows faster in proportional to y -1/2 as we approach the magnetic instability point than two-dimensional nearly antiferromagnetic metals with ln(1/y s ) dependence, where y and y s are the inverses of the reduced uniform and staggered magnetic susceptibilities, respectively. Our result is consistent with the Grueneisen's relation between the thermal expansion coefficient and the specific heat at low temperatures. In 2-dimensional electron gas we find that the thermal expansion coefficient is divergent with a finite y when the higher order term of non-interacting dynamical susceptibility is taken into account.

  6. Electronic Structure Evolution across the Peierls Metal-Insulator Transition in a Correlated Ferromagnet

    Directory of Open Access Journals (Sweden)

    P. A. Bhobe

    2015-10-01

    Full Text Available Transition metal compounds often undergo spin-charge-orbital ordering due to strong electron-electron correlations. In contrast, low-dimensional materials can exhibit a Peierls transition arising from low-energy electron-phonon-coupling-induced structural instabilities. We study the electronic structure of the tunnel framework compound K_{2}Cr_{8}O_{16}, which exhibits a temperature-dependent (T-dependent paramagnetic-to-ferromagnetic-metal transition at T_{C}=180  K and transforms into a ferromagnetic insulator below T_{MI}=95  K. We observe clear T-dependent dynamic valence (charge fluctuations from above T_{C} to T_{MI}, which effectively get pinned to an average nominal valence of Cr^{+3.75} (Cr^{4+}∶Cr^{3+} states in a 3∶1 ratio in the ferromagnetic-insulating phase. High-resolution laser photoemission shows a T-dependent BCS-type energy gap, with 2G(0∼3.5(k_{B}T_{MI}∼35  meV. First-principles band-structure calculations, using the experimentally estimated on-site Coulomb energy of U∼4  eV, establish the necessity of strong correlations and finite structural distortions for driving the metal-insulator transition. In spite of the strong correlations, the nonintegral occupancy (2.25 d-electrons/Cr and the half-metallic ferromagnetism in the t_{2g} up-spin band favor a low-energy Peierls metal-insulator transition.

  7. 1D ferromagnetic edge contacts to 2D graphene/h-BN heterostructures

    Science.gov (United States)

    Karpiak, Bogdan; Dankert, André; Cummings, Aron W.; Power, Stephen R.; Roche, Stephan; Dash, Saroj P.

    2018-03-01

    We report the fabrication of one-dimensional (1D) ferromagnetic edge contacts to two-dimensional (2D) graphene/h-BN heterostructures. While aiming to study spin injection/detection with 1D edge contacts, a spurious magnetoresistance signal was observed, which is found to originate from the local Hall effect in graphene due to fringe fields from ferromagnetic edge contacts and in the presence of charge current spreading in the nonlocal measurement configuration. Such behavior has been confirmed by the absence of a Hanle signal and gate-dependent magnetoresistance measurements that reveal a change in sign of the signal for the electron- and hole-doped regimes, which is in contrast to the expected behavior of the spin signal. Calculations show that the contact-induced fringe fields are typically on the order of hundreds of mT, but can be reduced below 100 mT with careful optimization of the contact geometry. There may be an additional contribution from magnetoresistance effects due to tunneling anisotropy in the contacts, which needs further investigation. These studies are useful for optimization of spin injection and detection in 2D material heterostructures through 1D edge contacts.

  8. Spin-glass transition in disordered terbium

    International Nuclear Information System (INIS)

    Hauser, J.J.

    1985-01-01

    While crystalline Tb is a helix antiferromagnet with a Neel temperature of 229 K which becomes ferromagnetic at 222 K, disordered Tb exhibits a spin-glass transition. The spin-glass freezing temperature ranges from 183 to 53 K, the lowest temperatures corresponding to the greatest degree of atomic disorder. These experiments constitute the first evidence for an elemental spin-glass. (author)

  9. Field noise near ferromagnetic films

    Science.gov (United States)

    McMichael, Robert; Liu, Hau-Jian; Yoon, Seungha

    Thermally driven magnetization fluctuations can be viewed as a nuisance noise source or as interesting physics. For example, mag noise in a field sensor may set the minimum detectable field of that sensor. On the other hand, the field noise spectrum reflects the dynamics of the magnetic components, which are essential for device operation. Here, we model the field noise spectrum near the surface of a magnetic film due to thermal spin waves, and we calculate its effect on the T1 relaxation rate of a nearby nitrogen-vacancy (NV) center spin. The model incorporates four components: the spin wave dispersion of the magnetization in a finite-thickness film, thermal excitation of spin waves, the coupling geometry between waves in the film and an external point dipole and finally, the relaxation dynamics of the NV spin. At a distance of 100 nm above a 50 nm thick permalloy film, we find that the strongest stray fields are along the film normal and parallel to the magnetization, on the order of 1 mA m-1 Hz- 1 / 2 or 1 nT Hz- 1 / 2, yielding relaxation times on the order of 10 μs. The spin wave field noise can dominate the intrinsic relaxation, (T1 1 ms) of the NV center spin.

