Linear and cubic dynamic susceptibilities in quantum spin glass
Busiello, G; Sushkova, V G
2001-01-01
The low temperature behaviour of the dynamic nonlinear (cubic) susceptibility chi sub 3 sup ' (omega, T) in quantum d-dimensional Ising spin glass with short-range interactions between spins is investigated in terms of the quantum droplet model and the quantum-mechanical nonlinear response theory is employed. We have revealed a glassy like behaviour of droplet dynamics. The frequency dependence of chi sub 3 sup ' (omega, T) is very remarkable, the temperature dependence is found at very low temperatures (quantum regime). The nonlinear response depends on the tunneling rate for a droplet which regulates the strength of quantum fluctuations. This response has a strong dependence on the distribution of droplet free energies and on the droplet length scale average. Implications for experiments in quantum spin glasses like disordered dipolar quantum Ising magnet LiHo sub x Y sub 1 sub - sub x F sub 4 and pseudospin are noted.
Xu, Chao; Kiselev, Valerij G; Möller, Harald E; Fiebach, Jochen B
2013-04-01
Perfusion measurements using dynamic susceptibility contrast imaging provide additional information about the mean vessel size of microvasculature when supplemented with a dual gradient echo (GE) - spin echo (SE) contrast. Dynamic increase in the corresponding transverse relaxation rate constant changes, ΔR2GE and ΔR2SE , forms a loop on the (Δ R2SE3/2, ΔR2GE ) plane, rather than a reversible line. The shape of the loop and the direction of its passage differentiate between healthy brain and pathological tissue, such as tumour and ischemic tissue. By considering a tree model of microvasculature, the direction of the loop is found to be influenced mainly by the relative arterial and venous blood volume, as well as the tracer bolus dispersion. A parameter Λ is proposed to characterize the direction and shape of the loop, which might be considered as a novel imaging marker for describing the pathology of cerebrovascular network.
Detection of topological states in two-dimensional Dirac systems by the dynamic spin susceptibility
Nakamura, Masaaki; Tokuno, Akiyuki
2016-08-01
We discuss dynamic spin susceptibility (DSS) in two-dimensional (2D) Dirac electrons with spin-orbit interactions to characterize topological insulators. The imaginary part of the DSS appears as an absorption rate in response to a transverse ac magnetic field, just as in an electron spin resonance experiment for localized spin systems. We found that when the system is in a static magnetic field, the topological state can be identified by an anomalous resonant peak of the imaginary part of the DSS as a function of the frequency of the transverse magnetic field ω . In the absence of a static magnetic field, the imaginary part of the DSS becomes a continuous function of ω with a threshold frequency ωc. In this case, the topological and the trivial phases can also be distinguished by the values of ωc and by the line shapes. Thus the DSS is an experimentally observable physical quantity to characterize a topological insulator directly from bulk properties, without observing a topological transition.
DYNAMICAL SPIN SUSCEPTIBILITY IN THE TD-LDA AND QSGW APPROXIMATIONS
Energy Technology Data Exchange (ETDEWEB)
SCHILFGAARDE, MARK VAN; KOTANI, TAKAO
2012-10-15
Abstract. This project was aimed at building the transverse dynamical spin susceptibility with the TD-LDA and the recently-developed Quasparticle Self-Consisent Approximations, which determines an optimum quasiparticle picture in a self-consistent manner within the GW approximation. Our main results were published into two papers, (J. Phys. Cond. Matt. 20, 95214 (2008), and Phys. Rev. B83, 060404(R) (2011). In the first paper we present spin wave dispersions for MnO, NiO, and -MnAs based on quasiparticle self-consistent GW approximation (QSGW). For MnO and NiO, QSGW results are in rather good agreement with experiments, in contrast to the LDA and LDA+U descriptions. For -MnAs, we find a collinear ferromagnetic ground state in QSGW, while this phase is unstable in the LDA. In the second, we apply TD-LDA to the CaFeAs2 the first attempt the first ab initio calculation of dynamical susceptibililty in a system with complex electronic structure Magnetic excitations in the striped phase of CaFe2As2 are studied as a function of local moment amplitude. We find a new kind of excitation: sharp resonances of Stoner-like (itinerant) excitations at energies comparable to the ´eel temperature, originating largely from a narrow band of Fe d states near the Fermi level, and coexisting with more conventional (localized) spin waves. Both kinds of excitations can show multiple branches, highlighting the inadequacy of a description based on a localized spin model.
Directory of Open Access Journals (Sweden)
Yen-Chu Huang
Full Text Available BACKGROUND: The aim of this study was to evaluate whether arterial spin labeling (ASL perfusion magnetic resonance imaging (MRI can reliably quantify perfusion deficit as compared to dynamic susceptibility contrast (DSC perfusion MRI. METHODS: Thirty-nine patients with acute ischemic stroke in the anterior circulation territory were recruited. All underwent ASL and DSC MRI perfusion scans within 30 hours after stroke onset and 31 patients underwent follow-up MRI scans. ASL cerebral blood flow (CBF and DSC time to maximum (T(max maps were used to calculate the perfusion defects. The ASL CBF lesion volume was compared to the DSC Tmax lesion volume by Pearson's correlation coefficient and likewise the ASL CBF and DSC T(max lesion volumes were compared to the final infarct sizes respectively. A repeated measures analysis of variance and least significant difference post hoc test was used to compare the mean lesion volumes among ASL CBF, DSC T(max >4-6 s and final infarct. RESULTS: Mean patient age was 72.6 years. The average time from stroke onset to MRI was 13.9 hours. The ASL lesion volume showed significant correlation with the DSC lesion volume for T(max >4, 5 and 6 s (r = 0.81, 0.82 and 0.80; p5 s (29.2 ml, p6 s (21.8 ml, p5 or 6 s were close to mean final infarct size. CONCLUSION: Quantitative measurement of ASL perfusion is well correlated with DSC perfusion. However, ASL perfusion may overestimate the perfusion defects and therefore further refinement of the true penumbra threshold and improved ASL technique are necessary before applying ASL in therapeutic trials.
Spin susceptibility of disordered gapped graphene systems
Grosu, I.; Biter, T. L.
2017-02-01
We calculate the spin susceptibility for the case of gapped graphene systems in the presence of disorder. The average single-particle density of states in gapped graphene with disorder was calculated, using the Born and the T-matrix approximations. The temperature dependence of the static spin susceptibility was analyzed. The influence of the chemical potential position and disorder is also discussed.
Energy Technology Data Exchange (ETDEWEB)
Goetti, Robert [University Children' s Hospital Zurich, Department of Diagnostic Imaging, Zurich (Switzerland); University Hospital Zurich, Department of Diagnostic and Interventional Radiology, Zurich (Switzerland); O' Gorman, Ruth [University Children' s Hospital Zurich, Center for MR Research, Zurich (Switzerland); Khan, Nadia [University Children' s Hospital Zurich, Moyamoya Center, Division of Neurosurgery, Department of Surgery, Zurich (Switzerland); Kellenberger, Christian J.; Scheer, Ianina [University Children' s Hospital Zurich, Department of Diagnostic Imaging, Zurich (Switzerland)
2013-05-15
This study seeks to evaluate the diagnostic accuracy of cerebral perfusion imaging with arterial spin labelling (ASL) MR imaging in children with moyamoya disease compared to dynamic susceptibility contrast (DSC) imaging. Ten children (7 females; age, 9.2 {+-} 5.4 years) with moyamoya disease underwent cerebral perfusion imaging with ASL and DSC on a 3-T MRI scanner in the same session. Cerebral perfusion images were acquired with ASL (pulsed continuous 3D ASL sequence, 32 axial slices, TR = 5.5 s, TE = 25 ms, FOV = 24 cm, matrix = 128 x 128) and DSC (gradient echo EPI sequence, 35 volumes of 28 axial slices, TR = 2,000 ms, TE = 36 ms, FOV = 24 cm, matrix = 96 x 96, 0.2 ml/kg Gd-DOTA). Cerebral blood flow maps were generated. ASL and DSC images were qualitatively assessed regarding perfusion of left and right ACA, MCA, and PCA territories by two independent readers using a 3-point-Likert scale and quantitative relative cerebral blood flow (rCBF) was calculated. Correlation between ASL and DSC for qualitative and quantitative assessment and the accuracy of ASL for the detection of reduced perfusion per territory with DSC serving as the standard of reference were calculated. With a good interreader agreement ({kappa} = 0.62) qualitative perfusion assessment with ASL and DSC showed a strong and significant correlation ({rho} = 0.77; p < 0.001), as did quantitative rCBF (r = 0.79; p < 0.001). ASL showed a sensitivity, specificity and accuracy of 94 %, 93 %, and 93 % for the detection of reduced perfusion per territory. In children with moyamoya disease, unenhanced ASL enables the detection of reduced perfusion per vascular territory with a good accuracy compared to contrast-enhanced DSC. (orig.)
Dynamic nuclear spin polarization
Energy Technology Data Exchange (ETDEWEB)
Stuhrmann, H.B. [GKSS-Forschungszentrum Geesthacht GmbH (Germany)
1996-11-01
Polarized neutron scattering from dynamic polarized targets has been applied to various hydrogenous materials at different laboratories. In situ structures of macromolecular components have been determined by nuclear spin contrast variation with an unprecedented precision. The experiments of selective nuclear spin depolarisation not only opened a new dimension to structural studies but also revealed phenomena related to propagation of nuclear spin polarization and the interplay of nuclear polarisation with the electronic spin system. The observation of electron spin label dependent nuclear spin polarisation domains by NMR and polarized neutron scattering opens a way to generalize the method of nuclear spin contrast variation and most importantly it avoids precontrasting by specific deuteration. It also likely might tell us more about the mechanism of dynamic nuclear spin polarisation. (author) 4 figs., refs.
White, Carissa M; Pope, Whitney B; Zaw, Taryar; Qiao, Joe; Naeini, Kourosh M; Lai, Albert; Nghiemphu, Phioanh L; Wang, J J; Cloughesy, Timothy F; Ellingson, Benjamin M
2014-01-01
The objective of the current study was to evaluate the regional and voxel-wise correlation between dynamic susceptibility contrast (DSC) and arterial spin labeling (ASL) perfusion magnetic resonance imaging (MRI) measurement of cerebral blood flow (CBF) in patients with brain tumors. Thirty patients with histologically verified brain tumors were evaluated in the current study. DSC-MRI was performed by first using a preload dose of gadolinium contrast, then collecting a dynamic image acquisition during a bolus of contrast, followed by posthoc contrast agent leakage correction. Pseudocontinuous ASL was collected using 30 pairs of tag and control acquisition using a 3-dimensional gradient-echo spin-echo (GRASE) acquisition. All images were registered to a high-resolution anatomical atlas. Average CBF measurements within regions of contrast-enhancement and T2 hyperintensity were evaluated between the two modalities. Additionally, voxel-wise correlation between CBF measurements obtained with DSC and ASL were assessed. Results demonstrated a positive linear correlation between DSC and ASL measurements of CBF when regional average values were compared; however, a statistically significant voxel-wise correlation was only observed in around 30-40% of patients. These results suggest DSC and ASL may provide regionally similar, but spatially different measurements of CBF.
Dynamical theory of spin relaxation
Field, Timothy R.; Bain, Alex D.
2013-02-01
The dynamics of a spin system is usually calculated using the density matrix. However, the usual formulation in terms of the density matrix predicts that the signal will decay to zero, and does not address the issue of individual spin dynamics. Using stochastic calculus, we develop a dynamical theory of spin relaxation, the origins of which lie in the component spin fluctuations. This entails consideration of random pure states for individual protons, and how these pure states are correctly combined when the density matrix is formulated. Both the lattice and the spins are treated quantum mechanically. Such treatment incorporates both the processes of spin-spin and (finite temperature) spin-lattice relaxation. Our results reveal the intimate connections between spin noise and conventional spin relaxation.
Spin dynamics in general relativity
Saravanan, S.
2016-01-01
Since all astrophysical objects spin, it is important to study the dynamics of spinning objects in curved space-time. The dynamics of spinning particles are described with a covariant Hamiltonian formalism. In this formalism, the closed set of equations of motion are obtained from Poisson-Dirac
Energy Technology Data Exchange (ETDEWEB)
Xiao, Hua-Feng [302 Hospital of Chinese People' s Liberation Army, Department of Radiology, Beijing (China); Chen, Zhi-Ye; Wang, Yu-Lin; Wang, Yan; Ma, Lin [People' s Liberation Army General Hospital, Department of Radiology, Beijing (China); Lou, Xin [People' s Liberation Army General Hospital, Department of Radiology, Beijing (China); University of California, Department of Neurology, Los Angeles, CA (United States); Gui, Qiu-Ping [People' s Liberation Army General Hospital, Department of Pathology, Beijing (China); Shi, Kai-Ning; Zhou, Zhen-Yu; Zheng, Dan-Dan [General Electric Healthcare (China) Co., Ltd., Beijing; Wang, Danny J.J. [University of California, Department of Neurology, Los Angeles, CA (United States)
2015-12-15
We hypothesized that three-dimensional pseudocontinuous arterial spin labelling (pCASL) may have similar efficacy in astrocytic tumour grading as dynamic susceptibility contrast-enhanced perfusion-weighted imaging (DSC-PWI), and the grading accuracy may be further improved when combined with apparent diffusion coefficient (ADC) values. Forty-three patients with astrocytic tumours were studied using diffusion weighted imaging (DWI), pCASL, and DSC-PWI. Histograms of ADC and normalized tumour cerebral blood flow values (nCBF on pCASL and nrCBF on DSC-PWI) were measured and analyzed. The mean 10 % ADC value was the DWI parameter that provided the best differentiation between low-grade astrocytoma (LGA) and high-grade astrocytoma (HGA). The nCBF and nrCBF (1.810 ± 0.979 and 2.070 ± 1.048) in LGA were significantly lower than those (4.505 ± 2.270 and 5.922 ± 2.630) in HGA. For differentiation between LGA and HGA, the cutoff values of 0.764 x 10{sup -3} mm{sup 2}/s for mean 10 % ADC, 2.374 for nCBF, and 3.464 for nrCBF provided the optimal accuracy (74.4 %, 86.1 %, and 88.6 %, respectively). Combining the ADC values with nCBF or nrCBF could further improve the grading accuracy to 97.7 % or 95.3 %, respectively. pCASL is an alternative to DSC-PWI for astrocytic tumour grading. The combination of DWI and contrast-free pCASL offers a valuable choice in patients with risk factors. (orig.)
From spin flip excitations to the spin susceptibility enhancement of a two-dimensional electron gas.
Perez, F; Aku-leh, C; Richards, D; Jusserand, B; Smith, L C; Wolverson, D; Karczewski, G
2007-07-13
The g-factor enhancement of the spin-polarized two-dimensional electron gas was measured directly over a wide range of spin polarizations, using spin flip resonant Raman scattering spectroscopy on two-dimensional electron gases embedded in Cd(1-x)Mn(x)Te semimagnetic quantum wells. At zero Raman transferred momentum, the single-particle spin flip excitation, energy Z*, coexists in the Raman spectrum with the spin flip wave of energy Z, the bare giant Zeeman splitting. We compare the measured g-factor enhancement with recent spin-susceptibility enhancement theories and deduce the spin-polarization dependence of the mass renormalization.
Magnetic Nanostructures Spin Dynamics and Spin Transport
Farle, Michael
2013-01-01
Nanomagnetism and spintronics is a rapidly expanding and increasingly important field of research with many applications already on the market and many more to be expected in the near future. This field started in the mid-1980s with the discovery of the GMR effect, recently awarded with the Nobel prize to Albert Fert and Peter Grünberg. The present volume covers the most important and most timely aspects of magnetic heterostructures, including spin torque effects, spin injection, spin transport, spin fluctuations, proximity effects, and electrical control of spin valves. The chapters are written by internationally recognized experts in their respective fields and provide an overview of the latest status.
Yoshitake, Junki; Nasu, Joji; Motome, Yukitoshi
2016-10-01
Experimental identification of quantum spin liquids remains a challenge, as the pristine nature is to be seen in asymptotically low temperatures. We here theoretically show that the precursor of quantum spin liquids appears in the spin dynamics in the paramagnetic state over a wide temperature range. Using the cluster dynamical mean-field theory and the continuous-time quantum Monte Carlo method, which are newly developed in the Majorana fermion representation, we calculate the dynamical spin structure factor, relaxation rate in nuclear magnetic resonance, and magnetic susceptibility for the honeycomb Kitaev model whose ground state is a canonical example of the quantum spin liquid. We find that dynamical spin correlations show peculiar temperature and frequency dependence even below the temperature where static correlations saturate. The results provide the experimentally accessible symptoms of the fluctuating fractionalized spins evincing the quantum spin liquids.
Microscopic studies of nonlocal spin dynamics and spin transport (invited)
Energy Technology Data Exchange (ETDEWEB)
Adur, Rohan; Du, Chunhui; Cardellino, Jeremy; Scozzaro, Nicolas; Wolfe, Christopher S.; Wang, Hailong; Herman, Michael; Bhallamudi, Vidya P.; Pelekhov, Denis V.; Yang, Fengyuan; Hammel, P. Chris, E-mail: hammel@physics.osu.edu [Department of Physics, The Ohio State University, Columbus, Ohio 43210 (United States)
2015-05-07
Understanding the behavior of spins coupling across interfaces in the study of spin current generation and transport is a fundamental challenge that is important for spintronics applications. The transfer of spin angular momentum from a ferromagnet into an adjacent normal material as a consequence of the precession of the magnetization of the ferromagnet is a process known as spin pumping. We find that, in certain circumstances, the insertion of an intervening normal metal can enhance spin pumping between an excited ferromagnetic magnetization and a normal metal layer as a consequence of improved spin conductance matching. We have studied this using inverse spin Hall effect and enhanced damping measurements. Scanned probe magnetic resonance techniques are a complementary tool in this context offering high resolution magnetic resonance imaging, localized spin excitation, and direct measurement of spin lifetimes or damping. Localized magnetic resonance studies of size-dependent spin dynamics in the absence of lithographic confinement in both ferromagnets and paramagnets reveal the close relationship between spin transport and spin lifetime at microscopic length scales. Finally, detection of ferromagnetic resonance of a ferromagnetic film using the photoluminescence of nitrogen vacancy spins in neighboring nanodiamonds demonstrates long-range spin transport between insulating materials, indicating the complexity and generality of spin transport in diverse, spatially separated, material systems.
Microscopic studies of nonlocal spin dynamics and spin transport (invited)
Adur, Rohan; Du, Chunhui; Cardellino, Jeremy; Scozzaro, Nicolas; Wolfe, Christopher S.; Wang, Hailong; Herman, Michael; Bhallamudi, Vidya P.; Pelekhov, Denis V.; Yang, Fengyuan; Hammel, P. Chris
2015-05-01
Understanding the behavior of spins coupling across interfaces in the study of spin current generation and transport is a fundamental challenge that is important for spintronics applications. The transfer of spin angular momentum from a ferromagnet into an adjacent normal material as a consequence of the precession of the magnetization of the ferromagnet is a process known as spin pumping. We find that, in certain circumstances, the insertion of an intervening normal metal can enhance spin pumping between an excited ferromagnetic magnetization and a normal metal layer as a consequence of improved spin conductance matching. We have studied this using inverse spin Hall effect and enhanced damping measurements. Scanned probe magnetic resonance techniques are a complementary tool in this context offering high resolution magnetic resonance imaging, localized spin excitation, and direct measurement of spin lifetimes or damping. Localized magnetic resonance studies of size-dependent spin dynamics in the absence of lithographic confinement in both ferromagnets and paramagnets reveal the close relationship between spin transport and spin lifetime at microscopic length scales. Finally, detection of ferromagnetic resonance of a ferromagnetic film using the photoluminescence of nitrogen vacancy spins in neighboring nanodiamonds demonstrates long-range spin transport between insulating materials, indicating the complexity and generality of spin transport in diverse, spatially separated, material systems.
Spin dynamics simulations at AGS
Energy Technology Data Exchange (ETDEWEB)
Huang, H.; MacKay, W.W.; Meot, F.; Roser, T.
2010-05-23
To preserve proton polarization through acceleration, it is important to have a correct model of the process. It has been known that with the insertion of the two helical partial Siberian snakes in the Alternating Gradient Synchrotron (AGS), the MAD model of AGS can not deal with a field map with offset orbit. The stepwise ray-tracing code Zgoubi provides a tool to represent the real electromagnetic fields in the modeling of the optics and spin dynamics for the AGS. Numerical experiments of resonance crossing, including spin dynamics in presence of the snakes and Q-jump, have been performed in AGS lattice models, using Zgoubi. This contribution reports on various results so obtained.
Billoire, A; Marinari, E
2003-01-01
We investigate the large deviation behaviour of the overlap probability density in the Sherrington-Kirkpatrick (SK) model using the coupled replica scheme, and we compare with the results of a large-scale numerical simulation. In the spin glass phase we show that, generically, for any model with continuous replica symmetry breaking (RSB), 1/N log P sub N (q)approx -A(|q| - q sub E sub A) sup 3 , and we compute the first correction to the expansion of A in powers of T sub c - T for the SK model. We also study the paramagnetic phase, where results are obtained in the replica symmetric scheme that do not involve an expansion in powers of q - q sub E sub A or T sub c - T. Finally we give precise semi-analytical estimates of P(|q| = 1). The overall agreement between the various points of view is very satisfactory.
High-field spin dynamics of antiferromagnetic quantum spin chains
DEFF Research Database (Denmark)
Enderle, M.; Regnault, L.P.; Broholm, C.;
2000-01-01
The characteristic internal order of macroscopic quantum ground states in one-dimensional spin systems is usually not directly accessible, but reflected in the spin dynamics and the field dependence of the magnetic excitations. In high magnetic fields quantum phase transitions are expected. We...... present recent work on the high-field spin dynamics of the S = I antiferromagnetic Heisenberg chains NENP (Haldane ground state) and CsNiCl3 (quasi-1D HAF close to the quantum critical point), the uniform S = 1/2 chain CTS, and the spin-Peierls system CuGeO3. (C) 2000 Elsevier Science B,V. All rights...
Electronic spin susceptibility of metallic superconductive nano-particles
Institute of Scientific and Technical Information of China (English)
Li Feng; Chen Zhi-Qian; Li Qing
2006-01-01
We have observed the thermodynamic properties of metallic superconductive nano-particles in the grand canonical ensemble; and the level distribution and the level correlation between the discrete electronic energy levels are considered in the calculation of the electronic spin susceptibility of the ensemble numerically. The quantum effect, even-odd effect and other special effects existing in the metallic nano-particles are also studied in this article.
Spin anisotropy and slow dynamics in spin glasses.
Bert, F; Dupuis, V; Vincent, E; Hammann, J; Bouchaud, J-P
2004-04-23
We report on an extensive study of the influence of spin anisotropy on spin glass aging dynamics. New temperature cycle experiments allow us to compare quantitatively the memory effect in four Heisenberg spin glasses with various degrees of random anisotropy and one Ising spin glass. The sharpness of the memory effect appears to decrease continuously with the spin anisotropy. Besides, the spin glass coherence length is determined by magnetic field change experiments for the first time in the Ising sample. For three representative samples, from Heisenberg to Ising spin glasses, we can consistently account for both sets of experiments (temperature cycle and magnetic field change) using a single expression for the growth of the coherence length with time.
Nonlinear dynamic susceptibilities of interacting and noninteracting magnetic nanoparticles
Joensson, P; García-Palacios, J L; Svedlindh, P
2000-01-01
The linear and cubic dynamic susceptibilities of solid dispersions of nanosized maghemite gamma-Fe sub 2 O sub 3 particles have been measured for three samples with a volume concentration of magnetic particles ranging from 0.3% to 17%, in order to study the effect of dipole-dipole interactions. Significant differences between the dynamic response of the samples are observed. While the linear and cubic dynamic susceptibilities of the most dilute sample compare reasonably well with the corresponding expressions proposed by Raikher and Stepanov for noninteracting particles, the nonlinear dynamic response of the most concentrated sample exhibits at low temperatures similar features as observed in a Ag(11 at% Mn) spin glass.
Spin Dynamics in Confined Magnetic Structures III
Hillebrands, Burkard
2006-01-01
This third volume of Spin Dynamics in Confined Magnetic Structures addresses central aspects of spin-dynamic phenomena, including recent new developments, on a tutorial level. Researchers will find a comprehensive compilation of the current work in the field. Introductory chapters help newcomers to understand the basic concepts. The more advanced chapters give the current state of the art of spin dynamic issues ranging from the femtosecond to the microsecond regime. This volume concentrates on new experimental techniques such as ferromagnetic-resonance-force microscopy and two-photon photoemission, as well as on aspects of precessional switching, spin-wave excitation, vortex dynamics, spin relaxation, domain-wall dynamics in nanowires and their applications to magnetic logic devices. An important chapter is devoted to the presently very hot subject of the spin-transfer torque, combining the physics of electronic transport and micromagnetics. The comprehensive presentation of these developments makes this volu...
Thermal Spin Dynamics of Yttrium Iron Garnet
Barker, Joseph; Bauer, Gerrit E. W.
2016-11-01
The magnetic insulator yttrium iron garnet can be grown with near perfection and is therefore and ideal conduit for spin currents. It is a complex material with 20 magnetic moments in the unit cell. In spite of being a ferrimagnet, YIG is almost always modeled as a simple ferromagnet with a single spin wave mode. We use the method of atomistic spin dynamics to study the temperature evolution of the full spin wave spectrum, in quantitative agreement with neutron scattering experiments. The antiferromagnetic or optical mode is found to suppress the spin Seebeck effect at room temperature and beyond due to thermally pumped spin currents with opposite polarization to the ferromagnetic mode.
Dynamical spin-spin coupling of quantum dots
Grigoryan, Vahram; Xiao, Jiang; A spintronics Group Team
2014-03-01
We carried out a nested Schrieffer-Wolff transformation of an Anderson two-impurity Hamiltonian to study the spin-spin coupling between two dynamical quantum dots under the influence of rotating transverse magnetic field. As a result of the rotating field, we predict a novel Ising type spin-spin coupling mechanism between quantum dots, whose strength is tunable via the magnitude of the rotating field. Due to its dynamical origin, this new coupling mechanism is qualitatively different from the all existing static couplings such as RKKY, while the strength could be comparable to the strength of the RKKY coupling. The dynamical coupling with the intristic RKKY coupling enables to construct a four level system of maximally entangled Bell states in a controllable manner. This work was supported by the special funds for the Major State Basic Research Project of China (No. 2011CB925601) and the National Natural Science Foundation of China (Grants No. 11004036 and No. 91121002).
Spin dynamics in driven composite multiferroics
Energy Technology Data Exchange (ETDEWEB)
Wang, Zidong, E-mail: Zidong.Wang@auckland.ac.nz; Grimson, Malcolm J. [Department of Physics, The University of Auckland, Auckland 1010 (New Zealand)
2015-09-28
A spin dynamics approach has been used to study the behavior of the magnetic spins and the electric pseudo-spins in a 1-D composite multiferroic chain with a linear magneto-electric coupling at the interface. The response is investigated with either external magnetic or electric fields driving the system. The spin dynamics is based on the Landau-Lifshitz-Gilbert equation. A Gaussian white noise is later added into the dynamic process to include the thermal effects. The interface requires a closer inspection of the magneto-electric effects. Thus, we construct a 2-D ladder model to describe the behavior of the magnetic spins and the electric pseudo-spins with different magneto-electric couplings.
Spin, Isospin and Strong Interaction Dynamics
Directory of Open Access Journals (Sweden)
Comay E.
2011-10-01
Full Text Available The structure of spin and isospin is analyzed. Although both spin and isospin are related to the same SU(2 group, they represent different dynamical effects. The Wigner-Racah algebra is used for providing a description of bound states of several Dirac particles in general and of the proton state in particular. Isospin states of the four ∆ (1232 baryons are discussed. The work explains the small contribution of quarks spin to the overall proton spin (the proton spin crisis. It is also proved that the addition of QCD’s color is not required for a construction of an antisymmetric state for the ∆ ++ (1232 baryon.
Dynamic specific heat of frustrated Ising spin rings
Ismail, G
2003-01-01
The dynamic specific heat C(omega) is calculated exactly for rings of six coupled Ising spins within Glauber dynamics. We used the response of the internal energy to small temperature oscillations to find C(omega). The spin glass (SG) and disordered ferromagnetic (DFM) rings showed here have four energy minima and thus four diverging relaxation times in the time evolution of magnetization and three such times in the evolution of energy. The properties of the real and imaginary parts of dynamic specific heat are investigated for different temperatures and frequencies. The dynamic susceptibility is affected by the longest relaxing mode while the dynamic specific heat is not. Our results confirm that C(omega) is sensitive only to rapidly relaxing processes for ferromagnetic (FM) and anti-ferromagnetic (AFM) cases. (Author)
Coherent spin mixing dynamics in thermal $^{87}$Rb spin-1 and spin-2 gases
He, Xiaodong; Li, Xiaoke; Wang, Fudong; Xu, Zhifang; Wang, Dajun
2015-01-01
We study the non-equilibrium coherent spin mixing dynamics in ferromagnetic spin-1 and antiferromagnetic spin-2 thermal gases of ultracold $^{87}$Rb atoms. Long lasting spin population oscillations with magnetic field dependent resonances are observed in both cases. Our observations are well reproduced by Boltzmann equations of the Wigner distribution function. Compared to the equation of motion of spinor Bose-Einstein condensates, the only difference here is a factor of two increase in the spin-dependent interaction, which is confirmed directly in the spin-2 case by measuring the relation between the oscillation amplitude and the sample's density.
Theoretical model study of dynamic ferromagnetic susceptibility in mono-layer graphene
Sahu, Sivabrata; Parashar, S. K. S.; Rout, G. C.
2016-04-01
We report here a microscopic theoretical study of dynamic ferromagnetic spin susceptibility of electrons for graphene systems, which deal with a tight-binding model Hamiltonian consisting of the hopping of electrons up to third-nearest-neighbors, impurity and substrate effects besides Coulomb interaction of electrons at A-and B- sub- lattices. The spin susceptibility involves four two-particle Green's functions, which are calculated by Zubarev's Green's function technique. The up and down electron occupancies at A and B sub-lattices are computed numerically and self-consistently. The temperature dependent susceptibility shows a pronounced peak at Curie temperature for critical Coulomb interaction Uc = 2.2t1.
Nonergodic dynamics of nuclear spin 1/2 with equal constants of spin-spin interaction
Rudavets, M G
2002-01-01
The exact solution of the nuclear spins polarization evolution in the system with the similar q-constant spin-spin interaction (SSI) between all spin pairs is obtained in the case when only one (the first) spin was polarized at the initial time moment. It is shown that polarization of the first spin P sub 1 (t) has the form of periodical pulsations in the time with the 4 pi/g period. The P sub 1 (t) function changes in each period from the initial value P(0) = 1 up to 1/3 value during the time period of the t approx = 4 pi/Ng order, when the spins number is N >= 1 and remains in the P sub 1 (t) 1/3 state practically during the whole period. The simple classical model within the frames of the average field theory explains the physical cause of the nonergodic dynamics of the considered system
Spin dynamics and spin freezing at ferromagnetic quantum phase transitions
Schmakat, P.; Wagner, M.; Ritz, R.; Bauer, A.; Brando, M.; Deppe, M.; Duncan, W.; Duvinage, C.; Franz, C.; Geibel, C.; Grosche, F. M.; Hirschberger, M.; Hradil, K.; Meven, M.; Neubauer, A.; Schulz, M.; Senyshyn, A.; Süllow, S.; Pedersen, B.; Böni, P.; Pfleiderer, C.
2015-07-01
We report selected experimental results on the spin dynamics and spin freezing at ferromagnetic quantum phase transitions to illustrate some of the most prominent escape routes by which ferromagnetic quantum criticality is avoided in real materials. In the transition metal Heusler compound Fe2TiSn we observe evidence for incipient ferromagnetic quantum criticality. High pressure studies in MnSi reveal empirical evidence for a topological non-Fermi liquid state without quantum criticality. Single crystals of the hexagonal Laves phase compound Nb1- y Fe2+ y provide evidence of a ferromagnetic to spin density wave transition as a function of slight compositional changes. Last but not least, neutron depolarisation imaging in CePd1- x Rh x underscore evidence taken from the bulk properties of the formation of a Kondo cluster glass.
Decoherence dynamics of a single spin versus spin ensemble
Dobrovitski, V.V.; Feiguin, A.E.; Awschalom, D.D.; Hanson, R.
2008-01-01
We study decoherence of central spins by a spin bath, focusing on the difference between measurement of a single central spin and measurement of a large number of central spins (as found in typical spin-resonance experiments). For a dilute spin bath, the single spin demonstrates Gaussian free-induct
Decoherence dynamics of a single spin versus spin ensemble
Dobrovitski, V.V.; Feiguin, A.E.; Awschalom, D.D.; Hanson, R.
2008-01-01
We study decoherence of central spins by a spin bath, focusing on the difference between measurement of a single central spin and measurement of a large number of central spins (as found in typical spin-resonance experiments). For a dilute spin bath, the single spin demonstrates Gaussian
Spin dynamics in geometrically frustrated antiferromagnetic pyrochlores
Gardner, J. S.; Ehlers, G.; Bramwell, S. T.; Gaulin, B. D.
2004-03-01
We have studied the spin dynamics of several antiferromagnetic pyrochlore oxides. These magnets are geometrically frustrated and only reach their ground states at temperatures much lower than that expected from mean field theory. Here we present data on the magnetic nature, especially the spin dynamics of Tb2Ti2O7, Gd2Ti2O7 and Y2Mo2O7. In these systems the ground states are found to be very different. Y2Mo2O7 freezes completely into a spin glass-like state, Tb2Ti2O7 is a cooperative paramagnetic and remains dynamic down to 15 mK and Gd2Ti2O7 enters a unique partially ordered state at {\\sim }1 K.
Use of piloted simulation for studies of fighter departure/spin susceptibility
Gilbert, W. P.; Nguyen, L. T.
1978-01-01
The NASA-Langley Research Center has incorporated into its stall/spin research program on military airplanes the use of piloted, fixed-base simulation to complement the existing matrix of unique research testing techniques. The piloted simulations of fighter stall/departure flight dynamics are conducted on the Langley Differential Maneuvering Simulator (DMS). The objectives of the simulation research are reviewed. The rationale underlying the simulation methods and procedures used in the evaluation of airplane characteristics is presented. The evaluation steps used to assess fighter stall/departure characteristics are discussed. Simulation results are presented to illustrate the flight dynamics phenomena dealt with. The considerable experience accumulated in the conduct of piloted stall/departure simulation indicates that simulation provides a realistic evaluation of an airplane's maneuverability at high angles of attack and an assessment of the departure and spin susceptibility of the airplane. This realism is obtained by providing the pilot a complete simulation of the airplane and control system which can be flown using a realistic cockpit and visual display in simulations of demanding air combat maneuvering tasks. The use of the piloted simulation methods and procedures described were found very effective in identifying stability and control problem areas and in developing automatic control concepts to alleviate many of these problems. A good level of correlation between simulated flight dynamics and flight test results were obtained over the many fighter configurations studied in the simulator.
Dynamics of the classical planar spin chain
Raedt, Bart De; Raedt, Hans De
1978-01-01
In this paper we pay attention to the classical one-dimensional planar spin system and, in particular, to the dynamics of such a model. We use the Monte Carlo method to calculate the static correlation functions, needed to determine the relaxation functions completely. We are then able to give the r
Controlled spatial separation of spins and coherent dynamics in spin-orbit-coupled nanostructures
Lo, Shun-Tsung; Chen, Chin-Hung; Fan, Ju-Chun; Smith, L. W.; Creeth, G. L.; Chang, Che-Wei; Pepper, M.; Griffiths, J. P.; Farrer, I.; Beere, H. E.; Jones, G. A. C.; Ritchie, D. A.; Chen, Tse-Ming
2017-07-01
The spatial separation of electron spins followed by the control of their individual spin dynamics has recently emerged as an essential ingredient in many proposals for spin-based technologies because it would enable both of the two spin species to be simultaneously utilized, distinct from most of the current spintronic studies and technologies wherein only one spin species could be handled at a time. Here we demonstrate that the spatial spin splitting of a coherent beam of electrons can be achieved and controlled using the interplay between an external magnetic field and Rashba spin-orbit interaction in semiconductor nanostructures. The technique of transverse magnetic focusing is used to detect this spin separation. More notably, our ability to engineer the spin-orbit interactions enables us to simultaneously manipulate and probe the coherent spin dynamics of both spin species and hence their correlation, which could open a route towards spintronics and spin-based quantum information processing.
Spin dynamics of bilayer manganites
Indian Academy of Sciences (India)
Tapan Chatterji
2004-07-01
The results of inelastic and quasi-elastic neutron scattering investigations on the 40% hole-doped quasi-2D bilayer manganites La1.2Sr1.8Mn2O7 have been reviewed. The complete set of exchange interactions have been determined on the basis of a localized Heisenberg model. However, the spin wave dispersion in La1.2Sr1.8Mn2O7 shows softening close to the zone boundary and are also heavily damped especially close to the zone boundary and deviate from that expected for a simple Heisenberg model. A minimal double exchange model including quantum corrections can reproduce these effects qualitatively but falls short of quantitative agreement.
Spin dynamics and spin freezing in the triangular lattice antiferromagnets FeGa2S4 and NiGa2S4
Zhao, Songrui; Dalmas de Réotier, P.; Yaouanc, A.; MacLaughlin, D. E.; Mackie, J. M.; Bernal, O. O.; Nambu, Y.; Higo, T.; Nakatsuji, S.
2012-08-01
Magnetic susceptibility and muon spin relaxation (μSR) experiments have been carried out on the quasi-2D triangular-lattice spin S=2 antiferromagnet FeGa2S4. The μSR data indicate a sharp onset of a frozen or nearly frozen spin state at T*=31(2) K, twice the spin-glass-like freezing temperature Tf=16(1) K. The susceptibility becomes field dependent below T*, but no sharp anomaly is observed in any bulk property. A similar transition is observed in μSR data from the spin-1 isomorph NiGa2S4. In both compounds the dynamic muon spin relaxation rate λd(T) above T* agrees well with a calculation of spin-lattice relaxation by Chubukov, Sachdev, and Senthil in the renormalized classical regime of a 2D frustrated quantum antiferromagnet. There is no firm evidence for other mechanisms. At low temperatures, λd(T) becomes temperature independent in both compounds, indicating persistence of spin dynamics. Scaling of λd(T) between the two compounds is observed from ˜Tf to ˜1.5T*. Although the μSR data by themselves cannot exclude a truly static spin component below T*, together with the susceptibility data they are consistent with a slowly fluctuating “spin gel” regime between Tf and T*. Such a regime and the absence of a divergence in λd(T) at T* are features of two unconventional mechanisms: (1) binding/unbinding of Z2 vortex excitations, and (2) impurity spins in a nonmagnetic spin-nematic ground state. The absence of a sharp anomaly or history dependence at T* in the susceptibility of FeGa2S4, and the weakness of such phenomena in NiGa2S4, strongly suggest transitions to low-temperature phases with unconventional dynamics.
Structurally dynamic spin market networks
Horváth, D
2007-01-01
The agent-based model of price dynamics on a directed evolving complex network is suggested and studied by direct simulation. The resulting stationary regime is maintained as a result of the balance between the extremal dynamics, adaptivity of strategic variables and reconnection rules. For some properly selected parametric combination the network displays small-world phenomenon with high mean clustering coefficient and power-law node degree distribution. The mechanism of repeated random walk through network combined with a fitness recognition is proposed and tested to generate modular multi-leader market. The simulations suggest that dynamics of fitness is the slowest process that manifests itself in the volatility clustering of the log-price returns.
Structurally Dynamic Spin Market Networks
Horváth, Denis; Kuscsik, Zoltán
The agent-based model of stock price dynamics on a directed evolving complex network is suggested and studied by direct simulation. The stationary regime is maintained as a result of the balance between the extremal dynamics, adaptivity of strategic variables and reconnection rules. The inherent structure of node agent "brain" is modeled by a recursive neural network with local and global inputs and feedback connections. For specific parametric combination the complex network displays small-world phenomenon combined with scale-free behavior. The identification of a local leader (network hub, agent whose strategies are frequently adapted by its neighbors) is carried out by repeated random walk process through network. The simulations show empirically relevant dynamics of price returns and volatility clustering. The additional emerging aspects of stylized market statistics are Zipfian distributions of fitness.
Spin Dynamics of Electrons Confined in Silicon Heterostructures
Jock, Ryan Michael
The spin states of electrons confined in silicon heterostructures have shown promise as qubits for quantum information processing. Recently, a host of single and few electron silicon quantum dot device architectures have arisen as implementations for quantum computation. These devices often combine regions of low density two-dimensional (2D) electrons, localized electrons, and interfaces depleted of electrons. Electron spin resonance (ESR) is a unique tool for probing the spin dynamics of both mobile and localized electrons at silicon heterointerfaces and investigating the effects limiting the ability to control electrons and their spin states in these structures. We use a continuous wave ESR method to examine localized 2D electron band-tail states at Si/SiO 2 interfaces in large area metal-oxide-semiconductor transistors. We compare two devices, fabricated in different laboratories, which display similar low temperature (4.2 K) peak mobilities. We find that one of the devices displays a smaller band-tail density of confined states and a shallower characteristic confinement. Thus, ESR reveals a difference in device quality, which is not apparent from mobility measurements, and is a valuable tool for evaluating the interface quality in Si/SiO2 heterostructures. Additionally, we use pulsed ESR techniques to study the spin dynamics of electrons confined in Si/SiGe heterostructures. For mobile 2D electrons, the density-dependent Dyakonov-Perel mechanism dominates spin relaxation. At low 2D densities, stronger electron-electron interactions cause an increase in the electron effective mass, leading to an increase in spin susceptibility. For very low densities, natural disorder localizes electrons at the silicon heterointerface. Naturally localized electrons in these structures display short spin relaxation times (ensembles of around 108 quantum dots in Si/SiGe heterostructures. By tailoring the device structure, a long electron spin relaxation time (T1 = 1.4 ms) is
Coherent spin dynamics in semiconductor quantum dots
Energy Technology Data Exchange (ETDEWEB)
Amand, T.; Senes, M.; Marie, X.; Renucci, P. [Laboratoire de Nanophysique, Magnetisme et Optoelectronique-LPMC, INSA, 135 avenue de Rangueil, 31077 Toulouse cedex 4 (France); Urbaszek, B. [Laboratoire de Nanophysique, Magnetisme et Optoelectronique-LPMC, INSA, 135 avenue de Rangueil, 31077 Toulouse cedex 4 (France); Department of Physics, Heriot-Watt University, Edinburgh EH14 4AS (United Kingdom); Krebs, O.; Laurent, S.; Voisin, P. [Laboratoire de Photonique et Nanostructures, route de Nozay, 91460 Marcoussis (France); Warburton, R.J. [Department of Physics, Heriot-Watt University, Edinburgh EH14 4AS (United Kingdom)
2005-05-01
The anisotropic exchange interaction (AEI) between electrons and holes is shown to play a central role in quantum dots (QDs) spin dynamics. In neutral QDs, AEI is at the origin of spin quantum beats observed under resonant excitation between the lowest energy doublet of linearly dipole-active eigenstates. In negatively charged QDs, AEI is at the origin of QD emission with opposite helicity to the optic al excitation, under non-resonant excitation conditions. Finally, the possibility of leaving a spin information in the system after recombination of the photo-injected electron-hole pair is discussed with respect to the type and the level of the doping. (copyright 2005 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)
Dynamic Feedback in Ferromagnet-Spin Hall Metal Heterostructures
Cheng, Ran; Zhu, Jian-Gang; Xiao, Di
2016-08-01
In ferromagnet-normal-metal heterostructures, spin pumping and spin-transfer torques are two reciprocal processes that occur concomitantly. Their interplay introduces a dynamic feedback effect interconnecting energy dissipation channels of both magnetization and current. By solving the spin diffusion process in the presence of the spin Hall effect in the normal metal, we show that the dynamic feedback gives rise to (i) a nonlinear magnetic damping that is crucial to sustain uniform steady-state oscillations of a spin Hall oscillator at large angles and (ii) a frequency-dependent spin Hall magnetoimpedance that reduces to the spin Hall magnetoresistance in the dc limit.
Combined molecular dynamics-spin dynamics simulations of bcc iron
Energy Technology Data Exchange (ETDEWEB)
Perera, Meewanage Dilina N [ORNL; Yin, Junqi [ORNL; Landau, David P [University of Georgia, Athens, GA; Nicholson, Don M [ORNL; Stocks, George Malcolm [ORNL; Eisenbach, Markus [ORNL; Brown, Greg [ORNL
2014-01-01
Using a classical model that treats translational and spin degrees of freedom on an equal footing, we study phonon-magnon interactions in BCC iron with combined molecular and spin dynamics methods. The atomic interactions are modeled via an empirical many-body potential while spin dependent interactions are established through a Hamiltonian of the Heisenberg form with a distance dependent magnetic exchange interaction obtained from first principles electronic structure calculations. The temporal evolution of translational and spin degrees of freedom was determined by numerically solving the coupled equations of motion, using an algorithm based on the second order Suzuki-Trotter decomposition of the exponential operators. By calculating Fourier transforms of space- and time-displaced correlation functions, we demonstrate that the the presence of lattice vibrations leads to noticeable softening and damping of spin wave modes. As a result of the interplay between lattice and spin subsystems, we also observe additional longitudinal spin wave excitations, with frequencies which coincide with that of the longitudinal lattice vibrations.
NMR probe for dynamic-angle spinning
Mueller, K. T.; Chingas, G. C.; Pines, A.
1991-06-01
We describe the design of a probe for dynamic-angle spinning (DAS) NMR experiments, comprised of a spinning cylindrical sample holder whose axis may be reoriented rapidly between discrete directions within the bore of a superconducting magnet. This allows the refocusing of nuclear spin magnetization that evolves under anisotropic interactions such as chemical shift anisotropy and quadrupolar coupling, providing high resolution NMR spectra for quadrupolar nuclei in solid materials. The probe includes an axial air delivery system to bearing and drive jets which support and spin a rotor containing the sample. Axis reorientation is accomplished with a pulley attached to the probehead and coupled to a stepping motor outside of the magnet. The choice of motor and gear ratio is based on an analysis of the moments of inertia of the motor and load, the desired angular resolution, and simplicity of design. Control of angular accuracy and precision are discussed, as well as the efficiency of radiofrequency irradiation and detection. High resolution DAS spectra of oxygen-17 and aluminum-27 nuclei in polycrystalline minerals illustrate the experimental capabilities.
Quantification of entanglement from magnetic susceptibility for a Heisenberg spin 1/2 system
Energy Technology Data Exchange (ETDEWEB)
Chakraborty, Tanmoy; Singh, Harkirat; Das, Diptaranjan; Sen, Tamal K. [Indian Institute of Science Education and Research (IISER) Kolkata, Mohanpur Campus, PO BCKV Campus Main Office, Mohanpur – 741252, Nadia, West Bengal (India); Mitra, Chiranjib, E-mail: chiranjib@iiserkol.ac.in [Indian Institute of Science Education and Research (IISER) Kolkata, Mohanpur Campus, PO BCKV Campus Main Office, Mohanpur – 741252, Nadia, West Bengal (India)
2012-10-01
We report temperature and magnetic field dependent magnetization and quantification of entanglement from the experimental data for dichloro (thiazole) copper (II), a Heisenberg spin chain system. The plot of magnetic susceptibility vs. temperature indicates an infinite spin chain. Isothermal magnetization measurements (as functions of magnetic field) were performed at various temperatures below the antiferromagnetic (AFM) ordering, where the AFM correlations persist significantly. These magnetization curves are fitted to the Bonner–Fisher model. Magnetic susceptibility is used as an entanglement witness to quantify the amount of entanglement in the system. -- Highlights: ► Magnetic properties of a Heisenberg spin chain system are studied. ► Experimental data is fitted to theoretical models. ► Magnetic susceptibility is used as a macroscopic witness of entanglement. ► Entanglement is extracted from experimental data.
Dynamics of Spin-2 Bose-Einstein Condensates
Institute of Scientific and Technical Information of China (English)
无
2007-01-01
We numerically simulate the dynamics of a spin-2 Bose-Einstein condensate. We find that the initial phase plays an important role in the spin component oscillations. The spin mixing processes can fully cancel out due to quantum interference when taking some initial special phase. In all the spin mixing processes, the total spin is conversed.When the initial population is mainly occupied by a component with the maximal or minimal magnetic quantum number,the oscillations of spin components cannot happen due to the total spin conversation. The presence of quadratic Zeeman energy terms suppresses some spin mixing processes so that the oscillations of spin components are suppressed in some initial spin configuration. However, the linear Zecman energy terms have no effects on the spin mixing processes.
Dynamical picture of spin Hall effect based on quantum spin vorticity theory
Directory of Open Access Journals (Sweden)
Masahiro Fukuda
2016-02-01
Full Text Available It is proposed that the dynamical picture of the spin Hall effect can be explained as the generation of the spin vorticity by the applied electric field on the basis of the “quantum spin vorticity theory”, which describes the equation of motion of local spin and the vorticity of spin in the framework of quantum field theory. Similarly, it is proposed that the dynamical picture of the inverse spin Hall effect can be explained as the acceleration of the electron by the rotation of the spin torque density as driving force accompanying the generation of the spin vorticity. These explanations may help us to understand spin phenomena in condensed matter and molecular systems from a unified viewpoint.
Competition between Bose-Einstein Condensation and Spin Dynamics.
Naylor, B; Brewczyk, M; Gajda, M; Gorceix, O; Maréchal, E; Vernac, L; Laburthe-Tolra, B
2016-10-28
We study the impact of spin-exchange collisions on the dynamics of Bose-Einstein condensation by rapidly cooling a chromium multicomponent Bose gas. Despite relatively strong spin-dependent interactions, the critical temperature for Bose-Einstein condensation is reached before the spin degrees of freedom fully thermalize. The increase in density due to Bose-Einstein condensation then triggers spin dynamics, hampering the formation of condensates in spin-excited states. Small metastable spinor condensates are, nevertheless, produced, and they manifest in strong spin fluctuations.
Spin dynamics in a two-dimensional quantum gas
DEFF Research Database (Denmark)
Pedersen, Poul Lindholm; Gajdacz, Miroslav; Deuretzbacher, Frank
2014-01-01
We have investigated spin dynamics in a two-dimensional quantum gas. Through spin-changing collisions, two clouds with opposite spin orientations are spontaneously created in a Bose-Einstein condensate. After ballistic expansion, both clouds acquire ring-shaped density distributions with superimp......We have investigated spin dynamics in a two-dimensional quantum gas. Through spin-changing collisions, two clouds with opposite spin orientations are spontaneously created in a Bose-Einstein condensate. After ballistic expansion, both clouds acquire ring-shaped density distributions...
Spin dynamics in the anisotropic spin glass Fe2TiO5
DEFF Research Database (Denmark)
Yeshurun, Y.; Tholence, J. L.; Kjems, Jørgen;
1985-01-01
We have studied spin-freezing phenomena along the magnetic easy axis of the insulating spin glass Fe2TiOS by magnetisation, AC susceptibility and neutron scattering experiments. The characteristic measurement time for these techniques varies over more than fourteen orders of magnitude. The results...
Doping Induced Spin State Transition in LaCoO3: Dynamical Mean-Field Study
Augustinský, P.; Křápek, V.; Kuneš, J.
2013-06-01
Hole and electron doped LaCoO3 is studied using dynamical mean-field theory. The one-particle spectra are analyzed and compared to the available experimental data, in particular the x-ray absorption spectra. Analyzing the temporal spin-spin correlation functions we find the atomic intermediate spin state is not important for the observed Curie-Weiss susceptibility. Contrary to the commonly held view about the roles played by the t2g and eg electrons we find narrow quasiparticle bands of t2g character crossing the Fermi level accompanied by strongly damped eg excitations.
Susceptibility of the 2D spin-1 / 2 Heisenberg antiferromagnet with an impurity.
Höglund, Kaj H; Sandvik, Anders W
2003-08-15
We use a quantum Monte Carlo method (stochastic series expansion) to study the effects of a magnetic or nonmagnetic impurity on the magnetic susceptibility of the two-dimensional Heisenberg antiferromagnet. At low temperatures, we find a log-divergent contribution to the transverse susceptibility. We also introduce an effective few-spin model that can quantitatively capture the differences between magnetic and nonmagnetic impurities at high and intermediate temperatures.
