WorldWideScience

Sample records for electron energy losses

  1. electron energy-loss spectroscopy

    International Nuclear Information System (INIS)

    Egerton, R.

    1997-01-01

    As part of a commemorative series of articles to mark the hundredth anniversary of the discovery of the electron, this article describes the use of electron energy-loss spectroscopy. The physical and chemical properties of materials can be studied by considering the energy that electrons use as they travel through a solid, often in conjunction with other analytical techniques. The technique is often combined with electron diffraction and high-resolution imaging and can be used to provide elemental identification down to the atomic scale. 6 figs

  2. Electron energy-loss spectroscopy

    International Nuclear Information System (INIS)

    Egerton, R.

    1997-01-01

    As part of the commemorative series of articles to mark the hundredth anniversary of the discovery of the electron, this article discusses electron energy-loss spectroscopy. The physical and chemical properties of materials can be studied by considering the energy that electrons use as they travel through a solid, often in conjunction with other analytical techniques. The technique is often combined with electron diffraction and high-resolution imaging and can be used to provide elemental identification down to the atomic scale. (UK)

  3. Depth sectioning using electron energy loss spectroscopy

    International Nuclear Information System (INIS)

    D'Alfonso, A J; Findlay, S D; Allen, L J; Cosgriff, E C; Kirkland, A I; Nellist, P D; Oxley, M P

    2008-01-01

    The continued development of electron probe aberration correctors for scanning transmission electron microscopy has enabled finer electron probes, allowing atomic resolution column-by-column electron energy loss spectroscopy. Finer electron probes have also led to a decrease in the probe depth of focus, facilitating optical slicing or depth sectioning of samples. The inclusion of post specimen aberration corrected image forming lenses allows for scanning confocal electron microscopy with further improved depth resolution and selectivity. We show that in both scanning transmission electron microscopy and scanning confocal electron microscopy geometries, by performing a three dimensional raster scan through a specimen and detecting electrons scattered with a characteristic energy loss, it will be possible to determine the location of isolated impurities embedded within the bulk.

  4. Coherence in electron energy loss spectrometry

    International Nuclear Information System (INIS)

    Schattschneider, P.; Werner, W.S.M.

    2005-01-01

    Coherence effects in electron energy loss spectrometry (EELS) and in energy filtering are largely neglected although they occur frequently due to Bragg scattering in crystals. We discuss how coherence in the inelastically scattered wave field can be described by the mixed dynamic form factor (MDFF), and how it relates to the density matrix of the scattered electrons. Among the many aspects of 'inelastic coherence' are filtered high-resolution images, dipole-forbidden transitions, coherence in plasma excitations, errors in chemical microanalysis, coherent double plasmons, and circular dichroism

  5. Electron energy-loss spectra in molecular fluorine

    Science.gov (United States)

    Nishimura, H.; Cartwright, D. C.; Trajmar, S.

    1979-01-01

    Electron energy-loss spectra in molecular fluorine, for energy losses from 0 to 17.0 eV, have been taken at incident electron energies of 30, 50, and 90 eV and scattering angles from 5 to 140 deg. Features in the spectra above 11.5 eV energy loss agree well with the assignments recently made from optical spectroscopy. Excitations of many of the eleven repulsive valence excited electronic states are observed and their location correlates reasonably well with recent theoretical results. Several of these excitations have been observed for the first time and four features, for which there are no identifications, appear in the spectra.

  6. Performance of the electron energy-loss spectrometer

    International Nuclear Information System (INIS)

    Tanaka, H.; Huebner, R.H.

    1977-01-01

    Performance characteristics of the electron energy-loss spectrometer incorporating a new high-resolution hemispherical monochromator are reported. The apparatus achieved an energy-resolution of 25 meV in the elastic scattering mode, and angular distributions of elastically scattered electrons were in excellent agreement with previous workers. Preliminary energy-loss spectra for several atmospheric gases demonstrate the excellent versatility and stable operation of the improved system. 12 references

  7. Energy loss and thermalization of low-energy electrons

    International Nuclear Information System (INIS)

    LaVerne, J.A.; Mozumder, A.; Notre Dame Univ., IN

    1984-01-01

    Various processes involved in the moderation of low-energy electrons (< 10 keV in energy) have been delineated in gaseous and liquid media. The discussion proceeds in two stages. The first stage ends and the second stage begins when the electron energy equals the first excitation potential of the medium. The second stage ends with thermalization. Cross sections for electronic excitation and for the excitation (and de-excitation) of sub-electronic processes have been evaluated and incorporated in suitable stopping power and transport theories. Comparison between experiment and theory and intercomparisons between theories and experiments have been provided where possible. (author)

  8. Data Acquisition System for Electron Energy Loss Coincident Spectrometers

    International Nuclear Information System (INIS)

    Zhang Chi; Yu Xiaoqi; Yang Tao

    2005-01-01

    A Data Acquisition System (DAQ) for electron energy loss coincident spectrometers (EELCS) has been developed. The system is composed of a Multiplex Time-Digital Converter (TDC) that measures the flying time of positive and negative ions and a one-dimension position-sensitive detector that records the energy loss of scattering electrons. The experimental data are buffered in a first-in-first-out (FIFO) memory module, then transferred from the FIFO memory to PC by the USB interface. The DAQ system can record the flying time of several ions in one collision, and allows of different data collection modes. The system has been demonstrated at the Electron Energy Loss Coincident Spectrometers at the Laboratory of Atomic and Molecular Physics, USTC. A detail description of the whole system is given and experimental results shown

  9. Surface energy loss processes in XPS studied by absolute reflection electron energy loss spectroscopy

    International Nuclear Information System (INIS)

    Nagatomi, T.; Goto, K.

    2010-01-01

    The results of the investigation of the inelastic interaction of 300-3000 eV electrons with the Ni and Au surfaces by the analysis of absolute reflection electron energy loss spectroscopy (REELS) spectra were described. The present analysis enables the inelastic mean free path (IMFP), surface excitation parameter (SEP) and differential SEP (DSEP) to be obtained simultaneously from an absolute REELS spectrum. The obtained IMFPs for Ni and Au showed a good agreement with those calculated using the TPP-2M predictive equation. The present SEPs determined for Ni and Au were fitted to the Chen's formula describing the dependence of the SEP on the electron energy, and material parameters for Ni and Au in Chen's formula were proposed. The present DESPs were compared with the theoretical results, and a reasonable agreement between the experimentally determined DSEPs and theoretical results was confirmed. The MC modeling of calculating the REELS spectrum, in which energy loss processes due to surface excitations are taken into account, was also described. The IMFP, SEP and DSEP determined by the present absolute REELS analysis were employed to describe energy loss processes by inelastic scattering in the proposed MC simulation. The simulated REELS spectra were found to be in a good agreement with the experimental spectra for both Ni and Au.

  10. Nonequilibrium electron energy-loss kinetics in metal clusters

    CERN Document Server

    Guillon, C; Fatti, N D; Vallee, F

    2003-01-01

    Ultrafast energy exchanges of a non-Fermi electron gas with the lattice are investigated in silver clusters with sizes ranging from 4 to 26 nm using a femtosecond pump-probe technique. The results yield evidence for a cluster-size-dependent slowing down of the short-time energy losses of the electron gas when it is strongly athermal. A constant rate is eventually reached after a few hundred femtoseconds, consistent with the electron gas internal thermalization kinetics, this behaviour reflecting evolution from an individual to a collective electron-lattice type of coupling. The timescale of this transient regime is reduced in small nanoparticles, in agreement with speeding up of the electron-electron interactions with size reduction. The experimental results are in quantitative agreement with numerical simulations of the electron kinetics.

  11. Electron energy loss spectroscopy of gold nanoparticles on graphene

    International Nuclear Information System (INIS)

    DeJarnette, Drew; Roper, D. Keith

    2014-01-01

    Plasmon excitation decay by absorption, scattering, and hot electron transfer has been distinguished from effects induced by incident photons for gold nanoparticles on graphene monolayer using electron energy loss spectroscopy (EELS). Gold nano-ellipses were evaporated onto lithographed graphene, which was transferred onto a silicon nitride transmission electron microscopy grid. Plasmon decay from lithographed nanoparticles measured with EELS was compared in the absence and presence of the graphene monolayer. Measured decay values compared favorably with estimated radiative and non-radiative contributions to decay in the absence of graphene. Graphene significantly enhanced low-energy plasmon decay, increasing mode width 38%, but did not affect higher energy plasmon or dark mode decay. This decay beyond expected radiative and non-radiative mechanisms was attributed to hot electron transfer, and had quantum efficiency of 20%, consistent with previous reports

  12. The Generalized Multipole Technique for the Simulation of Low-Loss Electron Energy Loss Spectroscopy

    DEFF Research Database (Denmark)

    Kiewidt, Lars; Karamehmedovic, Mirza

    2018-01-01

    In this study, we demonstrate the use of a Generalized Multipole Technique (GMT) to simulate low-loss Electron Energy Loss Spectroscopy (EELS) spectra of isolated spheriodal nanoparticles. The GMT provides certain properties, such as semi-analytical description of the electromagnetic fields...

  13. Construction of energy loss function for low-energy electrons in helium

    Energy Technology Data Exchange (ETDEWEB)

    Dayashankar, [Bhabha Atomic Research Centre, Bombay (India). Div. of Radiation Protection

    1976-02-01

    The energy loss function for electrons in the energy range from 50 eV to 1 keV in helium gas has been constructed by considering separately the energy loss in overcoming the ionization threshold, the loss manifested as kinetic energy of secondary electrons and the loss in the discrete state excitations. This has been done by utilizing recent measurements of Opal et al. on the energy spectrum of secondary electrons and incorporating the experimental data on cross sections for twenty-four excited states. The present results of the energy loss function are in good agreement with the Bethe formula for energies above 500 eV. For lower energies, where the Bethe formula is not applicable, the present results should be particularly useful.

  14. Electronic energy loss of fast molecules in matter

    International Nuclear Information System (INIS)

    Steinbeck, J.

    1975-06-01

    In high velocity collisions of molecular ions the correlated motion influence of the ion cores on the electronic energy loss is investigated. The stopping power in first Born approximation for a random arrangement of target atoms can be formulated in terms of the inelastic electronic structure factor. In treating the target atoms in Hartree-Fock approximation each electron can be regarded as stopping the ion independent of all other electrons without restriction by the Pauli principle. A second equivalent formulation of the stopping power leads to the dielectric function of the target. The results are applied to the stopping of H 2 + -ions. For vanishing distance between the two protons the stopping power per particle is twice that for single proton collisions. For distances in the order of the Bohr radius the correlated stopping power may even be smaller than for uncorrelated protons. With increasing distances the correlation influence vanishes. The stopping of H 2 + -ions in C, Si and Ge is discussed using Clementi wave functions for the core electrons and a free electron approximation with Lindhard's dielectric function for the valence electrons. The comparison with the only experimental result available for H 2 + in C at 300 keV yields qualitative agreement. (orig.) [de

  15. Probing Plasmonic Nanostructures with Electron Energy - Loss Spectroscopy

    DEFF Research Database (Denmark)

    Raza, Søren

    for nonlocal response. The experimental work comprises the use of electron energy-loss spectroscopy (EELS) to excite and study both localized and propagating surface plasmons in metal structures. Following a short introduction, we present the theoretical foundation to describe nonlocal response in Maxwell......, dimer with nanometer-sized gaps, core-shell nanowire with ultrathin metal shell, and a thin metal film. In all cases we compare the nonlocal models with the local-response approximation. Below the plasma frequency, we find that the distance between the induced positive and negative surface charges...

  16. Characteristic losses of electrons energy under reflection from leadsilicate glasses

    International Nuclear Information System (INIS)

    Gusarov, A.I.; Mashkov, V.A.; Pronin, V.P.; Tyutikov, A.M.

    1986-01-01

    The spectra of characteristic losses of energy (CLE) for the case of electron reflection from the surface of leadsilicate glasses of the composition xPbOx(1-x)SiO 2 , depending on molar concentration of lead oxide x, has been calculated for the first time. It is shown that the given model of glass energy structure permits to describe correctly general behaviour of CLE spectrum. However, the energy of plasma maximum measured experimentally remains approximately constant. The behaviour can be conditioned by ω 0 dependence on x[4], which has not been taken into account, and (or) by a slower change in ΔE, than it has been assumed. Further refining of theory and experiment is required to solve the problem

  17. EELOSS: the program for calculation of electron energy loss data

    International Nuclear Information System (INIS)

    Tanaka, Shun-ichi

    1980-10-01

    A computer code EELOSS has been developed to obtain the electron energy loss data required for shielding and dosimetry of beta- and gamma-rays in nuclear plants. With this code, the following data are obtainable for any energy from 0.01 to 15 MeV in any medium (metal, insulator, gas, compound, or mixture) composed of any choice of 69 elements with atomic number 1 -- 94: a) Collision stopping power, b) Restricted collision stopping power, c) Radiative stopping power, and d) Bremsstrahlung production cross section. The availability of bremsstrahlung production cross section data obtained by the EELOSS code is demonstrated by the comparison of calculated gamma-ray spectrum with measured one in Pb layer, where electron-photon cascade is included implicitly. As a result, it is concluded that the uncertainty in the bremsstrahlung production cross sections is negligible in the practical shielding calculations of gamma rays of energy less than 15 MeV, since the bremsstrahlung production cross sections increase with the gamma-ray energy and the uncertainty for them decreases with increasing the gamma-ray energy. Furthermore, the accuracy of output data of the EELOSS code is evaluated in comparison with experimental data, and satisfactory agreements are observed concerning the stopping power. (J.P.N.)

  18. Electron energy-loss spectroscopy on fullerenes and fullerene compounds

    International Nuclear Information System (INIS)

    Armbruster, J.

    1996-03-01

    A few years ago, a new form of pure carbon, the fullerenes, has been discovered, which shows many fascinating properties. Within this work the spatial and electronic structure of some selected fullerene compounds have been investigated by electron-energy-loss spectroscopy in transmission. Phase pure samples of alkali intercalated fullerides A x C 60 (A=Na, K, Cs) have been prepared using vacuum distillation. Measruements of K 3 C 60 show a dispersion of the charge carrier plasmon close to zero. This can be explained by calculations, which take into account both band structure and local-field (inhomogeneity) effects. The importance of the molecular structure can also be seen from the A 4 C 60 compounds, where the non-metallic properties are explained by a splitting of the t 1u and t 1g derived bands that is caused by electron-correlation and Jahn-Teller effects. First measurements of the electronic structure of Na x C 60 (x>6) are presented and reveal a complete transfer from the sodium atoms but an incomplete transfer onto the C 60 molecules. This behaviour can be explained by taking into account additional electronic states that are situated between the sodium atoms in the octahedral sites and are predicted by calculations using local density approximation. The crystal structure of the higher fullerenes C 76 and C 84 is found to be face-centered cubic

  19. Atomic column resolved electron energy-loss spectroscopy

    International Nuclear Information System (INIS)

    Duscher, G.; Pennycook, S.J.; Browning, N.D.

    1998-01-01

    Spatially resolved electron energy-loss spectroscopy (EELS) is rapidly developing into a unique and powerful tool to characterize internal interfaces. Because atomic column resolved Z-contrast imaging can be performed simultaneously with EELS in the scanning transmission electron microscope, this combination allows the atomic structure to be correlated with the electronic structure, and thus the local properties of interfaces or defects can be determined directly. However, the ability to characterize interfaces and defects at that level requires not only high spatial resolution but also the exact knowledge of the beam location, from where the spectrum is obtained. Here we discuss several examples progressing from cases where the limitation in spatial resolution is given by the microscopes or the nature of the sample, to one example of impurity atoms at a grain boundary, which show intensity and fine structure changes from atomic column to atomic column. Such data can be interpreted as changes in valence of the impurity, depending on its exact site in the boundary plane. Analysis ofthis nature is a valuable first step in understanding the microscopic structural, optical and electronic properties of materials. (orig.)

  20. Secondary electron emission studied by secondary electron energy loss coincidence spectroscopy (SE2ELCS)

    International Nuclear Information System (INIS)

    Khalid, R.

    2013-01-01

    Emission of secondary electrons is of importance in many branches of fundamental and applied science. It is widely applied in the electron microscope for the investigation of the structure and electronic state of solid surfaces and particle detection in electron multiplier devices, and generally it is related to the energy dissipation of energetic particles moving inside a solid. The process of secondary electron emission is a complex physical phenomenon, difficult to measure experimentally and treat theoretically with satisfactory accuracy. The secondary electron spectrum measured with single electron spectroscopy does not provide detailed information of the energy loss processes responsible for the emission of secondary electrons. This information can be accessed when two correlated electron pairs are measured in coincidence and the pair consists of a backscattered electron after a given energy loss and a resulting emitted secondary electron. To investigate the mechanisms responsible for the emission of secondary electrons, a reflection (e,2e) coincidence spectrometer named Secondary Electron Electron Energy Loss Coincidence Spectrometer (SE2ELCS) has been developed in the framework of this thesis which allows one to uncover the relation between the features in the spectra which are due to energy losses and true secondary electron emission structures. The correlated electron pairs are measured with a hemispherical mirror analyzer (HMA) and a time of flight analyzer (TOF) by employing a continuous electron beam. An effort has been made to increase the coincidence count rate by increasing the effective solid angle of the TOF analyzer and optimizing the experimental parameters to get optimum energy resolution. Double differential coincidence spectra for a number of materials namely, nearly free electron metals (Al, Si), noble metals (Ag, Au, Cu, W) and highly oriented pyrolytic graphite (HOPG) have been measured using this coincidence spectrometer. The

  1. Study of optical and electronic properties of nickel from reflection electron energy loss spectra

    Science.gov (United States)

    Xu, H.; Yang, L. H.; Da, B.; Tóth, J.; Tőkési, K.; Ding, Z. J.

    2017-09-01

    We use the classical Monte Carlo transport model of electrons moving near the surface and inside solids to reproduce the measured reflection electron energy-loss spectroscopy (REELS) spectra. With the combination of the classical transport model and the Markov chain Monte Carlo (MCMC) sampling of oscillator parameters the so-called reverse Monte Carlo (RMC) method was developed, and used to obtain optical constants of Ni in this work. A systematic study of the electronic and optical properties of Ni has been performed in an energy loss range of 0-200 eV from the measured REELS spectra at primary energies of 1000 eV, 2000 eV and 3000 eV. The reliability of our method was tested by comparing our results with the previous data. Moreover, the accuracy of our optical data has been confirmed by applying oscillator strength-sum rule and perfect-screening-sum rule.

  2. Communication: Investigation of the electron momentum density distribution of nanodiamonds by electron energy-loss spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Feng, Zhenbao; Yang, Bing; Lin, Yangming; Su, Dangsheng, E-mail: dssu@imr.ac.cn [Shenyang National Laboratory of Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Wenhua Road 72, Shenyang 110016 (China)

    2015-12-07

    The electron momentum distribution of detonation nanodiamonds (DND) was investigated by recording electron energy-loss spectra at large momentum transfer in the transmission electron microscope (TEM), which is known as electron Compton scattering from solid (ECOSS). Compton profile of diamond film obtained by ECOSS was found in good agreement with prior photon experimental measurement and theoretical calculation that for bulk diamond. Compared to the diamond film, the valence Compton profile of DND was found to be narrower, which indicates a more delocalization of the ground-state charge density for the latter. Combining with other TEM characterizations such as high-resolution transmission electron spectroscopy, diffraction, and energy dispersive X-ray spectroscopy measurements, ECOSS was shown to be a great potential technique to study ground-state electronic properties of nanomaterials.

  3. Microanalysis by spectroscopy of transmitted electron energy losses

    International Nuclear Information System (INIS)

    Colliex, C.; Trebbia, P.

    1978-01-01

    Among the various signals which, in a transmission electron microscope, result from the interactions between the primary beam of well defined energy E 0 and the sample, the spectrum of the energy distribution of the electrons transmitted contains useful informations on the chemical and physical properties of the sample. Consequently the adaptation of an energy dispersive system on an electron microscope enables new fields of research to be investigated, particularly a localised chemical analysis technique with a space resolution scale equal to that of the electron microscope. It is this second aspect that we suggest describing in particular here. Already, this technique appears to be indispensable in the problems arising from the analysis of very small quantities of matter: detection limits in the order of 10 -19 to 10 -20 g (around 100 to 1000 atoms) would seem to be resonably possible [fr

  4. Precessed electron beam electron energy loss spectroscopy of graphene: Beyond channelling effects

    Energy Technology Data Exchange (ETDEWEB)

    Yedra, Ll.; Estradé, S., E-mail: sestrade@ub.edu [LENS, MIND-IN2UB, Departament d' Electrònica, Universitat de Barcelona, Martí i Franquès 1, 08028 Barcelona (Spain); TEM-MAT, CCiT, Universitat de Barcelona, Solé i Sabarís 1, 08028 Barcelona (Spain); Torruella, P.; Eljarrat, A.; Peiró, F. [LENS, MIND-IN2UB, Departament d' Electrònica, Universitat de Barcelona, Martí i Franquès 1, 08028 Barcelona (Spain); Darbal, A. D. [AppFive LLC, 1095 W Rio Salado Pkway, Suite 110, Tempe, Arizona 85281 (United States); Weiss, J. K. [AppFive LLC, 1095 W Rio Salado Pkway, Suite 110, Tempe, Arizona 85281 (United States); NanoMEGAS SPRL, Blvd. Edmond Machtens 79, B-1080 Brussels (Belgium)

    2014-08-04

    The effects of beam precession on the Electron Energy Loss Spectroscopy (EELS) signal of the carbon K edge in a 2 monolayer graphene sheet are studied. In a previous work, we demonstrated the use of precession to compensate for the channeling-induced reduction of EELS signal when in zone axis. In the case of graphene, no enhancement of EELS signal is found in the usual experimental conditions, as graphene is not thick enough to present channeling effects. Interestingly, though it is found that precession makes it possible to increase the collection angle, and, thus, the overall signal, without a loss of signal-to-background ratio.

  5. First principles study of electronic properties, interband transitions and electron energy loss of α-graphyne

    Science.gov (United States)

    Behzad, Somayeh

    2016-04-01

    The electronic and optical properties of α-graphyne sheet are investigated by using density functional theory. The results confirm that α-graphyne sheet is a zero-gap semimetal. The optical properties of the α-graphyne sheet such as dielectric function, refraction index, electron energy loss function, reflectivity, absorption coefficient and extinction index are calculated for both parallel and perpendicular electric field polarizations. The optical spectra are strongly anisotropic along these two polarizations. For (E ∥ x), absorption edge is at 0 eV, while there is no absorption below 8 eV for (E ∥ z).

  6. Low-dose electron energy-loss spectroscopy using electron counting direct detectors.

    Science.gov (United States)

    Maigné, Alan; Wolf, Matthias

    2018-03-01

    Since the development of parallel electron energy loss spectroscopy (EELS), charge-coupled devices (CCDs) have been the default detectors for EELS. With the recent development of electron-counting direct-detection cameras, micrographs can be acquired under very low electron doses at significantly improved signal-to-noise ratio. In spectroscopy, in particular in combination with a monochromator, the signal can be extremely weak and the detection limit is principally defined by noise introduced by the detector. Here we report the use of an electron-counting direct-detection camera for EEL spectroscopy. We studied the oxygen K edge of amorphous ice and obtained a signal noise ratio up to 10 times higher than with a conventional CCD.We report the application of electron counting to record time-resolved EEL spectra of a biological protein embedded in amorphous ice, revealing chemical changes observed in situ while exposed by the electron beam. A change in the fine structure of nitrogen K and the carbon K edges were recorded during irradiation. A concentration of 3 at% nitrogen was detected with a total electron dose of only 1.7 e-/Å2, extending the boundaries of EELS signal detection at low electron doses.

  7. Electron transport in furfural: dependence of the electron ranges on the cross sections and the energy loss distribution functions

    Science.gov (United States)

    Ellis-Gibbings, L.; Krupa, K.; Colmenares, R.; Blanco, F.; Muńoz, A.; Mendes, M.; Ferreira da Silva, F.; Limá Vieira, P.; Jones, D. B.; Brunger, M. J.; García, G.

    2016-09-01

    Recent theoretical and experimental studies have provided a complete set of differential and integral electron scattering cross section data from furfural over a broad energy range. The energy loss distribution functions have been determined in this study by averaging electron energy loss spectra for different incident energies and scattering angles. All these data have been used as input parameters for an event by event Monte Carlo simulation procedure to obtain the electron energy deposition patterns and electron ranges in liquid furfural. The dependence of these results on the input cross sections is then analysed to determine the uncertainty of the simulated values.

  8. Electronic and optical properties of Fe, Pd, and Ti studied by reflection electron energy loss spectroscopy

    International Nuclear Information System (INIS)

    Tahir, Dahlang; Kraaer, Jens; Tougaard, Sven

    2014-01-01

    We have studied the electronic and optical properties of Fe, Pd, and Ti by reflection electron energy-loss spectroscopy (REELS). REELS spectra recorded for primary energies in the range from 300 eV to 10 keV were corrected for multiple inelastically scattered electrons to determine the effective inelastic-scattering cross section. The dielectric functions and optical properties were determined by comparing the experimental inelastic-electron scattering cross section with a simulated cross section calculated within the semi-classical dielectric response model in which the only input is Im(−1/ε) by using the QUEELS-ε(k,ω)-REELS software package. The complex dielectric functions ε(k,ω), in the 0–100 eV energy range, for Fe, Pd, and Ti were determined from the derived Im(−1/ε) by Kramers-Kronig transformation and then the refractive index n and extinction coefficient k. The validity of the applied model was previously tested and found to give consistent results when applied to REELS spectra at energies between 300 and 1000 eV taken at widely different experimental geometries. In the present paper, we provide, for the first time, a further test on its validity and find that the model also gives consistent results when applied to REELS spectra in the full range of primary electron energies from 300 eV to 10000 eV. This gives confidence in the validity of the applied method.

  9. Electron loss from multiply protonated lysozyme ions in high energy collisions with molecular oxygen

    DEFF Research Database (Denmark)

    Hvelplund, P; Nielsen, SB; Sørensen, M

    2001-01-01

    We report on the electron loss from multiply protonated lysozyme ions Lys-Hn(n)+ (n = 7 - 17) and the concomitant formation of Lys-Hn(n+1)+. in high-energy collisions with molecular oxygen (laboratory kinetic energy = 50 x n keV). The cross section for electron loss increases with the charge state...... of the precursor from n = 7 to n = 11 and then remains constant when n increases further. The absolute size of the cross section ranges from 100 to 200 A2. The electron loss is modeled as an electron transfer process between lysozyme cations and molecular oxygen....

  10. Bremsstrahlung spectra from thick-target electron beams with noncollisional energy losses

    International Nuclear Information System (INIS)

    Brown, J.C.; MacKinnon, A.L.

    1985-01-01

    We consider what can be learned from the bremsstrahlung radiation of fast electrons in a thick target, generalized to include electron energy losses additional to collisions. We show that the observed photon spectrum can, in principle, be inverted to yield an integral functional of the electron spectrum and the effective energy loss rate. In the light of this result, there seems no reason to suppose, in the absence of a priori information to the contrary, that the photon spectrum is symptomatic more of the fast electron distribution than of the energy loss processes. In cases where the electron injection spectrum is known on independent observational or theoretical grounds, it is possible to infer an effective, ''phenomenological'' energy loss function. In the more general case, however, fullest possible modeling of the physical situation and comparison of the resulting spectrum with observations is all that can be attempted

  11. Calculated and experimental low-loss electron energy loss spectra of dislocations in diamond and GaN

    CERN Document Server

    Jones, R; Gutiérrez-Sosa, A; Bangert, U; Heggie, M I; Blumenau, A T; Frauenheim, T; Briddon, P R

    2002-01-01

    First-principles calculations of electron energy loss (EEL) spectra for bulk GaN and diamond are compared with experimental spectra acquired with a scanning tunnelling electron microscope offering ultra-high-energy resolution in low-loss energy spectroscopy. The theoretical bulk low-loss EEL spectra, in the E sub g to 10 eV range, are in good agreement with experimental data. Spatially resolved spectra from dislocated regions in both materials are distinct from bulk spectra. The main effects are, however, confined to energy losses lying above the band edge. The calculated spectra for low-energy dislocations in diamond are consistent with the experimental observations, but difficulties remain in understanding the spectra of threading dislocations in GaN.

  12. Electron energy loss spectroscopy microanalysis and imaging in the transmission electron microscope: example of biological applications

    International Nuclear Information System (INIS)

    Diociaiuti, Marco

    2005-01-01

    This paper reports original results obtained in our laboratory over the past few years in the application of both electron energy loss spectroscopy (EELS) and electron spectroscopy imaging (ESI) to biological samples, performed in two transmission electron microscopes (TEM) equipped with high-resolution electron filters and spectrometers: a Gatan model 607 single magnetic sector double focusing EEL serial spectrometer attached to a Philips 430 TEM and a Zeiss EM902 Energy Filtering TEM. The primary interest was on the possibility offered by the combined application of these spectroscopic techniques with those offered by the TEM. In particular, the electron beam focusing available in a TEM allowed us to perform EELS and ESI on very small sample volumes, where high-resolution imaging and electron diffraction techniques can provide important structural information. I show that ESI was able to improve TEM performance, due to the reduced chromatic aberration and the possibility of avoiding the sample staining procedure. Finally, the analysis of the oscillating extended energy loss fine structure (EXELFS) beyond the ionization edges characterizing the EELS spectra allowed me, in a manner very similar to the extended X-ray absorption fine structure (EXAFS) analysis of the X-ray absorption spectra, to obtain short-range structural information for such light elements of biological interest as O or Fe. The Philips EM430 (250-300 keV) TEM was used to perform EELS microanalysis on Ca, P, O, Fe, Al and Si. The assessment of the detection limits of this method was obtained working with well-characterized samples containing Ca and P, and mimicking the actual cellular matrix. I applied EELS microanalysis to Ca detection in bone tissue during the mineralization process and to P detection in the cellular membrane of erythrocytes treated with an anti-tumoral drug, demonstrating that the cellular membrane is a drug target. I applied EELS microanalysis and selected area electron

  13. Depth-selective X-ray absorption spectroscopy by detection of energy-loss Auger electrons

    Energy Technology Data Exchange (ETDEWEB)

    Isomura, Noritake, E-mail: isomura@mosk.tytlabs.co.jp [Toyota Central R& D Labs., Inc., 41-1 Yokomichi, Nagakute, Aichi 480-1192 (Japan); Soejima, Narumasa; Iwasaki, Shiro [Toyota Central R& D Labs., Inc., 41-1 Yokomichi, Nagakute, Aichi 480-1192 (Japan); Nomoto, Toyokazu; Murai, Takaaki [Aichi Synchrotron Radiation Center (AichiSR), 250-3 Minamiyamaguchi-cho, Seto, Aichi 489-0965 (Japan); Kimoto, Yasuji [Toyota Central R& D Labs., Inc., 41-1 Yokomichi, Nagakute, Aichi 480-1192 (Japan)

    2015-11-15

    Graphical abstract: - Highlights: • A unique XAS method is proposed for depth profiling of chemical states. • PEY mode detecting energy-loss electrons enables a variation in the probe depth. • Si K-edge XAS spectra of the Si{sub 3}N{sub 4}/SiO{sub 2}/Si multilayer films have been investigated. • Deeper information was obtained in the spectra measured at larger energy loss. • Probe depth could be changed by the selection of the energy of detected electrons. - Abstract: A unique X-ray absorption spectroscopy (XAS) method is proposed for depth profiling of chemical states in material surfaces. Partial electron yield mode detecting energy-loss Auger electrons, called the inelastic electron yield (IEY) mode, enables a variation in the probe depth. As an example, Si K-edge XAS spectra for a well-defined multilayer sample (Si{sub 3}N{sub 4}/SiO{sub 2}/Si) have been investigated using this method at various kinetic energies. We found that the peaks assigned to the layers from the top layer to the substrate appeared in the spectra in the order of increasing energy loss relative to the Auger electrons. Thus, the probe depth can be changed by the selection of the kinetic energy of the energy loss electrons in IEY-XAS.

  14. Depth-selective X-ray absorption spectroscopy by detection of energy-loss Auger electrons

    International Nuclear Information System (INIS)

    Isomura, Noritake; Soejima, Narumasa; Iwasaki, Shiro; Nomoto, Toyokazu; Murai, Takaaki; Kimoto, Yasuji

    2015-01-01

    Graphical abstract: - Highlights: • A unique XAS method is proposed for depth profiling of chemical states. • PEY mode detecting energy-loss electrons enables a variation in the probe depth. • Si K-edge XAS spectra of the Si_3N_4/SiO_2/Si multilayer films have been investigated. • Deeper information was obtained in the spectra measured at larger energy loss. • Probe depth could be changed by the selection of the energy of detected electrons. - Abstract: A unique X-ray absorption spectroscopy (XAS) method is proposed for depth profiling of chemical states in material surfaces. Partial electron yield mode detecting energy-loss Auger electrons, called the inelastic electron yield (IEY) mode, enables a variation in the probe depth. As an example, Si K-edge XAS spectra for a well-defined multilayer sample (Si_3N_4/SiO_2/Si) have been investigated using this method at various kinetic energies. We found that the peaks assigned to the layers from the top layer to the substrate appeared in the spectra in the order of increasing energy loss relative to the Auger electrons. Thus, the probe depth can be changed by the selection of the kinetic energy of the energy loss electrons in IEY-XAS.

  15. Optimization of Monochromated TEM for Ultimate Resolution Imaging and Ultrahigh Resolution Electron Energy Loss Spectroscopy

    KAUST Repository

    Lopatin, Sergei; Cheng, Bin; Liu, Wei-Ting; Tsai, Meng-Lin; He, Jr-Hau; Chuvilin, Andrey

    2017-01-01

    The performance of a monochromated transmission electron microscope with Wien type monochromator is optimized to achieve an extremely narrow energy spread of electron beam and an ultrahigh energy resolution with spectroscopy. The energy spread in the beam is improved by almost an order of magnitude as compared to specified values. The optimization involves both the monochromator and the electron energy loss detection system. We demonstrate boosted capability of optimized systems with respect to ultra-low loss EELS and sub-angstrom resolution imaging (in a combination with spherical aberration correction).

  16. Optimization of Monochromated TEM for Ultimate Resolution Imaging and Ultrahigh Resolution Electron Energy Loss Spectroscopy

    KAUST Repository

    Lopatin, Sergei

    2017-09-01

    The performance of a monochromated transmission electron microscope with Wien type monochromator is optimized to achieve an extremely narrow energy spread of electron beam and an ultrahigh energy resolution with spectroscopy. The energy spread in the beam is improved by almost an order of magnitude as compared to specified values. The optimization involves both the monochromator and the electron energy loss detection system. We demonstrate boosted capability of optimized systems with respect to ultra-low loss EELS and sub-angstrom resolution imaging (in a combination with spherical aberration correction).

  17. Electron energy-loss spectrometry at the frontier of spatial and energy resolution

    International Nuclear Information System (INIS)

    Hofer, F.; Grogger, W.; Kothleitner, G.

    2004-01-01

    Full text: Electron energy-loss spectroscopy (EELS) in the transmission electron microscope (TEM) is now used routinely as a means of measuring chemical and structural properties of very small regions of a thin specimen. The power of this technique depends significantly on two parameters: its spatial resolution and the energy resolution available in the spectrum and in the energy-filtered TEM (EFTEM) image. The cold field emission source and the Schottky emitter have made an energy resolution below 1 eV possible and it is now feasible to obtain data with a spatial resolution close to atomic dimensions, given the right instrumentation and specimen. EFTEM allows to record elemental maps at sub-nanometre resolution, being mainly limited by chromatic and spherical aberration of the objective lens and by delocalization of inelastic scattering. Recently the possibility of correcting spherical and even chromatic aberrations of electron lenses has become a practical reality thus improving the point resolution of the TEM to below 0.1 nm. The other limiting factor for EFTEM resolution is delocalization. However, recent measurements show that resolution values in the range of 1 nm and below can be achieved, even for energy-losses of only a few eV. In terms of energy-resolution, EELS and EFTEM compare less favourably with other spectroscopies. For common TEMs, the overall energy-resolution is mainly determined by the energy width of the electron source, typically between 0.5 and 1.5 eV. For comparison, synchrotron x-ray sources and beam line spectrometers, provide a resolution well below 0.1 eV for absorption spectroscopy. During the early sixties, the energy spread of an electron beam could be reduced by incorporating an energy-filter into the illumination system, but the system lacked spatial resolution. Later developments combined high energy resolution in the range of 0.1 eV with improved spatial resolution. Recently, FEI introduced a new high resolution EELS system based

  18. Electron energy-loss spectroscopy of branched gap plasmon resonators

    DEFF Research Database (Denmark)

    Raza, Søren; Esfandyarpour, Majid; Koh, Ai Leen

    2016-01-01

    The miniaturization of integrated optical circuits below the diffraction limit for high-speed manipulation of information is one of the cornerstones in plasmonics research. By coupling to surface plasmons supported on nanostructured metallic surfaces, light can be confined to the nanoscale......, enabling the potential interface to electronic circuits. In particular, gap surface plasmons propagating in an air gap sandwiched between metal layers have shown extraordinary mode confinement with significant propagation length. In this work, we unveil the optical properties of gap surface plasmons...... in silver nanoslot structures with widths of only 25 nm. We fabricate linear, branched and cross-shaped nanoslot waveguide components, which all support resonances due to interference of counter-propagating gap plasmons. By exploiting the superior spatial resolution of a scanning transmission electron...

  19. Characteristic electron energy losses in monoatomic antimony films on (110) and (112) tungsten faces

    International Nuclear Information System (INIS)

    Gorodetskij, D.A.; Gorchinskij, A.D.; Shevlyakov, S.A.

    1981-01-01

    Complex investigations of antimony condensation on a monoatomical clean surface of tungsten monocrystals are carried out. The completion of a physical antimony monolayer has been controlled by the methods of Auger-electron spectroscopy and slow electron diffraction. It is shown that at submonolayer coatings a collectivization of valent electrons occurs leading to appearance of peaks of surface and volumetric plasmons in the energy losses spectrum. The anomalous cencentrational dependence of antimony ionization peak intensity has been found. The origin of previously unexplored peaks in the energy losses spectrum is discussed [ru

  20. First-Principles Vibrational Electron Energy Loss Spectroscopy of β -Guanine

    Science.gov (United States)

    Radtke, G.; Taverna, D.; Lazzeri, M.; Balan, E.

    2017-07-01

    A general approach to model vibrational electron energy loss spectra obtained using an electron beam positioned away from the specimen is presented. The energy-loss probability of the fast electron is evaluated using first-principles quantum mechanical calculations (density functional theory) of the dielectric response of the specimen. The validity of the method is assessed using recently measured anhydrous β -guanine, an important molecular solid used by animals to produce structural colors. The good agreement between theory and experiments lays the basis for a quantitative interpretation of this spectroscopy in complex systems.

  1. Two types of charge transfer excitations in low dimensional cuprates: an electron energy-loss study

    Czech Academy of Sciences Publication Activity Database

    Knupfer, M.; Fink, J.; Drechsler, S.-L.; Hayn, R.; Málek, Jiří; Moskvin, A.S.

    137-140, - (2004), s. 469-473 ISSN 0368-2048 Institutional research plan: CEZ:AV0Z1010914 Keywords : cuprates * electronic excitations * electron energy-loss spectroscopy Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.069, year: 2004

  2. Characteristic electron energy loss in lanthanum films adsorbed on tungsten (110) single crystal

    International Nuclear Information System (INIS)

    Gorodetskij, D.A.; Gorchinskij, A.D.; Kobylyanskij, A.V.

    1988-01-01

    The spectrum of electron energy loss (ELS) in a wide range of energy loss 0-150 eV has been studied for La films adsorbed on W(110) single crystal with the coverage Θ from submonolayer to a few monolayers. The concentration dependence of loss energy peaks amplitude of different nature has been studied for the adsorption of rare earth element on refractory substrate. It has been shown that the essential information for the interpretation of the energy loss nature may be obtained by the investigation of such dependences for La adsorption on W(110). It is found that the surface and bulk plasmons peaks appear in ELS of La-W(110) system before the completion of the physical monolayer. Thus, the collectivization of valence electrons in the rare earth element film at the transition metal surface ensues for the submonolayer coverage like in the case of collective processes in alkali and alkaline earth element films

  3. Evolutionary developments in x ray and electron energy loss microanalysis instrumentation for the analytical electron microscope

    Science.gov (United States)

    Zaluzec, Nester J.

    Developments in instrumentation for both X ray Dispersive and Electron Energy Loss Spectroscopy (XEDS/EELS) over the last ten years have given the experimentalist a greatly enhanced set of analytical tools for characterization. Microanalysts have waited for nearly two decades now in the hope of getting a true analytical microscope and the development of 300 to 400 kV instruments should have allowed us to attain this goal. Unfortunately, this has not generally been the case. While there have been some major improvements in the techniques, there has also been some devolution in the modern AEM (Analytical Electron Microscope). In XEDS, the majority of today's instruments are still plagued by the hole count effect, which was first described in detail over fifteen years ago. The magnitude of this problem can still reach the 20 percent level for medium atomic number species in a conventional off-the-shelf intermediate voltage AEM. This is an absurd situation and the manufacturers should be severely criticized. Part of the blame, however, also rests on the AEM community for not having come up with a universally agreed upon standard test procedure. Fortunately, such a test procedure is in the early stages of refinement. The proposed test specimen consists of an evaporated Cr film approx. 500 to 1000A thick supported upon a 3mm diameter Molybdenum 200 micron aperture.

  4. Target electron collision effects on energy loss straggling of protons in an electron gas at any degeneracy

    International Nuclear Information System (INIS)

    Barriga-Carrasco, Manuel D.

    2008-01-01

    The purpose of the present paper is to describe the effects of target electron collisions on proton energy loss straggling in plasmas at any degeneracy. Targets are considered fully ionized so electronic energy loss is only due to the free electrons. The analysis is focused on targets with electronic density around solid values n e ≅10 23 cm -3 and with temperature around T≅10 eV; these targets are in the limit of weakly coupled electron gases. These types of plasma targets have not been studied extensively, though they are very important for inertial confinement fusion. The energy loss straggling is obtained from an exact quantum-mechanical evaluation, which takes into account the degeneracy of the target plasma, and later it is compared with common classical and degenerate approximations. Then electron collisions in the exact quantum-mechanical straggling calculation are considered. Now the energy loss straggling is enhanced for energies smaller than the energy before the maximum, then decreases around this maximum, and finally tends to the same values with respect to noncollisional calculation. Differences with the same results but not taking into account these collisions are as far as 17% in the cases analyzed. As an example, proton range distributions have been calculated to show the importance of an accurate energy straggling calculation

  5. Surface plasmon modes of a single silver nanorod: An electron energy loss study

    DEFF Research Database (Denmark)

    Nicoletti, Olivia; Wubs, Martijn; Mortensen, N. Asger

    2011-01-01

    We present an electron energy loss study using energy filtered TEM of spatially resolved surface plasmon excitations on a silver nanorod of aspect ratio 14.2 resting on a 30 nm thick silicon nitride membrane. Our results show that the excitation is quantized as resonant modes whose intensity maxima...

  6. Determining the band gap and mean kinetic energy of atoms from reflection electron energy loss spectra

    Energy Technology Data Exchange (ETDEWEB)

    Vos, M. [Atomic and Molecular Physics Laboratories, Research School of Physics and Engineering, Australian National University, Canberra ACT (Australia); Marmitt, G. G. [Atomic and Molecular Physics Laboratories, Research School of Physics and Engineering, Australian National University, Canberra ACT (Australia); Instituto de Fisica da Universidade Federal do Rio Grande do Sul, Avenida Bento Goncalves 9500, 91501-970 Porto Alegre, RS (Brazil); Finkelstein, Y. [Nuclear Research Center — Negev, Beer-Sheva 84190 (Israel); Moreh, R. [Physics Department, Ben-Gurion University of the Negev, Beer-Sheva 84105 (Israel)

    2015-09-14

    Reflection electron energy loss spectra from some insulating materials (CaCO{sub 3}, Li{sub 2}CO{sub 3}, and SiO{sub 2}) taken at relatively high incoming electron energies (5–40 keV) are analyzed. Here, one is bulk sensitive and a well-defined onset of inelastic excitations is observed from which one can infer the value of the band gap. An estimate of the band gap was obtained by fitting the spectra with a procedure that includes the recoil shift and recoil broadening affecting these measurements. The width of the elastic peak is directly connected to the mean kinetic energy of the atom in the material (Doppler broadening). The experimentally obtained mean kinetic energies of the O, C, Li, Ca, and Si atoms are compared with the calculated ones, and good agreement is found, especially if the effect of multiple scattering is taken into account. It is demonstrated experimentally that the onset of the inelastic excitation is also affected by Doppler broadening. Aided by this understanding, we can obtain a good fit of the elastic peak and the onset of inelastic excitations. For SiO{sub 2}, good agreement is obtained with the well-established value of the band gap (8.9 eV) only if it is assumed that the intensity near the edge scales as (E − E{sub gap}){sup 1.5}. For CaCO{sub 3}, the band gap obtained here (7 eV) is about 1 eV larger than the previous experimental value, whereas the value for Li{sub 2}CO{sub 3} (7.5 eV) is the first experimental estimate.

  7. Determining the band gap and mean kinetic energy of atoms from reflection electron energy loss spectra

    International Nuclear Information System (INIS)

    Vos, M.; Marmitt, G. G.; Finkelstein, Y.; Moreh, R.

    2015-01-01

    Reflection electron energy loss spectra from some insulating materials (CaCO 3 , Li 2 CO 3 , and SiO 2 ) taken at relatively high incoming electron energies (5–40 keV) are analyzed. Here, one is bulk sensitive and a well-defined onset of inelastic excitations is observed from which one can infer the value of the band gap. An estimate of the band gap was obtained by fitting the spectra with a procedure that includes the recoil shift and recoil broadening affecting these measurements. The width of the elastic peak is directly connected to the mean kinetic energy of the atom in the material (Doppler broadening). The experimentally obtained mean kinetic energies of the O, C, Li, Ca, and Si atoms are compared with the calculated ones, and good agreement is found, especially if the effect of multiple scattering is taken into account. It is demonstrated experimentally that the onset of the inelastic excitation is also affected by Doppler broadening. Aided by this understanding, we can obtain a good fit of the elastic peak and the onset of inelastic excitations. For SiO 2 , good agreement is obtained with the well-established value of the band gap (8.9 eV) only if it is assumed that the intensity near the edge scales as (E − E gap ) 1.5 . For CaCO 3 , the band gap obtained here (7 eV) is about 1 eV larger than the previous experimental value, whereas the value for Li 2 CO 3 (7.5 eV) is the first experimental estimate

  8. Simulation of electron energy loss spectra of nanomaterials with linear-scaling density functional theory

    International Nuclear Information System (INIS)

    Tait, E W; Payne, M C; Ratcliff, L E; Haynes, P D; Hine, N D M

    2016-01-01

    Experimental techniques for electron energy loss spectroscopy (EELS) combine high energy resolution with high spatial resolution. They are therefore powerful tools for investigating the local electronic structure of complex systems such as nanostructures, interfaces and even individual defects. Interpretation of experimental electron energy loss spectra is often challenging and can require theoretical modelling of candidate structures, which themselves may be large and complex, beyond the capabilities of traditional cubic-scaling density functional theory. In this work, we present functionality to compute electron energy loss spectra within the onetep linear-scaling density functional theory code. We first demonstrate that simulated spectra agree with those computed using conventional plane wave pseudopotential methods to a high degree of precision. The ability of onetep to tackle large problems is then exploited to investigate convergence of spectra with respect to supercell size. Finally, we apply the novel functionality to a study of the electron energy loss spectra of defects on the (1 0 1) surface of an anatase slab and determine concentrations of defects which might be experimentally detectable. (paper)

  9. The energy-deposition model. Electron loss of heavy ions in collisions with neutral atoms at low and intermediate energies

    International Nuclear Information System (INIS)

    Shevelko, V.P.; Litsarev, M.S.; Kato, D.; Tawara, H.

    2010-09-01

    Single- and multiple-electron loss processes in collisions of heavy many-electron ions (positive and negative) in collisions with neutral atoms at low and intermediate energies are considered using the energy-deposition model. The DEPOSIT computer code, created earlier to calculate electron-loss cross sections at high projectile energies, is extended for low and intermediate energies. A description of a new version of DEPOSIT code is given, and the limits of validity for collision velocity in the model are discussed. Calculated electron-loss cross sections for heavy ions and atoms (N + , Ar + , Xe + , U + , U 28+ , W, W + , Ge - , Au - ), colliding with neutral atoms (He, Ne, Ar, W) are compared with available experimental and theoretical data at energies E > 10 keV/u. It is found that in most cases the agreement between experimental data and the present model is within a factor of 2. Combining results obtained by the DEPOSIT code at low and intermediate energies with those by the LOSS-R code at high energies (relativistic Born approximation), recommended electron-loss cross sections in a wide range of collision energy are presented. (author)

  10. Vacuum ultra-violet and electron energy loss spectroscopy of gaseous and solid organic compounds

    International Nuclear Information System (INIS)

    Koch, E.E.; Otto, A.

    1976-01-01

    The experimental arrangements used by the authors for the study of optical vacuum ultra-violet and electron energy loss spectra of organic compounds are described and some theoretical aspects of studies of higher excited states are considered. Results for alkanes, benzene, naphthalene, anthracene and some more complex hydrocarbons are reviewed. Recent results obtained by reflection and electron energy loss spectroscopy for single crystals of anthracene are included and their relevance for gas phase work as well as for the understanding of exciton effects in organic solids is described. (author)

  11. Distributions of energy losses of electrons and pions in the CBM TRD

    International Nuclear Information System (INIS)

    Akishina, E.P.; Akishina, T.P.; Ivanov, V.V.; Denisova, O.Yu.

    2007-01-01

    The distributions of energy losses of electrons and pions in the TRD detector of the CBM experiment are considered. We analyze the measurements of the energy deposits in one-layer TRD prototype obtained during the test beam (GSI, Darmstadt, February 2006) and Monte Carlo simulations for the n-layered TRD realized with the help of GEANT in frames of the CBM ROOT. We show that 1) energy losses both for real measurements and GEANT simulations are approximated with a high accuracy by a log-normal distribution for π and a weighted sum of two log-normal distributions for e; 2) GEANT simulations noticeably differ from real measurements and, as a result, we have a significant loss in the efficiency of the e/π identification. A procedure to control and correct the process of the energy deposit of electrons in the TRD is developed

  12. Electron energy-loss spectroscopy of quasi-one-dimensional cuprates and vanadates

    International Nuclear Information System (INIS)

    Atzkern, S.

    2001-01-01

    In a combination of experimental and theoretical methods in this thesis the electronic structures of quasi-one-dimensional cuprates and vanadates were studied. For this the momentum-dependent loss function was measured by means of the electron energy-loss spectroscopy in transmission on monocrystals of Li 2 CuO 2 , CuGeO 3 , V 2 O 5 and α'-NaVO 5 . The comparison of the experimental data with results from band-structure and cluster calculations allowed conclusions on the mobility and correlations of the electrons in these systems

  13. Electronic properties of Mn-phthalocyanine–C60 bulk heterojunctions: Combining photoemission and electron energy-loss spectroscopy

    International Nuclear Information System (INIS)

    Roth, Friedrich; Herzig, Melanie; Knupfer, Martin; Lupulescu, Cosmin; Darlatt, Erik; Gottwald, Alexander; Eberhardt, Wolfgang

    2015-01-01

    The electronic properties of co-evaporated mixtures (blends) of manganese phthalocyanine and the fullerene C 60 (MnPc:C 60 ) have been studied as a function of the concentration of the two constituents using two supplementary electron spectroscopic methods, photoemission spectroscopy (PES) and electron energy-loss spectroscopy (EELS) in transmission. Our PES measurements provide a detailed picture of the electronic structure measured with different excitation energies as well as different mixing ratios between MnPc and C 60 . Besides a relative energy shift, the occupied electronic states of the two materials remain essentially unchanged. The observed energy level alignment is different compared to that of the related CuPc:C 60 bulk heterojunction. Moreover, the results from our EELS investigations show that, despite the rather small interface interaction, the MnPc related electronic excitation spectrum changes significantly by admixing C 60 to MnPc thin films

  14. High-resolution monochromated electron energy-loss spectroscopy of organic photovoltaic materials.

    Science.gov (United States)

    Alexander, Jessica A; Scheltens, Frank J; Drummy, Lawrence F; Durstock, Michael F; Hage, Fredrik S; Ramasse, Quentin M; McComb, David W

    2017-09-01

    Advances in electron monochromator technology are providing opportunities for high energy resolution (10 - 200meV) electron energy-loss spectroscopy (EELS) to be performed in the scanning transmission electron microscope (STEM). The energy-loss near-edge structure in core-loss spectroscopy is often limited by core-hole lifetimes rather than the energy spread of the incident illumination. However, in the valence-loss region, the reduced width of the zero loss peak makes it possible to resolve clearly and unambiguously spectral features at very low energy-losses (photovoltaics (OPVs): poly(3-hexlythiophene) (P3HT), [6,6] phenyl-C 61 butyric acid methyl ester (PCBM), copper phthalocyanine (CuPc), and fullerene (C 60 ). Data was collected on two different monochromated instruments - a Nion UltraSTEM 100 MC 'HERMES' and a FEI Titan 3 60-300 Image-Corrected S/TEM - using energy resolutions (as defined by the zero loss peak full-width at half-maximum) of 35meV and 175meV, respectively. The data was acquired to allow deconvolution of plural scattering, and Kramers-Kronig analysis was utilized to extract the complex dielectric functions. The real and imaginary parts of the complex dielectric functions obtained from the two instruments were compared to evaluate if the enhanced resolution in the Nion provides new opto-electronic information for these organic materials. The differences between the spectra are discussed, and the implications for STEM-EELS studies of advanced materials are considered. Copyright © 2017 Elsevier B.V. All rights reserved.

  15. Angle-resolved electron energy loss spectroscopy in hexagonal boron nitride

    Science.gov (United States)

    Fossard, Frédéric; Sponza, Lorenzo; Schué, Léonard; Attaccalite, Claudio; Ducastelle, François; Barjon, Julien; Loiseau, Annick

    2017-09-01

    Electron energy loss spectra were measured on hexagonal boron nitride single crystals employing an electron energy loss spectroscopic setup composed of an electron microscope equipped with a monochromator and an in-column filter. This setup provides high-quality energy-loss spectra and allows also for the imaging of energy-filtered diffraction patterns. These two acquisition modes provide complementary pieces of information, offering a global view of excitations in reciprocal space. As an example of the capabilities of the method we show how easily the core loss spectra at the K edges of boron and nitrogen can be measured and imaged. Low losses associated with interband and/or plasmon excitations are also measured. This energy range allows us to illustrate that our method provides results whose quality is comparable to that obtained from nonresonant x-ray inelastic scattering but with advantageous specificities such as an enhanced sensitivity at low q and a much greater simplicity and versatility that make it well adapted to the study of two-dimensional materials and related heterostructures. Finally, by comparing theoretical calculations to our measures, we are able to relate the range of applicability of ab initio calculations to the anisotropy of the sample and assess the level of approximation required for a proper simulation of our acquisition method.

  16. Impact of stand-by energy losses in electronic devices on smart network performance

    Directory of Open Access Journals (Sweden)

    Mandić-Lukić Jasmina S.

    2012-01-01

    Full Text Available Limited energy resources and environmental concerns due to ever increasing energy consumption, more and more emphasis is being put on energy savings. Smart networks are promoted worldwide as a powerful tool used to improve the energy efficiency through consumption management, as well as to enable the distributed power generation, primarily based on renewable energy sources, to be optimally explored. To make it possible for the smart networks to function, a large number of electronic devices is needed to operate or to be in their stand-by mode. The consumption of these devices is added to the consumption of many other electronic devices already in use in households and offices, thus giving rise to the overall power consumption and threatening to counteract the primary function of smart networks. This paper addresses the consumption of particular electronic devices, with an emphasis placed on their thermal losses when in stand-by mode and their total share in the overall power consumption in certain countries. The thermal losses of electronic devices in their stand-by mode are usually neglected, but it seems theoretically possible that a massive increase in their number can impact net performance of the future smart networks considerably so that above an optimum level of energy savings achieved by their penetration, total consumption begins to increase. Based on the current stand-by energy losses from the existing electronic devices, we propose that the future penetration of smart networks be optimized taking also into account losses from their own electronic devices, required to operate in stand-by mode.

  17. Electron Energy-Loss Spectroscopy: Fundamentals and applications in the characterization of minerals

    International Nuclear Information System (INIS)

    Krishnan, K.M.

    1989-04-01

    The combined use of an energy-loss spectrometer and an analytical electron microscope with fine probe forming capabilities provides a wealth of information about the sample at high spatial resolution. Fundamental principles governing the physics of the interaction between the fast electron and a thin foil sample, to account for the fine structure in the inelastically scattered fast electron distribution (Electron-Energy Loss Spectroscopy, EELS), will be reviewed. General application of EELS is in the area of low atomic number elements (Z < 11) microanalysis, where it significantly complements the more widely used Energy Dispersive X-ray Spectroscopy (EDXS). However, a careful analysis of the low loss plasmon oscillations and the fine structure in the core-loss edges, can provide additional information related to the bonding and electronic structure of the sample. An illustration of this is presented from our study of Cδ diamond residue from the Allende carbonaceous chondrite. Combination of EELS with channeling effects can provide specific site occupation/valence information in crystalline materials. Details of this novel crystallographic method will be outlined and illustrated with an example of the study of chromite spinels. Finally, some pertinent experimental details will be discussed. 7 figs

  18. Some thoughts on source monochromation and the implications for electron energy loss spectroscopy

    CERN Document Server

    Brydson, R; Brown, A

    2003-01-01

    We briefly outline the factors determining the intrinsic widths of features in electron energy loss near edge structure (ELNES) measured by electron energy loss spectroscopy (EELS) in the transmission electron microscope (TEM). We have made estimates of the differing contributions of both the initial and final state lifetime effects in the ELNES ionisation processes and also show how these may be combined with the instrumental energy resolution. We discuss the potential benefits of source monochromation for ELNES measurements via a comparison of these theoretical estimates with experimental spectra from the literature. We show that for certain core level excitations, solid state broadening mechanisms may be the fundamental limiting factor for resolving fine detail in ELNES. (orig.)

  19. Electronic energy loss spectra from mono-layer to few layers of phosphorene

    International Nuclear Information System (INIS)

    Mohan, Brij; Thakur, Rajesh; Ahluwalia, P. K.

    2016-01-01

    Using first principles calculations, electronic and optical properties of few-layers phosphorene has been investigated. Electronic band structure show a moderate band gap of 0.9 eV in monolayer phosphorene which decreases with increasing number of layers. Optical properties of few-layers of phosphorene in infrared and visible region shows tunability with number of layers. Electron energy loss function has been plotted and huge red shift in plasmonic behaviours is found. These tunable electronic and optical properties of few-layers of phosphorene can be useful for the applications of optoelectronic devices.

  20. Electronic energy loss spectra from mono-layer to few layers of phosphorene

    Energy Technology Data Exchange (ETDEWEB)

    Mohan, Brij, E-mail: brijmohanhpu@yahoo.com; Thakur, Rajesh; Ahluwalia, P. K. [Department of Physics, Himachal Pradesh University, Shimla (HP) India 171005 (India)

    2016-05-23

    Using first principles calculations, electronic and optical properties of few-layers phosphorene has been investigated. Electronic band structure show a moderate band gap of 0.9 eV in monolayer phosphorene which decreases with increasing number of layers. Optical properties of few-layers of phosphorene in infrared and visible region shows tunability with number of layers. Electron energy loss function has been plotted and huge red shift in plasmonic behaviours is found. These tunable electronic and optical properties of few-layers of phosphorene can be useful for the applications of optoelectronic devices.

  1. On FEL integral equation and electron energy loss in intermediate gain regime

    International Nuclear Information System (INIS)

    Takao, Masaru

    1994-03-01

    The FEL pendulum equation in a intermediate gain small signal regime is investigated. By calculating the energy loss of the electron beam in terms of the solution of the pendulum equation, we confirm the consistency of the FEL equation in intermediate gain regime. (author)

  2. Quantification of the boron speciation in alkali borosilicate glasses by electron energy loss spectroscopy

    DEFF Research Database (Denmark)

    Cheng, D.S.; Yang, G.; Zhao, Y.Q.

    2015-01-01

    developed a method based on electron energy loss spectroscopy (EELS) data acquisition and analyses, which enables determination of the boron speciation in a series of ternary alkali borosilicate glasses with constant molar ratios. A script for the fast acquisition of EELS has been designed, from which...

  3. Spin flip inelastic scattering in electron energy loss spectroscopy of a ferromagnetic metal

    International Nuclear Information System (INIS)

    Bocchetta, C.J.; Tosatti, E.; Yin, S.

    1986-11-01

    A model ferromagnetic metal is used to calculate the spin-polarization which occurs during inelastic electron-metal scattering with the production of an electron-hole pair. The polarization is found to have contributions from unequal spin-flip as well as non-flip energy loss rates. Our results indicate an asymmetry of the order of a few percent with parameters roughly modelling iron. (author)

  4. Spin-flip inelastic scattering in electron energy loss spectroscopy of a ferromagnetic metal

    International Nuclear Information System (INIS)

    Yin, S.; Tosatti, E.

    1981-08-01

    We calculate the spin polarization occuring during electron inelastic scattering from electron-hole pairs in a model ferromagnetic metal. The polarization is found to have contributions from unequal spin flip as well as non-flip energy loss rates. Our results indicate an asymmetry of the order of a few percent with parameters roughly modeling Fsub(e). The possibilities of comparison with experiments in the presence of simultaneous spin-polarizing elastic scattering are discussed. (author)

  5. Design and performance of a spin-polarized electron energy loss spectrometer with high momentum resolution

    Energy Technology Data Exchange (ETDEWEB)

    Vasilyev, D.; Kirschner, J. [Max-Planck-Institut für Mikrostrukturphysik, Weinberg 2, 06120 Halle (Germany)

    2016-08-15

    We describe a new “complete” spin-polarized electron energy loss spectrometer comprising a spin-polarized primary electron source, an imaging electron analyzer, and a spin analyzer of the “spin-polarizing mirror” type. Unlike previous instruments, we have a high momentum resolution of less than 0.04 Å{sup −1}, at an energy resolution of 90-130 meV. Unlike all previous studies which reported rather broad featureless data in both energy and angle dependence, we find richly structured spectra depending sensitively on small changes of the primary energy, the kinetic energy after scattering, and of the angle of incidence. The key factor is the momentum resolution.

  6. Electron-energy-loss spectral library and its application to materials science

    Energy Technology Data Exchange (ETDEWEB)

    Zaluzec, N.J.

    1983-09-01

    An electron energy loss spectral library can be an invaluable tool in materials research from a fundamental as well as a practical standpoint. Although it will not alleviate all the complications associated with quantification, this type of library can help to elucidate details of spectral profiles previously found intractable. This work was supported by the US Department of Energy. The author also wishes to express his gratitude to the organizing committee for partial financial support provided to attend this meeting.

  7. Measurement of the band gap by reflection electron energy loss spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Vos, Maarten, E-mail: maarten.vos@anu.edu.au [Electronic Materials Engineering Department, Research School of Physics and Engineering, The Australian National University, Canberra 0200 (Australia); King, Sean W. [Logic Technology Development, Intel Corporation, Hillsboro, OR 97124 (United States); French, Benjamin L. [Ocotillo Materials Laboratory, Intel Corporation, Chandler, AZ 85248 (United States)

    2016-10-15

    Highlights: • Semiconductors are measured (without surface preparation) using REELS. • At low beam energies it is difficult to measure band gap due to surface impurities. • At very high energies it is difficult to measure band gap due to recoil effect. • At intermediate energies (around 5 keV) one obtains a good estimate of the band gap. - Abstract: We investigate the possibilities of measuring the band gap of a variety of semiconductors and insulators by reflection electron energy loss spectroscopy without additional surface preparation. The band gap is a bulk property, whereas reflection energy loss spectroscopy is generally considered a surface sensitive technique. By changing the energy of the incoming electrons, the degree of surface sensitivity can be varied. Here, we present case studies to determine the optimum condition for the determination of the band gap. At very large incoming electron energies recoil effects interfere with the band gap determination, whereas at very low energies surface effects are obscuring the band gap without surface preparation. Using an incoming energy of 5 keV a reasonable estimate of the band gap is obtained in most cases.

  8. Measurement of the band gap by reflection electron energy loss spectroscopy

    International Nuclear Information System (INIS)

    Vos, Maarten; King, Sean W.; French, Benjamin L.

    2016-01-01

    Highlights: • Semiconductors are measured (without surface preparation) using REELS. • At low beam energies it is difficult to measure band gap due to surface impurities. • At very high energies it is difficult to measure band gap due to recoil effect. • At intermediate energies (around 5 keV) one obtains a good estimate of the band gap. - Abstract: We investigate the possibilities of measuring the band gap of a variety of semiconductors and insulators by reflection electron energy loss spectroscopy without additional surface preparation. The band gap is a bulk property, whereas reflection energy loss spectroscopy is generally considered a surface sensitive technique. By changing the energy of the incoming electrons, the degree of surface sensitivity can be varied. Here, we present case studies to determine the optimum condition for the determination of the band gap. At very large incoming electron energies recoil effects interfere with the band gap determination, whereas at very low energies surface effects are obscuring the band gap without surface preparation. Using an incoming energy of 5 keV a reasonable estimate of the band gap is obtained in most cases.

  9. Electron emission and energy loss in grazing collisions of protons with insulator surfaces

    International Nuclear Information System (INIS)

    Gravielle, M. S.; Miraglia, J. E.; Aldazabal, I.; Arnau, A.; Ponce, V. H.; Aumayr, F.; Lederer, S.; Winter, H.

    2007-01-01

    Electron emission from LiF, KCl, and KI crystal surfaces during grazing collisions of swift protons is studied using a first-order distorted-wave formalism. Owing to the localized character of the electronic structure of these surfaces, we propose a model that allows us to describe the process as a sequence of atomic transitions from different target ions. Experimental results are presented for electron emission from LiF and KI and energy loss from KI surfaces. Calculations show reasonable agreement with these experimental data. The role played by the charge of the incident particle is also investigated

  10. Low-energy electron energy losses and inelastic mean free paths in zinc, selenium, and zinc selenide

    Energy Technology Data Exchange (ETDEWEB)

    Bourke, J.D.; Chantler, C.T., E-mail: chantler@unimelb.edu.au

    2014-10-15

    We compute low-energy optical energy loss spectra for the elemental solids zinc and selenium, and for the binary compound zinc selenide. The optical data are transformed via a constrained partial-pole algorithm to produce momentum-dependent electron energy loss spectra and electron inelastic mean free paths. This enables a comparison between the electron scattering behaviour in a compound solid and its constituent elements. Results cannot be explained by aggregation methods or commonly used universal curves, and prove that new approaches are required. Our work demonstrates new capabilities for the determination of fundamental material properties for a range of structures previously inaccessible to established theoretical models, and at energy levels inaccessible to most experimental techniques.

