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Sample records for emitting natural radionuclide

  1. Natural gamma-emitting radionuclides in egyptian cement

    International Nuclear Information System (INIS)

    El Arabi, A.M.; Abbady, A.; El Kamel, A.H.; Nosier, A.; Moustafa, A.

    2005-01-01

    Samples of cement manufactured in Egypt and the various raw materials, which compose the product, have been analyzed using gamma-spectroscopy, in order to determine the concentration of natural radionuclides and associated radiological hazard. The mean of specific activity due to all the three radionuclides (226 R a, 232 T h and 40 K ) were found to be 20±4 , 11± 2, 320 ± 18 (gypsum), 41 ±8, 27± 5, 410± 27 (clay), 58 ± 11, 18 3, 321± 20 (Iron ore) and 37.6 ± 6, 11.8 ± 3, 178.6 ± 15 Bq.kg-1 (Portland cement), respectively. 40 K concentration could not be detected in Slag; limestone; Sulphate resistant cement; Clinker and White cement, while the mean activity concentrations of 226 R a and 232 T h are 239 ± 16, 48.7 ± 7; 31.5 ±5, 10 ± 2; 47 ± 7, 20 ± 4; 23 ± 5, 10.4 ± 3 and 23 ± 5, 11 ±3 Bq.kg-1, respectively. The measured activity concentrations of these natural radionuclides were compared with data of some countries. The present values are in the same range and sometimes less than those in other countries

  2. Natural gamma-emitting radionuclides in egyptian cement

    International Nuclear Information System (INIS)

    El-Arabi, A.M.; Abbady, A.; El-Kamel, A.H.; Nosier, A.; Moustafa, A.

    2005-01-01

    Samples of cement manufactured in Egypt and the various raw materials, which compose the product, have been analyzed using gamma-spectroscopy, in order to determine the concentration of natural radionuclides and associated radiological hazard. The mean of specific activity due to all the three radionuclides (226 R a, 232 T h and 40 K ) were found to be 20 ± 4 , 11 ± 2, 320 ± 18 (gypsum), 41 ± 8, 27 ± 5, 410 ± 27 (clay), 58 ± 11, 18 3, 321 ± 20 (Iron ore) and 37.6 ± 6, 11.8 ± 3, 178.6 ± 15 Bq.kg-1 (Portland cement), respectively. 40 K concentration could not be detected in Slag; limestone; Sulphate resistant cement; Clinker and White cement, while the mean activity concentrations of 226 R a and 232 T h are 239 ± 16, 48.7 ± 7; 31.5 ± 5, 10 ± 2; 47 3 ± 7, 20 ± 4; 23 ± 5, 10.4 ± 3 and 23 ± 5, 11 ± 3 Bq.kg-1, respectively. The measured activity concentrations of these natural radionuclides were compared with data of some countries. The present values are in the same range and sometimes less than those in other countries

  3. External exposure doses due to gamma emitting natural radionuclides in some Egyptian building materials.

    Science.gov (United States)

    Moharram, B M; Suliman, M N; Zahran, N F; Shennawy, S E; El Sayed, A R

    2012-01-01

    Using of building materials containing naturally occurring radionuclides as (238)U, (232)Th and (40)K and their progeny results in an external exposures of the housing of such buildings. In the present study, indoor dose rates for typical Egyptian rooms are calculated using the analytical method and activity concentrations of natural radionuclides in some building materials. Uniform chemical composition of the walls, floor and ceiling as well as uniform mass concentrations of the radionuclides in walls, floor and ceiling assumed. Different room models are assumed to discuss variation of indoor dose rates according to variation in room construction. Activity concentrations of (238)U, (232)Th and (40)K content in eight samples representative Clay soil and different building materials used in most recent Egyptian building were measured using Inductively Coupled Plasma-Mass Spectrometry (ICP-MS). The specific activity for (238)U, (232)Th and (40)K, from the selected samples, were in the range 14.15-60.64, 2.75-84.66 and 7.35-554.4Bqkg(-1), respectively. The average indoor absorbed dose rates in air ranged from 0.005μGyh(-1) to 0.071μGyh(-1) and the corresponding population-weighted annual effective dose due to external gamma radiation varies from 0.025 to 0.345mSv. An outdoor dose rate for typical building samples in addition to some radiological hazards has been introduced for comparison. Copyright © 2011 Elsevier Ltd. All rights reserved.

  4. Alpha Emitting Radionuclides and Radiopharmaceuticals for Therapy

    International Nuclear Information System (INIS)

    Chérel, Michel; Barbet, Jacques

    2013-01-01

    Today, cancer treatments mainly rely on surgery or external beam radiation to remove or destroy bulky tumors. Chemotherapy is given when tumours cannot be removed or when dissemination is suspected. However, these approaches cannot permanently treat all cancers and relapse occurs in up to 50% of the patients’ population. Radioimmunotherapy (RIT) and peptide receptor radionuclide therapy (PRRT) are effective against some disseminated and metastatic diseases, although they are rarely curative. Most preclinical and clinical developments in this field have involved electron-emitting radionuclides, particularly iodine-131, yttrium-90 and lutetium-177. The large range of the electrons emitted by these radionuclides reduces their efficacy against very small tumour cell clusters or isolated tumour cells present in residual disease and in many haematological tumours (leukaemia, myeloma). The range of alpha particles in biological tissues is very short, less than 0.1 mm, which makes alpha emitters theoretically ideal for treatment of such isolated tumour cells or micro-clusters of malignant cells. Thus, over the last decade, a growing interest for the use of alpha-emitting radionuclides has emerged. Research on targeted alpha therapy (TAT) began years ago in Nantes through cooperation between Subatech, a nuclear physics laboratory, CRCNA, a cancer research centre with a nuclear oncology team and ITU (Karlsruhe, Germany). CD138 was demonstrated as a potential target antigen for Multiple Myeloma, which is a target of huge clinical interest particularly suited for TAT because of the disseminated nature of the disease consisting primarily of isolated cells and small clusters of tumour cells mainly localized in the bone marrow. Thus anti-CD138 antibodies were labelled with bismuth-213 from actinium-225/bismuth-213 generators provided by ITU and used to target multiple myeloma cells. In vitro studies showed cell cycle arrest, synergism with chemotherapy and very little induction

  5. Doses of external exposure in Jordan house due to gamma-emitting natural radionuclides in building materials.

    Science.gov (United States)

    Al-Jundi, J; Ulanovsky, A; Pröhl, G

    2009-10-01

    The use of building materials containing naturally occurring radionuclides as (40)K, (232)Th, and (238)U and their progeny results in external exposures of the residents of such buildings. In the present study, indoor dose rates for a typical Jordan concrete room are calculated using Monte Carlo method. Uniform chemical composition of the walls, floor and ceiling as well as uniform mass concentrations of the radionuclides in walls, floor and ceiling are assumed. Using activity concentrations of natural radionuclides typical for the Jordan houses and assuming them to be in secular equilibrium with their progeny, the maximum annual effective doses are estimated to be 0.16, 0.12 and 0.22 mSv a(-1) for (40)K, (232)Th- and (238)U-series, respectively. In a total, the maximum annual effective indoor dose due to external gamma-radiation is 0.50 mSv a(-1). Additionally, organ dose coefficients are calculated for all organs considered in ICRP Publication 74. Breast, skin and eye lenses have the maximum equivalent dose rate values due to indoor exposures caused by the natural radionuclides, while equivalent dose rates for uterus, colon (LLI) and small intestine are found to be the smallest. More specifically, organ dose rates (nSv a(-1)per Bq kg(-1)) vary from 0.044 to 0.060 for (40)K, from 0.44 to 0.60 for radionuclides from (238)U-series and from 0.60 to 0.81 for radionuclides from (232)Th-series. The obtained organ and effective dose conversion coefficients can be conveniently used in practical dose assessment tasks for the rooms of similar geometry and varying activity concentrations and local-specific occupancy factors.

  6. Positron emitting radionuclides for South Africa

    International Nuclear Information System (INIS)

    Wynchbank, S.; Van der Walt, T.N.; Sharpey-Shafer, J.

    2004-01-01

    Full text: In South Africa there are currently two projects underway to supply and utilise positron emitting radionuclides for imaging in clinical nuclear medicine facilities. The advantages and applications of such radio nuclides are numerous and well known. However the premier initial application will be to employ 1BF, at first in the compound fluorine-18 fluorodeoxyglucose ( 18 F)-FDG, for patients with cancers and neoplasms. The two projects are sited at iThemba LABS, where production of a generator supplying 66 Ga and the provision of ( 18 F]-FDG, are in an advanced state of planning; the former already fully financed by the Innovation Fund of the National Research Foundation. The two positron emitting radionuclides, 18 F and 68 Ge, will be produced using a cyclotron induced reaction on 1802 and Ga, respectively, at iThemba LABS. The 68 Ge/ 68 Ga generator consists of an anion exchanger loaded with 68 Ge, which decays to 68 Ga. The resulting radiopharmaceuticals, ( 18 F]-FDG and 68 Ga citrate, will be produced by the Radionuclide Production Group of iThemba LABS, using well described methods. However the structures and processes to be used in the generator to provide 68 Ga are novel and will be explained. Initially provision of the CBF]-FDG will be to selected clinical medicine facilities in the Western Cape and Gauteng. It should be noted that the logistical problems of providing this radiopharmaceutical (which are much complicated by its short half life of 109.7 min) to Gauteng, were shown to be surmountable in the 1970s, by a regular delivery of 18 F between Gauteng and Cape Town, after the advent of a commercial service using jet aircraft. The obvious requirement that there should be appropriate nuclear medicine facilities to image patients, at the sites to which the positron emitting radiopharmaceuticals will be supplied, has been addressed. Proposed solutions will be outlined, in terms of a dedicated positron emission tomography (PET) camera and a gamma

  7. Concentration levels of alpha emitting radionuclides in natural waters. Implications in the use of various radionuclides of reference for the determination of total alpha activity index

    International Nuclear Information System (INIS)

    Corbacho, J. A.; Baeza, A.; Guillen, J.; Valles, I.; Serrano, I.; Camacho, A.; Montana, M.

    2013-01-01

    The present study was carried out a statistical evaluation of the natural radioactive contents of a large number of water samples collected at different points of the Spanish geography, in order to meet its controlling radioactive composition and assessing the implications of total alpha activity index can have in this type of samples. (Author)

  8. The sources and fate of radionuclides emitted to the atmosphere

    International Nuclear Information System (INIS)

    Sandalls, J.

    2001-01-01

    The thesis represents an account of the sources and fate of radionuclides entering the atmosphere, and indicates where the candidate, through his own work, has contributed to the overall picture. The sources of the natural and man-made radionuclides found in the atmosphere are identified. New data on emissions from UK coal-fired power stations and UK steel works are reported. Radionuclides produced in nuclear fission and released to the atmosphere in the detonation of nuclear weapons, in nuclear accidents, and through routine discharges from nuclear sites have added to the atmospheric burden of radioactive materials; both acute and chronic low-level emissions are discussed. The various natural processes which remove radionuclides from the atmosphere are described. Soon after release, many radioactive materials become attached to the atmospheric aerosol, but others undergo gas-phase reactions. Some gases are sufficiently long-lived in the troposphere as to find their way into the stratosphere where their fate may be determined by the short-wave radiation from the sun. The nature of the particles of fuel emitted to the atmosphere in the explosion and fire at the Chernobyl nuclear power plant in 1986 are discussed, together with the associated environmental problems. The ground is the major sink for radionuclides leaving the atmosphere, and the behaviour of the more radiologically important radionuclides following deposition is described with special reference to: (i) fallout in both the urban and living environments; (ii) the pathways which may lead to contamination of the food chain; (iii) how the fuel particle fallout from Chernobyl was unique in nuclear accidents; (iv) soil-to-plant transfer of radioelements and (v) how radiation exposure of man can be mitigated in both the contaminated urban and rural environments. (author)

  9. The distribution and abundance of gamma emitting radionuclides in Lake Ontario sediments

    International Nuclear Information System (INIS)

    McKinley, R.S.

    1985-03-01

    The distribution of gamma emitting radionuclides in Lake Ontario sediments was investigated. Samples were collected using a systematic design in the vicinity of Pickering and Darlington, and supplemented by lakewide offshore samples. Naturally occurring 40 K was the predominant source of gamma activity. 60 Co was the only potentially CANDU released radionuclide which showed a distributional association with the Pickering 'A' NGS discharge

  10. Natural activity in Hudson River estuary samples and their influence on the detection limits for gamma emitting radionuclides using NaI gamma spectrometry

    International Nuclear Information System (INIS)

    Wrenn, M.E.; Jinks, S.M.; Hairr, L.M.; Paschoa, A.S.; Lentsch, J.W.

    1972-01-01

    Sources of natural radioactivity in Hudson River Estuary are described. The technique of analysis for gamma spectrometry of environmental samples is presented and its pros and cons discussed. The distribution of natural radioactivity in water, biota and sediment was reported as well as the role played by the vertical distribution of cesium-137 in sediments as an indicator of the rate of sedimentation. The effect of the presence of natural radionuclides on the detection limits of man-made nuclides in the Hudson River environment is thoroughly examined. The results obtained with a 4-in. sodium iodide well crystal housed in a low background mercury shielding compare favorably with a more sophisticated Ge(Li) system which uses anticoincidence, as far as the analysis of environmental samples is concerned. (U.S.)

  11. Natural radionuclides in groundwaters

    International Nuclear Information System (INIS)

    Laul, J.C.

    1990-01-01

    The U-234 and Th-230 radionuclides are highly retarded by factors of 10 4 to 10 5 in basalt groundwater (Hanford) and briny groundwaters from Texas and geothermal brine from the Salton Sea Geothermal Field (SSGF). In basalt groundwaters (low ionic strength), Ra is highly sorbed, while in brines (high ionic strength), Ra is soluble. This is probably because the sorption sites are saturated with Na + and Cl - ions and RaCl 2 is soluble in brines. Pb-210 is soluble in SSGF brine, probably as a chloride complex. The U-234/Th-230 ratios in basalt groundwaters and brines from Texas and SSGF are nearly unity, indicating that U is in the +4 state, suggesting a reducing environment for these aquifers. 19 refs., 3 figs

  12. Natural radionuclides in groundwaters

    International Nuclear Information System (INIS)

    Laul, J.C.

    1992-01-01

    The 234 U and 230 Th radionuclides are highly retarded by factors of 10 4 to 10 5 in basalt groundwater (Hanford) and briny groundwaters from Texas, and geothermal brine form the Salton Sea Geothermal Field (SSGF). In basalt groundwaters (low ionic strength), Ra is highly sorbed, while in brines (high ionic strength), Ra is soluble. This is probably because the sorption sites are saturated with Na + and Cl - ions, and RaCl 2 is soluble in brines. 210 Pb is soluble in SSGF brine, probably as a chloride complex. The 234 U/ 230 Th ratios in basalt groundwaters and brines from Texas and SSGF are nearly unity, indicating that U is in the +4 state, suggesting a reducing environment for these aquifers. (author) 19 refs.; 3 figs

  13. Naturally occurring radionuclides in food

    International Nuclear Information System (INIS)

    Djujic, I.

    1995-01-01

    The naturally occurring radionuclides are the major source of radiation exposure to humans. The principal way of natural radiation exposure is the inhalation of 222 Rn decay products (about 85% of the total). The remainder is equally divided between internally deposited radionuclides, cosmic and terrestrial sources. In the present study, the content of 40 K, 210 Pb, 226 Ra, 230 Th, 232 Th and 238 U in representative food samples (milk, pork, beef, potatoes, wheat and corn flour) and samples of different food items that do not represent entire national production but provide interesting additional data for approximative calculation of naturally occurring radionuclide intake is presented. Daily weight of food eaten, participation of food groups, as well as daily intake by food of mentioned naturally occurring radionuclides in the Serbian diet was obtained on the base of house hold budget surveys. The result obtained for daily intake estimates in mBq for Serbian population are 78.1 ( 40 K), 38.2( 210 Pb), 52.3( 226 Ra), 2.0( 230 Th) and 12.5( 238 U). (author)

  14. Toxicity of inhaled alpha-emitting radionuclides - Status report

    International Nuclear Information System (INIS)

    Muggenburg, B.A.; Mewhinney, J.A.; Guilmette, R.A.; Gillett, N.A.; Diel, J.H.; Lundgren, D.L.; Hahn, F.F.; Boecker, B.B.; McClellan, R.O.

    1988-01-01

    The toxicity of inhaled alpha-emitting radionuclides is being investigated in a series of interrelated dose-response studies. Dogs, rodents, and nonhuman primates have been exposed to monodisperse or polydisperse aerosols of the oxides of 239 Pu, 238 Pu, 241 Am, or 244 Cm to measure the relative importance of average organ dose, local dose around particles, specific activity, chemical form, particle size, and number of particles inhaled to the development of biological effects. The influence of animal species, age at exposure, and pre-existing lung disease, as well as the effects of repeated exposure, are also being studied, because they may influence the toxicity of these radionuclides. (author)

  15. Metabolism and biological effects of alpha-emitting radionuclides

    Energy Technology Data Exchange (ETDEWEB)

    Bair, W. J.

    1979-05-01

    The emphasis of much of the current and planned research on the toxicity of alpha-emitting radionuclides is directed toward the complexities of actual and potential conditions of occupational environmental exposures of human beings. These, as well as the more limited studies on mechanisms of biological transport and effects, should increase our ability to predict health risks more accurately and to deal more confidently with human exposures, if and when they occur.

  16. Toxicity studies of inhaled beta-emitting radionuclides - Status report

    Energy Technology Data Exchange (ETDEWEB)

    Hahn, F F; Boeker, B B; Gillett, N A; Griffith, W C; Lundgren, D L; McClellan, R O; Muggenburg, B A; Snipes, M B

    1988-12-01

    The effects of beta-emitting radionuclides inhaled in either a relatively soluble form ({sup 90}SrCl{sub 2}, {sup 144}CeCl{sub 3}, {sup 91}yl{sub 3}, or {sup 137}CsCl) or in a relatively insoluble form ({sup 90}Y, {sup 91}Y, {sup 144}Ce or {sup 90}Sr in fused aluminosilicate particles [FAP]) have been studied in laboratory animals. The results showed that the total beta dose and the dose-rate pattern can modify both the neoplastic and non-neoplastic effects of inhaled beta-emitting radionuclides. In addition, the solubility and chemical characteristics of the radionuclides influence which organs are affected. Effects are seen primarily in organs where the radionuclide is ultimately accumulated, e.g., lung, bone, liver, or tracheobronchial lymph nodes. In addition, effects may be seen in organs where there is little accumulation, but where the radiation dose may still be high, e.g., nasal epithelium and heart. Studies of inhaled {sup 144}Ce-FAP in four different species showed that, compared to mice and dogs, lung tumor risk factors are very low for Syrian hamsters and high for rats. Studies of mice, Syrian hamsters, rats, and dogs repeatedly exposed to aerosols of {sup 144}Ce-FAP showed that lung tumor incidence correlates better with cumulative dose to the lung than with dose rate. Most of the studies in this program are nearing completion and full analyses are in progress. (author)

  17. Activity concentrations and mean annual effective dose from gamma-emitting radionuclides in the Lebanese diet

    International Nuclear Information System (INIS)

    Nasreddine, L.; Hwalla, N.; El Samad, O.; Baydoun, R.; Hamze, M.; Parent-Massin, D.

    2008-01-01

    Since the primary factor contributing to the internal effective dose in the human organism is contaminated food, the control of radionuclides in food represents the most important means of protection. This study was conducted to determine the levels of the dietary exposure of the Lebanese population to gamma-emitting radioisotopes. The activity concentrations of gamma-emitting radioisotopes have been measured in food samples that represent the market basket of an adult urban population in Lebanon. The artificial radionuclide 137 Cs was measured above detection limits in only fish, meat and milk-based deserts. The most abundant natural radionuclide was 40 K (31-121 Bq kg -1 ), with the highest content in fish and meat samples. The annual mean effective dose contributed by 40 K in the reference typical diet was estimated equal to 186 μSv y -1 , a value reasonably consistent with findings reported by several other countries. (authors)

  18. Dietary intake of natural radionuclides

    Energy Technology Data Exchange (ETDEWEB)

    Smith-Briggs, J L; Bradley, E J [National Radiological Protection Board, Chilton (UK)

    1984-09-01

    The levels of the natural radionuclides, radium-226, lead-210 and polonium-210 were measured in food samples collected for a National Food Survey, thus reflecting current consumption patterns in the UK. Daily intakes of radium-226, lead-210 and inferred values of polonium-210 were calculated for 20 food groups. From these data, the annual effective dose equivalents from radium-226, lead-210 and polonium-210 in the UK diet were estimated to be 3..mu..Sv, 41..mu..Sv and 13..mu..Sv respectively.

  19. Dietary intake of natural radionuclides

    International Nuclear Information System (INIS)

    Smith-Briggs, J.L.; Bradley, E.J.

    1984-01-01

    The levels of the natural radionuclides, radium-226, lead-210 and polonium-210 were measured in food samples collected for a National Food Survey, thus reflecting current consumption patterns in the UK. Daily intakes of radium-226, lead-210 and inferred values of polonium-210 were calculated for 20 food groups. From these data, the annual effective dose equivalents from radium-226, lead-210 and polonium-210 in the UK diet were estimated to be 3μSv, 41μSv and 13μSv respectively. (U.K.)

  20. Lifetime health risks from internally deposited beta-emitting radionuclides

    International Nuclear Information System (INIS)

    Boecker, B.B.; Griffith, W.C.; Hahn, F.F.; Nikula, K.J.; Lundgren, D.L.; Muggenburg, B.A.

    1997-01-01

    Much of our knowledge on the lifetime health risks resulting from internal depositions of beta- and gamma-emitting radionuclides has come from studies in laboratory animals conducted to provide information not available from human epidemiological studies. This paper is focused primarily on results of experiments in which laboratory animals (dogs and rodents) were exposed once, briefly, by inhalation or intravenous injection to an individual fission-product radionuclide and were studied for radionuclide metabolism, dosimetry, and lifetime health effects. The relative importance of many dose- and effect-modifying factors was studied. The main long-term biological effects were cancers in the organs and tissues receiving the highest doses. Results for three different patterns of irradiation (skeleton, lung, and whole-body) are presented. The risks of bone cancers produced by 90 Sr are compared with those from 238 Pu in dogs. Lung cancer risks for several beta emitters inhaled in a relatively insoluble form by dogs are compared with results for 144 CeO 2 inhaled by rats. Late-occurring biological effects from the relatively uniform whole-body irradiation from intravenously injected 137 Cs are also presented. In addition to radionuclide-specific results, cross-cutting analyses of these studies provide valuable information on broader issues such as dose protraction, relative biological effectiveness, threshold considerations, and inter-species comparisons including extrapolation to human exposure situations. (authors)

  1. Illicit Trafficking of Natural Radionuclides

    International Nuclear Information System (INIS)

    Friedrich, Steinhaeusler; Lyudmila, Zaitseva

    2008-01-01

    Natural radionuclides have been subject to trafficking worldwide, involving natural uranium ore (U 238), processed uranium (yellow cake), low enriched uranium ( 20% U 235), radium (Ra 226), polonium (Po 210), and natural thorium ore (Th 232). An important prerequisite to successful illicit trafficking activities is access to a suitable logistical infrastructure enabling an undercover shipment of radioactive materials and, in case of trafficking natural uranium or thorium ore, capable of transporting large volumes of material. Covert en route diversion of an authorised uranium transport, together with covert diversion of uranium concentrate from an operating or closed uranium mines or mills, are subject of case studies. Such cases, involving Israel, Iran, Pakistan and Libya, have been analyzed in terms of international actors involved and methods deployed. Using international incident data contained in the Database on Nuclear Smuggling, Theft and Orphan Radiation Sources (DSTO) and international experience gained from the fight against drug trafficking, a generic Trafficking Pathway Model (TPM) is developed for trafficking of natural radionuclides. The TPM covers the complete trafficking cycle, ranging from material diversion, covert material transport, material concealment, and all associated operational procedures. The model subdivides the trafficking cycle into five phases: (1) Material diversion by insider(s) or initiation by outsider(s); (2) Covert transport; (3) Material brokerage; (4) Material sale; (5) Material delivery. An Action Plan is recommended, addressing the strengthening of the national infrastructure for material protection and accounting, development of higher standards of good governance, and needs for improving the control system deployed by customs, border guards and security forces

  2. Illicit Trafficking of Natural Radionuclides

    Science.gov (United States)

    Friedrich, Steinhäusler; Lyudmila, Zaitseva

    2008-08-01

    Natural radionuclides have been subject to trafficking worldwide, involving natural uranium ore (U 238), processed uranium (yellow cake), low enriched uranium (20% U 235), radium (Ra 226), polonium (Po 210), and natural thorium ore (Th 232). An important prerequisite to successful illicit trafficking activities is access to a suitable logistical infrastructure enabling an undercover shipment of radioactive materials and, in case of trafficking natural uranium or thorium ore, capable of transporting large volumes of material. Covert en route diversion of an authorised uranium transport, together with covert diversion of uranium concentrate from an operating or closed uranium mines or mills, are subject of case studies. Such cases, involving Israel, Iran, Pakistan and Libya, have been analyzed in terms of international actors involved and methods deployed. Using international incident data contained in the Database on Nuclear Smuggling, Theft and Orphan Radiation Sources (DSTO) and international experience gained from the fight against drug trafficking, a generic Trafficking Pathway Model (TPM) is developed for trafficking of natural radionuclides. The TPM covers the complete trafficking cycle, ranging from material diversion, covert material transport, material concealment, and all associated operational procedures. The model subdivides the trafficking cycle into five phases: (1) Material diversion by insider(s) or initiation by outsider(s); (2) Covert transport; (3) Material brokerage; (4) Material sale; (5) Material delivery. An Action Plan is recommended, addressing the strengthening of the national infrastructure for material protection and accounting, development of higher standards of good governance, and needs for improving the control system deployed by customs, border guards and security forces.

  3. Direct measurement of γ-emitting radionuclides in waste drum

    International Nuclear Information System (INIS)

    Ma Ruwei; Mao Yong; Zhang Xiuzhen; Xia Xiaobin; Guo Caiping; Han Yueqin

    1993-01-01

    The low-level rad waste produced from nuclear power plant, nuclear facilities, and in the process of their decommissioning is stored in waste depository. For the safety of transport and storage of these wastes, some test must be done. One of them is to analyse the kinds and activities of radionuclides in each waste drum. Segmented scanning gamma spectrum analysis can be used for direct measurement of gamma-emitting radionuclides in drum. Gamma emitters such as Co-60, Cs-137, Ra-226 can be measured directly from outside of drum. A method and system for direct measuring gamma emitters in waste drum are described, and measuring apparatus and measurement results as well

  4. Toxicity of inhaled alpha-emitting radionuclides - Status report

    Energy Technology Data Exchange (ETDEWEB)

    Muggenburg, B A; Mewhinney, J A; Guilmette, R A; Gillett, N A; Diel, J H; Lundgren, D L; Hahn, F F; Boecker, B B; McClellan, R O

    1988-12-01

    The toxicity of inhaled alpha-emitting radionuclides is being investigated in a series of interrelated dose-response studies. Dogs, rodents, and nonhuman primates have been exposed to monodisperse or polydisperse aerosols of the oxides of {sup 239}Pu, {sup 238}Pu, {sup 241}Am, or {sup 244}Cm to measure the relative importance of average organ dose, local dose around particles, specific activity, chemical form, particle size, and number of particles inhaled to the development of biological effects. The influence of animal species, age at exposure, and pre-existing lung disease, as well as the effects of repeated exposure, are also being studied, because they may influence the toxicity of these radionuclides. (author)

  5. Natural and anthropogenic radionuclides in the environment

    International Nuclear Information System (INIS)

    Hille, R.

    1984-01-01

    A survey is given on the actual knowledge about occurence and environmental relevancy of the most important radionuclides from natural and anthropogenic origin. The contribution of AGF installation is emphasized. (orig.) [de

  6. Determination of natural occurring radionuclides concentrations

    International Nuclear Information System (INIS)

    Stajic, J.; Markovic, V.; Krstic, D.; Nikezic, D.

    2011-01-01

    Tobacco smoke contains certain concentrations of naturally occurring radionuclides from radioactive chains of uranium and thorium - 214 Pb, 214 Bi, 228 Ac, 208 Tl, 226 Ra, 232 Th and 40 K. Inhaling of tobacco smoke leads to internal exposure of man. In order to estimate absorbed dose of irradiation it is necessary to determine concentrations of radionuclides present in the tobacco leaves. In this paper specific activities of naturally occurring radionuclides were measured in tobacco samples from cigarettes which are used in Serbia. [sr

  7. Gamma emitting radionuclides of the Test Reactor Area leaching ponds

    International Nuclear Information System (INIS)

    Millard, J.B.; Whicker, F.W.; Markham, O.D.

    1978-01-01

    Radioactive leaching ponds adjacent to the Test Reactor Area (TRA) located on the Idaho National Engineering Laboratory (INEL) Site were investigated to determine the seasonal distribution and ecological behavior of gamma emitting radionuclides. The potential hazards to man and the environment were considered through the biological export of radioactive materials from the ponds. Both biotic and abiotic pond compartments were sampled. Fall and winter biomass estimates showed that benthic periphyton comprised 52%, macrophytes and littoral vegetation 35%, and seston 10% of the total for all biotic compartments. Concentrations and concentration factors (CFs) for fall and winter are presented for Cr-51, Co-60, Zr-95, I-131, Cs-137, Ba-140, and Ce-141. Concentrations and CFs ranged over seven orders of magnitude for the various nuclides and compartments. Seston and zooplankton had the highest concentrations followed by periphyton, sediment, macrophytes, littoral plants, willow, and filtered water. Arthropods had variable concentrations and CFs. Significant seasonal differences were observed for concentrations and CFs in seston, macrophytes, and littoral vegetation. A compartmental inventory of total gamma emitting activity accounted for 254 Ci (9.25 TBq) of the 731 Ci (24.8 TBq) estimated to remain in the ponds at the time of sampling. Filtered water and surface sediments contained 99% of the total radioactivity, while periphyton and seston had most of the remaining 1%. An estimate of the avian export rate of radioactivity from the TRA ponds showed that potentially harvestable mourning doves had the lowest rate with 0.02 μCi/y. External tissues of migratory waterfowl were found to contribute 90% of the total exported activity for all birds. The total avian export rate was estimated to be 1350 μCi/y during 1975

  8. Calibration and operation of continuous air monitors for alpha-emitting radionuclides

    International Nuclear Information System (INIS)

    Hoover, M.D.; Newton, G.J.

    1993-01-01

    Spectrometer-based continuous air monitors have improved our capabilities for detecting aerosols of alpha-emitting radionuclides. This paper describes basic requirements and statistical limitations in the sensitivity of alpha continuous air monitors, and presents a technical basis for selecting the energy window for detection of uranium and plutonium aerosols, correcting for interference from airborne dust, selecting filters with low pressure drop and good front surface collection characteristics, and properly using electroplated calibration sources. Sensitivity limits are described for detecting uranium or plutonium aerosols in the presence of increased concentrations of naturally occurring, alpha-emitting radon progeny radionuclides. Decreasing the lower energy boundary of the detection window from 4.3 MeV to 2.7 MeV improves by a factor of three the detection of plutonium in the presence of dust, while causing minimal additional interference from ambient radon progeny. Selection of the Millipore Fluoropore teflon membrane filter reduces both pressure drop and interference from ambient radon progeny by up to a factor of two. Field collection of ambient radon progeny can be used to verify the proper energy of alpha emissions from electroplated calibration sources. In the absence of energy verification, errors in instrument calibration may result from solid state diffusion of the electroplated calibration radionuclide into the substrate plate

  9. Natural and Synthetic Barriers to Immobilize Radionuclides

    International Nuclear Information System (INIS)

    Um, W.

    2011-01-01

    The experiments of weathering of glass waste form and the reacted sediments with simulated glass leachates show that radionuclide sequestration can be significantly enhanced by promoting the formation of secondary precipitates. In addition, synthetic phosphate-bearing nanoporous material exhibits high stability at temperature and has a very high K d value for U(VI) removal. Both natural and synthetic barrier materials can be used as additional efficient adsorbents for retarding transport of radionuclides for various contaminated waste streams and waste forms present at U. S. Department of Energy clean-up sites and the proposed geologic radioactive waste disposal facility. In the radioactive waste repository facility, natural or synthetic materials are planned to be used as a barrier material to immobilize and retard radionuclide release. The getter material can be used to selectively scavenge the radionuclide of interest from a liquid waste stream and subsequently incorporate the loaded getters in a cementitious or various monolithic waste forms. Also, the getter material is to reduce the release of radionuclides from monolithic waste forms. Also, the getter material is to reduce the release of radionuclides from monolithic waste forms. Also, the getter material is to reduce the release of radionuclides form monolithic waste forms by being emplaced as a backfill barrier material around the wastes or waste form to minimize the potential around the wastes or waste form to minimize the potential hazard of leached radioactive wastes. The barrier material should be highly efficient to sequester radionuclides and possess physical and chemical stability for long-term exposure to severe weathering conditions. Because potential leaching of radionuclides depends on various environmental and weathering conditions of the near-field repository, the barrier materials must be durable and not disintegrate under a range of moisture, temperature, pressure, radiation, Eh, ph. and

  10. Method of measuring the disintegration rate of a beta-emitting radionuclide in a liquid sample

    International Nuclear Information System (INIS)

    Horrocks, D.L.

    1980-01-01

    A novel liquid scintillation counting method of measuring the disintegration rate of a beta-emitting radionuclide is described which involves counting the sample at at least two different quench levels. (UK)

  11. Radionuclides incorporation in activated natural nanotubes

    International Nuclear Information System (INIS)

    Silva, Jose Parra

    2016-01-01

    Natural palygorskite nanotubes show suitable physical and chemical properties and characteristics to be use as potential nanosorbent and immobilization matrix for the concentration and solidification of radionuclides present in nuclear wastes. In the development process of materials with sorption properties for the incorporation and subsequent immobilization of radionuclides, the most important steps are related with the generation of active sites simultaneously to the increase of the specific surface area and suitable heat treatment to producing the structural folding. This study evaluated the determining parameters and conditions for the activation process of the natural palygorskite nanotubes aiming at the sorption of radionuclides in the nanotubes structure and subsequent evaluation of the parameters involve in the structural folding by heat treatments. The optimized results about the maximum sorption capacity of nickel in activated natural nanotubes show that these structures are apt and suitable for incorporation of radionuclides similar to nickel. By this study is verified that the optimization of the acid activation process is fundamental to improve the sorption capacities for specifics radionuclides by activated natural nanotubes. Acid activation condition optimized maintaining structural integrity was able to remove around 33.3 wt.% of magnesium cations, equivalent to 6.30·10 -4 g·mol -1 , increasing in 42.8% the specific surface area and incorporating the same molar concentration of nickel present in the liquid radioactive waste at 80 min. (author)

  12. Natural radionuclides concentration in underground mine materials

    Energy Technology Data Exchange (ETDEWEB)

    Santos, T.O.; Rocha, Z.; Taveira, N.F.; Takahashi, L.C.; Pineiro, M.M., E-mail: talitaolsantos@yahoo.com.br, E-mail: rochaz@cdtn.br, E-mail: mayarapinheiroduarte@gmail.com, E-mail: lauratakahashi@hotmail.com, E-mail: natyfontaveira@hotmail.com [Centro de Desenvolvimento da Tecnologia Nuclear (CDTN/CNEN-MG), Belo Horizonte, MG (Brazil); Borges, P.F.; Cruz, P.; Gouvea, V.A.; Siqueira, J.B., E-mail: vgouvea@cnen.gov.br, E-mail: flavia.borges@cnen.gov.br, E-mail: pcruz@cnen.gov.br, E-mail: jbsiquei@cnen.gov.br [Comissão Nacional de Energia Nuclear (CNEN), Rio de Janeiro, RJ (Brazil)

    2017-07-01

    Natural Radionuclides are present in earth's environment since its origin. The main radionuclides present are {sup 40}K, as well as, {sup 238}U and {sup 232}Th with their decay products. These radionuclides occur in minerals in different activity concentration associated with geological and geochemical conditions, appearing at different levels from point to point in the world. Underground mines may present a high natural background radiation which is due to the presence of these radiogenic heavy minerals. To address this concern, this work outlines on the characterization of the natural radionuclides presence in underground mines in Brazil which are located in many cases on higher radiation levels bed rocks. The radon concentration was measured by using E-PERM Electrets Ion Chamber, AlphaGUARD and CR-39 track etch detectors. The radon progeny was determined by using DOSEman detector. Radon concentration measurement in groundwater was performed by using RAD7 detector. The {sup 238}U and {sup 232}Th activity concentration in ore and soil samples were determined by using Neutron Activation Analysis using TRIGA MARK I IPR-R1 Reactor. Gamma spectrometry was used to determine {sup 226}Ra, {sup 228}Ra and {sup 40}K activity concentrations. The results show that the natural radioactivity varies considerably from mine to mine and that there are not risks of radiological damage for exposed workers in these cases. Based on these data, recommendations for Brazilian regulatory standards are presented. (author)

  13. Natural radionuclides concentration in underground mine materials

    International Nuclear Information System (INIS)

    Santos, T.O.; Rocha, Z.; Taveira, N.F.; Takahashi, L.C.; Pineiro, M.M.; Borges, P.F.; Cruz, P.; Gouvea, V.A.; Siqueira, J.B.

    2017-01-01

    Natural Radionuclides are present in earth's environment since its origin. The main radionuclides present are 40 K, as well as, 238 U and 232 Th with their decay products. These radionuclides occur in minerals in different activity concentration associated with geological and geochemical conditions, appearing at different levels from point to point in the world. Underground mines may present a high natural background radiation which is due to the presence of these radiogenic heavy minerals. To address this concern, this work outlines on the characterization of the natural radionuclides presence in underground mines in Brazil which are located in many cases on higher radiation levels bed rocks. The radon concentration was measured by using E-PERM Electrets Ion Chamber, AlphaGUARD and CR-39 track etch detectors. The radon progeny was determined by using DOSEman detector. Radon concentration measurement in groundwater was performed by using RAD7 detector. The 238 U and 232 Th activity concentration in ore and soil samples were determined by using Neutron Activation Analysis using TRIGA MARK I IPR-R1 Reactor. Gamma spectrometry was used to determine 226 Ra, 228 Ra and 40 K activity concentrations. The results show that the natural radioactivity varies considerably from mine to mine and that there are not risks of radiological damage for exposed workers in these cases. Based on these data, recommendations for Brazilian regulatory standards are presented. (author)

  14. Dosimetry of beta emitting radionuclides for use in balloon angioplasty

    International Nuclear Information System (INIS)

    Fox, R.A.

    1997-01-01

    The dose at varying distances from the surface of an infinite cylinder containing 90 Y, 32 P and 188 Re respectively is calculated using published scaled point dose kernels for these three radionuclides. It is shown that all are suitable radionuclides for use in the irradiation of arteries subsequent to balloon angioplasty. All three may be used as a radioactive liquid in the angioplasty balloon, thereby simplifying the procedure and enabling a uniform radiation dose to be given to the arterial wall. It is however shown that there is a rapid reduction in dose with distance from the arterial wall which demands careful specification of the prescribed radiation dose. A similar rapid reduction with distance is also found with a central radioactive wire or with a radioactive stent containing the same radionuclides. (author)

  15. Comparison of bone tumors induced by beta-emitting or alpha-emitting radionuclides: Schemes of pathogenesis

    International Nuclear Information System (INIS)

    Gillett, N.A.; Muggenburg, B.A.; Pool, R.R.; Hahn, F.F.

    1988-01-01

    Life-span studies in Beagle dogs have documented the occurrence of bone tumors following exposure to bone-seeking alpha- or beta-emitting radionuclides administered by different routes of exposure. Bone tumors from dogs in four different life-span studies were analyzed according to tumor phenotype, tumor location, radiographic appearance, incidence of metastasis, and association with radiation osteodystrophy. Marked differences in these parameters were observed that did not correlate with differences in radionuclide type, route of exposure, or duration of radionuclide uptake. Radiation osteodystrophy, which is postulated to be a preneoplastic lesion, was not a significant component in one of the studies. Analysis of the data from these four studies suggests that at least two different mechanisms of bone tumor pathogenesis occur for radiation-induced bone tumors. (author)

  16. Natural analogues and radionuclide transport model validation

    International Nuclear Information System (INIS)

    Lever, D.A.

    1987-08-01

    In this paper, some possible roles for natural analogues are discussed from the point of view of those involved with the development of mathematical models for radionuclide transport and with the use of these models in repository safety assessments. The characteristic features of a safety assessment are outlined in order to address the questions of where natural analogues can be used to improve our understanding of the processes involved and where they can assist in validating the models that are used. Natural analogues have the potential to provide useful information about some critical processes, especially long-term chemical processes and migration rates. There is likely to be considerable uncertainty and ambiguity associated with the interpretation of natural analogues, and thus it is their general features which should be emphasized, and models with appropriate levels of sophistication should be used. Experience gained in modelling the Koongarra uranium deposit in northern Australia is drawn upon. (author)

  17. Traces of natural radionuclides in animal food

    Science.gov (United States)

    Merli, Isabella Desan; da Silveira, Marcilei A. Guazzelli; Medina, Nilberto H.

    2014-11-01

    Naturally occurring radioactive materials are present everywhere, e.g., in soil, air, housing materials, food, etc. Therefore, human beings and animals receive internal exposure from radioactive elements inside their bodies through breathing and alimentation. Gamma radiation has enough energy to remove an electron from the atom and compromise the rearrangement of electrons in the search for a more stable configuration which can disturb molecule chemical bonding. Food ingestion is one of the most common forms of radioisotopes absorption. The goal of this work is the measurement of natural gamma radiation rates from natural radioisotopes present in animal food. To determine the concentration of natural radionuclides present in animal food gamma-ray spectrometry was applied. We have prepared animal food samples for poultry, fish, dogs, cats and cattle. The two highest total ingestion effective doses observed refers to a sample of mineral salt cattle, 95.3(15) μSv/year, rabbit chow, with a value of 48(5) μSv/year, and cattle mineral salt, with a value of 69(7) μSv/year, while the annual total dose value from terrestrial intake radionuclide is of the order of 290 μSv/year.

  18. Traces of natural radionuclides in animal food

    International Nuclear Information System (INIS)

    Merli, Isabella Desan; Guazzelli da Silveira, Marcilei A.; Medina, Nilberto H.

    2014-01-01

    Naturally occurring radioactive materials are present everywhere, e.g., in soil, air, housing materials, food, etc. Therefore, human beings and animals receive internal exposure from radioactive elements inside their bodies through breathing and alimentation. Gamma radiation has enough energy to remove an electron from the atom and compromise the rearrangement of electrons in the search for a more stable configuration which can disturb molecule chemical bonding. Food ingestion is one of the most common forms of radioisotopes absorption. The goal of this work is the measurement of natural gamma radiation rates from natural radioisotopes present in animal food. To determine the concentration of natural radionuclides present in animal food gamma-ray spectrometry was applied. We have prepared animal food samples for poultry, fish, dogs, cats and cattle. The two highest total ingestion effective doses observed refers to a sample of mineral salt cattle, 95.3(15) μSv/year, rabbit chow, with a value of 48(5) μSv/year, and cattle mineral salt, with a value of 69(7) μSv/year, while the annual total dose value from terrestrial intake radionuclide is of the order of 290 μSv/year

  19. Traces of natural radionuclides in animal food

    Energy Technology Data Exchange (ETDEWEB)

    Merli, Isabella Desan; Guazzelli da Silveira, Marcilei A. [Centro Universitário da FEI, São Bernardo do Campo (Brazil); Medina, Nilberto H. [Instituto de Física da USP, São Paulo (Brazil)

    2014-11-11

    Naturally occurring radioactive materials are present everywhere, e.g., in soil, air, housing materials, food, etc. Therefore, human beings and animals receive internal exposure from radioactive elements inside their bodies through breathing and alimentation. Gamma radiation has enough energy to remove an electron from the atom and compromise the rearrangement of electrons in the search for a more stable configuration which can disturb molecule chemical bonding. Food ingestion is one of the most common forms of radioisotopes absorption. The goal of this work is the measurement of natural gamma radiation rates from natural radioisotopes present in animal food. To determine the concentration of natural radionuclides present in animal food gamma-ray spectrometry was applied. We have prepared animal food samples for poultry, fish, dogs, cats and cattle. The two highest total ingestion effective doses observed refers to a sample of mineral salt cattle, 95.3(15) μSv/year, rabbit chow, with a value of 48(5) μSv/year, and cattle mineral salt, with a value of 69(7) μSv/year, while the annual total dose value from terrestrial intake radionuclide is of the order of 290 μSv/year.

  20. ''Strong gammas''. List of strong gamma-rays emitted from radionuclides. Documentation of the PC diskette

    International Nuclear Information System (INIS)

    Ichimiya, T.; Narita, T.; Kitao, K.

    1994-01-01

    The PC diskette containing the ''List of strong gamma-rays emitted from radionuclides'' as published by T. Narita et al. in the report JAERI-M-94-059, March 1994, is described. The diskette is available from the IAEA Nuclear Data Section, costfree, upon request. (author)

  1. Environmental impact of natural radionuclides from the fossil fuel power plants

    International Nuclear Information System (INIS)

    Antic, D.

    1989-01-01

    A set of experimental data for selected coals in Yugoslavia is used for this study. The impact of natural radionuclides emitted from the coal fired power plants with these coals is analysed. Simple models are used to asses annual doses at the maximum concentration points. The calculated values are compared with the values from the literature for similar calculations (author)

  2. Natural radionuclides in the UK marine environment

    Energy Technology Data Exchange (ETDEWEB)

    Rollo, S F.N.; Camplin, W C; Allington, D J; Young, A K [Ministry of Agriculture, Fisheries and Food, Lowestoft (United Kingdom). Fisheries Radiobiological Lab.

    1992-01-01

    The importance of natural radionuclides giving rise to radiation exposure of man from marine consumption pathways has been known for some time. However, the extent of surveys of levels in marine biota has been limited. This paper presents new data on concentrations of natural radionuclides in fish, shellfish and seaweeds taken from coastal sampling locations in the U.K. Sampling included areas where levels due to natural sources would be predominant, but efforts were made to study potential sources of technologically enhanced discharges to seas and rivers, particularly the phosphogypsum plant at Whitehaven in Cumbria. The highest concentrations (up to 371 Bq.kg[sup -1] (wet) [sup 210]Po) were observed in winkles near Whitehaven. The general levels at sites remote from known sources were much lower. Monthly concentrations in molluscs at a single location were elevated by approximately a factor of 2 during the summer months. An assessment of the expected doses to members of the public from marine consumption pathways is made. (author).

  3. Reuse of Material Containing Natural Radionuclides - 12444

    Energy Technology Data Exchange (ETDEWEB)

    Metlyaev, E.G.; Novikova, N.J. [Burnasyan Federal Medical Biophysical Centre, Moscow (Russian Federation)

    2012-07-01

    Disposal of and use of wastes containing natural radioactive material (NORM) or technologically enhanced natural radioactive material (TENORM) with excessive natural background as a building material is very important in the supervision body activity. At the present time, the residents of Octyabrsky village are under resettlement. This village is located just near the Priargunsky mining and chemical combine (Ltd. 'PPGHO'), one of the oldest uranium mines in our country. The vacated wooden houses in the village are demolished and partly used as a building material. To address the issue of potential radiation hazard of the wooden beams originating from demolition of houses in Octyabrsky village, the contents of the natural radionuclides (K-40, Th-232, Ra-226, U- 238) are being determined in samples of the wooden beams of houses. The NORM contents in the wooden house samples are higher, on average, than their content in the reference sample of the fresh wood shavings, but the range of values is rather large. According to the classification of waste containing the natural radionuclides, its evaluation is based on the effective specific activity. At the effective specific activity lower 1.5 kBq/kg and gamma dose rate lower 70 μR/h, the material is not considered as waste and can be used in building by 1 - 3 classes depending upon A{sub eff} value. At 1.5 kBq/kg < A{sub eff} ≤ 4 kBq/kg (4 class), the wooden beams might be used for the purpose of the industrial building, if sum of ratios between the radionuclide specific activity and its specific activity of minimum significance is lower than unit. The material classified as the waste containing the natural radionuclides has A{sub eff} higher 1.5 kBq /kg, and its usage for the purpose of house-building and road construction is forbidden. As for the ash classification and its future usage, such usage is unreasonable, because, according to the provided material, more than 50% of ash samples are considered as

  4. Bioaccumulation of gamma emitting radionuclides in Polysiphonia fucoides

    International Nuclear Information System (INIS)

    Tamara Zalewska

    2014-01-01

    The article presents the results of a study on the bioaccumulation abilities of Polysiphonia fucoides, a red algae specific to the southern Baltic Sea, towards (of) gamma emitting isotopes. A laboratory experiment was carried out to determine changes in the activities of some isotopes - 54 Mn, 57 Co, 65 Zn, 110m Ag, 113 Sn, 134 Cs, 137 Cs and 241 Am - occurring in P. fucoides exposed to a seawater medium containing these isotopes over the course of 1 month. All analyzed isotopes showed the greatest increase of radioactive activity in plant tissue in the first 24 h of exposure. The temporary concentration factors of cesium isotopes were increasing linearly during the experiment from 114 to 274 in the case of 137 Cs, and from 144 to 351 in the case of 134 Cs. The level of the initial concentration factor of cesium isotopes in the plant proved to be independent of the initial concentration of the isotope in seawater and it took the lowest (125 dm 3 kg -1 ) level among the studied isotopes. In the case of a mixture of gamma emitting isotopes, a linear relation between the individual isotope activity in P. fucoides and its initial concentration in seawater was established after the first day of exposure; the isotopes initial concentration factors ranged from 767 to 874 dm 3 kg -1 . Having reached the maximal concentration level, a statistically significant decline in radioactivity concentrations of the five isotopes in the plant tissue was observed. A half-life of biological removal of the isotopes from the plant tissue was established at: 3.8 days in the case of 54 Mn, 4 days- 57 Co, 4 days- 60 Co, 4.2 days- 137 Cs and 241 Am-3.5 days. (author)

  5. Natural radio-nuclides in drinking water

    International Nuclear Information System (INIS)

    Deflorin, O.

    2003-01-01

    This article discusses the presence of radio-nuclides in Switzerland's drinking water. The article describes research done into the natural radioactivity to be found in various drinking water samples taken from the public water supply in the Canton of Grisons in eastern Switzerland. The various natural nuclides to be expected are listed and the methods used to take the samples are described. The results of the analysis are presented in the form of sketches showing the geographical distribution of the nuclide samples. Diagrams of the cumulative frequency of the quantities of nuclides found are presented, as are such diagrams for the yearly radioactive doses that the population is exposed to. The results and their consequences for the water supply are discussed in detail and further investigations to be made in the region are proposed

  6. Natural radionuclides as dirt tracers in sugar cane consignments

    International Nuclear Information System (INIS)

    Bacchi, M.A.; Fernandes, E.A.N.

    1998-01-01

    Soil is usually carried out to the mills, as an impurity in sugar cane, leading to economic drawbacks for the industry. The quantification of this dirt is important to identify its causes and for routine quality control. Several methods have been used for this purpose, however, no single one has been pointed out as an industrial standard. The use of a γ-ray emitting radionuclide of natural occurence was investigated and, after several soil and cane radioactivity analyses, 212 Pb was chosen as the best tracer. Calibration curves developed with the addition of soil in clean cane, from 0 to 10% (dry mass), demonstrated the linearity of the method. Analyses of eleven samples taken from consignments showed that the procedure was consistent and reliable when compared to the traditional ash method. (author)

  7. An improved in situ method for determining depth distributions of gamma-ray emitting radionuclides

    International Nuclear Information System (INIS)

    Benke, R.R.; Kearfott, K.J.

    2001-01-01

    In situ gamma-ray spectrometry determines the quantities of radionuclides in some medium with a portable detector. The main limitation of in situ gamma-ray spectrometry lies in determining the depth distribution of radionuclides. This limitation is addressed by developing an improved in situ method for determining the depth distributions of gamma-ray emitting radionuclides in large area sources. This paper implements a unique collimator design with conventional radiation detection equipment. Cylindrically symmetric collimators were fabricated to allow only those gamma-rays emitted from a selected range of polar angles (measured off the detector axis) to be detected. Positioned with its axis normal to surface of the media, each collimator enables the detection of gamma-rays emitted from a different range of polar angles and preferential depths. Previous in situ methods require a priori knowledge of the depth distribution shape. However, the absolute method presented in this paper determines the depth distribution as a histogram and does not rely on such assumptions. Other advantages over previous in situ methods are that this method only requires a single gamma-ray emission, provides more detailed depth information, and offers a superior ability for characterizing complex depth distributions. Collimated spectrometer measurements of buried area sources demonstrated the ability of the method to yield accurate depth information. Based on the results of actual measurements, this method increases the potential of in situ gamma-ray spectrometry as an independent characterization tool in situations with unknown radionuclide depth distributions

  8. Natural radionuclides in drinking water in Argentina

    International Nuclear Information System (INIS)

    Bomben, A.M.; Palacios, M.A.

    2000-01-01

    As part of the national survey to evaluate natural radioactivity in the environment, concentration levels of natural uranium and 226 Ra have been analyzed in over 300 drinking water samples taken from different locations in Argentina. 226 Ra was determined by 222 Rn emanation and liquid scintillation counting, and natural uranium by a fluorimetric procedure. Values ranging from 0.03 to 24 μg.l -1 of natural uranium and from 0.06 to 50 μg.l -1 , were measured on drinking water samples taken from tap water systems and private wells, respectively. Concentrations up to 15 mBq.l -1 and to 22 mBq.l -1 of 226 Ra were found in drinking water samples taken from tap water systems and private wells, respectively. These values are compared with the reference values accepted for drinking water. Based on the water intake rate, the age distribution and the measured concentrations, an annual collective effective dose of 1.9 man Sv and an individual committed effective dose of 0.49 μSv.y -1 were calculated for the city of Buenos Aires adult inhabitants, for the ingestion of both natural radionuclides analyzed in drinking water. (author)

  9. Dose assessment on natural radiation, natural radionuclide, and artificial radionuclide released by Fukushima nuclear accident

    International Nuclear Information System (INIS)

    Hosoda, Masahiro; Tokonami, Shinji; Furukawa, Masahide

    2012-01-01

    Various radionuclides are distributed in environmental materials such as soil, rock, and water. People are exposed every day to natural radiation. According to the UNSCEAR 2008 report, Sources of Ionizing Radiation, natural radiation sources are categorized as terrestrial gamma-rays, radon, cosmic rays and food. The effective dose from radon, thoron and its decay products is about 50% of all natural radiation exposure. Consciousness of the Japanese public toward radiation exposure has significantly increased since the start of the Fukushima Dai-ichi Nuclear Power Station accident. In this paper, the nationwide survey and dose estimation for terrestrial gamma-rays and radon are summarized. External dose from artificial radionuclides released by the Fukushima accident are also reported. (author)

  10. Natural systems prediction of radionuclide migration

    International Nuclear Information System (INIS)

    Ewing, R.C.

    1991-01-01

    This paper reviews the application (and limitations) of data from natural systems to the verification of performance assessments, particularly as they apply to the evaluation of the long-term performance of waste forms, backfill, canister materials, and finally, the integrity of the repository itself. Two specific examples, the corrosion of borosilicate glass and the formation of alteration products of spent fuel, will be discussed. In both cases, inferences are of three types: 1) directly applicable data (i.e. radiation effects, stable phase assemblages): 2) inferences based on the analogous behaviour of the natural and repository systems (e.g. long-term corrosion rate); 3) specific identification of new phenomena that could not have been anticipated from the short term laboratory data (i.e. new mechanisms for the retention or release of radionuclides). The latter can only be derived from the observation of natural systems. Finally, specific attention will be paid to the limitations in the use of natural systems, particularly as the spatial and temporal scales expand, and to the inherent limitations of prediction and verification. (J.P.N.)

  11. Natural radionuclides in Brazilian underground mines

    International Nuclear Information System (INIS)

    Santos, Talita de Oliveira

    2015-01-01

    Rock, soil and water contain "2"3"8U and "2"3"2Th and their decay products. The distribution of these radionuclides differs in terms of activity concentration depending on the mineral type and origin. All ore processing releases long and short half-life radionuclides, mainly radon and its progeny. It is important to monitor this gas and its decay products in underground mines in order to assess the radiological hazards of the exposed workers. On this concern, the present work outlines the characterization of brazilian underground mines with relation to natural radionuclides, specially radon and its progeny. The radon concentration was measured by using E-PERM Electrets Ion Chamber (Radelec), AlphaGUARD (Saphymo GmbH) and CR-39 (Landauer) track etch detectors. The radon progeny was determined by using DOSEman detector. The equilibrium state between radon and its progeny was calculated. Based on these data, the total effective dose for miners was estimated. Moreover, the contribution from the main sources to the radon level inside mines was evaluated. For this, the following detectors were used: measurements of radon concentrations in soil gas were carried out by using AlphaGUARD detector; "2"2"6Ra ("2"1"4Bi), "2"3"2Th e "4"0K specific activity in ore and soil samples were determined by using gamma-ray spectrometry HPGe detector (Canberra); and radon concentration in groundwater samples was performed by using RAD7 (Durridge Inc.). The radon concentration ranged from 113 to 8171 Bq.m"-"3 and the Equilibrium Equivalent Concentration varied from 76 to 1174 Bq.m"-"3. The equilibrium factor mean value was 0.4 (0.2 -0.7). The workers estimated total effective dose ranged from 1 to 22 mSv.a"-"1 (mean 10 mSv.a"-"1). Therefore, results show the importance to assess continually and permanently the radon and its progeny behavior and the need to adopt safety measurements against natural radiation in underground mines environment. (author)

  12. Migration of heavy natural radionuclides in a humid climatic zone

    International Nuclear Information System (INIS)

    Titaeva, N.A.; Alexakhin, R.M.; Taskaev, A.I.; Maslov, V.I.

    1980-01-01

    Regularities and biochemical peculiarities of the migrations of heavy natural radionuclides in the environment are examined, with special reference to two regions in a humid climatic zone representing natural patterns of radionuclide distribution and to four plots artificially contaminated with high levels of natural radioactivity more than 20 years previously. It was determined that the migration of thorium, uranium, and radium isotopes through the rock-water-soil-plant system is dependent on many physiochemical properties of these radionuclides, their compounds, and the local environment. Isotopic activity ratios provide a useful tool for studying the direction of radionuclide migration and its influence on observed distribution patterns

  13. Determination of γ-rays emitting radionuclides in surface water: application of a quantitative biosensing method

    International Nuclear Information System (INIS)

    Wolterbeek, H. Th.; Van der Meer, A. J. G. M.

    1995-01-01

    A quantitative biosensing method has been developed for the determination of γ-rays emitting radionuclides in surface water. The method is based on the concept that at equilibrium the specific radioactivity in the biosensor is equal to the specific radioactivity in water. The method consists of the measurement of both the radionuclide and the related stable isotope (element) in the biosensor and the determination of the element in water. This three-way analysis eliminates problems such as unpredictable biosensor behaviour, effects of water elemental composition or further abiotic parameters on accumulation levels: what remains is the generally high enrichment (bioaccumulation factor BCF) of elements and radionuclides in the biosensor material. Using water plants, the method is shown to be three to five orders of magnitude more sensitive than the direct analysis of water. (author)

  14. Determination of {gamma}-rays emitting radionuclides in surface water: application of a quantitative biosensing method

    Energy Technology Data Exchange (ETDEWEB)

    Wolterbeek, H Th; Van der Meer, A. J. G. M. [Delft University of Technology, Interfaculty Reactor Institute, Mekelweg 15, 2629 JB Delft (Netherlands)

    1995-12-01

    A quantitative biosensing method has been developed for the determination of {gamma}-rays emitting radionuclides in surface water. The method is based on the concept that at equilibrium the specific radioactivity in the biosensor is equal to the specific radioactivity in water. The method consists of the measurement of both the radionuclide and the related stable isotope (element) in the biosensor and the determination of the element in water. This three-way analysis eliminates problems such as unpredictable biosensor behaviour, effects of water elemental composition or further abiotic parameters on accumulation levels: what remains is the generally high enrichment (bioaccumulation factor BCF) of elements and radionuclides in the biosensor material. Using water plants, the method is shown to be three to five orders of magnitude more sensitive than the direct analysis of water. (author)

  15. Mechanisms of radionuclide transition in natural environment

    International Nuclear Information System (INIS)

    Pacyna, J.

    1974-01-01

    Mechanisms of radionuclide transition in various elements of the environment have been dealt with in an ecological aspect. The knowledge of the radionuclide propagation tracks will make possible to ascertain precisely causes and effects of the radiation and to reduce the contamination value. Particular attention has been paid to test methods. (author)

  16. Natural radionuclides in Austrian bottled mineral waters

    International Nuclear Information System (INIS)

    Gabriele Wallner; Tania Jabbar

    2010-01-01

    All commercially available mineral waters of Austrian origin were investigated with regard to the natural radionuclides 228 Ra, 226 Ra, 210 Pb, 210 Po, 238 U and 234 U. From 1 to 1.5 L of sample the nuclides were extracted and measured sequentially: the radium isotopes as well as 210 Pb were measured by liquid scintillation counting after separation on a membrane loaded with element-selective particles (Empore Radium Disks), 210 Po was determined by α-particle spectroscopy after spontaneous deposition onto a copper planchette and uranium was determined also by α-particle spectroscopy after anion separation and microprecipitation with NdF 3 . The calculated committed effective doses for adults, teens and babies were compared to the total indicative dose of 0.1 mSv/year given in the EC Drinking Water Directive. The dominant portion of the committed effective dose was due to 228 Ra. Highly mineralised waters showed also higher 226 Ra and 228 Ra levels. (author)

  17. Report of a Technical Meeting on ''Alpha emitting radionuclides and radiopharmaceuticals for therapy''

    International Nuclear Information System (INIS)

    2013-01-01

    Considering the high potential of α-emitters for future development of radionuclide therapy, the International Atomic Energy Agency (IAEA) organized a Technical Meeting on ‘Alpha Emitting Radionuclides and Radiopharmaceuticals for Therapy’, from June 24 to 28, 2013, at IAEA Headquarters in Vienna with the purpose of gathering eminent Experts in the field and discuss with them the status and future perspectives of the field. Sixteen Experts and two External Observers from ten different countries, and four IAEA Technical Officers attended this meeting. Outstanding lectures have been presented covering all relevant aspects of α-therapy, which were followed by extensive discussions and analysis. Selected arguments encompassed production methods and availability of alpha-emitting radionuclides, labelling chemistry of alpha-emittting radioelements, design and development of target-specific radiopharmaceuticals, physical principles of alpha-particle dosimetry and advanced dosimetric models, biological effects of alpha radiation at the cellular level, on-going preclinical and clinical studies with new radiopharmaceuticals, results of clinical trials on the use of radium-223 chloride solutions for the treatment of metastatic bone cancer. The broad scientific background of invited components of the Experts’ panel conferred a strong interdisciplinary trait to the overall discussion and stimulated a critical analysis of this emerging unexplored field. Results of this comprehensive overview on alpha therapy, including recommendations to the Agency on suitable initiatives that may help to promote and spread the knowledge to Members States on this emerging therapeutic modality, are summarized in the present Report

  18. Seasonal distribution and uptake of gamma emitting radionuclides at the test reactor area leaching ponds

    International Nuclear Information System (INIS)

    Millard, J.B.

    1986-01-01

    Radioactive leaching ponds adjacent to the Test Reactor Area (TRA) located on the Idaho National Engineering Laboratory (INEL) site were investigated to determine the seasonal distribution and ecological behavior of gamma emitting radionuclides in various pond compartments. The physical, chemical and biological properties of the TRA ponds were documented including basic morphometry, water chemistry and species identification. Penetrating radiation exposure rates at the ponds ranged from 35 to 65 mR/d at the water surface and up to 3400 mR/d one meter above bottom sediments. Seasonal concentrations and concentration ratios were determined for 16 principle radionuclides in filtered water, sediment, seston, zooplankton, net plankton, nannoplankton, periphyton, macrophytes, thistle, speedwell and willow. Seston and nannoplankton had the highest concentration ratios with substantial decreases observed for higher trophic level compartments. Significant (P < 0.01 to P < 0.001) seasonal effects wee found for concentration ratios. Radionuclides without nutrient analogs had the highest ratios in spring for periphyton, macrophytes and littoral plants. Concentration ratios were highest in summer, fall or winter for radionuclides with nutrient analogs

  19. Final report proficiency test on the determination of α, β and γ-emitting radionuclides

    International Nuclear Information System (INIS)

    Shakhashiro, A.; Trinkl, A.; Benesch, T.; Sansone, U.

    2005-06-01

    A proficiency test on the determination of α, β and γ-emitting radionuclides was organised within the frame of the Technical Cooperation project: RAS/9/024 'Environmental Radiation Monitoring and Regional Data Base' to evaluate the analytical performance of 14 laboratories from 12 Asian countries. This report summarises the performance evaluation of the participating laboratories. Analytical data evaluation of this proficiency test showed that 58% of all reported results obtained a 'Passed' final score for both the trueness and precision criteria applied to this exercise. (author)

  20. Application of Monte Carlo simulation to the standardization of positron emitting radionuclides

    International Nuclear Information System (INIS)

    Tongu, Margareth Lika Onishi

    2009-01-01

    Since 1967, the Nuclear Metrology Laboratory (LNM) at the Nuclear and Energy Research (IPEN) in Sao Paulo, Brazil, has developed radionuclide standardization methods and measurements of the Gamma-ray emission probabilities per decay by means of 4πβ-γ coincidence system, a high accuracy primary method for determining disintegration rate of radionuclides of interest. In 2001 the LNM started a research field on modeling, based on Monte Carlo method, of all the system components, including radiation detectors and radionuclide decay processes. This methodology allows the simulation of the detection process in a 4πβ-γ system, determining theoretically the observed activity as a function of the 4πβ detector efficiency, enabling the prediction of the behavior of the extrapolation curve and optimizing a detailed planning of the experiment before starting the measurements. One of the objectives of the present work is the improvement of the 4π proportional counter modeling, presenting a detailed description of the source holder and radioactive source material, as well as absorbers placed around the source. The simulation of radiation transport through the detectors has been carried out using code MCNPX. The main focus of the present work is on Monte Carlo modeling of the standardization of positron emitting radionuclides associated (or not) with electron capture and accompanied (or not) by the emission of Gamma radiation. One difficulty in this modeling is to simulate the detection of the annihilation Gamma ray, which arise in the process of positron absorption within the 4π detector. The methodology was applied to radionuclides 18 F and 22 Na. (author)

  1. Concentration levels of alpha emitting radionuclides in natural waters. Implications in the use of various radionuclides of reference for the determination of total alpha activity index; Niveles de concentracion de radionucleidos emisores alfa en aguas de origen natural. Implicaciones en el uso de los distintos radionucleidos de referencia para la determinacion del indice de actividad total alfa

    Energy Technology Data Exchange (ETDEWEB)

    Corbacho, J. A.; Baeza, A.; Guillen, J.; Valles, I.; Serrano, I.; Camacho, A.; Montana, M.

    2013-07-01

    The present study was carried out a statistical evaluation of the natural radioactive contents of a large number of water samples collected at different points of the Spanish geography, in order to meet its controlling radioactive composition and assessing the implications of total alpha activity index can have in this type of samples. (Author)

  2. Measurement of beta emitting radionuclides in dose calibrators routinely used in nuclear medicine departments

    International Nuclear Information System (INIS)

    Tastan, S.; Soylu, A.; Kucuk, O.; Ibis, E.

    2004-01-01

    Full text: Radionuclides for diagnostics purposes like Tc-99m, Tl-201, Ga-67 and In-111 are measured by using ionization type of dose calibrators. Therapeutic radionuclides, which emit both beta and gamma rays are detected by the same type of dose calibrators. Other therapeutic products like Y-90, P-32 and Sr-89 are pure beta emitters and they are gaining wider utility because various new therapy radiopharmaceuticals are being developed. The type of container material, like glass or plastic, may seriously affect radioactivity measurement due to attenuation, Since it is crucial to give the exact amount of radioactivity to the patient for therapy purposes, dedicated dose calibrators are specially manufactured for the measurement of these radionuclides. But these measuring systems are not widely available in nuclear medicine centers where therapy is applied to the patient. It is a known fact that dose calibrators routinely used in nuclear medicine departments can be calibrated for vials and syringes using standard sources of the same radioisotope. The method of calibration of Y-90 measurement for two ionization chamber dose calibrators available in the institute will be summarized in this presentation

  3. Measurement of beta emitting radionuclides in dose calibrators routinely used in nuclear medicine departments

    International Nuclear Information System (INIS)

    Tastan, S.; Soylu, A.; Kucuk, O.; Ibis, E.

    2004-01-01

    Radionuclides for diagnostics purposes like Tc-99m, Tl-201, Ga-67 and In-111 are measured by using ionization type of dose calibrators. Therapeutic radionuclides, which emit both beta and gamma rays are detected by the same type of dose calibrators. Other therapeutic products like Y-90, P-32 and Sr-89 are pure beta emitters and they are gaining wider utility because various new therapy radiopharmaceuticals are being developed. The type of container material, like glass or plastic, may seriously affect radioactivity measurement due to attenuation, Since it is crucial to give the exact amount of radioactivity to the patient for therapy purposes, dedicated dose calibrators are specially manufactured for the measurement of these radionuclides. But these measuring systems are not widely available in nuclear medicine centers where therapy is applied to the patient. It is a known fact that dose calibrators routinely used in nuclear medicine departments can be calibrated for vials and syringes using standard sources of the same radioisotope. The method of calibration of Y-90 measurement for two ionization chamber dose calibrators available in the institute will be summarized in this presentation. (author)

  4. Colloidal nature of radionuclides in seawater

    International Nuclear Information System (INIS)

    Feldman, I.

    1976-01-01

    There is considerable doubt that equilibrium calculations, i.e., employing solubility products and complex-ion stability constants, are valid for the submicro concentrations of radionuclides in seawater. The existence of radiocolloids should be expected in seawater. The great tendency of radiocolloids to adsorb onto finely-divided hydrous oxides makes their formation of significance in seawater, especially for artificial radionuclides. The subject of radiocolloid formation is reviewed in this chapter. It is shown that the 226 Ra/ 230 Th/U relationship found in seawater can be explained from the fact that the tendencies of these elements to form radiocolloids in seawater should decrease in order thorium > radium much greater than uranium. This explanation is much simpler than the prevailing oceanographic one. The theories for radiocolloid formation are discussed. The recent theory of Jones and Healy for the adsorption of hydrolyzable metal ions onto hydrous oxides is reviewed briefly, and its relevance to radiocolloid formation is pointed out

  5. Exposure-dose research for radionuclides in natural gas

    International Nuclear Information System (INIS)

    McNelis, D.N.; Patzer, R.G.

    1969-01-01

    The fate determination of specific radionuclides in natural gas stimulated by underground engineering applications is being examined. An experimental program, now in its initial stages, is using gas artificially labeled with krypton-85 and tritium under simulated domestic situations. The following topics are being investigated in this study: 1. The concentration of the radionuclides in a gas-heated home. 2. The build-up of contamination on appliances in the kitchen environment. 3. The concentration in foods as a function of radionuclide, food type and preparation. 4. The maximum exposure plausible under specified conditions. (author)

  6. Exposure-dose research for radionuclides in natural gas

    Energy Technology Data Exchange (ETDEWEB)

    McNelis, D N; Patzer, R G [Southwestern Radiological Health Laboratory, U.S. Public Health Service, Las Vegas, NV (United States)

    1969-07-01

    The fate determination of specific radionuclides in natural gas stimulated by underground engineering applications is being examined. An experimental program, now in its initial stages, is using gas artificially labeled with krypton-85 and tritium under simulated domestic situations. The following topics are being investigated in this study: 1. The concentration of the radionuclides in a gas-heated home. 2. The build-up of contamination on appliances in the kitchen environment. 3. The concentration in foods as a function of radionuclide, food type and preparation. 4. The maximum exposure plausible under specified conditions. (author)

  7. Naturally occurring radionuclides in agricultural products: An overview

    International Nuclear Information System (INIS)

    Hanlon, E.A.

    1994-01-01

    Low levels of naturally occurring radionuclides exist in phosphatic clays, a by-product of phosphatic mining and beneficiation processes. Concerns about these radionuclides entering the human food chain were an immediate research priority before the phosphate clays could be reclaimed for intensive agricultural purposes. Efforts included the assembly of a large body of data from both sons and plants, part of which were produced by the Polk County (Florida) Mined Lands Agricultural Research/Demonstration Project MLAR/DP. Additional detailed studies involving dairy and beef cattle (Bos taurus) were conducted by researchers working with the MLAR/DP. A national symposium was conducted in which data concerning the MLAR/DP work and other research projects also dealing with naturally occurring radionuclides in agriculture could be discussed. The symposium included invited review papers dealing with the identification of radionuclide geological origins, the geochemistry and movement of radionuclides within the environment, mechanisms of plant uptake, entry points into the food chain, and evaluation of dose and risk assessment to the consumer of low levels of radionuclides. The risk to human health of an individual obtaining 0.1 of his or her dietary intake from crops produced on phosphatic clays increased by 1 in 5 x 10 6 /yr above a control individual consuming no food grown on phosphatic clays. Leaf tissues were found to be generally higher than fruit, grain, or root tissues. The natural range in radionuclide content among various food types was greater than the difference in radionuclides content between the same food produced on phosphatic clays vs. natural soils. 19 refs

  8. Evaluation of natural radionuclides in selected regions of Slovak Republic

    International Nuclear Information System (INIS)

    Porubcanova, B.; Mojzes, A.; Nikodemova, D.

    2014-01-01

    Slovakian part of Western Carpathian is an area typical for very various geological structures. This fact is also reflected on values of natural radionuclide concentrations. Our paper was focused on evaluation and collection of data about activities of different natural radionuclides (uranium, thorium and potassium) and on the description of rocks which cause it. For research purposes were offered the results obtained from middle and eastern Slovakia which includes different types of rocks with various values of radioactive concentrations. Consequently these data were processed and shown by maps that represent the values of natural radioactivity in the studied areas. (authors)

  9. Evaluation of natural radionuclides in selected regions of Slovak Republic

    International Nuclear Information System (INIS)

    Porubcanova, B.; Nikodemova, D.; Mojzes, A.

    2014-01-01

    Slovakian part of Western Carpathian is an area typical for very various geological structures. This fact is also reflected on values of natural radionuclide concentrations. Our poster was focused on evaluation and collection of data about activities of different natural radionuclides (uranium, thorium and potassium) and on the description of rocks which cause it. For research purposes were offered the results obtained from middle and eastern Slovakia which includes different types of rocks with various values of radioactive concentrations. Consequently these data were processed and shown by maps that represent the values of natural radioactivity in the studied areas. (authors)

  10. Analyses for some transuranic and natural radionuclides in the environmental samples

    International Nuclear Information System (INIS)

    Harley, J.H.