Law, J M; Benner, H; Kremer, R K
2013-02-13
The temperature dependence of the spin susceptibilities of S = 1, 3/2, 2, 5/2 and 7/2 Heisenberg antiferromagnetic 1D spins chains with nearest-neighbor coupling was simulated via quantum Monte Carlo calculations, within the reduced temperature range of 0.005 ≤ T* ≤ 100, and fitted to a Padé approximation with deviations between the simulated and fitted data of the same order of magnitude as or smaller than the quantum Monte Carlo simulation error. To demonstrate the practicality of our theoretical findings, we compare these results with the susceptibility of the well known 1D chain compound TMMC ([(CH(3))(4)N[MnCl(3)
Glassy Spin Dynamics in Geometrically Frustrated Buckled Colloidal Crystals
Zhou, Di; Wang, Feng; Li, Bo; Lou, Xiaojie; Han, Yilong
2017-04-01
Geometrical frustration arises when the lattice geometry prevents local interaction energies from minimizing simultaneously. Whether and how geometrically frustrated spins or charges in clean crystals exhibit glassy dynamics remain elusive due to the lack of measurements on microscopic dynamics. Here, we employ buckled monolayer colloidal crystals to mimic frustrated antiferromagnetic Ising spins on triangular lattices and measure single-spin dynamics using video microscopy. Both attractive and repulsive colloidal crystals buckled into zigzag stripes with glassy dynamics at low effective temperatures in experiment and simulation. The simple local spin configurations enable uncovering correlations among structure, dynamics, and soft vibrational modes. Machine learning analysis further reveals facilitated dynamics to be an important mechanism of structural relaxation. Moreover, our simulation reveals a similar structure and dynamics in lattice Coulomb liquids. Hence, spin-lattice coupling and long-range interaction can similarly lift degeneracy, induce a rugged landscape, and, thus, produce glassy dynamics.
Wheeler-Feynman dynamics of spin-1/2 particles
Energy Technology Data Exchange (ETDEWEB)
Van Alstine, P.; Crater, H.W.
1986-02-15
By combining a supersymmetric description of a spinning particle in an external field with an appropriate modification of the ''adjunct field'' of Wheeler and Feynman, we construct a many-time relativistic dynamics for arbitrary numbers of spin-(1/2) and spinless particles in mutual scalar or vector interaction. Quantization of the slow-motion approximation to the dynamics of two spinning particles reproduces the corresponding field-theoretic (Bethe-Salpeter) dynamics through order U.
Wheeler-Feynman dynamics of spin-1/2 particles
van Alstine, Peter; Crater, Horace W.
1986-02-01
By combining a supersymmetric description of a spinning particle in an external field with an appropriate modification of the ``adjunct field'' of Wheeler and Feynman, we construct a many-time relativistic dynamics for arbitrary numbers of spin-(1/2) and spinless particles in mutual scalar or vector interaction. Quantization of the slow-motion approximation to the dynamics of two spinning particles reproduces the corresponding field-theoretic (Bethe-Salpeter) dynamics through order α4.
Electrical detection of magnetization dynamics via spin rectification effects
Harder, Michael; Gui, Yongsheng; Hu, Can-Ming
2016-11-01
The purpose of this article is to review the current status of a frontier in dynamic spintronics and contemporary magnetism, in which much progress has been made in the past decade, based on the creation of a variety of micro and nanostructured devices that enable electrical detection of magnetization dynamics. The primary focus is on the physics of spin rectification effects, which are well suited for studying magnetization dynamics and spin transport in a variety of magnetic materials and spintronic devices. Intended to be intelligible to a broad audience, the paper begins with a pedagogical introduction, comparing the methods of electrical detection of charge and spin dynamics in semiconductors and magnetic materials respectively. After that it provides a comprehensive account of the theoretical study of both the angular dependence and line shape of electrically detected ferromagnetic resonance (FMR), which is summarized in a handbook format easy to be used for analysing experimental data. We then review and examine the similarity and differences of various spin rectification effects found in ferromagnetic films, magnetic bilayers and magnetic tunnel junctions, including a discussion of how to properly distinguish spin rectification from the spin pumping/inverse spin Hall effect generated voltage. After this we review the broad applications of rectification effects for studying spin waves, nonlinear dynamics, domain wall dynamics, spin current, and microwave imaging. We also discuss spin rectification in ferromagnetic semiconductors. The paper concludes with both historical and future perspectives, by summarizing and comparing three generations of FMR spectroscopy which have been developed for studying magnetization dynamics.
Spin dynamics of an ultra-small nanoscale molecular magnet
Directory of Open Access Journals (Sweden)
Ciftja Orion
2007-01-01
Full Text Available AbstractWe present mathematical transformations which allow us to calculate the spin dynamics of an ultra-small nanoscale molecular magnet consisting of a dimer system of classical (high Heisenberg spins. We derive exact analytic expressions (in integral form for the time-dependent spin autocorrelation function and several other quantities. The properties of the time-dependent spin autocorrelation function in terms of various coupling parameters and temperature are discussed in detail.
SD-CAS: Spin Dynamics by Computer Algebra System.
Filip, Xenia; Filip, Claudiu
2010-11-01
A computer algebra tool for describing the Liouville-space quantum evolution of nuclear 1/2-spins is introduced and implemented within a computational framework named Spin Dynamics by Computer Algebra System (SD-CAS). A distinctive feature compared with numerical and previous computer algebra approaches to solving spin dynamics problems results from the fact that no matrix representation for spin operators is used in SD-CAS, which determines a full symbolic character to the performed computations. Spin correlations are stored in SD-CAS as four-entry nested lists of which size increases linearly with the number of spins into the system and are easily mapped into analytical expressions in terms of spin operator products. For the so defined SD-CAS spin correlations a set of specialized functions and procedures is introduced that are essential for implementing basic spin algebra operations, such as the spin operator products, commutators, and scalar products. They provide results in an abstract algebraic form: specific procedures to quantitatively evaluate such symbolic expressions with respect to the involved spin interaction parameters and experimental conditions are also discussed. Although the main focus in the present work is on laying the foundation for spin dynamics symbolic computation in NMR based on a non-matrix formalism, practical aspects are also considered throughout the theoretical development process. In particular, specific SD-CAS routines have been implemented using the YACAS computer algebra package (http://yacas.sourceforge.net), and their functionality was demonstrated on a few illustrative examples.
The classical and quantum dynamics of molecular spins on graphene
Cervetti, Christian; Rettori, Angelo; Pini, Maria Gloria; Cornia, Andrea; Repollés, Ana; Luis, Fernando; Dressel, Martin; Rauschenbach, Stephan; Kern, Klaus; Burghard, Marko; Bogani, Lapo
2015-01-01
Controlling the dynamics of spins on surfaces is pivotal to the design of spintronic1 and quantum computing2 devices. Proposed schemes involve the interaction of spins with graphene to enable surface-state spintronics3,4, and electrical spin-manipulation4-11. However, the influence of the graphene environment on the spin systems has yet to be unraveled12. Here we explore the spin-graphene interaction by studying the classical and quantum dynamics of molecular magnets13 on graphene. While the static spin response remains unaltered, the quantum spin dynamics and associated selection rules are profoundly modulated. The couplings to graphene phonons, to other spins, and to Dirac fermions are quantified using a newly-developed model. Coupling to Dirac electrons introduces a dominant quantum-relaxation channel that, by driving the spins over Villain’s threshold, gives rise to fully-coherent, resonant spin tunneling. Our findings provide fundamental insight into the interaction between spins and graphene, establishing the basis for electrical spin-manipulation in graphene nanodevices. PMID:26641019
Spin dynamics in 122-type iron-based superconductors
Energy Technology Data Exchange (ETDEWEB)
Park, Jitae
2012-07-16
In this thesis, we present the experimental data on four different iron-based SC materials. It is mainly about the magnetic-dynamics study in the FeSC that is assumed to be among the most crucial ingredients for superconductivity in this system. Thus, the main goal of this thesis is to figure out the exact relationship between spin dynamics and superconductivity, and then further to realize what is the contribution of magnetic fluctuations for superconductivity by providing experimental data for modeling a microscopic mechanism of electron pairing in the FeSC system. In Chap. 2, we first discuss basic characteristics of FeSC, such as crystal structure and electron band-structure by briefly reviewing the relevant literature. Then, an introduction about magnetic and SC phases will follow based on the generic phase diagram. Details about current understanding of magnetic ground state in the parent compounds will be discussed in terms of spin-wave excitations which would be important when we are considering the spin dynamics in doped materials. To study magnetic dynamics in FeSC, we employed the inelastic-neutron-scattering (INS) method which can uniquely probe the underlying spin dynamics in the four dimensional energy and momentum space in a wide range. By taking advantage of the well developed theory for the magnetic neutron-scattering process, one can quantify the imaginary part of spin susceptibility that is an essential physical quantity the description of elementary magnetic excitations and can be compared with theoretical calculations directly. Moreover, the technique's energy-resolving scale spans over the most relevant energy range of magnetic fluctuations (from 0 to 100 meV). For these reasons, neutron scattering is a very powerful technique for magnetism study, and we introduce how neutron-scattering experiment works theoretically and practically in Chap. 3. For a slightly underdoped Ba{sub 1-x}K{sub x}Fe{sub 2}As{sub 2} compound, we report the phase
Electron-spin dynamics in elliptically polarized light waves
Bauke, Heiko; Grobe, Rainer
2014-01-01
We investigate the coupling of the spin angular momentum of light beams with elliptical polarization to the spin degree of freedom of free electrons. It is shown that this coupling, which is of similar origin as the well-known spin-orbit coupling, can lead to spin precession. The spin-precession frequency is proportional to the product of the laser-field's intensity and its spin density. The electron-spin dynamics is analyzed by employing exact numerical methods as well as time-dependent perturbation theory based on the fully relativistic Dirac equation and on the nonrelativistic Pauli equation that is amended by a relativistic correction that accounts for the light's spin density.
Giant dynamical Zeeman split in inverse spin valves
Wang, X. R.
2008-01-01
The inversion of a spin valve device is proposed. Opposite to a conventional spin valve of a non-magnetic spacer sandwiched between two ferromagnetic metals, an inverse spin valve is a ferromagnet sandwiched between two non-magnetic metals. It is predicted that, under a bias, the chemical potentials of spin-up and spin-down electrons in the metals split at metal-ferromagnet interfaces, a dynamical Zeeman effect. This split is of the order of an applied bias. Thus, there should be no problem o...
Spin susceptibility of underdoped cuprate superconductors: Insights from a stripe-ordered crystal
Hücker, M.; Gu, G. D.; Tranquada, J. M.
2008-12-01
We report a detailed study of the temperature and magnetic-field dependence of the spin susceptibility for a single crystal of La1.875Ba0.125CuO4 . From a quantitative analysis, we find that the temperature-dependent anisotropy of the susceptibility, observed in both the paramagnetic and stripe-ordered phases, directly indicates that localized Cu moments dominate the magnetic response. A field-induced spin-flop transition provides further corroboration for the role of local moments. Contrary to previous analyses of data from polycrystalline samples, we find that a commonly assumed isotropic and temperature-independent contribution from free carriers, if present, must be quite small. Our conclusion is strengthened by extending the quantitative analysis to include crystals of La2-xBaxCuO4 with x=0.095 and 0.155. On the basis of our results, we present a revised interpretation of the temperature and doping dependence of the spin susceptibility in La2-x(Sr,Ba)xCuO4 .
Mizushima, Takeshi
2014-11-01
We here illustrate the relation between odd-frequency spin-triplet even-parity (OTE) Cooper pairs and anomalous surface magnetic response in time-reversal-invariant (TRI) spin-triplet superfluids and superconductors. The spin susceptibility generally consists of two contributions: even-frequency odd-parity pair amplitudes and odd-frequency even-parity pair amplitudes. The OTE pair amplitudes are absent in the bulk region, but ubiquitously exist in the surface and interface region as Andreev bound states. We here clarify that additional discrete symmetries, originating from the internal symmetry and point-group symmetry, impose strong constraint on the OTE pair amplitudes emergent in the surface of TRI superfluids and superconductors. As a result of the symmetry constraint, the magnetic response of the OTE pairs yields Ising-like anisotropy. For the topological phase of the 3He -B in a restricted geometry, the coupling of the OTE pair amplitudes to an applied field is prohibited by an additional discrete symmetry. Once the discrete symmetry is broken, however, the OTE pairs start to couple to the applied field, which anomalously enhances surface spin susceptibility. Furthermore, we extend this theory to TRI superconductors, where the corresponding discrete symmetry is the mirror reflection symmetry.
Spin-dynamics simulations of the antiferromagnetic triangular XY model*
Nho, Kwangsik; Landau, D. P.
2002-03-01
Using Monte Carlo and spin-dynamics methods, we have simulated the dynamic behavior of the classical, antiferromagnetic XY model on a triangular lattice. The temporal evolutions of spin configurations were obtained by solving numerically the coupled equations of motion for each spin using fourth-order Suzuki-Trotter decompositions of exponential operators. From space-and time-displaced spin-spin correlation functions and their space-time Fourier transforms we obtained the dynamic structure factor S(q,w) for momentum q and frequency w. Below T_c, where long-range order appears in the staggered chirality[1], S(q,w) exhibits very strong and sharp spin-wave peaks in the in-plane-component S^xx. We also observe two-spin-wave peaks at low w and an almost dispersionless domain-wall peak at high w. Above T_c, a weak spin-wave peak persists but the domain-wall peak disappears for all q. We have calculated the dispersion relation and the linewidth of the spin-wave peak in S^xx by fitting the line shape to simple Lorentzians. *Supported by NSF [1] D.H. Lee, J.D. Joannopoulos, J.W. Negele, and D.P. Landau, Phys. Rev. Lett. 52, 433 (1984)
Spin currents and magnetization dynamics in multilayer systems
van der Bijl, E.
2014-01-01
In this Thesis the interplay between spin currents and magnetization dynamics is investigated theoretically. With the help of a simple model the relevant physical phenomena are introduced. From this model it can be deduced that in systems with small spin-orbit coupling, current-induced torques on
Toward Ultrafast Spin Dynamics in Low Dimensional Semiconductors
Chiu, Yi-Hsin
Since the discovery of long spin relaxation times of itinerant electrons up to 100 nanoseconds and spin diffusion lengths over 100 mum in GaAs, extraordinary advances in semiconductor spintronics have been made in the past one and half decades. Incorporating spins in semiconductors requires the following essential capabilities: (i) injection of spins into semiconductors, (ii) manipulation of spins, and (iii) sensitive detection of spin coherence. The solutions to these challenges lie in a deeper understanding of spin interactions and spin relaxation in semiconductors as well as appropriate tools to probe spin dynamics. In particular, recent experiments have suggested the important role of dimensionality in spin dynamics. For example, spin-orbit interaction, the dominant source of spin relaxation in most II-VI and III-V semiconductors, has been shown to be significantly suppressed in reduced dimensions. Low-dimensional semiconductors are therefore appealing candidates for exploring spin physics and device applications. This dissertation aims at exploring spin dynamics in low dimensional semiconductor systems using time-resolved optical techniques. The time resolution allows for a direct measurement of the equilibrium and non-equilibrium carrier spins and various spin interactions in the time domain. Optical approaches are also a natural fit for probing optically active nanostructures where electric approaches can often encounter challenges. For instance, fabricating electric contacts with nanostructures is a proven challenge because of their reduced size and modified electronic structure. This dissertation is divided into three sections targeting an ultimate goal of employing optical methods to explore spin dynamics in low dimensional semiconductors. First, the time-resolved Kerr rotation technique is employed to study spin relaxation in Fe/MgO/GaAs heterostructures. The results reveal rich interactions between the GaAs electron spins, nuclear spins, and the
Transistor-based metamaterials with dynamically tunable nonlinear susceptibility
Barrett, John P.; Katko, Alexander R.; Cummer, Steven A.
2016-08-01
We present the design, analysis, and experimental demonstration of an electromagnetic metamaterial with a dynamically tunable effective nonlinear susceptibility. Split-ring resonators loaded with transistors are shown theoretically and experimentally to act as metamaterials with a second-order nonlinear susceptibility that can be adjusted through the use of a bias voltage. Measurements confirm that this allows for the design of a nonlinear metamaterial with adjustable mixing efficiency.
Domain-wall spin dynamics in kagome antiferromagnets.
Lhotel, E; Simonet, V; Ortloff, J; Canals, B; Paulsen, C; Suard, E; Hansen, T; Price, D J; Wood, P T; Powell, A K; Ballou, R
2011-12-16
We report magnetization and neutron scattering measurements down to 60 mK on a new family of Fe based kagome antiferromagnets, in which a strong local spin anisotropy combined with a low exchange path network connectivity lead to domain walls intersecting the kagome planes through strings of free spins. These produce unfamiliar slow spin dynamics in the ordered phase, evolving from exchange-released spin flips towards a cooperative behavior on decreasing the temperature, probably due to the onset of long-range dipolar interaction. A domain structure of independent magnetic grains is obtained that could be generic to other frustrated magnets.
Spin motive force driven by skyrmion dynamics in magnetic nanodisks
Shimada, Yuhki; Ohe, Jun-ichiro
2015-05-01
The spin motive force driven by the dynamics of the skyrmion structure formed in a nanomagnetic disk is numerically investigated. Due to the existence of the magnetic structure along the disk edge, the collective mode of the magnetization is modified from that of the bulk skyrmion lattice obtained by using the periodic boundary condition. For a single-skyrmion disk, the dynamics of the skyrmion core and the edge magnetization induce the spin motive force, and a measurable AC voltage is obtained by two probes on the disk. For a multi-skyrmions disk, the phase-locked collective mode of skyrmions is found in the lowest resonant frequency where the amplitude of the AC voltage is enhanced by the cascade effect of the spin motive force. We also investigate the effect of the Rashba spin-orbit coupling on the spin motive force.
NMR with generalized dynamics of spin and spatial coordinates
Energy Technology Data Exchange (ETDEWEB)
Lee, Chang Jae
1987-11-01
This work is concerned with theoretical and experimental aspects of the generalized dynamics of nuclear spin and spatial coordinates under magnetic-field pulses and mechanical motions. The main text begins with an introduction to the concept of ''fictitious'' interactions. A systematic method for constructing fictitious spin-1/2 operators is given. The interaction of spins with a quantized-field is described. The concept of the fictitious interactions under the irradiation of multiple pulses is utilized to design sequences for selectively averaging linear and bilinear operators. Relations between the low-field sequences and high-field iterative schemes are clarified. These relations and the transformation properties of the spin operators are exploited to develop schemes for heteronuclear decoupling of multi-level systems. The resulting schemes are evaluated for heteronuclear decoupling of a dilute spin-1/2 from a spin-1 in liquid crystal samples and from a homonuclear spin-1/2 pair in liquids. A relation between the spin and the spatial variables is discussed. The transformation properties of the spin operators are applied to spatial coordinates and utilized to develop methods for removing the orientational dependence responsible for line broadening in a powder sample. Elimination of the second order quadrupole effects, as well as the first order anisotropies is discussed. It is shown that various sources of line broadening can effectively be eliminated by spinning and/or hopping the sample about judiciously chosen axes along with appropriate radio-frequency pulse sequences.
Institute of Scientific and Technical Information of China (English)
王敏; 王德杭; 洪汛宁; 王建伟
2011-01-01
Objective:To compare the arterial spin labeling and dynamic susceptibility contrast-enhanced MR imaging and explore the clinical application of arterial spin labeling (ASL) technique in the preoperation of tumor grade in brain gliomas. Methods: Twenty-three patients with gliomas ( all the cases were verified histologically, including 17 patients of highgrade gliomas, 6 patients of low-grade gliomas) were routinely examined by 3. 0 T MRI including ASL and DSC before operation. The maximal cerebral blood flow of solid regions of tumor (TBFmax) and the cerebral blood flow of opposite white matter, opposite grey matter and opposite hemisphere were measured on maps. Results: All of 23 cases demonstrated agreement between ASL and DSC MR imagings. The ratio of TBFmax/ opposite white matter CBF, TBFmax/opposite there was statistical difference between high-grade and low-grade gliomas. The threshold of TBFmax/opposite white matter CBF, TBFmax/opposite grey matter CBF, TBF max/opposite hemisphere CBF were 3. 06 , 0. 46 and 1. 31 respectively, the diagnosis sensibility were 100％, 88. 2％ and lOO％ respectively, and the specificity were 83. 3％, 83. 3％ and 100 ％ respectively by ASL technique. Conclusion : The noninvasive and repcatable ASL technique was almost as sensitive as DSC MRI in detecting brain gliomas perfusing abnormaliries. It is helpful to give the grade of gliomas before operation.%目的:对照研究动脉自旋标记(arterial spin labeling,ASL)与动态磁敏感对比增强(dynamic susceptibility contrast-enhanced,DSC)灌注成像技术在脑胶质瘤中的灌注特点,探讨ASL在脑胶质瘤术前分级中的临床应用价值.方法:使用3.0T MR成像系统对23例脑胶质瘤患者(术后病理证实高级别胶质瘤17例,低级别胶质瘤6例)术前行常规扫描外,加扫ASL及DSC灌注检查,测量肿瘤实质部分最大肿瘤血流量(maximal tumor blood flow,TBFmax)以及对侧白质、对侧灰质、对侧半球的血流量(cerebral blood
Spin tune mapping as a novel tool to probe the spin dynamics in storage rings
Saleev, A.; Nikolaev, N. N.; Rathmann, F.; Augustyniak, W.; Bagdasarian, Z.; Bai, M.; Barion, L.; Berz, M.; Chekmenev, S.; Ciullo, G.; Dymov, S.; Eversmann, D.; Gaisser, M.; Gebel, R.; Grigoryev, K.; Grzonka, D.; Guidoboni, G.; Heberling, D.; Hejny, V.; Hempelmann, N.; Hetzel, J.; Hinder, F.; Kacharava, A.; Kamerdzhiev, V.; Keshelashvili, I.; Koop, I.; Kulikov, A.; Lehrach, A.; Lenisa, P.; Lomidze, N.; Lorentz, B.; Maanen, P.; Macharashvili, G.; Magiera, A.; Mchedlishvili, D.; Mey, S.; Müller, F.; Nass, A.; Pesce, A.; Prasuhn, D.; Pretz, J.; Rosenthal, M.; Schmidt, V.; Semertzidis, Y.; Senichev, Y.; Shmakova, V.; Silenko, A.; Slim, J.; Soltner, H.; Stahl, A.; Stassen, R.; Stephenson, E.; Stockhorst, H.; Ströher, H.; Tabidze, M.; Tagliente, G.; Talman, R.; Engblom, P. Thörngren; Trinkel, F.; Uzikov, Yu.; Valdau, Yu.; Valetov, E.; Vassiliev, A.; Weidemann, C.; Wrońska, A.; Wüstner, P.; Zuprański, P.; Zurek, M.; JEDI Collaboration
2017-07-01
Precision experiments, such as the search for electric dipole moments of charged particles using storage rings, demand for an understanding of the spin dynamics with unprecedented accuracy. The ultimate aim is to measure the electric dipole moments with a sensitivity up to 15 orders in magnitude better than the magnetic dipole moment of the stored particles. This formidable task requires an understanding of the background to the signal of the electric dipole from rotations of the spins in the spurious magnetic fields of a storage ring. One of the observables, especially sensitive to the imperfection magnetic fields in the ring is the angular orientation of stable spin axis. Up to now, the stable spin axis has never been determined experimentally, and in addition, the JEDI collaboration for the first time succeeded to quantify the background signals that stem from false rotations of the magnetic dipole moments in the horizontal and longitudinal imperfection magnetic fields of the storage ring. To this end, we developed a new method based on the spin tune response of a machine to artificially applied longitudinal magnetic fields. This novel technique, called spin tune mapping, emerges as a very powerful tool to probe the spin dynamics in storage rings. The technique was experimentally tested in 2014 using polarized deuterons stored in the cooler synchrotron COSY, and for the first time, the angular orientation of the stable spin axis at two different locations in the ring has been determined to an unprecedented accuracy of better than 2.8 μ rad .
Spin dynamics in the kagome compound YBaCo{sub 3}AlO{sub 7}
Energy Technology Data Exchange (ETDEWEB)
Iakovleva, M.; Vavilova, E. [IFW Dresden (Germany); Zavoisky Physical-Technical Institute, Kazan (Russian Federation); Grafe, H.J.; Kataev, V.; Buechner, B. [IFW Dresden (Germany); Valldor, M. [MPI CPfS, Dresden (Germany)
2015-07-01
YBaCo{sub 3}AlO{sub 7} is a transition metal oxide compound with a magnetic kagome substructure where unconventional ground states such as a spin liquid can be expected. We have investigated the ground state and low energy spin dynamics of this material by {sup 27}Al nuclear magnetic resonance spectroscopy. The characteristic features of the spectral shape and of the relaxation rate temperature dependences show that short-range quasi static correlations occur in the system but not a long-range antiferromagnetic order. We compare our NMR results with AC and DC susceptibility measurements and discuss a possible realization of a spin glass state due to intrinsic structural disorder in this material.
Variation of the dynamic susceptibility along an isochrone
DEFF Research Database (Denmark)
Bailey, Nicholas; Schrøder, Thomas; Dyre, J. C.
2014-01-01
Koperwas et al. showed in a recent paper [Phys. Rev. Lett. 111, 125701 (2013)] that the dynamic susceptibility χ4 as estimated by dielectric measurements for certain glass-forming liquids decreases substantially with increasing pressure along a curve of constant relaxation time. This observation...
The spin-temperature theory of dynamic nuclear polarization and nuclear spin-lattice relaxation
Byvik, C. E.; Wollan, D. S.
1974-01-01
A detailed derivation of the equations governing dynamic nuclear polarization (DNP) and nuclear spin lattice relaxation by use of the spin temperature theory has been carried to second order in a perturbation expansion of the density matrix. Nuclear spin diffusion in the rapid diffusion limit and the effects of the coupling of the electron dipole-dipole reservoir (EDDR) with the nuclear spins are incorporated. The complete expression for the dynamic nuclear polarization has been derived and then examined in detail for the limit of well resolved solid effect transitions. Exactly at the solid effect transition peaks, the conventional solid-effect DNP results are obtained, but with EDDR effects on the nuclear relaxation and DNP leakage factor included. Explicit EDDR contributions to DNP are discussed, and a new DNP effect is predicted.
Nematic ordering dynamics of an antiferromagnetic spin-1 condensate
Symes, L. M.; Blakie, P. B.
2017-07-01
We consider the formation of order in a quasi-two-dimensional antiferromagnetic spin-1 condensate quenched from an easy-axis to an easy-plane nematic phase. We define the relevant order parameter to quantify the spin-nematic degrees of freedom and study the evolution of the spin-nematic and superfluid order during the coarsening dynamics using numerical simulations. We observe dynamical scaling in the late-time dynamics, with both types of order extending across the system with a diffusive growth law. We identify half-quantum vortices as the relevant topological defects of the ordering dynamics and demonstrate that the growth of both types of order is determined by the mutual annihilation of these vortices.
Coupled spin, elastic and charge dynamics in magnetic nanostructures
Kamra, A.
2015-01-01
In this Thesis, I address the interaction of magnetic degrees of freedom with charge current and elastic dynamics in hybrid systems composed of magnetic and non-magnetic materials. The objective, invariably, is to control and study spin dynamics using charge and elastic degrees of freedom. In certai
Spin Dynamics in an Ordered Stripe Phase
Tranquada, J. M.; Wochner, P.; Buttrey, D. J.
1997-09-01
Inelastic neutron scattering has been used to measure the low-energy spin excitations in the ordered charge-stripe phase of La2NiO4+δ with δ = 0.133. Spin-wave-like excitations disperse away from the incommensurate magnetic superlattice points with a velocity ~60% of that in the δ = 0 compound. Incommensurate inelastic peaks remain well resolved up to at least twice the magnetic ordering temperature. Paramagnetic scattering from a δ = 0.105 sample, which has a Néel-ordered ground state, shows anomalies suggestive of incipient stripe correlations. Similarities between these results and measurements on superconducting cuprates are discussed.
Generating quantum states through spin chain dynamics
Kay, Alastair
2017-04-01
The spin chain is a theoretical work-horse of the physicist, providing a convenient, tractable model that yields insight into a host of physical phenomena including conduction, frustration, superconductivity, topological phases, localisation, phase transitions, quantum chaos and even string theory. Our ultimate aim, however, is not just to understand the properties of a physical system, but to harness it for our own ends. We therefore study the possibilities for engineering a special class of spin chain, envisaging the potential for this to feedback into the original physical systems. We pay particular attention to the generation of multipartite entangled states such as the W (Dicke) state, superposed over multiple sites of the chain.
Strong ties promote the epidemic prevalence in susceptible-infected-susceptible spreading dynamics
Cui, Ai-Xiang; Zhou, Tao
2013-01-01
Understanding spreading dynamics will benefit society as a whole in better preventing and controlling diseases, as well as facilitating the socially responsible information while depressing destructive rumors. In network-based spreading dynamics, edges with different weights may play far different roles: a friend from afar usually brings novel stories, and an intimate relationship is highly risky for a flu epidemic. In this article, we propose a weighted susceptible-infected-susceptible model on complex networks, where the weight of an edge is defined by the topological proximity of the two associated nodes. Each infected individual is allowed to select limited number of neighbors to contact, and a tunable parameter is introduced to control the preference to contact through high-weight or low-weight edges. Experimental results on six real networks show that the epidemic prevalence can be largely promoted when strong ties are favored in the spreading process. By comparing with two statistical null models respe...
Entanglement dynamics via semiclassical propagators in systems of two spins
Ribeiro, A D
2012-01-01
We analyze the dynamical generation of entanglement in systems of two interacting spins initially prepared in a product of spin coherent states. For arbitrary time-independent Hamiltonians, we derive a semiclassical expression for the purity of the reduced density matrix as function of time. The final formula, subsidiary to the linear entropy, shows that the short-time dynamics of entanglement depends exclusively on the stability of trajectories governed by the underlying classical Hamiltonian. Also, this semiclassical measure is shown to reproduce the general properties of its quantum counterpart and give the expected result in the large spin limit. The accuracy of the semiclassical formula is further illustrated in a problem of phase exchange for two particles of spin $j$.
Simulation of Spin-orbit Dynamics in Storage Rings
Ivanov, A.; Andrianov, S.; Senichev, Yu.
2016-09-01
In the article a mapping approach based on nonlinear matrix integration for longterm spin-orbit dynamics simulation is briefly described. Using this technique the nonlinear effects of spin dynamics in an electrostatics storage ring are investigated. Namely, the fringe fields, the energy conservation law and the random field errors are considered. The necessity of examination of such effects arises, for example, in the storage ring design for search the Electrical Dipole Moment of proton and deuteron. The EDM ring is proposed to measure EDM using the spin transformation of polarized particle in the magneto-electrostatic elements of the ring. The article consists of short description of the spin-orbit simulation results based on the nonlinear model.
Chaos and dynamics of spinning particles in Kerr spacetime
Han, Wen-Biao
2010-01-01
We study chaos dynamics of spinning particles in Kerr spacetime of rotating black holes use the Papapetrou equations by numerical integration. Because of spin, this system exists many chaos solutions, and exhibits some exceptional dynamic character. We investigate the relations between the orbits chaos and the spin magnitude S, pericenter, polar angle and Kerr rotation parameter a by means of a kind of brand new Fast Lyapulov Indicator (FLI) which is defined in general relativity. The classical definition of Lyapulov exponent (LE) perhaps fails in curve spacetime. And we emphasize that the Poincar\\'e sections cannot be used to detect chaos for this case. Via calculations, some new interesting conclusions are found: though chaos is easier to emerge with bigger S, but not always depends on S monotonically; the Kerr parameter a has a contrary action on the chaos occurrence. Furthermore, the spin of particles can destroy the symmetry of the orbits about the equatorial plane. And for some special initial condition...
Yoshitake, Junki; Nasu, Joji; Kato, Yasuyuki; Motome, Yukitoshi
2017-07-01
A prominent feature of quantum spin liquids is fractionalization of the spin degree of freedom. Fractionalized excitations have their own dynamics in different energy scales, and hence, affect finite-temperature (T ) properties in a peculiar manner even in the paramagnetic state harboring the quantum spin liquid state. We here present a comprehensive theoretical study of the spin dynamics in a wide T range for the Kitaev model on a honeycomb lattice, whose ground state is a quantum spin liquid. In this model, the fractionalization occurs to break up quantum spins into itinerant matter fermions and localized Z2 fluxes, which results in two crossovers at very different T scales. Extending the previous study for the isotropic coupling case [J. Yoshitake, J. Nasu, and Y. Motome, Phys. Rev. Lett. 117, 157203 (2016), 10.1103/PhysRevLett.117.157203], we calculate the dynamical spin structure factor S (q ,ω ) , the NMR relaxation rate 1 /T1 , and the magnetic susceptibility χ while changing the anisotropy in the exchange coupling constants, by using the dynamical mean-field theory based on a Majorana fermion representation. We describe the details of the methodology including the continuous-time quantum Monte Carlo method for computing dynamical spin correlations and the maximum entropy method for analytic continuation. We confirm that the combined method provides accurate results in a wide T range including the region where the spins are fractionalized. We find that also in the anisotropic cases the system exhibits peculiar behaviors below the high-T crossover whose temperature is comparable to the average of the exchange constants: S (q ,ω ) shows an inelastic response at the energy scale of the averaged exchange constant, 1 /T1 continues to grow even though the equal-time spin correlations are saturated and almost T independent, and χ deviates from the Curie-Weiss behavior. In particular, when the exchange interaction in one direction is stronger than the other two
Quantum Computation and Quantum Spin Dynamics
Raedt, Hans De; Michielsen, Kristel; Hams, Anthony; Miyashita, Seiji; Saito, Keiji
2001-01-01
We analyze the stability of quantum computations on physically realizable quantum computers by simulating quantum spin models representing quantum computer hardware. Examples of logically identical implementations of the controlled-NOT operation are used to demonstrate that the results of a quantum
Quantum Computation and Quantum Spin Dynamics
Raedt, Hans De; Michielsen, Kristel; Hams, Anthony; Miyashita, Seiji; Saito, Keiji
2001-01-01
We analyze the stability of quantum computations on physically realizable quantum computers by simulating quantum spin models representing quantum computer hardware. Examples of logically identical implementations of the controlled-NOT operation are used to demonstrate that the results of a quantum
Optically induced dynamic nuclear spin polarisation in diamond
Scheuer, Jochen; Schwartz, Ilai; Chen, Qiong; Schulze-Sünninghausen, David; Carl, Patrick; Höfer, Peter; Retzker, Alexander; Sumiya, Hitoshi; Isoya, Junichi; Luy, Burkhard; Plenio, Martin B.; Naydenov, Boris; Jelezko, Fedor
2016-01-01
The sensitivity of magnetic resonance imaging (MRI) depends strongly on nuclear spin polarisation and, motivated by this observation, dynamical nuclear spin polarisation has recently been applied to enhance MRI protocols (Kurhanewicz et al 2011 Neoplasia 13 81). Nuclear spins associated with the 13C carbon isotope (nuclear spin I = 1/2) in diamond possess uniquely long spin lattice relaxation times (Reynhardt and High 2011 Prog. Nucl. Magn. Reson. Spectrosc. 38 37). If they are present in diamond nanocrystals, especially when strongly polarised, they form a promising contrast agent for MRI. Current schemes for achieving nuclear polarisation, however, require cryogenic temperatures. Here we demonstrate an efficient scheme that realises optically induced 13C nuclear spin hyperpolarisation in diamond at room temperature and low ambient magnetic field. Optical pumping of a nitrogen-vacancy centre creates a continuously renewable electron spin polarisation which can be transferred to surrounding 13C nuclear spins. Importantly for future applications we also realise polarisation protocols that are robust against an unknown misalignment between magnetic field and crystal axis.
Kim, Tae Heon; Grünberg, Peter; Han, Song Hee; Cho, Beongki
2016-10-01
The spin-torque driven dynamics of antiferromagnets with Dzyaloshinskii-Moriya interaction (DMI) were investigated based on the Landau-Lifshitz-Gilbert-Slonczewski equation with antiferromagnetic and ferromagnetic order parameters (l and m, respectively). We demonstrate that antiferromagnets including DMI can be described by a 2-dimensional pendulum model of l. Because m is coupled with l, together with DMI and exchange energy, close examination of m provides fundamental understanding of its dynamics in linear and nonlinear regimes. Furthermore, we discuss magnetization reversal as a function of DMI and anisotropy energy induced by a spin current pulse.
Kim, Tae Heon; Grünberg, Peter; Han, Song Hee; Cho, Beongki
2016-01-01
The spin-torque driven dynamics of antiferromagnets with Dzyaloshinskii-Moriya interaction (DMI) were investigated based on the Landau-Lifshitz-Gilbert-Slonczewski equation with antiferromagnetic and ferromagnetic order parameters (l and m, respectively). We demonstrate that antiferromagnets including DMI can be described by a 2-dimensional pendulum model of l. Because m is coupled with l, together with DMI and exchange energy, close examination of m provides fundamental understanding of its dynamics in linear and nonlinear regimes. Furthermore, we discuss magnetization reversal as a function of DMI and anisotropy energy induced by a spin current pulse. PMID:27713522
Mondal, Ritwik; Berritta, Marco; Oppeneer, Peter M.
2016-10-01
Starting from the Dirac-Kohn-Sham equation, we derive the relativistic equation of motion of spin angular momentum in a magnetic solid under an external electromagnetic field. This equation of motion can be rewritten in the form of the well-known Landau-Lifshitz-Gilbert equation for a harmonic external magnetic field and leads to a more general magnetization dynamics equation for a general time-dependent magnetic field. In both cases there is an electronic spin-relaxation term which stems from the spin-orbit interaction. We thus rigorously derive, from fundamental principles, a general expression for the anisotropic damping tensor which is shown to contain an isotropic Gilbert contribution as well as an anisotropic Ising-like and a chiral, Dzyaloshinskii-Moriya-like contribution. The expression for the spin relaxation tensor comprises furthermore both electronic interband and intraband transitions. We also show that when the externally applied electromagnetic field possesses spin angular momentum, this will lead to an optical spin torque exerted on the spin moment.
Spin-dynamics simulations of the triangular antiferromagnetic XY model*
Nho, Kwangsik; Landau, D. P.
2003-03-01
Using Monte Carlo and spin-dynamics methods, we have studied the dynamic behavior of the classical, antiferromagnetic XY model on a triangular lattice. The temporal evolutions of spin configurations were obtained by solving numerically the coupled equations of motion for each spin using fourth-order Suzuki-Trotter decompositions of exponential operators. We calculated the dynamic structure factor S(q,w) for momentum q and frequency w. Below T_KT (Kosteritz-Thouless transition), both the in-plane (S^xx) and out-of-plane (S^zz) components exhibit very strong and sharp spin-wave peaks. Well above T_KT, S^xx and S^zz apparently display a central peak, and spin-wave signatures are still seen in S^zz. In addition, we also observed an almost dispersionless domain-wall peak at high w below Tc (Ising transition), where long-range order appears in the staggered chirality[1]. We found that our results demonstrate the consistency of the dynamic finite-size scaling theory for the characteristic frequency wm and S(q,w). *Supported by NSF [1] D.H. Lee, J.D. Joannopoulos, J.W. Negele, and D.P. Landau, Phys. Rev. Lett. 52, 433 (1984)
The dynamics of a spinning particle in a linear in spin Hamiltonian approximation
Lukes-Gerakopoulos, Georgios; Patsis, Panos A; Seyrich, Jonathan
2016-01-01
We investigate for order and chaos the dynamical system of a spinning test particle of mass $m$ moving in the spacetime background of a Kerr black hole of mass M. This system is approximated in our investigation by the linear in spin Hamiltonian function provided in [E. Barausse, and A. Buonanno, Phys.Rev. D 81, 084024 (2010)]. We study the corresponding phase space by using 2D projections on a surface of section and the method of color and rotation on a 4D Poincar\\'e section. Various topological structures coming from the non-integrability of the linear in spin Hamiltonian are found and discussed. Moreover, an interesting result is that from the value of the dimensionless spin $S/(m M)=10^{-4}$ of the particle and below, the impact of the non-integrability of the system on the motion of the particle seems to be negligible.
Magnetization dynamics and spin pumping induced by standing elastic waves
Azovtsev, A. V.; Pertsev, N. A.
2016-11-01
The magnetization dynamics induced by standing elastic waves excited in a thin ferromagnetic film is described with the aid of micromagnetic simulations taking into account the magnetoelastic coupling between spins and lattice strains. Our calculations are based on the numerical solution of the Landau-Lifshitz-Gilbert equation comprising the damping term and the effective magnetic field with all relevant contributions. The simulations have been performed for 2-nm-thick F e81G a19 film dynamically strained by longitudinal and transverse standing waves with various frequencies, which span a wide range around the resonance frequency νres of coherent magnetization precession in unstrained F e81G a19 film. It is found that standing elastic waves give rise to complex local magnetization dynamics and spatially inhomogeneous dynamic patterns in the form of standing spin waves with the same wavelength. Remarkably, the amplitude of magnetization precession does not go to zero at nodes of these spin waves, which cannot be precisely described by simple analytical formulae. In the steady-state regime, magnetization oscillates with the frequency of the elastic wave, except in the case of longitudinal waves with frequencies well below νres, where the magnetization precesses with variable frequency strongly exceeding the wave frequency. The results obtained for the magnetization dynamics driven by elastic waves are used to calculate the spin current pumped from the dynamically strained ferromagnet into adjacent paramagnetic metal. Numerical calculations demonstrate that the transverse charge current in the paramagnetic layer, which is created by the spin current via inverse spin Hall effect, is high enough to be measured experimentally.
Spin tune mapping as a novel tool to probe the spin dynamics in storage rings
Directory of Open Access Journals (Sweden)
2017-07-01
Full Text Available Precision experiments, such as the search for electric dipole moments of charged particles using storage rings, demand for an understanding of the spin dynamics with unprecedented accuracy. The ultimate aim is to measure the electric dipole moments with a sensitivity up to 15 orders in magnitude better than the magnetic dipole moment of the stored particles. This formidable task requires an understanding of the background to the signal of the electric dipole from rotations of the spins in the spurious magnetic fields of a storage ring. One of the observables, especially sensitive to the imperfection magnetic fields in the ring is the angular orientation of stable spin axis. Up to now, the stable spin axis has never been determined experimentally, and in addition, the JEDI collaboration for the first time succeeded to quantify the background signals that stem from false rotations of the magnetic dipole moments in the horizontal and longitudinal imperfection magnetic fields of the storage ring. To this end, we developed a new method based on the spin tune response of a machine to artificially applied longitudinal magnetic fields. This novel technique, called spin tune mapping, emerges as a very powerful tool to probe the spin dynamics in storage rings. The technique was experimentally tested in 2014 using polarized deuterons stored in the cooler synchrotron COSY, and for the first time, the angular orientation of the stable spin axis at two different locations in the ring has been determined to an unprecedented accuracy of better than 2.8 μ rad.
Spin Glasses : Statics and Dynamics : Summer School
Bovier, Anton
2009-01-01
Over the last decade, spin glass theory has turned from a fascinating part of t- oretical physics to a ?ourishing and rapidly growing subject of probability theory as well. These developments have been triggered to a large part by the mathem- ical understanding gained on the fascinating and previously mysterious “Parisi solution” of the Sherrington–Kirkpatrick mean ?eld model of spin glasses, due to the work of Guerra, Talagrand, and others. At the same time, new aspects and applications of the methods developed there have come up. The presentvolumecollects a number of reviewsaswellas shorterarticlesby lecturers at a summer school on spin glasses that was held in July 2007 in Paris. These articles range from pedagogical introductions to state of the art papers, covering the latest developments. In their whole, they give a nice overview on the current state of the ?eld from the mathematical side. The review by Bovier and Kurkova gives a concise introduction to mean ?eld models, starting with the Curie–...
Dynamic susceptibility of onion in ferromagnetic elliptical nanoring
Mu, Congpu; Song, Jiefang; Xu, Jianghong; Wen, Fusheng
2016-06-01
Micromagnetic simulation was performed to investigate the equilibrium state and dynamic susceptibility spectra of magnetic elliptical nanoring. There are two equilibrium states (onion and vortex) obtained in elliptical nanoring. The onion state can be used to record information in MRAM. And it is important to investigate the dynamic susceptibility spectra of onion state, which is closely related to writing and reading speed of magnetic memory devices. Those results show that two or three resonance peaks are found under different thickness of elliptical nanoring with onion state, respectively. The low resonance frequency of two resonance peaks is increasing with the arm width of the elliptical ring, but is decreasing with the thickness. However, the high frequency of two resonance peaks is decreasing with the arm width of the elliptical ring.
Dynamic susceptibility of onion in ferromagnetic elliptical nanoring
Directory of Open Access Journals (Sweden)
Congpu Mu
2016-06-01
Full Text Available Micromagnetic simulation was performed to investigate the equilibrium state and dynamic susceptibility spectra of magnetic elliptical nanoring. There are two equilibrium states (onion and vortex obtained in elliptical nanoring. The onion state can be used to record information in MRAM. And it is important to investigate the dynamic susceptibility spectra of onion state, which is closely related to writing and reading speed of magnetic memory devices. Those results show that two or three resonance peaks are found under different thickness of elliptical nanoring with onion state, respectively. The low resonance frequency of two resonance peaks is increasing with the arm width of the elliptical ring, but is decreasing with the thickness. However, the high frequency of two resonance peaks is decreasing with the arm width of the elliptical ring.
Solving the Dynamic Correlation Problem of the Susceptible-Infected-Susceptible Model on Networks
Cai, Chao-Ran; Chen, Michael Z Q; Holme, Petter; Guan, Jian-Yue
2016-01-01
The Susceptible-Infected-Susceptible model is a canonical model for emerging disease outbreaks. Such outbreaks are naturally modeled as taking place on networks. A theoretical challenge in network epidemiology is the dynamic correlations coming from that if one node is occupied, or infected (for disease spreading models), then its neighbors are likely to be occupied. By combining two theoretical approaches---the heterogeneous mean-field theory and the effective degree method---we are able to include these correlations in an analytical solution of the SIS model. We derive accurate expressions for the average prevalence (fraction of infected) and epidemic threshold. We also discuss how to generalize the approach to a larger class of stochastic population models.
Nonlinear dynamics of spin transfer nano-oscillators
Indian Academy of Sciences (India)
B Subash; V K Chandrasekar; M Lakshmanan
2015-03-01
The evolution equation of a ferromagnetic spin system described by Heisenberg nearest-neighbour interaction is given by Landau–Lifshitz–Gilbert (LLG) equation, which is a fascinating nonlinear dynamical system. For a nanomagnetic trilayer structure (spin valve or pillar) an additional torque term due to spin-polarized current has been suggested by Slonczewski, which gives rise to a rich variety of dynamics in the free layer. Under appropriate conditions the spin-polarized current gives a time-varying resistance to the magnetic structure thereby inducing magnetization oscillations of frequency which lies in the microwave region. Such a device is called a spin transfer nanooscillator (STNO). However, this interesting nanoscale level source of microwaves lacks efficiency due to its low emitting power typically of the order of nWs. To over-come this difficulty, one has to consider the collective dynamics of synchronized arrays/networks of STNOs as suggested by Fert and coworkers so that the power can be enhanced 2 times that of a single STNO. We show that this goal can be achieved by applying a common microwave magnetic field to an array of STNOs. In order to make the system technically more feasible to practical level integration with CMOS circuits, we establish suitable electrical connections between the oscillators. Although the electrical connection makes the system more complex, the applied microwave magnetic field drives the system to synchronization in large regions of parameter space.
Molecular dynamics, spin dynamics study of phonon-magnon interactions in BCC iron
Perera, Dilina; Landau, David P.; Stocks, G. Malcolm; Nicholson, Don; Eisenbach, Markus; Yin, Junqi
2013-03-01
By combining an atomistic many-body potential (Finnis-Sinclair) with a classical Heisenberg-like spin Hamiltonian, we perform combined molecular and spin dynamics simulations to investigate phonon-magnon interactions in BCC iron. The coupling between atomic and spin degrees of freedom is established via a distance dependent exchange interaction derived from first principles electronic structure calculations. Coupled equations of motion are integrated using a second order Suzuki-Trotter decomposition of the exponential time evolution operator. To investigate the effect of lattice vibrations on spin wave spectrum, we calculate spin-spin and density-density dynamic structure factors S(q, ω), and compare that to the results obtained from pure spin dynamics simulations performed on a rigid lattice. In the presence of lattice vibrations, we observe an additional peak in the longitudinal spin-spin dynamic structure factor which coincides with the peak position in density-density dynanmic structure factor. Research sponsored by the U.S. Department of Energy, Office of Basic Energy Sciences, Materials Sciences and Engineering Division, ''Center for Defect Physics,'' an Energy Frontier Research Center
Electron spin coherence and effect of spin polarization on electron relaxation dynamics in GaAs
Teng, Lihua; Wang, Xia; Ge, Weikun; Lai, Tianshu
2011-09-01
Time-resolved circularly and linearly polarized pump-probe spectroscopy is used to study the evolution of the electron spin coherence and electron relaxation dynamics in bulk GaAs at 9.6 K. In particular, their dependence on photon energy (or electron excess energy) is carefully investigated. The absorption quantum beats which are observed in circularly polarized pump-probe spectroscopy are obtained, reflecting the dephasing of the electron spin coherence. A circularly dichromatic pump-probe model is developed with both the spin-polarization-dependent band-filling and band-gap renormalization effects being taken into account. The model is used to simulate the differential transmission spectra for the collinearly polarized, co-helicity circularly polarized and cross-helicity circularly polarized pump-probe configurations, respectively. It is found that the model simulates well the features of the absorption quantum beats for a spin-dependent thermalized distribution of the photocreated carriers by a circularly polarized pump pulse, such as the variation of the oscillatory amplitude and phase reversal of the absorption quantum beats with photon energy increase. The simulation is in good agreement with our experimental results and reveals the effect of spin polarization on electron relaxation dynamics.
Spin dynamics in a Curie-switch.
Kravets, A F; Tovstolytkin, A I; Dzhezherya, Yu I; Polishchuk, D M; Kozak, I M; Korenivski, V
2015-11-11
Ferromagnetic resonance properties of F1/f/F2/AF multilayers, where weakly ferromagnetic spacer f is sandwiched between strongly ferromagnetic layers F1 and F2, with F1 being magnetically soft and F2-magnetically hard due to exchange pinning to antiferromagnetic layer AF, are investigated. Spacer-mediated exchange coupling is shown to strongly affect the resonance fields of both F1 and F2 layers. Our theoretical calculations as well as measurements show that the key magnetic parameters of the spacer, which govern the ferromagnetic resonance in F1/f/F2/AF, are the magnetic exchange length (Λ), effective saturation magnetization at T = 0 (m0) and effective Curie temperature (T(C)(eff)). The values of these key parameters are deduced from the experimental data for multilayers with f = Ni(x)Cu(100-x), for the key ranges in the Ni-concentration (x = 54 ÷ 70 at. %) and spacer thickness (d = 3 ÷ 6 nm). The results obtained provide a deeper insight into thermally-controlled spin precession and switching in magnetic nanostructures, with potential applications in spin-based oscillators and memory devices.
Magnetization dynamics of imprinted non-collinear spin textures
Energy Technology Data Exchange (ETDEWEB)
Streubel, Robert, E-mail: r.streubel@ifw-dresden.de; Kopte, Martin; Makarov, Denys, E-mail: d.makarov@ifw-dresden.de [Institute for Integrative Nanosciences, IFW Dresden, 01069 Dresden (Germany); Fischer, Peter [Center for X-Ray Optics, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Physics Department, UC Santa Cruz, Santa Cruz, California 95064 (United States); Schmidt, Oliver G. [Institute for Integrative Nanosciences, IFW Dresden, 01069 Dresden (Germany); Material Systems for Nanoelectronics, Chemnitz University of Technology, 09107 Chemnitz (Germany)
2015-09-14
We study the magnetization dynamics of non-collinear spin textures realized via imprint of the magnetic vortex state in soft permalloy into magnetically hard out-of-plane magnetized Co/Pd nanopatterned heterostructures. Tuning the interlayer exchange coupling between soft- and hard-magnetic subsystems provides means to tailor the magnetic state in the Co/Pd stack from being vortex- to donut-like with different core sizes. While the imprinted vortex spin texture leads to the dynamics similar to the one observed for vortices in permalloy disks, the donut-like state causes the appearance of two gyrofrequencies characteristic of the early and later stages of the magnetization dynamics. The dynamics are described using the Thiele equation supported by the full scale micromagnetic simulations by taking into account an enlarged core size of the donut states compared to magnetic vortices.
Spin dynamics in storage rings and linear accelerators
Energy Technology Data Exchange (ETDEWEB)
Irwin, J.
1994-04-01
The purpose of these lectures is to survey the subject of spin dynamics in accelerators: to give a sense of the underlying physics, the typical analytic and numeric methods used, and an overview of results achieved. Consideration will be limited to electrons and protons. Examples of experimental and theoretical results in both linear and circular machines are included.
Dynamical theory of spin noise and relaxation - prospects for real time NMR measurements
Field, Timothy
2014-03-01
The dynamics of a spin system is usually calculated using the density matrix. However, the usual formulation in terms of the density matrix predicts that the signal will decay to zero, and does not address the stochastic dynamics of individual spins. Spin fluctuations are to be viewed as an intrinsic quantum mechanical property of such systems immersed in random magnetic environments, and are observed as ``spin noise'' in the absence of any radio frequency (RF) excitation. Using stochastic calculus we develop a dynamical theory of spin noise and relaxation whose origins lie in the component spin fluctuations. This entails consideration of random pure states for individual protons, and how these pure states are correctly combined when the density matrix is formulated. Both the lattice and the spins are treated quantum mechanically. Such treatment incorporates both the processes of spin-spin and (finite temperature) spin-lattice relaxation. Our results reveal the intimate connections between spin noise and conventional spin relaxation, in terms of a modified spin density (MSD), distinct from the density matrix, which is necessary to describe non-ensemble averaged properties of spin systems. With the prospect of ultra-fast digitization, the role of spin noise in real time parameter extraction for (NMR) spin systems, and the advantage over standard techniques, is of essential importance, especially for systems containing a small number of spins. In this presentation we outline prospects for harnessing the recent dynamical theory in terms of spin noise measurement, with attention to real time properties.