  11. Low-energy electron energy losses and inelastic mean free paths in zinc, selenium, and zinc selenide

    International Nuclear Information System (INIS)

    Bourke, J.D.; Chantler, C.T.

    2014-01-01

    We compute low-energy optical energy loss spectra for the elemental solids zinc and selenium, and for the binary compound zinc selenide. The optical data are transformed via a constrained partial-pole algorithm to produce momentum-dependent electron energy loss spectra and electron inelastic mean free paths. This enables a comparison between the electron scattering behaviour in a compound solid and its constituent elements. Results cannot be explained by aggregation methods or commonly used universal curves, and prove that new approaches are required. Our work demonstrates new capabilities for the determination of fundamental material properties for a range of structures previously inaccessible to established theoretical models, and at energy levels inaccessible to most experimental techniques

  12. Structural defects in multiferroic BiMnO3 studied by transmission electron microscopy and electron energy-loss spectroscopy

    International Nuclear Information System (INIS)

    Yang, H.; Chi, Z. H.; Yao, L. D.; Zhang, W.; Li, F. Y.; Jin, C. Q.; Yu, R. C.

    2006-01-01

    The multiferroic material BiMnO 3 synthesized under high pressure has been systematically studied by transmission electron microscopy and electron energy-loss spectroscopy, and some important structural defects are revealed in this multiferroic material. The frequently observed defects are characterized to be Σ3(111) twin boundaries, Ruddlesden-Popper [Acta Crystallogr. 11, 54 (1958)] antiphase boundaries, and a p p superdislocations connected with a small segment of Ruddlesden-Popper defect. These defects are present initially in the as-synthesized sample. In addition, we find that ordered voids (oxygen vacancies) are easily introduced into the multiferroic BiMnO 3 by electron-beam irradiation

  13. Defect production and subsequent effects induced by electronic energy loss of swift heavy ion

    International Nuclear Information System (INIS)

    Hou Mingdong; Liu Jie; Sun Youmei; Yin Jingmin; Yao Huijun; Duan Jinglai; Mo Dan; Zhang Ling; Chen Yanfeng; Chinese Academy of Sciences, Beijing

    2008-01-01

    Swift heavy ion in matter is one of forfront fields of nuclear physics in the world. A series of new phenomena were discovered in recent years. The history and sta- tus on the development of this field were reviewed. Electronic energy loss effects induced by swift heavy ion irradiation, such as defect production and evolution, ion latent track formation, phase transformation and anisotropy plastic deformation were introduced emphatically. A trend of future investigation was explored. (authors)

  14. Independent component analysis: A new possibility for analysing series of electron energy loss spectra

    International Nuclear Information System (INIS)

    Bonnet, Nogl; Nuzillard, Danielle

    2005-01-01

    A complementary approach is proposed for analysing series of electron energy-loss spectra that can be recorded with the spectrum-line technique, across an interface for instance. This approach, called blind source separation (BSS) or independent component analysis (ICA), complements two existing methods: the spatial difference approach and multivariate statistical analysis. The principle of the technique is presented and illustrations are given through one simulated example and one real example

  15. Deconvolution of overlapping features in electron energy-loss spectra: the determination of absolute differential cross sections for electron-impact excitation of electronic states of molecules

    International Nuclear Information System (INIS)

    Campbell, L.; Brunger, M.J.; Teubner, O.J.P.; Mojarrabi, B.

    1996-06-01

    A set of three computer programs is reported which allow for the deconvolution of overlapping molecular electronic state structure in electron energy-loss spectra, even in highly perturbed systems. This procedure enables extraction of absolute differential cross sections for electron-impact excitation of electronic states of diatomic molecules from electron energy-loss spectra. The first code in the sequence uses the Rydberg-Klein-Rees procedure to generate potential energy curves from spectroscopic constants, while the second calculates Franck-Condon factors by numerical solution of the Schroedinger equation, given the potential energy curves. The third, given these Franck-Condon factors, the previously calculated relevant energies for the vibrational levels of the respective electronic states and the experimental energy-loss spectra, extracts the differential cross sections for each state. Each program can be run independently, or the three can run in sequence to determine these cross sections from the spectroscopic constants and the experimental energy-loss spectra. The application of these programs to the specific case of electron scattering from nitric oxide (NO) is demonstrated. 25 refs., 2 tabs., 2 figs

  16. Multivariate statistical analysis of electron energy-loss spectroscopy in anisotropic materials

    International Nuclear Information System (INIS)

    Hu Xuerang; Sun Yuekui; Yuan Jun

    2008-01-01

    Recently, an expression has been developed to take into account the complex dependence of the fine structure in core-level electron energy-loss spectroscopy (EELS) in anisotropic materials on specimen orientation and spectral collection conditions [Y. Sun, J. Yuan, Phys. Rev. B 71 (2005) 125109]. One application of this expression is the development of a phenomenological theory of magic-angle electron energy-loss spectroscopy (MAEELS), which can be used to extract the isotropically averaged spectral information for materials with arbitrary anisotropy. Here we use this expression to extract not only the isotropically averaged spectral information, but also the anisotropic spectral components, without the restriction of MAEELS. The application is based on a multivariate statistical analysis of core-level EELS for anisotropic materials. To demonstrate the applicability of this approach, we have conducted a study on a set of carbon K-edge spectra of multi-wall carbon nanotube (MWCNT) acquired with energy-loss spectroscopic profiling (ELSP) technique and successfully extracted both the averaged and dichroic spectral components of the wrapped graphite-like sheets. Our result shows that this can be a practical alternative to MAEELS for the study of electronic structure of anisotropic materials, in particular for those nanostructures made of layered materials

  17. Electron Energy Loss Spectroscopy imaging of surface plasmons at the nanometer scale

    Energy Technology Data Exchange (ETDEWEB)

    Colliex, Christian, E-mail: christian.colliex@u-psud.fr; Kociak, Mathieu; Stéphan, Odile

    2016-03-15

    Since their first realization, electron microscopes have demonstrated their unique ability to map with highest spatial resolution (sub-atomic in most recent instruments) the position of atoms as a consequence of the strong scattering of the incident high energy electrons by the nuclei of the material under investigation. When interacting with the electron clouds either on atomic orbitals or delocalized over the specimen, the associated energy transfer, measured and analyzed as an energy loss (Electron Energy Loss Spectroscopy) gives access to analytical properties (atom identification, electron states symmetry and localization). In the moderate energy-loss domain (corresponding to an optical spectral domain from the infrared (IR) to the rather far ultra violet (UV), EELS spectra exhibit characteristic collective excitations of the rather-free electron gas, known as plasmons. Boundary conditions, such as surfaces and/or interfaces between metallic and dielectric media, generate localized surface charge oscillations, surface plasmons (SP), which are associated with confined electric fields. This domain of research has been extraordinarily revived over the past few years as a consequence of the burst of interest for structures and devices guiding, enhancing and controlling light at the sub-wavelength scale. The present review focuses on the study of these surface plasmons with an electron microscopy-based approach which associates spectroscopy and mapping at the level of a single and well-defined nano-object, typically at the nanometer scale i.e. much improved with respect to standard, and even near-field, optical techniques. After calling to mind some early studies, we will briefly mention a few basic aspects of the required instrumentation and associated theoretical tools to interpret the very rich data sets recorded with the latest generation of (Scanning)TEM microscopes. The following paragraphs will review in more detail the results obtained on simple planar and

  18. Electron Energy Loss Spectroscopy imaging of surface plasmons at the nanometer scale.

    Science.gov (United States)

    Colliex, Christian; Kociak, Mathieu; Stéphan, Odile

    2016-03-01

    Since their first realization, electron microscopes have demonstrated their unique ability to map with highest spatial resolution (sub-atomic in most recent instruments) the position of atoms as a consequence of the strong scattering of the incident high energy electrons by the nuclei of the material under investigation. When interacting with the electron clouds either on atomic orbitals or delocalized over the specimen, the associated energy transfer, measured and analyzed as an energy loss (Electron Energy Loss Spectroscopy) gives access to analytical properties (atom identification, electron states symmetry and localization). In the moderate energy-loss domain (corresponding to an optical spectral domain from the infrared (IR) to the rather far ultra violet (UV), EELS spectra exhibit characteristic collective excitations of the rather-free electron gas, known as plasmons. Boundary conditions, such as surfaces and/or interfaces between metallic and dielectric media, generate localized surface charge oscillations, surface plasmons (SP), which are associated with confined electric fields. This domain of research has been extraordinarily revived over the past few years as a consequence of the burst of interest for structures and devices guiding, enhancing and controlling light at the sub-wavelength scale. The present review focuses on the study of these surface plasmons with an electron microscopy-based approach which associates spectroscopy and mapping at the level of a single and well-defined nano-object, typically at the nanometer scale i.e. much improved with respect to standard, and even near-field, optical techniques. After calling to mind some early studies, we will briefly mention a few basic aspects of the required instrumentation and associated theoretical tools to interpret the very rich data sets recorded with the latest generation of (Scanning)TEM microscopes. The following paragraphs will review in more detail the results obtained on simple planar and

  19. Electron Energy Loss Spectroscopy imaging of surface plasmons at the nanometer scale

    International Nuclear Information System (INIS)

    Colliex, Christian; Kociak, Mathieu; Stéphan, Odile

    2016-01-01

    Since their first realization, electron microscopes have demonstrated their unique ability to map with highest spatial resolution (sub-atomic in most recent instruments) the position of atoms as a consequence of the strong scattering of the incident high energy electrons by the nuclei of the material under investigation. When interacting with the electron clouds either on atomic orbitals or delocalized over the specimen, the associated energy transfer, measured and analyzed as an energy loss (Electron Energy Loss Spectroscopy) gives access to analytical properties (atom identification, electron states symmetry and localization). In the moderate energy-loss domain (corresponding to an optical spectral domain from the infrared (IR) to the rather far ultra violet (UV), EELS spectra exhibit characteristic collective excitations of the rather-free electron gas, known as plasmons. Boundary conditions, such as surfaces and/or interfaces between metallic and dielectric media, generate localized surface charge oscillations, surface plasmons (SP), which are associated with confined electric fields. This domain of research has been extraordinarily revived over the past few years as a consequence of the burst of interest for structures and devices guiding, enhancing and controlling light at the sub-wavelength scale. The present review focuses on the study of these surface plasmons with an electron microscopy-based approach which associates spectroscopy and mapping at the level of a single and well-defined nano-object, typically at the nanometer scale i.e. much improved with respect to standard, and even near-field, optical techniques. After calling to mind some early studies, we will briefly mention a few basic aspects of the required instrumentation and associated theoretical tools to interpret the very rich data sets recorded with the latest generation of (Scanning)TEM microscopes. The following paragraphs will review in more detail the results obtained on simple planar and

  20. Time-of-flight electron energy loss spectroscopy using TM110 deflection cavities

    Directory of Open Access Journals (Sweden)

    W. Verhoeven

    2016-09-01

    Full Text Available We demonstrate the use of two TM110 resonant cavities to generate ultrashort electron pulses and subsequently measure electron energy losses in a time-of-flight type of setup. The method utilizes two synchronized microwave cavities separated by a drift space of 1.45 m. The setup has an energy resolution of 12 ± 2 eV FWHM at 30 keV, with an upper limit for the temporal resolution of 2.7 ± 0.4 ps. Both the time and energy resolution are currently limited by the brightness of the tungsten filament electron gun used. Through simulations, it is shown that an energy resolution of 0.95 eV and a temporal resolution of 110 fs can be achieved using an electron gun with a higher brightness. With this, a new method is provided for time-resolved electron spectroscopy without the need for elaborate laser setups or expensive magnetic spectrometers.

  1. Investigation of Deuterium Implantation into Beryllium Sample by Electron Energy Loss Spectroscopy

    Science.gov (United States)

    Afanas'ev, V. P.; Gryazev, A. S.; Kaplya, P. S.; Köppen, M.; Ridzel, O. Yu; Subbotin, N. Yu; Hansen, P.

    2017-11-01

    Quantitative analysis of hydrogen isotopes in first wall as well as in construction materials of future fusion devices plays a crucial role to understand the evolution of those materials under operation conditions. A quantitative understanding of hydrogen in materials is also an important issue for storing energy as well as for fuel cells. A combination of Electron Energy Loss Spectroscopy (EELS) and Elastic Peak Electron Spectroscopy (EPES) is presented in this study to tackle these problems of modern material research for energy production and storage. Accurate inelastic scattering background subtraction is a key part of the presented quantitative measurement of the Be/D ratio. The differential inelastic scattering cross-section is determined by the fitting procedure. The fitting procedure is based on the iterative solution of the direct problem and minimization of the residual between computed and measured spectra. This study also takes into account the difference in electron energy loss laws for surface and bulk. The inelastic scattering cross-sections for different doses of deuterium ions in beryllium substrate (5.5·1021 m-2 and 2.01·1022 m-2) were defined in a two-layered model. The analysis is carried out for the EELS spectra. Relative concentration of D atoms is defined.

  2. Radiative interaction of a focused relativistic electron beam in energy-loss spectroscopy of nanoscopic platelets

    International Nuclear Information System (INIS)

    Itskovsky, M. A.; Maniv, T.; Cohen, H.

    2008-01-01

    A quantum-mechanical scattering theory for relativistic, highly focused electron beams in the vacuum near nanoscopic platelets is presented, revealing an excitation mechanism due to the electron wave scattering from the platelet edges. Radiative electromagnetic excitations within the light cone are shown to arise, allowed by the breakdown of momentum conservation along the beam axis in the inelastic-scattering process. Calculated for metallic (silver and gold) and insulating (SiO 2 and MgO) nanoplatelets, radiative features are revealed above the main surface-plasmon-polariton peak, and dramatic enhancements in the electron-energy-loss probability at gaps of the 'classical' spectra are found. The corresponding radiation should be detectable in the vacuum far-field zone, with e beams exploited as sensitive 'tip detectors' of electronically excited nanostructures

  3. Radiative interaction of a focused relativistic electron beam in energy-loss spectroscopy of nanoscopic platelets

    Science.gov (United States)

    Itskovsky, M. A.; Cohen, H.; Maniv, T.

    2008-07-01

    A quantum-mechanical scattering theory for relativistic, highly focused electron beams in the vacuum near nanoscopic platelets is presented, revealing an excitation mechanism due to the electron wave scattering from the platelet edges. Radiative electromagnetic excitations within the light cone are shown to arise, allowed by the breakdown of momentum conservation along the beam axis in the inelastic-scattering process. Calculated for metallic (silver and gold) and insulating ( SiO2 and MgO) nanoplatelets, radiative features are revealed above the main surface-plasmon-polariton peak, and dramatic enhancements in the electron-energy-loss probability at gaps of the “classical” spectra are found. The corresponding radiation should be detectable in the vacuum far-field zone, with e beams exploited as sensitive “tip detectors” of electronically excited nanostructures.

  4. Simulation of Probe Position-Dependent Electron Energy-Loss Fine Structure

    Energy Technology Data Exchange (ETDEWEB)

    Oxley, M. P.; Kapetanakis, M. D.; Prange, Micah P.; Varela, M.; Pennycook, Stephen J.; Pantelides, Sokrates T.

    2014-03-31

    We present a theoretical framework for calculating probe-position-dependent electron energy-loss near-edge structure for the scanning transmission electron microscope by combining density functional theory with dynamical scattering theory. We show how simpler approaches to calculating near-edge structure fail to include the fundamental physics needed to understand the evolution of near-edge structure as a function of probe position and investigate the dependence of near-edge structure on probe size. It is within this framework that density functional theory should be presented, in order to ensure that variations of near-edge structure are truly due to local electronic structure and how much from the diffraction and focusing of the electron beam.

  5. Analytical modeling of electron energy loss spectroscopy of graphene: Ab initio study versus extended hydrodynamic model.

    Science.gov (United States)

    Djordjević, Tijana; Radović, Ivan; Despoja, Vito; Lyon, Keenan; Borka, Duško; Mišković, Zoran L

    2018-01-01

    We present an analytical modeling of the electron energy loss (EEL) spectroscopy data for free-standing graphene obtained by scanning transmission electron microscope. The probability density for energy loss of fast electrons traversing graphene under normal incidence is evaluated using an optical approximation based on the conductivity of graphene given in the local, i.e., frequency-dependent form derived by both a two-dimensional, two-fluid extended hydrodynamic (eHD) model and an ab initio method. We compare the results for the real and imaginary parts of the optical conductivity in graphene obtained by these two methods. The calculated probability density is directly compared with the EEL spectra from three independent experiments and we find very good agreement, especially in the case of the eHD model. Furthermore, we point out that the subtraction of the zero-loss peak from the experimental EEL spectra has a strong influence on the analytical model for the EEL spectroscopy data. Copyright © 2017 Elsevier B.V. All rights reserved.

  6. Mapping bright and dark modes in gold nanoparticle chains using electron energy loss spectroscopy.

    Science.gov (United States)

    Barrow, Steven J; Rossouw, David; Funston, Alison M; Botton, Gianluigi A; Mulvaney, Paul

    2014-07-09

    We present a scanning transmission electron microscopy-electron energy loss spectroscopy (STEM-EELS) investigation of gold nanosphere chains with lengths varying from 1 to 5 particles. We show localized EELS signals from the chains and identify energy-loss peaks arising due to l = 1, 2, 3, 4, and 5 plasmon modes through the use of EELS mapping. We also show the evolution of the energy of these modes as the length of a given chain increases, and we find that a chain containing N particles can accommodate at least N experimentally observable modes, in addition to the transverse mode. As the chain length is increased by the addition of one more gold particle to the chain, the new N + 1 mode becomes the highest energy mode, while the existing modes lower their energy and eventually asymptote as they delocalize along the chain. We also show that modes become increasingly difficult to detect with the EELS technique as l approaches N. The data are compared to numerical simulations.

  7. Effects of target electron collisions on energy loss straggling in plasmas of all degeneracies

    Energy Technology Data Exchange (ETDEWEB)

    Barriga Carrasco, Manuel D. [E.T.S.I. Industriales, Universisdad de Castilla La Mancha, Ciudad Real E13071 (Spain)]. E-mail: ManuelD.Barriga@uclm.es

    2007-07-01

    The purpose of the present paper is to describe the effects of target electron collisions on the energy loss straggling in plasmas of any degeneracy. We focus our analysis on targets that are in the limit of weakly coupled electron gases, where the random phase approximation can be applied. This type of plasmas targets has not been studied extensively, though they are very important for inertial confinement fusion. The energy loss straggling is obtained from an exact quantum mechanical evaluation, which takes into account the degeneracy of the target plasma, and later it is compared with common classical and degenerate approximations. Also we consider electron collisions in the exact quantum mechanical straggling calculation. Now the maximum straggling occurs at velocities smaller than for the calculations without considering collisions for all kinds of plasmas analyzed. The straggling remains equal or enhances for velocities less than or equal to the velocity at maximum while is slightly decreases for higher velocities. Differences are significant in all cases, that can let large errors creep on in further energy deposition and projectile range studies.

  8. Effects of target electron collisions on energy loss straggling in plasmas of all degeneracies

    International Nuclear Information System (INIS)

    Barriga Carrasco, Manuel D.

    2007-01-01

    The purpose of the present paper is to describe the effects of target electron collisions on the energy loss straggling in plasmas of any degeneracy. We focus our analysis on targets that are in the limit of weakly coupled electron gases, where the random phase approximation can be applied. This type of plasmas targets has not been studied extensively, though they are very important for inertial confinement fusion. The energy loss straggling is obtained from an exact quantum mechanical evaluation, which takes into account the degeneracy of the target plasma, and later it is compared with common classical and degenerate approximations. Also we consider electron collisions in the exact quantum mechanical straggling calculation. Now the maximum straggling occurs at velocities smaller than for the calculations without considering collisions for all kinds of plasmas analyzed. The straggling remains equal or enhances for velocities less than or equal to the velocity at maximum while is slightly decreases for higher velocities. Differences are significant in all cases, that can let large errors creep on in further energy deposition and projectile range studies

  9. Electronic energy loss of the latent track in heavy ion-irradiated polyimide

    International Nuclear Information System (INIS)

    Sun Youmei; Liu Jie; Zhang Chonghong; Wang Zhiguang; Jin Yunfan; Duan Jinglai; Song Yin

    2005-01-01

    In the interaction process of a swift heavy ion (SHI) and polymer, a latent track with radius of several nanometers appears near the ion trajectory due to the dense ionization and excitation. To describe the role of electronic energy loss (dE/dX) e , multi-layer stacks (with different dE/dX) of polyimide (PI) films were irradiated by different SHIs (1.158 GeV Fe 56 and 1.755 GeV Xe 136 ) under vacuum at room temperature. Chemical changes of modified PI films were studied by Fourier Transform Infrared (FTIR) spectroscopy. The main feature of SHI irradiation is the degradation of the functional group and creation of alkyne. The chain disruption rate of PI was investigated in the fluence range from 1 x 10 11 to 6 x 10 12 ions/cm 2 and a wider energy stopping power range (2.2 to 5.2 keV/nm for Fe 56 ions and 8.6 to 11.3 keV/nm for Xe 136 ions). Alkyne formation was observed over the electronic energy loss range of interest. Assuming the saturated track model (the damage process only occur in a cylinder of area σ), the mean degradation and alkyne formation radii in tracks were deduced for Fe and Xe ion irradiation, respectively. The results were validated by the thermal spike model and the threshold electronic energy loss of track formation S et in PI was deduced. The analysis of the irradiated PI films shows that the predictions of the thermal spike model are in qualitative agreement with the curve shape of experimental results. (authors)

  10. Electron energy loss spectroscopy of excitons in two-dimensional-semiconductors as a function of temperature

    KAUST Repository

    Tizei, Luiz H. G.; Lin, Yung-Chang; Lu, Ang-Yd; Li, Lain-Jong; Suenaga, Kazu

    2016-01-01

    We have explored the benefits of performing monochromated Electron Energy Loss Spectroscopy(EELS) in samples at cryogenic temperatures. As an example, we have observed the excitonic absorption peaks in single layer Transition Metal Dichalcogenides. These peaks appear separated by small energies due to spin orbit coupling. We have been able to distinguish the split for MoS2 below 300 K and for MoSe2 below 220 K. However, the distinction between peaks is only clear at 150 K. We have measured the change in absorption threshold between 150 K and 770 K for MoS2 and MoSe2. We discuss the effect of carbon and ice contamination in EELSspectra. The increased spectral resolution available made possible with modern monochromators in electron microscopes will require the development of stable sample holders which reaches temperatures far below that of liquid nitrogen.

  11. Electron energy loss spectroscopy of excitons in two-dimensional-semiconductors as a function of temperature

    KAUST Repository

    Tizei, Luiz H. G.

    2016-04-21

    We have explored the benefits of performing monochromated Electron Energy Loss Spectroscopy(EELS) in samples at cryogenic temperatures. As an example, we have observed the excitonic absorption peaks in single layer Transition Metal Dichalcogenides. These peaks appear separated by small energies due to spin orbit coupling. We have been able to distinguish the split for MoS2 below 300 K and for MoSe2 below 220 K. However, the distinction between peaks is only clear at 150 K. We have measured the change in absorption threshold between 150 K and 770 K for MoS2 and MoSe2. We discuss the effect of carbon and ice contamination in EELSspectra. The increased spectral resolution available made possible with modern monochromators in electron microscopes will require the development of stable sample holders which reaches temperatures far below that of liquid nitrogen.

  12. Direct observation and theory of trajectory-dependent electronic energy losses in medium-energy ion scattering.

    Science.gov (United States)

    Hentz, A; Parkinson, G S; Quinn, P D; Muñoz-Márquez, M A; Woodruff, D P; Grande, P L; Schiwietz, G; Bailey, P; Noakes, T C Q

    2009-03-06

    The energy spectrum associated with scattering of 100 keV H+ ions from the outermost few atomic layers of Cu(111) in different scattering geometries provides direct evidence of trajectory-dependent electronic energy loss. Theoretical simulations, combining standard Monte Carlo calculations of the elastic scattering trajectories with coupled-channel calculations to describe inner-shell ionization and excitation as a function of impact parameter, reproduce the effects well and provide a means for far more complete analysis of medium-energy ion scattering data.

  13. Study of semiconductor valence plasmon line shapes via electron energy-loss spectroscopy in the transmission electron microscope

    International Nuclear Information System (INIS)

    Kundmann, M.K.

    1988-11-01

    Electron energy-loss spectra of the semiconductors Si, AlAs, GaAs, InAs, InP, and Ge are examined in detail in the regime of outer-shell and plasmon energy losses (0--100eV). Particular emphasis is placed on modeling and analyzing the shapes of the bulk valence plasmon lines. A line shape model based on early work by Froehlich is derived and compared to single-scattering probability distributions extracted from the measured spectra. Model and data are found to be in excellent agreement, thus pointing the way to systematic characterization of the plasmon component of EELS spectra. The model is applied to three separate investigations. 82 refs

  14. Application of electron energy loss spectroscopy for single wall carbon nanotubes (review)

    International Nuclear Information System (INIS)

    Mittal, N.; Jain, S.; Mittal, J.

    2015-01-01

    Electron energy loss spectroscopy (EELS) is among the few techniques that are available for the characterization of modified single wall carbon nanotubes (SWCNTs) having nanometer dimensions (~1-3 nm). CNTs can be modified either by surface functionalization or coating, between bundles of nanotubes by doping, intercalation and fully or partially filling the central core. EELS is an exclusive technique for the identification, composition analysis, and crystallization studies of the chemicals and materials used for the modification of SWCNTs. The present paper serves as a compendium of research work on the application of EELS for the characterization of modified SWCNTs. (authors)

  15. Electron energy-loss spectroscopy study of NiTi shape memory alloys

    International Nuclear Information System (INIS)

    Yang, Z.Q.; Schryvers, D.

    2008-01-01

    Electron energy loss spectroscopy (EELS) investigations were carried out on NiTi shape memory alloys. The composition of lens-shaped precipitates is determined to be Ni 4 Ti 3 by model-based EELS quantification, and the Ni-depleted zone in the B2 matrix surrounding the Ni 4 Ti 3 precipitates was quantified. The Young's modulus Y m of the B2 matrix with 51 at.% Ni and the Ni 4 Ti 3 precipitates was evaluated to be about 124 and 175 GPa, respectively. The intensity of the Ni L 3 edge for the precipitate is slightly higher than that for the B2 phase

  16. Energy loss of a high charge bunched electron beam in plasma: Simulations, scaling, and accelerating wakefields

    Directory of Open Access Journals (Sweden)

    J. B. Rosenzweig

    2004-06-01

    Full Text Available The energy loss and gain of a beam in the nonlinear, “blowout” regime of the plasma wakefield accelerator, which features ultrahigh accelerating fields, linear transverse focusing forces, and nonlinear plasma motion, has been asserted, through previous observations in simulations, to scale linearly with beam charge. Additionally, from a recent analysis by Barov et al., it has been concluded that for an infinitesimally short beam, the energy loss is indeed predicted to scale linearly with beam charge for arbitrarily large beam charge. This scaling is predicted to hold despite the onset of a relativistic, nonlinear response by the plasma, when the number of beam particles occupying a cubic plasma skin depth exceeds that of plasma electrons within the same volume. This paper is intended to explore the deviations from linear energy loss using 2D particle-in-cell simulations that arise in the case of experimentally relevant finite length beams. The peak accelerating field in the plasma wave excited behind the finite-length beam is also examined, with the artifact of wave spiking adding to the apparent persistence of linear scaling of the peak field amplitude into the nonlinear regime. At large enough normalized charge, the linear scaling of both decelerating and accelerating fields collapses, with serious consequences for plasma wave excitation efficiency. Using the results of parametric particle-in-cell studies, the implications of these results for observing severe deviations from linear scaling in present and planned experiments are discussed.

  17. Quantitative nanoscale water mapping in frozen-hydrated skin by low-loss electron energy-loss spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Yakovlev, Sergey [Department of Chemical Engineering and Materials Science, Stevens Institute of Technology, Hoboken, NJ 07030 (United States); Misra, Manoj; Shi, Shanling [Unilever Research and Development, Trumbull, CT 06611 (United States); Firlar, Emre [Department of Chemical Engineering and Materials Science, Stevens Institute of Technology, Hoboken, NJ 07030 (United States); Libera, Matthew, E-mail: mlibera@stevens.edu [Department of Chemical Engineering and Materials Science, Stevens Institute of Technology, Hoboken, NJ 07030 (United States)

    2010-06-15

    Spatially resolved low-loss electron energy-loss spectroscopy (EELS) is a powerful method to quantitatively determine the water distribution in frozen-hydrated biological materials at high spatial resolution. However, hydrated tissue, particularly its hydrophilic protein-rich component, is very sensitive to electron radiation. This sensitivity has traditionally limited the achievable spatial resolution because of the relatively high noise associated with low-dose data acquisition. We show that the damage caused by high-dose data acquisition affects the accuracy of a multiple-least-squares (MLS) compositional analysis because of inaccuracies in the reference spectrum used to represent the protein. Higher spatial resolution combined with more accurate compositional analysis can be achieved if a reference spectrum is used that better represents the electron-beam-damaged protein component under frozen-hydrated conditions rather than one separately collected from dry protein under low-dose conditions. We thus introduce a method to extract the best-fitting protein reference spectrum from an experimental spectrum dataset. This method can be used when the MLS-fitting problem is sufficiently constrained so that the only unknown is the reference spectrum for the protein component. We apply this approach to map the distribution of water in cryo-sections obtained from frozen-hydrated tissue of porcine skin. The raw spectral data were collected at doses up to 10{sup 5} e/nm{sup 2} despite the fact that observable damage begins at doses as low as 10{sup 3} e/nm{sup 2}. The resulting spatial resolution of 10 nm is 5-10 times better than that in previous studies of frozen-hydrated tissue and is sufficient to resolve sub-cellular water fluctuations as well as the inter-cellular lipid-rich regions of skin where water-mediated processes are believed to play a significant role in the phenotype of keratinocytes in the stratum corneum.

  18. Quantitative nanoscale water mapping in frozen-hydrated skin by low-loss electron energy-loss spectroscopy

    International Nuclear Information System (INIS)

    Yakovlev, Sergey; Misra, Manoj; Shi, Shanling; Firlar, Emre; Libera, Matthew

    2010-01-01

    Spatially resolved low-loss electron energy-loss spectroscopy (EELS) is a powerful method to quantitatively determine the water distribution in frozen-hydrated biological materials at high spatial resolution. However, hydrated tissue, particularly its hydrophilic protein-rich component, is very sensitive to electron radiation. This sensitivity has traditionally limited the achievable spatial resolution because of the relatively high noise associated with low-dose data acquisition. We show that the damage caused by high-dose data acquisition affects the accuracy of a multiple-least-squares (MLS) compositional analysis because of inaccuracies in the reference spectrum used to represent the protein. Higher spatial resolution combined with more accurate compositional analysis can be achieved if a reference spectrum is used that better represents the electron-beam-damaged protein component under frozen-hydrated conditions rather than one separately collected from dry protein under low-dose conditions. We thus introduce a method to extract the best-fitting protein reference spectrum from an experimental spectrum dataset. This method can be used when the MLS-fitting problem is sufficiently constrained so that the only unknown is the reference spectrum for the protein component. We apply this approach to map the distribution of water in cryo-sections obtained from frozen-hydrated tissue of porcine skin. The raw spectral data were collected at doses up to 10 5 e/nm 2 despite the fact that observable damage begins at doses as low as 10 3 e/nm 2 . The resulting spatial resolution of 10 nm is 5-10 times better than that in previous studies of frozen-hydrated tissue and is sufficient to resolve sub-cellular water fluctuations as well as the inter-cellular lipid-rich regions of skin where water-mediated processes are believed to play a significant role in the phenotype of keratinocytes in the stratum corneum.

  19. Impact of potassium doping on the electronic structure of tetracene and pentacene: An electron energy-loss study

    Energy Technology Data Exchange (ETDEWEB)

    Roth, Friedrich, E-mail: Friedrich.Roth@cfel.de [Center for Free-Electron Laser Science / DESY, Notkestraße 85, D-22607 Hamburg (Germany); Knupfer, Martin, E-mail: M.Knupfer@ifw-dresden.de [IFW Dresden, P.O. Box 270116, D-01171 Dresden (Germany)

    2015-10-21

    We report the doping induced changes of the electronic structure of tetracene and pentacene probed by electron energy-loss spectroscopy in transmission. A comparison between the dynamic response of undoped and potassium-intercalated tetracene and pentacene emphasizes the appearance of a new excitation feature in the former gap upon potassium addition. Interestingly, the momentum dependency of this new excitation shows a negative dispersion. Moreover, the analysis of the C 1s and K 2p core-level excitation results in a significantly lower doping level compared to potassium doped picene, a recently discovered superconductor. Therefore, the present electronic structure investigations open a new pathway to better understand the exceptional differences between acenes and phenacene and their divergent behavior upon alkali doping.

  20. High resolution electron energy loss spectroscopy of clean and hydrogen covered Si(001) surfaces: first principles calculations.

    Science.gov (United States)

    Patterson, C H

    2012-09-07

    Surface phonons, conductivities, and loss functions are calculated for reconstructed (2×1), p(2×2) and c(4×2) clean Si(001) surfaces, and (2×1) H and D covered Si(001) surfaces. Surface conductivities perpendicular to the surface are significantly smaller than conductivities parallel to the surface. The surface loss function is compared to high resolution electron energy loss measurements. There is good agreement between calculated loss functions and experiment for H and D covered surfaces. However, agreement between experimental data from different groups and between theory and experiment is poor for clean Si(001) surfaces. Formalisms for calculating electron energy loss spectra are reviewed and the mechanism of electron energy losses to surface vibrations is discussed.

  1. Energy-filtered real- and k-space secondary and energy-loss electron imaging with Dual Emission Electron spectro-Microscope: Cs/Mo(110)

    Energy Technology Data Exchange (ETDEWEB)

    Grzelakowski, Krzysztof P., E-mail: k.grzelakowski@opticon-nanotechnology.com

    2016-05-15

    Since its introduction the importance of complementary k{sub ||}-space (LEED) and real space (LEEM) information in the investigation of surface science phenomena has been widely demonstrated over the last five decades. In this paper we report the application of a novel kind of electron spectromicroscope Dual Emission Electron spectroMicroscope (DEEM) with two independent electron optical channels for reciprocal and real space quasi-simultaneous imaging in investigation of a Cs covered Mo(110) single crystal by using the 800 eV electron beam from an “in-lens” electron gun system developed for the sample illumination. With the DEEM spectromicroscope it is possible to observe dynamic, irreversible processes at surfaces in the energy-filtered real space and in the corresponding energy-filtered k{sub ǁ}-space quasi-simultaneously in two independent imaging columns. The novel concept of the high energy electron beam sample illumination in the cathode lens based microscopes allows chemically selective imaging and analysis under laboratory conditions. - Highlights: • A novel concept of the electron sample illumination with “in-lens” e- gun is realized. • Quasi-simultaneous energy selective observation of the real- and k-space in EELS mode. • Observation of the energy filtered Auger electron diffraction at Cs atoms on Mo(110). • Energy-loss, Auger and secondary electron momentum microscopy is realized.

  2. Nanoscale probing of bandgap states on oxide particles using electron energy-loss spectroscopy.

    Science.gov (United States)

    Liu, Qianlang; March, Katia; Crozier, Peter A

    2017-07-01

    Surface and near-surface electronic states were probed with nanometer spatial resolution in MgO and TiO 2 anatase nanoparticles using ultra-high energy resolution electron energy-loss spectroscopy (EELS) coupled to a scanning transmission electron microscope (STEM). This combination allows the surface electronic structure determined with spectroscopy to be correlated with nanoparticle size, morphology, facet etc. By acquiring the spectra in aloof beam mode, radiation damage to the surface can be significantly reduced while maintaining the nanometer spatial resolution. MgO and TiO 2 showed very different bandgap features associated with the surface/sub-surface layer of the nanoparticles. Spectral simulations based on dielectric theory and density of states models showed that a plateau feature found in the pre-bandgap region in the spectra from (100) surfaces of 60nm MgO nanocubes is consistent with a thin hydroxide surface layer. The spectroscopy shows that this hydroxide species gives rise to a broad filled surface state at 1.1eV above the MgO valence band. At the surfaces of TiO 2 nanoparticles, pronounced peaks were observed in the bandgap region, which could not be well fitted to defect states. In this case, the high refractive index and large particle size may make Cherenkov or guided light modes the likely causes of the peaks. Copyright © 2016 Elsevier B.V. All rights reserved.

  3. Detection of water and its derivatives on individual nanoparticles using vibrational electron energy-loss spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Crozier, Peter A., E-mail: crozier@asu.edu [School for the Engineering of Matter, Transport and Energy, Arizona State University, 501 E. Tyler Mall, Tempe, AZ 85287-6106 (United States); Aoki, Toshihiro [LeRoy Eyring Center for Solid State Science, Arizona State University, Tempe, AZ 85287-1704 (United States); Liu, Qianlang [School for the Engineering of Matter, Transport and Energy, Arizona State University, 501 E. Tyler Mall, Tempe, AZ 85287-6106 (United States)

    2016-10-15

    Understanding the role of water, hydrate and hydroxyl species on nanoparticle surfaces and interfaces is very important in both physical and life sciences. Detecting the presence of oxygen-hydrogen species with nanometer resolution is extremely challenging at present. Here we show that the recently developed vibrational electron energy-loss spectroscopy using subnanometer focused electron beams can be employed to spectroscopically identify the local presence and variation of OH species on nanoscale surfaces. The hydrogen-oxygen fingerprint can be correlated with highly localized structural and morphological information obtained from electron imaging. Moreover, the current approach exploits the aloof beam mode of spectral acquisition which does not require direct electron irradiation of the sample thus greatly reducing beam damage to the OH bond. These findings open the door for using electron microscopy to probe local hydroxyl and hydrate species on nanoscale organic and inorganic structures. - Highlights: • High spatial resolution spectroscopic detection of water related species in nanoparticles. • Detection of OH stretch modes with vibrational EELS. • Differentiation between hydrate and hydroxide species on or on nanoparticles. • Detection of hydrate on a single 60 nm oxide nanoparticle of MgO. • Use of aloof beam EELS to minimize radiation damage.

  4. The effects of high electronic energy loss on the chemical modification of polyimide

    CERN Document Server

    SunYouMei; Jin Yun Fan; Liu Chang Long; LiuJie; Wang Zhi Guang; Zhang Qi; Zhu Zhi Yong

    2002-01-01

    In order to observe the role of electronic energy loss (dE/dX) sub e on chemical modification of polyimide (PI), the multi-layer stacks (corresponding to different dE/dX) were irradiated by different swift heavy ions (1.37 GeV Ar sup 4 sup 0 , 1.98 GeV Kr sup 8 sup 4 , 1.755 GeV Xe sup 1 sup 3 sup 6 and 2.636 GeV U sup 2 sup 3 sup 8) under vacuum and room temperature. The chemical changes of modified PI films were studied by Fourier transform infrared (FTIR) and ultraviolet/visible (UV/Vis) absorption spectroscopy. The degradation of PI was investigated in the fluence range from 1x10 sup 1 sup 0 to 5.5x10 sup 1 sup 2 ions/cm sup 2 and different electronic energy loss from 0.77 to 11.5 keV/nm. The FTIR results show the absorbance of the typical function group decrease exponentially as a function of fluence. The alkyne end group was found after irradiation and its formation radii were 5.6 and 5.9 nm corresponding to 8.8 and 11.5 keV/nm Xe irradiation respectively. UV/Vis analysis indicates the radiation induced...

  5. Mapping boron in silicon solar cells using electron energy-loss spectroscopy

    DEFF Research Database (Denmark)

    in the energies of plasmon peaks in the low loss region [5]. We use these approaches to characterize both a thick n-p junction and the 10-nm-thick p-doped layer of a working solar cell. [1] U. Kroll, C. Bucher, S. Benagli, I. Schönbächler, J. Meier, A. Shah, J. Ballutaud, A. Howling, Ch. Hollenstein, A. Büchel, M......Amorphous silicon solar cells typically consist of stacked layers deposited on plastic or metallic substrates making sample preparation for transmission electron microscopy (TEM) difficult. The amorphous silicon layer - the active part of the solar cell - is sandwiched between 10-nm-thick n- and p...... resolution using TEM is highly challenging [3]. Recently, scanning TEM (STEM) combined with electron energy-loss spectroscopy (EELS) and spherical aberration-correction has allowed the direct detection of dopant concentration of 10^20cm-3 in 65-nm-wide silicon devices [4]. Here, we prepare TEM samples...

  6. Characteristic electron energy loss spectra in SiC buried layers formed by C+ implantation into crystalline silicon

    International Nuclear Information System (INIS)

    Yan Hui; Chen Guanghua; Kwok, R.W.M.

    1998-01-01

    SiC buried layers were synthesized by a metal vapor vacuum arc ion source, with C + ions implanted into crystalline Si substrates. According to X-ray photoelectron spectroscopy, the characteristic electron energy loss spectra of the SiC buried layers were studied. It was found that the characteristic electron energy loss spectra depend on the profiles of the carbon content, and correlate well with the order of the buried layers

  7. Order enables efficient electron-hole separation at an organic heterojunction with a small energy loss

    KAUST Repository

    Menke, S. Matthew

    2018-01-12

    Donor–acceptor organic solar cells often show low open-circuit voltages (VOC) relative to their optical energy gap (Eg) that limit power conversion efficiencies to ~12%. This energy loss is partly attributed to the offset between Eg and that of intermolecular charge transfer (CT) states at the donor–acceptor interface. Here we study charge generation occurring in PIPCP:PC61BM, a system with a very low driving energy for initial charge separation (Eg−ECT ~ 50 meV) and a high internal quantum efficiency (ηIQE ~ 80%). We track the strength of the electric field generated between the separating electron-hole pair by following the transient electroabsorption optical response, and find that while localised CT states are formed rapidly (<100 fs) after photoexcitation, free charges are not generated until 5 ps after photogeneration. In PIPCP:PC61BM, electronic disorder is low (Urbach energy <27 meV) and we consider that free charge separation is able to outcompete trap-assisted non-radiative recombination of the CT state.

  8. Order enables efficient electron-hole separation at an organic heterojunction with a small energy loss

    KAUST Repository

    Menke, S. Matthew; Cheminal, Alexandre; Conaghan, Patrick; Ran, Niva A.; Greehnam, Neil C.; Bazan, Guillermo C.; Nguyen, Thuc-Quyen; Rao, Akshay; Friend, Richard H.

    2018-01-01

    Donor–acceptor organic solar cells often show low open-circuit voltages (VOC) relative to their optical energy gap (Eg) that limit power conversion efficiencies to ~12%. This energy loss is partly attributed to the offset between Eg and that of intermolecular charge transfer (CT) states at the donor–acceptor interface. Here we study charge generation occurring in PIPCP:PC61BM, a system with a very low driving energy for initial charge separation (Eg−ECT ~ 50 meV) and a high internal quantum efficiency (ηIQE ~ 80%). We track the strength of the electric field generated between the separating electron-hole pair by following the transient electroabsorption optical response, and find that while localised CT states are formed rapidly (<100 fs) after photoexcitation, free charges are not generated until 5 ps after photogeneration. In PIPCP:PC61BM, electronic disorder is low (Urbach energy <27 meV) and we consider that free charge separation is able to outcompete trap-assisted non-radiative recombination of the CT state.

  9. Nanoscale probing of bandgap states on oxide particles using electron energy-loss spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Liu, Qianlang [School for the Engineering of Matter, Transport and Energy, Arizona State University, 85287 AZ (United States); March, Katia [Laboratoire de Physique des Solides, Bâtiment 510, Université Paris-Sud, 91405 Orsay Cedex (France); Crozier, Peter A., E-mail: CROZIER@asu.edu [School for the Engineering of Matter, Transport and Energy, Arizona State University, 85287 AZ (United States)

    2017-07-15

    Surface and near-surface electronic states were probed with nanometer spatial resolution in MgO and TiO{sub 2} anatase nanoparticles using ultra-high energy resolution electron energy-loss spectroscopy (EELS) coupled to a scanning transmission electron microscope (STEM). This combination allows the surface electronic structure determined with spectroscopy to be correlated with nanoparticle size, morphology, facet etc. By acquiring the spectra in aloof beam mode, radiation damage to the surface can be significantly reduced while maintaining the nanometer spatial resolution. MgO and TiO{sub 2} showed very different bandgap features associated with the surface/sub-surface layer of the nanoparticles. Spectral simulations based on dielectric theory and density of states models showed that a plateau feature found in the pre-bandgap region in the spectra from (100) surfaces of 60 nm MgO nanocubes is consistent with a thin hydroxide surface layer. The spectroscopy shows that this hydroxide species gives rise to a broad filled surface state at 1.1 eV above the MgO valence band. At the surfaces of TiO{sub 2} nanoparticles, pronounced peaks were observed in the bandgap region, which could not be well fitted to defect states. In this case, the high refractive index and large particle size may make Cherenkov or guided light modes the likely causes of the peaks. - Highlights: • Bandgap states detected with aloof beam monochromated EELS on oxide nanoparticle surfaces. • Dielectric theory applied to simulate the spectra and interpret surface structure. • Density of states models also be employed to understand the surface electronic structure. • In MgO, one states associate with water species was found close to the valence band edge. • In anatase, two mid-gap states associated with point defects were found.

  10. Improved calculations of the electronic and nuclear energy losses for light ions penetrating H and He targets at intermediate velocities

    Energy Technology Data Exchange (ETDEWEB)

    Grande, P.L. [Rio Grande do Sul Univ., Porto Alegre, RS (Brazil). Inst. de Fisica; Schiwietz, G. [Hahn-Meitner-Institut Berlin GmbH (Germany). Dept. FD

    1994-06-01

    A review is given on the use of the coupled-channel method to calculate the electronic and nuclear energy loss of ions penetrating the matter. This first principle calculation based on an expansion of the time dependent electronic wavefunction in terms of atomic orbitals has been applied to evaluate the impact parameter dependence of the electronic energy loss, the stopping cross-section and the fluctuation is energy loss of ions colliding with H and He atoms at energies of 10 keV/amu to 500 keV/amu. The results have been compared to experimental data as well as to others existing models, local density approximation in an electron gas target, harmonic oscillator target treatment and first order plane-wave-Born approximation. (author). 63 refs, 11 figs.

  11. Temperature-dependent surface structure, composition, and electronic properties of the clean SrTiO3(111) crystal face: Low-energy-electron diffraction, Auger-electron spectroscopy, electron energy loss, and ultraviolet-photoelectron spectroscopy studies

    International Nuclear Information System (INIS)

    Lo, W.J.; Somorjai, G.A.

    1978-01-01

    Low-energy-electron diffraction, Auger-electron spectroscopy, electron-energy-loss, and ultraviolet-photoelectron spectroscopies were used to study the structure, composition, and electron energy distribution of a clean single-crystal (111) face of strontium titanate (perovskite). The dependence of the surface chemical composition on the temperature has been observed along with corresponding changes in the surface electronic properties. High-temperature Ar-ion bombardment causes an irreversible change in the surface structure, stoichiometry, and electron energy distribution. In contrast to the TiO 2 surface, there are always significant concentrations of Ti 3+ in an annealed ordered SrTiO 3 (111) surface. This stable active Ti 3+ monolayer on top of a substrate with large surface dipole potential makes SrTiO 3 superior to TiO 2 when used as a photoanode in the photoelectrochemical cell

  12. Electron energy-loss spectroscopy of single nanocrystals: mapping of tin allotropes

    Science.gov (United States)

    Roesgaard, Søren; Ramasse, Quentin; Chevallier, Jacques; Fyhn, Mogens; Julsgaard, Brian

    2018-05-01

    Using monochromated electron energy-loss spectroscopy (EELS), we are able to map different allotropes in Sn-nanocrystals embedded in Si. It is demonstrated that α-Sn and β-Sn, as well as an interface related plasmon, can be distinguished in embedded Sn-nanostructures. The EELS data is interpreted by standard non-negative matrix factorization followed by a manual Lorentzian decomposition. The decomposition allows for a more physical understanding of the EELS mapping without reducing the level of information. Extending the analysis from a reference system to smaller nanocrystals demonstrates that allotrope determination in nanoscale systems down below 5 nm is possible. Such local information proves the use of monochromated EELS mapping as a powerful technique to study nanoscale systems. This possibility enables investigation of small nanostructures that cannot be investigated through other means, allowing for a better understanding and thus leading to realizations that can result in nanomaterials with improved properties.

  13. The data acquisition system used in one-dimension multichannel fast electron energy loss spectrometer

    International Nuclear Information System (INIS)

    Jiang Weichun; Zhu Linfan; Zhang Yijun; Xu Kezuo

    2010-01-01

    It describes a data acquisition system used in one dimension multichannel fast electron energy loss spectrometer, which can work in scan acquisition mode and static acquisition mode. The timing precision of the scan mode is less than 4 μs by utilizing the gated signal generated by data acquisition card DAQ2010 and an AND logic circuit. A timer card PCI8554 is used to synchronize the data acquisition card and the personal computer. The scan voltage supply is controlled by the personal computer through the RS232 interface. The multithreading technology is used in the acquisition software in order to improve the accommodating-err ability of the acquisition system. A satisfactory test result is given. (authors)

  14. Tensor decompositions for the analysis of atomic resolution electron energy loss spectra

    Energy Technology Data Exchange (ETDEWEB)

    Spiegelberg, Jakob; Rusz, Ján [Department of Physics and Astronomy, Uppsala University, Box 516, S-751 20 Uppsala (Sweden); Pelckmans, Kristiaan [Department of Information Technology, Uppsala University, Box 337, S-751 05 Uppsala (Sweden)

    2017-04-15

    A selection of tensor decomposition techniques is presented for the detection of weak signals in electron energy loss spectroscopy (EELS) data. The focus of the analysis lies on the correct representation of the simulated spatial structure. An analysis scheme for EEL spectra combining two-dimensional and n-way decomposition methods is proposed. In particular, the performance of robust principal component analysis (ROBPCA), Tucker Decompositions using orthogonality constraints (Multilinear Singular Value Decomposition (MLSVD)) and Tucker decomposition without imposed constraints, canonical polyadic decomposition (CPD) and block term decompositions (BTD) on synthetic as well as experimental data is examined. - Highlights: • A scheme for compression and analysis of EELS or EDX data is proposed. • Several tensor decomposition techniques are presented for BSS on hyperspectral data. • Robust PCA and MLSVD are discussed for denoising of raw data.

  15. Monte Carlo Simulations of Electron Energy-Loss Spectra with the Addition of Fine Structure from Density Functional Theory Calculations.

    Science.gov (United States)

    Attarian Shandiz, Mohammad; Guinel, Maxime J-F; Ahmadi, Majid; Gauvin, Raynald

    2016-02-01

    A new approach is presented to introduce the fine structure of core-loss excitations into the electron energy-loss spectra of ionization edges by Monte Carlo simulations based on an optical oscillator model. The optical oscillator strength is refined using the calculated electron energy-loss near-edge structure by density functional theory calculations. This approach can predict the effects of multiple scattering and thickness on the fine structure of ionization edges. In addition, effects of the fitting range for background removal and the integration range under the ionization edge on signal-to-noise ratio are investigated.

  16. Joint density of states of wide-band-gap materials by electron energy loss spectroscopy

    International Nuclear Information System (INIS)

    Fan, X.D.; Peng, J.L.; Bursill, L.A.

    1998-01-01

    Kramers-Kronig analysis for parallel electron energy loss spectroscopy (PEELS) data is developed as a software package. When used with a JEOL 4000EX high-resolution transmission electron microscope (HRTEM) operating at 100 keV this allows us to obtain the dielectric function of relatively wide band gap materials with an energy resolution of approx 1.4 eV. The imaginary part of the dielectric function allows the magnitude of the band gap to be determined as well as the joint-density-of-states function. Routines for obtaining three variations of the joint-density of states function, which may be used to predict the optical and dielectric response for angle-resolved or angle-integration scattering geometries are also described. Applications are presented for diamond, aluminum nitride (AlN), quartz (SiO 2 ) and sapphire (Al 2 O 3 ). The results are compared with values of the band gap and density of states results for these materials obtained with other techniques. (authors)

  17. Direct Detection Electron Energy-Loss Spectroscopy: A Method to Push the Limits of Resolution and Sensitivity.

    Science.gov (United States)

    Hart, James L; Lang, Andrew C; Leff, Asher C; Longo, Paolo; Trevor, Colin; Twesten, Ray D; Taheri, Mitra L

    2017-08-15

    In many cases, electron counting with direct detection sensors offers improved resolution, lower noise, and higher pixel density compared to conventional, indirect detection sensors for electron microscopy applications. Direct detection technology has previously been utilized, with great success, for imaging and diffraction, but potential advantages for spectroscopy remain unexplored. Here we compare the performance of a direct detection sensor operated in counting mode and an indirect detection sensor (scintillator/fiber-optic/CCD) for electron energy-loss spectroscopy. Clear improvements in measured detective quantum efficiency and combined energy resolution/energy field-of-view are offered by counting mode direct detection, showing promise for efficient spectrum imaging, low-dose mapping of beam-sensitive specimens, trace element analysis, and time-resolved spectroscopy. Despite the limited counting rate imposed by the readout electronics, we show that both core-loss and low-loss spectral acquisition are practical. These developments will benefit biologists, chemists, physicists, and materials scientists alike.

  18. Interpolation formulas for quantities related to radiative energy-loss of electrons

    International Nuclear Information System (INIS)

    Tabata, T.; Ito, R.

    1977-01-01

    An interpolation formula is given for the quantity PHIsub(rad)/PHI(bar) that is proportional to the radiative energy-loss divided by the total energy of the incident electron. Errors caused by the formula have been checked for three sets of values of PHIsub(rad)/PHI(bar) which have been computed by Berger and Seltzer with different empirical corrections to reduce Born-approximation errors. Incident energies from 1 keV to 1000 MeV and atomic numbers of material from 1 to 92 have been considered. Values of six parameters in the formula have been determined by using Tschebyschev's criterion of approximation, and the maximum error has been found to be less than 1.9% for the intermediate set with Aiginger-Rester correction as well as for the no-correction set. A table of parameters in the case of the Aiginger-Rester set is provided for 59 elements. An interpolation formula for the Aginger-Rester correction factor is also given. (Auth.)

  19. Electronic energy states of HfSe/sub 2/ and NbSe/sub 2/ by low energy electron loss spectroscopy study

    Energy Technology Data Exchange (ETDEWEB)

    Ito, T; Iwami, M; Hiraki, A [Osaka Univ., Suita (Japan). Faculty of Engineering

    1981-06-01

    Low energy electron loss spectroscopy (ELS) study was performed on 1T-HfSe/sub 2/ (group IVB metal compound) and 2H-NbSe/sub 2/ (group VB metal compound) by using incident electron energies of 30-250 eV. From the loss data in the second derivative form, maxima in density-of-states in the conduction band of the compounds were deduced through the information on the filled core states by X-ray photoelectron spectroscopy. The conduction band of the transition-metal dichalcogenides could be divided into two parts. The results are discussed in relation to the previous work on WS/sub 2/ (group VIB metal compound), and also to proposals based on band calculations and experimental studies on the transition-metal dichalcogenides with constituent metals of group IVB, VB and VIB.

  20. Impact of stand-by energy losses in electronic devices on smart network performance

    OpenAIRE

    Mandić-Lukić Jasmina S.; Pantović Vladan S.; Vasiljević Željko S.

    2012-01-01

    Limited energy resources and environmental concerns due to ever increasing energy consumption, more and more emphasis is being put on energy savings. Smart networks are promoted worldwide as a powerful tool used to improve the energy efficiency through consumption management, as well as to enable the distributed power generation, primarily based on renewable energy sources, to be optimally explored. To make it possible for the smart networks to function, a large number of electronic dev...

  1. Characterisation of nano-structured titanium and aluminium nitride coatings by indentation, transmission electron microscopy and electron energy loss spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Girleanu, M., E-mail: maria.girleanu@uha.fr [Mecanique, Materiaux et Procedes de Fabrication, LPMT (EA CNRS 4365), Universite de Haute Alsace, 61 rue Albert Camus, F-68093 Mulhouse (France); Pac, M.-J.; Louis, P. [Mecanique, Materiaux et Procedes de Fabrication, LPMT (EA CNRS 4365), Universite de Haute Alsace, 61 rue Albert Camus, F-68093 Mulhouse (France); Ersen, O.; Werckmann, J. [Departement Structures et Interfaces, IPCMS (UMR CNRS 7504), Universite de Strasbourg, 23 rue du Loess, F-67087 Strasbourg (France); Rousselot, C. [Departement Micro Nano Sciences et Systemes, FEMTO-ST (UMR CNRS 6174), Universite de Franche-Comte, BP 71427, F-25211 Montbeliard (France); Tuilier, M.-H. [Mecanique, Materiaux et Procedes de Fabrication, LPMT (EA CNRS 4365), Universite de Haute Alsace, 61 rue Albert Camus, F-68093 Mulhouse (France)

    2011-07-01

    Titanium and aluminium nitride Ti{sub 1-x}Al{sub x}N films deposited by radiofrequency magnetron reactive sputtering onto steel substrate are examined by transmission electron microscopy over all the range of composition (x = 0, 0.5, 0.68, 0.86, 1). The deposition parameters are optimised in order to grow nitride films with low stress over all the composition range. Transmission electron microscopy cross-section images of Vickers indentation prints performed on that set of coatings show the evolution of their damage behaviour as increasing x Al content. Cubic Ti-rich nitrides consist of small grains clustered in rather large columns sliding along each other during indentation. Hexagonal Al-rich films grow in thinner columns which can be bent under the Vickers tip. Indentation tests carried out on TiN and AlN films are simulated using finite element modelling. Particular aspects of shear stresses and displacements in the coating/substrate are investigated. The growth mode and the nanostructure of two typical films, TiN and Ti{sub 0.14}Al{sub 0.86}N, are studied in detail by combining transmission electron microscopy cross-sections and plan views. Electron energy loss spectrum taken across Ti{sub 0.14}Al{sub 0.86}N film suggests that a part of nitrogen atoms is in cubic-like local environment though the lattice symmetry of Al-rich coatings is hexagonal. The poorly crystallised domains containing Ti and N atoms in cubic-like environment are obviously located in grain boundaries and afford protection of the coating against cracking.

  2. Characterisation of nano-structured titanium and aluminium nitride coatings by indentation, transmission electron microscopy and electron energy loss spectroscopy

    International Nuclear Information System (INIS)

    Girleanu, M.; Pac, M.-J.; Louis, P.; Ersen, O.; Werckmann, J.; Rousselot, C.; Tuilier, M.-H.

    2011-01-01

    Titanium and aluminium nitride Ti 1-x Al x N films deposited by radiofrequency magnetron reactive sputtering onto steel substrate are examined by transmission electron microscopy over all the range of composition (x = 0, 0.5, 0.68, 0.86, 1). The deposition parameters are optimised in order to grow nitride films with low stress over all the composition range. Transmission electron microscopy cross-section images of Vickers indentation prints performed on that set of coatings show the evolution of their damage behaviour as increasing x Al content. Cubic Ti-rich nitrides consist of small grains clustered in rather large columns sliding along each other during indentation. Hexagonal Al-rich films grow in thinner columns which can be bent under the Vickers tip. Indentation tests carried out on TiN and AlN films are simulated using finite element modelling. Particular aspects of shear stresses and displacements in the coating/substrate are investigated. The growth mode and the nanostructure of two typical films, TiN and Ti 0.14 Al 0.86 N, are studied in detail by combining transmission electron microscopy cross-sections and plan views. Electron energy loss spectrum taken across Ti 0.14 Al 0.86 N film suggests that a part of nitrogen atoms is in cubic-like local environment though the lattice symmetry of Al-rich coatings is hexagonal. The poorly crystallised domains containing Ti and N atoms in cubic-like environment are obviously located in grain boundaries and afford protection of the coating against cracking.

  3. Perturbation of the energy loss spectra for an accelerated electron beam due to the photo injector exit

    CERN Document Server

    Salah, W

    2003-01-01

    The influence of the photo-injector exit hall on the energy loss for an accelerated electron beam is investigated, by calculating the total energy transferred from the electrons to the wakefields, which are driven by the beam. The obtained energy loss is compared to those previously obtained for a 'pill-box' cavity. This comparison shows that the influence of this hall, in terms of energy loss, varies over the beam length. It is strongest in the middle of the beam and decreases towards both ends. In consequence of this perturbation, the center of the beam is displaced from its initial position during the first phase (t < 200 ps) where the exit aperture has no effect to a new equilibrium position which takes place at 200 < t < 250 ps. (author)

  4. Experimental investigation of the trapping and energy loss mechanisms of intense relativistic electron rings in hydrogen gas and plasma

    International Nuclear Information System (INIS)

    Smith, A.C. Jr.

    1977-01-01

    The results of an experimental study on the trapping and energy loss mechanisms of intense, relativistic electron rings confined in Astron-like magnetic field geometries are presented. The work is subdivided into four sections: gas trapping; average ring electron energetics; plasma trapping, and hollow-beam cusp-injection into gas and plasma. The mechanisms by which the injected beam coalesces into a current ring in the existing Cornell RECE-Berta facility are considered. To investigate the nature of ring electron energy loss mechanisms following completion of the trapping process, a diagnostic was developed utilizing multi-foil X-ray absorption spectroscopy to analyze the Bremsstrahlung generated by the electrons as they impinge upon a thin tungsten wire target suspended in the circulating current. Finally, a set of preliminary experimental results is presented in which an annular electron beam was passed through a coaxial, non-adiabatic magnetic cusp located at one end of a magnetic mirror well

  5. Electronic energy loss of low velocity H+ beams in Al, Ag, Sb, Au and Bi

    International Nuclear Information System (INIS)

    Valdes, J.E.; Martinez Tamayo, G.; Lantschner, G.H.; Eckardt, J.C.; Arista, N.R.

    1993-01-01

    The energy loss of H + ions in thin polycrystalline Al, Sb, Ag, Au and Bi films has been determined in the energy range below 10 keV. This low-energy range is of special interest to fill a lack of low-energy experimental data and test various theoretical predictions and semiempirical formulas. We find that the general theoretical prediction of a velocity-proportional dependence of energy loss does not hold for all targets studied in this work. The velocity-proportionality is better satisfied for Al, Sb and Bi, whereas a departure from such dependence is observed at lower energies for Ag and Au targets. The results obtained here are in good general agreement with nonlinear stopping power calculations based on density functional theory. Comparison with semiempirical predictions, and other experimental results are also done. (orig.)

  6. Study of real space wave functions with electron energy loss spectrometry

    Energy Technology Data Exchange (ETDEWEB)

    Löffler, S.

    2013-07-01

    In this work, new methods to study the real space wave functions of electrons in a solid using transmission electron microscopy (TEM) and electron energy loss spectrometry (EELS) are presented. To this end, the theory of both elastic and inelastic electron scattering is treated in a density-matrix formalism. In the process, the central quantities of inelastic electron scattering - the mixed dynamic form factor (MDFF) and the double differential scattering cross section (DDSCS) - are introduced. In addition to the formal theory, several approximations and simplifications, as well as their respective validities, are discussed. Furthermore, a method for diagonalizing the mixed dynamic form factor is described, which allows calculating high resolution energy filtered TEM images with unprecedented accuracy. Subsequently, several applications of the aforementioned theory to real-world examples are presented. On the one hand, the example of Silicon serves to demonstrate how the radial wave functions in the bulk can be measured; the agreement with the theoretical predictions proves to be very good. On the other hand, the determination of the wave functions' azimuthal dependence is derived. It turns out that the symmetry of the system under investigation is crucial to the success of this endeavor. With the new techniques presented here, it will be possible to measure electronic properties with atomic resolution, which can be of great importance, particularly in material science. (author) [German] In der vorliegenden Arbeit werden neue Methoden vorgestellt, mit deren Hilfe Elektronenwellenfunktionen in Festkörpern mittels Transmissionselektronenmikroskopie (TEM) und Elektronenenergieverlustspektrometrie (EELS) direkt im Realraum vermessen werden können. Zu diesem Zweck wird sowohl die Theorie der elastischen Elektronenbeugung als auch die der inelastischen Elektronenstreuung im Dichtematrixformalismus dargestellt. Dabei werden die zentralen Größen der inelastischen

  7. Internal Energy Loss of the Electrons Ejected in Neutrinoless Double Beta Decay

    International Nuclear Information System (INIS)

    Drukarev, E. G.; Amusia, M. Ya.; Chernysheva, L. V.

    2017-01-01

    The excitations of the electron shell in neutrinoless double beta decay shifts the limiting energy available for ejected electrons. We present the general equations for this shift and make computations for the decays of two nuclei—germanium and xenon. (author)

  8. Vibrational Surface Electron-Energy-Loss Spectroscopy Probes Confined Surface-Phonon Modes

    Directory of Open Access Journals (Sweden)

    Hugo Lourenço-Martins

    2017-12-01

    Full Text Available Recently, two reports [Krivanek et al. Nature (London 514, 209 (2014NATUAS0028-083610.1038/nature13870, Lagos et al. Nature (London 543, 529 (2017NATUAS0028-083610.1038/nature21699] have demonstrated the amazing possibility to probe vibrational excitations from nanoparticles with a spatial resolution much smaller than the corresponding free-space phonon wavelength using electron-energy-loss spectroscopy (EELS. While Lagos et al. evidenced a strong spatial and spectral modulation of the EELS signal over a nanoparticle, Krivanek et al. did not. Here, we show that discrepancies among different EELS experiments as well as their relation to optical near- and far-field optical experiments [Dai et al. Science 343, 1125 (2014SCIEAS0036-807510.1126/science.1246833] can be understood by introducing the concept of confined bright and dark surface phonon modes, whose density of states is probed by EELS. Such a concise formalism is the vibrational counterpart of the broadly used formalism for localized surface plasmons [Ouyang and Isaacson Philos. Mag. B 60, 481 (1989PMABDJ1364-281210.1080/13642818908205921, García de Abajo and Aizpurua Phys. Rev. B 56, 15873 (1997PRBMDO0163-182910.1103/PhysRevB.56.15873, García de Abajo and Kociak Phys. Rev. Lett. 100, 106804 (2008PRLTAO0031-900710.1103/PhysRevLett.100.106804, Boudarham and Kociak Phys. Rev. B 85, 245447 (2012PRBMDO1098-012110.1103/PhysRevB.85.245447]; it makes it straightforward to predict or interpret phenomena already known for localized surface plasmons such as environment-related energy shifts or the possibility of 3D mapping of the related surface charge densities [Collins et al. ACS Photonics 2, 1628 (2015APCHD52330-402210.1021/acsphotonics.5b00421].