  10. Strain engineered magnetic tunnel junctions and spin-orbit torque switching (Conference Presentation)

    Science.gov (United States)

    Wu, Yang; Narayanapillai, Kulothungasagaran; Elyasi, Mehrdad; Qiu, Xuepeng; Yang, Hyunsoo

    2016-10-01

    The efficient generation of pure spin currents and manipulation of the magnetization dynamics of magnetic structures is of central importance in the field of spintronics. The spin-orbit effect is one of the promising ways to generate spin currents, in which a charge current can be converted to a transverse spin current due to the spin-orbit interaction. We investigate the spin dynamics in the presence of strong spin-orbit coupling materials such as LaAlO3/SrTiO3 oxide heterostructures. Angle dependent magnetoresistance measurements are employed to detect and understand the current-induced spin-orbit torques, and an effective field of 2.35 T is observed for a dc-current of 200 uA. In order to understand the interaction between light and spin currents, we use a femtosecond laser to excite an ultrafast transient spin current and subsequent terahertz (THz) emission in nonmagnet (NM)/ferromagnet (FM)/oxide heterostructures. The THz emission strongly relies on spin-orbit interaction, and is tailored by the magnitude and sign of the effective spin Hall angle of the NM. Our results can be utilized for ultrafast spintronic devices and tunable THz sources.

  11. Room-temperature ferromagnetic properties of Cu-doped ZnO rod ...

    Indian Academy of Sciences (India)

    The rod arrays have exhibited room-temperature ferromagnetic behaviour with the remanence of 0.926 × 10-3 emu/cm3. We suggest that the exchange interaction between local spin-polarized electrons (such as the electrons of Cu2+ ions) and conductive electrons is the cause of room-temperature ferromagnetism.

  12. Emergent spin-1 trimerized valence bond crystal in the spin-1/2 Heisenberg model on the star lattice

    Science.gov (United States)

    Ran, Shi-Ju; Li, Wei; Gong, Shou-Shu; Weichselbaum, Andreas; von Delft, Jan; Su, Gang

    2018-02-01

    We explore the frustrated spin-1/2 Heisenberg model on the star lattice with antiferromagnetic (AF) couplings inside each triangle and ferromagnetic (FM) intertriangle couplings (Jefrustration from the AF interactions inside each triangle, but trigger a fully gapped inversion-symmetry-breaking trimerized valence bond crystal (TVBC) with emergent spin-1 degrees of freedom. We discover that with strengthening Je, the system exhibits a universal scaling behavior either with or without a magnetic field h : the order parameter, the five critical fields that separate the Je-h ground-state phase diagram into six phases, and the excitation gap obtained by low-temperature specific heat, all depend exponentially on Je. Our work implies that the spin-1 VBCs can be stabilized by introducing small FM couplings in the geometrically frustrated spin-1/2 systems.

  13. Ferromagnetic states of p-type silicon doped with Mn

    International Nuclear Information System (INIS)

    Yunusov, Z. A.; Yuldashev, Sh. U.; Igamberdiev, Kh. T.; Kwon, Y. H.; Kang, T. W.; Bakhadyrkhanov, M. K.; Isamov, S. B.; Zikrillaev, N. F.

    2014-01-01

    In this work, the ferromagnetic states of Mn-doped p-type silicon samples were investigated. Two different types of ferromagnetic states have been observed in Si (Mn, B). The samples with a relatively high concentration of Mn revealed a ferromagnetic state with a Curie temperature above room temperature, and that ferromagnetism was due to the Mn x B y ferromagnetic clusters. The samples with a moderate concentration of Mn at low temperatures revealed a ferromagnetic state that was mediated by carriers (holes). The samples demonstrated the anomalous Hall effect at temperatures below 100 K and had a negative magneto-resistivity peak at a temperature close to the Curie temperature. The thermal diffusivity measurements demonstrated the existence of a second-order phase transition in the samples with a moderate Mn concentration. The specific heat's critical exponent α = 0.5, determined from the thermal diffusivity measurements, confirmed the long-range nature of the magnetic exchange interaction in these samples.