    1978-01-01

    There is considerable present and expected future interest in the contamination of the environment with transuranic elements, particularly plutonium and americium. In addition, the alpha-emitting natural radionuclides are the usual standard of comparison for such transuranic element contamination. The present paper reviews the quality of data available for evaluating the distribution of transuranic elements and some natural radioactive elements in the environment. The overall quality cannot be documented for most programs and the data that are available indicate that the quality is poor. The fact that a few programs maintain high quality analyses indicates that the cause is poor analytical work rather than poor methods of analysis. (author)

  11. NATIONAL EMISSION STANDARDS FOR HAZARDOUS AIR POLLUTANTS (NESHAP) SUBPART H RADIONUCLIDES POTENTIAL TO EMIT CALCULATIONS

    Energy Technology Data Exchange (ETDEWEB)

    EARLEY JN

    2008-07-23

    This document provides an update of the status of stacks on the Hanford Site and the potential radionuclide emissions, i.e., emissions that could occur with no control devices in place. This review shows the calculations that determined whether the total effective dose equivalent (TEDE) received by the maximum public receptor as a result of potential emissions from any one of these stacks would exceed 0.1 millirem/year. Such stacks require continuous monitoring of the effluent, or other monitoring, to meet the requirements of Washington Administrative code (WAC) 246-247-035(1)(a)(ii) and WAC 246-247-075(1), -(2), and -(6). This revised update reviews the potential-to-emit (PTE) calculations of 31 stacks for Fluor Hanford, Inc. Of those 31 stacks, 11 have the potential to cause a TEDE greater than 0.1 mrem/year.

  12. NATIONAL EMISSION STANDARDS FOR HAZARDOUS AIR POLLUTANTS (NESHAP) SUBPART H; RADIONUCLIDES POTENTIAL-TO-EMIT CALCULATIONS

    International Nuclear Information System (INIS)

    EARLEY JN

    2008-01-01

    This document provides an update of the status of stacks on the Hanford Site and the potential radionuclide emissions, i.e., emissions that could occur with no control devices in place. This review shows the calculations that determined whether the total effective dose equivalent (TEDE) received by the maximum public receptor as a result of potential emissions from any one of these stacks would exceed 0.1 millirem/year. Such stacks require continuous monitoring of the effluent, or other monitoring, to meet the requirements of Washington Administrative code (WAC) 246-247-035(1)(a)(ii) and WAC 246-247-075(1), -(2), and -(6). This revised update reviews the potential-to-emit (PTE) calculations of 31 stacks for Fluor Hanford, Inc. Of those 31 stacks, 11 have the potential to cause a TEDE greater than 0.1 mrem/year

  13. Method for measuring the disintegration rate of a beta-emitting radionuclide in a liquid sample

    International Nuclear Information System (INIS)

    1977-01-01

    A method of measuring the distintegration rate of a beta-emitting radionuclide in a liquid sample by counting at least two differently quenched versions of the sample. In each counting operation the sample is counted in the presence of and in the absence of a standard radioactive source. A pulse height (PH) corresponding to a unique point on the pulse height spectrum generated in the presence of the standard is determined. A zero threshold sample count rate (CPM) is derived by counting the sample once in a counting window having a zero threshold lower limit. Normalized values of the measured pulse heights (PH) are developed and correlated with the corresponding counts (CPM) to determine the pulse count for a normalized pulse height value of zero and hence the sample disintegration rate

  14. External tandem target system for efficient production of short-lived positron emitting radionuclides

    International Nuclear Information System (INIS)

    Koh, K.; Dwyer, J.; Finn, R.; Sheh, Y.; Sinnreich, J.; Wooten, T.

    1983-01-01

    Recent developments in radiopharmaceutical chemistry allow the incorporation of short-lived, positron-emitting radionuclides into a variety of compounds which when used with a positron emission tomograph provide a means of monitoring physiological disorders by a standard technique. To effectively meet the increased ''in-house'' clinical demands while maintaining a production schedule, a tandem target was designed and has been installed for the simultaneous ''on-line'' preparation of oxygen-15 labelled compounds such as CO 2 15 , H 2 O 15 ; and nitrogen-13 labelled compounds such as 13 NH 3 , 13 N 2 O, and 13 N 2 . The processing time required for the synthesis of the nitrogen-13 products as compared to the essentially instantaneous formation of oxygen-15 labelled compounds has provided the necessary time delay for clinical utilization. The characterisitcs of this external tandem target system as well as the automation for the dual processing are presented

  15. Method of measuring the disinteration rate of beta-emitting radionuclide in a liquid sample

    International Nuclear Information System (INIS)

    Horrocks, D.L.

    1977-01-01

    A method of measuring the disintegration rate of a beta-emitting radionuclide in a liquid sample by counting at least two differently quenched versions of the sample is described. In each counting operation the sample is counted in the presence of and in the absence of a standard radioactive source. A pulse height (PH) corresponding to a unique point on the pulse height spectrum generated in the presence of the standard is determined. A zero threshold sample count rate (CPM) is derived by counting the sample once in a counting window having a zero threshold lower limit. Normalized values of the measured pulse heights (PH) are developed and correlated with the corresponding pulse counts (CPM) to determine the pulse count for a normalized pulse height value of zero and hence the sample disintegration rate

  16. Health effect of exposure to internally deposited alpha-emitting radionuclides

    International Nuclear Information System (INIS)

    Iwata, Shiro

    1989-01-01

    The health effect of exposure on human population to internally deposited alpha-emitting radionuclides and their decay products has been considered as most hazardous radiation effect. However, the harmful late effects by the intake of radioactive nuclides are not definite in the epidemiological and clinical viewpoint. Only two cases, radium and thorium, have since long been noted for their deletrious effects to man. As the former, it has been first reported that dial workers in USA using 226 Ra can suffer from 'radiumjaw' which is a cancer of the bone of jaws. Another radium isotope, 224 Ra, was used for a medical reason as therapy against turberculosis of bone to German children during the years 1946∼1950, and has given rise to bone cancer. As the latter, Thorotrast (the commercial name of a colloidal thorium dioxide preparation), introduced for angiography in 1929 and utilized until about 1950, was found to cause malignant hepatic tumors, liver cirrhosis and blood diseases such as some kinds of leukemia and anemia. In Japan, the former cases have seldom found though, the latter cases are assumed over 1000. Especially, Thorotrast administered war-wounded ex-servicemen in World War II have been beyond 300 persons. The epidemiological and clinico-pathological studies have been demonstrated by the research Group on Biological Effect of Thorium in Special Project Research on Energy, Japan, as a fundamental study of the safe treatment of nuclear fuel materials. The resultant data of the study and risk evaluation of liver cancer for Japanese Thorotrast administered patients are reviewed related to that of another alpha-emitting radionuclides. (author)

  17. Quality assurance in the analysis of natural radionuclides - measures and results

    Energy Technology Data Exchange (ETDEWEB)

    Bothe, M [Nuclear Engineering and Analytics Rossendorf, Inc. (VKTA), Dresden (Germany)

    1997-03-01

    In the Laboratory for Environmental and Radionuclide Analytics we analyze several natural and also some artificial radionuclides in different materials. For the determination of radionuclides we use various analytical methods. (orig./DG)

  18. Evaluation of natural radionuclide contents in the building industry

    International Nuclear Information System (INIS)

    Mrnustik, J.

    1990-01-01

    A model was adopted to calculate the effective annual dose equivalent for inhabitants of rooms built from three combinations of building materials with different natural radionuclide contents. The mean natural radionuclide contents of Czech building materials were assessed based on extensive data. The vast majority of materials satisfy the requirement that the annual dose equivalent lie within the 1-2 mSv range. Materials with average radionuclide contents contribute to the radiation burden of the population approximately twofold with respect to the natural background, which is acceptable. Raw materials used for the production of building materials must be checked for radioactivity, this checking, however, should be sensible; hasty purchases of expensive measuring instrumentation, establishment of specialized institutions, etc., as a response to public phobia is unreasonable. (P.A.). 2 tabs

  19. Natural radionuclide distribution in phosphate fertilizer and superphosphate production technology

    Energy Technology Data Exchange (ETDEWEB)

    Lisachenko, Eh P; Ponikarova, T M; Lisitsyna, Yu Z

    1987-01-01

    The obtained data on the natural radionuclide distribution by phosphate fertilizer and superphosphate production process stages testify to phosphate fertilizer enrichment 2-4 times in relation to initial ore, depending in the raw material used. In this case uranium and thorium series element concentration value (in equilibrium with their decomposition products), proposed as a regulating one in phosphorus-containing fertilizers, is not achieved. However, the fact of lurichment as it is and the enrichment factor, stated in the course of the work, should be taken into account for evaluation of phosphorite new deposit raw material with higher concentrations of natural radionuclides. Natural radionuclide separation in the enrichment process and superphosphate production is not revealed.

  20. Analyses of human exposures to alpha-emitting radionuclides from nuclear fuel cycles

    International Nuclear Information System (INIS)

    Cuddihy, R.G.; McClellan, R.O.; Griffith, W.C.; Hoover, M.D.

    1977-01-01

    Human populations may potentially be exposed to alpha-emitting radionuclides released to the environment from a variety of activities associated with nuclear fuel cycles. Generally, the most important exposure pathway is by way of inhalation. This can occur soon after release of these substances or after they have been deposited on ground surfaces and resuspended with soil particles. Estimating the potential magnitude of these exposures is usually done through the use of mathematical models accounting for the dispersion of the released material through the environment and its uptake by people living near the nuclear facilities. Studies described in this paper suggest that these exposures can probably be estimated within a factor of 10 based upon our previous experience with measured human organ levels of other trace metals taken up from the environment. It should also be noted that variability among individuals within the population may result in a few percent accumulating more than 10 times the geometric mean of the internal organ radionuclide burdens

  1. Natural radionuclides in ground water in western Spain

    International Nuclear Information System (INIS)

    Fernandez, F.; Lozano, J.C.; Gomez, J.M.G.

    1992-01-01

    A survey of natural radioactivity in drinking water was carried out in a granitic area in western Spain covering the so-called greywacke-schist complex. This region is known to be rich in uranium ores, such that natural radionuclides should be expected in the groundwater. During 1988, 345 water samples were collected from the water supplies of 115 different villages. These samples were analysed for gross alpha U, Th and Ra. The average concentrations of radionuclides were found to be 5-30 times higher in groundwater from bedrock than in groundwater from soil. The results indicate that Ra makes the highest contribution to the effective dose equivalent. (author)

  2. Natural radionuclides in ground water in western Spain

    Energy Technology Data Exchange (ETDEWEB)

    Fernandez, F.; Lozano, J.C.; Gomez, J.M.G. (Salamanca Univ. (Spain). Lab. de Radioactividad Ambiental)

    1992-01-01

    A survey of natural radioactivity in drinking water was carried out in a granitic area in western Spain covering the so-called greywacke-schist complex. This region is known to be rich in uranium ores, such that natural radionuclides should be expected in the groundwater. During 1988, 345 water samples were collected from the water supplies of 115 different villages. These samples were analysed for gross alpha U, Th and Ra. The average concentrations of radionuclides were found to be 5-30 times higher in groundwater from bedrock than in groundwater from soil. The results indicate that Ra makes the highest contribution to the effective dose equivalent. (author).

  3. Measurements of radionuclide activity by the (e-α, β, γ, Lx) coincidence method using electrons with energies of a few eV emitted from radionuclides

    International Nuclear Information System (INIS)

    Frolov, E.A.

    1994-01-01

    A study was made of the possibility of measuring radionuclide activities by the method of coincidence of electrons with energies of a few eV emitted from the valence shells of radioactive atoms with nuclear radiations. The low energy electrons were detected with a detector equipped with microchannel plates with trochoidal focusing of an original design. Photons were detected with NaI(TI) detectors. A 100 μm thick plastic scintillator was used to detect beta- and alpha-particles. The investigation shows that it is possible to use this method for accurate measurements of radionuclide activity. (orig.)

  4. Correlation Water Velocity and TSS with Natural Radionuclides Activity

    International Nuclear Information System (INIS)

    Tri Harningsih; Muzakky; Agus Taftazani

    2007-01-01

    Correlation water velocity and TSS with natural radionuclides activity has been studied. For that purpose, the study is to correlation water velocity and TSS with radionuclides on water and sediment samples in alongside river Code Yogyakarta. This research selected radionuclides, for examples Ra-226, Pb-212, Ac- 228, and K-40. Election of this radionuclides to spread over gamma gross composition alongside river of Code. Gamma gross influenced by water velocity and TSS, so that require to correct between water velocity and TSS to radionuclides. Sampling water and sediment conducted when dry season of August, 2006 at 11 locations, start from Boyong Bridge until Pacar Bridge. Result of analysis showed that water velocity range from 8-1070 L/dt and TSS range from 2.81 E-06 - 8.02 E-04 mg/L. The accumulation of radionuclides in water samples non correction water velocity for Ra-226: 0.302-2.861 Bq/L, Pb-212: 0.400-3.390 Bq/L, Ac- 228: 0.0029-0.0047 Bq/L and K-40: 0.780-9.178 Bq/L. The accumulation of radionuclide in water samples correction water velocity for Ra-226: 1.112-70.454 Bq/L, Pb-212: 0.850-77.113 Bq/L, Ac-228: 0.7187- 60.859 Bq/L and K-40: 2.420-208.8 Bq/L. While distribution of radionuclide in sediment for the Ra-226: 0.0012-0.0211 Bq/kg, Pb-212: 0.0017-0.0371 Bq/kg, Ac-228: 0.0021-0.0073 Bq/kg and K-40: 0.0006-0.0084 Bq/kg. (author)

  5. Estimate of the annual effective dose for natural radionuclides of anthropogenic origin in the Bay of Cadiz

    International Nuclear Information System (INIS)

    Rodrigo, J. F.; Martinez-Ramos, C.; Barbero, L.; Casas-Ruiz, M.

    2011-01-01

    Knowledge of radioactivity levels in soils has a double interest: on the one hand, allows you to set the reference values ??(base Linne) from a region or geographic area, and secondly, to evaluate the external radiation dose received by the population and biota, through appropriate dosimetric model. The natural radioactivity, especially the radionuclides in the natural series. The aim of this study is to determine the levels of gamma emitting radionuclides in marine sediments of the Bay of Cadiz, and dose rates from external radiation received in the areas studied. (Author)

  6. Natural radionuclides in food in an area with high concentrations of radionuclides

    International Nuclear Information System (INIS)

    Pereira, W.S.; Moraes, S.R.; Cavalcante, J.J.V.; Kelecom, A.; Silva, A.X. da; Lopez, J.M.; Filgueiras, R.; Carmo, A.S.

    2017-01-01

    Areas of high natural radiation expose the local population to doses greater than the world average. One of the routes of exposure is food intake. The activity concentration (AC) of 5 natural radionuclides in 7 types of foods was analyzed. The highest CA measured was 2.40 Bq.kg -1 for the U nat in the potato. The multivariate statistic identified two groups: (U nat e 232 Th) and [( 210 Pb and 228 Ra) and 226 Ra

  7. Natural radionuclides in soils from Sao Paulo State cerrado forest

    International Nuclear Information System (INIS)

    Miranda, Marcia V.F.E.S.; Farias, Emerson E.G. de; Cantinha, Rebeca S.; Franca, Elvis J. de

    2015-01-01

    Considering the long life history, forests should be preferentially evaluated for the monitoring of radionuclides, mainly artificial radioisotopes. However, little is known about nuclides from Uranium and Thorium series, as well as, K-40, in soils from the Sao Paulo State forests. Soils are the main reservoir of natural radionuclides for vegetation, thereby deserving attention. Taking into account the advantages of High-Resolution Gamma-ray Spectrometry (HRGS), diverse radionuclides can be quantified simultaneously. In this work natural radionuclides in soils from the Estacao Ecologica de Assis were evaluated by HRGS. Samples of 0-10 cm depth were collected under crown projection of most abundant tree species of long-term plots installed within the Estacao Ecologica de Assis, Sao Paulo State, Brazil. After drying and milling until 0.5 mm particle size, test portions of 30 g were transferred to polypropylene vials, sealed with silicone and kept under controlled conditions until 30 days to achieve secular equilibrium. A group of gamma-ray spectrometers was used to analyze about 27 samples by 80,000 seconds. Activity concentrations of Pb-214, Ac-228 and K-40 and their respective expanded analytical uncertainties at the 95% confidence level were calculated by Genie software from Canberra. Abnormal values were not detected for radionuclides in soils samples, however K-40 activity concentrations changed considerably due to the mineral cycling, in which K and, consequently K-40, is mainly stocked in vegetation in spite of soils. (author)

  8. Natural radionuclides in soils from Sao Paulo State cerrado forest

    Energy Technology Data Exchange (ETDEWEB)

    Miranda, Marcia V.F.E.S.; Farias, Emerson E.G. de; Cantinha, Rebeca S.; Franca, Elvis J. de, E-mail: mvaleria@cnen.gov.br, E-mail: emersonemiliano@yahoo.com.br, E-mail: rebecanuclear@gmail.com, E-mail: ejfranca@cnen.gov.br [Centro Regional de Ciencias Nucleares do Nordeste (CRCN-NE/CNEN-PE), Recife, PE (Brazil)

    2015-07-01

    Considering the long life history, forests should be preferentially evaluated for the monitoring of radionuclides, mainly artificial radioisotopes. However, little is known about nuclides from Uranium and Thorium series, as well as, K-40, in soils from the Sao Paulo State forests. Soils are the main reservoir of natural radionuclides for vegetation, thereby deserving attention. Taking into account the advantages of High-Resolution Gamma-ray Spectrometry (HRGS), diverse radionuclides can be quantified simultaneously. In this work natural radionuclides in soils from the Estacao Ecologica de Assis were evaluated by HRGS. Samples of 0-10 cm depth were collected under crown projection of most abundant tree species of long-term plots installed within the Estacao Ecologica de Assis, Sao Paulo State, Brazil. After drying and milling until 0.5 mm particle size, test portions of 30 g were transferred to polypropylene vials, sealed with silicone and kept under controlled conditions until 30 days to achieve secular equilibrium. A group of gamma-ray spectrometers was used to analyze about 27 samples by 80,000 seconds. Activity concentrations of Pb-214, Ac-228 and K-40 and their respective expanded analytical uncertainties at the 95% confidence level were calculated by Genie software from Canberra. Abnormal values were not detected for radionuclides in soils samples, however K-40 activity concentrations changed considerably due to the mineral cycling, in which K and, consequently K-40, is mainly stocked in vegetation in spite of soils. (author)

  9. ALMERA Proficiency Test: Determination of Gamma Emitting Radionuclides in Simulated Air Filters

    International Nuclear Information System (INIS)

    2010-01-01

    The activity concentration of radionuclides in air is a critical factor in assessing the air quality and the potential impact of possible pollutants. Air is in fact one of the main pathways for human exposure to radioactivity. Radioactivity may be present in the atmosphere due to natural processes; intentional (low level) anthropogenic release; or as a consequence of nuclear or radiological incident. The resulting environmental impact should be considered carefully to ensure safety and compliance with environmental regulations. A reliable determination of radionuclides in air is necessary for regular monitoring of air quality to comply with radiation protection and environmental regulations. This proficiency test (PT) is one of the series of the ALMERA network proficiency tests organised on regular basis by the Terrestrial Environment Laboratory in Seibersdorf, designed to assess the technical capacity of ALMERA Members in analysing radionuclides to identify any analytical problems and to support ALMERA laboratories to maintain their preparedness to provide rapid and reliable analytical results. The range of simulated air filters used in this PT for analysis has been mainly at environmental level. The PT set consisted of four filters. The participating laboratories were requested to analyze Mn-54, Co-57, Fe-59, Co-60, Zn-65, Cd-109, Ba-133, Cs-134, Cs-137, Eu-152 and Am-241 in filters 01, 02 and 03. The participants were informed that only some of the listed radionuclides were present in the filters and the levels of the radionuclides were such that they could be measured within a 6-hour measurement period using a conventional HPGe gammaspectrometer of 35% relative efficiency. Filter 04, was containing only Co-60 and Ba-133 with known activities to the participants, had to be used as a control for the efficiency calibration. The tasks of IAEA were to prepare and distribute the simulated air filters to the participating laboratories, to collect and interpret

  10. Radiation exposure by man-modified materials containing natural radionuclides

    Energy Technology Data Exchange (ETDEWEB)

    Becker, D.E. [Technical Inspection Agency of Bavaria, Munich (Germany); Eder, E. [Government of Bavaria, Ministry for State Development and Environmental Affairs Development, Munich (Germany); Reichelt, A. [Technical Inspection Agency of Bavaria, Munich (Germany)

    1992-07-01

    More than one hundred materials, containing natural radioactive nuclides, are being investigated due to radiation exposure to people. This paper deals with thoriated gas mantles and shows that the radiation exposure by inhalation of radionuclides released while burning and exchange is not negligible. (author)

  11. Radiochemical techniques for determining some naturally occurring radionuclides in marine environmental materials

    Energy Technology Data Exchange (ETDEWEB)

    Baker, C W [Ministry of Agriculture, Fisheries and Food, Lowestoft (UK). Fisheries Lab.

    1984-06-15

    The determination of some of the naturally-occurring, alpha-emitting radionuclides in marine environmental materials, is of interest for several reasons. Radium and radon nuclides are potentially useful as oceanographic tracers. Lead and thorium nuclides may be used to study sedimentation rates, mixing processes and bioturbation in sediments. Radium and polonium nuclides are incorporated into food chains and the data may provide a perspective against which to assess the significance, for marine organisms, of exposure to radiation in a marine radioactive waste disposal situation. This paper discusses the manner in which samples are taken, and the radiochemical methods which have been employed to measure the nuclides, together with some data produced.

  12. Gamma-emitting radionuclides in the bottom sediments of some Finnish lakes

    International Nuclear Information System (INIS)

    Ilus, E.; Puhakainen, M.; Saxen, R.

    1993-10-01

    In 1988 and 1990 bottom sediment and surface water samples were taken from eight large lakes representing all five categories of deposition regions contaminated by the chernobyl fallout in Finland. All samples were analysed for gamma-emitting radionuclides. The 137 Cs concentrations in surface waters varied in 1988 from 20 to 310 Bq/m 3 and in 1990 from 78 to 170 Bq/m 3 . The other radionuclides of Chernobyl origin detected in water samples were 106 Ru, 125 Sb and 134 Cs. In the sediments the total amount of 137 Cs per square metre varied in 1988 from 1100 to 160 000 Bq/m 2 and in 1990 from 14 000 to 250 000 Bq/m 2 . The maximum values were in Lake Pyhaejaervi. The maximum concentration of 137 Cs in the surface layer of sediment (0-2cm) was 55 700 Bq/kg dry wt in Lake Naesijaervi. In addition to the cesium isotopes 137 Cs and 134 Cs , Chernobyl derived 106 Ru, 125 Sb amd 144 Ce were detected i the surface layer of sediment in most lakes. 54 Mn, 60 Co and 110m Ag were also detected in some lakes situated in the regions most contaminated by the Chernobyl fallout. In 1988 the maximum concentrations of 137 Cs and 134 Cs were in the uppermost layer of sediment (0-2cm) at almost all stations. In 1990, the cesium peaks already occurred at many stations in the second slice (2-5cm), which may indicate downward diffusion of cesium in sediments or mixing of sediment layers during sampling. The most important factors affecting cesium values in sediments were the local amount of deposition and the type of sediment. This study did not reveal any correletion between the maximum depth of the lake and the area of the lake with the cesium amounts in the sediments. (orig.). (23 refs., 10 figs., 6 tabs.)

  13. Natural radionuclide distribution in Brazilian commercial granites

    International Nuclear Information System (INIS)

    Anjos, R.M.; Veiga, R.; Soares, T.; Santos, A.M.A.; Aguiar, J.G.; Frasca, M.H.B.O.; Brage, J.A.P.; Uzeda, D.; Mangia, L.; Facure, A.; Mosquera, B.; Carvalho, C.; Gomes, P.R.S.

    2005-01-01

    The dimension stones sector in Brazil produces several varieties of granites, marbles, slates and basalts. More than half of this production corresponds to around 200 different commercial types of granites with specific names, geographical and geological origins and mineral compositions. The well-known natural radioactivity present in rocks, where high radiation levels are associated with igneous rocks such as granite, can be used to determine their general petrologic features. This subject is important in environmental radiological protection, since granites are widely used as building and ornamental stones. In this paper, it is applied to correlate the petrographic characteristics of commercial granites with their corresponding dose rates for natural radioactivity. Amounts of thorium, uranium and potassium concentrations have been reported in several Brazilian commercial granite samples

  14. Uptake and dosimetry of Auger emitting diagnostic radionuclides (in particular indium-111) in human male germ cells

    International Nuclear Information System (INIS)

    Nettleton, J.S.; Lawson, R.S.; Prescott, M.C.; Hoyes, K.P.; Morris, I.D.

    2000-01-01

    This paper concerns the uptake and dosimetry of Auger electron emitting radionuclides which are used during routine diagnostic nuclear medicine procedures, in human testes and spermatozoa (sperm). A computer model was developed to calculate the doses to sperm heads from cellular localisation of the Auger electron emitting radionuclides 99m Tc, 111 In, 123 I and 201 Tl. An assumption of ellipsoidal geometry was made to approximate the sperm head. S Factors were determined for differing sub-cellular localisations of radionuclide. The S-Factors determined were then combined with in-vitro data for quantification of radionuclide uptake for 99m Tc pertechnetate, 111 In chloride and 201 Tl chloride, to estimate in-vivo doses to sperm heads following intravenous administration of radionuclide in typical diagnostic quantities. The uptake and resulting cellular radiation dose of 111 In (from the chloride) was significantly larger than the other radionuclides in the chemical forms investigated. Further investigations were carried out to determine localisation of 111 In on sperm. The results of these experiments indicate that the radiation dose to mature sperm following administration of 111 In pharmaceuticals for diagnostic purposes might be large enough to result in DNA damage which is not expressed until after fertilisation of an oocyte. Consideration should therefore be given to providing some contraceptive advice following diagnostic administrations of this radionuclide. In order to consider the possible effects of these radionuclides on other spermatogenic cells, further studies were undertaken to obtain in-vivo data for quantification of 111 In chloride and 201 Tl chloride uptake into the human testis following intravenous administration. Conventional dosimetry was then used to estimate testicular radiation dose using our values of percentage uptake. The results obtained indicate that the values of testicular radiation doses quoted by ICRP for 111 In might be too low by

  15. Influence of radiation-dose pattern from inhaled beta--gamma-emitting radionuclides on canine peripheral lymphocytes

    International Nuclear Information System (INIS)

    Jones, R.K.; Boecker, B.B.; Pickrell, J.A.; Hobbs, C.H.; McClellan, R.O.

    1976-01-01

    As part of studies assess the biological hazards associated with inhaled radionuclides, periodic hematologic evaluations were performed on beagle dogs given a single nose-only exposure to aerosols of beta--gamma-emitting isotopes. The physical form and specific radionuclides selected produced radiation-dose patterns representative of those which might be encountered in the event of human accidental exposures. Dogs received graded lung burdens of either 90 Y, 91 Y, 144 Ce, or 90 Sr, each in fused clay. Differences in the effective half-lives of these radionuclides resulted in a spectrum of cumulative radiation doses to lung delivered at a variety of dose rates. Since the form in which the radionuclides were inhaled was relatively insoluble, the lung and intrathoracic tissues represented the primary recipient of the dose. Regardless of the effective half-life of radionuclide retention, a dose-related depression of peripheral lymphocytes was observed at various times after inhalation exposure. The time at which maximum depression and subsequent recovery occurred, however, was most directly related to the effective half-life of the radionuclide. Of special interest was the persistence of lymphopenia through 2 1 / 2 years after exposure to 144 Ce and 90 Sr in fused clay where, other than tracheobronchial lymph nodes, the lymphoid tissue received very little radiation dose. The possible mechanisms responsible for lymphocyte depression from these various radiation-dose patterns are discussed

  16. Investigation of natural radionuclide contents in soil in China

    International Nuclear Information System (INIS)

    Pan Sanming; Liu Ruye

    1992-01-01

    The survey of natural radionuclide contents in soil in China (1983-1990) is a part of investigation of environmental natural radioactivity level on China. The results of the investigation area as follows: (1) The average content of natural radionuclides 238 U, 226 Ra, 232 Th and 40 K(area weighted) and its standard deviation for single measurement is 39.5 and 34.4,36.5 and 22.0, 49.1 and 27.6, 580.0 and 202.0 Bq.kg -1 ,respectively.(2) The content of natural radionuclides is apparently correlated to the types of soil-forming rock. The analysis results from 1552 soil samples of soil-forming rock show that: the content of 238 U, 226 Ra, 232 Th and 40 K for magmatic rock type is the highest, 238 U, 226 Ra and 232 Th of metamorphic rock type higher, sedimentary rock type the lowest. However, the content of 40 K of sedimentary rock type is more higher, magmatic rock type the lowest. In magmatic rock type, the content of 238 U, 226 Ra, 232 Th of granite and acidic magmatic rock type, and the content of 40 K of acidic and alkaline magmatic rock type are higher. (3) The analysis results from 9613 various types of soil samples show that for crimson soil of ferralsol wind soil of rock soil-forming order at northern part is lower. For frigid dessert soil of alpine soil order, alpine dessert soil, and the burozem, dark burozem and drab soil of alfisol order and semialfisol order, the content of 40 K is shown to be higher, and it is lower for latosol of ferralsol order, crimson soil, yellow soil and various lime soil. (4) The geographical distribution of the natural radionuclide content in soil appears apparently regional

  17. Migration of uranium daughter radionuclides in natural sediments

    International Nuclear Information System (INIS)

    Colley, S.; Thomson, J.

    1991-01-01

    An irregular concentration/depth profile of uranium in deep-sea turbidities, previously elucidated, has been exploited to obtain in-situ effective diffusion coefficients for the long-lived members of the 238 U natural series. The findings are relevant to the assessment of deep-sea sediments as potential repositories for high-level radioactive waste, because waste actinides decay through the same chains of daughter radionuclides as natural actinides. This work was part of the CEC Mirage project-Second phase, Natural analogues research area

  18. The transport of natural radionuclides from soil to plants

    International Nuclear Information System (INIS)

    Bikit, I.; Conkic, Lj.; Slivka, J.; Krmar, M.

    1995-01-01

    The transport and accumulation processes of Ra-226, U-238, Th-232 and K-40 from soil to plants have been studied. Plant samples with consumable parts grown below surface have been bred in natural conditions on soil with enhanced levels of natural radioactivity (barren soil of the uranium mine Gabrovnica-Kalna). An intensive transport of heavy natural radionuclides from soil to the roots was established. The transfer factors for U-238 and Ra-226 have been much bigger than for Th-232. The most intensive uptake was registered for beet root. (author)

  19. An determination of man-made γ-emitting radionuclides in coal fly ash and standard solution

    International Nuclear Information System (INIS)

    Xu Cuihua; Zhou Qiang

    2004-01-01

    We participated an international comparison on the determination of man-made γ-emitting radionuclides in coal fly ash and in standard solution organized by the Analytical Quality Control Service of the IAEA in 2002. The sample was dispensed in 100.0 ± 0.1 g aliquots in plastic container and was spiked with known amounts of certified standard γ-emitting radionuclides 54 Mn, 57 Co, 60 Co, 65 Zn, 88 Y, 134 Cs, 137 Cs and 241 Am. The determination of the anthropogenic )γ-emitting radionuclides in the test samples was carried out with an ORTEC gamma-ray spectrometry system coupled with a HPGe detector with resolution of 1.75 keV and relative efficiency of 55% for 137 Cs, located in a 10 cm thick lead container. The energy and efficiency calibration were with home-made volume calibration sources containing some of the radionuclides to be analyzed. The analysis procedure is described elsewhere. Table 1 lists the results of the determination and the comparisons with IAEA reference data and evaluation. Overall our results are agreeable in ±8.6% with the IAEA reference data, except for 60 Co. The differences for 60 Co was -10.8%. It may be caused by the 60 Co calibration source made with residual of quiet old standard solution. The difference for 241 Am is due to self-absorption in the fly ash sample. This bias was small for the solution sample. For standard solution sample, the results are agreeable within ±3.7% for all radionuclides except for 60 Co, being 12%. (authors)

  20. Technogenic and natural radionuclides in Black Sea sediments and algae

    International Nuclear Information System (INIS)

    Strezov, A.; Stoilova, T.; Petkov, N.; Hristoskova, M.

    1999-01-01

    Technogenic and natural emitters have been monitored since 1991 in marine samples from the Bulgarian Black Sea coast by low level gamma and alpha spectroscopy. The radionuclide content was determined in bottom sediment samples from 35 reference locations in the spring, summer and autumn during six consecutive years. Samples were collected and data obtained for the main Black Sea resorts and the main dwelling places along the Bulgarian Black Sea shore

  1. Environmental effects of radionuclides--observations on natural ecosystems.

    Science.gov (United States)

    Copplestone, D; Toal, M E; Johnson, M S; Jackson, D; Jones, S R

    2000-03-01

    To better quantify risk to non-human species from exposure to environmental radioactivity, understanding of the behaviour of radionuclides in the biosphere needs to be increased. This study outlines current thinking on ecological risk assessment (ERA) methodology and applies the indicator species or critical groups approach to biota inhabiting a semi-natural coniferous woodland contaminated with the radionuclides 137Cs, 238Pu, 239+240Pu and 241Am. The majority of these radionuclides originate from routine aerial emissions from the nuclear fuel reprocessing plant at BNFL, Sellafield, Cumbria, UK. Radionuclide activity concentrations have been determined in biota from the woodland and estimates of absorbed dose rates (mGy d(-1)) have been calculated using the dosimetric models outlined. Dose rates to the key indicator species, Oniscus asellus, Carabus violaceous and Apodemus sylvaticus (detritivorous invertebrate, predatory invertebrate and the granivorous wood mouse) have been determined at 3.0 x 10(-3) mGy d(-1), 2.2 x 10(-3) mGy d(-1) and 1.0 x 10(-3) mGy d(-1) respectively. The values are at least three orders of magnitude lower than the 1 mGy d(-1) level below which no observable effects on populations in a terrestrial ecosystem are thought to occur. Limitations of this approach are discussed.

  2. Environmental effects of radionuclides - observations on natural ecosystems

    International Nuclear Information System (INIS)

    Copplestone, D.; Toal, M.E.; Johnson, M.S.; Jackson, D.; Jones, S.R.

    2000-01-01

    To better quantify risk to non-human species from exposure to environmental radioactivity, understanding of the behaviour of radionuclides in the biosphere needs to be increased. This study outlines current thinking on ecological risk assessment (ERA) methodology and applies the indicator species or critical groups approach to biota inhabiting a semi-natural coniferous woodland contaminated with the radionuclides 137 Cs, 238 Pu, 239+240 Pu and 241 Am. The majority of these radionuclides originate from routine aerial emissions from the nuclear fuel reprocessing plant at BNFL, Sellafield, Cumbria, UK. Radionuclide activity concentrations have been determined in biota from the woodland and estimates of absorbed dose rates (mGy d -1 ) have been calculated using the dosimetric models outlined. Dose rates to the key indicator species, Oniscus asellus, Carabus violaceous and Apodemus sylvaticus (detritivorous invertebrate, predatory invertebrate and the granivorous wood mouse) have been determined at 3.0x10 -3 mGy d -1 , 2.2x10 -3 mGy d -1 and 1.0x10 -3 mGy d -1 respectively. The values are at least three orders of magnitude lower than the 1 mGy d -1 level below which no observable effects on populations in a terrestrial ecosystem are thought to occur. Limitations of this approach are discussed. (author)

  3. Environmental effects of radionuclides - observations on natural ecosystems

    Energy Technology Data Exchange (ETDEWEB)

    Copplestone, D. [Industrial Ecology Research Centre, School of Biological Sciences, University of Liverpool, Liverpool L69 3BX (United Kingdom). E-mail: copplest at liv.ac.uk; Toal, M.E.; Johnson, M.S. [Industrial Ecology Research Centre, School of Biological Sciences, University of Liverpool, Liverpool L69 3BX (United Kingdom); Jackson, D.; Jones, S.R. [Westlakes Scientific Consulting, Princess Royal Building, Westlakes Science and Technology Park, Moor Row, Cumbria CA24 3LN (United Kingdom)

    2000-03-01

    To better quantify risk to non-human species from exposure to environmental radioactivity, understanding of the behaviour of radionuclides in the biosphere needs to be increased. This study outlines current thinking on ecological risk assessment (ERA) methodology and applies the indicator species or critical groups approach to biota inhabiting a semi-natural coniferous woodland contaminated with the radionuclides {sup 137}Cs, {sup 238}Pu, {sup 239+240}Pu and {sup 241}Am. The majority of these radionuclides originate from routine aerial emissions from the nuclear fuel reprocessing plant at BNFL, Sellafield, Cumbria, UK. Radionuclide activity concentrations have been determined in biota from the woodland and estimates of absorbed dose rates (mGy d{sup -1}) have been calculated using the dosimetric models outlined. Dose rates to the key indicator species, Oniscus asellus, Carabus violaceous and Apodemus sylvaticus (detritivorous invertebrate, predatory invertebrate and the granivorous wood mouse) have been determined at 3.0x10{sup -3} mGy d{sup -1}, 2.2x10{sup -3} mGy d{sup -1} and 1.0x10{sup -3} mGy d{sup -1} respectively. The values are at least three orders of magnitude lower than the 1 mGy d{sup -1} level below which no observable effects on populations in a terrestrial ecosystem are thought to occur. Limitations of this approach are discussed. (author)

  4. Natural background gamma-ray spectrum. List of gamma-rays ordered in energy from natural radionuclides

    International Nuclear Information System (INIS)

    Ichimiya, Tsutomu; Narita, Tsutomu; Kitao, Kensuke.

    1998-03-01

    A quick index to γ-rays and X-rays from natural radionuclides is presented. In the list, γ-rays are arranged in order of increasing energy. The list also contains γ-rays from radioactive nuclides produced in a germanium detector and its surrounding materials by interaction with cosmic neutrons, as well as direct γ-rays from interaction with the neutrons. Artificial radioactive nuclides emitting γ-rays with same or near energy value as that of the natural γ-rays and X-rays are also listed. In appendix, γ-ray spectra from a rock, uranium ore, thorium, monazite and uraninite and also background spectra obtained with germanium detectors placed in iron or lead shield have been given. The list is designed for use in γ-ray spectroscopy under the conditions of highly natural background, such as in-situ environmental radiation monitoring or low-level activity measurements, with a germanium detector. (author)

  5. Natural background gamma-ray spectrum. List of gamma-rays ordered in energy from natural radionuclides

    Energy Technology Data Exchange (ETDEWEB)

    Ichimiya, Tsutomu [Japan Radioisotope Association, Tokyo (Japan); Narita, Tsutomu; Kitao, Kensuke

    1998-03-01

    A quick index to {gamma}-rays and X-rays from natural radionuclides is presented. In the list, {gamma}-rays are arranged in order of increasing energy. The list also contains {gamma}-rays from radioactive nuclides produced in a germanium detector and its surrounding materials by interaction with cosmic neutrons, as well as direct {gamma}-rays from interaction with the neutrons. Artificial radioactive nuclides emitting {gamma}-rays with same or near energy value as that of the natural {gamma}-rays and X-rays are also listed. In appendix, {gamma}-ray spectra from a rock, uranium ore, thorium, monazite and uraninite and also background spectra obtained with germanium detectors placed in iron or lead shield have been given. The list is designed for use in {gamma}-ray spectroscopy under the conditions of highly natural background, such as in-situ environmental radiation monitoring or low-level activity measurements, with a germanium detector. (author)

  6. Accelerator based production of auger-electron-emitting isotopes for radionuclide therapy

    International Nuclear Information System (INIS)

    Thisgaard, H.

    2008-08-01

    In this research project the focus has been on the identification and production of new, unconventional Auger-electron-emitting isotopes for targeted radionuclide therapy of cancer. Based on 1st principles dosimetry calculations on the subcellular level, the Auger-emitter 119Sb has been identified as a potent candidate for therapy. The corresponding imaging analogue 117Sb has been shown from planar scintigraphy and single-photon emission computed tomography (SPECT) to be suitable for SPECT-based dosimetry of a future Sb-labeled radiopharmaceutical. The production method of these radioisotopes has been developed using a low-energy cyclotron via the nuclear reactions 119Sn(p,n)119Sb and 117Sn(p,n)117Sb including measurements of the excitation function for the former reaction. Moreover, a new high-yield radiochemical separation method has been developed to allow the subsequent separation of the produced 119Sb from the enriched 119Sn target material with high radionuclidic- and chemical purity. A method that also allows efficient recovery of the 119Sn for recycling. To demonstrate the ability of producing therapeutic quantities of 119Sb and other radioisotopes for therapy with a low-energy cyclotron, two new 'High Power' cyclotron targets were developed in this study. The target development was primarily based on theoretical thermal modeling calculations using finite-element-analysis software. With these targets, I have shown that it will be possible to produce several tens of GBq of therapeutics isotopes (e.g. 119Sb or 64Cu) using the PETtrace cyclotron commonly found at the larger PET-centers in the hospitals. Finally, research in a new method to measure the radiotoxicity of Auger-emitters invitro using cellular microinjection has been carried out. The purpose of this method is to be able to experimentally evaluate and compare the potency of the new and unconventional Auger-emitters (e.g. 119Sb). However, due to experimental complications, the development of this

  7. Accelerator based production of auger-electron-emitting isotopes for radionuclide therapy

    Energy Technology Data Exchange (ETDEWEB)

    Thisgaard, H.

    2008-08-15

    In this research project the focus has been on the identification and production of new, unconventional Auger-electron-emitting isotopes for targeted radionuclide therapy of cancer. Based on 1st principles dosimetry calculations on the subcellular level, the Auger-emitter 119Sb has been identified as a potent candidate for therapy. The corresponding imaging analogue 117Sb has been shown from planar scintigraphy and single-photon emission computed tomography (SPECT) to be suitable for SPECT-based dosimetry of a future Sb-labeled radiopharmaceutical. The production method of these radioisotopes has been developed using a low-energy cyclotron via the nuclear reactions 119Sn(p,n)119Sb and 117Sn(p,n)117Sb including measurements of the excitation function for the former reaction. Moreover, a new high-yield radiochemical separation method has been developed to allow the subsequent separation of the produced 119Sb from the enriched 119Sn target material with high radionuclidic- and chemical purity. A method that also allows efficient recovery of the 119Sn for recycling. To demonstrate the ability of producing therapeutic quantities of 119Sb and other radioisotopes for therapy with a low-energy cyclotron, two new 'High Power' cyclotron targets were developed in this study. The target development was primarily based on theoretical thermal modeling calculations using finite-element-analysis software. With these targets, I have shown that it will be possible to produce several tens of GBq of therapeutics isotopes (e.g. 119Sb or 64Cu) using the PETtrace cyclotron commonly found at the larger PET-centers in the hospitals. Finally, research in a new method to measure the radiotoxicity of Auger-emitters invitro using cellular microinjection has been carried out. The purpose of this method is to be able to experimentally evaluate and compare the potency of the new and unconventional Auger-emitters (e.g. 119Sb). However, due to experimental complications, the development

  8. Development of positron emitting radionuclides for imaging with improved positron detectors

    International Nuclear Information System (INIS)

    Yano, Y.

    1976-10-01

    Recent advances in positron cameras and positron ring detectors for transverse section reconstruction have created renewed interest in positron emitting radionuclides. This paper reports on: generator-produced 82 Rb; cyclotron-produced 62 Zn; and reactor-produced 64 Cu. Investigation of the 82 Sr (25 d)-- 82 Rb (75 s) generator determined the elution characteristics for Bio-Rex 70, a weakly acidic carboxylic cation exchanger, using 2% NaCl as the eluent. The yield of 82 Rb and the breakthrough of 82 Sr were determined for newly prepared columns and for long term elution conditions. Spallation-produced 82 Sr was used to charge a compact 82 Rb generator to obtain multi-millicurie amounts of 82 Rb for myocardial imaging. Zinc accumulates in the islet cells of the pancreas and in the prostate. Zinc-62 was produced by protons on Cu foil and separated by column chromatography. Zinc-62 was administered as the amino acid chelates and as the ZnCl 2 to tumor and normal animals. Tissue distribution was determined for various times after intravenous injection. Pancreas-liver images of 62 Zn-histidine uptake were obtained in animals with the gamma camera and the liver uptake of /sup 99m/Tc sulfur colloid was computer subtracted to image the pancreas alone. The positron camera imaged uptake of 62 Zn-histidine in the prostate of a dog at 20 h. 64 Cu was chelated to asparagine, a requirement of leukemic cells, and administered to lymphoma mice. Uptake in tumor and various tissues was determined and compared with the uptake of 67 Ga citrate under the same conditions. 64 Cu-asparagine had better tumor-to-soft tissue ratios than 67 Ga-citrate

  9. Determination of naturally occurring radionuclides in El-Sin Water

    International Nuclear Information System (INIS)

    Al-Masri, M.S.; Al-Rayyes, A.H.

    2000-01-01

    Naturally occurring radionuclides levels have been determined in El-Sin water for the period of 1995 and 1996. water samples were collected from four sites, which are the main drinking water sources of the area. Radon concentration was found to vary between 0.88 Bq/1 in Lattakia main water supply site and 8.4 Bq/1 in El-Sin springs.The highest values found for other radionuclides were 51.6 mBq/1, 18.6 mB/1 and 24.8 mBq/1 for sup 2 sup 2 sup 6 Ra, sup 2 sup 1 sup 0 Po and total uranium (sup 2 sup 3 sup 4 U and sup 2 sup 3 sup 8 U) respectively. These levels are much lower than the maximum permissible levels in drinking water set by international organization.(author)

  10. Determination of natural radionuclides in lichen samples of Carnoparmelia Texana

    International Nuclear Information System (INIS)

    Alencar, Marcos M.; Damatto, Sandra R.; Mazzilli, Barbara P.

    2009-01-01

    Lichen plays an important role in studies of environmental pollution. It can be used for the evaluation of air contaminants, including heavy metals and radionuclides. The main objective of this study is to verify the possibility of using the lichen species Canoparmelia Texana for the assessment of natural radionuclides of the U and Th decay series in air in the vicinity of Instituto de Pesquisas Energeticas e Nucleares (IPEN) installations. IPEN has as major activity to perform research in the field of the nuclear fuel cycle, and therefore deals with natural radionuclides of the U and Th series. The content of 238 U, 234 U, 230 Th, 210 Po and 232 Th in lichen samples were determined by alpha spectrometry after a radiochemical separation. Ra isotopes and 210 Pb were determined by gross alpha and beta counting after a radiochemical separation and measurement on a low background gas flow proportional detector. The results obtained for 238 U varied from 2.4 ± 0.4 Bq kg -1 to 6.6 ± 0.1 Bq kg -1 and from 4.4 ± 0.3 Bq kg -1 to 12.1 ± 2.6 Bq kg -1 , for 232 Th. For 226 Ra varied from 13 ± 1 Bq kg -1 to 38 ± 2 Bq kg -1 and from 200 ± 13 Bq kg -1 to 351 ± 12 Bqkg -1 for 228 Ra. The results obtained were compared with data obtained for the same radionuclides in lichen samples in an area affected by TENORM industry and can be considered as background for this lichen species. It can be concluded that the control of atmospheric discharges of IPEN facilities has been effective along the years, giving no evidence of radiological environmental impact. (author)

  11. Natural decay series radionuclide studies at the Needle's Eye natural analogue site

    International Nuclear Information System (INIS)

    MacKenzie, A.B.; Scott, R.D.; Houston, C.M.; Hooker, P.J.

    1991-01-01

    This report covers work on a natural radioactive geochemical system and has been carried out with the aim of improving confidence in using predictive models of radionuclide migration in the geosphere. It is one of a series being produced and is concerned with the U/Th decay series characterization of the hydrothermal mineral veins and the movement of these radionuclides into post-glacial flood plain deposits

  12. An assessment of natural radionuclides in water of Langat River estuary, Selangor

    Energy Technology Data Exchange (ETDEWEB)

    Hamzah, Zaini, E-mail: tengkuliana88@gmail.com; Rosli, Tengku Nurliana Tuan Mohd, E-mail: tengkuliana88@gmail.com; Saat, Ahmad, E-mail: tengkuliana88@gmail.com; Wood, Ab. Khalik, E-mail: tengkuliana88@gmail.com [Faculty of Applied Sciences, Universiti Teknologi MARA, 40450 Shah Alam, Selangor (Malaysia)

    2014-02-12

    An estuary is an area that has a free connection with the open sea and it is a dynamic semi-enclosed coastal bodies. Ex-mining, aquaculture and industrial areas in Selangor are the sources of pollutants discharged into the estuary water. Radionuclides are considered as pollutants to the estuary water. Gamma radiations emitted by natural radionuclides through their decaying process may give impact to human. The radiological effect of natural radionuclides which are {sup 226}Ra, {sup 228}Ra, {sup 40}K, {sup 238}U and {sup 232}Th, were explored by determining the respective activity concentrations in filtered water along the Langat estuary, Selangor. Meanwhile, in- situ water quality parameters such as temperature, dissolve oxygen (DO), salinity, total suspended solid (TSS), pH and turbidity were measured by using YSI portable multi probes meter. The activity concentration of {sup 226}Ra, {sup 228}Ra and {sup 40}K were determined by using gamma-ray spectrometry with high-purity germanium (HPGe) detector. The activity concentrations of {sup 226}Ra, {sup 228}Ra and {sup 40}K in samples are in the range of 0.17 - 0.67 Bq/L, 0.16 - 0.97 Bq/L and 1.22 - 5.57 Bq/L respectively. On the other hand, the concentrations of uranium-238 and thorium-232 were determined by using Energy Dispersive X-ray Fluorescence Spectrometry (EDXRF). The thorium concentrations are between 0.17 ppm to 0.28 ppm and uranium concentrations were 0.25 ppm to 0.31 ppm. The results show activity concentrations of radionuclides are slightly high near the river estuary. The Radium Equivalent, Absorbed Dose Rate, External Hazard Index, and Annual Effective Dose of {sup 226}Ra, {sup 228}Ra and {sup 40}K are also studied.

  13. Natural radionuclides in Italian diet and their annual intake

    International Nuclear Information System (INIS)

    Donatella Desideri; Maria Assunta Meli; Carla Roselli; Laura Feduzi; Nevio Forini; Alba Rongoni

    2014-01-01

    This study was dedicated to the evaluation of the background activity concentration of natural radionuclides as 228 Ra and 228 Th of 232 Th family, 226 Ra of 238 U family and 40 K in the Italian daily diet. These radionuclides were determined by gamma spectrometry. 40 K activity concentration, in the samples taken into account in the present paper, ranged between 70.5 (milk) and 181.1 Bq kg ww -1 (pasta), 226 Ra activity concentration ranged between 1.1 (milk) and 5.7 Bq kg ww -1 (pasta), 228 Ra and 228 Th activity concentration, in the same samples, ranged between 0.7 (milk) and 3.7 Bq kg ww -1 (pasta) and between 1.4 (milk) and 6.1 Bq kg ww -1 (flours) respectively. The annual intake of every radionuclide from foodstuffs ingestion was also calculated. The 94-95 % of the total intake comes from 40 K. For adults and children, the highest activity intake of all radioisotopes was from grain products, for infants it was from milk products. (author)

  14. Natural and artificial radionuclides in soils from Parana State, Brazil

    International Nuclear Information System (INIS)

    Schuch, L.A.; Barreto, W.O.; Cardoso, A.

    1994-01-01

    Soil samples from Parana State, Brazil, were collected in 1991 and compared with others collected at some location in March 1977 and at the end of 1983. Pedological analyses were practiced on the samples and 137 Cs and 232 Th, 226 Ra and 40 K activities were determined by gamma-ray spectrometry. A latitude dependence of 137 Cs was found as well. It was impossible to determine the 137 Cs contribution from Chernobyl nuclear accident because of low fallout and intense leaching, erosion and re-suspension in soils of regions with high annual precipitation. Natural radionuclides did not show such effects. (author) 39 refs; 6 tabs

  15. Determination of dose rates from natural radionuclides in dental materials

    International Nuclear Information System (INIS)

    Veronese, I.; Guzzi, G.; Giussani, A.; Cantone, M.C.; Ripamonti, D.

    2006-01-01

    Different types of materials used for dental prosthetics restoration, including feldspathic ceramics, glass ceramics, zirconia-based ceramics, alumina-based ceramics, and resin-based materials, were investigated with regard to content of natural radionuclides by means of thermoluminescence beta dosimetry and gamma spectrometry. The gross beta dose rate from feldspathic and glass ceramics was about ten times higher than the background measurement, whereas resin-based materials generated negligible beta dose rate, similarly to natural tooth samples. The specific activity of uranium and thorium was significantly below the levels found in the period when addition of uranium to dental porcelain materials was still permitted. The high-beta dose levels observed in feldspathic porcelains and glass ceramics are thus mainly ascribable to 4 K, naturally present in these specimens. Although the measured values are below the recommended limits, results indicate that patients with prostheses are subject to higher dose levels than other members of the population. Alumina- and zirconia-based ceramics might be a promising alternative, as they have generally lower beta dose rates than the conventional porcelain materials. However, the dosimetry results, which imply the presence of inhomogeneously distributed clusters of radionuclides in the sample matrix, and the still unsuitable structural properties call for further optimization of these materials

  16. Reference Material IAEA 434: Naturally Occurring Radionuclides in Phosphogypsum

    International Nuclear Information System (INIS)

    2010-01-01

    Phosphogypsum is generated as a by-product of the phosphoric acid based fertilizer industry. The discharge of phosphogypsum on earth surface deposits is a potential source of enhanced natural radiation and heavy metals, and the resulting environmental impact should be considered carefully to ensure safety and compliance with environmental regulations. In addition, phosphogypsum can be used to make several building materials and it is used in agriculture as a conditioner to maintain soil productivity in areas where soils are poor and erode easily. A reliable determination of naturally occurring radionuclides in phosphogypsum is necessary to comply with the radiation protection and environmental regulations. The IAEA-434 will assist laboratories in the IAEA Member States in validating their analytical methods for the determination of naturally occurring radionuclides in phosphogypsum and to control the quality of the produced analytical results. Reference values for the massic activities and associated standard uncertainties were established for: Pb-210, Ra-226, Th-230, U-234 and U-238. During sample production and certification, the requirements for reference material production and certification as stated in ISO guides 34 and 35 were taken into account. This report summarizes the preparation and certification process

  17. Natural decay series radionuclide studies at the Needle's Eye Natural Analogue Site, II, 1989-1991

    International Nuclear Information System (INIS)

    MacKenzie, A.B.; Whitton, A.M.; Shimmield, T.M.; Jemielita, R.A.; Scott, R.D.; Hooker, P.J.

    1991-12-01

    HMIP has a research programme investigating some naturally radioactive sites as geochemical analogues of radionuclide migration. The objective is to test thermodynamic databases and computer codes used for modelling radionuclide migration under environmental conditions. This report describes the study of transport and retardation processes affecting natural radionuclides, mainly uranium (U), in the vicinity of pitchblende veins in the cliff at Needle's Eye on the Solway Coast, SW Scotland. The natural decay series results from this study have been used to develop a well constrained geochemical model within which the codes can be tested. A conceptual geochemical model for the behaviour of U at the site was developed in stage I of the study; work in stage II is concerned with improving the information available on the U source term, groundwater chemistry, U aqueous phase specification, U retardation by fracture-lining minerals during fissure flow of groundwater, U-organic associations and loss of U from the site by stream drainage. (author)

  18. A sensitive and quantitative biosensing method for the determination of {gamma}-ray emitting radionuclides in surface water

    Energy Technology Data Exchange (ETDEWEB)

    Wolterbeek, H.Th.; Meer, A.J.G.M. van der [Technische Univ. Delft (Netherlands). Interfacultair Reactor Inst.

    1996-11-01

    A quantitative and sensitive biosensing method has been developed for the determination of {gamma}-ray emitting radionuclides in surface water. The method is based on the concept that at equilibrium the specific radioactivity in the biosensor is equal to the specific radioactivity in water. The method consists of the measurement of both the radionuclide and the element in the biosensor and the determination of the element level in water. This three-way analysis eliminates problems such as unpredictable biosensor behaviour, effects of water elemental composition or further abiotic parameters: what remains is the generally high enrichment (bioaccumulation factor BCF) of elements and radionuclides in the biosensor material. Measurements were performed with floating water plants (Azolla filiculoides Lamk., Spirodela polyrhiza/Lemna sp.) and the fully submerged water plant Ceratophyllum demersum L., which were sampled from ditch water. Concentrations of elements and radionuclides were determined in both water and biosensor plants, using Neutron Activation Analysis (NAA), ICP-MS, and {gamma}-ray spectrometry, respectively. For the latter, both 1 litre samples (Marinelli-geometry) and 1 cm{sup 3} samples (well-type detectors) were applied in measurements. (author).

  19. A sensitive and quantitative biosensing method for the determination of γ-ray emitting radionuclides in surface water

    International Nuclear Information System (INIS)

    Wolterbeek, H.Th.; Meer, A.J.G.M. van der

    1996-01-01

    A quantitative and sensitive biosensing method has been developed for the determination of γ-ray emitting radionuclides in surface water. The method is based on the concept that at equilibrium the specific radioactivity in the biosensor is equal to the specific radioactivity in water. The method consists of the measurement of both the radionuclide and the element in the biosensor and the determination of the element level in water. This three-way analysis eliminates problems such as unpredictable biosensor behaviour, effects of water elemental composition or further abiotic parameters: what remains is the generally high enrichment (bioaccumulation factor BCF) of elements and radionuclides in the biosensor material. Measurements were performed with floating water plants (Azolla filiculoides Lamk., Spirodela polyrhiza/Lemna sp.) and the fully submerged water plant Ceratophyllum demersum L., which were sampled from ditch water. Concentrations of elements and radionuclides were determined in both water and biosensor plants, using Neutron Activation Analysis (NAA), ICP-MS, and γ-ray spectrometry, respectively. For the latter, both 1 litre samples (Marinelli-geometry) and 1 cm 3 samples (well-type detectors) were applied in measurements. (author)

  20. Public Health Goal for Naturally Occurring Radionuclides in Groundwater

    International Nuclear Information System (INIS)

    Kamel, N.H.M.; Omar, H.A.; El-Baset, L.A.

    2008-01-01

    Naturally occurring and man-made radionuclide in groundwater may have a health hazardous to some residents. The objective of this work is to provide criteria for safety of drinking-water with respect to the chemical parameters and the radionuclide content. The annual effective dose for the consumption of drinking water was considered. Ground water samples were selected from different sites in Egypt, that have the most population, it were taken from aquifer regions along Giza sites in Egypt. Chemical analyses for the major anions, cations, and the radiological analyses were tested . Activity concentrations (Bq/l) of the gross alpha and the gross beta activities of our investigated samples were compared with the maximum contaminant level (MCL) of the world health organization (WHO). Some of the water samples were found to have a higher of gross beta and alpha particles than the MCL. Alpha activity were found depending on to the total dissolved solids (TDS) content of the water samples. Gamma activity concentrations were analyzed using low background germanium detector, the higher of activity values was found in some investigated samples is due to increasing of 226 Ra and 228 Ra activities. Tritium activity concentrations also were measured using soft beta liquid scintillation counter, it was found lower than the MCL. Our investigated samples were found to have a higher concentrations of the phosphate, nitrites, iron, and manganese contents than the maximum permissible limit, all the ground water samples were found to have a higher of silica and alumina content. Commercial carbon powder and natural clay materials were tested as ion exchangers for the removal of inorganic contaminants in the ground water samples. Clay materials was found to have a higher selectivity than activated carbon for the removal of radionuclides, phosphates, nitrites, and manganese content at the ground water samples

  1. Estimate of S-values for children due to six positron emitting radionuclides used in PET examinations

    Science.gov (United States)

    Belinato, Walmir; Santos, William S.; Perini, Ana P.; Neves, Lucio P.; Caldas, Linda V. E.; Souza, Divanizia N.

    2017-11-01

    Positron emission tomography (PET) has revolutionized the diagnosis of cancer since its conception. When combined with computed tomography (CT), PET/CT performed in children produces highly accurate diagnoses from images of regions affected by malignant tumors. Considering the high risk to children when exposed to ionizing radiation, a dosimetric study for PET/CT procedures is necessary. Specific absorbed fractions (SAF) were determined for monoenergetic photons and positrons, as well as the S-values for six positron emitting radionuclides (11C, 13N, 18F, 68Ga, 82Rb, 15O), and 22 source organs. The study was performed for six pediatric anthropomorphic hybrid models, including the newborn and 1 year hermaphrodite, 5 and 10-year-old male and female, using the Monte Carlo N-Particle eXtended code (MCNPX, version 2.7.0). The results of the SAF in source organs and S-values for all organs showed to be inversely related to the age of the phantoms, which includes the variation of body weight. The results also showed that radionuclides with higher energy peak emission produces larger auto absorbed S-values due to local dose deposition by positron decay. The S-values for the source organs are considerably larger due to the interaction of tissue with non-penetrating particles (electrons and positrons) and present a linear relationship with the phantom body masses. The results of the S-values determined for positron-emitting radionuclides can be used to assess the radiation dose delivered to pediatric patients subjected to PET examination in clinical settings. The novelty of this work is associated with the determination of auto absorbed S-values, in six new pediatric virtual anthropomorphic phantoms, for six emitting positrons, commonly employed in PET exams.

  2. Risk Due to Radiological Terror Attacks With Natural Radionuclides

    Science.gov (United States)

    Friedrich, Steinhäusler; Stan, Rydell; Lyudmila, Zaitseva

    2008-08-01

    The naturally occurring radionuclides radium (Ra-226) and polonium (Po-210) have the potential to be used for criminal acts. Analysis of international incident data contained in the Database on Nuclear Smuggling, Theft and Orphan Radiation Sources (CSTO), operated at the University of Salzburg, shows that several acts of murder and terrorism with natural radionuclides have already been carried out in Europe and Russia. Five different modes of attack (T) are possible: (1) Covert irradiation of an individual in order to deliver a high individual dose; (2) Covert irradiation of a group of persons delivering a large collective dose; (3) Contamination of food or drink; (4) Generation of radioactive aerosols or solutions; (5) Combination of Ra-226 with conventional explosives (Dirty Bomb). This paper assesses the risk (R) of such criminal acts in terms of: (a) Probability of terrorist motivation deploying a certain attack mode T; (b) Probability of success by the terrorists for the selected attack mode T; (c) Primary damage consequence (C) to the attacked target (activity, dose); (d) Secondary damage consequence (C') to the attacked target (psychological and socio-economic effects); (e) Probability that the consequences (C, C') cannot be brought under control, resulting in a failure to manage successfully the emergency situation due to logistical and/or technical deficits in implementing adequate countermeasures. Extensive computer modelling is used to determine the potential impact of such a criminal attack on directly affected victims and on the environment.

  3. Risk Due to Radiological Terror Attacks With Natural Radionuclides

    International Nuclear Information System (INIS)

    Friedrich, Steinhaeusler; Lyudmila, Zaitseva; Stan, Rydell

    2008-01-01

    The naturally occurring radionuclides radium (Ra-226) and polonium (Po-210) have the potential to be used for criminal acts. Analysis of international incident data contained in the Database on Nuclear Smuggling, Theft and Orphan Radiation Sources (CSTO), operated at the University of Salzburg, shows that several acts of murder and terrorism with natural radionuclides have already been carried out in Europe and Russia. Five different modes of attack (T) are possible: (1) Covert irradiation of an individual in order to deliver a high individual dose; (2) Covert irradiation of a group of persons delivering a large collective dose; (3) Contamination of food or drink; (4) Generation of radioactive aerosols or solutions; (5) Combination of Ra-226 with conventional explosives (Dirty Bomb).This paper assesses the risk (R) of such criminal acts in terms of: (a) Probability of terrorist motivation deploying a certain attack mode T; (b) Probability of success by the terrorists for the selected attack mode T; (c) Primary damage consequence (C) to the attacked target (activity, dose); (d) Secondary damage consequence (C') to the attacked target (psychological and socio-economic effects); (e) Probability that the consequences (C, C') cannot be brought under control, resulting in a failure to manage successfully the emergency situation due to logistical and/or technical deficits in implementing adequate countermeasures. Extensive computer modelling is used to determine the potential impact of such a criminal attack on directly affected victims and on the environment

  4. Radionuclide data

    International Nuclear Information System (INIS)

    Anon.

    1992-01-01

    Chapter 8 presents tables on selected alpha, beta, gamma and x-ray emitters by increasing energy; information on specific activity for selected radionuclides; naturally occurring radionuclides; the natural decay series; and the artificially produced neptunium series. A table of alpha emitters is listed by increasing atomic number and by energy. The table of β emitters presented is useful in identifying β emitters whose energies and possibly half-lives have been determined by standard laboratory techniques. It is also a handy guide to β-emitting isotopes for applications requiring specific half-lives and/or energies. Gamma rays for radionuclides of importance to radiological assessments and radiation protection are listed by increasing energy. The energies and branching ratios are important for radionuclide determinations with gamma spectrometry detectors. This section also presents a table of x-ray energies which are useful for radiochemical analyses. A number of nuclides emit x-rays as part of their decay scheme. These x-rays may be counted with Ar proportional counters, Ge planar or n-type Ge co-axial detectors, or thin crystal NaI(T1) scintillation counters. In both cases, spectral measurements can be made and both qualitative and quantitative information obtained on the sample. Nuclear decay data (energy and probability by radiation type) for more than one hundred radionuclides that are important to health physicists are presented in a schematic manner

  5. Natural radionuclides in Syrian diet and their daily intake

    International Nuclear Information System (INIS)

    Al-Masri, M.S.; Mukallati, H.; Al-Hamwi, A.; Khalili, H.; Hassan, M.; Assaf, H.; Amin, Y.; Nashawati, A.

    2004-01-01

    More than one hundred different food stuffs (meat, vegetables cereals, seafood,..) have been collected during 1998, 1999 and 2000 and analyzed for radioactivity as part of the National Food Monitoring Program in Syria. Results have shown that most of the observed concentrations were within the range of the worldwide values with the exception of relatively high levels of 210 Po being observed in fish, vegetables, mushrooms, herbs and flowers. The daily intakes of the radionuclides studied have been evaluated. Relatively high values, in comparison with some countries, were found for 210 Po (1.9 Bq/day). This is due to high content of 210 Po in wheat (2.3 Bq/kg) consumed by Syrians, the daily consumption of wheat by Syrians is about 526 g. In addition, natural and artificial radionuclides in some manufactured food of Syrian infant and their intake rates have been determined. Seventeen manufactured food and eleven types of canned milk were collected from the local market and their radioactivity analyzed. 210 Po activity concentration varied between 0.38 and 2.89 Bq/kg dry wt. in canned milk while the highest concentration in infant food was found to be 1.69 Bq/kg dry wt. Other radionuclide concentrations were below the limit of detection of 3 Bq/kg dry wt. and 4 Bq/kg dry wt. for 22' 6Ra and 228 Ra, respectively, while uranium concentration varied between 2.2 and 10.5 μg/kg dry wt. in milk samples and 0.78-6.0 μg/kg dry wt. in other food samples. (author)

  6. Natural analogue studies of the role of colloids, natural organics and microorganisms on radionuclide transport

    International Nuclear Information System (INIS)

    McCarthy, J.F.

    1994-01-01

    Colloids may be important as a geochemical transport mechanism for radionuclides at geological repositories if they are (1) present in the groundwater, (2) stable with respect to both colloidal and chemical stabilities, (3) capable of adsorbing radionuclides, especially if the sorption is irreversible, and (4) mobile in the subsurface. The available evidence from natural analogue and other field studies relevant to these issues is reviewed, as is the potential role of mobile microorganisms (open-quotes biocolloidsclose quotes) on radionuclide migration. Studies have demonstrated that colloids are ubiquitous in groundwater, although colloid concentrations in deep, geochemically stable systems may be too low to affect radionuclide transport. However, even low colloid populations cannot be dismissed as a potential concern because colloids appear to be stable, and many radionuclides that adsorb to colloids are not readily desorbed over long periods. Field studies offer somewhat equivocal evidence concerning colloid mobility and cannot prove or disprove the significance of colloid transport in the far-field environment. Additional research is needed at new sites to properly represent a repository far-field. Performance assessment would benefit from natural analogue studies to examine colloid behavior at sites encompassing a suite of probable groundwater chemistries and that mimic the types of formations selected for radioactive waste repositories

  7. Natural Radionuclides in Private Wells | RadTown USA | US ...

    Science.gov (United States)

    2017-08-07

    About 15 percent of Americans use private wells as their main source of drinking water. Those who use private wells should remember: Test for radionuclides every three years. Take appropriate steps if radionuclide levels are higher than EPA's limits.

  8. Radiation doses to aquatic organisms from natural radionuclides

    International Nuclear Information System (INIS)

    Brown, J E; Jones, S R; Saxen, R; Thoerring, H; Batlle, J Vives i

    2004-01-01

    A framework for protection of the environment is likely to require a methodology for assessing dose rates arising from naturally occurring radionuclides. This paper addresses this issue for European aquatic environments through a process of (a) data collation, mainly with respect to levels of radioactivity in water sediments and aquatic flora and fauna, (b) the use of suitable distribution coefficients, concentration factors and global data where data gaps are present and (c) the utilisation of a reference organism approach whereby a finite number of suitable geometries are selected to allow dose per unit concentration factors to be derived and subsequent absorbed dose calculations (weighted or unweighted) to be made. The majority of the calculated absorbed dose, for both marine and freshwater organisms, arises from internally incorporated alpha emitters, with 210 Po and 226 Ra being the major contributors. Calculated doses are somewhat higher for freshwater compared to marine organisms, and the range of doses is also much greater. This reflects both the much greater variability of radionuclide concentrations in freshwater as compared to seawater, and also variability or uncertainty in concentration factor values. This work has revealed a number of substantial gaps in published empirical data especially for European aquatic environments

  9. Activity measurement and effective dose modelling of natural radionuclides in building material

    International Nuclear Information System (INIS)

    Maringer, F.J.; Baumgartner, A.; Rechberger, F.; Seidel, C.; Stietka, M.

    2013-01-01

    In this paper the assessment of natural radionuclides' activity concentration in building materials, calibration requirements and related indoor exposure dose models is presented. Particular attention is turned to specific improvements in low-level gamma-ray spectrometry to determine the activity concentration of necessary natural radionuclides in building materials with adequate measurement uncertainties. Different approaches for the modelling of the effective dose indoor due to external radiation resulted from natural radionuclides in building material and results of actual building material assessments are shown. - Highlights: • Dose models for indoor radiation exposure due to natural radionuclides in building materials. • Strategies and methods in radionuclide metrology, activity measurement and dose modelling. • Selection of appropriate parameters in radiation protection standards for building materials. • Scientific-based limitations of indoor exposure due to natural radionuclides in building materials

  10. 238 U 92 radionuclide handbook. Natural Uranium and environment

    International Nuclear Information System (INIS)

    Garnier-Laplace, J.; Colle, C.; Morello, M.

    2001-01-01

    This handbook summarizes the behaviour of the chemical element in the main compartments of land and aquatic ecosystems, under the two following assumptions: isotopic discrimination is negligible (this is validated for most of the examined elements); when the element possesses stable isotopes, the behaviour analogy between its stable and radioactive isotopes is implicitly admitted, knowing that, for elements existing at the natural state, the chemical form and the emitting media of the anthropic effluents are susceptible of implying other transfer processes than those identified for the natural stable element. The handbook gives information on the chemical and nuclear characteristics of the element, its origins, the concentrations in the environment, the mobility and bio-availability in land ecosystems (soils, plants, animals) and aquatic ecosystems (waters, sediments, plants, animals)

  11. Life-span health effects of relatively soluble forms of internally deposited beta-emitting radionuclides

    International Nuclear Information System (INIS)

    Boecker, B.B.; Muggenburg, B.A.; Hahn, F.F.; Nikula, K.J.; Griffith, W.C.

    1991-01-01

    As part of a large research effort to study the lifetime health risks of inhaled radionuclides, Beagle dogs inhaled 90 SrCl 2 or 144 CeCl 3 or were injected intravenously with 137 CsCl. Because these three compounds were soluble in body fluids, the resulting widely differing patterns of radionuclide distribution and dose reflected tissue affinities of the elements involved. Long-term health effects, predominantly cancers, were seen in the organs receiving the highest doses. Investigations are continuing on the extent to which other less irradiated organs may have also been affected

  12. Committed effective dose from naturally occuring radionuclides in shellfish

    International Nuclear Information System (INIS)

    Khandaker, Mayeen Uddin; Wahib, Norfadira Binti; Amin, Yusoff Mohd.; Bradley, D.A.

    2013-01-01

    Recognizing their importance in the average Malaysian daily diet, the radioactivity concentrations in mollusc- and crustacean-based food have been determined for key naturally occuring radionuclides. Fresh samples collected from various maritime locations around peninsular Malaysia have been processed using standard procedures; the radionuclide concentrations being determined using an HPGe γ-ray spectrometer. For molluscs, assuming secular equilibrium, the range of activities of 238 U ( 226 Ra), 232 Th ( 228 Ra) and 40 K were found to be 3.28±0.35 to 5.34±0.52, 1.20±0.21 to 2.44±0.21 and 118±6 to 281±14 Bq kg −1 dry weight, respectively. The respective values for crustaceans were 3.02±0.57 to 4.70±0.52, 1.38±0.21 to 2.40±0.35 and 216±11 to 316±15 Bq kg −1 . The estimated average daily intake of radioactivity from consumption of molluscs are 0.37 Bq kg −1 for 238 U ( 226 Ra), 0.16 Bq kg −1 for 232 Th ( 228 Ra) and 18 Bq kg −1 for 40 K; the respective daily intake values from crustaceans are 0.36 Bq kg −1 , 0.16 Bq kg −1 and 23 Bq kg −1 . Associated annual committed effective doses from molluscs are estimated to be in the range 21.3 to 34.7 μSv for 226 Ra, 19.3 to 39.1 μSv for 228 Ra and 17.0 to 40.4 μSv for 40 K. For crustaceans, the respective dose ranges are 19.6 to 30.5 μSv, 22.0 to 38.4 μSv and 31.1 to 45.5 μSv, being some several times world average values. - Highlights: ► Activity concentrations of naturally occuring radionuclides were assessed for shellfish. ► 238 U, 232 Th, 40 K intake via shellfish showed several times higher than world averages. ► Committed effective doses due to the ingestions of 238 U, 232 Th, 40 K are the first report in Malaysia. ► Estimated committed effective dose also showed higher values than the world average

  13. The role of natural organics in radionuclide migration in natural aquifer systems

    International Nuclear Information System (INIS)

    Choppin, G.R.

    1992-01-01

    The wide variety of organic compounds present in natural waters is assessed for the role they may play in radionuclide and, especially, actinide migration. Some natural analog and environmental data are briefly reviewed for evaluation of the effect of organics in these systems. The binding constants and the kinetics of complexation of actinides by humics are discussed in terms of probable effects on actinide migration. The role of organics in redox, and in sorption, is also considered. (orig.)

  14. Tracking the complete revolution of surface westerlies over Northern Hemisphere using radionuclides emitted from Fukushima

    International Nuclear Information System (INIS)

    Hernández-Ceballos, M.A.; Hong, G.H.; Lozano, R.L.; Kim, Y.I.; Lee, H.M.; Kim, S.H.; Yeh, S.-W.; Bolívar, J.P.; Baskaran, M.