  9. Time evolution of the characteristic electron energy losses spectra of the electrons scattered on polycrystal samples of Al mechanically cleaned in vacuum

    International Nuclear Information System (INIS)

    Szczesny, R.; Baranowski, A.; Beliczynski, J.

    1982-01-01

    Measurements by the reflection technique of characteristic electron energy losses (CEEL) with a primary electron beam of energy E 0 =1 keV have been carried out on polycrystal samples of Al. The sample surfaces have been mechanically cleaned in a dinamical vacuum of the order 10 -6 Tr before each measurement. The CEEL spectra have been corrected for the resolving power of the apparatus by the deconvolution method. We have ascertained that the measuring technique and elaboration data method are useful for quickly obtaining the plasmon energy loss spectrum for an investigated material. (author)

  10. Local secondary-electron emission spectra of graphite and gold surfaces obtained using the Scanning Probe Energy Loss Spectrometer (SPELS)

    International Nuclear Information System (INIS)

    Lawton, J J; Pulisciano, A; Palmer, R E

    2009-01-01

    Secondary-electron emission (SEE) spectra have been obtained with the Scanning Probe Energy Loss Spectrometer at a tip-sample distance of only 50 nm. Such short working distances are required for the best theoretical spatial resolution (<10 nm). The SEE spectra of graphite, obtained as a function of tip bias voltage, are shown to correspond to unoccupied states in the electronic band structure. The SEE spectra of thin gold films demonstrate the capability of identifying (carbonaceous) surface contamination with this technique.

  11. Local secondary-electron emission spectra of graphite and gold surfaces obtained using the Scanning Probe Energy Loss Spectrometer (SPELS)

    Energy Technology Data Exchange (ETDEWEB)

    Lawton, J J; Pulisciano, A; Palmer, R E, E-mail: R.E.Palmer@bham.ac.u [Nanoscale Physics Research Laboratory, School of Physics and Astronomy, University of Birmingham, Birmingham B15 2TT (United Kingdom)

    2009-11-25

    Secondary-electron emission (SEE) spectra have been obtained with the Scanning Probe Energy Loss Spectrometer at a tip-sample distance of only 50 nm. Such short working distances are required for the best theoretical spatial resolution (<10 nm). The SEE spectra of graphite, obtained as a function of tip bias voltage, are shown to correspond to unoccupied states in the electronic band structure. The SEE spectra of thin gold films demonstrate the capability of identifying (carbonaceous) surface contamination with this technique.

  12. Energy loss and online directional track visualization of fast electrons with the pixel detector Timepix

    Czech Academy of Sciences Publication Activity Database

    Granja, C.; Krist, Pavel; Chvátil, David; Šolc, J.; Pospíšil, S.; Jakubek, J.; Opalka, L.

    2013-01-01

    Roč. 59, DEC (2013), s. 245-261 ISSN 1350-4487 Institutional support: RVO:61389005 Keywords : interaction of radiation with matter * dE/dx detectors * particle tracking detectors * hybrid pixel detectors * active nuclear emulsion * energy loss Subject RIV: BG - Nuclear, Atomic and Molecular Physics, Colliders Impact factor: 1.140, year: 2013

  13. Interpretation of monoclinic hafnia valence electron energy-loss spectra by time-dependent density functional theory

    Science.gov (United States)

    Hung, L.; Guedj, C.; Bernier, N.; Blaise, P.; Olevano, V.; Sottile, F.

    2016-04-01

    We present the valence electron energy-loss spectrum and the dielectric function of monoclinic hafnia (m -HfO2) obtained from time-dependent density-functional theory (TDDFT) predictions and compared to energy-filtered spectroscopic imaging measurements in a high-resolution transmission-electron microscope. Fermi's golden rule density-functional theory (DFT) calculations can capture the qualitative features of the energy-loss spectrum, but we find that TDDFT, which accounts for local-field effects, provides nearly quantitative agreement with experiment. Using the DFT density of states and TDDFT dielectric functions, we characterize the excitations that result in the m -HfO2 energy-loss spectrum. The sole plasmon occurs between 13 and 16 eV, although the peaks ˜28 and above 40 eV are also due to collective excitations. We furthermore elaborate on the first-principles techniques used, their accuracy, and remaining discrepancies among spectra. More specifically, we assess the influence of Hf semicore electrons (5 p and 4 f ) on the energy-loss spectrum, and find that the inclusion of transitions from the 4 f band damps the energy-loss intensity in the region above 13 eV. We study the impact of many-body effects in a DFT framework using the adiabatic local-density approximation (ALDA) exchange-correlation kernel, as well as from a many-body perspective using "scissors operators" matched to an ab initio G W calculation to account for self-energy corrections. These results demonstrate some cancellation of errors between self-energy and excitonic effects, even for excitations from the Hf 4 f shell. We also simulate the dispersion with increasing momentum transfer for plasmon and collective excitation peaks.

  14. Quantum-size effects in the energy loss of charged particles interacting with a confined two-dimensional electron gas

    International Nuclear Information System (INIS)

    Borisov, A. G.; Juaristi, J. I.; Muino, R. Diez; Sanchez-Portal, D.; Echenique, P. M.

    2006-01-01

    Time-dependent density-functional theory is used to calculate quantum-size effects in the energy loss of antiprotons interacting with a confined two-dimensional electron gas. The antiprotons follow a trajectory normal to jellium circular clusters of variable size, crossing every cluster at its geometrical center. Analysis of the characteristic time scales that define the process is made. For high-enough velocities, the interaction time between the projectile and the target electrons is shorter than the time needed for the density excitation to travel along the cluster. The finite-size object then behaves as an infinite system, and no quantum-size effects appear in the energy loss. For small velocities, the discretization of levels in the cluster plays a role and the energy loss does depend on the system size. A comparison to results obtained using linear theory of screening is made, and the relative contributions of electron-hole pair and plasmon excitations to the total energy loss are analyzed. This comparison also allows us to show the importance of a nonlinear treatment of the screening in the interaction process

  15. Phonon spectrum of single-crystalline FeSe probed by high-resolution electron energy-loss spectroscopy

    Science.gov (United States)

    Zakeri, Khalil; Engelhardt, Tobias; Le Tacon, Matthieu; Wolf, Thomas

    2018-06-01

    Utilizing high-resolution electron energy-loss spectroscopy (HREELS) we measure the phonon frequencies of β-FeSe(001), cleaved under ultra-high vacuum conditions. At the zone center (Γ bar-point) three prominent loss features are observed at loss energies of about ≃ 20.5 and 25.6 and 40 meV. Based on the scattering selection rules we assign the observed loss features to the A1g, B1g, and A2u phonon modes of β-FeSe(001). The experimentally measured phonon frequencies do not agree with the results of density functional based calculations in which a nonmagnetic, a checkerboard or a strip antiferromagnetic order is assumed for β-FeSe(001). Our measurements suggest that, similar to the other Fe-based materials, magnetism has a profound impact on the lattice dynamics of β-FeSe(001).

  16. Electronic excitation of furfural as probed by high-resolution vacuum ultraviolet spectroscopy, electron energy loss spectroscopy, and ab initio calculations

    Science.gov (United States)

    Ferreira da Silva, F.; Lange, E.; Limão-Vieira, P.; Jones, N. C.; Hoffmann, S. V.; Hubin-Franskin, M.-J.; Delwiche, J.; Brunger, M. J.; Neves, R. F. C.; Lopes, M. C. A.; de Oliveira, E. M.; da Costa, R. F.; Varella, M. T. do N.; Bettega, M. H. F.; Blanco, F.; García, G.; Lima, M. A. P.; Jones, D. B.

    2015-10-01

    The electronic spectroscopy of isolated furfural (2-furaldehyde) in the gas phase has been investigated using high-resolution photoabsorption spectroscopy in the 3.5-10.8 eV energy-range, with absolute cross section measurements derived. Electron energy loss spectra are also measured over a range of kinematical conditions. Those energy loss spectra are used to derive differential cross sections and in turn generalised oscillator strengths. These experiments are supported by ab initio calculations in order to assign the excited states of the neutral molecule. The good agreement between the theoretical results and the measurements allows us to provide the first quantitative assignment of the electronic state spectroscopy of furfural over an extended energy range.

  17. Electronic excitation of furfural as probed by high-resolution vacuum ultraviolet spectroscopy, electron energy loss spectroscopy, and ab initio calculations

    International Nuclear Information System (INIS)

    Ferreira da Silva, F.; Lange, E.; Limão-Vieira, P.; Jones, N. C.; Hoffmann, S. V.; Hubin-Franskin, M.-J.; Delwiche, J.; Brunger, M. J.

    2015-01-01

    The electronic spectroscopy of isolated furfural (2-furaldehyde) in the gas phase has been investigated using high-resolution photoabsorption spectroscopy in the 3.5–10.8 eV energy-range, with absolute cross section measurements derived. Electron energy loss spectra are also measured over a range of kinematical conditions. Those energy loss spectra are used to derive differential cross sections and in turn generalised oscillator strengths. These experiments are supported by ab initio calculations in order to assign the excited states of the neutral molecule. The good agreement between the theoretical results and the measurements allows us to provide the first quantitative assignment of the electronic state spectroscopy of furfural over an extended energy range

  18. Electronic excitation of furfural as probed by high-resolution vacuum ultraviolet spectroscopy, electron energy loss spectroscopy, and ab initio calculations

    Energy Technology Data Exchange (ETDEWEB)

    Ferreira da Silva, F.; Lange, E. [Laboratório de Colisões Atómicas e Moleculares, CEFITEC, Departamento de Física, Faculdade de Ciências e Tecnologia, Universidade Nova de Lisboa, 2829-516 Caparica (Portugal); Limão-Vieira, P., E-mail: plimaovieira@fct.unl.pt, E-mail: michael.brunger@flinders.edu.au, E-mail: maplima@ifi.unicamp.br [Laboratório de Colisões Atómicas e Moleculares, CEFITEC, Departamento de Física, Faculdade de Ciências e Tecnologia, Universidade Nova de Lisboa, 2829-516 Caparica (Portugal); School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, South Australia 5001 (Australia); Jones, N. C.; Hoffmann, S. V. [ISA, Department of Physics and Astronomy, Aarhus University, Ny Munkegade, DK-8000 Århus C (Denmark); Hubin-Franskin, M.-J.; Delwiche, J. [Départment de Chimie, Institut de Chimie-Bât. B6C, Université de Liège, B-4000 Liège 1 (Belgium); Brunger, M. J., E-mail: plimaovieira@fct.unl.pt, E-mail: michael.brunger@flinders.edu.au, E-mail: maplima@ifi.unicamp.br [School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, South Australia 5001 (Australia); Institute of Mathematical Sciences, University of Malaya, 50603 Kuala Lumpur (Malaysia); and others

    2015-10-14

    The electronic spectroscopy of isolated furfural (2-furaldehyde) in the gas phase has been investigated using high-resolution photoabsorption spectroscopy in the 3.5–10.8 eV energy-range, with absolute cross section measurements derived. Electron energy loss spectra are also measured over a range of kinematical conditions. Those energy loss spectra are used to derive differential cross sections and in turn generalised oscillator strengths. These experiments are supported by ab initio calculations in order to assign the excited states of the neutral molecule. The good agreement between the theoretical results and the measurements allows us to provide the first quantitative assignment of the electronic state spectroscopy of furfural over an extended energy range.

  19. Vicinage effects in energy loss and electron emission during grazing scattering of heavy molecular ions from a solid surface

    International Nuclear Information System (INIS)

    Song Yuanhong; Wang Younian; Miskovic, Z.L.

    2005-01-01

    Vicinage effects in the energy loss and the electron emission spectra are studied in the presence of Coulomb explosion of swift, heavy molecular ions, during their grazing scattering from a solid surface. The dynamic response of the surface is treated by means of the dielectric theory within the specular reflection model using the plasmon pole approximation for the bulk dielectric function, whereas the angle-resolved energy spectra of the electrons emitted from the surface are obtained on the basis of the first-order, time-dependent perturbation theory. The evolution of the charge states of the constituent ions in the molecule during scattering is described by a nonequilibrium extension of the Brandt-Kitagawa model. The molecule scattering trajectories and the corresponding Coulomb explosion dynamics are evaluated for the cases of the internuclear axis being either aligned in the beam direction or randomly oriented in the directions parallel to the surface. Our calculations show that the vicinage effect in the energy loss is generally weaker for heavy molecules than for light molecules. In addition, there is clear evidence of the negative vicinage effect in both the energy loss and the energy spectra of the emitted electrons for molecular ions at lower speeds and with the axis aligned in the direction of motion

  20. Relativistic effects in the energy loss of a fast charged particle moving parallel to a two-dimensional electron gas

    Science.gov (United States)

    Mišković, Zoran L.; Akbari, Kamran; Segui, Silvina; Gervasoni, Juana L.; Arista, Néstor R.

    2018-05-01

    We present a fully relativistic formulation for the energy loss rate of a charged particle moving parallel to a sheet containing two-dimensional electron gas, allowing that its in-plane polarization may be described by different longitudinal and transverse conductivities. We apply our formulation to the case of a doped graphene layer in the terahertz range of frequencies, where excitation of the Dirac plasmon polariton (DPP) in graphene plays a major role. By using the Drude model with zero damping we evaluate the energy loss rate due to excitation of the DPP, and show that the retardation effects are important when the incident particle speed and its distance from graphene both increase. Interestingly, the retarded energy loss rate obtained in this manner may be both larger and smaller than its non-retarded counterpart for different combinations of the particle speed and distance.

  1. Evidence for CO formation in irradiated methanol and acetone: contribution of low-energy electron-energy-loss spectroscopy to γ-radiolysis

    International Nuclear Information System (INIS)

    Jay-Gerin, J.-P.; Fraser, M.-J.; Michaud, M.; Sanche, L.; Swiderek, P.; Ferradini, C.

    1997-01-01

    Energy-loss spectra for low-energy electrons incident on acetone condensed on a multilayer film of argon, and on a methanol film deposited on a metallic substrate, are reported. In both cases, the formation of carbon monoxide has been detected. These results are directly related to those obtained in the liquid-phase γ-radiolysis of the two compounds. (author)

  2. Electron Energy Loss and One- and Two-Photon Excited SERS Probing of “Hot” Plasmonic Silver Nanoaggregates

    DEFF Research Database (Denmark)

    Kadkhodazadeh, Shima; Wagner, Jakob Birkedal; Joseph, Virginia

    2013-01-01

    in an optical experiment and electron energy loss intensity at energies corresponding to excitation wavelengths used for optical probing. This inverse relation exists independent on specific nanoaggregate geometries and is mainly controlled by the gap size between the particles forming the aggregate. The ratio...... between two- and one-photon excited SERS measured at different excitation wavelengths provides information about local fields in the hottest spots and their dependence on the photon energy. Our data verify experimentally the predicted increase of local optical fields in the hot spots with increasing wave...

  3. Band gap and defect states of MgO thin films investigated using reflection electron energy loss spectroscopy

    Directory of Open Access Journals (Sweden)

    Sung Heo

    2015-07-01

    Full Text Available The band gap and defect states of MgO thin films were investigated by using reflection electron energy loss spectroscopy (REELS and high-energy resolution REELS (HR-REELS. HR-REELS with a primary electron energy of 0.3 keV revealed that the surface F center (FS energy was located at approximately 4.2 eV above the valence band maximum (VBM and the surface band gap width (EgS was approximately 6.3 eV. The bulk F center (FB energy was located approximately 4.9 eV above the VBM and the bulk band gap width was about 7.8 eV, when measured by REELS with 3 keV primary electrons. From a first-principles calculation, we confirmed that the 4.2 eV and 4.9 eV peaks were FS and FB, induced by oxygen vacancies. We also experimentally demonstrated that the HR-REELS peak height increases with increasing number of oxygen vacancies. Finally, we calculated the secondary electron emission yields (γ for various noble gases. He and Ne were not influenced by the defect states owing to their higher ionization energies, but Ar, Kr, and Xe exhibited a stronger dependence on the defect states owing to their small ionization energies.

  4. Radiation effects in nuclear materials: Role of nuclear and electronic energy losses and their synergy

    Energy Technology Data Exchange (ETDEWEB)

    Thomé, Lionel [Centre de Spectrométrie Nucléaire et de Spectrométrie de Masse, CNRS-IN2P3-Université Paris-Sud; Debelle, Aurelien [Universite Paris Sud, Orsay, France; Garrido, Frederico [Universite Paris Sud, Orsay, France; Mylonas, Stamatis [Universite Paris Sud, Orsay, France; Décamps, B. [Universite Paris Sud, Orsay, France; Bachelet, C. [Universite Paris Sud, Orsay, France; Sattonnay, G. [LEMHE/ICMMO, Université Paris-Sud, Bât. Orsay, France; Moll, Sandra [French Atomic Energy Commission (CEA), Centre de Saclay, Gif sur Yvette; Pellegrino, S. [French Atomic Energy Commission (CEA); Miro, S. [French Atomic Energy Commission (CEA); Trocellier, P. [French Atomic Energy Commission (CEA); Serruys, Y. [French Atomic Energy Commission (CEA); Velisa, G. [French Atomic Energy Commission (CEA); Grygiel, C. [CNRS, France; Monnet, I. [CIMAP, CEA-CNRS-Université de Caen, France; Toulemonde, Marcel [French Atomic Energy Commission (CEA), French National Centre for Scientific Research (CNRS)-ENSICAE; Simon, P. [CEMHTI, CNRS, France; Jagielski, Jacek [Institute for Electronic Materials Technology; Jozwik-Biala, Iwona [Institute for Electronic Materials Technology; Nowicki, Lech [Soltan Institute for Nuclear Studies, Swierk, Poland; Behar, M. [Instituto de Fisica, Universidade Federal do Rio Grande do Sul, Porto Alegre,; Weber, William J [ORNL; Zhang, Yanwen [ORNL; Backman, Marie [University of Tennessee, Knoxville (UTK); Nordlund, Kai [University of Helsinki; Djurabekova, Flyura [University of Helsinki

    2013-01-01

    Ceramic oxides and carbides are promising matrices for the immobilization and/or transmutation of nuclear wastes, cladding materials for gas-cooled fission reactors and structural components for fusion reactors. For these applications there is a need of fundamental data concerning the behavior of nuclear ceramics upon irradiation. This article is focused on the presentation of a few remarkable examples regarding ion-beam modifications of nuclear ceramics with an emphasis on the mechanisms leading to damage creation and phase transformations. Results obtained by combining advanced techniques (Rutherford backscattering spectrometry and channeling, X-ray diffraction, transmission electron microscopy, Raman spectroscopy) concern irradiations in a broad energy range (from keV to GeV) with the aim of exploring both nuclear collision (Sn) and electronic excitation (Se) regimes. Finally, the daunting challenge of the demonstration of the existence of synergistic effects between Sn and Se is tackled by discussing the healing due to intense electronic energy deposition (SHIBIEC) and by reporting results recently obtained in dual-beam irradiation (DBI) experiments.

  5. Chirality effect on electron phonon relaxation, energy loss, and thermopower in single and bilayer graphene in BG regime

    Science.gov (United States)

    Ansari, Meenhaz; Ashraf, S. S. Z.

    2017-10-01

    We investigate the energy dependent electron-phonon relaxation rate, energy loss rate, and phonon drag thermopower in single layer graphene (SLG) and bilayer graphene (BLG) under the Bloch-Gruneisen (BG) regime through coupling to acoustic phonons interacting via the Deformation potential in the Boltzmann transport equation approach. We find that the consideration of the chiral nature of electrons alters the temperature dependencies in two-dimensional structures of SLG and BLG from that shown by other conventional 2DEG system. Our investigations indicate that the BG analytical results are valid for temperatures far below the BG limit (˜TBG/4) which is in conformity with a recent experimental investigation for SLG [C. B. McKitterick et al., Phys. Rev. B 93, 075410 (2016)]. For temperatures above this renewed limit (˜TBG/4), there is observed a suppression in energy loss rate and thermo power in SLG, but enhancement is observed in relaxation rate and thermopower in BLG, while a suppression in the energy loss rate is observed in BLG. This strong nonmonotonic temperature dependence in SLG has also been experimentally observed within the BG limit [Q. Ma et al., Phys. Rev. Lett. 112, 247401 (2014)].

  6. A reverse Monte Carlo method for deriving optical constants of solids from reflection electron energy-loss spectroscopy spectra

    International Nuclear Information System (INIS)

    Da, B.; Sun, Y.; Ding, Z. J.; Mao, S. F.; Zhang, Z. M.; Jin, H.; Yoshikawa, H.; Tanuma, S.

    2013-01-01

    A reverse Monte Carlo (RMC) method is developed to obtain the energy loss function (ELF) and optical constants from a measured reflection electron energy-loss spectroscopy (REELS) spectrum by an iterative Monte Carlo (MC) simulation procedure. The method combines the simulated annealing method, i.e., a Markov chain Monte Carlo (MCMC) sampling of oscillator parameters, surface and bulk excitation weighting factors, and band gap energy, with a conventional MC simulation of electron interaction with solids, which acts as a single step of MCMC sampling in this RMC method. To examine the reliability of this method, we have verified that the output data of the dielectric function are essentially independent of the initial values of the trial parameters, which is a basic property of a MCMC method. The optical constants derived for SiO 2 in the energy loss range of 8-90 eV are in good agreement with other available data, and relevant bulk ELFs are checked by oscillator strength-sum and perfect-screening-sum rules. Our results show that the dielectric function can be obtained by the RMC method even with a wide range of initial trial parameters. The RMC method is thus a general and effective method for determining the optical properties of solids from REELS measurements.

  7. Many-Body Theory of Proton-Generated Point Defects for Losses of Electron Energy and Photons in Quantum Wells

    Science.gov (United States)

    Huang, Danhong; Iurov, Andrii; Gao, Fei; Gumbs, Godfrey; Cardimona, D. A.

    2018-02-01

    The effects of point defects on the loss of either energies of ballistic electron beams or incident photons are studied by using a many-body theory in a multi-quantum-well system. This theory includes the defect-induced vertex correction to a bare polarization function of electrons within the ladder approximation, and the intralayer and interlayer screening of defect-electron interactions is also taken into account in the random-phase approximation. The numerical results of defect effects on both energy-loss and optical-absorption spectra are presented and analyzed for various defect densities, numbers of quantum wells, and wave vectors. The diffusion-reaction equation is employed for calculating distributions of point defects in a layered structure. For completeness, the production rate for Frenkel-pair defects and their initial concentration are obtained based on atomic-level molecular-dynamics simulations. By combining the defect-effect, diffusion-reaction, and molecular-dynamics models with an available space-weather-forecast model, it will be possible in the future to enable specific designing for electronic and optoelectronic quantum devices that will be operated in space with radiation-hardening protection and, therefore, effectively extend the lifetime of these satellite onboard electronic and optoelectronic devices. Specifically, this theory can lead to a better characterization of quantum-well photodetectors not only for high quantum efficiency and low dark current density but also for radiation tolerance or mitigating the effects of the radiation.

  8. Electron energy-loss spectroscopy characterization and microwave absorption of iron-filled carbon-nitrogen nanotubes

    International Nuclear Information System (INIS)

    Che Renchao; Liang Chongyun; Shi Honglong; Zhou Xingui; Yang Xinan

    2007-01-01

    Iron-filled carbon-nitrogen (Fe/CN x ) nanotubes and iron-filled carbon (Fe/C) nanotubes were synthesized at 900 deg. C through a pyrolysis reaction of ferrocene/acetonitrile and ferrocene/xylene, respectively. The differences of structure and composition between the Fe/CN x nanotubes and Fe/C nanotubes were investigated by transmission electron microscopy and electron energy-loss spectroscopy (EELS). It was found that the morphology of Fe/CN x nanotubes is more corrugated than that of the Fe/C nanotubes due to the incorporation of nitrogen. By comparing the Fe L 2,3 electron energy-loss spectra of Fe/CN x nanotubes to those of the Fe/C nanotubes, the electron states at the interface between Fe and the tubular wall of both Fe/CN x nanotubes and Fe/C nanotubes were investigated. At the boundary between Fe and the wall of a CN x nanotube, the additional electrons contributed from the doped 'pyridinic-like' nitrogen might transfer to the empty 3d orbital of the encapsulated iron, therefore leading to an intensity suppression of the iron L 2,3 edge and an intensity enhancement of the carbon K edge. However, such an effect could not be found in Fe/C nanotubes. Microwave absorption properties of both Fe/CN x and Fe/C nanocomposites at 2-18 GHz band were studied

  9. Free electrons and ionic liquids: study of excited states by means of electron-energy loss spectroscopy and the density functional theory multireference configuration interaction method.

    Science.gov (United States)

    Regeta, Khrystyna; Bannwarth, Christoph; Grimme, Stefan; Allan, Michael

    2015-06-28

    The technique of low energy (0-30 eV) electron impact spectroscopy, originally developed for gas phase molecules, is applied to room temperature ionic liquids (IL). Electron energy loss (EEL) spectra recorded near threshold, by collecting 0-2 eV electrons, are largely continuous, assigned to excitation of a quasi-continuum of high overtones and combination vibrations of low-frequency modes. EEL spectra recorded by collecting 10 eV electrons show predominantly discrete vibrational and electronic bands. The vibrational energy-loss spectra correspond well to IR spectra except for a broadening (∼0.04 eV) caused by the liquid surroundings, and enhanced overtone activity indicating a contribution from resonant excitation mechanism. The spectra of four representative ILs were recorded in the energy range of electronic excitations and compared to density functional theory multireference configuration interaction (DFT/MRCI) calculations, with good agreement. The spectra up to about 8 eV are dominated by π-π* transitions of the aromatic cations. The lowest bands were identified as triplet states. The spectral region 2-8 eV was empty in the case of a cation without π orbitals. The EEL spectrum of a saturated solution of methylene green in an IL band showed the methylene green EEL band at 2 eV, indicating that ILs may be used as a host to study nonvolatile compounds by this technique in the future.

  10. Preliminary report on electron energy-loss measurements for CCl3, CCl2F2, CCl3F

    International Nuclear Information System (INIS)

    Bushnell, D.L. Jr.; Huebner, R.H.; Celotta, R.J.; Mielczarek, S.R.

    1975-01-01

    Currently, nation-wide research efforts are devoted to studying the possible ozone (O 3 ) depletion in the stratosphere by the chemical action of chlorine atoms released from CCl 2 F 2 or CCl 3 F upon absorption of ultraviolet radiation. Since electron-impact data taken in the forward scattering direction can be used to derive oscillator strengths and thus to yield apparent photoabsorption cross sections, such an analysis for CCl 2 F 2 , CCLl 3 F, and CClF 3 was carried out. Oscillator-strength distributions were obtained between 5 and 20 eV and are compared to available photoabsorption data. Certain photoabsorption values agree very well with these electron-impact data, but other optical studies deviate in some spectral regions by as much as a factor of 5. Also, the electron energy-loss spectrum reveals electronic transitions previously undetected by photoabsorption

  11. Electron-energy-loss and optical-transmittance investigation of Bi2Sr2CaCu2O8

    International Nuclear Information System (INIS)

    Wang, Y.; Feng, G.; Ritter, A.L.

    1990-01-01

    The energy-loss function Im(-1/ε) of Bi 2 Sr 2 CaCu 2 O 8 has been measured over the range E loss =0.8 to 80 eV by transmission electron-energy-loss spectroscopy (EELS) (nonimaging). The energy and momentum resolution were 0.1 eV and 0.04 A -1 , respectively. The low-energy spectra (E loss ≤3 eV) were studied as a function of momentum transfer (0.1 A -1 ≤q≤0.3 A -1 ). A well-defined peak in the loss function at E loss ∼1 eV is observed to disperse with momentum proportional to q 2 . This excitation is analyzed in terms of both an intracell, charge-transfer exciton model and the free-carrier (plasmon) model. The derived effective mass of the exciton m tot /m congruent 1.0 is far too small for a localized exciton. Using the free-carrier model and random-phase-approximation expressions for the dispersion coefficient, the carrier density and carrier effective mass can be determined separately. From our data and similar measurements by Nuecker et al. [Phys. Rev. B 39, 12 379 (1989)], it is found that the effective mass roughly scales with carrier density. A heuristic model is introduced based on the assumption that low-energy gaps exist in portions of the Fermi surface due to structural instabilities. The model suggests how the effective mass could appear to scale with carrier density and why a single Drude term (with frequency-independent effective mass) does not describe the mid- to far-infrared optical spectra. Finally, the optical transmittance of the EELS sample was measured and the spectra analyzed in terms of the free-carrier model

  12. Reflection electron energy loss spectroscopy as efficient technique for the determination of optical properties of polystyrene intermixed with gold nanoparticles

    Energy Technology Data Exchange (ETDEWEB)

    Deris, Jamileh [Department of Physics, Yasouj University, Yasouj 75918-74831 (Iran, Islamic Republic of); Hajati, Shaaker, E-mail: Hajati@mail.yu.ac.ir [Department of Physics, Yasouj University, Yasouj 75918-74831 (Iran, Islamic Republic of); Department of Semiconductors, Materials and Energy Research Center, Karaj 3177983634 (Iran, Islamic Republic of)

    2017-01-15

    Highlights: • Reflection Electron Energy Loss Spectroscopy of nano-metalized polymer. • Determination of real part of the dielectric function of nanostructured sample. • Determination of imaginary part of the dielectric function of nanostructured sample. • Determination of refractive index and coefficient of extinction of the sample. • Determination of reflection and absorption coefficients of nano-metalized Polymer. - Abstract: The electronic properties (electron inelastic cross section, energy loss function) of a nano-metalized polystyrene obtained by reflection electron energy loss spectroscopy (REELS) in a previous study [J. Deris, S. Hajati, S. Tougaard, V. Zaporojtchenko, Appl. Surf. Sci. 377 (2016) 44–47], which relies on the Yubero-Tougaard method, were used in the complementary application of Kramers-Kronig transformation to determine its optical properties such as the real part (ε{sub 1}) and imaginary part (ε{sub 2}) of the dielectric function (ε), refractive index (n), coefficients of extinction (k), reflection (R) and absorption (μ). The degree of intermixing of polystyrene thin film and gold nanoparticles of sizes 5.5 nm was controlled by annealing the sample to achieve a morphology in which the nanoparticles were homogeneously distributed within polystyrene. It is worth noting that no data are available on the optical properties of metalized polymers such as gold nanoparticles intermixed with polystyrene. Therefore, this work is of high importance in terms of both the sample studied here and the method applied. The advantage of the method applied here is that no information on the lateral distribution of the nanocomposite sample is required. This means that the REELS technique has been presented here to suitably, efficiently and easily obtain the optical properties of such nano-metalized polymer in which the metal nanoparticles have been vertically well distributed (homogeneous in depth). Therefore, for vertically homogeneous and

  13. Energy losses in switches

    International Nuclear Information System (INIS)

    Martin, T.H.; Seamen, J.F.; Jobe, D.O.

    1993-01-01

    The authors experiments show energy losses between 2 and 10 times that of the resistive time predictions. The experiments used hydrogen, helium, air, nitrogen, SF 6 polyethylene, and water for the switching dielectric. Previously underestimated switch losses have caused over predicting the accelerator outputs. Accurate estimation of these losses is now necessary for new high-efficiency pulsed power devices where the switching losses constitute the major portion of the total energy loss. They found that the switch energy losses scale as (V peak I peak ) 1.1846 . When using this scaling, the energy losses in any of the tested dielectrics are almost the same. This relationship is valid for several orders of magnitude and suggested a theoretical basis for these results. Currents up to .65 MA, with voltages to 3 MV were applied to various gaps during these experiments. The authors data and the developed theory indicates that the switch power loss continues for a much longer time than the resistive time, with peak power loss generally occurring at peak current in a ranging discharge instead of the early current time. All of the experiments were circuit code modeled after developing a new switch loss version based on the theory. The circuit code predicts switch energy loss and peak currents as a function of time. During analysis of the data they noticed slight constant offsets between the theory and data that depended on the dielectric. They modified the plasma conductivity for each tested dielectric to lessen this offset

  14. Quantitative analysis of reflection electron energy loss spectra to determine electronic and optical properties of Fe–Ni alloy thin films

    International Nuclear Information System (INIS)

    Tahir, Dahlang; Oh, Sukh Kun; Kang, Hee Jae; Tougaard, Sven

    2016-01-01

    Highlights: • Electronic and optical properties of Fe-Ni alloy thin films grown on Si (1 0 0) were studied via quantitative analyses of reflection electron energy loss spectra (REELS). • The energy loss functions (ELF) are dominated by a plasmon peak at 23.6 eV for Fe and moves gradually to lower energies in Fe-Ni alloys towards the bulk plasmon energy of Ni at 20.5 eV. • Fe has a strong effect on the dielectric and optical properties of Fe-Ni alloy thin films even for an alloy with 72% Ni. Electronic and optical properties of Fe-Ni alloy thin films grown on Si (1 0 0) were studied via quantitative analyses of reflection electron energy loss spectra (REELS). - Abstract: Electronic and optical properties of Fe–Ni alloy thin films grown on Si (1 0 0) by ion beam sputter deposition were studied via quantitative analyses of reflection electron energy loss spectra (REELS). The analysis was carried out by using the QUASES-XS-REELS and QUEELS-ε(k,ω)-REELS softwares to determine the energy loss function (ELF) and the dielectric functions and optical properties by analyzing the experimental spectra. For Ni, the ELF shows peaks around 3.6, 7.5, 11.7, 20.5, 27.5, 67 and 78 eV. The peak positions of the ELF for Fe_2_8Ni_7_2 are similar to those of Fe_5_1Ni_4_9, even though there is a small peak shift from 18.5 eV for Fe_5_1Ni_4_9 to 18.7 eV for Fe_2_8Ni_7_2. A plot of n, k, ε_1, and ε_2 shows that the QUEELS-ε(k,ω)-REELS software for analysis of REELS spectra is useful for the study of optical properties of transition metal alloys. For Fe–Ni alloy with high Ni concentration (Fe_2_8Ni_7_2), ε_1, and ε_2 have strong similarities with those of Fe. This indicates that the presence of Fe in the Fe–Ni alloy thin films has a strong effect.

  15. Effect of the van der Waals interaction on the electron energy-loss near edge structure theoretical calculation.

    Science.gov (United States)

    Katsukura, Hirotaka; Miyata, Tomohiro; Tomita, Kota; Mizoguchi, Teruyasu

    2017-07-01

    The effect of the van der Waals (vdW) interaction on the simulation of the electron energy-loss near edge structure (ELNES) by a first-principles band-structure calculation is reported. The effect of the vdW interaction is considered by the Tkatchenko-Scheffler scheme, and the change of the spectrum profile and the energy shift are discussed. We perform calculations on systems in the solid, liquid and gaseous states. The transition energy shifts to lower energy by approximately 0.1eV in the condensed (solid and liquid) systems by introducing the vdW effect into the calculation, whereas the energy shift in the gaseous models is negligible owing to the long intermolecular distance. We reveal that the vdW interaction exhibits a larger effect on the excited state than the ground state owing to the presence of an excited electron in the unoccupied band. Moreover, the vdW effect is found to depend on the local electron density and the molecular coordination. In addition, this study suggests that the detection of the vdW interactions exhibited within materials is possible by a very stable and high resolution observation. Copyright © 2016 Elsevier B.V. All rights reserved.

  16. Determination of the parametric region in which runaway electron energy losses are dominated by bremsstrahlung radiation in tokamaks

    International Nuclear Information System (INIS)

    Fernandez-Gomez, I.; Martin-Solis, J. R.; Sanchez, R.

    2007-01-01

    It has been recently argued that, at sufficiently large parallel electric fields, bremsstrahlung radiation can greatly reduce the maximum energy that runaway electrons can gain in tokamaks [M. Bakhtiari et al., Phys. Plasmas 12, 102503 (2005)]. In this contribution, the work of these authors is extended to show that the region where bremsstrahlung radiation dominate runaway energy losses is however more restricted than reported by them. Expressions will be provided for the limits of this region within the parameter space spanned by the background density and parallel electric field, as a function of the rest of the plasma parameters. It will be shown that the background density has to be above a certain critical value and that the parallel electric field must lie within a range of values, below and above which synchrotron radiation dominate the runaway energy losses. Finally, it will be demonstrated that typical disruption parameters lie within this region and, as a result, bremsstrahlung losses still play an important role in controlling the runaway energy

  17. Electron-beam-induced reduction of Fe3+ in iron phosphate dihydrate, ferrihydrite, haemosiderin and ferritin as revealed by electron energy-loss spectroscopy

    International Nuclear Information System (INIS)

    Pan, Ying-Hsi; Vaughan, Gareth; Brydson, Rik; Bleloch, Andrew; Gass, Mhairi; Sader, Kasim; Brown, Andy

    2010-01-01

    The effect of high-energy electron irradiation on ferritin/haemosiderin cores (in an iron-overloaded human liver biopsy), its mineral analogue; six-line ferrihydrite (6LFh), and iron phosphate dihydrate (which has similar octahedral ferric iron to oxygen coordination to that in ferrihydrite and ferritin/haemosiderin cores) has been investigated using electron energy-loss spectroscopy (EELS). Fe L 2,3 -ionisation edges were recorded on two types of electron microscope: a 200 keV transmission electron microscope (TEM) and a 100 keV scanning transmission electron microscope (STEM), in order to investigate the damage mechanisms in operation and to establish a methodology for minimum specimen alteration during analytical electron microscopic characterisation. A specimen damage mechanism dominated by radiolysis that results in the preferential loss of iron co-ordinating ligands (O, OH and H 2 O) is discussed. The net result of irradiation is structural re-organisation and reduction of iron within the iron hydroxides. At sufficiently low electron fluence and particularly in the lower incident energy, finer probe diameter STEM, the alteration is shown to be minimal. All the materials examined exhibit damage which as a function of cumulative fluence is best fitted by an inverse power-law, implying that several chemical and structural changes occur in response to the electron beam and we suggest that these are governed by secondary processes arising from the primary ionisation event. This work affirms that electron fluence and current density should be considered when measuring mixed valence ratios with EELS.

  18. Electron-beam-induced reduction of Fe{sup 3+} in iron phosphate dihydrate, ferrihydrite, haemosiderin and ferritin as revealed by electron energy-loss spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Pan, Ying-Hsi; Vaughan, Gareth; Brydson, Rik [Institute for Materials Research, SPEME, University of Leeds, Leeds LS2 9JT (United Kingdom); Bleloch, Andrew; Gass, Mhairi [SuperSTEM, Daresbury Laboratories, Warrington WA4 4AD (United Kingdom); Sader, Kasim [Institute for Materials Research, SPEME, University of Leeds, Leeds LS2 9JT (United Kingdom); SuperSTEM, Daresbury Laboratories, Warrington WA4 4AD (United Kingdom); Brown, Andy, E-mail: a.p.brown@leeds.ac.uk [Institute for Materials Research, SPEME, University of Leeds, Leeds LS2 9JT (United Kingdom)

    2010-07-15

    The effect of high-energy electron irradiation on ferritin/haemosiderin cores (in an iron-overloaded human liver biopsy), its mineral analogue; six-line ferrihydrite (6LFh), and iron phosphate dihydrate (which has similar octahedral ferric iron to oxygen coordination to that in ferrihydrite and ferritin/haemosiderin cores) has been investigated using electron energy-loss spectroscopy (EELS). Fe L{sub 2,3}-ionisation edges were recorded on two types of electron microscope: a 200 keV transmission electron microscope (TEM) and a 100 keV scanning transmission electron microscope (STEM), in order to investigate the damage mechanisms in operation and to establish a methodology for minimum specimen alteration during analytical electron microscopic characterisation. A specimen damage mechanism dominated by radiolysis that results in the preferential loss of iron co-ordinating ligands (O, OH and H{sub 2}O) is discussed. The net result of irradiation is structural re-organisation and reduction of iron within the iron hydroxides. At sufficiently low electron fluence and particularly in the lower incident energy, finer probe diameter STEM, the alteration is shown to be minimal. All the materials examined exhibit damage which as a function of cumulative fluence is best fitted by an inverse power-law, implying that several chemical and structural changes occur in response to the electron beam and we suggest that these are governed by secondary processes arising from the primary ionisation event. This work affirms that electron fluence and current density should be considered when measuring mixed valence ratios with EELS.

  19. Effect of the van der Waals interaction on the electron energy-loss near edge structure theoretical calculation

    Energy Technology Data Exchange (ETDEWEB)

    Katsukura, Hirotaka; Miyata, Tomohiro; Tomita, Kota; Mizoguchi, Teruyasu, E-mail: teru@iis.u-tokyo.ac.jp

    2017-07-15

    The effect of the van der Waals (vdW) interaction on the simulation of the electron energy-loss near edge structure (ELNES) by a first-principles band-structure calculation is reported. The effect of the vdW interaction is considered by the Tkatchenko-Scheffler scheme, and the change of the spectrum profile and the energy shift are discussed. We perform calculations on systems in the solid, liquid and gaseous states. The transition energy shifts to lower energy by approximately 0.1 eV in the condensed (solid and liquid) systems by introducing the vdW effect into the calculation, whereas the energy shift in the gaseous models is negligible owing to the long intermolecular distance. We reveal that the vdW interaction exhibits a larger effect on the excited state than the ground state owing to the presence of an excited electron in the unoccupied band. Moreover, the vdW effect is found to depend on the local electron density and the molecular coordination. In addition, this study suggests that the detection of the vdW interactions exhibited within materials is possible by a very stable and high resolution observation. - Highlights: • Effect of van der Waals (vdW) interaction in ELNES calculation is investigated. • The vdW interaction influences more to the excited state owing to the presence of excited electron. • The vdW interaction makes spectral shift to lower energy side by 0.1–0.01 eV. • The vdW interaction is negligible in gaseous materials due to long intermolecular distance.

  20. Identification of hydrogen and deuterium at the surface of water ice by reflection electron energy loss spectroscopy

    International Nuclear Information System (INIS)

    Yubero, F.; Toekesi, K.

    2009-01-01

    Complete text of publication follows. The study of elastically backscattered electrons from surfaces by reflection electron energy loss spectroscopy (REELS) has been recently recommended as an alternative technique to quantify the H content at the surface of a-C:H and polymer samples. This analysis is based on the fact that the energy loss of the incident electrons due to the recoil effect depends on the atomic mass of the particular atom present at the surface. The observed difference in recoil energies between H and O atoms (about 2 eV for 1.5 keV primary electrons) can be easily measured with standard electron spectrometers used in surface analysis. In this paper we go one step forward to explore if, with the same experimental approach, it is possible to differentiate between hydrogen and deuterium (D) in the surface region of a sample. This capability could be important for technological fields such as surface functionalization, where it is desired to distinguish between H and D at surfaces after interaction with labeled compounds. We have chosen normal and deuterated water as test labeled compounds because this polar molecule is of key importance in numerous surface reactions. It has been shown that H and D can be easily distinguished at the surface of water ice [4] using standard REELS measurements with 1000 - 1650 eV primary-electron energies, i.e., a surface analytical technique. Differences in recoil energies of the O - H and O - D atom pairs present in H 2 O and D 2 O have been found to agree with MC simulations (see Fig.1). There are many possible applications of H and D detection by REELS. Among many others, this study opens the possibility of nondestructive studies of deuterium-labeled atoms present or adsorbed on surfaces. For example, studies of H incorporation into a polymer or carbonbased surface after plasma activation with gas mixtures with several labeled molecules containing H atoms. Acknowledgements F.Y. thanks the Spanish Ministry of Science

  1. Studying substrate effects on localized surface plasmons in an individual silver nanoparticle using electron energy-loss spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Fujiyoshi, Yoshifumi; Nemoto, Takashi; Kurata, Hiroki, E-mail: kurata@eels.kuicr.kyoto-u.ac.jp

    2017-04-15

    In this study, electron energy-loss spectroscopy (EELS) in conjunction with scanning transmission electron microscopy (STEM) was used to investigate surface plasmons in a single silver nanoparticle (NP) on a magnesium oxide substrate, employing an incident electron trajectory parallel to the substrate surface. This parallel irradiation allowed a direct exploration of the substrate effects on localized surface plasmon (LSP) excitations as a function of the distance from the substrate. The presence of the substrate was found to lower the symmetry of the system, such that the resonance energies of LSPs were dependent on the polarization direction relative to the substrate surface. The resulting mode splitting could be detected by applying different electron trajectories, providing results similar to those previously obtained from optical studies using polarized light. However, the LSP maps obtained by STEM-EELS analysis show an asymmetric intensity distribution with the highest intensity at the top surface of the NP (that is, far from the substrate), a result that is not predicted by optical simulations. We show that modifications of the applied electric field by the substrate cause this asymmetric intensity distribution in the LSP maps.

  2. Tracking of boron-labelled monoclonal antibodies by energy loss spectroscopy in the electron microscope: a preliminary report

    International Nuclear Information System (INIS)

    Moore, D.E.; Dawes, A.L.; Chandler, A.K.; Bradstock, K.F.

    1990-01-01

    A technique is being developed, based on electron energy loss spectroscopy in the transmission electron microscope, whereby the binding of monoclonal antibodies to their specific receptors and any subsequent movement or endocytosis can be studied in cell culture. The method requires that antibodies be labelled with a low atomic number element, such as boron. Two procedures have been established enabling up to 1200 boron atoms to be attached per antibody molecule without affecting the immunoreactivity. In the first method, dodecaborane cages are attached to polyornithine bridging molecules which in turn are covalently bound to the antibody using a photosensitive reagent. The second technique makes use of the extremely high biotin-avidin affinity by attaching biotin to the antibody and dodecaborane cages to avidin before mixing the two components. 13 refs., 2 figs

  3. The uniformity study of non-oxide thin film at device level using electron energy loss spectroscopy

    Science.gov (United States)

    Li, Zhi-Peng; Zheng, Yuankai; Li, Shaoping; Wang, Haifeng

    2018-05-01

    Electron energy loss spectroscopy (EELS) has been widely used as a chemical analysis technique to characterize materials chemical properties, such as element valence states, atoms/ions bonding environment. This study provides a new method to characterize physical properties (i.e., film uniformity, grain orientations) of non-oxide thin films in the magnetic device by using EELS microanalysis on scanning transmission electron microscope. This method is based on analyzing white line ratio of spectra and related extended energy loss fine structures so as to correlate it with thin film uniformity. This new approach can provide an effective and sensitive method to monitor/characterize thin film quality (i.e., uniformity) at atomic level for thin film development, which is especially useful for examining ultra-thin films (i.e., several nanometers) or embedded films in devices for industry applications. More importantly, this technique enables development of quantitative characterization of thin film uniformity and it would be a remarkably useful technique for examining various types of devices for industrial applications.

  4. Direct characterization of the energy level alignments and molecular components in an organic hetero-junction by integrated photoemission spectroscopy and reflection electron energy loss spectroscopy analysis.

    Science.gov (United States)

    Yun, Dong-Jin; Shin, Weon-Ho; Bulliard, Xavier; Park, Jong Hwan; Kim, Seyun; Chung, Jae Gwan; Kim, Yongsu; Heo, Sung; Kim, Seong Heon

    2016-08-26

    A novel, direct method for the characterization of the energy level alignments at bulk-heterojunction (BHJ)/electrode interfaces on the basis of electronic spectroscopy measurements is proposed. The home-made in situ photoemission system is used to perform x-ray/ultraviolet photoemission spectroscopy (XPS/UPS), reflection electron energy loss spectroscopy (REELS) and inverse photoemission spectroscopy of organic-semiconductors (OSCs) deposited onto a Au substrate. Through this analysis system, we are able to obtain the electronic structures of a boron subphthalocyanine chloride:fullerene (SubPC:C60) BHJ and those of the separate OSC/electrode structures (SubPC/Au and C60/Au). Morphology and chemical composition analyses confirm that the original SubPC and C60 electronic structures remain unchanged in the electrodes prepared. Using this technique, we ascertain that the position and area of the nearest peak to the Fermi energy (EF = 0 eV) in the UPS (REELS) spectra of SubPC:C60 BHJ provide information on the highest occupied molecular orbital level (optical band gap) and combination ratio of the materials, respectively. Thus, extracting the adjusted spectrum from the corresponding SubPC:C60 BHJ UPS (REELS) spectrum reveals its electronic structure, equivalent to that of the C60 materials. This novel analytical approach allows complete energy-level determination for each combination ratio by separating its electronic structure information from the BHJ spectrum.

  5. High-resolution electron-energy-loss spectroscopy studies of clean and hydrogen-covered tungsten (100) surfaces

    International Nuclear Information System (INIS)

    Woods, J.P.

    1986-01-01

    High-resolution (10-meV FWHM) low-energy (≤ 100eV) electrons are scattered from the tungsten (100) surface. Electron-energy-loss spectroscopy (EELS) selection rules are utilized to identify vibrational modes of the surface tungsten atoms. A 36-meV mode is measured on the c(2 X 2) thermally reconstructed surface and is modeled as an overtone of the 18-meV mode at M in the surface Brillouin zone. The superstructure of the reconstructed surface allows this mode to be observed in specular scattering. The surface tungsten atoms return to their bulk lateral positions with saturated hydrogen (β 1 phase) adsorption; and a 26-meV mode identified is due to the perpendicular vibration of the surface tungsten layers. The clean-room temperature surface does not display either low-energy vibrations and the surface is modeled as disordered. The three β 1 phase hydrogen vibrations are observed and a new vibration at 118 meV is identified. The 118-meV cross section displays characteristics of a parallel mode, but calculations show this assignment to be erroneous. There are two hydrogen atoms for each surface tungsten atom in the β 1 phase, and lattice-dynamical calculations show that the 118-meV mode is due to a hydrogen-zone edge vibration. The predicted breakdown of the parallel hydrogen vibration selection rule was not observed

  6. Multiple scattering in electron fluid and energy loss in multi-ionic targets

    Energy Technology Data Exchange (ETDEWEB)

    Deutsch, C., E-mail: claude.deutsch@u-psud.fr [LPGP, UParis-Sud, 91405-Orsay (France); Tahir, N.A. [GSI, 1Planck Str., 64291-Darmstadt (Germany); Barriga-Carrasco, M. [ETSII, UCastilla-la-Mancha, 13071 Ciudad-Real (Spain); Ceban, V. [LPGP, UParis-Sud, 91405-Orsay (France); Fromy, P. [CRI, UParis-Sud, 91405-Orsay (France); Gilles, D. [CEA/Saclay/DSM/IRFU/SAP, 91191-Gif-s-Yvette (France); Leger, D. [Laboratoire Monthouy, UValenciennes-Hainaut Cambresis (France); Maynard, G. [LPGP, UParis-Sud, 91405-Orsay (France); Tashev, B. [Department of Physics, KazNu, Tole Bi82, Almaty (Kazakhstan); Volpe, L. [Department of Physics, UMilano-Bicocca, Milano 20126 (Italy)

    2014-01-01

    Extensions of the standard stopping model (SSM) for ion projectiles interacting with dense targets of timely concern for ICF and WDM are reviewed. They include multiple scattering on partially degenerate electrons, low velocity ion slowing down in demixing H–He mixtures within Jovian planets core or multiionic target such as Kapton.

  7. Multiple scattering in electron fluid and energy loss in multi-ionic targets

    International Nuclear Information System (INIS)

    Deutsch, C.; Tahir, N.A.; Barriga-Carrasco, M.; Ceban, V.; Fromy, P.; Gilles, D.; Leger, D.; Maynard, G.; Tashev, B.; Volpe, L.

    2014-01-01

    Extensions of the standard stopping model (SSM) for ion projectiles interacting with dense targets of timely concern for ICF and WDM are reviewed. They include multiple scattering on partially degenerate electrons, low velocity ion slowing down in demixing H–He mixtures within Jovian planets core or multiionic target such as Kapton

  8. Energy-loss magnetic chiral dichroism (EMCD): magnetic chiral dichroism in the electron microscope

    Czech Academy of Sciences Publication Activity Database

    Rubino, S.; Schattschneider, P.; Stöger-Pollach, M.; Hébert, S.; Rusz, Ján; Calmels, L.; Warot-Fonrose, B.; Houdellier, F.; Serin, V.; Novák, Pavel

    2008-01-01

    Roč. 23, č. 10 (2008), s. 2582-2590 ISSN 0884-2914 EU Projects: European Commission(XE) 508971 - CHIRALTEM Institutional research plan: CEZ:AV0Z10100521 Keywords : magnetic circular dichroism * transmission electron microscopy Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.743, year: 2008

  9. Quantitative analysis with electron energy-loss: spectroscopic imaging and its application in pathology

    NARCIS (Netherlands)

    A.L.D. Beckers (Guus)

    1995-01-01

    textabstractAfter the invention of the transmission electron microscope (TEM) in 1931 by Ruska and Knoll, it took about 20 years to develop the inslmment into a tool for ultrastructural research. In material science this led to the ability to visualize and investigate atomic arrangements through the

  10. The effects of electron transfer on the energy loss of slow He2+, C2+, and C4+ ions penetrating a graphene fragment

    International Nuclear Information System (INIS)

    Mao, Fei; Zhang, Chao; Gao, Cong-Zhang; Dai, Jinxia; Zhang, Feng-Shou

    2014-01-01

    Electronic energy loss in the collision processes of slow ions with a graphene fragment is investigated by combining ab initio time-dependent density functional theory calculations for electrons with molecular dynamics simulations for ions in real time and real space. We study the electronic energy loss of slow He 2+ , C 2+ , and C 4+ ions penetrating the graphene fragment as a function of the ion velocity, and establish the velocity-proportional energy loss for low-charged ions down to 0.1 a.u. One mechanism clarified in the simulations for electron transfer is polarization capture, which is effective for bare ions at low velocities. The other one is resonance capture, by which the incident ion can capture electrons from the graphene fragment to its electron affinity levels, which have the same, or nearly the same, energy as those of the electron donor levels. The results demonstrate that the nonlinear behavior of energy loss of C 4+ is attributed to the large number of electrons captured by this multi-charged ion during the collision. (paper)

  11. Far-field interaction of focused relativistic electron beams in electron energy loss spectroscopy of nanoscopic platelets

    OpenAIRE

    Itskovsky, M. A.; Cohen, H.; Maniv, T.

    2008-01-01

    A quantum mechanical scattering theory for relativistic, highly focused electron beams near nanoscopic platelets is presented, revealing a new excitation mechanism due to the electron wave scattering from the platelet edges. Radiative electromagnetic excitations within the light cone are shown to arise, allowed by the breakdown of momentum conservation along the beam axis in the inelastic scattering process. Calculated for metallic (silver and gold) and insulating (SiO2 and MgO) nanoplatelets...

  12. Plasmonic nanoengineering in hollow metal nanostructures: an electron energy-loss spectroscopy study

    OpenAIRE

    Genç, Aziz; Universitat Autònoma de Barcelona. Departament de Física

    2015-01-01

    Resumen en Español Las nanoestructuras metálicas están siendo objeto de gran atención dada su capacidad para generar resonancias plasmónicas, que son oscilaciones colectivas de electrones alojados en la banda de conducción en un metal excitado por efecto de un campo electromagnético. El creciente interés entorno a las nanoestructuras metálicas como fuentes de plasmones, ha resultado en el desarrollo de un nuevo campo, la plasmónica, definida como la ciencia y tecnología de la generación, cont...

  13. Energy loss of pions and electrons of 1 to 6 GeV/c in drift chambers operated with Xe,CO2(15\\%)

    CERN Document Server

    Andronic, A; Braun-Munzinger, P; Bucher, D; Busch, O; Catanescu, V; Ciobanu, M; Daues, H W; Emschermann, D; Fateev, O V; Foka, Y; Garabatos, C; Gunji, T; Herrmann, N; Inuzuka, M; Kislov, E; Lindenstruth, V; Ludolphs, W; Mahmoud, T; Petracek, V; Petrovici, M; Rusanov, I R; Sandoval, A; Santo, R; Schicker, R; Simon, R S; Smykov, L P; Soltveit, H K; Stachel, J; Stelzer, H; Tsiledakis, G; Vulpescu, B; Wessels, J P; Windelband, B; Xu, C; Zaudtke, O; Zanevsky, Yu; Yurevich, V

    2004-01-01

    We present measurements of the energy loss of pions and electrons in drift chambers operated with a Xe,CO2(15%) mixture. The measurements are carried out for particle momenta from 1 to 6 GeV/c using prototype drift chambers for the ALICE TRD. Microscopic calculations are performed using input parameters calculated with GEANT3. These calculations reproduce well the measured average and most probable values for pions, but a higher Fermi plateau is required in order to reproduce our electron data. The widths of the measured distributions are smaller for data compared to the calculations. The electron/pion identification performance using the energy loss is also presented.

  14. Electron-beam induced amorphization of stishovite: Silicon-coordination change observed using Si K-edge extended electron energy-loss fine structure

    Science.gov (United States)

    van Aken, P. A.; Sharp, T. G.; Seifert, F.

    The analysis of the extended energy-loss fine structure (EXELFS) of the Si K-edge for sixfold-coordinated Si in synthetic stishovite and fourfold-coordinated Si in natural α-quartz is reported by using electron energy-loss spectroscopy (EELS) in combination with transmission electron microscopy (TEM). The stishovite Si K-edge EXELFS spectra were measured as a time-dependent series to document irradiation-induced amorphization. The amorphization was also investigated through the change in Si K- and O K-edge energy-loss near edge structure (ELNES). For α-quartz, in contrast to stishovite, electron irradiation-induced vitrification, verified by selected area electron diffraction (SAED), produced no detectable changes of the EXELFS. The Si K-edge EXELFS were analysed with the classical extended X-ray absorption fine structure (EXAFS) treatment and compared to ab initio curve-waved multiple-scattering (MS) calculations of EXAFS spectra for stishovite and α-quartz. Highly accurate information on the local atomic environment of the silicon atoms during the irradiation-induced amorphization of stishovite is obtained from the EXELFS structure parameters (Si-O bond distances, coordination numbers and Debye-Waller factors). The mean Si-O bond distance R and mean Si coordination number N changes from R=0.1775 nm and N=6 for stishovite through a disordered intermediate state (R 0.172 nm and N 5) to R 0.167 nm and N 4.5 for a nearly amorphous state similar to α-quartz (R=0.1609 nm and N=4). During the amorphization process, the Debye-Waller factor (DWF) passes through a maximum value of as it changes from for sixfold to for fourfold coordination of Si. This increase in Debye-Waller factor indicates an increase in mean-square relative displacement (MSRD) between the central silicon atom and its oxygen neighbours that is consistent with the presence of an intermediate structural state with fivefold coordination of Si. The distribution of coordination states can be estimated by

  15. Fluctuating Charge-Order in Optimally Doped Bi- 2212 Revealed by Momentum-resolved Electron Energy Loss Spectroscopy

    Science.gov (United States)

    Husain, Ali; Vig, Sean; Kogar, Anshul; Mishra, Vivek; Rak, Melinda; Mitrano, Matteo; Johnson, Peter; Gu, Genda; Fradkin, Eduardo; Norman, Michael; Abbamonte, Peter

    Static charge order is a ubiquitous feature of the underdoped cuprates. However, at optimal doping, charge-order has been thought to be completely suppressed, suggesting an interplay between the charge-ordering and superconducting order parameters. Using Momentum-resolved Electron Energy Loss Spectroscopy (M-EELS) we show the existence of diffuse fluctuating charge-order in the optimally doped cuprate Bi2Sr2CaCu2O8+δ (Bi-2212) at low-temperature. We present full momentum-space maps of both elastic and inelastic scattering at room temperature and below the superconducting transition with 4meV resolution. We show that the ``rods'' of diffuse scattering indicate nematic-like fluctuations, and the energy width defines a fluctuation timescale of 160 fs. We discuss the implications of fluctuating charge-order on the dynamics at optimal doping. This work was supported by the Gordon and Betty Moore Foundation's EPiQS Initiative through Grant GBMF-4542. An early prototype of the M-EELS instrument was supported by the DOE Center for Emergent Superconductivity under Award No. DE-AC02-98CH10886.

  16. Optical Dark-Field and Electron Energy Loss Imaging and Spectroscopy of Symmetry-Forbidden Modes in Loaded Nanogap Antennas.

    Science.gov (United States)

    Brintlinger, Todd; Herzing, Andrew A; Long, James P; Vurgaftman, Igor; Stroud, Rhonda; Simpkins, B S

    2015-06-23

    We have produced large numbers of hybrid metal-semiconductor nanogap antennas using a scalable electrochemical approach and systematically characterized the spectral and spatial character of their plasmonic modes with optical dark-field scattering, electron energy loss spectroscopy with principal component analysis, and full wave simulations. The coordination of these techniques reveal that these nanostructures support degenerate transverse modes which split due to substrate interactions, a longitudinal mode which scales with antenna length, and a symmetry-forbidden gap-localized transverse mode. This gap-localized transverse mode arises from mode splitting of transverse resonances supported on both antenna arms and is confined to the gap load enabling (i) delivery of substantial energy to the gap material and (ii) the possibility of tuning the antenna resonance via active modulation of the gap material's optical properties. The resonant position of this symmetry-forbidden mode is sensitive to gap size, dielectric strength of the gap material, and is highly suppressed in air-gapped structures which may explain its absence from the literature to date. Understanding the complex modal structure supported on hybrid nanosystems is necessary to enable the multifunctional components many seek.

  17. High energy-resolution electron energy-loss spectroscopy study of the dielectric properties of bulk and nanoparticle LaB6 in the near-infrared region

    International Nuclear Information System (INIS)

    Sato, Yohei; Terauchi, Masami; Mukai, Masaki; Kaneyama, Toshikatsu; Adachi, Kenji

    2011-01-01

    The dielectric properties of LaB 6 crystals and the plasmonic behavior of LaB 6 nanoparticles, which have been applied to solar heat-shielding filters, were studied by high energy-resolution electron energy-loss spectroscopy (HR-EELS). An EELS spectrum of a LaB 6 crystal showed a peak at 2.0 eV, which was attributed to volume plasmon excitation of carrier electrons. EELS spectra of single LaB 6 nanoparticles showed peaks at 1.1-1.4 eV depending on the dielectric effect from the substrates. The peaks were assigned to dipole oscillation excitations. These peak energies almost coincided with the peak energy of optical absorption of a heat-shielding filter with LaB 6 nanoparticles. On the other hand, those energies were a smaller than a dipole oscillation energy predicted using the dielectric function of bulk LaB 6 crystal. It is suggested that the lower energy than expected is due to an excitation at 1.2 eV, which was observed for oxidized LaB 6 area. -- Highlights: → The dielectric properties of LaB 6 nanoparticles applied to solar heat-shielding filters were studied by HR-EELS. → Plasmon peak energies of the LaB 6 nanoparticles were almost equal to optical absorption energy of a heat-shielding filter. → From this result, near-infrared optical absorption of the filter is due to the surface dipole mode of the nanoparticles.

  18. Electron energy-loss spectroscopy on n-type doped high-temperature superconductors and related systems

    International Nuclear Information System (INIS)

    Alexander, M.

    1992-08-01

    Electron-enery loss spectroscopy measurements on n-type doped high temperature superconductors, their undoped parent compounds, Y-doped Bi 2 Sr 2 CaCu 2 O 8 and some rare earth oxides are presented. The undoped parent compounds Ln 2 CuO 4 (Ln = Pr, Nd, Sm) are charge transfer insulators with a charge transfer energy gap of 1.4 eV. The conduction band lies in the CuO 2 plane and has mainly Cu3d x 2 -y 2 character. O2p x,y states are slightly hybridized with this band. Upon partially substituting the trivalent Ln ions by tetravalent Ce or Th and monovalent F for the O ions, electron doping of the CuO 2 plane occurs with the electrons having mainly Cu3d character. A rigid band behaviour is proposed by several band structure calculations could be ruled out, as well as the occurence of so called 'mid-gap' states appearing inside the band gap between the valence and conduction bands. The position of the Fermi level was found to be at the bottom of the conduction bands. No measurable influence of the reduction process, necessary to obtain superconductivity, was detected in the unoccupied density of states. Characteristics shifts of the measured oxygen and copper edges were correlated with crossing the metal-insulator transition. These shifts are most probably caused by an improved screening capacity of the free charge carriers. A similar effect was also observed in Y-doped Bi 2 Sr 2 CaCu 2 O 8 . Thus, it was possible to show that the disappearance of the valence band hole states upon doping did not occur in a rigid-band-like manner. The low energy excitations in Nd 1.85 Ce 0.15 CuO 4-δ showed a plasmon like excitation at about 1 eV as well as a reduction and an energy shift of the charge transfer excitation. The dispersion of this plasmon excitation was determined. (orig.)

  19. Electron-beam induced amorphization of stishovite: Silicon-coordination change observed using Si K-edge extended electron energy-loss fine structure

    International Nuclear Information System (INIS)

    Aken, P.A. van; Sharp, T.G.; Seifert, F.