  14. Controlling entangled spin-orbit coupling of 5 d states with interfacial heterostructure engineering

    Science.gov (United States)

    Kim, J.-W.; Choi, Y.; Chun, S. H.; Haskel, D.; Yi, D.; Ramesh, R.; Liu, J.; Ryan, P. J.

    2018-03-01

    The combination of strong electron correlations in 3 d transition-metal oxides and spin-orbit interactions in the 5 d counterpart can give rise to exotic electronic and magnetic properties. Here, the nature of emerging phenomena at the interface between SrIr O3 (SIO) and L a2 /3S r1 /3Mn O3 (LSMO) is presented. Nominally, SIO with strong spin-orbit interaction is metallic and nonmagnetic on the verge of a metal-insulator transition, whereas LSMO is metallic and ferromagnetic with itinerant character and high spin polarization. In the 1:1 LSMO/SIO superlattice, we observe ferromagnetic Mn moments with an insulating behavior, accompanied by antiferromagnetic ordering in SIO. Element-resolved x-ray magnetic circular dichroism proves that there is a weak net ferromagnetic Ir moment aligned antiparallel to the Mn counterpart. The branching ratio shows the formation of molecular orbitals between the Mn and Ir layers modifying the Ir 5 d electronic configuration through the mixture of t2 g and eg states, resulting in a deviation from Jeff=1 /2 . This result demonstrates a pathway to manipulate the spin-orbit entanglement in 5 d states with two-dimensional 3 d spin-polarized electrons through heterostructure design.

  15. Single- and double-island ferromagnetic single-electron transistors

    International Nuclear Information System (INIS)

    Barnas, J.; Weymann, I.; Wisniewska, J.; Kowalik, M.; Kunert, H.W.

    2006-01-01

    Electronic transport in a ferromagnetic single-electron transistor has been considered theoretically in the sequential tunneling regime. The device consists of two external leads and one or two islands as the central part, connected to the leads by tunneling barriers. External gates are additionally attached to the islands. Generally, the two external electrodes and the islands can be ferromagnetic with arbitrary orientation of the corresponding magnetic moments. We have carried out detailed theoretical analysis of the current-voltage characteristics and spin-valve magnetoresistance in the limit of fast spin relaxation on the islands. Asymmetry in tunneling probabilities of spin-majority and spin-minority electrons leads to interesting features in the transport characteristics, like for instance magnetoresistance oscillations with the bias and gate voltages, negative differential resistance, and others

  16. Spin-dependent transport properties of a GaMnAs-based vertical spin metal-oxide-semiconductor field-effect transistor structure

    International Nuclear Information System (INIS)

    Kanaki, Toshiki; Asahara, Hirokatsu; Ohya, Shinobu; Tanaka, Masaaki

    2015-01-01

    We fabricate a vertical spin metal-oxide-semiconductor field-effect transistor (spin-MOSFET) structure, which is composed of an epitaxial single-crystal heterostructure with a ferromagnetic-semiconductor GaMnAs source/drain, and investigate its spin-dependent transport properties. We modulate the drain-source current I DS by ∼±0.5% with a gate-source voltage of ±10.8 V and also modulate I DS by up to 60% with changing the magnetization configuration of the GaMnAs source/drain at 3.5 K. The magnetoresistance ratio is more than two orders of magnitude higher than that obtained in the previous studies on spin MOSFETs. Our result shows that a vertical structure is one of the hopeful candidates for spin MOSFET when the device size is reduced to a sub-micron or nanometer scale

  17. Magnons, Spin Current and Spin Seebeck Effect

    Science.gov (United States)