Energy Technology Data Exchange (ETDEWEB)
Nabavizadeh, Seyed Ali; Edgar, J.C.; Vossough, Arastoo [University of Pennsylvania, Department of Radiology, Philadelphia, PA (United States); Children' s Hospital of Philadelphia, Department of Radiology, Philadelphia, PA (United States)
2014-10-15
The objectives of the study are to investigate the application of susceptibility-weighted imaging (SWI) and arterial spin labeling (ASL) imaging in the assessment of shunting and the draining veins in pediatric patients with arteriovenous shunting and compare the utility of SWI and ASL with conventional MR and digital subtraction angiography (DSA). This study is a retrospective study of 19 pediatric patients with arteriovenous shunting on brain MRI who were also evaluated with DSA. We assessed the ability of conventional MRI sequences, susceptibility magnitude images, phase-filtered SWI images, and pulsed ASL images in the detection of arteriovenous (AV) shunting, number of draining veins and drainage pathways in comparison to DSA. The mean number of detected draining veins on DSA (3.63) was significantly higher compared to SWI phase-filtered image (mean = 2.72), susceptibility magnitude image (mean = 2.92), ASL (mean = 1.76) and conventional MRI (2.47) (p < 0.05). Pairwise comparison of DSA difference scores (i.e., difference between MR modalities in the number of missed draining veins) revealed no difference between the MR modalities (p > 0.05). ASL was the only method that correctly identified superficial and deep venous drainage in all patients. Regarding detection of shunting, ASL, SWI phase-filtered, and magnitude images demonstrated shunting in 100, 83, and 84 % of patients, respectively. SWI depicts a higher number of draining vein compared to conventional MR pulse sequences. ASL is a sensitive approach in showing 100 % sensitivity in the detection of AV shunting and in the diagnosis of the pattern of venous drainage. The present findings suggest the added utility of both SWI and ASL in the assessment of AV shunting. (orig.)
Covariant hamiltonian spin dynamics in curved space–time
Energy Technology Data Exchange (ETDEWEB)
D' Ambrosi, G., E-mail: gdambros@nikhef.nl [Nikhef, Science Park 105, Amsterdam (Netherlands); Satish Kumar, S., E-mail: satish@lorentz.leidenuniv.nl [Lorentz Institute, Leiden University, Niels Bohrweg 2, Leiden (Netherlands); Holten, J.W. van, E-mail: t32@nikhef.nl [Nikhef, Science Park 105, Amsterdam (Netherlands); Lorentz Institute, Leiden University, Niels Bohrweg 2, Leiden (Netherlands)
2015-04-09
The dynamics of spinning particles in curved space–time is discussed, emphasizing the hamiltonian formulation. Different choices of hamiltonians allow for the description of different gravitating systems. We give full results for the simplest case with minimal hamiltonian, constructing constants of motion including spin. The analysis is illustrated by the example of motion in Schwarzschild space–time. We also discuss a non-minimal extension of the hamiltonian giving rise to a gravitational equivalent of the Stern–Gerlach force. We show that this extension respects a large class of known constants of motion for the minimal case.
Covariant hamiltonian spin dynamics in curved space-time
d'Ambrosi, G; van Holten, J W
2015-01-01
The dynamics of spinning particles in curved space-time is discussed, emphasizing the hamiltonian formulation. Different choices of hamiltonians allow for the description of different gravitating systems. We give full results for the simplest case with minimal hamiltonian, constructing constants of motion including spin. The analysis is illustrated by the example of motion in Schwarzschild space-time. We also discuss a non-minimal extension of the hamiltonian giving rise to a gravitational equivalent of the Stern-Gerlach force. We show that this extension respects a large class of known constants of motion for the minimal case.
Computer studies of multiple-quantum spin dynamics
Energy Technology Data Exchange (ETDEWEB)
Murdoch, J.B.
1982-11-01
The excitation and detection of multiple-quantum (MQ) transitions in Fourier transform NMR spectroscopy is an interesting problem in the quantum mechanical dynamics of spin systems as well as an important new technique for investigation of molecular structure. In particular, multiple-quantum spectroscopy can be used to simplify overly complex spectra or to separate the various interactions between a nucleus and its environment. The emphasis of this work is on computer simulation of spin-system evolution to better relate theory and experiment.
Shi, Caiyun; Xie, Guoxi; Zhang, Yongqin; Zhang, Xiaoyong; Chen, Min; Su, Shi; Dong, Ying; Liu, Xin; Ji, Jim
2017-04-01
This study aims to develop an accelerated susceptibility-based positive contrast MR imaging method for visualizing MR compatible metallic devices. A modified fast spin echo sequence is used to accelerate data acquisition. Each readout gradient in the modified fast spin echo is slightly shifted by a short distance T shift. Phase changes accumulated within T shift are then used to calculate the susceptibility map by using a kernel deconvolution algorithm with a regularized ℓ1 minimization. To evaluate the proposed fast spin echo method, three phantom experiments were conducted and compared to a spin echo based technique and the gold standard CT for visualizing biopsy needles and brachytherapy seeds. Compared to the spin echo based technique, the data sampling speed of the proposed method was faster by 2–4 times while still being able to accurately visualize and identify the location of the biopsy needle and brachytherapy seeds. These results were confirmed by CT images of the same devices. Results also demonstrated that the proposed fast spin echo method can achieve good visualization of the brachytherapy seeds in positive contrast and in different orientations. It is also capable of correctly differentiating brachytherapy seeds from other similar structures on conventional magnitude images.
Spin transfer torques and spin dynamics in point contacts and spin-flop tunnel junctions
Konovalenko, Alexander
2008-01-01
The first part of this thesis is an experimental study of the spin-dependent transport in magnetic point contacts. Nano-contacts are produced micromechanically, by bringing a sharpened non-magnetic (N) tip into contact with a ferromagnetic (F) film. The magnetic and magneto-transport properties of such N/F nanocontacts are studied using transport spectroscopy, spanning the ballistic, diffusive, and thermal transport regimes. Single N/F interfaces can exhibit current driven magnetic excitation...
Spin dynamics in highly frustrated pyrochlore magnets
Petit, Sylvain; Guitteny, Solène; Robert, Julien; Bonville, Pierre; Decorse, Claudia; Ollivier, Jacques; Mutka, Hannu; Mirebeau, Isabelle
2015-01-01
This paper aims at showing the complementarity between time-of-flight and triple-axis neutron scattering experiments, on the basis of two topical examples in the field of geometrical magnetic frustration. Rare earth pyrochlore magnets R2Ti2O7 (R is a rare earth) play a prominent role in this field, as they form model systems showing a rich variety of ground states, depending on the balance between dipolar, exchange interactions and crystal field. We first review the case of the XY antiferromagnet Er2 Ti2 O7. Here a transition towards a Néel state is observed, possibly induced by an order-by-disorder mechanism. Effective exchange parameters can be extracted from S(Q,ω). We then examine the case of the spin liquid Tb2 Ti2 O7. Recent experiments reveal a complex ground state characterized by "pinch points" and supporting a low energy excitation. These studies demonstrate the existence of a coupling between crystal field transitions and a transverse acoustic phonon mode.
A Flight Dynamic Model of Aircraft Spinning
1990-06-01
Australia, Library Australian Airlines, Library Qantas Airways Limited Hawker de Havilland Aust. Pty Ltd, Victoria, Library Hawker de Havilland Aust. Pty...3. MARTIN, C.A. ; Modelling Aircraft Dynamics. ARL-AERO-TECH- MEMO-400 July 1988 4. HULTBERG, R.S. ; Rotary Balance Data and Analysis for the
Dynamic magnetic hysteresis and nonlinear susceptibility of antiferromagnetic nanoparticles
Kalmykov, Yuri P.; Ouari, Bachir; Titov, Serguey V.
2016-08-01
The nonlinear ac stationary response of antiferromagnetic nanoparticles subjected to both external ac and dc fields of arbitrary strength and orientation is investigated using Brown's continuous diffusion model. The nonlinear complex susceptibility and dynamic magnetic hysteresis (DMH) loops of an individual antiferromagnetic nanoparticle are evaluated and compared with the linear regime for extensive ranges of the anisotropy, the ac and dc magnetic fields, damping, and the specific antiferromagnetic parameter. It is shown that the shape and area of the DMH loops of antiferromagnetic particles are substantially altered by applying a dc field that permits tuning of the specific magnetic power loss in the nanoparticles.
Spin Dynamics in Graphene and Graphene like Nanocarbon Doped with Nitrogen the ESR Analysis
Alegaonkar, Ashwini P; Pardeshi, Satish K; Alegaonkar, Prashant S
2013-01-01
Nano engineered spin degree of freedom in carbon system may offer desired exchange coupling with optimum spin orbit interaction which is essential, to construct solid state qubits, for fault tolerant quantum computation. The purpose of this communication is to analyze spin dynamics of, basically, four types of systems, (i) Graphene (system with inversion symmetry), (ii) Graphene like nanocarbons (GNCs, broken inversion symmetry and heterostructure, sp2 and sp3, environment), and (iii) their nitrogen doped derivatives. The spin transport data was obtained using the electron spin resonance spectroscopy (ESR) technique, carried out over 123 to 473K temperature range. Analysis of shape, linewidths of dispersion derivatives,, and g factor anisotropy has been carried out. Spin parameters such as, spin spin relaxation time, spin lattice relaxation time, spin flip parameter,spin relaxation rate,spin, momentum relaxation rate,pseudo chemical potential, density of states, effective magnetic moment, spin concentration, ...
Spinning Flight Dynamics of Frisbees, Boomerangs, Samaras, and Skipping Stones
Lorenz, Ralph D
2006-01-01
More frisbees are sold each year than baseballs, basketballs, and footballs combined. Yet these familiar flying objects have subtle and clever aerodynamic and gyrodynamic properties which are only recently being documented by wind tunnel and other studies. In common with other rotating bodies discussed in this readily accessible book, they are typically not treated in textbooks of aeronautics and the literature is scattered in a variety of places. This book develops the theme of disc-wings and spinning aerospace vehicles in parallel. Many readers will have enjoyed these vehicles and their dynamics in recreational settings, so this book will be of wide interest. In addition to spinning objects of various shapes, several exotic manned aircraft with disc platforms have been proposed and prototypes built - these include a Nazi ‘secret weapon’ and the De Havilland Avrocar, also discussed in the book. Boomerangs represent another category of spinning aerodynamic body whose behavior can only be understood by cou...
Dynamical Decoupling of a single electron spin at room temperature
Naydenov, Boris; Hall, Liam T; Shin, Chang; Fedder, Helmut; Hollenberg, Lloyd C L; Jelezko, Fedor; Wrachtrup, Jörg
2010-01-01
Here we report the increase of the coherence time T$_2$ of a single electron spin at room temperature by using dynamical decoupling. We show that the Carr-Purcell-Meiboom-Gill (CPMG) pulse sequence can prolong the T$_2$ of a single Nitrogen-Vacancy center in diamond up to 2.44 ms compared to the Hahn echo measurement where T$_2 = 390~\\mu$s. Moreover, by performing spin locking experiments we demonstrate that with CPMG the maximum possible $T_2$ is reached. On the other hand, we do not observe strong increase of the coherence time in nanodiamonds, possibly due to the short spin lattice relaxation time $T_1=100~\\mu$s (compared to T$_1$ = 5.93 ms in bulk). An application for detecting low magnetic field is demonstrated, where we show that the sensitivity using the CPMG method is improved by about a factor of two compared to the Hahn echo method.
Nonequilibrium spin glass dynamics with the Janus computer
Yllanes, David; Belletti, F.; Cruz, A.; Fernandez, L. A.; Gordillo-Guerrero, A.; Guidetti, M.; Maiorano, A.; Mantovani, F.; Marinari, E.; Martin-Mayor, V.; Monforte, J.; Munoz Sudupe, A.; Navarro, D.; Parisi, G.; Perez-Gaviro, S.; Ruiz-Lorenzo, J. J.; Schifano, S. F.; Sciretti, D.; Tarancon, A.; Tripiccione, R.
2009-03-01
The out of equilibrium evolution of the Edwards-Anderson spin glass is followed for a tenth of a second, effectively halving the (logarithmic) temporal gap between previous simulations and experiments. In fact, we have been able to make safe predictions about the behavior at experimental times, using mild extrapolations. This work has been made possible by Janus, a special purpose computer designed by our collaboration. We have thoroughly studied the spin glass correlation functions and the growth of the coherence length for L 0 lattices in 3D,using L 4,40 lattices to check for finite size effects. We present clear evidence for a replicon correlator. Our main conclusion is that these spin glasses follow non-coarsening dynamics, at least up to the experimentally relevant time scales.
Dynamic-angle spinning and double rotation of quadrupolar nuclei
Energy Technology Data Exchange (ETDEWEB)
Mueller, K.T. (Lawrence Berkeley Lab., CA (United States) California Univ., Berkeley, CA (United States). Dept. of Chemistry)
1991-07-01
Nuclear magnetic resonance (NMR) spectroscopy of quadrupolar nuclei is complicated by the coupling of the electric quadrupole moment of the nucleus to local variations in the electric field. The quadrupolar interaction is a useful source of information about local molecular structure in solids, but it tends to broaden resonance lines causing crowding and overlap in NMR spectra. Magic- angle spinning, which is routinely used to produce high resolution spectra of spin-{1/2} nuclei like carbon-13 and silicon-29, is incapable of fully narrowing resonances from quadrupolar nuclei when anisotropic second-order quadrupolar interactions are present. Two new sample-spinning techniques are introduced here that completely average the second-order quadrupolar coupling. Narrow resonance lines are obtained and individual resonances from distinct nuclear sites are identified. In dynamic-angle spinning (DAS) a rotor containing a powdered sample is reoriented between discrete angles with respect to high magnetic field. Evolution under anisotropic interactions at the different angles cancels, leaving only the isotropic evolution of the spin system. In the second technique, double rotation (DOR), a small rotor spins within a larger rotor so that the sample traces out a complicated trajectory in space. The relative orientation of the rotors and the orientation of the larger rotor within the magnetic field are selected to average both first- and second-order anisotropic broadening. The theory of quadrupolar interactions, coherent averaging theory, and motional narrowing by sample reorientation are reviewed with emphasis on the chemical shift anisotropy and second-order quadrupolar interactions experienced by half-odd integer spin quadrupolar nuclei. The DAS and DOR techniques are introduced and illustrated with application to common quadrupolar systems such as sodium-23 and oxygen-17 nuclei in solids.
Introducing spin in Schrodinger dynamics of particle motion
Zaveri, Vikram H
2007-01-01
A non-perturbative relativistic atomic theory is presented in which Dirac's theory and Schrodinger theory are shown to originate from a common wave equation. Spin is successfully introduced in Schrodinger dynamics of particle motion and the resulting energy levels of Hydrogen atom are shown to be exactly same as that of Dirac's theory. The separation of new radial and angular wave equations in spherical polar coordinates is as simple as that of the Schrodinger theory. The solutions of the angular part of the wave equation are exactly same as that of the Schrodinger theory. The new theory accounts for the energy due to spin-orbit interaction as well as for the additional potential energy due to spin and spin-orbit coupling. Spin angular momentum operator is as neatly integrated into the equation of motion as the orbital angular momentum operator. This requires modification to classical Laplacian operator. Consequently the Dirac matrices and the k operator of Dirac's theory are dispensed with. The theory also p...
Dynamics of spinning compact binaries in general relativity
Hartl, Michael David
This thesis investigates the dynamics of binary systems composed of spinning compact objects in the context of general relativity. Compact binaries are promising sources of gravitational radiation for both ground- and space-based gravitational-wave detectors. If the dynamics of these systems were chaotic, the number of waveform templates needed to match a given gravitational-wave signal would grow exponentially with increasing detection sensitivity, rendering the preferred matched filter detection method computationally impractical. It is therefore urgent to understand whether the binary dynamics can be chaotic, and, if so, how prevalent this chaos is. We first consider the dynamics of a spinning compact object orbiting a much more massive rotating black hole, as modeled by the Papapetrou equations in Kerr spacetime. We find that many initial conditions lead to positive Lyapunov exponents, indicating chaotic dynamics. Despite the formal existence of chaotic solutions, we find that chaos occurs only for physically unrealistic values of the small body's spin. As a result, chaos will not affect theoretical templates in the extreme mass-ratio limit for which the Papapetrou equations are valid. We next consider the dynamics of spinning black-hole binaries, as modeled by the post-Newtonian (PN) equations, which are valid for orbital velocities much smaller than the speed of light. We study thoroughly the special case of quasi-circular orbits with comparable mass ratios. Our survey shows that chaos occurs in a negligible fraction of possible configurations, and only for such small radii that the PN approximation is likely to be invalid. As a result, at least in the case of comparable mass black-hole binaries, theoretical templates will not be significantly affected by chaos. In a final, self-contained chapter, we discuss various methods for the calculation of Lyapunov exponents in systems of ordinary differential equations. We introduce several new techniques applicable
Chaos and dynamics of spinning particles in Kerr spacetime
Han, Wenbiao
2008-09-01
We study chaos dynamics of spinning particles in Kerr spacetime of rotating black holes use the Papapetrou equations by numerical integration. Because of spin, this system exists many chaos solutions, and exhibits some exceptional dynamic character. We investigate the relations between the orbits chaos and the spin magnitude S, pericenter, polar angle and Kerr rotation parameter a by means of a kind of brand new Fast Lyapulov Indicator (FLI) which is defined in general relativity. The classical definition of Lyapulov exponent (LE) perhaps fails in curve spacetime. And we emphasize that the Poincaré sections cannot be used to detect chaos for this case. Via calculations, some new interesting conclusions are found: though chaos is easier to emerge with bigger S, but not always depends on S monotonically; the Kerr parameter a has a contrary action on the chaos occurrence. Furthermore, the spin of particles can destroy the symmetry of the orbits about the equatorial plane. And for some special initial conditions, the orbits have equilibrium points.
Institute of Scientific and Technical Information of China (English)
GE Rong-Chun; LI Chuan-Feng; GUO Guang-Can
2012-01-01
We investigate the dynamics of entanglement,quantum correlation and classical correlation for the one-dimensional XY model in a transverse magnetic field.With the initial state polarized along the z axis,we find that the first maximum of the classical correlation between the nearest neighbor sites peaks around the critical point for large anisotropy parameter.It may indicate the quantum phase transition.For all kinds of correlation,we find that their behaviors between the nearest neighbor sites are significantly different from those of the next-nearestneighbor sites.
Quantum spin dynamics in a spin-orbit-coupled Bose-Einstein condensate
Poon, Ting Fung Jeffrey; Liu, Xiong-Jun
2016-06-01
Spin-orbit-coupled bosons can exhibit rich equilibrium phases at low temperature and in the presence of particle-particle interactions. In the case with a 1D synthetic spin-orbit interaction, it has been observed that the ground state of a Bose gas can be a normal phase, stripe phase, or magnetized phase in different parameter regimes. The magnetized states are doubly degenerate and consist of a many-particle two-state system. In this work, we investigate the nonequilibrium quantum dynamics by switching on a simple one-dimensional optical lattice potential as external perturbation to induce resonant couplings between the magnetized phases, and predict a quantum spin dynamics which cannot be obtained in the single-particle systems. In particular, due to particle-particle interactions, the transition of the Bose condensate from one magnetized phase to the other is forbidden when the external perturbation strength is less than a critical value, and a full transition can occur only when the perturbation exceeds such critical strength. This phenomenon manifests itself a dynamical phase transition, with the order parameter defined by the time-averaged magnetization over an oscillation period, and the critical point behavior being exactly solvable. The thermal fluctuations are also considered in detail. From numerical simulations and exact analytic studies we show that the predicted many-body effects can be well observed with the current experiments.
Zeisner, J.; Brockmann, M.; Zimmermann, S.; Weiße, A.; Thede, M.; Ressouche, E.; Povarov, K. Yu.; Zheludev, A.; Klümper, A.; Büchner, B.; Kataev, V.; Göhmann, F.
2017-07-01
We compare theoretical results for electron spin resonance (ESR) properties of the Heisenberg-Ising Hamiltonian with ESR experiments on the quasi-one-dimensional magnet Cu (py) 2Br2 (CPB). Our measurements were performed over a wide frequency and temperature range giving insight into the spin dynamics, spin structure, and magnetic anisotropy of this compound. By analyzing the angular dependence of ESR parameters (resonance shift and linewidth) at room temperature, we show that the two weakly coupled inequivalent spin-chain types inside the compound are well described by Heisenberg-Ising chains with their magnetic anisotropy axes perpendicular to the chain direction and almost perpendicular to each other. We further determine the full g tensor from these data. In addition, the angular dependence of the linewidth at high temperatures gives us access to the exponent of the algebraic decay of a dynamical correlation function of the isotropic Heisenberg chain. From the temperature dependence of static susceptibilities, we extract the strength of the exchange coupling (J /kB=52.0 K ) and the anisotropy parameter (δ ≈-0.02 ) of the model Hamiltonian. An independent compatible value of δ is obtained by comparing the exact prediction for the resonance shift at low temperatures with high-frequency ESR data recorded at 4 K . The spin structure in the ordered state implied by the two (almost) perpendicular anisotropy axes is in accordance with the propagation vector determined from neutron scattering experiments. In addition to undoped samples, we study the impact of partial substitution of Br by Cl ions on spin dynamics. From the dependence of the ESR linewidth on the doping level, we infer an effective decoupling of the anisotropic component J δ from the isotropic exchange J in these systems.
The quark susceptibility in a generalized dynamical quasiparticle model
Berrehrah, Hamza; Bratkovskaya, Elena; Steinert, Thorsten
2015-01-01
The quark susceptibility $\\chi_q$ at zero and finite quark chemical potential provides a critical benchmark to determine the quark-gluon-plasma (QGP) degrees of freedom in relation to the results from lattice QCD (lQCD) in addition to the equation of state and transport coefficients. Here we extend the familiar dynamical-quasiparticle model (DQPM) to partonic propagators that explicitly depend on the three-momentum with respect to the partonic medium at rest in order to match perturbative QCD (pQCD) at high momenta. Within the extended dynamical-quasi-particle model (DQPM$^*$) we reproduce simultaneously the lQCD results for the quark number density and susceptibility and the QGP pressure at zero and finite (but small) chemical potential $\\mu_q$. The shear viscosity $\\eta$ and the electric conductivity $\\sigma_e$ from the extended quasiparticle model (DQPM$^*$) also turn out in close agreement with lattice results for $\\mu_q$ =0. The DQPM$^*$, furthermore, allows to evaluate the momentum $p$, temperature $T$ ...
Matsuno, Genki; Kobayashi, Akito
2017-01-01
The nontrivial properties of interband spin fluctuations are studied by the random phase approximation in a Hubbard model describing the molecular conductor α-(BEDT-TTF)2I3, where wave functions are based on the four sublattices named A, A', B, and C in a two-dimensional BEDT-TTF molecular plane. It is found that the ferrimagnetic polarization observed by a recent NMR measurement emerges only if there exist cross terms among intra- and inter-band irreducible susceptibility matrix elements in the presence of the on-site Coulomb interaction U. It is also found that the nontrivial sign of the interband components of the spin susceptibility, being negative only for the B sublattice, is closely related to the characteristic phase structure of wave functions in the Dirac fermion system with multisublattices. The negative value of the spin susceptibility on the B sublattice observed in the experiment is associated with this negative interband susceptibility, which comes from the excitations in the gentle-slope region of the energy dispersion connecting the Dirac points with saddle points in the first Brillouin zone.
Spacetime Dynamics from Spin Dynamics: Cosmological Constant and Neutrino Mass
Crawford, James
2003-04-01
Two fundamental unresolved issues in gravitational physics are the origin of the cosmological constant (dark energy), whose existence is suggested by the observed acceleration of the universe, and the origin of the particle masses, which we now know includes the neutrinos. Since all matter particles are represented by spinor fields, it seems natural to inquire whether the gravitational interaction of the spinor fields can illuminate these issues. Therefore we consider the possibility that the spin curvature is fundamental, and show that by relaxing the Schrödinger condition (covariant constancy of the Dirac matrices) it is possible to obtain both spacetime curvature and torsion as parts of the spin curvature. We assume a scale invariant Lagrangian composed of the standard Yang-Mills Lagrangian for the spin curvature and the massless Dirac Lagrangian for the spinors. An exact vacuum cosmological solution to the associated field equations is found which exhibits exponential acceleration of the universe and gives a minimum mass for all spinors.
Five-Axis, Three-Magnetic-Bearing Dynamic Spin Rig
Morrison, Carlos R.; Provenza, Andrew; Kurkov, Anatole; Mehmed, Oral; Johnson, Dexter; Montague, Gerald; Duffy, Kirsten; Jansen, Ralph
2005-01-01
The Five-Axis, Three-Magnetic-Bearing Dynamic Spin Rig is an apparatus for vibration testing of turbomachine blades in a vacuum at rotational speeds from 0 to 40,000 rpm. This rig includes (1) a vertically oriented shaft on which is mounted an assembly comprising a rotor holding the blades to be tested, (2) two actively controlled heteropolar radial magnetic bearings at opposite ends of the shaft, and (3) an actively controlled magnetic thrust bearing at the upper end of the shaft. This rig is a more capable successor to a prior apparatus, denoted the Dynamic Spin Rig (DSR), that included a vertically oriented shaft with a mechanical thrust bearing at the upper end and a single actively controlled heteropolar radial magnetic bearing at the lower end.
Optimal control of stochastic magnetization dynamics by spin current
Wang, Yong; Zhang, Fu-Chun
2013-05-01
Fluctuation-induced stochastic magnetization dynamics plays an important role in spintronics devices. Here we propose that it can be optimally controlled by spin currents to minimize or maximize the Freidlin-Wentzell action functional of the system hence to increase or decrease the probability of the large fluctuations. We apply this method to study the thermally activated magnetization switching problem and to demonstrate the merits of the optimal control strategy.
Exciton spin dynamics in ZnO epilayers
Energy Technology Data Exchange (ETDEWEB)
Lagarde, D.; Lombez, L.; Balocchi, A.; Renucci, P.; Carrere, H.; Amand, T.; Marie, X. [Laboratoire de Nanophysique, Magnetisme et Optoelectronique, INSA, 135 avenue de Rangueil, 31077 Toulouse Cedex 4 (France); Mei, Z.X.; Du, X.L.; Xue, Q.K. [Institute of Physics, Chinese Academy of Sciences and National Center for Nano-Science and Technology, Beijing 100080 (China)
2007-07-01
We used time-resolved optical orientation experiments to study the low temperature spin dynamics of a ZnO epilayer. The sample shows a circular polarisation of the donor-bound exciton of 11% with a decay time of 275 ps. A very narrow spectral dependence of the initial polarisation and a rapid decrease of the polarisation decay time with temperature are also observed. (copyright 2007 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)
Spin dynamics in the quantum spin system KCu{sub 5}V{sub 3}O{sub 13}
Energy Technology Data Exchange (ETDEWEB)
Klauss, H.-H.; Lemmens, P.; Birke, M.; Baabe, D.; Mienert, D.; Litterst, F.J.; Amato, A.; Pommer, J.; Ionescu, A.; Choi, K.-Y.; Guentherodt, G.; Kageyama, H.; Hiroi, Z.; Takigawa, M
2003-02-01
The complex Oxo-Cu-vanadate KCu{sub 5}V{sub 3}O{sub 13} with 5 independent Cu-sites (s=((1)/(2))) per unit cell has an exchange topology described as a ladder of spin tetrahedra or triangles. Magnetic susceptibility measurements on single crystals show a steplike anomaly at 213 K and an antiferromagnetic transition at 7.5 K. ZF {mu}SR reveals only nuclear relaxation above 10 K and two spontaneous precession signals in the long range ordered regime. Below 3.7 K, a spin reorientation leads to a broad frequency distribution typical for an incommensurate spin structure.
Probing of incomplete fusion dynamics by spin-distribution measurement
Energy Technology Data Exchange (ETDEWEB)
Singh, Pushpendra P. [Accelerator Laboratory, Department of Physics, A.M. University, Aligarh (UP) 202002 (India); NP Group, Inter-University Accelerator Center, PO Box 10502, New Delhi 110067 (India)], E-mail: pushpendrapsingh@gmail.com; Singh, B.P. [Accelerator Laboratory, Department of Physics, A.M. University, Aligarh (UP) 202002 (India)], E-mail: bpsinghamu@gmail.com; Sharma, M.K.; Gupta, Unnati [Accelerator Laboratory, Department of Physics, A.M. University, Aligarh (UP) 202002 (India); Kumar, Rakesh [NP Group, Inter-University Accelerator Center, PO Box 10502, New Delhi 110067 (India); Singh, D. [Accelerator Laboratory, Department of Physics, A.M. University, Aligarh (UP) 202002 (India); Singh, R.P.; Murlithar, S. [NP Group, Inter-University Accelerator Center, PO Box 10502, New Delhi 110067 (India); Ansari, M.A.; Prasad, R. [Accelerator Laboratory, Department of Physics, A.M. University, Aligarh (UP) 202002 (India); Bhowmik, R.K. [NP Group, Inter-University Accelerator Center, PO Box 10502, New Delhi 110067 (India)], E-mail: ranjan@iuac.ernet.in
2009-01-12
Aiming to probe incomplete fusion dynamics in {sup 16}O + {sup 169}Tm system, spin-distributions of various reaction products populated via xn-, {alpha}/2{alpha}xn-channels have been measured at E{approx}5.6MeV/nucleon. Prompt {gamma}-rays in coincidence with fast charged particles (Z=1,2) have been recorded to achieve the information about involved reaction processes on the basis of their experimentally observed spin-populations during de-excitation. The experimentally observed spin-distributions for direct-{alpha}-emitting channels (associated with incomplete fusion) have been found to be distinctly different than that observed for fusion-evaporation (complete fusion) channels. The mean value of driving input angular momenta associated with various direct-{alpha}/2{alpha}xn-channels have been found to be higher than that observed for fusion-evaporation xn/{alpha}xn-channels, and increases with direct-{alpha}-multiplicity in forward cone. Experimentally measured, normalized production yields of fusion-evaporation xn/{alpha}xn-channels have been found to be in good agreement with the predictions of theoretical model code PACE4. Further, in order to understand the feeding probability in both complete and incomplete fusion reaction products, an attempt has been made to generate feeding intensity profiles from spin-distribution data. It has been observed that the complete fusion products are strongly fed over a broad spin range, while incomplete fusion products are found to be less fed and/or the population of lower spin states are strongly hindered.
Second post-Newtonian Lagrangian dynamics of spinning compact binaries
Energy Technology Data Exchange (ETDEWEB)
Huang, Li; Wu, Xin [Nanchang University, Department of Physics and Institute of Astronomy, Nanchang (China); Ma, DaZhu [Hubei University for Nationalities, School of Science, Enshi (China)
2016-09-15
The leading-order spin-orbit coupling is included in a post-Newtonian Lagrangian formulation of spinning compact binaries, which consists of the Newtonian term, first post-Newtonian (1PN) and 2PN non-spin terms and 2PN spin-spin coupling. This leads to a 3PN spin-spin coupling occurring in the derived Hamiltonian. The spin-spin couplings are mainly responsible for chaos in the Hamiltonians. However, the 3PN spin-spin Hamiltonian is small and has different signs, compared with the 2PN spin-spin Hamiltonian equivalent to the 2PN spin-spin Lagrangian. As a result, the probability of the occurrence of chaos in the Lagrangian formulation without the spin-orbit coupling is larger than that in the Lagrangian formulation with the spin-orbit coupling. Numerical evidences support this claim. (orig.)
SPILADY: A parallel CPU and GPU code for spin-lattice magnetic molecular dynamics simulations
Ma, Pui-Wai; Dudarev, S. L.; Woo, C. H.
2016-10-01
Spin-lattice dynamics generalizes molecular dynamics to magnetic materials, where dynamic variables describing an evolving atomic system include not only coordinates and velocities of atoms but also directions and magnitudes of atomic magnetic moments (spins). Spin-lattice dynamics simulates the collective time evolution of spins and atoms, taking into account the effect of non-collinear magnetism on interatomic forces. Applications of the method include atomistic models for defects, dislocations and surfaces in magnetic materials, thermally activated diffusion of defects, magnetic phase transitions, and various magnetic and lattice relaxation phenomena. Spin-lattice dynamics retains all the capabilities of molecular dynamics, adding to them the treatment of non-collinear magnetic degrees of freedom. The spin-lattice dynamics time integration algorithm uses symplectic Suzuki-Trotter decomposition of atomic coordinate, velocity and spin evolution operators, and delivers highly accurate numerical solutions of dynamic evolution equations over extended intervals of time. The code is parallelized in coordinate and spin spaces, and is written in OpenMP C/C++ for CPU and in CUDA C/C++ for Nvidia GPU implementations. Temperatures of atoms and spins are controlled by Langevin thermostats. Conduction electrons are treated by coupling the discrete spin-lattice dynamics equations for atoms and spins to the heat transfer equation for the electrons. Worked examples include simulations of thermalization of ferromagnetic bcc iron, the dynamics of laser pulse demagnetization, and collision cascades.
Dynamical TAP equations for non-equilibrium Ising spin glasses
DEFF Research Database (Denmark)
Roudi, Yasser; Hertz, John
2011-01-01
equations take the form of self consistent equations for magnetizations at time t+1, given the magnetizations at time t. In the asynchronously updated model, the TAP equations determine the time derivatives of the magnetizations at each time, again via self consistent equations, given the current values......We derive and study dynamical TAP equations for Ising spin glasses obeying both synchronous and asynchronous dynamics using a generating functional approach. The system can have an asymmetric coupling matrix, and the external fields can be time-dependent. In the synchronously updated model, the TAP...
Pulse Control Assisted Dynamical Decoupling in a Central Spin Model
Li, Zhao-Yan; Wei, Yong-Bo; Wang, Zhao-Ming; Gu, Yong-Jian; Li, Wen-Dong; Ma, Xiao-Ping
2017-02-01
We study pulse control assisted dynamical decoupling through a central spin model in a total Hilbert space. We find that the effective decoupling can be realized by applying a sequence of external pulses. Compared with the bang-bang control which needs infinite strength and infinitesimal short pulses, we show that there is a large parameter space that allows an effective nonperturbative dynamical control. Furthermore, our numerical calculation shows that the reliability can be held for random pulses, such as random pulse time interval or random strength.
Cloud Susceptibilities to Ice Nuclei: Microphysical Effects and Dynamical Feedbacks
Paukert, Marco; Hoose, Corinna
2015-04-01
The impact of aerosols on cloud properties is currently not well established. This is largely attributed to the interdependencies of aerosols and cloud microphysical processes, among which primary ice formation contributes to considerable uncertainties. Although it is known that in a large range of thermodynamic conditions aerosol particles are required to initiate ice formation, identifying and characterizing the effect of specific ice nuclei is among current scientific efforts. Here we attempt to quantify the change of cloud properties with varying aerosol background concentrations. We adapt the concept of susceptibilities for mixed-phase and ice clouds, defining the susceptibility as the derivation of a macrophysical quantity with respect to ice nucleating aerosol concentrations. A focus of our study is the use of different model approaches in order to identify the distinct contributions of both cloud microphysics and cloud-dynamical feedbacks to the overall susceptibility. The classical method is the direct comparison of two independent model runs, where the whole range of microphysical and cloud-dynamical feedbacks contributes to different cloud properties in a perturbed simulation. Our alternative method relies on a single simulation which incorporates multiple executions of the microphysical scheme within the same time step, each "perturbed microphysics" scheme with varying aerosol concentrations and an additional set of cloud particle tracers. Since in the latter case the model dynamics are held constant and only microphysical feedbacks contribute to the properties of perturbed clouds, we can distinguish between the pure microphysical effect and the dynamical enhancement or suppression. For a persistent Arctic mixed-phase stratocumulus cloud layer which is expected to be particularly sensitive to feedback cycles, we show an enhancement of the cloud susceptibility to ice nucleating particles by dynamics of around 50%, but a decay of the enhancement with time
Nonlinear Dynamics of Dipoles in Microtubules: Pseudo-Spin Model
Nesterov, Alexander I; Berman, Gennady P; Mavromatos, Nick E
2016-01-01
We perform a theoretical study of the dynamics of the electric field excitations in a microtubule by taking into consideration the realistic cylindrical geometry, dipole-dipole interactions of the tubulin-based protein heterodimers, the radial electric field produced by the solvent, and a possible degeneracy of energy states of individual heterodimers. The consideration is done in the frames of the classical pseudo-spin model. We derive the system of nonlinear dynamical ordinary differential equations of motion for interacting dipoles, and the continuum version of these equations. We obtain the solutions of these equations in the form of snoidal waves, solitons, kinks, and localized spikes. Our results will help to a better understanding of the functional properties of microtubules including the motor protein dynamics and the information transfer processes. Our considerations are based on classical dynamics. Some speculations on the role of possible quantum effects are also made.
Lengthscale dependence of dynamic four-point susceptibilities in glass formers
Chandler, David; Juan P Garrahan; Jack, Robert L.; Maibaum, Lutz; Pan, Albert C.
2006-01-01
Dynamical four-point susceptibilities measure the extent of spatial correlations in the dynamics of glass forming systems. We show how these susceptibilities depend on the length scales that necessarily form part of their definition. The behaviour of these susceptibilities is estimated by means of an analysis in terms of renewal processes within the context of dynamic facilitation. The analytic results are confirmed by numerical simulations of an atomistic model glass-former, and of two kinet...
Coherent spin-rotational dynamics of oxygen super rotors
Milner, Alexander A; Milner, Valery
2014-01-01
We use state- and time-resolved coherent Raman spectroscopy to study the rotational dynamics of oxygen molecules in ultra-high rotational states. While it is possible to reach rotational quantum numbers up to $N \\approx 50$ by increasing the gas temperature to 1500 K, low population levels and gas densities result in correspondingly weak optical response. By spinning O$_2$ molecules with an optical centrifuge, we efficiently excite extreme rotational states with $N\\leqslant 109$ in high-density room temperature ensembles. Fast molecular rotation results in the enhanced robustness of the created rotational wave packets against collisions, enabling us to observe the effects of weak spin-rotation coupling in the coherent rotational dynamics of oxygen. The decay rate of spin-rotation coherence due to collisions is measured as a function of the molecular angular momentum and explained in terms of the general scaling law. We find that at high values of $N$, the rotational decoherence of oxygen is much faster than t...
precession: Dynamics of spinning black-hole binaries with python
Gerosa, Davide; Kesden, Michael
2016-06-01
We present the numerical code precession, a new open-source python module to study the dynamics of precessing black-hole binaries in the post-Newtonian regime. The code provides a comprehensive toolbox to (i) study the evolution of the black-hole spins along their precession cycles, (ii) perform gravitational-wave-driven binary inspirals using both orbit-averaged and precession-averaged integrations, and (iii) predict the properties of the merger remnant through fitting formulas obtained from numerical-relativity simulations. precession is a ready-to-use tool to add the black-hole spin dynamics to larger-scale numerical studies such as gravitational-wave parameter estimation codes, population synthesis models to predict gravitational-wave event rates, galaxy merger trees and cosmological simulations of structure formation. precession provides fast and reliable integration methods to propagate statistical samples of black-hole binaries from/to large separations where they form to/from small separations where they become detectable, thus linking gravitational-wave observations of spinning black-hole binaries to their astrophysical formation history. The code is also a useful tool to compute initial parameters for numerical-relativity simulations targeting specific precessing systems. precession can be installed from the python Package Index, and it is freely distributed under version control on github, where further documentation is provided.
Spin Particle in an Absorbing Environment
Amooshahi, M.
2015-10-01
The quantum dynamics of a localized spin Particle interacting with an absorbing environment is investigated. The quantum Langevin-Schrödinger equation for spin is obtained. The susceptibility function of the environment is calculated in terms of the coupling function of the spin and the environment. it is shown that the susceptibility function satisfies the Kramers-Kronig relations. Spontaneous emission and the shift frequency of the spin is obtained in terms of the imaginary part of the susceptibility function in frequency domain. Some transition probabilities between the spin states are calculated when the absorbing environment is in the thermal state.
Dynamics and decoherence of a single spin-qubit in a tunable environment
Ratschbacher, L; Carcagni, L; Silver, J M; Zipkes, C; Köhl, M
2013-01-01
We report on the immersion of a spin-qubit encoded in a single trapped ion into a spin-polarized neutral atom environment, which possesses both continuous (motional) and discrete (spin) degrees of freedom. The environment is widely tunable and offers the possibility of a precise microscopic description, both of which allows us to understand dynamics and decoherence from first principles. We observe the spin dynamics of the qubit and measure the decoherence times (T1 and T2), which are determined by the spin-exchange interaction as well as by an unexpectedly strong spin-nonconserving coupling mechanism.
Energy Technology Data Exchange (ETDEWEB)
Melnikov, N.B., E-mail: melnikov@cs.msu.su [Lomonosov Moscow State University, Moscow 119991 (Russian Federation); Reser, B.I., E-mail: reser@imp.uran.ru [Miheev Institute of Metal Physics, Ural Branch of Russian Academy of Sciences, Ekaterinburg 620990 (Russian Federation); Paradezhenko, G.V., E-mail: gparadezhenko@cs.msu.su [Lomonosov Moscow State University, Moscow 119991 (Russian Federation)
2016-08-01
To study the spin-density correlations in the ferromagnetic metals above the Curie temperature, we relate the spin correlator and neutron scattering cross-section. In the dynamic spin-fluctuation theory, we obtain explicit expressions for the effective and local magnetic moments and spatial spin-density correlator. Our theoretical results are demonstrated by the example of bcc Fe. The effective and local moments are found in good agreement with results of polarized neutron scattering experiment over a wide temperature range. The calculated short-range order is small (up to 4 Å) and slowly decreases with temperature.
2016-01-01
We present a new open-source Python package for exact diagonalization and quantum dynamics of spin(-photon) chains, called QuSpin, supporting the use of various symmetries and (imaginary) time evolution for chains up to 32 sites in length. The package is well-suited to study, among others, quantum quenches at finite and infinite times, the Eigenstate Thermalisation hypothesis, many-body localisation and other dynamical phase transitions, periodically-driven (Floquet) systems, adiabatic and co...
Random walk approach to spin dynamics in a two-dimensional electron gas with spin-orbit coupling
Energy Technology Data Exchange (ETDEWEB)
Yang, Luyi; Orenstein, J.; Lee, Dung-Hai
2010-09-27
We introduce and solve a semiclassical random walk (RW) model that describes the dynamics of spin polarization waves in zinc-blende semiconductor quantum wells. We derive the dispersion relations for these waves, including the Rashba, linear and cubic Dresselhaus spin-orbit interactions, as well as the effects of an electric field applied parallel to the spin polarization wave vector. In agreement with calculations based on quantum kinetic theory [P. Kleinert and V. V. Bryksin, Phys. Rev. B 76, 205326 (2007)], the RW approach predicts that spin waves acquire a phase velocity in the presence of the field that crosses zero at a nonzero wave vector, q{sub 0}. In addition, we show that the spin-wave decay rate is independent of field at q{sub 0} but increases as (q-q{sub 0}){sup 2} for q {ne} q{sub 0}. These predictions can be tested experimentally by suitable transient spin grating experiments.
Sayad, Mohammad; Potthoff, Michael
2015-11-01
The real-time dynamics of a classical spin in an external magnetic field and local exchange coupled to an extended one-dimensional system of non-interacting conduction electrons is studied numerically. Retardation effects in the coupled electron-spin dynamics are shown to be the source for the relaxation of the spin in the magnetic field. Total energy and spin is conserved in the non-adiabatic process. Approaching the new local ground state is therefore accompanied by the emission of dispersive wave packets of excitations carrying energy and spin and propagating through the lattice with Fermi velocity. While the spin dynamics in the regime of strong exchange coupling J is rather complex and governed by an emergent new time scale, the motion of the spin for weak J is regular and qualitatively well described by the Landau-Lifschitz-Gilbert (LLG) equation. Quantitatively, however, the full quantum-classical hybrid dynamics differs from the LLG approach. This is understood as a breakdown of weak-coupling perturbation theory in J in the course of time. Furthermore, it is shown that the concept of the Gilbert damping parameter is ill-defined for the case of a one-dimensional system.
Cone Algorithm of Spinning Vehicles under Dynamic Coning Environment
Directory of Open Access Journals (Sweden)
Shuang-biao Zhang
2015-01-01
Full Text Available Due to the fact that attitude error of vehicles has an intense trend of divergence when vehicles undergo worsening coning environment, in this paper, the model of dynamic coning environment is derived firstly. Then, through investigation of the effect on Euler attitude algorithm for the equivalency of traditional attitude algorithm, it is found that attitude error is actually the roll angle error including drifting error and oscillating error, which is induced directly by dynamic coning environment and further affects the pitch angle and yaw angle through transferring. Based on definition of the cone frame and cone attitude, a cone algorithm is proposed by rotation relationship to calculate cone attitude, and the relationship between cone attitude and Euler attitude of spinning vehicle is established. Through numerical simulations with different conditions of dynamic coning environment, it is shown that the induced error of Euler attitude fluctuates by the variation of precession and nutation, especially by that of nutation, and the oscillating frequency of roll angle error is twice that of pitch angle error and yaw angle error. In addition, the rotation angle is more competent to describe the spinning process of vehicles under coning environment than Euler angle gamma, and the real pitch angle and yaw angle are calculated finally.
On the spin-axis dynamics of a Moonless Earth
Energy Technology Data Exchange (ETDEWEB)
Li, Gongjie; Batygin, Konstantin, E-mail: gli@cfa.harvard.edu [Harvard-Smithsonian Center for Astrophysics, The Institute for Theory and Computation, 60 Garden Street, Cambridge, MA 02138 (United States)
2014-07-20
The variation of a planet's obliquity is influenced by the existence of satellites with a high mass ratio. For instance, Earth's obliquity is stabilized by the Moon and would undergo chaotic variations in the Moon's absence. In turn, such variations can lead to large-scale changes in the atmospheric circulation, rendering spin-axis dynamics a central issue for understanding climate. The relevant quantity for dynamically forced climate change is the rate of chaotic diffusion. Accordingly, here we re-examine the spin-axis evolution of a Moonless Earth within the context of a simplified perturbative framework. We present analytical estimates of the characteristic Lyapunov coefficient as well as the chaotic diffusion rate and demonstrate that even in absence of the Moon, the stochastic change in Earth's obliquity is sufficiently slow to not preclude long-term habitability. Our calculations are consistent with published numerical experiments and illustrate the putative system's underlying dynamical structure in a simple and intuitive manner.
Dynamic nuclear polarization studies on deuterated nitroxyl spin probes.
David Jebaraj, D; Utsumi, Hideo; Milton Franklin Benial, A
2017-10-01
Detailed dynamic nuclear polarization and electron spin resonance studies were carried out for 3-carbamoyl-2,2,5,5-tetramethyl-pyrrolidine-1-oxyl, 3-carboxy-2,2,5,5-tetramethyl-pyrrolidine-1-oxyl,3-methoxycarbonyl-2,2,5,5-tetramethy pyrolidine-1-oxyl nitroxyl radicals and their corresponding deuterated nitroxyl radicals, used in Overhauser-enhanced magnetic resonance imaging for the first time. The dynamic nuclear polarization parameters such as dynamic nuclear polarization (DNP) factor, longitudinal relaxivity, saturation parameter, leakage factor and coupling factor were estimated for deuterated nitroxyl radicals. DNP enhancement increases with agent concentration up to 3 mm and decreases above 3 mm. The proton spin-lattice relaxation time and the longitudinal relaxivity parameters were estimated. The leakage factor increases with increasing agent concentration up to 3 mm and reaches plateau in the region 3-5 mm. The coupling parameter shows the interaction between the electron and nuclear spins to be mainly dipolar in origin. DNP spectrum exhibits that the full width at half maximum values are higher for undeuterated nitroxyl radicals compared with deuterated nitroxyl radicals, which leads to the increase in DNP enhancement. The ESR parameters such as, the line width, line shape, signal intensity ratio, rotational correlation time, hyperfine coupling constant and g-factor were calculated. The narrow line width was observed for deuterated nitroxyl radicals compared with undeuterated nitroxyl radicals, which leads to the higher saturation parameter value and DNP enhancement. The novelty of the work permits clear understanding of the DNP parameters determining the higher DNP enhancement compared with the undeuterated nitroxyl radicals. Copyright © 2017 John Wiley & Sons, Ltd. Copyright © 2017 John Wiley & Sons, Ltd.
Local factorisation of the dynamics of quantum spin systems
Bachmann, Sven; Bluhm, Andreas
2017-07-01
Motivated by the study of area laws for the entanglement entropy of gapped ground states of quantum spin systems and their stability, we prove that the unitary cocycle generated by a local time-dependent Hamiltonian can be approximated, for any finite set X, by a tensor product of the corresponding unitaries in X and its complement, multiplied by a dynamics strictly supported in the neighbourhood of the surface ∂ X . The error decays almost exponentially in the size of the neighbourhood and grows with the square of the area |∂ X |2.
Energy Technology Data Exchange (ETDEWEB)
Bourges, P.; Sidis, Y. [Laboratoire Leon Brillouin (LLB) - Centre d`Etudes de Saclay, 91 - Gif-sur-Yvette (France); Regnault, L.P.; Henry, J.Y.; Burlet, P. [CEA Centre d`Etudes de Grenoble, 38 (France). Dept. de Recherche Fondamentale sur la Matiere Condensee; Vettier, C. [European Synchrotron Research Facility, 38 -Grenoble (France)
1994-12-31
The spin dynamics in single-crystals of YBa{sub 2}Cu{sub 3}O{sub 6+x} has been successfully investigated, by inelastic neutron scattering (INS) experiments, as a function of temperature in the metallic state over the whole doping range from the weakly-doped to the heavily-doped and the over-doped regimes. Dynamical AF-correlations persist in all the metallic states. The imaginary part of the magnetic susceptibility, {chi}{sup ``}, consists of two contributions which have different doping and temperature dependences. At low temperature, {chi}{sup ``} exhibits an energy gap in any superconducting samples which becomes much weaker close to the insulating-metallic transition. To emphasize the characteristic features of the spin dynamics in YBCO, INS results obtained elsewhere are compared with the experiments. Several theoretical approaches, which intend to describe the energy lineshape of the dynamical magnetic susceptibility, are also discussed. (authors). 6 figs., 51 refs.
Dynamics of open quantum spin systems : An assessment of the quantum master equation approach
Zhao, P.; De Raedt, H.; Miyashita, S.; Jin, F.; Michielsen, K.
2016-01-01
Data of the numerical solution of the time-dependent Schrodinger equation of a system containing one spin-1/2 particle interacting with a bath of up to 32 spin-1/2 particles is used to construct a Markovian quantum master equation describing the dynamics of the system spin. The procedure of obtainin
Some Aspects of Dynamics of Nitrogen-14 Quadrupolar Spin-System
Energy Technology Data Exchange (ETDEWEB)
Rudakov, T. N., E-mail: trudakov@qrsciences.com; Hayes, P. A.; Chisholm, W. P. [QRSciences Limited (Australia)
2004-12-15
This is a study of the behaviour of nuclear quadrupole resonance (NQR) signals in the 'observation windows' of multi-pulse sequence for a nitrogen-14 spin-system. Obtained results revealed steady state (SS) and spin echo (SE) components of the signal. The results contribute to the understanding the dynamic properties of the quadrupolar spin-system.
Dynamical supersymmetry of the spin particle-magnetic field interaction
Energy Technology Data Exchange (ETDEWEB)
Ngome, J-P; Horvathy, P A [Laboratoire de Mathematiques et de Physique Theorique, Universite Francois-Rabelais Tours, Federation Denis Poisson, CNRS Parc de Grandmont, 37200 Tours (France); Van Holten, J W, E-mail: juste.ngome@lmpt.univ-tours.f, E-mail: horvathy@lmpt.univ-tours.f, E-mail: t32@nikhef.n [NIKHEF, PO Box 41882, 1009 DB Amsterdam (Netherlands)
2010-07-16
We study the dynamical and supersymmetries of a fermion in a D = d = 3-dimensional monopole background. The Hamiltonian also involves an additional spin-orbit coupling term, which is parameterized by the gyromagnetic ratio. We construct the superinvariants associated with the system using a SUSY extension of a previously proposed algorithm, based on Grassmann-valued Killing tensors. Conserved quantities arise for certain definite values of the gyromagnetic factor: N=1 SUSY requires g = 2; a Kepler-type dynamical symmetry only arises, however, for the anomalous values g = 0 and g = 4. The two anomalous systems can be unified into an N=2 SUSY system built by doubling the number of Grassmann variables. For D = d = 2, the planar system also exhibits an N=2 supersymmetry without Grassmann variable doubling.