    1998-01-01

    The analysis of the extended energy-loss fine structure (EXELFS) of the Si K-edge for sixfold-coordinated Si in synthetic stishovite and fourfold-coordinated Si in natural α-quartz is reported by using electron energy-loss spectroscopy (EELS) in combination with transmission electron microscopy (TEM). The stishovite Si K-edge EXELFS spectra were measured as a time-dependent series to document irradiation-induced amorphization. The amorphization was also investigated through the change in Si K- and O K-edge energy-loss near edge structure (ELNES). For α-quartz, in contrast to stishovite, electron irradiation-induced vitrification, produced no detectable changes of the EXELFS. The Si K-edge EXELFS were analysed with the classical extended X-ray absorption fine structure (EXAFS) treatment and compared to ab initio curve-waved multiple-scattering (MS) calculations of EXAFS spectra for stishovite and α-quartz. Highly accurate information on the local atomic environment of the silicon atoms during the irradiation-induced amorphization of stishovite is obtained from the EXELFS structure parameters The mean Si-O bond distance R and mean Si coordination number N changes from R=0.1775 nm and N=6 for stishovite through a disordered intermediate state (R∼0.172 nm and N∼5) to R∼0.167 nm and N∼4.5 for a nearly amorphous state similar to α-quartz (R=0.1609 nm and N=4). During the amorphization process, the Debye-Waller factor (DWF) passes through a maximum value of σ N 2 ∼83.8pm 2 as it changes from σ st 2 =51.8pm 2 for sixfold to σ qu 2 =18.4pm 2 for fourfold coordination of Si. This increase in Debye-Waller factor indicates an increase in mean-square relative displacement (MSRD) between the central silicon atom and its oxygen neighbours. Using the EXELFS data for amorphization, a new method is developed to derive the relative amounts of Si coordinations in high-pressure minerals with mixed coordination. For the radiation-induced amorphization process of

  20. Electronic structure of metastable bcc Cu–Cr alloy thin films: Comparison of electron energy-loss spectroscopy and first-principles calculations

    Energy Technology Data Exchange (ETDEWEB)

    Liebscher, C.H.; Freysoldt, C. [Max-Planck-Institut für Eisenforschung GmbH, 40237 Düsseldorf (Germany); Dennenwaldt, T. [Institute of Condensed Matter Physics and Interdisciplinary Center for Electron Microscopy, Ecole Polytechnique Fédérale de Lausanne, 1015 Lausanne (Switzerland); Harzer, T.P.; Dehm, G. [Max-Planck-Institut für Eisenforschung GmbH, 40237 Düsseldorf (Germany)

    2017-07-15

    Metastable Cu–Cr alloy thin films with nominal thickness of 300 nm and composition of Cu{sub 67}Cr{sub 33} (at%) are obtained by co-evaporation using molecular beam epitaxy. The microstructure, chemical phase separation and electronic structure are investigated by transmission electron microscopy (TEM). The thin film adopts the body-centered cubic crystal structure and consists of columnar grains with ~50 nm diameter. Aberration-corrected scanning TEM in combination with energy dispersive X-ray spectroscopy confirms compositional fluctuations within the grains. Cu- and Cr-rich domains with composition of Cu{sub 85}Cr{sub 15} (at%) and Cu{sub 42}Cr{sub 58} (at%) and domain size of 1–5 nm are observed. The alignment of the interface between the Cu- and Cr-rich domains shows a preference for {110}-type habit plane. The electronic structure of the Cu–Cr thin films is investigated by electron energy loss spectroscopy (EELS) and is contrasted to an fcc-Cu reference sample. The experimental EEL spectra are compared to spectra computed by density functional theory. The main differences between bcc-and fcc-Cu are related to differences in van Hove singularities in the electron density of states. In Cu–Cr solid solutions with bcc crystal structure a single peak after the L{sub 3}-edge, corresponding to a van Hove singularity at the N-point of the first Brillouin zone is observed. Spectra computed for pure bcc-Cu and random Cu–Cr solid solutions with 10 at% Cr confirm the experimental observations. The calculated spectrum for a perfect Cu{sub 50}Cr{sub 50} (at%) random structure shows a shift in the van Hove singularity towards higher energy by developing a Cu–Cr d-band that lies between the delocalized d-bands of Cu and Cr. - Highlights: • Compositional fluctuations on the order of 1–5 nm in Cu- and Cr-rich domains are observed. • EELS determines a single van Hove singularity for bcc Cu–Cr solid solutions. • The electronic structure is dominated by d

  1. Localization of calcium in the cyanobiont and gonidial zone of Cycas revoluta Thunb. by microelectrodes, chlorotetracycline, electron spectroscopic imaging and electron energy loss spectroscopy

    International Nuclear Information System (INIS)

    Caiola, M.G.; Canini, A.; Brandizzi, F.

    1994-01-01

    Ionic calcium concentration was measured in the gonidial zone of fresh coralloid roots by means of calcium microelectrodes. It was 10 -6 M in the apical segments of coralloid roots and increased to 10 -5 M in the gonidial zones of median and basal segments. Loosely membrane-bound calcium was evidenced by using chloro-tetracycline (CTC) or ethylene glycol-bis-(β-aminoethyl ether)-N,N,N',N'-tetraacetic acid (EGTA) and CTC, in cell walls of columnar cells of Cycas and in the cytoplasm of cyanobiont. Sub-cellular localization of calcium was obtained by electron spectroscopic imaging (ESI) and electron energy loss spectroscopy (EELS) analyses applied at transmission electron microscopy on thin, unstained sections of gonidial zone of coralloid roots. By means of these techniques, bound-calcium was detected inside the mucilage of apical and median segments whereas, in the basal segments, it was completely absent. In the heterocysts of apical segments of coralloid, calcium was localized on the envelope, cell walls, thylakoids and cyanophycin granules. In the gonidial zone of the basal segments, dead or degenerating heterocysts completely lacked calcium. Therefore, the high ionic calcium amounts detected in the gonidial zone of median and basal segments could represent a minor calcium uptake by the cells or release by lysed ones. The decreases in nitrogenase activity recorded in the median and basal segments of the coralloid roots paralleled the decrease in calcium amount in heterocyst envelope. (authors)

  2. Two dimensional CCD [charged coupled device] arrays as parallel detectors in electron energy loss and x-ray wavelength dispersive spectroscopy

    International Nuclear Information System (INIS)

    Zaluzec, N.J.

    1988-08-01

    Parallel detection systems for spectroscopy have generally been based upon linear detector arrays. Replacing the linear arrays with two dimensional systems yields more complicated devices; however, there are corresponding benefits which can be realized for both x-ray and electron energy loss spectroscopy. The operational design of these systems, as well as preliminary results from the construction of such a device used for electron spectroscopy, are presented. 10 refs., 8 figs

  3. Modelling Energy Loss Mechanisms and a Determination of the Electron Energy Scale for the CDF Run II W Mass Measurement

    Energy Technology Data Exchange (ETDEWEB)

    Riddick, Thomas [Univ. College London, Bloomsbury (United Kingdom)

    2012-06-15

    The calibration of the calorimeter energy scale is vital to measuring the mass of the W boson at CDF Run II. For the second measurement of the W boson mass at CDF Run II, two independent simulations were developed. This thesis presents a detailed description of the modification and validation of Bremsstrahlung and pair production modelling in one of these simulations, UCL Fast Simulation, comparing to both geant4 and real data where appropriate. The total systematic uncertainty on the measurement of the W boson mass in the W → eve channel from residual inaccuracies in Bremsstrahlung modelling is estimated as 6.2 ±3.2 MeV/c2 and the total systematic uncertainty from residual inaccuracies in pair production modelling is estimated as 2.8± 2.7 MeV=c2. Two independent methods are used to calibrate the calorimeter energy scale in UCL Fast Simulation; the results of these two methods are compared to produce a measurement of the Z boson mass as a cross-check on the accuracy of the simulation.

  4. Design and construction of a high-stability, low-noise power supply for use with high-resolution electron energy loss spectrometers

    International Nuclear Information System (INIS)

    Katz, J.E.; Davies, P.W.; Crowell, J.E.; Somorjai, G.A.

    1982-01-01

    The design and construction of a high-stability, low-noise power supply which provides potentials for the lens and analyzer elements of a 127 0 Ehrhardt-type high-resolution electron energy loss spectrometer (HREELS) is described. The supply incorporates a filament emission-control circuit and facilities for measuring electron beam current at each spectrometer element, thus facilitating optimal tuning of the spectrometer. Spectra obtained using this supply are shown to have a four-fold improvement in signal-to-noise ratio and a higher resolution of the vibrational loss features when compared with spectra taken using a previously existing supply based on passive potential divider networks

  5. Investigation of ionization losses of shower electrons in electron-photon shower developed in liquid xenon by gamma quanta in the energy range 1600-3400 MeV

    International Nuclear Information System (INIS)

    Okhrymenko, L.S.; Slowinski, B.; Strugalski, Z.; Sredniawa, B.

    1975-01-01

    Results of the investigation of differential distributions of ionization losses and the corresponding fluctuations for shower electrons in the longitudinal development of electron-photon showers produced by gamma-quanta of energies Esub(γ)=1600-3400 MeV in liquid xenon are given. A simple and convenient from the methodical point of view two-parametric function, approximating the observed distribution has been obtained. The independence of the fluctuations of ionization losses of shower electrons on the energy of gamma-quanta in the investigated interval of Esub(γ) values has been found

  6. The electronic stopping powers and angular energy-loss dependence of helium and lithium ions in the silicon crystal

    Czech Academy of Sciences Publication Activity Database

    Mikšová, Romana; Macková, Anna; Malinský, Petr

    2017-01-01

    Roč. 406, SEP (2017), s. 179-184 ISSN 0168-583X R&D Projects: GA MŠk LM2015056; GA ČR GA15-01602S Institutional support: RVO:61389005 Keywords : energy -loss measurement * SOI material * RBS-channelling Subject RIV: BG - Nuclear , Atomic and Molecular Physics, Colliders OBOR OECD: Nuclear physics Impact factor: 1.109, year: 2016

  7. Energy-loss return gate via liquid dielectric polarization.

    Science.gov (United States)

    Kim, Taehun; Yong, Hyungseok; Kim, Banseok; Kim, Dongseob; Choi, Dukhyun; Park, Yong Tae; Lee, Sangmin

    2018-04-12

    There has been much research on renewable energy-harvesting techniques. However, owing to increasing energy demands, significant energy-related issues remain to be solved. Efforts aimed at reducing the amount of energy loss in electric/electronic systems are essential for reducing energy consumption and protecting the environment. Here, we design an energy-loss return gate system that reduces energy loss from electric/electronic systems by utilizing the polarization of liquid dielectrics. The use of a liquid dielectric material in the energy-loss return gate generates electrostatic potential energy while reducing the dielectric loss of the electric/electronic system. Hence, an energy-loss return gate can make breakthrough impacts possible by amplifying energy-harvesting efficiency, lowering the power consumption of electronics, and storing the returned energy. Our study indicates the potential for enhancing energy-harvesting technologies for electric/electronics systems, while increasing the widespread development of these systems.

  8. Use of a silicon surface-barrier detector for measurement of high-energy end loss electrons in a tandem mirror

    International Nuclear Information System (INIS)

    Saito, T.; Kiwamoto, Y.; Honda, T.; Kasugai, A.; Kurihara, K.; Miyoshi, S.

    1991-01-01

    An apparatus for the measurement of high-energy electrons (10--500 keV) with a silicon surface-barrier detector is described. The apparatus has special features. In particular, a fast CAMAC transient digitizer is used to directly record the wave form of a pulse train from the detector and then pulse heights are analyzed with a computer instead of on a conventional pulse height analyzer. With this method the system is capable of detecting electrons with a count rate as high as ∼300--400 kilocounts/s without serious deterioration of performance. Moreover, piled up signals are reliably eliminated from analysis. The system has been applied to measure electron-cyclotron-resonance-heating-induced end loss electrons in the GAMMA 10 tandem mirror and has yielded information relating to electron heating and diffusion in velocity space

  9. High-Resolution Electron Energy Loss Studies of Oxygen, Hydrogen, Nitrogen, Nitric Oxide, and Nitrous Oxide Adsorption on Germanium Surfaces.

    Science.gov (United States)

    Entringer, Anthony G.

    The first high resolution electron energy loss spectroscopy (HREELS) studies of the oxidation and nitridation of germanium surfaces are reported. Both single crystal Ge(111) and disordered surfaces were studied. Surfaces were exposed to H, O_2, NO, N _2O, and N, after cleaning in ultra-high vacuum. The Ge surfaces were found to be non-reactive to molecular hydrogen (H_2) at room temperature. Exposure to atomic hydrogen (H) resulted hydrogen adsorption as demonstrated by the presence of Ge-H vibrational modes. The HREEL spectrum of the native oxide of Ge characteristic of nu -GeO_2 was obtained by heating the oxide to 200^circC. Three peaks were observed at 33, 62, and 106 meV for molecular oxygen (O_2) adsorbed on clean Ge(111) at room temperature. These peaks are indicative of dissociative bonding and a dominant Ge-O-Ge bridge structure. Subsequent hydrogen exposure resulted in a shift of the Ge-H stretch from its isolated value of 247 meV to 267 meV, indicative of a dominant +3 oxidation state. A high density of dangling bonds and defects and deeper oxygen penetration at the amorphous Ge surface result in a dilute bridge structure with a predominant +1 oxidation state for similar exposures. Molecules of N_2O decompose at the surfaces to desorbed N_2 molecules and chemisorbed oxygen atoms. In contrast, both oxygen and nitrogen are detected at the surfaces following exposure to NO molecules. Both NO and N_2O appear to dissociate and bond at the top surface layer. Molecular nitrogen (N_2) does not react with the Ge surfaces, however, a precursor Ge nitride is observed at room temperature following exposure to nitrogen atoms and ions. Removal of oxygen by heating of the NO-exposed surface to 550^circC enabled the identification of the Ge-N vibrational modes. These modes show a structure similar to that of germanium nitride. This spectrum is also identical to that of the N-exposed surface heated to 550^circC. Surface phonon modes of the narrow-gap semiconducting

  10. Time dependent formulation of the energy loss by an accelerated intense electron beam just emitted by the cathode of RF-FEL photoinjector

    Energy Technology Data Exchange (ETDEWEB)

    Salah, Wa' el [Physics Department, Hashemite University, Zarqa 13115 (Jordan)]. E-mail: wael_salahh@hotmail.com; Coacolo, J.-L. [Institut de Physique Nucleaire d' Orsay, 91406 Orsay Cedex (France); Hallak, A.B. [Physics Department, Hashemite University, Zarqa 13115 (Jordan); Al-Obaid, M. [Physics Department, Hashemite University, Zarqa 13115 (Jordan)

    2006-08-01

    The energy loss by an accelerated electron bunch of a conical shape propagating in the laser-driven RF-photoinjector is expressed in terms of an expansion of the vector and scalar potentials into a series of eigenfunctions of the empty unit 'pill-box' cavity. A versatile and simple analytical formula which can be easily applied to a bunch of any shape is obtained.

  11. Recovery effects due to the interaction between nuclear and electronic energy losses in SiC irradiated with a dual-ion beam

    Energy Technology Data Exchange (ETDEWEB)

    Thomé, Lionel, E-mail: thome@csnsm.in2p3.fr; Debelle, Aurélien; Garrido, Frédérico; Sattonnay, Gaël; Mylonas, Stamatis [Centre de Sciences Nucléaires et de Sciences de la Matière, CNRS-IN2P3-Université Paris-Sud, Bât. 108, F-91405 Orsay (France); Velisa, Gihan [CEA, DEN, Service de Recherches de Métallurgie Physique, Laboratoire JANNUS, F-91191 Gif-sur-Yvette (France); Horia Hulubei National Institute for Physics and Nuclear Engineering, P.O.B. MG-6, 077125 Magurele (Romania); Miro, Sandrine; Trocellier, Patrick; Serruys, Yves [CEA, DEN, Service de Recherches de Métallurgie Physique, Laboratoire JANNUS, F-91191 Gif-sur-Yvette (France)

    2015-03-14

    Single and dual-beam ion irradiations of silicon carbide (SiC) were performed to study possible Synergetic effects between Nuclear (S{sub n}) and Electronic (S{sub e}) Energy Losses. Results obtained combining Rutherford backscattering in channeling conditions, Raman spectroscopy, and transmission electron microscopy techniques show that dual-beam irradiation of SiC induces a dramatic change in the final sample microstructure with a substantial decrease of radiation damage as compared to single-beam irradiation. Actually, a defective layer containing dislocations is formed upon dual-beam irradiation (S{sub n} and S{sub e}), whereas single low-energy irradiation (S{sub n} alone) or even sequential (S{sub n} + S{sub e}) irradiations lead to full amorphization. The healing process is ascribed to the electronic excitation arising from the electronic energy loss of swift ions. These results shed new light on the long-standing puzzling problem of the existence of a possible synergy between S{sub n} and S{sub e} in ion-irradiation experiments. This work is interesting for both fundamental understanding of the ion-solid interactions and technological applications in the nuclear industry where recovery S{sub n}/S{sub e} effects may preserve the integrity of nuclear devices.

  12. Observability of localized magnetoplasmons in quantum dots: Scrutinizing the eligibility of far-infrared, Raman, and electron-energy-loss spectroscopies

    Directory of Open Access Journals (Sweden)

    Manvir S. Kushwaha

    2016-03-01

    Full Text Available We investigate a one-component, quasi-zero dimensional, quantum plasma exposed to a parabolic potential and an applied magnetic field in the symmetric gauge. If the size of such a system as can be realized in the semiconducting quantum dots is on the order of the de-Broglie wavelength, the electronic and optical properties become highly tunable. Then the quantum size effects challenge the observation of many-particle phenomena such as the magneto-optical absorption, Raman intensity, and electron energy-loss spectrum. An exact analytical solution of the problem leads us to infer that these many-particle phenomena are, in fact, dictated by the generalized Kohn’s theorem (GKT in the long-wavelength limit. Maneuvering the confinement and/or the magnetic field furnishes the resonance energies capable of being explored with the FIR, Raman, and/or electron-energy-loss spectroscopy. This implies that either of these probes is competent in observing the localized magnetoplasmons in the system. As an application of the rigorous analytical diagnosis of the system, we have presented various pertinent single-particle, such as Fock-Darwin spectrum, Fermi energy, zigzag excitation spectrum, and magneto-optical transitions, and the many-particle phenomena, such as magneto-optical absorption, Raman intensity, and electron energy-loss probability. In the latter, the energy position of the resonance peaks is observed to be independent of the electron-electron interactions and hence of the number of electrons in the quantum dot in compliance with the GKT. It is found that both confinement potential and magnetic field play a decisive role in influencing the aforementioned many-particle phenomena. Specifically, increasing (decreasing the strength of the confining potential is found to be analogous to shrinking (expanding the size of the quantum dots and results into a blue (red shift in the respective spectra. Intensifying the magnetic field has two-fold effects in

  13. Observability of localized magnetoplasmons in quantum dots: Scrutinizing the eligibility of far-infrared, Raman, and electron-energy-loss spectroscopies

    Energy Technology Data Exchange (ETDEWEB)

    Kushwaha, Manvir S. [Department of Physics and Astronomy, Rice University, P.O. Box 1892, Houston, Texas 77251 (United States)

    2016-03-15

    We investigate a one-component, quasi-zero dimensional, quantum plasma exposed to a parabolic potential and an applied magnetic field in the symmetric gauge. If the size of such a system as can be realized in the semiconducting quantum dots is on the order of the de-Broglie wavelength, the electronic and optical properties become highly tunable. Then the quantum size effects challenge the observation of many-particle phenomena such as the magneto-optical absorption, Raman intensity, and electron energy-loss spectrum. An exact analytical solution of the problem leads us to infer that these many-particle phenomena are, in fact, dictated by the generalized Kohn’s theorem (GKT) in the long-wavelength limit. Maneuvering the confinement and/or the magnetic field furnishes the resonance energies capable of being explored with the FIR, Raman, and/or electron-energy-loss spectroscopy. This implies that either of these probes is competent in observing the localized magnetoplasmons in the system. As an application of the rigorous analytical diagnosis of the system, we have presented various pertinent single-particle, such as Fock-Darwin spectrum, Fermi energy, zigzag excitation spectrum, and magneto-optical transitions, and the many-particle phenomena, such as magneto-optical absorption, Raman intensity, and electron energy-loss probability. In the latter, the energy position of the resonance peaks is observed to be independent of the electron-electron interactions and hence of the number of electrons in the quantum dot in compliance with the GKT. It is found that both confinement potential and magnetic field play a decisive role in influencing the aforementioned many-particle phenomena. Specifically, increasing (decreasing) the strength of the confining potential is found to be analogous to shrinking (expanding) the size of the quantum dots and results into a blue (red) shift in the respective spectra. Intensifying the magnetic field has two-fold effects in the resonance

  14. Relativistic energy loss in a dispersive medium

    DEFF Research Database (Denmark)

    Houlrik, Jens Madsen

    2002-01-01

    The electron energy loss in a dispersive medium is obtained using macroscopic electrodynamics taking advantage of a static frame of reference. Relativistic corrections are described in terms of a dispersive Lorentz factor obtained by replacing the vacuum velocity c by the characteristic phase...... velocity c/n, where n is the complex index of refraction. The angle-resolved energy-loss spectrum of a Drude conductor is analyzed in detail and it is shown that the low-energy peak due to Ohmic losses is enhanced compared to the classical approximation....

  15. Loss of cellular transformation efficiency induced by DNA irradiation with low-energy (10 eV) electrons.

    Science.gov (United States)

    Kouass Sahbani, Saloua; Sanche, Leon; Cloutier, Pierre; Bass, Andrew D; Hunting, Darel J

    2014-11-20

    Low energy electrons (LEEs) of energies less than 20 eV are generated in large quantities by ionizing radiation in biological matter. While LEEs are known to induce single (SSBs) and double strand breaks (DSBs) in DNA, their ability to inactivate cells by inducing nonreparable lethal damage has not yet been demonstrated. Here we observe the effect of LEEs on the functionality of DNA, by measuring the efficiency of transforming Escherichia coli with a [pGEM-3Zf (-)] plasmid irradiated with 10 eV electrons. Highly ordered DNA films were prepared on pyrolitic graphite by molecular self-assembly using 1,3-diaminopropane ions (Dap(2+)). The uniformity of these films permits the inactivation of approximately 50% of the plasmids compared to transforming cluster damage into DSBs by digestion with repair enzymes, also occurred relatively infrequently. The exact nature of the lethal damage remains unknown, but it is probably a form of compact cluster damage in which the lesions are too close to be revealed by purified repair enzymes. In addition, this damage is either not repaired or is misrepaired by E. coli, since it results in plasmid inactivation, when they contain an average of three lesions. Comparison with previous results from a similar experiment performed with γ-irradiated plasmids indicates that the type of clustered DNA lesions, created directly on cellular DNA by LEEs, may be more difficult to repair than those produced by other species from radiolysis.

  16. 3D spectrum imaging of multi-wall carbon nanotube coupled π-surface modes utilising electron energy-loss spectra acquired using a STEM/Enfina system

    International Nuclear Information System (INIS)

    Seepujak, A.; Bangert, U.; Gutierrez-Sosa, A.; Harvey, A.J.; Blank, V.D.; Kulnitskiy, B.A.; Batov, D.V.

    2005-01-01

    Numerous studies have utilised electron energy-loss (EEL) spectra acquired in the plasmon (2-10 eV) regime in order to probe delocalised π-electronic states of multi-wall carbon nanotubes (MWCNTs). Interpretation of electron energy loss (EEL) spectra of MWCNTs in the 2-10 eV regime. Carbon (accepted for publication); Blank et al. J. Appl. Phys. 91 (2002) 1657). In the present contribution, EEL spectra were acquired from a 2D raster defined on a bottle-shaped MWCNT, using a Gatan UHV Enfina system attached to a dedicated scanning transmission electron microscope (STEM). The technique utilised to isolate and sequentially filter each of the volume and surface resonances is described in detail. Utilising a scale for the intensity of a filtered mode enables one to 'see' the distribution of each resonance in the raster. This enables striking 3D resonance-filtered spectrum images (SIs) of π-collective modes to be observed. Red-shift of the lower energy split π-surface resonance provides explicit evidence of π-surface mode coupling predicted for thin graphitic films (Lucas et al. Phys. Rev. B 49 (1994) 2888). Resonance-filtered SIs are also compared to non-filtered SIs with suppressed surface contributions, acquired utilising a displaced collector aperture. The present filtering technique is seen to isolate surface contributions more effectively, and without the significant loss of statistics, associated with the displaced collector aperture mode. Isolation of collective modes utilising 3D resonance-filtered spectrum imaging, demonstrates a valuable method for 'pinpointing' the location of discrete modes in irregularly shaped nanostructures

  17. Deterministic models for energy-loss straggling

    International Nuclear Information System (INIS)

    Prinja, A.K.; Gleicher, F.; Dunham, G.; Morel, J.E.

    1999-01-01

    Inelastic ion interactions with target electrons are dominated by extremely small energy transfers that are difficult to resolve numerically. The continuous-slowing-down (CSD) approximation is then commonly employed, which, however, only preserves the mean energy loss per collision through the stopping power, S(E) = ∫ 0 ∞ dEprime (E minus Eprime) σ s (E → Eprime). To accommodate energy loss straggling, a Gaussian distribution with the correct mean-squared energy loss (akin to a Fokker-Planck approximation in energy) is commonly used in continuous-energy Monte Carlo codes. Although this model has the unphysical feature that ions can be upscattered, it nevertheless yields accurate results. A multigroup model for energy loss straggling was recently presented for use in multigroup Monte Carlo codes or in deterministic codes that use multigroup data. The method has the advantage that the mean and mean-squared energy loss are preserved without unphysical upscatter and hence is computationally efficient. Results for energy spectra compared extremely well with Gaussian distributions under the idealized conditions for which the Gaussian may be considered to be exact. Here, the authors present more consistent comparisons by extending the method to accommodate upscatter and, further, compare both methods with exact solutions obtained from an analog Monte Carlo simulation, for a straight-ahead transport problem

  18. Simulation of loss electron in vacuum magnetically insulated transmission lines

    International Nuclear Information System (INIS)

    Zhang Pengfei; Li Yongdong; Liu Chunliang; Wang Hongguang; Guo Fan; Yang Hailiang; Qiu Aici; Su Zhaofeng; Sun Jianfeng; Sun Jiang; Gao Yi

    2011-01-01

    In the beginning of magnetic insulated period, loss electron in coaxial vacuum magnetically insulated transmission line (MITL) strikes anode and the bremsstrahlung photons are generated in the mean time. Based on the self-limited flow model, velocity in direction of energy transport, energy spectrum and angular distribution of loss electron are simulated by PIC code, energy spectrum of bremsstrahlung photons as well calculated though Monte Carlo method. Computational results show that the velocity of loss electron is less than 2.998 x 108 m/s, the angular excursion of electron is not much in a board extent of energy spectrum. These results show an indirect diagnosis of vacuum insulted transmission line working status based on loss electron bremsstrahlung. (authors)

  19. Loss of energy business

    International Nuclear Information System (INIS)

    Beer, G.

    2010-01-01

    Russian PM Vladimir Putin, euphoric about the signing of the 25-year contract for the use of Ukrainian seaports by the Russian Navy, announced several new strategic bilateral projects. The new partnership between the two countries might be a disappointment for those who were hoping for new Slovak energy business development in cooperation with Moscow. Representatives of the Russian company TVEL frequently visited the Slovak Ministry of Economy last year, discussing the idea of a nuclear fuel production plant in Slovakia. The factory was supposed to make fuel for the growing number of Russian reactors throughout Europe and utilize the recently discovered uranium deposits near Kosice. However, since Mr. Putin unveiled the idea of creating a Russian-Ukrainian nuclear holding at the site of the Khmelnitskaya Nuclear Power Plant, Slovakia will probably not become the gate to the EU for Russia's atomic business. Owners of the Slovak uranium deposit site are losing business too. And not only does the Slovak-Russian nuclear cooperation seem to be completely lost, but the gas transfer business is unclear too. Last week, the Russian gas company Gazprom showed that its selling prices are a matter of political bargaining rather than fair market value. Similar to low prices for the extremely friendly Belarus, Ukraine earned a $100 discount and in exchange for the Black Sea deal it will be paying only $236 per thousand cubic meters of the commodity. Russia thus gave up roughly $3 billion this year. Slovakia has nothing to offer in exchange for such a deal. Not only price creation but also the construction of gas pipelines through Europe remains a political issue for Russians. With plans to bypass Ukraine and Slovakia, the only safe future for the local transit system can be the result of an idea to pool Gazprom and Ukrainian Naftohaz transit assets together with a stock swap. (author)

  20. Energy losses on tokamak startup

    International Nuclear Information System (INIS)

    Murray, J.G.; Rothe, K.E.; Bronner, G.

    1983-01-01

    During the startup of a tokamak reactor using poloidal field (PF) coils to induce plasma currents, the conducting structures carry induced currents. The associated energy losses in the circuits must be provided by the startup coils and the PF system. This paper provides quantitative and comparitive values for the energies required as a function of the thickness or resistivity of the torus shells

  1. The role of symmetry in the theory of inelastic high-energy electron scattering and its application to atomic-resolution core-loss imaging.

    Science.gov (United States)

    Dwyer, C

    2015-04-01

    The inelastic scattering of a high-energy electron in a solid constitutes a bipartite quantum system with an intrinsically large number of excitations, posing a considerable challenge for theorists. It is demonstrated how and why the utilization of symmetries, or approximate symmetries, can lead to significant improvements in both the description of the scattering physics and the efficiency of numerical computations. These ideas are explored thoroughly for the case of core-loss excitations, where it is shown that the coupled angular momentum basis leads to dramatic improvements over the bases employed in previous work. The resulting gains in efficiency are demonstrated explicitly for K-, L- and M-shell excitations, including such excitations in the context of atomic-resolution imaging in the scanning transmission electron microscope. The utilization of other symmetries is also discussed. Copyright © 2014 Elsevier B.V. All rights reserved.

  2. World offshore energy loss statistics

    International Nuclear Information System (INIS)

    Kaiser, Mark J.

    2007-01-01

    Offshore operations present a unique set of environmental conditions and adverse exposure not observed in a land environment taking place in a confined space in a hostile environment under the constant danger of catastrophe and loss. It is possible to engineer some risks to a very low threshold of probability, but losses and unforeseen events can never be entirely eliminated because of cost considerations, the human factor, and environmental uncertainty. Risk events occur infrequently but have the potential of generating large losses, as evident by the 2005 hurricane season in the Gulf of Mexico, which was the most destructive and costliest natural disaster in the history of offshore production. The purpose of this paper is to provide a statistical assessment of energy losses in offshore basins using the Willis Energy Loss database. A description of the loss categories and causes of property damage are provided, followed by a statistical assessment of damage and loss broken out by region, cause, and loss category for the time horizon 1970-2004. The impact of the 2004-2005 hurricane season in the Gulf of Mexico is summarized

  3. High-resolution parallel electron energy-loss spectroscopy of MnL2,3-edges in inorganic manganese compounds

    International Nuclear Information System (INIS)

    Garvie, L.A.J.; Craven, A.J.

    1994-01-01

    Parallel electron energy-loss spectroscopy (PEELS) in a scanning transmission electron microscope (STEM) was used to record the Mn L 2,3 -edges from a range of natural and synthetic manganese containing materials, covering valences 0, II, III, IV and VII, with an energy resolution of ca. 0.5 eV. The Mn L 2,3 electron-loss near-edge structure (ELNES) of these edges provided a sensitive fingerprint of its valence. The Mn 2+ L 2,3 -edges show little sensitivity to the local site symmetry of the ligands surrounding the manganese. This is illustrated by comparing the Mn L 2,3 -edges from 4-, 6-and 8-fold coordinated Mn 2+ . In contrast, the Mn L 3 -edges from Mn 3+ and Mn 4+ containing minerals exhibited ELNES that are interpreted in terms of a crystals-field splitting of the 3d electrons, governed by the symmetry of the surrounding ligands. The Mn L 3 -edges for octahedrally coordinated Mn 2+ , Mn 3+ and Mn 4+ showed variations in their ELNES that were sensitive to the crystal-field strength. The crystal-field strength (10Q) was measured from these edges and compared very well with published optically determinted values. The magnitude of 10Dq measured from the Mn L 3 -edges and their O K-edge prepeaks of the manganese oxides were almost identical. This further confirms that the value of 10Dq measured at the Mn L 3 -edge is correct. Selected spectra are compared with theoretical 2p atomic multiplet spectra and the differences and similarities are explained in terms of the covalency and site symmetry of the manganese. The Mn L 3 -edges allow the valence of the manganese to be ascertained, even in multivalent state materials, and can also be used to dtermin 10Dq. (orig.)

  4. Loss energy states of nonstationary quantum systems

    International Nuclear Information System (INIS)

    Dodonov, V.V.; Man'ko, V.I.

    1978-01-01

    The concept of loss energy states is introduced. The loss energy states of the quantum harmonic damping oscillator are considered in detail. The method of constructing the loss energy states for general multidimensional quadratic nonstationary quantum systems is briefly discussed

  5. Stopping power and energy loss cross section of a point charge penetrating through a dense medium of bound electrons

    International Nuclear Information System (INIS)

    Belkacem, A.; Sigmund, P.; Odense Univ.

    1989-01-01

    We have derived the dielectric function ε(k,ω) in the Lindhard approximation for a medium consisting of electrons individually bound by harmonic forces. The dielectric function is expressible in terms of a hypergeometric series and approaches well-known results in the limits of negligible binding, large momentum transfer, and long wavelength, respectively. The stopping power of a moving point charge scales very well with the shifted resonance frequency α 0 = (ω O 2 + ω P 2 ) 1/2 (ω O = oscillator frequency; ω P = plasma frequency) that follows from classical dispersion theory. The results differ noticeably from free-electron behavior even at rather high electron density. The discrete excitation levels of an isolated harmonic oscillator are increasingly shifted and broadened with increasing electron density. 15 refs., 2 figs

  6. Electron energy loss spectroscopy of CH3N2CH3 adsorbed on Ni(100), Ni(111), Cr(100), Cr(111)

    International Nuclear Information System (INIS)

    Schulz, M.A.

    1985-07-01

    A study of the adsorption of CH 3 N 2 CH 3 on Ni(100), Ni(111), Cr(100), and Cr(111) using high resolution electron energy loss spectroscopy (EELS) is presented. Under approximately the same conditions of coverage, the vibrational spectra of CH 3 N 2 CH 3 on these four surfaces are quite distinct from one another, implying that the CH 3 N 2 CH 3 -substrate interaction is very sensitive to the physical and electronic structure of each surface. In addition to the room temperature studies, the evolution of surface species on the Ni(100) surface in the temperature range 300 to 425 K was studied. Analysis of the Ni(100) spectra indicates that molecular adsorption, probably through the N lone pair, occurs at room temperature. Spectra taken after annealing the CH 3 N 2 CH 3 -Ni(100) surfaces indicate that CH and CN bond scission occurred at the elevated temperatures. Decomposition of CH 3 N 2 CH 3 takes place on the Ni(111), Cr(100), and Cr(111) surfaces at room temperature, as evidenced by the intensity of the carbon-metal stretch in the corresponding spectra. Possible identities of coadsorbed dissociation products are considered. The stable coverage of surface species on all four surfaces at 300 K is less than one monolayer. A general description of an electron energy loss (EEL) spectrometer is given. Followed by a more specific discussion of some recent modifications to the EEL monochromator assembly used in this laboratory. Both the previous configuration of our monochromator and the new version are briefly described, as an aid to understanding the motivation for the changes as well as the differences in operation of the two versions. For clarity, the new monochromator design is referred to as variable pass, while the previous design is referred to as double pass. A modified tuning procedure for the new monochromator is also presented. 58 refs., 11 figs

  7. Mechanical energy losses in plastically deformed and electron plus neutron irradiated high purity single crystalline molybdenum at elevated temperatures

    Energy Technology Data Exchange (ETDEWEB)

    Zelada, Griselda I. [Laboratorio de Materiales, Escuela de Ingenieria Electrica, Facultad de Ciencias Exactas, Ingenieria y Agrimensura, Universidad Nacional de Rosario, Avda. Pellegrini 250, 2000 Rosario (Argentina); Lambri, Osvaldo Agustin [Laboratorio de Materiales, Escuela de Ingenieria Electrica, Facultad de Ciencias Exactas, Ingenieria y Agrimensura, Universidad Nacional de Rosario, Avda. Pellegrini 250, 2000 Rosario (Argentina); Instituto de Fisica Rosario - CONICET, Member of the CONICET& #x27; s Research Staff, Avda. Pellegrini 250, 2000 Rosario (Argentina); Bozzano, Patricia B. [Laboratorio de Microscopia Electronica, Unidad de Actividad Materiales, Centro Atomico Constituyentes, Comision Nacional de Energia Atomica, Avda. Gral. Paz 1499, 1650 San Martin (Argentina); Garcia, Jose Angel [Departamento de Fisica Aplicada II, Facultad de Ciencias y Tecnologia, Universidad del Pais Vasco, Apdo. 644, 48080 Bilbao, Pais Vasco (Spain)

    2012-10-15

    Mechanical spectroscopy (MS) and transmission electron microscopy (TEM) studies have been performed in plastically deformed and electron plus neutron irradiated high purity single crystalline molybdenum, oriented for single slip, in order to study the dislocation dynamics in the temperature range within one third of the melting temperature. A damping peak related to the interaction of dislocation lines with both prismatic loops and tangles of dislocations was found. The peak temperature ranges between 900 and 1050 K, for an oscillating frequency of about 1 Hz. (Copyright copyright 2012 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  8. Energy loss spectroscopy applied to surface studies

    International Nuclear Information System (INIS)

    Lecante, J.

    1975-01-01

    The analysis of energy losses suffered by slow electrons (5eV to 300eV) back-scattered by single crystal surfaces appears to be a powerful method for surfaces studies. The inelastic scattering of these slow electrons limits their escape depth to the surface region. After a review of the basic excitation processes due to the interaction between electrons and surfaces (phonons, plasmons and electronic transitions) a brief discussion is given about the instruments needed for this electrons spectroscopy. Finally some experimental results are listed and it is shown that the comparison of the results given by ELS with other surface sensitive methods such as UPS is very fruitful and new information can be obtained. The improvement of theoretical studies on surface excitations due to slow electrons will provide in the next future the possibility of analysing in a more quantitative way the results given by ELS [fr

  9. Evidences of the influence of the electronic stopping power in the elastic energy loss in thin films of amorphous carbon

    International Nuclear Information System (INIS)

    Grande, P.L.; Fichtner, P.F.P.; Behar, M.; Zawislak, E.F.C.

    1988-01-01

    Measurements of deepness of implanted ions in carbon films, show the possibility that the energy elastic component given to the medium, could be affected by the ineslastic stopping parcel, which could cause a total stopping power, smaller than the expected. (A.C.A.S.) [pt

  10. The substrate effect in electron energy-loss spectroscopy of localized surface plasmons in gold and silver nanoparticles

    DEFF Research Database (Denmark)

    Kadkhodazadeh, Shima; Christensen, Thomas; Beleggia, Marco

    2017-01-01

    , as in optical measurements, the substrate material can modify the acquired signal. Here, we have investigated how the EELS signal recorded from supported silver and gold spheroidal nanoparticles at different electron beam impact parameter positions is affected by the choice of a dielectric substrate material...... and thickness. Consistent with previous optical studies, the presence of a dielectric substrate is found to redshift localized surface plasmons, increase their line-widths, and lead to increased prominence of higher order modes. The extent of these modifications heightens with increasing substrate permittivity...

  11. Energy loss spectroscopy applied to surface studies

    International Nuclear Information System (INIS)

    Lecante, J.

    1975-01-01

    The analysis of energy losses suffered by slow electrons (5 eV to 300 eV) back-scattered by single crystal surfaces appears to be a powerful method for surfaces studies. The inelastic scattering of these slow electrons limits their escape depth to the surface region which is defined here. After a review of the basic excitation processes due to the interaction between electrons and surfaces (phonons, plasmons and electronic transitions) a brief discussion is given about the instruments needed for this electron spectroscopy. Finally some experimental results are listed and it is shown that the comparison of the results given by ELS with other surface sensitive methods such as UPS is very fruitful and new information can be obtained [fr

  12. Ion irradiation of carbides ZrC and TiC. Effects of electronic and nuclear energy losses

    International Nuclear Information System (INIS)

    Pellegrino-Chateau, Stephanie

    2015-01-01

    This study is focused on the ceramic refractory transition metals, such as titanium carbide and zirconium envisaged to their strength characteristics under extreme conditions. These ceramics are subject to various sources of radiation (neutrons, fission products, the alpha decays) in future generation reactors IV high temperature reactor and gas cooled reactor. Radiation encountered in the reactor can be simulated by external irradiation with particle accelerators, using various ions in a wide energy range. These instruments can reproduce in controlled conditions damage suffered by structural nuclear materials. (author) [fr

  13. Auroral electron energies

    International Nuclear Information System (INIS)

    McEwan, D.J.; Duncan, C.N.; Montalbetti, R.

    1981-01-01

    Auroral electron characteristic energies determined from ground-based photometer measurements of the ratio of 5577 A OI and 4278 A N 2 + emissions are compared with electron energies measured during two rocket flights into pulsating aurora. Electron spectra with Maxwellian energy distributions were observed in both flights with an increase in characteristic energy during each pulsation. During the first flight on February 15, 1980 values of E 0 ranging from 1.4 keV at pulsation minima to 1.8 keV at pulsation maxima were inferred from the 5577/4278 ratios, in good agreement with rocket measurements. During the second flight on February 23, direct electron energy measurements yielded E 0 values of 1.8 keV rising to 2.1 keV at pulsation maxima. The photometric ratio measurements in this case gave inferred E 0 values about 0.5 keV lower. This apparent discrepancy is considered due to cloud cover which impaired the absolute emission intensity measurements. It is concluded that the 5577/4278 ratio does yield a meaningful measure of the characteristic energy of incoming electrons. This ratio technique, when added to the more sensitive 6300/4278 ratio technique usable in stable auroras can now provide more complete monitoring of electron influx characteristics. (auth)

  14. Estimation of fluctuation in restricted energy loss

    International Nuclear Information System (INIS)

    Doke, T.; Hayashi, T.; Nagata, K.

    1983-01-01

    Restricted Energy Loss (REL) is defined as an energy loss [(dE/dX)/sub E//sub delta/<ν/] that produced the delta-rays of energies less than some specified energy ν and is often used as a simple measure of track structure. For example, REL is a measure of track formation threshold in plastic track detector and the growth rate of track in chemical etching solution is considered to depend only on REL given along the track. Using a stack of elastic sheets, recently, it became possible to identify isotopes of incident particles. In that case, the limit of mass resolution is determined by fluctuation of REL in the length of etch pit produced along the path of particle. A computer program was developed to calculate the probability distribution for energy deposition in absorber allowing for electron escape. In this calculation, it is assumed that all electrons with energies greater than a certain value epsilon/sub d/ escape. This means that this calculation directly gives the fluctuation of REL. Therefore, we tried to use the computer program to estimate the ultimate mass resolution in plastic detector. In this paper, we show firstly the comparison of ASB's calculation with the experimental results obtained by a gas counter and next the results of estimation of ultimate mass resolution in plastic detectors

  15. Plasma electron losses in a multidipole plasma

    International Nuclear Information System (INIS)

    Haworth, M.D.

    1983-01-01

    The magnitude of the plasma electron cusp losses in a multidipole plasma device is determined by using a plasma electron heating technique. This method consists of suddenly generating approximately monoenergetic test electrons inside the multidipole plasma, which is in a steady-state equilibrium prior to the introduction of the test electrons. The Coulomb collisions between the test electrons and the plasma electrons result in heating the plasma electrons. The experimentally measured time evolution of the plasma electron temperature is compared with that predicted by a kinetic-theory model which calculates the time evolution of the test electron and the plasma electron distribution functions. The analytical solution of the plasma electron heating rate when the test electrons are first introduced into the plasma predicts that there is no dependence on ion mass. Experimental results in helium, neon, argon, and krypton multidipole plasmas confirm this prediction. The time-evolved solution of the kinetic equations must be solved numerically, and these results (when coupled with the experimental heating results) show that the plasma electron cusp-loss width is on the order of an electron Larmor radius

  16. The degree of 5f electron localization in URu2Si2: electron energy-loss spectroscopy and spin-orbit sum rule analysis

    Energy Technology Data Exchange (ETDEWEB)

    Jeffries, J R; Moore, K T; Butch, N P; Maple, M B

    2010-05-19

    We examine the degree of 5f electron localization in URu{sub 2}Si{sub 2} using spin-orbit sum rule analysis of the U N{sub 4,5} (4d {yields} 5f) edge. When compared to {alpha}-U metal, US, USe, and UTe, which have increasing localization of the 5f states, we find that the 5f states of URu{sub 2}Si{sub 2} are more localized, although not entirely. Spin-orbit analysis shows that intermediate coupling is the correct angular momentum coupling mechanism for URu{sub 2}Si{sub 2} when the 5f electron count is between 2.6 and 2.8. These results have direct ramifications for theoretical assessment of the hidden order state of URu{sub 2}Si{sub 2}, where the degree of localization of the 5f electrons and their contribution to the Fermi surface are critical.

  17. Dynamical observation of lithium insertion/extraction reaction during charge-discharge processes in Li-ion batteries by in situ spatially resolved electron energy-loss spectroscopy.

    Science.gov (United States)

    Shimoyamada, Atsushi; Yamamoto, Kazuo; Yoshida, Ryuji; Kato, Takehisa; Iriyama, Yasutoshi; Hirayama, Tsukasa

    2015-12-01

    All-solid-state Li-ion batteries (LIBs) with solid electrolytes are expected to be the next generation devices to overcome serious issues facing conventional LIBs with liquid electrolytes. However, the large Li-ion transfer resistance at the electrode/solid-electrolyte interfaces causes low power density and prevents practical use. In-situ-formed negative electrodes prepared by decomposing the solid electrolyte Li(1+x+3z)Alx(Ti,Ge)(2-x)Si(3z)P(3-z)O12 (LASGTP) with an excess Li-ion insertion reaction are effective electrodes providing low Li-ion transfer resistance at the interfaces. Prior to our work, however, it had still been unclear how the negative electrodes were formed in the parent solid electrolytes. Here, we succeeded in dynamically visualizing the formation by in situ spatially resolved electron energy-loss spectroscopy in a transmission electron microscope mode (SR-TEM-EELS). The Li-ions were gradually inserted into the solid electrolyte region around 400 nm from the negative current-collector/solid-electrolyte interface in the charge process. Some of the ions were then extracted in the discharge process, and the rest were diffused such that the distribution was almost flat, resulting in the negative electrodes. The redox reaction of Ti(4+)/Ti(3+) in the solid electrolyte was also observed in situ during the Li insertion/extraction processes. The in situ SR-TEM-EELS revealed the mechanism of the electrochemical reaction in solid-state batteries. © The Author 2015. Published by Oxford University Press on behalf of The Japanese Society of Microscopy. All rights reserved. For permissions, please e-mail: journals.permissions@oup.com.

  18. Antiscreening mode of projectile-electron loss

    International Nuclear Information System (INIS)

    Montanari, C.C.; Miraglia, J.E.; Arista, N.R.

    2003-01-01

    The inelastic contribution of target electrons to different electronic processes in the projectile is obtained by employing the local-density approximation as usually applied in the dielectric formalism. Projectile-electron-loss cross sections due to the electron-electron interaction are calculated and compared with those obtained by using atomic antiscreening theories. We also calculate ionization cross sections and stopping power for bare ions impinging on different gases. The good agreement with the experimental data and the simplicity of the local-density approximation make it an efficient method for describing inelastic processes of gaseous target electrons. It is expected to be useful for targets with large atomic number. In this case, the number of possible final states to be considered by the traditional atomic methods makes it a tough task to be tackled. On the contrary, the more electrons the target has, the better the local plasma approximation is expected to be

  19. Trapped electron losses by interactions with coherent VLF waves

    International Nuclear Information System (INIS)

    Walt, M.; Inan, U.S.; Voss, H.D.

    1996-01-01

    VLF whistler waves from lightning enter the magnetosphere and cause the precipitation of energetic trapped electrons by pitch angle scattering. These events, known as Lightning-induced Electron Precipitation (LEP) have been detected by satellite and rocket instruments and by perturbations of VLF waves traveling in the earth-ionosphere waveguide. Detailed comparison of precipitating electron energy spectra and time dependence are in general agreement with calculations of trapped electron interactions with ducted whistler waves. In particular the temporal structure of the precipitation and the dynamic energy spectra of the electrons confirm this interpretation of the phenomena. There are discrepancies between observed and measured electron flux intensities and pitch angle distributions, but these quantities are sensitive to unknown wave intensities and trapped particle fluxes near the loss cone angle. The overall effect of lightning generated VLF waves on the lifetime of trapped electrons is still uncertain. The flux of electrons deflected into the bounce loss cone by a discrete whistler wave has been measured in a few cases. However, the area of the precipitation region is not known, and thus the total number of electrons lost in an LEP event can only be estimated. While the LEP events are dramatic, more important effects on trapped electrons may arise from the small but numerous deflections which increase the pitch angle diffusion rate of the electron population. copyright 1996 American Institute of Physics

  20. Trapped electron losses by interactions with coherent VLF waves

    Science.gov (United States)

    Walt, M.; Inan, U. S.; Voss, H. D.

    1996-07-01

    VLF whistler waves from lightning enter the magnetosphere and cause the precipitation of energetic trapped electrons by pitch angle scattering. These events, known as Lightning-induced Electron Precipitation (LEP) have been detected by satellite and rocket instruments and by perturbations of VLF waves traveling in the earth-ionosphere waveguide. Detailed comparison of precipitating electron energy spectra and time dependence are in general agreement with calculations of trapped electron interactions with ducted whistler waves. In particular the temporal structure of the precipitation and the dynamic energy spectra of the electrons confirm this interpretation of the phenomena. There are discrepancies between observed and measured electron flux intensities and pitch angle distributions, but these quantities are sensitive to unknown wave intensities and trapped particle fluxes near the loss cone angle. The overall effect of lightning generated VLF waves on the lifetime of trapped electrons is still uncertain. The flux of electrons deflected into the bounce loss cone by a discrete whistler wave has been measured in a few cases. However, the area of the precipitation region is not known, and thus the total number of electrons lost in an LEP event can only be estimated. While the LEP events are dramatic, more important effects on trapped electrons may arise from the small but numerous deflections which increase the pitch angle diffusion rate of the electron population.

  1. Electron energies in metals

    International Nuclear Information System (INIS)

    Mahan, G.D.; Tennessee Univ., Knoxville, TN

    1991-01-01

    The modern era of electron-electron interactions began a decade ago. Plummer's group initiated a program of using angular resolved photoemission to examine the band structure of the simple metals. Beginning with aluminum, and carrying on to sodium and potassium, they always found that the occupied energy bands were much narrower than expected. For example, the compressed energy bands for metallic potassium suggest a band effective mass of m* = 1.33m e . This should be compared to the band mass found from optical conductivity m*/m e = 1.01 ± 0.01. The discrepancy between these results is startling. It was this great difference which started my group doing calculations. Our program was two-fold. On one hand, we reanalyzed the experimental data, in order to see if Plummer's result was an experimental artifact. On the other hand, we completely redid the electron-electron self-energy calculations for simple metals, using the most modern choices of local-field corrections and vertex corrections. Our results will be reported in these lectures. They can be summarized as following: Our calculations give the same effective masses as the older calculations, so the theory is relatively unchanged; Our analysis of the experiments suggests that the recent measurements of band narrowing are an experimental artifact. 38 refs., 9 figs

  2. Effects of dynamic diffraction conditions on magnetic parameter determination in a double perovskite Sr_2FeMoO_6 using electron energy-loss magnetic chiral dichroism

    International Nuclear Information System (INIS)

    Wang, Z.C.; Zhong, X.Y.; Jin, L.; Chen, X.F.; Moritomo, Y.; Mayer, J.

    2017-01-01

    Electron energy-loss magnetic chiral dichroism (EMCD) spectroscopy, which is similar to the well-established X-ray magnetic circular dichroism spectroscopy (XMCD), can determine the quantitative magnetic parameters of materials with high spatial resolution. One of the major obstacles in quantitative analysis using the EMCD technique is the relatively poor signal-to-noise ratio (SNR), compared to XMCD. Here, in the example of a double perovskite Sr_2FeMoO_6, we predicted the optimal dynamical diffraction conditions such as sample thickness, crystallographic orientation and detection aperture position by theoretical simulations. By using the optimized conditions, we showed that the SNR of experimental EMCD spectra can be significantly improved and the error of quantitative magnetic parameter determined by EMCD technique can be remarkably lowered. Our results demonstrate that, with enhanced SNR, the EMCD technique can be a unique tool to understand the structure-property relationship of magnetic materials particularly in the high-density magnetic recording and spintronic devices by quantitatively determining magnetic structure and properties at the nanometer scale. - Highlights: • We demonstrate how to choose the optimal experimental conditions by using dynamical diffraction calculations in Sr_2FeMoO_6. • With optimized diffraction conditions, the signal-to-noise ratio of experimental EMCD spectra has been significantly improved. • We have determined orbital to spin magnetic moment ratio of Sr_2FeMoO_6 quantitatively. • We have discussed the effects of dynamical diffraction conditions on the error bar of quantitative magnetic parameters.

  3. Assessing electron beam sensitivity for SrTiO{sub 3} and La{sub 0.7}Sr{sub 0.3}MnO{sub 3} using electron energy loss spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Nord, Magnus, E-mail: magnunor@gmail.com [Department of Physics, NTNU, Trondheim (Norway); Vullum, Per Erik [Department of Physics, NTNU, Trondheim (Norway); Materials and Chemistry, SINTEF, Trondheim (Norway); Hallsteinsen, Ingrid; Tybell, Thomas [Department of Electronics and Telecommunications, NTNU, Trondheim (Norway); Holmestad, Randi [Department of Physics, NTNU, Trondheim (Norway)

    2016-10-15

    Thresholds for beam damage have been assessed for La{sub 0.7}Sr{sub 0.3}MnO{sub 3} and SrTiO{sub 3} as a function of electron probe current and exposure time at 80 and 200 kV acceleration voltage. The materials were exposed to an intense electron probe by aberration corrected scanning transmission electron microscopy (STEM) with simultaneous acquisition of electron energy loss spectroscopy (EELS) data. Electron beam damage was identified by changes of the core loss fine structure after quantification by a refined and improved model based approach. At 200 kV acceleration voltage, damage in SrTiO{sub 3} was identified by changes both in the EEL fine structure and by contrast changes in the STEM images. However, the changes in the STEM image contrast as introduced by minor damage can be difficult to detect under several common experimental conditions. No damage was observed in SrTiO{sub 3} at 80 kV acceleration voltage, independent of probe current and exposure time. In La{sub 0.7}Sr{sub 0.3}MnO{sub 3}, beam damage was observed at both 80 and 200 kV acceleration voltages. This damage was observed by large changes in the EEL fine structure, but not by any detectable changes in the STEM images. The typical method to validate if damage has been introduced during acquisitions is to compare STEM images prior to and after spectroscopy. Quantifications in this work show that this method possibly can result in misinterpretation of beam damage as changes of material properties. - Highlights: • We studied the effects of a TEM electron beam on a perovskite heterostructure. • Using an improved ELNES quantification method, subtle changes could be observed. • On LSMO changes were observed in the ELNES, but none in the STEM-HAADF. • For STO changes were observed in both ELNES and STEM-HAADF. • This shows beam damage can be misinterpreted as material properties.

  4. Energy loss in grazing proton-surface collisions

    Energy Technology Data Exchange (ETDEWEB)

    Juaristi, J I [Dept. Fisica de Materiales, Facultad de Quimicas, UPV/EHU, San Sebastian (Spain); Garcia de Abajo, F J [Dept. Ciencias de la Computacion e Inteligencia Artificial, Facultad de Informatica, UPV/EHU, San Sebastian (Spain)

    1994-05-01

    The energy loss of fast protons, with energy E > 100 keV, specularly reflected on a solid surface with glancing angle of incidence of the order of a mrad is analysed on theoretical grounds. Two different contributions can be distinguished: (i) energy losses originating from the interaction with the valence band, accounted for through an induced force, and (ii) the excitation of electron bound states of the target atoms. The results are compared with available experimental data. (orig.)

  5. Energy loss in grazing proton-surface collisions

    International Nuclear Information System (INIS)

    Juaristi, J.I.; Garcia de Abajo, F.J.

    1994-01-01

    The energy loss of fast protons, with energy E > 100 keV, specularly reflected on a solid surface with glancing angle of incidence of the order of a mrad is analysed on theoretical grounds. Two different contributions can be distinguished: i) energy losses originating from the interaction with the valence band, accounted for through an induced force, and ii) the excitation of electron bound states of the target atoms. The results are compared with available experimental data. (orig.)

  6. Comments on GUT monopole energy loss and ionization

    International Nuclear Information System (INIS)

    Hagstrom, R.

    1982-01-01

    A few comments about the likely behavior of the electromagnetic energy loss and ionization rates of super-slowly moving magnetic monopoles are presented. The questions of energy loss rates and ionization rates for super-low monopoles passing through matter are considered, concentrating on aspects of these issues which affect practical detection techniques. It is worthwhile here to emphasize that there is a potentially great distinction between energy loss rates and ionization rates and that the magnitude of this distinction is really the great issue which must be settled in order to understand the significance of experimental results from present and proposed investigations of the slow monopole question. Energy loss here means the total dE/dX of the projectile due to interactions with the electrons of the slowing medium. To the extent that nuclear collisions can be neglected, this so-called electronic energy loss is the relevant quantity in questions about whether monopoles stop within the earth's crust, whether they are slowed by interstellar plasmas, or the signal in a truly calorimetric measurement (measuring temperature rises along the trajectory), etc. Most of our successful detection techniques depend upon the promotion of ground state electrons into states which lie above some energy gap in the material of the detector: electrons must be knocked completely free from the gas atoms in a proportional chamber gas, electrons must be promoted to a higher band in solid scintillator plastics. These processes are generically identified as ionization

  7. Calculated and experimental electron energy-loss spectra of La2O3, La(OH)3, and LaOF nanophases in high permittivity lanthanum-based oxide layers

    Science.gov (United States)

    Calmels, L.; Coulon, P. E.; Schamm-Chardon, S.

    2011-06-01

    Using first principles methods, the O K energy-loss near-edge structure of cubic and hexagonal La2O3, La(OH)3, and LaOF phases have been calculated. These calculations support the identification of nanocrystalline phases evidenced experimentally by electron energy-loss spectroscopy (EELS) performed in a transmission electron microscope. The nanocrystals have been observed in atomic layer deposited La2O3 thin films developed for advanced metal-oxide-semiconductor field effect transistor applications. The presence of the nanophases can be explained by the hygroscopicity and the particular reactivity with fluorine of La2O3. These calculations provide a set of EELS fingerprints which will be useful for local phase identification in La2O3-based materials.

  8. New approach to energy loss measurements

    CERN Document Server

    Trzaska, W H; Alanko, T; Mutterer, M; Raeisaenen, J; Tjurin, G; Wojdyr, M

    2002-01-01

    A new approach to energy loss measurements is proposed. In the same experiment electronic stopping force (power) in gold, nickel, carbon, polycarbonate and Havar for sup 4 sup 0 Ar, sup 2 sup 8 Si, sup 1 sup 6 O, sup 4 He and sup 1 H ions in the energy range 0.12-11 MeV/u has been measured. In this paper we give the full results for gold, nickel, and carbon and for sup 4 sup 0 Ar, sup 1 sup 6 O, sup 4 He and sup 1 H ions. Good agreement of the measured stopping force values for light ions with literature data is interpreted as the positive test of the experimental technique. The same technique used with heavy ions yields agreement with the published data only for energies above 1 MeV/u. At lower energies we observe progressively increasing discrepancy. This discrepancy is removed completely as soon as we neglect pulse height defect compensation. This observation makes us believe that the majority of the published results as well as semi-empirical calculations based on them (like the popular SRIM) may be in er...

  9. Proton energy loss in multilayer graphene and carbon nanotubes

    Science.gov (United States)

    Uribe, Juan D.; Mery, Mario; Fierro, Bernardo; Cardoso-Gil, Raul; Abril, Isabel; Garcia-Molina, Rafael; Valdés, Jorge E.; Esaulov, Vladimir A.

    2018-02-01

    Results of a study of electronic energy loss of low keV protons interacting with multilayer graphene targets are presented. Proton energy loss shows an unexpectedly high value as compared with measurements in amorphous carbon and carbon nanotubes. Furthermore, we observe a classical linear behavior of the energy loss with the ion velocity but with an apparent velocity threshold around 0.1 a.u., which is not observed in other carbon allotropes. This suggests low dimensionality effects which can be due to the extraordinary graphene properties.

  10. Heavy quark energy loss in nuclear medium

    International Nuclear Information System (INIS)

    Zhang, Benr-Wei; Wang, Enke; Wang, Xin-Nian

    2003-01-01

    Multiple scattering, modified fragmentation functions and radiative energy loss of a heavy quark propagating in a nuclear medium are investigated in perturbative QCD. Because of the quark mass dependence of the gluon formation time, the medium size dependence of heavy quark energy loss is found to change from a linear to a quadratic form when the initial energy and momentum scale are increased relative to the quark mass. The radiative energy loss is also significantly suppressed relative to a light quark due to the suppression of collinear gluon emission by a heavy quark

  11. Equilibration Influence on Jet Energy Loss

    International Nuclear Information System (INIS)

    Cheng Luan; Wang Enke

    2010-01-01

    With the initial conditions in the chemical non-equilibrated medium and Bjorken expanding medium at RHIC, we investigate the consequence for parton evolution. With considering the parton equilibration, we obtain the time dependence of the opacity when the jet propagates through the QGP medium. The parton equilibration affect the jet energy loss with detailed balance evidently. Both parton energy loss from stimulated emission in the chemical non-equilibrated expanding medium and in Bjorken expanding medium are linear dependent on the propagating distance rather than square dependent in the static medium. This will increase the energy and propagating distance dependence of the parton energy loss.

  12. Electron loss from hydrogen-like highly charged ions in collisions with electrons, protons and light atoms

    Science.gov (United States)

    Lyashchenko, K. N.; Andreev, O. Yu; Voitkiv, A. B.

    2018-03-01

    We consider electron loss from a hydrogen-like highly charged ion (HCI) in relativistic collisions with hydrogen and helium in the range of impact velocities v min ≤ v ≤ v max (v min and v max correspond to the threshold energy ε th for electron loss in collisions with a free electron and to ≈5 ε th, respectively) where any reliable data for loss cross sections are absent. In this range, where the loss process is characterized by large momentum transfers, we express it in terms of electron loss in collisions with equivelocity protons and electrons and explore by performing a detailed comparative study of these subprocesses. Our results, in particular, show that: (i) compared to equivelocity electrons protons are more effective in inducing electron loss, (ii) the relative effectiveness of electron projectiles grows with increase in the atomic number of a HCI, (iii) collisions with protons and electrons lead to a qualitatively different population of the final-state-electron momentum space and even when the total loss cross sections in these collisions become already equal the spectra of the outgoing electrons still remain quite different in almost the entire volume of the final-state-electron momentum space, (iv) in collisions with hydrogen and helium the contributions to the loss process from the interactions with the nucleus and the electron(s) of the atom could be rather well separated in a substantial part of the final-state-electron momentum space.

  13. The energy cost of quantum information losses

    Science.gov (United States)

    Romanelli, Alejandro; de Lima Marquezino, Franklin; Portugal, Renato; Donangelo, Raul

    2018-05-01

    We explore the energy cost of the information loss resulting from the passage of an initial density operator to a reduced one. We use the concept of entanglement temperature in order to obtain a lower bound for the energy change associated with this operation. We determine the minimal energy required for the case of the information losses associated with the trace over the space coordinates of a two-dimensional quantum walk.

  14. Electron-impact excitation of multiply-charged ions using energy loss in merged beams: e + Si3+(3s2S1/2) → e + Si3+(3p2P1/2,3/2)

    International Nuclear Information System (INIS)

    Wahlin, E.K.; Thompson, J.S.; Dunn, G.H.; Phaneuf, R.A.; Gregory, D.C.; Smith, A.C.H.

    1990-01-01

    For the first time absolute total cross sections for electron-impact excitation of a multiply-charged ion have been measured using an electron-energy-loss technique. Measurements were made near threshold for the process e + Si 3+ (3s 2 S 1/2 ) → e + Si 3+ (3p 2 P 1/2 , 3/2 ) -- 8.88 eV. The 10 -15 cm 2 measured cross section agrees with results of 7-state close coupling calculations to better than the ±20% (90% CL) total uncertainty of the measurements. Convoluting the theoretical curve with a Gaussian energy distribution indicates an energy width of 0.15 approx-lt ΔE approx-lt 0.20 eV. 12 refs., 2 figs

  15. Chlorine loss and mass loss from polyvinylchloride and polyvinylidenchloride under the electron beam

    International Nuclear Information System (INIS)

    Lindberg, K.A.H.; Bertilsson, H.E.

    1985-01-01

    The loss of chlorine during the irradiation of PVC and PVDC in the electron microscope has been measured by the decay of the X-ray chlorine Kα signal. A number of factors affecting the measured beam damage curves have been considered and the experimental errors reduced to +- 10%. The results show that the chlorine decay curves can be best described by the sum of two exponentials, corresponding to the two different chlorine decay processes, these being: the dehydrochlorination of the polymer molecules and the dehydrochlorination of the polyene structure formed by the beam damage. The higher initial chlorine content of PVDC compared to PVC will result in a larger amount of chlorine atoms reacting with the polyene structure, which is more stable in the electron beam than the undamaged polymer. The chlorine loss, measured by X-ray analysis, has been compared to the mass loss, measured by energy loss analysis, and also with the volume changes of isolated spherical PVC particles. It has been concluded that the mass loss is almost entirely due to chlorine loss and that the residual structure has a density similar to the undamaged PVC. (author)

  16. Cross sections of electron loss and capture for beams of O+ in water vapor from the energy range of 0,2 to 1,2 MeV

    International Nuclear Information System (INIS)

    Oliveira, Vitor Jesus de

    2015-01-01

    The study of the interactions between atoms and molecules is important for the knowledge of the cross sections of the processes that contribute to the deposition of energy by charged particle beams used in radiotherapy planning and transport particle simulation codes. Heavy ions, such as oxygen, induce many cellular and molecular damages in human cells.as a result of interaction between the projectile and atoms and molecules. The use of proton and carbon as the projectile interacting with water molecules is well characterized, however there are few studies with oxygen ions. In this work we are interested in the study of electron loss (projectile ionization) and electron capture with charge state 1+. The Pelletron accelerator of 1.7 MeV from the Federal University of Rio de Janeiro housed in the Atomic and Molecular collisions Laboratory (LACAM) has been used, which can accelerate atomic and molecular ions up to speeds of the order of hundredths of light speed, and consists of the source of negative ions, the Wien filter, the accelerator itself and the magnet load selector. The detection device used to evaluate the processes of interaction (capture and loss) between the beam of the O + and the water molecule is a Microchannel Plate (MCP) at the position sensitive anode. The collisions of O + beans are being studied in the range of 0.2 to 1.2 MeV with water vapor (Z = 10). Were obtained the respective absolute cross sections for electron loss and electron capture and compared with the cross sections of the molecule methane (CH4 → Z = 10), the isoelectronic water molecule. The experimental results show an agreement between the measurements with water and methane. Comparisons were made with results of theoretical models for electron loss using the 'Free Collision Model' and for capture the Bohr and Lindhard model. The theoretical results for electron loss show an agreement of experimental data with the model used. The model of Bohr and Lindhard describes

  17. Quantifying the Precipitation Loss of Radiation Belt Electrons during a Rapid Dropout Event

    Science.gov (United States)

    Pham, K. H.; Tu, W.; Xiang, Z.