    Maekawa, Sadamichi

    2012-02-01

    When metals and semiconductors are placed in a temperature gradient, the electric voltage is generated. This mechanism to convert heat into electricity, the so-called Seebeck effect, has attracted much attention recently as the mechanism for utilizing wasted heat energy. [1]. Ferromagnetic insulators are good conductors of spin current, i.e., the flow of electron spins [2]. When they are placed in a temperature gradient, generated are magnons, spin current and the spin voltage [3], i.e., spin accumulation. Once the spin voltage is converted into the electric voltage by inverse spin Hall effect in attached metal films such as Pt, the electric voltage is obtained from heat energy [4-5]. This is called the spin Seebeck effect. Here, we present the linear-response theory of spin Seebeck effect based on the fluctuation-dissipation theorem [6-8] and discuss a variety of the devices. [4pt] [1] S. Maekawa et al, Physics of Transition Metal Oxides (Springer, 2004). [0pt] [2] S. Maekawa: Nature Materials 8, 777 (2009). [0pt] [3] Concept in Spin Electronics, eds. S. Maekawa (Oxford University Press, 2006). [0pt] [4] K. Uchida et al., Nature 455, 778 (2008). [0pt] [5] K. Uchida et al., Nature Materials 9, 894 (2010) [0pt] [6] H. Adachi et al., APL 97, 252506 (2010) and Phys. Rev. B 83, 094410 (2011). [0pt] [7] J. Ohe et al., Phys. Rev. B (2011) [0pt] [8] K. Uchida et al., Appl. Phys. Lett. 97, 104419 (2010).

  18. Carrier Dynamics in Narrow Gap Ferromagnetic Semiconductors

    Science.gov (United States)

    Saha, D.; Pan, X.; Sanders, G. D.; Stanton, C. J.; Bhowmick, M.; Merritt, T.; Khodaparast, G. A.; Feeser, C.; Wessels, B. W.; McGill, S.

    2012-02-01

    Narrow gap ferromagnetic semiconductors are promising materials for spin photonic and spin transport devices because of their small effective masses, small energy gap, and high carrier mobility. We use time resolved differential transmission (TRDT) experiments to study carrier dynamics in ferromagnetic InMnAs and InMnSb. Electronic structure for InMnAs and InMnSb is calculated using an 8-band Pidgeon-Brown model generalized to include the effects of an external magnetic field. Our model includes the effects of the ferromagnetic Mn ions and their coupling to electrons and holes with or without an external magnetic field. Optical transitions are calculated from Fermi's Golden rule and interband transitions at a given pump or probe laser energy are identified. This allows us to understand a sign change seen in the TRDT. Our results show that 1) Phase-Space Filling, 2) Band Gap Renormalization and 3) Free Carrier Absorption all contribute to the TRDT and that the relative importance of these effects depends on the laser probe energy.

  19. Itinerant Ferromagnetism in Ultracold Fermi Gases

    DEFF Research Database (Denmark)

    Heiselberg, Henning

    2012-01-01

    Itinerant ferromagnetism in cold Fermi gases with repulsive interactions is studied applying the Jastrow-Slater approximation generalized to finite polarization and temperature. For two components at zero temperature a second order transition is found at akF ≃ 0.90 compatible with QMC. Thermodyna......Itinerant ferromagnetism in cold Fermi gases with repulsive interactions is studied applying the Jastrow-Slater approximation generalized to finite polarization and temperature. For two components at zero temperature a second order transition is found at akF ≃ 0.90 compatible with QMC...

  20. Transport and pairing properties of helical edges with proximity induced superconductivity and ferromagnetism

    Energy Technology Data Exchange (ETDEWEB)

    Keidel, Felix; Burset, Pablo; Trauzettel, Bjoern [Institute of Theoretical Physics and Astrophysics, University of Wuerzburg, 97074 Wuerzburg (Germany); Crepin, Francois [Laboratoire de Physique Theorique de la Matiere Condensee, UPMC, Sorbonne Universites, 75252 Paris (France)

    2016-07-01

    The scientific interest in Quantum Spin Hall systems is far from declining. While these certainly are fascinating by themselves, there is plenty of new and exciting physics to arise when superconductivity and ferromagnetism are brought into the game. The strong constraint of helicity in the edge states of a two-dimensional topological insulator is responsible for an intimate relation between the allowed scattering processes in a hybrid junction and the parameters of the system, namely the superconducting order parameter and the magnetic field. In our work, we study a helical liquid in proximity to a conventional s-wave superconductor and ferromagnetic insulators by means of a Green's function analysis. The ferromagnet gives rise to sub-gap Andreev/Majorana bound states and non-local crossed Andreev reflection (CAR), both of which decisively affect the pairing and transport properties of the junction. As a result, the simple s-wave symmetry of the superconductor is enriched and unconventional odd-frequency triplet superconductivity emerges. Strikingly, we have identified a setup that favors CAR over electron co-tunneling and may allow for the indirect measurement of the symmetries of the superconducting order parameter.