PRECESSION. Dynamics of spinning black-hole binaries with python
Gerosa, Davide
2016-01-01
We present the numerical code PRECESSION: a new open-source python module to study the dynamics of precessing black-hole binaries in the post-Newtonian regime. The code provides a comprehensive toolbox to (i) study the evolution of the black-hole spins along their precession cycles, (ii) perform gravitational-wave driven binary inspirals using both orbit-averaged and precession-averaged integrations, and (iii) predict the properties of the merger remnant through fitting formulae obtained from numerical-relativity simulations. PRECESSION is a ready-to-use tool to add the black-hole spin dynamics to larger-scale numerical studies such as gravitational-wave parameter estimation codes, population synthesis models to predict gravitational-wave event rates, galaxy merger trees and cosmological simulations of structure formation. PRECESSION provides fast and reliable integration methods to propagate statistical samples of black-hole binaries from/to large separations where they form to/from small separations where t...
Storch, Natalia I.; Lai, Dong; Anderson, Kassandra R.
2017-03-01
Many exoplanetary systems containing hot Jupiters (HJs) exhibit significant misalignment between the spin axes of the host stars and the orbital angular momentum axes of the planets ('spin-orbit misalignment'). High-eccentricity migration involving Lidov-Kozai oscillations of the planet's orbit induced by a distant perturber is a possible channel for producing such misaligned HJ systems. Previous works have shown that the dynamical evolution of the stellar spin axis during the high-e migration plays a dominant role in generating the observed spin-orbit misalignment. Numerical studies have also revealed various patterns of the evolution of the stellar spin axis leading to the final misalignment. Here, we develop an analytic theory to elucidate the evolution of spin-orbit misalignment during the Lidov-Kozai migration of planets in stellar binaries. Secular spin-orbit resonances play a key role in the misalignment evolution. We include the effects of short-range forces and tidal dissipation, and categorize the different possible paths to spin-orbit misalignment as a function of various physical parameters (e.g. planet mass and stellar rotation period). We identify five distinct spin-orbit evolution paths and outcomes, only two of which are capable of producing retrograde orbits. We show that these paths to misalignment and the outcomes depend only on two dimensionless parameters, which compare the stellar spin precession frequency with the rate of change of the planet's orbital axis, and the Lidov-Kozai oscillation frequency. Our analysis reveals a number of novel phenomena for the stellar spin evolution, ranging from bifurcation, adiabatic advection, to fully chaotic evolution of spin-orbit angles.
Multi-spin-state dynamics during insulator-metal crossover in LaCoO3
Doi, A.; Fujioka, J.; Fukuda, T.; Tsutsui, S.; Okuyama, D.; Taguchi, Y.; Arima, T.; Baron, A. Q. R.; Tokura, Y.
2014-08-01
We have investigated the dynamics of spin-state crossover (SSC) for perovskite LaCoO3 through optical phonons by means of infrared and inelastic x-ray spectroscopy. Upon thermally induced SSC, anomalously dispersionless Co-O bond stretching phonons coupled to the thermally excited spin state have been identified. The enhanced spin-state fluctuation irrespective of the presence of a clear charge gap suggests the emergence of complex spin-state disproportionation involving low-, intermediate-, and high-spin states due to the strong correlation among thermally activated spin states.
Dynamical spin injection at a quasi-one-dimensional ferromagnet-graphene interface
Energy Technology Data Exchange (ETDEWEB)
Singh, S.; Ahmadi, A.; Mucciolo, E. R.; Barco, E. del [Department of Physics, University of Central Florida, Orlando, Florida 32816 (United States); Cherian, C. T. [Department of Physics, National University of Singapore, 2 Science Drive 3, Singapore 117542 (Singapore); Graphene Research Center, National University of Singapore, Singapore 117542 (Singapore); Özyilmaz, B. [Department of Physics, National University of Singapore, 2 Science Drive 3, Singapore 117542 (Singapore); NanoCore, 4 Engineering Drive 3, National University of Singapore, Singapore 117576 (Singapore); Graphene Research Center, National University of Singapore, Singapore 117542 (Singapore); NUS Graduate School for Integrative Sciences and Engineering (NGS), National University of Singapore, Singapore 117456 (Singapore)
2015-01-19
We present a study of dynamical spin injection from a three-dimensional ferromagnet into two-dimensional single-layer graphene. Comparative ferromagnetic resonance (FMR) studies of ferromagnet/graphene strips buried underneath the central line of a coplanar waveguide show that the FMR linewidth broadening is the largest when the graphene layer protrudes laterally away from the ferromagnetic strip, indicating that the spin current is injected into the graphene areas away from the area directly underneath the ferromagnet being excited. Our results confirm that the observed damping is indeed a signature of dynamical spin injection, wherein a pure spin current is pumped into the single-layer graphene from the precessing magnetization of the ferromagnet. The observed spin pumping efficiency is difficult to reconcile with the expected backflow of spins according to the standard spin pumping theory and the characteristics of graphene, and constitutes an enigma for spin pumping in two-dimensional structures.
Phonon-magnon interactions in body centered cubic iron: A combined molecular and spin dynamics study
Energy Technology Data Exchange (ETDEWEB)
Perera, Dilina, E-mail: dilinanp@physast.uga.edu; Landau, David P. [Center for Simulational Physics, The University of Georgia, Georgia 30602 (United States); Nicholson, Don M.; Malcolm Stocks, G.; Eisenbach, Markus; Yin, Junqi [Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 (United States); Brown, Gregory [Florida State University, Tallahassee, Florida 32306 (United States)
2014-05-07
Combining an atomistic many-body potential with a classical spin Hamiltonian parameterized by first principles calculations, molecular-spin dynamics computer simulations were performed to investigate phonon-magnon interactions in body centered cubic iron. Results obtained for spin-spin and density-density dynamic structure factors show that noticeable softening and damping of magnon modes occur due to the presence of lattice vibrations. Furthermore, as a result of the phonon-magnon coupling, additional longitudinal spin wave excitations are observed, with the same frequencies as the longitudinal phonon modes.
Phonon-magnon interactions in BCC iron: A combined molecular and spin dynamics study
Energy Technology Data Exchange (ETDEWEB)
Perera, Meewanage Dilina N [ORNL; Landau, David P [University of Georgia, Athens, GA; Nicholson, Don M [ORNL; Stocks, George Malcolm [ORNL; Eisenbach, Markus [ORNL; Yin, Junqi [ORNL; Brown, Greg [ORNL
2014-01-01
Combining an atomistic many-body potential with a classical spin Hamiltonian pa- rameterized by first principles calculations, molecular-spin dynamics computer sim- ulations were performed to investigate phonon-magnon interactions in BCC iron. Results obtained for spin-spin and density-density dynamic structure factors show that noticeable softening and damping of magnon modes occur due to the presence of lattice vibrations. Furthermore, as a result of the phonon-magnon coupling, addi- tional longitudinal spin wave excitations are observed, with the same frequencies as the longitudinal phonon modes.
Dynamics of High-Order Spin-Orbit Couplings about Linear Momenta in Compact Binary Systems*
Huang, Li; Wu, Xin; Mei, Li-Jie; Huang, Guo-Qing
2017-09-01
This paper relates to the post-Newtonian Hamiltonian dynamics of spinning compact binaries, consisting of the Newtonian Kepler problem and the leading, next-to-leading and next-to-next-to-leading order spin-orbit couplings as linear functions of spins and momenta. When this Hamiltonian form is transformed to a Lagrangian form, besides the terms corresponding to the same order terms in the Hamiltonian, several additional terms, third post-Newtonian (3PN), 4PN, 5PN, 6PN and 7PN order spin-spin coupling terms, yield in the Lagrangian. That means that the Hamiltonian is nonequivalent to the Lagrangian at the same PN order but is exactly equivalent to the full Lagrangian without any truncations. The full Lagrangian without the spin-spin couplings truncated is integrable and regular. Whereas it is non-integrable and becomes possibly chaotic when any one of the spin-spin terms is dropped. These results are also supported numerically.
Spin dynamics in perovskites, pyrochlores, and layered manganites
Energy Technology Data Exchange (ETDEWEB)
Oseroff, S. B. [San Diego State University, San Diego, California 29182-8062 (United States); Moreno, N. O. [Instituto de Fisica ' ' Gleb Wataghin' ' UNICAMP, Campinas, Sao Paulo 13083-970, (Brazil); Pagliuso, P. G. [Instituto de Fisica ' ' Gleb Wataghin' ' UNICAMP, Campinas, Sao Paulo 13083-970, (Brazil); Rettori, C. [Instituto de Fisica ' ' Gleb Wataghin' ' UNICAMP, Campinas, Sao Paulo 13083-970, (Brazil); Huber, D. L. [University of Wisconsin-Madison, Madison, Wisconsin 53706 (United States); Gardner, J. S. [Los Alamos National Laboratory, Los Alamos, New Mexico 87545 (United States); Sarrao, J. L. [Los Alamos National Laboratory, Los Alamos, New Mexico 87545 (United States); Thompson, J. D. [Los Alamos National Laboratory, Los Alamos, New Mexico 87545 (United States); Causa, M. T. [Centro Atomico Bariloche and Instituto Balseiro, Comision Nacional de Energia Atomica and Universidad Nacional de Cuyo, 8400 San Carlos de Bariloche, (Argentina); Alejandro, G. [Centro Atomico Bariloche and Instituto Balseiro, Comision Nacional de Energia Atomica and Universidad Nacional de Cuyo, 8400 San Carlos de Bariloche, (Argentina)] (and others)
2000-05-01
High temperature electron spin resonance (ESR) and magnetic susceptibility ({chi}) are analyzed for manganites related with colossal magnetoresistance (CMR). The properties of compounds with different crystalline structures: three-dimensional (3D) perovskites, pyrochlore, and La{sub 1.2}Sr{sub 1.8}Mn{sub 2}O{sub 7}, a two-dimensional layer, are compared. In the paramagnetic regime, and outside the critical regions associated with phase transitions, the temperature dependence of the ESR linewidth presents a universal behavior dominated by the variations of {chi}(T), {delta}H{sub pp}(T)=[C/T{chi}(T)]{delta}H{sub pp}({infinity}). The high temperature limit of the linewidth, {delta}H{sub pp}({infinity}), is related to the parameters of the Hamiltonian describing the interactions of the spin system. The role played by magnetic anisotropy, isotropic superexchange, and double exchange is revealed and discussed in the analysis of the experimental data. In CMR and non-CMR pyrochlores, {delta}H{sub pp}({infinity}){proportional_to}{omega}{sub p}{sup 2}/J where J is proportional to the Curie-Weiss temperature, including the hybridization mechanism producing CMR. Instead, {delta}H{sub pp}({infinity}) of CMR perovskites seems not to be affected by the double-exchange interaction. In contrast with the 3D perovskites, the ESR linewidth and resonance field of La{sub 1.2}Sr{sub 1.8}Mn{sub 2}O{sub 7}, a bilayer compound, although isotropic at high temperatures, becomes anisotropic for T{sub c}=125 K
Spin-charge coupled dynamics driven by a time-dependent magnetization
Tölle, Sebastian; Eckern, Ulrich; Gorini, Cosimo
2017-03-01
The spin-charge coupled dynamics in a thin, magnetized metallic system are investigated. The effective driving force acting on the charge carriers is generated by a dynamical magnetic texture, which can be induced, e.g., by a magnetic material in contact with a normal-metal system. We consider a general inversion-asymmetric substrate/normal-metal/magnet structure, which, by specifying the precise nature of each layer, can mimic various experimentally employed setups. Inversion symmetry breaking gives rise to an effective Rashba spin-orbit interaction. We derive general spin-charge kinetic equations which show that such spin-orbit interaction, together with anisotropic Elliott-Yafet spin relaxation, yields significant corrections to the magnetization-induced dynamics. In particular, we present a consistent treatment of the spin density and spin current contributions to the equations of motion, inter alia, identifying a term in the effective force which appears due to a spin current polarized parallel to the magnetization. This "inverse-spin-filter" contribution depends markedly on the parameter which describes the anisotropy in spin relaxation. To further highlight the physical meaning of the different contributions, the spin-pumping configuration of typical experimental setups is analyzed in detail. In the two-dimensional limit the buildup of dc voltage is dominated by the spin-galvanic (inverse Edelstein) effect. A measuring scheme that could isolate this contribution is discussed.
Morais, C. V.; Zimmer, F. M.; Lazo, M. J.; Magalhães, S. G.; Nobre, F. D.
2016-06-01
The behavior of the nonlinear susceptibility χ3 and its relation to the spin-glass transition temperature Tf in the presence of random fields are investigated. To accomplish this task, the Sherrington-Kirkpatrick model is studied through the replica formalism, within a one-step replica-symmetry-breaking procedure. In addition, the dependence of the Almeida-Thouless eigenvalue λAT (replicon) on the random fields is analyzed. Particularly, in the absence of random fields, the temperature Tf can be traced by a divergence in the spin-glass susceptibility χSG, which presents a term inversely proportional to the replicon λAT. As a result of a relation between χSG and χ3, the latter also presents a divergence at Tf, which comes as a direct consequence of λAT=0 at Tf. However, our results show that, in the presence of random fields, χ3 presents a rounded maximum at a temperature T* which does not coincide with the spin-glass transition temperature Tf (i.e., T*>Tf for a given applied random field). Thus, the maximum value of χ3 at T* reflects the effects of the random fields in the paramagnetic phase instead of the nontrivial ergodicity breaking associated with the spin-glass phase transition. It is also shown that χ3 still maintains a dependence on the replicon λAT, although in a more complicated way as compared with the case without random fields. These results are discussed in view of recent observations in the LiHoxY1 -xF4 compound.
Spin probe dynamics of n-hexadecane in confined geometry
Lukešová, Miroslava; Švajdlenková, Helena; Sippel, Pit; Macová, Eva; Berek, Dušan; Loidl, Alois; Bartoš, Josef
2015-02-01
A combined study of the rotational dynamics of the stable free radical 2,2,6,6-tetramethyl-1-piperidinyloxy (TEMPO) and the phase behavior of n-hexadecane (n-HXD) in the bulk and the confined states in a series of silica gels (SG) by means of ESR and DSC is presented. A slow to fast motion transition of the spin probe TEMPO in the bulk n-HXD occurs at T50 G,bulk ≪ Tm,bulk, i.e., well below the melting temperature due to its trapping and localized mobility in the interlamellar gap of the crystallites [J. Bartoš, H. Švajdlenková, M. Zaleski, M. Edelmann, M. Lukešová, Physica B 430, 99 (2013)]. On the other hand, the dynamics of the TEMPO in the confined systems is strongly slowing down with T50 G (Dpore) >Tm(Dpore) and slightly increases with the pore size Dpore = 60, 100 and 300 Å of the SG's. At the same time, both the corresponding melting temperature, Tm (Dpore), and melting enthalpy, ΔHm (Dpore), decrease with Dpore together with the mutual anti-correlation between T50 G and Tm as a function of the inverse of pore diameter, 1/Dpore. Moreover, the dynamic heterogeneity of the TEMPO in the confined state below T50 G (Dpore) is closely related to the phase transformation. The strong slowing down of the spin probe motion likely results from its preferential localization at the interface layer of the matrix pore due to specific interaction of TEMPO molecules with the polar silanol groups of the SG matrix. This is supported by special study on a series of the variously filled n-HXD/SG systems, other similar experimental findings as well as by theoretical spectral argument.
Energy Technology Data Exchange (ETDEWEB)
Cofield, M.L.; Bryan, P.S.
1986-02-03
We have determined the value of the ground-state zero-field splitting parameter D for several high-spin d/sup 4/ Mn(III) compounds from average susceptibility measurements down to 5 K with a SQUID magnetometer. The zero-field splittings in these compounds are similar to some results reported for Mn(III) porphyrins and are insensitive to ligand structure and axial halide binding, in contrast to what has been reported for the analogous Fe(III) compounds. (orig./HBR).
Tseng, K. F.; Keller, T.; Walters, A. C.; Birgeneau, R. J.; Keimer, B.
2016-07-01
We report a neutron spin-echo study of the critical dynamics in the S =5/2 antiferromagnets MnF2 and Rb2MnF4 with three-dimensional (3D) and two-dimensional (2D) spin systems, respectively, in zero external field. Both compounds are Heisenberg antiferromagnets with a small uniaxial anisotropy resulting from dipolar spin-spin interactions, which leads to a crossover in the critical dynamics close to the Néel temperature, TN. By taking advantage of the μ eV energy resolution of the spin-echo spectrometer, we have determined the dynamical critical exponents z for both longitudinal and transverse fluctuations. In MnF2, both the characteristic temperature for crossover from 3D Heisenberg to 3D Ising behavior and the exponents z in both regimes are consistent with predictions from the dynamical scaling theory. The amplitude ratio of longitudinal and transverse fluctuations also agrees with predictions. In Rb2MnF4 , the critical dynamics crosses over from the expected 2D Heisenberg behavior for T ≫TN to a scaling regime with exponent z =1.387 (4 ) , which has not been predicted by theory and may indicate the influence of long-range dipolar interactions.
Higher-order spin and charge dynamics in a quantum dot-lead hybrid system.
Otsuka, Tomohiro; Nakajima, Takashi; Delbecq, Matthieu R; Amaha, Shinichi; Yoneda, Jun; Takeda, Kenta; Allison, Giles; Stano, Peter; Noiri, Akito; Ito, Takumi; Loss, Daniel; Ludwig, Arne; Wieck, Andreas D; Tarucha, Seigo
2017-09-22
Understanding the dynamics of open quantum systems is important and challenging in basic physics and applications for quantum devices and quantum computing. Semiconductor quantum dots offer a good platform to explore the physics of open quantum systems because we can tune parameters including the coupling to the environment or leads. Here, we apply the fast single-shot measurement techniques from spin qubit experiments to explore the spin and charge dynamics due to tunnel coupling to a lead in a quantum dot-lead hybrid system. We experimentally observe both spin and charge time evolution via first- and second-order tunneling processes, and reveal the dynamics of the spin-flip through the intermediate state. These results enable and stimulate the exploration of spin dynamics in dot-lead hybrid systems, and may offer useful resources for spin manipulation and simulation of open quantum systems.
Energy Technology Data Exchange (ETDEWEB)
Artzi, Moran [Tel Aviv Sourasky Medical Center, Functional Brain Center, The Wohl Institute for Advanced Imaging, Tel Aviv (Israel); Tel Aviv University, Sackler Faculty of Medicine, Tel Aviv (Israel); Liberman, Gilad; Vitinshtein, Faina; Aizenstein, Orna [Tel Aviv Sourasky Medical Center, Functional Brain Center, The Wohl Institute for Advanced Imaging, Tel Aviv (Israel); Nadav, Guy [Tel Aviv Sourasky Medical Center, Functional Brain Center, The Wohl Institute for Advanced Imaging, Tel Aviv (Israel); Tel Aviv University, Faculty of Engineering, Tel Aviv (Israel); Blumenthal, Deborah T.; Bokstein, Felix [Tel Aviv Sourasky Medical Center, Neuro-Oncology Service, Tel Aviv (Israel); Bashat, Dafna Ben [Tel Aviv Sourasky Medical Center, Functional Brain Center, The Wohl Institute for Advanced Imaging, Tel Aviv (Israel); Tel Aviv University, Sackler Faculty of Medicine and Sagol School of Neuroscience, Tel Aviv (Israel)
2015-07-15
Cerebral blood volume (CBV) is an important parameter for the assessment of brain tumors, usually obtained using dynamic susceptibility contrast (DSC) MRI. However, this method often suffers from low spatial resolution and high sensitivity to susceptibility artifacts and usually does not take into account the effect of tissue permeability. The plasma volume (v{sub p}) can also be extracted from dynamic contrast enhancement (DCE) MRI. The aim of this study was to investigate whether DCE can be used for the measurement of cerebral blood volume in place of DSC for the assessment of patients with brain tumors. Twenty-eight subjects (17 healthy subjects and 11 patients with glioblastoma) were scanned using DCE and DSC. v{sub p} and CBV values were measured and compared in different brain components in healthy subjects and in the tumor area in patients. Significant high correlations were detected between v{sub p} and CBV in healthy subjects in the different brain components; white matter, gray matter, and arteries, correlating with the known increased tissue vascularity, and within the tumor area in patients. This work proposes the use of DCE as an alternative method to DSC for the assessment of blood volume, given the advantages of its higher spatial resolution, its lower sensitivity to susceptibility artifacts, and its ability to provide additional information regarding tissue permeability. (orig.)
Energy Technology Data Exchange (ETDEWEB)
Jungfleisch, Matthias B. [Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA; Zhang, Wei [Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA; Ding, Junjia [Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA; Jiang, Wanjun [Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA; Sklenar, Joseph [Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA; Department of Physics and Astronomy, Northwestern University, Evanston, Illinois 60208, USA; Pearson, John E. [Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA; Ketterson, John B. [Department of Physics and Astronomy, Northwestern University, Evanston, Illinois 60208, USA; Hoffmann, Axel [Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439, USA
2016-02-01
The understanding of spin dynamics in laterally confined structures on sub-micron length scales has become a significant aspect of the development of novel magnetic storage technologies. Numerous ferromagnetic resonance measurements, optical characterization by Kerr microscopy and Brillouin light scattering spectroscopy and x-ray studies were carried out to detect the dynamics in patterned magnetic antidot lattices. Here, we investigate Oersted-field driven spin dynamics in rectangular Ni80Fe20/Pt antidot lattices with different lattice parameters by electrical means. When the system is driven to resonance, a dc voltage across the length of the sample is detected that changes its sign upon field reversal, which is in agreement with a rectification mechanism based on the inverse spin Hall effect. Furthermore, we show that the voltage output scales linearly with the applied microwave drive in the investigated range of powers. Our findings have direct implications on the development of engineered magnonics applications and devices.
Spin dynamics of an individual Cr atom in a semiconductor quantum dot under optical excitation
Energy Technology Data Exchange (ETDEWEB)
Lafuente-Sampietro, A. [Université Grenoble Alpes, Institut Néel, F-38000 Grenoble (France); CNRS, Institut Néel, F-38000 Grenoble (France); Institute of Materials Science, University of Tsukuba, 305-8573 Tsukuba (Japan); Utsumi, H.; Kuroda, S. [Institute of Materials Science, University of Tsukuba, 305-8573 Tsukuba (Japan); Boukari, H.; Besombes, L., E-mail: lucien.besombes@grenoble.cnrs.fr [Université Grenoble Alpes, Institut Néel, F-38000 Grenoble (France); CNRS, Institut Néel, F-38000 Grenoble (France)
2016-08-01
We studied the spin dynamics of a Cr atom incorporated in a II-VI semiconductor quantum dot using photon correlation techniques. We used recently developed singly Cr-doped CdTe/ZnTe quantum dots to access the spin of an individual magnetic atom. Auto-correlation of the photons emitted by the quantum dot under continuous wave optical excitation reveals fluctuations of the localized spin with a timescale in the 10 ns range. Cross-correlation gives quantitative transfer time between Cr spin states. A calculation of the time dependence of the spin levels population in Cr-doped quantum dots shows that the observed spin dynamics is dominated by the exciton-Cr interaction. These measurements also provide a lower bound in the 20 ns range for the intrinsic Cr spin relaxation time.
Dynamic magnetic susceptibility of systems with long-range magnetic order
Energy Technology Data Exchange (ETDEWEB)
Vannette, Matthew Dano [Iowa State Univ., Ames, IA (United States)
2009-01-01
The utility of the TDR as an instrument in the study of magnetically ordered materials has been expanded beyond the simple demonstration purposes. Results of static applied magnetic field dependent measurements of the dynamic magnetic susceptibility, χ, of various ferromagnetic (FM) and antiferromagnetic (AFM) materials showing a range of transition temperatures (1-800 K) are presented. Data was collected primarily with a tunnel diode resonator (TDR) at different radio-frequencies (~10-30 MHz). In the vicinity of T_{C} local moment ferromagnets show a very sharp, narrow peak in χ which is suppressed in amplitude and shifted to higher temperatures as the static bias field is increased. Unexpectedly, critical scaling analysis fails for these data. It is seen that these data are frequency dependent, however there is no simple method whereby measurement frequency can be changed in a controllable fashion. In contrast, itinerant ferromagnets show a broad maximum in χ well below T_{C} which is suppressed and shifts to lower temperatures as the dc bias field is increased. The data on itinerant ferromagnets is fitted to a semi-phenomenological model that suggests the sample response is dominated by the uncompensated minority spins in the conduction band. Concluding remarks suggest possible scenarios to achieve frequency resolved data using the TDR as well as other fields in which the apparatus may be exploited.
Zero-dimensional spin accumulation and spin dynamics in a mesoscopic metal island
Zaffalon, M; van Wees, BJ
2003-01-01
We have measured electron spin accumulation at 4.2 K and at room temperature in an aluminum island with all dimensions (400 nmx400 nmx30 nm) smaller than the spin relaxation length. For the first time, we obtain uniform spin accumulation in a four-terminal lateral device with a magnitude exceeding t
Institute of Scientific and Technical Information of China (English)
LIU Bang-gui; ZHANG Kai-cheng; LI Ying
2007-01-01
The Kinetic Monte Carlo (KMC) method based on the transition-state theory, powerful and famous for sim-ulating atomic epitaxial growth of thin films and nanostruc-tures, was used recently to simulate the nanoferromagnetism and magnetization dynamics of nanomagnets with giant mag-netic anisotropy. We present a brief introduction to the KMC method and show how to reformulate it for nanoscale spin systems. Large enough magnetic anisotropy, observed exper-imentally and shown theoretically in terms of first-principle calculation, is not only essential to stabilize spin orientation but also necessary in making the transition-state barriers dur-ing spin reversals for spin KMC simulation. We show two applications of the spin KMC method to monatomic spin chains and spin-polarized-current controlled composite nano-magnets with giant magnetic anisotropy. This spin KMC method can be applied to other anisotropic nanomagnets and composite nanomagnets as long as their magnetic anisotropy energies are large enough.
Kiselev, Egor I.; Scheurer, Mathias S.; Wölfle, Peter; Schmalian, Jörg
2017-03-01
An ordered state in the spin sector that breaks parity without breaking time-reversal symmetry, i.e., that can be considered dynamically generated spin-orbit coupling, was proposed to explain puzzling observations in a range of different systems. Here, we derive severe restrictions for such a state that follow from a Ward identity related to spin conservation. It is shown that l =1 spin-Pomeranchuk instabilities are not possible in nonrelativistic systems since the response of spin-current fluctuations is entirely incoherent and nonsingular. This rules out relativistic spin-orbit coupling as an emergent low-energy phenomenon. We illustrate the exotic physical properties of the remaining higher-angular-momentum analogs of spin-orbit coupling and derive a geometric constraint for spin-orbit vectors in lattice systems.
Spin Dynamics simulations of the dynamic properties of classical models for magnetic materials
Bunker, Alex; Landau, D. P.
1998-03-01
The Spin Dynamics simulation technique, which has had considerable success for the study of critical properties of classical Heisenberg antiferromagnets(A. Bunker, K. Chen, and D. P. Landau Phys. Rev. B) \\underline54, 9259 (1996), has been used to determine more general properties for a wider range of materials. A general spin dynamics program has been developed which can determine the dynamic structure factor, S(q,ω), in the [100], [110], and [111] directions for a wide range of classical magnetic models at any temperature desired. We have simulated the magnetic dynamics in the ordered phase of the isotropic Heisenberg model with both ferromagnetic and antiferromagnetic coupling on L×L×L BCC and SC lattices. Outside of the critical regime relatively small lattice sizes of L = 12, 24 could be used. From our simulation we have determined the stiffness coefficient and the spin relaxation rate which were compared to both experimental(J. Als-Nielsen in Phase Transitions and Critical Phenomena), ed. C. Domb, M. S. Green, Academic Press, (1976) and theoretical results. We have performed the same simulation with anisotropy appropriate for MnF2 and FeF_2. Research supported in part by the NSF
Melnikov, Alexey; Razdolski, Ilya; Alekhin, Alexandr; Ilin, Nikita; Meyburg, Jan; Diesing, Detlef; Roddatis, Vladimir; Rungger, Ivan; Stamenova, Maria; Sanvito, Stefano; Bovensiepen, Uwe
2016-10-01
Further development of spintronics requires miniaturization and reduction of characteristic timescales of spin dynamics combining the nanometer spatial and femtosecond temporal ranges. These demands shift the focus of interest towards the fundamental open question of the interaction of femtosecond spin current (SC) pulses with a ferromagnet (FM). The spatio-temporal properties of the spin transfer torque (STT) exerted by ultrashort SC pulses on the FM open the time domain for studying STT fingerprint on spatially non-uniform magnetization dynamics. Using the sensitivity of magneto-induced second harmonic generation to SC, we develop technique for SC monitoring. With 20 fs resolution, we demonstrate the generation of 250 fs-long SC pulses in Fe/Au/Fe/MgO(001) structures. Their temporal profile indicates (i) nearly-ballistic hot electron transport in Au and (ii) that the pulse duration is primarily determined by the thermalization time of laser-excited hot carriers in Fe. Together with strongly spin-dependent Fe/Au interface transmission calculated for these carriers, this suggests the non-thermal spin-dependent Seebeck effect dominating the generation of ultrashort SC pulses. The analysis of SC transmission/reflection at the Au/Fe interface shows that hot electron spins orthogonal to the Fe magnetization rotate gaining huge parallel (anti-parallel) projection in transmitted (reflected) SC. This is accompanied by a STT-induced perturbation of the magnetization localized at the interface, which excites the inhomogeneous high-frequency spin dynamics in the FM. Time-resolved magneto-optical studies reveal the excitation of several standing spin wave modes in the Fe film with their spectrum extending up to 0.6 THz and indicating the STT spatial confinement to 2 nm.
Storch, Natalia I; Anderson, Kassandra R
2016-01-01
Many exoplanetary systems containing hot Jupiters (HJs) exhibit significant misalignment between the spin axes of the host stars and the orbital angular momentum axes of the planets ("spin-orbit misalignment"). High-eccentricity migration involving Lidov-Kozai oscillations of the planet's orbit induced by a distant perturber is a possible channel for producing such misaligned HJ systems. Previous works have shown that the dynamical evolution of the stellar spin axis during the high-$e$ migration plays a dominant role in generating the observed spin-orbit misalignment. Numerical studies have also revealed various patterns of the evolution of the stellar spin axis leading to the final misalignment. Here we develop an analytic theory to elucidate the evolution of spin-orbit misalignment during the Lidov-Kozai migration of planets in stellar binaries. Secular spin-orbit resonances play a key role in the misalignment evolution. We include the effects of short-range forces and tidal dissipation, and categorize the ...
Influence of Impurity Spin Dynamics on Quantum Transport in Epitaxial Graphene.
Lara-Avila, Samuel; Kubatkin, Sergey; Kashuba, Oleksiy; Folk, Joshua A; Lüscher, Silvia; Yakimova, Rositza; Janssen, T J B M; Tzalenchuk, Alexander; Fal'ko, Vladimir
2015-09-04
Experimental evidence from both spin-valve and quantum transport measurements points towards unexpectedly fast spin relaxation in graphene. We report magnetotransport studies of epitaxial graphene on SiC in a vector magnetic field showing that spin relaxation, detected using weak-localization analysis, is suppressed by an in-plane magnetic field B(∥), and thereby proving that it is caused at least in part by spinful scatterers. A nonmonotonic dependence of the effective decoherence rate on B(∥) reveals the intricate role of the scatterers' spin dynamics in forming the interference correction to the conductivity, an effect that has gone unnoticed in earlier weak localization studies.
Exact results for spin dynamics and fractionalization in the Kitaev Model.
Baskaran, G; Mandal, Saptarshi; Shankar, R
2007-06-15
We present certain exact analytical results for dynamical spin correlation functions in the Kitaev Model. It is the first result of its kind in nontrivial quantum spin models. The result is also novel: in spite of the presence of gapless propagating Majorana fermion excitations, dynamical two spin correlation functions are identically zero beyond nearest neighbor separation. This shows existence of a gapless but short range spin liquid. An unusual, all energy scale fractionalization of a spin-flip quanta, into two infinitely massive pi fluxes and a dynamical Majorana fermion, is shown to occur. As the Kitaev Model exemplifies topological quantum computation, our result presents new insights into qubit dynamics and generation of topological excitations.
Tracking excited-state charge and spin dynamics in iron coordination complexes
DEFF Research Database (Denmark)
Zhang, Wenkai; Alonso-Mori, Roberto; Bergmann, Uwe
2014-01-01
to spin state, can elucidate the spin crossover dynamics of [Fe(2,2'-bipyridine)(3)](2+) on photoinduced metal-to-ligand charge transfer excitation. We are able to track the charge and spin dynamics, and establish the critical role of intermediate spin states in the crossover mechanism. We anticipate......Crucial to many light-driven processes in transition metal complexes is the absorption and dissipation of energy by 3d electrons(1-4). But a detailed understanding of such non-equilibrium excited-state dynamics and their interplay with structural changes is challenging: a multitude of excited...... states and possible transitions result in phenomena too complex to unravel when faced with the indirect sensitivity of optical spectroscopy to spin dynamics(5) and the flux limitations of ultrafast X-ray sources(6,7). Such a situation exists for archetypal poly-pyridyl iron complexes, such as [Fe(2...
Two dimensional electron spin resonance: Structure and dynamics of biomolecules
Saxena, Sunil; Freed, Jack H.
1998-03-01
The potential of two dimensional (2D) electron spin resonance (ESR) for measuring the structural properties and slow dynamics of labeled biomolecules will be presented. Specifically, it will be shown how the recently developed method of double quantum (DQ) 2D ESR (S. Saxena and J. H. Freed, J. Chem. Phys. 107), 1317, (1997) can be used to measure large interelectron distances in bilabeled peptides. The need for DQ ESR spectroscopy, as well as the challenges and advantages of this method will be discussed. The elucidation of the slow reorientational dynamics of this peptide (S. Saxena and J. H. Freed, J. Phys. Chem. A, 101) 7998 (1997) in a glassy medium using COSY and 2D ELDOR ESR spectroscopy will be demonstrated. The contributions to the homogeneous relaxation time, T_2, from the overall and/or internal rotations of the nitroxide can be distinguished from the COSY spectrum. The growth of spectral diffusion cross-peaks^2 with mixing time in the 2D ELDOR spectra can be used to directly determine a correlation time from the experiment which can be related to the rotational correlation time.
Coupled spin-light dynamics in cavity optomagnonics
Viola Kusminskiy, Silvia; Tang, Hong X.; Marquardt, Florian
2016-09-01
Experiments during the past 2 years have shown strong resonant photon-magnon coupling in microwave cavities, while coupling in the optical regime was demonstrated very recently for the first time. Unlike with microwaves, the coupling in optical cavities is parametric, akin to optomechanical systems. This line of research promises to evolve into a new field of optomagnonics, aimed at the coherent manipulation of elementary magnetic excitations in solid-state systems by optical means. In this work we derive the microscopic optomagnonic Hamiltonian. In the linear regime the system reduces to the well-known optomechanical case, with remarkably large coupling. Going beyond that, we study the optically induced nonlinear classical dynamics of a macrospin. In the fast-cavity regime we obtain an effective equation of motion for the spin and show that the light field induces a dissipative term reminiscent of Gilbert damping. The induced dissipation coefficient, however, can change sign on the Bloch sphere, giving rise to self-sustained oscillations. When the full dynamics of the system is considered, the system can enter a chaotic regime by successive period doubling of the oscillations.
Ness, H; Dash, L K
2012-03-23
We calculate the nonequilibrium charge transport properties of nanoscale junctions in the steady state and extend the concept of charge susceptibility to the nonequilibrium conditions. We show that the nonequilibrium charge susceptibility is related to the nonlinear dynamical conductance. In spectroscopic terms, both contain the same features versus applied bias when charge fluctuation occurs in the corresponding electronic resonances. However, we show that, while the conductance exhibits features at biases corresponding to inelastic scattering with no charge fluctuations, the nonequilibrium charge susceptibility does not. We suggest that measuring both the nonequilibrium conductance and charge susceptibility in the same experiment will permit us to differentiate between different scattering processes in quantum transport.
Energy Technology Data Exchange (ETDEWEB)
Martinez-Blanco, D.; Gorria, P. [Departamento de Fisica, Universidad de Oviedo, Calvo Sotelo, s/n, 33007 Oviedo (Spain); Fernandez-Martinez, Alejandro [Lawrence Livermore National Laboratory 7000 East Avenue, Livermore, CA 9455 (United States); Perez, M.J. [Departamento de Fisica, Universidad de Oviedo, Calvo Sotelo, s/n, 33007 Oviedo (Spain); Cuello, Gabriel J. [Institut Laue-Langevin, BP 156, 6, rue Jules Horowitz, 38042 Grenoble Cedex 9 (France); Blanco, J.A., E-mail: jabr@uniovi.es [Departamento de Fisica, Universidad de Oviedo, Calvo Sotelo, s/n, 33007 Oviedo (Spain)
2011-06-15
Research highlights: > Spin-glass-like behaviour o owing an re-entrant spin-glass transition. > No critical divergence observed in the maxima of the real and magnetic susceptibility on ball milled Fe{sub 30}Cr{sub 70}. > High temperature Curie-Weiss behavior of the magnetic susceptibility on ball milled Fe{sub 30}Cr{sub 70}. > Moderate shift of the freezing temperature per frequency in ball milled Fe{sub 30}Cr{sub 70} obtained from the temperature dependence of the real magnetic susceptibility - Abstract: Nominal nanostructured Fe{sub 30}Cr{sub 70} obtained from ball milling during 110 h has been investigated from dc magnetization and ac magnetic susceptibility. The as-milled sample is not monophasic and is formed of two phases, Fe{sub 20{+-}2}Cr{sub 80{+-}2} ({approx}86 {+-} 2%) and iron ({approx}14 {+-} 2%). The ac susceptibility measurements show evidence of a re-entrant spin-glass-like transition for the Fe{sub 20}Cr{sub 80} phase below 30 K. The shift of the freezing temperature per frequency decade is moderate when compared to that found in conventional spin-glass alloys. A Vogel-Fulcher activation process can be used to explain the frequency variation. The results are also analyzed in terms of Cole-Cole formalism for extracting information of relaxation time ({tau} {approx} 10{sup -5} to 10{sup -4} s).
Wang, Jiongjiong; Li, Lin; Roc, Anne C; Alsop, David C; Tang, Kathy; Butler, Norman S; Schnall, Mitchell D; Detre, John A
2004-01-01
Arterial spin labeling (ASL) perfusion contrast is not based on susceptibility effects and can therefore be used to study brain function in regions of high static inhomogeneity. As a proof of concept, single-shot spin-echo echo-planar imaging (EPI) acquisition was carried out with a multislice continuous ASL (CASL) method at 1.5T. A bilateral finger tapping paradigm was used in the presence of an exogenously induced susceptibility artifact over left motor cortex. The spin-echo CASL technique was compared with a regular gradient-echo EPI sequence with the same slice thickness, as well as other imaging methods using thin slices and spin-echo acquisitions. The results demonstrate improved functional sensitivity and efficiency of the spin-echo CASL approach as compared with gradient-echo EPI techniques, and a trend of improved sensitivity as compared with spin-echo EPI approach in the brain regions affected by the susceptibility artifact. ASL images, either with or without subtraction of the control, provide a robust alternative to blood oxygenation level dependant (BOLD) methods for activation imaging in regions of high static field inhomogeneity.
Electron spin dynamics in GaAsN and InGaAsN structures
Energy Technology Data Exchange (ETDEWEB)
Lagarde, D.; Lombez, L.; Marie, X.; Balocchi, A.; Amand, T. [Laboratoire de Nanophysique, Magnetisme et Optoelectronique, INSA 135 avenue de Rangueil 31077 Toulouse Cedex 4 (France); Kalevich, V.K.; Shiryaev, A.; Ivchenko, E.; Egorov, A. [A.F. Ioffe Physico-Technical Institute, 194021 St-Petersburg (Russian Federation)
2007-01-15
We report on optical orientation experiments in undoped GaAsN epilayers and InGaAsN quantum wells (QW), showing that a strong electron spin polarisation can persist at room temperature. We demonstrate that the spin dynamics in these dilute nitride structures is governed by a spin-dependent recombination process of free conduction electrons on deep paramagnetic centres. (copyright 2007 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)
Spin dynamics and magneto-optical response in charge-neutral tunnel-coupled quantum dots
Gawełczyk, Michał; Machnikowski, Paweł
2017-04-01
We model the electron and hole spin dynamics in an undoped double quantum dot structure, considering the carrier tunneling between quantum dots. Taking the presence of an additional in-plane or tilted magnetic field into account, we enable the simulation of magneto-optical experiments, like the time-resolved Kerr rotation measurement, which are currently performed on such structures to probe the temporal spin dynamics. With our model, we reproduce the experimentally observed effect of the extension of the spin polarization lifetime caused by spatial charge separation, which may occur in structures of this type. Moreover, we provide a number of qualitative predictions concerning the necessary conditions for observation of this effect as well as about possible channels of its suppression, including the spin–orbit coupling, which leads to tunneling of carriers accompanied by a spin flip. We also consider the impact of the magnetic field tilting, which results in an interesting spin polarization dynamics.
Secular precessing compact binary dynamics, spin and orbital angular momentum flip-flops
Tápai, Márton; Gergely, László Árpád
2016-01-01
We derive the conservative secular evolution of precessing compact binaries to second post-Newtonian order accuracy, with leading-order spin-orbit, spin-spin and mass quadrupole-monopole contributions included. The emerging closed system of first-order differential equations evolves the pairs of polar and azimuthal angles of the spin and orbital angular momentum vectors together with the periastron angle. In contrast with the instantaneous dynamics, the secular dynamics is autonomous. This secular dynamics reliably characterizes the system over timescales starting from a few times the radial period to several precessional periods, but less than the radiation reaction timescale. We numerically compare the instantaneous and secular evolutions and estimate the number of periods for which dissipation has no significant effect, e.g. the conservative timescale. We apply the analytic equations to study the spin flip-flop effect, recently found by numerical relativity methods. Our investigations show that the effect ...
Pumping dynamics of nuclear spins in GaAs quantum wells
Mocek, Raphael W; Cascio, Giovanni; Suter, Dieter
2016-01-01
Irradiating a semiconductor with circularly polarized light creates spin-polarized charge carriers. If the material contains atoms with non-zero nuclear spin, they interact with the electron spins via the hyperfine coupling. Here, we consider GaAs/AlGaAs quantum wells, where the conduction-band electron spins interact with three different types of nuclear spins. The hyperfine interaction drives a transfer of spin polarization to the nuclear spins, which therefore acquire a polarization that is comparable to that of the electron spins. In this paper, we analyze the dynamics of the optical pumping process in the presence of an external magnetic field while irradiating a single quantum well with a circularly polarized laser. We measure the time dependence of the photoluminescence polarization to monitor the buildup of the nuclear spin polarization and thus the average hyperfine interaction acting on the electron spins. We present a simple model that adequately describes the dynamics of this process and is in goo...
Collective dynamics of solid-state spin chains and ensembles in quantum information processing
Ping, Yuting
This thesis is concerned with the collective dynamics in different spin chains and spin ensembles in solid-state materials. The focus is on the manipulation of electron spins, through spin-spin and spin-photon couplings controlled by voltage potentials or electromagnetic fields. A brief review of various systems is provided to describe the possible physical implementation of the ideas, and also outlines the basis of the adopted effective interaction models. The first two ideas presented explore the collective behaviour of non-interacting spin chains with external couplings. One focuses on mapping the identical state of spin-singlet pairs in two currents onto two distant, static spins downstream, creating distributed entanglement that may be accessed. The other studies a quantum memory consisting of an array of non-interacting, static spins, which may encode and decode multiple flying spins. Both chains could effectively `enhance' weak couplings in a cumulative fashion, and neither scheme requires active quantum control. Moreover, the distributed entanglement generated can offer larger separation between the qubits than more conventional protocols that only exploit the tunnelling effects between quantum dots. The quantum memory can also `smooth' the statistical fluctuations in the effects of local errors when the stored information is spread. Next, an interacting chain of static spins with nearest-neighbour interactions is introduced to connect distant end spins. Previously, it has been shown that this approach provides a cubic speed-up when compared with the direct coupling between the target spins. The practicality of this scheme is investigated by analysing realistic error effects via numerical simulations, and from that perspective relaxation of the nearest-neighbour assumption is proposed. Finally, a non-interacting electron spin ensemble is reviewed as a quantum memory to store single photons from an on-chip stripline cavity. It is then promoted to a full
Non-commutative dynamics of spinning D0 branes
Loh, D; Sahakian, V V; Loh, Duane; Rudolfa, Kit; Sahakian, Vatche
2004-01-01
Rotational dynamics is known to polarize D0 branes into higher dimensional fuzzy Dp-branes: the tension forces between D0 branes provide the centripetal acceleration, and a puffed up spinning configuration stabilizes. In this work, we consider a rotating cylindrical formation of finite height, wrapping a compact cycle of the background space along the axis of rotation. We find a myriad of interesting results: an intriguing relation between the angular speed, the geometry of the cylinder, and the scale of non-commutativity; instabilities for small radii in relation to the height of the cylinder - reminiscent of the Gregory-LaFlamme phenomenon; a critical radius corresponding to the case where the area of the cylinder is proportional to the number of D0 branes - reminiscent of Matrix black holes; and no power radiated away through D0 brane charge. The instabilities appear to lead to the lateral collapse of the cylinder into possibly a slinky configuration, akin to the Matrix string.
Anomalous magnetic structure and spin dynamics in magnetoelectric LiFePO_{4}
DEFF Research Database (Denmark)
Toft-Petersen, Rasmus; Reehuis, Manfred; Jensen, Thomas Bagger Stibius
2015-01-01
We report significant details of the magnetic structure and spin dynamics of LiFePO4 obtained by single-crystal neutron scattering. Our results confirm a previously reported collinear rotation of the spins away from the principal b axis, and they determine that the rotation is toward the a axis...
Quark Number Susceptibilities with Domain-Wall Fermions
Hegde, Prasad; Schmidt, Christian
2008-01-01
We present results from calculations of different quark number and hadronic susceptibilities on 2+1-flavor dynamical domain wall ensembles. We find that the iso-spin and electric charge susceptibilities are especially well suited to determine the transition temperature, as these quantities show only small statistical errors. Moreover, the transition values of the coupling obtained from iso-spin and electrical charge susceptibilities are in good agreement with the one obtained from the chiral condensate.
Energy Technology Data Exchange (ETDEWEB)
Onufrieva, F.
1994-12-31
Spin dynamics in cuprates is analysed in the framework of a new theory (based on the t-t`-J model and the diagrammatic technique for Hubbard operators) developed to treat correctly strong electron correlations within CuO{sub 2} plane. The dynamic magnetic susceptibility is determined by two contributions different in nature, the ``localized`` and ``itinerant`` ones. The ``itinerant`` contribution reflects a response in the spin susceptibility on Cu related to the propagating carrier quasiparticles. The ``localized`` contribution reflects the existence of short-range correlations between localized spins. As a result of their competition, the spin dynamics evolves continuously within the metallic state from a normal-metal behaviour at high doping (overdoped regime) to a quantum spin-liquid-type dynamics with magnon-like excitations at low doping through a non-Fermi-liquid behaviour in all intermediate regimes. The picture of the spin dynamics in the metallic state of cuprates as a whole and in details in concern to INS and NMR experimental data is presented. Many exotic features of {chi}({Kappa},{omega}) revealed by these experiments find a natural explanation within the proposed scenario. (author). 64 refs., 17 figs.
Dynamic neutron scattering on incoherent systems using efficient resonance spin flip techniques
Energy Technology Data Exchange (ETDEWEB)
Häussler, Wolfgang [Heinz Maier-Leibnitz Zentrum, Technische Universität München, D-85748 Garching, Germany and Physik-Department E21, Technische Universität München, D-85748 Garching (Germany); Kredler, Lukas [Physik-Department E21, Technische Universität München, D-85748 Garching (Germany)
2014-05-15
We have performed numerical ray-tracing Monte-Carlo-simulations of incoherent dynamic neutron scattering experiments. We intend to optimize the efficiency of incoherent measurements depending on the fraction of neutrons scattered without and with spin flip at the sample. In addition to conventional spin echo, we have numerically and experimentally studied oscillating intensity techniques. The results point out the advantages of these different spin echo variants and are an important prerequisite for neutron resonance spin echo instruments like RESEDA (FRM II, Munich), to choose the most efficient technique depending on the scattering vector range and the properties of the sample system under study.
Spin transport and dynamics in the F/N junction
Li, Hua; Bedell, Kevin
2015-03-01
We study the spin transport in the low temperature regime (often referred to as the precession-dominated regime) between a ferromagnetic Fermi liquid (FFL) and a normal metal metallic Fermi liquid (NFL), the F/N junction, which is considered one of the basic spintronic devices. In particular, we explore the propagation of spin waves and transport of magnetization through the interface of the F/N junction where non-equilibrium spin polarization is created on the normal metal side of the junction by spin injection. We calculate the probable spin wave modes in the precession-dominated regime on both sides of the junction especially on the NFL side where the system is out of equilibrium. Proper boundary conditions at the interface are introduced to establish the transport of the spin properties through the F/N junction. In the end, a possible transmission conduction electron spin resonance experiment is suggested on the F/N junction to see if the predicted spin wave modes could propagate through the junction.
Spin Transport and Dynamics in Antiferromagnetic Metals and Magnetic Insulators
Swaving, A.C.|info:eu-repo/dai/nl/313938083
2012-01-01
It is demonstrated that in an antiferromagnetic metal a steady-state transport current generates a current-induced out-of-plane spin density, resulting in torques on the magnetization. This spin density is parameterized by a velocity that is proportional to the current. The generalization of the
Spin transport and dynamics in magnetic insulator/metal systems
Vlietstra, Nynke
2016-01-01
In present electronics, mostly the charge of electrons is used as a carrier of information. However, the charge of electrons is not the only property of electrons; each electron also carries angular momentum, called spin. In the past decades, the possibility of using the spin of electrons as a
Spin transport and dynamics in magnetic insulator/metal systems
Vlietstra, Nynke
2016-01-01
In present electronics, mostly the charge of electrons is used as a carrier of information. However, the charge of electrons is not the only property of electrons; each electron also carries angular momentum, called spin. In the past decades, the possibility of using the spin of electrons as a carri
Magnetization dynamics of topological defects and the spin solid in a kagome artificial spin ice
Bhat, V. S.; Heimbach, F.; Stasinopoulos, I.; Grundler, D.
2016-04-01
We report broadband spin-wave spectroscopy on kagome artificial spin ice (ASI) made of large arrays of interconnected Ni80Fe20 nanobars. Spectra taken in saturated and disordered states exhibit a series of resonances with characteristic magnetic field dependencies. Making use of micromagnetic simulations, we identify resonances that reflect the spin-solid-state and monopole-antimonopole pairs on Dirac strings. The latter resonances allow for the generation of highly charged vertices in ASIs via microwave-assisted switching. Our findings open further perspectives for fundamental studies on ASIs and their usage in reprogrammable magnonics.
Directory of Open Access Journals (Sweden)
Alex Förster
Full Text Available Transient global amnesia (TGA is a transitory, short-lasting neurological disorder characterized by a sudden onset of antero- and retrograde amnesia. Perfusion abnormalities in TGA have been evaluated mainly by use of positron emission tomography (PET or single-photon emission computed tomography (SPECT. In the present study we explore the value of dynamic susceptibility contrast perfusion-weighted MRI (PWI in TGA in the acute phase.From a MRI report database we identified TGA patients who underwent MRI including PWI in the acute phase and compared these to control subjects. Quantitative perfusion maps (cerebral blood flow (CBF and volume (CBV were generated and analyzed by use of Signal Processing In NMR-Software (SPIN. CBF and CBV values in subcortical brain regions were assessed by use of VOI created in FIRST, a model-based segmentation tool in the Oxford Centre for Functional Magnetic Resonance Imaging of the Brain (FMRIB Software Library (FSL.Five TGA patients were included (2 men, 3 women. On PWI, no relevant perfusion alterations were found by visual inspection in TGA patients. Group comparisons for possible differences between TGA patients and control subjects showed significant lower rCBF values bilaterally in the hippocampus, in the left thalamus and globus pallidus as well as bilaterally in the putamen and the left caudate nucleus. Correspondingly, significant lower rCBV values were observed bilaterally in the hippocampus and the putamen as well as in the left caudate nucleus. Group comparisons for possible side differences in rCBF and rCBV values in TGA patients revealed a significant lower rCBV value in the left caudate nucleus.Mere visual inspection of PWI is not sufficient for the assessment of perfusion changes in TGA in the acute phase. Group comparisons with healthy control subjects might be useful to detect subtle perfusion changes on PWI in TGA patients. However, this should be confirmed in larger data sets and serial PWI
Energy Technology Data Exchange (ETDEWEB)
Berard, A.; Grandati, Y.; Mohrbach, H. [Universite Paul Verlaine, Institut de Physique, Laboratoire de Physique Moleculaire et des Collisions, ICPMB, IF CNRS 2843, Metz, Cedex 3 (France); Ghosh, Subir [Indian Statistical Institute, Physics and Applied Mathematics Unit, Kolkata (India); Pal, Probir [S.N. Bose National Centre for Basic Sciences, Kolkata (India)
2011-11-15
In this paper we have considered the dynamics of an anomalous (g{ne}2) charged relativistic spinning particle in the presence of an external electromagnetic field. A constraint analysis is done and the complete set of Dirac brackets are provided that generate the canonical Lorentz algebra and dynamics through Hamiltonian equations of motion. The spin-induced effective curvature of spacetime and its possible connection with Analogue Gravity models are commented upon. (orig.)