    2017-12-01

    Relativistic electron flux in the radiation belt can drop by orders of magnitude within the timespan of hours. In this study, we used the drift-diffusion model that includes azimuthal drift and pitch angle diffusion of electrons to simulate low-altitude electron distribution observed by POES/MetOp satellites for rapid radiation belt electron dropout event occurring on May 1, 2013. The event shows fast dropout of MeV energy electrons at L>4 over a few hours, observed by the Van Allen Probes mission. By simulating the electron distributions observed by multiple POES satellites, we resolve the precipitation loss with both high spatial and temporal resolution and a range of energies. We estimate the pitch angle diffusion coefficients as a function of energy, pitch angle, and L-shell, and calculate corresponding electron lifetimes during the event. The simulation results show fast electron precipitation loss at L>4 during the electron dropout, with estimated electron lifetimes on the order of half an hour for MeV energies. The electron loss rate show strong energy dependence with faster loss at higher energies, which suggest that this dropout event is dominated by quick and localized scattering process that prefers higher energy electrons. The estimated pitch angle diffusion rates from the model are then compared with in situ wave measurements from Van Allen Probes to uncover the underlying wave-particle-interaction mechanisms that are responsible for the fast electron precipitation. Comparing the resolved precipitation loss with the observed electron dropouts at high altitudes, our results will suggest the relative role of electron precipitation loss and outward radial diffusion to the radiation belt dropouts during storm and non-storm times, in addition to its energy and L dependence.

  18. Applications of energy loss contrast STIM

    International Nuclear Information System (INIS)

    Bench, G.; Saint, A.; Legge, G.J.F.; Cholewa, M.

    1992-01-01

    Scanning Transmission Ion Microscopy (STIM) with energy loss contrast is a quantitative imaging technique. A focussed MeV ion microbeam is scanned over the sample and measured energy losses of residual ions at each beam location are used to provide the contrast in the image. The technique is highly efficient as almost every ion carries useful information from which quantitative data can be obtained. The high efficiency of data collection at present necessitates the use of small beam currents. Therefore small apertures can be used and fine spatial resolution can be achieved. High efficiency also makes it possible to collect large data sets for high definition imaging with a small radiation dose. Owing to the simple relationship between energy loss and areal density, STIM with energy loss contrast can provide a quantitative image that can be used to obtain areal density information on the sample. These areal density maps can be used not only to provide a high resolution image of the sample but also to normalise Particle Induced Xray Emission (PIXE) data. The small radiation dose required to form these areal density maps also allows one to use STIM with energy loss contrast to quantitatively monitor ion beam induced specimen changes caused by higher doses and dose rates used in other microanalytical techniques. STIM with energy loss contrast also provides the possibility of stereo imaging and ion microtomography. STIM has also been used in conjunction with channeling to explore transmission channeling in thin crystals. This paper will discuss these applications of STIM with energy loss contrast and look at further developments from them

  19. Direct band gap measurement of Cu(In,Ga)(Se,S)2 thin films using high-resolution reflection electron energy loss spectroscopy

    International Nuclear Information System (INIS)

    Heo, Sung; Lee, Hyung-Ik; Park, Jong-Bong; Ko, Dong-Su; Chung, JaeGwan; Kim, KiHong; Kim, Seong Heon; Yun, Dong-Jin; Ham, YongNam; Park, Gyeong Su; Song, Taewon; Lee, Dongho; Nam, Junggyu; Kang, Hee Jae; Choi, Pyung-Ho; Choi, Byoung-Deog

    2015-01-01

    To investigate the band gap profile of Cu(In 1−x ,Ga x )(Se 1−y S y ) 2 of various compositions, we measured the band gap profile directly as a function of in-depth using high-resolution reflection energy loss spectroscopy (HR-REELS), which was compared with the band gap profile calculated based on the auger depth profile. The band gap profile is a double-graded band gap as a function of in-depth. The calculated band gap obtained from the auger depth profile seems to be larger than that by HR-REELS. Calculated band gaps are to measure the average band gap of the spatially different varying compositions with respect to considering its void fraction. But, the results obtained using HR-REELS are to be affected by the low band gap (i.e., out of void) rather than large one (i.e., near void). Our findings suggest an analytical method to directly determine the band gap profile as function of in-depth

  20. Direct band gap measurement of Cu(In,Ga)(Se,S){sub 2} thin films using high-resolution reflection electron energy loss spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Heo, Sung [Analytical Engineering Group, Samsung Advanced Institute of Technology, 130 Samsung-ro, Yeongtong-gu, Suwon-si, Gyeonggi-do 443-803 (Korea, Republic of); College of Information and Communication Engineering, Sungkyunkwan University, Cheoncheon-dong 300, Jangan-gu, Suwon 440-746 (Korea, Republic of); Lee, Hyung-Ik; Park, Jong-Bong; Ko, Dong-Su; Chung, JaeGwan; Kim, KiHong; Kim, Seong Heon; Yun, Dong-Jin; Ham, YongNam; Park, Gyeong Su [Analytical Engineering Group, Samsung Advanced Institute of Technology, 130 Samsung-ro, Yeongtong-gu, Suwon-si, Gyeonggi-do 443-803 (Korea, Republic of); Song, Taewon [Energy lab, Samsung Advanced Institute of Technology, 130 Samsung-ro, Yeongtong-gu, Suwon-si, Gyeonggi-do 443-803 (Korea, Republic of); Lee, Dongho, E-mail: dhlee0333@gmail.com; Nam, Junggyu [PV Development Team, Energy Solution Business Division, Samsung SDI, 467 Beonyeong-ro, Cheonan-si, Chungcheongnam-do 331-330 (Korea, Republic of); Kang, Hee Jae [Department of Physics, Chungbuk National University, Gaesin-dong, Heungdeok-gu, Cheongju, 361-763 (Korea, Republic of); Choi, Pyung-Ho; Choi, Byoung-Deog, E-mail: bdchoi@skku.edu [College of Information and Communication Engineering, Sungkyunkwan University, Cheoncheon-dong 300, Jangan-gu, Suwon 440-746 (Korea, Republic of)

    2015-06-29

    To investigate the band gap profile of Cu(In{sub 1−x},Ga{sub x})(Se{sub 1−y}S{sub y}){sub 2} of various compositions, we measured the band gap profile directly as a function of in-depth using high-resolution reflection energy loss spectroscopy (HR-REELS), which was compared with the band gap profile calculated based on the auger depth profile. The band gap profile is a double-graded band gap as a function of in-depth. The calculated band gap obtained from the auger depth profile seems to be larger than that by HR-REELS. Calculated band gaps are to measure the average band gap of the spatially different varying compositions with respect to considering its void fraction. But, the results obtained using HR-REELS are to be affected by the low band gap (i.e., out of void) rather than large one (i.e., near void). Our findings suggest an analytical method to directly determine the band gap profile as function of in-depth.

  1. Energy loss of muons in the energy range 1-10000 GeV

    International Nuclear Information System (INIS)

    Lohmann, W.; Kopp, R.; Voss, R.

    1985-01-01

    A summary is given of the most recent formulae for the cross-sections contributing to the energy loss of muons in matter, notably due to electro-magnetic interactions (ionization, bremsstrahlung and electron-pair production) and nuclear interactions. Computed energy losses dE/dx are tabulated for muons with energy between 1 GeV and 10,000 GeV in a number of materials commonly used in high-energy physics experiments. In comparison with earlier tables, these show deviations that grow with energy and amount to several per cent at 200 GeV muon energy. (orig.)

  2. Observations of discrete energy loss effects in spectra of positrons reflected from solid surfaces

    International Nuclear Information System (INIS)

    Dale, J.M.; Hulett, L.D.; Pendyala, S.

    1980-01-01

    Surfaces of tungsten and silicon have been bombarded with monoenergetic beams of positrons and electrons. Spectra of reflected particles show energy loss tails with discrete peaks at kinetic energies about 15 eV lower than that of the elastic peaks. In the higher energy loss range for tungsten, positron spectra show fine structure that is not apparent in the electron spectra. This suggests that the positrons are losing energy through mechanisms different from that of the electrons

  3. X-ray emission reduction and photon dose lowering by energy loss of fast electrons induced by return current during the interaction of a short-pulse high-intensity laser on a metal solid target

    Science.gov (United States)

    Compant La Fontaine, A.

    2018-04-01

    During the interaction of a short-pulse high-intensity laser with the preplasma produced by the pulse's pedestal in front of a high-Z metal solid target, high-energy electrons are produced, which in turn create an X-ray source by interacting with the atoms of the converter target. The current brought by the hot electrons is almost completely neutralized by a return current j → driven by the background electrons of the conductive target, and the force exerted on the hot electrons by the electric field E → which induces Ohmic heating j → .E → , produced by the background electrons, reduces the energy of the hot electrons and thus lowers the X-ray emission and photon dose. This effect is analyzed here by means of a simple 1-D temperature model which contains the most significant terms of the relativistic Fokker-Planck equation with electron multiple scattering, and the energy equations of ions, hot, and cold electrons are then solved numerically. This Ohmic heating energy loss fraction τOh is introduced as a corrective term in an improved photon dose model. For instance, for a ps laser pulse with 10 μm spot size, the dose obtained with a tantalum target is reduced by less than about 10% to 40% by the Ohmic heating, depending upon the plasma scale length, target thickness, laser parameters, and in particular its spot size. The laser and plasma parameters may be optimized to limit the effect of Ohmic heating, for instance at a small plasma scale length or small laser spot size. Conversely, others regimes not suitable for dose production are identified. For instance, the resistive heating is enhanced in a foam target or at a long plasma scale length and high laser spot size and intensity, as the mean emission angle θ0 of the incident hot electron bunch given by the ponderomotive force is small; thus, the dose produced by a laser interacting in a gas jet may be inhibited under these circumstances. The resistive heating may also be maximized in order to reduce

  4. An overview of heavy quark energy loss puzzle at RHIC

    International Nuclear Information System (INIS)

    Djordjevic, Magdalena

    2006-01-01

    We give a theoretical overview of the heavy quark tomography puzzle posed by recent non-photonic single electron data from central Au+Au collisions at √s = 200A GeV. We show that radiative energy loss mechanisms alone are not able to explain large single electron suppression data, as long as realistic parameter values are assumed. We argue that a combined collisional and radiative pQCD approach can solve a substantial part of the non-photonic single electron puzzle

  5. Energy loss and charge exchange processes of high energy heavy ions channeled in crystals

    International Nuclear Information System (INIS)

    Poizat, J.C.; Andriamonje, S.; Anne, R.; Faria, N.V.d.C.; Chevallier, M.; Cohen, C.; Dural, J.; Farizon-Mazuy, B.; Gaillard, M.J.; Genre, R.; Hage-Ali, M.; Kirsch, R.; L'hoir, A.; Mory, J.; Moulin, J.; Quere, Y.; Remillieux, J.; Schmaus, D.; Toulemonde, M.

    1990-01-01

    The interaction of moving ions with single crystals is very sensitive to the orientation of the incident beam with respect to the crystalline directions of the target. Our experiments show that high energy heavy ion channeling deeply modifies their slowing down and charge exchange processes. This is due to the fact that channeled ions interact only with outershell target electrons, which means that the electron density they experience is very low and that the binding energy, and then the momentum distribution of these electrons, are quite different from the corresponding average values associated to random incidence. The two experimental studies presented here show the reduction of the energy loss rate for fast channeled heavy ions and illustrate the two aspects of channeling effects on charge exchange, the reduction of electron loss on one hand, and of electron capture on the other hand

  6. Examining Relativistic Electron Loss in the Outer Radiation Belt

    Science.gov (United States)

    Green, J. C.; Onsager, T. G.; O'Brien, P.

    2003-12-01

    Since the discovery of earth's radiation belts researchers have sought to identify the mechanisms that dictate the seemingly erratic relativistic electron flux levels in the outer belt. Contrary to intuition, relativistic electron flux levels do not always increase during geomagnetic storms even though these storms signify enhanced energy input from the solar wind to the magnetosphere [Reeves et al., 2003; O'Brien et al., 2001]. The fickle response of the radiation belt electrons to geomagnetic activity suggests that flux levels are determined by the outcome of a continuous competition between acceleration and loss. Some progress has been made developing and testing acceleration mechanisms but little is known about how relativistic electrons are lost. We examine relativistic electron losses in the outer belt focusing our attention on flux decrease events of the type first described by Onsager et al. [2002]. The study showed a sudden decrease of geosynchronous >2MeV electron flux occurring simultaneously with local stretching of the magnetic field. The decrease was first observed near 15:00 MLT and progressed to all local times after a period of ˜10 hours. Expanding on the work of Onsager et al. [2002], we have identified ˜ 51 such flux decrease events in the GOES and LANL data and present the results of a superposed epoch analysis of solar wind data, geomagnetic activity indicators, and locally measured magnetic field and plasma data. The analysis shows that flux decreases occur after 1-2 days of quiet condition. They begin when either the solar wind dynamic pressure increases or Bz turns southward pushing hot dense plasma earthward to form a partial ring current and stretched magnetic field at dusk. Adiabatic electron motion in response to the stretched magnetic field may explain the initial flux reduction; however, often the flux does not recover with the magnetic field recovery, indicating that true loss from the magnetosphere is occurring. Using Polar and

  7. Microgrids: Energy management by loss minimization technique

    Energy Technology Data Exchange (ETDEWEB)

    Basu, A.K. [Electrical Engineering Dept., Jadavpur University & 20/2, Khanpur Road, Kolkata 700047 (India); Chowdhury, S.; Chowdhury, S.P. [Electrical Engineering Department, University of Cape Town & Private Bag X3, Menzies Building, Room-517, Rondebosch, Cape Town 7701 (India)

    2011-07-01

    Energy management is a techno-economic issue, which dictates, in the context of microgrids, how optimal investment in technology front could bring optimal power quality and reliability (PQR) of supply to the consumers. Investment in distributed energy resources (DERs), with their connection to the utility grid at optimal locations and with optimal sizes, saves energy in the form of line loss reduction. Line loss reduction is the indirect benefit to the microgrid owner who may recover it as an incentive from utility. The present paper focuses on planning of optimal siting and sizing of DERs based on minimization of line loss. Optimal siting is done, here, on the loss sensitivity index (LSI) method and optimal sizing by differential evolution (DE) algorithms, which is, again, compared with particle swarm optimization (PSO) technique. Studies are conducted on 6-bus and 14-bus radial networks under islanded mode of operation with electric demand profile. Islanding helps planning of DER capacity of microgrid, which is self-sufficient to cater its own consumers without utility's support.

  8. Turbulent energy losses during orchard heating

    Energy Technology Data Exchange (ETDEWEB)

    Bland, W.L.

    1979-01-01

    Two rapid-response drag anemometers and low time constant thermocouples, all at 4 m above a heated orchard floor, sampled wind component in the vertical direction and temperature at 30 Hz. The turbulent heat flux calculated revealed not more than 10% of the heat lost from the orchard was via turbulent transort. The observations failed to support previous estimates that at least a third of the energy applied was lost through turbulent transport. Underestimation of heat loss due to mean flow and a newly revealed flux due to spatial variations in the mean flow may explain the unaccounted for loss.

  9. 19 CFR 360.108 - Loss of electronic licensing privileges.

    Science.gov (United States)

    2010-04-01

    ... 19 Customs Duties 3 2010-04-01 2010-04-01 false Loss of electronic licensing privileges. 360.108 Section 360.108 Customs Duties INTERNATIONAL TRADE ADMINISTRATION, DEPARTMENT OF COMMERCE STEEL IMPORT MONITORING AND ANALYSIS SYSTEM § 360.108 Loss of electronic licensing privileges. Should Commerce determine...

  10. Low energy electron transport in furfural

    Science.gov (United States)

    Lozano, Ana I.; Krupa, Kateryna; Ferreira da Silva, Filipe; Limão-Vieira, Paulo; Blanco, Francisco; Muñoz, Antonio; Jones, Darryl B.; Brunger, Michael J.; García, Gustavo

    2017-09-01

    We report on an initial investigation into the transport of electrons through a gas cell containing 1 mTorr of gaseous furfural. Results from our Monte Carlo simulation are implicitly checked against those from a corresponding electron transmission measurement. To enable this simulation a self-consistent cross section data base was constructed. This data base is benchmarked through new total cross section measurements which are also described here. In addition, again to facilitate the simulation, our preferred energy loss distribution function is presented and discussed.

  11. Formation of a superhigh energy electron spectrum in the Galaxy

    International Nuclear Information System (INIS)

    Agaronyan, F.A.; Ambartsumyan, A.S.

    1985-01-01

    The formation of superhigh energy electron spectrum in the disk of the galaxy and halo is considered. A different behaviour of the electron spectrum within the framework of capture models in disk or halo, in the energy region E> or approximately 10 5 GeV is revealed due to the account of relativistic corrections ir the energy losses of electrons during the inverse Compton scattering. A comparison with the existing experimental data is carried out

  12. Experimental study of single-electron loss by Ar+ ions in rare-gas atoms

    Science.gov (United States)

    Reyes, P. G.; Castillo, F.; Martínez, H.

    2001-04-01

    Absolute differential and total cross sections for single-electron loss were measured for Ar+ ions on rare-gas atoms in the laboratory energy range of 1.5 to 5.0 keV. The electron loss cross sections for all the targets studied are found to be in the order of magnitude between 10-19 and 10-22 cm2, and show a monotonically increasing behaviour as a function of the incident energy. The behaviour of the total single-electron loss cross sections with the atomic target number, Zt, shows different dependences as the collision energy increases. In all cases the present results display experimental evidence of saturation in the single-electron loss cross section as the atomic number of the target increases.

  13. Limiting energy loss distributions for multiphoton channeling radiation

    International Nuclear Information System (INIS)

    Bondarenco, M.V.

    2015-01-01

    Recent results in the theory of multiphoton spectra for coherent radiation sources are overviewed, with the emphasis on channeling radiation. For the latter case, the importance of the order of resummation and averaging is emphasized. Limiting shapes of multiphoton spectra at high intensity are discussed for different channeling regimes. In some spectral regions, there emerges a correspondence between the radiative energy loss and the electron integrals of motion

  14. Nanoscale investigation of the degradation mechanism of a historical chrome yellow paint by quantitative electron energy loss spectroscopy mapping of chromium species.

    Science.gov (United States)

    Tan, Haiyan; Tian, He; Verbeeck, Jo; Monico, Letizia; Janssens, Koen; Van Tendeloo, Gustaaf

    2013-10-18

    Getting the picture: The investigation of 100 year old chrome yellow paint by transmission electron microscopy and spectroscopy has led to the identification of four types of core-shell particles. This nanoscale investigation has allowed a mechanism to be proposed for the darkening of some bright yellow colors in Van Gogh's paintings (e.g. in Falling leaves (Les Alyscamps), 1888). Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  15. Comprehensive Power Losses Model for Electronic Power Transformer

    DEFF Research Database (Denmark)

    Yue, Quanyou; Li, Canbing; Cao, Yijia

    2018-01-01

    and considering the impact of the non-unity power factor and the three-phase unbalanced current, the overall power losses in the distribution network when using the EPT to replace the conventional transformer is analyzed, and the conditions in which the application of the EPT can cause less power losses...... reduced power losses in the distribution network require a comprehensive consideration when comparing the power losses of theEPT and conventional transformer. In this paper, a comprehensive power losses analysis model for the EPT in distribution networks is proposed. By analyzing the EPT self-losses......The electronic power transformer (EPT) has highe rpower losses than the conventional transformer. However, the EPT can correct the power factor, compensate the unbalanced current and reduce the line power losses in the distribution network.Therefore, the higher losses of the EPT and the consequent...

  16. Comprehensive Power Losses Model for Electronic Power Transformer

    DEFF Research Database (Denmark)

    Yue, Quanyou; Li, Canbing; Cao, Yijia

    2018-01-01

    The electronic power transformer (EPT) has highe rpower losses than the conventional transformer. However, the EPT can correct the power factor, compensate the unbalanced current and reduce the line power losses in the distribution network.Therefore, the higher losses of the EPT and the consequent...... reduced power losses in the distribution network require a comprehensive consideration when comparing the power losses of theEPT and conventional transformer. In this paper, a comprehensive power losses analysis model for the EPT in distribution networks is proposed. By analyzing the EPT self......-losses and considering the impact of the non-unity power factor and the three-phase unbalanced current, the overall power losses in the distribution network when using the EPT to replace the conventional transformer is analyzed, and the conditions in which the application of the EPT can cause less power losses...

  17. High energy polarized electron beams

    International Nuclear Information System (INIS)

    Rossmanith, R.

    1987-01-01

    In nearly all high energy electron storage rings the effect of beam polarization by synchrotron radiation has been measured. The buildup time for polarization in storage rings is of the order of 10 6 to 10 7 revolutions; the spins must remain aligned over this time in order to avoid depolarization. Even extremely small spin deviations per revolution can add up and cause depolarization. The injection and the acceleration of polarized electrons in linacs is much easier. Although some improvements are still necessary, reliable polarized electron sources with sufficiently high intensity and polarization are available. With the linac-type machines SLC at Stanford and CEBAF in Virginia, experiments with polarized electrons will be possible

  18. Diffraction of high energy electrons

    International Nuclear Information System (INIS)

    Bourret, A.

    1981-10-01

    The diffraction of electrons by a crystal is examined to study its structure. As the electron-substance interaction is strong, it must be treated in a dynamic manner. Using the N waves theory and physical optics the base equations giving the wave at the outlet are deduced for a perfect crystal and their equivalence is shown. The more complex case of an imperfect crystal is then envisaged in these two approaches. In both cases, only the diffraction of high energy electrons ( > 50 KeV) are considered since in the diffraction of slow electrons back scattering cannot be ignored. Taking into account an increasingly greater number of beams, through fast calculations computer techniques, enables images to be simulated in very varied conditions. The general use of the Fast Fourier Transform has given a clear cut practical advantage to the multi-layer method [fr

  19. Sawtooth-induced loss of runaway electrons in tokamaks

    International Nuclear Information System (INIS)

    Yan Longwen; Shi Bingren; Jiao Yiming

    2001-01-01

    A model based on banana orbit loss has been proposed to explain the sawtooth effect on the loss of the runaway electrons in tokamaks. Circulating runaway electrons can be transferred into the trapped ones due to magnetic perturbation during sawtooth crashes, then they are repelled to the limiter via toroidal precession drift with a time delay. This model may also clarify the hard X-ray oscillations correlated with the m = 2 mode and the hard X-ray bursts during outer disruptions

  20. Magnetic energy analyser for slow electrons

    International Nuclear Information System (INIS)

    Limberg, W.

    1974-08-01

    A differential spectrometer with high time and energy resolution has been developed using the principle of energy analysis with a longitudinal homogeneous magnetic field. This way it is possible to measure the energy distribution of low energy electrons (eV-range) in the presence of high energy electrons without distortions by secondary electrons. The functioning and application of the analyzer is demonstrated by measuring the energy distributions of slow electrons emitted by a filament. (orig.) [de

  1. Loss mechanism of the superthermal electrons across the separatrix into the scrape-off layer in DIVA

    International Nuclear Information System (INIS)

    Yamamoto, Shin; Sengoku, Seio; Kimura, Haruyuki; Shimomura, Yasuo; Maeda, Hikosuke

    1977-10-01

    Behavior of superthermal electrons is investigated by using X-ray measurement and electrostatic energy analyser. Superthermal electrons are divided into two groups; i.e. high energy electrons (10 keV - 100 keV) and epithermal electrons (150 eV - 500 eV). Loss flux of the epithermal electrons is obtained and their loss is shown to be explained by destruction of magnetic surfaces near the separatrix due to non-axisymmetric perturbations. Two-dimensional path of high energy electrons is obtained and the effects of non-axisymmetric perturbations on the drift surface are described. (auth.)

  2. Optimal Allocation of Renewable Energy Sources for Energy Loss Minimization

    Directory of Open Access Journals (Sweden)

    Vaiju Kalkhambkar

    2017-03-01

    Full Text Available Optimal allocation of renewable distributed generation (RDG, i.e., solar and the wind in a distribution system becomes challenging due to intermittent generation and uncertainty of loads. This paper proposes an optimal allocation methodology for single and hybrid RDGs for energy loss minimization. The deterministic generation-load model integrated with optimal power flow provides optimal solutions for single and hybrid RDG. Considering the complexity of the proposed nonlinear, constrained optimization problem, it is solved by a robust and high performance meta-heuristic, Symbiotic Organisms Search (SOS algorithm. Results obtained from SOS algorithm offer optimal solutions than Genetic Algorithm (GA, Particle Swarm Optimization (PSO and Firefly Algorithm (FFA. Economic analysis is carried out to quantify the economic benefits of energy loss minimization over the life span of RDGs.

  3. Electron clouds in high energy hadron accelerators

    Energy Technology Data Exchange (ETDEWEB)

    Petrov, Fedor

    2013-08-29

    The formation of electron clouds in accelerators operating with positrons and positively charge ions is a well-known problem. Depending on the parameters of the beam the electron cloud manifests itself differently. In this thesis the electron cloud phenomenon is studied for the CERN Super Proton Synchrotron (SPS) and Large Hadron Collider (LHC) conditions, and for the heavy-ion synchrotron SIS-100 as a part of the FAIR complex in Darmstadt, Germany. Under the FAIR conditions the extensive use of slow extraction will be made. After the acceleration the beam will be debunched and continuously extracted to the experimental area. During this process, residual gas electrons can accumulate in the electric field of the beam. If this accumulation is not prevented, then at some point the beam can become unstable. Under the SPS and LHC conditions the beam is always bunched. The accumulation of electron cloud happens due to secondary electron emission. At the time when this thesis was being written the electron cloud was known to limit the maximum intensity of the two machines. During the operation with 25 ns bunch spacing, the electron cloud was causing significant beam quality deterioration. At moderate intensities below the instability threshold the electron cloud was responsible for the bunch energy loss. In the framework of this thesis it was found that the instability thresholds of the coasting beams with similar space charge tune shifts, emittances and energies are identical. First of their kind simulations of the effect of Coulomb collisions on electron cloud density in coasting beams were performed. It was found that for any hadron coasting beam one can choose vacuum conditions that will limit the accumulation of the electron cloud below the instability threshold. We call such conditions the ''good'' vacuum regime. In application to SIS-100 the design pressure 10{sup -12} mbar corresponds to the good vacuum regime. The transition to the bad vacuum

  4. Energy Loss of Coasting Gold Ions and Deuterons in RHIC

    CERN Document Server

    Abreu, N P; Brown, K; Burkhardt, H; Butler, J; Fischer, W; Harvey, M; Tepikian, S

    2008-01-01

    The total energy loss of coasting gold ion beams at two different energies and deuterons at one energy were measured at RHIC, corresponding to a gamma of 75.2, 107.4 and 108.7 respectively. We describe the experiment and observations and compare the measured total energy loss with expectations from ionization losses at the residual gas, the energy loss due to impedance and synchrotron radiation. We find that the measured energy losses are below what is expected from free space synchrotron radiation. We believe that this shows evidence for suppression of synchrotron radiation which is cut off at long wavelength by the presence of the conducting beam pipe.

  5. Low energy electron transport in furfural

    International Nuclear Information System (INIS)

    Lozano, A.I.; Garcia, G.; Krupa, K.; Ferreira da Silva, F.; Limao-Vieira, P.; Blanco, F.; Munoz, A.; Jones, D.B.; Brunger, M.J.

    2017-01-01

    The cyclic configuration of the furfural molecule is similar to the 5-membered ring structure constituting the sugar units of the DNA helix, hence its importance in biology. In this paper, we report on an initial investigation into the transport of electrons through a gas cell containing 1 mtorr of gaseous furfural. Results from our Monte Carlo simulation are implicitly checked against those from a corresponding electron transmission measurement. To enable this simulation a self-consistent cross section data base was constructed. This data base is benchmarked through new total cross section measurements which are also described here. In addition, again to facilitate the simulation, our preferred energy loss distribution function is presented and discussed

  6. Electron Linacs for High Energy Physics

    International Nuclear Information System (INIS)

    Wilson, Perry B.

    2011-01-01

    The purpose of this article is to introduce some of the basic physical principles underlying the operation of electron linear accelerators (electron linacs). Electron linacs have applications ranging from linacs with an energy of a few MeV, such that the electrons are approximately relativistic, to future electron-positron linear colliders having a collision energy in the several-TeV energy range. For the most part, only the main accelerating linac is treated in this article.

  7. Implementing tactical plans to improve water-energy loss management

    OpenAIRE

    Loureiro, D.; Alegre, H.; Silva, M. S.; Ribeiro, R.; Mamade, A.; Poças, A.

    2015-01-01

    Water utilities are aware of the water-energy loss relevance in supply systems. However, they still mainly focus on daily water loss control (real and apparent losses), without considering the impact on embedded energy. Moreover, they are mostly concerned with the economic dimension and, in most cases, tend to disregard the impact that water-energy loss may have on the quality of service, communication with the customers, social awareness, water quality and environment. This paper focuses on ...

  8. Absolute single electron loss in collisions of Ar+ with various atoms

    Science.gov (United States)

    Reyes, P. G.; Martínez, H.; Castillo, F.

    2001-07-01

    Absolute differential and total cross sections for single electron loss were measured for Ar+ ions on various atoms in the energy range of 1.5 to 5.0 keV. The laboratory angular scan for the distributions ranged from -2.5 to 2.5 degrees. The measured differential cross sections have been integrated over the experimental angular range providing absolute total cross sections. The behavior of the total electron loss cross sections with the target atomic number, Zt, shows different dependences as the collision energy increases. In all cases it displays a saturation as Zt increases.

  9. Energy-loss measurements with heavy ions at relativistic energies

    International Nuclear Information System (INIS)

    Blank, B.; Gaimard, J.J.; Geissel, H.; Muenzenberg, G.; Schmidt, K.H.; Stelzer, H.; Suemmerer; Clerc, H.G.; Hanelt, E.; Steiner, M.; Voss, B.

    1990-03-01

    Using the magnetic spectrometer SPES I at SATURNE, energy-loss measurements have been performed for projectiles of 40 Ar (401 MeV/u), 36 P (362 MeV/u), 15 N (149 MeV/u), 11 Li (131 MeV/u) and 8 Li, 9 Li (130 MeV/u) in carbon, aluminum and lead targets. The experimental results are compared to calculations based on a modified relativistic Bethe formula and to a semi-empirical formula using a Z 2 scaling law for the stopping power and an effective charge parametrization for the heavy ions. (orig.)

  10. Power Electronics, Energy Harvesting and Renewable Energies Laboratory

    Data.gov (United States)

    Federal Laboratory Consortium — The research in the Power Electronics, Energy Harvesting and Renewable Energies Laboratory (PEHREL) is mainly focused on investigation, modeling, simulation, design,...

  11. Improving a radiative plus collisional energy loss model for application to RHIC and LHC

    International Nuclear Information System (INIS)

    Wicks, Simon; Gyulassy, Miklos

    2007-01-01

    With the QGP opacity computed perturbatively and with the global entropy constraints imposed by the observed dN ch /dy ∼ 1000, radiative energy loss alone cannot account for the observed suppression of single non-photonic electrons. Collisional energy loss is comparable in magnitude to radiative loss for both light and heavy jets. Two aspects that significantly affect the collisional energy loss are examined: the role of fluctuations and the effect of introducing a running QCD coupling as opposed to the fixed α s = 0.3 used previously

  12. A proximal retarding field analyzer for scanning probe energy loss spectroscopy

    Science.gov (United States)

    Bauer, Karl; Murphy, Shane; Palmer, Richard E.

    2017-03-01

    A compact proximal retarding field analyzer for scanning probe energy loss spectroscopy measurements is described. Using the scanning tunneling microscope (STM) tip as a field emission (FE) electron source in conjunction with this analyzer, which is placed at a glancing angle to the surface plane, FE sample current and electron reflectivity imaging may be performed simultaneously. This is demonstrated in measurements of Ag nanostructures prepared on graphite by electron-beam lithography, where a material contrast of 13% is observed, with a lateral resolution of 25 nm, between the silver and graphite in electron reflectivity images. Topological contrast mechanisms such as edge enhancement and shadowing are also observed, giving rise to additional features in the electron reflectivity images. The same instrument configuration has been used to measure electron energy loss spectra on bare graphite, where the zero loss peak, π band plasmon loss peak and secondary electron peaks are observed. Using this simple and compact analyzer an STM, with sufficient open access to the tip-sample junction, may easily be augmented to provide simultaneous elemental and topographic mapping, supplementing STM image measurements with FE sample current and electron reflectivity images, as well as electron energy loss spectroscopy measurements, in the same instrument.

  13. Secondary Electron Emission Beam Loss Monitor for LHC

    CERN Document Server

    Dehning, B; Holzer, E B; Kramer, Daniel

    2008-01-01

    Beam Loss Monitoring (BLM) system is a vital part of the active protection of the LHC accelerators' elements. It should provide the number of particles lost from the primary hadron beam by measuring the radiation field induced by their interaction with matter surrounding the beam pipe. The LHC BLM system will use ionization chambers as standard detectors but in the areas where very high dose rates are expected, the Secondary Emission Monitor (SEM) chambers will be employed because of their high linearity, low sensitivity and fast response. The SEM needs a high vacuum for proper operation and has to be functional for up to 20 years, therefore all the components were designed according to the UHV requirements and a getter pump was included. The SEM electrodes are made of Ti because of its Secondary Emission Yield (SEY) stability. The sensitivity of the SEM was modeled in Geant4 via the Photo-Absorption Ionization module together with custom parameterization of the very low energy secondary electron production. ...

  14. Angular distribution of scattered electron and medium energy electron spectroscopy for metals

    International Nuclear Information System (INIS)

    Oguri, Takeo; Ishioka, Hisamichi; Fukuda, Hisashi; Irako, Mitsuhiro

    1986-01-01

    The angular distribution (AD) of scattered electrons produced by medium energy incident electrons (E P = 50 ∼ 300 eV) from polycrystalline Ti, Fe, Ni, Cu and Au were obtained by the angle-resolved medium energy electron spectrometer. The AD of the energy loss peaks are similar figures to AD of the elastically reflected electron peaks. Therefore, the exchanged electrons produced by the knock-on collision between the incident electrons and those of metals without momentum transfer are observed as the energy loss spectra (ELS). This interpretation differs from the inconsequent interpretation by the dielectric theory or the interband transition. The information depth and penetration length are obtained from AD of the Auger electron peaks. The contribution of the surface to spectra is 3 % at the maximum for E P = 50 eV. The true secondary peaks representing the secondary electron emission spectroscopy (SES) are caused by the emissions of the energetic electrons (kT e ≥ 4 eV), and SES is the inversion of ELS. The established fundamental view is that the medium energy electron spectra represent the total bulk density of states. (author)

  15. Gamma rays from relativistic electrons undergoing Compton losses in isotropic photon fields

    International Nuclear Information System (INIS)

    Zdziarski, A.A.

    1989-01-01

    The kinetic equation describing Compton losses of relativistic electrons in an isotropic field of soft background photons is solved exactly including both continuous energy losses in the classical Thomson regime and catastrophic losses in the quantum Klein-Nishina regime. This extends the previous treatments of this problem, which assumed the validity of either one of these regimes alone. The problem is relevant to astrophysical sources containing relativistic electrons. Analytical solutions for the steady state electron and gamma-ray spectra in the case of power-law soft photons and monoenergetic and power-law electron injections are obtained. Numerical solutions are presented for monoenergetic, blackbody, and power-law soft photons. A comparison between the numerical and the available analytic solutions is made. 15 refs

  16. Electron loss from heavy heliumlike projectiles in ultrarelativistic collisions with many-electron atomic targets

    International Nuclear Information System (INIS)

    Mueller, C.; Gruen, N.; Voitkiv, A.B.

    2002-01-01

    We study single- and double-electron loss from heavy heliumlike projectiles in ultrarelativistic collisions with neutral many-electron target atoms. The simultaneous interaction of the target with two projectile electrons is found to be the dominant process in the double-electron loss provided the atomic number of the projectile, Z p , that of the target, Z t , and the collision velocity, v, satisfy the condition Z p Z t /v>0.4. It is shown that for a wide range of projectile and target atomic numbers the asymptotic double-to-single loss ratio strongly depends on the target atomic number but is nearly independent of the nuclear charge of the projectile. It is also demonstrated that many-photon exchange between the target and each of the projectile electrons considerably influences the double loss in collisions with very heavy targets

  17. Thermalisation of high energy electrons and positrons in water vapour

    Science.gov (United States)

    Munoz, A.; Blanco, F.; Limao-Vieira, P.; Thorn, P. A.; Brunger, M. J.; Buckman, S. J.; Garcia, G.

    2008-07-01

    In this study we describe a method to simulate single electron tracks of electrons in molecular gases, particularly in water vapour, from relatively high energies, where Born (Inokuti 1971) approximation is supposed to be valid, down to thermal energies paying special attention to the low energy secondary electrons which are abundantly generated along the energy degradation procedure. Experimental electron scattering cross sections (Munoz et al. 2007) and energy loss spectra (Thorn et al. 2007) have been determined, where possible, to be used as input parameters of the simulating program. These experimental data have been complemented with optical potential calculation (Blanco and Garcia 2003) providing a complete set of interaction probability functions for each type of collision which could take place in the considered energy range: elastic, ionization, electronic excitation, vibrational and rotational excitation. From the simulated track structure (Munoz et al. 2005) information about energy deposition and radiation damage at the molecular level can be derived. A similar procedure is proposed to the study of single positron tracks in gases. Due to the lack of experimental data for positron interaction with molecules, especially for those related to energy loss and excitation cross sections, some distribution probability data have been derived from those of electron scattering by introducing positron characteristics as positroniun formation. Preliminary results for argon are presented discussing also the utility of the model to biomedical applications based on positron emitters.

  18. High-energy electron diffraction and microscopy

    CERN Document Server

    Peng, L M; Whelan, M J

    2011-01-01

    This book provides a comprehensive introduction to high energy electron diffraction and elastic and inelastic scattering of high energy electrons, with particular emphasis on applications to modern electron microscopy. Starting from a survey of fundamental phenomena, the authors introduce the most important concepts underlying modern understanding of high energy electron diffraction. Dynamical diffraction in transmission (THEED) and reflection (RHEED) geometries is treated using ageneral matrix theory, where computer programs and worked examples are provided to illustrate the concepts and to f

  19. Power electronics for renewable energy systems

    DEFF Research Database (Denmark)

    Iov, Florin; Blaabjerg, Frede

    2009-01-01

    sources from the conventional, fossil (and short term) based energy sources to renewable energy resources. Another is to use high efficient power electronics in power generation, power transmission/distribution and end-user application. This paper discuss some of the most emerging renewable energy sources......, wind energy and photovoltaics, which by means of power electronics are changing from being minor energy sources to be acting as important power sources in the energy system....

  20. Acceleration and loss of relativistic electrons during small geomagnetic storms.

    Science.gov (United States)

    Anderson, B R; Millan, R M; Reeves, G D; Friedel, R H W

    2015-12-16

    Past studies of radiation belt relativistic electrons have favored active storm time periods, while the effects of small geomagnetic storms ( D s t  > -50 nT) have not been statistically characterized. In this timely study, given the current weak solar cycle, we identify 342 small storms from 1989 through 2000 and quantify the corresponding change in relativistic electron flux at geosynchronous orbit. Surprisingly, small storms can be equally as effective as large storms at enhancing and depleting fluxes. Slight differences exist, as small storms are 10% less likely to result in flux enhancement and 10% more likely to result in flux depletion than large storms. Nevertheless, it is clear that neither acceleration nor loss mechanisms scale with storm drivers as would be expected. Small geomagnetic storms play a significant role in radiation belt relativistic electron dynamics and provide opportunities to gain new insights into the complex balance of acceleration and loss processes.

  1. Effects of dynamic diffraction conditions on magnetic parameter determination in a double perovskite Sr{sub 2}FeMoO{sub 6} using electron energy-loss magnetic chiral dichroism

    Energy Technology Data Exchange (ETDEWEB)

    Wang, Z.C. [National Center for Electron Microscopy in Beijing, Key Laboratory of Advanced Materials (MOE), The State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing 100084 (China); Zhong, X.Y., E-mail: xyzhong@mail.tsinghua.edu.cn [National Center for Electron Microscopy in Beijing, Key Laboratory of Advanced Materials (MOE), The State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing 100084 (China); Jin, L. [Peter Grünberg Institute and Ernst Ruska-Centre for Microscopy and Spectroscopy with Electrons (ER-C), Forschungszentrum Jülich, 52425 Jülich (Germany); Chen, X.F. [National Center for Electron Microscopy in Beijing, Key Laboratory of Advanced Materials (MOE), The State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing 100084 (China); Moritomo, Y. [Graduate School of Pure & Applied Science and Faculty of Pure & Applied Science, University of Tsukuba, Tennodai 1-1-1, Tsukuba, Ibaraki 305-7571 (Japan); Mayer, J. [Peter Grünberg Institute and Ernst Ruska-Centre for Microscopy and Spectroscopy with Electrons (ER-C), Forschungszentrum Jülich, 52425 Jülich (Germany); Central Facility for Electron Microscopy, RWTH Aachen University, 52074 Aachen (Germany)

    2017-05-15

    Electron energy-loss magnetic chiral dichroism (EMCD) spectroscopy, which is similar to the well-established X-ray magnetic circular dichroism spectroscopy (XMCD), can determine the quantitative magnetic parameters of materials with high spatial resolution. One of the major obstacles in quantitative analysis using the EMCD technique is the relatively poor signal-to-noise ratio (SNR), compared to XMCD. Here, in the example of a double perovskite Sr{sub 2}FeMoO{sub 6}, we predicted the optimal dynamical diffraction conditions such as sample thickness, crystallographic orientation and detection aperture position by theoretical simulations. By using the optimized conditions, we showed that the SNR of experimental EMCD spectra can be significantly improved and the error of quantitative magnetic parameter determined by EMCD technique can be remarkably lowered. Our results demonstrate that, with enhanced SNR, the EMCD technique can be a unique tool to understand the structure-property relationship of magnetic materials particularly in the high-density magnetic recording and spintronic devices by quantitatively determining magnetic structure and properties at the nanometer scale. - Highlights: • We demonstrate how to choose the optimal experimental conditions by using dynamical diffraction calculations in Sr{sub 2}FeMoO{sub 6}. • With optimized diffraction conditions, the signal-to-noise ratio of experimental EMCD spectra has been significantly improved. • We have determined orbital to spin magnetic moment ratio of Sr{sub 2}FeMoO{sub 6} quantitatively. • We have discussed the effects of dynamical diffraction conditions on the error bar of quantitative magnetic parameters.

  2. Energy loss of MeV protons specularly reflected from metal surfaces

    International Nuclear Information System (INIS)

    Juaristi, J.I.; Garcia de Abajo, F.J.; Echenique, P.M.

    1996-01-01

    A parameter-free model is presented to study the energy loss of fast protons specularly reflected from metal surfaces. The contributions to the energy loss from excitation of valence-band electrons and ionization of localized target-atom electronic states are calculated separately. The former is calculated from the induced surface wake potential using linear response theory and the specular-reflection model, while the latter is calculated in the first Born approximation. The results obtained are in good agreement with available experimental data. However, the experimental qualitative trend of the energy loss as a function of the angle of incidence is obtained when the valence-band electron model is replaced by localized target atom electron states, though with a worse quantitative agreement. copyright 1996 The American Physical Society

  3. Local energy losses at positive and negative steps in subcritical ...

    African Journals Online (AJOL)

    Local energy losses occur when there is a transition in open channel flow. Even though local losses in subcritical open channel flow due to changes in channel width have been studied, to date no studies have been reported for losses due to changes in bed elevations. Steps are commonly used in engineering applications ...

  4. Energy losses of superconducting power transmission cables in the grid

    DEFF Research Database (Denmark)

    Østergaard, Jacob; Okholm, Jan; Lomholt, Karin

    2001-01-01

    One of the obvious motives for development of superconducting power transmission cables is reduction of transmission losses. Loss components in superconducting cables as well as in conventional cables have been examined. These losses are used for calculating the total energy losses of conventional...... as well as superconducting cables when they are placed in the electric power transmission network. It is concluded that high load connections are necessary to obtain energy saving by the use of HTSC cables. For selected high load connections, an energy saving of 40% is expected. It is shown...

  5. Distorted wave calculations for electron loss process induced by bare ion impact on biological targets

    International Nuclear Information System (INIS)

    Monti, J.M.; Tachino, C.A.; Hanssen, J.; Fojón, O.A.; Galassi, M.E.; Champion, C.; Rivarola, R.D.

    2014-01-01

    Distorted wave models are employed to investigate the electron loss process induced by bare ions on biological targets. The two main reactions which contribute to this process, namely, the single electron ionization as well as the single electron capture are here studied. In order to further assess the validity of the theoretical descriptions used, the influence of particular mechanisms are studied, like dynamic screening for the case of electron ionization and energy deposition on the target by the impacting projectile for the electron capture one. Results are compared with existing experimental data. - Highlights: ► Distorted wave models are used to investigate ion-molecule collisions. ► Differential and total cross-sections for capture and ionization are evaluated. ► The influence of dynamic screening is determined. ► Capture reaction dominates the mean energy deposited by the projectile on the target

  6. Production and energy loss of strange and heavy quarks

    International Nuclear Information System (INIS)

    2010-01-01

    Data taken over the last several years have demonstrated that RHIC has created a hot, dense medium with partonic degrees of freedom. Identified particle spectra at high transverse momentum (p T ) and heavy flavor that are thought to be well-calibrated probes thus serve as ideal tools to study the properties of the medium. We present p T distributions of particle ratios in p+p collisions from the STAR experiment to understand the particle production mechanisms. These measurements will also constrain fragmentation functions in hadron-hardon collisions. In heavy-ion collisions, we highlight (1) recent measurements of strange hadrons and heavy flavor decay electrons up to high p T to study jet interaction with the medium and explore partonic energy loss mechanisms, and (2) Υ and high p T J/ψ measurements to study the effect of color screening and other possible production mechanisms.

  7. Electrons with continuous energy distribution from energetic heavy ion collisions

    International Nuclear Information System (INIS)

    Berenyi, D.

    1984-01-01

    The properties and origin of continuous electron spectrum emitted in high energy heavy ion collisions are reviewed. The basic processes causing the characteristic regions of the continuous spectrum are described. The contribution of electrons ejected from the target and from the projectile are investigated in detail in the cases of light and heavy projectiles. The recently recognized mechanisms, electron-capture-to-continuum (ECC) and electron-loss-to-continuum (ELC), leading to a cusp in forward direction, and their theoretical interpretations are discussed. The importance of data from ion-atom collisions in the field of atomic physics and in applications are briefly summarized. (D.Gy)

  8. Energy-dependent losses in pulsed-feedback preamplifiers

    International Nuclear Information System (INIS)

    Landis, D.A.; Madden, N.W.; Goulding, F.S.

    1978-11-01

    Energy dependent counting losses occur in most pulsed-feedback preamplifiers due to the loss of those pulses which activate the recharge system. A pulsed-feedback system that overcomes this inefficiency is described. Pulsed-light feedback as used with germanium gamma-ray spectrometers is discussed as used at high energies and high rates where those losses become significant. Experimental results are presented

  9. Attainment of Electron Beam Suitable for Medium Energy Electron Cooling

    International Nuclear Information System (INIS)

    Seletskiy, Sergey M.; Rochester U.

    2005-01-01

    Electron cooling of charged particle beams is a well-established technique at electron energies of up to 300 keV. However, up to the present time the advance of electron cooling to the MeV-range energies has remained a purely theoretical possibility. The electron cooling project at Fermilab has recently demonstrated the first cooling of 8.9 GeV/c antiprotons in the Recycler ring, and therefore, has proved the validity of the idea of relativistic electron cooling. The Recycler Electron Cooler (REC) is the key component of the Tevatron Run II luminosity upgrade project. Its performance depends critically on the quality of electron beam. A stable electron beam of 4.3 MeV carrying 0.5 A of DC current is required. The beam suitable for the Recycler Electron Cooler must have an angular spread not exceeding 200 (micro)rad. The full-scale prototype of the REC was designed, built and tested at Fermilab in the Wideband laboratory to study the feasibility of attaining the high-quality electron beam. In this thesis I describe various aspects of development of the Fermilab electron cooling system, and the techniques used to obtain the electron beam suitable for the cooling process. In particular I emphasize those aspects of the work for which I was principally responsible. Chapter 1 is an introduction where I describe briefly the theory and the history of electron cooling, and derive the requirements to the quality of electron beam and requirements to the basic parameters of the Recycler Electron Cooler. Chapter 2 is devoted to the theoretical consideration of the motion of electrons in the cooling section, description of the cooling section and of the measurement of the magnetic fields. In Chapter 3 I consider different factors that increase the effective electron angle in the cooling section and suggest certain algorithms for the suppression of parasitic angles. Chapter 4 is devoted to the measurements of the energy of the electron beam. In the concluding Chapter 5 I review

  10. Experimental study of single-electron loss by Ar{sup +} ions in rare-gas atoms

    Energy Technology Data Exchange (ETDEWEB)

    Reyes, P.G. [Facultad de Ciencias, UNAM, Coyoacan (Mexico); Castillo, F. [Instituto de Ciencias Nucleares, UNAM, Coyoacan (Mexico); Martinez, H. [Centro de Ciencias Fisicas, UNAM, Cuernavaca, Morelos (Mexico)]. E-mail: hm@fis.unam.mx

    2001-04-28

    Absolute differential and total cross sections for single-electron loss were measured for Ar{sup +} ions on rare-gas atoms in the laboratory energy range of 1.5 to 5.0 keV. The electron loss cross sections for all the targets studied are found to be in the order of magnitude between 10{sup -19} and 10{sup -22} cm{sup 2}, and show a monotonically increasing behaviour as a function of the incident energy. The behaviour of the total single-electron loss cross sections with the atomic target number, Z{sub t}, shows different dependences as the collision energy increases. In all cases the present results display experimental evidence of saturation in the single-electron loss cross section as the atomic number of the target increases. (author)

  11. Power Electronics for Renewable Energy Systems

    DEFF Research Database (Denmark)

    Choi, U. M.; Lee, K. B.; Blaabjerg, Frede

    2012-01-01

    The use of renewable energy sources are increased because of the depletion of natural resources and the increasing pollution level from energy production. The wind energy and the solar energy are most widely used among the renewable energy sources. Power electronics is needed in almost all kinds...... of renewable energy system. It controls the renewable source and interfaces with the load effectively, which can be grid-connected or van work in stand-alone mode. In this presentation, overview of wind and photovoltaic energy systems are introduced. Next, the power electronic circuits behind the most common...

  12. Inelastic energy loss in large angle scattering of Ar9+ ions from Au(1 1 1) crystal

    International Nuclear Information System (INIS)

    Pesic, Z.D.; Anton, J.; Bremer, J.H.; Hoffmann, V.; Stolterfoht, N.; Vikor, Gy.; Schuch, R.

    2003-01-01

    The azimuthal angle dependence of the energy loss in large-angle scattering of slow (v∼0.06 a.u.) Ar 9+ ions from a Au(1 1 1) single crystal was investigated. Regarding the kinematics of quasi-single collisions, the smallest energy loss is expected for the azimuthal orientations which correspond to the closest packed atomic row of the crystal. This agrees with the prediction of a trajectory simulation (Marlowe code), but the experimental results don't show such dependence. Thus, we discuss possible inelastic processes as image charge energy gain, electronic energy loss in close collision and the electronic energy loss in the interaction with the electron gas. The observed azimuthal dependence is explained by the change of the electronic stopping power due to the variation of effective electron density sampled by the projectile

  13. Elucidating Jet Energy Loss Using Jets Prospects from ATLAS

    CERN Document Server

    Grau, N

    2009-01-01

    Jets at the LHC are expected to provide the testing ground for studying QCD energy loss. In this contribution, we briefly outline the strategy that will be used to measure jets in ATLAS and how we will go about studying energy loss. We describe the utility of measuring the jet $R_{AA}$, the fragmentation function, and heavy flavor jets. Utilizing the collision energy provided by the LHC and the nearly hermetic and highly segmented calorimeter, ATLAS is expected to make important contributions to the understanding of parton energy loss using fully reconstructed jets.

  14. Elucidating Jet Energy Loss Using Jets: Prospects from ATLAS

    International Nuclear Information System (INIS)

    Grau, N.

    2009-01-01

    Jets at the LHC are expected to provide the testing ground for studying QCD energy loss. In this contribution, we briefly outline the strategy that will be used to measure jets in ATLAS and how we will go about studying energy loss. We describe the utility of measuring the jet R AA , the fragmentation function, and heavy flavor jets. Utilizing the collision energy provided by the LHC and the nearly hermetic and highly segmented calorimeter, ATLAS is expected to make important contributions to the understanding of parton energy loss using fully reconstructed jets.

  15. Energy loss of charged particles to molecular gas targets

    International Nuclear Information System (INIS)

    Sigmund, P.

    1976-01-01

    The energy loss spectrum of fast charged particles penetrating a dilute molecular gas target has been analysed theoretically, with a homogeneous gas mixture in the state of complete dissociation as a reference standard. It is shown that the geometrical structure of molecules causes the energy-loss straggling and higher moments over the energy-loss spectrum to be greater than the corresponding quantities for a completely dissociated gas of equal composition. Such deviations from additivity are shown to be most pronounced at energies around the stopping-power maximum. There is found supporting evidence in the experimental literature. (Auth.)

  16. LRSPC, Proton High-Energy Loss in Matter

    International Nuclear Information System (INIS)

    2001-01-01

    1 - Description of program or function: The LRSPC program is designed to estimate the energy loss, due to ionization and excitation, and the range of charged particles passing through matter. The code treats protons in elements or mixtures composed of elements with atomic numbers ranging from 1 to 100. The results for protons are generally valid from 1 MeV to 100 GeV. The code may be extended to treat other charged particles such as muons, pions, hyperons, deuterons, tritons and alphas by changing the particle mass, charge and range at 2 MeV. 2 - Method of solution: Stopping power is calculated from the Bethe-Bloch equation with shell and density corrections included. Range is calculated by integrating the reciprocal of the stopping power from an initial value at 2 MeV. The K-shell correction is taken from Walske's data. The L-shell and higher shell corrections are adjusted to fit low energy measurements fro 30 elements. The density correction is calculated by a method similar to that of Sternheimer, differing chiefly in the large number of electron shells considered. LRSPC computes improved proton range and stopping power data for use in the proton penetration code, LPPC (CCC-0051). It is packages separately and may be requested independently. 3 - Restrictions on the complexity of the problem: Number of elements in mixture ≤ 10, Atomic number of element ≤ 100, Number of energy points ≤ 500

  17. Attainment of Electron Beam Suitable for Medium Energy Electron Cooling

    Energy Technology Data Exchange (ETDEWEB)

    Seletskiy, Sergei M. [Univ. of Rochester, NY (United States)

    2005-01-01

    Electron cooling of charged particle beams is a well-established technique at electron energies of up to 300 keV. However, up to the present time the advance of electron cooling to the MeV-range energies has remained a purely theoretical possibility. The electron cooling project at Fermilab has recently demonstrated the ¯rst cooling of 8.9 GeV/c antiprotons in the Recycler ring, and therefore, has proved the validity of the idea of relativistic electron cool- ing. The Recycler Electron Cooler (REC) is the key component of the Teva- tron Run II luminosity upgrade project. Its performance depends critically on the quality of electron beam. A stable electron beam of 4.3 MeV car- rying 0.5 A of DC current is required. The beam suitable for the Recycler Electron Cooler must have an angular spread not exceeding 200 ¹rad. The full-scale prototype of the REC was designed, built and tested at Fermilab in the Wideband laboratory to study the feasibility of attaining the high-quality electron beam. In this thesis I describe various aspects of development of the Fermilab electron cooling system, and the techniques used to obtain the electron beam suitable for the cooling process. In particular I emphasize those aspects of the work for which I was principally responsible.

  18. Resonance effects in projectile-electron loss in relativistic collisions with excited atoms

    International Nuclear Information System (INIS)

    Voitkiv, A B

    2005-01-01

    The theory of electron loss from projectile-ions in relativistic ion-atom collisions is extended to the case of collisions with excited atoms. The main feature of such collisions is a resonance which can emerge between electron transitions in the ion and atom. The resonance becomes possible due to the Doppler effect and has a well-defined impact energy threshold. In the resonance case, the ion-atom interaction is transmitted by the radiation field and the range of this interaction becomes extremely long. Because of this the presence of other atoms in the target medium and the size of the space occupied by the medium have to be taken into account and it turns out that microscopic loss cross sections may be strongly dependent on such macroscopic parameters as the target density, temperature and size. We consider both the total and differential loss cross sections and show that the resonance can have a strong impact on the angular and energy distributions of electrons emitted from the projectiles and the total number of electron loss events

  19. The energy broadening resulting from electron stripping process of a low energy Au- beam

    International Nuclear Information System (INIS)

    Taniike, Akira; Sasao, Mamiko; Hamada, Yasuji; Fujita, Junji; Wada, Motoi.

    1994-12-01

    Energy loss spectra of Au + ions produced from Au - ions by electron stripping in He, Ar, Kr and Xe have been measured in the impact energy range of 24-44 keV. The energy broadening of the Au + beam increases as the beam energy increases, and the spectrum shows a narrower energy width for heavy target atoms. The dependence of the spectrum width upon the beam energy and that upon the target mass are well described by the calculation based on the unified potential and semi-classical internal energy transfer model of Firsov's. (author)

  20. Inelastic vibrational bulk and surface losses of swift electrons in ionic nanostructures

    Science.gov (United States)

    Hohenester, Ulrich; Trügler, Andreas; Batson, Philip E.; Lagos, Maureen J.

    2018-04-01

    In a recent paper [Lagos et al., Nature (London) 543, 533 (2017), 10.1038/nature21699] we have used electron energy loss spectroscopy with sub-10 meV energy and atomic spatial resolution to map optical and acoustic, bulk and surface vibrational modes in magnesium oxide nanocubes. We found that a local dielectric description works well for the simulation of aloof geometries, similar to related work for surface plasmons and surface plasmon polaritons, while for intersecting geometries such a description fails to reproduce the rich spectral features associated with excitation of bulk acoustic and optical phonons. To account for scatterings with a finite momentum exchange, in this paper we investigate molecular and lattice dynamics simulations of bulk losses in magnesium-oxide nanocubes using a rigid-ion description and investigate the loss spectra for intersecting electron beams. From our analysis we can evaluate the capability of electron energy loss spectroscopy for the investigation of phonon modes at the nanoscale, and we discuss shortcomings of our simplified approach as well as directions for future investigations.

  1. Electron Beam Return-Current Losses in Solar Flares: Initial Comparison of Analytical and Numerical Results

    Science.gov (United States)

    Holman, Gordon

    2010-01-01

    Accelerated electrons play an important role in the energetics of solar flares. Understanding the process or processes that accelerate these electrons to high, nonthermal energies also depends on understanding the evolution of these electrons between the acceleration region and the region where they are observed through their hard X-ray or radio emission. Energy losses in the co-spatial electric field that drives the current-neutralizing return current can flatten the electron distribution toward low energies. This in turn flattens the corresponding bremsstrahlung hard X-ray spectrum toward low energies. The lost electron beam energy also enhances heating in the coronal part of the flare loop. Extending earlier work by Knight & Sturrock (1977), Emslie (1980), Diakonov & Somov (1988), and Litvinenko & Somov (1991), I have derived analytical and semi-analytical results for the nonthermal electron distribution function and the self-consistent electric field strength in the presence of a steady-state return-current. I review these results, presented previously at the 2009 SPD Meeting in Boulder, CO, and compare them and computed X-ray spectra with numerical results obtained by Zharkova & Gordovskii (2005, 2006). The phYSical significance of similarities and differences in the results will be emphasized. This work is supported by NASA's Heliophysics Guest Investigator Program and the RHESSI Project.

  2. Electron correlation energy in confined two-electron systems

    Energy Technology Data Exchange (ETDEWEB)

    Wilson, C.L. [Chemistry Program, Centre College, 600 West Walnut Street, Danville, KY 40422 (United States); Montgomery, H.E., E-mail: ed.montgomery@centre.ed [Chemistry Program, Centre College, 600 West Walnut Street, Danville, KY 40422 (United States); Sen, K.D. [School of Chemistry, University of Hyderabad, Hyderabad 500 046 (India); Thompson, D.C. [Chemistry Systems and High Performance Computing, Boehringer Ingelheim Pharamaceuticals Inc., 900 Ridgebury Road, Ridgefield, CT 06877 (United States)

    2010-09-27

    Radial, angular and total correlation energies are calculated for four two-electron systems with atomic numbers Z=0-3 confined within an impenetrable sphere of radius R. We report accurate results for the non-relativistic, restricted Hartree-Fock and radial limit energies over a range of confinement radii from 0.05-10a{sub 0}. At small R, the correlation energies approach limiting values that are independent of Z while at intermediate R, systems with Z{>=}1 exhibit a characteristic maximum in the correlation energy resulting from an increase in the angular correlation energy which is offset by a decrease in the radial correlation energy.

  3. Electron capture and energy-gain spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Taulbjerg, K.

    1989-01-01

    The applicability of translation energy spectroscopy as a tool to determine individual reaction cross sections in atomic collisions is analyzed with special emphasis on the electron capture process in highly charged ion collisions. A condition is derived to separate between higher collision energies where translation energy spectroscopy is problem free and lower energies where strong overlap of individual spectra features prohibits an analysis of the total translation energy spectrum by means of a simple deconvolution procedure. 8 refs., 6 figs.

  4. Measurements of energy losses, distributions of energy loss and additivity of energy losses for 50 to 150 keV protons in hydrogen and nine hydrocarbon gases

    International Nuclear Information System (INIS)

    Thorngate, J.H.

    1976-05-01

    Measurements of energy-loss distributions were made for 51, 102, and 153 keV protons traversing hydrogen, methane, ethyne (acetylene), ethene (ethylene), ethane, propyne (methyl acetylene), propadiene (allene), propene (propylene), cyclopropane and propane. The objectives were to test the theories of energy-loss distribution in this energy range and to see if the type of carbon bonding in a hydrocarbon molecule affects the shape of the distribution. Stopping powers and stopping cross sections were also measured at these energies and at 76.5 and 127.5 keV to determine effects of chemical binding. All of the measurements were made at the gas density required to give a 4 percent energy loss. The mean energy, second central moment (a measure of the width of the distribution), and the third central moment (a measure of the skew) were calculated from the measured energy-loss distributions. Stopping power values, calculated using the mean energy, compared reasonably well with those calculated from the Bethe stopping power theory. For the second and third central moments, the best agreement between measurement and theory was when the classical scattering probability was used for the calculations, but even these did not agree well. In all cases, variations were found in the data that could be correlated to the type of carbon binding in the molecule. The differences were statistically significant at a 99 percent confidence interval for the stopping powers and second central moments measured with 51 keV protons. Similar trends were noted at other energies and for the third central moment, but the differences were not statistically significant at the 99 percent confidence interval

  5. Holographic energy loss in non-relativistic backgrounds

    Energy Technology Data Exchange (ETDEWEB)

    Atashi, Mahdi; Fadafan, Kazem Bitaghsir; Farahbodnia, Mitra [Shahrood University of Technology, Physics Department, P.O. Box 3619995161, Shahrood (Iran, Islamic Republic of)

    2017-03-15

    In this paper, we study some aspects of energy loss in non-relativistic theories from holography. We analyze the energy lost by a rotating heavy point particle along a circle of radius l with angular velocity ω in theories with general dynamical exponent z and hyperscaling violation exponent θ. It is shown that this problem provides a novel perspective on the energy loss in such theories. A general computation at zero and finite temperature is done and it is shown how the total energy loss rate depends non-trivially on two characteristic exponents (z,θ). We find that at zero temperature there is a special radius l{sub c} where the energy loss is independent of different values of (θ,z). Also at zero temperature, there is a crossover between a regime in which the energy loss is dominated by the linear drag force and by the radiation because of the acceleration of the rotating particle. We find that the energy loss of the particle decreases by increasing θ and z. We note that, unlike in the zero temperature, there is no special radius l{sub c} at finite temperature case. (orig.)

  6. Ultrafast Electron Dynamics in Solar Energy Conversion.

    Science.gov (United States)

    Ponseca, Carlito S; Chábera, Pavel; Uhlig, Jens; Persson, Petter; Sundström, Villy

    2017-08-23

    Electrons are the workhorses of solar energy conversion. Conversion of the energy of light to electricity in photovoltaics, or to energy-rich molecules (solar fuel) through photocatalytic processes, invariably starts with photoinduced generation of energy-rich electrons. The harvesting of these electrons in practical devices rests on a series of electron transfer processes whose dynamics and efficiencies determine the function of materials and devices. To capture the energy of a photogenerated electron-hole pair in a solar cell material, charges of opposite sign have to be separated against electrostatic attractions, prevented from recombining and being transported through the active material to electrodes where they can be extracted. In photocatalytic solar fuel production, these electron processes are coupled to chemical reactions leading to storage of the energy of light in chemical bonds. With the focus on the ultrafast time scale, we here discuss the light-induced electron processes underlying the function of several molecular and hybrid materials currently under development for solar energy applications in dye or quantum dot-sensitized solar cells, polymer-fullerene polymer solar cells, organometal halide perovskite solar cells, and finally some photocatalytic systems.

  7. Dependence of electron inelastic mean free paths on electron energy and materials at low energy region, 1

    International Nuclear Information System (INIS)

    Tanuma, Shigeo; Powell, C.J.; Penn, D.R.

    1990-01-01

    We have proposed a general formula of electron inelastic mean free path (IMFP) to describe the calculated IMFPs over the 50-2000 eV energy range based on the Inokuti's modified Bethe formula for the inelastic scattering cross section. The IMFPs for 50-2000 eV electrons in 27 elements were calculated using Penn's algorithm. The IMFP dependence on electron energy in the range 50-200 eV varies considerably from material to material. These variations are associated with substantial differences in the electron energy-loss functions amongst the material. We also found that the modified Bethe formula by Inokuti could be fitted to the calculated IMFPs in the range 50-2000 eV within 3% relative error. (author)

  8. Evaluating the Role and Effects of Precipitation on Relativistic Electron Losses during Storms

    Science.gov (United States)

    Chen, Y.; Fu, X.

    2016-12-01

    Theoretic studies have suggested that during storm times various waves (e.g., whistler-mode chorus and electromagnetic ion cyclotron waves) can cause significant precipitation of relativistic ( MeV) electrons that are originally trapped inside the outer radiation belt. However, the role of precipitation and its quantitative contribution to the losses of outer-belt electrons remain open questions. In this study, we tackle these questions by systemically examining the latest wave and electron in-situ, simultaneous observations made at different altitudes by Van Allen Probes from near equator, NOAA POES at low Earth orbits near/across electron loss cone, and BARREL under the mesosphere. After calibrating with DEMTER observations, we first confirm and quantify the response of POES MEPED proton channels to MeV electrons. Next, we identify a list of precipitation events from BARREL and POES measurements, examine the temporal adn spatial relation between the two data sets, and estimate the intensities of electron precipitation with ascertained uncertainties. Then, from Van Allen Probes data, we select another list of dropout events during storms. By cross checking the above two lists, we are able to determine the causal relation between precipitation and dropouts through individual case as well as statistical studies so as to quantify the contributions from precipitation. This study mainly focuses on the relatively small L-shells with positive phase space density radial gradient in order to alleviate the impacts from outward radial diffusion and adiabatic effects. Based upon the recent discovery of cross-energy cross-pitch angle coherence, we pay particular attention to the cross-term diffusions which may account for the extra "loss" needed by observed MeV electron dropouts. Results from this observational study will advance our knowledge on the loss mechanism of outer-belt electrons, and thus lay down another stepping stone towards high-fidelity physics-based models for

  9. Kramers-Kronig transform for the surface energy loss function

    International Nuclear Information System (INIS)

    Tan, G.L.; DeNoyer, L.K.; French, R.H.; Guittet, M.J.; Gautier-Soyer, M.