    2012-01-01

    Massive amounts of anthropogenic radionuclides were released from the nuclear reactors located in Fukushima (northeastern Japan) between 12 and 16 March 2011 following the earthquake and tsunami. Ground level air radioactivity was monitored around the globe immediately after the Fukushima accident. This global effort provided a unique opportunity to trace the surface air mass movement at different sites in the Northern Hemisphere. Based on surface air radioactivity measurements around the globe and the air mass backward trajectory analysis of the Fukushima radioactive plume at various places in the Northern Hemisphere by employing the Hybrid Single-Particle Lagrangian Integrated Trajectory model, we show for the first time, that the uninterrupted complete revolution of the mid-latitude Surface Westerlies took place in less than 21 days, with an average zonal velocity of > 60 km/h. The position and circulation time scale of Surface Westerlies are of wide interest to a large number of global researchers including meteorologists, atmospheric researchers and global climate modellers. -- Highlights: ► Evidence of the South Korea contamination with released radiocesium from Fukushima. ► Field samples and air mass analysis were utilized to elucidate the transport of those radionuclides. ► Characterization of the air mass movements at different sites at the Earth's surface. ► Verification of the uninterrupted complete revolution of the artificial radionuclides released in Fukushima. ► Quantification of the velocity of the artificial radionuclides released in Fukushima.

  15. Tracking the complete revolution of surface westerlies over Northern Hemisphere using radionuclides emitted from Fukushima

    Energy Technology Data Exchange (ETDEWEB)

    Hernandez-Ceballos, M.A. [Department of Applied Physics, University of Huelva, Huelva (Spain); Hong, G.H. [Korea Ocean Research and Development Institute, Ansan 426-744 (Korea, Republic of); Lozano, R.L. [Department of Applied Physics, University of Huelva, Huelva (Spain); Kim, Y.I. [Korea Ocean Research and Development Institute, Uljin 767-813 (Korea, Republic of); Lee, H.M.; Kim, S.H. [Korea Ocean Research and Development Institute, Ansan 426-744 (Korea, Republic of); Yeh, S.-W. [Department of Environmental Marine Science, Hanyang University, Ansan, 426-791 (Korea, Republic of); Bolivar, J.P., E-mail: bolivar@uhu.es [Department of Applied Physics, University of Huelva, Huelva (Spain); Baskaran, M. [Department of Geology, Wayne State University, Detroit, Michigan (United States)

    2012-11-01

    Massive amounts of anthropogenic radionuclides were released from the nuclear reactors located in Fukushima (northeastern Japan) between 12 and 16 March 2011 following the earthquake and tsunami. Ground level air radioactivity was monitored around the globe immediately after the Fukushima accident. This global effort provided a unique opportunity to trace the surface air mass movement at different sites in the Northern Hemisphere. Based on surface air radioactivity measurements around the globe and the air mass backward trajectory analysis of the Fukushima radioactive plume at various places in the Northern Hemisphere by employing the Hybrid Single-Particle Lagrangian Integrated Trajectory model, we show for the first time, that the uninterrupted complete revolution of the mid-latitude Surface Westerlies took place in less than 21 days, with an average zonal velocity of > 60 km/h. The position and circulation time scale of Surface Westerlies are of wide interest to a large number of global researchers including meteorologists, atmospheric researchers and global climate modellers. -- Highlights: Black-Right-Pointing-Pointer Evidence of the South Korea contamination with released radiocesium from Fukushima. Black-Right-Pointing-Pointer Field samples and air mass analysis were utilized to elucidate the transport of those radionuclides. Black-Right-Pointing-Pointer Characterization of the air mass movements at different sites at the Earth's surface. Black-Right-Pointing-Pointer Verification of the uninterrupted complete revolution of the artificial radionuclides released in Fukushima. Black-Right-Pointing-Pointer Quantification of the velocity of the artificial radionuclides released in Fukushima.

  16. Natural radionuclides in the human body; Natuerliche Radionuklide im menschlichen Koerper

    Energy Technology Data Exchange (ETDEWEB)

    Voelkle, Hansruedi [Fribourg Univ. (Switzerland). Physikdept.

    2017-08-01

    Natural radionuclides in the human body produce worldwide a medium annual radiation exposure of 0.31 mSv. 0.17 mSv are due to potassium-40 (K-40) per year, 0.12 mSv per year are due to radionuclides from the uranium and thorium decay series, less than 0.02 mSv due to cosmogenic radionuclides. Natural radioactivity is therefore the largest exposure source, anthropogenic exposure is comparatively marginal.

  17. Analysis of natural radionuclides and lead in foods and diets

    International Nuclear Information System (INIS)

    Bueno, Luciana

    1999-01-01

    The main purpose of the present study was to determine the lead-210, polonium-210 and lead concentrations in foods and diets. Consumption of food is generally the main route by which radionuclides can enter the human organism. Precision and accuracy of the methods developed were verifies by the analysis of reference materials from the International Atomic Energy Agency (IAEA). The method for polonium-210 analysis consisted of sample dissolution by using a microwave digester (open system) employing concentrated nitric acid and hydrogen peroxide, evaporation almost dryness, addition of hydrochloric acid, polonium deposition onto silver disc for six hours and counting by alpha spectrometry. Lead was analysed by atomic absorption technique. After sample dissolution in a microwave digester (using concentrated nitric acid and hydrogen peroxide) and dilution to 50 ml, 20μl of the sample was injected in a pyrolytic graphite furnace - atomic absorption spectrophotometer equipped with Zeeman background correction. The assessment of the contaminants in foods and diets allowed to estimate the intake of these elements and for the radionuclides were also evaluated the radiation doses that the individuals selected were exposed by the food consumption. The effective dose for lead-210 by diets intake ranged from 1.3 to 4.3 μSv/year, corresponding to 25% of the resulting from polonium-210 intake. The dose due to the both natural radionuclides varied from 6.8 to 23.0 μSv/year. These values are in good agreement with the literature data. The value estimated by the United Nations Scientific Committee on Effects of Atomic Radiation (UNSCEAR, 1993) that is 60 μSv and lower than the dose of 0.02 Sv, limit established by ICRP, 1980. The lead levels found in the majority of the Brazilian foods are in good agreement with the values published by CONAT and FAO/WHO. However, some foods such as bean, potato, papaya, apple and rice present levels above of the recommended values by the Public

  18. Elimination of man-made radionuclides from natural waters by applying a standard coagulation-flocculation process

    International Nuclear Information System (INIS)

    Baeza, A.; Miro, C.; Salas, A.; Fernandez, M.; Herranz, M.; Legarda, F.

    2004-01-01

    Effectiveness of potable water treatment processes that consist of the stages of coagulation-flocculation-decantation, using iron-based coagulants, in eliminating gamma-emitting man-made radioisotopes of cesium, strontium, and americium from two natural waters with different degrees of mineralization was studied. The resulting decontamination was found to depend on the chemical behavior of each of the radionuclides considered, on the pH at which the process of coagulation is carried out, and on the concentration of the other stable cations present. (author)

  19. Investigation and assessment of natural radionuclides in groundwater and geothermal fluid of Tianjin city

    International Nuclear Information System (INIS)

    Wang Xiao; Duan Xigui; Gao Liang; Yang Yuxin

    2012-01-01

    Investigation on the specific activities of natural radionuclides in the groundwater and geothermal fluids of Tianjin city were conducted. Based on the investigation, internal dose level posed by drinking the water and fluid to local public was evaluated. Results show the specific activities of natural radionuclides in the groundwater and geothermal fluid of Tianjin city is under control, no abnormal radioactivity discovered. (authors)

  20. Harvard--MIT research program in short-lived radiopharmaceuticals. Progress report, September 1, 1977--April 30, 1978. [/sup 99m/Tc, positron-emitting radionuclides

    Energy Technology Data Exchange (ETDEWEB)

    Adelstein, S.J.; Brownell, G.L.

    1978-05-01

    Progress is reported on the following studies: chemistry studies designed to achieve a more complete understanding of the fundamental chemistry of technetium in order to facilitate the design of future radiopharmaceuticals incorporating the radionuclide /sup 99m/Tc; the development of new radiopharmaceuticals intended to improve image quality and lower radiation doses by the use of short-lived radionuclides and disease-specific agents; the development of short-lived positron-emitting radionuclides which offer advantages in transverse section imaging of regional physiological processes; and studies of the toxic effects of particulate radiation.

  1. A review of measurement and characterisation of airborne long-lived alpha-emitting radionuclides

    International Nuclear Information System (INIS)

    Bigu, J.

    1993-01-01

    Sampling principles, monitoring instrumentation and characterisation of Long-Lived Radioactive Dust (LLRD) generated in U-Th mine and mill operations are discussed. Methods and techniques for the quantification, radionuclide identification and the study of other important characteristics of LLRD (e.g., electrical charge) are reviewed. Furthermore, field and laboratory measurements and methods of radiation dose assessment are revised. Some emphasis is placed in this work on occupational worker exposure assessment and the principles, methods and techniques of 'external' radiation exposure, internal dosimetry, and dosimetric models. It is clear that in spite of constant advances in the several areas which are the subject of this paper, there is still considerable room for improvement. For example, there is no universally accepted sampling protocol and sampler for routine LLRD monitoring for occupational hygiene exposure calculation purposes. Other areas for improvement could include calibration of instrumentation and improved sensitivity in radionuclide quantification and identification. 105 refs., 6 tabs., 3 figs

  2. Gamma emitting radionuclides in fruits and vegetables produced in the Canary Islands: domestic consequences

    International Nuclear Information System (INIS)

    Triguero-Perez, M.; Duarte-Rodriguez, X.; Lopez-Perez, M.; Hernandez-Armas, J.

    2011-01-01

    Determine the possible effects due to ingestion of radionuclides that can be found in health food is of interest from the viewpoint of radiation protection of the population. these determinations and analysis of the consequences on the health of people and jobs has led to studies that have had consequences in the form of rules to follow and values have to be attended to limit dictated by national and international agencies. (Author)

  3. Behavior of natural radionuclides in wastewater treatment plants

    International Nuclear Information System (INIS)

    Camacho, A.; Montaña, M.; Vallés, I.; Devesa, R.; Céspedes-Sánchez, R.; Serrano, I.; Blázquez, S.; Barjola, V.

    2012-01-01

    56 samples, including influent, primary effluent, secondary effluent and final effluent wastewater from two Spanish municipal wastewater treatment plants (WWTPs), were analyzed to assess both the occurrence and behavior of natural radioactivity during 12 sampling campaigns carried out over the period 2007–2010. Influent and final effluent wastewaters were sampled by taking into account the hydraulic residence time within the WWTP. A wide range of gross alpha activities (15–129 mBq/L) and gross beta activities (477–983 mBq/L) in liquid samples were obtained. A correlation analysis between radioactivity in liquid samples and the performance characteristics of the WWTPs was performed. The results in liquid samples showed that gross beta activities were not influenced by treatment in the studied WWTPs. However, gross alpha activities behave differently and an increase was detected in the effluent values compared with influent wastewater. This behavior was due to the increase in the total dissolved uranium produced during secondary treatment. The results indicate that the radiological characteristics of the effluents do not present a significant radiological risk and make them suitable for future applications. - Highlights: ► Liquids from WWTPs were analyzed to know the behavior of natural radionuclides. ► Gross beta activities were not influenced by treatment in the studied WWTPs. ► Increase in gross alpha activity was observed due to uranium desorption/solubilisation. ► Correlation between gross alpha activity and the chemical oxygen demand was found

  4. Method for measuring the decay rate of a radionuclide emitting β-rays in a liquid sample

    International Nuclear Information System (INIS)

    Horrocks, D.

    1977-01-01

    With this method the decay rate of a radionuclide emitting β-rays, e.g. 3 H or 14 C, in a liquid sample can be measured by means of liquid scintillation counters, at least two different versions of the sample being used with quench effect (shifting of the Compton spectrum). For this purpose each sample is counted with and without a radioactive standard source, e.g. 137 Cs. Then a pulse height will be determined corresponding to a selected point in the pulse height spectrum if the standard source is present. The determination of a zero-threshold sample count rate is then performed by counting the sample in a counting window. In addition standardized values of the measured pulse heights are derived and put in mathematical relation to corresponding pulse count rates, the pulse count rate for a standardized pulse height value thus becoming zero and the sample decay rate in this way being determined. (DG) 891 HP [de

  5. Natural and anthropogenic radionuclide activity concentrations in the New Zealand diet.

    Science.gov (United States)

    Pearson, Andrew J; Gaw, Sally; Hermanspahn, Nikolaus; Glover, Chris N

    2016-01-01

    To support New Zealand's food safety monitoring regime, a survey was undertaken to establish radionuclide activity concentrations across the New Zealand diet. This survey was undertaken to better understand the radioactivity content of the modern diet and also to assess the suitability of the current use of milk as a sentinel for dietary radionuclide trends. Thirteen radionuclides were analysed in 40 common food commodities, including animal products, fruits, vegetables, cereal grains and seafood. Activity was detected for (137)Caesium, (90)Strontium and (131)Iodine. No other anthropogenic radionuclides were detected. Activity concentrations of the three natural radionuclides of Uranium and the daughter radionuclide (210)Polonium were detected in the majority of food sampled, with a large variation in magnitude. The maximum activity concentrations were detected in shellfish for all these radionuclides. Based on the established activity concentrations and ranges, the New Zealand diet contains activity concentrations of anthropogenic radionuclides far below the Codex Alimentarius guideline levels. Activity concentrations obtained for milk support its continued use as a sentinel for monitoring fallout radionuclides in terrestrial agriculture. The significant levels of natural and anthropogenic radionuclide activity concentrations detected in finfish and molluscs support undertaking further research to identify a suitable sentinel for New Zealand seafood monitoring. Copyright © 2015 The Authors. Published by Elsevier Ltd.. All rights reserved.

  6. Monte Carlo simulation of different positron emitting radionuclides incorporated in a soft tissue volume

    International Nuclear Information System (INIS)

    Olaya D, H.; Martinez O, S. A.; Sevilla M, A. C.; Vega C, H. R.

    2015-10-01

    Monte Carlo calculations were carried out where compounds with positron-emitters radionuclides, like FDG ( 18 F), Acetate ( 11 C), and Ammonium ( 13 N), were incorporated into a soft tissue volume, in the aim to estimate the type of particles produced their energies, their mean free paths, and the absorbed dose at different distances with respect to the center of the volume. The volume was modeled with a radius larger than the maximum range of positrons in order to produce 0.511 keV annihilation gamma-ray photons. With the obtained results the equivalent dose, in various organs and tissues able to metabolize different radiopharmaceutical drugs, can be estimated. (Author)

  7. Accelerator based Production of Auger-Electron-emitting Isotopes for Radionuclide Therapy

    DEFF Research Database (Denmark)

    Thisgaard, Helge

    Sb from the enriched 119Sn target material with high radionuclidic- and chemical purity. A method that also allows efficient recovery of the 119Sn for recycling. To demonstrate the ability of producing therapeutic quantities of 119Sb and other radioisotopes for therapy with a low-energy cyclotron...... isotopes (e.g. 119Sb or 64Cu) using the PETtrace cyclotron commonly found at the larger PET-centers in the hospitals. Finally, research in a new method to measure the radiotoxicity of Auger-emitters invitro using cellular microinjection has been carried out. The purpose of this method is to be able...

  8. Natural radionuclides in soil profiles surrounding the largest coal-fired power plant in Serbia

    OpenAIRE

    Tanić Milan N.; Janković-Mandić Ljiljana J.; Gajić Boško A.; Daković Marko Z.; Dragović Snežana D.; Bačić Goran G.

    2016-01-01

    This study evaluates the influence of the largest Serbian coal-fired power plant on radionuclide concentrations in soil profiles up to 50 cm in depth. Thirty soil profiles were sampled from the plant surroundings (up to 10 km distance) and analyzed using standard methods for soil physicochemical properties and gamma ray spectrometry for specific activities of natural radionuclides (40K, 226Ra and 232Th). Spatial and vertical distribution of radionuclides wa...

  9. Natural radionuclides near a coal-fired power station

    International Nuclear Information System (INIS)

    Smith-Briggs, J.L.

    1984-01-01

    A previous assessment of the radiological consequences of the emission of natural radionuclides from coal-fired power stations had indicated that 210 Pb was the main contributor to the maximum individual dose. This dose arose from the consumption of foodstuffs particularly cattle liver contaminated by deposited fly ash. Uncertainty surrounded some of the factors used in the assessment, and a limited environmental monitoring programme was recommended to improve it. An experiment has been performed to measure the specific activities of 210 Pb and 210 Po in livers from cattle that had grazed in a field near Didcot power station. Livers from cattle in the Cotswold region have been measured for comparison. The specific activities of 210 Pb and 210 Po in soil and grass samples from both areas have also been measured at three-monthly intervals over a year. No statistically significant increases were observed in the 210 Pb and 210 Po levels in liver, soil or grass samples which could be attributed to the operation of the power station. Transfer coefficients for 210 Pb from forage to liver were about two orders of magnitude less than that used in the original assessment, and the transfer coefficients for 210 Po about a factor a two less. (orig.)

  10. Committed effective dose from naturally occuring radionuclides in shellfish

    Science.gov (United States)

    Khandaker, Mayeen Uddin; Wahib, Norfadira Binti; Amin, Yusoff Mohd.; Bradley, D. A.

    2013-07-01

    Recognizing their importance in the average Malaysian daily diet, the radioactivity concentrations in mollusc- and crustacean-based food have been determined for key naturally occuring radionuclides. Fresh samples collected from various maritime locations around peninsular Malaysia have been processed using standard procedures; the radionuclide concentrations being determined using an HPGe γ-ray spectrometer. For molluscs, assuming secular equilibrium, the range of activities of 238U (226Ra), 232Th (228Ra) and 40K were found to be 3.28±0.35 to 5.34±0.52, 1.20±0.21 to 2.44±0.21 and 118±6 to 281±14 Bq kg-1 dry weight, respectively. The respective values for crustaceans were 3.02±0.57 to 4.70±0.52, 1.38±0.21 to 2.40±0.35 and 216±11 to 316±15 Bq kg-1. The estimated average daily intake of radioactivity from consumption of molluscs are 0.37 Bq kg-1 for 238U (226Ra), 0.16 Bq kg-1 for 232Th (228Ra) and 18 Bq kg-1 for 40K; the respective daily intake values from crustaceans are 0.36 Bq kg-1, 0.16 Bq kg-1 and 23 Bq kg-1. Associated annual committed effective doses from molluscs are estimated to be in the range 21.3 to 34.7 μSv for 226Ra, 19.3 to 39.1 μSv for 228Ra and 17.0 to 40.4 μSv for 40K. For crustaceans, the respective dose ranges are 19.6 to 30.5 μSv, 22.0 to 38.4 μSv and 31.1 to 45.5 μSv, being some several times world average values.

  11. Preliminary identification of contaminating α- and β-emitting radionuclides in nuclear facilities to be decommissioned through Digital Autoradiography

    International Nuclear Information System (INIS)

    Haudebourg, Raphael; Fichet, Pascal

    2016-01-01

    In previous publications, we presented how Digital Autoradiography (DA) could be of the most useful help in a preparation to decommissioning context: with this technique, a radiological mapping of the facility to dismantle can be obtained at a rate of around 2 weeks/100 m 2 . The technique is sensitive to all types of radioactivity (including α and 3 H- or 14 C-emitted β) and to both labile and fixed radioactivity. The method (radiosensitive screens exposure followed by a scanning step at the laboratory in a small-size device) neither involves nuclear material transportation, neither produces wastes, nor requires operators' presence during signal acquisition. The purpose is to accurately locate possible contamination spots, in order to relevantly perform targeted sampling and thus limit destructive analyses runs at the laboratory. In the latest developments, additional methods were implemented to analyze various nuclear samples (wastes, blocks, rubbles, pieces of furniture, drilled cores...) through this technique, to preliminary check for contamination, and to evaluate contamination location, homogeneity, and activity. These methods have proven themselves relevant and useful to build appropriate analyses and optimized decontamination protocols at the LASE (Laboratory of Analyses and Operators' Support). In this paper, we propose a new autoradiographic tool providing the identification of the contaminating radionuclide of a sample or an area, based on the stacking of several screens. The decrease of the signal screen after screen could be considered specific to one radionuclide. Modeling results obtained through Monte Carlo N-Particle transport code (MCNP) were in excellent agreement with experimental results obtained with sealed sources. Moreover, a method was developed to scan all the screens in the stack in only one run (instead of as many runs as screens) to shorten analysis duration. In the case of non-penetrating radiations (α particles, 3 H- or

  12. Natural and anthropogenic radionuclide activity concentrations in the New Zealand diet

    International Nuclear Information System (INIS)

    Pearson, Andrew J.; Gaw, Sally; Hermanspahn, Nikolaus; Glover, Chris N.

    2016-01-01

    To support New Zealand's food safety monitoring regime, a survey was undertaken to establish radionuclide activity concentrations across the New Zealand diet. This survey was undertaken to better understand the radioactivity content of the modern diet and also to assess the suitability of the current use of milk as a sentinel for dietary radionuclide trends. Thirteen radionuclides were analysed in 40 common food commodities, including animal products, fruits, vegetables, cereal grains and seafood. Activity was detected for 137 Caesium, 90 Strontium and 131 Iodine. No other anthropogenic radionuclides were detected. Activity concentrations of the three natural radionuclides of Uranium and the daughter radionuclide 210 Polonium were detected in the majority of food sampled, with a large variation in magnitude. The maximum activity concentrations were detected in shellfish for all these radionuclides. Based on the established activity concentrations and ranges, the New Zealand diet contains activity concentrations of anthropogenic radionuclides far below the Codex Alimentarius guideline levels. Activity concentrations obtained for milk support its continued use as a sentinel for monitoring fallout radionuclides in terrestrial agriculture. The significant levels of natural and anthropogenic radionuclide activity concentrations detected in finfish and molluscs support undertaking further research to identify a suitable sentinel for New Zealand seafood monitoring. - Highlights: • A radionuclide monitoring program was undertaken across the New Zealand food supply. • 40 food types were analysed for 13 radionuclides. • 137 Cs was present in 15% of foods (range: 0.05–0.44Bq/kg). • Anthropogenic radionuclides displayed compliance with international limits. • 210 Po, 234 U and 238 U were present in most foods with large ranges of activities.

  13. Monte Carlo simulation of different positron emitting radionuclides incorporated in a soft tissue volume

    Energy Technology Data Exchange (ETDEWEB)

    Olaya D, H.; Martinez O, S. A. [Universidad Pedagogica y Tecnologica de Colombia, Grupo de Fisica Nuclear Aplicada y Simulacion, Av. Central del Norte 39-115, 150003 Tunja, Boyaca (Colombia); Sevilla M, A. C. [Universidad Nacional de Colombia, Departamento de Fisica, Grupo CRYOMAG, 111321 Bogota D. C. (Colombia); Vega C, H. R., E-mail: grupo.finuas@uptc.edu.co [Universidad Autonoma de Zacatecas, Unidad Academica de Estudios Nucleares, Cipres No. 10, Fracc. La Penuela, 98060 Zacatecas, Zac. (Mexico)

    2015-10-15

    Monte Carlo calculations were carried out where compounds with positron-emitters radionuclides, like FDG ({sup 18}F), Acetate ({sup 11}C), and Ammonium ({sup 13}N), were incorporated into a soft tissue volume, in the aim to estimate the type of particles produced their energies, their mean free paths, and the absorbed dose at different distances with respect to the center of the volume. The volume was modeled with a radius larger than the maximum range of positrons in order to produce 0.511 keV annihilation gamma-ray photons. With the obtained results the equivalent dose, in various organs and tissues able to metabolize different radiopharmaceutical drugs, can be estimated. (Author)

  14. The relative effectiveness of inhaled alpha- and beta-emitting radionuclides in producing lung cancer

    International Nuclear Information System (INIS)

    Boecker, B.B.; Hahn, F.F.; Muggenburg, B.A.; Guilmetter, R.A.; Griffith, W.C.; McClellan, R.O.

    1988-01-01

    Proper assessment of a long-term human health risks associated with inhaled radionuclides requires knowledge of dose to critical cells and tissues and relationships between dose and effect for different biological end points. Results from epidemiological studies of exposed human populations provided important information for such assessments. However, because the types of exposures are limited, these results need to be supplemented with more detailed information on dosimetry and biological effects available through studies in laboratory animals and in vitro systems. To provide health risk information for inhaled fission product and actinide aerosols, life-span studies are being conducted using beagle dogs and other species at the Lovelace Inhalation Toxicology Research Institute (ITRI). Results of two life-span studies in dogs involving inhalation of the beta emitter 91 Y in fused aluminosilicate particles or the alpha emitter 239 PuO 2 are reported here

  15. Induction of cancers in the rat after inhalation of alpha-emitting radionuclides

    International Nuclear Information System (INIS)

    Morin, M.; Nenot, J.C.; Masse, R.; Nolibe, D.; Metivier, H.; Lafuma, J.

    1976-01-01

    Experiments have been conducted for several years on the toxic action of inhaled alpha-emitters on laboratory rats. The inhaled radionuclides were 239 Pu, 238 Pu and 241 Am in oxide and nitrate form. The initial alveolar activities varied to give total activities ranging from 1 to 200 thousand million alpha-particles per gram of lung. Variations, depending on the physico-chemical form of the nuclides, in the space and time distributions of the dose are observed. The influence of the two parameters on life span reduction, latency time and frequency of cancer occurrence, initial location of tumours and their histological types were studied. A theoretical model relating the cancerogenous effect to the dose is compared with experimental data. (author)

  16. Atmospheric transport of radionuclides emitted due to wildfires near the Chernobyl Nuclear Power Plant in 2015

    Science.gov (United States)

    Evangeliou, Nikolaos; Zibtsev, Sergey; Myroniuk, Viktor; Zhurba, Marina; Hamburger, Thomas; Stohl, Andreas; Balkanski, Yves; Paugam, Ronan; Mousseau, Timothy A.; Møller, Anders P.; Kireev, Sergey I.

    2016-04-01

    In 2015, two major fires in the Chernobyl Exclusion Zone (CEZ) have caused concerns about the secondary radioactive contamination that might have spread over Europe. The total active burned area was estimated to be about 15,000 hectares, of which 9000 hectares burned in April and 6000 hectares in August. The present paper aims to assess, for the first time, the transport and impact of these fires over Europe. For this reason, direct observations of the prevailing deposition levels of 137Cs and 90Sr, 238Pu, 239Pu, 240Pu and 241Am in the CEZ were processed together with burned area estimates. Based on literature reports, we made the conservative assumption that 20% of the deposited labile radionuclides 137Cs and 90Sr, and 10% of the more refractory 238Pu, 239Pu, 240Pu and 241Am, were resuspended by the fires. We estimate that about 10.9 TBq of 137Cs, 1.5 TBq of 90Sr, 7.8 GBq of 238Pu, 6.3 GBq of 239Pu, 9.4 GBq of 240Pu and 29.7 GBq of 241Am were released from both fire events. These releases could be classified as of "Level 3" on the relative INES (International Nuclear Events Scale) scale, which corresponds to a serious incident, in which non-lethal deterministic effects are expected from radiation. To simulate the dispersion of the resuspended radionuclides in the atmosphere and their deposition onto the terrestrial environment, we used a Lagrangian dispersion model. Spring fires redistributed radionuclides over the northern and eastern parts of Europe, while the summer fires also affected Central and Southern Europe. The more labile elements escaped more easily from the CEZ and then reached and deposited in areas far from the source, whereas the larger refractory particles were removed more efficiently from the atmosphere and thus did mainly affect the CEZ and its vicinity. For the spring 2015 fires, we estimate that about 80% of 137Cs and 90Sr and about 69% of 238Pu, 239Pu, 240Pu and 241Am were deposited over areas outside the CEZ. 93% of the labile and 97% of

  17. The assessment of low-level contamination from gamma-emitting radionuclides

    International Nuclear Information System (INIS)

    Gray, P.W.

    1989-01-01

    The objective of this research was to evaluate a new analytical technique to improve the radionuclide activity estimate from area measurements of small-area spectral peaks obtained using multi-channel spectrometry. These improvements are based on the application of Bayesian peak fitting, a method of peak fitting that allows the information contained in a spectrum to be used more fully than is possible with the method of gross counting currently employed. The study carried out showed that activity estimates and confidence intervals for activity could be more precisely defined, and the time-related costs reduced up to 50% when making activity measurements by the peak-fitting method (for a fixed detection limit) instead of gross counting. Testing of the method under real conditions would be the logical follow-up to the work achieved

  18. Field studies about radionuclide migration natural analogues and faults in clays

    International Nuclear Information System (INIS)

    Williams, G.M.; Hooker, P.J.; Brightman, M.A.

    1990-01-01

    This report puts together final reports of CEC contracts about the following topics: in situ determination of the effects of organics on the mobility of radionuclides in controlled conditions of groundwater flow (Drigg site); natural analogue studies of radionuclide migration (Loch Lomond, Broubster, Needle's Eye); faults in clays: their detection and characterization (Down Ampney site)

  19. Incorporation monitoring, above all for naturally occuring radionuclides; Inkorporationsueberwachung, vor allem bei natuerlichen radioaktiven Stoffen

    Energy Technology Data Exchange (ETDEWEB)

    Breustedt, Bastian [Karlsruher Institut fuer Technologie (KIT), Eggenstein-Leopoldshafen (Germany). Inst. fuer Strahlenforschung; Buchholz, Werner [Bundesamt fuer Strahlenschutz, Oberschleissheim (Germany). FB Strahlenschutz und Gesundheit; Burow, Mechthild [Forschungszentrum Juelich GmbH (Germany). Geschaeftsbereich ' ' Sicherheit und Strahlenschutz' ' ; and others

    2017-08-01

    The contribution of the main topic deals with further development of ICRP-models and standardization of regulations in the field of incorporation monitoring. Natural radionuclides, medically used radionuclides and quality assurance, will be discussed. The planning and realization of a shielding chamber for a whole body counter is presented.

  20. Content of naturally occurring radionuclides in samples taken from world historical sites

    International Nuclear Information System (INIS)

    Nikolic, J.; Jankovic, M.; Todorovic, D.; Sarap, N.

    2011-01-01

    This paper presents the results of the investigation of naturally occurring radionuclides content in different samples taken from the historical sites in Iran, China, Syria and Jordan. Samples contained different natural materials used in masonry, for making artefacts for personal use as well as water, sand and mud from the Dead sea. The aim was to ascertain the content of naturally occurring radionuclides, calculation of hazard indexes and their comparison to the values recommended and obtained in modern days materials [sr

  1. The biotic factors role in radionuclide migration of natural-vegetable complexes

    International Nuclear Information System (INIS)

    Yakushev, B.I.; Kazej, A.I.; Sak, M.M.; Kuz'mich, O.T.; Golushko, R.M.

    1992-01-01

    In Byelorussiyn from first months after the Chernobyl' accident investigation are conducting on the radionuclide de dynamics in the soil-plant-soil system. The isotope composition of soil contamination density and specific plants radioactivity are studying, the radionuclide migration dynamic through the soil profile is investigating. The data are shown on considerable reduction of the plants radioactivity (1986-91 years) in connection with the reduction in the soil contamination density with gamma-spectrum radionuclides, accounting for Ce-144, Pr-144, Ru-106, Cs-134 decay; information is done on gamma-spectrum radionuclides of organs in natural pine and meadows system. It is shown, that the radionuclides are actively absorbed by roots in a zone of the highest radionuclide concentration and are delivered into the overground plant parts, then actively are removed into environment in the breathing process. 11 refs.; 4 tabs

  2. Activity measurement and effective dose modelling of natural radionuclides in building material.

    Science.gov (United States)

    Maringer, F J; Baumgartner, A; Rechberger, F; Seidel, C; Stietka, M

    2013-11-01

    In this paper the assessment of natural radionuclides' activity concentration in building materials, calibration requirements and related indoor exposure dose models is presented. Particular attention is turned to specific improvements in low-level gamma-ray spectrometry to determine the activity concentration of necessary natural radionuclides in building materials with adequate measurement uncertainties. Different approaches for the modelling of the effective dose indoor due to external radiation resulted from natural radionuclides in building material and results of actual building material assessments are shown. Copyright © 2013 Elsevier Ltd. All rights reserved.

  3. Natural radionuclides in soil profiles surrounding the largest coal-fired power plant in Serbia

    Directory of Open Access Journals (Sweden)

    Tanić Milan N.

    2016-01-01

    Full Text Available This study evaluates the influence of the largest Serbian coal-fired power plant on radionuclide concentrations in soil profiles up to 50 cm in depth. Thirty soil profiles were sampled from the plant surroundings (up to 10 km distance and analyzed using standard methods for soil physicochemical properties and gamma ray spectrometry for specific activities of natural radionuclides (40K, 226Ra and 232Th. Spatial and vertical distribution of radionuclides was determined and analyzed to show the relations between the specific activities in the soil and soil properties and the most influential factors of natural radionuclide variability were identified. The radiological indices for surface soil were calculated and radiological risk assessment was performed. The measured specific activities were similar to values of background levels for Serbia. The sampling depth did not show any significant influence on specific activities of natural radionuclides. The strongest predictor of specific activities of the investigated radionuclides was soil granulometry. All parameters of radiological risk assessment were below the recommended values and adopted limits. It appears that the coal-fired power plant does not have a significant impact on the spatial and vertical distribution of natural radionuclides in the area of interest, but technologically enhanced natural radioactivity as a consequence of the plant operations was identified within the first 1.5 km from the power plant. [Projekat Ministarstva nauke Republike Srbije br. III43009 i br. III41005

  4. Relation of forms of compounds of heavy natural radionuclides in soils

    International Nuclear Information System (INIS)

    Arkhipov, N.P.; Fedorova, T.A.; Fevraleva, L.T.

    1986-01-01

    Results of studying forms of 238 U, 232 Th, 226 Ra, 210 Po, 210 Pb compounds in nonfertilized soils (under control) and in soils fertilized with ammophos containing increased amount of the mentioned radionuclides are given. The study was performed in main-year field experiment with sandy ashen gray soil and leached chernozemic soil. It is shown that a main share of radionuclides in nonfertilized soils is presened with tightly bound compounds and compounds bound with sesquioxide compounds. After 5 years labelled natural radionuclides introduced into the ammophos composition are in a more mobile state as compared with radionuclides in nonfertilized soil and they are presented with acid-soluble and bound with humus compound forms. Systematical application of fertilizers during along-term period results in the concentration increase of heavy natural radionuclides in soil

  5. Natural radionuclides in select matrices of terrestrial food chain around Kudankulam nuclear power station, India

    International Nuclear Information System (INIS)

    Ross, E.M.; Wesley, S.G.

    2016-01-01

    Natural radionuclides entering the food chain are mostly derived from the soil. There is a variation in soil radionuclide content in different geographic regions. Uptake of radionuclides by plants also varies from species to species and depends on many factors. Human food and animal feed derived from such regions may have varying levels of radionuclides. Intake of food/feed will be reflected in the next consumer level of the food chain. Such studies are essential around a nuclear power plant where there can be exposure from natural as well as artificial radionuclides. In this study an effort was taken to study the intake and excretion of 40 K, 226 Ra and 228 Ra levels along the soil-grass-cow pathway

  6. Naturally Occurring Radionuclides in Pottery, Ceramic and Glasswares Produced in Bangladesh

    International Nuclear Information System (INIS)

    Chowdhury, M.I.; Reaz, Rafia; Kamal, M.; Alam, M.N.; Mustafa, M.N.

    2005-01-01

    The concentrations of naturally occurring radionuclides were measured using gamma spectrometry in the finished products of pottery, glass, ceramic and tiles. Ceramic and pottery utensils, tiles, basin and glassware contained naturally occurring radionuclides. Pottery is produced from local clay materials, but ceramic, tiles, basin and glassware's are made from both local and imported raw materials. Radium and thorium radionuclides are concentrated during the making of pottery from the clay materials due to calcination. Radionuclides concentrated more in the highly calcined pottery products than the low calcined products. Glassware products contained very low quantities of radionuclides comparing with the ceramic and pottery products. Study on radioactivity in the pottery, ceramic and glassware products is important in the assessment of possible radiological hazards to human health. The knowledge is essential for the development of standards and guidelines for the use and management of these materials. (author)

  7. Direct internal dosimetry. A new way for routine incorporation monitoring of γ-emitting radionuclides

    International Nuclear Information System (INIS)

    Doerfel, H.

    1996-01-01

    The INDOS detector system offers the following advantages with respect to routine incorporation monitoring: The measurement is performed automatically and there is no need for trained staff. The measuring time is short and thus a relative large number of persons may be monitored with a relative high measuring frequency. First estimates of the individual effective dose equivalent rate are available immediately after the measurement. 1) The direct determination of the dose equivalent in principle is more precise than the conventional procedures for internal dosimetry, because (i) the retention of radionuclides in the body may be measured explicitly and (ii) the dependence of the dose equivalent on the body proportions is corrected implicitly. 2) The measuring procedure is comparable to the external dosimetry with respect to accuracy and lower limit of detection. Thus, the results of internal and external dosimetry can be summed up in an easy and reasonable manner. 3) The detector system can be installed in any building; it also can be installed as a mobile unit in a car or a container for long distance transportation by aircraft or train. 4) Last but not least, the cost for monitoring with INDOS is much lower than for the conventional monitoring procedures using whole body counters. (author)

  8. Strand breaks in plasmid DNA following positional changes of Auger-electron-emitting radionuclides

    International Nuclear Information System (INIS)

    Adelstein, S.J.; Kassis, A.I.

    1996-01-01

    The purpose of our studies is to elucidate the kinetics of DNA strand breaks caused by low-energy Auger electron emitters in close proximity to DNA. Previously we have studied the DNA break yields in plasmids after the decay of indium-111 bound to DNA or free in solution. In this work, we compare the DNA break yields in supercoiled DNA of iodine-125 decaying close to DNA following DNA intercalation, minor-groove binding, or surface binding, and at a distance form DNA. Supercoiled DNA, stored at 4 C to accumulate radiation dose from the decay of 125 I, was then resolved by gel electrophoresis into supercoiled, nicked circular, and linear forms, representing undamaged DNA, single-strand breaks, and double-strand breaks respectively. DNA-intercalated or groove-bound 125 I is more effective than surface-bound radionuclide or 125 I free in solution. The hydroxyl radical scavenger DMSO protects against damage by 125 I free in solution but has minimal effect on damage by groove-bound 125 I. (orig.)

  9. Influence of variations in dose and dose rates on biological effects of inhaled beta-emitting radionuclides

    International Nuclear Information System (INIS)

    McClellan, R.O.; Benjamin, S.A.; Boecker, B.B.; Hahn, F.F.; Hobbs, C.H.; Jones, R.K.; Lundgren, D.L.

    1976-01-01

    The biological effects of inhaled β-emitting radionuclides, 90 Y, 91 Y, 144 Ce and 90 Sr, are being investigated in beagle dogs that received single acute exposures at 12 to 14 months of age. The aerosols studied have included 91 YC1 3 , 144 CeC1 3 , 90 SrC1 2 , and 90 Y, 91 Y, 144 Ce or 90 Sr in aluminosilicate particles. Thus, 91 YCl 3 , 144 CeCl 3 and the aluminosilicate containing radionuclide particles all resulted in significant exposures to lung; 91 YC1 3 , 144 CeC1 3 an 90 SrC1 2 resulted in significant exposures to bone; 91 YC1 3 and 144 CeC1 3 resulted in significant exposures to liver. The higher initial doserate exposures have been more effective than low dose-rate exposures on a per-rad basis in producing early effects. To date ( 144 CeO 2 , it was observed that, on a μCi initial lung burden per kilogram body weight basis, mice did not develop pulmonary tumours whereas beagle dogs did. To fid out the reason for this observation mice have been repeatedly exposed by inhalation to 144 CeO 2 to maintain lung burdens of 144 Ce that resulted in radiation dose rates similar to that observed in beagle dogs. Several of the repeatedly exposed mice developed malignant pulmonary tumours. Thus, with similar dose rates and cumulative doses to the lung, mice and dogs responded in a similar manner to chronic β radiation

  10. Natural Radionuclides in Meadow and Pasture land in the Nordic countries

    DEFF Research Database (Denmark)

    Rosén, Klas; Villanueva, José - Luis Gutiérrez; Sundell-Bergman, Synnöve

    transfer for pasture land under the different conditions that prevail in the Nordic countries. The potential health hazards due to chronic ingestion of low concentrations of naturally occurring radionuclides are fairly unknown but the results of this study may provide valuable background information...... for assessing these radiation risks. The aim of this project has been to gain knowledge on the status of natural radionuclides in meadow and pasture land and in grassland plants in different Nordic countries and on the transfer of these radionuclides from soil/water to man via the milk/food chain (soil- meadow/pasture...... grass –cow-milk). Limited data are available on the mobility and the transfer of naturally occurring radionuclides in the ecosystems of the agricultural land. In addition, information concerning the concentrations in meat and dairy products is of interest for assessing exposures of humans to natural...

  11. Radionuclide releases from natural analogues of spent nuclear fuel

    International Nuclear Information System (INIS)

    Curtis, D.B.; Fabryka-Martin, J.; Dixon, P.; Aguilar, R.; Rokop, D.; Cramer, J.

    1993-01-01

    Measures of 99 Tc, 129 I, 239 Pu and U concentrations in rock samples from uranium deposits at Cigar Lake and Koongarra have been used to study processes of radionuclide release from uranium minerals. Rates of release have been immeasurably slow at Cigar Lake. At Koongarra release rates appear to have been faster, producing small deficiencies of 99 Tc, and larger ones of 129 I. The inferred differences in radionuclide release rates are consistent with expected differences in uranium mineral degradation rates produced by the differing hydrogeochemical environments at the two sites

  12. Production and Applications of Long-Lived Positron-Emitting Radionuclides

    Science.gov (United States)

    Graves, Stephen A.

    Positron emission tomography (PET) is a medical imaging modality capable of determining the in vivo spatial distribution of a biologically relevant molecule which has been labeled with a positron-emitting isotope. The use of molecules such as monoclonal antibodies and nanoparticles for therapeutic and diagnostic applications has expanded preclinically in recent years. As these larger molecules tend to have longer circulation times and slow clearance kinetics, positron-emitting isotopes with half-lives longer than conventional medical radioisotopes are required for PET applications. This dissertation details methods for the production of 51Mn (t1/2: 45.4 min), 52gMn (t1/2: 5.59 d), 64Cu (t1/2: 12.7 h), 76Br (t1/2: 16.2 h), 89Zr (t1/2: 3.27 d), and 194Au (t1/2: 38.0 h) on low-energy medical cyclotrons, including targetry considerations, radiochemical separation methods, and analysis of resulting purity. Pursuant to the production of these isotopes, several instrumentation developments have been made including implementation of an automatic nuclide identification library for gamma spectroscopy; development of methods for dead time correction and background estimation in auto-gamma counting; and the creation of a new linearly-filled Derenzo-type PET phantom. Measurement of the radioactive half-lives of 51Mn and 52gMn are presented in addition to their use in a variety of preclinical molecular imaging applications, including immunoPET, stem cell tracking, functional beta-cell mass determination, and probing the impact of isoflurane on acute pancreatic function. An analytic model of effective specific activity is formed and tested against preliminary trace metal analysis results. Measurements of excitation functions for the large-scale production of medically relevant isotopes, including 52gMn, at the Los Alamos National Laboratory Isotope Production Facility (100 MeV p+) are presented. The results described herein have enabled and informed a variety of novel

  13. Natural radionuclides in meadow and pasture land in the Nordic countries

    International Nuclear Information System (INIS)

    Rosen, K.; Gutierrez Villanueva, J.-L.; Sundell-Bergman, S.

    2012-06-01

    The amount of natural radionuclides in the environment differs between the Nordic countries as shown by previous investigations and also by this study. Agricultural areas of high natural background are predominantly found in Sweden, Southern Finland and Norway while low background areas are typical for Iceland and Denmark. Thus, this study offers possibilities for studying behaviour of natural radionuclides under different conditions such as the influence of different soil types as well as the husbandry. Furthermore the areas also enable studying environmental behaviour of radium and other natural radionuclides under seemingly steady state conditions. However, migration and accumulation of natural radionuclides in cultivated soil is complex involving various processes. Thus, a long term goal of this study was to identify the implications of some of these processes by determining the soil to plant transfer for pasture land under the different conditions that prevail in the Nordic countries. The potential health hazards due to chronic ingestion of low concentrations of naturally occurring radionuclides are fairly unknown but the results of this study may provide valuable background information for assessing these radiation risks. The aim of this project has been to gain knowledge on the status of natural radionuclides in meadow and pasture land and in grassland plants in different Nordic countries and on the transfer of these radionuclides from soil/water to man via the milk/food chain (soil- meadow/pasture grass -cow-milk). Limited data are available on the mobility and the transfer of naturally occurring radionuclides in the ecosystems of the agricultural land. In addition, information concerning the concentrations in meat and dairy products is of interest for assessing exposures of humans to natural radionuclides. Soil characteristics are known to have significant impact on the mobility and uptake of natural radionuclides. Therefore, the uptake in relation to

  14. Natural radionuclides in meadow and pasture land in the Nordic countries

    Energy Technology Data Exchange (ETDEWEB)

    Rosen, K.; Gutierrez Villanueva, J.-L.; Sundell-Bergman, S. [Swedish Univ. of Agricultural Sciences (SLU) (Sweden)] [and others

    2012-06-15

    The amount of natural radionuclides in the environment differs between the Nordic countries as shown by previous investigations and also by this study. Agricultural areas of high natural background are predominantly found in Sweden, Southern Finland and Norway while low background areas are typical for Iceland and Denmark. Thus, this study offers possibilities for studying behaviour of natural radionuclides under different conditions such as the influence of different soil types as well as the husbandry. Furthermore the areas also enable studying environmental behaviour of radium and other natural radionuclides under seemingly steady state conditions. However, migration and accumulation of natural radionuclides in cultivated soil is complex involving various processes. Thus, a long term goal of this study was to identify the implications of some of these processes by determining the soil to plant transfer for pasture land under the different conditions that prevail in the Nordic countries. The potential health hazards due to chronic ingestion of low concentrations of naturally occurring radionuclides are fairly unknown but the results of this study may provide valuable background information for assessing these radiation risks. The aim of this project has been to gain knowledge on the status of natural radionuclides in meadow and pasture land and in grassland plants in different Nordic countries and on the transfer of these radionuclides from soil/water to man via the milk/food chain (soil- meadow/pasture grass -cow-milk). Limited data are available on the mobility and the transfer of naturally occurring radionuclides in the ecosystems of the agricultural land. In addition, information concerning the concentrations in meat and dairy products is of interest for assessing exposures of humans to natural radionuclides. Soil characteristics are known to have significant impact on the mobility and uptake of natural radionuclides. Therefore, the uptake in relation to

  15. Standardization of sequential separation of naturally occurring radionuclides in drinking water

    International Nuclear Information System (INIS)

    Nair, Madhu G.; Rao, D.D.; Sathyapriya, R.S.; Sarkar, P.K.

    2012-01-01

    Human are constantly exposed to radiation originating from natural or manmade sources. The main contribution for internal dose is due to radionuclides from uranium and thorium series in drinking water. The distribution of these elements varies depending on the geological and physiological characteristics of the aquifer. With increased concern for radiological safety of public, it is necessary to evaluate the naturally occurring radionuclides in the drinking water

  16. The enrichment of natural radionuclides in oil shale-fired power plants in Estonia – The impact of new circulating fluidized bed technology

    International Nuclear Information System (INIS)

    Vaasma, Taavi; Kiisk, Madis; Meriste, Tõnis; Tkaczyk, Alan Henry

    2014-01-01

    Burning oil shale to produce electricity has a dominant position in Estonia's energy sector. Around 90% of the overall electric energy production originates from the Narva Power Plants. The technology in use has been significantly renovated – two older types of pulverized fuel burning (PF) energy production units were replaced with new circulating fluidized bed (CFB) technology. Additional filter systems have been added to PF boilers to reduce emissions. Oil shale contains various amounts of natural radionuclides. These radionuclides concentrate and become enriched in different boiler ash fractions. More volatile isotopes will be partially emitted to the atmosphere via flue gases and fly ash. To our knowledge, there has been no previous study for CFB boiler systems on natural radionuclide enrichment and their atmospheric emissions. Ash samples were collected from Eesti Power Plant's CFB boiler. These samples were processed and analyzed with gamma spectrometry. Activity concentrations (Bq/kg) and enrichment factors were calculated for the 238 U ( 238 U, 226 Ra, 210 Pb) and 232 Th ( 232 Th, 228 Ra) family radionuclides and for 40 K in different CFB boiler ash fractions. Results from the CFB boiler ash sample analysis showed an increase in the activity concentrations and enrichment factors (up to 4.5) from the furnace toward the electrostatic precipitator block. The volatile radionuclide ( 210 Pb and 40 K) activity concentrations in CFB boilers were evenly distributed in finer ash fractions. Activity balance calculations showed discrepancies between input (via oil shale) and output (via ash fractions) activities for some radionuclides ( 238 U, 226 Ra, 210 Pb). This refers to a situation where the missing part of the activity (around 20% for these radionuclides) is emitted to the atmosphere. Also different behavior patterns were detected for the two Ra isotopes, 226 Ra and 228 Ra. A part of 226 Ra input activity, unlike 228 Ra, was undetectable in the solid

  17. Radionuclide transport and retention in natural rock formations. Ruprechtov site

    International Nuclear Information System (INIS)

    Noseck, U.; Brasser, T.

    2006-05-01

    Deep geological disposal is based on a multi-barrier concept in which clay materials often play an important role as geological barriers. Detailed investigations of suitable geological analogues may lead to a better understanding of the complex interrelations between transport and sorption of radionuclides in argillaceous media under natural conditions, and especially on very long-term scales relevant for Performance assessment (PA). The Ruprechtov site was chosen because its geological and geochemical conditions are similar to sedimentary sequences which cover often potential host rocks for underground waste repositories. It is situated in the north-western part of the Czech Republic in a Tertiary basin of the Eger (Ohre) rift composed of clay and organic material (coal, lignite), with places of high uranium conentrations. With a bilateral project this site has been investigated by GRS, Germany and NRI, Czech Republic in order to identify the main mobilisation/immobilisation processes for PA-relevant elements, namely uranium. The work presented here is a continuation of the previous project phase. In this last project phase the site investigation was limited to a small area of about 200 m 3 . Three exploration boreholes and two boreholes for detailed investigation were available at that time. The main intention of the new project phase was to enlarge the investigation area, in order to better understand the structure and the hydrogeochemical conditions of the overall system. On the one hand this includes the characterisation of the hydrogeological conditions in order to understand the regional groundwater flow and potential uranium transport processes on a larger spatial scale. Therefore the spatial extension of uranium-rich layers, water-bearing horizons and lithological units as well as groundwater ages and flow directions need to be determined. On that basis a conceptual model for the groundwater flow at Ruprechtov site can be developed. On the other hand it

  18. Natural radionuclides in the environment and problems of uranium mining

    International Nuclear Information System (INIS)

    Bowie, S.H.U.

    1981-01-01

    The subject is discussed under the headings: introduction (U-238, U-235, Th-232, K-40, and their decay products); distribution of radionuclides; α, β and γ radiation; uranium in rocks; uranium in soil and water; uranium mining (hazards of uranium and radon during mining and in tailings); assessment of risk. (U.K.)

  19. Study on natural radionuclide activities in meat samples consumed in Sao Paulo City, Brazil

    International Nuclear Information System (INIS)

    Rosa, Mychelle M.L.; Taddei, Maria HelenaT.

    2015-01-01

    Consumption of food is usually the most important route by which natural and artificial radionuclides can enter the human body. An assessment of radionuclide levels in different foods and diets is therefore important to estimate the intake of these radionuclides by man. The contamination by radionuclides can occur via the food chain (soil, root, plant and animal), with emphasis to the long half-life radionuclides, which can also have their transfer through the animal meat. The inclusion of meat in human nutrition is important because it is an excellent source of high quality protein, nutrient related to construction and cell regeneration. This work aims the determination of natural radionuclides ( 234 U, 235 U, 238 U, 228 Th, 230 Th, 232 Th, 226 Ra, 228 Ra, and 210 Pb) in meat samples. Five groups of samples were analyzed, such as cattle meat (beef), fish, pork, poultry, and processed meat, after radiochemical separation followed by alpha or alpha beta spectrophotometry, and total count quantification. The determination of these radionuclides is very important because they are products of the natural decay series of 238 U and 232 Th, being easily found in meat samples. (author)

  20. Study on natural radionuclide activities in meat samples consumed in Sao Paulo City, Brazil

    Energy Technology Data Exchange (ETDEWEB)

    Rosa, Mychelle M.L.; Taddei, Maria HelenaT. [Comissao Nacional de Energia Nuclear (LAPOC/CNEN), Pocos de Caldas, MG (Brazil). Laboratorio de Pocos de Caldas; Avegliano, Roseane P.; Maihara, Vera A., E-mail: mychelle@cnen.gov.br [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP), Sao Paulo, SP (Brazil)

    2015-07-01

    Consumption of food is usually the most important route by which natural and artificial radionuclides can enter the human body. An assessment of radionuclide levels in different foods and diets is therefore important to estimate the intake of these radionuclides by man. The contamination by radionuclides can occur via the food chain (soil, root, plant and animal), with emphasis to the long half-life radionuclides, which can also have their transfer through the animal meat. The inclusion of meat in human nutrition is important because it is an excellent source of high quality protein, nutrient related to construction and cell regeneration. This work aims the determination of natural radionuclides ({sup 234}U, {sup 235}U, {sup 238}U, {sup 228}Th, {sup 230}Th, {sup 232}Th, {sup 226}Ra, {sup 228}Ra, and {sup 210}Pb) in meat samples. Five groups of samples were analyzed, such as cattle meat (beef), fish, pork, poultry, and processed meat, after radiochemical separation followed by alpha or alpha beta spectrophotometry, and total count quantification. The determination of these radionuclides is very important because they are products of the natural decay series of {sup 238}U and {sup 232}Th, being easily found in meat samples. (author)

  1. Levels and effects of natural radionuclides in soil samples of Garhwal Himalaya

    International Nuclear Information System (INIS)

    Manjulata Yadav; Mukesh Rawat; Anoop Dangwal; Mukesh Prasad; Gusain, G.S.; Ramola, R.C.

    2014-01-01

    Distribution of natural radionuclide gives significant parameter to assess the presence of gamma radioactivity and its radiological effect in our environment. Natural radionuclides are present in the form of 226 Ra, 232 Th and 40 K in soil, rocks, water, air, and building materials. Distribution of natural radionuclides depends on the type of minerals present in the soil and rocks. For this purpose gamma spectrometer is used as tool for finding the concentration of these radionuclides. The activity concentration of naturally occurring radionuclides 226 Ra, 232 Th and 40 K in these soil samples were found to vary from of 8 ± 1 Bq/kg to 50 ± 10 Bq/kg with an average 20 Bq/kg, 7 ± 1-88 ± 16 Bq/kg with an Average 26 Bq/kg and 115 ± 18-885 ± 132 Bq/kg with an average 329 Bq/kg, respectively. In this paper, we are presenting the radiological effect due to distribution of natural radionuclide present in soil of Garhwal Himalaya. (author)

  2. Natural radionuclides and toxic elements in transboundary rivers of Kazakhstan.

    Science.gov (United States)

    Solodukhin, V; Poznyak, V; Kabirova, G; Stepanov, V; Ryazanova, L; Lennik, S; Liventsova, A; Bychenko, A; Zheltov, D

    2015-06-01

    The paper reports on the study of radionuclide and elemental composition of water, bottom sediment and soil samples collected at the border areas of the following transboundary rivers in Kazakhstan: Chagan, Ural, Ilek, Tobol, Ayat, Irtysh, Emel, Ili, Tekes, Shu, Karabalta, Talas and Syrdarya. The employed analyses include the following methods: instrumental gamma-ray spectrometry, radiochemical analysis, neutron activation analysis, XRF and the inductively coupled plasma mass spectrometry (ICP-MS). Evidence of water environment contamination with radionuclides and toxic elements has been revealed in many of the studied rivers both in Kazakhstan and in adjacent countries. Transboundary transfer of the contaminants is most likely related to local industry (uranium mining and processing) and the presence of radioactive substances in the river basins. © The Author 2015. Published by Oxford University Press. All rights reserved. For Permissions, please email: journals.permissions@oup.com.

  3. Natural-series radionuclides in traditional North Australian aboriginal foods

    International Nuclear Information System (INIS)

    Murray, A.S.; Johnston, A.; Hancock, G.J.; Martin, P.

    1997-01-01

    Activity concentrations of the radionuclides 226 Ra, 210 Pb, 210 Po, 238 U, 234 U, 230 Th, 232 Th and 227 Ac were measured in edible flesh of traditional Aboriginal food items from the Magela and Cooper Creek systems in the tropical Northern Territory of Australia. Fish, buffalo, pig, magpie goose, filesnake, goanna, turtle, freshwater shrimp and freshwater crocodile were studied. Activity concentrations in water were also measured to enable the calculation of concentration ratios (CRs).For most edible flesh samples, activity concentrations followed the approximate order: 210 Po>> 226210 [ 234 Usimilar 238 [ 230 Thsimilar 232 Th]. The 210 Po/ 210 Pb activity ratio was particularly high (greater than 100) for pig flesh. CRs for fish species fall into two groups. Group 1 (bony bream and sleepy cod) had CRs about five times higher than for group 2 (eight other species). CRs for turtle flesh were similar to those for fish in group 1, while those for turtle liver were about a factor of 10 higher. CRs for magpie goose, filesnake, freshwater shrimp, goanna and crocodile flesh were also of the same order as for fish in groups 1 or 2.Calculations of dose resulting from release of wastewaters from uranium mining operations in the region show that the dominant pathway would be uptake of radionuclides, especially 226 Ra, by freshwater mussels, followed by radionuclide uptake by fish. (Copyright (c) 1997 Elsevier Science B.V., Amsterdam. All rights reserved.)

  4. Partitioning behaviour of natural radionuclides during combustion of coal in thermal power plants

    International Nuclear Information System (INIS)

    Sahu, S.K.; Tiwari, M.; Bhangare, R.C.; Ajmal, P.Y.; Pandit, G.G.

    2014-01-01

    All fossil fuels contain low levels of naturally occurring radioactive substances. The environmental impact of radionuclide-containing waste products from coal combustion is an important issue. These radionuclides vaporize in the hot portions of the coal combustor and then return to the solid phase in cooler downstream zones. Indian coal used in power plants generally has high ash yield (35-45%) and is of low quality. In the burning process of coal, minerals undergo thermal decomposition, fusion, disintegration, and agglomeration. A major portion of elements in the boiler enter into slag or bottom ash, and the rest of the inorganic materials find their way into the flue gas, in fly ash or vapor. Fly and bottom ash are significant sources of exposure to these radionuclides. In the present study, coal and ash samples collected from six thermal power stations were analyzed to determine their natural radioactivity content and the partitioning behavior of these radionuclides was carried out by tracing their activities in fly and bottom ashes. The partitioning of radionuclides is strongly dependent on the size of associated ash particle. Polonium-210 was mostly associated with the finest fraction and showed large variation with particle size whereas 232 Th showed least dependence on the particle size. The high activities of all radionuclides in fly ashes than that of bottom ashes thus may be due to strong affinity of the nuclides towards the finer particle fractions. All the radionuclide distribution favored small particle sizes

  5. Removal of natural radionuclides from drinking water from private wells in Finland

    International Nuclear Information System (INIS)

    Huikuri, Pia; Salonen, Laina; Turtiainen, Tuukka

    1999-01-01

    Removal of natural radionuclides is often necessary in Finland when household water is taken from a drilled well. Removal of radionuclides by various methods from Finnish groundwaters were studied in a EU-research project, TENAWA. The results indicated that radon can be removed very efficiently (up to 99%) by applying aeration or granular activated carbon (GAC) filtration. Uranium and radium were also removed (over 94%) by using strong base anion (SBA) and strong acid cation (SAC) resins. The capability of reverse osmosis (RO) equipment to remove radionuclides was over 90% for uranium, radium and polonium. The water quality analyses indicated that water quality remained mostly good during the water treatment. (au)

  6. The enrichment behavior of natural radionuclides in pulverized oil shale-fired power plants

    International Nuclear Information System (INIS)

    Vaasma, Taavi; Kiisk, Madis; Meriste, Tõnis; Tkaczyk, Alan Henry

    2014-01-01

    The oil shale industry is the largest producer of NORM (Naturally Occurring Radioactive Material) waste in Estonia. Approximately 11–12 million tons of oil shale containing various amounts of natural radionuclides is burned annually in the Narva oil shale-fired power plants, which accounts for approximately 90% of Estonian electricity production. The radionuclide behavior characteristics change during the fuel combustion process, which redistributes the radionuclides between different ash fractions. Out of 24 operational boilers in the power plants, four use circulating fluidized bed (CFB) technology and twenty use pulverized fuel (PF) technology. Over the past decade, the PF boilers have been renovated, with the main objective to increase the efficiency of the filter systems. Between 2009 and 2012, electrostatic precipitators (ESP) in four PF energy blocks were replaced with novel integrated desulphurization technology (NID) for the efficient removal of fly ash and SO 2 from flue gases. Using gamma spectrometry, activity concentrations and enrichment factors for the 238 U ( 238 U, 226 Ra, 210 Pb) and 232 Th ( 232 Th, 228 Ra) family radionuclides as well as 40 K were measured and analyzed in different PF boiler ash fractions. The radionuclide activity concentrations in the ash samples increased from the furnace toward the back end of the flue gas duct. The highest values in different PF boiler ash fractions were in the last field of the ESP and in the NID ash, where radionuclide enrichment factors were up to 4.2 and 3.3, respectively. The acquired and analyzed data on radionuclide activity concentrations in different PF boiler ashes (operating with an ESP and a NID system) compared to CFB boiler ashes provides an indication that changes in the fuel (oil shale) composition and boiler working parameters, as well as technological enhancements in Estonian oil shale fired power plants, have had a combined effect on the distribution patterns of natural radionuclides in

  7. The Palmottu natural analogue project. Progress report 1996. The behaviour of natural radionuclides in and around uranium deposits, Nr. 10

    International Nuclear Information System (INIS)

    Lampinen, P.; Ruskeeniemi, T.; Blomqvist, R.

    1997-01-01

    The report summarises the activities carried out in the Palmottu Natural Analogue project in 1996. Efforts has mainly been directed toward the hydrogeological and hydrogeochemical studies of the site. Other activities in 1996 have included up-dating the structural model of the site and radionuclide migration studies. The topical summaries documented are: (1) Hydrogeological studies, (2) Up-dating the structural model of the site, (3) Hydrogeochemical studies at Palmottu, and (4) Radionuclide migration studies. (41 refs.)

  8. Natural radionuclides in an eucalyptus forest located in the south of Spain

    International Nuclear Information System (INIS)

    Vaca, F.; Manjon, G.; Garcia-Leon, M.

    2001-01-01

    Eucalyptus forests can be considered as the main source of raw material for the pulp industry of Spain. This environment was selected for a radioactivity study because natural and artificial radionuclides can be transferred into the pulp mills, associated with raw material, wood and barks, where they are concentrated by industrial processes, becoming a cause of doses. Radionuclide concentration of natural radionuclides ( 238 U, 234 U, 228 Th, 230 Th, 232 Th) were determined by alpha- and gamma-spectrometry. Well-established radiochemical procedures were applied to environmental samples in order to isolate these radionuclides. A comparison between 228 Th activity, determined by gamma-spectrometry, and 232 Th activity, determined by alpha-spectrometry, was used as quality control parameter for analyses. The concentration factors were finally evaluated from experimental data.

  9. Naturally occurring radionuclides in pasture soil, feed ingredients and milk of dairy cattle

    Energy Technology Data Exchange (ETDEWEB)

    Turtiainen, T.; Kostiainen, E.; Solatie, D. [STUK-Radiation and Nuclear Safety Authority (Finland)

    2014-07-01

    Naturally occurring radionuclides are generally considered being respective part of the environment and hence no statutory monitoring of their levels are required in food products. Therefore, limited data are available on the naturally occurring radionuclides in food. Dairy products constitute a significant portion of Finnish diet (400-500 g/d) and hence it is reasonable to study radionuclide levels in milk in more detail. Contrary to caesium, strontium and iodine, few transfer coefficients are available in the literature for naturally occurring radionuclide transfer to cow's milk. The renaissance of mining industry in Finland has raised a question among the public about the baseline values of naturally occurring radionuclides in Finnish agricultural products. The objective of this study was to investigate naturally occurring radionuclides in the components of dairy cattle diet and milk and calculate their transfer to milk. This information is needed for regulating the permitted discharges to the environment and for setting up monitoring programs if any unplanned discharges are released. In modern dairy farming, cattle are fed a precise diet in order to maximize milk production and quality and to achieve cost-effectiveness. Therefore, several different components are found in dairy cattle's diet and pasture grass concentrations are not sufficient for calculating radionuclide transfer to cow's milk. In this study, we carried out comprehensive sampling at four dairy farms each representing different areas of natural radiation background. The pasture soils were characterized and measured for natural radioactivity. Samples were taken from cattle's total diet (including e.g. pasture grass, water, silage, mineral forage) and milk. Document available in abstract form only. (authors)

  10. Environmental methodology. Sampling and preparing fresh water organisms. Measuring of emitting radionuclides

    International Nuclear Information System (INIS)

    Foulquier, Luc; Philippot, J.C.; Baudin-Jaulent, Yvette.

    1982-05-01

    This paper provides some initial responses to questions asked by users of radioecological documents. By using aquatic plants and fish drawn ''in situ'' the authors' results often reveal very low activity levels; they make a point of knowing how to deal with such levels, since the fundamental objective is to interpret transfer mechanisms. The establishment of the environmental level of radioactivity requires that the write-ups produced demonstrate the use of reproducible methods, and contain results for which the extent of reliability is clearly specified. Aquatic plants and fish are, among all fresh water organisms, the most interesting links in the study of artificial and natural radioactivity. By systematically using concrete examples, this work reaffirms the precautions that should be taken in a site study. Once the objective is clearly defined, the properties to give to the sampling can be specified [fr

  11. Radiotherapy Based On α Emitting Radionuclides: Geant4 For Dosimetry And Micro-/Nano-Dosimetry

    International Nuclear Information System (INIS)

    Guatelli, Susanna

    2013-01-01

    Possible physics approaches to evaluate the efficacy of TAT are dosimetry, microdosimetry and nanodosimetry. Dosimetry is adequate when mean absorbed dose to a macroscopic target volume is important to understand the biological effect of radiation. General purpose Monte Carlo (MC) codes, based on condensed history approach, are a very useful, cost effective tool to solve dosimetric problems. The condensed history approach is based on the use of multiple scattering theories to calculate the energy losses and angular changes in the direction of the particle. The short α particle range and high LET make the microdosimetric approach more suitable than dosimetry to study TAT from first physics principles, as this approach takes into account the stochastic nature of energy deposition at cellular level

  12. A survey of natural terrestrial and airborne radionuclides in moss samples from the peninsular Thailand.

    Science.gov (United States)

    Wattanavatee, Komrit; Krmar, Miodrag; Bhongsuwan, Tripob

    2017-10-01

    The aim of this study was to determine the activity concentrations of natural terrestrial radionuclides ( 238 U, 226 Ra, 232 Th and 40 K) and airborne radionuclides ( 210 Pb, 210 Pb ex and 7 Be) in natural terrestrial mosses. The collected moss samples (46) representing 17 species were collected from 17 sampling localities in the National Parks and Wildlife Sanctuaries of Thailand, situated in the mountainous areas between the northern and the southern ends of peninsular Thailand (∼7-12 °N, 99-102 °E). Activity concentrations of radionuclides in the samples were measured using a low background gamma spectrometer. The results revealed non-uniform spatial distributions of all the radionuclides in the study area. Principal component analysis and cluster analysis revealed two distinct origins for the studied radionuclides, and furthermore, the Pearson correlations were strong within 226 Ra, 232 Th, 238 U and 40 K as well as within 210 Pb and 210 Pb ex , but there was no significant correlation between these two groups. Also 7 Be was uncorrelated to the others, as expected due to different origins of the airborne and terrestrial radionuclides. The radionuclide activities of moss samples varied by moss species, topography, geology, and meteorology of each sampling area. The observed abnormally high concentrations of some radionuclides probably indicate that the concentrations of airborne and terrestrial radionuclides in moss samples were directly related to local geological features of the sampling site, or that high levels of 7 Be were most probably linked with topography and regional NE monsoonal winds from mainland China. Copyright © 2017 Elsevier Ltd. All rights reserved.

  13. Natural radionuclides in effluents release by a deactivated uranium mine

    Energy Technology Data Exchange (ETDEWEB)

    Pereira, Wagner S.; Kelecom, Alphonse; Silva, Ademir X.; Lopes, José M.; Pinto, Carlos E.C.; Py Júnior, Delcy A.; Antunes, Marcos M., E-mail: pereiraws@gmail.com, E-mail: caerjbr@gmail.com, E-mail: wspereira@inb.gov.br, E-mail: delcy@inb.gov.br, E-mail: Antunes@inb.gov.br, E-mail: lararapls@hotmail.com, E-mail: Ademir@nuclear.ufrj.br, E-mail: marqueslopes@yahoo.com.br [Universidade Veiga de Almeida (UVA), Rio de Janeiro, RJ (Brazil); Indústrias Nucleares do Brasil (COMAP.N/FCN/INB), Resende RJ (Brazil). Fábrica de Combustível Nuclear. Coordenação de Meio Ambiente e Proteção Radiológica Ambiental; Universidade Federal Fluminense (LARARA-PLS/UFF), Niterói, RJ (Brazil). Laboratório de Radiobiologia e Radiometria; Coordenacao de Pos-Graduacao e Pesquisa de Engenharia (COPPE/UFRJ), Rio de Janeiro, RJ (Brazil). Programa de Engenharia Nuclear

    2017-07-01

    The Ore Treatment Unit (OTU) is a mine and deactivated uranium plant in the city of Caldas, Minas Gerais, Brazil. This facility possesses three points of release of liquid effluents containing radionuclides: point 014, 025 and 076. At these points, the values of activity concentrations (AC) of the radionuclides U{sub nat}, {sup 226}Ra, {sup 210}Pb, {sup 232}Th and {sup 228}Ra were analyzed in 2012. The evaluation of point 014 by univariate statistics pointed four groups. [U{sub nat} > {sup 228}Ra > ({sup 226}Ra = {sup 210}Pb) >{sup 232}Th]. The multivariate statistics separated the radionuclides into two groups: [(U{sub nat} and {sup 232}Th) and ({sup 226}Ra, {sup 228}Ra and {sup 210}Pb)]. At point 025, the univariate statistics described three groups: [Un{sub at} > ({sup 228}Ra = {sup 210}Pb) > ({sup 226}Ra = {sup 232}Th)] and the multivariate analysis also described three but different groups: [(U{sub nat} and {sup 228}Ra), ({sup 226}Ra and {sup 210}Pb) and {sup 232}Th]. In turn, point 076 showed another behavior. The univariate analysis showed only two groups: [(U{sub nat}) > ({sup 226}Ra, {sup 228}Ra, {sup 210}Pb, {sup 232}Th)]. Differently, the multivariate statistics defined three groups: [(U{sub nat} and {sup 232}Th), ({sup 226}Ra and {sup 228}Ra) and {sup 210}Pb].Thus, statistical analysis showed that each point has releases of effluents with different characteristics. Both the behaviors of releases, based on multivariate statistics, and of the AC magnitudes, based on the univariate statistics, are different between the points. The only common features were the greater magnitude of uranium and the smaller magnitude of thorium. (author)

  14. Natural-series radionuclides in traditional North Australian aboriginal foods

    Energy Technology Data Exchange (ETDEWEB)

    Murray, A.S.; Johnston, A.; Hancock, G.J.; Martin, P. [Environmental Research Institute of the Supervising Scientist (ERISS), Jabiru (Australia)

    1997-07-01

    Activity concentrations of the radionuclides {sup 226}Ra, {sup 210}Pb, {sup 210}Po, {sup 238}U, {sup 234}U, {sup 230}Th, {sup 232}Th and {sup 227}Ac were measured in edible flesh of traditional Aboriginal food items from the Magela and Cooper Creek systems in the tropical Northern Territory of Australia. Fish, buffalo, pig, magpie goose, filesnake, goanna, turtle, freshwater shrimp and freshwater crocodile were studied. Activity concentrations in water were also measured to enable the calculation of concentration ratios (CRs).For most edible flesh samples, activity concentrations followed the approximate order: {sup 210}Po>>{sup 226210}[{sup 234}Usimilar{sup 238}[{sup 230}Thsimilar{sup 232}Th]. The {sup 210}Po/{sup 210}Pb activity ratio was particularly high (greater than 100) for pig flesh. CRs for fish species fall into two groups. Group 1 (bony bream and sleepy cod) had CRs about five times higher than for group 2 (eight other species). CRs for turtle flesh were similar to those for fish in group 1, while those for turtle liver were about a factor of 10 higher. CRs for magpie goose, filesnake, freshwater shrimp, goanna and crocodile flesh were also of the same order as for fish in groups 1 or 2.Calculations of dose resulting from release of wastewaters from uranium mining operations in the region show that the dominant pathway would be uptake of radionuclides, especially {sup 226}Ra, by freshwater mussels, followed by radionuclide uptake by fish. (Copyright (c) 1997 Elsevier Science B.V., Amsterdam. All rights reserved.)

  15. Distribution of natural radionuclide in soil of Ukhimath region of Garhwali Himalaya and its radiological implications

    International Nuclear Information System (INIS)

    Yadav, Manjulata; Rawat, Mukesh; Prasad, Mukesh; Dangwal, Anoop; Gusain, G.S.; Ramola, R.C.

    2014-01-01

    The naturally occurring radionuclides present in soil include 226 Ra, 232 Th and 40 K some of these radionuclides are transferred to man through food chain or inhalations, while the extraterrestrial radiation originate from outer space as primary cosmic rays. External exposure will occur as a result of irradiation, and internal exposure will occurs as result of inhalation. Therefore, the assessment of gamma radiations dose from natural sources is of particular importance as natural radiation is the largest contributor to the external dose of world population

  16. Radioactivity in papers: the concentration and source of naturally occurring radionuclides

    International Nuclear Information System (INIS)

    Kobashi, Asaya

    2005-01-01

    The radioactivities of naturally occurring radionuclides ( 226 Ra, 228 Ra, 228 Th and 40 K) in papers such as magazines, newspapers, and copying papers produced in Japan were determined by gamma-ray spectrometry to obtain information on radioactivity level of papers. The X-ray diffraction measurement of the samples was also carried out to elucidate the source of radionuclides contained in them. The average 226 Ra, 228 Ra, 228 Th, and 40 K contents of pocket-sized books were 6.4, 21.5, 23.7, and 18.8 Bq kg -1 , respectively, and those of other kinds of samples were near to or less than the values. The 228 Th content was generally somewhat higher than the 228 Ra content. Possibly 228 Ra was leached from the raw materials of the papers to water during their production in preference to 228 Th. The concentrations of the naturally occurring radionuclides were correlated to each other. The X-ray diffraction study showed that kaolinite, talc, and calcite were contained in the papers. The kaolinite content of the samples was correlated to the concentrations of the naturally occurring radionuclides, indicating that the naturally occurring radionuclides in the paper samples were mainly brought with kaolinite used as filler or coating pigment in the papers. The regression analysis of the data showed that the natural radioactivity content of filler kaolinite was higher than that of pigment kaolinite. (author)

  17. Measurement of natural radionuclides in U.K. diet.

    Science.gov (United States)

    Smith-Briggs, J L; Bradley, E J

    1984-05-01

    The levels of radium-226, lead-210 and polonium-210 in the U.K. diet have been determined. The important food groups contributing to the intake of these radionuclides have been identified. Seventy-five percent of the daily intake of radium-226 is derived from beverages, cereals, other vegetables, bread, sugars and preserves. Seventy-five percent of the intake of lead-210 and polonium-210 is derived from bread, milk, cereals, beverages, other vegetables, sugars and preserves, and meat products. The average daily intakes of these radionuclides are tentatively calculated to be 30 mBq for radium-226 and 82 mBq for both lead-210 and polonium-210. These levels are compared with data from other countries. The annual effective dose equivalents resulting from the intakes are approximately 3 muSv for radium-226 and 54 muSv from lead-210 and polonium-210 together. The differences between these doses and other current estimates are discussed.