Energy Technology Data Exchange (ETDEWEB)
Adelnia, Fatemeh; Lascialfari, Alessandro [Dipartimento di Fisica, Università degli Studi di Milano and INSTM, Milano (Italy); Dipartimento di Fisica, Università degli Studi di Pavia and INSTM, Pavia (Italy); Mariani, Manuel [Dipartimento di Fisica e Astronomia, Università di Bologna, Bologna (Italy); Ammannato, Luca; Caneschi, Andrea; Rovai, Donella [Dipartimento di Chimica, Università degli Studi di Firenze and INSTM, Firenze (Italy); Winpenny, Richard; Timco, Grigore [School of Chemistry, The University of Manchester, Manchester (United Kingdom); Corti, Maurizio, E-mail: maurizio.corti@unipv.it; Borsa, Ferdinando [Dipartimento di Fisica, Università degli Studi di Pavia and INSTM, Pavia (Italy)
2015-05-07
We present the room temperature proton nuclear magnetic resonance (NMR) nuclear spin-lattice relaxation rate (NSLR) results in two 1D spin chains: the Heisenberg antiferromagnetic (AFM) Eu(hfac){sub 3}NITEt and the magnetically frustrated Gd(hfac){sub 3}NITEt. The NSLR as a function of external magnetic field can be interpreted very well in terms of high temperature spin dynamics dominated by a long time persistence of the decay of the two-spin correlation function due to the conservation of the total spin value for isotropic Heisenberg chains. The high temperature spin dynamics are also investigated in Heisenberg AFM molecular rings. In both Cr{sub 8} closed ring and in Cr{sub 7}Cd and Cr{sub 8}Zn open rings, i.e., model systems for a finite spin segment, an enhancement of the low frequency spectral density is found consistent with spin diffusion but the high cut-off frequency due to intermolecular anisotropic interactions prevents a detailed analysis of the spin diffusion regime.
Fong, C. F.; Ota, Y.; Iwamoto, S.; Arakawa, Y.
2017-06-01
Optically induced dynamic nuclear spin polarization (DNP) in a semiconductor quantum dot (QD) requires many cycles of excitation of spin polarized carriers and carrier recombination. As such, the radiative lifetime of the exciton containing the electron becomes one of the limiting factors of DNP. In principle, changing the radiative lifetime of the exciton will affect DNP and thus the nuclear spin polarization. Here, we demonstrate the manipulation of DNP in single QDs through the engineering of the photonic environment using two-dimensional photonic crystals. We find that the achievable degree of nuclear spin polarization can be controlled through the modification of exciton radiative lifetime. Our results show the promise of achieving a higher degree of nuclear spin polarization via photonic environment engineering, with implications on spin-based quantum information processing.
Spin dynamics of heavy-holes in (InGa)As quantum dots
Energy Technology Data Exchange (ETDEWEB)
Dahbashi, Ramin; Wiegand, Julia; Huebner, Jens; Oestreich, Michael [Insitute for Solid State Physics, Leibniz Universitaet Hannover, Appelstr. 2, D-30167 Hannover (Germany); Marie, Xavier [Universite de Toulouse, INSA, UPS, CNRS, LPCNO, 135 avenue de Rangueil, F-31077 Toulouse (France); Pierz, Klaus; Schumacher, Hans Werner [Physikalisch Technische Bundesanstalt, Bundesallee 100, D-38116 Braunschweig (Germany)
2013-07-01
The spin dynamics of heavy-holes confined in (InGa)As quantum dots (QDs) are of particular interest for future applications in solid state quantum information processing. We employ spin noise spectroscopy as a quantum non-demolition experiment to get access to the intrinsic spin dynamics. The spin noise method is transferred from ensembles of QDs to single dot heavy-hole measurements. Numerical simulations show an extremely long spin dephasing time if light absorption is negligible. The investigated QDs are characterized by polarization resolved photoluminescence measurements and via a Hanbury Brown-Twiss setup. The discharging of the QDs via Auger recombination due to residual light absorption is deactivated by co-pumping the dots with low intensity light.
Unified dynamics of electrons and photons via Zitterbewegung and spin-orbit interaction
Leary, C. C.; Smith, Karl H.
2014-02-01
We show that when an electron or photon propagates in a cylindrically symmetric waveguide, it experiences both a Zitterbewegung effect and a spin-orbit interaction leading to identical propagation dynamics for both particles. Applying a unified perturbative approach to both particles simultaneously, we find that to first order in perturbation theory, their Hamiltonians each contain identical Darwin (Zitterbewegung) and spin-orbit terms, resulting in the unification of their dynamics. The presence of the Zitterbewegung effect may be interpreted physically as the delocalization of the electron on the scale of its Compton wavelength, or the delocalization of the photon on the scale of its wavelength in the waveguide. The presence of the spin-orbit interaction leads to the prediction of several rotational effects: the spatial or time evolution of either particle's spin or polarization vector is controlled by the sign of its orbital angular momentum quantum number or, conversely, its spatial wave function is controlled by its spin angular momentum.
Weyl fermions and spin dynamics of metallic ferromagnet SrRuO3
Itoh, Shinichi; Endoh, Yasuo; Yokoo, Tetsuya; Ibuka, Soshi; Park, Je-Geun; Kaneko, Yoshio; Takahashi, Kei S.; Tokura, Yoshinori; Nagaosa, Naoto
2016-06-01
Weyl fermions that emerge at band crossings in momentum space caused by the spin-orbit interaction act as magnetic monopoles of the Berry curvature and contribute to a variety of novel transport phenomena such as anomalous Hall effect and magnetoresistance. However, their roles in other physical properties remain mostly unexplored. Here, we provide evidence by neutron Brillouin scattering that the spin dynamics of the metallic ferromagnet SrRuO3 in the very low energy range of milli-electron volts is closely relevant to Weyl fermions near Fermi energy. Although the observed spin wave dispersion is well described by the quadratic momentum dependence, the temperature dependence of the spin wave gap shows a nonmonotonous behaviour, which can be related to that of the anomalous Hall conductivity. This shows that the spin dynamics directly reflects the crucial role of Weyl fermions in the metallic ferromagnet.
Faithful solid state optical memory with dynamically decoupled spin wave storage.
Lovrić, Marko; Suter, Dieter; Ferrier, Alban; Goldner, Philippe
2013-07-12
We report a high fidelity optical memory in which dynamical decoupling is used to extend the storage time. This is demonstrated in a rare-earth doped crystal in which optical coherences were transferred to nuclear spin coherences and then protected against environmental noise by dynamical decoupling, leading to storage times of up to 4.2 ms. An interference experiment shows that relative phases of input pulses are preserved through the whole storage and retrieval process with a visibility ≈1, demonstrating the usefulness of dynamical decoupling for extending the storage time of quantum memories. We also show that dynamical decoupling sequences insensitive to initial spin coherence increase retrieval efficiency.
Energy Technology Data Exchange (ETDEWEB)
Sierra-Bermúdez, Sergio [Department of Chemical Engineering, University of Puerto Rico, P.O. Box 9000 Mayaguez, PR 00681 PR (United States); Maldonado-Camargo, Lorena P. [Department of Chemical Engineering, University of Florida, 1006 Center Drive, Gainesville, FL 32603 (United States); Orange, François [Department of Physics and Nanoscopy Facility, College of Natural Sciences, University of Puerto Rico, PO Box 70377, San Juan, PR 00936-8377 (United States); Guinel, Maxime J.-F. [Department of Physics and Nanoscopy Facility, College of Natural Sciences, University of Puerto Rico, PO Box 70377, San Juan, PR 00936-8377 (United States); Department of Chemistry, College of Natural Sciences, University of Puerto Rico, PO Box 70377, San Juan, PR 00936-8377 (United States); Rinaldi, Carlos, E-mail: carlos.rinaldi@bme.ufl.edu [J. Crayton Pruitt Family Department of Biomedical Engineering, University of Florida, PO Box 116131, Gainesville, FL 32611-6131 (United States)
2015-03-15
Aggregation of magnetic nanoparticles in polymer melts was assessed using dynamic magnetic susceptibility measurements. Magnetic nanocomposites consisting of polybutadiene/CoFe{sub 2}O{sub 4} and polystyrene/CoFe{sub 2}O{sub 4} mixtures were prepared using different techniques and characterized using dynamic magnetic susceptibility measurements. The presence of nanoparticle aggregates determined using magnetic measurements was confirmed with transmission electron microscopy examinations. The results were in good agreement with predictions from the Flory–Huggins interaction parameters. - Highlights: • Oleic acid coated magnetic nanoparticles (MNPs) were dispersed in polymer melts. • MNPs dispersed well in polybutadiene but not in polystyrene. • Dynamic magnetic susceptibility (DMS) measurements assessed presence of aggregates. • DMS predictions were confirmed by transmission electron microscopy. • The Flory-Huggins interaction parameter correlated with MNP dispersion.
Magnetism of metals in the dynamic spin-fluctuation theory
Melnikov, N. B.; Reser, B. I.
2016-12-01
We overview new developments in spin-fluctuation theory, which describes magnetic properties of ferromagnetic metals at finite temperatures. We present a detailed analysis of the underlying techniques and compare numerical results with experiment.
Effect of a cosmic string on spin dynamics
Chowdhury, Debashree; Basu, B.
2014-12-01
In the present paper, we have investigated the role of the cosmic string on spin current and Hall electric field. Due to the background cosmic string, the modified electric field of the system generates renormalized spin-orbit coupling, which induces a modified non-Abelian gauge field. The defect causes a change in the Aharonov-Bohm and Aharonov-Casher phases appearing due to the modified electromagnetic field. In addition, for a time varying electric field we perform explicit analytic calculations to derive the exact form of spin electric field and spin current, which is defect parameter dependent and of oscillating type. Furthermore, in an asymmetric crystal within the Drude model approach we investigate the dependence of the cosmic string parameters on cosmic string induced Hall electric field.
Atom-diatom scattering dynamics of spinning molecules
Energy Technology Data Exchange (ETDEWEB)
Eyles, C. J. [Institut für Chemie und Biochemie, Freie Universität Berlin, 14195 Berlin (Germany); Floß, J.; Averbukh, I. Sh. [Department of Chemical Physics, Weizmann Institute of Science, Rehovot 76100 (Israel); Leibscher, M. [Institut für Theoretische Physik, Leibniz Universität Hannover, 30167 Hannover (Germany)
2015-01-14
We present full quantum mechanical scattering calculations using spinning molecules as target states for nuclear spin selective atom-diatom scattering of reactive D+H{sub 2} and F+H{sub 2} collisions. Molecules can be forced to rotate uni-directionally by chiral trains of short, non-resonant laser pulses, with different nuclear spin isomers rotating in opposite directions. The calculations we present are based on rotational wavepackets that can be created in this manner. As our simulations show, target molecules with opposite sense of rotation are predominantly scattered in opposite directions, opening routes for spatially and quantum state selective scattering of close chemical species. Moreover, two-dimensional state resolved differential cross sections reveal detailed information about the scattering mechanisms, which can be explained to a large degree by a classical vector model for scattering with spinning molecules.
Dynamics of an all-optical atomic spin gyroscope.
Fang, Jiancheng; Wan, Shuangai; Yuan, Heng
2013-10-20
We present the transfer function of an all-optical atomic spin gyroscope through a series of differential equations and validate the transfer function by experimental test. A transfer function is the basis for further control system design. We build the differential equations based on a complete set of Bloch equations describing the all-optical atomic spin gyroscope, and obtain the transfer function through application of the Laplace transformation to these differential equations. Moreover, we experimentally validate the transfer function in an all-optical Cs-Xe129 atomic spin gyroscope through a series of step responses. This transfer function is convenient for analysis of the form of control system required. Furthermore, it is available for the design of the control system specifically to improve the performance of all-optical atomic spin gyroscopes.
Spin effects on the dynamics of compact binaries
Steinhoff, Jan
2015-01-01
Compact binaries are the most promising source for the advanced gravitational wave detectors, which will start operating this year. The influence of spin on the binary evolution is an important consequence of general relativity and can be large. It is argued that the spin supplementary condition, which is related to the observer dependence of the center, gives rise to a gauge symmetry in the action principle of spinning point-particles. These spinning point-particles serve as an analytic model for extended bodies. The internal structure can be modelled by augmenting the point-particle with higher-order multipole moments. Consequences of the recently discovered universal (equation of state independent) relations between the multipole moments of neutron stars are discussed.
Photoexcited Eu2+ spin dynamics in EuFe2As2
Pogrebna, A.; Mertelj, T.; Cao, G.; Xu, Z. A.; Mihailovic, D.
2014-06-01
Employing temperature dependent time-resolved optical femtosecond spectroscopy, we investigated the quasiparticle and Eu2+ spin relaxation dynamics in EuFe2As2 (EFA). As previously reported in other undoped iron-based pnictides, we observe the quasiparticle relaxation bottleneck due to the charge gap opening in the spin density wave (SDW) state below T SDW = 189 K. Below the Eu2+ antiferromagnetic (AFM) spin ordering temperature, T AFM = 19 K, we observe another slower relaxation component, which we attribute to the Eu2+ AFM order dynamics. The slow dynamics of this component suggests a weak coupling between the Eu2+ spins and the carriers in the Fe- d derived bands.
Energy Technology Data Exchange (ETDEWEB)
Jungfleisch, Matthias B., E-mail: jungfleisch@anl.gov; Zhang, Wei; Ding, Junjia; Jiang, Wanjun; Pearson, John E.; Hoffmann, Axel [Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439 (United States); Sklenar, Joseph [Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439 (United States); Department of Physics and Astronomy, Northwestern University, Evanston, Illinois 60208 (United States); Ketterson, John B. [Department of Physics and Astronomy, Northwestern University, Evanston, Illinois 60208 (United States)
2016-02-01
The understanding of spin dynamics in laterally confined structures on sub-micron length scales has become a significant aspect of the development of novel magnetic storage technologies. Numerous ferromagnetic resonance measurements, optical characterization by Kerr microscopy and Brillouin light scattering spectroscopy, and x-ray studies were carried out to detect the dynamics in patterned magnetic antidot lattices. Here, we investigate Oersted-field driven spin dynamics in rectangular Ni{sub 80}Fe{sub 20}/Pt antidot lattices with different lattice parameters by electrical means and compare them to micromagnetic simulations. When the system is driven to resonance, a dc voltage across the length of the sample is detected that changes its sign upon field reversal, which is in agreement with a rectification mechanism based on the inverse spin Hall effect. Furthermore, we show that the voltage output scales linearly with the applied microwave drive in the investigated range of powers. Our findings have direct implications on the development of engineered magnonics applications and devices.
Collective dynamics in atomistic models with coupled translational and spin degrees of freedom
Perera, Dilina; Nicholson, Don M.; Eisenbach, Markus; Stocks, G. Malcolm; Landau, David P.
2017-01-01
Using an atomistic model that simultaneously treats the dynamics of translational and spin degrees of freedom, we perform combined molecular and spin dynamics simulations to investigate the mutual influence of the phonons and magnons on their respective frequency spectra and lifetimes in ferromagnetic bcc iron. By calculating the Fourier transforms of the space- and time-displaced correlation functions, the characteristic frequencies and the linewidths of the vibrational and magnetic excitation modes were determined. Comparison of the results with that of the stand-alone molecular dynamics and spin dynamics simulations reveals that the dynamic interplay between the phonons and magnons leads to a shift in the respective frequency spectra and a decrease in the lifetimes. Moreover, in the presence of lattice vibrations, additional longitudinal magnetic excitations were observed with the same frequencies as the longitudinal phonons.
Rényi information flow in the Ising model with single-spin dynamics
Deng, Zehui; Wu, Jinshan; Guo, Wenan
2014-12-01
The n -index Rényi mutual information and transfer entropies for the two-dimensional kinetic Ising model with arbitrary single-spin dynamics in the thermodynamic limit are derived as functions of ensemble averages of observables and spin-flip probabilities. Cluster Monte Carlo algorithms with different dynamics from the single-spin dynamics are thus applicable to estimate the transfer entropies. By means of Monte Carlo simulations with the Wolff algorithm, we calculate the information flows in the Ising model with the Metropolis dynamics and the Glauber dynamics, respectively. We find that not only the global Rényi transfer entropy, but also the pairwise Rényi transfer entropy, peaks in the disorder phase.
Mikolasek, Mirko; Nicolazzi, William; Terki, Férial; Molnár, Gábor; Bousseksou, Azzedine
2017-07-01
In the first part of this work, an experimental study of the lattice dynamics of spin crossover nanoparticles was performed using the nuclear inelastic scattering (NIS). A size dependence of low energy phonon modes appears under 10 nm, but its origin is not well understood. In this paper, we investigate the phonon confinement effects in the framework of molecular dynamics simulations by modeling three-dimensional nanoparticles considering a cubic lattice with an octahedral pattern. The vibrational density of states is computed and compared to the experiment. The simulations allow one to highlight both the role of the phonon quantification and the role of the size and shape distributions of particles on the extracted parameters leading to a better understanding of the experimental results.
Nonlinear damping effects in spin torque dynamics of magnetic tunnel junctions
Barsukov, Igor; Chen, Yu-Jin; Lee, Han Kyu; Goncalves, Alexandre; Katine, Jordan; Arias, Rodrigo; Ivanov, Boris; Krivorotov, Ilya
2015-03-01
Performance of nanoscale spin torque devices such as memory (STT-MRAM) and auto-oscillators critically depends on magnetic relaxation. It is commonly assumed that magnetization dynamics in the presence of spin torque can be understood as simple competition between antidamping arising from spin torque and Gilbert damping of the free layer. However our experiments reveal that the situation is more complex and that nonlinear damping processes in the free layer of magnetic tunnel junction (MTJ) nanopillars can strongly alter spin torque driven dynamics. We study elliptical MTJ nanopillars with in-plane magnetizations of the free layer and SAF layers by spin torque ferromagnetic resonance. We find an excitation spectrum associated with standing spin waves of the free layer. By varying the external field, the energy of a higher-order spin wave mode becomes twice the energy of the main mode. This opens up a nonlinear, resonant relaxation channel, giving rise to a damping increase of approximately 20 percent. With increasing spin torque provided by a DC bias current, we find that this relaxation channel competes with antidamping in a nonlinear manner, increasingly contributing to and even dominating the relaxation at subcritical currents.
Theory of spin dynamics of magnetic adatoms traced by time-resolved scanning tunneling spectroscopy
Schüler, Michael; Berakdar, Jamal
2012-01-01
The inelastic scanning tunneling microscopy (STM) has been shown recently (Loth et al. Science 329, 1628 (2010)) to be extendable as to access the nanosecond, spin-resolved dynamics of magnetic adatoms and molecules. Here we analyze theoretically this novel tool by considering the time-resolved spin dynamics of a single adsorbed Fe atom excited by a tunneling current pulse from a spin-polarized STM tip. The adatom spin-configuration can be controlled and probed by applying voltage pulses between the substrate and the spin-polarized STM tip. We demonstrate how, in a pump-probe manner, the relaxation dynamics of the sample spin is manifested in the spin-dependent tunneling current. Our model calculations are based on the scattering theory in a wave-packet formulation. The scheme is nonpertubative and hence, is valid for all voltages. The numerical results for the tunneling probability and the conductance are contrasted with the prediction of simple analytical models and compared with experiments.
Materials optimization and ghz spin dynamics of metallic ferromagnetic thin film heterostructures
Cheng, Cheng
Metallic ferromagnetic (FM) thin film heterostructures play an important role in emerging magnetoelectronic devices, which introduce the spin degree of freedom of electrons into conventional charge-based electronic devices. As the majority of magnetoelectronic devices operate in the GHz frequency range, it is critical to understand the high-frequency magnetization dynamics in these structures. In this thesis, we start with the static magnetic properties of FM thin films and their optimization via the field-sputtering process incorporating a specially designed in-situ electromagnet. We focus on the origins of anisotropy and hysteresis/coercivity in soft magnetic thin films, which are most relevant to magentic susceptibility and power dissipation in applications in the sub-GHz frequency regime, such as magnetic-core integrated inductors. Next we explore GHz magnetization dynamics in thin-film heterostructures, both in semi-infinite samples and confined geometries. All investigations are rooted in the Landau-Lifshitz-Gilbert (LLG) equation, the equation of motion for magnetization. The phenomenological Gilbert damping parameter in the LLG equation has been interpreted, since the 1970's, in terms of the electrical resistivity. We present the first interpretation of the size effect in Gilbert damping in single metallic FM films based on this electron theory of damping. The LLG equation is intrinsically nonlinear, which provides possibilities for rf signal processing. We analyze the frequency doubling effect at small-angle magnetization precession from the first-order expansion of the LLG equation, and demonstrate second harmonic generation from Ni81 Fe19 (Permalloy) thin film under ferromagnetic resonance (FMR), three orders of magnitude more efficient than in ferrites traditionally used in rf devices. Though the efficiency is less than in semiconductor devices, we provide field- and frequency-selectivity in the second harmonic generation. To address further the
Bartley, David L
2016-01-01
The Bohm/de Broglie theory of deterministic non-relativistic quantum mechanics is broadened to accommodate the free-particle Dirac equation. As with the spin-0 theory, an effective particle rest-mass scalar field in the presence of the spin-1/2 pilot wave is allowed, together with the assumption that the convective current component describes ensemble dynamics. Non-positive excursions of the ensemble density for extreme cases of positive-energy solutions of the Dirac equation are interpreted in terms of virtual-like pair creation and annihilation beneath the Compton wavelength. A specific second-rank tensor is defined in terms of the Dirac spinors for generalizing from simply a quantum potential to a stress tensor required to account for the force of pilot wave on particle. A simple dependence of the stress tensor on a two-component spin pseudovector field is determined. Consistency is found with an earlier non-relativistic theory of objects with spin.
Golysheva, Elena A.; Shevelev, Georgiy Yu.; Dzuba, Sergei A.
2017-08-01
In glassy substances and biological media, dynamical transitions are observed in neutron scattering that manifests itself as deviations of the translational mean-squared displacement, , of hydrogen atoms from harmonic dynamics. In biological media, the deviation occurs at two temperature intervals, at ˜100-150 K and at ˜170-230 K, and it is attributed to the motion of methyl groups in the former case and to the transition from harmonic to anharmonic or diffusive motions in the latter case. In this work, electron spin echo (ESE) spectroscopy—a pulsed version of electron paramagnetic resonance—is applied to study the spin relaxation of nitroxide spin probes and labels introduced in molecular glass former o-terphenyl and in protein lysozyme. The anisotropic contribution to the rate of the two-pulse ESE decay, ΔW, is induced by spin relaxation appearing because of restricted orientational stochastic molecular motion; it is proportional to τc, where is the mean-squared angle of reorientation of the nitroxide molecule around the equilibrium position and τc is the correlation time of reorientation. The ESE time window allows us to study motions with τc τc temperature dependence shows a transition near 240 K, which is in agreement with the literature data on . For spin probes of essentially different size, the obtained data were found to be close, which evidences that motion is cooperative, involving a nanocluster of several neighboring molecules. For the dry lysozyme, the τc values below 260 K were found to linearly depend on the temperature in the same way as it was observed in neutron scattering for . As spin relaxation is influenced only by stochastic motion, the harmonic motions seen in ESE must be overdamped. In the hydrated lysozyme, ESE data show transitions near 130 K for all nitroxides, near 160 K for the probe located in the hydration layer, and near 180 K for the label in the protein interior. For this system, the two latter transitions are not
Spin currents and magnon dynamics in insulating magnets
Nakata, Kouki; Simon, Pascal; Loss, Daniel
2017-03-01
Nambu–Goldstone theorem provides gapless modes to both relativistic and nonrelativistic systems. The Nambu–Goldstone bosons in insulating magnets are called magnons or spin-waves and play a key role in magnetization transport. We review here our past works on magnetization transport in insulating magnets and also add new insights, with a particular focus on magnon transport. We summarize in detail the magnon counterparts of electron transport, such as the Wiedemann–Franz law, the Onsager reciprocal relation between the Seebeck and Peltier coefficients, the Hall effects, the superconducting state, the Josephson effects, and the persistent quantized current in a ring to list a few. Focusing on the electromagnetism of moving magnons, i.e. magnetic dipoles, we theoretically propose a way to directly measure magnon currents. As a consequence of the Mermin–Wagner–Hohenberg theorem, spin transport is drastically altered in one-dimensional antiferromagnetic (AF) spin-1/2 chains; where the Néel order is destroyed by quantum fluctuations and a quasiparticle magnon-like picture breaks down. Instead, the low-energy collective excitations of the AF spin chain are described by a Tomonaga–Luttinger liquid (TLL) which provides the spin transport properties in such antiferromagnets some universal features at low enough temperature. Finally, we enumerate open issues and provide a platform to discuss the future directions of magnonics.
Dynamics of Polymer Blend Film Formation During Spin Coating
Mouhamad, Youmna; Clarke, Nigel; Jones, Richard A. L.; Geoghegan, Mark
2012-02-01
Spin casting is a process broadly used to obtain a uniform film on a flat substrate. A homogeneous film results from the balance between centrifugal and viscous forces. Here we revisit the Meyerhofer model of the spin casting process by taking in account the centrifugal forces, a uniform time dependent evaporation rate, and account for the changes in viscosity using the Huggins intrinsic viscosity. Time resolved light reflectometry is used to monitor the thickness changes of a polystyrene-poly(methyl methacrylate)(which we denote as PS and PMMA) film initially dissolved in toluene and spin cast for ten seconds at 1000 rpm. The experimental data are in good agreement with the model. We also investigate how the volume fraction of PS and PMMA influences the thinning of the film during spin casting. A distinct change in the temporal evolution of thickness as a function of time delimits the first phase of the spin casting process where centrifugal forces are dominant from a second phase dominated by the solvent evaporation. This hypothesis is supported by in-situ off specular scattering data. The time at which this change from centrifugal to evaporation-dominated behaviour is delayed as the volume fraction of PMMA increases.
Dynamics of antiferromagnetic skyrmion driven by the spin Hall effect
Jin, Chendong; Song, Chengkun; Wang, Jianbo; Liu, Qingfang
2016-10-01
Magnetic skyrmion moved by the spin-Hall effect is promising for the application of the generation racetrack memories. However, the Magnus force causes a deflected motion of skyrmion, which limits its application. Here, we create an antiferromagnetic skyrmion by injecting a spin-polarized pulse in the nanostripe and investigate the spin Hall effect-induced motion of antiferromagnetic skyrmion by micromagnetic simulations. In contrast to ferromagnetic skyrmion, we find that the antiferromagnetic skyrmion has three evident advantages: (i) the minimum driving current density of antiferromagnetic skyrmion is about two orders smaller than the ferromagnetic skyrmion; (ii) the velocity of the antiferromagnetic skyrmion is about 57 times larger than the ferromagnetic skyrmion driven by the same value of current density; (iii) antiferromagnetic skyrmion can be driven by the spin Hall effect without the influence of Magnus force. In addition, antiferromagnetic skyrmion can move around the pinning sites due to its property of topological protection. Our results present the understanding of antiferromagnetic skyrmion motion driven by the spin Hall effect and may also contribute to the development of antiferromagnetic skyrmion-based racetrack memories.
Kumar, D. Sanjeev; Mukhopadhyay, Soma; Chatterjee, Ashok
2016-11-01
The magnetization and susceptibility of a two-electron parabolic quantum dot are studied in the presence of electron-electron and spin-orbit interactions as a function of magnetic field and temperature. The spin-orbit interactions are treated by a unitary transformation and an exactly soluble parabolic interaction model is considered to mimic the electron-electron interaction. The theory is finally applied to an InAs quantum dot. Magnetization and susceptibility are calculated using canonical ensemble approach. Our results show that Temperature has no effect on magnetization and susceptibility in the diamagnetic regime whereas electron-electron interaction reduces them. The temperature however reduces the height of the paramagnetic peak. The Rashba spin-orbit interaction is shown to shift the paramagnetic peak towards higher magnetic fields whereas the Dresselhaus spin-orbit interaction shifts it to the lower magnetic field side. Spin-orbit interaction has no effect on magnetization and susceptibility at larger temperatures.
Influence of the black hole spin on the chaotic particle dynamics within a dipolar halo
Nag, Sankhasubhra; Sinha, Siddhartha; Ananda, Deepika B.; Das, Tapas K.
2017-04-01
We investigate the role of the spin angular momentum of astrophysical black holes in controlling the special relativistic chaotic dynamics of test particles moving under the influence of a post-Newtonian pseudo-Kerr black hole potential, along with a perturbative potential created by an asymmetrically placed (dipolar) halo. Proposing a Lyapunov-like exponent to be the effective measure of the degree of chaos observed in the system under consideration, it has been found that black hole spin anti-correlates with the degree of chaos for the aforementioned dynamics. Our findings have been explained applying the general principles of dynamical systems analysis.
Influence of the black hole spin on the chaotic particle dynamics within a dipolar halo
Nag, Sankhasubhra; Ananda, Deepika B; Das, Tapas K
2016-01-01
We investigate the role of the spin angular momentum of astrophysical black holes in controlling the special relativistic chaotic dynamics of test particles moving under the influence of a post-Newtonian pseudo-Kerr black hole potential, along with a perturbative potential created by a asymmetrically placed (dipolar) halo. Proposing a Lyapunov-like exponent to be the effective measure of the degree of chaos observed in the system under consideration, it has been found that black hole spin anti-correlates with the degree of chaos for the aforementioned dynamics. Our findings have been explained applying the general principles of dynamical systems analysis.
Dynamics of Genuine Three-Qubit Entanglement in Ising Spin Systems
Institute of Scientific and Technical Information of China (English)
PANG Chao-Yang; LI Yu-Liang
2006-01-01
We investigate the dynamics of genuine three-qubit entanglement in the Ising model of three spins. A scheme is presented for generating the genuine three-qubit entanglement by the nearest-neighbour couplings. The effect of magnetic fields on the dynamics of genuine three-qubit entanglement is also discussed.
Exact solutions for spin-1/2 systems using dynamical manipulation techniques
Fernández-Cesar, C; Rosas-Ortiz, Oscar
1997-01-01
The dynamics of purely spin-1/2 systems in homogeneous magnetic fields is analysed through inverse techniques. The generation of exact solutions using this method is explored. Some cases of the "evolution loops", dynamical processes for which any state evolves cyclically, are presented, and the corresponding geometric phases are evaluated.
Comparison of quantum and classical relaxation in spin dynamics.
Wieser, R
2013-04-01
The classical Landau-Lifshitz equation with a damping term has been derived from the time evolution of a quantum mechanical wave function under the assumption of a non-Hermitian Hamilton operator. Further, the trajectory of a classical spin (S) has been compared with the expectation value of the spin operator (Ŝ). A good agreement between classical and quantum mechanical trajectories can be found for Hamiltonians linear in Ŝ or S, respectively. Quadratic or higher order terms in the Hamiltonian result in a disagreement.
Spin-cast bulk heterojunction solar cells: A dynamical investigation
Chou, Kang Wei
2013-02-22
Spin-coating is extensively used in the lab-based manufacture of organic solar cells, including most of the record-setting solution-processed cells. We report the first direct observation of photoactive layer formation as it occurs during spin-coating. The study provides new insight into mechanisms and kinetics of bulk heterojunction formation, which may be crucial for its successful transfer to scalable printing processes. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Low frequency spin dynamics in the quantum magnet copper pyrazine dinitrate
Energy Technology Data Exchange (ETDEWEB)
Kuehne, H.; Klauss, H.H. [Institut fuer Festkoerperphysik, TU Dresden Dresden (Germany); Institut fuer Physik der Kondensierten Materie, TU Braunschweig (Germany); Guenther, M. [Institut fuer Festkoerperphysik, TU Dresden Dresden (Germany); Grossjohann, S.; Brenig, W. [Institut fuer Theoretische Physik, TU Braunschweig (Germany); Litterst, F.J. [Institut fuer Physik der Kondensierten Materie, TU Braunschweig (Germany); Reyes, A.P.; Kuhns, P.L. [National High Magnetic Field Laboratory, Tallahassee, FL (United States); Turnbull, M.M.; Landee, C.P. [Carlson School of Chemistry and Department of Physics, Clark University, Worcester, MA (United States)
2010-03-15
The S = 1/2 antiferromagnetic Heisenberg chain exhibits a magnetic field driven quantum critical point. We study the low frequency spin dynamics in copper pyrazine dinitrate (CuPzN), a realization of this model system of quantum magnetism, by means of {sup 13}C-NMR spectroscopy. Measurements of the nuclear spin-lattice relaxation rate T{sub 1}{sup -} {sup 1} in the vicinity of the saturation field are compared with quantum Monte Carlo calculations of the dynamic structure factor. Both show a strong divergence of low energy excitations at temperatures in the quantum regime. The analysis of the anisotropic T{sub 1}{sup -} {sup 1}-rates and frequency shifts allows one to disentangle the contributions from transverse and longitudinal spin fluctuations for a selective study and to determine the transfer of delocalized spin moments from copper to the neighboring nitrogen atoms. (Abstract Copyright [2010], Wiley Periodicals, Inc.)
Energy Technology Data Exchange (ETDEWEB)
Pohlit, Merlin, E-mail: pohlit@physik.uni-frankfurt.de; Porrati, Fabrizio; Huth, Michael; Müller, Jens [Institute of Physics, Goethe-University Frankfurt, Frankfurt/Main (Germany); Stockem, Irina; Schröder, Christian [Bielefeld Institute for Applied Materials Research, FH Bielefeld-University of Applied Sciences, Bielefeld (Germany)
2016-10-14
We study the magnetization dynamics of a spin ice cluster which is a building block of an artificial square spin ice fabricated by focused electron-beam-induced deposition both experimentally and theoretically. The spin ice cluster is composed of twelve interacting Co nanoislands grown directly on top of a high-resolution micro-Hall sensor. By employing micromagnetic simulations and a macrospin model, we calculate the magnetization and the experimentally investigated stray field emanating from a single nanoisland. The parameters determined from a comparison with the experimental hysteresis loop are used to derive an effective single-dipole macrospin model that allows us to investigate the dynamics of the spin ice cluster. Our model reproduces the experimentally observed non-deterministic sequences in the magnetization curves as well as the distinct temperature dependence of the hysteresis loop.
Pohlit, Merlin; Stockem, Irina; Porrati, Fabrizio; Huth, Michael; Schröder, Christian; Müller, Jens
2016-10-01
We study the magnetization dynamics of a spin ice cluster which is a building block of an artificial square spin ice fabricated by focused electron-beam-induced deposition both experimentally and theoretically. The spin ice cluster is composed of twelve interacting Co nanoislands grown directly on top of a high-resolution micro-Hall sensor. By employing micromagnetic simulations and a macrospin model, we calculate the magnetization and the experimentally investigated stray field emanating from a single nanoisland. The parameters determined from a comparison with the experimental hysteresis loop are used to derive an effective single-dipole macrospin model that allows us to investigate the dynamics of the spin ice cluster. Our model reproduces the experimentally observed non-deterministic sequences in the magnetization curves as well as the distinct temperature dependence of the hysteresis loop.
Dynamical skyrmion state in a spin current nano-oscillator with perpendicular magnetic anisotropy.
Liu, R H; Lim, W L; Urazhdin, S
2015-04-03
We study the spectral characteristics of spin current nano-oscillators based on the Pt/[Co/Ni] magnetic multilayer with perpendicular magnetic anisotropy. By varying the applied magnetic field and current, both localized and propagating spin wave modes of the oscillation are achieved. At small fields, we observe an abrupt onset of the modulation sidebands. We use micromagnetic simulations to identify this state as a dynamical magnetic skyrmion stabilized in the active device region by spin current injection, whose current-induced dynamics is accompanied by the gyrotropic motion of the core due to the skew deflection. Our results demonstrate a practical route for controllable skyrmion manipulation by spin current in magnetic thin films.
Magnetic correlation, excitation and slow dynamics in concentrated spin-glass alloys
Indian Academy of Sciences (India)
Kiyoichiro Motoya
2004-07-01
Three kinds of neutron scattering experiments have been performed to clarify the role of magnetic clusters on the various properties of re-entrant spin-glasses. The presence of two kinds of spin-wave excitations, the limitations of magnetic phase diagrams and the mechanism of slow dynamics have been discussed based on the results of in-elastic scattering, diffuse scattering and time-resolved small-angle scattering experiments, respectively.
Semiclassical dynamics of a spin-1/2 in an arbitrary magnetic field
Alscher, Adrian; Grabert, Hermann
1999-01-01
The spin coherent state path integral describing the dynamics of a spin-1/2-system in a magnetic field of arbitrary time-dependence is considered. Defining the path integral as the limit of a Wiener regularized expression, the semiclassical approximation leads to a continuous minimal action path with jumps at the endpoints. The resulting semiclassical propagator is shown to coincide with the exact quantum mechanical propagator. A non-linear transformation of the angle variables allows for a d...
Spin dynamics and hyperfine interaction in InAs semiconductor quantum dots
Energy Technology Data Exchange (ETDEWEB)
Eble, B.; Krebs, O.; Voisin, P.; Lemaitre, A.; Kudelski, A. [CNRS - Laboratoire de Photonique et Nanostructures, Route de Nozay, 91460 Marcoussis (France); Braun, P.F.; Lombez, L.; Marie, X.; Urbaszek, B.; Amand, T.; Lagarde, D.; Renucci, P. [Laboratoire de Nanophysique Magnetisme et Optoelectronique, INSA, 31077 Toulouse Cedex 4 (France); Kowalik, K. [CNRS - Laboratoire de Photonique et Nanostructures, Route de Nozay, 91460 Marcoussis (France); Institute of Experimental Physics, Warsaw University, Hoza 69, 00-681 Warsaw (Poland); Kalevich, V.K.; Kavokin, K.V. [Ioffe Institute, Politekhnicheskaya 26, St-Petersburg 194021 (Russian Federation)
2006-08-15
We present a detailed study of the hyperfine interaction between carrier and nuclear spins in InAs semiconductor quantum dots. Time resolved measurements on excitons in positively charged quantum dots show the electron spin relaxation due to random fluctuations of the spin orientation of the nuclei in the quantum dot. A complimentary aspect of the hyperfine interaction can be uncovered in single dot continuous wave photoluminescence experiments in a weak magnetic field, namely the Overhauser shift due to the dynamic polarisation of the nuclei following excitation with circularly polarised light. (copyright 2006 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)
Generating highly polarized nuclear spins in solution using dynamic nuclear polarization
DEFF Research Database (Denmark)
Wolber, J.; Ellner, F.; Fridlund, B.;
2004-01-01
and other low-γ nuclei. Subsequent to the DNP process, the solid sample is dissolved rapidly with a warm solvent to create a solution of molecules with highly polarized nuclear spins. Two main applications are proposed: high-resolution liquid state NMR with enhanced sensitivity, and the use......A method to generate strongly polarized nuclear spins in solution has been developed, using Dynamic Nuclear Polarization (DNP) at a temperature of 1.2K, and at a field of 3.354T, corresponding to an electron spin resonance frequency of 94GHz. Trityl radicals are used to directly polarize 13C...
First-principles approach to noncollinear magnetism: Towards spin dynamics
DEFF Research Database (Denmark)
Sharma, S.; Dewhurst, J.K.; Ambrosch-Draxl, C.;
2007-01-01
A description of noncollinear magnetism in the framework of spin-density functional theory is presented for the exact exchange energy functional which depends explicitly on two-component spinor orbitals. The equations for the effective Kohn-Sham scalar potential and magnetic field are derived...
Computational fluid dynamics model of the spinning pipe gas lens
CSIR Research Space (South Africa)
Mafusire, C
2010-08-01
Full Text Available When a metal horizontal pipe is heated and spun along its axis, a graded refractive index distribution is generated which is can be used as a lens, thus its name, the spinning pipe gas lens (SPGL). Previous experimental results of its performance...
Two-level system in spin baths: non-adiabatic dynamics and heat transport.
Segal, Dvira
2014-04-28
We study the non-adiabatic dynamics of a two-state subsystem in a bath of independent spins using the non-interacting blip approximation, and derive an exact analytic expression for the relevant memory kernel. We show that in the thermodynamic limit, when the subsystem-bath coupling is diluted (uniformly) over many (infinite) degrees of freedom, our expression reduces to known results, corresponding to the harmonic bath with an effective, temperature-dependent, spectral density function. We then proceed and study the heat current characteristics in the out-of-equilibrium spin-spin-bath model, with a two-state subsystem bridging two thermal spin-baths of different temperatures. We compare the behavior of this model to the case of a spin connecting boson baths, and demonstrate pronounced qualitative differences between the two models. Specifically, we focus on the development of the thermal diode effect, and show that the spin-spin-bath model cannot support it at weak (subsystem-bath) coupling, while in the intermediate-strong coupling regime its rectifying performance outplays the spin-boson model.
Chekhovich, Evgeny A.
2017-06-01
Dynamics of nuclear spin decoherence and nuclear spin flip-flops in self-assembled InGaAs/GaAs quantum dots are studied experimentally using optically detected nuclear magnetic resonance (NMR). Nuclear spin-echo decay times are found to be in the range 1-4 ms. This is a factor of ~3 longer than in strain-free GaAs/AlGaAs structures and is shown to result from strain-induced quadrupolar effects that suppress nuclear spin flip-flops. The correlation times of the flip-flops are examined using a novel frequency-comb NMR technique and are found to exceed 1 s, a factor of ~1000 longer than in strain-free structures. These findings complement recent studies of electron spin coherence and reveal the paradoxical dual role of the quadrupolar effects in self-assembled quantum dots: large increase of the nuclear spin bath coherence and at the same time significant reduction of the electron spin-qubit coherence. Approaches to increasing electron spin coherence are discussed. In particular the nanohole filled GaAs/AlGaAs quantum dots are an attractive option: while their optical quality matches the self-assembled dots the quadrupolar effects measured in NMR spectra are a factor of 1000 smaller.
Wang, H; Kühn, O
2016-01-01
Recent developments in attosecond spectroscopy yield access to the correlated motion of electrons on their intrinsic time scales. Spin-flip dynamics is usually considered in the context of valence electronic states, where spin-orbit coupling is weak and processes related to the electron spin are usually driven by nuclear motion. However, for core-excited states, where the core hole has a nonzero angular momentum, spin-orbit coupling is strong enough to drive spin-flips on a much shorter time scale. Using density matrix based time-dependent restricted active space configuration interaction including spin-orbit coupling, we address an unprecedentedly short spin-crossover for the example of L-edge (2p$\\rightarrow$3d) excited states of a prototypical Fe(II) complex. This process occurs on a time scale, which is faster than that of Auger decay ($\\sim$4\\,fs) treated here explicitly. Modest variations of carrier frequency and pulse duration can lead to substantial changes in the spin-state yield, suggesting its cont...
Harms, Enno; Bernuzzi, Sebastiano; Nagar, Alessandro
2016-01-01
We consider a spinning test-body in circular motion around a nonrotating black hole and analyze different prescriptions for the body's dynamics. We compare, for the first time, the Mathisson-Papapetrou formalism under the Tulczyjew spin-supplementary-condition (SSC), the Pirani SSC and the Ohashi-Kyrian-Semerak SSC, and the spinning particle limit of the effective-one-body Hamiltonian of [Phys.~Rev.~D.90,~044018(2014)]. We analyze the four different dynamics in terms of the ISCO shifts and in terms of the coordinate invariant binding energies, separating higher-order spin contributions from spin-orbit contributions. The asymptotic gravitational wave fluxes produced by the spinning body are computed by solving the inhomogeneous $(2+1)D$ Teukolsky equation and contrasted for the different cases. For small orbital frequencies $\\Omega$, all the prescriptions reduce to the same dynamics and the same radiation fluxes. For large frequencies, ${x \\equiv (M \\Omega)^{2/3} >0.1 }$, where $M$ is the black hole mass, and ...
Belykh, V. V.; Evers, E.; Yakovlev, D. R.; Fobbe, F.; Greilich, A.; Bayer, M.
2016-12-01
We develop an extended pump-probe Faraday rotation technique to study submicrosecond electron spin dynamics with picosecond time resolution in a wide range of magnetic fields. The electron spin dephasing time T2* and the longitudinal spin relaxation time T1, both approaching 250 ns in weak fields, are measured thereby in n -type bulk GaAs. By tailoring the pump pulse train through increasing the contained number of pulses, the buildup of resonant spin amplification is demonstrated for the electron spin polarization. The spin precession amplitude in high magnetic fields applied in the Voigt geometry shows a nonmonotonic dynamics deviating strongly from a monoexponential decay and revealing slow beatings. The beatings indicate a two spin component behavior with a g -factor difference of Δ g ˜4 ×10-4 , much smaller than the Δ g expected for free and donor-bound electrons. This g -factor variation indicates efficient, but incomplete spin exchange averaging.
Mi, Qixi; Chernick, Erin T; McCamant, David W; Weiss, Emily A; Ratner, Mark A; Wasielewski, Michael R
2006-06-15
The stable free radical 2,2,6,6-tetramethylpiperidinoxyl (TEMPO, T*) was covalently attached to the electron acceptor in a donor-chromophore-acceptor (D-C-A) system, MeOAn-6ANI-Phn-A-T*, having well-defined distances between each component, where MeOAn = p-methoxyaniline, 6ANI = 4-(N-piperidinyl)naphthalene-l,8-dicarboximide, Ph = 2,5-dimethylphenyl (n = 0,1), and A = naphthalene-1,8:4,5-bis(dicarboximide) (NI) or pyromellitimide (PI). Using both time-resolved optical and EPR spectroscopy, we show that T* influences the spin dynamics of the photogenerated triradical states 2,4(MeOAn+*-6ANI-Phn-A-*-T*), resulting in modulation of the charge recombination rate within the triradical compared with the corresponding biradical lacking T*. The observed spin-spin exchange interaction between the photogenerated radicals MeOAn+* and A-* is not altered by the presence of T*, which interacts most strongly with A-* and accelerates radical pair intersystem crossing. Charge recombination within the triradicals results in the formation of 2,4(MeOAn-6ANI-Phn-3*NI-T*) or 2,4(MeOAn-3*6ANI-Phn-PI-T*) in which T* is strongly spin polarized in emission. Normally, the spin dynamics of correlated radical pairs do not produce a net spin polarization; however, the rate at which the net spin polarization appears on T* closely follows the photogenerated radical ion pair decay rate. This effect is attributed to antiferromagnetic coupling between T* and the local triplet state 3NI, which is populated following charge recombination. These results are explained using a switch in the spin basis set between the triradical and the three-spin charge recombination product having both T* and 3*NI or 3*6ANI present.
Optimal Controller Tested for a Magnetically Suspended Five-Axis Dynamic Spin Rig
Choi, Benjamin B.
2003-01-01
NASA Glenn Research Center's Structural Mechanics and Dynamics Branch has developed a fully suspended magnetic bearing system for their Dynamic Spin Rig, which performs vibration tests of turbomachinery blades and components under spinning conditions in a vacuum. Two heteropolar radial magnetic bearings and a thrust magnetic bearing and the associated control system were integrated into the Dynamic Spin Rig to provide magnetic excitation as well as noncontact magnetic suspension of the 35-lb vertical rotor with blades to induce turbomachinery blade vibration (ref. 1). The new system can provide longer run times at higher speeds and larger vibration amplitudes for rotating blades. Also, it was proven that bearing mechanical life was substantially extended and flexibility was increased in the excitation orientation (direction and phasing).
Spin distributions and dynamics in domain walls guided by soft magnetic nanowire structures
Yang, Jusang; Erskine, James L.
2017-01-01
Numerical simulations are used to investigate static and dynamic properties of spin distributions within domain walls confined by rectangular cross section Permalloy nanowire conduits having widths up to 1000 nm and thickness up to 50 nm. Phase boundaries and critical regions associated with domain-wall spin distributions of various topologies [transverse (or asymmetric transverse), vortex, double-vortex, triple-vortex and cross-tie] are accurately determined using high-performance computing resources. Mobility curves are calculated that characterize domain-wall propagation for an interesting region of the spin texture phase diagram: 20 nm thick nanowires with widths of 60-700 nm at axial drive fields extending to 150 Oe. The simulations (and corresponding experiments, which are discussed), reveal new propagating fixed configuration domain-wall topologies with enhanced velocity. Effects of temperature on the spin distributions and dynamics are explored, by conducting simulations that include separately varying temperature-dependent parameters (saturation magnetization and exchange constant) and simulating effects of temperature-dependent fluctuations using the Langevin dynamics feature of the simulation code. Related temperature-dependent experiments are discussed. The simulation studies demonstrate a close connection between static and (field-driven) dynamic spin configurations in nanowire-confined domain walls and demonstrate the importance of exploring model-system parameter space at high numerical precision.
On the dynamics of spin-glass models of neural networks
Jongen, Greetje
1999-10-01
In the first part of the thesis we have studied the parallel dynamics of the Q-Ising spin-glass model of an attractor neural network. The pattern retrieval is seen as a dynamical process of the spins in order to arrive at a configuration similar to one of the embedded patterns. The similarity is expressed by order parameters. Using a probabilistic signal-to-noise analysis we have calculated the time evolution of the order parameters for the asymmetrically and symmetrically diluted architectures and the fully connected architecture. For the first one we have obtained a closed-form solution. For the other architectures feedback correlations of the spins prevent such a closed-form solution, but we have developed a recursive scheme determining the complete time evolution of the order parameters, without any approximation. For these symmetric architectures we have also derived equilibrium fixed-point equations under certain conditions on the noise in the system. They are the same as those obtained in the replica-symmetric mean-field theory. In the second part of the thesis we have applied the replica-symmetric mean-field theory to the XY spin glass with coupled dynamics. In such a model both spins and couplings evolve stochastically, according to coupled equations, but on different time scales. We have defined relevant order parameters and derived a phase diagram. The system exhibits two different spin-glass phases: one describing freezing of the spins only, and one describing freezing of both spins and couplings. Finally, we have calculated the de Almeida-Thouless lines indicating replica-symmetry breaking.
Effect of modularity on the Glauber dynamics of the dilute spin glass model
Energy Technology Data Exchange (ETDEWEB)
Park, Jeong-Man [The Catholic University of Korea, Bucheon (Korea, Republic of)
2014-11-15
We study the Glauber dynamics of the dilute, infinite-ranged spin glass model, the so-called dilute Sherrington-Kirkpatrick (dSK) model. The dSK model has sparse couplings and can be classified by the modularity (M) of the coupling matrix. We investigate the effect of the modularity on the relaxation dynamics starting from a random initial state. By using the Glauber dynamics and the replica method, we derive the relaxation dynamics equations for the magnetization (m) and the energy per spin (r), in addition to the equation for the spin glass order parameter (q{sub α}β). In the replica symmetric (RS) analysis, we find that there are two solutions for the RS spin glass order parameter (q): q = 0 which is stable for r < 1/2 and q = (-1+4r{sup 2})/(32r{sup 4}) which is stable for r > 1/2 in the non-modular system and q = 0 which is stable for r < 1/ SQRT(8) and q = (-1+8r{sup 2})/(128r{sup 4}) which is stable for r > 1/ SQRT(8) in the completely modular system. By substituting the proper q values into the equations for r, we find that the relaxation dynamics of r depends on the modularity, M. These results suggest that, in the context of evolutionary theory, the modularity may emerge spontaneously in the point-mutation-only framework (Glauber dynamics) under a changing environment.
Effect of modularity on the Glauber dynamics of the dilute spin glass model
Park, Jeong-Man
2014-11-01
We study the Glauber dynamics of the dilute, infinite-ranged spin glass model, the so-called dilute Sherrington-Kirkpatrick (dSK) model. The dSK model has sparse couplings and can be classified by the modularity ( M) of the coupling matrix. We investigate the effect of the modularity on the relaxation dynamics starting from a random initial state. By using the Glauber dynamics and the replica method, we derive the relaxation dynamics equations for the magnetization ( m) and the energy per spin ( r), in addition to the equation for the spin glass order parameter ( q αβ ). In the replica symmetric (RS) analysis, we find that there are two solutions for the RS spin glass order parameter ( q): q = 0which is stable for r 1/2 in the non-modular system and q = 0 which is stable for r 1/ in the completely modular system. By substituting the proper q values into the equations for r, we find that the relaxation dynamics of r depends on the modularity, M. These results suggest that, in the context of evolutionary theory, the modularity may emerge spontaneously in the point-mutation-only framework (Glauber dynamics) under a changing environment.