    2005-01-01

    A new pair of Kramers-Kronig (KK) dispersion relationships for the transformation of surface energy loss function Im[-1/(ε + 1)] has been proposed. The validity of the new surface KK transform is confirmed, using both a Lorentz oscillator model and the surface energy loss functions determined from the experimental complex dielectric function of SrTiO 3 and tungsten metal. The interband transition strength spectra (J cv ) have been derived either directly from the original complex dielectric function or from the derived dielectric function obtained from the KK transform of the surface energy loss function. The original J cv trace and post-J cv trace overlapped together for the three modes, indicating that the new surface Kramers-Kronig dispersion relationship is valid for the surface energy loss function

  10. Local energy losses at positive and negative steps in subcritical ...

    African Journals Online (AJOL)

    2010-04-22

    Apr 22, 2010 ... channel flow due to changes in channel width have been studied, to date no studies have been reported for losses due to changes in bed elevations. .... of these studies report on numerical modelling of flow over transitions. ... that the frictional losses are negligible, the energy equation between Sections (1) ...

  11. NaI(Tl) electron energy resolution

    CERN Document Server

    Mengesha, W

    2002-01-01

    NaI(Tl) electron energy resolution eta sub e was measured using the Modified Compton Coincidence Technique (MCCT). The MCCT allowed detection of nearly monoenergetic internal electrons resulting from the scattering of incident 662 keV gamma rays within a primary NaI(Tl) detector. Scattered gamma rays were detected using a secondary HPGe detector in a coincidence mode. Measurements were carried out for electron energies ranging from 16 to 438 keV, by varying the scattering angle. Measured HPGe coincidence spectra were deconvolved to determine the scattered energy spectra from the NaI(Tl) detector. Subsequently, the NaI(Tl) electron energy spectra were determined by subtracting the energy of scattered spectra from the incident source energy (662 keV). Using chi-squared minimization, iterative deconvolution of the internal electron energy spectra from the measured NaI(Tl) spectra was then used to determine eta sub e at the electron energy of interest. eta sub e values determined using this technique represent va...

  12. Monte Carlo electron-transport calculations for clinical beams using energy grouping

    Energy Technology Data Exchange (ETDEWEB)

    Teng, S P; Anderson, D W; Lindstrom, D G

    1986-01-01

    A Monte Carlo program has been utilized to study the penetration of broad electron beams into a water phantom. The MORSE-E code, originally developed for neutron and photon transport, was chosen for adaptation to electrons because of its versatility. The electron energy degradation model employed logarithmic spacing of electron energy groups and included effects of elastic scattering, inelastic-moderate-energy-loss-processes and inelastic-large-energy-loss-processes (catastrophic). Energy straggling and angular deflections were modeled from group to group, using the Moeller cross section for energy loss, and Goudsmit-Saunderson theory to describe angular deflections. The resulting energy- and electron-deposition distributions in depth were obtained at 10 and 20 MeV and are compared with ETRAN results and broad beam experimental data from clinical accelerators.

  13. Model calculation for energy loss in ion-surface collisions

    International Nuclear Information System (INIS)

    Miraglia, J.E.; Gravielle, M.S.

    2003-01-01

    The so-called local plasma approximation is generalized to deal with projectiles colliding with surfaces of amorphous solids and with a specific crystalline structure (plannar channeling). Energy loss of protons grazingly colliding with aluminum, SnTe alloy, and LiF surfaces is investigated. The calculations agree quite well with previous theoretical results and explain the experimental findings of energy loss for aluminum and SnTe alloy, but they fall short to explain the data for LiF surfaces

  14. Can Low Energy Electrons Affect High Energy Physics Accelerators?

    International Nuclear Information System (INIS)

    Cimino, Roberto

    2004-01-01

    The properties of the electrons participating in the build up of an electron cloud (EC) inside the beam-pipe have become an increasingly important issue for present and future accelerators whose performance may be limited by this effect. The EC formation and evolution are determined by the wall-surface properties of the accelerator vacuum chamber. Thus, the accurate modeling of these surface properties is an indispensible input to simulation codes aimed at the correct prediction of build-up thresholds, electron-induced instability or EC heat load. In this letter, we present the results of surface measurements performed on a prototype of the beam screen adopted for the Large Hadron Collider (LHC), which presently is under construction at CERN. We have measured the total secondary electron yield (SEY) as well as the related energy distribution curves (EDC) of the secondary electrons as a function of incident electron energy. Attention has been paid, for the first time in this context, to the probability at which low-energy electrons (<∼ 20 eV) impacting on the wall create secondaries or are elastically reflected. It is shown that the ratio of reflected to true-secondary electrons increases for decreasing energy and that the SEY approaches unity in the limit of zero primary electron energy

  15. Reactions induced by low energy electrons in cryogenic films

    International Nuclear Information System (INIS)

    Bass, A.D.; Sanche, L.

    2003-01-01

    We review recent research on reactions (including dissociation) initiated by low-energy electron bombardment of monolayer and multilayer molecular solids at cryogenic temperatures. With incident electrons of energies below 20 eV, dissociation is observed by the electron stimulated desorption (ESD) of anions from target films and is attributed to the processes of dissociative electron attachment (DEA) and to dipolar dissociation. It is shown that DEA to condensed molecules is sensitive to environmental factors such as the identity of co-adsorbed species and film morphology. The effects of image-charge induced polarization on cross-sections for DEA to CH3Cl are also discussed. Taking as examples, the electron-induced production of CO within multilayer films of methanol and acetone, it is shown that the detection of electronic excited states by high resolution electron energy loss spectroscopy can be used to monitor electron beam damage. In particular, the incident energy dependence of the CO indicates that below 19 eV, dissociation proceeds via the decay of transient negative ions (TNI) into electronically excited dissociative states. The electron induced dissociation of biomolecular targets is also considered, taking as examples the ribose analog tetrahydrofuran and DNA bases adenine and thymine, cytosine and guanine. The ESD of anions from such films also show dissociation via the formation of TNI. In multilayer molecular solids, fragment species resulting from dissociation, may react with neighboring molecules, as is demonstrated in anion ESD measurements from films containing O 2 and various hydrocarbon molecules. X-ray photoelectron spectroscopy measurements reported for electron irradiated monolayers of H 2 O and CF 4 on a Si - H passivated surface further show that DEA is an important initial step in the electron-induced chemisorption of fragment species

  16. Radiative energy loss of neighboring subjets arXiv

    CERN Document Server

    Mehtar-Tani, Yacine

    We compute the in-medium energy loss probability distribution of two neighboring subjets at leading order, in the large-$N_c$ approximation. Our result exhibits a gradual onset of color decoherence of the system and accounts for two expected limiting cases. When the angular separation is smaller than the characteristic angle for medium-induced radiation, the two-pronged substructure lose energy coherently as a single color charge, namely that of the parent parton. At large angular separation the two subjets lose energy independently. Our result is a first step towards quantifying effects of energy loss as a result of the fluctuation of the multi-parton jet substructure and therefore goes beyond the standard approach to jet quenching based on single parton energy loss. We briefly discuss applications to jet observables in heavy-ion collisions.

  17. Probing low-energy hyperbolic polaritons in van der Waals crystals with an electron microscope.

    Science.gov (United States)

    Govyadinov, Alexander A; Konečná, Andrea; Chuvilin, Andrey; Vélez, Saül; Dolado, Irene; Nikitin, Alexey Y; Lopatin, Sergei; Casanova, Fèlix; Hueso, Luis E; Aizpurua, Javier; Hillenbrand, Rainer

    2017-07-21

    Van der Waals materials exhibit intriguing structural, electronic, and photonic properties. Electron energy loss spectroscopy within scanning transmission electron microscopy allows for nanoscale mapping of such properties. However, its detection is typically limited to energy losses in the eV range-too large for probing low-energy excitations such as phonons or mid-infrared plasmons. Here, we adapt a conventional instrument to probe energy loss down to 100 meV, and map phononic states in hexagonal boron nitride, a representative van der Waals material. The boron nitride spectra depend on the flake thickness and on the distance of the electron beam to the flake edges. To explain these observations, we developed a classical response theory that describes the interaction of fast electrons with (anisotropic) van der Waals slabs, revealing that the electron energy loss is dominated by excitation of hyperbolic phonon polaritons, and not of bulk phonons as often reported. Thus, our work is of fundamental importance for interpreting future low-energy loss spectra of van der Waals materials.Here the authors adapt a STEM-EELS system to probe energy loss down to 100 meV, and apply it to map phononic states in hexagonal boron nitride, revealing that the electron loss is dominated by hyperbolic phonon polaritons.

  18. Probing low-energy hyperbolic polaritons in van der Waals crystals with an electron microscope

    KAUST Repository

    Govyadinov, Alexander A.

    2017-07-14

    Van der Waals materials exhibit intriguing structural, electronic, and photonic properties. Electron energy loss spectroscopy within scanning transmission electron microscopy allows for nanoscale mapping of such properties. However, its detection is typically limited to energy losses in the eV range-too large for probing low-energy excitations such as phonons or mid-infrared plasmons. Here, we adapt a conventional instrument to probe energy loss down to 100 meV, and map phononic states in hexagonal boron nitride, a representative van der Waals material. The boron nitride spectra depend on the flake thickness and on the distance of the electron beam to the flake edges. To explain these observations, we developed a classical response theory that describes the interaction of fast electrons with (anisotropic) van der Waals slabs, revealing that the electron energy loss is dominated by excitation of hyperbolic phonon polaritons, and not of bulk phonons as often reported. Thus, our work is of fundamental importance for interpreting future low-energy loss spectra of van der Waals materials.Here the authors adapt a STEM-EELS system to probe energy loss down to 100 meV, and apply it to map phononic states in hexagonal boron nitride, revealing that the electron loss is dominated by hyperbolic phonon polaritons.

  19. Probing low-energy hyperbolic polaritons in van der Waals crystals with an electron microscope

    KAUST Repository

    Govyadinov, Alexander A.; Konečná , Andrea; Chuvilin, Andrey; Vé lez, Saü l; Dolado, Irene; Nikitin, Alexey Y.; Lopatin, Sergei; Casanova, Fè lix; Hueso, Luis E.; Aizpurua, Javier; Hillenbrand, Rainer

    2017-01-01

    Van der Waals materials exhibit intriguing structural, electronic, and photonic properties. Electron energy loss spectroscopy within scanning transmission electron microscopy allows for nanoscale mapping of such properties. However, its detection is typically limited to energy losses in the eV range-too large for probing low-energy excitations such as phonons or mid-infrared plasmons. Here, we adapt a conventional instrument to probe energy loss down to 100 meV, and map phononic states in hexagonal boron nitride, a representative van der Waals material. The boron nitride spectra depend on the flake thickness and on the distance of the electron beam to the flake edges. To explain these observations, we developed a classical response theory that describes the interaction of fast electrons with (anisotropic) van der Waals slabs, revealing that the electron energy loss is dominated by excitation of hyperbolic phonon polaritons, and not of bulk phonons as often reported. Thus, our work is of fundamental importance for interpreting future low-energy loss spectra of van der Waals materials.Here the authors adapt a STEM-EELS system to probe energy loss down to 100 meV, and apply it to map phononic states in hexagonal boron nitride, revealing that the electron loss is dominated by hyperbolic phonon polaritons.

  20. The distribution of infered energetic electron loss with respect to plasmapause location: BARREL results.

    Science.gov (United States)

    Halford, A. J.; Malaspina, D.; Sibeck, D. G.

    2017-12-01

    One of the long outstanding challenges of understanding the inner magnetosphere is accurately describing radiation belt dynamics. This enterprise can seem daunting as many have stated: "if you've seen one storm you've seen one storm". And although much progress has been made over the last half century since the discovery of the radiation belts, there is still ongoing debate about the relative importance of different loss and source mechanisms. Here we will consider one part of radiation belt dynamics, the loss of electrons ( 30 keV to MeV) to the upper atmosphere and endeavor to identify the relative importance of the different loss mechanisms. As demonstrated in often used cartoon diagrams, and previous studies, many radiation belt loss mechanisms such as chorus, hiss, and EMIC waves are thought to have specific MLT and L dependencies as well as dependence on geomagnetic conditions. Many of these loss mechanisms are identifiable through the energies and time scales in which they precipitate electrons. Thus we expect that the observed electron precipiation should follow similar MLT and L patterns as what caused the loss and not show something completely unexpected such as Atlantis rising out of the Columbia River. Here we will examine the location and geomagnetic conditions under which the Balloon Array for Relativistic Radiation Belt Electron Loss (BARREL) inferred radiation belt electron precipitation. The BARREL mission consisted of 4 campaigns, two in Antarctica and 2 in Sweden, for a total of 55 launches. The flights conducted in Antarctica took advantage of the circumpolar winds allowing for the payloads to cross a range of L-values from L > 2.5 onto open field lines, while the Swedish campaigns were held during turn around where the balloons stayed near L = 5.8. We will present the distribution of precipitation with respect to L and MLT as well as with respect to the boundary of the plasmapause as new work has shown that this boundary clearly separates

  1. Electron loss mechanisms in collisions of He+ ions with various targets

    International Nuclear Information System (INIS)

    Sant'Anna, M.M.; Melo, W.S.; Santos, A.C.F.; Sigaud, G.M.; Montenegro, E.C.

    1995-01-01

    The electron loss of high-velocity ions by neutral atoms is due to two different and competing mechanisms. In the screening mode, the electron loss is basically due to the nucleus-electron interaction, with the target electrons assuming the passive role of decreasing the Coulomb field of the target nucleus in the vicinity of the projectile active electron. For a fixed projectile velocity, this contribution is expected to give a non-linear dependence with the target atomic number Z 2 due to the incomplete screening at the impact parameter region where the projectile ionization is more likely to occur. Within first-order theories, if the screening is completely absent, the expected dependence would be Z 2 2 ; with screening, it should scale between Z 2 and Z 2 2 . On the other hand, in the antiscreening mode, where the loss is due to the action of the target electrons and the target nucleus plays no active role, the expected dependence would be approximately linear with Z 2 . Thus, for first-order theories, the expected overall dependence with Z 2 would be dominated by the screening mode as Z 2 increases. We have measured total electron-loss cross sections of He + ions impinging upon He, Ne, Ar, Kr and Xe targets in the energy range from 1.0 to 4.0 MeV to complement previous measurements and the results point towards a much smaller contribution from the screening mode than expected from first-order theories, possibly due to a saturation effect manifested only in the screening channel. (orig.)

  2. Food irradiation by low energy electrons

    International Nuclear Information System (INIS)

    Bird, J.R.

    1985-01-01

    For some special cases, the use of low energy electrons has advantages over the use of gamma-rays or higher energy electrons for the direct irradiation of food. These advantages arise from details of the interaction processes which are responsible for the production of physical, chemical and biological effects. Factors involved include depth of penetration, dose distribution, irradiation geometry, the possible production of radioactivity and costs

  3. Surface sterilization by low energy electron beams

    International Nuclear Information System (INIS)

    Sekiguchi, Masayuki; Tabei, Masae

    1989-01-01

    The germicidal effectiveness of low energy electron beams (175 KV) against bacterial cells was investigated. The dry spores of Bacillus pumilus ATCC 27142 and Bacillus globigii ATCC 9372 inoculated on carrier materials and irradiated by gamma rays showed the exponential type of survival curves whereas they showed sigmoidal ones when exposed to low energy electron beams. When similarly irradiated, the wet spores inoculated on membrane filter showed the same survival curves as the dry spores inoculated on carrier materials. The wet vegetative cells of Escherichia coli ATCC 25922 showed exponential curves when exposed to gamma and electron beam irradiation. Low energy electron beams in air showed little differences from nitrogen stream in their germicidal effectiveness against dry spores of B. pumilus. The D values of B. pumilus spores inoculated on metal plates decreased as the amounts of backscattering electrons from the plates increased. There was adequate correlation between the D value (linear region of survival curve), average D value (6D/6) and 1% survival dose and backscattering factor. Depth dose profile and backscatterig dose of low energy electron beams were measured by radiochromic dye film dosimeter (RCD). These figures were not always in accord with the observed germicidal effectiveness against B. pumilus spores because of varying thickness of RCD and spores inoculated on carrier material. The dry spores were very thin and this thinness was useful in evaluating the behavior of low energy electrons. (author)

  4. High energy electron multibeam diffraction and imaging

    International Nuclear Information System (INIS)

    Bourret, Alain.

    1980-04-01

    The different theories of dynamical scattering of electrons are firstly reviewed with special reference to their basis and the validity of the different approximations. Then after a short description of the different experimental set ups, structural analysis and the investigation of the optical potential by means of high energy electrons will be surveyed

  5. Electron energy-distribution functions in gases

    International Nuclear Information System (INIS)

    Pitchford, L.C.

    1981-01-01

    Numerical calculation of the electron energy distribution functions in the regime of drift tube experiments is discussed. The discussion is limited to constant applied fields and values of E/N (ratio of electric field strength to neutral density) low enough that electron growth due to ionization can be neglected

  6. Analytic approach to auroral electron transport and energy degradation

    International Nuclear Information System (INIS)

    Stamnes, K.

    1980-01-01

    The interaction of a beam of auroral electrons with the atmosphere is described by the linear transport equation, encompassing discrete energy loss, multiple scattering, and secondary electrons. A solution to the transport equation provides the electron intensity as a function of altitude, pitch angle (with respect to the geomagnetic field) and energy. A multi-stream (discrete ordinate) approximation to the transport equation is developed. An analytic solution is obtained in this approximation. The computational scheme obtained by combining the present transport code with the energy degradation method of Swartz (1979) conserves energy identically. The theory provides a framework within which angular distributions can be easily calculated and interpreted. Thus, a detailed study of the angular distributions of 'non-absorbed' electrons (i.e., electrons that have lost just a small fraction of their incident energy) reveals a systematic variation with incident angle and energy, and with penetration depth. The present approach also gives simple yet accurate solutions in low order multi-stream approximations. The accuracy of the four-stream approximation is generally within a few per cent, whereas two-stream results for backscattered mean intensities and fluxes are accurate to within 10-15%. (author)

  7. Compact multi-energy electron linear accelerators

    International Nuclear Information System (INIS)

    Tanabe, E.; Hamm, R.W.

    1985-01-01

    Two distinctly different concepts that have been developed for compact multi-energy, single-section, standing-wave electron linear accelerator structures are presented. These new concepts, which utilize (a) variable nearest neighbor couplings and (b) accelerating field phase switching, provide the capability of continuously varying the electron output energy from the accelerator without degrading the energy spectrum. These techniques also provide the means for continuously varying the energy spectrum while maintaining a given average electron energy, and have been tested successfully with several accelerators of length from 0.1 m to 1.9 m. Theoretical amd experimental results from these accelerators, and demonstrated applications of these techniques to medical and industrial linear accelerator technology will be described. In addition, possible new applications available to research and industry from these techniques are presented. (orig.)

  8. A Bench Measurement of the Energy Loss of a Stored Beam to a Cavity

    Energy Technology Data Exchange (ETDEWEB)

    Sands, M; Rees, J.; /SLAC

    2016-12-19

    A rather simple electronic bench experiment is proposed for obtaining a measure of the impulse energy loss of a stored particle bunch to an rf cavity or other vacuum-chamber structure--the so-called "cavity radiation". The proposed method is analyzed in some detail.

  9. Vibrational and electronic excitation of hexatriacontane thin films by low energy electron impact

    International Nuclear Information System (INIS)

    Vilar, M.R.; Schott, M.; Pfluger, P.

    1990-01-01

    Thin polycrystalline films of hexatriacontane (HTC) were irradiated with low energy (E=0.5--15 eV) electrons, and off-specular backscattered electron spectra were measured. Below E∼7 eV, single and multiple vibrational excitations only are observed, which relax the electrons down to the bottom of the HTC conduction band. Due to the negative electron affinity of HTC, thermal electrons are emitted into vacuum. Structure in the backscattered electron current at kinetic energies about 1.5 and 4 eV are associated to conduction band density of states. Above E∼7 eV, the dominant losses correspond to electronic excitations, excitons, or above a threshold (energy of the electron inside the HTC film) at 9.2±0.1 eV, electron--hole pair generation. The latter process is very efficient and reaches a yield of the order of one ∼11 eV. Evidence for chemical reaction above E∼4 eV is observed

  10. High energy electron positron physics

    International Nuclear Information System (INIS)

    Ali, A.; Soding, P.

    1987-01-01

    With the termination of the physics program at PETRA in a year from now, and with the start of TRISTAN and the SLC and later LEP, an era of e/sup +/e/sup -/ physics will come to an end and a new one begins. The field is changing from a field of a few specialists, to becoming one of the mainstream efforts of the high energy community. It seems appropriate at this moment to summarize what has been learned over the past years, in a way more useful to any high energy physicist in particular to newcomers in the e/sup +/e/sup -/ field. This is the purpose of the book. This book should be used as a reference for future workers in the field of e/sup +/e/sup -/ interactions. It includes the most relevant data, parametrizations, theoretical background, and a chapter on detectors. Contents: Foreword; Detectors for High Energy e/sup +/e/sup -/ Physics; Lepton Pair Production and Electroweak Parameters; Hadron Production, Strong and Electroweak Properties; tau Physics; Recent Results on the Charm Sector; Bottom Physics; Lifetime Measurements of tau, Charmed and Beauty Hadrons; Υ Spectroscopy; Hadronic Decays of the Υ; Quark and Gluon Fragmentation in the e/sup +/e/sup -/ Continuum; Jet Production and QCD; Two Photon Physics; Search for New Particles

  11. Electron energy distribution function, effective electron temperature, and dust charge in the temporal afterglow of a plasma

    International Nuclear Information System (INIS)

    Denysenko, I. B.; Azarenkov, N. A.; Kersten, H.

    2016-01-01

    Analytical expressions describing the variation of electron energy distribution function (EEDF) in an afterglow of a plasma are obtained. Especially, the case when the electron energy loss is mainly due to momentum-transfer electron-neutral collisions is considered. The study is carried out for different EEDFs in the steady state, including Maxwellian and Druyvesteyn distributions. The analytical results are not only obtained for the case when the rate for momentum-transfer electron-neutral collisions is independent on electron energy but also for the case when the collisions are a power function of electron energy. Using analytical expressions for the EEDF, the effective electron temperature and charge of the dust particles, which are assumed to be present in plasma, are calculated for different afterglow durations. An analytical expression for the rate describing collection of electrons by dust particles for the case when the rate for momentum-transfer electron-neutral collisions is independent on electron energy is also derived. The EEDF profile and, as a result, the effective electron temperature and dust charge are sufficiently different in the cases when the rate for momentum-transfer electron-neutral collisions is independent on electron energy and when the rate is a power function of electron energy.

  12. Energy loss of ions by electric-field fluctuations in a magnetized plasma.

    Science.gov (United States)

    Nersisyan, Hrachya B; Deutsch, Claude

    2011-06-01

    The results of a theoretical investigation of the energy loss of charged particles in a magnetized classical plasma due to the electric-field fluctuations are reported. The energy loss for a test particle is calculated through the linear-response theory. At vanishing magnetic field, the electric-field fluctuations lead to an energy gain of the charged particle for all velocities. It has been shown that in the presence of strong magnetic field, this effect occurs only at low velocities. In the case of high velocities, the test particle systematically loses its energy due to the interaction with a stochastic electric field. The net effect of the fluctuations is the systematic reduction of the total energy loss (i.e., the sum of the polarization and stochastic energy losses) at vanishing magnetic field and reduction or enhancement at strong field, depending on the velocity of the particle. It is found that the energy loss of the slow heavy ion contains an anomalous term that depends logarithmically on the projectile mass. The physical origin of this anomalous term is the coupling between the cyclotron motion of the plasma electrons and the long-wavelength, low-frequency fluctuations produced by the projectile ion. This effect may strongly enhance the stochastic energy gain of the particle.

  13. Energy spectra variations of high energy electrons in magnetic storms observed by ARASE and HIMAWARI

    Science.gov (United States)

    Takashima, T.; Higashio, N.; Mitani, T.; Nagatsuma, T.; Yoshizumi, M.

    2017-12-01

    The ARASE spacecraft was launched in December 20, 2016 to investigate mechanisms for acceleration and loss of relativistic electrons in the radiation belts during space storms. The six particle instruments with wide energy range (a few eV to 10MeV) are onboard the ARASE spacecraft. Especially, two particle instruments, HEP and XEP observe high energy electron with energy range from 70keV to over 10Mev. Those instruments observed several geomagnetic storms caused by coronal hole high speed streams or coronal mass ejections from March in 2017. The relativistic electrons in the outer radiation belt were disappeared/increased and their energy spectra were changed dynamically in some storms observed by XEP/HEP onboard the ARASE spacecraft. In the same time, SEDA-e with energy range 200keV-4.5MeV for electron on board the HIMAWARI-8, Japanese weather satellite on GEO, observed increase of relativistic electron in different local time. We will report on energy spectra variations of high energy electrons including calibrations of differential flux between XEP and HEP and discuss comparisons with energy spectra between ARAE and HIMAWARI that observed each storm in different local time.

  14. Golden mean energy equals highest atomic electron orbital energy

    Energy Technology Data Exchange (ETDEWEB)

    Malinowski, Leonard J. [Interdisciplinary Research Club, P.O. Box 371, Monroeville, PA 15146 (United States)], E-mail: LJMalinowski@gmail.com

    2009-12-15

    The golden mean numerical value {phi} = 0.5({radical}5 - 1) has been given a physical manifestation through E infinity theory. This short paper relates the golden mean energy 0.618034 MeV to atomic electron orbitals.

  15. Golden mean energy equals highest atomic electron orbital energy

    International Nuclear Information System (INIS)

    Malinowski, Leonard J.

    2009-01-01

    The golden mean numerical value φ = 0.5(√5 - 1) has been given a physical manifestation through E infinity theory. This short paper relates the golden mean energy 0.618034 MeV to atomic electron orbitals.

  16. Energy-Efficiency Options for Insurance Loss Prevention

    Energy Technology Data Exchange (ETDEWEB)

    Mills, E. [Ernest Orlando Lawrence Berkeley National Lab., CA (United States). Environmental Energy Technologies Div.; Knoepfel, I. [Swiss Reinsurance Co., Zurich (Switzerland)

    1997-06-09

    Energy-efficiency improvements offer the insurance industry two areas of opportunity: reducing ordinary claims and avoiding greenhouse gas emissions that could precipitate natural disaster losses resulting from global climate change. We present three vehicles for taking advantage of this opportunity, including research and development, in- house energy management, and provision of key information to insurance customers and risk managers. The complementary role for renewable energy systems is also introduced.

  17. Electron energy measurements in pulsating auroras

    International Nuclear Information System (INIS)

    McEwan, D.J.; Yee, E.; Whalen, B.A.; Yau, A.W.

    1981-01-01

    Electron spectra were obtained during two rocket flights into pulsating aurora from Southend, Saskatchewan. The first rocket launched at 1143:24 UT on February 15, 1980 flew into an aurora of background intensity 275 R of N 2 + 4278 A and showing regular pulsations with about a 17 s period. Electron spectra of Maxwellian energy distributions were observed with an average E 0 = 1.5 keV, rising to 1.8 keV during the pulsations. There was one-to-one correspondence between the electron energy modulation and the observed optical pulsations. The second rocket, launched at 1009:10 UT on February 23, flew into a diffuse auroral surface of intensity 800 R of N 2 + 4278 A and with somewhat irregular pulsations. The electron spectra were again of Maxwellian energy distribution with an average E 0 = 1.8 keV increasing to 2.1 keV during the pulsations. The results from these flights suggest that pulsating auroras occurring in the morning sector may be quite commonly excited by low energy electrons. The optical pulsations are due to periodic increases in the energy of the electrons with the source of modulation in the vicintiy of the geomagnetic equatorial plane. (auth)

  18. Electron-atom scattering at intermediate energies

    International Nuclear Information System (INIS)

    Kingston, A.E.; Walters, H.R.J.

    1982-01-01

    The problems of intermediate energy scattering are approached from the low and high energy ends. At low intermediate energies difficulties associated with the use of pseudostates and correlation terms are discussed, special consideration being given to nonphysical pseudoresonances. Perturbation methods appropriate to high intermediate energies are described and attempts to extend these high energy approximations down to low intermediate energies are studied. It is shown how the importance of electron exchange effects develops with decreasing energy. The problem of assessing the 'effective completeness' of pseudostate sets at intermediate energies is mentioned and an instructive analysis of a 2p pseudostate approximation to elastic e - -H scattering is given. It is suggested that at low energies the Pauli Exclusion Principle can act to hide short range defects in pseudostate approximations. (author)

  19. Low Energy Electron Cooler for NICA Booster

    CERN Document Server

    Denisov, A P

    2017-01-01

    BINP has developed an electron cooler to increase the ion accumulation efficiency in the NICA (Nuclotron-based Ion Collider fAcility) heavy ion booster (JINR, Dubna). Adjustment of the cooler magnetic system provides highly homogeneous magnetic field in the cooling section B trans/B long ≤ 4∙10-5 which is vital for efficient electron cooling. First experiments with an electron beam performed at BINP demonstrated the target DC current of 500 mA and electron energy 6 keV.

  20. The impact of cell culture equipment on energy loss.

    Science.gov (United States)

    Davies, Lleucu B; Kiernan, Michael N; Bishop, Joanna C; Thornton, Catherine A; Morgan, Gareth

    2014-01-01

    Light energy of discrete wavelengths supplied via lasers and broadband intense pulsed light have been used therapeutically for many years. In vitro models complement clinical studies, especially for the elucidation of underlying mechanisms of action. Clarification that light energy reaches the cells is necessary when developing protocols for the treatment of cells using in vitro models. Few studies report on energy loss in cell culture equipment. The ability of energy from light with therapeutic potential to reach cells in culture needs to be determined; this includes determining the proportion of light energy lost within standard cell culture media and cell culture vessels. The energy absorption of cell culture media, with/without the pH indicator dye phenol red, and the loss of energy within different plastics and glassware used typically for in vitro cell culture were investigated using intense pulsed light and a yellow pulsed dye laser. Media containing phenol red have a distinctive absorption peak (560 nm) absent in phenol red-free media and restored by the addition of phenol red. For both light sources, energy loss was lowest in standard polystyrene tissue culture flasks or multi-well plates and highest in polypropylene vessels or glass tubes. The effects of phenol red-free media on the absorption of energy varied with the light source used. Phenol red-free media are the media of choice; polystyrene vessels with flat surfaces such as culture flasks or multi-well plates should be used in preference to polypropylene or glass vessels.

  1. Uncertainty, loss aversion, and markets for energy efficiency

    International Nuclear Information System (INIS)

    Greene, David L.

    2011-01-01

    Increasing energy efficiency is critical to mitigating greenhouse gas emissions from fossil-fuel combustion, reducing oil dependence, and achieving a sustainable global energy system. The tendency of markets to neglect apparently cost-effective energy efficiency options has been called the 'efficiency gap' or 'energy paradox.' The market for energy efficiency in new, energy-using durable goods, however, appears to have a bias that leads to undervaluation of future energy savings relative to their expected value. This paper argues that the bias is chiefly produced by the combination of substantial uncertainty about the net value of future fuel savings and the loss aversion of typical consumers. This framework relies on the theory of context-dependent preferences. The uncertainty-loss aversion bias against energy efficiency is quantifiable, making it potentially correctible by policy measures. The welfare economics of such policies remains unresolved. Data on the costs of increased fuel economy of new passenger cars, taken from a National Research Council study, illustrate how an apparently cost-effective increase in energy efficiency would be uninteresting to loss-averse consumers.

  2. Photoelectron energy-loss study of the Bi2CaSr2Cu2O8 superconductor

    International Nuclear Information System (INIS)

    Shen, Z.; Lindberg, P.A.P.; Dessau, D.S.; Lindau, I.; Spicer, W.E.; Mitzi, D.B.; Bozovic, I.; Kapitulnik, A.

    1989-01-01

    Using energy-loss spectroscopy of photoelectrons from a single crystal of Bi 2 CaSr 2 Cu 2 O 8 , we show that the electronic structure of the near-surface region is the same as that of the bulk. Utilizing the fact that photoelectrons of different elements are excited at different locations in the unit cell, we identify the energy-loss features as due to valence plasmon excitations, and one-electron excitations by comparing the photoelectron energy-loss spectra of the different elements

  3. Electron energy recuperation in gyrodevices

    International Nuclear Information System (INIS)

    Savilov, A. V.; Nusinovich, G. S.; Sinitsyn, O. V.

    2008-01-01

    For many applications of gyrodevices, it is extremely important to increase their overall efficiency and reduce the power consumption. Therefore, at present, there are many gyrotrons operating with depressed collectors. These gyrotrons and their depressed collectors are typically designed with the use of available numerical codes. This paper is devoted to the analysis of the energy recuperation in gyrotrons, which is performed with the use of the Hamiltonian formalism. Such consideration gives some insight into the physics of gyrodevices and can be useful for estimating the benefits from utilizing depressed collectors. Both single-cavity gyromonotrons and multicavity gyrodevices in which the last cavity is excited by a prebunched beam are analyzed. Special attention is paid to a three-cavity, frequency-quadrupling gyrodevice.

  4. A precise measurement of 180 GeV muon energy losses in iron

    Czech Academy of Sciences Publication Activity Database

    Amaral, P.; Amorim, A.; Davídek, T.; Krivková, P.; Leitner, R.; Lokajíček, Miloš; Němeček, Stanislav; Suk, M.; Valkar, S.; Zaitsev, A.

    2001-01-01

    Roč. 20, - (2001), s. 487-495 ISSN 1434-6044 R&D Projects: GA MPO RP-4210/69 Institutional research plan: CEZ:AV0Z1010920 Keywords : energy loss spectrum * muons * hadron Tile calorimeter * CERN SPS * production of electron-positron pairs * energetic knock-on elecktrons * ion elastic form factor correction Subject RIV: BF - Elementary Particles and High Energy Physics Impact factor: 5.194, year: 2001

  5. High-Energy Electron Beam Application to Air Pollutants Removal

    International Nuclear Information System (INIS)

    Ighigeanu, D.; Martin, D.; Manaila, E.; Craciun, G.; Calinescu, I.

    2009-01-01

    The advantage of electron beam (EB) process in pollutants removal is connected to its high efficiency to transfer high amount of energy directly into the matter under treatment. Disadvantage which is mostly related to high investment cost of accelerator may be effectively overcome in future as the result of use accelerator new developments. The potential use of medium to high-energy high power EB accelerators for air pollutants removal is demonstrated in [1]. The lower electrical efficiencies of accelerators with higher energies are partially compensated by the lower electron energy losses in the beam windows. In addition, accelerators with higher electron energies can provide higher beam powers with lower beam currents [1]. The total EB energy losses (backscattering, windows and in the intervening air space) are substantially lower with higher EB incident energy. The useful EB energy is under 50% for 0.5 MeV and about 95% above 3 MeV. In view of these arguments we decided to study the application of high energy EB for air pollutants removal. Two electron beam accelerators are available for our studies: electron linear accelerators ALIN-10 and ALID-7, built in the Electron Accelerator Laboratory, INFLPR, Bucharest, Romania. Both accelerators are of traveling-wave type, operating at a wavelength of 10 cm. They utilize tunable S-band magnetrons, EEV M 5125 type, delivering 2 MW of power in 4 μ pulses. The accelerating structure is a disk-loaded tube operating in the 2 mode. The optimum values of the EB peak current IEB and EB energy EEB to produce maximum output power PEB for a fixed pulse duration EB and repetition frequency fEB are as follows: for ALIN-10: EEB = 6.23 MeV; IEB =75 mA; PEB 164 W (fEB = 100 Hz, EB = 3.5 s) and for ALID-7: EEB 5.5 MeV; IEB = 130 mA; PEB = 670 W (fEB = 250 Hz, EB = 3.75 s). This paper presents a special designed installation, named SDI-1, and several representative results obtained by high energy EB application to SO 2 , NOx and VOCs

  6. Low energy electron scattering from fuels

    International Nuclear Information System (INIS)

    Lopes, M. Cristina A.; Silva, Daniel G.M.; Coelho, Rafael F.; Duque, Humberto V.; Santos, Rodrigo R. dos; Ribeiro, Thiago M.

    2011-01-01

    Full text. Accurate and precise values of absolute total cross section (TCS) represent important information in many scientific and technological applications. In our case, for example, we are motivated to provide such information for electron-fuel collision processes which are specifically relevant to modeling spark ignition in alcohol-fuelled internal combustion engines. Many electron scattering TCS measurements are presently available for a diverse range of atomic and molecular targets. However, lack of data for important bio-molecular targets still remains. Disagreements between the available TCS data for the alcohols have prompted several studies of electron scattering collision of slow electrons with these molecules which are currently important in applications as bio- fuels. This relevance, which has attracted much attention, has been one of the subjects of a recent collaboration between experimental and theoretical groups in the USA and Brazil. Recently this collaboration reported first measurements and calculations of differential cross sections for elastic low-energy (rotationally unresolved) electron scattering by several primary alcohols. In this work we address methanol and ethanol TCSs at low energy range and report additional studies of resonant structure in ethanol using the detection of metastable states produced by electron impact excitation with high energy resolution. We have recently constructed a TCS apparatus in our laboratory at Universidade Federal de Juiz de Fora, Brazil, based on the well-known linear transmission technique. The experimental setup is based on the measurement of the attenuation of a collimated electron beam through a gas cell containing the atoms or molecules to be studied at a given pressure. It consists essentially of an electron gun, a gas cell and an electron energy analyzer composed of an array of decelerating electrostatic lenses, a cylindrical dispersive 127o analyzer and a Faraday cup. To our knowledge, there exist

  7. Low energy electron scattering from fuels

    Energy Technology Data Exchange (ETDEWEB)

    Lopes, M. Cristina A.; Silva, Daniel G.M.; Coelho, Rafael F.; Duque, Humberto V.; Santos, Rodrigo R. dos; Ribeiro, Thiago M. [Universidade Federal de Juiz de Fora (UFJF), MG (Brazil). Dept. de Fisica; Yates, Brent; Hong, Ling; Khakoo, Murtadha A. [California State University at Fullerton, CA (US). Physics Department; Bettega, Marcio H.F. [Universidade Federal do Parana (UFPR), Curitiba, PR (Brazil). Dept. de Fisica; Costa, Romarly F. da [Universidade Federal do ABC (UFABC), Santo Andre, SP (Brazil). Centro de Ciencias Naturais e Humanas; Lima, Marco A.P. [Laboratorio Nacional de Ciencia e Tecnologia do Bioetanol (CTBE/CNPEM), Campinas, SP (Brazil)

    2011-07-01

    Full text. Accurate and precise values of absolute total cross section (TCS) represent important information in many scientific and technological applications. In our case, for example, we are motivated to provide such information for electron-fuel collision processes which are specifically relevant to modeling spark ignition in alcohol-fuelled internal combustion engines. Many electron scattering TCS measurements are presently available for a diverse range of atomic and molecular targets. However, lack of data for important bio-molecular targets still remains. Disagreements between the available TCS data for the alcohols have prompted several studies of electron scattering collision of slow electrons with these molecules which are currently important in applications as bio- fuels. This relevance, which has attracted much attention, has been one of the subjects of a recent collaboration between experimental and theoretical groups in the USA and Brazil. Recently this collaboration reported first measurements and calculations of differential cross sections for elastic low-energy (rotationally unresolved) electron scattering by several primary alcohols. In this work we address methanol and ethanol TCSs at low energy range and report additional studies of resonant structure in ethanol using the detection of metastable states produced by electron impact excitation with high energy resolution. We have recently constructed a TCS apparatus in our laboratory at Universidade Federal de Juiz de Fora, Brazil, based on the well-known linear transmission technique. The experimental setup is based on the measurement of the attenuation of a collimated electron beam through a gas cell containing the atoms or molecules to be studied at a given pressure. It consists essentially of an electron gun, a gas cell and an electron energy analyzer composed of an array of decelerating electrostatic lenses, a cylindrical dispersive 127o analyzer and a Faraday cup. To our knowledge, there exist

  8. Electron scattering from sodium at intermediate energies

    International Nuclear Information System (INIS)

    Mitroy, J.; McCarthy, I.E.

    1986-10-01

    A comprehensive comparison is made between theoretical calculations and experimental data for intermediate energy (≥ 10 eV) electron scattering from sodium vapour. The theoretical predictions of coupled-channels calculations (including one, two or four channels) do not agree with experimental values of the differential cross sections for elastic scattering or the resonant 3s to 3p excitation. Increasingly-more-sophisticated calculations, incorporating electron correlations in the target states, and also including core-excited states in the close-coupling expansion, are done at a few selected energies in an attempt to isolate the cause of the discrepancies between theory and experiment. It is found that these more-sophisticated calculations give essentially the same results as the two- and four-channel calculations using Hartree-Fock wavefunctions. Comparison of the sodium high-energy elastic differential cross sections with those of neon suggests that the sodium differential cross section experiments may suffer from systematic errors. There is also disagreement, at the higher energies, between theoretical values for the scattering parameters and those that are derived from laser-excited superelastic scattering and electron photon coincidence experiments. When allowance is made for the finite acceptance angle of the electron spectrometers used in the experiments by convoluting the theory with a function representing the distribution of electrons entering the electron spectrometer it is found that the magnitudes of the differences between theory and experiment are reduced

  9. Allotropic effects on the energy loss of swift H+ and He+ ion beams through thin foils

    International Nuclear Information System (INIS)

    Garcia-Molina, Rafael; Abril, Isabel; Denton, Cristian D.; Heredia-Avalos, Santiago

    2006-01-01

    We have developed a theoretical treatment and a simulation code to study the energy loss of swift H + and He + ion beams interacting with thin foils of different carbon allotropes. The former is based on the dielectric formalism, and the latter combines Monte Carlo with the numerical solution of the motion equation for each projectile to describe its trajectory and interactions through the target. The capabilities of both methods are assessed by the reasonably good agreement between their predictions and the experimental results, for a wide range of projectile energies and target characteristics. Firstly, we apply the theoretical procedure to calculate the stopping cross sections for H + and He + beams in foils of different allotropic forms of carbon (such as diamond, graphite, amorphous carbon, glassy carbon and C 60 -fullerite), as a function of the projectile energy. We take into account the electronic structure of the projectile, as well as the different charge states it can acquire, the energy loss associated to the electronic capture and loss processes, the polarization of the projectile, and a realistic description of the target. On the other hand, the simulation code is used to evaluate the energy distributions of swift H + and He + ion beams when traversing several foils of the above mentioned allotropic forms of carbon, in order to analyze the influence of the chemical and physical state of the target in the projectile energy loss. These allotropic effects are found to become more important around the maximum of the stopping cross-section

  10. Toroidal electron beam energy storage for controlled fusion

    International Nuclear Information System (INIS)

    Clark, W.; Korn, P.; Mondelli, A.; Rostoker, N.

    1976-01-01

    In the presence of an external magnetic field stable equilibria exist for an unneutralized electron beam with ν/γ >1. As a result, it is in principle, possible to store very large quantities of energy in relatively small volumes by confining an unneutralized electron beam in a Tokamak-like device. The energy is stored principally in the electrostatic and self-magnetic fields associated with the beam and is available for rapid heating of pellets for controlled fusion. The large electrostatic potential well in such a device would be sufficient to contain energetic alpha particles, thereby reducing reactor wall bombardment. This approach also avoids plasma loss and wall bombardment by charge exchange neutrals. The conceptual design of an electrostatic Tokamak fusion reactor (ETFR) is discussed. A small toroidal device (the STP machine) has been constructed to test the principles involved. Preliminary experiments on this device have produced electron densities approximately 10% of those required in a reactor

  11. Daily pattern of energy distribution and weight loss.

    Science.gov (United States)

    Raynor, Hollie A; Li, Fan; Cardoso, Chelsi

    2018-08-01

    Timing of energy intake, a temporal dietary pattern, may enhance health. Eating a greater amount of energy earlier and a smaller amount of energy later in the day, a behavioral circadian rhythm, may assist with chronoenhancement. Chronoenhancement seeks to enhance entrainment (synchronization) of biological and behavioral circadian rhythms. In humans, research reports that eating a greater amount of energy early and a smaller amount of energy later in the day increases dietary induced thermogenesis, improves cardiometabolic outcomes, and enhances weight loss. However, little human research has examined if this eating pattern enhances regularity of biological circadian rhythm. In a randomized controlled 8-week pilot study, the influence of energy distribution timing on weight loss and regularity of sleep onset and wake times (marker for biological circadian rhythm) was examined. Within an hypocaloric, three-meal prescription, participants (n = 8) were assigned to either: 1) Morning: 50%, 30%, and 20% of kcal at breakfast, lunch, and dinner, respectively; or 2) Evening: 20%, 30%, and 50% of kcal at breakfast, lunch, and dinner, respectively. Percent weight loss and regularity of sleep onset and wake times were significantly (p energy distribution timing on health, longer studies conducted in free-living participants, with dietary intake assessed using time-stamped methods, that include measures of the circadian timing system are needed. This small review is based upon a symposium presentation at the Society of the Study of Ingestive Behavior in 2017. Copyright © 2018 Elsevier Inc. All rights reserved.

  12. Electronic market places in the energy

    International Nuclear Information System (INIS)

    Mons, L.

    2001-12-01

    Electronic market places in the energy domain occurred at the end of the 90's in the US and have started to develop in Europe in the year 2000. About 60 platforms are registered today and this development can be explained by the advantages raised by such an infrastructure: simplification of purchase procedures, reduction of delays in the purchase decision, reduction of administrative costs etc.. However, today none of these electronic market places is profitable and several have closed down. On the other hand, this tool will certainly become necessary in the future and all energy actors are developing projects in this way. This study analyzes the electronic market places phenomenon in the energy domain using 10 market places examples with their key-factors of success. It draws out a complete status of the initiatives developed today and presents some scenarios of evolution. (J.S.)

  13. Molecular dynamics simulations of the role of electronic losses in damage creation of ion irradiated Tungsten

    International Nuclear Information System (INIS)

    Maya, P.N.; Deshpande, S.P

    2014-01-01

    Damage creation due to the irradiation of 14 MeV fusion neutrons and the subsequent mechanical failure and alteration of the fuel retention properties of tungsten plasma-facing materials is one of the major concerns of the fusion reactors. In addition to nuclear reactions and the subsequent transmutations, the energetic neutron impars its kinetic energy either partly or completely to a lattice tungsten atom thereby creating a primary knock-on atom (PKA) which, is considered as the onset of damage creation in the lattice. The PKA continues to undergo collisions with the lattice atoms which eventually leads to a collision cascade. In order to understand the collision process, one often simulates such systems using surrogate ions, such as energetic W ions itself, in particle accelerators and due to the experimental constraints (such as the stability of the beam) one often has to opt for high energetic ion beams (∼ 30 MeV) which surpasses the PKA energies created by neutron (∼100s of KeV) in W. Hence it is important to distinguish how the very high energetic tungsten atoms interact with the lattice atoms in comparison with the low energy PKA created by the neutron. One of the key difference is that at higher energies the electronic losses become important which decides the collision dynamics. In this presentation the effect of electronic losses in the damage creation using molecular dynamics simulations have been discussed

  14. Beam energy loss to parasitic modes in SPEAR II

    International Nuclear Information System (INIS)

    Allen, M.A.; Paterson, J.M.; Rees, J.R.; Wilson, P.B.

    1975-01-01

    The energy loss due to the excitation of parasitic modes in the SPEAR II rf cavities and vacuum chamber components was measured by observing the shift in synchronous phase angle as a function of circulating beam current and accelerating cavity voltage. The resulting parasitic mode loss resistance is 5 M OMEGA at a bunch length of 6.5 cm. The loss resistance varies with bunch length sigma/sub z/ approximately as exp(-0.3 sigma/sub z/). If the measured result is compared with reasonable theoretical predictions, it may be inferred that the major portion of the parasitic loss takes place in ring vacuum components rather than in the rf cavities. (auth)

  15. Energy Drinks, Weight Loss, and Disordered Eating Behaviors

    Science.gov (United States)

    Jeffers, Amy J.; Vatalaro Hill, Katherine E.; Benotsch, Eric G.

    2014-01-01

    Objective: The present study examined energy drink consumption and relations with weight loss attempts and behaviors, body image, and eating disorders. Participants/Methods: This is a secondary analysis using data from 856 undergraduate students who completed the American College Health Association-National College Health Assessment II…

  16. Acceleration and energy loss in N = 4 SYM

    International Nuclear Information System (INIS)

    Chernicoff, Mariano; Gueijosa, Alberto

    2009-01-01

    This contribution is based on two talks given at the XIII Mexican School of Particles and Fields. We revisit some of the results presented in [19], concerning the rate of energy loss of an accelerating quark in strongly-coupled N = 4 super-Yang-Mills.

  17. Acceleration and energy loss in N = 4 SYM

    Science.gov (United States)

    Chernicoff, Mariano; Güijosa, Alberto

    2009-04-01

    This contribution is based on two talks given at the XIII Mexican School of Particles and Fields. We revisit some of the results presented in [19], concerning the rate of energy loss of an accelerating quark in strongly-coupled N = 4 super-Yang-Mills.

  18. Rotating gravity currents. Part 1. Energy loss theory

    Science.gov (United States)

    Martin, J. R.; Lane-Serff, G. F.

    2005-01-01

    A comprehensive energy loss theory for gravity currents in rotating rectangular channels is presented. The model is an extension of the non-rotating energy loss theory of Benjamin (J. Fluid Mech. vol. 31, 1968, p. 209) and the steady-state dissipationless theory of rotating gravity currents of Hacker (PhD thesis, 1996). The theory assumes the fluid is inviscid, there is no shear within the current, and the Boussinesq approximation is made. Dissipation is introduced using a simple method. A head loss term is introduced into the Bernoulli equation and it is assumed that the energy loss is uniform across the stream. Conservation of momentum, volume flux and potential vorticity between upstream and downstream locations is then considered. By allowing for energy dissipation, results are obtained for channels of arbitrary depth and width (relative to the current). The results match those from earlier workers in the two limits of (i) zero rotation (but including dissipation) and (ii) zero dissipation (but including rotation). Three types of flow are identified as the effect of rotation increases, characterized in terms of the location of the outcropping interface between the gravity current and the ambient fluid on the channel boundaries. The parameters for transitions between these cases are quantified, as is the detailed behaviour of the flow in all cases. In particular, the speed of the current can be predicted for any given channel depth and width. As the channel depth increases, the predicted Froude number tends to surd 2, as for non-rotating flows.

  19. Experimental investigation of energy loss and end loss physics in a linear theta pinch. Scientific report 81-3

    International Nuclear Information System (INIS)

    Jacoby, B.A.

    1981-01-01

    The results of an experimental study of particle and thermal loss processes from a 50-cm long theta pinch are presented. The plasma was generated with a 40-mTorr fill of deuterium in a 3.81 cm radius discharge tube; 67% Z-preionization was followed by a main current discharge that produced a 23-kG peak magnetic field in 4.75 μsec. The electron density and temperature in the plasma column at the end of dynamic implosion were characterized by 1.0 x 10 16 cm -3 and 20 eV, respectively. This was followed by adiabatic compression which occurred with the particle and energy loss of interest. The diagnostics employed in this experiment were Thomson scattering, continuum radiation spectroscopy, local magnetic-field probes, local pressure probes, and diamagnetic loops. Axial temperature and density profiles were mapped from the coil into the end region

  20. Nonlinear energy loss of highly charged heavy ions

    International Nuclear Information System (INIS)

    Zwicknagel, G.Guenter.

    2000-01-01

    For slow, highly charged heavy ions strong coupling effects in the energy transfer from the projectile-ion to an electron target plasma become important. A theoretical description of this nonlinear ion stopping has to go beyond the standard approaches like the dielectric linear response or the binary collision model which are strictly valid only at weak ion-target coupling. Here we outline an improved treatment which is based on a suitable combination of binary collision and linear response contributions. As has been verified for isotropic, nonmagnetized electron plasmas by comparison with simulations, this approach well reproduces the essential features of nonlinear stopping up to moderate coupling strength. Its extension to anisotropic, magnetized electron plasmas basically involves the fully numerical determination of the momentum and energy transfer in binary ion-electron collisions in the presence of a magnetic field. First results of such calculations are presented and discussed

  1. Anisotropic pitch angle distribution of ~100 keV microburst electrons in the loss cone: measurements from STSAT-1

    Directory of Open Access Journals (Sweden)

    J. J. Lee

    2012-11-01

    Full Text Available Electron microburst energy spectra in the range of 170 keV to 360 keV have been measured using two solid-state detectors onboard the low-altitude (680 km, polar-orbiting Korean STSAT-1 (Science and Technology SATellite-1. Applying a unique capability of the spacecraft attitude control system, microburst energy spectra have been accurately resolved into two components: perpendicular to and parallel to the geomagnetic field direction. The former measures trapped electrons and the latter those electrons with pitch angles in the loss cone and precipitating into atmosphere. It is found that the perpendicular component energy spectra are harder than the parallel component and the loss cone is not completely filled by the electrons in the energy range of 170 keV to 360 keV. These results have been modeled assuming a wave-particle cyclotron resonance mechanism, where higher energy electrons travelling within a magnetic flux tube interact with whistler mode waves at higher latitudes (lower altitudes. Our results suggest that because higher energy (relativistic microbursts do not fill the loss cone completely, only a small portion of electrons is able to reach low altitude (~100 km atmosphere. Thus assuming that low energy microbursts and relativistic microbursts are created by cyclotron resonance with chorus elements (but at different locations, the low energy portion of the microburst spectrum will dominate at low altitudes. This explains why relativistic microbursts have not been observed by balloon experiments, which typically float at altitudes of ~30 km and measure only X-ray flux produced by collisions between neutral atmospheric particles and precipitating electrons.

  2. High energy electron irradiation of flowable materials

    International Nuclear Information System (INIS)

    Offermann, B.P.

    1975-01-01

    In order to efficiently irradiate a flowable material with high energy electrons, a hollow body is disposed in a container for the material and the material is caused to flow in the form of a thin layer across a surface of the body from or to the interior of the container while the material flowing across the body surface is irradiated. (U.S.)

  3. Applications for Energy Recovering Free Electron Lasers

    Energy Technology Data Exchange (ETDEWEB)

    George Neil

    2007-08-01

    The availability of high-power, high-brilliance sources of tunable photons from energy-recovered Free Electron Lasers is opening up whole new fields of application of accelerators in industry. This talk will review some of the ideas that are already being put into production, and some of the newer ideas that are still under development.

  4. Multiple loss processes of relativistic electrons outside the heart of outer radiation belt during a storm sudden commencement

    International Nuclear Information System (INIS)

    Yu, J.

    2015-01-01

    By examining the compression-induced changes in the electron phase space density and pitch angle distribution observed by two satellites of Van Allen Probes (RBSP-A/B), we find that the relativistic electrons (>2 MeV) outside the heart of outer radiation belt (L*≥5) undergo multiple losses during a storm sudden commencement. The relativistic electron loss mainly occurs in the field-aligned direction (pitch angle α < 30° or >150°), and the flux decay of the field-aligned electrons is independent of the spatial location variations of the two satellites. However, the relativistic electrons in the pitch angle range of 30°–150° increase (decrease) with the decreasing (increasing) geocentric distance (|ΔL|<0.25) of the RBSP-B (RBSP-A) location, and the electron fluxes in the quasi-perpendicular direction display energy-dispersive oscillations in the Pc5 period range (2–10 min). The relativistic electron loss is confirmed by the decrease of electron phase space density at high-L shell after the magnetospheric compressions, and their loss is associated with the intense plasmaspheric hiss, electromagnetic ion cyclotron (EMIC) waves, relativistic electron precipitation (observed by POES/NOAA satellites at 850 km), and magnetic field fluctuations in the Pc5 band. Finally, the intense EMIC waves and whistler mode hiss jointly cause the rapidly pitch angle scattering loss of the relativistic electrons within 10 h. Moreover, the Pc5 ULF waves also lead to the slowly outward radial diffusion of the relativistic electrons in the high-L region with a negative electron phase space density gradient.

  5. Energy loss to parasitic modes of accelerating cavities

    International Nuclear Information System (INIS)

    Sands, M.

    1974-01-01

    At the maximum stored current, each circulating beam in PEP will consist of three bunches, each about 10 cm long containing 1.5 /times/ 10 12 particles. The large electric charge carried by such a bunch (2.5 /times/ 10/sup /minus/7/ coulomb) will, because of its short length, give rise to a large transient excitation of hundreds of parasitic modes in the accelerating cavities. The energy loss of the stored beam to the cavities from this process may be comparable to the loss to synchrotron radiation, and may, therefore, require a significant increase in power from the accelerating rf system. In this note I considered three aspects of this effect. First, an attempt is made to estimate the magnitude of the energy loss of a bunch in a single passage through the accelerating cavities. Then, I consider the effects of the periodic passages of the bunches in a single stored beam. And finally, I look at the consequences of storing two counter-rotating beams. The general conclusions are that the magnitude energy loss to the parasitic modes is serious, though probably not disastrous; and that, in general, the separate stored bunches will act incoherently. 2 refs., 7 figs

  6. Energy exchange in strongly coupled plasmas with electron drift

    International Nuclear Information System (INIS)

    Akbari-Moghanjoughi, M.; Ghorbanalilu, M.

    2015-01-01

    In this paper, the generalized viscoelastic collisional quantum hydrodynamic model is employed in order to investigate the linear dielectric response of a quantum plasma in the presence of strong electron-beam plasma interactions. The generalized Chandrasekhar's relativistic degeneracy pressure together with the electron-exchange and Coulomb interaction effects are taken into account in order to extend current research to a wide range of plasma number density relevant to big planetary cores and astrophysical compact objects. The previously calculated shear viscosity and the electron-ion collision frequencies are used for strongly coupled ion fluid. The effect of the electron-beam velocity on complex linear dielectric function is found to be profound. This effect is clearly interpreted in terms of the wave-particle interactions and their energy-exchange according to the sign of the imaginary dielectric function, which is closely related to the wave attenuation coefficient in plasmas. Such kinetic effect is also shown to be in close connection with the stopping power of a charged-particle beam in a quantum plasma. The effect of many independent plasma parameters, such as the ion charge-state, electron beam-velocity, and relativistic degeneracy, is shown to be significant on the growing/damping of plasma instability or energy loss/gain of the electron-beam

  7. Photoelectron Energy Loss in Al(002) Revisited: Retrieval of the Single Plasmon Loss Energy Distribution by a Fourier Transform Method

    Science.gov (United States)

    Santana, Victor Mancir da Silva; David, Denis; de Almeida, Jailton Souza; Godet, Christian

    2018-06-01

    A Fourier transform (FT) algorithm is proposed to retrieve the energy loss function (ELF) of solid surfaces from experimental X-ray photoelectron spectra. The intensity measured over a broad energy range towards lower kinetic energies results from convolution of four spectral distributions: photoemission line shape, multiple plasmon loss probability, X-ray source line structure and Gaussian broadening of the photoelectron analyzer. The FT of the measured XPS spectrum, including the zero-loss peak and all inelastic scattering mechanisms, being a mathematical function of the respective FT of X-ray source, photoemission line shape, multiple plasmon loss function, and Gaussian broadening of the photoelectron analyzer, the proposed algorithm gives straightforward access to the bulk ELF and effective dielectric function of the solid, assuming identical ELF for intrinsic and extrinsic plasmon excitations. This method is applied to aluminum single crystal Al(002) where the photoemission line shape has been computed accurately beyond the Doniach-Sunjic approximation using the Mahan-Wertheim-Citrin approach which takes into account the density of states near the Fermi level; the only adjustable parameters are the singularity index and the broadening energy D (inverse hole lifetime). After correction for surface plasmon excitations, the q-averaged bulk loss function, q , of Al(002) differs from the optical value Im[- 1 / ɛ( E, q = 0)] and is well described by the Lindhard-Mermin dispersion relation. A quality criterion of the inversion algorithm is given by the capability of observing weak interband transitions close to the zero-loss peak, namely at 0.65 and 1.65 eV in ɛ( E, q) as found in optical spectra and ab initio calculations of aluminum.

  8. Photoelectron Energy Loss in Al(002) Revisited: Retrieval of the Single Plasmon Loss Energy Distribution by a Fourier Transform Method

    Science.gov (United States)

    Santana, Victor Mancir da Silva; David, Denis; de Almeida, Jailton Souza; Godet, Christian

    2018-04-01

    A Fourier transform (FT) algorithm is proposed to retrieve the energy loss function (ELF) of solid surfaces from experimental X-ray photoelectron spectra. The intensity measured over a broad energy range towards lower kinetic energies results from convolution of four spectral distributions: photoemission line shape, multiple plasmon loss probability, X-ray source line structure and Gaussian broadening of the photoelectron analyzer. The FT of the measured XPS spectrum, including the zero-loss peak and all inelastic scattering mechanisms, being a mathematical function of the respective FT of X-ray source, photoemission line shape, multiple plasmon loss function, and Gaussian broadening of the photoelectron analyzer, the proposed algorithm gives straightforward access to the bulk ELF and effective dielectric function of the solid, assuming identical ELF for intrinsic and extrinsic plasmon excitations. This method is applied to aluminum single crystal Al(002) where the photoemission line shape has been computed accurately beyond the Doniach-Sunjic approximation using the Mahan-Wertheim-Citrin approach which takes into account the density of states near the Fermi level; the only adjustable parameters are the singularity index and the broadening energy D (inverse hole lifetime). After correction for surface plasmon excitations, the q-averaged bulk loss function, q , of Al(002) differs from the optical value Im[- 1 / ɛ(E, q = 0)] and is well described by the Lindhard-Mermin dispersion relation. A quality criterion of the inversion algorithm is given by the capability of observing weak interband transitions close to the zero-loss peak, namely at 0.65 and 1.65 eV in ɛ(E, q) as found in optical spectra and ab initio calculations of aluminum.

  9. Energy loss distributions of 7 TeV protons channeled in a bent silicon crystals

    Directory of Open Access Journals (Sweden)

    Stojanov Nace

    2013-01-01

    Full Text Available The energy loss distributions of relativistic protons axially channeled through the bent Si crystals, with the constant curvature radius, R = 50 m, are studied here. The proton energy is 7 TeV and the thickness of the crystal is varied from 1 mm to 5 mm, which corresponds to the reduced crystal thickness, L, from 2.1 to 10.6, respectively. The proton energy was chosen in accordance with the large hadron collider project, at the European Organization for Nuclear Research, in Geneva, Switzerland. The energy loss distributions of the channeled protons were generated by the computer simulation method using the numerical solution of the proton equations of motion in the transverse plane. Dispersion of the proton scattering angle caused by its collisions with the crystal’s electrons was taken into account. [Projekat Ministarstva nauke Republike Srbije, br. III 45006

  10. Study of the electron energy distribution function in plasma produced by a rf discharge in a mixture of inert gases

    International Nuclear Information System (INIS)

    Vagner, S.D.; Ignat'ev, B.K.

    1983-01-01

    Electron energy distribution functions (EEDF) are recorded in an rf discharge in a mixture of neon and argon. The rates of different ionization processes and the energy losses of the electrons in the bulk of the discharge are calculated. The experimentally recorded electron energy distribution functions are compared with distributions calculated using a nonlocal theory. The effect of an rf voltage in the probe circuit on the recorded electron energy distribution functions is investigated experimentally

  11. Influence of damping on proton energy loss in plasmas of all degeneracies

    International Nuclear Information System (INIS)

    Barriga-Carrasco, Manuel D.

    2007-01-01

    The purpose of the present paper is to describe the effects of electron-electron collisions on the stopping power of plasmas of any degeneracy. Plasma targets are considered fully ionized so electronic stopping is only due to the free electrons. We focus our analysis on plasmas which electronic density is around solid values n e ≅10 23 cm -3 and which temperature is around T≅10 eV; these plasmas are in the limit of weakly coupled plasmas. This type of plasma has not been studied extensively though it is very important for inertial confinement fusion. The electronic stopping is obtained from an exact quantum mechanical evaluation, which takes into account the degeneracy of the target plasma, and later it is compared with common classical and degenerate approximations. Differences are around 30% in some cases which can produce bigger mistakes in further energy deposition and projectile range studies. Then we consider electron-electron collisions in the exact quantum mechanical electronic stopping calculation. Now the maximum stopping occurs at velocities smaller than for the calculations without considering collisions for all kinds of plasmas analyzed. The energy loss enhances for velocities smaller than the velocity at maximum while decreases for higher velocities. Latter effects are magnified with increasing collision frequency. Differences with the same results for the case of not taking into account collisions are around 20% in the analyzed cases

  12. Electron-ion recombination at low energy

    International Nuclear Information System (INIS)

    Andersen, L.H.

    1993-01-01

    The work is based on results obtained with a merged-beams experiment. A beam of electronics with a well characterized density and energy distribution was merged with a fast, monoenergetic ion beam. Results have been obtained for radiative recombination and dielectronic recombination at low relative energies (0 to ∼70eV). The obtained energy resolution was improved by about a factor of 30. High vacuum technology was used to suppress interactions with electrons from the environments. The velocity distribution of the electron beam was determined. State-selective dielectronic-recombination measurements were performable. Recombination processes were studied. The theoretical background for radiative recombination and Kramers' theory are reviewed. The quantum mechanical result and its relation to the semiclassical theory is discussed. Radiative recombination was also measured with several different non-bare ions, and the applicability of the semiclassical theory to non-bare ions was investigated. The use of an effective charge is discussed. For dielectronic recombination, the standard theoretical approach in the isolated resonance and independent-processes approximation is debated. The applicability of this method was tested. The theory was able to reproduce most of the experimental data except when the recombination process was sensitive to couplings between different electronic configurations. The influence of external perturbing electrostatic fields is discussed. (AB) (31 refs.)