  18. Natural radionuclides in effluents release by a deactivated uranium mine

    International Nuclear Information System (INIS)

    Pereira, Wagner S.; Kelecom, Alphonse; Silva, Ademir X.; Lopes, José M.; Pinto, Carlos E.C.; Py Júnior, Delcy A.; Antunes, Marcos M.; Indústrias Nucleares do Brasil; Universidade Federal Fluminense; Coordenacao de Pos-Graduacao e Pesquisa de Engenharia

    2017-01-01

    The Ore Treatment Unit (OTU) is a mine and deactivated uranium plant in the city of Caldas, Minas Gerais, Brazil. This facility possesses three points of release of liquid effluents containing radionuclides: point 014, 025 and 076. At these points, the values of activity concentrations (AC) of the radionuclides U_n_a_t, "2"2"6Ra, "2"1"0Pb, "2"3"2Th and "2"2"8Ra were analyzed in 2012. The evaluation of point 014 by univariate statistics pointed four groups. [U_n_a_t > "2"2"8Ra > ("2"2"6Ra = "2"1"0Pb) >"2"3"2Th]. The multivariate statistics separated the radionuclides into two groups: [(U_n_a_t and "2"3"2Th) and ("2"2"6Ra, "2"2"8Ra and "2"1"0Pb)]. At point 025, the univariate statistics described three groups: [Un_a_t > ("2"2"8Ra = "2"1"0Pb) > ("2"2"6Ra = "2"3"2Th)] and the multivariate analysis also described three but different groups: [(U_n_a_t and "2"2"8Ra), ("2"2"6Ra and "2"1"0Pb) and "2"3"2Th]. In turn, point 076 showed another behavior. The univariate analysis showed only two groups: [(U_n_a_t) > ("2"2"6Ra, "2"2"8Ra, "2"1"0Pb, "2"3"2Th)]. Differently, the multivariate statistics defined three groups: [(U_n_a_t and "2"3"2Th), ("2"2"6Ra and "2"2"8Ra) and "2"1"0Pb].Thus, statistical analysis showed that each point has releases of effluents with different characteristics. Both the behaviors of releases, based on multivariate statistics, and of the AC magnitudes, based on the univariate statistics, are different between the points. The only common features were the greater magnitude of uranium and the smaller magnitude of thorium. (author)

  19. Relative contributions of natural and waste-derived organics to the subsurface transport of radionuclides

    International Nuclear Information System (INIS)

    Toste, A.P.; Myers, R.B.

    1985-06-01

    Our laboratory is studying the role of organic compounds in the subsurface transport of radionuclides at shallow-land burial sites of low-level nuclear waste, including a commercial site at Maxey Flats, Kentucky, and an aqueous waste disposal site. At the Maxey Flats site, several radionuclides, notably Pu and 60 Co, appear to exist as anionic, organic complexes. Waste-derived organics, particularly chelating agents such as EDTA, HEDTA and associated degradation products (e.g., ED3A), are abundant in aqueous waste leachates and appear to account for the complexation. EDTA, and probably other waste-derived chelating agents as well, are chelated to the Pu and 60 Co in the leachates, potentially mobilizing these radionuclides. In contrast, at the low-level aqueous waste disposal site, naturally-occurring organics, ranging from low molecular weight (MW) acids to high MW humic acids, account for the bulk of the groundwater's organic content. Certain radionuclides, notably 60 Co, 103 Ru and 125 Sb, are mobile as anionic complexes. These radionuclides are clearly associated with higher MW organics, presumably humic and fulvic acids with nominal MW's > 1000. It is clear, therefore, that naturally-occurring organics may play an important role in radionuclide transport, particularly at nuclear waste burial sites containing little in the way of waste-derived organics

  20. Distribution of natural and artificial radionuclides in chernozem soil/crop system from stationary experiments.

    Science.gov (United States)

    Sarap, Nataša B; Rajačić, Milica M; Đalović, Ivica G; Šeremešić, Srđan I; Đorđević, Aleksandar R; Janković, Marija M; Daković, Marko Z

    2016-09-01

    The present paper focuses on the determination of radiological characteristics of cultivated chernozem soil and crops from long-term field experiments, taking into account the importance of distribution and transfer of radionuclides in the soil-plant system, especially in agricultural cropland. The investigation was performed on the experimental fields where maize, winter wheat, and rapeseed were cultivated. Analysis of radioactivity included determination of the gross alpha and beta activity as a screening method, as well as the activities of the following radionuclides: natural ((210)Pb, (235)U, (238)U, (226)Ra, (232)Th, (40)K, (7)Be) and artificial ((90)Sr and (137)Cs). The activities of natural and artificial ((137)Cs) radionuclides were determined by gamma spectrometry, while the artificial radionuclide (90)Sr was determined by a radiochemical analytical method. Based on the obtained results for the specific activity of (40)K, (137)Cs, and (90)Sr, accumulation factors for these radionuclides were calculated in order to estimate transfer of radionuclides from soil to crops. The results of performed analyses showed that there is no increase of radioactivity that could endanger the food production through the grown crops.

  1. Distribution of anthropogenic and naturally occurring radionuclides in soils and lakes of Central Spitsbergen (Arctic)

    International Nuclear Information System (INIS)

    Lokas, Edyta

    2017-01-01

    This work provides the first results on activity concentrations, inventories and activity ratios of the artificial and natural fallout ("1"3"7Cs, "2"3"8Pu, "2"3"9"+"2"4"0Pu, "2"4"1Am, "2"1"0Pb) and lithogenic radionuclides ("2"2"6Ra, "2"2"8Ra, "4"0K) in soils and lake sediments of the inland Spitsbergen. The depths of activity peaks of the artificial radionuclides point to accumulation of up to 10 cm thick deposits during last 50 years. The activity ratios of the radionuclides suggest global fallout as their source. Despite low annual precipitation the inventories of fallout radionuclides in sites not affected by the secondary deposition agree with those reported from the more humid areas of Spitsbergen. (author)

  2. Transformation processes influencing physico-chemical forms of radionuclides and trace elements in natural water systems

    International Nuclear Information System (INIS)

    Salbu, B.; Riise, G.; Oughton, D.H.

    1995-01-01

    In order to assess short and long term consequences of radionuclides and trace elements introduced to aquatic systems, knowledge on source terms, key factors and key processes influencing the speciation is essential. The mobility, bioavailability and subsequent transfer into food chains depend on the physico-chemical forms on radionuclides and trace metals. In addition, transformation processes and especially the interaction with natural organic matter (NOM) influences the distribution pattern. Furthermore, the prevailing climate conditions, e.g. episodic events and temperature are vital for fluxes and for the kinetics of the transformation processes. In the present work processes in catchments and processes associated with acidification, episodic events, climate conditions (temperature) and mixing zone phenomena influencing the speciation of radionuclides and trace metals are highlighted. These processes should be highly relevant for assessing far field consequences of radionuclides potentially released from disposal sites. (authors). 21 refs., 8 figs., 1 tab

  3. Microbial transformations of natural organic compounds and radionuclides in subsurface environments

    International Nuclear Information System (INIS)

    Francis, A.J.

    1985-10-01

    A major national concern in the subsurface disposal of energy wastes is the contamination of ground and surface waters by waste leachates containing radionuclides, toxic metals, and organic compounds. Microorganisms play an important role in the transformation of organic compounds, radionuclides, and toxic metals present in the waste and affect their mobility in subsurface environments. Microbial processes involved in dissolution, mobilization, and immobilization of toxic metals under aerobic and anaerobic conditions are briefly reviewed. Metal complexing agents and several organic acids produced by microbial action affect mobilization of radionuclides and toxic metals in subsurface environments. Information on the persistence of and biodegradation rates of synthetic as well as microbiologically produced complexing agents is scarce but important in determining the mobility of metal organic complexes in subsoils. Several gaps in knowledge in the area of microbial transformation of naturally occurring organics, radionuclides, and toxic metals have been identified, and further basic research has been suggested. 31 refs., 1 fig., 3 tabs

  4. Natural radionuclide distribution in soils of Gudalore, India

    International Nuclear Information System (INIS)

    Selvasekarapandian, S.; Sivakumar, R.; Manikandan, N.M.; Meenakshisundaram, V.; Raghunath, V.M.; Gajendran, V.

    2000-01-01

    The concentration of primordial radionuclides in soil samples of Gudalore Taluk in the Udagamandalam district has been measured from the gamma ray spectrum of the soil. The mean activities of 232 Th, 238 U and 40 K are 75.3±44.1, 37.7±10.1 and 195.2±85.1 Bq kg -1 dry weight, respectively. The average outdoor absorbed dose rate in air at a height of 1 m above ground is 74.3±27.8 nGy h -1 , corresponding to an annual effective dose equivalent of 455.6 μSv. The dose equivalent ranges from 168.3 to 1250.5 μSv. The results have been compared with other global radioactivity measurements and evaluations

  5. Natural radionuclide distribution in soils of Gudalore, India

    Energy Technology Data Exchange (ETDEWEB)

    Selvasekarapandian, S. E-mail: spandian@bharathi.ernet.in; Sivakumar, R.; Manikandan, N.M.; Meenakshisundaram, V.; Raghunath, V.M.; Gajendran, V

    2000-02-01

    The concentration of primordial radionuclides in soil samples of Gudalore Taluk in the Udagamandalam district has been measured from the gamma ray spectrum of the soil. The mean activities of {sup 232}Th, {sup 238}U and {sup 40}K are 75.3{+-}44.1, 37.7{+-}10.1 and 195.2{+-}85.1 Bq kg{sup -1} dry weight, respectively. The average outdoor absorbed dose rate in air at a height of 1 m above ground is 74.3{+-}27.8 nGy h{sup -1}, corresponding to an annual effective dose equivalent of 455.6 {mu}Sv. The dose equivalent ranges from 168.3 to 1250.5 {mu}Sv. The results have been compared with other global radioactivity measurements and evaluations.

  6. Determination of distribution coefficient (Kd's) of some artificial and naturally occurring radionuclide in fresh and marine coastal water sediment

    International Nuclear Information System (INIS)

    Al-Masri, M. S.; Mamish, S; Haleem, M. A.

    2004-12-01

    Distribution coefficients of artificial and natural radionuclides in fresh and marine water sediment are used in modeling radionuclide dispersion in water system, and the radiation risk and environmental investigating of impact of radioactive emissions, due to routine operations of nuclear plants or disposal and burial of radioactive waste in the environment. In the present work, distribution coefficient of uranium, lead, polonium, radium (naturally occurring radionuclides that may be emitted into the Syrian environment by the phosphate and oil industry with relatively high concentrations) and caesium 137 and strontium 85, in fresh water sediment (Euphrates River, Orantos River and Mzzerib Lake) and marine coastal water (Lattakia, Tartous and Banias). Distribution coefficients were found to vary between (5.8-17.18)*10 3 , (2.2-8.11)*10 3 , (0.22-2.08)*10 3 , (0.16-0.19)*10 3 , (0.38-0.69)*10 3 and 49-312 for polonium, lead, uranium, radium, cesium and strontium respectively. Results have indicated that most measurement distribution coefficients in the present study were lower than those values reported in IAEA documents for marine coastal sediment. In addition, variations of Kd's with aqueous phase composition and sediment elemental and mineralogical composition and its total organic materials content have been studied, where liner correlation coefficients for each isotope with different parameters have been determined. The obtained data reported in this study can be used for radioactive contaminants dispersion and transfer in Syrian river, lake and coast to assess risks to public due to discharges of the phosphate and oil industry into the Syrian environment. (Authors)

  7. Occupational exposure to natural radionuclides due to mining activities in Ibadan, Southwestern Nigeria

    International Nuclear Information System (INIS)

    Ademola, J.A.; Okpalaonwuka, N.E.

    2010-01-01

    The activity concentrations of potassium, uranium and thorium in minerals and soil samples from a mining site in Ibadan, Southwestern Nigeria were measured using gamma ray spectroscopy method. Effective dose per annum has been calculated from the activity concentrations of dominant gamma-emitting natural radionuclides, potassium, uranium and thorium. Samples collected include minerals (beryl, quartz and feldspar), soil samples from the mining pits, heaps and undisturbed land around the mining site. The activity concentrations of 40 K, 238 U and 232 Th, respectively in Bq kg-1 in the mineral samples were as follows: 1985 ± 16, 4.8 ± 0.9 and 11.8 ± 5.8 for beryl sample, 115.1 ± 27.9, 5.0 ± 1.3 and 6.3 ± 5.0 for feldspar samples and 1421 ± 122, 40 K, 238 U and 232 Th, respectively, were 314.2 ± 5.7, 27.7 ± 2.6 and 11.5 ± 5.9 Bq kg-1 for soil samples from the pits and 278.1 ± 5.4, 21.1 ± 2.0 and 15.3 ± 7.5 Bq kg-1 for soil samples from heaps. The mean activity concentrations of soil samples from the undisturbed land around the mining site were 194.3 ± 25.2, 14.5 ± 5.1 and 13.3 ± 5.9 Bq kg-1 for 40 K, 238 U and 232 Th, respectively. The effective dose to which the miners are exposed according to exposure scenarios were calculated as 89.9 μSv y-1 for digging and handling of soil and mineral samples in the pit and 63.6 μSv y-1 for handling of soil and mineral samples at the heaps. (authors)

  8. Hydrothermal alterations as natural analogues of radionuclide migration in granitic rocks

    International Nuclear Information System (INIS)

    Piantone, P.

    1989-01-01

    The document is the final report of the project Hydrothermal alteration systems as analogues of nuclear waste repositories in granitic rocks which was the subject of contract n 0 F1 1 W/0072-F (CD) performed at shared cost between the Bureau de Recherches Geologiques et Minieres (BRGM), the Commissariat a l'Energie Atomique and the Commission of the European Communities as part of the MIRAGE programme. This study is the continuation of a preliminary study made by BRGM in 1986 and which concerned the same programme. The data given in this report were obtained from the study of the infilling and hydrothermalized walls of a mineralized vein located at Fombillou, Lot Department, in the French Massif Central. A satisfactory model of the processes generated by hydrothermal alteration then by climatic weathering such as formation of new minerals, flow of elements and variations in volume, was thus built. The mobility of elements displaying physical and chemical properties similar to those of radionuclides present in high-level radioactive waste was studied. A preliminary thermodynamic simulation of mineral transformations and transfers of matter during hydrothermal alteration was performed using the calculation code CEQCSY (Chemical EQuilibrium in Complex SYstem). This simulation is based on the values of the main physical and chemical parameters deduced from the analysis of the natural system. On the basis of the results obtained from Fombillou, an appraisal was made of the response of the granitic environment which has been disturbed by a hydrothermal system produced by heat emitted by the storage of high-level radio-active waste as well as its potential capacities of retention in case of possible leakage

  9. Mapping of Natural Radionuclides using Noise Adjusted Singular Value Decomposition, NASVD

    DEFF Research Database (Denmark)

    Aage, Helle Karina

    2006-01-01

    Mapping of natural radionuclides from airborne gamma spectrometry suffer from random ”noise” in the spectra due to short measurement times. This is partly compensated for by using large volume detectors to improve the counting statistics. One method of further improving the quality of the measured...... spectra is to remove from the spectra a large fraction of this random noise using a special variant of Singular Value Decomposition: Noise Adjusted Singular Value Decomposition. In 1997-1999 the natural radionuclides on the Danish Island of Bornholm were mapped using a combination of the standard 3...

  10. Sediment studies at Bikini Atoll part 3. Inventories of some long-lived gamma-emitting radionuclides associated with lagoon surface sediments

    Energy Technology Data Exchange (ETDEWEB)

    Noshkin, V.E.

    1997-12-01

    Surface sediment samples were collected during 1979 from 87 locations in the lagoon at Bikini Atoll. The collections were made to better define the concentrations and distribution of long-lived radionuclides associated with the bottom material and to show what modifications occurred to the composition of the surface sediment from the nuclear testing program conducted by the United States at the Atoll between 1946 and 1958. This is the last of three reports on Bikini sediment studies. In this report, we discuss the concentrations and inventories of the residual long-lived gamma-emitting radionuclides in sediments from the lagoon. The gamma-emitting radionuclides detected most frequently in sediments collected in 1979, in addition to Americium-241 ({sup 241}Am) (discussed in the second report of this series), included Cesium-137 ({sup 137}Cs), Bismuth-207 ({sup 207}Bi), Europium-155 ({sup 155}Eu), and Cobalt-60 ({sup 60}Co). Other man-made, gamma-emitting radionuclides such as Europium-152,154 ({sup 152,154}Eu), Antimony-125 ({sup 125}Sb), and Rhodium-101,102m ({sup 101,102m}Rh) were occasionally measured above detection limits in sediments near test site locations. The mean inventories for {sup 137}Cs, {sup 207}Ei, {sup 155}Eu, and {sup 60}Co in the surface 4 cm of the lagoon sediment to be 1.7, 0.56, 7.76, and 0.74 TBq, respectively. By June 1997, radioactive decay would reduce these values to 1.1, 0.38, 0.62, and 0.07 TBq, respectively. Some additional loss results from a combination of different processes that continuously mobilize and return some amount of the radionuclides to the water column. The water and dissolved constituents are removed from the lagoon through channels and exchange with the surface waters of the north equatorial Pacific Ocean. Highest levels of these radionuclides are found in surface deposits lagoonward of the Bravo Crater. Lowest concentrations and inventories are associated with sediment lagoonward of the eastern reef. The quantities in

  11. Contents of natural and anthropological radionuclides in uncultivated soils in the eastern part of Bulgaria

    International Nuclear Information System (INIS)

    Todorov, P.; Georgieva, D.; Yaneva, B.

    2006-01-01

    Bulgaria is a country which is located in the Eastern part of Europe. The lay shape of Bulgaria is very various, regarding to the lay shape, rock types and some human activities it defines content of radionuclides in uncultivated soils. Natural radionuclides in these soils are: U 238, Ra 226, Th 232 and K 40. The main anthropological source of radionuclides in these soils is Cs 137. There are no normative documents about limit concentrations of these radionuclides in uncultivated soils. So the actual concentrations are compared with some background concentrations, as a result from a lot of studies in the past. Valuation of natural and anthropological radionuclides is made by determination of their special activity in soil samples from the 0 - 20 cm layer by using the nondestructive gamma spectro metrological analysis. Specific activity of U 238 is defined by its daughter product - Th 234, specific activity of Ra 226 by Pb 214 and Bi 214, of Th 232 by Ac 228 and Pb 212, and specific activity of K-40 and Cs 137 by gamma spectro metrological analysis. In the last years there was made a systematic and valuation of concentrations of these radionuclides. There were examined more than 500 samples each year in the investigated area. Concentrations for U 238 vary from 4 to 64 Bq/kg, for Ra 226 from 7 to 54 Bq/kg, for Th 232 from 12 to 67 Bq/kg, for K 40 from 72 to 1106 Bq/kg. For Cs 137, the concentrations vary from 2 to 234 Bq/kg. During this analysis there were no indices of natural radionuclides above the limit concentrations - background concentrations typical for the different regions

  12. Assessment of Natural radionuclides in Powdered milk Consumed in Iraq

    Energy Technology Data Exchange (ETDEWEB)

    Amin, Sahar A.; Al-ani, Rana R. [Environmental Research Center, University of Technology, Baghdad (Iraq); AL-kafaje, Mohammed S.M. [Department of Laser Engineering and Electronic Optics, University of Technology (Iraq)

    2014-07-01

    The activity concentrations of {sup 226}Ra, {sup 232}Th, and {sup 40}K radionuclides were measured for 10 brands of powdered milk samples consumed in Iraq, which are imported from different countries. The main detected activity corresponding to {sup 40}K with average activity of 290.661 BqKg{sup -1}, while the average activities of {sup 226}Ra and {sup 232}Th were below the detection level (B.D.L.). Results are compared with those of different countries worldwide. The total average annual effective doses due to intake of {sup 40}K from the ingestion of the powdered milk for children (2-7, 7-12, 12-17)y and adults (≥ 17 y) were estimated to be 82.21, 50.90, 29.75 and 22.55 μSvy{sup -1}, respectively. These results indicate no significant radiation dose to the public. The resulting data may serve as base-line levels of activity concentration in powdered milk in the area of study. (authors)

  13. Measurement of natural and artificial radionuclide concentrations in meat consumed in Hong Kong

    International Nuclear Information System (INIS)

    Mao, S.Y.; Yu, K.N.

    1995-01-01

    Radionuclides in meat are determined using the EG and G ORTEC photon spectrometer system. Most of the naturally occurring radionuclides are found to have specific activities below the detectable limit. For our samples, 40 K is found to have values ranging from 295-407 Bq/kg, 172-423 Bq/kg and 172-282 Bq/kg for beef, pork and chicken meat samples, respectively, while 137 Cs has values from 0.19-2 Bq/kg, 0.34-0.71 Bq/kg and 0.12-0.53 Bq/kg, respectively. The estimated weighted committed dose equivalent due to the ingestion of natural radionuclides and 137 Cs in meat is 137 Cs in both sexes are less than the level recommended by the International Commission on Radiological Protection. (author)

  14. The NIST natural-matrix radionuclide standard reference material program for ocean studies

    International Nuclear Information System (INIS)

    Inn, K.G.W.; Zhichao Lin; Zhongyu Wu; MacMahon, C.; Filliben, J.J.; Krey, P.; Feiner, M.; Harvey, J.

    2001-01-01

    In 1997, the Low-level Working Group of the International Committee on Radionuclide Metrology met in Boston, MA (USA) to define the characteristics of a new set of environmental radioactivity reference materials. These reference materials were to provide the radiochemist with the same analytical challenges faced when assaying environmental samples. It was decided that radionuclide bearing natural materials should be collected from sites where there had been sufficient time for natural processes to redistribute the various chemically different species of the radionuclides. Over the succeeding years, the National Institute of Standards and Technology (NIST), in cooperation with other highly experienced laboratories, certified and issued a number of these as low-level radioactivity Standard Reference Materials (SRMs) for fission and activation product and actinide concentrations. The experience of certifying these SRMs has given NIST the opportunity to compare radioanalytical methods and learn of their limitations. NIST convened an international workshop in 1994 to define the natural-matrix radionuclide SRM needs for ocean studies. The highest priorities proposed at the workshop were for sediment, shellfish, seaweed, fish flesh and water matrix SRMs certified for mBq per sample concentrations of 90 Sr, 137 Cs and 239 Pu + 240 Pu. The most recent low-level environmental radionuclide SRM issued by NIST, Ocean Sediment (SRM 4357) has certified and uncertified values for the following 22 radionuclides: 40 K, 90 Sr, 129 I, 137 Cs, 155 Eu, 210 Pb, 210 Po, 212 Pb, 214 Bi, 226 Ra, 228 Ra, 228 Th, 230 Th, 232 Th, 234 U, 235 U, 237 Np, 238 U, 238 Pu, 239 Pu + 240 Pu, and 241 Am. The uncertainties for a number of the certified radionuclides are non-symmetrical and relatively large because of the non-normal distribution of reported values. NIST is continuing its efforts to provide the ocean studies community with additional natural matrix radionuclide SRMs. The freeze

  15. Natural attenuation of metals and radionuclides: Report from a workshop held by Sandia National Laboratories

    Energy Technology Data Exchange (ETDEWEB)

    Brady, P.V.; Borns, D.J. [Sandia National Labs., Albuquerque, NM (United States). Geochemistry Dept.

    1997-11-01

    Natural attenuation is increasingly applied to remediate contaminated soils and ground waters. Roughly 25% of Superfund groundwater remedies in 1995 involved some type of monitored natural attenuation, compared to almost none 5 years ago. Remediation by natural attenuation (RNA) requires clear evidence that contaminant levels are decreasing sufficiently over time, a defensible explanation of the attenuation mechanism, long-term monitoring, and a contingency plan at the very least. Although the primary focus of implementation has to date been the biodegradation of organic contaminants, there is a wealth of scientific evidence that natural processes reduce the bioavailability of contaminant metals and radionuclides. Natural attenuation of metals and radionuclides is likely to revolve around sorption, solubility, biologic uptake and dilution controls over contaminant availability. Some of these processes can be applied to actively remediate sites. Others, such as phytoremediation, are likely to be ineffective. RNA of metals and radionuclides is likely to require specialized site characterization to construct contaminant and site-specific conceptual models of contaminant behavior. Ideally, conceptual models should be refined such that contaminant attenuation can be confidently predicted into the future. The technical approach to RNA of metals and radionuclides is explored here.

  16. Natural attenuation of metals and radionuclides: Report from a workshop held by Sandia National Laboratories

    International Nuclear Information System (INIS)

    Brady, P.V.; Borns, D.J.

    1997-11-01

    Natural attenuation is increasingly applied to remediate contaminated soils and ground waters. Roughly 25% of Superfund groundwater remedies in 1995 involved some type of monitored natural attenuation, compared to almost none 5 years ago. Remediation by natural attenuation (RNA) requires clear evidence that contaminant levels are decreasing sufficiently over time, a defensible explanation of the attenuation mechanism, long-term monitoring, and a contingency plan at the very least. Although the primary focus of implementation has to date been the biodegradation of organic contaminants, there is a wealth of scientific evidence that natural processes reduce the bioavailability of contaminant metals and radionuclides. Natural attenuation of metals and radionuclides is likely to revolve around sorption, solubility, biologic uptake and dilution controls over contaminant availability. Some of these processes can be applied to actively remediate sites. Others, such as phytoremediation, are likely to be ineffective. RNA of metals and radionuclides is likely to require specialized site characterization to construct contaminant and site-specific conceptual models of contaminant behavior. Ideally, conceptual models should be refined such that contaminant attenuation can be confidently predicted into the future. The technical approach to RNA of metals and radionuclides is explored here

  17. Bioaccumulation of some natural radionuclides in short-antenna grasshoppers (Acrididae family, class Ortoptera)

    International Nuclear Information System (INIS)

    Dimitrova, M.; Markova, E.

    1996-01-01

    The seasonal accumulation of radioactive elements of uranium-radium line in representatives of larval stages of different species of Acrididae family has been examined. This group of invertebrates is a good bioindicator of radionuclides accumulation and could be used successfully as an ecological evaluation. The monitoring sites are typical for the region of Etropole (where the uranium mine 'Elatsite' is situated) and offer information about the natural radiation background as well as about an eventual radiation pollution. Two years examination has been carried out during spring, summer and autumn on natural grass ecosystem (one of them just above the mentioned uranium mine). The gamma-spectrometric analysis of seventeen samples have shown the presence of U-238, Ra-226, Pb-214 and Bi-214. The minimal detectable activity of these radionuclides was calculated, resp. 0.25Bq, 0.49Bq, 0.07Bq and 0.12Bq. All experimental data for the four radionuclides are reliable considering Currie criterion. The meadow close to the uranium mine has shown maximal radiation background, while the control samples from nearby region have shown no presence of radionuclides. The accumulation of the radionuclides from U-Ra line is seasonal, more expressed in autumn. This fact could be explained by the biological maturity of this species in the end of summer. It has been found that the ionizing radiation in the natural biocenoses is not only an individual irritant, but also has an effect of a radioecological factor of the environment. The examinations show a redistribution of the natural radionuclides resulting from economic activities. 17 refs., 3 tabs., 3 figs

  18. Natural radionuclides monitoring in Lombardia drinking water by liquid scintillation technique

    International Nuclear Information System (INIS)

    Forte, M.; Rusconi, R.; Bellinsona, S.; Sgorbati, G.

    2002-01-01

    Concern about total radionuclides content in water intended for human consumption has been brought to public attention by the recent Council Directive 98/83/EC, subsequently enforced through an Italian law (DL 31, February 2., 2001). Parameter values have been fixed for Tritium content and total indicative dose: the Directive points out that the total indicative dose must be evaluated excluding Tritium, 4 0K , 1 4C , Radon and its decay products, but including all other natural series radionuclides. Maximum concentration values for Radon are separately proposed in Commission Recommendation 2001/928/Euratom. Tritium determination follows a well established procedure, standardised by International Standard Organisation (ISO 9698, 1989). On the contrary, total indicative dose evaluation requires more specific and cumbersome procedures for the measurement of radioactivity content, with special regard to natural series radionuclides. The large number of possibly involved radionuclides and the good sensitivities required make the application of traditional analytical techniques unsuitable in view of a large scale monitoring program. World Health Organisation (WHO 1993 and 1996) guidelines for drinking water suggest performing an indirect evaluation of committed dose by measuring alpha and beta gross radioactivity and checking compliance to derived limit values; the proposed limit values are 0,1 Bq/l for gross alpha and 1 Bq/l for gross beta radioactivity. Nevertheless, it is desirable to identify single radionuclides contribution to alpha and beta activity in order to perform more accurate measurements of committed dose

  19. ALMERA Proficiency Test: Determination of Natural and Artificial Radionuclides in Soil and Water. IAEA-TEL-2011-04

    International Nuclear Information System (INIS)

    2013-01-01

    The Analytical Laboratories for the Measurement of Environmental Radioactivity (ALMERA) network is a cooperative effort of analytical laboratories worldwide. Members of the network are nominated by their respective Member States on the expectation of providing reliable and timely analysis of environmental samples in the event of an accidental or intentional release of radioactivity. The ALMERA network consists of 131 laboratories representing 81 Member States at December 2012. The IAEA's Environment Laboratories in Seibersdorf and Monaco are the central coordinators of the ALMERA network activities. The IAEA helps the ALMERA network to maintain their readiness by coordinating activities, including the organization of meetings, development of standardized methods of sample collection and analysis, and organization of interlaboratory comparison exercises and proficiency tests as tools for external quality control. IAEA proficiency tests and interlaboratory comparison exercises are organized on a regular basis specifically for the members of the ALMERA network. At least one exercise is organized per year by the IAEA for the ALMERA network. These exercises are designed to monitor and to demonstrate the performance and analytical capabilities of the network members, and to identify gaps and problem areas where further development is needed. The ALMERA proficiency tests enable ALMERA members to report their results on gamma emitting radionuclides in a very short time frame, i.e. three days, which is what would be required for emergency response. This publication presents the results of the ALMERA proficiency test IAEA-TEL-2011-04 on the determination of natural and artificial radionuclides in water and soil. The methodologies, data evaluation approach, summary evaluation of each radionuclide and individual evaluation reports for each laboratory are also described

  20. Determination of natural radionuclide level in industrial waste slags and evaluation of comprehensive utilization

    International Nuclear Information System (INIS)

    Li Ruixiang; Liu Xinhua; Gan Lin

    1994-09-01

    Natural radionuclide contents were measured in various industrial waste slags in China by a low background HPGe γ spectrometer and the radiological impact was estimated for some comprehensive utilization of these slags. Most waste slags can be used for building materials except for tailing and waste rock form nuclear industry

  1. Levels of natural radionuclides in soil samples around a phosphate fertilizer plant

    International Nuclear Information System (INIS)

    Ajmal, P.Y.; Sahu, S.K.; Bhangare, R.C.; Pandit, G.G.; Puranik, V.D.

    2010-01-01

    The present study is aimed at the determination of the activity levels of primordial radionuclides in soil from various locations around a phosphate fertilizer plant and also to figure out the external dose rate due to natural gamma background in the area by mapping the dose rates with the geographical co-ordinates within the plant premises

  2. Natural and artificial radionuclides in southern of Gulf of Mexico marine sediments

    International Nuclear Information System (INIS)

    Rodriguez-Espinosa, P.F.; Vidal-Lorandi, V.M.V.; Vidal-Lorandi, F.V.

    1999-01-01

    Preliminary results of quantitative analysis of natural and artificial radionuclides in sediment cores of the Southern Gulf of Mexico, reveal the presence of 22.01 Bq/kg 226 Ra, 15.56 Bq/kg 214 Bi, 18.17 Bq/kg 214 Pb, 485.81 Bq/kg 40 K and 2.84 Bq/kg 137 Cs

  3. MCNP modelling of scintillation-detector gamma-ray spectra from natural radionuclides

    NARCIS (Netherlands)

    Hendriks, Peter; Maucec, M; de Meijer, RJ

    gamma-ray spectra of natural radionuclides are simulated for a BGO detector in a borehole geometry using the Monte Carlo code MCNP. All gamma-ray emissions of the decay of K-40 and the series of Th-232 and U-238 are used to describe the source. A procedure is proposed which excludes the

  4. Decision making algorithm of the rehabilitation of agricultural lands contaminated with heavy natural radionuclides

    International Nuclear Information System (INIS)

    Khomutyinyin, Yu.V.; Yivanov, Yu.O.; Kirichenko, V.K.

    2013-01-01

    Problem of rehabilitation of agricultural land contaminated with heavy natural radionuclides ( 210 Pb, 210 Po, 226 Ra, 232 Th, 238 U) was considered. Algorithm of decision making support on advisability of rehabilitation of mentioned land was suggested. Proposed algorithm was tested on the base of agricultural farmlands located in the affected zone of Pridneprovsky Chemicals Plant and its tailing dumps

  5. Natural radionuclides in some romanian medicinal mineral water

    Energy Technology Data Exchange (ETDEWEB)

    Botezatu, E.; Iacob, O. [Institute of Public Health, Iasi (Romania)

    2006-07-01

    Radioactive minerals occur irregularly in the bedrock, similar to other minerals and they dissolve easily in water. Bedrock contains naturally occurring radioactivity including uranium, thorium, radium and potassium. The natural radioactivity results from water passing through deposits of naturally occurring radioactive materials.Many mineral water springs are traditionally used as drinking mineral water sources in the area.During the period from 1997 to 2000, we accomplished a study that had as basic objectives the radioacty control of the drinking mineral waters according to existing standards and evaluation of doses to population by ingestion of mineral water (bottled waters commercially available for human intake and some spring waters).For this reason, we were interested in finding out the extent to which these waters can be a natural radiation source. This survey aimed at assessing the radioactive content of these waters and their contribution to the population exposure.The presented data contribute to a national database concerning the natural radioactive content of Romanian mineral waters. A hypothetical person that undergoes a cure of mineral water by ingestion, inhalation and immersion is receiving an average supplementary dose of 3 {mu}Sv over background radiation of 2,512 {mu}Sv.y{sup -1} due to all natural radiation sources in Romania. The contribution of mineral water used in therapeutic purposes to the natural irradiation of population is very slight, almost insignificant. This supports the conclusion that these spring mineral waters can be used without any restrictions for drinking or bathing / washing for medical therapy of ailing persons even other sources of exposure are also taken into account. (N.C.)

  6. The effect of dose protraction on the incidence of lung carcinomas in beagle dogs with internally deposited β-emitting radionuclides

    International Nuclear Information System (INIS)

    Griffith, W.C.; Boecker, B.B.; Hahn, F.F.; Muggenburg, B.A.; Snipes, M.B.

    1992-01-01

    Studies using Beagle dogs were conducted to understand health effects when lung is the primary organ irradiated after inhaling insoluble radioactive particles containing one of four β-emitting radionuclides, 90 Y, 91 Y, 144 Ce, or 90 Sr. The low-LET β irradiation was delivered over a wide range of total doses and dose rate patterns that protracted the dose to lung from about 1 wk to several years. The tumor incidence rates for lung carcinomas were estimated using a proportional hazard rate model. These studies suggest that dose protraction only affects production of lung carcinomas at doses above 50 Gy

  7. Distribution of natural radionuclides in sediment around Sultan Azlan Shah coal-fired power plant coastal water area in Manjung, Perak

    International Nuclear Information System (INIS)

    Zaini Hamzah; Anisa Abdullah; Abdul Khalik Wood; Ahmad Saat

    2013-01-01

    Full-text: A rapid and simple analytical method for the determination of the natural radionuclides in sediment around Sultan Azlan Shah Coal-Fired Power Plant coastal water area in Manjung, Perak of Malaysia was carried out by Energy Dispersive X-ray Fluorescence (EDXRF) technique. The concentration of radionuclides contents in the marine ecosystem can be adversely affect human health and the environment when exposed through food chain. Furthermore, radionuclide is an atom with an unstable nucleus and they are naturally origin undergoes radioactive decay and emits a gamma ray or subatomic particles radiated from a coal fired power plant activity that contained in raw coal, fly ash and bottom ash, where a potential risk exposed into the atmosphere. However, coal is a heat source for electric power generation and operation of a coal burning power plant is one of the sources radiation contaminations and leads to a distributes of natural radionuclides. Sediment particle is a common pollutant that settles at the bottom of body water can be degrades water quality and demanding of oxygen in the marine ecosystem. Ten points of sediment cores will be taken along the coastal area in the study. The results of present study showed the concentration of natural radionuclides 238 U and 232 Th in surface sediment samples were in the ranged between 2.47 to 3.80 mg/ kg and 8.84 to 12.49 mg/ kg respectively. Thus, based on the concentration value obtained it can be determines assessment of potential hazard and radioactivity level in the future. (author)

  8. Natural radionuclides in mangrove soils from the State of Pernambuco, Brazil

    International Nuclear Information System (INIS)

    Paiva, J.D.S. de; Sousa, E.E.; Farias, E.E.G. de; Carmo, A.M.; Souza, E.M.; Franca, E.J. De

    2016-01-01

    Mangroves are essential for protecting coastal environments and biodiversity; however few studies encompass the distribution of radionuclides in soils from these ecosystems. By applying high resolution gamma-ray spectrometry, natural radionuclides were quantified in soils from the Chico Science Mangrove and Rio Formoso Mangrove (RFM), areas subjected to different human impacts. The activity concentrations of 226 Ra and 228 Ra were quite similar for the mangroves despite the differences found for 40 K. Moreover, no correlation with the environmental impacts on the mangroves was observed, although RFM soil was 40 K-enriched compared to deep sediments from other estuaries in the world. (author)

  9. Application of Monte Carlo simulation to the standardization of positron emitting radionuclides; Aplicacao do metodo de Monte Carlo na padronizacao de radionuclideos emissores de positrons

    Energy Technology Data Exchange (ETDEWEB)

    Tongu, Margareth Lika Onishi

    2009-07-01

    Since 1967, the Nuclear Metrology Laboratory (LNM) at the Nuclear and Energy Research (IPEN) in Sao Paulo, Brazil, has developed radionuclide standardization methods and measurements of the Gamma-ray emission probabilities per decay by means of 4{pi}{beta}-{gamma} coincidence system, a high accuracy primary method for determining disintegration rate of radionuclides of interest. In 2001 the LNM started a research field on modeling, based on Monte Carlo method, of all the system components, including radiation detectors and radionuclide decay processes. This methodology allows the simulation of the detection process in a 4{pi}{beta}-{gamma} system, determining theoretically the observed activity as a function of the 4{pi}{beta} detector efficiency, enabling the prediction of the behavior of the extrapolation curve and optimizing a detailed planning of the experiment before starting the measurements. One of the objectives of the present work is the improvement of the 4{pi} proportional counter modeling, presenting a detailed description of the source holder and radioactive source material, as well as absorbers placed around the source. The simulation of radiation transport through the detectors has been carried out using code MCNPX. The main focus of the present work is on Monte Carlo modeling of the standardization of positron emitting radionuclides associated (or not) with electron capture and accompanied (or not) by the emission of Gamma radiation. One difficulty in this modeling is to simulate the detection of the annihilation Gamma ray, which arise in the process of positron absorption within the 4{pi} detector. The methodology was applied to radionuclides {sup 18}F and {sup 22}Na. (author)

  10. IAEA programme of natural matrix reference materials for the determination of radionuclides

    International Nuclear Information System (INIS)

    Strachnov, V.; Valkovic, V.; LaRosa, J.; Dekner, R.; Zeisler, R.

    1993-01-01

    The International Atomic Energy Agency has been providing analytical quality control services (AQCS) to its Member States since the 1960's. The AQCS programme distributes reference materials (RMs), organizes intercomparison runs, and provides training courses for quality assurance in chemical analysis and radioactivity measurements of food, biological, environmental and marine materials. This paper focusses on those aspects of the subject dealing with reference materials and intercomparison runs for the determination of radionuclides. Nineteen natural matrix reference materials are available for the determination of radionuclides. Twelve new intercomparison and reference materials are in preparation or under consideration. The radionuclides of interest include: K-40, Mn-54, Co-60, Sr-90, Tc-99, Ru-106, Ba-133, Cs-134, Cs-137, Pb-210, Ra-226, Th-228, Th-232, Pu-238, Pu-239 + 240. (orig.)

  11. Assessment and the levels of radioactivity of natural radionuclides in drinking waters in China

    International Nuclear Information System (INIS)

    Liu Yulan

    1989-03-01

    In order to assess the levels of radioactivity of natural radionuclides in drinking waters and to estimate the internal doses of the population of China from ingestion, 1650 samples of waters were collected from normal radiation background areas of 28 provinces or autonomous regions of China. Radioactivity levels of U, Th, 226 Ra and 40 K in drinking waters were determined. The levels and the characteristics of distribution of 4 radionuclides are given. The results show that radioactivity levels in the southeast China are lower than in the north and northwest China. The average radioactivity levles of the 4 radionuclides in China close to the average levels given in UNSCEAR 1986 report. The result of estimation of internal doses from ingestion in the population of China is below the corresponding results given in UNSCEAR 1986 report, but near the result given by ICRP

  12. High levels of natural radionuclides in a deep-sea infaunal xenophyophore

    Energy Technology Data Exchange (ETDEWEB)

    Swinbanks, D D; Shirayama, Y

    1986-03-27

    The paper concerns the high levels of natural radionuclides in a deep-sea infaunal xenophyophore from the Izu-Ogasawara Trench. Measured /sup 210/Po activities and barium contents of various parts of Occultammina profunda and the surrounding sediment are given, together with their estimated /sup 210/Pb and /sup 226/Ra activities. The data suggest that xenophyphores are probably subject to unusually high levels of natural radiation.

  13. Natural Radionuclides and Heavy Metals Pollution in Seawater at Kuala Langat Coastal Area

    International Nuclear Information System (INIS)

    Sabarina Md Yunus; Zaini Hamzah; Ab Khalik Hj Wood; Ahmad Saat

    2015-01-01

    Rapid industrial developments along the Langat river basin play an important role in contributing to the increases of pollution loading at Kuala Langat coastal area. The major pollutant sources in this area may be originating from human activities such as industrial discharge, domestic sewage, construction, agriculture and pig farming near the tributaries that affects the water quality. In addition, Langat and Semenyih rivers flow through the mining and ex-mining area, which is related to the source of natural radionuclides contamination. Heavy metals in the aquatic environment and more likely to enter the food chain. This study is focusing to the levels of radionuclides and heavy metals in seawater. The samples were collected using appropriate water sampler, which is then acidified until pH 2 and filtered using cellulose acetate 0.45 μm. The concentration of these radionuclides and heavy metals were determined using Inductive Coupled Plasma Mass Spectrometer (ICPMS) after dilution. In general, the radionuclides and heavy metals concentrations are lower than Malaysia Marine Water Quality Standard (MMWQS) except for few locations where the concentration levels above the standards. The higher concentration of pollutant in the seawater may have a toxic effect on sensitive plants and living organisms. The results of pollution levels of these radionuclides and heavy metals were also compared with other studies. (author)

  14. Soil and vegetation influence in plants natural radionuclides uptake at a uranium mining site

    Science.gov (United States)

    Charro, E.; Moyano, A.

    2017-12-01

    The main objective of this work is to investigate the uptake of several radionuclides by the vegetation characteristic of a dehesa ecosystem in uranium mining-impacted soils in Central-West of Spain. The activity concentration for 238U, 226Ra, 210Pb, 232Th, and 224Ra was measured in soil and vegetation samples using a Canberra n-type HPGe gamma-ray spectrometer. Transfer factors of natural radionuclides in different tissues (leaves, branches, twigs, and others) of native plants were evaluated. From these data, the influence of the mine, the physicochemical parameters of the soils and the type of vegetation were analyzed in order to explain the accumulation of radionuclides in the vegetation. A preferential uptake of 210Pb and 226Ra by plants, particularly by trees of the Quercus species (Quercus pyrenaica and Quercus ilex rotundifolia), has been observed, being the transfer factors for 226Ra and 210Pb in these tree species higher than those for other plants (like Pinus pinaster, Rubur ulmifolius and Populus sp.). The analysis of radionuclide contents and transfer factors in the vegetation showed no evidence of influence of the radionuclide concentration in soils, although it could be explained in terms of the type of plants and, in particular, of the tree's species, with special attention to the tree's rate of growth, being higher in slow growing species.

  15. Investigation of rare earth natural radionuclide in Gannan region, Jiangxi province

    International Nuclear Information System (INIS)

    Liu Huiping; Zhong Minglong; Hu Yongmei

    2014-01-01

    In order to identify the types, level and migration law of natural radionuclide in ionic rare earth during its development and utilization process, the natural radionuclide in raw ore, waste residues and wastewater of south ionic rare of Gannan region, Jiangxi province were investigated. The results showed that: the natural radionuclide in rare earth raw ore in An'yuan and Longnan is with high content, in which the specific activities of natural U, 226 Ra and 232 Th are 3.69 × l0 4 , 8.33 × l0 3 and 3,40 × l0 3 Bq/ kg respectively; And the specific activities of the acid-soluble slag are 2.58 × l0 4 , 2.81 × l0 4 and 2.75 × l0 4 Bq/kg respectively; The radioactive level of natural U and 232 Th in some rare earth tailings, and the specific activity of natural U in the neutralizing slag of some individual enterprises is higher than national standards' exemption level (1000 Bq/kg). Also, the total content of Th and U in the efflux wastewater of some rare earth enterprises efflux wastewater are higher than the national emission standards limit (0.1 mg/L). (authors)

  16. Ion exchange of radionuclides on natural and modified micaceous minerals

    International Nuclear Information System (INIS)

    Kojvula, R.; Lekhto, Yu.

    1998-01-01

    Interaction of 134 Cs, 85 Sr and 60 Co with three micaceous minerals: muscovites, biotites and phlogopite is studied. Two types of micaceous minerals: natural ones, wherein potassium is an exchange cation, and samples, converted into sodium form, are studied/ It is found that biotite and phlogopite in the sodium form are specified by high selectivity to cobalt with distribution coefficient above 10 5 ml/g, whereas the muscovite potassium form is characterized by high selectivity to cesium. Neither of the micaceous minerals is characterized by selectivity to strontium. Distribution coefficients strongly depend on pH of the medium

  17. Radiological monitoring: terrestrial natural radionuclides in Kinta District, Perak, Malaysia

    Energy Technology Data Exchange (ETDEWEB)

    Lee, Siak Kuan [Department of Physics, Faculty of Science, University Teknologi Malaysia, 81310 Skudai, Johor Bahru (Malaysia)], E-mail: sklee88@hotmail.com; Wagiran, Husin; Termizi Ramli, Ahmad; Heru Apriantoro, Nursama [Department of Physics, Faculty of Science, University Teknologi Malaysia, 81310 Skudai, Johor Bahru (Malaysia); Khalik Wood, A. [Malaysia Nuclear Agency, Bangi, 43000 Kajang, Selangor (Malaysia)

    2009-05-15

    Natural background gamma radiation and radioactivity concentrations were investigated from 2003 to 2005 in Kinta District, Perak, Malaysia. Sample locations were distant from any 'amang' processing plants. The external gamma dose rates ranged from 39 to 1039 nGy h{sup -1}. The mean external gamma dose rate was 222 {+-} 191 nGy h{sup -1}. Small areas of relatively enhanced activity were located having external gamma dose rates of up to 1039 {+-} 104 nGy h{sup -1}. The activity concentrations of {sup 238}U, {sup 232}Th and {sup 40}K were analyzed by using a high-resolution co-axial HPGe detector system. The activity concentration ranges were 12-426 Bq kg{sup -1} for {sup 238}U, 19-1377 Bq kg{sup -1} for {sup 232}Th and <19-2204 Bq kg{sup -1} for {sup 40} K. Based on the radioactivity levels determined, the gamma-absorbed dose rates in air at 1 m above the ground were calculated. The calculated dose rates and measured dose rates had a good correlation coefficient, R of 0.94. To evaluate the radiological hazard of the natural radioactivity, the radium equivalent activity, the gamma-absorbed dose rate and the mean population weighted dose rate were calculated. An isodose map for the Kinta District was also produced.

  18. Radiological monitoring: terrestrial natural radionuclides in Kinta District, Perak, Malaysia

    International Nuclear Information System (INIS)

    Lee, Siak Kuan; Wagiran, Husin; Termizi Ramli, Ahmad; Heru Apriantoro, Nursama; Khalik Wood, A.

    2009-01-01

    Natural background gamma radiation and radioactivity concentrations were investigated from 2003 to 2005 in Kinta District, Perak, Malaysia. Sample locations were distant from any 'amang' processing plants. The external gamma dose rates ranged from 39 to 1039 nGy h -1 . The mean external gamma dose rate was 222 ± 191 nGy h -1 . Small areas of relatively enhanced activity were located having external gamma dose rates of up to 1039 ± 104 nGy h -1 . The activity concentrations of 238 U, 232 Th and 40 K were analyzed by using a high-resolution co-axial HPGe detector system. The activity concentration ranges were 12-426 Bq kg -1 for 238 U, 19-1377 Bq kg -1 for 232 Th and -1 for 40 K. Based on the radioactivity levels determined, the gamma-absorbed dose rates in air at 1 m above the ground were calculated. The calculated dose rates and measured dose rates had a good correlation coefficient, R of 0.94. To evaluate the radiological hazard of the natural radioactivity, the radium equivalent activity, the gamma-absorbed dose rate and the mean population weighted dose rate were calculated. An isodose map for the Kinta District was also produced.

  19. Distribution of natural radionuclides and radiation level measurements in Karnataka State, India. An overview

    International Nuclear Information System (INIS)

    Rangaswamy, D.R.; Sannappa, J.

    2016-01-01

    The exposure of human beings to ionizing radiation from natural sources is a continuing and inescapable feature of life on earth. A large number of natural radioactivity measurements were conducted throughout world, in order to know their distribution and to assess their radiological health hazards. In this regard, considerable studies have been conducted by different research groups in Karnataka state and more data are reported. In this article, all the studies of natural radioactivity measurements have been combined and reviewed. The majority of the reported articles are about monitoring, distribution and assessment of the radiological health hazards of naturally occurring radionuclides. (author)

  20. Incorporation of natural radionuclides and rare earth element into a salt tolerant plant

    International Nuclear Information System (INIS)

    Summerton, A.P.

    1992-01-01

    A highly salt tolerant shrub, samphire (Halosarcia halocnemoides), found growing in the solid alkaline residues in an evaporation pond at a former uranium and monazite treatment plant, has been analysed for natural radionuclides and rare earths. The data obtained have been copared with that for plants from the local natural environment. Vegetation-to-soil concentration ratios have been determined. The radionuclide concentration ratios for samples from the contaminated site are similar to those from the natural environment. Significant differences have been noted in the case of the rare earth elements with an apparent preferential incorporation of the light rare earth elements into the plant growing in the chemical residues. (author) 10 refs.; 1 fig.; 2 tabs

  1. Calibration of gamma cameras for the evaluation of accidental intakes of high-energy photon emitting radionuclides by humans based on urine samples

    Energy Technology Data Exchange (ETDEWEB)

    Degenhardt, A.L.; Lucena, E.A.; Reis, A.A. dos; Souza, W.O.; Dantas, A.L.A.; Dantas, B.M., E-mail: bmdantas@ird.gov.br [Instituto de Radioproteção e Dosimetria (IRD/CNEN-RJ), Rio de Janeiro, RJ (Brazil). Div. de Dosimetria

    2017-07-01

    The prompt response to emergency situations involving suspicion of intakes of radionuclides requires the use of simple and rapid methods of internal monitoring of the exposed individuals. The use of gamma cameras to estimate intakes and committed doses was investigated by the Centers for Disease Control and Preventions (CDC) of the USA in 2010.The present study aims to develop a calibration protocol for gamma cameras to be applied on internal monitoring based on urine samples to evaluate the incorporation of high-energy photon emitting radionuclides in emergency situations. A gamma camera available in a public hospital located in the city of Rio de Janeiro was calibrated using a standard liquid source of {sup 152}Eu supplied by the LNMRI of the IRD.'Efficiency vs Energy' curves at 10 and 30 cm were obtained. Calibration factors, Minimum Detectable Activities and Minimum Detectable Effective Doses of the gamma camera were calculated for {sup 137}Cs and {sup 60}Co. The gamma camera evaluated in this work presents enough sensitivity to detect activities of such radionuclides at dose levels suitable to assess suspected accidental intakes. (author)

  2. Uptake of γ-emitting radionuclides by aquatic biota exposed to contaminated water before and after passage through the ground

    International Nuclear Information System (INIS)

    Cushing, C.E.; Rickard, W.H.; Watson, D.G.

    1984-01-01

    Three experimental systems were designed to investigate the differential accumulation of radionuclides by biota from low-level aqueous effluents after passage through the ground. One system received river water (control), one received dilute low-level radioactive effluents (trench), and the third received the low-level effluents after it had percolated through about 260 m or porous gravel (springs). Biota studied included filamentous green algae, clams (Corbicula), goldfish (Carassius auratus), carp (Cyprinus carpio), and Veronica. Trophic level differences in accumulation of the various radionuclides from the diluted trench water were not consistent but generally followed the pattern algae > goldfish > molluscs > carp. Cobalt-60 was accumulated to the highest level of any radionuclide, and accumulation levels at the three sites were directly related to the concentration of 60 Co in the water. Manganese-54, 59 Fe, and 106 Ru were also accumulated to measurable levels in biota at the springs site indicating their bioavailability after passage through the ground

  3. Absorbed dose evaluation of Auger electron-emitting radionuclides: impact of input decay spectra on dose point kernels and S-values.

    Science.gov (United States)

    Falzone, Nadia; Lee, Boon Q; Fernández-Varea, José M; Kartsonaki, Christiana; Stuchbery, Andrew E; Kibédi, Tibor; Vallis, Katherine A

    2017-03-21

    The aim of this study was to investigate the impact of decay data provided by the newly developed stochastic atomic relaxation model BrIccEmis on dose point kernels (DPKs - radial dose distribution around a unit point source) and S-values (absorbed dose per unit cumulated activity) of 14 Auger electron (AE) emitting radionuclides, namely 67 Ga, 80m Br, 89 Zr, 90 Nb, 99m Tc, 111 In, 117m Sn, 119 Sb, 123 I, 124 I, 125 I, 135 La, 195m Pt and 201 Tl. Radiation spectra were based on the nuclear decay data from the medical internal radiation dose (MIRD) RADTABS program and the BrIccEmis code, assuming both an isolated-atom and condensed-phase approach. DPKs were simulated with the PENELOPE Monte Carlo (MC) code using event-by-event electron and photon transport. S-values for concentric spherical cells of various sizes were derived from these DPKs using appropriate geometric reduction factors. The number of Auger and Coster-Kronig (CK) electrons and x-ray photons released per nuclear decay (yield) from MIRD-RADTABS were consistently higher than those calculated using BrIccEmis. DPKs for the electron spectra from BrIccEmis were considerably different from MIRD-RADTABS in the first few hundred nanometres from a point source where most of the Auger electrons are stopped. S-values were, however, not significantly impacted as the differences in DPKs in the sub-micrometre dimension were quickly diminished in larger dimensions. Overestimation in the total AE energy output by MIRD-RADTABS leads to higher predicted energy deposition by AE emitting radionuclides, especially in the immediate vicinity of the decaying radionuclides. This should be taken into account when MIRD-RADTABS data are used to simulate biological damage at nanoscale dimensions.

  4. Behaviour of natural radionuclides on activated carbon filter

    International Nuclear Information System (INIS)

    Haberer, K.; Akkermann-Kubillus, A.; Dahlheimer, A.

    1998-01-01

    To investigate the behaviour of radon in adsorption/desorption processes at filter systems based on different activated carbon types, measurements were focused on adsorption capacity, adsorption velocity, retain capability, interaction with ions (poisoning of active centers) and adsorption of radon daughters. Various activated carbon types derived from hard coal, brown coal, peat and wood, were used in adsorption tests runs with activated carbons which are applied in water treatment facilities. In laboratory tests, water facility filter conditions were simulated using pilot plant columns filled with different carbon types. A small scale laboratory column was installed at a natural water source with elevated activity. Tests runs were conducted under varying flow rates and with different amounts of carbon. A full-scale waterworks filter system operated for 6 months was investigated for radon decay products adsorbed on the carbon. The main results observed were: 1. The amount of radioactivity adsorbed depends upon the type of carbon, its granular size and the contact time between the activated carbon and water. The decontamination capacity was between 19% and 94%. 2. The DOC-levels of water influences the adsorbable radioactivity due to the poisoning of the active centers of the carbon. The adsorption velocity decreased down to 15%. 3. The maximum decontamination rate of the water under waterworks conditions was 60%. (orig.) [de

  5. Distribution of some artificial and natural radionuclides and trace elements in Syrian soils

    International Nuclear Information System (INIS)

    Al-Masri, M. S.; Shaik Khalil, H.; Amin, Y.; Ibrahim, S.; Hassan, M.

    2004-07-01

    Within the environmental monitoring program in Syria, about 115 surface soil and 38 profile soil samples were collected and analyzed during the period of 1998 to 2003 in order to determine the levels of natural and artificial radionuclides and some of trace elements (Cu, Zn, Cd, Pb). The concentrations of the natural radionuclides in the surface samples were found to vary from area to another and ranged from 2-50 Bq/kg, 4-228 Bq/kg, 4-55 Bq/kg, 1-143 Bq/kg and 96-672 Bq/kg for 224 Ra, 226 Ra, 228 Ra, 137 Cs and 04 K, respectively. While, the concentrations of the studied trace elements were varied between 0.5-5.6 mg/kg for U, 3.2-31.7 mg/kg for Pb, 14-141 mg/kg for Zn, 1.6-114 mg/kg for Cu and 0.25-2.7 mg/kg for Cd. Most of the reported values in this study were in the range of the natural uncontaminated surface soil concentrations and published values in many countries in the world. The results showed that the relation between the distribution of the natural radionuclides and depth was approximately the same for all radionuclides except for 137 Cs, which was extremely binded in the upper layers of soil. In addition, some differences in the concentrations of the studied trace elements with depth were observed. These differences may be due to the average of rainfall and the existence of some potential sources of contamination of such elements. However, the results of this study can be considered as a database for the natural background in Syria that helps to establish the radiation map of the country.(author)

  6. Cytogenetic studies of marine organisms in the areas with higher contents of natural radionuclides

    International Nuclear Information System (INIS)

    Tsytsugina, V.G.; Floru, Kh.; Polikarpov, G.G.; Chalulu, K.; Gorbenko, V.P.

    2004-01-01

    Chromosome aberrations in cells of marine crustaceans and worms have been studied at sites with a high natural radioactivity level (the Black Sea coast at the mountain Karadag in the Crimea and the Ikaria Island in the Aegean Sea, an area around the hydrothermal spa) as well as at sites with the normal natural radiation level. Higher level of chromosome mutagenesis was found in cells of Melita palmata embryos and in germ and somatic cells of Lycastopsis sp. juveniles in the area around the spa. Probably, chromosome aberrations were induced by higher concentrations of natural radionuclides and their radiation in the environment

  7. Natural radionuclides in rocks and soils of the high-mountain regions of the Great Caucasus

    Science.gov (United States)

    Asvarova, T. A.; Abdulaeva, A. S.; Magomedov, M. A.

    2012-06-01

    The results of the radioecological survey in the high-mountain regions of the Great Caucasus at the heights from 2200 to 3800 m a.s.l. are considered. This survey encompassed the territories of Dagestan, Azerbaijan, Georgia, Chechnya, Northern Ossetia-Alania, Kabardino-Balkaria, Karachay-Cherkessia, and the Stavropol and Krasnodar regions. The natural γ background radiation in the studied regions is subjected to considerable fluctuations and varies from 6 to 40 μR/h. The major regularities of the migration of natural radionuclides 238U, 232Th, 226Ra, and 40K in soils in dependence on the particular environmental conditions (the initial concentration of the radionuclides in the parent material; the intensity of pedogenesis; the intensity of the vertical and horizontal migration; and the geographic, climatic, and landscape-geochemical factors) are discussed.

  8. Natural-Series Radionuclides in Traditional Aboriginal Foods in Tropical Northern Australia: A Review

    Directory of Open Access Journals (Sweden)

    Paul Martin

    2004-01-01

    Full Text Available This paper gives a review of available information on natural-series radionuclides in traditional Aboriginal foods of northern Australia. Research on this topic has been carried out primarily for radiological impact assessment purposes in relation to uranium mining activities in the region. Many of the studies have concentrated on providing purely concentration data or concentration ratios, although more detailed uptake studies have been undertaken for freshwater mussels, turtles, and water lilies. The most-studied radionuclides are 238U and 226Ra. However, dose estimates based on current data highlight the importance of 210Po, particularly for the natural (nonmining-related dose. Data on uptake by terrestrial flora and fauna are scarce in comparison with aquatic organisms, and this knowledge gap will need to be addressed in relation to planning for uranium minesite rehabilitation.

  9. Lognormal distribution of natural radionuclides in freshwater ecosystems and coal-ash repositories

    International Nuclear Information System (INIS)

    Drndarski, N.; Lavi, N.

    1997-01-01

    This study summarizes and analyses data for natural radionuclides, 40 K, 226 Ra and 'Th, measured by gamma spectrometry in water samples, sediments and coal-ash samples collected from regional freshwater ecosystems and near-by coal-ash repositories during the last decade, 1986-1996, respectively. The frequency plots of natural radionuclide data, for which the hypothesis of the regional scale log normality was accepted, exhibited single population groups with exception of 226 Ra and 232 Th data for waters. Thus the presence of break points in the frequency distribution plots indicated that 226 Ra and 232 Th data for waters do not come from a single statistical population. Thereafter the hypothesis of log normality was accepted for the separate population groups of 226 Ra and '-32 Th in waters. (authors)

  10. Modelling the impact of discharges of technologically enhanced natural series radionuclides in the marine environment

    International Nuclear Information System (INIS)

    Scott, E.M.; Baxter, M.S.

    1997-01-01

    Natural radionuclides are used within the marine environment to study particle associated processes such as scavenging and sedimentary re-working (Th-234) and to date events and measure rates (Pb-210). In addition, Po-210 has been shown to make a significant contribution to the collective dose of the world population through consumption of marine products (fish). The interpretation of observed activity ratios in the environment is presented, based on earlier description. The natural marine system may however undergo a number of disturbances on a local scale due to discharges of technologically enhanced radionuclides from industrial processes such as phosphate ore processing and scaling in oil and gas production. Some work done to extend the original Bateman equations is shown to describe the behaviour of a decay series under a number of different types of perturbations, and the approach is demonstrated through simulation of a simple system. (author)

  11. Quantum-cascade laser photoacoustic detection of methane emitted from natural gas powered engines

    Science.gov (United States)

    Rocha, M. V.; Sthel, M. S.; Silva, M. G.; Paiva, L. B.; Pinheiro, F. W.; Miklòs, A.; Vargas, H.

    2012-03-01

    In this work we present a laser photoacoustic arrangement for the detection of the important greenhouse gas methane. A quantum-cascade laser and a differential photoacoustic cell were employed. A detection limit of 45 ppbv in nitrogen was achieved as well as a great selectivity. The same methodology was also tested in the detection of methane issued from natural gas powered vehicles (VNG) in Brazil, which demonstrates the excellent potential of this arrangement for greenhouse gas detection emitted from real sources.

  12. Weathering products of basic rocks as sorptive materials of natural radionuclides

    International Nuclear Information System (INIS)

    Omelianenko, B.I.; Niconov, B.S.; Ryzhov, B.I.; Shikina, N.D.

    1994-06-01

    The principal requirements for employing natural minerals as buffer and backfill material in high-level waste (HLW) repositories are high sorptive properties, low water permeability, relatively high thermal conductivity, and thermostability. The major task of the buffer is to prevent the penetration of radionuclides into groundwater. The authors of this report examined weathered basic rocks from three regions of Russia in consideration as a suitable radioactive waste barrier

  13. Natural Radionuclides and Isotopic Signatures for Determining Carbonaceous Aerosol Sources, Aerosol Lifetimes, and Washout Processes

    International Nuclear Information System (INIS)

    Gaffney, Jeffrey

    2012-01-01

    This is the final technical report. The project description is as follows: to determine the role of aerosol radiative forcing on climate, the processes that control their atmospheric concentrations must be understood, and aerosol sources need to be determined for mitigation. Measurements of naturally occurring radionuclides and stable isotopic signatures allow the sources, removal and transport processes, as well as atmospheric lifetimes of fine carbonaceous aerosols, to be evaluated.

  14. Determination of artificial and natural radionuclides and others trace elements in environmental samples form Antarctica

    International Nuclear Information System (INIS)

    Schuch, L.A.; Godoy, J.M.; Nordemann, D.J.R.

    1994-01-01

    The results of the radioactive elements concentrations, determined by gamma spectrometry and the others trace elements determined by neutron activation analysis of several environmental samples (soils, marine sediments, algae mosses and lichens) in Comandante Ferraz Antartica Station are presented. The high concentrations of Cs-137 were found in lichens and mosses samples and the soils and sediments showed concentrations of natural radionuclides. (C.G.C.). 8 refs, 1 fig, 3 tabs

  15. Natural Radionuclides and Isotopic Signatures for Determining Carbonaceous Aerosol Sources, Aerosol Lifetimes, and Washout Processes

    Energy Technology Data Exchange (ETDEWEB)

    Gaffney, Jeffrey [Univ. of Arkansas, Little Rock, AR (United States)

    2012-12-12

    This is the final technical report. The project description is as follows: to determine the role of aerosol radiative forcing on climate, the processes that control their atmospheric concentrations must be understood, and aerosol sources need to be determined for mitigation. Measurements of naturally occurring radionuclides and stable isotopic signatures allow the sources, removal and transport processes, as well as atmospheric lifetimes of fine carbonaceous aerosols, to be evaluated.

  16. Natural and man-made radionuclide concentrations in marine sediments of Gokova Bay, Aegean Turkish coast

    International Nuclear Information System (INIS)

    Tanbay, A.U.; Yener, G.; Mulsow, S.; Fowler, S.W.; Duman, M.

    1999-01-01

    The purpose of this research is to define a baseline study of selected radionuclides (natural and man made) on sediments collected along Goekova Bay. A total of six sediment cores (gravity corer) were collected, each sediment core was sliced in sections and 210 Po, 210 Pb, 226 Ra, 232 Th and 40 K and 137 Cs, 239,240 Pu, 238 Pu and 241 Am were determined for each layer of sediment

  17. MCNP modelling of scintillation-detector gamma-ray spectra from natural radionuclides.

    Science.gov (United States)

    Hendriks, P H G M; Maucec, M; de Meijer, R J

    2002-09-01

    gamma-ray spectra of natural radionuclides are simulated for a BGO detector in a borehole geometry using the Monte Carlo code MCNP. All gamma-ray emissions of the decay of 40K and the series of 232Th and 238U are used to describe the source. A procedure is proposed which excludes the time-consuming electron tracking in less relevant areas of the geometry. The simulated gamma-ray spectra are benchmarked against laboratory data.

  18. Individual and collective dose rates from naturally-occurring radionuclides in seafood

    International Nuclear Information System (INIS)

    Pentreath, R.J.; Camplin, W.C.; Allington, D.J.

    1989-01-01

    Although seafoods are not a large item in the UK diet, they are of interest because of the above-average quantities of naturally-occurring radionuclides which they contain -particularly shellfish. The single most important contributor is 210 Po; studies have therefore been made to examine the contribution which this nuclide makes to the dose received, both collectively and to individual high-rate consumers of shellfish. (author)

  19. Natural radionuclides in the South Indian foods and their annual dose

    Energy Technology Data Exchange (ETDEWEB)

    Shanthi, G., E-mail: shanthidickson@gmail.co [Department of Physics, Women' s Christian College, Nagercoil 629001, Tamil Nadu (India); Thampi Thanka Kumaran, J. [Department of Physics, NM Christian College, Marthandam 629165, Tamil Nadu (India); Gnana Raj, G. Allan [Department of Chemistry and Research Centre, Scott Christian College, Nagercoil 629003, Tamil Nadu (India); Maniyan, C.G [Health Physics Unit, Indian Rare Earths, Manavalakurichi 629252, Tamil Nadu (India)

    2010-07-21

    The study was carried out to evaluate the radioactivity concentration in the food crops grown in high-level natural radioactive area (HLNRA) in south west India. Food samples collected were analysed by means of a gamma spectroscopy and estimated annual dietary intakes of the radioisotopes {sup 226}Ra, {sup 228}Ra, {sup 228}Th and {sup 40}K. The annual intake of the food stuffs was estimated on the basis of their average annual consumption. Calculations were also made to determine the effective dose to an individual consuming such diets. The intakes of these radionuclides were calculated using the concentrations in south Indian foods and daily consumption rates of these foods. Daily intakes of these radionuclides were as follows: {sup 226}Ra, 0.001-1.87; {sup 228}Ra, 0.0023-1.26, {sup 228}Th, 0.01-14.09 {sup 40}K, 0.46-49.39 Bq/day. The daily internal dose resulting from ingestion of radionuclides in food was 4.92 {mu}Sv/day and the annual dose was 1.79 mSv/yr. The radionuclides with highest consumption is {sup 40}K.

  20. Natural radionuclides in the South Indian foods and their annual dose

    International Nuclear Information System (INIS)

    Shanthi, G.; Thampi Thanka Kumaran, J.; Gnana Raj, G. Allan; Maniyan, C.G

    2010-01-01

    The study was carried out to evaluate the radioactivity concentration in the food crops grown in high-level natural radioactive area (HLNRA) in south west India. Food samples collected were analysed by means of a gamma spectroscopy and estimated annual dietary intakes of the radioisotopes 226 Ra, 228 Ra, 228 Th and 40 K. The annual intake of the food stuffs was estimated on the basis of their average annual consumption. Calculations were also made to determine the effective dose to an individual consuming such diets. The intakes of these radionuclides were calculated using the concentrations in south Indian foods and daily consumption rates of these foods. Daily intakes of these radionuclides were as follows: 226 Ra, 0.001-1.87; 228 Ra, 0.0023-1.26, 228 Th, 0.01-14.09 40 K, 0.46-49.39 Bq/day. The daily internal dose resulting from ingestion of radionuclides in food was 4.92 μSv/day and the annual dose was 1.79 mSv/yr. The radionuclides with highest consumption is 40 K.

  1. Radiochemical and radioecological studies of natural and artificial alpha-emitting radionuclides

    International Nuclear Information System (INIS)

    Holm, E.; Persson, B.

    1980-01-01

    Transuranium elements, including uranium and thorium, were analyzed in both marine and terrestrial samples. Vertical profiles of 239+240 Pu, 241 Am, 230 Th, and 238 U, in the Pacific, the Mediterranean, and the Atlantic, measured by different investigators, were compared. Uptake of the fallout isotopes 241 Pu, 240+239 Pu, 238 Pu, and 241 Am in the lichen - reindeer food chain was studied. Americium and thorium exhibited similar biophysical behavior in the environment and in the water column, although the settling velocity for thorium was somewhat higher. Plutonium showed similar distribution in the water columns in different waters. The fraction of ingested plutonium which was retained in the body of reindeer was in good agreement with the value of 3 x 10 -5 predicted for man. Uranium showed a constant concentration in the water column, with a low affinity to particles in the water. The high concentration of uranium in reindeer tissues depended on high intake from drinking water and foodstuffs other than lichens

  2. Naturally occurring radionuclides transfer factor on aquatic flora and fauna in Nagarjuna Sagar Dam near proposed uranium mining site

    International Nuclear Information System (INIS)

    Arunachalam, Kantha Deivi

    2015-04-01

    Naturally occurring radioactive element can be found in low levels within all rock, soil, and water. The present work aims to understand the transfer of naturally occurring radionuclides in different compartments of environment reflecting its behaviour in different tropic levels. The understanding and evaluation of the possible interactions of various naturally occurring radionuclides were done in the world's third largest man-made dam, Nagarjuna Sagar, built on river Krishna located in Andhra Pradesh, India. The naturally occurring radionuclides such as Uranium ( 238 U), Polonium ( 210 Po), Radium ( 226 Ra), and Lead ( 210 Pb) were analyzed in different matrices (i.e) sediment, water, and fish. The measurement of the naturally occurring radionuclides in the environment can be used as a reference baseline for long-term monitoring in the entire aquatic ecosystem

  3. Natural radionuclides by gammaspectrometry in region of West-south Serbia, for 1998, 1997 and 1996

    Energy Technology Data Exchange (ETDEWEB)

    Tanaskovic, I.; Vukovic, D.M. [Institute of Occupational and Radiological Health, Deligradska 29, Belgrade, Yugoslavia, Faculty of Physical Chemistry, Studentski trg 12, Belgrade (Yugoslavia); Markovic, D. [Faculty of Physical Chemistry, Belgrade (Yugoslavia)

    2000-05-01

    Region of West Serbia, known as Uzicki region, as a agriculture and industry region, with cities: Uzice, Cacak, Kraljevo and Valjevo is important part of Yugoslavia for development. Radioactivity comes mostly from natural radionuclides and partly from long-lived radionuclides from non natural sources as a consequence of Chernobyl accident. Monitoring of environment has proceeded by vertical methodology. We analyzed: aerosol, soil, fallout (wet and dry deposition), rivers, lakes, drinking water, human and animal food. Results from analyze of samples of environment contains very low activity, actually activity of changes of basic signal. Results for 1998, 1997 and 1996 are: 1. Gamma dose was measure in Belgrade with median years values: 0.103 {mu}G/h (1998), 0.077 {mu}G/h (1997) and 0.0722 {mu}G/h (1996). 2. By gammaspectrometry analyze of air of months samples for each year, results shows activity of changes of basic signal. The signals are coming from natural radionuclides. 3. {sup 137}Cs, as a long lived radionuclide, with remarkable activity in soil analyzed from Zlatibor and result are :32.3-173 Bq/kg (1998), -Bq/kg (1997) and 33-122.7 Bq/kg (1996). 4. Activity in the rivers for these region not analyzed. 5. Activity of drinking waters, from city network shows low level of activity which comes from {sup 40}K, for both places. 6. Activity in human food, measured in yogurt, meats, bread and agricultural products comes from {sup 40}K Uzice 32.4-168 Bq/kg (1998), Bq/kg (1997) and 55.2-164 Bq/kg (1996). Activities of {sup 137}Cs are 1 Bq/kg. Results of analyze of animal food shows same results. The samples were collected according to methods determined by the Regulations. (author)

  4. Natural radionuclides by gammaspectrometry in region of West-south Serbia, for 1998, 1997 and 1996

    International Nuclear Information System (INIS)

    Tanaskovic, I.; Vukovic, D.M.; Markovic, D.