Energy Technology Data Exchange (ETDEWEB)
Pełka, Robert, E-mail: Robert.Pelka@ifj.edu.pl [H. Niewodniczański Institute of Nuclear Physics, Polish Academy of Sciences, E. Radzikowskiego 152, 31-342 Kraków (Poland); Rudowicz, Czesław [Faculty of Chemistry, A. Mickiewicz University, Umultowska 89B, 61-614 Poznań (Poland)
2016-09-15
The standardization idea is nowadays tacitly accepted in EMR area, however, its usefulness in magnetism studies has not been fully recognized as yet. This idea arises due to intrinsic features of orthorhombic Hamiltonians of any physical nature, including the crystal (ligand) field (CF/LF) Hamiltonians or the zero-field splitting (ZFS) ones. Standardization limits the ratio of the orthorhombic parameter to the axial one to a fixed range between 0 and a specific value that depends on the notation used. For the ZFS parameters expressed in the conventional spin Hamiltonian (SH) notation the ratio λ=E/D can always be limited to the range (0, ±1/3) by appropriate choice of coordinate system. Implications of standardization of orthorhombic spin Hamiltonians for interpretation of experimental magnetic susceptibility data are considered. Using a numerical example, we show the existence of alternative solutions for ZFS parameters potentially obtainable from fitting experimental magnetic data and discuss their importance. For the first time algebraic applications of the standardization to the expressions for magnetic susceptibility tensor derived earlier for localized spin models with S=1, 3/2, 2, 5/2 and with rhombic anisotropy are explored. The numerical and algebraic results allow us to formulate an 'invariance principle'. These considerations facilitate interpretation of experimental magnetic data and provide an additional check of correctness of analytical magnetic susceptibility expressions.
RosettaEPR: rotamer library for spin label structure and dynamics.
Directory of Open Access Journals (Sweden)
Nathan S Alexander
Full Text Available An increasingly used parameter in structural biology is the measurement of distances between spin labels bound to a protein. One limitation to these measurements is the unknown position of the spin label relative to the protein backbone. To overcome this drawback, we introduce a rotamer library of the methanethiosulfonate spin label (MTSSL into the protein modeling program Rosetta. Spin label rotamers were derived from conformations observed in crystal structures of spin labeled T4 lysozyme and previously published molecular dynamics simulations. Rosetta's ability to accurately recover spin label conformations and EPR measured distance distributions was evaluated against 19 experimentally determined MTSSL labeled structures of T4 lysozyme and the membrane protein LeuT and 73 distance distributions from T4 lysozyme and the membrane protein MsbA. For a site in the core of T4 lysozyme, the correct spin label conformation (Χ1 and Χ2 is recovered in 99.8% of trials. In surface positions 53% of the trajectories agree with crystallized conformations in Χ1 and Χ2. This level of recovery is on par with Rosetta performance for the 20 natural amino acids. In addition, Rosetta predicts the distance between two spin labels with a mean error of 4.4 Å. The width of the experimental distance distribution, which reflects the flexibility of the two spin labels, is predicted with a mean error of 1.3 Å. RosettaEPR makes full-atom spin label modeling available to a wide scientific community in conjunction with the powerful suite of modeling methods within Rosetta.
Crowell, Paul A.; Liu, Changjiang; Patel, Sahil; Peterson, Tim; Geppert, Chad C.; Christie, Kevin; Stecklein, Gordon; Palmstrøm, Chris J.
2016-10-01
A distinguishing feature of spin accumulation in ferromagnet-semiconductor devices is its precession in a magnetic field. This is the basis for detection techniques such as the Hanle effect, but these approaches become ineffective as the spin lifetime in the semiconductor decreases. For this reason, no electrical Hanle measurement has been demonstrated in GaAs at room temperature. We show here that by forcing the magnetization in the ferromagnet to precess at resonance instead of relying only on the Larmor precession of the spin accumulation in the semiconductor, an electrically generated spin accumulation can be detected up to 300 K. The injection bias and temperature dependence of the measured spin signal agree with those obtained using traditional methods. We further show that this new approach enables a measurement of short spin lifetimes (techniques. The measurements were carried out on epitaxial Heusler alloy (Co2FeSi or Co2MnSi)/n-GaAs heterostructures. Lateral spin valve devices were fabricated by electron beam and photolithography. We compare measurements carried out by the new FMR-based technique with traditional non-local and three-terminal Hanle measurements. A full model appropriate for the measurements will be introduced, and a broader discussion in the context of spin pumping experimenments will be included in the talk. The new technique provides a simple and powerful means for detecting spin accumulation at high temperatures. Reference: C. Liu, S. J. Patel, T. A. Peterson, C. C. Geppert, K. D. Christie, C. J. Palmstrøm, and P. A. Crowell, "Dynamic detection of electron spin accumulation in ferromagnet-semiconductor devices by ferromagnetic resonance," Nature Communications 7, 10296 (2016). http://dx.doi.org/10.1038/ncomms10296
Quasiclassical methods for spin-charge coupled dynamics in low-dimensional systems
Energy Technology Data Exchange (ETDEWEB)
Corini, Cosimo
2009-06-12
Spintronics is a new field of study whose broad aim is the manipulation of the spin degrees of freedom in solid state systems. One of its main goals is the realization of devices capable of exploiting, besides the charge, the carriers' - and possibly the nuclei's - spin. The presence of spin-orbit coupling in a system enables the spin and charge degrees of freedom to ''communicate'', a favorable situation if one is to realize such devices. More importantly, it offers the opportunity of doing so by relying solely on electric fields, whereas magnetic fields are otherwise required. Eminent examples of versatile systems with built-in and variously tunable spin-orbit interaction are two-dimensional electron - or hole - gases. The study of spin-charge coupled dynamics in such a context faces a large number of open questions, both of the fundamental and of the more practical type. To tackle the problem we rely on the quasiclassical formalism. This is an approximate quantum-field theoretical formulation with a solid microscopic foundation, perfectly suited for describing phenomena at the mesoscopic scale, and bearing a resemblance to standard Boltzmann theory which makes for physical transparency. Originally born to deal with transport in electron-phonon systems, we first generalize it to the case in which spin-orbit coupling is present, and then move on to apply it to specific situations and phenomena. Among these, to the description of the spin Hall effect and of voltage induced spin polarizations in two-dimensional electron gases under a variety of conditions - stationary or time-dependent, in the presence of magnetic and non-magnetic disorder, in the bulk or in confined geometries -, and to the problem of spin relaxation in narrow wires. (orig.)
Soh, Wee Tee; Peng, Bin; Ong, C. K.
2015-08-01
The spin rectification effect (SRE), a phenomenon that generates dc voltages from ac microwave fields incident onto a conducting ferromagnet, has attracted widespread attention due to its high sensitivity to ferromagnetic resonance (FMR) as well as its relevance to spintronics. Here, we report the non-local detection of yttrium iron garnet (YIG) spin dynamics by measuring SRE voltages from an adjacent conducting NiFe layer up to 200 nm thick. In particular, we detect, within the NiFe layer, SRE voltages stemming from magnetostatic surface spin waves (MSSWs) of the adjacent bulk YIG which are excited by a shorted coaxial probe. These non-local SRE voltages within the NiFe layer that originates from YIG MSSWs are present even in 200 nm-thick NiFe films with a 50 nm thick SiO2 spacer between NiFe and YIG, thus strongly ruling out the mechanism of spin-pumping induced inverse spin Hall effect in NiFe as the source of these voltages. This long-range influence of YIG dynamics is suggested to be mediated by dynamic fields generated from YIG spin precession near YIG/NiFe interface, which interacts with NiFe spins near the simultaneous resonance of both spins, to generate a non-local SRE voltage within the NiFe layer.
Directory of Open Access Journals (Sweden)
Wee Tee Soh
2015-08-01
Full Text Available The spin rectification effect (SRE, a phenomenon that generates dc voltages from ac microwave fields incident onto a conducting ferromagnet, has attracted widespread attention due to its high sensitivity to ferromagnetic resonance (FMR as well as its relevance to spintronics. Here, we report the non-local detection of yttrium iron garnet (YIG spin dynamics by measuring SRE voltages from an adjacent conducting NiFe layer up to 200 nm thick. In particular, we detect, within the NiFe layer, SRE voltages stemming from magnetostatic surface spin waves (MSSWs of the adjacent bulk YIG which are excited by a shorted coaxial probe. These non-local SRE voltages within the NiFe layer that originates from YIG MSSWs are present even in 200 nm-thick NiFe films with a 50 nm thick SiO2 spacer between NiFe and YIG, thus strongly ruling out the mechanism of spin-pumping induced inverse spin Hall effect in NiFe as the source of these voltages. This long-range influence of YIG dynamics is suggested to be mediated by dynamic fields generated from YIG spin precession near YIG/NiFe interface, which interacts with NiFe spins near the simultaneous resonance of both spins, to generate a non-local SRE voltage within the NiFe layer.
Energy Technology Data Exchange (ETDEWEB)
Soh, Wee Tee, E-mail: a0046479@u.nus.edu; Ong, C. K. [Center for Superconducting and Magnetic Materials, Department of Physics, National University of Singapore, 2 Science Drive 3, Singapore 117551 (Singapore); Peng, Bin [State Key Laboratory of Electronic Thin Films and Integrated Devices, University of Electronic Science and Technology of China, Chengdu 610054 (China)
2015-08-15
The spin rectification effect (SRE), a phenomenon that generates dc voltages from ac microwave fields incident onto a conducting ferromagnet, has attracted widespread attention due to its high sensitivity to ferromagnetic resonance (FMR) as well as its relevance to spintronics. Here, we report the non-local detection of yttrium iron garnet (YIG) spin dynamics by measuring SRE voltages from an adjacent conducting NiFe layer up to 200 nm thick. In particular, we detect, within the NiFe layer, SRE voltages stemming from magnetostatic surface spin waves (MSSWs) of the adjacent bulk YIG which are excited by a shorted coaxial probe. These non-local SRE voltages within the NiFe layer that originates from YIG MSSWs are present even in 200 nm-thick NiFe films with a 50 nm thick SiO{sub 2} spacer between NiFe and YIG, thus strongly ruling out the mechanism of spin-pumping induced inverse spin Hall effect in NiFe as the source of these voltages. This long-range influence of YIG dynamics is suggested to be mediated by dynamic fields generated from YIG spin precession near YIG/NiFe interface, which interacts with NiFe spins near the simultaneous resonance of both spins, to generate a non-local SRE voltage within the NiFe layer.
Yucesoy, Burcu; Machta, Jonathan; Katzgraber, Helmut G.
2013-01-01
We present the results of a large-scale numerical study of the equilibrium three-dimensional Edwards-Anderson Ising spin glass with Gaussian disorder. Using parallel tempering (replica exchange) Monte Carlo we measure various static, as well as dynamical quantities, such as the autocorrelation times and round-trip times for the parallel tempering Monte Carlo method. The correlation between static and dynamic observables for 5000 disorder realizations and up to 1000 spins down to temperatures at 20% of the critical temperature is examined. Our results show that autocorrelation times are directly correlated with the roughness of the free-energy landscape.
Yucesoy, Burcu; Machta, Jonathan; Katzgraber, Helmut G.
2012-02-01
We present the results of a large-scale numerical study of the equilibrium three-dimensional Ising spin glass with Gaussian disorder. Using replica exchange (parallel tempering) Monte Carlo, we measure various static, as well as dynamical quantities, such as the autocorrelation times and round-trip times for the replica exchange Monte Carlo method. The correlation between static and dynamic observables for 5000 disorder realizations (N <=10^3 spins) down to very low temperatures (T 0.2Tc) is examined. Our results show that autocorrelation times are directly correlated with the roughness of the free energy landscape. We also discuss the size dependence of several static quantities.
Gravitational radiation and angular momentum flux from a spinning dynamical black hole
Wang, Chih-Hung
2013-01-01
A four-dimensional asymptotic expansion scheme is used to study the next order effects of the nonlinearity near a spinning dynamical black hole. The angular momentum flux and energy flux formula are then obtained by asymptotic expansion and the compatibility of the coupling Newman-Penrose equations. After constructing the reference frame in terms of the compatible constant spinors, the energy-momentum flux is derived and it is related to the black hole area growth. Directly from the flux formula of the spinning dynamical horizon, we find that the physically reasonable condition on the positivity of the gravitational energy flux yields that the shear will monotonically decrease with time.
Bhattacharjee, Satadeep; Nordström, Lars; Fransson, Jonas
2012-02-03
We consider spin dynamics for implementation in an atomistic framework and we address the feasibility of capturing processes in the femtosecond regime by inclusion of moment of inertia. In the spirit of an s-d-like interaction between the magnetization and electron spin, we derive a generalized equation of motion for the magnetization dynamics in the semiclassical limit, which is nonlocal in both space and time. Using this result we retain a generalized Landau-Lifshitz-Gilbert equation, also including the moment of inertia, and demonstrate how the exchange interaction, damping, and moment of inertia, all can be calculated from first principles.
A Generalized Kawasaki-Type Dynamics with Spin-Pair Redistribution Mechanism
Institute of Scientific and Technical Information of China (English)
朱建阳; 朱涵
2002-01-01
We generalize Kawasaki's dynamics, spin-pair exchange mechanism, to a spin-pair redistribution mechanism,and we present a normalized redistribution probability. As an application, we treat the one-dimensional kinetic Gaussian model and obtain the exact diffusion equation and the temperature-dependent diffusion coefficient. We find that the diffusion process can slow down infinitely near the critical point and obtain the critical dynamic exponent z = 2 that is independent of the assumed mechanism, either Glauber-type or Kawasaki-type.
DEFF Research Database (Denmark)
Kawasaki, Yu; Gavilano, Jorge L.; Keller, Lukas
2011-01-01
We report a neutron diffraction and muon spin relaxation mu SR study of static and dynamical magnetic properties of BaCo2V2O8, a quasi-one-dimensional spin-chain system. A proposed model for the antiferromagnetic structure includes: a propagation vector (k) over right arrow (AF) = (0,0,1), indepe......We report a neutron diffraction and muon spin relaxation mu SR study of static and dynamical magnetic properties of BaCo2V2O8, a quasi-one-dimensional spin-chain system. A proposed model for the antiferromagnetic structure includes: a propagation vector (k) over right arrow (AF) = (0...... at different muon stopping sites. Muon time spectra measured at weak longitudinal fields and temperatures much higher than T-N can be well described using a single muon site with an exponential muon spin relaxation that gradually changes into an stretched exponential on approaching T-N. The temperature...
Energy Technology Data Exchange (ETDEWEB)
Vatansever, Erol [Dokuz Eylül University, Graduate School of Natural and Applied Sciences, TR-35160 Izmir (Turkey); Polat, Hamza, E-mail: hamza.polat@deu.edu.tr [Department of Physics, Dokuz Eylül University, TR-35160 Izmir (Turkey)
2015-10-15
Nonequilibrium phase transition properties of a mixed Ising ferrimagnetic model consisting of spin-1/2 and spin-3/2 on a square lattice under the existence of a time dependent oscillating magnetic field have been investigated by making use of Monte Carlo simulations with a single-spin flip Metropolis algorithm. A complete picture of dynamic phase boundary and magnetization profiles have been illustrated and the conditions of a dynamic compensation behavior have been discussed in detail. According to our simulation results, the considered system does not point out a dynamic compensation behavior, when it only includes the nearest-neighbor interaction, single-ion anisotropy and an oscillating magnetic field source. As the next-nearest-neighbor interaction between the spins-1/2 takes into account and exceeds a characteristic value which sensitively depends upon values of single-ion anisotropy and only of amplitude of external magnetic field, a dynamic compensation behavior occurs in the system. Finally, it is reported that it has not been found any evidence of dynamically first-order phase transition between dynamically ordered and disordered phases, which conflicts with the recently published molecular field investigation, for a wide range of selected system parameters. - Highlights: • Spin-1/2 and spin-3/2 Ising ferrimagnetic model is examined. • The system is exposed to time-dependent magnetic field. • Kinetic Monte Carlo simulation technique is used. • Any evidence of first-order phase transition has not been found.
Damour, Thibault; Schäfer, Gerhard
2008-01-01
Using a recent, novel Hamiltonian formulation of the gravitational interaction of spinning binaries, we extend the Effective One Body (EOB) description of the dynamics of two spinning black holes to next-to-leading order (NLO) in the spin-orbit interaction. The spin-dependent EOB Hamiltonian is constructed from four main ingredients: (i) a transformation between the ``effective'' Hamiltonian and the ``real'' one, (ii) a generalized effective Hamilton-Jacobi equation involving higher powers of the momenta, (iii) a Kerr-type effective metric (with Pad\\'e-resummed coefficients) which depends on the choice of some basic ``effective spin vector'' $\\bf{S}_{\\rm eff}$, and which is deformed by comparable-mass effects, and (iv) an additional effective spin-orbit interaction term involving another spin vector $\\bsigma$. As a first application of the new, NLO spin-dependent EOB Hamiltonian, we compute the binding energy of circular orbits (for parallel spins) as a function of the orbital frequency, and of the spin param...
Nonlinear Dynamics of Magnons observed by AC Spin Pumping in Magnetic Hybrid Structures
Vilela-Leao, L. H.; Cunha, R. O.; Azevedo, A.; Rodriguez-Suarez, R. L.; Rezende, S. M.
2015-03-01
The electron spin degree of freedom constitutes the basic means to carry and store information in the field of spintronics. In the spin pumping process, the microwave driven magnetization dynamics in a ferromagnetic film generates a spin current in an attached metallic layer that can be converted into a charge current by means of the inverse spin Hall effect and detected by a voltage signal. While the time independent component (DC) of the spin current has been widely investigated in a variety of material structures, recently it has been recognized that the alternating current (AC) component is much larger, though more difficult to detect, and has many attractive features. We report experiments with microwave driven DC and AC spin pumping in bilayers made of the insulating ferrimagnet yttrium iron garnet (YIG) and platinum that reveal the nonlinear dynamics involving the driven mode and a pair of magnon modes with half frequency. This process occurs when the frequency is lowered below a critical value so that a three-magnon splitting process with energy conservation is made possible. The results are explained by a model with coupled nonlinear equations describing the time evolution of the magnon modes.
Hyperfine and spin-orbit dynamics in GaAs double quantum dots
Shulman, Michael; Nichol, John; Harvey, Shannon; Pal, Arijeet; Halperin, Bertrand; Umansky, Vladimir; Yacoby, Amir
2015-03-01
Semiconductor quantum dots provide a unique platform for single-particle physics and many-body quantum mechanics. In particular, understanding the dynamics of a single electron interacting with a nuclear spin bath is key to improving spin-based quantum information processing, since the hyperfine interaction limits the performance of many spin qubits. We probe the electron-nuclear interaction by measuring the splitting at the anti-crossing between the electron singlet (S) and m =1 triplet (T +) states in a GaAs double quantum dot. Using Landau-Zener sweeps, we find that the size of this splitting varies by more than an order of magnitude depending on the magnitude and direction of the external magnetic field. These results are consistent with a competition between the spin orbit interaction and the hyperfine interaction, even though the extracted spin orbit length is much larger than the size of the double quantum dot. We confirm these results by using Landau-Zener sweeps to measure the high-frequency correlations in the S-T + splitting that arise from the Larmor precession of the nuclei. These unexpected results have implications for improving the performance of spin-based quantum information processing, as well as improving our understanding of the central spin problem.
Spin wave dynamics in Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes
Energy Technology Data Exchange (ETDEWEB)
Mi, Bin-Zhou, E-mail: mbzfjerry2008@126.com [Department of Basic Curriculum, North China Institute of Science and Technology, Beijing 101601 (China); Department of Physics, School of Mathematics and Physics, University of Science and Technology Beijing, Beijing 100083 (China)
2016-09-15
The spin wave dynamics, including the magnetization, spin wave dispersion relation, and energy level splitting, of Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes are systematically calculated by use of the double-time Green’s function method within the random phase approximation. The role of temperature, diameter of the tube, and wave vector on spin wave energy spectrum and energy level splitting are carefully analyzed. There are two categories of spin wave modes, which are quantized and degenerate, and the total number of independent magnon branches is dependent on diameter of the tube, caused by the physical symmetry of nanotubes. Moreover, the number of flat spin wave modes increases with diameter of the tube rising. The spin wave energy and the energy level splitting decrease with temperature rising, and become zero as temperature reaches the critical point. At any temperature, the energy level splitting varies with wave vector, and for a larger wave vector it is smaller. When pb=π, the boundary of first Brillouin zone, spin wave energies are degenerate, and the energy level splittings are zero.
Spin wave dynamics in Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes
Mi, Bin-Zhou
2016-09-01
The spin wave dynamics, including the magnetization, spin wave dispersion relation, and energy level splitting, of Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes are systematically calculated by use of the double-time Green's function method within the random phase approximation. The role of temperature, diameter of the tube, and wave vector on spin wave energy spectrum and energy level splitting are carefully analyzed. There are two categories of spin wave modes, which are quantized and degenerate, and the total number of independent magnon branches is dependent on diameter of the tube, caused by the physical symmetry of nanotubes. Moreover, the number of flat spin wave modes increases with diameter of the tube rising. The spin wave energy and the energy level splitting decrease with temperature rising, and become zero as temperature reaches the critical point. At any temperature, the energy level splitting varies with wave vector, and for a larger wave vector it is smaller. When pb=π, the boundary of first Brillouin zone, spin wave energies are degenerate, and the energy level splittings are zero.
Dynamic properties of magnets with spin S = 3/2 and non-Heisenberg isotropic interaction
Energy Technology Data Exchange (ETDEWEB)
Kosmachev, O. A.; Fridman, Yu. A., E-mail: yuriifridman@gmail.com [Vernadsky Taurida National University (Russian Federation); Galkina, E. G. [National Academy of Sciences of Ukraine, Institute of Physics (Ukraine); Ivanov, B. A. [National Academy of Sciences of Ukraine, Institute of Magnetism (Ukraine)
2015-02-15
The dynamic properties of a magnet with magnetic-ion spin of 3/2 and an isotropic spin interaction of a general form have been investigated. Only four phase states can be realized in the system under consideration at various relationships between the material parameters: the ferro- and antiferromagnetic phases with saturated spin and the states with tensor order parameters, the nematic and antinematic ones. For these phases, the spontaneous symmetry breaking is determined by the octupole order parameter containing the mean values trilinear in spin operator components at a given site. The spectra of elementary excitations have been determined in all phases. Additional branches of excitations arise in all four phase states.
Energy Technology Data Exchange (ETDEWEB)
Mance, Deni; Baldus, Marc, E-mail: m.baldus@uu.nl [NMR Spectroscopy, Bijvoet Center for Biomolecular Research, Department of Chemistry, Faculty of Science, Utrecht University, 3584 CH Utrecht (Netherlands); Gast, Peter; Huber, Martina [Department of Physics, Huygens-Kamerlingh Onnes Laboratory, Leiden University, PO Box 9504, 2300 RA Leiden (Netherlands); Ivanov, Konstantin L., E-mail: ivanov@tomo.nsc.ru [International Tomography Center, Siberian Branch of the Russian Academy of Science, Institutskaya 3a, Novosibirsk 630090, Russia and Novosibirsk State University, Pirogova 2, Novosibirsk 63009 (Russian Federation)
2015-06-21
We develop a theoretical description of Dynamic Nuclear Polarization (DNP) in solids under Magic Angle Spinning (MAS) to describe the magnetic field dependence of the DNP effect. The treatment is based on an efficient scheme for numerical solution of the Liouville-von Neumann equation, which explicitly takes into account the variation of magnetic interactions during the sample spinning. The dependence of the cross-effect MAS-DNP on various parameters, such as the hyperfine interaction, electron-electron dipolar interaction, microwave field strength, and electron spin relaxation rates, is analyzed. Electron spin relaxation rates are determined by electron paramagnetic resonance measurements, and calculations are compared to experimental data. Our results suggest that the observed nuclear magnetic resonance signal enhancements provided by MAS-DNP can be explained by discriminating between “bulk” and “core” nuclei and by taking into account the slow DNP build-up rate for the bulk nuclei.
Low field domain wall dynamics in artificial spin-ice basis structure
Energy Technology Data Exchange (ETDEWEB)
Kwon, J. [School of Physical and Mathematical Sciences, Nanyang Technological University, 21 Nanyang Link, Singapore 637371 (Singapore); School of Electrical and Electronic Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798 (Singapore); Goolaup, S.; Lim, G. J.; Kerk, I. S.; Lew, W. S., E-mail: wensiang@ntu.edu.sg [School of Physical and Mathematical Sciences, Nanyang Technological University, 21 Nanyang Link, Singapore 637371 (Singapore); Chang, C. H., E-mail: echchang@ntu.edu.sg [School of Electrical and Electronic Engineering, Nanyang Technological University, 50 Nanyang Avenue, Singapore 639798 (Singapore); Roy, K. [School of Electrical and Computer Engineering, Purdue University, West Lafayette, Indiana 47907 (United States)
2015-10-28
Artificial magnetic spin-ice nanostructures provide an ideal platform for the observation of magnetic monopoles. The formation of a magnetic monopole is governed by the motion of a magnetic charge carrier via the propagation of domain walls (DWs) in a lattice. To date, most experiments have been on the static visualization of DW propagation in the lattice. In this paper, we report on the low field dynamics of DW in a unit spin-ice structure measured by magnetoresistance changes. Our results show that reversible DW propagation can be initiated within the spin-ice basis. The initial magnetization configuration of the unit structure strongly influences the direction of DW motion in the branches. Single or multiple domain wall nucleation can be induced in the respective branches of the unit spin ice by the direction of the applied field.
Non-Markovian Dynamics in Chiral Quantum Networks with Spins and Photons
Ramos, Tomás; Hauke, Philipp; Pichler, Hannes; Zoller, Peter
2016-01-01
We study the dynamics of chiral quantum networks consisting of nodes coupled by unidirectional or asymmetric bidirectional quantum channels. In contrast to the familiar photonic networks consisting of driven two-level atoms exchanging photons via 1D photonic nanostructures, we propose and study a setup where interactions between the atoms are mediated by spin excitations (magnons) in 1D XX-spin chains representing a spin waveguide. While Markovian quantum network theory eliminates quantum channels as structureless reservoirs in a Born-Markov approximation to obtain a master equation for the nodes, we are interested in non-Markovian dynamics. This arises from the nonlinear character of the dispersion with band-edge effects, and from finite spin propagation velocities leading to time delays in interactions. To account for the non-Markovian dynamics we treat the quantum degrees of freedom of the nodes and connecting channel as a composite spin system with the surrounding of the quantum network as a Markovian bat...
Magnetization dynamics under heat current in metallic spin valves and in insulators
Yu, Haiming
Spin caloritronics, an emerging branch of spintronics, studying the addition of thermal effects to the electrical and magnetic properties of nanostructures, has recently seen a rapid development. It has been predicted by Hatami et al. that a heat current can exert a spin torque on the magnetization in a nanostructure, analogous to the well-known spin-transfer torque induced by an electrical current. We provided the experimental evidence for the thermal spin-transfer torque effect in spin valves, showing the switching field change with heat current. I will present measurements of the second harmonic voltage response of Co-Cu-Co pseudo-spinvalves deposited in the middle of Cu nanowires. Both the magnitude of the second harmonic response of the spin valve and the field value of the maximum response are found to be dependent on the heat current. Both effects show that the magnetization dynamics of the pseudo-spinvalves is influenced by the heat current. Thus, the data provide a quantitative estimate of the thermal spin torque exerted on the magnetization of the Co layers. In addition, I will present recent study on the magnetization dynamics in a magnetic insulator YIG film under in-plane heat current. The ferromagnetic resonance linewidth is found to be tuned by the applied temperature gradient, i.e. narrowing and broadening. This suggests that the Gilbert damping parameter is compensated or reinforced by the applied temperature gradient in respective direction. These observations can be understood as a heat-driven spin torque in magnetic insulators.
Kinetic theories for spin models for cooperative relaxation dynamics
Pitts, Steven Jerome
The facilitated kinetic Ising models with asymmetric spin flip constraints introduced by Jackle and co-workers [J. Jackle, S. Eisinger, Z. Phys. B 84, 115 (1991); J. Reiter, F. Mauch, J. Jackle, Physica A 184, 458 (1992)] exhibit complex relaxation behavior in their associated spin density time correlation functions. This includes the growth of relaxation times over many orders of magnitude when the thermodynamic control parameter is varied, and, in some cases, ergodic-nonergodic transitions. Relaxation equations for the time dependence of the spin density autocorrelation function for a set of these models are developed that relate this autocorrelation function to the irreducible memory function of Kawasaki [K. Kawasaki, Physica A 215, 61 (1995)] using a novel diagrammatic series approach. It is shown that the irreducible memory function in a theory of the relaxation of an autocorrelation function in a Markov model with detailed balance plays the same role as the part of the memory function approximated by a polynomial function of the autocorrelation function with positive coefficients in schematic simple mode coupling theories for supercooled liquids [W. Gotze, in Liquids, Freezing and the Glass Transition, D. Levesque, J. P. Hansen, J. Zinn-Justin eds., 287 (North Holland, New York, 1991)]. Sets of diagrams in the series for the irreducible memory function are summed which lead to approximations of this type. The behavior of these approximations is compared with known results from previous analytical calculations and from numerical simulations. For the simplest one dimensional model, relaxation equations that are closely related to schematic extended mode coupling theories [W. Gotze, ibid] are also derived using the diagrammatic series. Comparison of the results of these approximate theories with simulation data shows that these theories improve significantly on the results of the theories of the simple schematic mode coupling theory type. The potential
Dynamic Consequences of Optical Spin-Orbit Interaction
Sukhov, Sergey; Dogariu, Aristide
2015-01-01
When circularly polarized wave scatters off a sphere, the scattered field forms a vortex with spiraling energy flow. This is due to the transformation of spin angular momentum into orbital one. Here we demonstrate that during this scattering an anomalous force can be induced that acts in a direction perpendicular to the propagation of incident wave. The appearance of this lateral force is made possible by the presence of an interface in the vicinity of scattering object. Besides radiation pressure and tractor-beam pulling forces, this lateral force is another type of non-conservative force that can be produced with unstructured light beams.
Quantum dynamics and entanglement of spins on a square lattice
DEFF Research Database (Denmark)
Christensen, Niels Bech; Rønnow, Henrik Moodysson; McMorrow, Desmond Francis;
2007-01-01
Bulk magnetism in solids is fundamentally quantum mechanical in nature. Yet in many situations, including our everyday encounters with magnetic materials, quantum effects are masked, and it often suffices to think of magnetism in terms of the interaction between classical dipole moments. Whereas...... this intuition generally holds for ferromagnets, even as the size of the magnetic moment is reduced to that of a single electron spin (the quantum limit), it breaks down spectacularly for antiferromagnets, particularly in low dimensions. Considerable theoretical and experimental progress has been made...
Spin-orbit interactions and quantum spin dynamics in cold ion-atom collisions
Tscherbul, Timur V; Buchachenko, Alexei A
2015-01-01
We present accurate ab initio and quantum scattering calculations on a prototypical hybrid ion-atom system Yb$^+$-Rb, recently suggested as a promising candidate for the experimental study of open quantum systems, quantum information processing, and quantum simulation. We identify the second-oder spin-orbit (SO) interaction as the dominant source of hyperfine relaxation and decoherence in cold Yb$^+$-Rb collisions. Our results are in good agreement with recent experimental observations [L. Ratschbacher et al., Phys. Rev. Lett. 110, 160402 (2013)] of hyperfine relaxation rates of trapped Yb$^+$ immersed in an ultracold Rb gas. The calculated rates are 4 times smaller than predicted by the Langevin capture theory and display a weak $T^{-0.3}$ temperature dependence, indicating significant deviations from statistical behavior. Our analysis underscores the deleterious nature of the SO interaction and implies that light ion-atom combinations such as Yb$^+$-Li should be used to minimize hyperfine relaxation and dec...
NONLINEAR DYNAMIC SIMULATION OF AN AXIALLY SLIDE-SPIN ROCKET FLEXIBLE SYSTEM WITH CLEARANCE
Institute of Scientific and Technical Information of China (English)
Zhu Huailiang; Zhang Fuxiang
2005-01-01
A hybrid approach is presented to investigate the dynamic behavior of an axially slide-spin flexible rocket with nonlinear clearance. The equations of motion of the flexible rocket are derived based upon Euler-Bernoulli beam theory and Hamilton principle and the finite element method. The characteristics of clearance between the spinning rocket and launcher are considered to be piecewise linear. Numerical solution is developed by direct integration method and demonstrates the validity of the method. The coupled dynamic behavior of axial motion and transverse vibrations of rocket are analyzed, and the influences of axially moving acceleration, spin speed, linking stiffness of elastic "shoes", and the nonlinearity of clearance on the motion attitude of rocket are studied.
Dynamics of polymer film formation during spin coating
Energy Technology Data Exchange (ETDEWEB)
Mouhamad, Y.; Clarke, N.; Jones, R. A. L.; Geoghegan, M., E-mail: geoghegan@sheffield.ac.uk [Department of Physics and Astronomy, The University of Sheffield, Hicks Building, Hounsfield Road, Sheffield S3 7RH (United Kingdom); Mokarian-Tabari, P. [Materials Research Group, Department of Chemistry and the Tyndall National Institute, University College Cork, Cork (Ireland)
2014-09-28
Standard models explaining the spin coating of polymer solutions generally fail to describe the early stages of film formation, when hydrodynamic forces control the solution behavior. Using in situ light scattering alongside theoretical and semi-empirical models, it is shown that inertial forces (which initially cause a vertical gradient in the radial solvent velocity within the film) play a significant role in the rate of thinning of the solution. The development of thickness as a function of time of a solute-free liquid (toluene) and a blend of polystyrene and poly(methyl methacrylate) cast from toluene were fitted to different models as a function of toluene partial pressure. In the case of the formation of the polymer blend film, a concentration-dependent (Huggins) viscosity formula was used to account for changes in viscosity during spin coating. A semi-empirical model is introduced, which permits calculation of the solvent evaporation rate and the temporal evolution of the solute volume fraction and solution viscosity.
Bowlan, P.; Trugman, S. A.; Bowlan, J.; Zhu, J.-X.; Hur, N. J.; Taylor, A. J.; Yarotski, D. A.; Prasankumar, R. P.
2016-09-01
We demonstrate an approach for directly tracking antiferromagnetic (AFM) spin dynamics by measuring ultrafast changes in a magnon resonance. We test this idea on the multiferroic HoMnO3 by optically photoexciting electrons, after which changes in the spin order are probed with a THz pulse tuned to a magnon resonance. This reveals a photoinduced change in the magnon line shape that builds up over 5-12 picoseconds, which we show to be the spin-lattice thermalization time, indicating that electrons heat the spins via phonons. We compare our results to previous studies of spin-lattice thermalization in ferromagnetic manganites, giving insight into fundamental differences between the two systems. Our work sheds light on the microscopic mechanism governing spin-phonon interactions in AFMs and demonstrates a powerful approach for directly monitoring ultrafast spin dynamics.
A Model of Charge Transfer Excitons: Diffusion, Spin Dynamics, and Magnetic Field Effects
Lee, Chee Kong; Willard, Adam P
2016-01-01
In this letter we explore how the microscopic dynamics of charge transfer (CT) excitons are influenced by the presence of an external magnetic field in disordered molecular semiconductors. This influence is driven by the dynamic interplay between the spin and spatial degrees of freedom of the electron-hole pair. To account for this interplay we have developed a numerical framework that combines a traditional model of quantum spin dynamics with a coarse-grained model of stochastic charge transport. This combination provides a general and efficient methodology for simulating the effects of magnetic field on CT state dynamics, therefore providing a basis for revealing the microscopic origin of experimentally observed magnetic field effects. We demonstrate that simulations carried out on our model are capable of reproducing experimental results as well as generating theoretical predictions related to the efficiency of organic electronic materials.
Spin dynamics in p-doped InAs/GaAs quantum dots
Energy Technology Data Exchange (ETDEWEB)
Braun, P.F.; Lombez, L.; Marie, X.; Urbaszek, B.; Senes, M.; Amand, T. [Laboratoire de Nanophysique, Magnetisme et Optoelectronique, INSA 135 avenue de Rangueil, 31077 Toulouse cedex (France); Kalevich, V.; Kavokin, K.; Ustinov, V. [IOFFE Institute, Politekhnicheskaya 26, St. Petersburg 194021 (Russian Federation); Krebs, O.; Voisin, P. [Laboratoire de Photonique et Nanostructures, route de Nozay, 91460 Marcoussis (France)
2005-05-01
We have investigated the optical orientation dynamics of positively charged excitons in p-doped InAs/GaAs quantum dots. We observe a hole spin memory effect in photoluminescence experiments. (copyright 2005 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)
Dynamical symmetries and crossovers in a three-spin system with collective dissipation
Pigeon, S.; Xuereb, A.; Lesanovsky, I.; Garrahan, J. P.; De Chiara, G.; Paternostro, M.
2015-01-01
We consider the non-equilibrium dynamics of a simple system consisting of interacting spin-1/2 particles subjected to a collective damping. The model is close to situations that can be engineered in hybrid electro/opto-mechanical settings. Making use of large-deviation theory, we find a Gallavotti-Cohen symmetry in the dynamics of the system as well as evidence for the coexistence of two dynamical phases with different activity levels. We show that additional damping processes smooth out this behavior. Our analytical results are backed up by Monte Carlo simulations that reveal the nature of the trajectories contributing to the different dynamical phases.
Zhang, Hou-Dao; Xu, Rui-Xue; Zheng, Xiao; Yan, YiJing
2015-01-14
We consider the hybrid system-bath dynamics, based on the Yan's dissipaton formalism [Y. J. Yan, J. Chem. Phys. 140, 054105 (2014)]. This theory provides a unified quasi-particle treatment on three distinct classes of quantum bath, coupled nonperturbatively to arbitrary quantum systems. In this work, to study the entangled system and bath polarization and nonlinear Fano interference, we incorporate further the time-dependent light field, which interacts with both the molecular system and the collective bath dipoles directly. Numerical demonstrations are carried out on a two-level system, with comparison between phonon and exciton baths, in both linear and nonlinear Fano interference regimes.
Optimizing a dynamical decoupling protocol for solid-state electronic spin ensembles in diamond
Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.
2015-08-01
We demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to 77 K suppresses longitudinal spin relaxation T1 effects and DD microwave pulses are used to increase the transverse coherence time T2 from ˜0.7 ms up to ˜30 ms . We extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. Following a theoretical and experimental characterization of pulse and detuning errors, we compare the performance of various DD protocols. We identify that the optimal control scheme for preserving an arbitrary spin state is a recursive protocol, the concatenated version of the XY8 pulse sequence. The improved spin coherence might have an immediate impact on improvements of the sensitivities of ac magnetometry. Moreover, the protocol can be used on denser diamond samples to increase coherence times up to NV-NV interaction time scales, a major step towards the creation of quantum collective NV spin states.
Levi, Michele
2016-01-01
In this work we complete the spin dependent conservative dynamics of inspiralling compact binaries at the fourth post-Newtonian order, and in particular the recent derivation of the next-to-next-to-leading order spin-squared interaction potential. We derive the physical equations of motion of the position and the spin from a direct variation of the action. Further, we derive the quadratic in spin Hamiltonians, as well as their expressions in the center of mass frame. We construct the conserved integrals of motion, which form the Poincare algebra. This construction provided a consistency check for the validity of our result, which is crucial in particular in the current absence of another independent derivation of the next-to-next-to-leading order spin-squared interaction. Finally, we provide here the complete gauge invariant relations among the binding energy, angular momentum, and orbital frequency of an inspiralling binary with generic compact spinning components to the fourth post-Newtonian order. These hi...
Advances and applications of dynamic-angle spinning nuclear magnetic resonance
Energy Technology Data Exchange (ETDEWEB)
Baltisberger, J.H.
1993-06-01
This dissertation describes nuclear magnetic resonance experiments and theory which have been developed to study quadrupolar nuclei (those nuclei with spin greater than one-half) in the solid state. Primarily, the technique of dynamic-angle spinning (DAS) is extensively reviewed and expanded upon in this thesis. Specifically, the improvement in both the resolution (two-dimensional pure-absorptive phase methods and DAS angle choice) and sensitivity (pulse-sequence development), along with effective spinning speed enhancement (again through choice of DAS conditions or alternative multiple pulse schemes) of dynamic-angle spinning experiment was realized with both theory and experimental examples. The application of DAS to new types of nuclei (specifically the {sup 87}Rb and {sup 85}Rb nuclear spins) and materials (specifically amorphous solids) has also greatly expanded the possibilities of the use of DAS to study a larger range of materials. This dissertation is meant to demonstrate both recent advances and applications of the DAS technique, and by no means represents a comprehensive study of any particular chemical problem.
Quantum spin dynamics at terahertz frequencies in 2D hole gases and improper ferroelectrics
Lloyd-Hughes, J.
2015-08-01
Terahertz time-domain spectroscopy permits the excitations of novel materials to be examined with exquisite precision. Improper ferroelectric materials such as cupric oxide (CuO) exhibit complex magnetic ground states. CuO is antiferromagnetic below 213K, but has an incommensurate cycloidal magnetic phase between 213K and 230K. Remarkably, the cycloidal magnetic phase drives ferroelectricity, where the material becomes polar. Such improper multiferroics are of great contemporary interest, as a better understanding of the science of magnetoelectric materials may lead to their application in actuators, sensors and solid state memories. Improper multiferroics also have novel quasiparticle excitations: electromagnons form when spin-waves become electric-dipole active. By examining the dynamic response of spins as they interact with THz radiation we gain insights into the underlying physics of multi-ferroics. In contrast to improper ferroelectrics, where magnetism drives structural inversion asymmetry (SIA), two-dimensional electronic systems can exhibit non-degenerate spin states as a consequence of SIA created by strain and/or electric fields. We identify and explore the influence of the Rashba spin-orbit interaction upon cyclotron resonance at terahertz frequencies in high-mobility 2D hole gases in germanium quantum wells. An enhanced Rashba spin-orbit interaction can be linked to the strain of the quantum well, while a time-frequency decomposition method permitted the dynamical formation and decay of spin-split cyclotron resonances to be tracked on picosecond timescales. Long spin-decoherence times concurrent with high hole mobilities highlight the potential of Ge quantum wells in spintronics.
Static and dynamic properties of interacting spin-1 bosons in an optical lattice
Natu, Stefan S.; Pixley, J. H.; Das Sarma, S.
2015-04-01
We study the physics of interacting spin-1 bosons in an optical lattice using a variational Gutzwiller technique. We compute the mean-field ground state wave function and discuss the evolution of the condensate, spin, nematic, and singlet order parameters across the superfluid-Mott transition. We then extend the Gutzwiller method to derive the equations governing the dynamics of low energy excitations in the lattice. Linearizing these equations, we compute the excitation spectra in the superfluid and Mott phases for both ferromagnetic and antiferromagnetic spin-spin interactions. In the superfluid phase, we recover the known excitation spectrum obtained from Bogoliubov theory. In the nematic Mott phase, we obtain gapped, quadratically dispersing particle and hole-like collective modes, whereas in the singlet Mott phase, we obtain a nondispersive gapped mode, corresponding to the breaking of a singlet pair. For the ferromagnetic Mott insulator, the Gutzwiller mean-field theory only yields particle-hole-like modes but no Goldstone mode associated with long-range spin order. To overcome this limitation, we supplement the Gutzwiller theory with a Schwinger boson mean-field theory which captures superexchange-driven fluctuations. In addition to the gapped particle-hole-like modes, we obtain a gapless quadratically dispersing ferromagnetic spin-wave Goldstone mode. We discuss the evolution of the singlet gap, particle-hole gap, and the effective mass of the ferromagnetic Goldstone mode as the superfluid-Mott phase boundary is approached from the insulating side. We discuss the relevance and validity of Gutzwiller mean-field theories to spinful systems, and potential extensions of this framework to include more exotic physics which appears in the presence of spin-orbit coupling or artificial gauge fields.
Spin-current probe for phase transition in an insulator
Qiu, Zhiyong; Li, Jia; Hou, Dazhi; Arenholz, Elke; N'diaye, Alpha T.; Tan, Ali; Uchida, Ken-Ichi; Sato, Koji; Okamoto, Satoshi; Tserkovnyak, Yaroslav; Qiu, Z. Q.; Saitoh, Eiji
2016-08-01
Spin fluctuation and transition have always been one of the central topics of magnetism and condensed matter science. Experimentally, the spin fluctuation is found transcribed onto scattering intensity in the neutron-scattering process, which is represented by dynamical magnetic susceptibility and maximized at phase transitions. Importantly, a neutron carries spin without electric charge, and therefore it can bring spin into a sample without being disturbed by electric energy. However, large facilities such as a nuclear reactor are necessary. Here we show that spin pumping, frequently used in nanoscale spintronic devices, provides a desktop microprobe for spin transition; spin current is a flux of spin without an electric charge and its transport reflects spin excitation. We demonstrate detection of antiferromagnetic transition in ultra-thin CoO films via frequency-dependent spin-current transmission measurements, which provides a versatile probe for phase transition in an electric manner in minute devices.
Spin dynamics of ZnSe-ZnTe nanostructures grown by migration enhanced molecular beam epitaxy
Deligiannakis, Vasilios; Dhomkar, Siddharth; Ji, Haojie; Pagliero, Daniela; Kuskovsky, Igor L.; Meriles, Carlos A.; Tamargo, Maria C.
2017-03-01
We study the spin dynamics of ZnSe layers with embedded type-II ZnTe quantum dots using time resolved Kerr rotation (TRKR). Three samples were grown with an increasing amount of Te, which correlates with increased quantum dot (QD) density. Samples with a higher quantum dot density exhibit longer electron spin lifetimes, up to ˜1 ns at low temperatures. Tellurium isoelectronic centers, which form in the ZnSe spacer regions as a result of the growth conditions, were probed via spectrally dependent TRKR. Temperature dependent TRKR results show that samples with high QD density are not affected by an electron-hole exchange dephasing mechanism.
Equilibrium dynamics of the sub-Ohmic spin-boson model under bias
Zheng, Da-Chuan; Tong, Ning-Hua
2017-06-01
Using the bosonic numerical renormalization group method, we studied the equilibrium dynamical correlation function C(ω) of the spin operator σ z for the biased sub-Ohmic spin-boson model. The small-ω behavior C(ω )\\propto {ω }s is found to be universal and independent of the bias ɛ and the coupling strength α (except at the quantum critical point α ={α }{{c}} and ɛ = 0). Our NRG data also show C(ω )\\propto {χ }2{ω }s for a wide range of parameters, including the biased strong coupling regime (\\varepsilon \
Solvent interactions and protein dynamics in spin-labeled T4 lysozyme.
Stoica, I
2004-06-01
Aspects of T4 lysozyme dynamics and solvent interaction are investigated using atomically detailed Molecular Dynamics (MD) simulations. Two spin-labeled mutants of T4 lysozyme are analyzed (T4L-N40C and T4L-K48C), which have been found from electronic paramagnetic resonance (EPR) experiments to exhibit different mobilities at the site of spin probe attachment (N- and C-terminus of helix B, respectively). Similarities and differences in solvent distribution and diffusion around the spin label, as well as around exposed and buried residues within the protein, are discussed. The purpose is to capture possible strong interactions between the spin label (ring) and solvent molecules, which may affect EPR lineshapes. The effect of backbone motions on the water density profiles is also investigated. The focus is on the domain closure associated with the T4 lysozyme hinge-bending motion, which is analyzed by Essential Dynamics (ED). The N-terminus of helix B is found to be a "hinge" residue, which explains the high degree of flexibility and motional freedom at this site.
Deployment dynamics of a simplified spinning IKAROS solar sail via absolute coordinate based method
Institute of Scientific and Technical Information of China (English)
Jiang Zhao; Qiang Tian; Hai-Yan Hu
2013-01-01
The spinning solar sail of large scale has been well developed in recent years.Such a solar sail can be considered as a rigid-flexible multibody system mainly composed of a spinning central rigid hub,a number of flexible thin tethers,sail membranes,and tip masses.A simplified interplanetary kite-craft accelerated by radiation of the Sun (IKAROS) model is established in this study by using the absolute-coordinate-based (ACB) method that combines the natural coordinate formulation (NCF) describing the central rigid hub and the absolute nodal coordinate formulation (ANCF) describing flexible parts.The initial configuration of the system in the second-stage deployment is determined through both dynamic and static analyses.The huge set of stiff equations of system dynamics is solved by using the generalized-alpha method,and thus the deployment dynamics of the system can be well understood.
Order and thermalized dynamics in Heisenberg-like square and Kagomé spin ices.
Wysin, G M; Pereira, A R; Moura-Melo, W A; de Araujo, C I L
2015-02-25
Thermodynamic properties of a spin ice model on a Kagomé lattice are obtained from dynamic simulations and compared with properties in square lattice spin ice. The model assumes three-component Heisenberg-like dipoles of an array of planar magnetic islands situated on a Kagomé lattice. Ising variables are avoided. The island dipoles interact via long-range dipolar interactions and are restricted in their motion due to local shape anisotropies. We define various order parameters and obtain them and thermodynamic properties from the dynamics of the system via a Langevin equation, solved by the Heun algorithm. Generally, a slow cooling from high to low temperature does not lead to a particular state of order, even for a set of coupling parameters that gives well thermalized states and dynamics. At very low temperature, however, square ice is more likely to reach states near the ground state than Kagomé ice, for the same island coupling parameters.
Universality and extremal aging for dynamics of spin glasses on sub-exponential time scales
Arous, G Ben
2010-01-01
We consider Random Hopping Time (RHT) dynamics of the Sherrington - Kirkpatrick (SK) model and p-spin models of spin glasses. For any of these models and for any inverse temperature we prove that, on time scales that are sub-exponential in the dimension, the properly scaled clock process (time-change process) of the dynamics converges to an extremal process. Moreover, on these time scales, the system exhibits aging like behavior which we called extremal aging. In other words, the dynamics of these models ages as the random energy model (REM) does. Hence, by extension, this confirms Bouchaud's REM-like trap model as a universal aging mechanism for a wide range of systems which, for the first time, includes the SK model.
Nonequilibrium dynamical phase transition of 3D kinetic Ising/Heisenberg spin system
Institute of Scientific and Technical Information of China (English)
Shao Yuan-Zhi; Lai J. K. L.; Shek C. H.; Lin Guang-Ming; Lan Tu
2004-01-01
We have studied the nonequilibrium dynamic phase transitions of both three-dimensional (3D) kinetic Ising and Heisenberg spin systems in the presence of a perturbative magnetic field by Monte Carlo simulation. The feature of the phase transition is characterized by studying the distribution of the dynamical order parameter.In the case of anisotropic Ising spin system (ISS), the dynamic transition is discontinuous and continuous under low and high temperatures respectively, which indicates the existence of a tri-critical point (TCP) on the phase boundary separating low-temperature order phase and high-temperature disorder phase. The TCP shifts towards the higher temperature region with the decrease of frequency, I.e. TTCp=1.33×exp(-ω/30.7). In the case of the isotropic Heisenberg spin system (HSS), however, the situation on dynamic phase transition of HSS is quite different from that of ISS in that no stable dynamical phase transition was observed in kinetic HSS after a threshold time. The evolution of magnetization in the HSS driven by a symmetrical external field after a certain duration always tends asymptotically to a disorder state no matter what an initial state the system starts with. The threshold time τ depends upon the amplitude H0,reduced temperature T/TC and the frequency ωas τ=C·ωα·H-β0·(T/TC)-γ.
P. Arosio; M. Corti; Mariani, M; Orsini, F.; Bogani, L.; A. CANESCHI; Lago, J.; Lascialfari, A.
2015-01-01
The spin dynamics of the molecular magnetic chain [Dy(hfac)(3){NIT(C6H4OPh)}] were investigated by means of the Muon Spin Relaxation (mu+SR) technique. This system consists of a magnetic lattice of alternating Dy(III) ions and radical spins, and exhibits single-chain-magnet behavior. The magnetic properties of [Dy(hfac)(3){NIT(C6H4OPh)}] have been studied by measuring the magnetization vs. temperature at different applied magnetic fields (H - 5, 3500, and 16500 Oe) and by performing mu+SR exp...
Chiang, Yun-Wei; Shimoyama, Yuhei; Feigenson, Gerald W; Freed, Jack H
2004-10-01
The hydrated ternary lamellar lipid mixture of dipalmitoyl-PC/dilauroyl-PC/cholesterol (DPPC/DLPC/Chol) has been studied by electron spin resonance (ESR) to reveal the dynamic structure on a molecular level of the different phases that exist and coexist over virtually the full range of composition. The spectra for more than 100 different compositions at room temperature were analyzed by nonlinear least-squares fitting to provide the rotational diffusion rates and order parameters of the end-chain labeled phospholipid 16-PC. The ESR spectra exhibit substantial variation as a function of composition, even though the respective phases generally differ rather modestly from each other. The Lalpha and Lbeta phases are clearly distinguished, with the former exhibiting substantially lower ordering and greater motional rates, whereas the well-defined Lo phase exhibits the greatest ordering and relatively fast motional rates. Typically, smaller variations occur within a given phase. The ESR spectral analysis also yields phase boundaries and coexistence regions which are found to be consistent with previous results from fluorescence methods, although new features are found. Phase coexistence regions were in some cases confirmed by observing the existence of isosbestic points in the absorption mode ESR spectra from the phases. The dynamic structural properties of the DPPC-rich Lbeta and DLPC-rich Lalpha phases, within their two-phase coexistence region do not change with composition along a tie-line, but the ratio of the two phases follows the lever rule in accordance with thermodynamic principles. The analysis shows that 16-PC spin-label partitions nearly equally between the Lalpha and Lbeta phases, making it a useful probe for studying such coexisting phases. Extensive study of two-phase coexistence regions requires the determination of tie-lines, which were approximated in this study. However, a method is suggested to accurately determine the tie-lines by ESR.