  13. Can low energy electrons affect high energy physics accelerators?

    CERN Document Server

    Cimino, R; Furman, M A; Pivi, M; Ruggiero, F; Rumolo, Giovanni; Zimmermann, Frank

    2004-01-01

    The properties of the electrons participating in the build up of an electron cloud (EC) inside the beam-pipe have become an increasingly important issue for present and future accelerators whose performance may be limited by this effect. The EC formation and evolution are determined by the wall-surface properties of the accelerator vacuum chamber. Thus, the accurate modeling of these surface properties is an indispensible input to simulation codes aimed at the correct prediction of build-up thresholds, electron-induced instability or EC heat load. In this letter, we present the results of surface measurements performed on a prototype of the beam screen adopted for the Large Hadron Collider (LHC), which presently is under construction at CERN. We have measured the total secondary electron yield (SEY) as well as the related energy distribution curves (EDC) of the secondary electrons as a function of incident electron energy. Attention has been paid, for the first time in this context, to the probability at whic...

  14. Energy loss of carbon transmitted 1-MeV H2+ ions

    International Nuclear Information System (INIS)

    Fritz, M.; Kimura, K.; Susuki, Y.; Mannami, M.

    1994-01-01

    Energy losses of 1-MeV H 2 + ions passing through carbon foils of 2-8 μg/cm 2 thickness have been measured and show besides the linear increase with target thickness a 0.4 keV offset. The stopping power derived from the observed energy losses is 1.15 times as large as the sum of the stopping powers for two single H + of the same velocity. Calculations of the stopping powers for H 2 + ions and diprotons, using first Born approximation, indicate that the H 2 + ions lose the binding electron upon entrance into the foil, traverse the target as diprotons and recapture target electrons at the exit surface, a scenario also supported by the 0.4 keV offset at zero thickness. (author)

  15. An energy monitor for electron accelerators

    Energy Technology Data Exchange (ETDEWEB)

    Geske, G. (Friedrich-Schiller-Universitaet, Jena (German Democratic Republic). Klinik und Poliklinik des Bereiches Medizin)

    1990-09-01

    A monitor useful for checks of the energy selector scale of medical electron accelerators was developed and tested. It consists of a linear array of flat ionization chambers sandwiched between absorber plates of low-Z material. The first chamber at the electron beam entrance may be used to produce a reference signal S{sub r}, if not another suitable reference signal is taken. The following chambers are electrically connected and deliver the measuring signal S{sub m}. A clinical dosimeter can be used for recording current or charge. The energy-dependent electron range parameters R{sub p}, R{sub 50} and R{sub 80} in water vary as linear functions of the ratio reference singal/measuring signal. The best linear fit was obtained for the half value layer R{sub 50}. Three types of the energy monitor are described, and experimental results obtained with a linear accelerator and a betatron between 5 and 25 MeV are reported. Uncertainties for checks of R{sub 50} with a calibrated energy monitor were not larger than 1 to 2 mm. Theoretical considerations by a computer model support these results. (orig./HP).

  16. An energy monitor for electron accelerators

    International Nuclear Information System (INIS)

    Geske, G.

    1990-01-01

    A monitor useful for checks of the energy selector scale of medical electron accelerators was developed and tested. It consists of a linear array of flat ionization chambers sandwiched between absorber plates of low-Z material. The first chamber at the electron beam entrance may be used to produce a reference signal S r , if not another suitable reference signal is taken. The following chambers are electrically connected and deliver the measuring signal S m . A clinical dosimeter can be used for recording current or charge. The energy-dependent electron range parameters R p , R 50 and R 80 in water vary as linear functions of the ratio reference singal/measuring signal. The best linear fit was obtained for the half value layer R 50 . Three types of the energy monitor are described, and experimental results obtained with a linear accelerator and a betatron between 5 and 25 MeV are reported. Uncertainties for checks of R 50 with a calibrated energy monitor were not larger than 1 to 2 mm. Theoretical considerations by a computer model support these results. (orig./HP) [de

  17. Neutrino energy loss rate in a stellar plasma

    International Nuclear Information System (INIS)

    Esposito, S.; Mangano, G.; Miele, G.; Picardi, I.; Pisanti, O.

    2003-01-01

    We review the purely leptonic neutrino emission processes, contributing to the energy loss rate of the stellar plasma. We perform a complete analysis up to the first order in the electromagnetic coupling constant. In particular the radiative electromagnetic corrections, at order α, to the process e + e - →νν-bar at finite density and temperature have been computed. This process gives one of the main contributions to the cooling of stellar interior in the late stages of star evolution. As a result of the analysis we find that the corrections affect the energy loss rate, computed at tree level, by a factor (-4-1)% in the temperature and density region where the pair annihilation is the most efficient cooling mechanism

  18. High Energy Electron Detectors on Sphinx

    Science.gov (United States)

    Thompson, J. R.; Porte, A.; Zucchini, F.; Calamy, H.; Auriel, G.; Coleman, P. L.; Bayol, F.; Lalle, B.; Krishnan, M.; Wilson, K.

    2008-11-01

    Z-pinch plasma radiation sources are used to dose test objects with K-shell (˜1-4keV) x-rays. The implosion physics can produce high energy electrons (> 50keV), which could distort interpretation of the soft x-ray effects. We describe the design and implementation of a diagnostic suite to characterize the electron environment of Al wire and Ar gas puff z-pinches on Sphinx. The design used ITS calculations to model detector response to both soft x-rays and electrons and help set upper bounds to the spurious electron flux. Strategies to discriminate between the known soft x-ray emission and the suspected electron flux will be discussed. H.Calamy et al, ``Use of microsecond current prepulse for dramatic improvements of wire array Z-pinch implosion,'' Phys Plasmas 15, 012701 (2008) J.A.Halbleib et al, ``ITS: the integrated TIGER series of electron/photon transport codes-Version 3.0,'' IEEE Trans on Nuclear Sci, 39, 1025 (1992)

  19. Energy loss of 107Ag, 109Ag and 150Sm in Ni and Au

    International Nuclear Information System (INIS)

    Ribas, R.V.; Seale, W.A.; Roney, W.M.; Szanto, E.M.

    1979-01-01

    The stopping power of 107 Ag, 109 Ag and 150 Sm in nickel and gold was measured as a preliminary test of a new technique for measuring energy loss based on the γ-ray Dopppler shift. The analysis of the data was based on the theories of Lindhard, Scharff and Schiott for nuclear and electronic stopping. The results are compared with the semi-empirical predictions of Northcliffe and Schilling. (author) [pt

  20. Local energy equation for two-electron atoms and relation between kinetic energy and electron densities

    International Nuclear Information System (INIS)

    March, N.H.

    2002-08-01

    In early work, Dawson and March [J. Chem. Phys. 81, 5850 (1984)] proposed a local energy method for treating both Hartree-Fock and correlated electron theory. Here, an exactly solvable model two-electron atom with pure harmonic interactions is treated in its ground state in the above context. A functional relation between the kinetic energy density t(r) at the origin r=0 and the electron density p(r) at the same point then emerges. The same approach is applied to the Hookean atom; in which the two electrons repel with Coulombic energy e 2 /r 12 , with r 12 the interelectronic separation, but are still harmonically confined. Again the kinetic energy density t(r) is the focal point, but now generalization away from r=0 is also effected. Finally, brief comments are added about He-like atomic ions in the limit of large atomic number. (author)

  1. Impact-parameter dependence of energy loss for 625-keV H+ ions in Si single crystals

    International Nuclear Information System (INIS)

    Dygo, A.; Boshart, M.A.; Seiberling, L.E.; Kabachnik, N.M.

    1994-01-01

    The energy distributions for 625-keV H + ions transmitted through thin Si single crystals are studied for detailed angular scans through the left-angle 110 right-angle and left-angle 100 right-angle axial as well as the {111} and {110} planar channels. Well-resolved structures in the distributions taken near the left-angle 110 right-angle axial direction are observed. The experimental energy-loss distributions are very well reproduced by a Monte Carlo simulation using the semiclassical approximation model for core electrons and the two-component free-electron-gas model for valence electrons. The best fit to the data is obtained if the model energy losses are scaled up for core electrons and down for valence electrons by several percent. The experimental distributions can also be reproduced by assuming the mean excitation energy for distant collisions of the ion with core electrons equal to 1.4 times the binding energy for a given shell. No significant differences between the distributions obtained using the solid-state and free-atom valence electron densities have been found. The evolution of the distributions for the left-angle 110 right-angle axial scan is discussed in terms of ion trajectories and the flux distribution. Also, the azimuthally averaged mean energy loss is studied as a function of tilt angle with respect to the left-angle 110 right-angle axis

  2. Magnetic field structure influence on primary electron cusp losses for micro-scale discharges

    International Nuclear Information System (INIS)

    Dankongkakul, Ben; Araki, Samuel J.; Wirz, Richard E.

    2014-01-01

    An experimental effort was used to examine the primary electron loss behavior for micro-scale (≲3 cm diameter) discharges. The experiment uses an electron flood gun source and an axially aligned arrangement of ring-cusps to guide the electrons to a downstream point cusp. Measurements of the electron current collected at the point cusp show an unexpectedly complex loss pattern with azimuthally periodic structures. Additionally, in contrast to conventional theory for cusp losses, the overall radii of the measured collection areas are over an order of magnitude larger than the electron gyroradius. Comparing these results to Monte Carlo particle tracking simulations and a simplified analytical analysis shows that azimuthal asymmetries of the magnetic field far upstream of the collection surface can substantially affect the electron loss structure and overall loss area

  3. Probing hot dense matter with jet energy loss

    International Nuclear Information System (INIS)

    Levai, P.; Barnafoeldi, G.G.; Gyulassy, M.; Vitev, I.; Fai, G.; Zhang, Y.

    2002-01-01

    We study, in a pQCD calculation augmented by nuclear effects, the jet energy loss needed to reproduce the π 0 spectra in Au+Au collisions at large p T , measured by PHENIX at RHIC. The transverse width of the parton momentum distributions (intrinsic k T ) is used phenomenologically to obtain a reliable baseline pp result. Jet quenching is applied to the nuclear spectra (including shadowing and multiscattering) to fit the data. Latest results on fluctuating gluon radiation are considered to measure the opacity of the produced hot dense matter at RHIC energy. (orig.)

  4. Electron-induced hydrogen loss in uracil in a water cluster environment

    International Nuclear Information System (INIS)

    Smyth, M.; Kohanoff, J.; Fabrikant, I. I.

    2014-01-01

    Low-energy electron-impact hydrogen loss due to dissociative electron attachment (DEA) to the uracil and thymine molecules in a water cluster environment is investigated theoretically. Only the A ′ -resonance contribution, describing the near-threshold behavior of DEA, is incorporated. Calculations are based on the nonlocal complex potential theory and the multiple scattering theory, and are performed for a model target with basic properties of uracil and thymine, surrounded by five water molecules. The DEA cross section is strongly enhanced when the attaching molecule is embedded in a water cluster. This growth is due to two effects: the increase of the resonance lifetime and the negative shift in the resonance position due to interaction of the intermediate negative ion with the surrounding water molecules. A similar effect was earlier found in DEA to chlorofluorocarbons

  5. Electron-induced hydrogen loss in uracil in a water cluster environment

    Energy Technology Data Exchange (ETDEWEB)

    Smyth, M.; Kohanoff, J. [Atomistic Simulation Centre, Queen' s University Belfast, Belfast BT7 1NN, Northern Ireland (United Kingdom); Fabrikant, I. I., E-mail: ifabrikant1@unl.edu [Department of Physics and Astronomy, University of Nebraska, Lincoln, Nebraska 68588, USA and Department of Physical Sciences, The Open University, Walton Hall, Milton Keynes MK7 6AA (United Kingdom)

    2014-05-14

    Low-energy electron-impact hydrogen loss due to dissociative electron attachment (DEA) to the uracil and thymine molecules in a water cluster environment is investigated theoretically. Only the A{sup ′}-resonance contribution, describing the near-threshold behavior of DEA, is incorporated. Calculations are based on the nonlocal complex potential theory and the multiple scattering theory, and are performed for a model target with basic properties of uracil and thymine, surrounded by five water molecules. The DEA cross section is strongly enhanced when the attaching molecule is embedded in a water cluster. This growth is due to two effects: the increase of the resonance lifetime and the negative shift in the resonance position due to interaction of the intermediate negative ion with the surrounding water molecules. A similar effect was earlier found in DEA to chlorofluorocarbons.

  6. A precise measurement of 180 GeV muon energy losses in iron

    CERN Document Server

    Amaral, P; Anderson, K; Artikov, A; Benetta, R; Berglund, S R; Biscarat, C; Blanch, O; Blanchot, G; Bogush, A A; Bohm, C; Boldea, V; Borisov, O N; Bosman, M; Bromberg, C; Bravo, S; Budagov, Yu A; Burdin, S V; Calôba, L P; Camarena, F; Carvalho, J; Castillo, M V; Cavalli-Sforza, M; Cavasinni, V; Cerqueira, A S; Chadelas, R; Chirikov-Zorin, I E; Chlachidze, G; Cobal, M; Cogswell, F; Cologna, S; Constantinescu, S; Costanzo, D; Cowan, Brian; Crouau, M; Daudon, F; David, M; Davidek, T; Dawson, J; De, K; Delfino, M C; Del Prete, T; De Santo, A; Di Girolamo, B; Dita, S; Downing, R; Engström, M; Errede, D; Errede, S; Fassi, F; Fenyuk, A; Ferrer, A; Flaminio, Vincenzo; Flix, J; Garabik, R; Gil, I; Gildemeister, O; Glagoley, V; Gómez, A; González de la Hoz, S; Grabskii, V; Grenier, P; Hakopian, H H; Haney, M; Hellman, S; Henriques, A; Hébrard, C; Higón, E; Holik, P; Holmgren, S O; Hruska, I; Huston, J; Jon-And, K; Kakurin, S; Karyukhin, A N; Khubua, J I; Kopikov, S V; Krivkova, P; Kukhtin, V V; Kulchitskii, Yu A; Kuzmin, M V; Lami, S; Lapin, V; Lazzeroni, C; Lebedev, A; Leitner, R; Li, J; Lomakin, Yu F; Lomakina, O V; Lokajícek, M; López-Amengual, J M; Maio, A; Malyukov, S N; Marroquin, F; Mataix, L; Mazzoni, E; Merritt, F S; Miller, R; Minashvili, I A; Miralles, L; Montarou, G; Némécek, S; Nessi, Marzio; Onofre, A; Ostankov, A P; Pacheco, A; Pallin, D; Pantea, D; Paoletti, R; Park, I C; Pilcher, J E; Pinhão, J; Price, L; Proudfoot, J; Pukhov, O; Reinmuth, G; Renzoni, G; Richards, R; Roda, C; Roldán, J; Romance, J B; Romanov, V; Rosnet, P; Ruiz, H; Rusakovitch, N A; Sanchis, E; Sanders, H; Santoni, C; Santo, J; Says, L P; Seixas, J M; Selldén, B; Semenov, A A; Shcelchkov, A; Shochet, M J; Silva, J; Simaitis, V J; Sissakian, A N; Solodkov, A A; Solovyanov, O; Sosebee, M; Soustruznik, K; Spanó, F; Stanek, R; Starchenko, E A; Stavina, O P; Suk, M; Sykora, I; Tang, F; Tas, P; Thaler, J J; Thome-Filho, Z D; Tokar, S; Topilin, N D; Valklar, S; Varanda, M J; Vartapetian, A H; Vazeille, F; Vichou, I; Vinogradov, V; Vorozhtsov, S B; White, A; Wolters, H; Yamdagni, N; Yarygin, G; Yosef, C; Zaitsev, A

    2001-01-01

    The energy loss spectrum of 180 GeV muons has been measured with the 5.6 m long finely segmented Module 0 of the ATLAS hadron tile calorimeter at the CERN SPS. The differential probability dP/d nu per radiation length of a fractional energy loss nu = Delta E/sub mu //E /sub mu / has been measured in the range 0.025energy losses due to bremsstrahlung, production of electron-positron pairs, and energetic knock-on electrons. The iron elastic form factor correction Delta /sub Fe//sup el/=1.63+or-0.17/sub stat/+or-023/sub syst$/ -/sub 0.14 //sup +0.20//sub theor/ to muon bremsstrahlung in the region of no screening of the nucleus by atomic electrons has been measured for the first time, and is compared with different theoretical predictions. (31 refs).

  7. Energy Transformation in Molecular Electronic Systems

    Energy Technology Data Exchange (ETDEWEB)

    Kasha, Michael

    1999-05-17

    This laboratory has developed many new ideas and methods in the electronic spectroscopy of molecules. This report covers the contract period 1993-1995. A number of the projects were completed in 1996, and those papers are included in the report. The DOE contract was terminated at the end of 1995 owing to a reorganizational change eliminating nationally the projects under the Office of Health and Environmental Research, U. S. Department of Energy.

  8. Power Loss Analysis and Comparison of Segmented and Unsegmented Energy Coupling Coils for Wireless Energy Transfer.

    Science.gov (United States)

    Tang, Sai Chun; McDannold, Nathan J

    2015-03-01

    This paper investigated the power losses of unsegmented and segmented energy coupling coils for wireless energy transfer. Four 30-cm energy coupling coils with different winding separations, conductor cross-sectional areas, and number of turns were developed. The four coils were tested in both unsegmented and segmented configurations. The winding conduction and intrawinding dielectric losses of the coils were evaluated individually based on a well-established lumped circuit model. We found that the intrawinding dielectric loss can be as much as seven times higher than the winding conduction loss at 6.78 MHz when the unsegmented coil is tightly wound. The dielectric loss of an unsegmented coil can be reduced by increasing the winding separation or reducing the number of turns, but the power transfer capability is reduced because of the reduced magnetomotive force. Coil segmentation using resonant capacitors has recently been proposed to significantly reduce the operating voltage of a coil to a safe level in wireless energy transfer for medical implants. Here, we found that it can naturally eliminate the dielectric loss. The coil segmentation method and the power loss analysis used in this paper could be applied to the transmitting, receiving, and resonant coils in two- and four-coil energy transfer systems.

  9. Inelastic collisions of medium energy atomic elements. Qualitative model of energy losses during collisions

    International Nuclear Information System (INIS)

    Pustovit, A.N.

    2006-01-01

    A new approach to the theoretical description of energy losses of atomic particle of medium energy during their interaction with the substance is proposed. The corner-stone of this approach is the supposition that all of the collision processes have inelastic nature during particle movement through the substance, while the calculation of the atomic particles braking is based on the law of their dispersion and the laws of energy and momentum conservation at the inelastic collisions. It is shown that inelastic atomic collision there are three dispersion zones for the only potential interaction with different laws, which characterize energy losses. The application conditions of this approach are determined [ru

  10. Auger electron spectroscopy, ionization loss spectroscopy, appearance potential spectroscopy

    International Nuclear Information System (INIS)

    Riwan, R.

    1973-01-01

    The spectroscopy of surfaces using an incident electron beam is studied. The fundamental mechanisms are discussed together with the parameters involved in Auger emission: excitation of the atom, de-excitation by electron emission, and the migration of electrons towards the surface and their ejection. Some examples of applications are given (surface structures, metallurgy, chemical information). Two new techniques for analyzing surfaces are studied: ionization spectroscopy, and appearance potential spectroscopy [fr

  11. Beam Loss Calibration Studies for High Energy Proton Accelerators

    CERN Document Server

    Stockner, M

    2007-01-01

    CERN's Large Hadron Collider (LHC) is a proton collider with injection energy of 450 GeV and collision energy of 7 TeV. Superconducting magnets keep the particles circulating in two counter rotating beams, which cross each other at the Interaction Points (IP). Those complex magnets have been designed to contain both beams in one yoke within a cryostat. An unprecedented amount of energy will be stored in the circulating beams and in the magnet system. The LHC outperforms other existing accelerators in its maximum beam energy by a factor of 7 and in its beam intensity by a factor of 23. Even a loss of a small fraction of the beam particles may cause the transition from the superconducting to the normal conducting state of the coil or cause physical damage to machine components. The unique combination of these extreme beam parameters and the highly advanced superconducting technology has the consequence that the LHC needs a more efficient beam cleaning and beam loss measurement system than previous accelerators....

  12. Integrated simulation of ELM energy loss determined by pedestal MHD and SOL transport

    International Nuclear Information System (INIS)

    Hayashi, N.; Takizuka, T.; Ozeki, T.; Aiba, N.; Oyama, N.

    2007-01-01

    An integrated simulation code TOPICS-IB based on a transport code with a stability code for the peeling-ballooning modes and a scrape-off-layer (SOL) model has been developed to clarify self-consistent effects of edge localized modes (ELMs) and the SOL on the plasma performance. Experimentally observed collisionality dependence of the ELM energy loss is found to be caused by both the edge bootstrap current and the SOL transport. The bootstrap current decreases with an increase in collisionality and intensifies the magnetic shear at the pedestal region. The increase in the magnetic shear reduces the width of eigenfunctions of unstable modes, which results in the reduction of both the area of the ELM enhanced transport and the ELM enhanced transport near the separatrix. On the other hand, when an ELM crash occurs, the energy flows into the SOL and the SOL temperature rapidly increases. The increase in the SOL temperature lowers the ELM energy loss due to the flattening of the radial edge gradient. The parallel electron heat conduction determines how the SOL temperature increases. For higher collisionality, the conduction becomes lower and the SOL electron temperature increases more. By the above two mechanisms, the ELM energy loss decreases with increasing collisionality

  13. Competition Between Radial Loss and EMIC Wave Scattering of MeV Electrons During Strong CME-shock Driven Storms

    Science.gov (United States)

    Hudson, M. K.; Jaynes, A. N.; Li, Z.; Malaspina, D.; Millan, R. M.; Patel, M.; Qin, M.; Shen, X.; Wiltberger, M. J.

    2017-12-01

    The two strongest storms of Solar Cycle 24, 17 March and 22 June 2015, provide a contrast between magnetospheric response to CME-shocks at equinox and solstice. The 17 March CME-shock initiated storm produced a stronger ring current response with Dst = - 223 nT, while the 22 June CME-shock initiated storm reached a minimum Dst = - 204 nT. The Van Allen Probes ECT instrument measured a dropout in flux for both events which can be characterized by magnetopause loss at higher L values prior to strong recovery1. However, rapid loss is seen at L 3 for the June storm at high energies with maximum drop in the 5.2 MeV channel of the REPT instrument coincident with the observation of EMIC waves in the H+ band by the EMFISIS wave instrument. The rapid time scale of loss can be determined from the 65 minute delay in passage of the Probe A relative to the Probe B spacecraft. The distinct behavior of lower energy electrons at higher L values has been modeled with MHD-test particle simulations, while the rapid loss of higher energy electrons is examined in terms of the minimum resonant energy criterion for EMIC wave scattering, and compared with the timescale for loss due to EMIC wave scattering which has been modeled for other storm events.2 1Baker, D. N., et al. (2016), Highly relativistic radiation belt electron acceleration, transport, and loss: Large solar storm events of March and June 2015, J. Geophys. Res. Space Physics, 121, 6647-6660, doi:10.1002/2016JA022502. 2Li, Z., et al. (2014), Investigation of EMIC wave scattering as the cause for the BARREL 17 January 2013 relativistic electron precipitation event: A quantitative comparison of simulation with observations, Geophys. Res. Lett., 41, 8722-8729, doi:10.1002/2014GL062273.

  14. Projectile electron loss in collisions of light charged ions with helium

    International Nuclear Information System (INIS)

    Yin Yong-Zhi; Chen Xi-Meng; Wang Yun

    2014-01-01

    We investigate the single-electron loss processes of light charged ions (Li 1+,2+ , C 2+,3+,5+ , and O 2+,3+ ) in collisions with helium. To better understand the experimental results, we propose a theoretical model to calculate the cross section of projectile electron loss. In this model, an ionization radius of the incident ion was defined under the classical over-barrier model, and we developed ''strings'' to explain the processes of projectile electron loss, which is similar with the molecular over-barrier model. Theoretical calculations are in good agreement with the experimental results for the cross section of single-electron loss and the ratio of double-to-single ionization of helium associated with one-electron loss. (atomic and molecular physics)

  15. High Q diamond hemispherical resonators: fabrication and energy loss mechanisms

    International Nuclear Information System (INIS)

    Bernstein, Jonathan J; Bancu, Mirela G; Bauer, Joseph M; Cook, Eugene H; Kumar, Parshant; Nyinjee, Tenzin; Perlin, Gayatri E; Ricker, Joseph A; Teynor, William A; Weinberg, Marc S; Newton, Eric

    2015-01-01

    We have fabricated polycrystalline diamond hemispheres by hot-filament CVD (HFCVD) in spherical cavities wet-etched into a high temperature glass substrate CTE matched to silicon. Hemispherical resonators 1.4 mm in diameter have a Q of up to 143 000 in the fundamental wineglass mode, for a ringdown time of 2.4 s. Without trimming, resonators have the two degenerate wineglass modes frequency matched as close as 2 Hz, or 0.013% of the resonant frequency (∼16 kHz). Laser trimming was used to match resonant modes on hemispheres to 0.3 Hz. Experimental and FEA energy loss studies on cantilevers and hemispheres examine various energy loss mechanisms, showing that surface related losses are dominant. Diamond cantilevers with a Q of 400 000 and a ringdown time of 15.4 s were measured, showing the potential of polycrystalline diamond films for high Q resonators. These resonators show great promise for use as hemispherical resonant gyroscopes (HRGs) on a chip. (paper)

  16. Elastic energy loss and longitudinal straggling of a hard jet

    International Nuclear Information System (INIS)

    Majumder, A.

    2009-01-01

    The elastic energy loss encountered by jets produced in deep-inelastic scattering (DIS) off a large nucleus is studied in the collinear limit. In close analogy to the case of (nonradiative) transverse momentum broadening, which is dependent on the medium transport coefficient q, a class of medium enhanced higher twist operators which contribute to the nonradiative loss of the forward light-cone momentum of the jet (q - ) are identified and the leading correction in the limit of asymptotically high q - is isolated. Based on these operator products, a new transport coefficient e is motivated which quantifies the energy loss per unit length encountered by the hard jet. These operator products are then computed, explicitly, in the case of a similar hard jet traversing a deconfined quark-gluon plasma (QGP) in the hard-thermal-loop (HTL) approximation. This is followed by an evaluation of subleading contributions which are suppressed by the inverse light-cone momentum q - , which yields the longitudinal 'straggling', i.e., a slight change in light cone momentum due to the Brownian propagation through a medium with a fluctuating color field.

  17. Investigation of the energy loss and the charge state of high energy heavy ions in a hydrogen plasma

    International Nuclear Information System (INIS)

    Dietrich, K.G.

    1991-07-01

    For heavy ions with energy of 1.4 to 5.9 MeV/u the energy loss and charge state after transmission through a totally ionized hydrogen plasma are investigated. Plasma target was a Z-pinch device incorporated in the beam optics of the accelerator by a pumping system. In the 20 cm long pinch hydrogen plasmas with densities up to 1.5x10 19 cm -3 and temperatures above 5 eV are produced, with ionization efficiency higher than 99%. The ions pass the plasma on the symmetry axis of the plasma column through small apertures in the electrodes. The energy loss was measured by time-of-flight method, the plasma density by interferometry along the pinch axis. For the first time the ion charge after transmission through the plasma has been determined by a charge spectrometer being a combination of a dipole magnet and a position sensitive detector with high time resolution. A growth of the average charge of heavy ions in plasma higher than the equilibrium charge in cold gas was discovered, caused by a reduction of electron capture by fast heavy ions in ionized matter. The electron loss rates in plasma and cold gas are equal. (orig./AH) [de

  18. Calculations on charge state and energy loss of argon ions in partially and fully ionized carbon plasmas.

    Science.gov (United States)

    Barriga-Carrasco, Manuel D; Casas, David; Morales, Roberto

    2016-03-01

    The energy loss of argon ions in a target depends on their velocity and charge density. At the energies studied in this work, it depends mostly on the free and bound electrons in the target. Here the random-phase approximation is used for analyzing free electrons at any degeneracy. For the plasma-bound electrons, an interpolation between approximations for low and high energies is applied. The Brandt-Kitagawa (BK) model is employed to depict the projectile charge space distribution, and the stripping criterion of Kreussler et al. is used to determine its equilibrium charge state Q(eq). This latter criterion implies that the equilibrium charge state depends slightly on the electron density and temperature of the plasma. On the other hand, the effective charge Q(eff) is obtained as the ratio between the energy loss of the argon ion and that of the proton for the same plasma conditions. This effective charge Q(eff) is larger than the equilibrium charge state Q(eq) due to the incorporation of the BK charge distribution. Though our charge-state estimations are not exactly the same as the experimental values, our energy loss agrees quite well with the experiments. It is noticed that the energy loss in plasmas is higher than that in the same cold target of about, ∼42-62.5% and increases with carbon plasma ionization. This confirms the well-known enhanced plasma stopping. It is also observed that only a small part of this energy loss enhancement is due to an increase of the argon charge state, namely only ∼2.2 and 5.1%, for the partially and the fully ionized plasma, respectively. The other contribution is connected with a better energy transfer to the free electrons at plasma state than to the bound electrons at solid state of about, ∼38.8-57.4%, where higher values correspond to a fully ionized carbon plasma.

  19. Time-dependent density functional calculation of the energy loss of antiprotons colliding with metallic nanoshells

    International Nuclear Information System (INIS)

    Quijada, M.; Borisov, A.G.; Muino, R.D.

    2008-01-01

    Time-dependent density functional theory is used to study the interaction between antiprotons and metallic nanoshells. The ground state electronic properties of the nanoshell are obtained in the jellium approximation. The energy lost by the antiproton during the collision is calculated and compared to that suffered by antiprotons traveling in metal clusters. The resulting energy loss per unit path length of material in thin nanoshells is larger than the corresponding quantity for clusters. It is shown that the collision process can be interpreted as the antiproton crossing of two nearly bi-dimensional independent metallic systems. (copyright 2008 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

  20. CMOS circuits for piezoelectric energy harvesters efficient power extraction, interface modeling and loss analysis

    CERN Document Server

    Hehn, Thorsten

    2014-01-01

    This book deals with the challenge of exploiting ambient vibrational energy which can be used to power small and low-power electronic devices, e.g. wireless sensor nodes. Generally, particularly for low voltage amplitudes, low-loss rectification is required to achieve high conversion efficiency. In the special case of piezoelectric energy harvesting, pulsed charge extraction has the potential to extract more power compared to a single rectifier. For this purpose, a fully autonomous CMOS integrated interface circuit for piezoelectric generators which fulfills these requirements is presented.Due

  1. On a temporal evolution of the ultra-relativistic electron spectrum by action of synchrotron losses and turbulent acceleration

    International Nuclear Information System (INIS)

    Samsonov, A.M.; Fedorenko, V.N.

    1981-01-01

    The kinetic equation describing temporal evolution of the ultra-relativistic electrons' energy spectrum effected by synchrotron losses and turbulent acceleration is solved for the isotropic part of the electrons' distribution function. The original distribution is assumed to be given in the form of a power spectrum. Turbulence properties are stated by means of the turbulent acceleration coefficient depending on epsilon energy D(epsilon)=D 0 epsilon 3 which is related to the synchrotron losses coefficient b(epsilon)=b 0 epsilon 3 so that the isotropization of the distribution function is provided without essential acceleration of particles. The initial spectrum is conserved up to some values of time t and energy epsilon connected by inequality epsilonb 0 t 0 /D 0 -2 if epsilonD 0 t>>1 and b 0 >>D 0 . Finally, are possible applications of the solution to description of processes in supernova shells and radio galaxies are discussed [ru

  2. Technology Roadmap. Energy Loss Reduction and Recovery in Industrial Energy Systems

    Energy Technology Data Exchange (ETDEWEB)

    none,

    2004-11-01

    To help guide R&D decision-making and gain industry insights on the top opportunities for improved energy systems, ITP sponsored the Energy Loss Reduction and Recoveryin Energy Systems Roadmapping Workshopin April 2004 in Baltimore, Maryland. This Technology Roadmapis based largely on the results of the workshop and additional industrial energy studies supported by ITP and EERE. It summarizes industry feedback on the top opportunities for R&D investments in energy systems, and the potential for national impacts on energy use and the environment.

  3. Extended wave-packet model to calculate energy-loss moments of protons in matter

    Science.gov (United States)

    Archubi, C. D.; Arista, N. R.

    2017-12-01

    In this work we introduce modifications to the wave-packet method proposed by Kaneko to calculate the energy-loss moments of a projectile traversing a target which is represented in terms of Gaussian functions for the momentum distributions of electrons in the atomic shells. These modifications are introduced using the Levine and Louie technique to take into account the energy gaps corresponding to the different atomic levels of the target. We use the extended wave-packet model to evaluate the stopping power, the energy straggling, the inverse mean free path, and the ionization cross sections for protons in several targets, obtaining good agreements for all these quantities on an extensive energy range that covers low-, intermediate-, and high-energy regions. The extended wave-packet model proposed here provides a method to calculate in a very straightforward way all the significant terms of the inelastic interaction of light ions with any element of the periodic table.

  4. Energy losses in magnetically insulated transmission lines due to microparticles

    International Nuclear Information System (INIS)

    Gray, E.W.; Stinnett, R.W.

    1987-01-01

    We discuss the effects of high-velocity and hypervelocity microparticles in the magnetically insulated transmission lines of multiterawatt accelerators used for particle beam fusion and radiation effects simulation. These microparticles may be a possible source for plasma production near the anode and cathode in early stages of the voltage pulse, and current carriers during and after the power pulse, resulting in power flow losses. Losses in the current pulse, due to microparticles, are estimated to be approximately 12 mA/cm 2 (0.3 kA) as a lower limit, and --0.3 A/cm 2 (7.2 kA) for microparticle initiated, anode plasma positive ion transport. We have calculated the velocities reached by these microparticles and the effects on them of Van der Waals forces. Field emission from the particles and their effects on cathode and anode plasma formation have been examined. Particle collision with the electrodes is also examined in terms of plasma production, as in the electron deposition in the particles in transit across the anode-cathode gap. Blistering of the electrode surface, thought to be due to H - bombardment was also observed and appears to be consistent with losses due to negative ions previously reported by J. P. VanDevender, R. W. Stinnett, and R. J. Anderson [App. Phys. Lett. 38, 229 (1981)

  5. Timescale and magnitude of plasma thermal energy loss before and during disruptions in JET

    International Nuclear Information System (INIS)

    Riccardo, V.; Loarte, A.

    2005-01-01

    In this paper we analyse and discuss the thermal energy loss dynamics before and during JET disruptions that occurred between 2002 and 2004 in discharges which reached >4.5 MJ of thermal energy. We observe the slow thermal energy transients with diamagnetic loops and the fast ones with electron cyclotron emission and soft x-ray diagnostics. For most disruption types in JET, the plasma thermal energy at the time of the thermal quench is substantially less than that of the full performance plasma, typically in the range of 10-50% depending on plasma conditions and disruption type. The exceptions to this observation are disruptions in plasmas with a strong internal transport barrier (ITB) and in discharges terminating in a pure vertical displacement event, in which the plasma conserves a very high energy content up to the thermal quench. These disruption types are very sudden, leaving little scope for the combined action of soft plasma landing strategies and intrinsic performance degradation, both requiring >500 ms to be effective, to decrease the available thermal energy. The characteristic time for the loss of energy from the main plasma towards the PFCs in the thermal quench of JET disruptions is in the range 0.05-3.0 ms. The shortest timescales are typical of disruptions caused by excessive pressure peaking in ITB discharges. The available thermal energy fraction and thermal quench duration observed in JET can be processed (with due caution) into estimates for the projected PFC lifetime of the ITER target

  6. Extended defect related energy loss in CVD diamond revealed by spectrum imaging in a dedicated STEM

    International Nuclear Information System (INIS)

    Bangert, U.; Harvey, A.J.; Schreck, M.; Hoermann, F.

    2005-01-01

    This article aims at investigations of the low EEL region in the wide band gap system diamond. The advent of the UHV Enfina electron energy loss spectrometer combined with Digital Micrograph acquisition and processing software has made reliable detection of absorption losses below 10 eV possible. Incorporated into a dedicated STEM this instrumentation allows the acquisition of spectral information via spectrum maps (spectrum imaging) of sample areas hundreds of nanometers across, with nanometers pixel sizes, adequate spectrum statistics and 0.3 eV energy resolution, in direct correlation with microstructural features in the mapping area. We aim at discerning defect related losses at band gap energies, and discuss different routes to simultaneously process and analyse the spectra in a map. This involves extracting the zero loss peak from each spectrum and constructing ratio maps from the intensities in two energy windows, one defect related and one at a higher, crystal bandstructure dominated energy. This was applied to the residual spectrum maps and their first derivatives. Secondly, guided by theoretical EEL spectra calculations, the low loss spectra were fitted by a series of gaussian distributions. Pixel maps were constructed from amplitude ratios of gaussians, situated in the defect and the unaffected energy regime. The results demonstrate the existence of sp 2 -bonded carbon in the vicinity of stacking faults and partial dislocations in CVD diamond as well as additional states below conduction band, tailing deep into the band gap, at a node in a perfect dislocation. Calculated EEL spectra of shuffle dislocations give similar absorption features at 5-8 eV, and it is thought that this common feature is due to sp 2 -type bonding

  7. Dispersion self-energy of the electron

    International Nuclear Information System (INIS)

    Hawton, M.

    1991-01-01

    Electron mass renormalization and the Lamb shift have been investigated using the dispersion self-energy formalism. If shifts of both the electromagnetic field and quantum-mechanical transitions frequencies are considered, absorption from the electromagnetic field is canceled by emission due to atomic fluctuations. The frequencies of all modes are obtained from the self-consistency condition that the field seen by the electron is the same as the field produced by the expectation value of current. The radiation present can thus be viewed as arising from emission and subsequent reabsorption by matter. As developed here, the numerical predictions of dispersion theory are identical to those of quantum electrodynamics. The physical picture implied by dispersion theory is discussed in the context of semiclassical theories and quantum electrodynamics

  8. Initial electron energy spectra in water irradiated by photons with energies to 1 GeV

    International Nuclear Information System (INIS)

    Todo, A.S.; Hiromoto, G.; Turner, J.E.; Hamm, R.N.; Wright, H.A.

    1984-02-01

    This work was undertaken to provide basic physical data for use in the dosimetry of high-energy photons. Present and future sources of such photons are described, and the relevant literature is reviewed and summarized. Calculations were performed with a Monte Carlo computer code, PHOEL-3, which is also described. Tables of initial electron and positron energies are presented for monoenergetic photons undergoing single interactions in water. Photon energies to 1 GeV are treated. The code treats explicitly the production of electron-positron pairs, Compton scattering, photoelectric absorption, and the emission of Auger electrons following the occurrence of K-shell vacancies in oxygen. The tables give directly the information needed to specify the absolute single-collision kerma in water, which approximates tissue, at each photon energy. Results for continuous photon energy spectra can be obtained by using linear interpolation with the tables. (Continuous spectra can also be used directly in PHOEL-3.) The conditions under whch first-collision kerma approximate absorbed dose are discussed. A formula is given for estimating bremsstrahlung energy loss, one of the principal differences between kerma and absorbed dose in practical cases. 31 references, 4 figures, 18 tables

  9. Acceleration and Energy Loss in N=4 SYM

    OpenAIRE

    Chernicoff, Mariano; Guijosa, Alberto

    2009-01-01

    We give a brief overview of the results obtained in arXiv:0803.3070, concerning the rate of energy loss of an accelerating quark in strongly-coupled N=4 super-Yang-Mills, both at zero and finite temperature. For phenomenological purposes, our main result is that, when a quark is created within the plasma together with its corresponding antiquark, the quark starts feeling the plasma only after the q-\\bar{q} separation becomes larger than the (v-dependent) screening length, and from this point ...

  10. On selection rules and inelastic electron scattering at intermediate energies

    International Nuclear Information System (INIS)

    Nuroh, K.

    1986-12-01

    Correlation effects are included in the Bethe-Born theory for the generalized oscillator strength of inelastic scattering of electrons on atoms. The formulation is such as to allow for the calculation of relative line strengths of multiplets. It is used to analyze line strengths of the 4d → 4f transition in La 3+ and Ce 4+ within LS-coupling. The analysis indicates that only singlet states of the intermediate 4d 9 4f configuration are allowed. Calculated line strengths are compared with a recent core electron energy loss spectra of metallic La and tetravalent CeO 2 and there is an overall qualitative agreement between theory and experiment. (author). 11 refs, 4 figs, 2 tabs

  11. Angular dispersion and energy loss of H+ and He+ in metals

    International Nuclear Information System (INIS)

    Cantero, Esteban

    2006-01-01

    In this master thesis the effects produced when a light ion beam traverses a thin metallic film were studied.In particular, the interactions of low energy (E ≤ 10 keV) light ions (H + ,H 2 + , D + , He + ) with monocrystalline and also polycrystalline gold samples were investigated.In first place, the dependence of the stopping power with projectiles' velocity was studied, analyzing the threshold effect in the excitation of the 5d electrons in the channelling regime for energies between 0,4 and 9 keV.Next, the angular dispersion of ions in polycrystalline and monocrystalline films was measured and analyzed.Comparisons for different energies and projectiles were done, studying molecular and isotopic effects.Using Lindhard's channeling theory, a scale law for the angular dispersion of angles greater than the critical angle was found.Additionally, the angular dependence of the energy loss and the energy loss straggling of protons transmitted through monocrystals were measured.To explain the angular variations of these magnitudes a theoretical model based on the electronic density fluctuations inside the channel was developed [es

  12. Nanoscale Energy-Filtered Scanning Confocal Electron Microscopy Using a Double-Aberration-Corrected Transmission Electron Microscope

    International Nuclear Information System (INIS)

    Wang Peng; Behan, Gavin; Kirkland, Angus I.; Nellist, Peter D.; Takeguchi, Masaki; Hashimoto, Ayako; Mitsuishi, Kazutaka; Shimojo, Masayuki

    2010-01-01

    We demonstrate that a transmission electron microscope fitted with two spherical-aberration correctors can be operated as an energy-filtered scanning confocal electron microscope. A method for establishing this mode is described and initial results showing 3D chemical mapping with nanoscale sensitivity to height and thickness changes in a carbon film are presented. Importantly, uncorrected chromatic aberration does not limit the depth resolution of this technique and moreover performs an energy-filtering role, which is explained in terms of a combined depth and energy-loss response function.

  13. The role of energy losses in photosynthetic light harvesting

    Science.gov (United States)

    Krüger, T. P. J.; van Grondelle, R.

    2017-07-01

    Photosynthesis operates at the bottom of the food chain to convert the energy of light into carbohydrates at a remarkable global rate of about 130 TW. Nonetheless, the overall photosynthetic process has a conversion efficiency of a few percent at best, significantly less than bottom-up photovoltaic cells. The primary photosynthetic steps, consisting of light harvesting and charge separation, are often presented as having near-unity quantum efficiency but this holds only true under ideal conditions. In this review, we discuss the importance of energy loss mechanisms to establish robustness in photosynthetic light harvesting. Thermal energy dissipation of light-harvesting complexes (LHCs) in different environments is investigated and the relationships and contrasts between concentration quenching of high pigment concentrations, photoprotection (non-photochemical quenching), quenching due to protein aggregation, and fluorescence blinking are discussed. The role of charge-transfer states in light harvesting and energy dissipation is highlighted and the importance of controlled protein structural disorder to switch the light-harvesting antennae between effective light harvesters and efficient energy quenchers is underscored. The main LHC of plants, LHCII, is used as a prime example.

  14. The role of energy losses in photosynthetic light harvesting

    International Nuclear Information System (INIS)

    Krüger, T P J; Van Grondelle, R

    2017-01-01

    Photosynthesis operates at the bottom of the food chain to convert the energy of light into carbohydrates at a remarkable global rate of about 130 TW. Nonetheless, the overall photosynthetic process has a conversion efficiency of a few percent at best, significantly less than bottom-up photovoltaic cells. The primary photosynthetic steps, consisting of light harvesting and charge separation, are often presented as having near-unity quantum efficiency but this holds only true under ideal conditions. In this review, we discuss the importance of energy loss mechanisms to establish robustness in photosynthetic light harvesting. Thermal energy dissipation of light-harvesting complexes (LHCs) in different environments is investigated and the relationships and contrasts between concentration quenching of high pigment concentrations, photoprotection (non-photochemical quenching), quenching due to protein aggregation, and fluorescence blinking are discussed. The role of charge-transfer states in light harvesting and energy dissipation is highlighted and the importance of controlled protein structural disorder to switch the light-harvesting antennae between effective light harvesters and efficient energy quenchers is underscored. The main LHC of plants, LHCII, is used as a prime example. (topical review)

  15. Energy loss effect in high energy nuclear Drell-Yan process

    International Nuclear Information System (INIS)

    Duan, C.G.; Song, L.H.; Huo, L.J.; Li, G.L.

    2003-01-01

    The energy loss effect in nuclear matter, which is a nuclear effect apart from the nuclear effect on the parton distribution as in deep-inelastic scattering process, can be measured best by the nuclear dependence of the high energy nuclear Drell-Yan process. By means of the nuclear parton distribution studied only with lepton deep-inelastic scattering experimental data, the measured Drell-Yan production cross sections for 800 GeV proton incident on a variety of nuclear targets are analyzed within the Glauber framework which takes into account the energy loss of the beam proton. It is shown that the theoretical results with considering the energy loss effect are in good agreement with the FNAL E866 data. (orig.)

  16. Energy deposition model for low-energy electrons (10-10 000 eV) in air

    International Nuclear Information System (INIS)

    Roldan, A.; Perez, J.M.; Williart, A.; Blanco, F.; Garcia, G.

    2004-01-01

    An energy deposition model for electrons in air that can be useful in microdosimetric applications is presented in this study. The model is based on a Monte Carlo simulation of the single electron scattering processes that can take place with the molecular constituents of the air in the energy range 10-10 000 eV. The input parameters for this procedure have been the electron scattering cross sections, both differential and integral. These parameters were calculated using a model potential method which describes the electron scattering with the molecular constituent of air. The reliability of the calculated integral cross section values has been evaluated by comparison with direct total electron scattering cross-section measurements performed by us in a transmission beam experiment. Experimental energy loss spectra for electrons in air have been used as probability distribution functions to define the electron energy loss in single collision events. The resulting model has been applied to simulate the electron transport through a gas cell containing air at different pressures and the results have been compared with those observed in the experiments. Finally, as an example of its applicability to dosimetric issues, the energy deposition of 10 000 eV by means of successive collisions in a free air chamber has been simulated

  17. Loss of Energy Concentration in Nonlinear Evolution Beam Equations

    Science.gov (United States)

    Garrione, Maurizio; Gazzola, Filippo

    2017-12-01

    Motivated by the oscillations that were seen at the Tacoma Narrows Bridge, we introduce the notion of solutions with a prevailing mode for the nonlinear evolution beam equation u_{tt} + u_{xxxx} + f(u)= g(x, t) in bounded space-time intervals. We give a new definition of instability for these particular solutions, based on the loss of energy concentration on their prevailing mode. We distinguish between two different forms of energy transfer, one physiological (unavoidable and depending on the nonlinearity) and one due to the insurgence of instability. We then prove a theoretical result allowing to reduce the study of this kind of infinite-dimensional stability to that of a finite-dimensional approximation. With this background, we study the occurrence of instability for three different kinds of nonlinearities f and for some forcing terms g, highlighting some of their structural properties and performing some numerical simulations.

  18. Medical radiation dosimetry theory of charged particle collision energy loss

    CERN Document Server

    McParland, Brian J

    2014-01-01

    Accurate radiation dosimetry is a requirement of radiation oncology, diagnostic radiology and nuclear medicine. It is necessary so as to satisfy the needs of patient safety, therapeutic and diagnostic optimisation, and retrospective epidemiological studies of the biological effects resulting from low absorbed doses of ionising radiation. The radiation absorbed dose received by the patient is the ultimate consequence of the transfer of kinetic energy through collisions between energetic charged particles and atoms of the tissue being traversed. Thus, the ability of the medical physicist to both measure and calculate accurately patient dosimetry demands a deep understanding of the physics of charged particle interactions with matter. Interestingly, the physics of charged particle energy loss has an almost exclusively theoretical basis, thus necessitating an advanced theoretical understanding of the subject in order to apply it appropriately to the clinical regime. ​ Each year, about one-third of the worl...

  19. Resolving runaway electron distributions in space, time, and energy

    Science.gov (United States)

    Paz-Soldan, C.; Cooper, C. M.; Aleynikov, P.; Eidietis, N. W.; Lvovskiy, A.; Pace, D. C.; Brennan, D. P.; Hollmann, E. M.; Liu, C.; Moyer, R. A.; Shiraki, D.

    2018-05-01

    Areas of agreement and disagreement with present-day models of runaway electron (RE) evolution are revealed by measuring MeV-level bremsstrahlung radiation from runaway electrons (REs) with a pinhole camera. Spatially resolved measurements localize the RE beam, reveal energy-dependent RE transport, and can be used to perform full two-dimensional (energy and pitch-angle) inversions of the RE phase-space distribution. Energy-resolved measurements find qualitative agreement with modeling on the role of collisional and synchrotron damping in modifying the RE distribution shape. Measurements are consistent with predictions of phase-space attractors that accumulate REs, with non-monotonic features observed in the distribution. Temporally resolved measurements find qualitative agreement with modeling on the impact of collisional and synchrotron damping in varying the RE growth and decay rate. Anomalous RE loss is observed and found to be largest at low energy. Possible roles for kinetic instability or spatial transport to resolve these anomalies are discussed.

  20. Single atom spectroscopy: Decreased scattering delocalization at high energy losses, effects of atomic movement and X-ray fluorescence yield.

    Science.gov (United States)

    Tizei, Luiz H G; Iizumi, Yoko; Okazaki, Toshiya; Nakanishi, Ryo; Kitaura, Ryo; Shinohara, Hisanori; Suenaga, Kazu

    2016-01-01

    Single atom localization and identification is crucial in understanding effects which depend on the specific local environment of atoms. In advanced nanometer scale materials, the characteristics of individual atoms may play an important role. Here, we describe spectroscopic experiments (electron energy loss spectroscopy, EELS, and Energy Dispersed X-ray spectroscopy, EDX) using a low voltage transmission electron microscope designed towards single atom analysis. For EELS, we discuss the advantages of using lower primary electron energy (30 keV and 60 keV) and higher energy losses (above 800 eV). The effect of atomic movement is considered. Finally, we discuss the possibility of using atomically resolved EELS and EDX data to measure the fluorescence yield for X-ray emission. Copyright © 2015 Elsevier B.V. All rights reserved.

  1. Single atom spectroscopy: Decreased scattering delocalization at high energy losses, effects of atomic movement and X-ray fluorescence yield

    International Nuclear Information System (INIS)

    Tizei, Luiz H.G.; Iizumi, Yoko; Okazaki, Toshiya; Nakanishi, Ryo; Kitaura, Ryo; Shinohara, Hisanori; Suenaga, Kazu

    2016-01-01

    Single atom localization and identification is crucial in understanding effects which depend on the specific local environment of atoms. In advanced nanometer scale materials, the characteristics of individual atoms may play an important role. Here, we describe spectroscopic experiments (electron energy loss spectroscopy, EELS, and Energy Dispersed X-ray spectroscopy, EDX) using a low voltage transmission electron microscope designed towards single atom analysis. For EELS, we discuss the advantages of using lower primary electron energy (30 keV and 60 keV) and higher energy losses (above 800 eV). The effect of atomic movement is considered. Finally, we discuss the possibility of using atomically resolved EELS and EDX data to measure the fluorescence yield for X-ray emission.

  2. Modelling high-resolution electron microscopy based on core-loss spectroscopy

    International Nuclear Information System (INIS)

    Allen, L.J.; Findlay, S.D.; Oxley, M.P.; Witte, C.; Zaluzec, N.J.

    2006-01-01

    There are a number of factors affecting the formation of images based on core-loss spectroscopy in high-resolution electron microscopy. We demonstrate unambiguously the need to use a full nonlocal description of the effective core-loss interaction for experimental results obtained from high angular resolution electron channelling electron spectroscopy. The implications of this model are investigated for atomic resolution scanning transmission electron microscopy. Simulations are used to demonstrate that core-loss spectroscopy images formed using fine probes proposed for future microscopes can result in images that do not correspond visually with the structure that has led to their formation. In this context, we also examine the effect of varying detector geometries. The importance of the contribution to core-loss spectroscopy images by dechannelled or diffusely scattered electrons is reiterated here

  3. Nonequilibrium thermodynamics and energy efficiency in weight loss diets

    Directory of Open Access Journals (Sweden)

    Fine Eugene J

    2007-07-01

    Full Text Available Abstract Carbohydrate restriction as a strategy for control of obesity is based on two effects: a behavioral effect, spontaneous reduction in caloric intake and a metabolic effect, an apparent reduction in energy efficiency, greater weight loss per calorie consumed. Variable energy efficiency is established in many contexts (hormonal imbalance, weight regain and knock-out experiments in animal models, but in the area of the effect of macronutrient composition on weight loss, controversy remains. Resistance to the idea comes from a perception that variable weight loss on isocaloric diets would somehow violate the laws of thermodynamics, that is, only caloric intake is important ("a calorie is a calorie". Previous explanations of how the phenomenon occurs, based on equilibrium thermodynamics, emphasized the inefficiencies introduced by substrate cycling and requirements for increased gluconeogenesis. Living systems, however, are maintained far from equilibrium, and metabolism is controlled by the regulation of the rates of enzymatic reactions. The principles of nonequilibrium thermodynamics which emphasize kinetic fluxes as well as thermodynamic forces should therefore also be considered. Here we review the principles of nonequilibrium thermodynamics and provide an approach to the problem of maintenance and change in body mass by recasting the problem of TAG accumulation and breakdown in the adipocyte in the language of nonequilibrium thermodynamics. We describe adipocyte physiology in terms of cycling between an efficient storage mode and a dissipative mode. Experimentally, this is measured in the rate of fatty acid flux and fatty acid oxidation. Hormonal levels controlled by changes in dietary carbohydrate regulate the relative contributions of the efficient and dissipative parts of the cycle. While no experiment exists that measures all relevant variables, the model is supported by evidence in the literature that 1 dietary carbohydrate, via its

  4. Electron beam accelerator energy control system

    International Nuclear Information System (INIS)

    Sharma, Vijay; Rajan, Rehim; Acharya, S.; Mittal, K.C.

    2011-01-01

    A control system has been developed for the energy control of the electron beam accelerator using PLC. The accelerating voltage of 3 MV has been obtained by using parallel coupled voltage multiplier circuit. A autotransformer controlled variable 0-10 KV DC is fed to a tube based push pull oscillator to generate 120 Khz, 10 KV AC. Oscillator output voltage is stepped up to 0-300 KV/AC using a transformer. 0-300 KVAC is fed to the voltage multiplier column to generate the accelerating voltage at the dome 0-3 MV/DC. The control system has been designed to maintain the accelerator voltage same throughout the operation by adjusting the input voltage in close loop. Whenever there is any change in the output voltage either because of beam loading or arcing in the accelerator. The instantaneous accelerator voltage or energy is a direct proportional to 0-10 KVDC obtained from autotransformer. A PLC based control system with user settable energy level has been installed for 3 MeV, EB accelerator. The PLC takes the user defined energy value through a touch screen and compares it to the actual accelerating voltage (obtained using resistive divider). Depending upon the error the PLC generates the pulses to adjust the autotransformer to bring the actual voltage to the set value within the window of error (presently set to +/- 0.1%). (author)

  5. Electron energy deposition in the middle atmosphere

    International Nuclear Information System (INIS)

    Vampola, A.L.; Gorney, D.J.

    1983-01-01

    Spectra of locally precipating 36- to 317-keV electrons obtained by instrumentation on the S3-2 satellite are used to calculate energy deposition profiles as a function of latitude, longitude, and altitude. In the 70- to 90-km altitude, mid-latitude ionization due to these precipitating energetic electrons can be comparable to that due to direct solar H Lyman α. At night, the electrons produce ionization more than an order of magnitude greater than that expected from scattered H Lyman α. Maximum precipitation rates in the region of the South Atlantic Anomaly are of the order of 10 -2 erg/cm 2 s with a spectrum of form j(E) = 1.34 x 10 5 E/sup -2.27/ (keV). Southern hemisphere precipitation dominates that in the north for 1.1< L<6 except for regions of low local surface field in the northern hemisphere. Above L = 6, local time effects dominate: i.e., longitudinal effects due to the asymmetric magnetic field which are strong features below L = 6 disappear and are replaced by high-latitude precipitation events which are local time features

  6. Effect of inelastic energy losses on development of atom-atom collision cascades

    International Nuclear Information System (INIS)

    Marinyuk, V.V.; Remizovich, V.S.

    2001-01-01

    The problem of influence of inelastic energy losses (ionization braking) of particles on the development of atom-atom collision cascades in infinite medium was studied theoretically. Main attention was paid to study of angular and energy distributions of primary ions and cascade atoms in the presence of braking. Analytical calculations were made in the assumption that single scattering of particles occurs by solid balls law, while the value of electron braking ability of a medium is determined by the Lindhard formula. It is shown that account of braking (directly when solving the Boltzmann transport equation) changes in principle the previously obtained angular and energy spectra of ions and cascade atoms. Moreover, it is the braking that is the determining factor responsible for anisotropy of angular distributions of low-energy primary ions and cascade atoms [ru

  7. Inelastic energy loss of light particles scattered by solid surfaces at low energy: influence of the 'gap'

    International Nuclear Information System (INIS)

    Boudjema, M.; D'bichi, N.; Boudouma, Y.; Chami, A.C.; Arezki, B.; Khalal, K.; Benazeth, C.; Benoit-Cattin, P.

    2000-01-01

    The energy spectra of particles scattered by solid surfaces are used to determine the inelastic energy loss at low energy. Assuming the binary collision approximation, a modified TRIM code provides length distributions which are converted to time-of-flight (TOF) spectra by using the friction coefficient as an adjustable parameter. Owing to the nonlinear effects occurring in this energy range, the theoretical value of the electronic stopping power is performed from electron-particle scattering cross-section using a screened potential and so, the phase shifts, obtained self-consistently in the framework of density functional theory (DFT). In the case of He/a:Si interaction at 4 keV, the standard model leads to a largely overestimated value. This fact has been attributed to the presence of the electron energy gap E G and to the structure of the valence band. We verify this assumption in a non-static model involving all electrons of the valence band with a threshold condition v e '2 >v F 2 +2E G , where v F is the Fermi velocity and v e the electron velocity after scattering (non-static extended collisional model). The theoretical results agree very well with the experimental ones for He colliding three targets: a:Si, a:Ge and polycrystalline Ni at 4 keV. The calculations performed for the velocity range below 1 a.u. confirm the important role of the gap and the band structure in the lowering of stopping power at low velocity

  8. Experimental and theoretical study of the energy loss of C and O in Zn

    Energy Technology Data Exchange (ETDEWEB)

    Cantero, E. D.; Lantschner, G. H.; Arista, N. R. [Centro Atomico Bariloche and Instituto Balseiro, Comision Nacional de Energia Atomica, 8400 San Carlos de Bariloche (Argentina); Montanari, C. C.; Miraglia, J. E. [Instituto de Astronomia y Fisica del Espacio (CONICET-UBA), Buenos Aires (Argentina); Facultad de Ciencias Exactas y Naturales, Universidad de Buenos Aires, Buenos Aires (Argentina); Behar, M.; Fadanelli, R. C. [Instituto de Fisica, Universidade Federal do Rio Grande do Sul, Avenida Bento Goncalves 9500, Porto Alegre-RS (Brazil)

    2011-07-15

    We present a combined experimental-theoretical study of the energy loss of C and O ions in Zn in the energy range 50-1000 keV/amu. This contribution has a double purpose, experimental and theoretical. On the experimental side, we present stopping power measurements that fill a gap in the literature for these projectile-target combinations and cover an extended energy range, including the stopping maximum. On the theoretical side, we make a quantitative test on the applicability of various theoretical approaches to calculate the energy loss of heavy swift ions in solids. The description is performed using different models for valence and inner-shell electrons: a nonperturbative scattering calculation based on the transport cross section formalism to describe the Zn valence electron contribution, and two different models for the inner-shell contribution: the shellwise local plasma approximation (SLPA) and the convolution approximation for swift particles (CasP). The experimental results indicate that C is the limit for the applicability of the SLPA approach, which previously was successfully applied to projectiles from H to B. We find that this model clearly overestimates the stopping data for O ions. The origin of these discrepancies is related to the perturbative approximation involved in the SLPA. This shortcoming has been solved by using the nonperturbative CasP results to describe the inner-shell contribution, which yields a very good agreement with the experiments for both C and O ions.

  9. Optimization of power output and study of electron beam energy spread in a Free Electron Laser oscillator

    International Nuclear Information System (INIS)

    Abramovich, A.; Pinhasi, Y.; Yahalom, A.; Bar-Lev, D.; Efimov, S.; Gover, A.

    2001-01-01

    Design of a multi-stage depressed collector for efficient operation of a Free Electron Laser (FEL) oscillator requires knowledge of the electron beam energy distribution. This knowledge is necessary to determine the voltages of the depressed collector electrodes that optimize the collection efficiency and overall energy conversion efficiency of the FEL. The energy spread in the electron beam is due to interaction in the wiggler region, as electrons enter the interaction region at different phases relative to the EM wave. This interaction can be simulated well by a three-dimensional simulation code such as FEL3D. The main adjustable parameters that determine the electron beam energy spread after interaction are the e-beam current, the initial beam energy, and the quality factor of the resonator out-coupling coefficient. Using FEL3D, we study the influence of these parameters on the available radiation power and on the electron beam energy distribution at the undulator exit. Simulations performed for I=1.5 A, E=1.4 MeV, L=20% (Internal loss factor) showed that the highest radiated output power and smallest energy spread are attained for an output coupler transmission coefficient T m congruent with 30%

  10. Monte Carlo calculation of energy loss of hydrogen and helium ions transmitted under channelling conditions in silicon single crystal

    International Nuclear Information System (INIS)

    El Bounagui, O.; Erramli, H.

    2010-01-01

    In this work, we report on calculations of the electronic channelling energy loss of hydrogen and helium ions along Si and Si axial directions for the low energy range by using the Monte Carlo simulation code. Simulated and experimental data are compared for protons and He ions in the and axis of silicon. A reasonable agreement was found. Computer simulation was also employed to study the angular dependence of energy loss for 0.5, 0.8, 1, and 2 MeV channelled 4 He ions transmitted through a silicon crystal of 3 μm thickness along the axis.

  11. Contribution from individual nearby sources to the spectrum of high-energy cosmic-ray electrons

    International Nuclear Information System (INIS)

    Sedrati, R.; Attallah, R.

    2014-01-01

    In the last few years, very important data on high-energy cosmic-ray electrons and positrons from high-precision space-born and ground-based experiments have attracted a great deal of interest. These particles represent a unique probe for studying local comic-ray accelerators because they lose energy very rapidly. These energy losses reduce the lifetime so drastically that high-energy cosmic-ray electrons can attain the Earth only from rather local astrophysical sources. This work aims at calculating, by means of Monte Carlo simulation, the contribution from some known nearby astrophysical sources to the cosmic-ray electron/positron spectra at high energy (≥10GeV). The background to the electron energy spectrum from distant sources is determined with the help of the GALPROP code. The obtained numerical results are compared with a set of experimental data

  12. Contribution from individual nearby sources to the spectrum of high-energy cosmic-ray electrons

    Energy Technology Data Exchange (ETDEWEB)

    Sedrati, R., E-mail: rafik.sedrati@univ-annaba.org; Attallah, R.

    2014-04-01

    In the last few years, very important data on high-energy cosmic-ray electrons and positrons from high-precision space-born and ground-based experiments have attracted a great deal of interest. These particles represent a unique probe for studying local comic-ray accelerators because they lose energy very rapidly. These energy losses reduce the lifetime so drastically that high-energy cosmic-ray electrons can attain the Earth only from rather local astrophysical sources. This work aims at calculating, by means of Monte Carlo simulation, the contribution from some known nearby astrophysical sources to the cosmic-ray electron/positron spectra at high energy (≥10GeV). The background to the electron energy spectrum from distant sources is determined with the help of the GALPROP code. The obtained numerical results are compared with a set of experimental data.

  13. Energy loss and (de)coherence effects beyond eikonal approximation

    CERN Document Server

    Apolinário, Liliana; Milhano, Guilherme; Salgado, Carlos A.

    2014-01-01

    The parton branching process is known to be modified in the presence of a medium. Colour decoherence processes are known to determine the process of energy loss when the density of the medium is large enough to break the correlations between partons emitted from the same parent. In order to improve existing calculations that consider eikonal trajectories for both the emitter and the hardest emitted parton, we provide in this work, the calculation of all finite energy corrections for the gluon radiation off a quark in a QCD medium that exist in the small angle approximation and for static scattering centres. Using the path integral formalism, all particles are allowed to undergo Brownian motion in the transverse plane and the offspring allowed to carry an arbitrary fraction of the initial energy. The result is a general expression that contains both coherence and decoherence regimes that are controlled by the density of the medium and by the amount of broadening that each parton acquires independently.

  14. Observational evidence of competing source, loss, and transport processes for relativistic electrons in Earth's outer radiation belt

    Science.gov (United States)

    Turner, Drew; Mann, Ian; Usanova, Maria; Rodriguez, Juan; Henderson, Mike; Angelopoulos, Vassilis; Morley, Steven; Claudepierre, Seth; Li, Wen; Kellerman, Adam; Boyd, Alexander; Kim, Kyung-Chan

    source in the plasma sheet, and chorus waves. We show how sudden losses during outer belt dropout events are dominated at higher L-shells (L>~4) by magnetopause shadowing and outward radial transport, which is effective over the full ranges of energy and equatorial pitch angle of outer belt electrons, but at lower L-shells near the plasmapause, energy and pitch angle dependent losses can also occur and are consistent with rapid scattering by interactions between relativistic electrons and EMIC waves. We show cases demonstrating how these different processes occur simultaneously during active periods, with relative effects that vary as a function of L-shell and electron energy and pitch angle. Ultimately, our results highlight the complexity of competing source/acceleration, loss, and transport processes in Earth’s outer radiation belt and the necessity of using multipoint observations to disambiguate between them for future studies.

  15. Energy loss spectroscopy study of Si(111)--alkali metal interfaces at low temperatures

    International Nuclear Information System (INIS)

    Avci, R.