    2000-01-01

    Region of West Serbia, known as Uzicki region, as a agriculture and industry region, with cities: Uzice, Cacak, Kraljevo and Valjevo is important part of Yugoslavia for development. Radioactivity comes mostly from natural radionuclides and partly from long-lived radionuclides from non natural sources as a consequence of Chernobyl accident. Monitoring of environment has proceeded by vertical methodology. We analyzed: aerosol, soil, fallout (wet and dry deposition), rivers, lakes, drinking water, human and animal food. Results from analyze of samples of environment contains very low activity, actually activity of changes of basic signal. Results for 1998, 1997 and 1996 are: 1. Gamma dose was measure in Belgrade with median years values: 0.103 μG/h (1998), 0.077 μG/h (1997) and 0.0722 μG/h (1996). 2. By gammaspectrometry analyze of air of months samples for each year, results shows activity of changes of basic signal. The signals are coming from natural radionuclides. 3. 137 Cs, as a long lived radionuclide, with remarkable activity in soil analyzed from Zlatibor and result are :32.3-173 Bq/kg (1998), -Bq/kg (1997) and 33-122.7 Bq/kg (1996). 4. Activity in the rivers for these region not analyzed. 5. Activity of drinking waters, from city network shows low level of activity which comes from 40 K, for both places. 6. Activity in human food, measured in yogurt, meats, bread and agricultural products comes from 40 K Uzice 32.4-168 Bq/kg (1998), Bq/kg (1997) and 55.2-164 Bq/kg (1996). Activities of 137 Cs are 1 Bq/kg. Results of analyze of animal food shows same results. The samples were collected according to methods determined by the Regulations. (author)

  5. Colloid migration in groundwaters: Geochemical interactions of radionuclides with natural colloids. Final report

    International Nuclear Information System (INIS)

    Kim, J.J.; Longworth, G.; Hasler, S.E.; Gardiner, M.; Fritz, P.; Klotz, D.; Lazik, D.; Wolf, M.; Geyer, S.; Alexander, J.L.; Read, D.; Thomas, J.B.

    1994-08-01

    In this joint research programme the significance of groundwater colloids in far field radionuclide migration has been studied. The characterization, quantification and theoretical interpretation of colloid-borne transport phenomena for radionuclides were the main objectives of this research programme. Groundwaters, colloids and sediments were sampled from aquifer system overlying a saltdome in the Gorleben area in northern Germany and were characterized by various analytical methods (ICP-MS, ICP-AES, neutron activation analysis (NAA), DOC-Analyser, HPIC, potentiometric titration). Different natural isotopes ( 2 H, 3 H, 13 C, 14 C, 18 O, 34 S, U/Th decay series) were determined and their ratios were compared with one another in the order to ascertain the provenance of the groundwater colloids. The investigated groundwaters contain substantial amounts of colloids mainly composed of humic and fulvic acids loaded with various metal ions. The chemical interaction of radionuclide ions of various oxidation states (Am, Eu, for M(III), Th, Pu for M(IV), Np for M(V) and U for M(VI)) with groundwater colloids was investigated in order to elucidate the colloid facilitated migration behaviour of actinides in a given aquifer system. Transport process studies with generated pseudocolloids of radionuclides in various oxidation states were undertaken in scaled column experiments, pre-equilibrated with colloid rich Gorleben groundwater. A modelling programme was developed to predict chemical transport of radionuclides in the presence of humic colloids using a modified version of the CHEMTARD code. Modelling predictions have generated acceptable results for Eu, Am and U and poorer agreement between experimental and modelling results for Th and Np as a result of more limited data. (orig.)

  6. Colloid migration in groundwaters: Geochemical interactions of radionuclides with natural colloids. Final report

    Energy Technology Data Exchange (ETDEWEB)

    Kim, J.J. [Technische Univ. Muenchen, Garching (Germany). Inst. fuer Radiochemie; Delakowitz, B. [Technische Univ. Muenchen, Garching (Germany). Inst. fuer Radiochemie; Zeh, P. [Technische Univ. Muenchen, Garching (Germany). Inst. fuer Radiochemie; Probst, T. [Technische Univ. Muenchen, Garching (Germany). Inst. fuer Radiochemie; Lin, X. [Technische Univ. Muenchen, Garching (Germany). Inst. fuer Radiochemie; Ehrlicher, U. [Technische Univ. Muenchen, Garching (Germany). Inst. fuer Radiochemie; Schauer, C. [Technische Univ. Muenchen, Garching (Germany). Inst. fuer Radiochemie; Ivanovich, M. [AEA Environment and Energy, Harwell (United Kingdom); Longworth, G. [AEA Environment and Energy, Harwell (United Kingdom); Hasler, S.E. [AEA Environment and Energy, Harwell (United Kingdom); Gardiner, M. [AEA Decommissioning and Radwaste, Harwell (United Kingdom); Fritz, P. [Gesellschaft fuer Strahlen- und Umweltforschung mbH Muenchen, Neuherberg (Germany); Klotz, D. [Gesellschaft fuer Strahlen- und Umweltforschung mbH Muenchen, Neuherberg (Germany); Lazik, D. [Gesellschaft fuer Strahlen- und Umweltforschung mbH Muenchen, Neuherberg (Germany); Wolf, M. [Gesellschaft fuer Strahlen- und Umweltforschung mbH Muenchen, Neuherberg (Germany); Geyer, S. [Gesellschaft fuer Strahlen- und Umweltforschung mbH Muenchen, Neuherberg (Germany); Alexander, J.L. [Atkins (W.S.) Engineering Sciences, Epsom (United Kingdom); Read, D. [Atkins (W.S.) Engineering Sciences, Epsom (United Kingdom); Thomas, J.B. [Atkins (W.S.) Engineering Sciences, Epsom (United Kingdom)

    1994-08-01

    In this joint research programme the significance of groundwater colloids in far field radionuclide migration has been studied. The characterization, quantification and theoretical interpretation of colloid-borne transport phenomena for radionuclides were the main objectives of this research programme. Groundwaters, colloids and sediments were sampled from aquifer system overlying a saltdome in the Gorleben area in northern Germany and were characterized by various analytical methods (ICP-MS, ICP-AES, neutron activation analysis (NAA), DOC-Analyser, HPIC, potentiometric titration). Different natural isotopes ({sup 2}H, {sup 3}H, {sup 13}C, {sup 14}C, {sup 18}O, {sup 34}S, U/Th decay series) were determined and their ratios were compared with one another in the order to ascertain the provenance of the groundwater colloids. The investigated groundwaters contain substantial amounts of colloids mainly composed of humic and fulvic acids loaded with various metal ions. The chemical interaction of radionuclide ions of various oxidation states (Am, Eu, for M(III), Th, Pu for M(IV), Np for M(V) and U for M(VI)) with groundwater colloids was investigated in order to elucidate the colloid facilitated migration behaviour of actinides in a given aquifer system. Transport process studies with generated pseudocolloids of radionuclides in various oxidation states were undertaken in scaled column experiments, pre-equilibrated with colloid rich Gorleben groundwater. A modelling programme was developed to predict chemical transport of radionuclides in the presence of humic colloids using a modified version of the CHEMTARD code. Modelling predictions have generated acceptable results for Eu, Am and U and poorer agreement between experimental and modelling results for Th and Np as a result of more limited data. (orig.)

  7. Determination of naturally occurring radionuclides in soil samples of Ayranci, Turkey

    Science.gov (United States)

    Agar, Osman; Eke, Canel; Boztosun, Ismail; Emin Korkmaz, M.

    2015-04-01

    The specific activity, radiation hazard index and the annual effective dose of the naturally occurring radioactive elements (238U, 232Th and 40K) were determined in soil samples collected from 12 different locations in Ayranci region by using a NaI(Tl) gamma-ray spectrometer. The measured activity concentrations of the natural radionuclides in studied soil samples were compared with the corresponding results of different countries and the internationally reported values. From the analysis, it is found that these materials may be safely used as construction materials and do not pose significant radiation hazards.

  8. Natural radionuclides in an eucalyptus forest located in the south of Spain

    International Nuclear Information System (INIS)

    Vaca, F.; Manjon, G.; Garcia-Leon, M.

    2000-01-01

    A pulp mill and the forest from which the raw material for its operation is collected have been studied since 1992 with respect to the natural radioactivity involved. The activity concentrations of 234 U, 238 U, 228 Th, 230 Th, 232 Th in forest samples (soils, wood, barks), were determined using alpha and gamma spectrometry. Radium and thorium isotopes were analyzed using the conventional radiochemical method. For gamma spectrometry, the HPGe detector efficiency was determined using the generalized transmission method developed by Bolivar et al. The results obtained by the two techniques are presented. The natural radionuclide distribution, activity ratio and relative activities among the forest compartments (soil, wood and barks) are given

  9. The encounter and analysis of naturally occurring radionuclides in gas and oil production and processing

    International Nuclear Information System (INIS)

    Hartog, F.A.; Jonkers, G.; Knaepen, W.A.I.

    1996-01-01

    As a result of oil and gas production, radioactive daughter elements from the uranium and thorium decay series can be mobilized and transported away from the reservoir. Due to changes in flow regime, temperature, pressure or chemical environment NORs (Naturally Occurring Radionuclides) may build up in products, by-products or waste streams from gas and oil production and processing facilities. Products containing NORs are commonly denoted by the acronym NORM (Naturally Occurring Radioactive Materials). Main topics of this paper are: E and P (Exploration and Production) NORM characteristics; incentives for NORM analysis; NORM analysis; interlaboratory test programme; analysis techniques; results and conclusions of the test programme. 4 figs., 2 tabs

  10. Natural radionuclides concentration in agricultural products and water from the Monte Alegre region

    International Nuclear Information System (INIS)

    Gouvea, Vandir A.; Melo, Vicente P.; Binns, Donald A.C.; Santos, Pedro L. dos

    1997-01-01

    Measurements to determine the content of natural radionuclides were performed in agricultural products in the brazilian Central Amazon Basin Monte Alegre region, for the soil-plant transfer calculation. these measurements were concentrated in the Ingles de Souza agricultural settlement, were several uranium and thorium occurrences exist in geological formations called Monte Alegre and Faro. The values obtained in foodstuff cultivated in the anomalous region are 10 times higher than those ones observed in the Alenquer region, which is the chosen region due to its low level natural radioactivity and its proximity to the anomalous region. (author). 9 refs., 4 tabs

  11. Natural radionuclides in waste water discharged from coal-fired power plants in Serbia.

    Science.gov (United States)

    Janković, Marija M; Todorović, Dragana J; Sarap, Nataša B; Krneta Nikolić, Jelena D; Rajačić, Milica M; Pantelić, Gordana K

    2016-12-01

    Investigation of the natural radioactivity levels in water around power plants, as well as in plants, coal, ash, slag and soil, and to assess the associated radiation hazard is becoming an emerging and interesting topic. This paper is focused on the results of the radioactivity analysis in waste water samples from five coal-fired power plants in Serbia (Nikola Tesla A, Nikola Tesla B, Kolubara, Morava and Kostolac), which were analyzed in the period 2003-2015. River water samples taken upstream and downstream from the power plants, drain water and overflow water were analyzed. In the water samples gamma spectrometry analysis was performed as well as determination of gross alpha and beta activity. Natural radionuclide 40 K was detected by gamma spectrometry, while the concentrations of other radionuclides, 226 Ra, 235 U and 238 U, usually were below the minimum detection activity (MDA). 232 Th and artificial radionuclide 137 Cs were not detected in these samples. Gross alpha and beta activities were determined by the α/β low level proportional counter Thermo Eberline FHT 770 T. In the analyzed samples, gross alpha activity ranged from MDA to 0.47 Bq L - 1 , while the gross beta activity ranged from MDA to 1.55 Bq L - 1 .

  12. Natural radionuclides and 137Cs in moss and lichen in eastern Serbia

    Directory of Open Access Journals (Sweden)

    Čučulović Ana

    2012-01-01

    Full Text Available The paper presents the results of radionuclides determination in moss (Homolothecium sp., Hypnum Cupressiforme sp., and Brachythecium sp. and lichen (Cladonia sp. sampled in the region of Eastern Serbia during 1996-2010. The activities in moss are in the range of 100-500 Bq/kg d. w. for 40K, and 5-50 Bq/kg d. w. for 226Ra and 232Th, while the “soil-to-moss” transfer factors are 0.45 for 40K, 3 for 226Ra, and 0.3 for 232Th. The spatial distribution of the 137Cs activities is highly non-uniform; some values reach 500 Bq/kg d. w., with less than 10% of the samples, mainly the ones taken prior to 2000, with the activity above 1000 Bq/kg d. w. The variations in the content of natural radionuclides among the moss species are not significant. The frequency pattern of the activities of natural radionuclides in lichen is similar to the one in moss, but the activities in lichen are to some extent lower. The mean activity of 137Cs in lichen is below 400 Bq/kg d. w. The mean activities of 7Be in moss and lichen sampled in 2006 and 2008 are in the range of 41-122 Bq/kg d. w., with pronounced variations between the sampling sites.

  13. Radiological impact due to natural radionuclides (U and Th-isotopes) in soils from Salamanca, Mexico

    Energy Technology Data Exchange (ETDEWEB)

    Mandujano G, C. D.; Sosa, M. [Universidad de Guanajuato, Division de Ciencias e Ingenierias, Loma del Bosque 103, Col. Lomas del Campestre, 37150 Leon, Guanajuato (Mexico); Mantero, J.; Manjon, G.; Garcia T, R. [Universidad de Sevilla, Grupo en Fisica Nuclear Aplicada, Av. Reina Mercedes No. 2, 41012 Sevilla (Spain); Costilla, R., E-mail: cmandujano@fisica.ugto.mx [Universidad de Guanajuato, Division de Ciencias de la Vida, Departamento de Ciencias Ambientales, Ex-Hacienda El Copal Km 9 Irapuato-Silao, 36500 Irapuato, Guanajuato (Mexico)

    2015-10-15

    Full text: Activity concentrations of U ({sup 238}U, {sup 234}U) and Th ({sup 232}Th, {sup 230}Th) radionuclides in samples of superficial urban soils surrounding an industrial complex in Salamanca, Mexico have been determined. Levels of naturally occurring radionuclides (Norm) in the environment may be affected due to the presence of different industrial activities in this zone, representing a potential radiological risk for the population which should be evaluated. Alpha-particle Spectrometry with Pips detectors has been used for the radiometric characterization. A well established radiochemical procedure was used for the isolation of the radionuclides of interest. Alkali fusion for sample digestion, liquid-liquid extraction with Tbp (tri-butyl-phosphate) for U and Th isolation and electrodeposition in stainless steel dishes for measurement conditioning has been used. The results cover the ranges of 10-42, 12-60, 12-52 and 11-51 Bq·kg{sup -1} for {sup 238}U, {sup 234}U, {sup 230}Th, and {sup 232}Th respectively, being not observed any clear anthropogenic increments in relation with the values normally found in unaffected soils. Although there is disequilibrium between U isotopes and {sup 230}Th in some soil samples, it can be attributed to natural processes. The radiological impact of the industrial activities in the surrounding soils can be then evaluated as very low. Hence, from the Radiological Protection point of view, the soils studied do not represent a radiological risk for the health of the population. (Author)

  14. Determination of naturally occurring radionuclides in scales produced in oil industry

    Energy Technology Data Exchange (ETDEWEB)

    Al-Masri, M S; Ali, A F; Kitue, M; Kawash, A [Atomic Energy Commission, Dept. of Radiation Protection and Nuclear Safety, Damascus (Syrian Arab Republic)

    1997-04-01

    Scales produced by Oil production operations contain relatively high concentrations of natural radionuclides especially radium isotopes (Ra-226, Ra-228, Ra-224) and their daughters. These scales deposit in oil surface equipment such as separator tanks, tubular, and storage tanks. In this work, naturally occurring radionuclides and radiation exposure levels in some Syrian oil lines have been determined. Radiation measurements have shown high radiation exposure in some production sites and reached about 23 {mu}Sv/hr (production wellhead) which is higher than the normal background (0.09 - 012 {mu}Sv/hr). The highest value of the exposure around storage tanks was about o.5 {mu}Sv/hr. Moreover, the highest concentration of radionuclides in scales were found to be 47000 Bq/Kg and 55000 Bq/Kg for Ra-226 and Ra-228 respectively while in sludge samples, the Ra-226 concentration was about 24.2 Bq/Kg, a relatively very low activity. In addition, results have shown that soil contamination can occur by disposal of produced water to the surrounding environment. Furthermore, the present paper shows some of protection procedures, which should be followed by workers for radiation protection. (author). 10 refs., 4 tabs.

  15. Analysis of the Research Status and Topics on the Radionuclide Migration and Retardation in Natural Barriers

    International Nuclear Information System (INIS)

    Baik, Min Hoon; Park, Chung Kyun; Kim, Seung Soo; Lee, Seung Yeop; Lee, Jae Kwang

    2008-12-01

    In this report, recent research status for major developed countries in the high-level radioactive waste disposal including international organizations was investigated and analyzed in research topics for the radionuclide migration and retardation in natural barriers. Besides, recent research trends and future prospects were investigated for selected major 10 topics about the radionuclide migration and retardation processes. Based upon these investigations and analyses, future research goals and topics to be concentrated were presented. This report will be helpful for understanding our current research status and technical position and establishing future research direction and topics by analyzing domestic and foreign research status and trends. The results will also be utilized as basic information for establishing future policy and plans of the government for the high-level radioactive waste disposal

  16. Distribution of selected natural radionuclides in soil of the district Ziar nad Hronom

    International Nuclear Information System (INIS)

    Porubcanova, B.; Nikodemova, D.; Mojzes, A.

    2015-01-01

    Slovakia like a part of a difficult geological structure of the Western Carpathians is a typical place with a different field of radioactivity. The district Ziar nad Hronom belongs to regions which are characteristic by their high values of radioactivity in comparison with Slovakia. It is due to a geological background which is mostly compound from neovulcanites. In this area were measurement concentrations of uranium-238, thorium- 232 and potassium-40. Consequently, these values were shown by maps which reflect distribution of chosen radionuclides. Sequential research was focus on demographic processing. There turned out that in this area is increased number of deaths in particular due to malignancies. This fact can be affected by natural radionuclides which exist in this area. (authors)

  17. Study on radionuclides transport from natural evaporating ponds to the atmosphere

    International Nuclear Information System (INIS)

    Liu Keqiang; Zou Changgui

    1997-08-01

    The results of simulated experiments, field monitoring and radiation health risk evaluation of radionuclides transport to the atmosphere from the natural evaporating ponds of a certain nuclear factory, and the estimating method of releasing source strength are presented. The estimated results of radiation health risk show that the maximum individual annual risk is 6.5 x 10 -9 and the total collective annual risk within a radius of 20 km is 3.2 x 10 -5 person, which are caused by operation of the evaporating ponds. It should be pointed out that the above estimated results only refer to one operating year (1990). If the cumulative effect of radionuclides deposition in ground is considered, the risk will increase a little with time until the dynamic balance is achieved. (5 ref., 8 tabs.)

  18. Natural radionuclides from the coal in atmospheric environment of the coal fired power plants

    International Nuclear Information System (INIS)

    Antic, D.; Kostic-Soskic, M.; Milovanovic, S.; Telenta, B.

    1995-01-01

    The inhalation radiation exposure of the public in the vicinity of the selected coal fired power plants near from Belgrade (30-50 km) has been studied, using a set of data for natural radionuclides from the analysed power plants. A generalised model for analysis of radiological impact of an energy source, that includes the two-dimensional version of the cloud model, has been used for simulation of the transport of radionuclides released to the atmosphere. The inhalation dose rates for an adult are assessed and analysed during fast changeable meteorological conditions. A set of realistic meteorological conditions (wind, radiosonde sounding temperature, pressure, and humidity data) has been used for the numerical simulations. (author)

  19. Identification of some heavy metals and natural radionuclides levels in Mzerib lake environment

    International Nuclear Information System (INIS)

    Al-Nimeh, M.; Al-Rayyes, A.; Al-Masri, M. S.

    2002-01-01

    Some trace metals (Cd, Pb, Cu, and Zn) and natural radionuclides ( 238 U, 210 Po, 210 Pb) were measured in environmental samples from Mzerib lake during 1998. This will help in evaluating the water quality and the effects of agricultural and humanitarian activities on the lake environment. Results showed that the lake water is of a good quality. Trace metals levels in water, sediments, freshwater clam (Unio terminals), and fish (cyprinus Cario) fall within the accepted range, although they were higher in some sites due to the presence of a potential source for pollution (e.g. the restaurant). The clam soft tissue samples showed the highest levels of Cd. Carp fish gonads and gills also showed high levels of cadmium, while Carp fish samples showed the highest levels of zinc. radionuclides levels were low and in agreement with levels reported in previous local and international studies. (authors)

  20. Analysis of the Research Status and Topics on the Radionuclide Migration and Retardation in Natural Barriers

    Energy Technology Data Exchange (ETDEWEB)

    Baik, Min Hoon; Park, Chung Kyun; Kim, Seung Soo; Lee, Seung Yeop; Lee, Jae Kwang [Korea Atomic Energy Research Institute, Daejeon (Korea, Republic of)

    2008-12-15

    In this report, recent research status for major developed countries in the high-level radioactive waste disposal including international organizations was investigated and analyzed in research topics for the radionuclide migration and retardation in natural barriers. Besides, recent research trends and future prospects were investigated for selected major 10 topics about the radionuclide migration and retardation processes. Based upon these investigations and analyses, future research goals and topics to be concentrated were presented. This report will be helpful for understanding our current research status and technical position and establishing future research direction and topics by analyzing domestic and foreign research status and trends. The results will also be utilized as basic information for establishing future policy and plans of the government for the high-level radioactive waste disposal.

  1. Report on the IAEA-CU-2006-11 proficiency test on the determination of gamma emitting radionuclides in air filters

    International Nuclear Information System (INIS)

    Shakhashiro, A.; Kim, C.-K.; Sansone, U.; Ferrari, M.; Sill, D.

    2006-10-01

    This report summarises the results of the IAEA-CU-2006-11 proficiency test on the determination of gamma emitting radionuclides in air filters, organised within the frame of the IAEA Technical Cooperation project RER/8/009 ''Air Pollution Monitoring in the Mediterranean Region''. The proficiency test was conducted by the Reference Materials Group of the Chemistry Unit (Physics, Chemistry and Instrumentation Laboratory) of the IAEA's analytical laboratories located in Seibersdorf (Austria) in cooperation with the Radiological and Environmental Sciences Laboratory, Department of Energy in the United States of America. The objective of TC project RER/8/009 is to contribute to air quality improvement through the establishment of a network for air monitoring and the design of a remedial strategy where the monitoring shows poor air quality. A spiked air filter with known activities of gamma emitting radionuclides prepared by the Department of Energy of the United States of America was used in this proficiency test. 14 spiked filters were distributed to the participating laboratories in April 2006. The deadline for receiving the results from the participants was set at 31 July 2006. The participating laboratories were requested to analyse the samples employing the methods used in their routine work, so that their performance on the test samples could be directly related to the real performance of the laboratory. Each laboratory was given a confidential code to assure the anonymity of the evaluation results. From the 14 initially registered, 11 laboratories reported their results back to the IAEA. The analytical results of the participating laboratories were evaluated against the reference values assigned to the reference air filter, and a rating system was applied

  2. LOW CONTENT OF RADIONUCLIDES IN NATURAL ENVIRONMENT AND PRODUCTION AS A RATIONALE FOR DEVELOPMENT OF RECREATIONAL POTENTIAL OF NORTHERN BUKOVINA

    Directory of Open Access Journals (Sweden)

    Natalia OMEL’CHENKO

    2017-06-01

    Full Text Available Investigation on food products contamination by Cesium-137 and Strontium-90, detection of content of natural radionuclides (Radium-226, Thorium-232, Potassium-40 in raw materials and finished products of building industry, monitoring of some radionuclides content in soils of mountainous area of Northern Bukovina was carried out. All the results were analyzed and discussed in view of the life safety position. Data on radionuclides content in surrounding natural environment as well as in building and food industry production confirm Northern Bukovina territory’s attractiveness and safety for recreation areas development.

  3. Natural analogue approach for estimating the health risks from release and migration of radionuclides from radioactive waste

    International Nuclear Information System (INIS)

    Gilbert, T.L.

    1983-01-01

    The health risks from radioactive waste may be expressed as a sum of products of transfer factors that characterize the causal chain of events between disposal of radionuclides in a waste field and the consequent health effects. Model estimates for the transfer factors are commonly obtained by modeling transport and other mechanisms in the subsystems that form the links in the causal chain. Natural estimates of some conversion factors for naturally occurring radionuclides can be obtained from data on the concentrations of naturally occurring radionuclides in soil, food, and the human body. These model and natural estimates can be used with scaling procedures to estimate the uncertainties and to obtain better estimates of the values. The scaling procedures take into account the differences in the source characteristics for radionuclides in a waste field of limited size and for radionuclides generally distributed in the natural environment. The ratios of the natural estimates to the model estimates for several transfer factors and several radionuclides belonging to the U-238 decay series have been determined. These ratios range from 1/8 to 4/1 for food-concentration/source-concentration transfer factors for the food pathways and from 1 to 77 for dose-rate/source-concentration transfer factors for the internal radiation dose pathways to various organs. 14 references

  4. Worldwide Open Proficiency Test: Determination of Naturally Occurring Radionuclides in Phosphogypsum and Water

    International Nuclear Information System (INIS)

    2010-01-01

    A reliable determination of naturally occurring radionuclides in phosphogypsum is necessary to comply with the radiation protection and environmental regulations. This proficiency test (PT) is one of the series of the world wide proficiency tests organised every year by the IAEA Terrestrial Environment Laboratory. This series of PTs is designed to identify analytical problems, to support Member State laboratories to maintain their accreditation and to provide a forum for discussions regarding the analysis of naturally occurring radionuclides. The range of sample types available for analysis has been mainly at environmental levels. In this PT, the test item set consisted of six samples: one phosphogypsum (the IAEA-434 reference material) and five water samples spiked with natural radionuclides. The main task of the participating laboratories was to identify and traceably quantify the activity levels of radionuclides present in these matrices. The tasks of the IAEA were to prepare and distribute the samples to the participating laboratories, to collect and interpret analysis results and to compile a comprehensive report. The certified massic activity values of all radionuclides used in this PT were traceable to international standards of radioactivity. In this PT, 1800 test items (reference materials) were prepared and distributed to 300 laboratories from 76 countries in November 2008. The deadline for receiving the results from the participants was set at 15 May 2009. The participating laboratories were requested to analyse Ra-226, U-234 and U-238 in water samples 01 and 02, and gross alpha/beta in water samples 03, 04 and 05. In the phosphogypsum sample number 06 the participants were asked to analyse Pb-210, Ra-226, Th-230, U-234 and U-238. The analytical results of the participating laboratories were compared with the reference values assigned to the reference materials, and a rating system was applied. Three National Metrology Institutes (NMI) and six expert

  5. Treatment techniques for removing natural radionuclides from drinking water. Final report of the TENAWA project

    International Nuclear Information System (INIS)

    Annanmaeki, M.; Turtiainen, T.

    2000-01-01

    TENAWA project (Treatment Techniques for Removing Natural Radionuclides from Drinking Water) was carried out on a cost-shared basic with the European Commission (CEC) under the supervision of Directorate-General XII, Radiation Protection Unit. TENAWA project was started because in several European countries ground water supplies may contain high amounts of natural radionuclides. During the project both laboratory and field research was performed in order to test the applicability of different equipment and techniques for removing natural radionuclides from drinking water. The measurable objectives of the project were: to give recommendations on the most suitable methods for removing radon ( 222 Rn), uranium ( 238,234 U), radium ( 226 , 228 Ra), lead ( 210 Pb) and polonium ( 210 Po) from drinking water of different qualities (i.e. soft, hard, iron-, manganese- and humus-rich, acidic) to test commercially available equipment for its ability to remove radionuclides; to find new materials, absorbents and membranes effective in the removal of radionuclides and to issue guidelines for the treatment and disposal of radioactive wastes produced in water treatment. Radon could be removed efficiently (>95%) from domestic water supplies by both aeration and granular activated carbon (GAC) filtration. Defects in technical reliability or radon removal efficiency were observed in some aerators. The significant drawback of GAC filtration was the elevated gamma dose rates (up to 120 μSv/h) near the filter and the radioactivity of spent GAC. Aeration was found to be a suitable method for removing radon at waterworks, too. The removal efficiencies at waterworks where the aeration process was designed to remove radon or carbon dioxide were 67-99%. If the aeration process was properly designed, removal efficiencies higher than 95% could be attained. Uranium could best be removed (>95%) with strong basic anion exchange resins and radium by applying strong acidic cation exchange resins

  6. Treatment techniques for removing natural radionuclides from drinking water. Final report of the TENAWA project

    Energy Technology Data Exchange (ETDEWEB)

    Annanmaeki, M.; Turtiainen, T. [eds.

    2000-01-01

    TENAWA project (Treatment Techniques for Removing Natural Radionuclides from Drinking Water) was carried out on a cost-shared basic with the European Commission (CEC) under the supervision of Directorate-General XII, Radiation Protection Unit. TENAWA project was started because in several European countries ground water supplies may contain high amounts of natural radionuclides. During the project both laboratory and field research was performed in order to test the applicability of different equipment and techniques for removing natural radionuclides from drinking water. The measurable objectives of the project were: to give recommendations on the most suitable methods for removing radon ({sup 222}Rn), uranium ({sup 238,234}U), radium ({sup 226}, {sup 228}Ra), lead ({sup 210}Pb) and polonium ({sup 210}Po) from drinking water of different qualities (i.e. soft, hard, iron-, manganese- and humus-rich, acidic) to test commercially available equipment for its ability to remove radionuclides; to find new materials, absorbents and membranes effective in the removal of radionuclides and to issue guidelines for the treatment and disposal of radioactive wastes produced in water treatment. Radon could be removed efficiently (>95%) from domestic water supplies by both aeration and granular activated carbon (GAC) filtration. Defects in technical reliability or radon removal efficiency were observed in some aerators. The significant drawback of GAC filtration was the elevated gamma dose rates (up to 120 {mu}Sv/h) near the filter and the radioactivity of spent GAC. Aeration was found to be a suitable method for removing radon at waterworks, too. The removal efficiencies at waterworks where the aeration process was designed to remove radon or carbon dioxide were 67-99%. If the aeration process was properly designed, removal efficiencies higher than 95% could be attained. Uranium could best be removed (>95%) with strong basic anion exchange resins and radium by applying strong

  7. Natural sorbents as barriers against migration of radionuclides from radioactive waste repositories

    International Nuclear Information System (INIS)

    Stefanova, I.; Gradev, G.D.

    1993-01-01

    The sorption properties of Bulgarian inorganic sorbents - clinoptilolite, vermiculite, bentonite, glauconite, celadonite and loess, which can be used as buffer, backfill and sealing materials in radwaste repository are studied. Experimental data about sorption and desorption capacities, radiation and thermal stability of sorbents from different Bulgarian deposits are reported and compared. Clinoptilolite from Beli Plast and its sodium variety from Kostino and Moryantsi is recommended as a barrier against radionuclide migration from radwaste repository due to their high sorption capacity of 137 Ce, 90 Sr and 60 Co. The high selectivity of vermiculite for polyvalent ions ( 144 Ce, 59 Fe and 90 Sr) gives grounds to include the sorption on vermiculite as a second step in the ion exchange technology for low level laundry waste decontamination. Bentonite is studied as a proposed buffer, backfill and sealing material. Its selectivity for cesium is lower compared to those of clinoptilolite. Thus a tailored-made mixture of bentonite and clinoptilolite will act as a barrier against radionuclides in different oxidation state. Glauconite can be successfully used as a barrier against migration of 144 Ce, 90 Sr, 54 Mn and 65 Zn. Loess is also included in the study, as the Kozloduy NPP is sited on loess formation and it is a natural potential site for low and intermediate level waste burial. It is concludes that zeolites and clays of Bulgarian deposits can be used effectively against radionuclide migration from radioactive waste repositories. 59 refs., 5 tabs. (author)

  8. Natural radionuclides and heavy metals in vegetables of people diet from Rio de Janeiro, RJ, Brazil

    International Nuclear Information System (INIS)

    Santos, Eliane Eugenia dos

    2002-01-01

    The characterization of the population exposure to the natural radiation is of extreme importance to set reference levels as a base to a regulatory system. Foodstuff, particularly of vegetable origin, presents variable contents of chemical products, essentials and not essentials according to soil characteristics, agricultural practices, among others. The present work had the goal to establish a methodology that allows evaluating the incorporation of natural radionuclides and heavy metals by the Brazilian population consuming foodstuff from vegetal origin. The results indicate that doses due to the ingestion of natural radionuclides and heavy metals as well in vegetables and derived products consumed by the Rio de Janeiro population are below the reference values set by international organizations. Regarding U and Th decay chain exposure ( 238 U, 23T h, 228 Ra, 226 Ra, 210 Pb), it was estimated an effective dose of 14,5 μSv/a, being 228 Ra, 226 Ra, 210 Pb responsible by 96%. The K-40 ingestion dose was assessed as 103 μSv/a. The daily intake of metals was assess as 2870 μg/d for Zn, 2499 μg/d for Mn, 1064 μg/d Cu, 96 μg/d Ni, 14,8 μg/d Cr, 11 μg/d Cd e 4,8 μg/d Pb. The most consumed metals by the Rio de Janeiro city inhabitants are Zn, Mn e Cu. The proposed methodology to extend this effective dose to the main Brazilian cities is: 1) to select for special analysis at each region the more consumed fruits at each city, carrots, manioc, tomato and sugar; 2) to use as a base line for all country the results of natural radionuclides and heavy metals obtained in this work for vegetables and derived products at specific locations and/or imported and distributed throughout the country; 3) in relation to natural radionuclides, it is only necessary to analyze 228 Ra, 226 Ra, 210 Pb. (author)

  9. Review of research on impacts to biota of discharges of naturally occurring radionuclides in produced water to the marine environment

    International Nuclear Information System (INIS)

    Hosseini, Ali; Brown, Justin E.; Gwynn, Justin P.; Dowdall, Mark

    2012-01-01

    Produced water has been described as the largest volume waste stream in the exploration and production process of oil and gas. It is accompanied by discharges of naturally occurring radionuclides raising concerns over the potential radiological impacts of produced water on marine biota. In the Northern European marine environment, radioactivity in produced water has received substantial attention owing to the OSPAR Radioactive Substances Strategy which aims at achieving ‘concentrations in the environment near background values for naturally occurring radioactive substances’. This review provides an overview of published research on the impacts to biota from naturally occurring radionuclides discharged in produced water by the offshore oil and gas industry. In addition to summarising studies and data that deal directly with the issue of dose and effect, the review also considers studies related to the impact of added chemicals on the fate of discharged radionuclides. The review clearly illustrates that only a limited number of studies have investigated possible impacts on biota from naturally occurring radionuclides present in produced water. Hence, although these studies indicate that the risk to the environment from naturally occurring radionuclides discharged in produced water is negligible, the substantial uncertainties involved in the assessments of impact make it difficult to be conclusive. With regard to the complexity involved in the problem under consideration there is a pressing need to supplement existing data and acquire new knowledge. Finally, the present work identifies some knowledge gaps to indicate future research requirements. -- Highlights: ► Produced water from offshore oil industry contains naturally occurring radionuclides. ► Published research on the impacts to biota from these radionuclides is reviewed. ► Review includes impact of added chemicals on the fate of discharged radionuclides. ► Studies indicate negligible risk to biota

  10. Natural substrate lift-off technique for vertical light-emitting diodes

    Science.gov (United States)

    Lee, Chia-Yu; Lan, Yu-Pin; Tu, Po-Min; Hsu, Shih-Chieh; Lin, Chien-Chung; Kuo, Hao-Chung; Chi, Gou-Chung; Chang, Chun-Yen

    2014-04-01

    Hexagonal inverted pyramid (HIP) structures and the natural substrate lift-off (NSLO) technique were demonstrated on a GaN-based vertical light-emitting diode (VLED). The HIP structures were formed at the interface between GaN and the sapphire substrate by molten KOH wet etching. The threading dislocation density (TDD) estimated by transmission electron microscopy (TEM) was reduced to 1 × 108 cm-2. Raman spectroscopy indicated that the compressive strain from the bottom GaN/sapphire was effectively released through the HIP structure. With the adoption of the HIP structure and NSLO, the light output power and yield performance of leakage current could be further improved.

  11. Distribution of natural radionuclides on coats of Bushehr, Persian Gulf, Iran

    International Nuclear Information System (INIS)

    Abdi, M. R.; Faghihian, H.; Kamali, M.; Mostajaboddavati, M.; Hasanzadeh, A.

    2006-01-01

    :A reconnaissance study has been made on the distribution of 2 38U , 2 32T h, 4 0K , 1 37C s and geochemical features in soil and sediment samples at various locations on the coast of Bushehr in the Persian Gulf. In this study a gamma-ray spectrometer based on a High Purity Germanium detector and a PC based MCA and X-ray fluorescence (XRF) method were used. Estimation of the measured radionuclide content have been made for the absorbed dose rate of gamma radiation. The Activity concentration (A), the equivalent radium (R eq ), and the external hazard index (H ex ) which resulted from the natural radionuclides in soil and sediment are also calculated. The base-line data of radionuclides and heavy metals in view of the commissioning of nuclear and non-nuclear industries for the coast of Bushehr, which does not yet exist, was obtained. Activity concentration levels due to radionuclides were measured in 50 soil and sediment samples collected from this region. The measurement was performed with respect to their gamma radioactivity for a counting time of 24 hour intervals. From the accumulated spectra, activity concentration were determined for 4 0K (range from 108 to 520 Bq Kg -1 ), 1 37 Cs (from 6 to 40 Bq Kg 1 ), 2 38U (from 12 to 75 Bq Kg -1 ) and 2 32T h (from 8 to 33 Bq Kg -1 ) with the lowest limit detection (LLD) of, respectively, 68, 3.2, 4.3 and 4.3 Bq Kg -1 . The dose rate from ambient air at the soil ranges was between 14 to 44 nGy h -1 with an average of 30.56±7.86 nGy h -1

  12. Determination of Natural Levels of Radionuclides in Proposed Mushroom Reference Material (A Proficiency Test Exercise)

    International Nuclear Information System (INIS)

    Waheed, S.; Rahman, A.; Siddique, N.; Ahmad, S.; Zaidi, J.H.

    2006-08-01

    A proficiency test (PT) was organized within the framework of international Atomic Energy Agency (IAEA) project INT/1/054, entitled 'Preparation' of Reference Materials and Organization of Proficiency Test Rounds'. This exercise served to estimate the proficiency of the analytical laboratories from participating countries. This report presents the results of the proficiency test exercise on the proposed Mushroom Reference Material for the determination of natural levels of radionuclides. Laboratories from 6 different countries submitted data on the following three radionuclides: /sup 134/Cs, /sup 137/Cs, /sup 40/K. Results for /sup 134/Cs, 137/sup 137/Cs, and /sup 40/K in the mushroom reference material were reported by three or more participating laboratories and could be subjected to statistical evaluation. The original data of these raionuclides was subjected to a computer program 'Histo Vession 2.1' provided by IAEA. The four outlier tests i.e. Dixon, Grubbs, Skewness and Kurtosis were applied to the data sets. All values for these three radionuclides were accepted by the software. Consensus (overall) mean value, absolute standard deviation, relative standard deviation, standard error, median and range of values for these three radionuclides have been are obtained (at significance level 0.05). the consensus mean values and confidence intervals are given./sup 134/Cs: 4.4 Bq/kg (3.4-5.3 Bq/kg) /sup 137/Cs: 2899 Bq/kg (2740-3058 Bq/kg) /sup 40/K: 1136 Bq/kg (1046-1226 Bq/kg). (author)

  13. Content of Natural Radionuclides in Sediments in the Vicinity of a Former Uranium Mine

    International Nuclear Information System (INIS)

    Strok, M.; Planinsek, P.; Smodis, B.

    2011-01-01

    Former Slovenian uranium mine Zirovski vrh lies in the subalpine environment with relative high rainfall and population density. As a legacy of uranium mining, Jazbec and Borst waste piles were constructed in the vicinity of a former uranium mine. On the Jazbec waste pile, about 2.5 millions of tons of spoil, and 0.05 millions of tons of red mud were deposited. Average activity concentrations in spoil are 750 Bq/kg for 238U, 226Ra and 230Th, and in red mud 495 Bq/kg for 238U, 190 Bq/kg for 226Ra and 65100 Bq/kg for 230Th. On the Borst waste pile, about 0.6 millions of tons of uranium mill tailings (UMT) were deposited. Average activity concentrations in UMT are 995 Bq/kg for 238U, 8630 Bq/kg for 226Ra and 3930 Bq/kg for 230Th. Seepage waters with elevated radionuclide concentrations from both waste piles flow in the nearby streams Brebovscica and Todrascica. Todrascica outfalls into the Brebovscica and Brebovscica into the Poljanska Sora River. Due to the different biogeochemical processes, natural radionuclides from both waste piles can be transferred to the sediments of the affected streams. These processes are mainly driven by the sorption onto the particles and particles settling or by the direct diffusion to sediments. Therefore the aim of this work was to find out at which extent these processes occur in the specific case by comparing activity concentrations in sediments before and after inflow of seepage waters from both waste piles. In sediment samples, 238U, 234U, 230Th, 226Ra, 210Pb and 210Po activity concentrations were determined, using radiochemical separations followed by either alpha spectrometry or proportional counting. Results of the content of natural radionuclides in sediments in the vicinity of a former uranium mine showed that activity concentrations of all analyzed radionuclides were higher in sediments after the inflow of seepage waters from waste piles in Brebovscica and Todrascica stream. This was not the case for Poljanska Sora River

  14. Soil-to-plant transfer factors for natural radionuclides in the Brazilian cerrado region

    International Nuclear Information System (INIS)

    Jacomino, Vanusa M.F.; Oliveira, Kerley A.; Menezes, Maria Angela de B.; Mello, Jaime de; Silva, David F. da

    2009-01-01

    Large amounts of phosphogypsum produced have been attracting attention of Radiological Protection institutions and Environmental Protection agencies worldwide, given its high potential for environmental contamination. In Brazil, this material has been used for several decades, especially for agricultural purposes. Due to the presence of radionuclides in its composition, it is necessary to understand the mechanisms for natural radionuclide transfer in the soil/plant system and to evaluate if the use of phosphogypsum in soil contributes to increased exposition of humans to natural radioactivity. Experiments were accomplished in a greenhouse with lettuce cultivation in two types of soil (sandy and clayey) fertilized with four different amounts of phosphogypsum. Samples of phosphogypsum, soil, lettuce and drainage water were then analyzed for key radionuclides. 238 U and 232 Th analyses were carried out by Neutron Activation Analysis; 226 Ra, 228 Ra, and 210 Pb by analyzed by Gamma Spectrometry; and 210 Po by Alpha Spectrometry Technique. Finally, Transfer Factors of soil-plant were calculated as well as annual contribution to the effective dose due to the ingestion of lettuces. 22 '6Ra average specific activity in phosphogypsum samples (252 Bq kg -1 ) was below the maximum level recommended by USEPA, which is 370 Bq.kg -1 for agricultural use. Although most of the results for mean specific activity of radionuclides in lettuce presented values below the Minimum Detectable Activity (MDA), Transfer Factors were estimated for those conditions in which the mean specific activity proved to be superior to MDA. Values ranged from 1.8 10 -3 to 2.3 10 -2 for 232 Th; 3.5 10 - '2 to 4.1 10 -2 for 226 Ra, 2.4 10 -1 to 3.2 10 - '1 for 228 Ra, and 3.5 10 -2 to 8.5 10 -2 for 210 Po, depending on the type of soil used for planting vegetables. In general, results obtained in the present study indicated that mobility of radionuclides was low in both soils studied. Calculated effective

  15. Soil-to-plant transfer factors for natural radionuclides in the Brazilian cerrado region

    Energy Technology Data Exchange (ETDEWEB)

    Jacomino, Vanusa M.F.; Oliveira, Kerley A.; Menezes, Maria Angela de B., E-mail: vmfj@cdtn.b [Centro de Desenvolvimento da Tecnologia Nuclear (CDTN/CNEN-MG), Belo Horizonte, MG (Brazil); Mello, Jaime de; Silva, David F. da, E-mail: jwvmello@ufv.b [Universidade Federal de Vicosa (UFV), MG (Brazil). Dept. de Solos; Siqueira, Maria C.; Taddei, Maria H.; Dias, Fabiana F., E-mail: mc_quimica@hotmail.co, E-mail: mhtaddei@cnen.gov.b, E-mail: fdias@cnen.gov.b [Comissao Nacional de Energia Nuclear (CNEN-MG), Pocos de Caldas, MG (Brazil). Lab. de Pocos de Caldas (LAPOC)

    2009-07-01

    Large amounts of phosphogypsum produced have been attracting attention of Radiological Protection institutions and Environmental Protection agencies worldwide, given its high potential for environmental contamination. In Brazil, this material has been used for several decades, especially for agricultural purposes. Due to the presence of radionuclides in its composition, it is necessary to understand the mechanisms for natural radionuclide transfer in the soil/plant system and to evaluate if the use of phosphogypsum in soil contributes to increased exposition of humans to natural radioactivity. Experiments were accomplished in a greenhouse with lettuce cultivation in two types of soil (sandy and clayey) fertilized with four different amounts of phosphogypsum. Samples of phosphogypsum, soil, lettuce and drainage water were then analyzed for key radionuclides. {sup 238}U and {sup 232}Th analyses were carried out by Neutron Activation Analysis; {sup 226}Ra, {sup 228}Ra, and {sup 210}Pb by analyzed by Gamma Spectrometry; and {sup 210}Po by Alpha Spectrometry Technique. Finally, Transfer Factors of soil-plant were calculated as well as annual contribution to the effective dose due to the ingestion of lettuces. {sup 22}'6Ra average specific activity in phosphogypsum samples (252 Bq kg{sup -1}) was below the maximum level recommended by USEPA, which is 370 Bq.kg{sup -1} for agricultural use. Although most of the results for mean specific activity of radionuclides in lettuce presented values below the Minimum Detectable Activity (MDA), Transfer Factors were estimated for those conditions in which the mean specific activity proved to be superior to MDA. Values ranged from 1.8 10{sup -3} to 2.3 10{sup -2} for {sup 232}Th; 3.5 10{sup -}'2 to 4.1 10{sup -2} for {sup 226}Ra, 2.4 10{sup -1} to 3.2 10{sup -}'1 for {sup 228}Ra, and 3.5 10{sup -2} to 8.5 10{sup -2} for {sup 210}Po, depending on the type of soil used for planting vegetables. In general, results

  16. Determination of gamma emitting radionuclides in environmental air and precipitation samples with a Ge(Li) detector

    International Nuclear Information System (INIS)

    Hoetzl, H.; Rosner, G.; Winkler, R.; Sansoni, B.

    1977-01-01

    The concentrations of the radionuclides 7 Be, 54 Mn, 95 Zr, 95 Nb, 103 Ru, 106 Ru, 125 Sb, 137 Cs, 140 Ba/ 140 La, 141 Ce and 144 Ce in ground level air and of 7 Be, 95 Zr, 137 Cs and 144 Ce in precipitation were determined since 1970 and 1971 respectively at Neuherberg, 10 km north of Munich, by gamma spectrometry using a 60 cm 3 Ge(Li) detector. Dust samples were collected twice a month 1 m above ground from about 40,000 m 3 of air on 46 cm x 28 cm microsorbane filters and pressed to small cylinders of 35 cm 3 in size. Sensitivity of the procedure is of the order of 1 fCi/m 3 for air and of 10 pCi/m 2 per month for precipitation samples at a counting time of 1500 min. (author)

  17. Natural radionuclides in facilities of deep geothermal energy in Germany. Origin and occurrence

    International Nuclear Information System (INIS)

    Degering, Detlev; Koehler, Matthias

    2014-01-01

    Geothermal energy facilities use two inexhaustible energy reservoirs, the heat flux from the earth crust and earth core, originating from the gravitational process of the planet development 4.7 billion years ago, and on the other hand the continuous heat production as a consequence of the decay processes of natural radionuclides in the earth crust. The heat flux through the earth surface is in the range of 10 13 W, 50 to 70% originating from the radioactive decay. The constancy of this heat flux causes the attractiveness of the geothermal energy as base load energy production in comparison with other renewable energy sources.

  18. Transfer of radionuclides by terrestrial food products from semi-natural ecosystems to humans

    International Nuclear Information System (INIS)

    Howard, B.J.

    1996-01-01

    The potential radiological significance of radionuclide transfer to humans via foodstuffs derived from semi-natural ecosystems has become apparent since the Chernobyl accident. Foodchain models developed before this time usually did not take such transfers into account. The processes leading to contamination of food in these environments are complex and current understanding of the transfer mechanisms is incomplete. For these reasons the approach adopted in Chapter 3 is to represent, by means of aggregated parameters, the empirical relationships between ground deposits and concentration in the food product. 107 refs, 2 figs, 9 tabs

  19. New composite fibres for natural and waste waters decontamination from cesium radionuclides

    Directory of Open Access Journals (Sweden)

    Yu. V. Bondar

    2017-08-01

    Full Text Available New composite adsorbent based on modified polyacrylonitrile fibers is synthesized by in situ deposition of potassium-nickel ferrocyanide layer on the fibers’ surface. It is shown that the ferrocyanide phase forms a compact homogeneous layer on the fibers’ surface consisted of rounded nanoaggregates (∼ 40 - 50 nm. Composite fibers are chemically stable in both acidic and alkaline solutions. Sorption experiments have demonstrated that synthesized fibers are high-selective adsorbents and can be used for the purification of natural waters and high-salt solutions from cesium radionuclides.

  20. Natural and active chemical remediation of toxic metals and radionuclides in the aquatic environment

    International Nuclear Information System (INIS)

    McPherson, G.; Pintauro, P.; O'Connor, S.; Zhang, J.; Gonzales, R.; Flowers, G.

    1993-01-01

    The focus of this research is the non-biological, chemical remediation of toxic heavy metals and radionuclides in aquatic environments. This Tulane/Xavier group includes researchers from Chemistry, Chemical Engineering, and Geology. Active methods using novel zeolites and ion exchange membranes are currently being evaluated for use in removing heavy metals from natural waters. In addition, field and laboratory studies of metal ion exchange reactions and competitive, heavy metal adsorption on clay substrates are underway to determine sediment metal sequestering capacity. A summary of progress to date and future work is presented

  1. Natural and artificial radionuclides in the Suez Canal bottom sediments and stream water

    International Nuclear Information System (INIS)

    El-Tahawy, M.S.; Farouk, M.A.; Ibrahiem, N.M.; El-Mongey, S.A.M.

    1994-01-01

    Concentration of natural and artificial radionuclides in Suez Canal bottom sediments and stream water have been measured using γ spectrometers based on a hyper-pure Ge detector. The activity concentrations of 238 U series, 232 Th series and 40 K did not exceed 16.0, 15.5 and 500.0 Bq kg -1 dry weight for sediments. The activity concentration of 238 U series and 40 K did not exceed 0.6 and 18.0 Bq l -1 for stream water. (author)

  2. Natural and artificial radionuclides in the Suez Canal bottom sediments and stream water

    Science.gov (United States)

    El-Tahawy, M. S.; Farouk, M. A.; Ibrahiem, N. M.; El-Mongey, S. A. M.

    1994-07-01

    Concentration of natural and artificial radionuclides in Suez Canal bottom sediments and stream water have been measured using γ spectrometers based on a hyper-pure Ge detector. The activity concentrations of 238U series, 232Th series and 40K did not exceed 16.0, 15.5 and 500.0 Bq kg-1 dry weight for sediments. The activity concentration of 238U series and 40K did not exceed 0.6 and 18.0 Bq 1-1 for stream water.

  3. Natural radionuclides in soils - relation between soil properties and the activities

    International Nuclear Information System (INIS)

    Fujiyoshi, Ryoko; Nakayama, Masashi; Sawamura, Sadashi

    2000-01-01

    Vertical profiles of natural radionuclides (K-40 and Ra-226) have been investigated in a soil core with 8 m in depth to elucidate its relation to the bed rock activity and to several soil properties. Pattern of the Ra-226 activity with soil depth suggests inhomogeneity of this nuclide during the accumulating process. Radiometric sorption experiments with Pb-210 as a tracer gave the result that almost all Pb(II) in the soil solution disappeared to be sorbed to the soil components

  4. Natural radionuclides in bauxitic tailings (Red-Mud) in the Gulf of Corinth, Greece

    International Nuclear Information System (INIS)

    Papatheodorou, G.; Maratou, A.; Ferentinos, G.; Papaefthymiou, H.

    2004-01-01

    A detailed environmental survey was carried out in the central Gulf of Corinth in order to determine radionuclides in the bauxite ed-mud tailings which have been discharged on the sea floor by a Bauxite Processing Plant (Aluminio Ellados A.E). The discharge of bauxitic tailings via two pipelines at a water depth of 100 m, in Antikyra Bay (Northern Gulf of Corinth), has resulted in the formation of two red-mud mound-like deposits. The red-mud deposits at the mouth of the out falls, are not stable and very often red-mud masses are detached from the two main deposits and are transported to the Corinth central basin, by turbidity currents, at a water depth of 850 m and about 17 km away from the main deposits. Thus, at the Antikyra bay, the red-mud has formed a surficial veneer (0.5-2.0 cm) on the sea floor. On the Corinth central basin floor the red mud has formed successive red-mud layers which are interrupted by layers of natural mud. Fifteen gravity cores have been selected from the studied area and a number of bauxite samples have been collected from mines that supply the bauxite processing plant. Red-mud, natural mud and bauxite samples were analyzed for 238 U 226 Ra, 232 Th, 40 K, and 137 Cs by direct gamma spectrometry. The study of radionuclides concentrations has shown that: (a) the enrichment factor of radionuclides in the red-mud in the main deposit at the mouth of the out falls, in relation to bauxite samples, is about 2.0, (b) the enrichment factor of 238 U, 226 Ra and 232 Th in the red-mud in the main deposit and the central basin, in relation to natural sediments below, is visibly higher than 1.0 (2.0-19.0) whilst 40 K exhibits the opposite trend, and (c) the enrichment/dilution factor of radionuclides in the red-mud surficial veneer at the Antikyra Bay, in relation to the natural sediments below, is ranging between 0.4 and 3.5. (author)

  5. Bioaccumulation of some natural radionuclides in short-antenna grasshoppers (Acrididae family, class Ortoptera)

    International Nuclear Information System (INIS)

    Dimitrova, M.; Markova, E.; Bogdanova, V.

    1996-01-01

    The seasonal accumulation of radioactive elements of the uranium-radium order in representatives of larva stages of different species of of Acrididae family has been examined. The monitoring sites are typical of the region and gave a relevant information about the natural background radiation. The process begins in the end of spring when Acrididae enter on the most intensive phase of their functional development and accumulate lots of radioisotopes not only by food but also through respiratory system and whole-body surface. Among the radioisotopes radium has an average biological absorbability, uranium - a very slight one. This fact explains the high values of radium in the ecosystems examined. Despite its low absorbability coefficient 238 U is found to a considerable extent in the investigated organisms. Because of it high mobility in soil compared to Ra 226, uranium 238 accumulates in plants by water and through trophic chain passes into the living organisms. It is found also that Acrididae accumulate later, during autumn and Bi 214. So they are a reliable bio-indicator for the radionuclides U 238, Ra 226, Pb 214 and Bi 214. It has been found that the ionizing radiation at the natural biocenoses is not only an individual irritant but also has an effect of a radioecological factor of the environment. The examinations show redistribution of the natural radionuclides as a result of economic activities

  6. Natural attenuation of metals and radionuclides - An overview of the Sandia/DOE approach

    International Nuclear Information System (INIS)

    Waters, R.D.; Brady, P.V.; Borns, D.J.

    1998-02-01

    Sandia National Laboratories is developing guidelines that outline the technical basis for relying on natural attenuation for the remediation of metals and radionuclide-contaminated soils and groundwaters at US Department of Energy (DOE) sites for those specific cases where natural processes are effective at ameliorating soil and groundwater toxicity. Remediation by monitored natural attenuation (MNA) requires a clear identification of the specific reaction(s) by which contaminant levels are made less available as well as considerable long-term monitoring. Central to MNA is the development of a conceptual model describing the biogeochemical behavior of contaminant(s) in the subsurface. The conceptual model will be used to make testable predictions of contaminant availability over time. In many cases, comparison between this prediction and field measurements will provide the test of whether MNA is to be implemented. As a result, development of the conceptual model should guide site characterization activities as well as long-term monitoring

  7. Gamma ray doses proceeding from natural occurring radionuclides in closed environments

    International Nuclear Information System (INIS)

    Aguiar, Vitor Angelo P. de; Medina, Nilberto H.; Silveira, Marcilei A. Guazzelli da; Moreira, Ramon H.

    2009-01-01

    In this work we report on the application of gamma-ray spectrometry in the study of the effective dose coming from terrestrial natural elements present in building materials such as sand, cement, lime (CaO) and milled granitic stones. The major contribution to annual gamma-ray radiation effective dose is due to the natural occurring radionuclides 40 K, 232 Th and 238 U. Two spectrometry systems were employed to measure the gamma radiation: one with a 60% efficient GeHP detector and the second one with a 2''x2'' NaI(Tl) scintillator. The estimated effective dose coming from the three reference rooms assumed is 0.63 mSv/yr, proceeding from terrestrial natural elements. The principal gamma radiation sources are cement, sand and bricks. (author)

  8. Natural radionuclides by gammaspectrometry in the Belgrade, capital city in Yugoslavia for 1998, 1997 and 1996

    Energy Technology Data Exchange (ETDEWEB)

    Vukovic, D.M. [Institute for Occupational and Radiological Health, Belgrade (Yugoslavia); Markovic, D. [Faculty of Physical Chemistry, Belgrade (Yugoslavia)

    2000-05-01

    Region of Belgrade, 44 0 18' north width and 21 o 35' east length, 134 m under the sea, as a capital city of Yugoslavia is important part of monitoring of radioactivity in environment. Radioactivity comes mostly from natural radionuclides and partly from long-lived radionuclides from non natural sources as a consequence of Chernobyl accident. Monitoring of environment has proceeded by vertical methodology. We analyzed: aerosol, soil, fallout (wet and dry deposition), rivers, lakes, drinking water, human and animal food. Results from analyze of samples from environment contains very low activity, actually activity of changes of basic signal. Results for 1998, 1997 and 1996 are: 1. Gamma dose rate, with values from 0.072 {mu}G/h to 0.170 {mu}G/h, with median years values: 0.103 {mu}G/h (1998), 0.077 {mu}G/h (1997) and 0.072 {mu}G/h (1996). 2. By gammaspectrometry analyze of air as months samples for each year, results shows activity of changes of basic signal. The signals are coming from natural radionuclides. 3. {sup 137}Cs, as a long lived radionuclide, with remarkable activity in soil has values: 14-19 Bq/kg (1998), 12-111 Bq/kg (1997) and 7-39 Bq/kg (1996). 4. Activity in rivers Sava (Belgrade) and Danube (Zemun) belongs to {sup 40}K, while activities of {sup 137}Cs, {sup 226}Ra, {sup 232}Th, {sup 235}U and {sup 238}U are in traces. Activity of river sediment comes from {sup 137}Cs with values 0.4-46 Bq/kg of dry samples (river Danube). Activity in fish, mixture, white fish and others comes from {sup 40}K 55-100 Bq/kg and {sup 137}Cs 0.2-0.8 Bq/kg. 5. Activity of drinking waters, from city network shows low level of activity which comes from {sup 40}K. 6. Activity in milk comes from {sup 40}K 46.5-61.2 Bq/l (1998), 33-59 Bq/l (1997) and 31-54 Bq/l (1996). Activities of {sup 137}Cs are on the same level of detection. 7. Activity in the human food, measured in yogurt, meats, bread and agricultural products comes from {sup 40}K 44-310 Bq/kg (1998), 31

  9. Natural radionuclides by gammaspectrometry in the Belgrade, capital city in Yugoslavia for 1998, 1997 and 1996

    International Nuclear Information System (INIS)

    Vukovic, D.M.; Markovic, D.

    2000-01-01

    Region of Belgrade, 44 0 18' north width and 21 o 35' east length, 134 m under the sea, as a capital city of Yugoslavia is important part of monitoring of radioactivity in environment. Radioactivity comes mostly from natural radionuclides and partly from long-lived radionuclides from non natural sources as a consequence of Chernobyl accident. Monitoring of environment has proceeded by vertical methodology. We analyzed: aerosol, soil, fallout (wet and dry deposition), rivers, lakes, drinking water, human and animal food. Results from analyze of samples from environment contains very low activity, actually activity of changes of basic signal. Results for 1998, 1997 and 1996 are: 1. Gamma dose rate, with values from 0.072 μG/h to 0.170 μG/h, with median years values: 0.103 μG/h (1998), 0.077 μG/h (1997) and 0.072 μG/h (1996). 2. By gammaspectrometry analyze of air as months samples for each year, results shows activity of changes of basic signal. The signals are coming from natural radionuclides. 3. 137 Cs, as a long lived radionuclide, with remarkable activity in soil has values: 14-19 Bq/kg (1998), 12-111 Bq/kg (1997) and 7-39 Bq/kg (1996). 4. Activity in rivers Sava (Belgrade) and Danube (Zemun) belongs to 40 K, while activities of 137 Cs, 226 Ra, 232 Th, 235 U and 238 U are in traces. Activity of river sediment comes from 137 Cs with values 0.4-46 Bq/kg of dry samples (river Danube). Activity in fish, mixture, white fish and others comes from 40 K 55-100 Bq/kg and 137 Cs 0.2-0.8 Bq/kg. 5. Activity of drinking waters, from city network shows low level of activity which comes from 40 K. 6. Activity in milk comes from 40 K 46.5-61.2 Bq/l (1998), 33-59 Bq/l (1997) and 31-54 Bq/l (1996). Activities of 137 Cs are on the same level of detection. 7. Activity in the human food, measured in yogurt, meats, bread and agricultural products comes from 40 K 44-310 Bq/kg (1998), 31-238 Bq/kg (1997) and 36-122 Bq/kg (1996). Activities of 137 Cs are 1 Bq/kg. Results of analyze

  10. The radiological impact of naturally-occurring radionuclides in foods from the wild

    International Nuclear Information System (INIS)

    Green, N.; Hammond, D.J.; Davidson, M.F.; Wilkins, B.T.; Williams, B.

    2002-01-01

    Habit surveys have been conducted to identify people who make use of foodstuffs collected from the wild (free foods) in two areas of the UK: in the area around Chipping Norton in Oxfordshire, where levels of naturally-occurring radionuclides in soil were expected to be typical of the UK, and in the vicinity of Okehampton in Devon, where levels were known to be elevated. Individuals who make regular use of these foodstuffs were specifically identified, so that an estimate of typical and higher than average consumption rates could be derived. The naturally-occurring radionuclides of interest were 210 Po, 210 Pb, 234 U, 235 U, 238 U, 230 Th, 232 Th and 226 Ra. Samples of important foodstuffs were collected and the radionuclides of interest determined. The consumption rates were combined with the measured activity concentrations and published dose coefficients to estimate doses to average and higher than average consumers. These doses were compared with estimated doses reported in the Food Standards Agency's ongoing monitoring programme and with average doses to the population of the UK reviewed by NRPB. In total, 400 people were identified and between them they collected 54 different types of free food. Blackberries were by far the most common species collected, although various types of mushroom and nuts were also popular. On average, each collector from around Chipping Norton collected 2.1 different foods, and each from around Okehampton collected 2.2. On the basis of the habit survey, therefore, it would be reasonable to expect that any site, nuclear or otherwise, chosen for habit surveys, whether for radiological purposes or for any other contaminant, could have substantial numbers of people collecting free foods. In addition, the pattern of foods collected was very similar to previous studies, indicating similarities across England and Wales. Doses from the consumption of free foods were estimated. The annual doses estimated to have been received by a typical

  11. Natural radionuclides in coal and waste material originating from coal fired power plant

    International Nuclear Information System (INIS)

    Marovic, Gordana; Franic, Zdenko; Sencar, Jasminka; Petrinec, Branko; Bituh, Tomislav; Kovac, Jadranka

    2008-01-01

    This paper presents long-term investigations of natural radioactivity in coal, used for power production in the coal-fired power plant (CFPP) situated on the Adriatic coast, and resulting slag and ash. Activity concentrations of 40 K, 232 Th, 226 Ra and 238 U in used coal and resulting waste material have been measured for 25 years. As expected, it was demonstrated that the content of radionuclides in deposited bottom and filter ash material are closely related with radionuclide activity concentrations and mineral matter fraction in used coals. The external hazard index has been calculated and discussed for the slag and ash depository. During the first decade of operation of the CFPP has been used domestic coal produced in nearby area characterized by higher background radiation compared with the rest of Croatia. Therefore, the coal itself had relatively high 226 Ra and 238 U activity concentrations while potassium and thorium content was very low, 40 K activity concentrations being 2-9% and those of 232 Th 1-3% of total activity. As, in addition, the sulphur concentrations in coal were very high use of domestic coal was gradually abandoned till it was completely substituted by imported coal originated from various sources and of low natural radioactivity. Upon this, activity concentrations of uranium series radionuclides in deposited waste materials decreased significantly. Consequently, waste material i.e., slag and ash, generated in the last several years of coal fired power plant operation could be readily used in cement industry and as additive to other building materials, without any special restrictions according to the Croatian regulations dealing with building materials and European directives. (author)

  12. The radiological impact of naturally-occurring radionuclides in foods from the wild

    International Nuclear Information System (INIS)

    Green, N.; Hammond, D.J.; Davidson, M.F.; Wilkins, B.T.; Williams, B.

    2002-01-01

    Habit surveys have been conducted to identify people who make use of foodstuffs collected from the wild (free foods) in two areas of the UK: in the area around Chipping Norton in Oxfordshire, where levels of naturally-occurring radionuclides in soil were expected to be typical of the UK, and in the vicinity of Okehampton in Devon, where levels were known to be elevated. Individuals who make regular use of these foodstuffs were specifically identified, so that an estimate of typical and higher than average consumption rates could be derived. The naturally-occurring radionuclides of interest were 210 Po, 210 Pb, 234 U, 235 U, 238 U, 230 Th, 232 Th and 226 Ra. Samples of important foodstuffs were collected and the radionuclides of interest determined. The consumption rates were combined with the measured activity concentrations and published dose coefficients to estimate doses to average and higher than average consumers. These doses were compared with estimated doses reported in the Food Standards Agency's ongoing monitoring programme and with average doses to the population of the UK reviewed by NRPB. In total, 400 people were identified and between them they collected 54 different types of free food. Blackberries were by far the most common species collected, although various types of mushroom and nuts were also popular. On average, each collector from around Chipping Norton collected 2.1 different foods, and each from around Okehampton collected 2.2. On the basis of the habit survey, therefore, it would be reasonable to expect that any site, nuclear or otherwise, chosen for habit surveys, whether for radiological purposes or for any other contaminant, could have substantial numbers of people collecting free foods. In addition, the pattern of foods collected was very similar to previous studies, indicating similarities across England and Wales. (author)

  13. Natural radionuclides in major aquifer systems of the Parana sedimentary basin, Brazil

    International Nuclear Information System (INIS)

    Bonotto, Daniel Marcos

    2011-01-01

    This paper describes the natural radioactivity of groundwater occurring in sedimentary (Bauru and Guarani) and fractured rock (Serra Geral) aquifer systems in the Parana sedimentary basin, South America that is extensively used for drinking purposes, among others. The measurements of gross alpha and gross beta radioactivity as well the activity concentration of the natural dissolved radionuclides 40 K, 238 U, 234 U, 226 Ra, 222 Rn, 210 Po and 210 Pb were held in 80 tubular wells drilled in 21 municipalities located at Sao Paulo State and its border with Mato Grosso do Sul State in Brazil. Most of the gross alpha radioactivity data were below 1 mBq/L, whereas values exceeding the gross beta radioactivity detection limit of 30 mBq/L were found. The radioelement solubility in the studied systems varied according to the sequence radon>radium>other radionuclides and the higher porosity of sandstones relatively to basalts and diabases could justify the enhanced presence of dissolved radon in the porous aquifer. The implications of the data obtained in terms of standards established for defining the drinking water quality have also been discussed. The population-weighted average activity concentration for these radionuclides was compared to the guideline value of 0.1 mSv/yr for the total effective dose and discussed in terms of the choice of the dose conversion factors. - Highlights: → Integration of distinct radiometric data acquired in groundwaters. → Radiation dose in important hydrological resources in South America. → Contribution of 226 Ra for the more accentuated radiation dose in aquifers. → Dose factors for Rn and generation of values exceeding the maximum of 0.1 mSv/yr.

  14. Natural radionuclides in major aquifer systems of the Parana sedimentary basin, Brazil

    Energy Technology Data Exchange (ETDEWEB)

    Bonotto, Daniel Marcos, E-mail: danielbonotto@yahoo.com.br [Departamento de Petrologia e Metalogenia, IGCE-Instituto de Geociencias e Ciencias Exatas, UNESP-Universidade Estadual Paulista Julio de Mesquita Filho, Av. 24-A, No. 1515 - CP 178, CEP 13506-900-Rio Claro, SP (Brazil)

    2011-10-15

    This paper describes the natural radioactivity of groundwater occurring in sedimentary (Bauru and Guarani) and fractured rock (Serra Geral) aquifer systems in the Parana sedimentary basin, South America that is extensively used for drinking purposes, among others. The measurements of gross alpha and gross beta radioactivity as well the activity concentration of the natural dissolved radionuclides {sup 40}K, {sup 238}U, {sup 234}U, {sup 226}Ra, {sup 222}Rn, {sup 210}Po and {sup 210}Pb were held in 80 tubular wells drilled in 21 municipalities located at Sao Paulo State and its border with Mato Grosso do Sul State in Brazil. Most of the gross alpha radioactivity data were below 1 mBq/L, whereas values exceeding the gross beta radioactivity detection limit of 30 mBq/L were found. The radioelement solubility in the studied systems varied according to the sequence radon>radium>other radionuclides and the higher porosity of sandstones relatively to basalts and diabases could justify the enhanced presence of dissolved radon in the porous aquifer. The implications of the data obtained in terms of standards established for defining the drinking water quality have also been discussed. The population-weighted average activity concentration for these radionuclides was compared to the guideline value of 0.1 mSv/yr for the total effective dose and discussed in terms of the choice of the dose conversion factors. - Highlights: > Integration of distinct radiometric data acquired in groundwaters. > Radiation dose in important hydrological resources in South America. > Contribution of {sup 226}Ra for the more accentuated radiation dose in aquifers. > Dose factors for Rn and generation of values exceeding the maximum of 0.1 mSv/yr.

  15. The Palmottu natural analogue project. The behaviour of natural radionuclides in and around uranium deposits. Summary report 1992-1994

    Energy Technology Data Exchange (ETDEWEB)

    Blomqvist, R; Ruskeeniemi, T; Ahonen, L [Geological Survey of Finland, Espoo (Finland); Suksi, J [Helsinki Univ. (Finland). Lab. of Radiochemistry; Niini, H [Helsinki Univ. of Technology, Otaniemi (Finland). Lab. of Engineering Geology and Geophysics; Vuorinen, U [VTT Chemical Technology, Espoo (Finland); Jakobsson, K [Finnish Centre for Radiation and Nuclear Safety, Helsinki (Finland)

    1995-06-01

    The Palmottu U-Th mineralization at Nummi-Pusula, southwestern Finland, has been studied as a natural analogue to deep disposal of radioactive wastes since 1988. The report gives a summary of the results of investigations carried out during the years 1992-1994. The Palmottu Analogue Project aims at a more profound understanding of radionuclide transport processes in fractured crystalline bedrock. The essential factors controlling transport are groundwater flow and interaction between water and rock. Accordingly, the study includes structural interpretations based in part on geophysical measurements, hydrological studies including hydraulic downhole measurements, flow modelling, hydrogeochemical characterization of groundwater, uranium chemistry and colloid chemistry, mineralogical studies, geochemical interpretation and modelling, including paleohydrogeological aspects, and studies of radionuclide mobilization and migration processes including numerical simulations. The project has produced a large amount of data related to natural analogue aspects. The data obtained have already been utilized in developing logical conceptual ideas of the time frames and processes operating in the bedrock of the site. (61 refs., 24 figs., 8 tabs.).

  16. The Palmottu natural analogue project. The behaviour of natural radionuclides in and around uranium deposits. Summary report 1992-1994

    International Nuclear Information System (INIS)

    Blomqvist, R.; Ruskeeniemi, T.; Ahonen, L.; Suksi, J.; Jakobsson, K.

    1995-06-01

    The Palmottu U-Th mineralization at Nummi-Pusula, southwestern Finland, has been studied as a natural analogue to deep disposal of radioactive wastes since 1988. The report gives a summary of the results of investigations carried out during the years 1992-1994. The Palmottu Analogue Project aims at a more profound understanding of radionuclide transport processes in fractured crystalline bedrock. The essential factors controlling transport are groundwater flow and interaction between water and rock. Accordingly, the study includes structural interpretations based in part on geophysical measurements, hydrological studies including hydraulic downhole measurements, flow modelling, hydrogeochemical characterization of groundwater, uranium chemistry and colloid chemistry, mineralogical studies, geochemical interpretation and modelling, including paleohydrogeological aspects, and studies of radionuclide mobilization and migration processes including numerical simulations. The project has produced a large amount of data related to natural analogue aspects. The data obtained have already been utilized in developing logical conceptual ideas of the time frames and processes operating in the bedrock of the site. (61 refs., 24 figs., 8 tabs.)

  17. Balance of natural radionuclides in the brown coal based power generation and harmlessness of the residues and side product utilization

    International Nuclear Information System (INIS)

    Schulz, Hartmut; Kunze, Christian; Hummrich, Holger

    2017-01-01

    During brown coal combustion a partial enrichment of natural radionuclides occurs in different residues. Residues and side product from brown coal based power generation are used in different ways, for example filter ashes and gypsum from flue gas desulfurization facilities are used in the construction materials fabrication and slags for road construction. Detailed measurement and accounting of radionuclides in the mass throughputs in coal combustion power plants have shown that the utilized gypsum and filter ashes are harmless in radiologic aspects.

  18. Superluminescent light emitting diodes on naturally survived InGaN/GaN lateral nanowires

    Energy Technology Data Exchange (ETDEWEB)

    Banerjee, D.; Sankaranarayanan, S.; Khachariya, D.; Nadar, M. B.; Ganguly, S.; Saha, D., E-mail: dipankarsaha@iitb.ac.in [Applied Quantum Mechanics Laboratory, Centre of Excellence in Nanoelectronics, Indian Institute of Technology Bombay, Powai, Mumbai 400076 (India)

    2016-07-18

    We demonstrate a method for nanowire formation by natural selection during wet anisotropic chemical etching in boiling phosphoric acid. Nanowires of sub-10 nm lateral dimensions and lengths of 700 nm or more are naturally formed during the wet etching due to the convergence of the nearby crystallographic hexagonal etch pits. These nanowires are site controlled when formed in augmentation with dry etching. Temperature and power dependent photoluminescence characterizations confirm excitonic transitions up to room temperature. The exciton confinement is enhanced by using two-dimensional confinement whereby enforcing greater overlap of the electron-hole wave-functions. The surviving nanowires have less defects and a small temperature variation of the output electroluminescent light. We have observed superluminescent behaviour of the light emitting diodes formed on these nanowires. There is no observable efficiency roll off for current densities up to 400 A/cm{sup 2}.