Quantum spin dynamics and entanglement generation with hundreds of trapped ions
Bohnet, Justin G.; Sawyer, Brian C.; Britton, Joseph W.; Wall, Michael L.; Rey, Ana Maria; Foss-Feig, Michael; Bollinger, John J.
2016-06-01
Quantum simulation of spin models can provide insight into problems that are difficult or impossible to study with classical computers. Trapped ions are an established platform for quantum simulation, but only systems with fewer than 20 ions have demonstrated quantum correlations. We studied quantum spin dynamics arising from an engineered, homogeneous Ising interaction in a two-dimensional array of 9Be+ ions in a Penning trap. We verified entanglement in spin-squeezed states of up to 219 ions, directly observing 4.0 ± 0.9 decibels of spectroscopic enhancement, and observed states with non-Gaussian statistics consistent with oversqueezed states. The good agreement with ab initio theory that includes interactions and decoherence lays the groundwork for simulations of the transverse-field Ising model with variable-range interactions, which are generally intractable with classical methods.
Spin dynamics in Kapitza-Dirac scattering of electrons from bichromatic laser fields
Dellweg, Matthias M; Müller, Carsten
2016-01-01
Kapitza-Dirac scattering of nonrelativistic electrons from counterpropagating bichromatic laser waves of linear polarization i s studied. The focus lies on the electronic spin dynamics in the Bragg regime when the laser fields possess a frequency ratio of two. To this end, the time-dependent Pauli equation is solved numerically, both in coordinate space and momentum space. Our numerical results are corroborated by analytical derivations. We demonstrate that, for certain incident electron momenta, the scattering crucially relies on the electron spin which undergo es characteristic Rabi-like oscillations. A parameter regime is identified where the Rabi oscillations reach maximum amplitude. We also briefly discuss spin-dependent Kapitza-Dirac scattering of protons.
Dynamics of extended bodies with spin-induced quadrupole in Kerr spacetime: generic orbits
Han, Wen-Biao
2016-01-01
We discuss motions of extended bodies in Kerr spacetime by using Mathisson-Papapetrou-Dixon equations. We firstly solve the conditions for circular orbits, and calculate the orbital frequency shift due to the mass quadrupoles. The results show that we need not consider the spin-induced quadrupoles in extreme-mass-ratio inspirals for spatial gravitational wave detectors. We quantitatively investigate the temporal variation of rotational velocity of the extended body due to the coupling of quadrupole and background gravitational field. For generic orbits, we numerically integrate the Mathisson-Papapetrou-Dixon equations for evolving the motion of an extended body orbiting a Kerr black hole. By comparing with the monopole-dipole approximation, we reveal the influences of quadrupole moments of extended bodies on the orbital motion and chaotic dynamics of extreme-mass-ratio systems. We do not find any chaotic orbits for the extended bodies with physical spins and spin-induced quadrupoles. Possible implications for...
Skyrmion dynamics in a chiral magnet driven by periodically varying spin currents*
Zhu, Rui; Zhang, Yin-Yan
2016-12-01
In this work, we investigated the spin dynamics in a slab of chiral magnets induced by an alternating (ac) spin current. Periodic trajectories of the skyrmion in real space are discovered under the ac current as a result of the Magnus and viscous forces, which originate from the Gilbert damping, the spin transfer torque, and the β-nonadiabatic torque effects. The results are obtained by numerically solving the Landau-Lifshitz-Gilbert equation and can be explained by the Thiele equation characterizing the skyrmion core motion. Supplementary material in the form of one avi file available from the Journal web page at: http://dx.doi.org/10.1140/epjb/e2016-70467-9
Experimental test of the new analytic matrix formalism for spin dynamics
Directory of Open Access Journals (Sweden)
V. S. Morozov
2007-04-01
Full Text Available We recently started testing Chao’s proposed new matrix formalism for describing the spin dynamics due to a single spin resonance. The Chao formalism is probably the first fundamental improvement of the Froissart-Stora equation in that it allows analytic calculations of the beam polarization’s behavior inside a resonance. We tested the Chao formalism using a 1.85 GeV/c polarized deuteron beam stored in COSY, by sweeping an rf dipole’s frequency through 200 Hz, while varying the distance from the sweep’s end frequency to an rf-induced spin resonance’s central frequency. Since the Froissart-Stora equation itself can make no prediction inside a resonance, we compared our experimental data with the predictions of the Chao formalism and those of an empirical two-fluid model based on the Froissart-Stora equation. The data strongly favor the Chao formalism.
Quantum spin dynamics and entanglement generation with hundreds of trapped ions
Bohnet, Justin G; Britton, Joseph W; Wall, Michael L; Rey, Ana Maria; Foss-Feig, Michael; Bollinger, John J
2015-01-01
Quantum simulation of spin models can provide insight into complex problems that are difficult or impossible to study with classical computers. Trapped ions are an established platform for quantum simulation, but only systems with fewer than 20 ions have demonstrated quantum correlations. Here we study non-equilibrium, quantum spin dynamics arising from an engineered, homogeneous Ising interaction in a two-dimensional array of $^9$Be$^+$ ions in a Penning trap. We verify entanglement in the form of spin-squeezed states for up to 219 ions, directly observing 4.0$\\pm$0.9 dB of spectroscopic enhancement. We also observe evidence of non-Gaussian, over-squeezed states in the full counting statistics. We find good agreement with ab-initio theory that includes competition between entanglement and decoherence, laying the groundwork for simulations of the transverse-field Ising model with variable-range interactions, for which numerical solutions are, in general, classically intractable.
Valero, Rosendo; Truhlar, Donald G
2007-09-06
A diabatic representation is convenient in the study of electronically nonadiabatic chemical reactions because the diabatic energies and couplings are smooth functions of the nuclear coordinates and the couplings are scalar quantities. A method called the fourfold way was devised in our group to generate diabatic representations for spin-free electronic states. One drawback of diabatic states computed from the spin-free Hamiltonian, called a valence diabatic representation, for systems in which spin-orbit coupling cannot be ignored is that the couplings between the states are not zero in asymptotic regions, leading to difficulties in the calculation of reaction probabilities and other properties by semiclassical dynamics methods. Here we report an extension of the fourfold way to construct diabatic representations suitable for spin-coupled systems. In this article we formulate the method for the case of even-electron systems that yield pairs of fragments with doublet spin multiplicity. For this type of system, we introduce the further simplification of calculating the triplet diabatic energies in terms of the singlet diabatic energies via Slater's rules and assuming constant ratios of Coulomb to exchange integrals. Furthermore, the valence diabatic couplings in the triplet manifold are taken equal to the singlet ones. An important feature of the method is the introduction of scaling functions, as they allow one to deal with multibond reactions without having to include high-energy diabatic states. The global transformation matrix to the new diabatic representation, called the spin-valence diabatic representation, is constructed as the product of channel-specific transformation matrices, each one taken as the product of an asymptotic transformation matrix and a scaling function that depends on ratios of the spin-orbit splitting and the valence splittings. Thus the underlying basis functions are recoupled into suitable diabatic basis functions in a manner that
Dynamic nuclear spin polarization in the resonant laser excitation of an InGaAs quantum dot.
Högele, A; Kroner, M; Latta, C; Claassen, M; Carusotto, I; Bulutay, C; Imamoglu, A
2012-05-11
Resonant optical excitation of lowest-energy excitonic transitions in self-assembled quantum dots leads to nuclear spin polarization that is qualitatively different from the well-known optical orientation phenomena. By carrying out a comprehensive set of experiments, we demonstrate that nuclear spin polarization manifests itself in quantum dots subjected to finite external magnetic field as locking of the higher energy Zeeman transition to the driving laser field, as well as the avoidance of the resonance condition for the lower energy Zeeman branch. We interpret our findings on the basis of dynamic nuclear spin polarization originating from noncollinear hyperfine interaction and find excellent agreement between experiment and theory. Our results provide evidence for the significance of noncollinear hyperfine processes not only for nuclear spin diffusion and decay, but also for buildup dynamics of nuclear spin polarization in a coupled electron-nuclear spin system.
Replica exchange Monte Carlo simulations of the ising spin glass: Static and dynamic properties
Yucesoy, Burcu
Spin glasses have been the subject of intense study and considerable controversy for decades, and the low-temperature phase of short-range spin glasses is still poorly understood. Our main goal is to improve our understanding in this area and find an answer to the following question: Are there only a single pair or a countable infinity of pure states in the low temperature phase of the EA spin glass? To that aim we first start by introducing spin glasses and provide a brief history of their research, then proceed to describe our method of simulation, the parallel tempering Monte Carlo algorithm. Next, we present the results of a large-scale numerical study of the equilibrium three-dimensional Edwards-Anderson Ising spin glass with Gaussian disorder. In order to understand how the parallel tempering algorithm works, we measure various static, as well as dynamical quantities, such as the autocorrelation times and round-trip times for the parallel tempering Monte Carlo method. We examine the correlation between static and dynamic observables for ˜ 5000 disorder realizations and up to 1000 spins down to temperatures at 20% of the critical temperature, and our results show that autocorrelation times are directly correlated with the roughness of the free-energy landscape. In the following chapters, the three- and four-dimensional Edwards-Anderson and mean-field Sherrington-Kirkpatrick Ising spin glasses are studied again via large scale Monte Carlo simulations at low temperatures, deep within the spin glass phase. Performing a careful statistical analysis of several thousand independent disorder realizations and using an observable that detects peaks in the overlap distribution, we show that the Sherrington-Kirkpatrick and Edwards-Anderson models have a distinctly different low-temperature behavior. We arrive to the following conclusion: The structure of the spin-glass overlap distribution for the Edwards-Anderson model suggests that its low-temperature phase has only a
Institute of Scientific and Technical Information of China (English)
XIE Gang; HAN Ru-Shan
2001-01-01
We further calculate the dependence of xT on T in high magnetic fields,where X denotes susceptibility and T is temperature,using our previous research work - Green function's decoupling approximate approach,for the one-dimensional ferrimagnetic chain with alternating spins 1 and 1/2.We find a linear correlation in certain range of magnetic field between the temperature of xT maximum and the magnetic field.Moreover,we simply analyze its physical meaning by our approach.``
Discrete-time dynamic network model for the spread of susceptible-infective-recovered diseases
Chauhan, Sanjeev Kumar
2017-07-01
We propose a discrete-time dynamic network model describing the spread of susceptible-infective-recovered diseases in a population. We consider the case in which the nodes in the network change their links due to social mixing dynamics as well as in response to the disease. The model shows the behavior that, as we increase social mixing, disease spread is inhibited in certain cases, while in other cases it is enhanced. We also extend this dynamic network model to take into account the case of hidden infection. Here we find that, as expected, the disease spreads more readily if there is a time period after contracting the disease during which an individual is infective but is not known to have the disease.
Proton-driven spin diffusion in rotating solids via reversible and irreversible quantum dynamics.
Veshtort, Mikhail; Griffin, Robert G
2011-10-07
Proton-driven spin diffusion (PDSD) experiments in rotating solids have received a great deal of attention as a potential source of distance constraints in large biomolecules. However, the quantitative relationship between the molecular structure and observed spin diffusion has remained obscure due to the lack of an accurate theoretical description of the spin dynamics in these experiments. We start with presenting a detailed relaxation theory of PDSD in rotating solids that provides such a description. The theory applies to both conventional and radio-frequency-assisted PDSD experiments and extends to the non-Markovian regime to include such phenomena as rotational resonance (R(2)). The basic kinetic equation of the theory in the non-Markovian regime has the form of a memory function equation, with the role of the memory function played by the correlation function. The key assumption used in the derivation of this equation expresses the intuitive notion of the irreversible dissipation of coherences in macroscopic systems. Accurate expressions for the correlation functions and for the spin diffusion constants are given. The theory predicts that the spin diffusion constants governing the multi-site PDSD can be approximated by the constants observed in the two-site diffusion. Direct numerical simulations of PDSD dynamics via reversible Liouville-von Neumann equation are presented to support and compliment the theory. Remarkably, an exponential decay of the difference magnetization can be observed in such simulations in systems consisting of only 12 spins. This is a unique example of a real physical system whose typically macroscopic and apparently irreversible behavior can be traced via reversible microscopic dynamics. An accurate value for the spin diffusion constant can be usually obtained through direct simulations of PDSD in systems consisting of two (13)C nuclei and about ten (1)H nuclei from their nearest environment. Spin diffusion constants computed by this
Immense Magnetic Response of Exciplex Light Emission due to Correlated Spin-Charge Dynamics
Wang, Yifei; Sahin-Tiras, Kevser; Harmon, Nicholas J.; Wohlgenannt, Markus; Flatté, Michael E.
2016-01-01
As carriers slowly move through a disordered energy landscape in organic semiconductors, tiny spatial variations in spin dynamics relieve spin blocking at transport bottlenecks or in the electron-hole recombination process that produces light. Large room-temperature magnetic-field effects (MFEs) ensue in the conductivity and luminescence. Sources of variable spin dynamics generate much larger MFEs if their spatial structure is correlated on the nanoscale with the energetic sites governing conductivity or luminescence such as in coevaporated organic blends within which the electron resides on one molecule and the hole on the other (an exciplex). Here, we show that exciplex recombination in blends exhibiting thermally activated delayed fluorescence produces MFEs in excess of 60% at room temperature. In addition, effects greater than 4000% can be achieved by tuning the device's current-voltage response curve by device conditioning. Both of these immense MFEs are the largest reported values for their device type at room temperature. Our theory traces this MFE and its unusual temperature dependence to changes in spin mixing between triplet exciplexes and light-emitting singlet exciplexes. In contrast, spin mixing of excitons is energetically suppressed, and thus spin mixing produces comparatively weaker MFEs in materials emitting light from excitons by affecting the precursor pairs. Demonstration of immense MFEs in common organic blends provides a flexible and inexpensive pathway towards magnetic functionality and field sensitivity in current organic devices without patterning the constituent materials on the nanoscale. Magnetic fields increase the power efficiency of unconditioned devices by 30% at room temperature, also showing that magnetic fields may increase the efficiency of the thermally activated delayed fluorescence process.
X-ray imaging of spin currents and magnetisation dynamics at the nanoscale
Bonetti, Stefano
2017-04-01
Understanding how spins move in time and space is the aim of both fundamental and applied research in modern magnetism. Over the past three decades, research in this field has led to technological advances that have had a major impact on our society, while improving the understanding of the fundamentals of spin physics. However, important questions still remain unanswered, because it is experimentally challenging to directly observe spins and their motion with a combined high spatial and temporal resolution. In this article, we present an overview of the recent advances in x-ray microscopy that allow researchers to directly watch spins move in time and space at the microscopically relevant scales. We discuss scanning x-ray transmission microscopy (STXM) at resonant soft x-ray edges, which is available at most modern synchrotron light sources. This technique measures magnetic contrast through the x-ray magnetic circular dichroism (XMCD) effect at the resonant absorption edges, while focusing the x-ray radiation at the nanometre scale, and using the intrinsic pulsed structure of synchrotron-generated x-rays to create time-resolved images of magnetism at the nanoscale. In particular, we discuss how the presence of spin currents can be detected by imaging spin accumulation, and how the magnetisation dynamics in thin ferromagnetic films can be directly imaged. We discuss how a direct look at the phenomena allows for a deeper understanding of the the physics at play, that is not accessible to other, more indirect techniques. Finally, we present an overview of the exciting opportunities that lie ahead to further understand the fundamentals of novel spin physics, opportunities offered by the appearance of diffraction limited storage rings and free electron lasers.
Dynamic magnetization switching and spin wave excitations by voltage-induced torque
Shiota, Yoichi
2013-03-01
The effect of electric fields on ultrathin ferromagnetic metal layer is one of the promising approaches for manipulating the spin direction with low-energy consumption, localization, and coherent behavior. Several experimental approaches to realize it have been investigated using ferromagnetic semiconductors, magnetostriction together with piezo-electric materials, multiferroic materials, and ultrathin ferromagnetic layer. In this talk, we will present a dynamic control of spins by voltage-induced torque. We used the magnetic tunnel junctions with ultrathin ferromagnetic layer, which shows voltage-induced perpendicular magnetic anisotropy change. By applying the voltage to the junction, the magnetic easy-axis in the ultrathin ferromagnetic layer changes from in-plane to out-of-plane, which causes a precession of the spins. This precession resulted in a two-way toggle switching by determining an appropriate pulse length. On the other hand, an application of rf-voltage causes an excitation of a uniform spin-wave. Since the precession of spin associates with an oscillation in the resistance of the junction, the applied rf-signal is rectified and produces a dc-voltage. From the spectrum of the dc-voltage as a function of frequency, we could estimate the voltage-induced torque. This research was supported by CREST-JST, G-COE program, and JSPS for the fellowship. Collaborators include T. Nozaki, S. Miwa, F. Bonell, N. Mizuochi, T. Shinjo, and Y. Suzuki.
Charge Dynamics and Spin Blockade in a Hybrid Double Quantum Dot in Silicon
Directory of Open Access Journals (Sweden)
Matias Urdampilleta
2015-08-01
Full Text Available Electron spin qubits in silicon, whether in quantum dots or in donor atoms, have long been considered attractive qubits for the implementation of a quantum computer because of silicon’s “semiconductor vacuum” character and its compatibility with the microelectronics industry. While donor electron spins in silicon provide extremely long coherence times and access to the nuclear spin via the hyperfine interaction, quantum dots have the complementary advantages of fast electrical operations, tunability, and scalability. Here, we present an approach to a novel hybrid double quantum dot by coupling a donor to a lithographically patterned artificial atom. Using gate-based rf reflectometry, we probe the charge stability of this double quantum-dot system and the variation of quantum capacitance at the interdot charge transition. Using microwave spectroscopy, we find a tunnel coupling of 2.7 GHz and characterize the charge dynamics, which reveals a charge T_{2}^{*} of 200 ps and a relaxation time T_{1} of 100 ns. Additionally, we demonstrate a spin blockade at the inderdot transition, opening up the possibility to operate this coupled system as a singlet-triplet qubit or to transfer a coherent spin state between the quantum dot and the donor electron and nucleus.
New insights into electron spin dynamics in the presence of correlated noise.
Spezia, S; Adorno, D Persano; Pizzolato, N; Spagnolo, B
2012-02-08
The changes in the spin depolarization length in zinc-blende semiconductors when an external component of correlated noise is added to a static driving electric field are analyzed for different values of field strength, noise amplitude and correlation time. Electron dynamics is simulated by a Monte Carlo procedure which takes into account all the possible scattering phenomena of the hot electrons in the medium and includes the evolution of spin polarization. Spin depolarization is studied by examining the decay of the initial spin polarization of the conduction electrons through the D'yakonov-Perel process, the only relevant relaxation mechanism in III-V crystals. Our results show that, for electric field amplitudes lower than the Gunn field, the dephasing length shortens with increasing noise intensity. Moreover, a nonmonotonic behavior of spin depolarization length with the noise correlation time is found, characterized by a maximum variation for values of noise correlation time comparable with the dephasing time. Instead, in high field conditions, we find that, critically depending on the noise correlation time, external fluctuations can positively affect the relaxation length. The influence of the inclusion of the electron-electron scattering mechanism is also shown and discussed.
Finite-temperature dynamics and thermal intraband magnon scattering in Haldane spin-one chains
Becker, J.; Köhler, T.; Tiegel, A. C.; Manmana, S. R.; Wessel, S.; Honecker, A.
2017-08-01
The antiferromagnetic spin-one chain is considerably one of the most fundamental quantum many-body systems, with symmetry-protected topological order in the ground state. Here, we present results for its dynamical spin structure factor at finite temperatures, based on a combination of exact numerical diagonalization, matrix-product-state calculations, and quantum Monte Carlo simulations. Open finite chains exhibit a subgap band in the thermal spectral functions, indicative of localized edge states. Moreover, we observe the thermal activation of a distinct low-energy continuum contribution to the spin spectral function with an enhanced spectral weight at low momenta and its upper threshold. This emerging thermal spectral feature of the Haldane spin-one chain is shown to result from intraband magnon scattering due to the thermal population of the single-magnon branch, which features a large bandwidth-to-gap ratio. These findings are discussed with respect to possible future studies on spin-one chain compounds based on inelastic neutron scattering.
Tsurkan, V.; Prodan, L.; Felea, V.; Filippova, I.; Kravtsov, V.; Günther, A.; Widmann, S.; Krug von Nidda, H.-A.; Deisenhofer, J.; Loidl, A.
2017-08-01
We report structure, susceptibility, and specific heat studies of stoichiometric and off-stoichiometric poly- and single crystals of the A -site spinel compound FeS c2S4 . In stoichiometric samples, no long-range magnetic order is found down to 1.8 K. The magnetic susceptibility of these samples is field independent in the temperature range 10-400 K and does not show irreversible effects at low temperatures. In contrast, the magnetic susceptibility of samples with iron excess shows substantial field dependence at high temperatures and manifests a pronounced magnetic irreversibility at low temperatures with a difference between zero-field cooled (ZFC) and field cooled (FC) susceptibilities and a maximum at 10 K, reminiscent of a magnetic transition. Single-crystal x-ray diffraction of the stoichiometric samples revealed a single phase spinel structure without site inversion. In single crystalline samples with Fe excess, in addition to the main spinel phase, a second ordered single-crystal phase was detected with the diffraction pattern of a vacancy-ordered superstructure of iron sulfide, close to the 5C polytype F e9S10 . Specific heat studies reveal a broad anomaly, which evolves below 20 K in both stoichiometric and off-stoichiometric crystals. We show that the low-temperature specific heat can be well described by considering the low-lying spin-orbital electronic levels of F e2 + ions. Our results demonstrate significant influence of excess Fe ions on intrinsic magnetic behavior of FeS c2S4 and provide support for the spin-orbital liquid scenario proposed in earlier studies for the stoichiometric compound.
Pulse and quench induced dynamical phase transition in a chiral multiferroic spin chain
Azimi, M.; Sekania, M.; Mishra, S. K.; Chotorlishvili, L.; Toklikishvili, Z.; Berakdar, J.
2016-08-01
Quantum dynamics of magnetic order in a chiral multiferroic chain is studied. We consider two different scenarios: ultrashort terahertz excitations or a sudden electric field quench. Performing analytical and numerical exact diagonalization calculations, we trace the pulse induced spin dynamics and extract quantities that are relevant to quantum information processing. In particular, we analyze the dynamics of the system chirality, the von Neumann entropy, and the pairwise and many-body entanglement. If the characteristic frequencies of the generated states are noncommensurate, then a partial loss of pair concurrence occurs. Increasing the system size, this effect becomes even more pronounced. Many-particle entanglement and chirality are robust and persist in the incommensurate phase. To analyze the dynamical quantum transitions for the quenched and pulsed dynamics we combined the Weierstrass factorization technique for entire functions and the Lanczos exact diagonalization method. For a small system we obtained analytical results including the rate function of the Loschmidt echo. Exact numerical calculations for a system up to 40 spins confirm phase transition. Quench-induced dynamical transitions have been extensively studied recently. Here we show that related dynamical transitions can be achieved and controlled by appropriate electric field pulses.
Kawecki, M.; Gutfreund, P.; Adlmann, F. A.; Lindholm, E.; Longeville, S.; Lapp, A.; Wolff, M.
2016-09-01
Neutron Spin Echo spectroscopy provides unique insight into molecular and submolecular dynamics as well as intra- and inter-molecular interactions in soft matter. These dynamics may change drastically under shear flow. In particular in polymer physics a stress plateau is observed, which might be explained by an entanglement-disentanglement transition. However, such a transition is difficult to identify directly by experiments. Neutron Spin Echo has been proven to provide information about entanglement length and degree by probing the local dynamics of the polymer chains. Combining shear experiments and neutron spin echo is challenging since, first the beam polarisation has to be preserved during scattering and second, Doppler scattered neutrons may cause inelastic scattering. In this paper we present a new shear device adapted for these needs. We demonstrate that a high beam polarisation can be preserved and present first data on an entangled polymer solution under shear. To complement the experiments on the dynamics we present novel SANS data revealing shear- induced conformational changes in highly entangled polymers.
Imaging Spin Dynamics on the Nanoscale using X-Ray Microscopy
Directory of Open Access Journals (Sweden)
Hermann eStoll
2015-04-01
Full Text Available The dynamics of emergent magnetic quasiparticles, such as vortices, domain walls, and bubbles are studied by scanning transmission x-ray microscopy (STXM, combining magnetic (XMCD contrast with about 25 nm lateral resolution as well as 70 ps time resolution. Essential progress in the understanding of magnetic vortex dynamics is achieved by vortex core reversal observed by sub-GHz excitation of the vortex gyromode, either by ac magnetic fields or spin transfer torque. The basic switching scheme for this vortex core reversal is the generation of a vortex-antivortex pair. Much faster vortex core reversal is obtained by exciting azimuthal spin wave modes with (multi-GHz rotating magnetic fields or orthogonal monopolar field pulses in x and y direction, down to 45 ps in duration. In that way unidirectional vortex core reversal to the vortex core 'down' or 'up' state only can be achieved with switching times well below 100 ps. Coupled modes of interacting vortices mimic crystal properties. The individual vortex oscillators determine the properties of the ensemble, where the gyrotropic mode represents the fundamental excitation. By self-organized state formation we investigate distinct vortex core polarization configurations and understand these eigenmodes in an extended Thiele model. Analogies with photonic crystals are drawn. Oersted fields and spin-polarized currents are used to excite the dynamics of domain walls and magnetic bubbles. From the measured phase and amplitude of the displacement of domain walls we deduce the size of the non-adiabatic spin-transfer torque. For sensing applications, the displacement of domain walls is studied and a direct correlation between domain wall velocity and spin structure is found. Finally the synchronous displacement of multiple domain walls using perpendicular field pulses is demonstrated as a possible paradigm shift for magnetic memory and logic applications.
Imaging Spin Dynamics on the Nanoscale using X-Ray Microscopy
Stoll, Hermann; Noske, Matthias; Weigand, Markus; Richter, Kornel; Krüger, Benjamin; Reeve, Robert; Hänze, Max; Adolff, Christian; Stein, Falk-Ulrich; Meier, Guido; Kläui, Mathias; Schütz, Gisela
2015-04-01
The dynamics of emergent magnetic quasiparticles, such as vortices, domain walls, and bubbles are studied by scanning transmission x-ray microscopy (STXM), combining magnetic (XMCD) contrast with about 25 nm lateral resolution as well as 70 ps time resolution. Essential progress in the understanding of magnetic vortex dynamics is achieved by vortex core reversal observed by sub-GHz excitation of the vortex gyromode, either by ac magnetic fields or spin transfer torque. The basic switching scheme for this vortex core reversal is the generation of a vortex-antivortex pair. Much faster vortex core reversal is obtained by exciting azimuthal spin wave modes with (multi-GHz) rotating magnetic fields or orthogonal monopolar field pulses in x and y direction, down to 45 ps in duration. In that way unidirectional vortex core reversal to the vortex core 'down' or 'up' state only can be achieved with switching times well below 100 ps. Coupled modes of interacting vortices mimic crystal properties. The individual vortex oscillators determine the properties of the ensemble, where the gyrotropic mode represents the fundamental excitation. By self-organized state formation we investigate distinct vortex core polarization configurations and understand these eigenmodes in an extended Thiele model. Analogies with photonic crystals are drawn. Oersted fields and spin-polarized currents are used to excite the dynamics of domain walls and magnetic bubbles. From the measured phase and amplitude of the displacement of domain walls we deduce the size of the non-adiabatic spin-transfer torque. For sensing applications, the displacement of domain walls is studied and a direct correlation between domain wall velocity and spin structure is found. Finally the synchronous displacement of multiple domain walls using perpendicular field pulses is demonstrated as a possible paradigm shift for magnetic memory and logic applications.
McHaourab, Hassane S; Steed, P Ryan; Kazmier, Kelli
2011-11-09
Trapping membrane proteins in the confines of a crystal lattice obscures dynamic modes essential for interconversion between multiple conformations in the functional cycle. Moreover, lattice forces could conspire with detergent solubilization to stabilize a minor conformer in an ensemble thus confounding mechanistic interpretation. Spin labeling in conjunction with electron paramagnetic resonance (EPR) spectroscopy offers an exquisite window into membrane protein dynamics in the native-like environment of a lipid bilayer. Systematic application of spin labeling and EPR identifies sequence-specific secondary structures, defines their topology and their packing in the tertiary fold. Long range distance measurements (60 Å-80 Å) between pairs of spin labels enable quantitative analysis of equilibrium dynamics and triggered conformational changes. This review highlights the contribution of spin labeling to bridging structure and mechanism. Efforts to develop methods for determining structures from EPR restraints and to increase sensitivity and throughput promise to expand spin labeling applications in membrane protein structural biology.
Dynamics of asteroid family halos constrained by spin/shape models
Broz, Miroslav
2016-10-01
A number of asteroid families cannot be identified solely on the basis of the Hierarchical Clustering Method (HCM), because they have additional 'former' members in the surroundings which constitute a so called halo (e.g. Broz & Morbidelli 2013). They are usually mixed up with the background population which has to be taken into account too.Luckily, new photometric observations allow to derive new spin/shape models, which serve as independent constraints for dynamical models. For example, a recent census of the Eos family shows 43 core and 27 halo asteroids (including background) with known spin orientations.To this point, we present a complex spin-orbital model which includes full N-body dynamics and consequently accounts for all mean-motion, secular, or three-body gravitational resonances, the Yarkovsky drift, YORP effect, collisional reorientations and also spin-orbital interactions. These are especially important for the Koronis family. In this project, we make use of data from the DAMIT database and ProjectSoft Blue Eye 600 observatory.
Dynamics of open quantum spin systems: An assessment of the quantum master equation approach.
Zhao, P; De Raedt, H; Miyashita, S; Jin, F; Michielsen, K
2016-08-01
Data of the numerical solution of the time-dependent Schrödinger equation of a system containing one spin-1/2 particle interacting with a bath of up to 32 spin-1/2 particles is used to construct a Markovian quantum master equation describing the dynamics of the system spin. The procedure of obtaining this quantum master equation, which takes the form of a Bloch equation with time-independent coefficients, accounts for all non-Markovian effects inasmuch the general structure of the quantum master equation allows. Our simulation results show that, with a few rather exotic exceptions, the Bloch-type equation with time-independent coefficients provides a simple and accurate description of the dynamics of a spin-1/2 particle in contact with a thermal bath. A calculation of the coefficients that appear in the Redfield master equation in the Markovian limit shows that this perturbatively derived equation quantitatively differs from the numerically estimated Markovian master equation, the results of which agree very well with the solution of the time-dependent Schrödinger equation.
Coupled intertwiner dynamics - a toy model for coupling matter to spin foam models
Steinhaus, Sebastian
2015-01-01
The universal coupling of matter and gravity is one of the most important features of general relativity. In quantum gravity, in particular spin foams, matter couplings have been defined in the past, yet the mutual dynamics, in particular if matter and gravity are strongly coupled, are hardly explored, which is related to the definition of both matter and gravitational degrees of freedom on the discretisation. However extracting this mutual dynamics is crucial in testing the viability of the spin foam approach and also establishing connections to other discrete approaches such as lattice gauge theories. Therefore, we introduce a simple 2D toy model for Yang--Mills coupled to spin foams, namely an Ising model coupled to so--called intertwiner models defined for $\\text{SU}(2)_k$. The two systems are coupled by choosing the Ising coupling constant to depend on spin labels of the background, as these are interpreted as the edge lengths of the discretisation. We coarse grain this toy model via tensor network renor...
Random spin freezing in uranium intermetallic compound UCuSi
Energy Technology Data Exchange (ETDEWEB)
Li Dexin [Institute for Materials Research, Tohoku University, Oarai, Ibaraki 311-1313 (Japan); Nimori, Shigeki [Tsukuba Magnet Laboratory, National Institute for Materials Science, 3-13 Sakura, Tsukuba 305-0003 (Japan); Shiokawa, Yoshinobu [Institute for Materials Research, Tohoku University, Oarai, Ibaraki 311-1313 (Japan)
2006-03-29
The results of low-temperature ac susceptibility, dc magnetization, magnetic relaxation, specific heat, and electrical resistivity measurements on the uranium intermetallic compound UCuSi, a hexagonal CeCd{sub 2}-type non-magnetic atom disorder system, are reported. The results establish that a spin-glass state is formed in this compound at low temperature. Some dynamical parameters characterizing the spin freezing state of this system, such as static spin freezing temperature T{sub s}, critical exponent z{nu}, and activation energy E{sub a}, are determined from dynamical analysis of the ac susceptibility data. The observed properties are discussed based on a magnetic cluster model.
I. Advances in NMR Signal Processing. II. Spin Dynamics in Quantum Dissipative Systems
Energy Technology Data Exchange (ETDEWEB)
Lin, Yung-Ya [Univ. of California, Berkeley, CA (United States)
1998-11-01
Part I. Advances in IVMR Signal Processing. Improvements of sensitivity and resolution are two major objects in the development of NMR/MRI. A signal enhancement method is first presented which recovers signal from noise by a judicious combination of a priordmowledge to define the desired feasible solutions and a set theoretic estimation for restoring signal properties that have been lost due to noise contamination. The effect of noise can be significantly mitigated through the process of iteratively modifying the noisy data set to the smallest degree necessary so that it possesses a collection of prescribed properties and also lies closest to the original data set. A novel detection-estimation scheme is then introduced to analyze noisy and/or strongly damped or truncated FIDs. Based on exponential modeling, the number of signals is detected based on information estimated using the matrix pencil method. theory and the spectral parameters are Part II. Spin Dynamics in body dipole-coupled systems Quantum Dissipative Systems. Spin dynamics in manyconstitutes one of the most fundamental problems in magnetic resonance and condensed-matter physics. Its many-spin nature precludes any rigorous treatment. ‘Therefore, the spin-boson model is adopted to describe in the rotating frame the influence of the dipolar local fields on a tagged spin. Based on the polaronic transform and a perturbation treatment, an analytical solution is derived, suggesting the existence of self-trapped states in the. strong coupling limit, i.e., when transverse local field >> longitudinal local field. Such nonlinear phenomena originate from the joint action of the lattice fluctuations and the reaction field. Under semiclassical approximation, it is found that the main effect of the reaction field is the renormalization of the Hamiltonian of interest. Its direct consequence is the two-step relaxation process: the spin is initially localized in a quasiequilibrium state, which is later detrapped by
Garcia, Yann; Campbell, Stewart J; Lord, James S; Boland, Yves; Ksenofontov, Vadim; Gütlich, Philipp
2007-09-27
The thermal spin transition that occurs in the polymeric chain compound [Fe(NH(2)trz)3](NO3)2 above room temperature has been investigated by zero-field muon spin relaxation (microSR) over the temperature range approximately 8-402 K. The depolarization curves are best described by a Lorentzian and a Gaussian line that represent fast and slow components, respectively. The spin transition is associated with a hysteresis loop of width DeltaT = 34 K (T1/2 upward arrow = 346 K and T1/2 downward arrow = 312 K) that has been delineated by the temperature variation of the initial asymmetry parameter, in good agreement with previously published magnetic measurements. Zero-field and applied field (20-2000 Oe) microSR measurements show the presence of diamagnetic muon species and paramagnetic muonium radical species (A = 753 +/- 77 MHz) over the entire temperature range. Fast dynamics have been revealed in the high-spin state of [Fe(NH(2)trz)3](NO3)2 with the presence of a Gaussian relaxation mode that is mostly due to the dipolar interaction with static nuclear moments. This situation, where the muonium radicals are totally decoupled and not able to sense paramagnetic fluctuations, implies that the high-spin dynamics fall outside the muon time scale. Insights to the origin of the cooperative effects associated with the spin transition of [Fe(NH(2)trz)3](NO3)2 through muon implantation are presented.
Entanglement dynamics of electron spins in quantum dots under a nonuniform magnetic field
Energy Technology Data Exchange (ETDEWEB)
Zhou, Feng-Xue; Qi, Yi-Hong; Niu, Yue-Ping; Gong, Shang-Qing [East China University of Science and Technology, Shanghai (China); Qian, Jun [Chinese Academy of Sciences, Shanghai (China); Yu, Ting [Stevens Institute of Technology, Hoboken, NJ (United States)
2012-04-15
We investigate entanglement of two coupled electron spins in quantum dots (QDs) in the presence of an inhomogeneous magnetic field. The important effects of the inhomogeneous field are discussed for the dynamics of entanglement. Due to the system's symmetry, the inhomogeneity of the field is shown not to affect the evolution of entanglement for Φ-type Bell state while it plays a key role for Ψ-type Bell state. For the maximal entangled Bell states, the field is positive for the entanglement dynamics. The mean field can increase the entanglement revival for Φ-type Bell state while an inhomogeneous field can promote the entanglement revival for Ψ-type Bell state. For the unentangled initial states, the field is destructive for the entanglement generation induced by the coupling of the two spins.
Theoretical approaches to control spin dynamics in solid-state nuclear magnetic resonance
Indian Academy of Sciences (India)
Eugene Stephane Mananga
2015-12-01
This article reviews theoretical approaches for controlling spin dynamics in solid-state nuclear magnetic resonance. We present fundamental theories in the history of NMR, namely, the average Hamiltonian and Floquet theories. We also discuss emerging theories such as the Fer and Floquet-Magnus expansions. These theories allow one to solve the time-dependent Schrodinger equation, which is still the central problem in spin dynamics of solid-state NMR. Examples from the literature that highlight several applications of these theories are presented, and particular attention is paid to numerical integrators and propagator operators. The problem of time propagation calculated with Chebychev expansion and the future development of numerical directions with the Cayley transformation are considered. The bibliography includes 190 references.
Azevedo, F S; Castro, Luis B; Filgueiras, Cleverson; Cogollo, D
2015-01-01
The planar quantum dynamics of spin-1/2 neutral particle interacting with electrical fields is considered. A set of first order differential equations are obtained directly from the planar Dirac equation with nonminimum coupling. New solutions of this system, in particular, for the Aharonov-Casher effect, are found and discussed in detail. Pauli equation is also obtained by studying the motion of the particle when it describes a circular path of constant radius. We also analyze the planar dynamics in the full space, including the $r=0$ region. The self-adjoint extension method is used to obtain the energy levels and wave functions of the particle for two particular values for the self-adjoint extension parameter. The energy levels obtained are analogous to the Landau levels and explicitly depend on the spin projection parameter.
Dynamic Entanglement Evolution of Two-qubit XYZ Spin Chain in Markovian Environment
Yi-Chong, Ren
2015-01-01
We propose a new approach called Ket-Bra Entangled State (KBES) Method for converting master equation into Schr\\"{o}dinger-like equation. With this method, we investigate decoherence process and entanglement dynamics induced by a $2$-qubit spin chain that each qubit coupled with reservoir. The spin chain is an anisotropy $XYZ$ Heisenberg model in the external magnetic field $B$, the corresponding master equation is solved concisely by KBES method; Furthermore, the effects of anisotropy, temperature, external field and initial state on concurrence dynamics is analyzed in detail for the case that initial state is Extended Wenger-Like(EWL) state. Finally we research the coherence and concurrence of the final state (namely the density operator for time tend to infinite)
Porto, Rafael A
2007-01-01
In this comment we explain the discrepancy found between the results in arXiv:0712.1716v1 for the 3PN spin-spin potential and those previously derived in gr-qc/0604099. We point out that to compare one must include sub-leading lower order spin-orbit effects which contribute to the spin-spin potential once one transforms to the PN frame. When these effects are included the results in arXiv:0712.1716v1 do indeed reproduce those found in gr-qc/0604099.
Dynamical modelling and control of a spacecraft-mounted manipulator capturing a spinning satellite
Cyril, Xavier; Jaar, Gilbert J.; Misra, Arun K.
1995-01-01
Issues associated with the modelling and control of a spacecraft-mounted manipulator capturing a spinning satellite are presented. The Lagrangian formulation is used to derive the dynamical equations of the system immediately following the capture. The formulation is carried out by writing Lagrange's equations for the individual bodies, and then assembling them to obtain the constrained dynamical equations of the system. The non-working constraint forces/torques are then eliminated by using the natural orthogonal complement which produces a set of independent dynamical equations. A control algorithm whose objective is to produce a set of feedback-linearized, homogeneous and uncoupled equations is designed and implemented. The initial conditions of the state variables needed to achieve smooth berthing of the satellite are computed, and the dynamics simulation of both the controlled and uncontrolled systems is carried out. The manipulator's structural flexibility is included in the dynamics simulation model.
Dynamical thermal conductivity of the spin Lieb lattice
Yarmohammadi, Mohsen
2016-05-01
In the ferromagnetic insulator with the Dzyaloshinskii-Moriya interaction (DMI), we have theoretically investigated the dynamical thermal conductivity (DTC). In other words, we have investigated the frequency dependence of thermal conductivity, κ, of the Lieb lattice, a face-centered square lattice, subjected to a time dependence temperature gradient. Using linear response theory and Green's function approach, DTC has been obtained in the context of Heisenberg Hamiltonian. At low frequencies, DTC is found to be monotonically increasing with DMI strength (DMIS), temperature and next-nearest-neighbor (NNN) coupling. Also we have found that DTC includes a peak for different values of temperature, DMIS and NNN coupling. Furthermore we study the temperature dependence of thermal conductivity of Lieb lattice for different values of DMIS, NNN coupling and external magnetic filed. We witness a decrease in DTC with temperature due to the quantum effects in the system.
Rapid 3D dynamic arterial spin labeling with a sparse model-based image reconstruction.
Zhao, Li; Fielden, Samuel W; Feng, Xue; Wintermark, Max; Mugler, John P; Meyer, Craig H
2015-11-01
Dynamic arterial spin labeling (ASL) MRI measures the perfusion bolus at multiple observation times and yields accurate estimates of cerebral blood flow in the presence of variations in arterial transit time. ASL has intrinsically low signal-to-noise ratio (SNR) and is sensitive to motion, so that extensive signal averaging is typically required, leading to long scan times for dynamic ASL. The goal of this study was to develop an accelerated dynamic ASL method with improved SNR and robustness to motion using a model-based image reconstruction that exploits the inherent sparsity of dynamic ASL data. The first component of this method is a single-shot 3D turbo spin echo spiral pulse sequence accelerated using a combination of parallel imaging and compressed sensing. This pulse sequence was then incorporated into a dynamic pseudo continuous ASL acquisition acquired at multiple observation times, and the resulting images were jointly reconstructed enforcing a model of potential perfusion time courses. Performance of the technique was verified using a numerical phantom and it was validated on normal volunteers on a 3-Tesla scanner. In simulation, a spatial sparsity constraint improved SNR and reduced estimation errors. Combined with a model-based sparsity constraint, the proposed method further improved SNR, reduced estimation error and suppressed motion artifacts. Experimentally, the proposed method resulted in significant improvements, with scan times as short as 20s per time point. These results suggest that the model-based image reconstruction enables rapid dynamic ASL with improved accuracy and robustness.
Mikati, Abdul Ghani; Tan, Huan; Shenkar, Robert; Li, Luying; Zhang, Lingjiao; Guo, Xiaodong; Shi, Changbin; Liu, Tian; Wang, Yi; Shah, Akash; Edelman, Robert; Christoforidis, Gregory; Awad, Issam
2015-01-01
Background Hyperpermeability and iron deposition are two central pathophysiological phenomena in human cerebral cavernous malformation (CCM) disease. Here we used two novel magnetic resonance imaging (MRI) techniques to establish a relationship between these phenomena. Methods Subjects with CCM disease (4 sporadic and 18 familial) underwent MRI imaging using the Dynamic Contrast Enhanced Quantitative Perfusion (DCEQP) and Quantitative Susceptibility Mapping (QSM) techniques that measure hemodynamic factors of vessel leak and iron deposition respectively, previously demonstrated in CCM disease. Regions of interest encompassing the CCM lesions were analyzed using these techniques Results Susceptibility measured by QSM was positively correlated with permeability of lesions measured using DCEQP (r=0.49, p=<0.0001). The correlation was not affected by factors including familial predisposition, lesion volume, the contrast agent and the use of statin medication. Susceptibility was correlated with lesional blood volume (r=0.4, p=0.0001), but not with lesional blood flow. Conclusion The correlation between QSM and DCEQP suggests that the phenomena of permeability and iron deposition are related in CCM; hence “more leaky lesions” also manifest a more cumulative iron burden. These techniques might be used as biomarkers to monitor the course of this disease and the effect of therapy. PMID:24302484
Lattice dynamics and spin-phonon interactions in multiferroic RMn2O5: Shell model calculations
Litvinchuk, A. P.
2009-08-01
The results of the shell model lattice dynamics calculations of multiferroic RMn2O5 materials (space group Pbam) are reported. Theoretical even-parity eigenmode frequencies are compared with those obtained experimentally in polarized Raman scattering experiments for R=Ho,Dy. Analysis of displacement patterns allows to identify vibrational modes which facilitate spin-phonon coupling by modulating the Mn-Mn exchange interaction and provides explanation of the observed anomalous temperature behavior of phonons.
Microscopic spin model for the dynamics of the return distribution of the Korean stock market index
Yang, Jae-Suk; Chae, Seungbyung; Jung, Woo-Sung; Moon, Hie-Tae
2006-05-01
In this paper, we studied the dynamics of the log-return distribution of the Korean Composition Stock Price Index (KOSPI) from 1992 to 2004. Based on the microscopic spin model, we found that while the index during the late 1990s showed a power-law distribution, the distribution in the early 2000s was exponential. This change in distribution shape was caused by the duration and velocity, among other parameters, of the information that flowed into the market.
Magnetic soft x-ray microscopy-imaging fast spin dynamics inmagnetic nanostructures
Energy Technology Data Exchange (ETDEWEB)
Fischer, Peter; Kim, Dong-Hyun; Mesler, Brooke L.; Chao, Weilun; Sakdinawat, Anne E.; Anderson, Erik H.
2007-06-01
Magnetic soft X-ray microscopy combines 15nm spatial resolution with 70ps time resolution and elemental sensitivity. Fresnel zone plates are used as X-ray optics and X-ray magnetic circular dichroism serves as magnetic contrast mechanism. Thus scientifically interesting and technologically relevant low dimensional nanomagnetic systems can be imaged at fundamental length and ultrafast time scales in a unique way. Studies include magnetization reversal in magnetic multilayers, nanopatterned systems, vortex dynamics in nanoelements and spin current induced phenomena.
Spin blockade and coherent dynamics of high-spin states in a three-electron double quantum dot
Chen, Bao-Bao; Wang, Bao-Chuan; Cao, Gang; Li, Hai-Ou; Xiao, Ming; Guo, Guang-Can; Jiang, Hong-Wen; Hu, Xuedong; Guo, Guo-Ping
2017-01-01
Asymmetry in a three-electron double quantum dot (DQD) allows spin blockade, when spin-3/2 (quadruplet) states and spin-1/2 (doublet) states have different charge configurations. We have observed this DQD spin blockade near the (1,2)-(2,1) charge transition using a pulsed-gate technique and a charge sensor. We, then, use this spin blockade to detect Landau-Zener-Stückelberg interference and coherent oscillations between the spin quadruplet and doublet states. Such studies add to our understandings of coherence and control properties of three-spin states in a double dot, which, in turn, would benefit explorations into various qubit encoding schemes in semiconductor nanostructures.
Nonequilibrium Dynamical Phase Transition of a Three-Dimensional Kinetic Heisenberg Spin System
Institute of Scientific and Technical Information of China (English)
邵元智; 林光明; 蓝图; J.K.L Lai; C.H.Shek
2002-01-01
We systematically investigate the dynamical response of a three-dimensional kinetic isotropic Heisenberg spin system (ISS) to an external driving field by Monte Carlo numerical simulation. The dynamical response of the isotropic HSS differs obviously from those of the anisotropic Ising spin system in which no realstable ordered state and relevant dynamical phase transition were observed in the kinetic ISS. There is a threshold time after which the magnetization m(t) in the ISS driven by a symmetrical external field always tends asymptotically to a disorder state regardless of the initial state of the system. The threshold time depends on the reduced temperature T/TC of the investigated spin system, amplitude H0 and frequency of the external field, i.e. γ = C. ωα . H0-β. (T/TC)-γ.C is a constant equal to 0.0302 for a three-dimensional lattice and exponents а = 1.18 ± 0.01, β = 1.81 ± 0.01and γ = 1.68 ± 0.01.
Spin Dynamics of Kelvin's Pebbles, Jellett's Eggs, and Shiva's Lingam Stones
Brecher, Kenneth
2015-04-01
Study of the problem of the rise of the center of mass (COM) of spinning objects is said to have begun in the late nineteenth century. These early mathematical treatments aimed to explain the motion of the newly invented and patented ``tippe top.'' This semi-spheroidal top will invert when spun on a smooth surface while raising its COM. Because of the importance of friction in their dynamics, such non-holonomic systems are not readily amenable to analytic treatment, or of intuitive understanding. In notes written in 1844 - before the invention of the tippe top - Lord Kelvin (William Thomson) discussed the problem of the rising COM of spinning objects. He experimented with both oblate and prolate ellipsoidal pebbles, but did not publish a complete theoretical treatment of the problem. J. H. Jellett, in his 1872 book ``Theory of Friction,'' provided a partial account of the related problem of the rise of the COM for an egg-shaped (ovoid) object, making use of a new (adiabatic) invariant of the motion that he devised. Naturally occurring prolate ellipsoidal ``Lingam stones'' from the Narmada River in India exhibit similar counter-intuitive dynamical behavior. When spun around its minor axis in a horizontal plane, a Lingam stone will stand erect and spin around its major axis in a vertical position. This presentation will explore the history and some of the experimental facts and theoretical ideas about the rotational dynamics of such physical objects.
Oxygen-17 NMR in solids by dynamic-angle spinning and double rotation
Chmelka, B. F.; Mueller, K. T.; Pines, A.; Stebbins, J.; Wu, Y.; Zwanziger, J. W.
1989-05-01
IT is widely lamented that despite its unqualified success with spin-1/2 nuclei such as 13C, 29Si and31P, the popular NMR technique of magic-angle spinning (MAS) has experienced a somewhat restricted applicability among quadrupolar nuclei such as 17O, 23Na and 27A1 (refs 1-3). The resolution in the central (1/2 lrarr-1/2) transition of these non-integer quadrupolar spins under MAS is thought to be limited primarily by second-order quadrupolar broadening. Such effects of second-order spatial anisotropy cannot be eliminated by rotation about a fixed axis or by multiple-pulse techniques4,5. More general mechanisms of sample reorientation (refs 6-8 and A. Samoson and A. Pines, manuscript in preparation) can, however, make high-resolution NMR of quadrupolar nuclei feasible. MAS is implemented by spinning a sample about a single axis so that second-rank spherical harmonics (which give rise to first-order broadening through anisotropy of electrical and magnetic interactions) are averaged away. But dynamic-angle-spinning (DAS) and double-rotation (DOR) NMR involve spinning around two axes, averaging away both the second- and fourth-rank spherical harmonics, which are responsible for second-order broadening. Here we present the application of these new techniques to 17O in two minerals, cristobalite (SiO2) and diopside (CaMgSi2O6). This work goes beyond previous results on 23Na (ref. 8) by showing the first experimental results using DAS and by demonstrating the application of DOR to the resolution of distinct oxygen sites in an important class of oxide materials.
Energy Technology Data Exchange (ETDEWEB)
Renshaw, P.F.; Levin, J.M.; Kaufman, M.J.; Ross, M.H. [Brain Imaging Center, McLean Hospital, 115 Mill Street, Belmont, MA 02178 (United States); Lewis, R.F.; Harris, G.J. [Neuroimaging Research Laboratory, New England Medical Center, Boston, Massachusetts (United States)
1997-12-31
Dynamic susceptibility contrast magnetic resonance imaging (DSC MRI) provides a noninvasive means to create high resolution maps of the regional distribution of cerebral blood volume (CBV). Most DSC MRI studies conducted to date have focused on the evaluation of patients with cerebral neoplasms, ischemia or infarction, and epilepsy. However, preliminary work suggests that DSC MRI may also provide clinically important information for the evaluation of patients with neuropsychiatric disorders, especially dementia and schizophrenia. Additionally, with appropriate modification, DSC MRI may be used to reliably evaluate the effects of pharmacological challenges on cerebral hemodynamics. As pharmacotherapy is an important component in the treatment of a range of psychiatric disorders, the dynamic assessment of changes in cerebral perfusion associated with drug administration may ultimately lead to the development of ``brain function tests`` for a wide range of disorders. (orig.) With 4 figs., 50 refs.