    1986-01-01

    Studies are made at approx.150 K under ultrahigh vacuum conditions on a wide range of alkali metal coverages on Si(111)-7 x 7. Negative second-derivative backscattered electron energy loss spectroscopy is used with 100 eV primary electrons. The interaction of the alkali metals with the silicon substrate goes through two stages as a function of alkali coverage: In the initial coverages, for less than approx.0.3 monolayer of alkali atoms, the basic reaction is that of charge transfer from the alkali atoms to the Si surface with a loss peak at approx.3.3 eV associated with the charge transfer states. The second stage of reaction: starting after the depletion of all the Si surface states: falls in a coverage range between approx.0.3 and approx.1 monolayer, in which the formation of a metallic layer with a coverage-dependent loss feature at about 2 eV is observed. At still higher coverages, multiple surface and bulk plasmon excitations and their combinations are dominant. In the overall scattering processes most of the parallel momentum (approx.3 A -1 ) is transferred to the sample during the elastic backscattering from the surface, and all the losses are essentially attributed to the forward inelastic scattering before and/or after the elastic process takes place near the metal/Si interface

  16. A technique for determining electron losses for a 20 MeV microtron

    International Nuclear Information System (INIS)

    Harisha, P.; Nayak, A.R.; Mehta, S.K.; Soni, H.C.; Siddappa, K.

    1999-01-01

    A 22 orbit, 20 MeV electron microtron is used as a preaccelerator for the 700 MeV booster synchrotron at INDUS-1, CAT, Indore. Estimation of electron losses at the RF cavity from each orbit is important in obtaining the radiation doses from the body of the microtron. Radiation mapping of the microtron can be used to estimate these loss terms as an alternate to actual measurement by using a measuring probe. (author)

  17. Sanitation methods using high energy electron beams

    International Nuclear Information System (INIS)

    Levaillant, C.; Gallien, C.L.

    1979-01-01

    Short recycling of waste water and the use of liquid or dehydrated sludge as natural manure for agriculture or animal supplement feed is of great economical and ecological interest. It implies strong biological and chemical disinfection. Ionizing radiations produced by radioactive elements or linear accelerators can be used as a complement of conventional methods in the treatment of liquid and solid waste. An experiment conducted with high-energy electron-beam linear accelerators is presented. Degradation of undesirable metabolites in water occurs for a dose of 50 kRad. Undesirable seeds present in sludge are destroyed with a 200 kRad dose. A 300 kRad dose is sufficient for parasitic and bacterial disinfection (DL 90). Destruction of polio virus (DL 90) is obtained for 400 kRad. Higher doses (1000 to 2000 kRad) produce mineralization of toxic organic mercury, reduce some chemical toxic pollutants present in sludge and improve flocculation. (author)

  18. Benchmarking NaI(Tl) Electron Energy Resolution Measurements

    International Nuclear Information System (INIS)

    Mengesha, Wondwosen; Valentine, J D.

    2002-01-01

    A technique for validating electron energy resolution results measured using the modified Compton coincidence technique (MCCT) has been developed. This technique relies on comparing measured gamma-ray energy resolution with calculated values that were determined using the measured electron energy resolution results. These gamma-ray energy resolution calculations were based on Monte Carlo photon transport simulations, the measured NaI(Tl) electron response, a simplified cascade sequence, and the measured electron energy resolution results. To demonstrate this technique, MCCT-measured NaI(Tl) electron energy resolution results were used along with measured gamma-ray energy resolution results from the same NaI(Tl) crystal. Agreement to within 5% was observed for all energies considered between the calculated and measured gamma-ray energy resolution results for the NaI(Tl) crystal characterized. The calculated gamma-ray energy resolution results were also compared with previously published gamma-ray energy resolution measurements with good agreement (<10%). In addition to describing the validation technique that was developed in this study and the results, a brief review of the electron energy resolution measurements made using the MCCT is provided. Based on the results of this study, it is believed that the MCCT-measured electron energy resolution results are reliable. Thus, the MCCT and this validation technique can be used in the future to characterize the electron energy resolution of other scintillators and to determine NaI(Tl) intrinsic energy resolution

  19. Energy loss of heavy ion beams in plasma

    Energy Technology Data Exchange (ETDEWEB)

    Okada, T; Hotta, T [Tokyo Univ. of Agriculture and Technology, Koganei (Japan). Faculty of Technology

    1997-12-31

    The energy loss of heavy-ion beams (HIB) is studied by means of Vlasov theory and Particle-in-Cell (PIC) simulations in a plasma. The interaction of HIB with a plasma is of central importance for inertial confinement fusion (ICF). A number of studies on the HIB interaction with target plasma have been published. It is important for heavy-ion stopping that the effects of the non-linear interaction of HIB within the Vlasov theory are included. Reported are results of a numerical study of nonlinear effects to the stopping power for HIB in plasma. It is shown that the PIC simulations of collective effects of the stopping power are in a good agreement with the Vlasov theory. (author). 2 tabs., 1 fig., 5 refs.

  20. Surface characterization by energy distribution measurements of secondary electrons and of ion-induced electrons

    International Nuclear Information System (INIS)

    Bauer, H.E.; Seiler, H.

    1988-01-01

    Instruments for surface microanalysis (e.g. scanning electron or ion microprobes, emission electron or ion microscopes) use the current of emitted secondary electrons or of emitted ion-induced electrons for imaging of the analysed surface. These currents, integrating over all energies of the emitted low energy electrons, are however, not well suited to surface analytical purposes. On the contrary, the energy distribution of these electrons is extremely surface-sensitive with respect to shape, size, width, most probable energy, and cut-off energy. The energy distribution measurements were performed with a cylindrical mirror analyser and converted into N(E), if necessary. Presented are energy spectra of electrons released by electrons and argon ions of some contaminated and sputter cleaned metals, the change of the secondary electron energy distribution from oxidized aluminium to clean aluminium, and the change of the cut-off energy due to work function change of oxidized aluminium, and of a silver layer on a platinum sample. The energy distribution of the secondary electrons often shows detailed structures, probably due to low-energy Auger electrons, and is broader than the energy distribution of ion-induced electrons of the same object point. (author)

  1. Molecularly Stretchable Electronics for Energy and Healthcare

    Science.gov (United States)

    Lipomi, Darren

    The term ``plastic electronics'' masks the wide range of mechanical behavior possessed by films of π-conjugated (semiconducting) small molecules and polymers. Such materials are promising for biosensors, large-area displays, low-energy lighting, and low-cost photovoltaic modules. There is also an apparent trade-off between electronic performance and mechanical compliance in films of some of the best-performing semiconducting polymers, which fracture at tensile strains not significantly greater than those at which conventional inorganic semiconductors fail. The design of intrinsically deformable electronic materials-i.e., imagine a semiconducting rubber band-would facilitate roll-to-roll production, mechanical robustness for potable applications, and conformal bonding to curved surfaces. This seminar describes my group's efforts to understand and control the structural parameters that influence the mechanical properties of π-conjugated polymers. The techniques we employ include synthetic chemistry, spectroscopy and microstructural characterization, computation from the molecular to continuum level, and electrical measurements of devices. A complex picture emerges for the interplay between molecular structure, the way the process of solidification influences the morphology, and how molecular structure and morphology combine to produce a film with a given modulus, elastic range, ductility, and toughness. We are also exploring ways to introduce other properties into organic semiconductors that are inspired by biological tissue. That is, not just elasticity and toughness, but also biodegradability and the capacity for self-repair. The seminar will also touch on our use of self-assembled metallic nanoislands on graphene for ultra-sensitive mechanical sensing using piezoresistive and ``piezoplasmonic'' mechanisms. The applications for these materials are in detecting human motion and measuring the mechanics of cardiac and musculoskeletal cells. My group is broadly

  2. Energy transformation in molecular electronic systems

    International Nuclear Information System (INIS)

    Kasha, M.

    1985-01-01

    Our new optical pumping spectroscopy (steady state, and double-laser pulse) allows the production and study of the unstable rare tautomer in its ground and excited states, including picosecond dynamic studies. Molecules under study here included 7-azaindole (model for biological purines), 3-hydroxyflavone (model for plant flavones), lumichrome, and other heterocyclics. New detailed molecular mechanisms for proton transfer are derived, especially with catalytic assisting molecules. A new proton-transfer laser of extraordinary efficiency has become a side dividend, possibly worth of industrial development. The excited and highly reactive singlet molecular oxygen species 1 Δ/sub g/) has proven to be ubiquitous in chemical peroxide systems and in physically excited sensitizer-oxygen systems. Hyperbaric oxygen mechanisms in biology probably involve singlet oxygen. We have undertaken a spectroscopic study of tris - dibenzoylmethane chelates of Al, Gd, Eu, and Yb trivalent ions. These chelates offer a variety of electronic behaviors, from Z-effects on π-electron spin-orbital coupling (Al, Gd) to Weissman intramolecular energy transfer to 4f mestable levels (Eu, Gd). Elegant new spectroscopic resolution at 77K permits separation of tautomeric, parasitic self-absorption, dissociation, and cage effects to be resolved. 18 refs., 4 figs

  3. Electron capture, electron loss, and deexcitation of fast H(2 2S) and H(1 2S) atoms in collisions with molecular hydrogen and inert gases

    International Nuclear Information System (INIS)

    Roussel, F.; Pradel, P.; Spiess, G.

    1977-01-01

    Collisions of ground-state (1 2 S) and metastable (2 2 S) hydrogen atoms with rare gases and molecular hydrogen have been studied in the energy range 0.5--3.0 keV. For an acceptance angle of 55 mrad, the electron loss and the electron-capture cross sections of both H(1 2 S) and H(2 2 S) have been measured and compared with previous experimental values. The deexcitation cross section for H(2 2 S) has been deduced with the help of previously measured total-quenching cross sections for H(2 2 S). The ratio of the electron-capture cross sections for H(2 2 S) relative to H(1 2 S) is found to be very large for argon at low energies. The effects of large-angle scattering and of highly excited states of H are discussed

  4. Electron loss and capture from low-charge-state oxygen projectiles in methane

    International Nuclear Information System (INIS)

    Santos, A C F; Wolff, W; Sant’Anna, M M; Sigaud, G M; DuBois, R D

    2013-01-01

    Absolute cross sections for single- and double-electron loss and single- and multiple-electron capture of 15–1000 keV oxygen projectiles (q = −1, 0, 1, 2) colliding with the methane molecule are presented. The experimental data are used to examine cross-section scaling characteristics for the electron loss of various projectiles. In addition, a modified version of the free-collision model was employed for the calculation of the single- and total-electron-loss cross sections of oxygen projectiles presented in this work. The comparison of the calculated cross sections with the present experimental data shows very good agreement for projectile velocities above 1.0 au. The comparison of the present single-electron-capture cross sections with other projectiles having the same charge shows good agreement, and a common curve can be drawn through the different data sets. (paper)

  5. Absolute photoabsorption oscillator strengths by electron energy loss methods: the valence and S 2p and 2s inner shells of sulphur dioxide in the discrete and continuum regions (3.5-260 eV)

    International Nuclear Information System (INIS)

    Feng, R.; Cooper, G.; Burton, G.R.; Brion, C.E.; Avaldi, L.

    1999-01-01

    Absolute photoabsorption oscillator strengths (cross-sections) for the valence shell discrete and continuum regions of sulphur dioxide from 3.5 to 51 eV have been measured using high resolution (∼0.05 eV FWHM) dipole (e,e) spectroscopy. A wide-range spectrum, covering both the valence shell and the S 2p and 2s inner shells, has also been obtained from 5 to 260 eV at low resolution (∼1 eV FWHM), and this has been used to determine the absolute oscillator strength scale using valence shell TRK (i.e., S(0)) sum-rule normalization. The present measurements have been undertaken in order to investigate the recently discovered significant quantitative errors in our previously published low resolution dipole (e,e) work on sulphur dioxide (Cooper et al., Chem. Phys. 150 (1991) 237; 150 (1991) 251). These earlier measurements were also in poor agreement with other previously published direct photoabsorption measurements. We now report new absolute photoabsorption oscillator strengths using both high and low resolution dipole (e,e) spectroscopies. These new measurements cover a wider energy range and are much more consistent with the previously published direct photoabsorption measurements. The accuracy of our new measurements is confirmed by an S(-2) dipole sum-rule analysis which gives a static dipole polarizability for sulphur dioxide in excellent agreement (within 3.5%) with previously reported polarizability values. Other dipole sums S(u) (u=-1,-3 to -6,-8,-10) and logarithmic dipole sums L(u) (u=-1 to -6) are also determined from the presently reported absolute oscillator strength distributions. (Copyright (c) 1999 Elsevier Science B.V., Amsterdam. All rights reserved.)

  6. Towards hot electron mediated charge exchange in hyperthermal energy ion-surface interactions

    DEFF Research Database (Denmark)

    Ray, M. P.; Lake, R. E.; Thomsen, Lasse Bjørchmar

    2010-01-01

    shows that the primary energy loss mechanism is the atomic displacement of Au atoms in the thin film of the metal–oxide–semiconductor device. We propose that neutral particle detection of the scattered flux from a biased device could be a route to hot electron mediated charge exchange.......We have made Na + and He + ions incident on the surface of solid state tunnel junctions and measured the energy loss due to atomic displacement and electronic excitations. Each tunnel junction consists of an ultrathin film metal–oxide–semiconductor device which can be biased to create a band of hot...

  7. eV-TEM: Transmission electron microscopy in a low energy cathode lens instrument

    Energy Technology Data Exchange (ETDEWEB)

    Geelen, Daniël, E-mail: geelen@physics.leidenuniv.nl [Huygens-Kamerlingh Onnes Laboratory, Leiden Institute of Physics, Leiden University, P.O. Box 9504, 2300 RA Leiden (Netherlands); Thete, Aniket [Huygens-Kamerlingh Onnes Laboratory, Leiden Institute of Physics, Leiden University, P.O. Box 9504, 2300 RA Leiden (Netherlands); Schaff, Oliver; Kaiser, Alexander [SPECS GmbH, Voltastrasse 5, D-13355 Berlin (Germany); Molen, Sense Jan van der [Huygens-Kamerlingh Onnes Laboratory, Leiden Institute of Physics, Leiden University, P.O. Box 9504, 2300 RA Leiden (Netherlands); Tromp, Rudolf [IBM T.J. Watson Research Center, 1101 Kitchawan Road, P.O. Box 218, Yorktown Heights, NY 10598 (United States)

    2015-12-15

    We are developing a transmission electron microscope that operates at extremely low electron energies, 0–40 eV. We call this technique eV-TEM. Its feasibility is based on the fact that at very low electron energies the number of energy loss pathways decreases. Hence, the electron inelastic mean free path increases dramatically. eV-TEM will enable us to study elastic and inelastic interactions of electrons with thin samples. With the recent development of aberration correction in cathode lens instruments, a spatial resolution of a few nm appears within range, even for these very low electron energies. Such resolution will be highly relevant to study biological samples such as proteins and cell membranes. The low electron energies minimize adverse effects due to radiation damage. - Highlights: • We present a new way of performing low energy transmission electron microscopy in an aberration corrected LEEM/PEEM instrument. • We show a proof of principle where we measure transmitted electrons through a suspended graphene monolayer with a preliminary setup. • We present an improved setup design that provides better control of the incident electron beam.

  8. Fundamental harmonic electron cyclotron emission for hot, loss-cone type distributions

    International Nuclear Information System (INIS)

    Bornatici, M.; Ruffina, U.; Westerhof, E.

    1988-01-01

    Electron cyclotron emission (ECE) is an important diagnostic tool for the study of hot plasmas. ECE can be used not only to measure the electron temperature but also to obtain information about non-thermal characteristics of the electron distribution function. One such a nonthermal characteristic is a loss-cone anisotropy. Loss-cone anisotropy can give rise to unstable growth of electro-magnetic waves around the harmonics of the electron cyclotron resonance and to increased emissivity of electron cyclotron waves. In case of high electron temperatures, also the dispersion properties of the extraordinary (X-) mode arond the fundamental electron cyclotron resonance are changed due to loss-cone anisotropy. The consequences of these dispersion properties for the emissivity of the fundamental harmonic X-mode are analyzed for perpendicular propagation. The emissivity, is calculated for two types of distribution functions having a loss-cone anisotropy. These distribution functions are a relativistic Dory-Guest-Harris type distribution function and modified relativistic Maxwellian distribution having a loss-cone with rounded edges (author). 9 refs.; 2 figs

  9. Limits for Recombination in a Low Energy Loss Organic Heterojunction

    KAUST Repository

    Menke, S. Matthew; Sadhanala, Aditya; Nikolka, Mark; Ran, Niva A.; Ravva, Mahesh Kumar; Abdel-Azeim, Safwat; Stern, Hannah L.; Wang, Ming; Sirringhaus, Henning; Nguyen, Thuc-Quyen; Bredas, Jean-Luc; Bazan, Guillermo C.; Friend, Richard H.

    2016-01-01

    Donor-acceptor organic solar cells often show high quantum yields for charge collection, but relatively low open-circuit voltages (VOC) limit power conversion efficiencies to around 12%. We report here the behavior of a system, PIPCP:PC61BM, that exhibits very low electronic disorder (Urbach energy less than 27 meV), very high carrier mobilities in the blend (field-effect mobility for holes >10-2 cm2 V-1 s-1), and a very low driving energy for initial charge separation (50 meV). These characteristics should give excellent performance, and indeed, the VOC is high relative to the donor energy gap. However, we find the overall performance is limited by recombination, with formation of lower-lying triplet excitons on the donor accounting for 90% of the recombination. We find this is a bimolecular process that happens on time scales as short as 100 ps. Thus, although the absence of disorder and the associated high carrier mobility speeds up charge diffusion and extraction at the electrodes, which we measure as early as 1 ns, this also speeds up the recombination channel, giving overall a modest quantum yield of around 60%. We discuss strategies to remove the triplet exciton recombination channel.

  10. Limits for Recombination in a Low Energy Loss Organic Heterojunction

    KAUST Repository

    Menke, S. Matthew

    2016-11-03

    Donor-acceptor organic solar cells often show high quantum yields for charge collection, but relatively low open-circuit voltages (VOC) limit power conversion efficiencies to around 12%. We report here the behavior of a system, PIPCP:PC61BM, that exhibits very low electronic disorder (Urbach energy less than 27 meV), very high carrier mobilities in the blend (field-effect mobility for holes >10-2 cm2 V-1 s-1), and a very low driving energy for initial charge separation (50 meV). These characteristics should give excellent performance, and indeed, the VOC is high relative to the donor energy gap. However, we find the overall performance is limited by recombination, with formation of lower-lying triplet excitons on the donor accounting for 90% of the recombination. We find this is a bimolecular process that happens on time scales as short as 100 ps. Thus, although the absence of disorder and the associated high carrier mobility speeds up charge diffusion and extraction at the electrodes, which we measure as early as 1 ns, this also speeds up the recombination channel, giving overall a modest quantum yield of around 60%. We discuss strategies to remove the triplet exciton recombination channel.

  11. The interaction of low-energy electrons with fructose molecules

    Science.gov (United States)

    Chernyshova, I. V.; Kontrosh, E. E.; Markush, P. P.; Shpenik, O. B.

    2017-11-01

    Using a hypocycloidal electronic spectrometer, the interactions of low energy electrons (0-8.50 eV) with fructose molecules, namely, electron scattering and dissociative attachment, are studied. The results of these studies showed that the fragmentation of fructose molecules occurs effectively even at an electron energy close to zero. In the total electron-scattering cross section by molecules, resonance features (at energies 3.10 and 5.00 eV) were first observed near the formation thresholds of light ion fragments OH- and H-. The correlation of the features observed in the cross sections of electron scattering and dissociative attachment is analyzed.

  12. Equation satisfied by electron-electron mutual Coulomb repulsion energy density functional

    OpenAIRE

    Joubert, Daniel P.

    2011-01-01

    The electron-electron mutual Coulomb repulsion energy density functional satisfies an equation that links functionals and functional derivatives at N-electron and (N-1)-electron densities for densities determined from the same adiabatic scaled external potential for the N-electron system.

  13. Development of a secondary electron energy analyzer for a transmission electron microscope.

    Science.gov (United States)

    Magara, Hideyuki; Tomita, Takeshi; Kondo, Yukihito; Sato, Takafumi; Akase, Zentaro; Shindo, Daisuke

    2018-04-01

    A secondary electron (SE) energy analyzer was developed for a transmission electron microscope. The analyzer comprises a microchannel plate (MCP) for detecting electrons, a coil for collecting SEs emitted from the specimen, a tube for reducing the number of backscattered electrons incident on the MCP, and a retarding mesh for selecting the energy of SEs incident on the MCP. The detection of the SEs associated with charging phenomena around a charged specimen was attempted by performing electron holography and SE spectroscopy using the energy analyzer. The results suggest that it is possible to obtain the energy spectra of SEs using the analyzer and the charging states of a specimen by electron holography simultaneously.

  14. Structural Variations to a Donor Polymer with Low Energy Losses

    KAUST Repository

    Bazan, Guillermo C

    2017-08-01

    Two regioregular narrow band gap conjugated polymers with a D’-A-D-A repeat unit architecture, namely PIFCF and PSFCF, were designed and synthesized. Both polymers contain strictly organized fluorobenzo[c][1,2,5]thiadiazole (FBT) orientations and different solubilizing side chains for solution processing. Compared to the previously reported asymmetric pyridyl-[2,1,3]thiadiazole (PT) based regioregular polymer, namely PIPCP, PIFCF and PSFCF exhibit wider band gaps, tighter π-π stacking, and improved hole mobilities. When incorporated into solar cells with fullerene acceptors, the Eloss = Eg - eVoc values of PIFCF and PSFCF devices are increased compared to solar cells based on PIPCP. Determination of Ect in these solar cells reveals that, relative to PIPCP, PIFCF solar cells lose more energy from Eg - Ect, and PSFCF solar cells lose more energy from both Eg - Ect and Ect - eVoc. The close structural relationship between PIPCP and PIFCF provides an excellent framework to establish molecular features that impact the relationship between Eg and Ect. Theoretical calculations predict that Eloss of PIFCF:PC61BM would be higher than in the case of PIPCP:PC61BM, due to greater Eg - Ect. These findings provide insight into the design of high performance, low voltage loss photovoltaic polymeric materials with desirable optoelectronic properties.

  15. Study and realization of an electron gun at low energy

    International Nuclear Information System (INIS)

    Camus, P.

    1977-01-01

    This work presents the theoretical concepts and experimental design of an electron gun. This gun is working in the weak energy range and the focus position is independant of electron energy measurements and analysis methods of the electron beam are described [fr

  16. Modified electron acoustic field and energy applied to observation data

    Energy Technology Data Exchange (ETDEWEB)

    Abdelwahed, H. G., E-mail: hgomaa-eg@yahoo.com, E-mail: hgomaa-eg@mans.edu.eg [College of Science and Humanitarian Studies, Physics Department, Prince Sattam Bin Abdul Aziz University, Alkharj 11942 (Saudi Arabia); Theoretical Physics Research Group, Physics Department, Faculty of Science, Mansoura University, Mansoura 35516 (Egypt); El-Shewy, E. K. [Theoretical Physics Research Group, Physics Department, Faculty of Science, Mansoura University, Mansoura 35516 (Egypt)

    2016-08-15

    Improved electrostatic acoustic field and energy have been debated in vortex trapped hot electrons and fluid of cold electrons with pressure term plasmas. The perturbed higher-order modified-Korteweg-de Vries equation (PhomKdV) has been worked out. The effect of trapping and electron temperatures on the electro-field and energy properties in auroral plasmas has been inspected.

  17. Photon and electron collimator effects on electron output and abutting segments in energy modulated electron therapy

    International Nuclear Information System (INIS)

    Olofsson, Lennart; Karlsson, Magnus G.; Karlsson, Mikael

    2005-01-01

    In energy modulated electron therapy a large fraction of the segments will be arranged as abutting segments where inhomogeneities in segment matching regions must be kept as small as possible. Furthermore, the output variation between different segments should be minimized and must in all cases be well predicted. For electron therapy with add-on collimators, both the electron MLC (eMLC) and the photon MLC (xMLC) contribute to these effects when an xMLC tracking technique is utilized to reduce the x-ray induced leakage. Two add-on electron collimator geometries have been analyzed using Monte Carlo simulations: One isocentric eMLC geometry with an isocentric clearance of 35 cm and air or helium in the treatment head, and one conventional proximity geometry with a clearance of 5 cm and air in the treatment head. The electron fluence output for 22.5 MeV electrons is not significantly affected by the xMLC if the shielding margins are larger than 2-3 cm. For small field sizes and 9.6 MeV electrons, the isocentric design with helium in the treatment head or shielding margins larger than 3 cm is needed to avoid a reduced electron output. Dose inhomogeneity in the matching region of electron segments is, in general, small when collimator positions are adjusted to account for divergence in the field. The effect of xMLC tracking on the electron output can be made negligible while still obtaining a substantially reduced x-ray leakage contribution. Collimator scattering effects do not interfere significantly when abutting beam techniques are properly applied

  18. A Practical Core Loss Model for Filter Inductors of Power Electronic Converters

    DEFF Research Database (Denmark)

    Matsumori, Hiroaki; Shimizu, Toshihisa; Wang, Xiongfei

    2018-01-01

    This paper proposes a core loss model for filter inductors of power electronic converters. The model allows a computationally efficient analysis on the core loss of the inductor under the square voltage excitation and the premagnetization condition. First, the core loss of the filter inductor under...... buck chopper excitation is evaluated with the proposed model and compared with the conventional methods. The comparison shows that the proposed method results in a better core loss prediction under the premagnetized condition than that of conventional alternatives. Then, the core loss of the filter...... inductor with the pulsewidth modulated inverter excitation is evaluated, which shows that the proposed model not only accurately predicts the core loss but also identifies the hysteresis loss part. These results demonstrate that the approach can further be used for the development of magnetic materials...

  19. Electron loss process and cross section of multiply charged ions by neutral atoms

    International Nuclear Information System (INIS)

    Karashima, S.; Watanabe, T.

    1985-01-01

    The significance of experimental and theoretical results on the electron loss and capture of ions in matter plays an important role in the charge equilibrium problems of fusion plasma physics and of accelerator physics. In the report, we calculate electron stripping cross section by using the binary encounter approximation (BEA). Our treatment of the electron loss process is based on BEA, in which the nucleus of B screened by the surrounding electrons collides with electrons in the ion A sup(q+). The basic approximation in EBA is that the ion interacts with only one electron or nucleus of the target atom at a time. In the calculation for Li sup(2+) + H, we have found that EBA will give approximately reliable results. (Mori, K.)

  20. The Fracture Influence on the Energy Loss of Compressed Air Energy Storage in Hard Rock

    Directory of Open Access Journals (Sweden)

    Hehua Zhu

    2015-01-01

    Full Text Available A coupled nonisothermal gas flow and geomechanical numerical modeling is conducted to study the influence of fractures (joints on the complex thermohydromechanical (THM performance of underground compressed air energy storage (CAES in hard rock caverns. The air-filled chamber is modeled as porous media with high porosity, high permeability, and high thermal conductivity. The present analysis focuses on the CAES in hard rock caverns at relatively shallow depth, that is, ≤100 m, and the pressure in carven is significantly higher than ambient pore pressure. The influence of one discrete crack and multiple crackson energy loss analysis of cavern in hard rock media are carried out. Two conditions are considered during each storage and release cycle, namely, gas injection and production mass being equal and additional gas injection supplemented after each cycle. The influence of the crack location, the crack length, and the crack open width on the energy loss is studied.

  1. A Monte Carlo computer code for evaluating energy loss of 10 keV to 10 MeV ions in amorphous silicon materials

    International Nuclear Information System (INIS)

    Erramli, H.; Elbounagui, O.; Misdaq, M.A.; Merzouki, A.

    2007-01-01

    The basic concepts of a computer simulation code for determining the energy loss of ions in the 10 keV to 10 MeV energy range in amorphous silicon materials were presented and discussed. Data obtained were found in good agreement with those obtained by using a SRIM programme. Electronic and nuclear energy losses were evaluated. Variation of the energy loss as a function of the incident ion energy were studied. This new computer code is a good tool for evaluating stopping powers of various materials for light and heavy ions

  2. Electronic energy distribution function at high electron swarm energies in neon

    International Nuclear Information System (INIS)

    Brown, K.L.; Fletcher, J.

    1995-01-01

    Electron swarms moving through a gas under the influence of an applied electric field have been extensively investigated. Swarms at high energies, as measured by the ratio of the applied field to the gas number density, E/N, which are predominant in many applications have, in general, been neglected. Discharges at E/N in the range 300 0 < 133 Pa using a differentially pumped vacuum system in which the swarm electrons are extracted from the discharge and energy analysed in both a parallel plate retarded potential analyser and a cylindrical electrostatic analyser. Both pre-breakdown and post-breakdown discharges have been studied. Initial results indicate that as the discharge traverses breakdown no sudden change in the nature of the discharge occurs and that the discharge can be described by both a Monte Carlo simulation and by a Boltzmann treatment given by Phelps et al. (1987). 18 refs., 8 figs

  3. A Hall-current model of electron loss after POS opening into high-impedance loads

    International Nuclear Information System (INIS)

    Greenly, J.B.

    1989-01-01

    The author discusses how a self-consistent relativistic model of laminar Hall (E x B) electron flow across a POS plasma allows a loss mechanism after opening even in a strongly magnetically-insulated line, downstream of the remaining POS plasma. Opening is assumed to occur at the cathode, either by erosion or push-back. The loss results only when a large voltage appears after opening into a high impedance load. Then the difference in potential between the plasma, which is near anode potential, and the cathode results in an axial component of E at the load end of the plasma, which supports an E x B drift of electrons across the gap. The analytic model predicts that this loss should increase with higher voltage after opening, and could be eliminated only by removing the plasma from the gap, or eliminating cathode electron emission (both difficult), or by confining this downstream electron flow with an applied magnetic field

  4. Electronic configurations and energies in some thermodynamically correlated laves compounds

    International Nuclear Information System (INIS)

    Campbell, G.M.

    1979-04-01

    The known electronic configurations of simple elements in Laves compounds are correlated with those of the more complex systems to determine their electronic configurations and gaseous state promotion energies

  5. Electron energy-loss spectroscopy of branched gap plasmon resonators

    DEFF Research Database (Denmark)

    Raza, Søren; Esfandyarpour, Majid; Koh, Ai Leen

    2016-01-01

    The miniaturization of integrated optical circuits below the diffraction limit for high-speed manipulation of information is one of the cornerstones in plasmonics research. By coupling to surface plasmons supported on nanostructured metallic surfaces, light can be confined to the nanoscale, enabl...

  6. Daily energy expenditure and physical activity measured in Parkinson's disease patients with and without weight loss

    Science.gov (United States)

    Patients with Parkinson's disease (PD) commonly exhibit weight loss, which investigators attribute to various factors, including elevated resting energy expenditure. We tested the hypothesis that daily energy expenditure (DEE) and its components, resting energy expenditure (REF) and physical activit...

  7. Daily energy expenditure, physical activity, and weight loss in Parkinson's disease patients

    Science.gov (United States)

    Patients with Parkinson's disease (PD) commonly exhibit weight loss (WL) which investigators attribute to various factors, including elevated energy expenditure. We tested the hypothesis that daily energy expenditure (DEE) and its components, resting energy expenditure (REE) and physical activity (P...

  8. Calculation of W for low energy electrons in tissue-equivalent gas. [<10 keV

    Energy Technology Data Exchange (ETDEWEB)

    Dayashankar, [Bhabha Atomic Research Centre, Bombay (India). Div. of Radiation Protection

    1977-11-01

    The mean energy expended per ion pair formed (W-value) in the tissue-equivalent gas for incident electrons of energy up to 10 keV has been calculated in the continuous slowing-down approximation. The effect of secondary and tertiary electrons has been considered by utilizing recent measurements of Opal et al., (1971, J. Chem. Phys., 55,4100) on the energy spectra of low-energy secondary electrons and the Mott formula for the spectra of high-energy secondaries. The results, which are provisional in nature due to the limitations on the accuracy of the input cross-section data and the neglect of the discrete nature of energy loss process, are compared with the available measurements.

  9. Identification of relativistic charged particles by means of ionisation energy loss in proportional counters

    International Nuclear Information System (INIS)

    Bateman, J.E.

    1978-12-01

    A method is described of obtaining a useful degree of improvement in the particle discrimination capability of multiwire proportional counters. The normal multiple sampling technique using a suitable bias to combat the small magnitude of the relativistic rise in the ionization energy loss and the wide pulse height distributions obtained in thin gas counters requires a large number of samples for useful discrimination. In the method reported, this number is reduced by suppressing the delta ray contribution to the total charge pulse from the anode wire. A monte carlo model convoluting the 'delta ray suppressed' data from a one sample detector shows that when it is required to separate pions and electrons at 1 GeV/C with a detection efficiency for the electron of 90%, a 'suppressor' circuit can achieve a pion rejection ratio of 250:1 with 82 samples, whereas the truncated mean approach (lowest 70% of samples) requires 100 samples. (UK)

  10. Energy consumption of audiovisual devices in the residential sector: Economic impact of harmonic losses

    International Nuclear Information System (INIS)

    Santiago, I.; López-Rodríguez, M.A.; Gil-de-Castro, A.; Moreno-Munoz, A.; Luna-Rodríguez, J.J.

    2013-01-01

    In this work, energy losses and the economic consequences of the use of small appliances containing power electronics (PE) in the Spanish residential sector were estimated. Audiovisual devices emit harmonics, originating in the distribution system an increment in wiring losses and a greater demand in the total apparent power. Time Use Surveys (2009–10) conducted by the National Statistical Institute in Spain were used to obtain information about the activities occurring in Spanish homes regarding the use of audiovisual equipment. Moreover, measurements of different types of household appliances available in the PANDA database were also utilized, and the active and non-active annual power demand of these residential-sector devices were determined. Although a single audiovisual device has an almost negligible contribution, the aggregated actions of this type of appliances, whose total annual energy demand is greater than 4000 GWh, can be significant enough to be taken into account in any energy efficiency program. It was proven that a reduction in the total harmonic distortion in the distribution systems ranging from 50% to 5% can reduce energy losses significantly, with economic savings of around several million Euros. - Highlights: • Time Use Survey provides information about Spanish household electricity consumption. • The annual aggregated energy demand of audiovisual appliances is very significant. • TV use accounts for more than 80% of household audiovisual electricity consumption. • A reduction from 50% to 5% in the total harmonic distortion would have economic savings of around several million Euros. • Stricter regulations regarding harmonic emissions must be demanded

  11. X-ray Spectroscopic Characterization of Plasma for a Charged-Particle Energy-Loss Experiment

    Science.gov (United States)

    Hoffman, Nm; Lee, Cl; Wilson, Dc; Barnes, Cris W.; Petrasso, Rd; Li, C.; Hicks, D.

    2000-10-01

    We are pursuing an approach to a charged-particle energy-loss experiment in which charged fusion products from an imploded ICF capsule travel through a well characterized, spatially separate plasma. For this purpose, a fully ionized, uniform, nearly steady-state carbon-hydrogen plasma will be created by laser irradiation of a plastic foil. The temperature and density structure of this plasma must be determined accurately in order to relate observed energy losses to predictions of theory. Various methods for diagnosing the plasma are possible, including Thomson scattering. Alternatively, if a small admixture of higher-Z material such as chlorine is included in the plastic, x-ray spectroscopic techniques will allow the plasma's temperature and density to be determined. Electron temperature is inferred from the ratios of line strengths of various chlorine ion stages, while electron density is determined from the spectra of lithium-like satellite lines near the He beta line of helium-like chlorine. We present results from detailed-configuration accounting (DCA) models of line emission from C+H+Cl plasmas, and estimate the accuracy with which such plasmas can be characterized.

  12. Inelastic collisions of atomic particles at mean energies. Pt.1. Qualitative model of energy losses during a collision

    International Nuclear Information System (INIS)

    Pustovit, A.N.

    2005-01-01

    A new approach is proposed for description of the energy losses of mean-energy atomic particles during their interactions with atomic particles of solids. It is shown that all these interactions are inelastic ones and are determined by different scattering zones with different laws of energy loss dependences [ru

  13. Measurement of the energy loss of heavy ions in laser-produced plasmas

    Energy Technology Data Exchange (ETDEWEB)

    Knobloch-Maas, Renate

    2009-11-25

    The interaction of ions with plasma is not yet fully understood today, although it is important for inertial fusion technology. During recent years, the energy loss of heavy ions in plasma has therefore been a subject of research in the Laser and Plasma Physics group of Darmstadt University of Technology. Several experiments were carried out at the Gesellschaft fuer Schwerionenforschung (GSI) in Darmstadt using laser-created plasma, thereby taking advantage of the unique combination of GSI's accelerator facility and the laser system nhelix, which is also described in this work. The experiments focus on the measurement of the energy loss of medium heavy ions in a plasma created by directly heating a thin carbon foil with the nhelix laser, at an energy of about 50 J. In order to measure the energy loss using a time-of-flight method, a stop detector is used to register the arrival of the ion pulses after passing the plasma and a 12 m drift space. At the beginning of the work on this thesis, the ion detector types formerly used were found to be inadequately suited to the difficult task; this was changed during this thesis. The ion detector has to be able to temporarily resolve ion pulses with a frequency of 108 MHz and a width (FWHM) of 3 ns at a very low current. It also has to withstand the X-ray burst from the plasma with a dead time shorter than the difference between the X-ray and the ion time of flight between the plasma and the detector. In order to satisfy these and other demands, a new diamond detector was designed and has now been used for several measurements. In addition to the new detector, other improvements were made concerning the diagnostics and the laser. The laser-created plasma now reaches a maximum temperature exceeding 200 eV and a free electron density of up to 10{sup 22} cm{sup -3}. With this greatly improved setup, energy loss data could be obtained with a temporal resolution several times better than before, using an ion beam with a

  14. Measurement of the energy loss of heavy ions in laser-produced plasmas

    International Nuclear Information System (INIS)

    Knobloch-Maas, Renate

    2009-01-01

    The interaction of ions with plasma is not yet fully understood today, although it is important for inertial fusion technology. During recent years, the energy loss of heavy ions in plasma has therefore been a subject of research in the Laser and Plasma Physics group of Darmstadt University of Technology. Several experiments were carried out at the Gesellschaft fuer Schwerionenforschung (GSI) in Darmstadt using laser-created plasma, thereby taking advantage of the unique combination of GSI's accelerator facility and the laser system nhelix, which is also described in this work. The experiments focus on the measurement of the energy loss of medium heavy ions in a plasma created by directly heating a thin carbon foil with the nhelix laser, at an energy of about 50 J. In order to measure the energy loss using a time-of-flight method, a stop detector is used to register the arrival of the ion pulses after passing the plasma and a 12 m drift space. At the beginning of the work on this thesis, the ion detector types formerly used were found to be inadequately suited to the difficult task; this was changed during this thesis. The ion detector has to be able to temporarily resolve ion pulses with a frequency of 108 MHz and a width (FWHM) of 3 ns at a very low current. It also has to withstand the X-ray burst from the plasma with a dead time shorter than the difference between the X-ray and the ion time of flight between the plasma and the detector. In order to satisfy these and other demands, a new diamond detector was designed and has now been used for several measurements. In addition to the new detector, other improvements were made concerning the diagnostics and the laser. The laser-created plasma now reaches a maximum temperature exceeding 200 eV and a free electron density of up to 10 22 cm -3 . With this greatly improved setup, energy loss data could be obtained with a temporal resolution several times better than before, using an ion beam with a diameter of only

  15. Energy-loss measurement with the ZEUS Central Tracking Detector

    Energy Technology Data Exchange (ETDEWEB)

    Bartsch, D.

    2007-05-15

    The measurement of the specific energy loss due to ionisation, dE/dx, in a drift chamber is a very important tool for particle identification in final states of reactions between high energetic particles. Such identification requires a well understood dE/dx measurement including a precise knowledge of its uncertainties. Exploiting for the first time the full set of ZEUS data from the HERA operation between 1996 and 2005 twelve detector-related influences affecting the dE/dx measurement of the ZEUS Central Tracking Detector have been identified, separately studied and parameterised. A sophisticated iterative procedure has been developed to correct for these twelve effects, which takes into account the correlations between them. A universal parameterisation of the detector-specific Bethe-Bloch curve valid for all particle species has been extracted. In addition, the various contributions to the measurement uncertainty have been disentangled and determined. This yields the best achievable prediction for the single-track dE/dx resolution. For both the analysis of the measured data and the simulation of detector performance, the detailed understanding of the measurement and resolution of dE/dx gained in this work provides a tool with optimum power for particle identification in a physics studies. (orig.)

  16. Energy-loss measurement with the ZEUS Central Tracking Detector

    International Nuclear Information System (INIS)

    Bartsch, D.

    2007-05-01

    The measurement of the specific energy loss due to ionisation, dE/dx, in a drift chamber is a very important tool for particle identification in final states of reactions between high energetic particles. Such identification requires a well understood dE/dx measurement including a precise knowledge of its uncertainties. Exploiting for the first time the full set of ZEUS data from the HERA operation between 1996 and 2005 twelve detector-related influences affecting the dE/dx measurement of the ZEUS Central Tracking Detector have been identified, separately studied and parameterised. A sophisticated iterative procedure has been developed to correct for these twelve effects, which takes into account the correlations between them. A universal parameterisation of the detector-specific Bethe-Bloch curve valid for all particle species has been extracted. In addition, the various contributions to the measurement uncertainty have been disentangled and determined. This yields the best achievable prediction for the single-track dE/dx resolution. For both the analysis of the measured data and the simulation of detector performance, the detailed understanding of the measurement and resolution of dE/dx gained in this work provides a tool with optimum power for particle identification in a physics studies. (orig.)

  17. Electron polarimetry at low energies in Hall C at JLab

    International Nuclear Information System (INIS)

    Gaskell, D.

    2013-01-01

    Although the majority of Jefferson Lab experiments require multi-GeV electron beams, there have been a few opportunities to make electron beam polarization measurements at rather low energies. This proceedings will discuss some of the practical difficulties encountered in performing electron polarimetry via Mo/ller scattering at energies on the order of a few hundred MeV. Prospects for Compton polarimetry at very low energies will also be discussed. While Mo/ller scattering is likely the preferred method for electron polarimetry at energies below 500 MeV, there are certain aspects of the polarimeter and experiment design that must be carefully considered

  18. Enhanced O2 Loss at Mars Due to an Ambipolar Electric Field from Electron Heating

    Science.gov (United States)

    Ergun, R. E.; Andersson, L. A.; Fowler, C. M.; Woodson, A. K.; Weber, T. D.; Delory, G. T.; Andrews, D. J.; Eriksson, A. I.; Mcenulty, T.; Morooka, M. W.; hide

    2016-01-01

    Recent results from the MAVEN Langmuir Probe and Waves (LPW) instrument suggest higher than predicted electron temperatures (T sub e) in Mars dayside ionosphere above approx. 180 km in altitude. Correspondingly, measurements from Neutral Gas and Ion Mass Spectrometer (NGIMS) indicate significant abundances of O2+ up to approx. 500 km in altitude, suggesting that O2+ may be a principal ion loss mechanism of oxygen. In this article, we investigate the effects of the higher T(sub e) (which results from electron heating) and ion heating on ion outflow and loss. Numerical solutions show that plasma processes including ion heating and higher T(sub e) may greatly increase O2+ loss at Mars. In particular, enhanced T(sub e) in Mars ionosphere just above the exobase creates a substantial ambipolar electric field with a potential (e) of several k(sub b)T(sub e), which draws ions out of the region allowing for enhanced escape. With active solar wind, electron and ion heating, direct O2+ loss could match or exceed loss via dissociative recombination of O2+. These results suggest that direct loss of O2+ may have played a significant role in the loss of oxygen at Mars over time.

  19. Tantalum surface oxidation: Bond relaxation, energy entrapment, and electron polarization

    Energy Technology Data Exchange (ETDEWEB)

    Guo, Yongling [Key Laboratory of Low-Dimensional Materials and Application Technologies (Ministry of Education), Hunan Provincial Key Laboratory of Thin Film Materials and Devices, Faculty of Materials Science and Engineering, Xiangtan University, Hunan 411105 (China); Bo, Maolin [Yangtze Normal University, College of Mechanical and Electrical Engineering, Chongqing 408100 (China); Wang, Yan [School of Information and Electronic Engineering, Hunan University of Science and Technology, Hunan 411201 (China); Liu, Yonghui [Key Laboratory of Low-Dimensional Materials and Application Technologies (Ministry of Education), Hunan Provincial Key Laboratory of Thin Film Materials and Devices, Faculty of Materials Science and Engineering, Xiangtan University, Hunan 411105 (China); Sun, Chang Q. [NOVITAS, School of Electrical and Electronic Engineering, Nanyang Technological University, Singapore 639798 (Singapore); Huang, Yongli, E-mail: huangyongli@xtu.edu.cn [Key Laboratory of Low-Dimensional Materials and Application Technologies (Ministry of Education), Hunan Provincial Key Laboratory of Thin Film Materials and Devices, Faculty of Materials Science and Engineering, Xiangtan University, Hunan 411105 (China)

    2017-02-28

    Graphical abstract: The bond, electron and energy relaxation result in core level energy shift, local densification, quantum entrapment and electron polarization of bonding electrons. - Highlights: • Increasing the oxygen coverage lowers the adsorption energy associated with lattice reconstruction. • Electrons transfer from Ta surface atoms to sp-hydrated oxygen, creating dipole moment that decreases the work function. • Oxygen chemisorption modified valence density-of-state (DOS) for Ta with four excessive DOS features: O−Ta bonding, O{sup 2−} lone pairs, Ta+ electron holes, and the lone-pair polarized Ta dipoles. • The bond, electron and energy relaxation between surface undercoordinated atoms are responsible for core level energy shift, local densification, quantum entrapment and electron polarization of bonding electrons. - Abstract: A combination of photoelectron spectrometric analysis and density functional theory calculations has enabled reconciliation of the bond-energy-electron relaxation for the Ta(100, 110, 111) surfaces chemisorbed with oxygen at different coverages. Results show that increasing oxygen coverage lowers the adsorption energy associated with lattice reconstruction. Valence electrons transfer from Ta surface atoms to oxygen to create four excessive DOS features in terms of O−Ta bonding, lone pairs of oxygen, Ta{sup +} electron holes, and polarized Ta dipoles. Oxidation proceeds in the following dynamics: oxygen gets electrons from two neighboring Ta atoms left behind Ta{sup +}; the sp{sup 3}-orbital hybridization takes place with additional two electron lone pairs, the lone pairs polarize the other two Ta neighbors becoming dipoles. X-ray photoelectron spectral analysis results in the 4f binding energy of an isolated Ta atom and its shift upon bond formation and oxidation. Exercises provide not only a promising numerical approach for the quantitative information about the bond and electronic behavior but also consistent

  20. Tantalum surface oxidation: Bond relaxation, energy entrapment, and electron polarization

    International Nuclear Information System (INIS)

    Guo, Yongling; Bo, Maolin; Wang, Yan; Liu, Yonghui; Sun, Chang Q.; Huang, Yongli

    2017-01-01

    Graphical abstract: The bond, electron and energy relaxation result in core level energy shift, local densification, quantum entrapment and electron polarization of bonding electrons. - Highlights: • Increasing the oxygen coverage lowers the adsorption energy associated with lattice reconstruction. • Electrons transfer from Ta surface atoms to sp-hydrated oxygen, creating dipole moment that decreases the work function. • Oxygen chemisorption modified valence density-of-state (DOS) for Ta with four excessive DOS features: O−Ta bonding, O"2"− lone pairs, Ta+ electron holes, and the lone-pair polarized Ta dipoles. • The bond, electron and energy relaxation between surface undercoordinated atoms are responsible for core level energy shift, local densification, quantum entrapment and electron polarization of bonding electrons. - Abstract: A combination of photoelectron spectrometric analysis and density functional theory calculations has enabled reconciliation of the bond-energy-electron relaxation for the Ta(100, 110, 111) surfaces chemisorbed with oxygen at different coverages. Results show that increasing oxygen coverage lowers the adsorption energy associated with lattice reconstruction. Valence electrons transfer from Ta surface atoms to oxygen to create four excessive DOS features in terms of O−Ta bonding, lone pairs of oxygen, Ta"+ electron holes, and polarized Ta dipoles. Oxidation proceeds in the following dynamics: oxygen gets electrons from two neighboring Ta atoms left behind Ta"+; the sp"3-orbital hybridization takes place with additional two electron lone pairs, the lone pairs polarize the other two Ta neighbors becoming dipoles. X-ray photoelectron spectral analysis results in the 4f binding energy of an isolated Ta atom and its shift upon bond formation and oxidation. Exercises provide not only a promising numerical approach for the quantitative information about the bond and electronic behavior but also consistent insight into the

  1. Time integrated x-ray measurments of the very energetic electron end loss profile in TMX-U

    International Nuclear Information System (INIS)

    Osher, J.E.; Fabyan, J.

    1984-01-01

    The time-integrated 2-D profile of the thick-target bremsstrahlung produced by energetic end loss electrons has been measured during ECRH operation of TMX-U. Sheets of x-ray film and/or arrays of thermoluminescent dosimeters were placed on the outside of the end tank end wall to measure the relative spatial x-ray profile, with locally added filters of Pb to determine the effective mean x-ray energy. The purpose of this simple survey diagnostic was to allow deduction of the gross features of the ECRH region. The electron source functions needed to fit the x-ray data were modeled for various anchor cell radial distributions mapped along magnetic field lines to the elliptical plasma potential control plates or the Al end walls. The data are generally consistent with (1) major ECR heating in the central 25-cm-diam core, (2) a mean ECRH electron loss energy of 420 keV, and (3) an ECRH coupling efficiency to these hot electrons of greater than or equal to 10%

  2. Bipolar energy-loss measurements on cryostable, low-loss conductors

    Energy Technology Data Exchange (ETDEWEB)

    Wollan, J.J.

    1981-01-01

    Losses have been measured on a prototype conductor for the 20 MJ coil for conditions which simulate closely the actual coil field sweep. The data on the prototype II conductor indicates coil losses which exceed the coil specification. The application of certain correction factors reduces the projected losses within the specification for a 2 s reversal but not for a 1 s reversal. Verification of these corrections await measurements on the actual strand and completion of coil construction and testing.

  3. Power electronic converter systems for direct drive renewable energy applications

    DEFF Research Database (Denmark)

    Chen, Zhe

    2013-01-01

    This chapter presents power electronic conversion systems for wind and marine energy generation applications, in particular, direct drive generator energy conversion systems. Various topologies are presented and system design optimization and reliability are briefly discussed....

  4. LAT Perspectives in Detection of High Energy Cosmic Ray Electrons

    International Nuclear Information System (INIS)

    Moiseev, Alexander; Ormes, J.F.; Funk, Stefan

    2007-01-01

    The LAT science objectives and capabilities in the detection of high energy electrons in the energy range from 20 GeV to ∼1.5 TeV are presented. LAT simulations are used to establish the event selections. It is found that maintaining the efficiency of electron detection at the level of 30%, the residual hadron contamination does not exceed 2-3% of the electron flux. It is expected to collect ∼ ten million of electrons with the energy above 20 GeV for one year of observation. Precise spectrum reconstruction with collected electron statistics opens the unique opportunity to investigate several important problems such as models of IC radiation, revealing the signatures of nearby sources such as high energy cutoff in the electron spectrum, testing the propagation model, and search for KKDM particles decay through their contribution to the electron spectrum

  5. Energy loss of argon in a laser-generated carbon plasma.

    Science.gov (United States)

    Frank, A; Blazević, A; Grande, P L; Harres, K; Hessling, T; Hoffmann, D H H; Knobloch-Maas, R; Kuznetsov, P G; Nürnberg, F; Pelka, A; Schaumann, G; Schiwietz, G; Schökel, A; Schollmeier, M; Schumacher, D; Schütrumpf, J; Vatulin, V V; Vinokurov, O A; Roth, M

    2010-02-01

    The experimental data presented in this paper address the energy loss determination for argon at 4 MeV/u projectile energy in laser-generated carbon plasma covering a huge parameter range in density and temperature. Furthermore, a consistent theoretical description of the projectile charge state evolution via a Monte Carlo code is combined with an improved version of the CasP code that allows us to calculate the contributions to the stopping power of bound and free electrons for each projectile charge state. This approach gets rid of any effective charge description of the stopping power. Comparison of experimental data and theoretical results allows us to judge the influence of different plasma parameters.

  6. Investigation of electron-loss and photon scattering correction factors for FAC-IR-300 ionization chamber

    Science.gov (United States)

    Mohammadi, S. M.; Tavakoli-Anbaran, H.; Zeinali, H. Z.

    2017-02-01

    The parallel-plate free-air ionization chamber termed FAC-IR-300 was designed at the Atomic Energy Organization of Iran, AEOI. This chamber is used for low and medium X-ray dosimetry on the primary standard level. In order to evaluate the air-kerma, some correction factors such as electron-loss correction factor (ke) and photon scattering correction factor (ksc) are needed. ke factor corrects the charge loss from the collecting volume and ksc factor corrects the scattering of photons into collecting volume. In this work ke and ksc were estimated by Monte Carlo simulation. These correction factors are calculated for mono-energy photon. As a result of the simulation data, the ke and ksc values for FAC-IR-300 ionization chamber are 1.0704 and 0.9982, respectively.

  7. Investigation of electron-loss and photon scattering correction factors for FAC-IR-300 ionization chamber

    International Nuclear Information System (INIS)

    Mohammadi, S.M.; Tavakoli-Anbaran, H.; Zeinali, H.Z.

    2017-01-01

    The parallel-plate free-air ionization chamber termed FAC-IR-300 was designed at the Atomic Energy Organization of Iran, AEOI. This chamber is used for low and medium X-ray dosimetry on the primary standard level. In order to evaluate the air-kerma, some correction factors such as electron-loss correction factor (k e ) and photon scattering correction factor (k sc ) are needed. k e factor corrects the charge loss from the collecting volume and k sc factor corrects the scattering of photons into collecting volume. In this work k e and k sc were estimated by Monte Carlo simulation. These correction factors are calculated for mono-energy photon. As a result of the simulation data, the k e and k sc values for FAC-IR-300 ionization chamber are 1.0704 and 0.9982, respectively.

  8. Synthesis of Pt nanoparticles and their burrowing into Si due to synergistic effects of ion beam energy losses

    Directory of Open Access Journals (Sweden)

    Pravin Kumar

    2014-10-01

    Full Text Available We report the synthesis of Pt nanoparticles and their burrowing into silicon upon irradiation of a Pt–Si thin film with medium-energy neon ions at constant fluence (1.0 × 1017 ions/cm2. Several values of medium-energy neon ions were chosen in order to vary the ratio of the electronic energy loss to the nuclear energy loss (Se/Sn from 1 to 10. The irradiated films were characterized using Rutherford backscattering spectroscopy (RBS, atomic force microscopy (AFM, scanning electron microscopy (SEM, X-ray diffraction (XRD and high resolution transmission electron microscopy (HRTEM. A TEM image of a cross section of the film irradiated with Se/Sn = 1 shows ≈5 nm Pt NPs were buried up to ≈240 nm into the silicon. No silicide phase was detected in the XRD pattern of the film irradiated at the highest value of Se/Sn. The synergistic effect of the energy losses of the ion beam (molten zones are produced by Se, and sputtering and local defects are produced by Sn leading to the synthesis and burrowing of Pt NPs is evidenced. The Pt NP synthesis mechanism and their burrowing into the silicon is discussed in detail.

  9. Enhanced energy deposition symmetry by hot electron transport

    International Nuclear Information System (INIS)

    Wilson, D.; Mack, J.; Stover, E.; VanHulsteyn, D.; McCall, G.; Hauer, A.

    1981-01-01

    High energy electrons produced by resonance absorption carry the CO 2 laser energy absorbed in a laser fusion pellet. The symmetrization that can be achieved by lateral transport of the hot electrons as they deposit their energy is discussed. A K/sub α/ experiment shows a surprising symmetrization of energy deposition achieved by adding a thin layer of plastic to a copper sphere. Efforts to numerically model this effect are described

  10. Cross sections of electron loss and capture for beams of O{sup +} in water vapor from the energy range of 0,2 to 1,2 MeV; Secoes de choque de perda e captura eletronica para feixes de O{sup +} em vapor de agua em uma faixa de energia entre 0,2 e 1,2 MeV

    Energy Technology Data Exchange (ETDEWEB)

    Oliveira, Vitor Jesus de

    2015-06-01

    The study of the interactions between atoms and molecules is important for the knowledge of the cross sections of the processes that contribute to the deposition of energy by charged particle beams used in radiotherapy planning and transport particle simulation codes. Heavy ions, such as oxygen, induce many cellular and molecular damages in human cells.as a result of interaction between the projectile and atoms and molecules. The use of proton and carbon as the projectile interacting with water molecules is well characterized, however there are few studies with oxygen ions. In this work we are interested in the study of electron loss (projectile ionization) and electron capture with charge state 1+. The Pelletron accelerator of 1.7 MeV from the Federal University of Rio de Janeiro housed in the Atomic and Molecular collisions Laboratory (LACAM) has been used, which can accelerate atomic and molecular ions up to speeds of the order of hundredths of light speed, and consists of the source of negative ions, the Wien filter, the accelerator itself and the magnet load selector. The detection device used to evaluate the processes of interaction (capture and loss) between the beam of the O{sup +} and the water molecule is a Microchannel Plate (MCP) at the position sensitive anode. The collisions of O{sup +} beans are being studied in the range of 0.2 to 1.2 MeV with water vapor (Z = 10). Were obtained the respective absolute cross sections for electron loss and electron capture and compared with the cross sections of the molecule methane (CH4 → Z = 10), the isoelectronic water molecule. The experimental results show an agreement between the measurements with water and methane. Comparisons were made with results of theoretical models for electron loss using the 'Free Collision Model' and for capture the Bohr and Lindhard model. The theoretical results for electron loss show an agreement of experimental data with the model used. The model of Bohr and Lindhard

  11. High-Energy Electron Confinement in a Magnetic Cusp Configuration

    Directory of Open Access Journals (Sweden)

    Jaeyoung Park

    2015-06-01

    Full Text Available We report experimental results validating the concept that plasma confinement is enhanced in a magnetic cusp configuration when β (plasma pressure/magnetic field pressure is of order unity. This enhancement is required for a fusion power reactor based on cusp confinement to be feasible. The magnetic cusp configuration possesses a critical advantage: the plasma is stable to large scale perturbations. However, early work indicated that plasma loss rates in a reactor based on a cusp configuration were too large for net power production. Grad and others theorized that at high β a sharp boundary would form between the plasma and the magnetic field, leading to substantially smaller loss rates. While not able to confirm the details of Grad’s work, the current experiment does validate, for the first time, the conjecture that confinement is substantially improved at high β. This represents critical progress toward an understanding of the plasma dynamics in a high-β cusp system. We hope that these results will stimulate a renewed interest in the cusp configuration as a fusion confinement candidate. In addition, the enhanced high-energy electron confinement resolves a key impediment to progress of the Polywell fusion concept, which combines a high-β cusp configuration with electrostatic fusion for a compact, power-producing nuclear fusion reactor.

  12. Electron emission from materials at low excitation energies

    International Nuclear Information System (INIS)

    Urma, N.; Kijek, M.; Millar, J.J.

    1996-01-01

    Full text: An experimental system has been designed and developed with the purpose of measuring the total electron emission yield from materials at low energy excitation. In the first instance the reliability of the system was checked by measuring the total electron emission yield for a well defined surface (aluminium 99.45%). The obtained data was in the expected range given by the literature, and consequently the system will be used further for measuring the total electron yield for a range of materials with interest in the instrumentation industry. We intend to measure the total electron emission yield under electron bombardment as a function of incident electron energy up to 1200 eV, angle of incidence, state of the surface and environment to which the surface has been exposed. Dependence of emission on total electron irradiated dose is also of interest. For many practical application of the 'Secondary Electron Emission', the total electron yield is desired to be as large as possible. The above phenomenon has practical applicability in electron multiplier tube and Scanning electron microscopy - when by means of the variation of the yield of the emitted electrons one may produce visible images of small sample areas. The electron multiplier tube, is a device which utilises the above effect to detect and amplify both single particles and low currents streams of charged particles. The majority of electron tubes use electrons with low energy, hundreds of eV. Not a lot has been published in the literature about this regime and also about the emission when the impinging electrons have small energy, up to 1 KeV. The information obtained from the experimental measurements concerning the total electron emission yield is used to asses the investigated materials as a potential electron emitting surfaces or dynodes in an electron multiplier tube

  13. Influence of high energy electrons on ECRH in LHD

    Directory of Open Access Journals (Sweden)

    Ogasawara S.

    2012-09-01

    Full Text Available The central bulk electron temperature of more than 20 keV is achieved in LHD as a result of increasing the injection power and the lowering the electron density near 2 × 1018 m−3. Such collision-less regime is important from the aspect of the neoclassical transport and also the potential structure formation. The presences of appreciable amount of high energy electrons are indicated from hard X-ray PHA, and the discrepancy between the stored energy and kinetic energy estimated from Thomson scattering. ECE spectrum are also sensitive to the presence of high energy electrons and discussed by solving the radiation transfer equation. The ECRH power absorption to the bulk and the high energy electrons are dramatically affected by the acceleration and the confinement of high energy electrons. The heating mechanisms and the acceleration process of high energy electrons are discussed by comparing the experimental results and the ray tracing calculation under assumed various density and mean energy of high energy electrons.

  14. ELEC-2005: Electronics in High Energy Physics

    CERN Multimedia

    Monique Duval

    2004-01-01

    ELEC-2005 is a new course series on modern electronics, given by CERN physicists and engineers in the format of the successful ELEC-2002 course series, and within the framework of the 2005 Technical Training Programme. This comprehensive course series is designed for people who are not electronics specialists, for example physicists, engineers and technicians working at or visiting the laboratory, who use or will use electronics in their present or future activities, in particular in the context of the LHC accelerator and experiments. ELEC-2005 will composed of four Terms throughout the year: Winter Term: Introduction to electronics in HEP (January-February, 6 lectures) Spring Term: Integrated circuits and VLSI technology for physics (March, 6 lectures) Summer Term: System electronics for physics: Issues (May, 7 lectures) Winter Term: Electronics applications in HEP experiments (November-December, 10 lectures) Lectures within each Term will take place on Tuesdays and Thursdays, from 10:00 to 12:30. The...

  15. Study of high energy ion loss during hydrogen minority heating in TFTR

    International Nuclear Information System (INIS)

    Park, J.; Zweben, S.J.

    1994-03-01

    High energy ion loss during hydrogen minority ICRF heating is measured and compared with the loss of the D-D fusion products. During H minority heating a relatively large loss of high energy ions is observed at 45 degrees below the outer midplane, with or without simultaneous NBI heating. This increase is most likely due to a loss of the minority tail protons, a possible model for this process is described

  16. Ion energy loss at maximum stopping power in a laser-generated plasma

    International Nuclear Information System (INIS)

    Cayzac, W.

    2013-01-01

    In the frame of this thesis, a new experimental setup for the measurement of the energy loss of carbon ions at maximum stopping power in a hot laser-generated plasma has been developed and successfully tested. In this parameter range where the projectile velocity is of the same order of magnitude as the thermal velocity of the plasma free electrons, large uncertainties of up to 50% are present in the stopping-power description. To date, no experimental data are available to perform a theory benchmarking. Testing the different stopping theories is yet essential for inertial confinement fusion and in particular for the understanding of the alpha-particle heating of the thermonuclear fuel. Here, for the first time, precise measurements were carried out in a reproducible and entirely characterized beam-plasma configuration. It involved a nearly fully-stripped ion beam probing a homogeneous fully-ionized plasma. This plasma was generated by irradiating a thin carbon foil with two high-energy laser beams and features a maximum electron temperature of 200 eV. The plasma conditions were simulated with a two-dimensional radiative hydrodynamic code, while the ion-beam charge-state distribution was predicted by means of a Monte-Carlo code describing the charge-exchange processes of projectile ions in plasma. To probe at maximum stopping power, high-frequency pulsed ion bunches were decelerated to an energy of 0.5 MeV per nucleon. The ion energy loss was determined by a time-of-flight measurement using a specifically developed chemical-vapor-deposition diamond detector that was screened against any plasma radiation. A first experimental campaign was carried out using this newly developed platform, in which a precision better than 200 keV on the energy loss was reached. This allowed, via the knowledge of the plasma and of the beam parameters, to reliably test several stopping theories, either based on perturbation theory or on a nonlinear T-Matrix formalism. A preliminary

  17. Modelling low energy electron and positron tracks in biologically relevant media

    International Nuclear Information System (INIS)

    Blanco, F.; Munoz, A.; Almeida, D.; Ferreira da Silva, F.; Limao-Vieira, P.; Fuss, M.C.; Sanz, A.G.; Garcia, G.

    2013-01-01

    This colloquium describes an approach to incorporate into radiation damage models the effect of low and intermediate energy (0-100 eV) electrons and positrons, slowing down in biologically relevant materials (water and representative biomolecules). The core of the modelling procedure is a C++ computing programme named 'Low Energy Particle Track Simulation (LEPTS)', which is compatible with available general purpose Monte Carlo packages. Input parameters are carefully selected from theoretical and experimental cross section data and energy loss distribution functions. Data sources used for this purpose are reviewed showing examples of electron and positron cross section and energy loss data for interactions with different media of increasing complexity: atoms, molecules, clusters and condense matter. Finally, we show how such a model can be used to develop an effective dosimetric tool at the molecular level (i.e. nanodosimetry). Recent experimental developments to study the fragmentation induced in biologically material by charge transfer from neutrals and negative ions are also included. (authors)

  18. Evaluations of the electron energy distribution in multidipole plasmas

    International Nuclear Information System (INIS)

    Taylor, G.R.; Kessel, M.A.; Sealock, J.W.

    1980-01-01

    In a previous paper a preliminary evaluation of the electron energy distribution in multidipole plasmas was presented. A polynominal regression technique for evaluating the distribution function from Langmuir probe current-voltage characteristics was described. This paper presents an extension of that analysis and the evaluations of the electron energy distributions in multidipole argon and hydrogen plasmas

  19. Cascade-probabilistic function with taking unto account energy losses of ions. Chapter 3

    International Nuclear Information System (INIS)

    1998-01-01

    Mathematical simulation of cascade-probabilistic functions (CPF) for ions with taking into account of energy losses is carried out. Recommendations for CPF calculation on computer are given. Influence of both the interaction number on CPF domain and the interaction depth on CPF domain are determined. Contribution of energy losses into simplest CPF is estimated. Algorithm of radiation defects concentration calculation under ion irradiation with taking into consideration energy losses is cited

  20. Acute visual loss and intraretinal hemorrhages associated to energy drink consumption.

    Science.gov (United States)

    Pagano, Christina W; Wu, Max; Wu, Lihteh

    2017-12-01

    To report the association of acute visual loss secondary to intraretinal hemorrhages and energy drink consumption. Case report and literature review. A 48-year-old hypertensive man developed an elevation in systemic blood pressure, tachycardia, and acute visual loss secondary to intraretinal hemorrhages shortly after drinking several cans of energy drinks. High consumption of energy drinks may lead to intraretinal hemorrhages and acute visual loss.