  19. Distribution of natural radionuclides in soil around Sultan Azlan Shah Coal-Fired Power Plant at Manjung, Perak

    International Nuclear Information System (INIS)

    Zaini Hamzah; Fetri Zainal; Ahmad Saat; Abdul Khalik Wood

    2013-01-01

    Full-text: A radionuclide is an atom with an unstable nucleus which is created by excess energy. This radionuclide will undergo radioactive decay where gamma ray or sub atomic particles are released making them radioactive which can be harmful if the safe level is exceeded. This study was carried out in Manjung, Perak near Sultan Azlan Shah coal-fired power plant. Coal combustion from power plant generates emissions of potentially toxic radionuclides besides major pollutants which are particulates, sulphur and nitrogen oxides. It is noted that emission of particulates, sulphur and nitrogen oxides are strictly control. Soil is one of the most important media for plant to growth however soil is subject to contamination and its quality must be protected. The concentration of natural radionuclides in soil can be affected from coal combustion process from power plant in order to generate electricity. In this study, natural radionuclides concentration such as 238 U and 232 Th concentration in soil at nine points around this power plant were determined to assess radioactivity level and the possible radiation hazard to local population that residence in that area will be carried out in future study. Concentrations of natural radionuclides have been determined by using Energy Dispersive X-ray Fluorescence (EDXRF) technique. The concentration of 238 U in the area were in the ranged between 3.42 mg/ kg to 7.59 mg/ kg. While the concentration of 232 Th ranged from 12.19 mg/ kg to 21.67 mg/ kg respectively. (author)

  20. Zone peculiarities of natural conditions, affecting ran food stuffs and drinking water contamination with radionuclides

    International Nuclear Information System (INIS)

    Marej, A.N.

    1980-01-01

    The effect of natural conditions on the USSR territory connected with peculiar types of soil on the behaviour of radionuclides fallen from stratosphere is considered. Characteristics of tundra, taiga partially-wooded steppe, step.oe, mountain and semi-desert zones are presented. Peculiarities of soils in different geographical zones of the USSR conditioned by various properties and compositions have a significant effect on 90 Sr and especially 137 Cs migration intensity from the soil into plants and organisms of animals through biological chains. The administration of radionuclides in the ration with food stuffs obtained on the surface of reservoirs where zonality low is also rightful, is studied. It is established that indexes of 90 Sr and 137 Cs buildup in tissues of hydrobionts are in reverse dependence on calcium and potassium content in water. Therefore, maximum levels of 90 Sr and 137 Cs buildup in fish is characteristic of zones with the low content of these elements. The degree of water mineralization in ponds has a clear zonality which increases in the direction from the North to the South. The degree of pond well-drained nature is of great importance

  1. Heavy metal and natural radionuclide levels in urban soils from Cienfuegos city, Cuba

    International Nuclear Information System (INIS)

    Diaz Rizo, Oscar; Quintana Miranda, Eduardo; D Alessandro Rodriguez, Katia; Lopez Pino, Neivy; Arado Lopez, Juana O.; Alonso Hernandez, Carlos M.; Cartas Aguila, Hector

    2013-01-01

    Concentrations of heavy metals and natural radionuclides in topsoil (0-10cm) from Cienfuegos city, Cuba, were determined by using X-ray fluorescence analysis and gamma ray spectrometry, respectively. The measured results of heavy metals show that the mean concentrations of Ni, Cu, Zn and Pb in the studied soil samples are higher than their corresponding background values. The calculated results of integrated pollution index of heavy metals indicate that the studied soils present severely heavy metal contamination. The concentrations of 226Ra, 232Th and 40K in the studied soil samples range from 8.3 to 32.7, 3.7 to 10.7 and 129 to 356 Bq.kg-1 with an average of 22.6, 6.3 and 272 Bq.kg-1 , respectively, which are similar than the average concentrations reported for South-central Cuban soils. The air absorbed dose rate and the annual effective dose equivalent received by the local residents due to the natural radionuclides in soil are lesser than the worldwide established limits. A significantly positive 232Th-Cu and 232Th-Zn correlations were determined, indicating the possible presence of these elements pollution source in the area.(author)

  2. Soil depth profiles and radiological assessment of natural radionuclides in forest ecosystem

    International Nuclear Information System (INIS)

    Manigandan, P.K.; Chandar Shekar, B.

    2017-01-01

    We measured the distribution of three naturally occurring radionuclides, "2"3"8U, "2"3"2Th, and "4"0K, in soil samples collected from a rainforest in the Western Ghats of India. For each surface sample, we calculated average activity concentration, outdoor terrestrial γ dose rate, annual effective dose equivalent (AEDE), and radiation hazard index. The activity concentrations of surface samples were randomly distributed over space, but differed slightly with different soil depths. The concentration of "2"3"2Th and the average terrestrial γ dose rates were slightly higher than the world averages, so slightly high γ radiation appears to be a general characteristic of the Western Ghats. However, all radiological hazard indices were within the limits proposed by the International Commission on Radiological Protection. The results reported here indicate that, except for "2"3"2Th, the naturally occurring radionuclides in the forest soils of the Western Ghats were within the ranges specified by United Nations Scientific Committee on the Effects of Atomic Radiation for undisturbed virgin soils.

  3. Changes of ionizing radiation caused by natural radionuclides in the Curonian Spit

    International Nuclear Information System (INIS)

    Peciuliene, M.; Jasaitis, D.; Grigaliunaite-Vonseviciene, G. and others

    2005-01-01

    Taking into consideration a unique scenery of the Curonian Spit, dosimetric investigation of ionizing radiation caused by natural radionuclides is performed there. The influence of natural radionuclides present in the ground on the equivalent dose rate of gamma radiation in the ground surface air is established. Measurements of equivalent dose rate are carried out in the whole territory of the Curonian Spit in Lithuania. Especially numerous data have been collected on the coasts of the sea and bay, near them, in seaside dunes and by roads. The established equivalent dose rate values vary from 22 nSv/h (on the dune top) to 90 nSv/h (above an asphalt path). The values of the main gamma radiation source ( 40 K and 226 Ra) concentration are measured, and positive correlation of concentrations and equivalent dose rates in the ground surface air between 40 K and 2 '2 6 Ra is determinated. It is established that 40 K has the biggest influence on equivalent dose rate. The equivalent dose rate values in the ground surface air in the Curonian Spit are comparatively low (they can even be 1630 times lower in comparison to Guarapari beach, Brazil). (author)

  4. Determination of natural and artificial radionuclides in 3 earner ecosystems (Alcocebre; Vinaroz and Vandellos)

    International Nuclear Information System (INIS)

    Navarro, E.; Roldan, C.; Sanchez, E.

    1998-01-01

    The knowledge of the environmental radioactivity level represents one of the main objectives at the moment for the environmental investigation. To check the existence of possible polluting sources and their impact in the population is of high-priority interest. We have intended to check the existence or not of radioactive pollutants in bio-indicators (algae, limpets and mussels) of the marine environment of three towns located in the Mediterranean coast: Alcocebre and Vinaroz in the county of Castellon and Vandellos in the county of Tarragona where a nuclear group is located for electric power production. The specific activity measurement carried out during the biennium 1996-97 of the natural gamma emitters ''228 Ac (''232Th series), ''226Ra (''238U series), ''235U, ''40K and ''7Be, and of the artificial radionuclides ''60Co, and ''137 Cs, it corroborates the character bio-accumulator of these organisms. Natural and artificial radionuclides have been detected in quantities without radiological significance. (Author) 3 Refs

  5. Soil depth profiles and radiological assessment of natural radionuclides in forest ecosystem

    Energy Technology Data Exchange (ETDEWEB)

    Manigandan, P.K. [Al Musanna College of Technology, Muscat (Oman); Chandar Shekar, B. [Bharathiar Univ., Coimbatore (India). Kongunadu Arts and Science College

    2017-08-01

    We measured the distribution of three naturally occurring radionuclides, {sup 238}U, {sup 232}Th, and {sup 40}K, in soil samples collected from a rainforest in the Western Ghats of India. For each surface sample, we calculated average activity concentration, outdoor terrestrial γ dose rate, annual effective dose equivalent (AEDE), and radiation hazard index. The activity concentrations of surface samples were randomly distributed over space, but differed slightly with different soil depths. The concentration of {sup 232}Th and the average terrestrial γ dose rates were slightly higher than the world averages, so slightly high γ radiation appears to be a general characteristic of the Western Ghats. However, all radiological hazard indices were within the limits proposed by the International Commission on Radiological Protection. The results reported here indicate that, except for {sup 232}Th, the naturally occurring radionuclides in the forest soils of the Western Ghats were within the ranges specified by United Nations Scientific Committee on the Effects of Atomic Radiation for undisturbed virgin soils.

  6. Effects on elevating cancer risk in population exposed to natural radionuclide 226Ra if parent radionuclide 238U is entered the body by inhalation or ingestion

    International Nuclear Information System (INIS)

    Zupunski, Lj.; Trobok, M.; Gordanic, V.; Spasic-Jokic, V.; Sovilj, P.

    2009-01-01

    People have always been exposed to ionizing radiation originating from natural radionuclides including 238 U, 40 K, 232 Th that exist in earths crust. Although received doses are small, due to the fact that threshold does not exist, there is a certain risk of developing cancer. Purpose of this study was to measure 238 U concentrations in soil of Bela Crkva territory. Based on these measurements, risks of developing cancers are calculated using Monte Carlo method.(author) [sr

  7. Assessment of radiological significance of naturally occurring radionuclides in soil and rock matrices around Kakrapar environment

    International Nuclear Information System (INIS)

    Patra, A.K.; Jaison, T.J.; Baburajan, A.; Hegde, A.G.

    2008-01-01

    The activity and gamma-absorbed dose rate due to the naturally occurring radionuclides in the terrestrial environment such as 238 U, 232 Th and 40 K were determined in soil and rock samples collected around Kakrapar Atomic Power Plant site, using gamma-ray spectrometry. The mean concentration levels measured in Kakrapar soil from naturally occurring radioisotopes such as 238 U, 232 Th and 40 K are lower than the corresponding global average values obtained in worldwide soil. The external hazard index (Hex) and absorbed gamma dose rate in air outdoors is observed to be 0.04-0.18 and 3.1-14.1 nGy h -1 , respectively. (authors)

  8. Colloid and radionuclide retention mechanisms in fractured rock under near-natural flow conditions

    International Nuclear Information System (INIS)

    Delos, A.; Schaefer, T.; Geckeis, H.; Guimera, J.; Carrera, J.; Fanghaenel, T.

    2005-01-01

    Full text of publication follows: Experiments in fractured host rock (Grimsel Test Site, GTS, Switzerland) revealed that the colloid relevance for actinide migration is high due to the specific geochemical groundwater conditions [1]. However, even under such conditions it is found that retention of colloids and colloid-borne actinides becomes significant under near-natural groundwater flow rates (1-10 m/a) [2]. Underlying mechanisms of colloid and radionuclide retention are not well understood up to now. The present study co-funded by the NoE ACTINET-6 focuses on (i) the kinetics of actinide-colloid interactions and (ii) the relevance of matrix diffusion as a competition process to other retention mechanisms which affect the actinides behavior in fractured rock systems such as the Grimsel granodiorite. Colloid migration is studied with well defined model colloids as e.g. fluorescence dyed carboxylated polystyrene particles, and natural colloids extracted from bentonite (FEBEX) and from fracture filling material (GTS). In order to study the influence of matrix porosity on actinides migration, those experiments are performed in columns of well defined geometry filled with microporous unmodified silica spheres, porous ceramic material and natural fracture filling material from the GTS. The behaviour of actinides (Pu(IV) and Am(III)) sorbed onto bentonite colloids is investigated in column and batch experiments. All experiments are performed under anoxic conditions. Colloid characterization methods used in this study include the combination of photon correlation spectroscopy (PCS), laser-induced breakdown detection (LIBD), fluorimetry and field flow fractionation (FFF). Experimental results and their application to the parametrisation of reactive colloid transport models are discussed. [1] Geckeis H, Schaefer T, Hauser W, Rabung T, Missana T, Degueldre C, Moeri A, Eikenberg J, Fierz T, Alexander WR (2004) Results of the Colloid and Radionuclide Retention experiment

  9. The immigration model and its implications of natural radionuclides of coastal groundwater in Xiamen

    International Nuclear Information System (INIS)

    Cai Minggang; Huang Yipu; Chen Min; Liu Guangshan

    2004-01-01

    The natural radionuclides in groundwater systems are considered to reside in three pools: dissolved, sorbed (on rock surface), and solid. Transfer of radionuclides between the dissolved and solid pools is accomplished chiefly by dissolution, (co-)precipitation and/or a-recoil. The mass balance equations model of the natural radionuclides of dissolved and adsorbed phase reservoir in groundwater is established by setting certain conditions and parameters. The modeling equations form the basic of our assessment of the effects of sorption-desorption, dissolution-precipitation, and advection-diffusion in radionuclide transport in the groundwater. The interaction between groundwater and rock in Xiamen coastal aquifers were studied quantitatively using this model, which gave us reasonable explanation for the spatial distribution of natural radium, radon isotopes activities and their activities ratio. α-recoil supply rates of 222 Rn (P r,Rn-222 ) and 224 Ra (P α,Ra-224 ) range from 0.09 x 10 3 to 3.44 x 10 3 atoms·m -3 ·s -1 and from 0.13 x l0 3 to 4.91 x 10 3 atoms·m -3 ·s -1 , respectively. P α,Ra-224 is also found to be larger than P r,Rn-222 in every station, revealing that aquifer solids contain more thorium than uranium in studied area. Both of P r,Rn-222 and P α,Ra-224 of coastal groundwater decreased seaward, revealing a-recoil supplying rates of 222 Rn and 224 Ra by aquifers rock decreased gradually, which gave good explanation of the spatial distribution characters of above two nuclides. P r,Rn-222 /A Rn-222 increase seaward from 0.3 to 0.9 along the major paths, with the average value of 0.6. Such results reveal that the primary source of groundwater 222 Rn in these areas is α-recoil of 226 Ra decay in solid pool, and its relative increase along the paths. Another source of 222 Rn is 226 Ra decay in tile sorbed pool (R f,Ra-226 ·A Ra-226 ), which attributes about 40 percent of total source of coastal groundwater 222 Rn. P α,Ra-224 /A Ra-224 ranges

  10. The immigration model and its implications of natural radionuclides of coastal groundwater in Xiamen

    International Nuclear Information System (INIS)

    Cai Minggang; Huang Yipu; Chen Min; Liu Guangshan

    2005-01-01

    The natural radionuclides in groundwater systems are considered to reside in three pools: dissolved, sorbed (on rock surface), and solid. Transfer of radionuclides between the dissolved and solid pools is accomplished chiefly by dissolution. (co-)precipitation and/or α-recoil. The mass balance equations model of the natural radionuclides of dissolved and adsorbed phase reservoir in groundwater is established by setting certain conditions and parameters. The modeling equations form the basic of our assessment of the effects of sorption-desorption, dissolution-precipitation, and advection-diffusion in radionuclide transport in the groundwater. The interaction between groundwater and rock in Xiamen coastal aquifers were studied quantitatively using this model, which gave us reasonable explanation for the spatial distribution of natural radium, radon isotopes activities and their activities ratio. α-recoil supply rates of 222 Rn (P r,Rn-22 -2) and 224 Ra (P a,Ra-224 ) range from 0.09 x l0 3 to 3.44 x 10 3 atoms·m -3 ·s -1 and from 0.13 x 10 3 to 4.91 x 10 3 x 10 3 atoms·m -3 ·s -1 , respectively. P a,Ra-224 is also found to be larger than P r,Rn-222 in every station, revealing that aquifer solids contain more thorium than uranium in studied area. Both of P r,Rn-222 and P a,Ra-224 of coastal groundwater decreased seaward, revealing α-recoil supplying rates of 222 Rn and 224 Ra by aquifers rock decreased gradually, which gave good explanation of the spatial distribution characters of above two nuclides. P r,Rn-222 /A Rn-222 increase seaward from 0.3 to 0.9 along the major paths, with the average value of 0.6, Such results reveal that the primary source of groundwater 222 Rn in these areas is α-recoil of 226 Ra decay in solid pool, and its relative increase along the paths. Another source of 222 Rn is 226 Ra decay in the sorbed pool (R f,Ra-226 ·A Ra-226 ), which attributes about 40 per cent of total source of coastal groundwater 222 Rn. P α,Ra-224 /A Ra-224

  11. Dosimetry of bone metastases in targeted radionuclide therapy with alpha-emitting {sup 223}Ra-dichloride

    Energy Technology Data Exchange (ETDEWEB)

    Pacilio, Massimiliano [Azienda Ospealiera San Camillo Forlianini, Rome (Italy). Dept. of Medical Physics; Ventroni, Guido; Mango, Lucio [Azienda Ospealiera San Camillo Forlianini, Rome (Italy). Dept. of Nuclear Medicin; De Vincentis, Giuseppe; Di Castro, Elisabetta; Frantellizzi, Viviana; Follacchio, Giulia Anna; Garkavaya, Tatiana [Rome Univ. (Italy). Dept. of Radiological, Oncological and Anatomo Pathological Sciences; Cassano, Bartolomeo; Lorenzon, Leda [Rome Univ. (Italy). Postgraduate School of Medical Physics; Pellegrini, Rosanna; Pani, Roberto [Rome Univ. (Italy). Dept. of Molecular Medicine; Ialongo, Pasquale [Azienda Ospealiera San Camillo Forlianini, Rome (Italy). Dept. of Radiology

    2016-01-15

    Ra-dichloride is an alpha-emitting radiopharmaceutical used in the treatment of bone metastases from castration-resistant prostate cancer. Image-based dosimetric studies remain challenging because the emitted photons are few. The aim of this study was to implement a methodology for in-vivo quantitative planar imaging, and to assess the absorbed dose to lesions using the MIRD approach. The study included nine Caucasian patients with 24 lesions (6 humeral head lesions, 4 iliac wing lesions, 2 scapular lesions, 5 trochanter lesions, 3 vertebral lesions, 3 glenoid lesions, 1 coxofemoral lesion). The treatment consisted of six injections (one every 4 weeks) of 50 kBq per kg body weight. Gamma-camera calibrations for {sup 223}Ra included measurements of sensitivity and transmission curves. Patients were statically imaged for 30 min, using an MEGP collimator, double-peak acquisition, and filtering to improve the image quality. Lesions were delineated on {sup 99m}Tc-MDP whole-body images, and the ROIs superimposed on the {sup 223}Ra images after image coregistration. The activity was quantified with background, attenuation, and scatter correction. Absorbed doses were assessed deriving the S values from the S factors for soft-tissue spheres of OLINDA/EXM, evaluating the lesion volumes by delineation on the CT images. In 12 lesions with a wash-in phase the biokinetics were assumed to be biexponential, and to be monoexponential in the remainder. The optimal timing for serial acquisitions was between 1 and 5 h, between 18 and 24 h, between 48 and 60 h, and between 7 and 15 days. The error in cumulated activity neglecting the wash-in phase was between 2 % and 12 %. The mean effective half-life (T{sub 1/2eff}) of {sup 223}Ra was 8.2 days (range 5.5-11.4 days). The absorbed dose (D) after the first injection was 0.7 Gy (range 0.2-1.9 Gy). Considering the relative biological effectiveness (RBE) of alpha particles (RBE = 5), D{sub RBE} = 899 mGy/MBq (range 340-2,450 mGy/MBq). The

  12. A study of naturally occurring, radionuclide bearing deposits at Portland Creek, Newfoundland

    International Nuclear Information System (INIS)

    1985-01-01

    A small uraniferous peat deposit located near Portland Creek, Newfoundland was investigated as part of the National Uranium Tailings Program (NUTP). The purpose of the investigation was to provide data on naturally occurring uranium series radionuclides at a surface location that could be used to compare with the predictions of mathematical models. The investigation was carried out between August 18 and 30, 1984 by CBCL Limited with the assistance of Golder Associates, SENES Consultants Limited, Environmental Design Group and Monenco Analytical Laboratories. The investigation involved the determination of the geological and hydrogeological conditions of the deposit site and collection of soil, water and biological samples. The samples were analyzed for major element chemistry, uranium and its various decay series radionuclides including radium-226 and the ratio of uranium-234 to uranium-238. The uranium mineralization was found to be associated with a peat deposit that has accumulated in post-glacial time. The deposit is situated within a groundwater discharge zone at the toe of a granitic talus pile that extends downward from the Long Range Mountains. The concentration of uranium within the peat deposit was found to vary from 100 to 28000 ppm, however, the activities of the uranium decay series radionuclides were comparatively very low. Radium-226 activities were found to vary from 0.5 Bq/g to 15.0 Bq/g. Little influence from the deposit was noted in the surrounding water bodies, fish samples and vegetation. Based on the results of the study the uranium mineralization within the peat is considered to be the result of precipitation or adsorption from groundwater that had previously leached uranium from the granitic talus which forms the groundwater recharge zone. The major geochemical mechanism for deposition is considered to be associated with the strong reducing conditions encountered within the peat. Being a recent deposit (i.e. less than 10,000-15,000 years old

  13. Assessment of environmental impact models in natural occurring radionuclides solid wastes disposal from the mineral industry

    International Nuclear Information System (INIS)

    Pontedeiro, Elizabeth May Braga Dulley

    2006-07-01

    This work evaluates the behavior of wastes with naturally occurring radionuclides as generated by the mineral industry and their final disposal in landfills. An integrated methodology is used to predict the performance of an industrial landfill for disposal of wastes containing NORM/TENORM, and to define acceptable amounts that can be disposed at the landfill using long-term environmental assessment. The governing equations for radionuclide transport are solved analytically using the generalized integral transform technique. Results obtained for each compartment of the biogeosphere are validated with experimental results or compared to other classes of solutions. An impact analysis is performed in order to define the potential consequences of a landfill to the environment, considering not only the engineering characteristics of the waste deposit but also the exposure pathways and plausible scenarios in which the contaminants could migrate and reach the environment and the human population. The present work permits the development of a safety approach that can be used to derive quantitative waste acceptance criteria for the disposal of NORM/TENORM waste in landfills. (author)

  14. Transportation of natural radionuclides and rare earth light elements in the lagoon system of Buena, RJ

    International Nuclear Information System (INIS)

    Lauria, Dejanira da Costa

    1999-03-01

    it was investigated the transport of the series natural radionuclides and the earth rare light elements in a coastal lagoon system, located in a monazite rich region, in the coast north region of Rio de Janeiro state. The lagoon water showed off abnormal concentrations of radium isotopes and of the earth rare light elements (ERLEs). The longitudinal gradient of the Ra, of the ERLEs and of the major ion concentration's, whose data were obtained during two and half years of the research at the place, and the statistical analysis pointed to two mainly source as responsible for the water lagoon composition - the marine and the underground waters. The underground water supplies the radionuclides and ERLEs, possibly originated by monazite lixiviation. Based on the water speciation modeling, the results of laboratory adsorption on sediment experiments and the sediment characterization, the behavior of the radio isotopes, the ERLEs, U, Th e Pb-210, along of the lagoon, are discussed. It is also discussed the role of the aquatic macrophyte Typha dominguesis Pers in the nuclide uptake and the following liberation. (author)

  15. Natural radionuclides in the Brazilian coast region: 1. Estuarine complex Cananeia-Iguape, Sao Paulo State

    Energy Technology Data Exchange (ETDEWEB)

    Franca, E.J. de; Ferreira, Fabiano S.; Silva Neto, Paulo C.; Farias, Emerson E.G. de; Figueira, Rubens C.L.; Ribeiro, Andreza P., E-mail: ejfranca@cnen.gov.br, E-mail: biologofabiano10@gmail.com, E-mail: ptpoli@yahoo.com.br, E-mail: emersonemiliano@yahoo.com.br [Centro Regional de Ciencias Nucleares do Nordeste (CRCN-NE/CNEN-PE), Recife, PE (Brazil)

    2015-07-01

    Mangrove forests are of utmost important ecosystems for biogeochemical transport processes in a global scale because of the preferential transport via sediments and organic matter from continents to oceans. Such ecosystems are the richest biodiversity areas, in which bioaccumulation of chemical substances can be expected for some species, in this case, there is a lack of knowledge of natural radionuclides accumulation in mangrove vegetation. This work encompasses the first results obtained for the Estuarine Complex Cananeia-Iguape, a peculiar coast area of the Sao Paulo State, Brazil. In 2011, leaf samples of Rhyzophora mangle and Laguncularia racemosa trees with perimeter at the breast height higher than 15 cm were collected in the conservation unit Parque Estadual Ilha do Cardoso. Sample preparation consisted of leaf washing, oven-drying, milling in porcelain mortar at the particle size lower than 0.5 mm. Portions of 10 g were transferred to polyethylene vials of appropriate geometry for the analysis by high resolution gamma-ray spectrometry. Reference materials were analyzed together to evaluate the quality of the analytical procedure. K-40 was preferentially allocated in leaves. Some accumulation in leaves was noticed for Pb-210 and Ac-228 depending on the species, indicating differences of radionuclide distribution in the mangrove vegetation. (author)

  16. Natural and artificial radionuclides in forest and bog soils: tracers for migration processes and soil development

    International Nuclear Information System (INIS)

    Schleich, N.; Degering, D.; Unterricker, S.

    2000-01-01

    Radionuclide distributions in undisturbed forest and bog soils, mostly situated in Saxony, Germany (Erzgebirge), were studied. Low concentrations of naturally-occurring U and Th decay series nuclides, including 210 Pb, and artificial radioisotopes ( 125 Sb, 134 Cs, 137 Cs, 241 Am) were determined using low-level γ-spectrometry. In addition, the activities of 238 Pu and 239,240 Pu were determined by radiochemical separation and α-spectrometry. 14 C and excess 210 Pb dating methods were used to date the sampled bog profiles. The different radionuclides show characteristic depth distributions in the forest and bog soil horizons, which were sub-sampled as thin slices. 125 Sb, 241 Am, 238 Pu and 239,240 Pu are strongly fixed in soil organic matter. In spruce forest soils, the influence of soil horizons with distinct properties dominates the vertical time-dependent distribution. In ombrotrophic bogs, the peak positions correlated with the year of maximum input of each nuclide. The Sb, Am and Pu ''time markers'' and the 14 C and 210 Pb dating results correspond very well. Although Cs seems to be relatively mobile in organic as well as mineral forest soil horizons, it is enriched in the organic material. In ombrotrophic bogs, Cs is very mobile in the peat deposit. In Sphagnum peat, Cs is translocated continuously towards the growing apices of the Sphagnum mosses, where it is accumulated. (orig.)

  17. Influence of natural organic matter on the speciation of radionuclides in a geochemistry context

    International Nuclear Information System (INIS)

    Marang, L.

    2007-09-01

    The principal aim of this work is the study of the influence of natural organic matter, in particularly humic substances (HS), on the speciation of radionuclides (RN). The studied radionuclides are cobalt (II), europium (III) and uranium (VI). It has been shown that mobility and bioavailability of a metal are related to its speciation. The NICA-Donnan model describes metal ion binding to NOM: it accounts for NOM chemical heterogeneity, competition during binding and ionic strength effects. However the model has been calibrated with a limited number of experimental data for the RN. Indeed there is only a few speciation technique available for the study of the interactions RN-HS. Within the framework of this study, we have developed and optimised speciation technique (Flux Donnan Membrane Technique and the use of an un-solubilized humic acid) in order to acquire new experimental data, we have also studied the effect of the competition on RN speciation and finally we have tested the model capacity to predict the RN behavior in laboratory or in situ. (author)

  18. Influence of natural organic matter on the speciation of radionuclides in a geochemistry context

    International Nuclear Information System (INIS)

    Marang, L.

    2007-09-01

    The principal aim of this work is the study of the influence of natural organic matter, in particularly humic substances (HS), on the speciation of radionuclides (RN). The studied radionuclides are cobalt (II), europium (III) and uranium (VI). It has been shown that mobility and bioavailability of a metal are related to its speciation. The NICA-Donnan model describes metal ion binding to NOM: it accounts for NOM chemical heterogeneity, competition during binding and ionic strength effects. However the model has been calibrated with a limited number of experimental data for the RN. Indeed there is only a few speciation techniques available for the study of the interactions RN-HS. Within the framework of this study, we have developed and optimised speciation technique (Flux Donnan Membrane Technique and the use of an insolubilized humic acid) in order to acquire new experimental data, we have also studied the effect of the competition on RN speciation and finally we have tested the model capacity to predict the RN behavior in laboratory or in situ. (author)

  19. The concentration of natural radionuclides in various types of building materials in Slovakia

    Energy Technology Data Exchange (ETDEWEB)

    Cabanekova, H [Inst. of Peventive and Clinical Medicine, Bratislava (Slovakia)

    1996-12-31

    The concentration of the natural radionuclides in various types of building materials was determined by the gamma spectrometry analysis using 130 cm{sup 3} high purity germanium detector and MCA LIVIUS 2000. Radium-226 and thorium-232 was assessed through their progeny photo peaks. The specific activity of both nuclides as weighted average of their photo peaks was determined. Potassium-40 was measured directly via its 1460 keV peak. The radium equivalent activity was calculate from specific activities of radium-226, thorium-232 and potassium-40. All samples were measured in 4{sup p}i{sup g}eometry. The building materials and products were milled and screened with 2-3 mm sieve. After drying the samples were stored in 450 cm{sup 3} sealed polyethylene container for 30 days ingrowing period. The results of analysis are corrected to the background distribution and to the self absorption in the volume of the samples. The efficiency calibration is realized using the reference sources distributed by IAEA in Vienna and by the Institute for Radionuclide Production in Prague The measured activity concentrations of the buildings materials are given. There are shown the minimum and maximum values for different investigated materials. (J.K.) 4 tabs., 5 refs.

  20. Natural radionuclides distribution in the shelf and upper slope of southeast Brazil

    International Nuclear Information System (INIS)

    Cordero, Luisa M.; Figueira, Rubens C.L.; Mahiques, Michel M.; Tessler, Moyses G.

    2009-01-01

    In recent decades, Oceanography has been using a variety of radionuclides as tracers to understand the ocean dynamic processes, handling and disposal of sediments of seabed. In this context, the determination of natural radionuclides distributions ( 238 U, 232 Th and 40 K) has been carried out with sediments samples from the shelf and upper slope off Southeast Brazil using a gamma spectrometry technique. The samples were sliced into strata of 2 cm, dried, ground and properly packed to be analysed. The concentration of activities was performed in a hyperpure Ge detector with a resolution of 1,9 keV for the peak of 1332,3 keV of 60 Co, model GEM50P by EGG and ORTEC. The study area is located between latitudes 28 deg 40'S and 23 deg 00'S and extends from Cabo Frio (RJ) to Cabo de Santa Marta Grande (SC). The activity concentrations varied from 0,6 to 52,8 BqKg -1 for 238 U, from 1,6 to 50,9BqKg -1 for 232 Th and from 65,4 to 873,3 BqKg -1 for 40 K. From these results it is possible to establish a correlation between the depositional area dynamics and the samples size parameters. (author)

  1. Natural radionuclides in the Brazilian coast region: 1. Estuarine complex Cananeia-Iguape, Sao Paulo State

    International Nuclear Information System (INIS)

    Franca, E.J. de; Ferreira, Fabiano S.; Silva Neto, Paulo C.; Farias, Emerson E.G. de; Figueira, Rubens C.L.; Ribeiro, Andreza P.

    2015-01-01

    Mangrove forests are of utmost important ecosystems for biogeochemical transport processes in a global scale because of the preferential transport via sediments and organic matter from continents to oceans. Such ecosystems are the richest biodiversity areas, in which bioaccumulation of chemical substances can be expected for some species, in this case, there is a lack of knowledge of natural radionuclides accumulation in mangrove vegetation. This work encompasses the first results obtained for the Estuarine Complex Cananeia-Iguape, a peculiar coast area of the Sao Paulo State, Brazil. In 2011, leaf samples of Rhyzophora mangle and Laguncularia racemosa trees with perimeter at the breast height higher than 15 cm were collected in the conservation unit Parque Estadual Ilha do Cardoso. Sample preparation consisted of leaf washing, oven-drying, milling in porcelain mortar at the particle size lower than 0.5 mm. Portions of 10 g were transferred to polyethylene vials of appropriate geometry for the analysis by high resolution gamma-ray spectrometry. Reference materials were analyzed together to evaluate the quality of the analytical procedure. K-40 was preferentially allocated in leaves. Some accumulation in leaves was noticed for Pb-210 and Ac-228 depending on the species, indicating differences of radionuclide distribution in the mangrove vegetation. (author)

  2. Naturally Occurring Radionuclides and Rare Earth Elements Pattern in Weathered Japanese Soil Samples

    International Nuclear Information System (INIS)

    Sahoo, S.K.; Hosoda, M.; Takahashi, H.; Sorimachi, A.; Ishikawa, T.; Tokonami, S.; Uchida, S.

    2011-01-01

    From the viewpoint of radiation protection, determination of natural radionuclides e.g. thorium and uranium in soil samples are important. Accurate methods for determination of Th and U is gaining importance. The geochemical behavior of Th, U and rare earth elements (REEs) are relatively close to one another while compared to other elements in geological environment. Radioactive elements like 232 Th and 238 U along with their decay products (e.g. 226 Ra) are present in most of the environmental matrices and can be transferred to living bodies by different pathways that can lead to sources of exposure of man. Therefore, it is necessary to monitor these natural radionuclides in weathered soil samples to assess the possible hazards. The activity concentrations of 226 Ra, 228 Th, and 40 K in soils have been measured using a g γ-ray spectroscopy system with high purity germanium detector. The thorium, uranium and REEs were determined from the same sample using inductively coupled plasma mass spectrometry (ICP-MS). Granitic rocks contain higher amounts of Th, U and light REEs compared to other igneous rocks such as basalt and andesites. Therefore, it is necessary to understand the interaction between REEs and nature of soils, as soils are complex heterogeneous mixture of organic and inorganic solids, water and gases. In this paper, we have discussed about distribution pattern of 226 Ra, 232 Th and 238 U along with REEs in soil samples of weathered acid rock (granite and ryolite) collected from two prefectures in Japan: 1. Gifu and 2. Okinawa. (author)

  3. Determination of natural occurring radionuclide and heavy metals in drinking water in Malaysia

    International Nuclear Information System (INIS)

    Nur Suraya Ahmad

    2012-01-01

    The objective of this study is to ascertain the activity concentration of naturally occurring radionuclide and selected heavy metals selected mineral and drinking waters sample in Malaysia. The activity concentration of natural radionuclide (mBq/ L) was determined by Gamma Spectroscopy Systems while the concentration of heavy metal (mg/ L) was determined by the Induces Couple Plasma Mass Spectrometry (ICP-MS). The mineral and drinking water samples used in this study were Segar UKM, Giant, Ice Mountain (600 ml), Ice Mountain (1600 ml), Spritzer, Reverse Osmosis, and fresh tap water. The results of the study found 3 natural occurring radioactive materials (NORM) found for example - U-238, Ra-226 and Ra-228. The activity concentration determined was 0.00 mBq/ L to 1.71 mBq/ L for U-238, 0.00 - 32.46 mBq/ L for Ra-226 and 0.00 - 12.01 mBq/ L for Ra-228 respectively. The concentration of heavy metals Zn, Fe, As, Cl, Mn, Cu and Pb determined in this study were in the range of 0.000 - 0.003 mg/ L, 0.002-0.018 mg/ L, 0.000 - 0.007 mg/ L, 6.152 - 57.724 mg/ L, 0.000 - 0.016 μg/ L, 0.058 - 0.766 μg/ L and 0.000 - 0.380 μg/ L respectively. In general, the result of this study indicate that the activity concentration NORM and selected heavy metals in the studied mineral and drinking water samples were low and not exceed the limit set by World Organization (WHO) and Malaysian Food Regulations 1985. Thus, all the studied water samples complying the Malaysian drinking standard and safe to be consumed. (author)

  4. Controls of internal contamination from gamma-emitting radionuclides performed whole-body counter measures on children's population from Bjelorussia, Russia and Ucraina

    International Nuclear Information System (INIS)

    Tarroni, G.; Battisti, P.; Castellani, C.M.; Formignani, M.; Rampa, E.; Ticconi, R.

    1994-12-01

    This report summarizes the results obtained in 9 measurement campaigns, performed at the ENEA (Italian Agency for New Technologies, Energy and the Environment) centres of Bologna and Roma-Casaccia from April 1991 to September 1992, for the assessment of internal contamination from gamma-emitting radionuclides. Homogeneous samples were selected for the controls, each one representing the children's population from given area. 15 areas were investigated and 24 examined; 20 of them were from Bjelorussia. 266 children, 124 male and 142 female subjects, were controlled. The instruments were intercalibrated according to the body size, from 20.25 kg to 81 kg. Body contamination only from 1 37 Cs and 1 34 Cs was detected. Evaluations were performed in order to test appropriate use of ICRP caesium biokynetic model for children aged 8 to 15 years. Statistical distribution of body activity data were carefully analyzed. It is demonstrated that the data are well fitted by lognormal distribution and a difference between sexes in terms of activity. A significant difference between sexes was found in terms of activity intake

  5. Report on the IAEA-CU-2006-03 world-wide open proficiency test on the determination of gamma emitting radionuclides

    International Nuclear Information System (INIS)

    Shakhashiro, A.; Sansone, U.; Trinkl, A.; Makarewicz, M.; Yonezawa, C.; Kim, C.K.; Kis-Benedek, G.; Benesch, T.; Schorn, R.

    2007-05-01

    The results of analytical measurements play a vital role in our daily lives. Analytical data may be the basis upon which economic, legal or environmental management decisions are made, and they are essential in international trade, environmental protection, safe transportation, law enforcement, consumer safety and the preservation of human health. As an incorrect decision can be extremely costly and detrimental, it is essential that such measurements are accurate, reliable, cost effective and defensible. In addition, measurements performed by laboratories located worldwide should yield traceable and comparable results. Proficiency testing is a method for regularly assessing the accuracy of the analytical data produced by the laboratories of particular measurements. The IAEA-CU-2006-03 world-wide proficiency test (PT) on the determination of gamma emitting radionuclides in water grass and soil is conducted by the Chemistry Unit of the IAEA's Laboratories located in Seibersdorf (Austria), which is actively involved in the production and characterization of matrix reference materials of terrestrial origin, widely used for method validation and organization of proficiency tests and intercomparison studies. The Chemistry Unit is a part of the Physics, Chemistry and Instrumentation Laboratory. This report describes the sample preparation methodology, data evaluation approach, summary evaluation of each nuclide and individual evaluation report for each laboratory

  6. Almera Proficiency Test Determination of Naturally Occurring Radionuclides in Phosphogypsum and Water

    International Nuclear Information System (INIS)

    2010-01-01

    Phosphogypsum is generated as a by-product of the phosphoric acid based fertilizer industry. The discharge of phosphogypsum on earth surface deposits is a potential source of enhanced natural radiation and heavy metals, and the resulting environmental impact should be considered carefully to ensure safety and compliance with environmental regulations. A reliable determination of technologically enhanced naturally occurring radioactive materials in phosphogypsum is necessary to comply with the radiation protection and environmental regulations. This proficiency test (PT) is one of the series of the ALMERA network proficiency tests organised on a regular basis by the Chemistry Unit of the IAEA Terrestrial Environment Laboratory. These proficiency tests are designed to identify analytical problems, to support Member States laboratories to maintain their preparedness and to provide rapid and reliable analytical results. In this PT, the test item set consisted of six samples: one phosphogypsum (the IAEA-434 reference material) and five water samples spiked with natural radionuclides. The main task of the participating laboratories was to identify and quantify the activity levels of radionuclides present in these matrices. The tasks of IAEA were to prepare and distribute the samples to the participating laboratories, to collect and interpret analysis results and to compile a comprehensive report. The certified massic activity values of all radionuclides used in this PT were fulfilling the requirements of metrological traceability to international standards of radioactivity. In this PT, 306 test items (reference materials) were prepared and distributed to 52 participants from 40 countries in November 2008. The deadline for receiving the results from the participants was set to15 May 2009. For gross alpha/beta results the deadline was one working day from the date of sample delivery. The participating laboratories were requested to analyse Ra-226, U-234 and U-238 in water

  7. Radioactivity of some alpha, beta and gamma emitting radionuclides in surface marine sediments of different bays in Algeria

    International Nuclear Information System (INIS)

    Noureddine, A.; Baggoura, B.

    1999-01-01

    Samples of surface (0-15) cm marine sediments of different grain sizes, namely sand, muddy and fine sand, were collected in the western, central and east coast of Algeria, to measure concentrations of natural and artificial radioactivity. The aim of this study is to detect any radioactive contamination, its origin and also to determine the uptake of radioactivity by marine surface sediments

  8. Assessment and management of risks associated with exposures to Auger- and beta-emitting radionuclides. Recommendations and proposals for lines of research

    International Nuclear Information System (INIS)

    2010-01-01

    The assessment and management of risks associated with exposures to ionising radiation are defined by the general radiological protection system, proposed by the International Commission on Radiological Protection (ICRP). This system is regarded by a large majority of users as a robust system with well-established relevance for the management and prevention of exposures. Despite this, there are a number of dissenting voices, claiming that this system is not suitable for estimating the risks resulting from internal exposures, particularly when incorporated radionuclides decay, emitting electrons. Criticisms of the system particularly pertain to Auger- and beta-emitting radionuclides, the intake of which can occur during environmental and industrial exposures or, simply, during a medical use of ionising radiation for diagnostic or therapeutic purposes. These debates result from a lack of data in the fields of dosimetry and toxicology of these radionuclides. Auger and beta emitters can be distributed preferentially in certain tissue structures and even in certain cellular organelles, according to the vector with which they are associated. Given the limited range of electrons in matter, this heterogeneous distribution can generate highly localised energy depositions, not taken into account in conventional dosimetry methods, which make the assumption of uniform energy depositions. These specific physical and biochemical features of some of these radionuclides seem to influence their cellular toxicity directly. It is thus established that intranuclear distribution of iodine-125 is more effective for the induction of mutations or even cell death than a cytosolic distribution. This point is explained by the very short range of Auger electrons in matter (around a few dozen nm), which, in the case of an intranuclear distribution, would deliver all of their energy in the vicinity of the DNA, which, if affected, would be detrimental to the survival of the cell. The observation

  9. The Palmottu natural analogue project. Progress report 1995. The behaviour of natural radionuclides in and around uranium deposits, Nr. 9

    International Nuclear Information System (INIS)

    Ruskeeniemi, T.; Blomqvist, R.

    1996-01-01

    Natural analogue studies at Palmottu (in Finland) have concentrated on characterising the general geological, hydrogeological and radiochemical setting of the uranium mineralisation. Since 1992 a research program focusing on the hydrogeological characterisation of potential flow routes has been in progress, and the basis for a constrained flow system has already been identified. Sophisticated studies have also been performed on groundwater redox chemistry and matrix diffusion processes. The report consists of an introduction to the activities carried out in 1995 followed by topical summaries documented by the principal investigators in charge of each activity. The following summaries are included in the report (1) Hydrogeological studies at Palmottu, (2) Modelling of groundwater flow, (3) TV-logging of boreholes, (4) Mineralogical and petrological studies, (5) Radionuclide migration studies and (6) Humic substances. Full technical and scientific results are documented in appropriate topical reports and publications referred to in this Progress Report. (46 refs., 10 figs., 4 tabs.)

  10. Radionuclide toxicity

    International Nuclear Information System (INIS)

    Galle, P.

    1982-01-01

    The aim of this symposium was to review the radionuclide toxicity problems. Five topics were discussed: (1) natural and artificial radionuclides (origin, presence or emission in the environment, human irradiation); (2) environmental behaviour of radionuclides and transfer to man; (3) metabolism and toxicity of radionuclides (radioiodine, strontium, rare gas released from nuclear power plants, ruthenium-activation metals, rare earths, tritium, carbon 14, plutonium, americium, curium and einsteinium, neptunium, californium, uranium) cancerogenous effects of radon 222 and of its danghter products; (4) comparison of the hazards of various types of energy; (5) human epidemiology of radionuclide toxicity (bone cancer induction by radium, lung cancer induction by radon daughter products, liver cancer and leukaemia following the use of Thorotrast, thyroid cancer; other site of cancer induction by radionuclides) [fr

  11. Self-expandable covered metallic esophageal stent impregnated with beta-emitting radionuclide: an experimental study in canine esophagus

    International Nuclear Information System (INIS)

    Won, Je Hwan; Lee, Jong Doo; Wang, Hee Jung; Kim, Gui-Eon; Kim, Bong Wan; Yim, Hyunee; Han, Sang Keon; Park, Chan H.; Joh, Chul Woo; Kim, Kyung-Hwa; Park, Kyung Bae; Shin, Kyong-Min

    2002-01-01

    Purpose: A specially designed self-expandable covered metallic stent impregnated with the β-emitting radioisotope 166 Ho ( 166 Ho, energy: 1.85 and 1.76 MeV, T((1)/(2)): 26.8 h) was developed at our institute for the purpose of intraluminal palliative brachytherapy, as well as for treating malignant esophageal stricture and swallowing difficulty. The aim of this study was to evaluate the tissue response to brachytherapy and the safety of the radioactive metallic stent with regard to the normal canine esophagus before clinical application. Methods and Materials: 166 Ho was impregnated into the polyurethane membrane (50 μ thickness) covering the outer surface of a self-expandable metallic stent (diameter, 18 mm; length, 40 mm). Stents with radioactivity 4.0-7.8 mCi (Group A, n=15), 1.0-1.8 mCi (Group B, n 5), and 0.5-0.7 mCi (Group C, n=5) were placed in the esophagi of 25 healthy beagle dogs, and the stents were tightly anchored surgically to prevent migration. The estimated radiation dose calculated by Monte Carlo simulation was 194-383 Gy in Group A, 48-90 Gy in Group B, and 23-32 Gy in Group C. The dogs were killed 8-12 weeks after insertion of the stents, and histologic examinations of the esophageal walls were performed. Results: In Group A, 3 of 15 dogs died of wound infection, so specimens were obtained from only 12 dogs; all 12 cases showed esophageal stricture with mucosal ulceration. Microscopically, severe fibrosis and degeneration of the muscular propria were found in 3 dogs, complete fibrosis of the entire esophageal wall was found in 7 dogs, and esophageal fibrosis with radiation damage within periesophageal soft tissue was found in 2 dogs. However, esophageal perforation did not develop, despite extremely high radiation doses. In Group B, glandular atrophy and submucosal fibrosis were found, but the muscular layer was intact. In Group C, no histologic change was found in 3 dogs, but submucosal inflammation and glandular atrophy with intact mucosa

  12. Naturally Occurring Radionuclides of Ash Produced by Coal Combustion. The Case of the Kardia Mine in Northern Greece

    Science.gov (United States)

    Fotakis, M.; Tsikritzis, L.; Tzimkas, N.; Kolovos, N.; Tsikritzi, R.

    2008-08-01

    West Macedonia Lignite Center (WMLC), located in Northwest Greece, releases into the atmosphere about 21,400 tons/year of fly ash through the stacks of four coal fired plants. The lignite ash contains naturally occurring radionuclides, which are deposited on the WMLC basin. This work investigates the natural radioactivity of twenty six ash samples, laboratory produced from combustion of lignite, which was sampled perpendicularly to the benches of the Kardia mine. The concentrations of radionuclides 40K, 235U, 238U, 226Ra, 228Ra and 232Th, were measured spectroscopically and found round one order of magnitude as high as those of lignite. Subsequently the Radionuclide Partitioning Coefficients of radionuclides were calculated and it was found that they are higher for 232Th, 228Ra and 40K, because the latter have closer affinity with the inorganic matrix of lignite. During combustion up to one third of the naturally occurring radioisotopes escape from the solid phase into the flue gases. With comparison to relative global data, the investigated ash has been found to have relatively high radioactivity, but the emissions of the WMLC radionuclides contribute only 0.03% to the mean annual absorbed dose.

  13. Naturally Occurring Radionuclides of Ash Produced by Coal Combustion. The Case of the Kardia Mine in Northern Greece

    International Nuclear Information System (INIS)

    Fotakis, M.; Tsikritzis, L.; Tzimkas, N.; Kolovos, N.; Tsikritzi, R.

    2008-01-01

    West Macedonia Lignite Center (WMLC), located in Northwest Greece, releases into the atmosphere about 21,400 tons/year of fly ash through the stacks of four coal fired plants. The lignite ash contains naturally occurring radionuclides, which are deposited on the WMLC basin. This work investigates the natural radioactivity of twenty six ash samples, laboratory produced from combustion of lignite, which was sampled perpendicularly to the benches of the Kardia mine. The concentrations of radionuclides 40 K, 235 U, 238 U, 226 Ra, 228 Ra and 232 Th, were measured spectroscopically and found round one order of magnitude as high as those of lignite. Subsequently the Radionuclide Partitioning Coefficients of radionuclides were calculated and it was found that they are higher for 232 Th, 228 Ra and 40 K, because the latter have closer affinity with the inorganic matrix of lignite. During combustion up to one third of the naturally occurring radioisotopes escape from the solid phase into the flue gases. With comparison to relative global data, the investigated ash has been found to have relatively high radioactivity, but the emissions of the WMLC radionuclides contribute only 0.03% to the mean annual absorbed dose

  14. The assessment and management of risks associated with exposures to short-range Auger- and beta-emitting radionuclides. State of the art and proposals for lines of research

    International Nuclear Information System (INIS)

    Paquet, F; Biau, A; Barbey, P; Bardiès, M; Blanchardon, E; Chetioui, A; Lebaron-Jacobs, L; Pasquier, J L

    2013-01-01

    The assessment and management of risks associated with exposures to ionising radiation are defined by the general radiological protection system, proposed by the International Commission on Radiological Protection (ICRP). This system is regarded by a large majority of users as a robust system although there are a number of dissenting voices, claiming that it is not suitable for estimating the risks resulting from internal exposures. One of the specific issues of internal exposure involves short-range radiations such as Auger and beta particles. Auger- and beta-emitting radionuclides can be distributed preferentially in certain tissue structures and even in certain cellular organelles, according to their chemical nature and the vector with which they are associated. Given the limited range of the low-energy electrons in biological matter, this heterogeneous distribution can generate highly localised energy depositions and exacerbate radiotoxic responses at cellular level. These particularities in energy distribution and cellular responses are not taken into account by the conventional methods for the assessment of risk. Alternative systems have been proposed, based on dosimetry conducted at the cellular or even molecular level, whose purpose is to determine the energy deposition occurring within the DNA molecule. However, calculation of absorbed doses at the molecular level is not sufficient to ensure a better assessment of the risks incurred. Favouring such a microdosimetric approach for the risk assessments would require a comprehensive knowledge of the biological targets of radiation, the dose–response relationships at the various levels of organisation, and the mechanisms leading from cellular energy deposition to the appearance of a health detriment. The required knowledge is not fully available today and it is not yet possible to link an intracellular energy deposition to a probability of occurrence of health effects or to use methods based on cellular

  15. Determination of naturally occurring radionuclides in selected rocks from Hetaunda area, Central Nepal

    International Nuclear Information System (INIS)

    Wallova, G.

    2010-01-01

    The specific activities of the naturally occurring radionuclides 238 U, 232 Th, and 40 K were measured in rock samples from the Hetaunda area, central Nepal, by using gamma spectrometry. The specific activities were found to be in the range of 17 - 95 Bq.kg -1 for 238 U, 24 - 260 Bq.kg -1 for 232 Th and 32 - 541 Bq.kg -1 for 40 K. From these data absorbed dose rates in air and annual effective doses were calculated and compared with respective data from the United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) compilation. The results from our study open the door to the safe applicability of most of the investigated materials as a cheep building material. (author)

  16. Intercomparison of natural radionuclide measurements in marine sediment sample SD-N-1/2

    International Nuclear Information System (INIS)

    1985-06-01

    This intercomparison exercise was organized with the aim of providing to the participating laboratories a possibility of testing the performance of their analytical methods and to acquire basic data for establishing reference values for a number of natural radionuclides in the sediment material SD-N-1/2 from the North Sea floor. In tables are presented results expressed in mBq.g -1 on potassium, uranium isotopes, thorium-232 with the respective decay products, thorium-230, radium-226 and lead-210. Altogether 98 laboratories from 42 Member States joined this intercomparison. The results show generally good agreement, but more analytical work is needed to improve the present status of the lead-210 certification. Gamma and alpha spectroscopy were the most frequently used as the analytical techniques

  17. Natural analogues of radionuclide migration: reconnaissance study of sites (May 1985-March 1986)

    International Nuclear Information System (INIS)

    Hooker, P.J.; Ball, T.K.; Basham, I.R.; Bloodworth, A.J.; Roberts, P.D.; Ivanovich, M.

    1986-01-01

    Research into natural analogues of radionuclide migration provide data for supporting computer codes that describe the processes of transport and retardation. Such models are appropriate to the far-fields of shallow and deep radioactive waste repositories. The objective of this research project was to define locations within the UK and abroad worthy of detailed investigation. Site investigations and evaluations were carried out at a number of UK localities. The main focus of this survey has been on uraniferous veins in places at near surface where transport of uranium into sediments has occurred. Several uranium rich mineralisations associated with granite margins were visited in Cornwall, Devon and along the Solway Firth coast in Scotland; the disused U mine at South Terras in Cornwall and the coastal site at Needle's Eye near Dalbeattie are confirmed as future study sites. Results to hand from the sediments of Loch Lomand warrant further measurements of iodine and bromine in fresh cores. (author)

  18. Measurement of natural radionuclides in Malaysian bottled mineral water and consequent health risk estimation

    Energy Technology Data Exchange (ETDEWEB)

    Priharti, W.; Samat, S. B.; Yasir, M. S. [School of Applied Physics, Faculty of Science and Technology, Universiti Kebangsaan Malaysia, 43600 UKM Bangi, Selangor (Malaysia)

    2015-09-25

    The radionuclides of {sup 226}Ra, {sup 232}Th and {sup 40}K were measured in ten mineral water samples, of which from the radioactivity obtained, the ingestion doses for infants, children and adults were calculated and the cancer risk for the adult was estimated. Results showed that the calculated ingestion doses for the three age categories are much lower than the average worldwide ingestion exposure of 0.29 mSv/y and the estimated cancer risk is much lower than the cancer risk of 8.40 × 10{sup −3} (estimated from the total natural radiation dose of 2.40 mSv/y). The present study concludes that the bottled mineral water produced in Malaysia is safe for daily human consumption.

  19. The Spectroscopy Analysis of Natural Radionuclide in Some Agriculture Regions Homs City

    International Nuclear Information System (INIS)

    Soufan, A.

    2009-01-01

    Gamma Spectroscopy was utilized for assessment the radionuclide concentration ( K 40 , Ra 226 , Th 232 ..) in some agricultures regions in Homs City. The spectroscopy analysis carried on different samples from agricultures soil, black soil, red soil and........ and White soil chosen from different regions in Homs area. The study shows that all samples contain K 40 in large quantities, and Ra 226 , Th 232 in small quantities. The measurements showed that the dose varies between 942μSv/y for black soil and 524μSv/y for white soil. These results of the measurements have indicated that natural radioactivity in agricultures soils in Homs area are relatively normal and less than that estimated by another country in the world. (author)

  20. Naturally occurring radionuclides of paper ashes and their effect in the environment

    International Nuclear Information System (INIS)

    Kobashi, Asaya

    2011-01-01

    The concentrations of naturally occurring radionuclides ( 226 Ra, 228 Ra, 228 Th, and 40 K) in ashes of papers such as magazines and newspapers were determined from the nuclide concentrations in the papers and the ash contents of the papers. The average 226 Ra, 228 Ra, 228 Th, and 40 K concentrations in the 34 ashes were respectively 27, 68, 75, and 75Bq kg -1 . The radium equivalent activities of the ashes were calculated to evaluate the hazard of γ-ray radiation from the ashes in the environment. A copying paper sample showed a high radium equivalent activity of 602Bq kg -1 . However, the average radium equivalent activity was 140Bq kg -1 and was lower than the level that causes an environmental health problem. (author)

  1. Measurement of natural radionuclides in Malaysian bottled mineral water and consequent health risk estimation

    Science.gov (United States)

    Priharti, W.; Samat, S. B.; Yasir, M. S.

    2015-09-01

    The radionuclides of 226Ra, 232Th and 40K were measured in ten mineral water samples, of which from the radioactivity obtained, the ingestion doses for infants, children and adults were calculated and the cancer risk for the adult was estimated. Results showed that the calculated ingestion doses for the three age categories are much lower than the average worldwide ingestion exposure of 0.29 mSv/y and the estimated cancer risk is much lower than the cancer risk of 8.40 × 10-3 (estimated from the total natural radiation dose of 2.40 mSv/y). The present study concludes that the bottled mineral water produced in Malaysia is safe for daily human consumption.

  2. Natural radionuclide and radiological assessment of building materials in high background radiation areas of Ramsar, Iran.

    Science.gov (United States)

    Bavarnegin, Elham; Moghaddam, Masoud Vahabi; Fathabadi, Nasrin

    2013-04-01

    Building materials, collected from different sites in Ramsar, a northern coastal city in Iran, were analyzed for their natural radionuclide contents. The measurements were carried out using a high resolution high purity Germanium (HPGe) gamma-ray spectrometer system. The activity concentration of (226)Ra, (232)Th, and (40)K content varied from below the minimum detection limit up to 86,400 Bqkg(-1), 187 Bqkg(-1), and 1350 Bqkg(-1), respectively. The radiological hazards incurred from the use of these building materials were estimated through various radiation hazard indices. The result of this survey shows that values obtained for some samples are more than the internationally accepted maximum limits and as such, the use of them as a building material pose significant radiation hazard to individuals.

  3. Natural occurring radionuclide 210Po in the components of the Black Sea ecosystem

    International Nuclear Information System (INIS)

    Lazorenko, G. G.; Polikarpov, G. G.

    2006-01-01

    The interest to study of the behavior of naturally occurring radionuclide 2 10Po in marine ecosystem was caused by its main contribution to the doses of irradiation to hydrobionts. This work presents own data of 2 10Po concentrations determined in water, bottom sediments and hydrobionts of the Black Sea in 1998-2004. 2 10Po concentrations in water varied from 0.58 to 1.02 Bqxm - 3. Their range in bottom sediments from shelf zone and open part of the Black Sea was 11.5-496.5 Bqxkg - 1 dry weight with maximum in the North-West region. The range of 2 10Po concentrations in bottom sediments from the Eastern part of the Black Sea was 4.5-220 Bqxkg-1 dry weight. Concentration factors (CF) of 2 10Po in bottom sediments reached 10 4 -10 5 . 2 10Po concentrations in the Black Sea hydrobionts are reported and compared with published data in the same taxa. The range of 2 10Po concentrations in the Black Sea mesozooplankton was 1.7-3.5 Bqxkg - 1 wet weight. It was 1.9-2.9 Bqxkg - 1 wet weight in the representative species of macro plankton community, namely the ctenophore Beroe ovata. 2 10Po concentrations in the Black Sea fishes depend on their belonging to different ecological groups and decrease from pelagic species to demersal and bottom ones. 2 10Po concentrations in the Black Sea mollusks excluding small species Nana nerithea were on the highest levels determined in hydrobionts inhabiting in this region. Concentration factors of this radionuclide, estimated on a wet weight basis, reached values of 1.5x10 3 for macrophytes, 4x10 3 for total zooplankton, 10 3 -10 4 for the entire fishes, depending on their ecological groups affiliation and (3.0-6.7) x10 4 for mollusks. So, the ability of the Black Sea hydrobionts to accumulate natural radionuclide 2 10Po is comparable with that of similar species from others marine and oceanic areas

  4. Determination of soil screening levels for natural radionuclides in Minas Gerais state, Brazil

    International Nuclear Information System (INIS)

    Peixoto, Claudia Marques; Jacomino, Vanusa Maria Feliciano; Balaine, Fernando; Taddei, Maria Helena

    2013-01-01

    Soil screening levels express the levels of contaminant concentration in the soil, which guide the actions to be taken following investigation to confirm contamination. The list of toxic substances or elements under Brazilian legislation includes organics, volatile organics and metals but does not consider radioactive elements. Radioactive elements are all potentially carcinogenic and therefore need to be subject to legal control. The National Nuclear Energy Commission, the federal agency currently responsible for legislation regarding the control of Naturally-Occurring Radioactive Material (NORM) facilities does not establish guiding values for intervention in terms of soil activity concentration in the case of contamination with radioactive elements. In mining, the processing and treating of ores such as cassiterite, uranium, phosphate, niobium, and rare earths contribute to the generation of large amounts of NORM residues. Obviously, the improper disposal of these materials may lead to situations that result in soil and groundwater contamination and unnecessary exposure of the population in general. In order to establish guiding values for soil quality for natural radionuclides in the state of Minas Gerais, the study area included the entire state, which has unique characteristics related to the lithology, genesis, and morphology of the soils. These characteristics have tremendous influence on the petrogeochemistry of elements and radionuclides. A total of 110 soil samples were collected and analyzed in order to determine the activity concentration of U, Th, 226Ra, 228Ra e 210Pb. In general, it was possible to verify that the activity concentrations of U are higher than those of Th. This fact can be explained by the intense weathering that most of the state's soil has undergone and the chemical and geochemical characteristics of the two elements. The values obtained up to the present are higher than the reference values for soil quality adopted in other parts of

  5. The presence of some artificial and natural radionuclides in a Eucalyptus forest in the south of Spain

    International Nuclear Information System (INIS)

    Vaca, F.; Manjon, G.; Garcia-Leon, M.

    2001-01-01

    Long-lived artificial radionuclides ( 137 Cs, 90 Sr) were studied in a Eucalyptus plantation located in the south-west of Spain. Radionuclide concentrations were determined in different types of samples corresponding to specific forest components (soil, trees, herbs and litter). Depth profile distributions were obtained in two selected core soils. Two layers were separately measured in three other cores. The concentration factor, defined as the ratio between the mean activity concentration in a component and the mean activity concentration in the soil, was calculated for each component. The biomass of different components was estimated in order to evaluate the total density concentration (Bq/ha) of the artificial radionuclides ( 137 Cs, 90 Sr) in the Eucalyptus plantation. The transfer of the radionuclides between the different forest components can be inferred from the results. Additionally, other naturally occurring radionuclides ( 40 K, 226 Ra, 228 Ra, 228 Ac) were determined for comparison. Transport of radionuclides from forest to a nearby pulp mill is also discussed

  6. The natural radionuclide concentration and radon exhalation rate of Turkish natural stones

    International Nuclear Information System (INIS)

    Yasar, O.; Yaprak, G.; Guer, F.

    2006-01-01

    Geological materials usually contaminated with naturally occurring radioactive materials (NORM) have become a focus great attention. These NORM under certain conditions can reach hazardous contamination levels. Some contamination levels may be sufficiently severe that precautions must be taken. The Turkey has very important natural stones potential with over 5 billion m 3 marble reserves. According to 2002 giving data the number of Turkish stones export is 303 million US Dollars. In this regards, the present study deals with 120 Turkish natural stones. The studied samples were analyzed and the concentrations in Bq/kg dry weight of radioisotopes were determined by gamma-ray spectrometry using HPGe defector in Bq/kg dry weight. For the measurement of the radon exhalation rate, the 'can technique' using sensitive alpha sensitive LR-115 type II plastic defectors were used. The radium equivalent activity varied from 285 Bq/kg to 325 Bq/kg for granite samples and from 2 Bq/kg to 32 Bq/kg for marble samples. The value of radon exhalation rate ranged from 0.06 Bq/m 2 h - 1 to 0.46 Bq/m 2 h - 1 for garnite samples and from 0.006 Bq/m 2 h - 1 to 0.011 Bq/m 2 h - 1 for marble samples. According to the recommended values and the calculated external hazard index values the samples are acceptable for use as building materials and decoration

  7. Natural radionuclides by gammaspectrometry in region of Vojvodina, in Yugoslavia for 1998, 1997 and 1996

    International Nuclear Information System (INIS)

    Javorina, L.R.; Vukovic, D.M.; Markovic, D.

    2000-01-01

    Region of Vojvodina, as a agriculture region in Yugoslavia is important part of Yugoslavia. Monitoring of radioactivity in environment had established in the tree points: Novi Sad and Subotica as cities and Palic as a National park. Radioactivity comes mostly from natural radionuclides and partly from long-lived radionuclides from non natural sources as a consequence of Chernobyl accident. Monitoring of environment has proceeded by vertical methodology. We analyzed: aerosol, soil, fallout (wet and dry deposition), rivers, lakes, drinking water, human and animal food. Results from analyze of samples from environment contains very low activity, actually activity of changes of basic signal. Results for 1998, 1997 and 1996 are: 1. Gamma dose was measure in Belgrade with median years values: 0.103 μG/h (1998), 0.077 μG/h (1997) and 0.072 μG/h (1996). 2. By gammaspectrometry analyze of air of months samples for each year, results shows activity of changes of basic signal. The signals are coming from natural radionuclides. 3. 137 Cs, as a long lived radionuclide, with remarkable activity in soil are: Novi Sad 4.40-19.2 Bq/kg (1998), 8.2-16.3 Bq/kg (1997) and 5.0-10.8 Bq/kg (1996) and Palic 8.9-15.9 Bq/kg (1998), - Bq/kg (1997) and 5.02-13.4 Bq/kg (1996). 4. Activity in rivers Danube (Novi Sad) and Tisa (Kanjiza) belongs to 40 K, while activities of 137 Cs, 226 Ra, 232 Th, 235 U and 238 U are in traces. Activity of river sediment comes from 137 Cs with values 0.4-46 Bq/kg of dry samples (river Danube). Activity in fish, mixture, white fish and others comes from 40 K 55-100 Bq/kg and 137 Cs 0.2-0.8 Bq/kg. 5. Activity of drinking waters, from city network shows low level of activity which comes from 40 K, for both places. 6. Activity in milk comes from 40 K: Novi Sad 31-59 Bq/l (1998), 36-59 Bq/l (1997) and 28-49.42 Bq/l (1996). Activities of 137 Cs are on the same level of detection. 7. Activity in the human food, measured in yogurt, meats, bread and agricultural

  8. Natural radionuclides by gammaspectrometry in region of Vojvodina, in Yugoslavia for 1998, 1997 and 1996

    Energy Technology Data Exchange (ETDEWEB)

    Javorina, L.R.; Vukovic, D.M. [Institute of Occupational and Radiological Health, Deligradska 29, Belgrade, Yugoslavia, Faculty of Physical Chemistry, Studentski trg 12, Belgrade (Yugoslavia); Markovic, D. [Faculty of Physical Chemistry, Belgrade (Yugoslavia)

    2000-05-01

    Region of Vojvodina, as a agriculture region in Yugoslavia is important part of Yugoslavia. Monitoring of radioactivity in environment had established in the tree points: Novi Sad and Subotica as cities and Palic as a National park. Radioactivity comes mostly from natural radionuclides and partly from long-lived radionuclides from non natural sources as a consequence of Chernobyl accident. Monitoring of environment has proceeded by vertical methodology. We analyzed: aerosol, soil, fallout (wet and dry deposition), rivers, lakes, drinking water, human and animal food. Results from analyze of samples from environment contains very low activity, actually activity of changes of basic signal. Results for 1998, 1997 and 1996 are: 1. Gamma dose was measure in Belgrade with median years values: 0.103 {mu}G/h (1998), 0.077 {mu}G/h (1997) and 0.072 {mu}G/h (1996). 2. By gammaspectrometry analyze of air of months samples for each year, results shows activity of changes of basic signal. The signals are coming from natural radionuclides. 3. {sup 137}Cs, as a long lived radionuclide, with remarkable activity in soil are: Novi Sad 4.40-19.2 Bq/kg (1998), 8.2-16.3 Bq/kg (1997) and 5.0-10.8 Bq/kg (1996) and Palic 8.9-15.9 Bq/kg (1998), - Bq/kg (1997) and 5.02-13.4 Bq/kg (1996). 4. Activity in rivers Danube (Novi Sad) and Tisa (Kanjiza) belongs to {sup 40}K, while activities of {sup 137}Cs, {sup 226}Ra, {sup 232}Th, {sup 235}U and {sup 238}U are in traces. Activity of river sediment comes from {sup 137}Cs with values 0.4-46 Bq/kg of dry samples (river Danube). Activity in fish, mixture, white fish and others comes from {sup 40}K 55-100 Bq/kg and {sup 137}Cs 0.2-0.8 Bq/kg. 5. Activity of drinking waters, from city network shows low level of activity which comes from {sup 40}K, for both places. 6. Activity in milk comes from {sup 40}K: Novi Sad 31-59 Bq/l (1998), 36-59 Bq/l (1997) and 28-49.42 Bq/l (1996). Activities of {sup 137}Cs are on the same level of detection. 7. Activity in

  9. Natural radionuclides and 137Cs in commercialized edible mushrooms in Sao Paulo-Brazil

    International Nuclear Information System (INIS)

    Castro, Lilian Pavanelli de

    2008-01-01

    Artificial and natural radionuclides are commonly found in several compartments of the earth's crust. Some mushroom species have a high capacity to absorb radionuclides and toxic elements from the soil. Diet is considered as one of the main routes of radioactive contamination. Therefore, radioactivity measurements in the environment and in food are extremely important to monitor the radiation levels that human can be exposed to either directly or indirectly. Environmental bio monitoring has demonstrated that diverse organisms such as crustaceans, fish and mushrooms are useful when evaluating both the contamination and the quality of the ecosystems. There are actually several radionuclides that can be accumulated in mushrooms, including 40 K, 137 Cs, 232 Th and 238 U. There are few studies in the Southern hemisphere countries, on the natural and artificial radioactivity levels in mushrooms. The present study evaluated 40 K, 137 Cs, 232 Th and 238 U in commercialized edible mushrooms in the state of Sao Paulo, Brazil. The edible mushroom samples were acquired in different commercial establishments in the Sao Paulo metropolitan region, specifically in Municipal Markets. Some samples were acquired directly from producers located in the cities of Mogi das Cruzes, Mirandopolis, Suzano and Juquitiba. About 400g were collected for each edible mushroom species, which included Agaricus sp, Pleurotus sp and Lentinula sp species. All the samples were prepared and stored in polyethylene bottles for approximately 35 days, so that secular equilibrium could be established before counting. The 40 K, 137 Cs, 232 Th and 238 U gamma activities were measured by gamma spectrometry. The equipment consisted of a Hyper pure Germanium detector connected to an electronic system. The detector efficiency was obtained from measurements of reference materials: IAEA-300, IAEA-327 and IAEA-375. The results for the specific activities in edible mushrooms samples ranged fi-om 461 to 1535 Bq kg -1

  10. Estimation of the radionuclide content and radionuclide behaviour and the state of the wild nature in the Chernobyl' PNN region

    International Nuclear Information System (INIS)

    Martoshov, V.Z.; Smirnov, E.G.; Suvorova, L.N.; Tarasova, O.V.; Bogatova, L.V.; Torkhova, N.Yu.

    1992-01-01

    As a result radioactive isotope decay an isotope relation in the threw-out radioactive substance changes and to 1991 year is such that: strontium-90, ruthenium-106, Cs-137, cerium-144, plutonium-238,-239,-240; americium-231. Next years the dose commitments will be formed from Sr-90, Cs-137, Pu-239, Am-241. In soils of the thirty kilometer zone the content of the watersoluble Cs-137 do not change with time (0.1-1.0% from the radionuclide content in the soil. The watersoluble form content of Sr-90 is above, than of CS-137, 0.2-1.8%). Six-year investigations in the thirty kilometer, zone show that the Cs-137 concentration in the animal organisms is not changed. In relation to the previous trophic level Cs-137 accumulates in organisms of amphibians, reptiles and predatory mammals and don't in the herbivorous animal organism

  11. Effects of water treatment processes used at waterworks on natural radionuclide concentrations

    International Nuclear Information System (INIS)

    Haemaelaeinen, K.; Vesterbacka, P.; Maekelaeinen, I.; Arvela, H.

    2004-08-01

    The occurrence of uranium and other natural radionuclides in waters of waterworks and the effects of the conventional water treatment processes on radionuclide concentrations were investigated. Water samples were collected from 17 waterworks. Radionuclide concentrations of the collected samples were compared to the currently valid concentrations according to the Finnish regulation, ST guide 12.3. Similarly the measured concentrations were compared to the values presented in the 98/83/EC directive and in the Commission recommendation, 2001/928/Euratom. The guidelines based on chemical toxicity of uranium were also considered. This report presents a summary of the radionuclide concentrations in waters distributed by waterworks. Short-term and logn-term temporal variation of radionuclide levels in raw water were also investigated. Waterworks selected to this study used different kinds of raw water sources and a variety of water treatment processes. Water samples were collected from 46 water catchments which used groundwater in soil, artificial groundwater or groundwater in bedrock as a source of raw water. The most common water treatment used in these catchments was alkalization. Other treatment processes used were various types of filtrations (sand, anthracite, slow sand and membrane filtration) and aeration. Four of the catchments distributed water without treatment. Sampling was carried out in co-operation with local health inspectors and waterworks staff in spring 2002. Later that autumn, monitoring samples were collected from eight catchments. The maximum value for radon, presented in ST guide 12.3, was exceeded in three water catchments that used groundwater in bedrock as a source of raw water. No exceedings were found in those water catchments that use groundwater in soil or artificial groundwater. The limits of uranium and radium calculated from the total indicative dose (98/83/EC) were not exceeded but the guidelines for lead and polonium, given in the

  12. A study of gamma-emitting radionuclides present into the sediments and algae of the ''Baie de l'Orne'' (Central Normandy Coast) collecting during the years 1980 - 1982

    International Nuclear Information System (INIS)

    Lepy, M.C.

    1982-01-01

    The present status of some environmental effects of existing sources of gamma-emitting radionuclides, along the Central part of the Normandy Coast (Calvados shores and river Orne mouth) was determined. A systematic study was made on the behaviour of the marine sediments and brown alga 'Laminaria digitata' with regard to their properties as indicators of radioactive contamination. Marine sediments were collected into the river Orne at fixed locations and into the sea in and around the estuary from 1977 to 1982. Algae samples were picked up along the coast from 1980 to 1982, mostly on the western part of the Orne estuary. Dosimetry techniques employed have produced accurate and reliable results, despite the very low levels of activity involved. Gamma-emitting radionuclides present in the environment (chiefly 106 Ru, 137 Cs, 95 Zr) were identified and measured. Their behaviour into the marine sediments and into Laminaria Digitata were determined. This study provides evidence on the presence of numerous gamma-emitting radionuclides into the marine environment of the Central part of the Normandy coast, but, altogether with very low levels of radioactivity [fr

  13. Monte Carlo simulation of age-dependent radiation dose from alpha- and beta-emitting radionuclides to critical trabecular bone and bone marrow targets

    Science.gov (United States)

    Dant, James T.; Richardson, Richard B.; Nie, Linda H.

    2013-05-01

    Alpha (α) particles and low-energy beta (β) particles present minimal risk for external exposure. While these particles can induce leukemia and bone cancer due to internal exposure, they can also be beneficial for targeted radiation therapies. In this paper, a trabecular bone model is presented to investigate the radiation dose from bone- and marrow-seeking α and β emitters to different critical compartments (targets) of trabecular bone for different age groups. Two main issues are addressed with Monte Carlo simulations. The first is the absorption fractions (AFs) from bone and marrow to critical targets within the bone for different age groups. The other issue is the application of 223Ra for the radiotherapy treatment of bone metastases. Both a static model and a simulated bone remodeling process are established for trabecular bone. The results show significantly lower AFs from radionuclide sources in the bone volume to the peripheral marrow and the haematopoietic marrow for adults than for newborns and children. The AFs from sources on the bone surface and in the bone marrow to peripheral marrow and haematopoietic marrow also varies for adults and children depending on the energy of the particles. Regarding the use of 223Ra as a radionuclide for the radiotherapy of bone metastases, the simulations show a significantly higher dose from 223Ra and its progeny in forming bone to the target compartment of bone metastases than that from two other more commonly used β-emitting radiopharmaceuticals, 153Sm and 89Sr. There is also a slightly lower dose from 223Ra in forming bone to haematopoietic marrow than that from 153Sm and 89Sr. These results indicate a higher therapy efficiency and lower marrow toxicity from 223Ra and its progeny. In conclusion, age-related changes in bone dimension and cellularity seem to significantly affect the internal dose from α and β emitters in the bone and marrow to critical targets, and 223Ra may be a more efficient

  14. Natural radionuclides in soils of a forest fragment of Atlantic Forest under ecological restoration process

    International Nuclear Information System (INIS)

    Ferreira, F.S.; Lira, M.B.; Souza, E.M.; França, E.J.

    2017-01-01

    The natural radioactive isotopes come from the radioactive series of the 238 U (Uranium Series), the 235 U (Actinium Series) and the 232 Th (Thorium Series) series, or they can occur in isolation as is the case with the 40 K. Primordial radionuclides such as 40 K, 232 Th, 235 U and 238 U exist since the formation of the earth, being found in appreciable amounts in nature and in some cases may present a mass activity above the acceptable of environmental radiation. The objective of this work was to evaluate the mass activity of 40 K, 226 Ra and 228 Ra in the soils of a fragment of Atlantic Forest under ecological restoration process located in the Municipality of Paulista, PE, Brazil. Soil samples (0 - 15 cm) were collected under the projection of the treetops of the most abundant trees in the region. After drying and comminution, analytical portions of 40 g were transferred to polyethylene petri dishes, sealed and stored for 30 days to ensure secular equilibrium. Radioactivity was quantified by High Resolution Gamma Spectrometry - EGAR. The mean physical activities of 40 K, 226 Ra and 228 Ra were 12, 15 and 20 Bq kg -1 , respectively, for the surface soil of the Parque Natural Municipal Mata do Frio. The values found were lower than those found in mangroves in the state of Pernambuco and those considered normal for soils worldwide

  15. Modelling of natural organic matter-linked radionuclide transport in Boom clay

    International Nuclear Information System (INIS)

    Govaerts, J.; Maes, N.

    2012-01-01

    Document available in extended abstract form only. In the framework of the Belgian research program on long term management of high-level and/or long-lived radioactive wastes coordinated by ONDRAF/NIRAS, Boom Clay is investigated for its potential to host a deep geological disposal repository. In order to demonstrate the suitability of the Boom Clay as a host rock, the mobility of critical radionuclides in this clay layer has been the subject of research during many years. As actinides, lanthanides and transition metals are known to form strong complexes with organic substances, the influence of the Natural Organic Matter (NOM) present in Boom Clay on the mobility of these critical radionuclides is of crucial importance. Interaction of radionuclides with OM present in Boom Clay could on the one hand retard the migration due to complexation/colloid interaction with the immobile OM, and on the other hand the mobility and solubility of the radionuclide can be enhanced by the formation of complexes/colloids with the mobile OM. The conceptual understanding (and its numerical modelling) of the kinetic stability and transport of these complexes/colloids is therefore regarded as highly important for the the long-term safety assesment of the geological disposal. This can be broken down into two subproblems: 1. Describing the transport behaviour of mobile OM in Boom Clay; 2. Describing the interaction of RN with mobile OM and the transport behaviour of the resulting complexes in Boom Clay. The first part of this paper revolves around the first subproblem, where a robust model for the description of the migration behaviour of Natural Organic Matter (NOM) is derived based on data from column migration experiments using 14 C-labelled NOM Tracer solution, obtained in the framework of the EC TRANCOM-II project. Clay plugs of different lengths and different Darcy velocities were used. Inverse modelling with the MATLAB and COMSOL numerical code was done in order to identify the

  16. Agricultural handling and natural radionuclide contents on vegetables cultivated at Rio de Janeiro

    International Nuclear Information System (INIS)

    Ribeiro, Fernando Carlos Araujo

    2004-01-01

    The food consumption is an important way of internal exposition of human beings to ionizing radiation. The chemical fertilizers, mainly the phosphate, may contain uranium and thorium and their decay radioactive products in significant levels. This way, the amount of natural radionuclides in vegetables can increase as well as the dose due to food consumption to consumers. This research aims to investigate the level of radionuclides in vegetables which were grown under different tillages and to obtain information about radionuclides concentrations in Brazilian fertilizers as well as it aims to get data of transfer factors for vegetables cultivated in Brazil. In the phosphate fertilizer samples, the concentrations of 226 Ra varied from 35 to 430 Bq.kg -1 , whereas the 228 Ra concentrations ranged from 32 to 176 Bq.kg -1 . Among the phosphate fertilizers, the highest radium concentrations were found in the super phosphate one. The values of radium concentrations in organic fertilizers varied from 14 to 51 Bq.kg -1 for 226 Ra and from 34 to 142 Bq.kg -1 for 228 Ra. Among these fertilizers the highest concentrations were found in bovine manure Significant statistical differences were not observed between the concentration of 226 Ra and 228 Ra in the vegetables cultivated in conventional tillage and the ones cultivated in organic tillage. The same was observed for the soil-to-plant transfer factors, whose values were 2.56 E-02 for 226 Ra and 3.56 E-02 for 228 Ra for the bean crop, 3.74 E-02 for 226 Ra and 4.74 E-02 for 228 Ra to lettuce crop. For carrot, the 226 Ra transfer factor value for the two tillages was 5.79 E-02, while the value for 228 Ra in the organic tillage (1.14 E-01) was higher than the value observed in the conventional tillages (3.94 E-02). For the culture of the bean, the values of concentration found in the samples of the subsistence handling had been inferior to the values found in the conventional and organic tillage, demonstrating that as much the

  17. Radiosensitivity of Prostate Cancer Cell Lines for Irradiation from Beta Particle-emitting Radionuclide ¹⁷⁷Lu Compared to Alpha Particles and Gamma Rays.

    Science.gov (United States)

    Elgqvist, Jörgen; Timmermand, Oskar Vilhelmsson; Larsson, Erik; Strand, Sven-Erik

    2016-01-01

    The purpose of the present study was to investigate the radiosensitivity of the prostate cancer cell lines LNCaP, DU145, and PC3 when irradiated with beta particles emitted from (177)Lu, and to compare the effect with irradiation using alpha particles or gamma rays. Cells were irradiated with beta particles emitted from (177)Lu, alpha particles from (241)Am, or gamma rays from (137)Cs. A non-specific polyclonal antibody was labeled with (177)Lu and used to irradiate cells in suspension with beta particles. A previously described in-house developed alpha-particle irradiator based on a (241)Am source was used to irradiate cells with alpha particles. External gamma-ray irradiation was achieved using a standard (137)Cs irradiator. Cells were irradiated to absorbed doses equal to 0, 0.5, 1, 2, 4, 6, 8, or 10 Gy. The absorbed doses were calculated as mean absorbed doses. For evaluation of cell survival, the tetrazolium-based WST-1 assay was used. After irradiation, WST-1 was added to the cell solutions, incubated, and then measured for level of absorbance at 450 nm, indicating the live and viable cells. LNCaP, DU145, and PC3 cell lines all had similar patterns of survival for the different radiation types. No significant difference in surviving fractions were observed between cells treated with beta-particle and gamma-ray irradiation, represented for example by the surviving fraction values (mean±SD) at 2, 6, and 10 Gy (SF2, SF6, and SF10) for DU145 after beta-particle irradiation: 0.700±0.090, 0.186±0.050 and 0.056±0.010, respectively. A strong radiosensitivity to alpha particles was observed, with SF2 values of 0.048±0.008, 0.018±0.006 and 0.015±0.005 for LNCaP, DU145, and PC3, respectively. The surviving fractions after irradiation using beta particles or gamma rays did not differ significantly at the absorbed dose levels and dose rates used. Irradiation using alpha particles led to a high level of cell killing. The results show that the beta-particle emitter

  18. Correlations of natural radionuclides in soil with those in sediment from the Danube and nearby irrigation channels

    International Nuclear Information System (INIS)

    Krmar, M.; Varga, E.; Slivka, J.

    2013-01-01

    The correlation between activity concentrations of some natural radionuclides ( 238 U, 226 Ra, 232 Th, 40 K) measured in soil and in sediment taken from the Danube River and nearby irrigation channels was studied. The soil samples were collected from the northern part of Serbia and the sediment from the Serbian part of the Danube River and from the surrounding irrigation channels. The correlation between 238 U and other natural radionuclides in irrigation channel sediments was not as good as in the Danube. One of the possible explanations for this weak correlation can be the different chemical dynamics of 238 U in the irrigation channel sediment or changes of the 238 U activity concentration in irrigation channel sediment due to some human activities. The evaluation of ratios of activity concentrations of some natural radionuclides could be a more sensitive method for the determination of contaminant, rather than the straightforward analysis of activity concentrations. -- Highlights: ► 238 U, 232 Th and 40 K were measured in soil, Danube and surrounding channel sediment. ► Correlation of activity concentrations were observed. ► In cannel sediment natural radionuclides are not well correlated as in Danube one. ► Ratios of 238 U, 232 Th and 40 K can be good indicator for TENORM monitoring

  19. Influence of elevated radionuclide contamination on Natural Plant Polessky State Radioecological Reserve

    International Nuclear Information System (INIS)

    Goncharova, N.; Matsko, V.; Zhebrakova, I.; Montik, T.

    1998-01-01

    A group of meadow dominants was selected - representatives of the families Gramineae, Compositae, Primulaceae, Rosaceae, in which the 137 Cs migration from soil to overgrown phytomass relates closely with the sum of atmospheric precipitations. The fact has to be taken into account that in the conditions of chronic irradiation, the vegetation of the majority of meadow dominants (representatives of families of Gramineae and Leguminosae) is completed by the formation of valued seed posterity able to produce a new generation. The radiological situation in meadow grassland was evaluated in the territory of the Polessky State Radioecological Reserve. In a 9-year population monitoring experiment it was found that the radiosensitivity of different plants species was different due to the different specificity of the genetic systems and bioecological peculiarities of the species. The plant species with a narrow ecological amplitude, high ploidy, apomictic breeding are the most radiosensitive, as well as the plants which grow in Southern Belarus as a limit of their natural dissemination. Decrease in number was noted for the majority of such species, or elimination from plants communities. The anthropogenic load removal from the evacuation territories followed by the radical phytocenoses reconstruction is of ecological significance as the ionising radiation effect. It may be inferred that long-time chronic action of radionuclides on plants in the fallout zone will depend on specific features of their accumulation by some plant species, the age related radiosensitivity and some other factors, associated with their growing conditions such as soil types, forms of radionuclide fallout, chemical and physical effect

  20. Development of autoradiographic method for measuring sorption of radionuclides on natural fracture surfaces

    International Nuclear Information System (INIS)

    Muuronen, S.

    1983-11-01

    On the basis of positive results about sorption of radionuclides in rock thin sections an autoradiographic method applicable for measurement sorption of radionuclides on rough rock surfaces was developed. There is no method available because 1) a plane film cannot be used because due to the roughness of rock surfaces 2) rock samples used in this investigation cannot be studied with microscopes and 3) autoradiogram cannot be studied fixed on the surface of a rock sample because the colours of the minerals in the sample will interfere with the interpretation. This report discusses experimental work done to find an useful proedure. In the development of the method main emphasis was put on investigation of the following steps: 1) preparation of the sample for equilibration and spiking; 2) properties of the covering paint for the rock surface and 3) testing of autoradiographic methods using different nuclear emulsions. As the result of these experiments promising autoradiograms with gel emulsion for sawed rock surfaces and with stripping film for rough rock surfaces were obtained. The mineralogic disribution of sorbed activity is easily seen in autoradiograms. Much work must still be done to get reliable quantitative information from autoradiograms. For developing of the autoradiographic method sawed plane rock samples of quartz feldspar intergrowth, pegmatite and limestone were used. In addition core samples of tonalite and mica gneiss from Olkiluoto were utilized. The distribution coefficients (Ksub(a)) obtained for cesium were 560 x 10 -4 and 620 x 10 -4 m 3 /m 2 for tonalite and mica gneiss, respectively. The results are little higher but of the same order of magnitude as obtained by the autoradiographic method using rock thin sections and by the batch method using crused samples. The natural fracture surface sorption study is a logical step in determining the scaling factor from laboratory to field studies. Field data will be needed to determine whether laboratory

  1. Humic substances in natural waters and their complexation with trace metals and radionuclides: a review

    International Nuclear Information System (INIS)

    Boggs, S. Jr.; Livermore, D.; Seitz, M.G.

    1985-07-01

    Dissolved humic substances (humic and fulvic acids) occur in surface waters and groundwaters in concentrations ranging from less than 1 mg(C)/L to more than 100 mg(C)/L. Humic substances are strong complexing agents for many trace metals in the environment and are also capable of forming stable soluble complexes or chelates with radionuclides. Concentrations of humic materials as low as 1 mg(C)/L can produce a detectable increase in the mobility of some actinide elements by forming soluble complexes that inhibit sorption of the radionuclides onto rock materials. The stability of trace metal- or radionuclide-organic complexes is commonly measured by an empirically determined conditional stability constant (K'), which is based on the ratio of complexed metal (radionuclide) in solution to the product concentration of uncomplexed metal and humic complexant. Larger values of stability constants indicate greater complex stability. The stability of radionuclide-organic complexes is affected both by concentration variables and envionmental factors. In general, complexing is favored by increased of radionuclide, increased pH, and decreased ionic strength. Actinide elements are generally most soluble in their higher oxidation states. Radionuclides can also form stable, insoluble complexes with humic materials that tend to reduce radionuclide mobility. These insoluble complexes may be radionuclide-humate colloids that subsequently precipitate from solution, or complexes of radionuclides and humic substances that sorb to clay minerals or other soil particulates strongly enough to immobilize the radionuclides. Colloid formation appears to be favored by increased radionuclide concentration and lowered pH; however, the conditions that favor formation of insoluble complexes that sorb to particulates are still poorly understood. 129 refs., 25 figs., 19 tabs

  2. Study on the natural radionuclides in vegetables and food materials in Coonoor Taluk of Nilgiri Biosphere

    International Nuclear Information System (INIS)

    Sivakumar, R.; Selvasekarappandian, S.; Kannan, V.

    2005-01-01

    One of the important route through which radionuclides enter human body is food material. A considerable study on this aspect focuses on the natural radionuclides content since it is the major contributor to the total dose received by human beings. Natural radionuclides 226 Ra, 210 Po and 210 Pb in uranium series and 228 Ra in the thorium series exist ubiquitously in the environment and significantly contribute to the effective dose equivalent. The concentration of these radionuclides in different vegetables and food material collected in Coonoor taluk of Nilgiri Biosphere has been estimated. The concentration of 210 Po has been estimated by radiochemical separation followed by alpha counting. 210 Pb content in food material has been estimated by in growth of its daughter 210 Bi and followed by its counting by low background beta counting system. 228 Ra content has been estimated by chemical separation followed by, low background beta counting. 226 Ra has been estimated by chemical separation followed by emanation of 222 Rn and alpha counting. The vegetables and other food materials have been collected throught the study area Coonoor. The collected vegetable and food materials are coming under five categories such as leafy vegetable, tuberous vegetables, other vegetables, cereals and other food materials. The observed 210 Po concentration in the present study varies from 0.06 to 0.91 Ba/kg (fresh weight). The highest concentration of 210 Po (0.91 Bq/kg) has been observed in Tea collected at Thaimalai and the lowest value (0.06 Bq/kg) has been observed in carrot (root) collected at Bikole. The highest concentration of 210 Pb (1.12 Bq/kg) has been found in Cauliflower collected at Colocombai, while the least concentration of 210 Pb (0.12 Bq/kg) has been observed in Beans collected at Bikole. The Carrot coming under tuberous vegetable collected at Kateri have registered the highest value of 2.30 Bq/kg and the Cauliflower coming under leafy vegetable collected at

  3. Development of positron emitting radionuclides for imaging with improved positron detectors. [/sup 82/Rb, /sup 62/Zn, /sup 64/Cu, /sup 67/Ga

    Energy Technology Data Exchange (ETDEWEB)

    Yano, Y.

    1976-10-01

    Recent advances in positron cameras and positron ring detectors for transverse section reconstruction have created renewed interest in positron emitting radionuclides. This paper reports on: generator-produced /sup 82/Rb; cyclotron-produced /sup 62/Zn; and reactor-produced /sup 64/Cu. Investigation of the /sup 82/Sr (25 d)--/sup 82/Rb (75 s) generator determined the elution characteristics for Bio-Rex 70, a weakly acidic carboxylic cation exchanger, using 2% NaCl as the eluent. The yield of /sup 82/Rb and the breakthrough of /sup 82/Sr were determined for newly prepared columns and for long term elution conditions. Spallation-produced /sup 82/Sr was used to charge a compact /sup 82/Rb generator to obtain multi-millicurie amounts of /sup 82/Rb for myocardial imaging. Zinc accumulates in the islet cells of the pancreas and in the prostate. Zinc-62 was produced by protons on Cu foil and separated by column chromatography. Zinc-62 was administered as the amino acid chelates and as the ZnCl/sub 2/ to tumor and normal animals. Tissue distribution was determined for various times after intravenous injection. Pancreas-liver images of /sup 62/Zn-histidine uptake were obtained in animals with the gamma camera and the liver uptake of /sup 99m/Tc sulfur colloid was computer subtracted to image the pancreas alone. The positron camera imaged uptake of /sup 62/Zn-histidine in the prostate of a dog at 20 h. /sup 64/Cu was chelated to asparagine, a requirement of leukemic cells, and administered to lymphoma mice. Uptake in tumor and various tissues was determined and compared with the uptake of /sup 67/Ga citrate under the same conditions. /sup 64/Cu-asparagine had better tumor-to-soft tissue ratios than /sup 67/Ga-citrate.

  4. Report on the IAEA-CU-2006-08 proficiency test on the determination of gamma emitting radionuclides in sea water

    International Nuclear Information System (INIS)

    Shakhashiro, A.; Sansone, U.; Martin, P.; Makarewicz, M.; Mohagheghi, A.

    2007-03-01

    The Cooperative Monitoring Centre of Sandia National Laboratories of the United States (SNL) has initiated the Radiation Measurements Cross Calibration (RMCC) project. The RMCC aims to promote regional cooperation in the Middle East for preparedness for radiological emergencies. The International Atomic Energy Agency (IAEA) is cooperating with Sandia National Laboratories in this project. On a practical level, the initial aim of the RMCC is to establish a network of experts to cooperatively standardize nuclear monitoring and measurement capabilities in the Middle East by applying internationally recognized standards for laboratory radiation measurements. One of the project activities is to assist selected radiation measurement laboratories to participate in a quality assurance program and proficiency tests. During the second Workshop of the RMCC Project, organised by Sandia National Laboratories in Doha, Qatar, 12-17 November 2005, it was agreed to request the Chemistry Unit at the Agency's Seibersdorf laboratories to organise a special Proficiency Test (PT) for participants, for gamma-emitters in sea water. It is well known that proficiency testing is a method for regularly assessing the accuracy of the analytical data produced by the laboratories of particular measurements. According to the requirements of the RMCC project the IAEA-CU-2006-08 proficiency test (PT) on the determination of gamma emitting radionuclides in sea water was conducted by the Chemistry Unit of the IAEA's Laboratories located in Seibersdorf (Austria). The Chemistry Unit is actively involved in the production and characterization of matrix reference materials of terrestrial origin, widely used for method validation and organization of proficiency tests and intercomparison studies. The Chemistry Unit is a part of the Physics, Chemistry and Instrumentation Laboratory. This report describes the sample preparation methodology, data evaluation approach, summary evaluation of each nuclide and

  5. Utilization of natural hematite as reactive barrier for immobilization of radionuclides from radioactive liquid waste.

    Science.gov (United States)

    El Afifi, E M; Attallah, M F; Borai, E H

    2016-01-01

    Potential utilization of hematite as a natural material for immobilization of long-lived radionuclides from radioactive liquid waste was investigated. Hematite ore has been characterized by different analytical tools such as Fourier transformer infrared (FTIR), X-ray fluorescence (XRF), powder X-ray diffraction (XRD), thermogravimetry (TG) and differential thermal (DT) analysis, scanning electron microscopy (SEM) and BET-surface area. In this study, europium was used as REEs(III) and as a homolog of Am(III)-isotopes (such as (241)Am of 432.6 y, (242m)Am of 141 y and (243)Am of 7370 y). Micro particles of the hematite ore were used for treatment of radioactive waste containing (152+154)Eu(III). The results indicated that 96% (4.1 × 10(4) Bq) of (152+154)Eu(III) was efficiently retained onto hematite ore. Kinetic experiments indicated that the processes could be simulated by a pseudo-second-order model and suggested that the process may be chemisorption in nature. The applicability of Langmuir, Freundlich and Temkin models was investigated. It was found that Langmuir isotherm exhibited the best fit with the experimental results. It can be concluded that hematite is an economic and efficient reactive barrier for immobilization of long-lived radio isotopes of actinides and REEs(III). Copyright © 2015 Elsevier Ltd. All rights reserved.

  6. Natural and anthropogenic radionuclides in rocks and beach sands from Ezine region (Canakkale), Western Anatolia, Turkey

    Energy Technology Data Exchange (ETDEWEB)

    Orguen, Y. [Faculty of Mines, Istanbul Technical University (ITU), Ayazaga Kampusu, 34469-Istanbul (Turkey)]. E-mail: orgun@itu.edu.tr; Altinsoy, N. [Institute of Energy, Istanbul Technical University (ITU), Ayazaga Kampusu, 34469-Istanbul (Turkey); Sahin, S.Y. [Department of Geophysics, Engineering Faculty, Istanbul University, Istanbul (Turkey); Guengoer, Y. [Department of Geophysics, Engineering Faculty, Istanbul University, Istanbul (Turkey); Gueltekin, A.H. [Faculty of Mines, Istanbul Technical University (ITU), Ayazaga Kampusu, 34469-Istanbul (Turkey); Karahan, G. [Cekmece Nuclear Research and Training Center, P.O. Box 1, Atatuerk Airport, 34149-Istanbul (Turkey); Karacik, Z. [Faculty of Mines, Istanbul Technical University (ITU), Ayazaga Kampusu, 34469-Istanbul (Turkey)

    2007-06-15

    This paper represents the first reports on the natural and anthropogenic radionuclides in Kestanbol granitic pluton and surrounding rocks, and coastal region of the Ezine town. To assess the radiological hazard of the natural radioactivity, the radium equivalent activity, the absorbed dose rate and the external hazard index were calculated, and in situ gamma dose rates were measured. The high-activity concentrations were measured in the pluton and sands, which was originated mainly from the pluton, due to the presence of zircon, allanite, monazite, thorite, uranothorite and apatite. The average activity concentrations of {sup 238}U, {sup 232}Th and {sup 40}K are 174.78, 204.69 and 1171.95 Bq kg{sup -1} for pluton, and 290.36, 532.04 and 1160.75 Bq kg{sup -1} for sands, respectively. {sup 137}Cs in Ezine region ranged from 0-6.57 Bq kg{sup -1}. The average absorbed dose rate for the granitic and sand samples were calculated to be 251.6 and 527.92 nGy h{sup -1}, respectively. The maximum contribution to the total absorbed gamma dose rate in air was due to the {sup 232}Th (52.3% for pluton and 67.1% for sands). The Raeq activities of the pluton and sands are higher than the recommended maximum value of 370 Bq kg{sup -1} criterion limit of Raeq activity for building materials.

  7. Correlations between Natural Radionuclide Concentrations in Soil and Vine-Growth Potential

    International Nuclear Information System (INIS)

    Modisane, T.G.D.

    2008-01-01

    Stellenbosch district is known as one of the best wine-producing regions in South Africa and lies 45 km east of Cape Town. It has a large number of estates, of which one of them was earmarked for vineyard development and is of much importance to this study. Soil plays an important role in the development of the vine and ultimately the grapes harvested from the vine. It is therefore important to characterise vineyard soils (quantitatively and qualitatively) and to study the impact of soil properties on the vine. These properties include among others and of importance to this study, the soil ph, concentrations of trace elements, clay content and natural radioactivity concentrations (1). In this study correlations between radiometric data and traditional chemical data in vineyard soils used to infer growth potential were studied. Discussed below are experimental techniques used in the determination of activity concentration of natural radionuclide ( 40 K, 232 Th and 238 U) in soil, data analysis, results and conclusions

  8. Using hydrogeochemical data from natural environments to improve models of radionuclide speciation in groundwaters

    International Nuclear Information System (INIS)

    Read, D.; Hooker, P.

    1991-01-01

    It is essential that computer-based models used in the safety assessment of radioactive waste repositories accurately represent the processes occurring in real field systems. Confidence in long-term predictions of radionuclide migration will then depend upon the completeness of data available, particularly those obtained from the disposal site, and correct implementation of the model. The study of natural geochemical systems provides information on the adequacy of the underlying generic database and enhances our understanding of the transport mechanisms which form the basis of performance assessment. This paper concentrates on speciation-solubility modelling and describes four natural occurrences of uranium, each of which displays a different facet of uranium migration behaviour. The attributes of each site and the means by which uranium is immobilised are described. Retardation is highly species specific and this is illustrated through the use of site data in equilibrium speciation and coupled chemical transport calculations. Oxidation of U(IV) to U(VI) species promotes leaching of uranium ore at all the locations studied, emphasising the need to ensure that reducing conditions persist in a repository dominated by its actinide inventory. 5 figs., 46 refs

  9. Radiation dose to Malaysian infants from natural radionuclides via consumption of powdered milk

    Energy Technology Data Exchange (ETDEWEB)

    Uwatse, Onosohwo Bemigho; Olatunji, Michael Adekunle; Khandaker, Mayeen Uddin; Amin, Yusoff Mohd. [Department of Physics, University of Malaya, Kuala Lumpur 50603 (Malaysia)

    2015-04-24

    Milk is the basic food stuff for the infants because they generally consume more milk on a daily basis as its minerals and proteins are essential for their growth and development, therefore, it is very important to assess the natural radioactivity levels and the associated dose in the widely consumed powered infant’s milk. As a result, 14 brands of infant’s powdered milk were collected from different supermarkets around Selangor, Malaysia and analysed for {sup 226}Ra, {sup 232}Th and {sup 40}K activities. The obtained mean activity of {sup 226}Ra, {sup 232}Th and {sup 40}K are 3.05±1.84, 2.55±2.48 and 99.1±69.5 Bqkg{sup −1}, respectively. Among the analysed milk samples, the brand from Philippines (Lactogen) showed low level of radioactivity while Singaporean brand (S26 SMA Gold) showed the highest. The estimated mean annual effective doses due to the ingestion of natural radionuclides in the sampled milk are 635 and 111 µSv for infant ≤ 1y and infant 1-2y, respectively. The obtained dose value does not yet pose any significant radiological hazards to the population under investigation comparing with the 1.0 mSvy{sup −1} recommended by ICRP for all ages.

  10. Natural radionuclides in phosphatic fertilizer and their behaviour of absoption and accumulation in soils and crops

    International Nuclear Information System (INIS)

    Chen Jingjian; Zhu Yongyi; Yang Juncheng; Gu Baming

    1990-06-01

    The systematic data on the radioactivity of U, Th, Ra and 40 K in phosphate rocks, phosphatic fertilizers and soil are given. The radioactive composition and radioactivity in phosphatic fertilizers vary with different kinds of phosphatic fertilizers. The radioactive compositions in the phosphatic fertilizers made from phosphate rock are the same as that in the original phosphate rock, but the radioactivity is only 50∼60% of the original. The natural uranium in the compound fertilizer made from phosphoric acid is several times higher than that in the phosphate rock, and the other radionuclides were separated during the process of forming phosphoric acid. In soil, the radioactivity varies with the soil types. The U content is slightly higher in the south region with red earth and the 40 K is higher in the north region with black earth, but all are in normal level. Usually, the radioactivity of phosphate rock and phosphatic fertilizer is between the natural background of soil and the limitation of radioactive protection, but the radioactivity of 226 Ra in some phosphate rocks and phosphatic fertilizers in Guizhou and Hunan is higher than the permitted limitation set by the government

  11. A model for the calculation of the radiation dose from natural radionuclides in The Netherlands

    International Nuclear Information System (INIS)

    Ackers, J.G.

    1986-02-01

    A model has been developed to calculate the radiation dose incurred from natural radioactivity indoors and outdoors, expressed in effective dose equivalence/year. The model is applied on a three rooms dwelling characterized by interconnecting air flows and on a dwelling with crawlspace. In this model the distinct parameters are variable in order to allow the investigation of the relative influence. The calculated effective dose equivalent for an adult in the dwelling was calculated to be about 1.7 mSv/year, composed of 15% from cosmic radiation, 35% from terrestrial radioactivity, 20% from radioactivity in the body and 30% from natural radionuclides in building materials. The calculations show an enhancement of about a factor of two in radon concentration in air in a room which is ventilated by air from an adjacent room. It is also shown that the attachment rate of radon products to aerosols and the plate-out effect are relatively important parameters influencing the magnitude of the dose rate. (Auth.)

  12. Natural radionuclides in ceramic building materials available in Cuddalore district, Tamil Nadu, India.

    Science.gov (United States)

    Rajamannan, B; Viruthagiri, G; Suresh Jawahar, K

    2013-10-01

    The activity concentrations of radium, thorium and potassium can vary from material to material and they should be measured as the radiation is hazardous for human health. Thus, studies have been planned to obtain the radioactivity of ceramic building materials used in Cuddalore District, Tamilnadu, India. The radioactivity of some ceramic materials used in this region has been measured using a gamma-ray spectrometry, which contains an NaI(Tl) detector connected to multichannel analyzer. The specific activities of (226)Ra, (232)Th and (40)K, from the selected ceramic building materials, were in the range of 9.89-30.75, 24.68-70.4, 117.19-415.83 Bq kg(-1), respectively. The radium equivalent activity, absorbed gamma dose rate (D) and annual effective dose rate associated with the natural radionuclides are calculated to assess the radiation hazards of the natural radioactivity in the ceramic building materials. It was found that none of the results exceeds the recommended limit value.

  13. Radiation dose to Malaysian infants from natural radionuclides via consumption of powdered milk

    Science.gov (United States)

    Uwatse, Onosohwo Bemigho; Olatunji, Michael Adekunle; Khandaker, Mayeen Uddin; Amin, Yusoff Mohd.

    2015-04-01

    Milk is the basic food stuff for the infants because they generally consume more milk on a daily basis as its minerals and proteins are essential for their growth and development, therefore, it is very important to assess the natural radioactivity levels and the associated dose in the widely consumed powered infant's milk. As a result, 14 brands of infant's powdered milk were collected from different supermarkets around Selangor, Malaysia and analysed for 226Ra, 232Th and 40K activities. The obtained mean activity of 226Ra, 232Th and 40K are 3.05±1.84, 2.55±2.48 and 99.1±69.5 Bqkg-1, respectively. Among the analysed milk samples, the brand from Philippines (Lactogen) showed low level of radioactivity while Singaporean brand (S26 SMA Gold) showed the highest. The estimated mean annual effective doses due to the ingestion of natural radionuclides in the sampled milk are 635 and 111 µSv for infant ≤ 1y and infant 1-2y, respectively. The obtained dose value does not yet pose any significant radiological hazards to the population under investigation comparing with the 1.0 mSvy-1 recommended by ICRP for all ages.

  14. Radiation dose to Malaysian infants from natural radionuclides via consumption of powdered milk

    International Nuclear Information System (INIS)

    Uwatse, Onosohwo Bemigho; Olatunji, Michael Adekunle; Khandaker, Mayeen Uddin; Amin, Yusoff Mohd.

    2015-01-01

    Milk is the basic food stuff for the infants because they generally consume more milk on a daily basis as its minerals and proteins are essential for their growth and development, therefore, it is very important to assess the natural radioactivity levels and the associated dose in the widely consumed powered infant’s milk. As a result, 14 brands of infant’s powdered milk were collected from different supermarkets around Selangor, Malaysia and analysed for 226 Ra, 232 Th and 40 K activities. The obtained mean activity of 226 Ra, 232 Th and 40 K are 3.05±1.84, 2.55±2.48 and 99.1±69.5 Bqkg −1 , respectively. Among the analysed milk samples, the brand from Philippines (Lactogen) showed low level of radioactivity while Singaporean brand (S26 SMA Gold) showed the highest. The estimated mean annual effective doses due to the ingestion of natural radionuclides in the sampled milk are 635 and 111 µSv for infant ≤ 1y and infant 1-2y, respectively. The obtained dose value does not yet pose any significant radiological hazards to the population under investigation comparing with the 1.0 mSvy −1 recommended by ICRP for all ages

  15. Methods of measurement and evaluation of natural radionuclide contents in buildings, at building sites, and in building materials and water

    International Nuclear Information System (INIS)

    1998-01-01

    The recommendations should serve as guidelines for specifying the scope of measurement and ways of evaluating the measuring results when satisfying the relevant requirements laid down by the Czech Atomic Act (Act No. 18/1997) and Decree No. 184/1997 in the field of natural radiation sources occurring in the environment without deliberate use. The document consists of the following sections: Methodology for the measurement and assessment of natural exposure of persons in dwelling rooms of buildings; Methodology of determination of the radon risk of building sites; Principles of systematic measurement and evaluation of natural radionuclide contents of building materials; and Principles of systematic measurement and evaluation of natural radionuclide contents of supplied water. (P.A.)

  16. Natural and anthropogenic radionuclide distributions in the Nansen Basin, Artic Ocean: Scavenging rates and circulation timescales

    Science.gov (United States)

    Kirk Cochran, J.; Hirschberg, David J.; Livingston, Hugh D.; Buesseler, Ken O.; Key, Robert M.

    Determination of the naturally occurring radionuclides 232Th, 230Th, 228 Th and 210Pb, and the anthropogenic radionuclides 241Am, 239,240Pu, 134Cs and 137Cs in water samples collected across the Nansen Basin from the Barents Sea slope to the Gakkel Ridge provides tracers with which to characterize both scavenging rates and circulation timescales in this portion of the Arctic Ocean. Large volume water samples (˜ 15001) were filtered in situ to separate particulate (> 0.5 μm) and dissolved Th isotopes and 241Am. Thorium-230 displays increases in both particulate and dissolved activities with depth, with dissolved 230Th greater and particulate 230Th lower in the deep central Nansen Basin than at the Barents Sea slope. Dissolved 228Th activities also are greater relative to 228Ra, in the central basin. Residence times for Th relative to removal from solution onto particles are ˜1 year in surface water, ˜10 years in deep water adjacent to the Barents Sea slope, and ˜20 years in the Eurasian Basin Deep Water. Lead-210 in the central basin deep water also has a residence time of ˜20 years with respect to its removal from the water column. This texture of scavenging is reflected in distributions of the particle-reactive anthropogenic radionuclide 241Am, which shows higher activities relative to Pu in the central Nansen Basin than at the Barents Sea slope. Distributions Of 137Cs show more rapid mixing at the basin margins (Barents Sea slope in the south, Gakkel Ridge in the north) than in the basin interior. Cesium-137 is mixed throughout the water column adjacent to the Barents Sea slope and is present in low but detectable activities in the Eurasian Basin Deep Water in the central basin. At the time of sampling (1987) the surface water at all stations had been labeled with 134Cs released in the 1986 accident at the Chernobyl nuclear power station. In the ˜1 year since the introduction of Chernobyl 134Cs to the Nansen Basin, it had been mixed to depths of ˜800 m at

  17. Colloid migration in groundwaters: Geochemical interactions of radionuclides with natural colloids. 5. progress report. Period covered: July - December 1993

    Energy Technology Data Exchange (ETDEWEB)

    Kim, J.I. [Technische Univ. Muenchen, Garching (Germany); Delakowitz, B. [Technische Univ. Muenchen, Garching (Germany); Zeh, P. [Technische Univ. Muenchen, Garching (Germany); Probst, T. [Technische Univ. Muenchen, Garching (Germany); Lin, X. [Technische Univ. Muenchen, Garching (Germany); Ehrlicher, U. [Technische Univ. Muenchen, Garching (Germany); Schauer, C. [Technische Univ. Muenchen, Garching (Germany); Ivanovich, M. [Harwell Lab., AEA Environment and Energy, Oxon (United Kingdom); Longworth, G. [Harwell Lab., AEA Environment and Energy, Oxon (United Kingdom); Hasler, S.E. [Harwell Lab., AEA Environment and Energy, Oxon (United Kingdom); Gardiner, M. [Harwell Lab., AEA Decommissioning and RadWaste, Oxon (United Kingdom); Fritz, P. [GSF - Forschungszentrum fuer Umwelt und Gesundheit GmbH, Neuherberg (Germany); Klotz, D. [GSF - Forschungszentrum fuer Umwelt und Gesundheit GmbH, Neuherberg (Germany); Lazik, D. [GSF - Forschungszentrum fuer Umwelt und Gesundheit GmbH, Neuherberg (Germany); Wolf, M. [GSF - Forschungszentrum fuer Umwelt und Gesundheit GmbH, Neuherberg (Germany); Geyer, S. [GSF - Forschungszentrum fuer Umwelt und Gesundheit GmbH, Neuherberg (Germany); Alexander, J.L. [Atkins (W.S.) Engineering Sciences, Epsom (United Kingdom); Read, D. [Atkins (W.S.) Engineering Sciences, Epsom (United Kingdom); Thomas, J.B. [Atkins (W.S.) Engineering Sciences, Epsom (United Kingdom)

    1994-02-01

    The aim of the joint research programme is to determine the significance of groundwater colloids in far field radionuclide migration. The characterization, quantification and theoretical interpretation of colloid-borne transport phenomena of radionuclides in selected Gorleben aquifer systems are the main objectives of the present research programme. Gorleben aquifer systems are chosen because they are well characterized in terms of their hydrological and geological properties and because they contain substantial amounts of colloids of different chemical compositions as well as considerable quantities of chemical homologues and natural analogues of radionuclides, e.g. M(III), M(IV), M(VI), and Th and U decay series. The research tasks are investigated jointly by the four laboratories (listed below) in close coordination of experimental capacities of each laboratory. (orig.)

  18. Genotoxic endpoints in the earthworms sub-lethal assay to evaluate natural soils contaminated by metals and radionuclides

    Energy Technology Data Exchange (ETDEWEB)

    Lourenco, Joana I., E-mail: joanalourenco@ua.pt [CESAM and Departamento de Biologia, Universidade de Aveiro, Campus Universitario de Santiago, 3810-193 Aveiro (Portugal); Pereira, Ruth O., E-mail: ruthp@ua.pt [CESAM and Departamento de Biologia, Universidade de Aveiro, Campus Universitario de Santiago, 3810-193 Aveiro (Portugal); Silva, Ana C., E-mail: ana.cmj@ua.pt [CESAM and Departamento de Biologia, Universidade de Aveiro, Campus Universitario de Santiago, 3810-193 Aveiro (Portugal); Morgado, Jose M., E-mail: jmtmorgado@gmail.com [Centro de Histocompatibilidade do Centro, Praceta Prof. Mota Pinto, Edificio S. Jeronimo, 4o piso, Apartado 9041, 3001-301 Coimbra (Portugal); Carvalho, Fernando P., E-mail: fernando.carvalho@itn.pt [Instituto Tecnologico Nuclear, Estrada Nacional 10, 2686-953 Sacavem (Portugal); Oliveira, Joao M., E-mail: joaomota@itn.pt [Instituto Tecnologico Nuclear, Estrada Nacional 10, 2686-953 Sacavem (Portugal); Malta, Margarida P., E-mail: margm@itn.pt [Instituto Tecnologico Nuclear, Estrada Nacional 10, 2686-953 Sacavem (Portugal); Paiva, Artur A., E-mail: apaiva@histocentro.min-saude.pt [Centro de Histocompatibilidade do Centro, Praceta Prof. Mota Pinto, Edificio S. Jeronimo, 4o piso, Apartado 9041, 3001-301 Coimbra (Portugal); Mendo, Sonia A., E-mail: smendo@ua.pt [CESAM and Departamento de Biologia, Universidade de Aveiro, Campus Universitario de Santiago, 3810-193 Aveiro (Portugal); Goncalves, Fernando J., E-mail: fjmg@ua.pt [CESAM and Departamento de Biologia, Universidade de Aveiro, Campus Universitario de Santiago, 3810-193 Aveiro (Portugal)

    2011-02-15

    Eisenia andrei was exposed, for 56 days, to a contaminated soil from an abandoned uranium mine and to the natural reference soil LUFA 2.2. The organisms were sampled after 0, 1, 2, 7, 14 and 56 days of exposure, to assess metals bioaccumulation, coelomocytes DNA integrity and cytotoxicity. Radionuclides bioaccumulation and growth were also determined at 0 h, 14 and 56 days of exposure. Results have shown the bioaccumulation of metals and radionuclides, as well as, growth reduction, DNA damages and cytotoxicity in earthworms exposed to contaminated soil. The usefulness of the comet assay and flow cytometry, to evaluate the toxicity of contaminants such as metals and radionuclides in earthworms are herein reported. We also demonstrated that DNA strand breakage and immune cells frequency are important endpoints to be employed in the earthworm reproduction assay, for the evaluation of soil geno and cytotoxicity, as part of the risk assessment of contaminated areas. This is the first study that integrates DNA damage and cytotoxicity evaluation, growth and bioaccumulation of metals and radionuclides in a sub lethal assay, for earthworms exposed to soil contaminated with metals and radionuclides.

  19. Genotoxic endpoints in the earthworms sub-lethal assay to evaluate natural soils contaminated by metals and radionuclides

    International Nuclear Information System (INIS)

    Lourenco, Joana I.; Pereira, Ruth O.; Silva, Ana C.; Morgado, Jose M.; Carvalho, Fernando P.; Oliveira, Joao M.; Malta, Margarida P.; Paiva, Artur A.; Mendo, Sonia A.; Goncalves, Fernando J.

    2011-01-01

    Eisenia andrei was exposed, for 56 days, to a contaminated soil from an abandoned uranium mine and to the natural reference soil LUFA 2.2. The organisms were sampled after 0, 1, 2, 7, 14 and 56 days of exposure, to assess metals bioaccumulation, coelomocytes DNA integrity and cytotoxicity. Radionuclides bioaccumulation and growth were also determined at 0 h, 14 and 56 days of exposure. Results have shown the bioaccumulation of metals and radionuclides, as well as, growth reduction, DNA damages and cytotoxicity in earthworms exposed to contaminated soil. The usefulness of the comet assay and flow cytometry, to evaluate the toxicity of contaminants such as metals and radionuclides in earthworms are herein reported. We also demonstrated that DNA strand breakage and immune cells frequency are important endpoints to be employed in the earthworm reproduction assay, for the evaluation of soil geno and cytotoxicity, as part of the risk assessment of contaminated areas. This is the first study that integrates DNA damage and cytotoxicity evaluation, growth and bioaccumulation of metals and radionuclides in a sub lethal assay, for earthworms exposed to soil contaminated with metals and radionuclides.

  20. Performance assessment model development and parameter acquisition for analysis of the transport of natural radionuclides in a Mediterranean watershed

    International Nuclear Information System (INIS)

    Agueero, Almudena

    2005-01-01

    This paper describes the methodology developed to construct a model for predicting the behaviour of the natural radioisotopes of U, Th and Ra in a Mediterranean watershed. The methodology includes the development of the performance assessment model, obtaining water flow and radiological parameters based on experimental data and analysis of results. The model, which accounts for both water flows and mass balances of the radionuclides in a semi-natural environment, provides assessments of radionuclide behaviour in grassland and agricultural soils, rivers and reservoirs, including the processes of radionuclide migration through land and water and interactions between both. From field and laboratory data, it has been possible to obtain parameters for the driving processes considered in the model, water fluxes, source term definition, soil to plant transfer factors and distribution coefficient values. Ranges of parameter values obtained have shown good agreement with published literature data. This general methodological approach was developed to be extended to other radionuclides for the modelling of a biosphere watershed in the context of performance assessment of a High Level Waste (HLW) repository under Mediterranean climate conditions, as well as for forecasting radionuclide transport under similar Mediterranean conditions that will occur in the future in other areas. The application of sensitivity and uncertainty analysis was intended to identify key uncertainties with the aim of setting priorities for future research. The model results for the activity concentration in the reservoir indicate that for 238 U and 230 Th the most relevant parameter is the initial concentrations of the radionuclides in the reservoir sediments. However, for 226 Ra the most important parameter is the precipitation rate over the whole watershed

  1. Minimum detectable activities for natural radionuclides for IRIS-XP airborne gamma-spectrometer

    International Nuclear Information System (INIS)

    Ohera, Marcel; Sladek, Petr

    2009-01-01

    To subtract the 90 Sr background in the helicopter (the 90 Sr source is used as a freezing deposit indicator in Mi-17 helicopters), a spectrum at the altitude of more than 500 metre altitude above the ground for 10 minutes was acquired. The spectra at 50, 100 and 150 m altitude were corrected for the aircraft and the cosmics, stripping and height attenuation in K, U and Th peak windows. For IRIS-XP, better results have been obtained than presented so far. The new calculated minimum detectable activities (MDAs) are 114 Bq/kg for 40 K, 16 Bq/kg for 238 U and 8 Bq/kg for 232 Th at 95% confidence interval for 1 second spectra at 100 m altitude. This work deals with counting statistics and the estimate of the MDAs for natural radionuclides for the IRIS-XP airborne gamma-ray spectrometer (4 x 4 litre NaI(Tl)) produced by PICO Envirotec, Inc. in Toronto, Canada. The detection sensitivities (MDA) for 4 x 4 NaI(Tl) crystals at the altitude of 90 m presented by Pico Envirotec, Inc. are too high compared with the detection sensitivities presented by other airborne gamma-ray spectrometer producers. This was the reason why to calculate and verify the MDA for IRIS-XP. Firstly, the minimum detectable activities for IRIS-XP for 4 x 4 litre NaI(Tl) crystals were determined based on the data acquired on the calibration pads at the Holland Landing Airport in Toronto, Canada to test the method of calculation used. This method on calibration pads provides all available window sensitivities, stripping factors and counts in the natural radionuclide windows to verify the computing method. Secondly, the MDAs under the real flight conditions were also estimated for the IRIS-XP (4 x 4 litre NaI(Tl) crystals) which was delivered to the Czech Armed Forces. The MDAs were calculated based on the data acquired during the tests at the Military Training Area in Vyskov, Czech Republic. The data was collected at three different altitudes (50 m, 100 m and 150 m) when the Mi-17 helicopter with IRIS

  2. Distribution of natural and anthropogenic radionuclides in surficial sediments of Jakarta bay

    International Nuclear Information System (INIS)

    Ali Arman Lubis

    2006-01-01

    he concentration and distribution of natural and anthropogenic radionuclide in surficial sediments of Jakarta Bay were investigated with the aim of evaluating its level and environmental radioactivity. Sediments were sampled in 30 locations using Smith-McIntyre Grab sampler. Sediments were dried, homogenized and sealed for 1 month for equilibration and for the detection, analysis and data acquisition, a high purity germanium (HPGe) detector coupled with a high resolution multichannel analyzer (MCA) was used. Additionally, the grain sizes were analyzed by means of hydrometer. The result shows that the specific activity of 238 U, 226 Ra, 232 Th, 40 K and 137 Cs range from 6.71±1.01 Bq/kg to 28.63±4.29 Bq/kg, 6.46±0.97 Bq/kg to 28.21±4.23 Bq/kg, 16.62±2.49 Bq/kg to 40.46±6.07 Bq/kg, 115.80±12.16 Bq/kg to 358.69±30.49 Bq/kg, and 0.03±0.01 Bq/kg to 1.99±0.34 Bq/kg with the average value are 12.83±2.11 Bq/kg, 12.03±1.98 Bq/kg, 26.55±4.36 Bq/kg, 235.55±19.37 Bq/kg, and 0.77±0.13 Bq/kg, respectively. It shows that the activity of radionuclides in the research area are in natural level and the variation may be influenced by the grain size distribution in the sample. The absorbed dose rate and radium equivalent of gamma radiation was estimated to be 32.06±7.72 nano Grey/h and 68.14±11.20 Bq/kg, respectively. (author)

  3. Natural colloids in groundwater from granite and their potential impact on radionuclide transport

    International Nuclear Information System (INIS)

    Vilks, P.; Bachinski, D.B.

    1997-03-01

    AECL has submitted an Environmental Impact Statement (EIS) to evaluate the concept of nuclear fuel disposal at depth in crystalline rock of the Canadian Shield. As part of geochemical studies carried out in support of the EIS, the role of natural groundwater colloids (0.001 to 0.45 μm) and suspended particles (>0.45 μm) in radionuclide transport in granite rock has been investigated. This report summarizes the results of investigations carried out in groundwaters from the Whiteshell Research Area (WRA) of southern Manitoba and the Atikokan Research Area (ARA) of northwestern Ontario to determine the concentrations, size distributions, and compositions of natural particles in groundwaters from the Canadian Shield. Particles from groundwater were isolated by ultrafiltration under a nitrogen atmosphere and particle concentrations and size distributions were determined by filtration, and by laser-based particle counting and size analysis. Groundwaters from Canadian Shield granites contain particles in a broad range of sizes, with no one particular size being dominant. Particle compositions include aluminosilicates, Fe oxides, carbonate and organics. Suspended particles are most likely generated by the mobilization of fracture-lining minerals by groundwater flow, while colloids are formed by a combination of precipitation and mobilization of colloidal material from fracture surfaces. The average concentration of 0.01 to 0.45 μm colloids in WRA groundwaters was 1.05 ± 0.14 mg/L. Average colloid concentrations were slightly higher in the more highly fractured ARA, although the highest observed colloid concentration in the ARA was below the 7 mg/L maximum observed in a sample from the WRA. The existence of colloids in the 0.001 to 0.01 μm size range was demonstrated using the results of chemical analysis of particle concentrates and data obtained with the laser-based Ultrafine Particle Size Analyzer (UPA). The WRA groundwaters contain on average about 2.7 mg/L of 0

  4. A multielement analysis of natural radionuclides in an area of Pernambuco - Brazil

    International Nuclear Information System (INIS)

    Santos Junior, Jose Araujo dos; Menezes, Romulo Simoes Cezar

    2007-01-01

    Levels of natural radioactivity are the major cause of external exposure to gamma radiation. Based on this parameter, natural radioactivity of 238 U, 232 Th and 40 K were evaluated in a semiarid region of Pernambuco, Brazil, with the aim of obtaining radiometric monitoring of agricultural soils. For the analyses, the gamma spectrometry was utilized with a hyperpure germanium detector with an intrinsic efficiency of 27.7%. Seventy eight samples of soil that were collected in an area of approximately 55,500 m 2 , around an anomaly of uranium in rock, were analyzed. The activities of 238 U were evaluated by the 63 keV photopeak of 234 Th, that of 232 Th by the 338, 911 and 969 keV peak of 228 Ac, and that of 40 K by its 1,461 keV peak. The mean of the activities for these radionuclides were 91 Bq.kg -1 (median 88 Bq.kg -1 ) for the 238 U, 228 Bq.kg -1 (median 215 Bq.kg -1 ) for the 232 Th and 1,827 Bq.kg -1 (median 1,662 Bq.kg -1 ) for the 40 K. The anomalous rock did not present neither associated thorium nor potassium (values below the limit of detection: -1 of 232 Th and - '1 of 40 K), thus giving the characteristic of another natural radioactivity source. The obtained data allow to take important conclusions about the distribution of the radioactivity levels, to establish radioecological parameters. (author)

  5. Natural and anthropogenic radionuclides in Brazilian commercial dog food: preliminary results

    Energy Technology Data Exchange (ETDEWEB)

    Cavalcante, Fernanda; Pecequilo, Brigitte R.S. [Instituto de Pesquisas Energeticas e Nucleares - IPEN, Av. Professor Lineu Prestes 2242, 05508-000 Sao Paulo (Brazil)

    2014-07-01

    In recent decades, the exposure of non-human species to ionizing radiation, as well as its effects, has been given a different focus; on the one hand due to the increasing knowledge on different exposure situations that these species are subjected to and on the other hand, due to the concern regarding biodiversity and its protection. To estimate the effects of ionizing radiation over non-human biota, several key points must be considered, such as radionuclide concentration, dosimetry models, reference biota and others. A vast number of non-human individuals can be represented by reference organisms defined by different international organisms (UNSCEAR, ICRP and the FASSET project), to facilitate the assessment of exposure, absorbed dose and radiation effect for individuals from alike environments. There is, however, no specific representative for domestic animals, like dogs and cats. Brazil holds the second largest dog and cat population in the world, consuming over 2 million tons of feed every year. The Brazilian Association of the Industry of Products for Pets (ABINPET) foresees, for the year of 2013, an economic growth of 8.1% that may represent 0.34% of the gross domestic product (GDP). Animal food content and quality evaluations have been presented elsewhere, while no radiological study and the consequences from its ingestion have ever been conducted in the country. Hence, the present study will evaluate absorbed doses for domestic animals (i.e. dogs and cats) due to ingestion of food designed for them, by determining the radioactivity content of natural and anthropogenic cause. Initially, the activity concentrations in different brands of dry dog and cat food will be assessed by high resolution gamma spectrometry. Several brands usually consumed in Brazil were selected for the study. Eighteen dog food samples were prepared (crushed into powder and kiln dried) and tightly sealed in 100 mL high density polyethylene flasks, with a plan screw cap and bubble

  6. Cesium-137 and natural radionuclides in soils from southern Brazil and soils and others environmental samples from Antarctic

    International Nuclear Information System (INIS)

    Schuch, L.A.

    1993-04-01

    This work presents a study of environmental artificial and natural radioactivity levels in soil samples from the Southern Brazil and in soils and other environmental samples form Antarctica. Artificial radioactivity was determined by measuring Cs-137 which is a 30.1 year half-life man-made radionuclide produced in the past by atmospheric tests of nuclear weapons. Natural radioactivity was determined by measuring some radionuclides belonging to Th-232 and U-238 natural radioactive families, and of K-40 concentrations. Several types of soils from Southern Brazil; and soil samples, marine sediments, lichens, mosses and algae collected at King George and other nearby islands (South Shetland Archipelago, Antarctica) were analyzed. A gamma-ray spectrometer was used to measure radioactivity levels of the collected samples and its overall characteristics are analyzed in this work. (author)

  7. Hygienic assessment of using rocks with high content of natural radionuclides in road construction

    International Nuclear Information System (INIS)

    Kornilov, A.N.; Ryabchikov, S.G.

    1983-01-01

    Experimental investigations on radiation hygienic assessment of the possibilities of using rocks with an increased content of natural radionuclides (NRN) are carried out. At experimental road portions constructed using such rocks, γ-radiation levels have been measured and radioactive contamination of the ad-- jacent territory has been determined. The danger presented by such roads for highway engineering workers and population also has been assessed. The results obtained permit to express a possitive opinion on the use of solid wastes with an increased NRN content for construction of roads with asphalt coating. Rocks with specific α-activity 3 Bq/kg are recommended to be used for any types of road construction, whereas wastes with specific α-activity 3 Bq/kg - only for road construction in an industrial zone, between populated areas and for thoroughfares and highways. The use of wastes with a higher NRN content is unreasonable as it leads to a growth of annular dose to population and excessive exposure of construction workers engaged in highway engineering operations

  8. Ocean disposal option for bulk wastes containing naturally occurring radionuclides: an assessment case history

    International Nuclear Information System (INIS)

    Stull, E.A.; Merry-Libby, P.

    1985-01-01

    There are 180,000 m 3 of slightly contaminated radioactive wastes (36 pCi/g radium-226) currently stored at the US Department of Energy's Niagara Falls Storage Site (NFSS), near Lewiston, New York. These wastes resulted from the cleanup of soils that were contaminated above the guidelines for unrestricted use of property. An alternative to long-term management of these wastes on land is dispersal in the ocean. A scenario for ocean disposal is presented for excavation, transport, and emplacement of these wastes in an ocean disposal site. The potential fate of the wastes and impacts on the ocean environment are analyzed, and uncertainties in the development of two worst-case scenarios for dispersion and pathway analyses are discussed. Based on analysis of a worst-case pathway back to man, the incremental dose from ingesting fish containing naturally occurring radionuclides from ocean disposal of the NFSS wastes is insignificant. Ocean disposal of this type of waste appears to be a technically promising alternative to the long-term maintenance costs and eventual loss of containment associated with management in a near-surface land burial facility

  9. Natural radioactivity content and radionuclides leachability of bricks containing industrial waste

    International Nuclear Information System (INIS)

    Zalina Laili; Mohd Zaidi Ibrahim; Nur Azna Mahmud; Muhamat Omar

    2012-01-01

    A study have been carried out using gamma-ray spectrometric system to determine the natural radioactivity level in bricks made from industrial waste and their associated radiation hazard. Brick-1 and brick-2 contained waste from coal power plant and granite industry, respectively. The leachability of radionuclides from these bricks was also investigated. The activity concentration values of 226 Ra, 228 Ra, 232 Th, and 40 K are 64.25, 63.15, 67.9 and 254.19 Bq kg -1 , respectively in brick-1, and 193, 164.48, 164.63 and 1348.75 Bq kg -1 , respectively in brick-2. The radiation hazard indexes such as radium equivalent activities (Ra eq ), representative level index (I γr ), external hazard index (H ex ) and internal hazard index (H in ) were calculated and compared with the internationally approved values. Results indicate that brick-1 showed less radiological hazard than brick-2. This suggested that brick-1 could be used in building construction without exceeding the proposed criterion level. The leachability of 226 Ra for bricks showed the activity concentration slightly exceeded the limit generally used for industrial wastewater for example 1 BqL -1 . (author)

  10. Analysis of natural radionuclides in soil samples of Purola area of Garhwal Himalaya, India.

    Science.gov (United States)

    Yadav, Manjulata; Rawat, Mukesh; Dangwal, Anoop; Prasad, Mukesh; Gusain, G S; Ramola, R C

    2015-11-01

    Naturally occurring radioactive materials are widely spread in the earth's environment, being distributed in soil, rocks, water, air, plants and even within the human body. All of these sources have contributed to an increase in the levels of environmental radioactivity and population radiation doses. This paper presents the activity level due to the presence of (226)Ra, (232)Th and (40)K in soil samples of Purola area in Garhwal Himalaya region. The measured activity of (226)Ra, (232)Th and (40)K in collected soil samples of Purola was found to vary from 13±10 to 55±10 Bq kg(-1) with an average of 31±2 Bq kg(-1), 13±10 to 101±13 Bq kg(-1) with an average 30±3 Bq kg(-1) and 150±81 to 1310±154 Bq kg(-1) with an average 583±30 Bq kg(-1), respectively. The radium equivalent activity in collected soil samples was found to vary from 47 to 221 Bq kg(-1) with an average of 115 Bq kg(-1). The total absorbed gamma dose rate in this area was found to vary from 22 to 93 nGy h(-1) with an average of 55 nGy h(-1). The distribution of these radionuclides in the soil of study area is discussed in details. © The Author 2015. Published by Oxford University Press. All rights reserved. For Permissions, please email: journals.permissions@oup.com.

  11. Previous management practices for naturally occurring radionuclide wastes: current radiological status

    International Nuclear Information System (INIS)

    Goldsmith, W.A.; Crawford, D.J.; Haywood, F.F.; Leggett, R.Q.

    1979-01-01

    Many installations used during the early days of the United States atomic energy program have been released in recent years for unrestricted private uses. These installations include lands and buildings used for the storage of radioactive wastes resulting from refining and processing of uranium and thorium. Waste management practices at these sites in the 1940's and 1950's were not conducted with today's emphasis on as-low-as-reasonably-achievable (ALARA) principles. Consequently, many of these older waste storage areas are contaminated with naturally occurring radionuclides in concentrations which are orders of magnitude greater than those found ordinarily in the earth's crust. current and potential elevated human exposures at fifteen of these sites are due primarily to radon daughters and external-gamma radiation. A wide variety of exposure conditions may be found at these sites - ranging from slightly above background to more than thirty times the guidelines recommended for the public. Remedial actions are contemplated for a number of these sites where contamination levels or radiaion exposures exceed current guidelines

  12. Distribution of natural radionuclides in soils and beach sands of Abana-Çatalzeytin (Kastamonu)

    Energy Technology Data Exchange (ETDEWEB)

    Kurnaz, Aslı, E-mail: akurnaz@kastamonu.edu.tr; Özcan, Murat, E-mail: murat-ozcan@kastamonu.edu.tr; Çetiner, M. Atıf, E-mail: macetiner@kastamonu.edu.tr [Kastamonu University, Arts and Sciences Faculty, Department of Physics, Kastamonu (Turkey)

    2016-03-25

    A gamma spectrometric study of distribution of natural radionuclides in soil and beach sand samples collected from the terrestrial and coastal environment of Abana and Çatalzeytin counties of Kastamonu Province in Turkey was performed with the aim of estimating the radiation hazard of the tourist area and the concentrations of {sup 238}U, {sup 232}Th and {sup 40}K were determined. The activity concentrations of {sup 238}U, {sup 232}Th and {sup 40}K were determined in the ranges 14.95–56.0, 46.5–99.4 and 357.5–871.3 Bqkg{sup −1} for soil samples and the mean concentrations were ascertained as 42.34, 71.24 and 624.18 Bqkg{sup −1}, respectively. In sand samples, {sup 238}U, {sup 232}Th and {sup 40}K contents were varied in the ranges of 13.35-41.6, 30.9-53.4 and 275.5-601.3 Bqkg{sup −1} and the mean concentrations were ascertained as 20.57, 45.05 and 411.71 Bqkg{sup −1}, respectively. The mean annual effective doses were calculated as 113.08 and 69.16 µSvy{sup −1} for the soil and sand samples, respectively.

  13. Natural radionuclides in Austrian mineral water and their sequential measurement by fast methods

    International Nuclear Information System (INIS)

    Wallner, Gabriele; Wagner, Rosmarie; Katzlberger, Christian

    2008-01-01

    Ten samples of Austrian mineral water were investigated with regard to the natural radionuclides 228 Ra, 226 Ra, 210 Pb, 210 Po, 238 U and 234 U. The radium isotopes as well as 210 Pb were measured by liquid scintillation counting (LSC) after separation on a membrane loaded with element-selective particles (Empore TM Radium Disks) and 210 Po was determined by α-spectroscopy after spontaneous deposition onto a copper planchette. Uranium was determined by ICP-MS as well as by α-spectroscopy after ion separation and microprecipitation with NdF 3 . From the measured activity concentrations the committed effective doses for adults and babies were calculated and compared to the total indicative dose of 0.1 mSv/a given in the EC Drinking Water Directive as a maximum dose. The dominant portion of the committed effective dose was due to the radium isotopes; the dose from 228 Ra in most samples clearly exceeded the dose from 226 Ra

  14. Sensitivity analysis on retardation effect of natural barriers against radionuclide transport

    International Nuclear Information System (INIS)

    Hatanaka, K.

    1994-01-01

    The generic performance assessment of the geological disposal system for high level waste (HLW) in Japan has been carried out by the Power Reactor and Nuclear Fuel Development Corporation (PNC) in accordance with the overall HLW management program defined by the Atomic Energy Commission of Japan. The Japanese concept of the geological disposal system is based on a multi-barrier system which is composed of vitrified waste, carbon steel overpack, thick bentonite buffer and a variety of realistic geological conditions. The main objectives of the study are the detailed analysis of the performance of engineered barrier system (EBS) and the analysis of the performance of natural barrier system (NBS) and the evaluation of its compliance with the required overall system performance. Sensitivity analysis was carried out for the objectives to investigate the way and extent of the retardation in the release to biosphere by the effect of NBS, and to clarify the conditions which is sufficient to ensure that the overall system meets safety requirement. The radionuclide transport model in geological media, the sensitivity analysis, and the calculated results of the retardation effect of NBS in terms of the sensitivity parameters are reported. (K.I.)

  15. Disequilibrium study of natural radionuclides of uranium and thorium series in cores and briny groundwaters from Palo Duro Basin, Texas

    International Nuclear Information System (INIS)

    Laul, J.C.; Smith, M.R.

    1988-05-01

    The concentrations of natural radionuclides of the 238 U and /232/Th series are reported in several cores and in ten deep and five shallow briny groundwaters from various formations in the Palo Duro Basin. The formations include Granite Wash, Pennsylvanian Granite Wash, Wolfcamp Carbonate, Pennsylvanian Carbonate, Seven River, Queen Grayburg, San Andres, Yates and Salado. The natural radionuclide data in cores suggest that the radionuclides have not migrated or been leached for at least a period of about 1 million years. Relative to the U and Th concentrations in cores, the brines are depleted by a factor of 10 4 to 10 5 , indicating extremely low solubility of U and Th in brines. The natural radionuclide data in brines suggest that radium is not sorbed significantly and thus not retarded in nine deep brines. Radium is somewhat sorbed in one deep brine of Wolfcamp Carbonate and significantly sorbed in shallow brines. Relative to radium, the U, Th, Pb, Bi, and Po radionuclides are highly retarded by sorption. The retardation factors for 228 Th range from 10 2 to 10 3 , whereas those for 230 Th and 234 U range from 10 3 to 10 5 , depending on the formation. The 234 U/ 238 U ratios in these brines are constant at about 1.5. The magnitude of the 234 U/ 230 Th ratio appears to reflect the degree of redox state of the aquifer's environment. The 234 U/ 230 Th ratio in nine deep brines is about unity, suggesting that U, like Th +4 , is in the +4 state, which in turn suggests a reduced environment. 49 refs., 23 figs., 18 tabs

  16. State of radionuclides in seawater. Comparison of natural stable and artificial radioactive isotope s of mercury and zinc in natural waters of the arid zone of the USSR

    International Nuclear Information System (INIS)

    Rakhmatov, U; Khikmatov, K; Kist, A.A.; Kulmatov, R.A.; Teshabaev, S.T.; Volkov, A.A.

    1986-01-01

    This paper studies the state of stable and artificial radioactive isotopes of merury and zinc in natural waters of the arid zone of the USSR by radioactivity and radiochemical methods. Convergent results have been obtained for the dissolved forms of mercury and zinc in natural waters of the arid zone in a comparison of the results of radioactivation analysis and laboratory simulation using the radionuclides mercury-203 and zinc-65

  17. Survey on the radiation exposure of the respiratory tract by inhalation of natural radionuclides

    International Nuclear Information System (INIS)

    Poretti, G.

    1987-01-01

    During the last twenty years, work carried out on radiation exposure of the respiratory tract due to the inhaled, naturally occurring nuclides radon, thoron and short-lived daughters has become increasingly important, because the doses received in the respiratory tract, due mainly to the effect of α rays, reach values among the general population which are comparable to or even higher than the average exposures per year of a population undergoing X-ray diagnostic examinations. A brief introduction to the physical characteristics of the natural radiation nuclides reaching the bronchi and lungs with the inhaled air (Rn-220 - thoron and short lived daughters), and the deposition and clearance of the nuclides (often linked to aerosols), is followed by a discussion of the anatomical/physiological characteristics of the ''lung models'', thanks to which it is possible to calculate the energy quantities (i.e. doses) deposited by the α rays in the epithelium of the lungs and bronchi. In addition the retention mechanisms of the radionuclides (as free ions or as aerosols) are briefly described, and finally the calculations to determine the quantity of radioactivity remaining on the walls of the respiratory tract are given. The construction of dosimetric models requires relatively precise knowledge of the thickness of the mucus layers and of the distribution of the nuclides in the mucus, the ciliary movement, the depth in the tissue of the radiation-sensitive cells etc. On the basis of local doses it is then possible to calculate approximately the regional doses for bronchi, lungs and other organs (via blood, accessible by the nuclides before excretion) for the short lived daughters of Rn-222 and Rn-220. Determination of the mean effective dose equivalent requires, amongst other things, knowledge of the concentration of the nuclides in the inhaled air and the mean respiratory frequency of the members of a population. (orig./HSI)

  18. Effects of soil properties on natural radio-nuclides concentration in arid environment: a case study

    International Nuclear Information System (INIS)

    Khater, A.F.M.; Al-Sewaidan, H.A.I.; Al-Saif, A.S.; Diab, H.I.

    2008-01-01

    Soil samples were collected from an arid environment in the central region of Saudi Arabia, 28 samples from selected 14 locations in an agricultural farm. Two samples, one from cultivated land and the second from uncultivated land, of the same origin were collected from each location. This work aims at investigating the changes of soil properties due to dry-land use and its effects on naturally occurring radio-nuclides (NOR) concentration and distribution. The specific activity, in Bq/kg, of 226 Ra ( 238 U series), 228 gRa ( 232 Th series), 40 K and 137 Cs were measured using calibrated gamma-ray spectrometer. The soil physical and chemical properties [e.g. pH, EC, particle size distribution (clay, silt and sand percentages), CaCO 3 %, soluble cations (Ca, Mg, Na and K) and soluble anions (CO 3 , HCO 3 , Cl and SO 4 )] were determined. The radium equivalent activity, in Bq/kg, and absorbed dose rate one meter above the ground, in nGy/y, were calculated. Generally, there are not noticeable changes in soil properties due to agricultural activities or strong correlations between soil properties and NOR specific activities. That could be due to the sandy nature of the soil and the effects of adsorption-filtration processes on the behavior and the distribution pattern of NOR in arid environment. Therefore, the environmental impacts of different man-made activities on underground resources should be carefully considered due to the possible filtration behavior of different pollutants in dry-land environment. (author)(tk)

  19. Enrichment of naturally occurring radionuclides and trace elements in Yatagan and Yenikoy coal-fired thermal power plants, Turkey.

    Science.gov (United States)

    Ozden, Banu; Guler, Erkan; Vaasma, Taavi; Horvath, Maria; Kiisk, Madis; Kovacs, Tibor

    2018-08-01

    Coal, residues and waste produced by the combustion of the coal contain naturally occurring radionuclides such as 238 U, 226 Ra, 210 Pb, 232 Th and 40 K and trace elements such as Cd, Cr, Pb, Ni and Zn. In this work, coal and its combustion residues collected from Yatagan and Yenikoy coal fired thermal power plants (CPPs) in Turkey were studied to determine the concentrations of natural radionuclides and trace elements, and their enrichments factors to better understand the radionuclide concentration processes within the combustion system. In addition, the utilization of coal fly ash as a secondary raw material in building industry was also studied in terms of radiological aspects. Fly ash samples were taken at different stages along the emission control system of the thermal power plants. Activity concentrations of naturally occurring radionuclides were determined with Canberra Broad Energy Germanium (BEGe) detector BE3830-P and ORTEC Soloist PIPS type semiconductor detector. The particle size distribution and trace elements contents were determined in various ash fractions by the laser scattering particle size distribution analyzer and inductively coupled plasma (ICP-OES). From the obtained data, natural radionuclides tend to condense on fly ash with and the activity concentrations increase as the temperature drop in CPPs. Measured 210 Pb and 210 Po concentration varied between 186 ± 20-1153 ± 44 Bq kg -1 , and 56 ± 5-1174 ± 45 Bq kg -1 , respectively. The highest 210 Pb and 210 Po activity concentrations were determined in fly ash taken from the temporary storage point as 1153 ± 44 Bq kg -1 and 1174 ± 45 Bq kg -1 , respectively. There were significant differences in the activity concentrations of some natural radionuclide and trace elements (Pb and Zn) contents in ash fractions among the sampling point inside both of the plants (ANOVA, p ash sample analysis showed an increase activity concentration and enrichment factors towards the

  20. Studies on distribution coefficient (Kd) of naturally occurring radionuclides in geological matrices

    International Nuclear Information System (INIS)

    Pandit, G.G.

    2014-01-01

    Accurate prediction of fate and transport of toxic and radioactive metals in the subsurface of uranium tailing pond sites is critical to the assessment of environmental impact and to the development of effective remediation technologies. The mobility of radionuclides and toxic metals is enhanced by acidification of tailings due to sulphide oxidation catalysed by microbial activity. Due to infiltration of water, there is a possibility of leaching of these radionuclides and toxic metals from the tailings pond to the ground water. Sorption onto mineral surfaces is an important mechanism for reducing radionuclide concentrations along ground water flow paths and retarding radionuclide migration to the accessible environment. Reactive transport of ground water contaminants often assume that the reaction governing the retardation of a particular contaminant or radionuclide can be described by simple partitioning constant, K d . This constant is assumed to account for all the reversible sorption processes affecting transport of the contaminant. Experimental determination of site-specific K d values is absolutely essential for the accurate estimation of reactive transport of these contaminants. The results of such studies would be helpful to model migration of these pollutants and to estimate the radiation dose to members of the public through groundwater drinking pathway at different distances from the tailings pond. In the present study it is clearly observed that K d values of most of the radionuclides are strongly dependent on different soil and ground water parameters. The relationships generated between distribution coefficient values of different radionuclides and different soil and ground water parameters can be used to generate look up table. And these relationships can also be used for the prediction of K d values of different radionuclides by using the different physico-chemical parameters of soil and ground water of the particular location

  1. The use of lichens as bioindicators of atmospheric contamination by natural radionuclides and metals in a region impacted by TENORM

    International Nuclear Information System (INIS)

    Leonardo, Lucio

    2010-01-01

    The main aim of this thesis is to study the possibility of using lichen as bioindicator of atmospheric pollution in regions contaminated by radionuclides, metals and rare earth elements. Two regions were chosen, one in Pirapora do Bom Jesus, where a tin and lead industry is located, and a second one in Cubatao, where a phosphate fertilizer industrial complex is located. The two industries chosen are considered as TENORM - Technologically Enhanced Naturally Occurring Radioactive Material, since they can cause a significant increase in the natural radionuclides concentration in the industrial process, and consequently a potential increase in the radiation exposure in products, byproducts and residue. To achieve this aim, the radionuclides 238 U, 226 Ra, 210 Pb, 2' 3 2 Th and 228 Ra, rare earth elements and metals were analyzed in samples of raw material and residues from the installations, lichens and soils. Lichens and soil samples were analyzed by instrumental neutron activation analysis for the determination of uranium, thorium, rare earth elements and metals. The radionuclides 226 Ra, 228 Ra and 2 '1 0 Pb in soil samples were determined by gamma spectrometry and in lichen sample by radiochemical separation and gross alpha and beta counting on a gas flow proportional counter. The concentrations of 238 U (from 19 to 473 Bq kg -1 ), 226 Ra (from 21 to 265 Bq kg -1 ), 210 Pb (from 401 to 1461 Bq kg -1 ), 232 Th (from 15 to 574 Bq kg -1 ), 228 Ra (from 176 to 535 Bq kg'- 1 ), rare earth elements, Hf and Ta determined in lichen samples around the tin and lead industry show an enrichment in these elements. Therefore, the lichens can be used as a fingerprint of the atmospheric contamination. The results obtained for the lichen samples, in the Cubatao region, present a fingerprint mainly of 210 Pb, from industries of the region. The results obtained in this study showed that the lichens can be used as bioindicators of atmospheric pollution by radionuclides and trace

  2. An analysis of nature and mechanisms of the Lira objects territories' radionuclide contamination

    International Nuclear Information System (INIS)

    Kadyrzhanov, K.K; Tuleushev, A.Zh.; Lukashenko, S.N.; Solodukhin, V.P.; Kazachevskij, I.V.; Reznikov, S.V.

    2001-01-01

    In the paper the results of study of radioactive contamination of 'Lira' objects territories are presented. Obtained data are evidencing, that existing radiation situation does not presents a threat for operating personnel of both the occupied on the deposit and its objects furthermore for inhabitants of the closest localities. Therewith a radionuclides concentration in the soils on the examined areas is slightly exceeds the background values characteristic for this region. Two hypothesises for reveled radionuclide contamination have been considered: yield on the surface and distribution by territory immediately after explosion 137 Xe and 90 Kr inert gases - they are genetical predecessors of 137 Cs and 90 Sr, relatively; existence of a constant effluence of these radionuclides on a surface from a 'ditch cavities' of the 'Lira' objects by the zones of dis-consolidation and crack propagations in the earth crust. With purpose for these hypothesis correctness clarification the distribution of radionuclides by soil layer depth in the vicinities of militant wells (TK-2 and TK-5), as well as in the case and riverbed of the Berezovka river. There are not data confirm the hypothesis about possible constant radionuclides influent from a 'ditch cavities'. So, the hypothesis of the 'Lira' objects territories radionuclide contamination due to inert gases yield on the surface is a more rightful

  3. Naturally occurring radionuclides in food and drinking water from a thorium-rich area

    International Nuclear Information System (INIS)

    Costa Lauria, Dejanira da; Rochedo, Elaine R.R.; Godoy, Maria Luisa D.P.; Santos, Eliane E.; Hacon, Sandra S.

    2012-01-01

    This paper focuses on a survey of uranium and thorium decay chain radionuclides in food and drinking water from the thorium-rich (monazite-bearing) region of Buena, which is located in the state of Rio de Janeiro, Brazil. The radionuclide concentration values in the food and drinking water from Buena reached values higher than 100-fold the international reference values. The daily intake of radionuclides by the local population is similar to that of another high background radiation area in Brazil, but the intake is higher than that of residents from a normal background radiation area. Approximately 58 % of the food consumed by Buena inhabitants is produced locally. Based on that figure, locally produced food and the dilution of total radionuclides in the diet of residents caused by food importation are both highly relevant to a population's intake of radionuclides. The concentration values for 210 Pb and the radium isotopes in drinking water from Buena are among the highest values to be reported in the literature. 228 Ra is the most important radionuclide ingested with both food and water among the inhabitants of Buena. (orig.)

  4. Comparison of concentrations of natural and artificial radionuclides in Plankton from French Polynesian and Australian coastal waters

    International Nuclear Information System (INIS)

    Poletiko, C.; Twining, J.R.; Jeffree, R.A.

    1994-01-01

    Zooplankton samples from French Polynesian and Australian coastal waters were analysed for natural and artificial radionuclides. Quality control was assured by correlating replicate analyses between three laboratories and by participation in an international intercomparison exercise. Pu239/240 was detected sporadically among samples from both regions, with the highest levels being more consistently found in Tuamotu-Gambier samples. The artificial radionuclides Cs-137, Cs-134, Sr-90 and Co-60 were not detected. Of the natural nuclides, Ac-228 was detected in shallow continental waters off Northern Australia and an inverse relationship (P<0.02) was established between plankton density and their Po-210 concentration. (authors). 2 figs., 2 tabs., 9 refs

  5. Utility of γH2AX as a molecular marker of DNA double-strand breaks in nuclear medicine: applications to radionuclide therapy employing auger electron-emitting isotopes.

    Science.gov (United States)

    Mah, Li-Jeen; Orlowski, Christian; Ververis, Katherine; El-Osta, Assam; Karagiannis, Tom C

    2011-01-01

    There is an intense interest in the development of radiopharmaceuticals for cancer therapy. In particular, radiopharmaceuticals which involve targeting radionuclides specifically to cancer cells with the use of monoclonal antibodies (radioimmunotherapy) or peptides (targeted radiotherapy) are being widely investigated. For example, the ultra-short range Auger electron-emitting isotopes, which are discussed in this review, are being considered in the context of DNAtargeted radiotherapy. The efficient quantitative evaluation of the levels of damage caused by such potential radiopharmaceuticals is required for assessment of therapeutic efficacy and determination of relevant doses for successful treatment. The DNA double-strand break surrogate marker, γH2AX, has emerged as a useful biomonitor of damage and thus effectiveness of treatment, offering a highly specific and sensitive means of assessment. This review will cover the potential applications of γH2AX in nuclear medicine, in particular radionuclide therapy.

  6. Release of natural radionuclides in the Czech Republic - from water treatment plants where water from underground water sources is treated

    International Nuclear Information System (INIS)

    Sinaglova, R.

    2014-01-01

    In this abstract author deals with the treatment of drinking water in the Czech Republic with removing of natural radionuclides as well as with treatment of filter cartridges. The advantage of these technologies is that flushing is not required so no wastewater occurs. Used ion exchangers with higher content of uranium are processed in the chemical treatment of uranium ores, managed by DIAMO, state enterprise. (authors)

  7. Natural Radionuclides and 137Cs Concentrations in Rice in Jepara Residence and Internal Dose Estimation Intake by the People

    International Nuclear Information System (INIS)

    Leli-Nirwani; Minarni; Buchari

    2001-01-01

    The measurement of natural radionuclides and 137 Cs concentration in rice in Jepara residence and internal dose estimation intake by people have been conducted. The aim of the research is to determine internal dose estimation of natural radionuclides and 137 Cs intake by people in Jepara residence. By knowing the natural radionuclides and 137 Cs concentrations in rice at Jepara residence, the dose coefficient for adult from ICRP No.72 and the annual intake consumption take from the Indonesian food balance published by BPS, the internal dose from natural radionuclides and 137 Cs intake from food can be calculate concentration of 228 Th, 226 Ra and 137 Cs were found in Bayuran, with the average value was (2.00±0.21) x 10 -5 Bq/kg, (0.09±0.25) x 10 -5 Bq/kg, (19.00±0.06) x 10 -5 Bq/kg respectively the highest 40 K concentration was found in Pandansili with the average was about (8.40 ± 0.34) x 10 -5 Bq/kg. The estimation of equivalent doses from intake of 228 Th, 226 Ra, 40 K, and 137 Cs in rice were the highest in Bayuran the value the average values, respectively, was 0.0039 x 10 -5 μ Sv/yr, 18.09 X 10 -5 μ Sv/yr, 1.63 x 10 -5 μ Sv/yr, 172.38 x 10 -5 μ Sv/yr. Result in this measurement lowest comparing by recommendation IAEA in Safety Series No. 115 in 1996. (author)

  8. Investigation of natural radionuclides in foods and waters in China and evaluation of internal dose to public

    International Nuclear Information System (INIS)

    Zhu Changshou; Liu Yulan; Xu Ning; Hu Aiying; Kou Tiluo; Shi Zhongxin

    1992-12-01

    In order to obtain background radiation levels of natural radionuclides in foods and waters in China, the determination and analysis of water and food samples have been completed by organizations of radiological protection from 28 provinces, autonomous regions and three major cities. Ranges of specific activity of natural radionuclides for U, Th, Ra, K, Pb and Po are (2.2 ∼ 25.5) x 10 -2 Bq/kg, (0.5 ∼ 6.9) x 10 -2 Bq/kg, (3.4 ∼ 25.5) x 10 -2 Bq/kg, (25 ∼ 420) x 10 -2 Bq/kg, (3.9 ∼ 55) x 10 -2 Bq/kg and (2.7 ∼ 58) x 10 -2 Bq/kg, respectively. Samples of drinking water were taken from tap water or well. The average concentrations in tap water and well water are 2.8 x 10 -2 Bq/L and 3.7 x 10 -2 Bq/L for U, 0.8 x 10 -2 Bq/L and 1.3 x 10 -2 Bq/L for Ra, 0.07 x 10 -2 Bq/L and 0.06 x 10 -2 Bq/L for Th, 0. 3 x 10 -2 Bq/L and 1.1 x 10 -2 Bq/L for Pb and 0.3 Bq/L and 0.5 Bq/L for Po respectively. The annual intakes by ingestion have been calculated. The annual intake of male adult from six main natural radionuclides is about 205 Bq. Among them 64% of total intake of U is from drinking water. The contributions from grains to the total intake of Ra, Pb and Po are 55.7%, 59.7% and 70% respectively. The total annual average effective dose equivalent of 6 natural radionuclides for male adult in China is about 310 μSv

  9. Radionuclide Migration at the Rio Blanco Site, A Nuclear-stimulated Low-permeability Natural Gas Reservoir

    Energy Technology Data Exchange (ETDEWEB)

    Clay A. Cooper; Ming Ye; Jenny Chapman; Craig Shirley

    2005-10-01

    The U.S. Department of Energy and its predecessor agencies conducted a program in the 1960s and 1970s that evaluated technology for the nuclear stimulation of low-permeability gas reservoirs. The third and final project in the program, Project Rio Blanco, was conducted in Rio Blanco County, in northwestern Colorado. In this experiment, three 33-kiloton nuclear explosives were simultaneously detonated in a single emplacement well in the Mesaverde Group and Fort Union Formation, at depths of 1,780, 1,899, and 2,039 m below land surface on May 17, 1973. The objective of this work is to estimate lateral distances that tritium released from the detonations may have traveled in the subsurface and evaluate the possible effect of postulated natural-gas development on radionuclide migration. Other radionuclides were considered in the analysis, but the majority occur in relatively immobile forms (such as nuclear melt glass). Of the radionuclides present in the gas phase, tritium dominates in terms of quantity of radioactivity in the long term and contribution to possible whole body exposure. One simulation is performed for {sup 85}Kr, the second most abundant gaseous radionuclide produced after tritium.

  10. Metrology of natural radionuclides. Current challenges in radiation protection for industry and the environment; Metrologie natuerlicher Radionuklide. Aktuelle Herausforderungen fuer den Strahlenschutz in Industrie und Umwelt

    Energy Technology Data Exchange (ETDEWEB)

    Maringer, F.J. [Bundesamt fuer Eich- und Vermessungswesen, Wien (Austria). Referat fuer ionisierende Strahlung und Radioaktivitaet; Univ. fuer Bodenkultur, Wien (Austria). Low-Level Counting Lab. Arsenal; Moser, H.; Kabrt, F. [Bundesamt fuer Eich- und Vermessungswesen, Wien (Austria). Referat fuer ionisierende Strahlung und Radioaktivitaet; Baumgartner, A.; Stietka, M. [Univ. fuer Bodenkultur, Wien (Austria). Low-Level Counting Lab. Arsenal

    2015-07-01

    In a range of industrial branches increased activity concentrations of natural radionuclides occur in various NORM materials processed. The ICRP 103 recommendation, and subsequent the IAEA International Basic Safety Standards and the European Basic Safety Standards for Radiation Protection, raised new challenges in radiation protection concerning natural radionuclide metrology and activity measurement methods - in particular for natural decay chain radionuclides ({sup 238}U+, {sup 232}Th+, {sup 235}U+). Especially adequate traceability and optimized measurement uncertainties of applied activity measurement methods are of increasing concern. In this paper a review on radionuclide metrology of natural radionuclides and its implementation to end-user activity measurement methods and practice is presented. This includes an overview on current and emerging drivers, targets, challenges, deliverables, technologies and stakeholders in the field. Current research results on activity measurement standards and instrumentation for natural radionuclides, revised decay data, in-situ measurement methods, NORM reference materials, are covered as well as benefits of natural radionuclide metrology on radiation protection of workers and the public.

  11. Rapid detailed characterization of concrete shielding blocks utilizing internal natural radionuclides for calibration

    International Nuclear Information System (INIS)

    McDonald, R.J.; Smith, A.R.; Norman, E.B.; Cowles, D.

    1995-10-01

    Following many years of productive work, the SuperHILAC and Bevalac accelerators at Lawrence Berkeley National Laboratory were closed, leaving thousands of concrete shielding blocks available for reuse or disposal. The process history of these blocks as shielding precludes free release pending radiological characterization. This paper presents a method for the rapid characterization of gamma-ray-emitting radioisotopes in large samples of earth-like materials: concrete shielding blocks in this case. Active regions are identified with a sensitive radiation-survey instrument and then examined in detail with a high-efficiency lead-shielded Ge spectrometer. Naturally-occurring gamma-ray emissions from the decays of uranium, thorium, and potassium are used to calibrate the spectrometer. A simple relationship exists between the observed counting rate in a characteristic gamma ray and the activity in the block. This method, taking only tens of minutes per sample at the nano-Curie/gram sensitivity level, replaces much of the expensive coring and laboratory analysis methods needed otherwise

  12. Radiological impact of drinks intakes of naturally occurring radionuclides on adults of central zone of Malaysia

    International Nuclear Information System (INIS)

    Tawalbeh, A.A.; Samat, S.B.; Muhammad Samudi Yasir; Muhamat Omar

    2012-01-01

    Fifty three samples of different types of imported and locally produced drinks consumed in central zone of Malaysia were analyzed using gamma-ray spectrometry system. The measurement was conducted for 12 hours using a Canberra p-type high purity germanium (HPGe) gamma spectrometer with 30 % relative efficiency resolution of 1.8 keV at 1.33 MeV. The detector was connected to a computer with MCA card (Accuspec B) and Genie-2000 Analysis software of Canberra Industries, USA. The geometric means of daily intakes of 238 U, 232 Th and 40 K were 0.05, 0.08 and 27.23 respectively. Also the values give annual committed effective doses of 0.8, 6.5 and 61.53 μSv yr -1 for 238 U, 232 Th and 40 K, respectively for population in central zone of Malaysia. The net radiological impact of these radionuclides is 68.83 μSv yr -1 . This value gives cancer risk factor of 1.72 x 10 -7 . Also the value of net radiological impact gives loss of life expectancy of 0.43 days only. Whereas ICRP cancer risk factor for general public is 2.5 x 10 -3 and total risk involve from the all natural radiation sources based on global average annual radiation dose of 2.4 mSv yr -1 is 6.0 x 10 -3 . The estimated cancer risk shows that probability of increase of cancer risk from daily Malaysian drinks is only a minor fraction of ICRP values. Therefore the drink samples investigated here does not pose any significant health hazard and is considered radiologically safe for human consumption. (author)

  13. Radiation dose from natural and manmade radionuclides in the soil of NIAB, Faisalabad, Pakistan

    International Nuclear Information System (INIS)

    Akhtar, N.; Choudhry, M.A.; Orfi, S.D.; Waqas, M.

    2004-01-01

    Natural Radioactivity originates from extraterrestrial sources as well as from radioactive elements in the earth's crust. The amount of radioactivity in soil varies widely and is a source of continuous exposure to human beings. Amount of radioactivity in soil depends upon the type of soil and its uses. For the investigation of amount of radioactivity in the fertile soil, an area of about 100 hectares of land was selected in NIAB (Nuclear Institute for Agriculture and Biology) at Faisalabad, Pakistan. Soil samples were collected from the cultivated and fertilized land. Activity concentration was measured using a HPGe (high purity germanium) ray detector and a PC based MCA. Specific activity levels due to /sup 40/K, /sup 137/Cs, /sup 226/Ra and /sup 232/Th were determined in 125 fertilized soil samples collected at a spacing of about 4 hectares at the depth level of 0-25 cm with a step of 5 cm depth. Activity concentration of the concerned radionuclides for the NIAB soil is: /sup 40/K, 614.4 670.7 Bqkg/sup -1/; /sup 137/Cs, 2.1 3.1 Bqkg/sup -1/; /sup 226/Ra, 28.6 32.6 Bqkg/sup -1/; and /sup 232/Th, 51.6 60.3 Bqkg/sup -1/. Chemical analysis for concentration of Na, Ca and Mg was also carried out along with the measurement of electrical conductivity and pH of the soil samples. The absorbed dose in air at NIAB Farm is 75 nGyh/sup -1/ which is higher than the world average of 57 nGyh/sup -1/ but lies within the range (18-93) nGyh/sup -1/. (author)

  14. JGOFS IV. Subproject: natural radionuclides as tracers for particle dynamics in the water column. Final report

    International Nuclear Information System (INIS)

    Scholten, J.C.; Fietzke, J.; Mangini, A.; Stoffers, P.

    2000-01-01

    As part of the German JOINT GLOBAL OCEAN FLUX STUDY (JGOFS) the aim of the project was to investigate the particle dynamics in the water column, especially to estimate the trapping efficiencies of sediment traps deployed in the eastern North Atlantic (L1: 33 N 21 W; L2: 47 N 19.5 W; L3: 54,4 N 21,1 W; ESTOC: 29,07 N 15,25 W; OMEX: 49 N 12,5 W). This investigation was based on measurements of the distribution of natural radionuclides in the water column and in sediment traps. In the upper water column (≤1000 m) the 230 Th concentrations are similar at all locations investigated and a reversible scavenging model was able to describe the 230 Th distribution. In the deep water-column at L2 and L3 the 230 Th concentrations were significantly lower than predicted from the reversible scavenging model. The 230 Th concentrations here could be described by a scavenging-mixing model which assumes an advection of 230 Th depleted water masses and a rapid ventilation between 3 and 25 years. Based on two models, a mass balance for 230 Th and 231 Pa and a constant removal model, sediment trap efficiencies were calculated to be between 9% and 143%. The lowest efficiencies (9%-36%) were determined in the 500 m and 1000 m traps and no direct relation between water currents velocities and trapping biases were observed. The correction for trapping biases were found to be important for the understanding of the regional differences in the particle flux in the eastern north Atlantic. (orig.) [de

  15. The formation of ultra-fine particles during ozone-initiated oxidations with terpenes emitted from natural paint

    International Nuclear Information System (INIS)

    Lamorena, Rheo B.; Jung, Sang-Guen; Bae, Gwi-Nam; Lee, Woojin

    2007-01-01

    The formation of secondary products during the ozone-initiated oxidations with biogenic VOCs emitted from natural paint was investigated in this study. Mass spectrometry and infrared spectroscopy measurements have shown that the major components of gas-phase chemicals emitted from natural paint are monoterpenes including α- and β-pinenes, camphene, p-cymene, and limonene. A significant formation of gaseous carbonyl products and nano-sized particles (4.4-168 nm) was observed in the presence of ozone. Carboxylic acids were also observed to form during the reactions (i.e. formic acid at 0.170 ppm and acetic acid at 0.260 ppm). The formation of particles increased as the volume of paint introduced into a reaction chamber increased. A secondary increase in the particle number concentration was observed after 440 min, which suggests further partitioning of oxidation products (i.e. carboxylic acids) into the particles previously existing in the reaction chamber. The growth of particles increased as the mean particle diameter and particle mass concentrations increased during the reaction. The experimental results obtained in this study may provide insight into the potential exposure of occupants to irritating chemical compounds formed during the oxidations of biogenic VOCs emitted from natural paint in indoor environments

  16. Radionuclide accumulations in Clinch River fish

    International Nuclear Information System (INIS)

    Oakes, T.W.; Easterly, C.E.; Shank, K.E.

    1976-01-01

    Fish samples were collected from several locations above Melton Hill Dam, which is upstream from the liquid effluent release point of the Oak Ridge National Laboratory. The sampling locations were chosen to determine the accumulation of natural and man-made radionuclides in fish from areas in the Clinch River not influenced by the Laboratory's liquid effluents. Bass, carp, crappie, shad, bluegill, and other sunfish were collected; ten fish per species were composited to form a single sample for each location. The gamma-emitting radionuclide concentrations were determined by gamma-ray spectroscopy. Estimates of radiological dose to man subsequent to ingestion of these fish are made

  17. Computation Of The Residual Radionuclide Activity Within Three Natural Waterways At The Savannah River Site

    Energy Technology Data Exchange (ETDEWEB)

    Hiergesell, R. A.; Phifer, M. A.

    2014-01-07

    In 2010 a Composite Analysis (CA) of the U.S. Department of Energy’s (DOE’s) Savannah River Site (SRS) was completed. This investigation evaluated the dose impact of the anticipated SRS End State residual sources of radionuclides to offsite members of the public. Doses were assessed at the locations where SRS site streams discharge into the Savannah River at the perimeter of the SRS. Although the model developed to perform this computation indicated that the dose constraint of 0.3 mSv/yr (30 mrem/yr), associated with CA, was not approached at the Points of Assessment (POAs), a significant contribution to the total computed dose was derived from the radionuclides (primarily Cs-137) bound-up in the soil and sediment of the drainage corridors of several SRS streams. DOE’s Low Level Waste Federal Review Group (LFRG) reviewed the 2010 CA and identified several items to be addressed in the SRS Maintenance Program. One of the items recognized Cs-137 in the Lower Three Runs (LTR) Integrator Operable Unit (IOU), as a significant CA dose driver. The item made the recommendation that SRS update the estimated radionuclide inventory, including Cs-137, in the LTR IOU. That initial work has been completed and its radionuclide inventory refined. There are five additional streams at SRS and the next phase of the response to the LFRG concern was to obtain a more accurate inventory and distribution of radionuclides in three of those streams, Fourmile Branch (FMB), Pen Branch (PB) and Steel Creek (SC). Each of these streams is designated as an IOU, which are defined for the purpose of this investigation as the surface water bodies and associated wetlands, including the channel sediment, floodplain sed/soil, and related biota. If present, radionuclides associated with IOUs are adsorbed to the streambed sediment and soils of the shallow floodplains that lie immediately adjacent to stream channels. The scope of this effort included the evaluation of any previous sampling and

  18. Selected natural and fallout radionuclides in plant foods around the Kudankulam Nuclear Power Project, India.

    Science.gov (United States)

    Ross, E Mahiban; Raj, Y Lenin; Wesley, S Godwin; Rajan, M P

    2013-01-01

    The activity concentrations of certain radionuclides were quantified in some plant foods cultivated around Kudankulam, where a mega-nuclear power plant is being established. The activity concentrations were found more in the 'pulses' group and were the lowest in 'other vegetable' category. The annual effective dose was computed based on the activity concentration of radionuclides and it was found to be higher due to the consumption of cereals and pulses. Other vegetables, cereals, pulses and nuts recorded high transfer factors for the radionuclide (228)Ra. Fruits, leafy vegetables, tubers and roots, and palm embryo registered high transfer factors for (226)Ra. Group-wise activity concentration, radiation dose to the public and soil-plant-to-transfer factor are discussed in detail. Copyright © 2012 Elsevier Ltd. All rights reserved.

  19. Transfer of radionuclides to plants of natural ecosystems at the Semipalatinsk Test Site.

    Science.gov (United States)

    Larionova, N V; Lukashenko, S N; Kabdyrakova, A M; Kunduzbayeva, A Ye; Panitskiy, A V; Ivanova, A R

    2018-06-01

    A systematic study devoted to 137 Cs, 90 Sr, 241 Am, 239+240 Pu radionuclides in vegetation cover from several spots of the Semipalatinsk test site (STS) is summarised in this paper, highlighting the main findings obtained. The analysed spots are characterized by various types of radioactive contamination. Transfer factors (Tf) required for the quantitative description of the radionuclides transition from the soil to aboveground plant parts were determined, being found that, on average, the minimum Tf for all the radionuclides concerned were determined on the "Experimental Field" ground, followed by the determined ones in the "plumes" of radioactive fallout and in the conditionally "background" territories analysed. The highest transfer factors were characteristic of zones of radioactive streamflows and places of warfare radioactive agent (WRA) tests. On the other hand, ordering the radionuclide transferring factors in descending order, the following sequence was obtained: 90 Sr Tf > Cs Tf >  239+240 Pu Tf >  241 Am Tf, with the 90 Sr Tf, on the average, exceeding the 137 Cs Tf by 8 times and exceeding the 239+240 Pu Tf by up 16 times. 239+240 Pu Tf values were up to 3 times higher than the 241 Am Tf. The exception to the indicated radionuclide Tf descending order corresponded to places of WRA tests where Tf of radionuclides of interest by plants follows the sequence 90 Sr >  239+240 Pu >  137 Cs. Copyright © 2017 Elsevier Ltd. All rights reserved.

  20. Natural radionuclides in environmental media: a review of natural levels of radioactivity and background radiation levels and an assessment of factors affecting these levels

    International Nuclear Information System (INIS)

    Bradley, E.J.

    1993-01-01

    A review of the literature has been carried out to assemble the information available on the levels of naturally-occurring radionuclides in environmental media in the UK. Some data from other countries are included for comparison. The data are compiled on the basis of geographical origin into five main sectors: air; waters; vegetation; soils, rocks and sediments; and foodstuffs. A summary table is provided for each main section. (author)

  1. Influence of industry on pollution of the environment and human population with natural radionuclides and heavy metals

    International Nuclear Information System (INIS)

    Jaworowski, Z.

    1982-01-01

    The rate of fallout of 226 Ra depending on the distance from industrial emission sources has been evaluated. Contamination of soil with natural radionuclides in industrial and rural regions of Poland has been compared with the concentration of radionuclides in ash of aerophytic plants. An increase of airborne pollutants in precipitation in Southern Poland has been compared with an increase of the concentration of pollutants in pine trees. Samples of human bones from Southern Poland have been checked for contents of lead. It has been found that in 20th century concentration of lead decreased to a level not much higher than natural. The level of 226 Ra in Polish population had been decreasing during the last 100 years. This points to the conclusion that human skeleton is well protected as the level of radionuclides was not related to the level of environmental pollution. The concentration of 226 Ra in air is steadily increasing and an upward transport leads to its wide distribution. (E.G.M.)

  2. Soil-to-plant transfer factors of stable elements and naturally occurring radionuclides. (2) Rice collected in Japan

    International Nuclear Information System (INIS)

    Uchida, Shigeo; Tagami, Keiko; Hirai, Ikuko

    2007-01-01

    The critical paths of radionuclides and the critical foods in Japan are different from those in European and North American countries because agricultural products and food customs are different. Consequently, safety assessment in Japan is required to consider rice and vegetables as the critical foods. In this study, we measured soil-to-plant transfer factors (TFs) for rice using naturally existing elements as analogues of radionuclides under equilibrium conditions. Rice and associated soil samples were collected from 50 sampling sites throughout Japan and TFs of 36 and 34 elements for brown rice and white rice, respectively, were calculated on dry weight basis. Probability distributions of TFs of elements for brown rice and white rice were a log normal type. Except for As and Mo, the TFs for brown rice were usually lower than those for wheat and barley especially for K, Fe, Sr (t-test: p 90 Sr and 137 Cs observed in field experiments. Thus, the TFs of naturally existing elements can be used as TFs of those radionuclides which have been in contact with the environment for a long time and have reached equilibrium conditions. (author)

  3. Measurement of some water quality parameters related to natural radionuclides in aqueous environmental samples from former tin mining lake

    International Nuclear Information System (INIS)

    Zaini Hamzah; Masitah Alias; Ahmad Saat; Abdul Kadir Ishak

    2011-01-01

    The issue of water quality is a never ended issue and becoming more critical when considering the presence of natural radionuclides. Physical parameters and the levels of radionuclides may have some correlation and need further attention. In this study, the former tin mine lake in Kampong Gajah was chosen as a study area for its past historical background which might contribute to attenuation of the levels of natural radionuclides in water. The water samples were collected from different lakes using water sampler and some in-situ measurement were conducted to measure physical parameters as well as surface dose level. The water samples were analyzed for its gross alpha and gross beta activity concentrations using liquid scintillation counting and in-house cocktail method. Gross alpha and beta analyzed using in-house cocktail are in the range of 3.17 to 8.20 Bq/ L and 9.89 to 22.20 Bq/ L; 1.64 to 8.78 Bq/ L and 0.22 to 28.22 Bq/ L, respectively for preserved and un-preserved sample. The surface dose rate measured using survey meter is in the range of 0.07 to 0.21 μSv/ h and 0.07 to 0.2 μSv/ h for surface and 1 meter above the surface of the water, respectively. (Author)

  4. Soil-to-plant transfer factors of natural radionuclides (226Ra and 40K) in selected Thai medicinal plants.

    Science.gov (United States)

    Saenboonruang, Kiadtisak; Phonchanthuek, Endu; Prasandee, Kamonkhuan

    2018-04-01

    A soil-to-plant transfer factor (TF) is an important parameter that could be used to estimate radionuclides levels in medicinal plants. This work reports concentrations of natural radionuclides ( 226 Ra and 40 K) and TFs in six Thai medicinal plants grown in central Thailand using an HPGe gamma ray spectrometer. Either root, leaf, or flower parts of each medicinal plant were selected for use in the investigation according to their practical uses in traditional medicine. The results showed that due to K being essential in plants, 40 K had higher arithmetic means of activity concentrations and geometric means of TFs (geometric standard deviations in parentheses) of 610 ± 260 Bq kg -1 dry weight (DW) and 2.0 (1.4), respectively, than 226 Ra, which had the activity concentrations and TFs of 4.8 ± 2.6 Bq kg -1 DW and 0.17 (1.8), respectively. The results also showed that the leaves of medicinal plants had higher activity concentrations and TFs than root and flower parts, probably due to higher metabolic activities in leaves. Furthermore, there was good agreement between the results from the current work and other similar reports on medicinal plants. The information obtained from this work could strengthen knowledge of natural radionuclides in plants and particularly increase available TF data on Thai medicinal plants. Copyright © 2018 Elsevier Ltd. All rights reserved.

  5. Measurement of natural radionuclides in bricks and brick-making clays from Cuddalore district, Tamilnadu, India

    International Nuclear Information System (INIS)

    Viruthagirl, G.; Rajamanan, B.; Ravisankar, R.; Thilaivelavan, K.; Chandrasekaran, A.; Meenkshisundram, V.

    2010-01-01

    In India, bricks as building materials are mainly prepared by clay using the deposited sediments of rivers, and the radionuclide contents in bricks and brick-making clays should vary with origin and geological condition. In this paper, the radionuclide contents of these materials from river bank areas of Cuddalore district, Tamilnadu India are measured by gamma ray spectrometer using NaI (Tl) detector, and compared with those of other countries. The radiation hazard indices, which are evaluated by radium-equivalent (Raeq) activity, are lower than that of NEA-OECD. (authors)

  6. Ecological transfer of radionuclides and metals to free-living earthworm species in natural habitats rich in NORM

    Energy Technology Data Exchange (ETDEWEB)

    Mrdakovic Popic, Jelena, E-mail: jelena.mrdakovic.popic@umb.no; Salbu, Brit; Skipperud, Lindis

    2012-01-01

    Transfer of radionuclides ({sup 232}Th and {sup 238}U) and associated metals (As, Cd, Pb and Cr) from soil to free-living earthworm species was investigated in a thorium ({sup 232}Th) rich area in Norway. Sampling took place within former mining sites representing the technologically enhanced naturally occurring radioactive materials (TENORM), at undisturbed site with unique bedrock geology representing the naturally occurring radioactive materials (NORM) and at site outside the {sup 232}Th rich area taken as reference Background site. Soil analysis revealed the elevated levels of investigated elements at NORM and TENORM sites. Based on sequential extraction, uranium ({sup 238}U) and cadmium (Cd) were quite mobile, while the other elements were strongly associated with mineral components of soil. Four investigated earthworm species (Aporrectodea caliginosa, Aporrectodea rosea, Dendrodrilus rubidus and Lumbricus rubellus) showed large individual variability in the accumulation of radionuclides and metals. Differences in uptake by epigeic and endogeic species, as well as differences within same species from the NORM, TENORM and Background sites were also seen. Based on total concentrations in soil, the transfer factors (TF) were in ranges 0.03-0.08 and 0.09-0.25, for {sup 232}Th and {sup 238}U, respectively. TFs for lead (Pb), chromium (Cr) and arsenic (As) were low (less than 0.5), while TFs for Cd were higher (about 10). Using the ERICA tool, the estimated radiation exposure dose rate of the earthworms ranged from 2.2 to 3.9 {mu}Gy/h. The radiological risk for investigated earthworms was low (0.28). The obtained results demonstrated that free-living earthworm species can survive in soil containing elevated {sup 232}Th and {sup 238}U, as well As, Cd, Pb and Cr levels, although certain amount of radionuclides was accumulated within their bodies. The present investigation contributes to general better understanding of complex soil-to-biota transfer processes of

  7. Unsaturated zone waters from the Nopal I natural analog, Chihuahua, Mexico -- Implications for radionuclide mobility at Yucca Mountain

    Energy Technology Data Exchange (ETDEWEB)

    Pickett, D.A.; Murphy, W.M.

    1999-07-01

    Chemical and U-Th isotopic data on unsaturated zone waters from the Nopal I natural analog reveal effects of water-rock interaction and help constrain models of radionuclide release and transport at the site and, by analogy, at the proposed nuclear waste repository at Yucca Mountain. Geochemical reaction-path modeling indicates that, under oxidizing conditions, dissolution of uraninite (spent fuel analog) by these waters will lead to eventual schoepite precipitation regardless of initial silica concentration provided that groundwater is not continuously replenished. Thus, less soluble uranyl silicates may not dominate the initial alteration assemblage and keep dissolved U concentrations low. Uranium-series activity ratios are consistent with models of U transport at the site and display varying degrees of leaching versus recoil mobilization. Thorium concentrations may reflect the importance of colloidal transport of low-solubility radionuclides in the unsaturated zone.

  8. Unsaturated zone waters from the Nopal I natural analog, Chihuahua, Mexico -- Implications for radionuclide mobility at Yucca Mountain

    International Nuclear Information System (INIS)

    Pickett, D.A.; Murphy, W.M.

    1999-01-01

    Chemical and U-Th isotopic data on unsaturated zone waters from the Nopal I natural analog reveal effects of water-rock interaction and help constrain models of radionuclide release and transport at the site and, by analogy, at the proposed nuclear waste repository at Yucca Mountain. Geochemical reaction-path modeling indicates that, under oxidizing conditions, dissolution of uraninite (spent fuel analog) by these waters will lead to eventual schoepite precipitation regardless of initial silica concentration provided that groundwater is not continuously replenished. Thus, less soluble uranyl silicates may not dominate the initial alteration assemblage and keep dissolved U concentrations low. Uranium-series activity ratios are consistent with models of U transport at the site and display varying degrees of leaching versus recoil mobilization. Thorium concentrations may reflect the importance of colloidal transport of low-solubility radionuclides in the unsaturated zone

  9. Investigation of the environmental impacts of naturally occurring radionuclides in the processing of sulfide ores for gold using gamma spectrometry

    Energy Technology Data Exchange (ETDEWEB)

    Gbadago, J K; Darko, E O [Ghana Atomic Energy Commission, PO Box LG 80, Legon, Accra (Ghana); Faanhof, A [South African Nuclear Energy Corporation, PO Box 582, Pretoria 0001 (South Africa); Schandorf, C, E-mail: jgbada@yahoo.com [School of Nuclear and Allied Sciences, University of Ghana, Legon, Accra (Ghana)

    2011-09-01

    The possible environmental impacts of naturally occurring radionuclides on workers and a critical community, as a result of milling and processing sulfide ores for gold by a mining company at Bogoso in the western region of Ghana, have been investigated using gamma spectroscopy. Indicative doses for the workers during sulfide ore processing were calculated from the activity concentrations measured at both physical and chemical processing stages. The dose rate, annual effective dose equivalent, radium equivalent activity, external and internal hazard indices, and radioactivity level index for tailings, for the de-silted sediments of run-off from the vicinity of the tailings dam through the critical community, and for the soils of the critical community's basic schools were calculated and found to be lower than their respective permissible limits. The environmental impact of the radionuclides is therefore expected to be low in this mining environment.

  10. Investigation of the environmental impacts of naturally occurring radionuclides in the processing of sulfide ores for gold using gamma spectrometry

    International Nuclear Information System (INIS)

    Gbadago, J K; Darko, E O; Faanhof, A; Schandorf, C

    2011-01-01

    The possible environmental impacts of naturally occurring radionuclides on workers and a critical community, as a result of milling and processing sulfide ores for gold by a mining company at Bogoso in the western region of Ghana, have been investigated using gamma spectroscopy. Indicative doses for the workers during sulfide ore processing were calculated from the activity concentrations measured at both physical and chemical processing stages. The dose rate, annual effective dose equivalent, radium equivalent activity, external and internal hazard indices, and radioactivity level index for tailings, for the de-silted sediments of run-off from the vicinity of the tailings dam through the critical community, and for the soils of the critical community's basic schools were calculated and found to be lower than their respective permissible limits. The environmental impact of the radionuclides is therefore expected to be low in this mining environment.

  11. Statistical methods for determination of background levels for naturally occuring radionuclides in soil at a RCRA facility

    International Nuclear Information System (INIS)

    Guha, S.; Taylor, J.H.

    1996-01-01

    It is critical that summary statistics on background data, or background levels, be computed based on standardized and defensible statistical methods because background levels are frequently used in subsequent analyses and comparisons performed by separate analysts over time. The final background for naturally occurring radionuclide concentrations in soil at a RCRA facility, and the associated statistical methods used to estimate these concentrations, are presented. The primary objective is to describe, via a case study, the statistical methods used to estimate 95% upper tolerance limits (UTL) on radionuclide background soil data sets. A 95% UTL on background samples can be used as a screening level concentration in the absence of definitive soil cleanup criteria for naturally occurring radionuclides. The statistical methods are based exclusively on EPA guidance. This paper includes an introduction, a discussion of the analytical results for the radionuclides and a detailed description of the statistical analyses leading to the determination of 95% UTLs. Soil concentrations reported are based on validated data. Data sets are categorized as surficial soil; samples collected at depths from zero to one-half foot; and deep soil, samples collected from 3 to 5 feet. These data sets were tested for statistical outliers and underlying distributions were determined by using the chi-squared test for goodness-of-fit. UTLs for the data sets were then computed based on the percentage of non-detects and the appropriate best-fit distribution (lognormal, normal, or non-parametric). For data sets containing greater than approximately 50% nondetects, nonparametric UTLs were computed

  12. Natural radionuclides in grapes and wine of the Valley of Sao Francisco-PE, Brazil

    Energy Technology Data Exchange (ETDEWEB)

    Silveira, Patricia B.; Genezini, Frederico A.; Honorato, Eliane V.; Hazin, Clovis A.; Farias, Emerson E. [Centro Regional de Ciencias Nucleares do Nordeste (CRCN/CNEN-NE), Recife, PE (Brazil)]. E-mails: pbrandao@cnen.gov.br; fredzini@cnen.gov.br; valentim@cnen.gov.br; chazin@cnen.gov.br; emersonemiliano@yahoo.com.br; Belo, Michele T.; Lira, Marcia [Instituto de Tecnologia de Pernambuco ITEP-NE, Recife, PE (Brazil)]. E-mails: marcia@itep.br; michele@itep.br

    2007-07-01

    Wine is a widely consumed beverage around the world. Wine quality is influenced by many factors related to the specific production area: grape varieties, soil and climate, and vinicultural practices. Fruit contamination by radionuclides can result from various processes, mainly: direct deposition to fruit surfaces, absorption by the fruit skin and transport to the flesh, and deposition to soil, root uptake and transfer to fruit. For assessment studies the processes affecting the transfer of radioactivity from soil to fruits are often grouped into an aggregated parameter: the soil-to-fruit transfer factor (TF). It relates the radionuclide concentration in fruit to that in the soil. In this work, radionuclides were determined in musts and wines from three wine grape varieties: Castelao (red), Barbera (red) and Schomburguer (white), as well as in several materials in which their presence has direct or indirect influence on the final amount of these elements in wines, like soils where the vines were cultivated. Radionuclides were determined by using gamma-spectrometry with a high resolution detector (HPGe). (author)

  13. Natural radionuclides in grapes and wine of the Valley of Sao Francisco-PE, Brazil

    International Nuclear Information System (INIS)

    Silveira, Patricia B.; Genezini, Frederico A.; Honorato, Eliane V.; Hazin, Clovis A.; Farias, Emerson E.; fredzini@cnen.gov.br; valentim@cnen.gov.br; Belo, Michele T.; Lira, Marcia

    2007-01-01

    Wine is a widely consumed beverage around the world. Wine quality is influenced by many factors related to the specific production area: grape varieties, soil and climate, and vinicultural practices. Fruit contamination by radionuclides can result from various processes, mainly: direct deposition to fruit surfaces, absorption by the fruit skin and transport to the flesh, and deposition to soil, root uptake and transfer to fruit. For assessment studies the processes affecting the transfer of radioactivity from soil to fruits are often grouped into an aggregated parameter: the soil-to-fruit transfer factor (TF). It relates the radionuclide concentration in fruit to that in the soil. In this work, radionuclides were determined in musts and wines from three wine grape varieties: Castelao (red), Barbera (red) and Schomburguer (white), as well as in several materials in which their presence has direct or indirect influence on the final amount of these elements in wines, like soils where the vines were cultivated. Radionuclides were determined by using gamma-spectrometry with a high resolution detector (HPGe). (author)

  14. Selected natural and fallout radionuclides in plant foods around the Kudankulam Nuclear Power Project, India

    International Nuclear Information System (INIS)

    Ross, E. Mahiban; Raj, Y. Lenin; Wesley, S. Godwin; Rajan, M.P.

    2013-01-01

    The activity concentrations of certain radionuclides were quantified in some plant foods cultivated around Kudankulam, where a mega-nuclear power plant is being established. The activity concentrations were found more in the ‘pulses’ group and were the lowest in ‘other vegetable’ category. The annual effective dose was computed based on the activity concentration of radionuclides and it was found to be higher due to the consumption of cereals and pulses. Other vegetables, cereals, pulses and nuts recorded high transfer factors for the radionuclide 228 Ra. Fruits, leafy vegetables, tubers and roots, and palm embryo registered high transfer factors for 226 Ra. Group-wise activity concentration, radiation dose to the public and soil-plant-to-transfer factor are discussed in detail. Highlights: ► Fallout radionuclides ( 90 Sr and 137 Cs) were below the limit of detection. ► 228 Ra activities were higher than 226 Ra activity concentrations. ► ‘Pulses’ group (leguminous grains) was the highest accumulator of radium nuclides. ► 228 Ra transfer factor was higher in few groups while 226 Ra was higher in others.

  15. Species diversity of plant communities from territories with natural origin radionuclides contamination

    Energy Technology Data Exchange (ETDEWEB)

    Kaneva, A.V.; Belykh, E.S.; Maystrenko, T.A.; Grusdev, B.I.; Zainullin, V.G.; Vakhrusheva, O.M. [Institute of Biology, Komi Scientific Center, Ural Division of RAS, Syktyvkar, 167982 (Russian Federation); Oughton, D. [Norwegian University of Life Sciences, P.O. Box 5003, NO-1432 Aas (Norway)

    2014-07-01

    Since plants dominate every landscape, the impact of any environmental stressor on plants can directly affect the structure and function of an ecosystem, resulting in decreased primary productivity and degradation of wildlife habitat. The investigation goal of the present research was to study how vascular plant species' composition at a former radium mining site could be related to i) soil contamination with heavy metals and uranium and thorium decay chain radionuclides and ii) soil agrochemical properties. Between the 1930's and 1950's, the commercial extraction of radium, storage of the uranium mill tailings and radium production wastes, together with deactivation of the site with a mixture of sand and gravel completely destroyed plant communities in the vicinity of Vodny settlement (Komi Republic, Russia). The plant cover recovery started more than 60 years ago, and resulted in overgrowing with common grassland plant species. Three meadow sites were investigated, one with low contamination (on the territory of former radium production plant), one with high contamination (waste storage cell) and a reference sites out of the radiochemical plant zone of influence, but with similar natural conditions. Geo-botanical descriptions revealed 134 vascular plant species from 34 families in the meadow communities studied. The greatest richness was seen for Poaceae, Asteraceae, Rosaceae and Fabaceae families; others had 1-5 species. The highest richness in diversity was seen at reference sites with 95 vascular plant species. 87 species were registered on low contaminated sites and 75 species on high contaminated. Perennial herbs were the dominant life form on all the studied meadow communities. Arboreal species expansion in vegetation was noted at both experimental and reference sites. Shannon index calculations indicated a significant (p<0.05) decrease in species diversity on sample areas of the highly contaminated radioactive waste storage cell. Mean values

  16. Combined Natural Convection and Radiation Heat Transfer of Various Absorbing-Emitting-Scattering Media in a Square Cavity

    Directory of Open Access Journals (Sweden)

    Xianglong Liu

    2014-01-01

    Full Text Available A numerical model is developed to simulate combined natural convection and radiation heat transfer of various anisotropic absorbing-emitting-scattering media in a 2D square cavity based on the discrete ordinate (DO method and Boussinesq assumption. The effects of Rayleigh number, optical thickness, scattering ratio, scattering phase function, and aspect ratio of square cavity on the behaviors of heat transfer are studied. The results show that the heat transfer of absorbing-emitting-scattering media is the combined results of radiation and natural convection, which depends on the physical properties and the aspect ratio of the cavity. When the natural convection becomes significant, the convection heat transfer is enhanced, and the distributions of NuR and Nuc along the walls are obviously distorted. As the optical thickness increases, NuR along the hot wall decreases. As the scattering ratio decreases, the NuR along the walls decreases. At the higher aspect ratio, the more intensive thermal radiation and natural convection are formed, which increase the radiation and convection heat fluxes. This paper provides the theoretical research for the optimal thermal design and practical operation of the high temperature industrial equipments.

  17. Doses rate in contact with plastic syringes of 1, 2 and 5 mL for different beta and gamma emitting radionuclides

    International Nuclear Information System (INIS)

    Torres Berdeguez, Mirta; Ayra Pardo, Enrique; Falcon, Lazaro

    2008-01-01

    The objective of this paper is to calculate the dose rate in contact with plastic syringes of 1, 2 and 5 m L volume, unshielded and the dose rate in the same syringes after a lead or a Lucite shield of various thickness has been installed, depending on the emission of the radionuclide used. The radionuclides involved in the assessment were 32 P, 51 Cr, 90 Y, 99m Tc, 125 I, 131 I, 153 Sm, 186 Re, 188 Re, 169 Er and 177 Lu. The code used was the MCNP4C. The results are intended to be used by a Radiation Protection Officer wherever the radionuclides in question are handled to rapidly assess the dose in hands of the operators. (author)

  18. Health effects models for nuclear power plant accident consequence analysis. Modification of models resulting from addition of effects of exposure to alpha-emitting radionuclides: Revision 1, Part 2, Scientific bases for health effects models, Addendum 2

    Energy Technology Data Exchange (ETDEWEB)

    Abrahamson, S. [Wisconsin Univ., Madison, WI (United States); Bender, M.A. [Brookhaven National Lab., Upton, NY (United States); Boecker, B.B.; Scott, B.R. [Lovelace Biomedical and Environmental Research Inst., Albuquerque, NM (United States). Inhalation Toxicology Research Inst.; Gilbert, E.S. [Pacific Northwest Lab., Richland, WA (United States)

    1993-05-01

    The Nuclear Regulatory Commission (NRC) has sponsored several studies to identify and quantify, through the use of models, the potential health effects of accidental releases of radionuclides from nuclear power plants. The Reactor Safety Study provided the basis for most of the earlier estimates related to these health effects. Subsequent efforts by NRC-supported groups resulted in improved health effects models that were published in the report entitled {open_quotes}Health Effects Models for Nuclear Power Plant Consequence Analysis{close_quotes}, NUREG/CR-4214, 1985 and revised further in the 1989 report NUREG/CR-4214, Rev. 1, Part 2. The health effects models presented in the 1989 NUREG/CR-4214 report were developed for exposure to low-linear energy transfer (LET) (beta and gamma) radiation based on the best scientific information available at that time. Since the 1989 report was published, two addenda to that report have been prepared to (1) incorporate other scientific information related to low-LET health effects models and (2) extend the models to consider the possible health consequences of the addition of alpha-emitting radionuclides to the exposure source term. The first addendum report, entitled {open_quotes}Health Effects Models for Nuclear Power Plant Accident Consequence Analysis, Modifications of Models Resulting from Recent Reports on Health Effects of Ionizing Radiation, Low LET Radiation, Part 2: Scientific Bases for Health Effects Models,{close_quotes} was published in 1991 as NUREG/CR-4214, Rev. 1, Part 2, Addendum 1. This second addendum addresses the possibility that some fraction of the accident source term from an operating nuclear power plant comprises alpha-emitting radionuclides. Consideration of chronic high-LET exposure from alpha radiation as well as acute and chronic exposure to low-LET beta and gamma radiations is a reasonable extension of the health effects model.

  19. Spatial distribution of radionuclides in soil around a coal-fired power plant: lead 210, polonium 210, radium 226, thorium 232, kalium 40 emitted with the fly ash and cesium 137 from the worldwide weapon testing fallout

    Energy Technology Data Exchange (ETDEWEB)

    Bunzl, K.; Hoetzl, H.; Rosner, G.; Winkler, R.

    1984-09-01

    To determine the effect of airborne emissions of radionuclides from coal-fired power plants on the environment, the concentrations of the most important radionuclides were measured in soil samples from the local environments (0.4-5.2 km) as well as in fly ash. The spatial distribution of the radionuclides in the soil did not indicate any significantly increased concentrations in the area downwind of the plant compared to other areas; the ratios lead 210/radium 226 and polonium 210/radium 226 were within the range observed for unaffected soils. The emissions from the plant, though present, are obviously too small to significantly change the natural local distribution pattern of the radionuclides in the soil. A highly significant correlation between potassium 40 and thorium 232 was observed which was independent of the different types of soils found in this area. The concentration of cesium 137 in topsoil, which is the result of worldwide fallout from nuclear weapons testing, varied at some places even within a small distance (approx. 2 km) by up to one order of magnitude. Furthermore, it was observed that the concentration of cesium 137 in soils from cropland was on average a factor of 2 less than in those from grassland. This variability has to be considered in planning monitoring programs around nuclear power plants, which may also release this radionuclide. (A.V.)

  20. Assessment of the doses due to natural radionuclide in the green leafy vegetables of Domiasiat, Meghalaya India

    International Nuclear Information System (INIS)

    Kumar, N.; Chaturvedi, S.S.; Jha, S.K.

    2011-01-01

    A radiation dose assessment exercise was carried out for the Ipomea batata, Allium sativum, Dacaus carota, and Solanum tuberosum due to naturally available radionuclide 40 K, 238 U and 232 Th in the Domiasiat area of Meghalaya. The concentration of radionuclides in biota as well as corresponding soil was measured by precipitation method using NaI detector for continuous 12 months. Transfer factor was calculated and was, for 40 K(3.96E-05, 3.40E-05, 3.40E-05, 2.70E-05), for 232 Th(3.94E-05, 3.20E-05, 3.20E-054.93E-05), for 238 U(3.60E-05, 3.89E-05, 3.85E-054.57E-05), respectively in each biota due to each radionuclide. The point source dose distribution (source ↔ target) hypotheses was applied for the consideration of absorbed fraction. The generated data were modeled using the FASSET method and obtained dose was 8.42E-03, 8.36E-03, 7.78E-03, 7.74E-03 μGy h -1 , respectively and finally compared with the IAEA and UNSCEAR dataset for screening level dose for terrestrial biota. (author)

  1. Distribution of natural radionuclides and uranium activity ratio in Gulf of Thailand sediments as base line data

    Energy Technology Data Exchange (ETDEWEB)

    Sahoo, S.K.; Hideki, A. [National Institute of Radiological Sciences (Japan); Kritsananuwat, R.; Fukushi, M. [Tokyo Metropolitan University (Japan); Chanyotha, S.; Pangza, K. [Chulalongkorn University (Thailand)

    2014-07-01

    This paper reports distribution of naturally occurring radionuclides and uranium activity ratio in marine sediments from selected coast, along the Gulf of Thailand to establish baseline data. Thailand has a plan to construct nuclear power plants (NPPs) as well as coal-fired thermal power plants to generate adequate and reliable electricity supply for rapid growth of industrialization. Therefore, it is important to focus not only on security and adequacy of power system but also on environmental protection and monitoring and risk assessment. To carry out environmental monitoring, baseline data plays a significant role. These data should be established and available before set up of mega projects that could impact the environment and health. Therefore, we have collected samples from five areas in the Gulf of Thailand, which are proposed as potential sites, to set up power plants by Thailand government. A total number of fifty-four marine sediment samples were collected. Gamma spectroscopy was used to determine the concentration of natural radionuclides e.g. {sup 226}Ra, {sup 228}Ac and {sup 40}K. Activity concentrations of {sup 226}Ra, {sup 228}Ac and {sup 40}K vary from 2.91-67.17 Bq/kg with an average of 26.64±14.57 Bq/kg, 4.42-109.17 Bq/kg with an average of 43.79±23.92 Bq/kg and 3.36-1004.56 Bq/kg with an average of 393.56±208.04 Bq/kg, respectively. The radiation hazard parameters including absorbed dose rate (D), annual effective dose equivalent (AEDE), radium equivalent activity (AGDE) and external hazard index (Hex) were calculated and compared with the international recommended values. We have noticed that sediments from two sites characterized by similar geological nature of landforms with a rocky coast have higher concentration of natural radionuclides. Concentration of uranium was determined using the inductively coupled plasma mass spectrometry (ICP-MS) and isotopic composition of {sup 234}U/{sup 238}U and {sup 235}U/{sup 238}U were determined using

  2. The cleaning of the soils polluted by oil and radionuclides by natural sorbents

    International Nuclear Information System (INIS)

    Farajov, M.F.; Shamilov, E.N.; Abdullayev, A.S.; Huseynov, V.I.

    2005-01-01

    Full text : Problem of environmental pollution in oil extracting areas of Absheron peninsula became the very important discussion object lately. It this areas for many years oil and well waters were flowed to environmental areas caused a lot of pools in that areas and at the result the soil and plants were polluted with oil and radionuclides. By last years researches it was revealed that amount of radium 226 oil well water contains 10 - 500 Bq/l. Sometimes amount of radium 226 in polluted soils is increasing to 2000--5000 Bq/l and at the result it is raising probability of entering radionuclides by the way of migration from ground to plants into the nutrition chain cycle. Thus the polluted areas with oil and radionuclides and also when oil spills from oil-pipes by an accident the deactivation of soils is one of the main and most actual problems. In researches for cleaning of polluted soils with radionuclides for the first time were used the phyto sorbent modified breccias forms taken from Chaildag, Gobu, and Lokbatan mud volcano areas. The mineral contain of volcano mud generally consists of clay rocks -(kaolinit, montmorillonit, zeolite, chlorite, biotit) pyrite, and i.e.[2]. The polluted soil samples were taken in Surakhani region from area with the 150 mikroroentgen per hour radiation background. The contain and amount of radionuclides were determined with the radio spectrometer P rogress - Beta - Gamma . Polluted soil samples firstly are washed by hot water and HCl solution by mixing for 3-5 hours. At the next level by adding pieced sorbent into the solution is intensively mixing by mixer and putting for sedimentation for 24 hours. After sedimentation the stiring process is repeated by adding HCl on the sediment again. The soil is stirred by water for last time. Decomposed solutions from soil are adhering and are maked with sorbent again. Thus the soil is quite cleaned from oil and radionuclides by the sorbents we offer. At the same time this sorbents may be

  3. Mobility of radionuclides and trace elements in soil from legacy NORM and undisturbed naturally 232Th-rich sites.

    Science.gov (United States)

    Mrdakovic Popic, Jelena; Meland, Sondre; Salbu, Brit; Skipperud, Lindis

    2014-05-01

    Investigation of radionuclides (232Th and 238U) and trace elements (Cr, As and Pb) in soil from two legacy NORM (former mining sites) and one undisturbed naturally 232Th-rich site was conducted as a part of the ongoing environmental impact assessment in the Fen Complex area (Norway). The major objectives were to determine the radionuclide and trace element distribution and mobility in soils as well as to analyze possible differences between legacy NORM and surrounding undisturbed naturally 232Th-rich soils. Inhomogeneous soil distribution of radionuclides and trace elements was observed for each of the investigated sites. The concentration of 232Th was high (up to 1685 mg kg(-1), i.e., ∼7000 Bq kg(-1)) and exceeded the screening value for the radioactive waste material in Norway (1 Bq g(-1)). Based on the sequential extraction results, the majority of 232Th and trace elements were rather inert, irreversibly bound to soil. Uranium was found to be potentially more mobile, as it was associated with pH-sensitive soil phases, redox-sensitive amorphous soil phases and soil organic compounds. Comparison of the sequential extraction datasets from the three investigated sites revealed increased mobility of all analyzed elements at the legacy NORM sites in comparison with the undisturbed 232Th-rich site. Similarly, the distribution coefficients Kd (232Th) and Kd (238U) suggested elevated dissolution, mobility and transportation at the legacy NORM sites, especially at the decommissioned Nb-mining site (346 and 100 L kg(-1) for 232Th and 238U, respectively), while the higher sorption of radionuclides was demonstrated at the undisturbed 232Th-rich site (10,672 and 506 L kg(-1) for 232Th and 238U, respectively). In general, although the concentration ranges of radionuclides and trace elements were similarly wide both at the legacy NORM and at the undisturbed 232Th-rich sites, the results of soil sequential extractions together with Kd values supported the expected differences

  4. Effects of radionuclides on non-human biota and natural ecosystem

    International Nuclear Information System (INIS)

    Garnier-Laplace, J.; Adam, C.; Gilbin, R.; Denison, F.; Fortin, C.; Simon, O.

    2004-01-01

    The need for a system of radiological protection of the environment drives regulators to urge scientists on conceptualisation of methods to demonstrate that the environment is protected against radioactive contaminants. One of the major difficulties in the implementation of ecological risk assessment for radioactive pollutants is the lack of data for wildlife chronic internal exposure to alpha or beta emitters. Situations of such chronic internal exposure at low levels are likely to cause toxic responses distinct from those observed after acute exposure at high doses because of the bioaccumulation phenomena. Biochemical mechanisms can lead to a gradual accumulation of elements present at trace level in the external medium, inducing a highly localised deposit within tissues or cells. These highly localised accumulations of radionuclides, coupling radiological and chemical toxicities, particularly for heavy elements such as actinides, may give rise to particular biological responses of a cell group, capable of causing functional or structural abnormalities at higher hierarchical levels. The assessment of these bioaccumulation phenomena investigated within the ENVIRHOM programme launched two years ago at the Institute for Radioprotection and Nuclear Safety, is primordial with regard to internal exposure to radionuclides since they increase locally both the radionuclide concentration and the biological effect of the delivered dose. Gaps of knowledge within this field constitute a strong limitation to our capability to make a reasonable risk estimate. Internal doses cannot be accurately calculated and potentially associated biological effects at any organization level remain fairly unknown. As a result, derivation of ecologically relevant and knowledge-based predicted no-effect concentrations becomes a critical issue in ERA. The scope of this paper is to illustrate the relevance of the development of a greater depth of understanding of radionuclide fate and biological

  5. Applications of neutron activation analysis in determination of natural and man-made radionuclides

    International Nuclear Information System (INIS)

    Byrne, A. R.; Benedik, L.

    1998-01-01

    Neutron activation analysis (NAA), being essentially an isotopic and not an elemental method of analysis, is capable of determining a number of important radionuclides of radioecological interest with good precision and accuracy, by transformation into another, more easily quantifiable radionuclide. The nuclear characteristics which favour this technique may be summarized in an advantage factor relative to radiometric analysis of the original radioanalyte. Well known or hardly known examples include 235 U, 238 U, 232 Th, 230 Th, 129 I, 99 Tc, 237 Np and 231 Pa; a number of these are discussed and illustrated in analysis of real samples of environmental and biological origin. The advantages and drawbacks of this technique relative to conventional radiometric analysis and newer, mass spectrometric methods is also discussed. The value of NAA as an independent method in certification of radionuclide reference materials (where much remains to be done) is stressed. Where direct sample analysis is possible, NAA retains the important advantage of being essentially blank-free. Where pre-separation of the analyte is necessary, some suggestions for improving the reliability of pre-separation yields using internal, activable tracers are proposed. The use of NAA to allow 238 U and 232 Th to be used as endogenous (internal) radiotracers in alpha spectrometric analyses of uranium and thorium radioisotopes in radioecological studies is described, also allowing independent data sets to be obtained, of great value in quality control. (author)

  6. Natural Radionuclides in Slag/Ash Pile from Coal-Fired Power Plant Plomin

    International Nuclear Information System (INIS)

    Barisic, D.; Lulic, S.; Marovic, G.; Sencar, J.

    2001-01-01

    Full text: The coal slag/ash pile contains about one million tons of different (bottom ash, filter ash, gypsum) waste material deposited in vicinity of Plomin coal-fired power plant. Activities of 40 K, 228 Ra, 226 Ra and 238 U in materials deposited on slag/ash pile as well as in used coals were occasionally measured during past more than two and half decades of Plomin coal-fired plant operation. The radionuclides content in deposited bottom and filter ash material are related with radionuclide activities and mineral matter fraction in coals used. Up to the middle of nineties, the majority of coal used was anthracite from Istrian local mines. In that period, deposited waste material was characterised with relatively high 226 Ra and 238 U activities while potassium and thorium content was very low. When Istrian coal has been completely substituted with imported coal, uranium series radionuclide concentrations in deposited waste materials decreased significantly. Meanwhile, potassium and thorium activities in slag/ash pile material increased. It seems that slag/ash pile material generated in the last several years of Plomin coal-fired power plant operation could be generally used in cement industry without any special restriction. (author)

  7. The natural course of radionuclide bone scanning in the evaluation of total knee replacement--a 2 year prospective study

    DEFF Research Database (Denmark)

    Duus, B R; Boeckstyns, M; Stadeager, Carsten Preben

    1990-01-01

    In order to establish the natural course of radionuclide bone scanning images after total knee replacement 41 consecutive patients were scheduled for examination 3, 7, 12 and 24 months after surgery. The mean age was 69 years (range 50-80 years); the female:male ratio was 4:1. Thirty-two patients...... completed the entire program. A total of 143 99Tcm medronic acid complex scintigrams was performed. No significant difference between the grades of total scintigraphic uptake at any of the four examinations nor any difference between the first and the last examinations could be demonstrated (P = 0...

  8. Immune reactions of northern population under the effect of chronic irradiation by incorporated radionuclides of different nature

    International Nuclear Information System (INIS)

    Shubin, V.M.; Litver, B.Ya.; Troitskaya, M.N.

    1978-01-01

    Immunologic indices are studied among the indigenous population of the Far North and among temporary and permanent inhabitants of Leningrad in an attempt to identify the role of radiation from incorporated radionuclides entering the body along the ecologic chain. A number of alterations in immunologic reactivity have been found among reindeer breeders, for example some reductions in most of the studied factors of nonspecific humoral protection. These alterations have been of a compensatory nature and suggest that adaptation mechanisms are disturbed. The alterations are thought to result from the action of a number of unfavorable environmental factors. The contribution of the radiation factor is still uncertain

  9. Natural radionuclides near a coal-fired power station. [/sup 210/Po and /sup 210/Pb levels in cattle livers

    Energy Technology Data Exchange (ETDEWEB)

    Smith-Briggs, J L; Crick, M J [National Radiological Protection Board, Harwell (UK)

    1982-11-01

    Previous measurements have shown enhanced levels of /sup 210/Po and /sup 210/Pb from fly ash deposited in the environment around old coal-fired power stations. Preliminary results are presented for levels of /sup 210/Po and /sup 210/Pb in liver samples from cattle which had grazed for two to three years in a field adjacent to a modern power station. No significant difference in the levels of these natural radionuclides was found compared to liver samples obtained from cattle in a control area.

  10. Investigation of natural radionuclides in foods and waters in China and evaluation of internal dose to public

    Energy Technology Data Exchange (ETDEWEB)

    Changshou, Zhu; Yulan, Liu; Ning, Xu; Aiying, Hu; Tiluo, Kou; Zhongxin, Shi [Laboratory of Industrial Hygiene, Ministry of Public Health (China); and others

    1992-12-01

    In order to obtain background radiation levels of natural radionuclides in foods and waters in China, the determination and analysis of water and food samples have been completed by organizations of radiological protection from 28 provinces, autonomous regions and three major cities. Ranges of specific activity of natural radionuclides for U, Th, Ra, K, Pb and Po are (2.2 {approx} 25.5) x 10 {sup -2} Bq/kg, (0.5 {approx} 6.9) x 10{sup -2} Bq/kg, (3.4 {approx} 25.5) x 10 {sup -2} Bq/kg, (25 {approx} 420) x 10{sup -2} Bq/kg, (3.9 {approx} 55) x 10{sup -2} Bq/kg and (2.7 {approx} 58) x 10{sup -2} Bq/kg, respectively. Samples of drinking water were taken from tap water or well. The average concentrations in tap water and well water are 2.8 x 10{sup -2} Bq/L and 3.7 x 10{sup -2} Bq/L for U, 0.8 x 10{sup -2} Bq/L and 1.3 x 10{sup -2} Bq/L for Ra, 0.07 x 10{sup -2} Bq/L and 0.06 x 10{sup -2} Bq/L for Th, 0. 3 x 10{sup -2} Bq/L and 1.1 x 10{sup -2} Bq/L for Pb and 0.3 Bq/L and 0.5 Bq/L for Po respectively. The annual intakes by ingestion have been calculated. The annual intake of male adult from six main natural radionuclides is about 205 Bq. Among them 64% of total intake of U is from drinking water. The contributions from grains to the total intake of Ra, Pb and Po are 55.7%, 59.7% and 70% respectively. The total annual average effective dose equivalent of 6 natural radionuclides for male adult in China is about 310 {mu}Sv.

  11. Use of natural analogues to support radionuclide transport models for deep geological repositories for long lived radioactive wastes

    International Nuclear Information System (INIS)

    1999-10-01

    Plans to dispose high level and long lived radioactive wastes in deep geological repositories have raised a number of unique problems, mainly due to the very long time-scales which have to be considered. An important way to help to evaluate performance and provide confidence in the assessment of safety in the long term is to carry out natural analogue studies. Natural analogues can be regarded as long term natural experiments the results or outcome of which can be observed, but which, by definition, are uncontrolled by humans. Studies of natural analogues have been carried out for more than two decades, although the application of information from them is only relatively recently becoming scientifically well ordered. This report is part of a the IAEA's programme on radioactive waste management dealing with disposal system technology for high level and long lived radioactive waste. It presents the current status of natural analogue information in evaluating models for radionuclide transport by groundwater. In particular, emphasis is given to the most useful aspects of quantitative applications for model development and testing (geochemistry and coupled transport models). The report provides an overview of various natural analogues as reference for those planning to develop a research programme in this field. Recommendations are given on the use of natural analogues to engender confidence in the safety of disposal systems. This report is a follow up of Technical Reports Series No. 304 on Natural Analogues in Performance Assessments for the Disposal of Long Lived Radioactive Waste (1989)

  12. The detailed analysis of natural radionuclides dissolved in spa waters of the Kłodzko Valley, Sudety Mountains, Poland

    International Nuclear Information System (INIS)

    Walencik-Łata, A.; Kozłowska, B.; Dorda, J.; Przylibski, T.A.

    2016-01-01

    A survey was conducted to measure natural radioactivity in spa waters from the Kłodzko Valley. The main goal of this study was to determine the activity concentration of uranium, radium and radon isotopes in the investigated groundwaters. Samples were collected several times from 35 water intakes from 5 spas and 2 mineral water bottling plants. The authors examined whether the increased gamma radiation background, as well as the elevated values of radium and uranium content in reservoir rocks, have a significant impact on the natural radioactivity of these waters. The second objective of this research was to provide information about geochemistry of U, Ra, Rn radionuclides and the radiological and chemical risks incurred by ingestion of isotopes with drinking water. On the basis of results obtained, it is feasible to assess the health hazard posed by ingestion of natural radioactivity with drinking waters. Moreover, the data yielded by this research may be helpful in the process of verification of the application of these waters in balneotherapy. In addition, annual effective radiation doses resulting from the isotopes consumption were calculated on the basis of the evaluated activity concentrations. In dose assessment for uranium and radium isotopes, the authors provided values for different human age groups. The obtained uranium content in the investigated waters was compared with the currently valid regulations concerning the quality of drinking water. Based on the activity concentrations data, the activity isotopic ratios 234 U/ 238 U, 226 Ra/ 238 U, 222 Rn/ 238 U, 222 Rn/ 226 Ra and the correlations between radionuclides content were then examined. In brief, it may be concluded on the basis of the obtained results that radon solubility is inversely proportional to radium and uranium dissolution in environmental water circulation. The presented study allows conclusions to be drawn on the radionuclide circulation among different environmental biota: from

  13. The detailed analysis of natural radionuclides dissolved in spa waters of the Kłodzko Valley, Sudety Mountains, Poland

    Energy Technology Data Exchange (ETDEWEB)

    Walencik-Łata, A., E-mail: agata.walencik@us.edu.pl [University of Silesia, Institute of Physics, Department of Nuclear Physics and Its Applications, Uniwersytecka 4 St., 40-007 Katowice (Poland); Kozłowska, B.; Dorda, J. [University of Silesia, Institute of Physics, Department of Nuclear Physics and Its Applications, Uniwersytecka 4 St., 40-007 Katowice (Poland); Przylibski, T.A. [Wrocław University of Technology, Faculty of Geoengineering, Mining and Geology, Division of Geology and Mineral Waters, Wybrzeże S. Wyspiańskiego 27, 50-370 Wrocław (Poland)

    2016-11-01

    A survey was conducted to measure natural radioactivity in spa waters from the Kłodzko Valley. The main goal of this study was to determine the activity concentration of uranium, radium and radon isotopes in the investigated groundwaters. Samples were collected several times from 35 water intakes from 5 spas and 2 mineral water bottling plants. The authors examined whether the increased gamma radiation background, as well as the elevated values of radium and uranium content in reservoir rocks, have a significant impact on the natural radioactivity of these waters. The second objective of this research was to provide information about geochemistry of U, Ra, Rn radionuclides and the radiological and chemical risks incurred by ingestion of isotopes with drinking water. On the basis of results obtained, it is feasible to assess the health hazard posed by ingestion of natural radioactivity with drinking waters. Moreover, the data yielded by this research may be helpful in the process of verification of the application of these waters in balneotherapy. In addition, annual effective radiation doses resulting from the isotopes consumption were calculated on the basis of the evaluated activity concentrations. In dose assessment for uranium and radium isotopes, the authors provided values for different human age groups. The obtained uranium content in the investigated waters was compared with the currently valid regulations concerning the quality of drinking water. Based on the activity concentrations data, the activity isotopic ratios {sup 234}U/{sup 238}U, {sup 226}Ra/{sup 238}U, {sup 222}Rn/{sup 238}U, {sup 222}Rn/{sup 226}Ra and the correlations between radionuclides content were then examined. In brief, it may be concluded on the basis of the obtained results that radon solubility is inversely proportional to radium and uranium dissolution in environmental water circulation. The presented study allows conclusions to be drawn on the radionuclide circulation among

  14. Examinations on the removal of natural radionuclides from drinking water and overview on their distribution in Austria

    International Nuclear Information System (INIS)

    Staubmann, K.

    2002-09-01

    The objective of the thesis was to give an overview about available data regarding natural radioactivity in Austrian ground and spring water and to examine the capability of membrane processes, ion exchange processes and processes for iron and manganese removal to remove natural radionuclides from drinking water. There are already Austrian-wide data existing for the activity concentrations of radon-222 in ground- and spring water, only few values are available for radium-226 (Ra-226), lead-210 (Pb-210), uranium (U) and polonium-210 up til now. From the existing data it is to be expected that in Austria only in exceptions water treatment will be necessary. The tested reverse osmosis and nanofiltration systems removed between 95.6 % and 99.8 % of Ra-226, U and Pb-210 on the average. Laboratory scale experiments for ion exchange showed an essential influence of the concurrent ions in the water on the removal of the radionuclides. With water softeners (cation exchangers) Ra-226 to more than 90 % and Pb to more than 80 % could be removed. By the use of other ones than the standard cartridge fillings for pour-through-filters (ion exchangers) the radionuclides could be removed more selectively and more effectively and the influence on the chemical composition of the water could be minimized. In a laboratory scale experiment simulating the planned treatment process at a waterwork for the removal of iron and manganese Ra-226 was removed to 61%. At the examined processes often disadvantageous side effects onto the water quality which require a subsequent treatment were observed. During the operation of the systems it should be aimed at keeping the activity in the produced waste low so that no radiation protection relevant risk starts from that. (author)

  15. Fluctuation contents of phosphorus and natural radionuclide in the water column of the Mersing river, Johor, Malaysia

    International Nuclear Information System (INIS)

    Saili, Noor Affizah Bujang; Mohamed, Che Abd Rahim

    2013-01-01

    Studies on natural radionuclides such as 210 Po and 210 Pb with the concentration of phosphorus in water column related to suspended particulate matter (SPM) were carried out at the Mersing River, Johor, Malaysia. Sixteen water samples were collected from nine stations on the 4 th July 2010. 210 Po and 210 Pb activities varied between 0.76 to 2.24 mBq/L and 0.16 to 1.60 mBq/L respectively. The phosphorus concentrations, comprising total dissolved phosphorus (TDP), soluble reactive phosphorus (SRP) and dissolved organic phosphorus (DOP), were within the ranges of 6.06 to 23.31 μg/L, 2.24 to 13.42 μg/L and 0.47 to 16.10 μ/L, respectively. The concentration of TDP and salinity shows weak positive correlation (r = 0.39), perhaps due to the shallow depth of the Mersing River. There is a high positive correlation (r = 0.85) of 210 Po activity with SPM concentration and a moderately positive correlation (r =0.59) of 210 Po and TDP in water. The K d values in suspended particulate matter are much higher compare to that in dissolved phase, proving that the adsorption of radionuclides to particles is more dominant. This implies that SPM significantly influences the variation of the P compound and both radionuclides in the Mersing River. This corresponds with agricultural activities from palm oil estates; erosion of the river bank due to river runoff; advection of suspended particulates from surface sediment due to boat and ferry traffic at the jetties; sedimentation; domestic sewage from nearby terrestrial areas; and natural processes; all of which might have resulted in their introduction to the Mersing River. (author)

  16. Gamma emitting radionuclides in fruits and vegetables produced in the Canary Islands: domestic consequences; Radionuclidos emisores gamma en frutas y hortalizas producidas en Canarias: consecuencias dosimetricas

    Energy Technology Data Exchange (ETDEWEB)

    Triguero-Perez, M.; Duarte-Rodriguez, X.; Lopez-Perez, M.; Hernandez-Armas, J.

    2011-07-01

    Determine the possible effects due to ingestion of radionuclides that can be found in health food is of interest from the viewpoint of radiation protection of the population. these determinations and analysis of the consequences on the health of people and jobs has led to studies that have had consequences in the form of rules to follow and values have to be attended to limit dictated by national and international agencies. (Author)

  17. Natural and artificial radionuclides in selected Styrian soils and plants before and after the reactor accident in Chernobyl

    Energy Technology Data Exchange (ETDEWEB)

    Heinrich, G; Gries, A [Graz Univ. (Austria); Mueller, H J; Oswald, K [Technische Univ., Graz (Austria). Inst. fuer Theoretische Physik und Reaktorphysik

    1989-01-01

    This paper reports on natural radioactivity due to the uptake of {sup 40}K and the radionuclides of the {sup 238}U and {sup 232}Th series. Selected examples show the concentrations of radionuclides in soils, lower and higher plants before and after the Chernobyl accident. The changes in the amount of radioactivity which have occurred during the vegetation periods of 1987 and 1988 have been investigated. It is also demonstrated how the conditions have changed in the following two periods of growth. In leaves of deciduous trees which were directly contaminated in 1986 natural radioactivity is sometim