Cumulative quantum work-deficit versus entanglement in the dynamics of an infinite spin chain
Energy Technology Data Exchange (ETDEWEB)
Dhar, Himadri Shekhar [School of Physical Sciences, Jawaharlal Nehru University, New Delhi 110067 (India); Ghosh, Rupamanjari [School of Physical Sciences, Jawaharlal Nehru University, New Delhi 110067 (India); School of Natural Sciences, Shiv Nadar University, Gautam Budh Nagar, UP 203207 (India); Sen, Aditi [Harish-Chandra Research Institute, Chhatnag Road, Jhunsi, Allahabad 211019 (India); Sen, Ujjwal, E-mail: ujjwal@hri.res.in [Harish-Chandra Research Institute, Chhatnag Road, Jhunsi, Allahabad 211019 (India)
2014-03-01
We find that the dynamical phase transition (DPT) in nearest-neighbor bipartite entanglement of time-evolved states of the anisotropic infinite quantum XY spin chain, in a transverse time-dependent magnetic field, can be quantitatively characterized by the dynamics of an information-theoretic quantum correlation measure, namely, quantum work-deficit (QWD). We show that only those nonequilibrium states exhibit entanglement resurrection after death, on changing the field parameter during the DPT, for which the cumulative bipartite QWD is above a threshold. The results point to an interesting inter-relation between two quantum correlation measures that are conceptualized from different perspectives.
New Dynamic Spin Rig Capabilities Used to Determine Rotating Blade Dynamics
Provenza, Andrew J.
2004-01-01
The Dynamic Spin Rig Facility at the NASA Glenn Research Center is used to determine the structural response of rotating engine components without the effects of aerodynamic loading. Recently, this rig's capabilities were enhanced through the replacement of grease-lubricated ball bearings with magnetic bearings. Magnetic bearings offer a number of advantages--the most important here being that they not only fully support the rotor system, but excite it as well. Three magnetic bearings support the rotor and provide five axes of controlled motion: an x- and y-axis translation at each of two radial bearings and a z-axis translation in the vertical or axial direction. Sinusoidal excitation (most commonly used) can be imparted on the rotor through the radial magnetic bearings in either a fixed or rotating frame of reference. This excitation is added directly to the magnetic bearing control output. Since the rotor is fully levitated, large translations and rotations of the rotor system can be achieved. Some of the capabilities of this excitation system were determined and reported. The accelerations obtained at the tip of a titanium flat plate test article versus the swept sine excitation sent to both radial bearings in phase and perpendicular to the plane containing the two blades are shown. Recent tests required the excitation of fundamental bending and torsional blade resonances at rotor speeds up to 10,000 rpm. Successful fixed synchronous rotation of the excitation signal provided the best detectable blade resonant vibrations at excitation frequencies up to 1100 Hz for the particular blades of interest. A noncontacting laser measurement system was used to collect blade-tip motions. From these data, the amplitude and frequency of the motion could be determined as well as the blade damping properties. Damping could be determined using two methods: (1) free decay and (2) curve fitting the vibration amplitude as a function of frequency in and around the resonance of
Can cerebrovascular reactivity be assessed by dynamic susceptibility contrast-enhanced MRI?
Energy Technology Data Exchange (ETDEWEB)
Berthezene, Y.; Meyer, R.; Froment, J.C. [Department of Radiology, Creatis UMR CNRS 5515, Neurological Hospital, Lyon (France); Nighoghossian, N.; Trouillas, P. [Neurology, Cerebrovascular Disease and Ataxia Research Center, Neurological Hospital, Lyon (France); Damien, J.; Cinotti, L. [Department of Nuclear Medicine, Neurological Hospital, Lyon (France); Adeleine, P. [Medical Informatics Laboratory, UFR Alexis Carrel, Lyon (France)
1998-01-01
s The acetazolamide (ACZ) test is performed to evaluate the decrease in cerebral perfusion pressure (CPP) by investigation of vasomotor reactivity (VMR). Our aim was to study cerebral blood flow and blood volume changes induced by the ACZ test in healthy control subjects using dynamic susceptibility contrast-enhanced gradient-echo MRI (DSC-MRI). A FLASH sequence was used to produce susceptibility-weighted images during an intravenous injection of 0.1 mmol/kg gadopentetate dimeglumine (Gd-DTPA). After the first dynamic study, 1 g acetazolamide was given intravenously and 10 min later a second bolus of Gd-DTPA was injected. Using the indicator-dilution theory, relative cerebral blood volume and relative cerebral blood flow were estimated. In healthy subjects the ACZ test induced a significant increase in relative blood volume (from 80.5 {+-} 10.7 to 113.4 {+-} 11.9) and relative blood flow (from 5.73 {+-} 0.96 to 7.5 {+-} 0.97), symmetrically in the cerebral hemispheres. This approach might be promising in the understanding of cerebral haemodynamics in patients with vascular disorders. (orig.) With 1 fig., 3 tabs., 24 refs.
Fong, C. F.; Ota, Y.; Harbord, E.; Iwamoto, S.; Arakawa, Y.
2016-03-01
Repeated injection of spin-polarized carriers in a quantum dot (QD) leads to the polarization of nuclear spins, a process known as dynamic nuclear spin polarization (DNP). Here, we report the observation of p-shell carrier assisted DNP in single QDs at zero external magnetic field. The nuclear field—measured by using the Overhauser shift of the singly charged exciton state of the QDs—continues to increase, even after the carrier population in the s-shell saturates. This is also accompanied by an abrupt increase in nuclear spin buildup time as p-shell emission overtakes that of the s shell. We attribute the observation to p-shell electrons strongly altering the nuclear spin dynamics in the QD, supported by numerical simulation results based on a rate equation model of coupling between electron and nuclear spin system. Dynamic nuclear spin polarization with p-shell carriers could open up avenues for further control to increase the degree of nuclear spin polarization in QDs.
Alvarez, Gonzalo A
2007-01-01
The control of open quantum systems has a fundamental relevance for fields ranging from quantum information processing to nanotechnology. Typically, the system whose coherent dynamics one wants to manipulate, interacts with an environment that smoothly degrades its quantum dynamics. Thus, a precise understanding of the inner mechanisms of this process, called "decoherence", is critical to develop strategies to control the quantum dynamics. In this thesis we solved the generalized Liouville-von Neumann quantum master equation to obtain the dynamics of many-spin systems interacting with a spin bath. We also solve the spin dynamics within the Keldysh formalism. Both methods lead to identical solutions and together gave us the possibility to obtain numerous physical predictions that contrast well with Nuclear Magnetic Resonance experiments. We applied these tools for molecular characterizations, development of new numerical methodologies and the control of quantum dynamics in experimental implementations. But, mo...
Molecular-scale dynamics of light-induced spin cross-over in a two-dimensional layer
Bairagi, Kaushik; Iasco, Olga; Bellec, Amandine; Kartsev, Alexey; Li, Dongzhe; Lagoute, Jérôme; Chacon, Cyril; Girard, Yann; Rousset, Sylvie; Miserque, Frédéric; Dappe, Yannick J; Smogunov, Alexander; Barreteau, Cyrille; Boillot, Marie-Laure; Mallah, Talal; Repain, Vincent
2016-01-01
Spin cross-over molecules show the unique ability to switch between two spin states when submitted to external stimuli such as temperature, light or voltage. If controlled at the molecular scale, such switches would be of great interest for the development of genuine molecular devices in spintronics, sensing and for nanomechanics. Unfortunately, up to now, little is known on the behaviour of spin cross-over molecules organized in two dimensions and their ability to show cooperative transformation. Here we demonstrate that a combination of scanning tunnelling microscopy measurements and ab initio calculations allows discriminating unambiguously between both states by local vibrational spectroscopy. We also show that a single layer of spin cross-over molecules in contact with a metallic surface displays light-induced collective processes between two ordered mixed spin-state phases with two distinct timescale dynamics. These results open a way to molecular scale control of two-dimensional spin cross-over layers. PMID:27425776
Improving the coherence properties of solid-state spin ensembles via optimized dynamical decoupling
Farfurnik, D.; Jarmola, A.; Pham, L. M.; Wang, Z. H.; Dobrovitski, V. V.; Walsworth, R. L.; Budker, D.; Bar-Gill, N.
2016-04-01
In this work, we optimize a dynamical decoupling (DD) protocol to improve the spin coherence properties of a dense ensemble of nitrogen-vacancy (NV) centers in diamond. Using liquid nitrogen-based cooling and DD microwave pulses, we increase the transverse coherence time T2 from ˜ 0.7 ms up to ˜ 30 ms. We extend previous work of single-axis (Carr-Purcell-Meiboom-Gill) DD towards the preservation of arbitrary spin states. After performing a detailed analysis of pulse and detuning errors, we compare the performance of various DD protocols. We identify that the concatenated XY8 pulse sequences serves as the optimal control scheme for preserving an arbitrary spin state. Finally, we use the concatenated sequences to demonstrate an immediate improvement of the AC magnetic sensitivity up to a factor of two at 250 kHz. For future work, similar protocols may be used to increase coherence times up to NV-NV interaction time scales, a major step toward the creation of quantum collective NV spin states.
Hole dynamics and spin currents after ionization in strong circularly polarized laser fields
Barth, Ingo
2014-01-01
We apply the time-dependent analytical R-matrix theory to develop a movie of hole motion in a Kr atom upon ionization by strong circularly polarized field. We find rich hole dynamics, ranging from rotation to swinging motion. The motion of the hole depends on the final energy and the spin of the photoelectron and can be controlled by the laser frequency and intensity. Crucially, hole rotation is a purely non-adiabatic effect, completely missing in the framework of quasistatic (adiabatic) tunneling theories. We explore the possibility to use hole rotation as a clock for measuring ionization time. Analysing the relationship between the relative phases in different ionization channels we show that in the case of short-range electron-core interaction the hole is always initially aligned along the instantaneous direction of the laser field, signifying zero delays in ionization. Finally, we show that strong-field ionization in circular fields creates spin currents (i.e. different flow of spin-up and spin-down densi...
Solid effect in the electron spin dressed state: A new approach for dynamic nuclear polarization
Weis, V.; Bennati, M.; Rosay, M.; Griffin, R. G.
2000-10-01
We describe a new type of solid effect for dynamic nuclear polarization (DNP) that is based on simultaneous, near resonant microwave (mw) and radio frequency (rf) irradiation of a coupled electron nuclear spin system. The interaction of the electron spin with the mw field is treated as an electron spin dressed state. In contrast to the customary laboratory frame solid effect, it is possible to obtain nuclear polarization with the dressed state solid effect (DSSE) even in the absence of nonsecular hyperfine coupling. Efficient, selective excitation of dressed state transitions generates nuclear polarization in the nuclear laboratory frame on a time scale of tens of μs, depending on the strength of the electron-nuclear coupling, the mw and rf offset and field strength. The experiment employs both pulsed mw and rf irradiation at a repetition rate comparable to T1e-1, where T1e is the electronic spin lattice relaxation time. The DSSE is demonstrated on a perdeuterated BDPA radical in a protonated matrix of polystyrene.
Characterization of spin dynamics in stripe-ordered La2-xSrxNiO4
Woo, H.; Tranquada, J. M.; Boothroyd, A. T.; Nakajima, K.; Perring, T. G.; Frost, C.; Freeman, P. G.; Prabhakaran, D.; Yamada, K.
2004-03-01
Inelastic neutron scattering experiments at a spallation source have enabled us to measure the full momentum- and energy- dependent spectra of magnetic fluctuations in the charge- and spin-stripe ordered systems La_2-xSr_xNiO4 ( x=1/3 and x=0.275). Peaks in the dynamic magnetic response at incommensurate wavevectors and over a wide frequency range are commonly observed in the high-Tc superconductors YBa_2Cu_3O_6+x and La_2-xA_xCuO_4(A=Sr,Ba) , as well as in the static charge- and spin-striped system nickelates La_2-xSr_xNiO_4. High energy transfer up to 90meV with broad reciprocal spaces was observed. In addition to intrastripe and interstripe exchange interactions between neighboring Ni spins [1], exchange interactions between diagonal Ni spins (not through oxygen) are also considered. We will present a detailed measurement and analysis in the NiO2 plane. We acknowledge U.S.-DOE for financial support: contract # DE-AC02-98CH1088. [1] Boothroyd et al. Phys. Rev. B 67, 100407(R) (2003).
Nonequilibrium dynamics of spin-boson models from phase-space methods
Piñeiro Orioli, Asier; Safavi-Naini, Arghavan; Wall, Michael L.; Rey, Ana Maria
2017-09-01
An accurate description of the nonequilibrium dynamics of systems with coupled spin and bosonic degrees of freedom remains theoretically challenging, especially for large system sizes and in higher than one dimension. Phase-space methods such as the truncated Wigner approximation (TWA) have the advantage of being easily scalable and applicable to arbitrary dimensions. In this work we adapt the TWA to generic spin-boson models by making use of recently developed algorithms for discrete phase spaces [J. Schachenmayer, A. Pikovski, and A. M. Rey, Phys. Rev. X 5, 011022 (2015), 10.1103/PhysRevX.5.011022]. Furthermore we go beyond the standard TWA approximation by applying a scheme based on the Bogoliubov-Born-Green-Kirkwood-Yvon (BBGKY) hierarchy of equations to our coupled spin-boson model. This allows us, in principle, to study how systematically adding higher-order corrections improves the convergence of the method. To test various levels of approximation we study an exactly solvable spin-boson model, which is particularly relevant for trapped-ion arrays. Using TWA and its BBGKY extension we accurately reproduce the time evolution of a number of one- and two-point correlation functions in several dimensions and for an arbitrary number of bosonic modes.
Minority-spin dynamics in the nonhomogeneous Ising model: Diverging time scales and exponents
Mullick, Pratik; Sen, Parongama
2016-05-01
We investigate the dynamical behavior of the Ising model under a zero-temperature quench with the initial fraction of up spins 0 ≤x ≤1 . In one dimension, the known results for persistence probability are verified; it shows algebraic decay for both up and down spins asymptotically with different exponents. It is found that the conventional finite-size scaling is valid here. In two dimensions, however, the persistence probabilities are no longer algebraic; in particular for x ≤0.5 , persistence for the up (minority) spins shows the behavior Pmin(t ) ˜t-γexp[-(t/τ ) δ] with time t , while for the down (majority) spins, Pmaj(t ) approaches a finite value. We find that the timescale τ diverges as (xc-x ) -λ, where xc=0.5 and λ ≃2.31 . The exponent γ varies as θ2 d+c0(xc-x ) β where θ2 d≃0.215 is very close to the persistence exponent in two dimensions; β ≃1 . The results in two dimensions can be understood qualitatively by studying the exit probability, which for different system size is found to have the form E (x ) =f [(x/-xc xc) L1 /ν] , with ν ≈1.47 . This result suggests that τ ˜Lz ˜ , where z ˜=λ/ν =1.57 ±0.11 is an exponent not explored earlier.
Proskuryakov, Y. Y.; Kvon, Z. D.; Savchenko, A. K.
2003-01-01
In this work we have studied the parallel magnetoresistance of a 2DEG near a vicinal silicon surface. An unusual, linear magnetoconductance is observed in the fields up to $B = 15$ T, which we explain by the effect of spin olarization on impurity scattering. This linear magnetoresistance shows strong anomalies near the boundaries of the minigap in the electron spectrum of the vicinal system.
Brahms, N
2010-01-01
The dynamics of a large quantum spin coupled parametrically to an optical resonator is treated in analogy with the motion of a cantilever in cavity optomechanics. New spin optodynamic phenonmena are predicted, such as cavity-spin bistability, optodynamic spin-precession frequency shifts, coherent amplification and damping of spin, and the spin optodynamic squeezing of light.
Kinematical and dynamical aspects of higher-spin bound-state equations in holographic QCD
Energy Technology Data Exchange (ETDEWEB)
de Téramond, Guy F.; Dosch, Hans Günter; Brodsky, Stanley J.
2013-04-01
In this paper we derive holographic wave equations for hadrons with arbitrary spin starting from an effective action in a higher-dimensional space asymptotic to anti–de Sitter (AdS) space. Our procedure takes advantage of the local tangent frame, and it applies to all spins, including half-integer spins. An essential element is the mapping of the higher-dimensional equations of motion to the light-front Hamiltonian, thus allowing a clear distinction between the kinematical and dynamical aspects of the holographic approach to hadron physics. Accordingly, the nontrivial geometry of pure AdS space encodes the kinematics, and the additional deformations of AdS space encode the dynamics, including confinement. It thus becomes possible to identify the features of holographic QCD, which are independent of the specific mechanisms of conformal symmetry breaking. In particular, we account for some aspects of the striking similarities and differences observed in the systematics of the meson and baryon spectra.
Spin dynamics and magnetic correlation length in two-dimensional quantum heisenberg antiferromagnets
Carretta; Ciabattoni; Cuccoli; Mognaschi; Rigamonti; Tognetti; Verrucchi
2000-01-10
The correlated spin dynamics and temperature dependence of the correlation length xi(T) in two-dimensional quantum (S = 1/2) Heisenberg antiferromagnets (2DQHAF) on a square lattice are discussed in light of experimental results of proton spin lattice relaxation in copper formiate tetradeuterate. In this compound the exchange constant is much smaller than the one in recently studied 2DQHAF, such as La2CuO4 and Sr2CuO2Cl2. Thus the spin dynamics can be probed in detail over a wider temperature range. The NMR relaxation rates turn out to be in excellent agreement with a theoretical mode-coupling calculation. The deduced temperature behavior of xi(T) is in agreement with high-temperature expansions, quantum Monte Carlo simulations, and the pure quantum self-consistent harmonic approximation. Contrary to the predictions of the theories based on the nonlinear sigma model, no evidence of crossover between different quantum regimes is observed.
PRECESSION: Python toolbox for dynamics of spinning black-hole binaries
Gerosa, Davide; Kesden, Michael
2016-11-01
PRECESSION is a comprehensive toolbox for exploring the dynamics of precessing black-hole binaries in the post-Newtonian regime. It allows study of the evolution of the black-hole spins along their precession cycles, performs gravitational-wave-driven binary inspirals using both orbit-averaged and precession-averaged integrations, and predicts the properties of the merger remnant through fitting formulas obtained from numerical-relativity simulations. PRECESSION can add the black-hole spin dynamics to larger-scale numerical studies such as gravitational-wave parameter estimation codes, population synthesis models to predict gravitational-wave event rates, galaxy merger trees and cosmological simulations of structure formation, and provides fast and reliable integration methods to propagate statistical samples of black-hole binaries from/to large separations where they form to/from small separations where they become detectable, thus linking gravitational-wave observations of spinning black-hole binaries to their astrophysical formation history. The code is also useful for computing initial parameters for numerical-relativity simulations targeting specific precessing systems.
Dynamics of Bound Monopoles in Artificial Spin Ice: How to Store Energy in Dirac Strings.
Vedmedenko, E Y
2016-02-19
Dirac strings in spin ices are lines of reversed dipoles joining two quasiparticle excitations. These excitations behave as unbound emergent monopoles if the tension of Dirac strings vanishes. In this Letter, analytical and numerical analysis are used to study the dynamics of two-dimensional dipolar spin ices, artificially created analogs of bulk spin ice, in the regime of bound monopoles. It is shown that, in this regime, strings, rather than monopoles, are effective degrees of freedom explaining the finite-width band of Pauling states. A measurable prediction of path-time dependence of endpoints of a stretched and, then, released Dirac string is made and verified via simulations. It is shown that string dynamics is defined by the characteristic tension-to-mass ratio, which is determined by the fine structure constant and lattice dependent parameter. It is proposed to use string tension to achieve spontaneous magnetic currents. A concept of an energy storing device on the basis of this principle is proposed and illustrated by an experimental demonstration. A scheme of independent measurement at the nanoscale is proposed.
Tracking protein dynamics with photoconvertible Dendra2 on spinning disk confocal systems.
Woods, Elena; Courtney, Jane; Scholz, Dimitri; Hall, William W; Gautier, Virginie W
2014-12-01
Understanding the dynamic properties of cellular proteins in live cells and in real time is essential to delineate their function. In this context, we introduce the Fluorescence Recovery After Photobleaching-Photoactivation unit (Andor) combined with the Nikon Eclipse Ti E Spinning Disk (Andor) confocal microscope as an advantageous and robust platform to exploit the properties of the Dendra2 photoconvertible fluorescent protein (Evrogen) and analyse protein subcellular trafficking in living cells. A major advantage of the spinning disk confocal is the rapid acquisition speed, enabling high temporal resolution of cellular processes. Furthermore, photoconversion and imaging are less invasive on the spinning disk confocal as the cell exposition to illumination power is reduced, thereby minimizing photobleaching and increasing cell viability. We have tested this commercially available platform using experimental settings adapted to track the migration of fast trafficking proteins such as UBC9, Fibrillarin and have successfully characterized their differential motion between subnuclear structures. We describe here step-by-step procedures, with emphasis on cellular imaging parameters, to successfully perform the dynamic imaging and photoconversion of Dendra2-fused proteins at high spatial and temporal resolutions necessary to characterize the trafficking pathways of proteins. © 2014 The Authors. Journal of Microscopy published by John Wiley & Sons, Ltd on behalf of Royal Microscopical Society.
Analytical approach to the dynamics of facilitated spin models on random networks
Fennell, Peter G.; Gleeson, James P.; Cellai, Davide
2014-09-01
Facilitated spin models were introduced some decades ago to mimic systems characterized by a glass transition. Recent developments have shown that a class of facilitated spin models is also able to reproduce characteristic signatures of the structural relaxation properties of glass-forming liquids. While the equilibrium phase diagram of these models can be calculated analytically, the dynamics are usually investigated numerically. Here we propose a network-based approach, called approximate master equation (AME), to the dynamics of the Fredrickson-Andersen model. The approach correctly predicts the critical temperature at which the glass transition occurs. We also find excellent agreement between the theory and the numerical simulations for the transient regime, except in close proximity of the liquid-glass transition. Finally, we analytically characterize the critical clusters of the model and show that the departures between our AME approach and the Monte Carlo can be related to the large interface between blocked and unblocked spins at temperatures close to the glass transition.
Nanocluster building blocks of artificial square spin ice: Stray-field studies of thermal dynamics
Energy Technology Data Exchange (ETDEWEB)
Pohlit, Merlin, E-mail: pohlit@physik.uni-frankfurt.de; Porrati, Fabrizio; Huth, Michael; Müller, Jens [Institute of Physics, Goethe-University Frankfurt, Frankfurt/Main (Germany); Ohno, Yuzo; Ohno, Hideo [Laboratory for Nanoelectronics and Spintronics, Research Institute of Electrical Communication, Tohoku University, Sendai (Japan)
2015-05-07
We present measurements of the thermal dynamics of a Co-based single building block of an artificial square spin ice fabricated by focused electron-beam-induced deposition. We employ micro-Hall magnetometry, an ultra-sensitive tool to study the stray field emanating from magnetic nanostructures, as a new technique to access the dynamical properties during the magnetization reversal of the spin-ice nanocluster. The obtained hysteresis loop exhibits distinct steps, displaying a reduction of their “coercive field” with increasing temperature. Therefore, thermally unstable states could be repetitively prepared by relatively simple temperature and field protocols allowing one to investigate the statistics of their switching behavior within experimentally accessible timescales. For a selected switching event, we find a strong reduction of the so-prepared states' “survival time” with increasing temperature and magnetic field. Besides the possibility to control the lifetime of selected switching events at will, we find evidence for a more complex behavior caused by the special spin ice arrangement of the macrospins, i.e., that the magnetic reversal statistically follows distinct “paths” most likely driven by thermal perturbation.
Energy Technology Data Exchange (ETDEWEB)
Kumar, Punith V., E-mail: drvldayal@gmail.com; Manju, M. R., E-mail: drvldayal@gmail.com; Dayal, Vijaylakshmi, E-mail: drvldayal@gmail.com [Department of Physics, Maharaja Institute of Technology, Mysore-571438, Karnataka (India)
2014-04-24
We present a comprehensive study on origin of Spin Glass (SG) property in polycrystalline La{sub 0.5}Bi{sub 0.5}MnO{sub 3} perovskite oxide using linear and higher order ac susceptibility (χ) measurements. The third order harmonic susceptibility (χ{sub 3}) vs. temperature (K) with varying magnetic fields from 0.95 to 9.45 Oe and the divergence in their χ{sub 3} (max) allows us to infer the SG behavior occurring in the sample possibly due to co-operative freezing of the spins.
Spin dynamics of the Kondo insulator CeNiSn approaching the metallic phase
DEFF Research Database (Denmark)
Schröder, A.; Aeppli, G.; Mason, T.E.
1997-01-01
The spin dynamics of Kondo insulators has been studied by high-resolution magnetic neutron spectroscopy at a triple-axes spectrometer on CeNi1-xCuxSn single crystals using a vertical 9 T magnet. While upon doping (x = 0.13) the spin gap of the Kondo insulator CeNiSn collapses at the transition...... to an antiferromagnetic ordered metallic Kondo compound, no such instability is observed in CeNiSn in magnetic fields up to 9 T. Both the sharp magnetic excitations (at 2 and 4 meV) appear significantly broader for energy and momentum transfer at high fields, while the ground-state correlations (probed by chi'(0)) remain...
A Comparison Study of Magnetic Bearing Controllers for a Fully Suspended Dynamic Spin Rig
Choi, Benjamin; Johnson, Dexter; Morrison, Carlos; Mehmed, Oral; Huff, Dennis (Technical Monitor)
2002-01-01
NASA Glenn Research Center (GRC) has developed a fully suspended magnetic bearing system for the Dynamic Spin Rig (DSR) that is used to perform vibration tests of turbomachinery blades and components under spinning conditions in a vacuum. Two heteropolar radial magnetic bearings and a thrust bearing and the associated control system were integrated into the DSR to provide noncontact magnetic suspension and mechanical excitation of the 35 lb vertical rotor with blades to induce turbomachinery blade vibration. A simple proportional-integral-derivative (PID) controller with a special feature for multidirectional radial excitation worked very well to both support and shake the shaft with blades. However, more advanced controllers were developed and successfully tested to determine the optimal controller in terms of sensor and processing noise reduction, smaller rotor orbits, and energy savings for the system. The test results of a variety of controllers we demonstrated up to the rig's maximum allowable speed of 10,000 rpm are shown.
Attitude Dynamics of a Spinning Rocket with Internal Fluid Whirling Motion
Directory of Open Access Journals (Sweden)
Marius Ionut MARMUREANU
2014-06-01
Full Text Available This paper evaluates the impact that helical motion of fluid products of combustion within the combustion chamber of a rocket can have on the attitude dynamics of rocket systems. By developing the study presented by Sookgaew (2004, we determined the configuration of the Coriolis moment components, which catch the impact of the combustion product’s whirling motion, for the radial and centripetal propellant burn pattern specific to S-5M and S-5K solid rocket motors. We continue the investigation of the effects of internal whirling motion of fluid products of combustion on the attitude behavior of variable mass systems of the rocket type by examining the spin motion and transverse attitude motion of such systems. The results obtained show that internal fluid whirling motion can cause appreciable deviations in spin rate predictions, and also affects the frequencies of the transverse angular velocity components.
Schüler, M.; Pavlyukh, Y.; Berakdar, J.
2012-04-01
Inelastic scanning tunneling microscopy (STM) has recently been shown (Loth et al 2010 Science 329 1628) to be extendable to access the nanosecond, spin-resolved dynamics of magnetic adatoms and molecules. Here we analyze this novel tool theoretically by considering the time-resolved spin dynamics of a single adsorbed Fe atom excited by a tunneling current pulse from a spin-polarized STM tip. The adatom spin configuration can be controlled and probed by applying voltage pulses between the substrate and the spin-polarized STM tip. We demonstrate how, in a pump-probe manner, the relaxation dynamics of the sample spin is manifested in the spin-dependent tunneling current. Our model calculations are based on the scattering theory in a wave-packet formulation. The scheme is non-perturbative and, hence, is valid for all voltages. The numerical results for the tunneling probability and the conductance are contrasted with the predictions of simple analytical models and compared with experiments.
Mihailescu, M; Endo, H; Allgaier, J; Gompper, G; Stellbrink, J; Richter, D; Jakobs, B; Sottmann, T; Faragó, B
2002-01-01
Using neutron spin-echo (NSE) spectroscopy in combination with dynamic light scattering (DLS), we performed an extensive investigation of the bicontinuous phase in ternary water-surfactant-oil microemulsions, with extension to lamellar and droplet phases. The dynamical behavior of surfactant monolayers of decyl-polyglycol-ether (C sub 1 sub 0 E sub 4) molecules, or mixtures of surfactant with long amphiphilic block-copolymers of type poly-ethylene propylene/poly-ethylene oxide (PEP-PEO) was studied, under comparable conditions. The investigation techniques provide access to different length scales relative to the characteristic periodicity length of the microemulsion structure. Information on the elastic bending modulus is obtained from the local scale dynamics in view of existing theoretical descriptions and is found to be in accordance with small angle neutron scattering (SANS) studies. Evidence for the modified elastic properties and additional interaction of the amphiphilic layers due to the polymer is mo...
Teich, Lisa; Schröder, Christian
2015-11-13
The development of magnetoresistive sensors based on magnetic nanoparticles which are immersed in conductive gel matrices requires detailed information about the corresponding magnetoresistive properties in order to obtain optimal sensor sensitivities. Here, crucial parameters are the particle concentration, the viscosity of the gel matrix and the particle structure. Experimentally, it is not possible to obtain detailed information about the magnetic microstructure, i.e., orientations of the magnetic moments of the particles that define the magnetoresistive properties, however, by using numerical simulations one can study the magnetic microstructure theoretically, although this requires performing classical spin dynamics and molecular dynamics simulations simultaneously. Here, we present such an approach which allows us to calculate the orientation and the trajectory of every single magnetic nanoparticle. This enables us to study not only the static magnetic microstructure, but also the dynamics of the structuring process in the gel matrix itself. With our hybrid approach, arbitrary sensor configurations can be investigated and their magnetoresistive properties can be optimized.
Low-Energy Charge and Spin Dynamics in Quantum Confined Systems
Rice, William D.
Condensed matter systems exhibit a variety of dynamical phenomena at low energy scales, from gigahertz (GHz) to terahertz (THz) frequencies in particular, arising from complex interplay between charge, spin, and lattice. A large number of collective and elementary excitations in solids occur in this frequency range, which are further modified and enriched by scattering, interactions, and disorder. Recent advancements in spectroscopic methods for probing low-energy dynamics allow us to investigate novel aspects of charge and spin dynamics in solids. In this dissertation work, we used direct current (DC) conductivity, GHz, THz, and mid-infrared (MIR) techniques to provide significant new insights into interaction and disorder effects in low-dimensional systems. Specifically, we have studied temperature-dependent magnetoresistance (MR) and electron spin resonance (ESR) in single-wall carbon nanotubes (SWCNTs), intra-exciton scattering in InGaAs quantum wells, and high-field MIR-induced band gaps in graphene. Temperature-dependent resistance and MR were measured in an ensemble of SWCNTs from 0.3 to 350 K. The resistance temperature behavior followed a 3D variable range hopping (VRH) behavior from 0.3 to ˜100 K. A positive MR was observed at temperatures above 25 K and could be fit with a spin-dependent VRH model; negative MR was seen at low temperatures. In the GHz regime, the ESR linewidth for SWCNTs was observed to narrow by as much as 50% as the temperature was increased from 3 to 300 K, a phenomenon known as motional narrowing, suggesting that we are detecting the ESR of hopping spins. From the linewidth change versus temperature, we find the hopping frequency to be 285 GHz. For excitons in InGaAs quantum wells, we demonstrate the manipulation of intra-excitonic populations using intense, narrow-band THz pulses. The THz radiation temporarily quenches the 1s emission, which is then followed by an enhancement and subsequent decay of 2s emission. After the quenching
Urbanization susceptibility maps: a dynamic spatial decision support system for sustainable land use
Directory of Open Access Journals (Sweden)
M. Cerreta
2012-10-01
Full Text Available Recent developments in land consumption assessment identify the need to implement integrated evaluative approaches, with particular attention to the identification of multidimensional tools for guiding and managing sustainable land use. Policy decisions defining land use are mostly implemented through spatial planning and related zoning, and this involves trade-offs between many sectoral interests and conflicting challenges aimed at win-win solutions. In order to identify a decision-making process for land use allocation, the paper proposes a methodological approach for a Dynamic Spatial Decision Support System (DSDSS, named Integrated Spatial Assessment (ISA, supported by Geographical Information Systems (GIS combined with Analytic Hierarchy Process (AHP. Through the empirical investigation in an operative case study, an integrated evaluative approach implemented in a DSDSS helps to elaborate "urbanization susceptibility maps", where spatial analysis combined with a multi-criteria method proved to be useful for facing the main issues related to land consumption and minimizing environmental impacts of spatial planning.
Onufrieva, F.
2017-03-01
The paper is motivated by the observation of unusual and not well understood spin dynamics in low- and moderately doped high-Tc cuprates as well as by the discovery in these materials of a static incommensurate order for doping exceeding the insulator-metal boundary in the phase diagram. We develop a microscopic approach that allows us to treat accurately the quantum fluctuations in the spiral state developing upon doping the Mott-Neel insulator. We show that the spiral order of localized spins induces an off-diagonal order of mobile charges and a gap Δ ∝|Q | in their spectrum (Q is the spiral incommensurability wave vector defined with respect to QAF). Due to the dynamic spin-charge interaction the latter gap produces a feedback effect consisting in the appearence of a gap in the coherent spin excitation spectrum. As a result, the characteristic energy ωc=Δ appears, in the spin excitation spectra. It separates two components with qualitatively different behavior-above ωc, spin excitations are magnonlike and have an upward dispersion, below it, they are of the relaxation type and have a slight downward dispersion. The form of the dispersion is close to the form observed experimentally (by inelastic neutron scattering), which can be characterized as OPEN-hour-glass shaped or Y -shaped. There is no qualitative difference between the spin dynamics in the normal and SC states as far as doping is relatively low. There is no resonance. Other important features, including the incommensurability and uniaxial anisotropy of the low-energy spin excitations and the doping dependencies of the characteristic energy and wave vectors, are also close to those observed experimentally in low-doped cuprates. We show that the static spiral state becomes unstable at the critical doping nc. We show also that adopting the hypothesis about the presence of finite-energy spiral correlations in the paramagnetic state above nc and based on the results obtained for the static spiral state
Waiting time distribution revealing the internal spin dynamics in a double quantum dot
Ptaszyński, Krzysztof
2017-07-01
Waiting time distribution and the zero-frequency full counting statistics of unidirectional electron transport through a double quantum dot molecule attached to spin-polarized leads are analyzed using the quantum master equation. The waiting time distribution exhibits a nontrivial dependence on the value of the exchange coupling between the dots and the gradient of the applied magnetic field, which reveals the oscillations between the spin states of the molecule. The zero-frequency full counting statistics, on the other hand, is independent of the aforementioned quantities, thus giving no insight into the internal dynamics. The fact that the waiting time distribution and the zero-frequency full counting statistics give a nonequivalent information is associated with two factors. Firstly, it can be explained by the sensitivity to different timescales of the dynamics of the system. Secondly, it is associated with the presence of the correlation between subsequent waiting times, which makes the renewal theory, relating the full counting statistics and the waiting time distribution, no longer applicable. The study highlights the particular usefulness of the waiting time distribution for the analysis of the internal dynamics of mesoscopic systems.
Spin Dynamics Simulations of Multiple Echo Spacing Pulse Sequences in Grossly Inhomogeneous Fields
Heidler, R.; Bachman, H. N.; Johansen, Y.
2008-12-01
Pulse sequences with multiple lengths of echo spacings are used in oilfield NMR logging for diffusion-based NMR applications such as rock and fluid characterization. One specific implementation is the so-called diffusion editing sequence comprising two long echo spacings followed by a standard CPMG at a shorter echo spacing. The echoes in the CPMG portion contain signal from both the direct and stimulated echoes. Modern oilfield NMR logging tools are designed for continuous depth logging of earth formations by projecting both the static (B0) and dynamic (B1) fields into the formation. Both B0 and B1 profiles are grossly inhomogeneous which results in non-steady-state behavior in the early echoes. The spin dynamics effects present a challenge for processing the echo amplitudes to measure porosity (amplitude extrapolated to zero time) and attenuations for fluid or pore size characterization. In this work we describe a calculation of the spin dynamics of the diffusion editing sequence with two long echo spacings. The calculation takes into account full B1 and B0 field maps, and comparisons will be made for sensors and parameters typical of oilfield logging tools and environments.
Spin dynamics in weakly and strongly interacting NiO nanoparticles
DEFF Research Database (Denmark)
Bahl, Christian Robert Haffenden; Lefmann, Kim; Kuhn, Luise Theil;
2006-01-01
The spin dynamics of plate-shaped nanoparticles of NiO has been studied by inelastic neutron scattering and Mossbauer spectroscopy. A value of the in-plane anisotropy energy constant significantly larger than the bulk value has been measured. The temperature and field dependence of the energy...... of the antiferromagnetic resonance mode associated with this in-plane anisotropy has been studied. Both Mossbauer spectroscopy and neutron scattering data show that the magnetic fluctuations are strongly affected by the strength of interparticle interactions....
Metal Atom Dynamics and Spin-Lattice Relaxation in Multilayer Sandwich Compounds
Energy Technology Data Exchange (ETDEWEB)
Nowik, Israel; Herber, Rolfe H., E-mail: HERBER@VMS.HUJI.AC.il [Hebrew University of Jerusalem, Racah Institute of Physics (Israel)
2004-12-15
Temperature-dependent {sup 57}Fe Moessbauer spectroscopy has been used to elucidate the hyperfine parameters and dynamical behavior of the metal atom in several organo-iron complexes which have one or more {eta}{sup 5} P{sub 5} ring structures as ligated groups. The spin-lattice relaxation of the (paramagnetic) one-electron oxidation products occurs on a time scale fast compared to {tau}{sub 1/2} (ME) at temperatures in the range 85 < T < 320 K.
Charges and currents in quantum spin chains: late-time dynamics and spontaneous currents
Fagotti, Maurizio
2017-01-01
We review the structure of the conservation laws in noninteracting spin chains and unveil a formal expression for the corresponding currents. We briefly discuss how interactions affect the picture. In the second part, we explore the effects of a localized defect. We show that the emergence of spontaneous currents near the defect undermines any description of the late-time dynamics by means of a stationary state in a finite chain. In particular, the diagonal ensemble does not work. Finally, we provide numerical evidence that simple generic localized defects are not sufficient to induce thermalization.
Instrumentation for solid-state dynamic nuclear polarization with magic angle spinning NMR
Rosay, Melanie; Blank, Monica; Engelke, Frank
2016-03-01
Advances in dynamic nuclear polarization (DNP) instrumentation and methodology have been key factors in the recent growth of solid-state DNP NMR applications. We review the current state of the art of solid-state DNP NMR instrumentation primarily based on available commercial platforms. We start with a general system overview, including options for microwave sources and DNP NMR probes, and then focus on specific developments for DNP at 100 K with magic angle spinning (MAS). Gyrotron microwave sources, passive components to transmit microwaves, the DNP MAS probe, a cooling device for low-temperature MAS, and sample preparation procedures including radicals for DNP are considered.
Molecular dynamics in rod-like liquid crystals probed by muon spin resonance spectroscopy.
McKenzie, Iain; Scheuermann, Robert; Sedlak, Kamil; Stoykov, Alexey
2011-08-01
Muoniated spin probes were produced by the addition of muonium (Mu) to two rod-like liquid crystals: N-(4-methoxybenzylidene)-4'-n-butylaniline (MBBA) and cholesteryl nonanoate (CN). Avoided level crossing muon spin resonance spectroscopy was used to characterize the muoniated spin probes and to probe dynamics at the molecular level. In MBBA Mu adds predominantly to the carbon of the bridging imine group and the muon and methylene proton hyperfine coupling constants (hfccs) of the resulting radical shift in the nematic phase due to the dipolar hyperfine coupling, the ordering of the molecules along the applied magnetic field and fluctuations about the local director. The amplitude of these fluctuations in in the nematic phase of MBBA is determined from the temperature dependence of the methylene proton hfcc. Mu adds to the double bond of the steroidal ring system of CN and the temperature dependence of the Δ(1) line width provides information about the amplitude of the fluctuations about the local director in the chiral nematic phase and the slow isotropic reorientation in the isotropic phase.
Dynamical correlation functions of the quadratic coupling spin-Boson model
Zheng, Da-Chuan; Tong, Ning-Hua
2017-06-01
The spin-boson model with quadratic coupling is studied using the bosonic numerical renormalization group method. We focus on the dynamical auto-correlation functions {C}O(ω ), with the operator \\hat{O} taken as {\\hat{{{σ }}}}x, {\\hat{{{σ }}}}z, and \\hat{X}, respectively. In the weak-coupling regime α exponents y O of these correlation functions are obtained as {y}{{{σ }}x}={y}{{{σ }}z}=1-2s and {y}X=-s, respectively. Here s is the bath index and X is the boson displacement operator. Close to the spin flip point, the high frequency peak of {C}{{{σ }}x}(ω ) is broadened significantly and the line shape changes qualitatively, showing enhanced dephasing at the spin flip point. Project supported by the National Key Basic Research Program of China (Grant No. 2012CB921704), the National Natural Science Foundation of China (Grant No. 11374362), the Fundamental Research Funds for the Central Universities, China, and the Research Funds of Renmin University of China (Grant No. 15XNLQ03).
Magnetic Dynamics of Single-Domain Planar Spin-Transfer Devices
Bazaliy, Ya. B.
2008-03-01
We study spin-transfer devices with dynamic magnets characterized by large easy-plane anisotropy. This situation is standard for planar devices where it arises due to the shape anisotropy. Dominating easy-plane anisotropy keeps the motion of the magnetic moment close to the easy plane, with small out-of-plane deviations. As a result, it is possible to approximately describe magnetization vector by the in-plane angle and derive an effective one dimensional equation for that angle in the absence [1] and in the presence [2] of spin-transfer torques. Effective description maps a spin-transfer device problem onto a problem of an ``effective particle'' moving in external potential with variable friction coefficient. The advantage of such a description is that the motion of the effective particle can be qualitatively understood by applying the usual energy conservation and dissipation arguments. We show how the effective description produces analytic results for current induced precession states [3] and predicts unconventional ``stabilization by repulsion'' of static states [2]. // [1] C. J. Garcia-Cervera, Weinan E, J. Appl. Phys. 90, 370 (2001). [2] Ya. B. Bazaliy, Phys. Rev. B 76, 140402(R) (2007). [3] Ya. B. Bazaliy, arXiv:0705.0508, to be published in Appl. Phys. Lett. (2007).
Hou, Kai; Wang, Huiyi; Lin, Yunyin; Chen, Shaohua; Yang, Shengyuan; Cheng, Yanhua; Hsiao, Benjamin S; Zhu, Meifang
2016-10-14
Hydrogel microfibers have been considered as a potential biomaterial to spatiotemporally biomimic 1D native tissues such as nerves and muscles which are always assembled hierarchically and have anisotropic response to external stimuli. To produce facile hydrogel microfibers in a mathematical manner, a novel dynamic-crosslinking-spinning (DCS) method is demonstrated for direct fabrication of size-controllable fibers from poly(ethylene glycol diacrylate) oligomer in large scale, without microfluidic template and in a biofriendly environment. The diameter of fibers can be precisely controlled by adjusting the spinning parameters. Anisotropic swelling property is also dependent on inhomogeneous structure generated in spinning process. Comparing with bulk hydrogels, the resulting fibers exhibit superior rapid water adsorption property, which can be attributed to the large surface area/volume ratio of fiber. This novel DCS method is one-step technology suitable for large-scale production of anisotropic hydrogel fibers which has a promising application in the area such as biomaterials. © 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
Spin dynamics of S = 1/2 kagome lattice antiferromagnets observed by high-field ESR
Energy Technology Data Exchange (ETDEWEB)
Ohta, Hitoshi [Molecular Photoscience Research Center, Kobe University, Kobe 657-8501 (Japan); Graduate School of Science, Kobe University, Kobe 657-8501 (Japan); Zhang, Wei-min [Graduate School of Science, Kobe University, Kobe 657-8501 (Japan); Okubo, Susumu; Fujisawa, Masashi [Molecular Photoscience Research Center, Kobe University, Kobe 657-8501 (Japan); Sakurai, Takahiro [Center for Supports to Research and Education Activities, Kobe University, Kobe 657-8501 (Japan); Okamoto, Yoshihiko; Yoshida, Hiroyuki; Hiroi, Zenji [Institute for Solid State Physics (ISSP), University of Tokyo, Kashiwa, Chiba 277-8581 (Japan)
2010-03-15
Due to the existence of strong spin frustration in a system, the spin dynamics of S = 1/2 kagome lattice antiferromagnet at low temperature has attracted much interest. High-field ESR has been measured on its model substances, Cu{sub 3}V{sub 2}O{sub 7}(OH){sub 2} . 2H{sub 2}O (volborthite) and BaCu{sub 3}V{sub 2}O{sub 3}(OH){sub 2} (vesignieite), down to 1.8 K using pulsed magnetic fields up to 16 T. The measurements are performed for 160 and 315 GHz using polycrys-talline samples. Although both samples showed the g-shift and the change of linewidth at low temperature, volborthite showed a small gap excitation of the order of 40 GHz (1.9 K) while vesignieite showed a paramagnetic behavior down to 1.9 K. Observed difference will be discussed in connection with the crystal structure, and the possible spin liquid state in vesignieite will be discussed. (Abstract Copyright [2010], Wiley Periodicals, Inc.)
Khaneja, Navin
2017-03-06
In this paper, we study some control problems related to the control of coupled spin dynamics in the presence of relaxation and decoherence in nuclear magnetic resonance spectroscopy. The decoherence is modelled through a master equation. We study some model problems, whereby, through an appropriate choice of state variables, the system is reduced to a control system, where the state enters linearly and controls quadratically. We study this quadratic control system. Study of this system gives us explicit bounds on how close a coupled spin system can be driven to its target state and how much coherence and polarization can be transferred between coupled spins. Optimal control for the quadratic control system can be understood as the separation of closed cones, and we show how the derived results on optimal efficiency can be interpreted in this formulation. Finally, we study some finite-time optimal control problems for the quadratic control system.This article is part of the themed issue 'Horizons of cybernetical physics'.
Khaneja, Navin
2017-03-01
In this paper, we study some control problems related to the control of coupled spin dynamics in the presence of relaxation and decoherence in nuclear magnetic resonance spectroscopy. The decoherence is modelled through a master equation. We study some model problems, whereby, through an appropriate choice of state variables, the system is reduced to a control system, where the state enters linearly and controls quadratically. We study this quadratic control system. Study of this system gives us explicit bounds on how close a coupled spin system can be driven to its target state and how much coherence and polarization can be transferred between coupled spins. Optimal control for the quadratic control system can be understood as the separation of closed cones, and we show how the derived results on optimal efficiency can be interpreted in this formulation. Finally, we study some finite-time optimal control problems for the quadratic control system. This article is part of the themed issue 'Horizons of cybernetical physics'.
Experimental investigation of magnetic anisotropy in spin vortex discs
Energy Technology Data Exchange (ETDEWEB)
Garraud, N., E-mail: ngarraud@ufl.edu; Arnold, D. P. [Department of Electrical and Computer Engineering, University of Florida, Gainesville, Florida 32611 (United States)
2014-05-07
We present experimental 2D vector vibrating sample magnetometer measurements to demonstrate the shape anisotropy effects occurring in micrometer-diameter supermalloy spin vortex discs. Measurements made for different disc sizes and orientations confirm the out-of-plane susceptibility is several orders of magnitude smaller than the in-plane susceptibility. These results validate with a high certitude that spin vortices with high diameter to thickness ratio retain in-plane-only magnetization, even when subjected to fields in the out-of-plane direction. These results contribute to further computational simulations of the dynamics of spin vortex structures in colloidal suspensions where external fields may be applied in any arbitrary direction.
Wieser, R
2017-05-04
A self-consistent mean field theory is introduced and used to investigate the thermodynamics and spin dynamics of an S = 1 quantum spin system with a magnetic Skyrmion. The temperature dependence of the Skyrmion profile as well as the phase diagram are calculated. In addition, the spin dynamics of a magnetic Skyrmion is described by solving the time dependent Schrödinger equation with additional damping term. The Skyrmion annihilation process driven by an electric field is used to compare the trajectories of the quantum mechanical simulation with a semi-classical description for the spin expectation values using a differential equation similar to the classical Landau-Lifshitz-Gilbert equation.
Albert, Brice J; Pahng, Seong Ho; Alaniva, Nicholas; Sesti, Erika L; Rand, Peter W; Saliba, Edward P; Scott, Faith J; Choi, Eric J; Barnes, Alexander B
2017-10-01
Cryogenic sample temperatures can enhance NMR sensitivity by extending spin relaxation times to improve dynamic nuclear polarization (DNP) and by increasing Boltzmann spin polarization. We have developed an efficient heat exchanger with a liquid nitrogen consumption rate of only 90L per day to perform magic-angle spinning (MAS) DNP experiments below 85K. In this heat exchanger implementation, cold exhaust gas from the NMR probe is returned to the outer portion of a counterflow coil within an intermediate cooling stage to improve cooling efficiency of the spinning and variable temperature gases. The heat exchange within the counterflow coil is calculated with computational fluid dynamics to optimize the heat transfer. Experimental results using the novel counterflow heat exchanger demonstrate MAS DNP signal enhancements of 328±3 at 81±2K, and 276±4 at 105±2K. Copyright © 2017 Elsevier Inc. All rights reserved.
Kuprov, Ilya
2008-11-01
We extend the recently proposed state-space restriction (SSR) technique for quantum spin dynamics simulations [Kuprov et al., J. Magn. Reson. 189 (2007) 241-250] to include on-the-fly detection and elimination of unpopulated dimensions from the system density matrix. Further improvements in spin dynamics simulation speed, frequently by several orders of magnitude, are demonstrated. The proposed zero track elimination (ZTE) procedure is computationally inexpensive, reversible, numerically stable and easy to add to any existing simulation code. We demonstrate that it belongs to the same family of Krylov subspace techniques as the well-known Lanczos basis pruning procedure. The combined SSR + ZTE algorithm is recommended for simulations of NMR, EPR and Spin Chemistry experiments on systems containing between 10 and 10 4 coupled spins.
Vortex Dynamics in a Spin-Orbit-Coupled Bose-Einstein Condensate
Fetter, Alexander L.
2015-07-01
Vortices in a one-component dilute atomic ultracold Bose-Einstein condensate (BEC) usually arise as a response to externally driven rotation. Apart from a few special situations, these vortices are singly quantized with unit circulation (Fetter, Rev Mod Phys 81, 647-691, 2009). Recently, the NIST group has constructed a two-component BEC with a spin-orbit-coupled Hamiltonian involving Pauli matrices (Spielman, Phys Rev A 79, 063613, 2009; Y.-J. Lin et al., Nature 462, 628-632, 2009; Y.-J. Lin et al., Nature 471, 83-87, 2011), and I here study the dynamics of a two-component vortex in such a spin-orbit-coupled condensate. These spin-orbit-coupled BECs use an applied magnetic field to split the hyperfine levels. Hence, they rely on a focused laser beam to trap the atoms. In addition, two Raman laser beams create an effective (or synthetic) gauge potential. The resulting spin-orbit Hamiltonian is discussed in some detail. The various laser beams are fixed in the laboratory, so that it is not feasible to nucleate a vortex by an applied rotation that would need to rotate all the laser beams and the magnetic field. In a one-component BEC, a vortex can also be created by a thermal quench, starting from the normal state and suddenly cooling deep into the condensed state (Freilich et al., Science 329, 1182-1185, 2010). I propose that a similar method would work for a vortex in a spin-orbit-coupled BEC. Such a vortex has two components, and each has its own circulation quantum number (typically ). If both components have the same circulation, I find that the composite vortex should execute uniform precession, like that observed in a single-component BEC (Freilich et al., Science 329, 1182-1185, 2010). In contrast, if one component has unit circulation and the other has zero circulation, then some fraction of the dynamical vortex trajectories should eventually leave the condensate, providing clear experimental evidence for this unusual vortex structure. In the context of
Lafuente-Sampietro, A.; Boukari, H.; Besombes, L.
2017-06-01
We analyze, through resonant photoluminescence, the spin dynamics of an individual magnetic atom (Mn) coupled to a hole in a semiconductor quantum dot. The hybrid Mn hole spin and the positively charged exciton in a CdTe/ZnTe quantum dot form an ensemble of Λ systems which can be addressed optically. Autocorrelation of the resonant photoluminescence and resonant optical pumping experiments are used to study the spin relaxation channels in this multilevel spin system. We identified for the hybrid Mn hole spin an efficient relaxation channel driven by the interplay of the Mn hole exchange interaction and the coupling to acoustic phonons. We also show that the optical Λ systems are connected through inefficient spin flips than can be enhanced under weak transverse magnetic field. The dynamics of the resonant photoluminescence in a p -doped magnetic quantum dot is well described by a complete rate equation model. Our results suggest that long-lived hybrid Mn hole spin could be obtained in quantum dot systems with large heavy-hole/light-hole splitting.
Energy Technology Data Exchange (ETDEWEB)
Neumann, A.U.; Derrida, B.
1988-10-01
We study the time evolution of two configurations submitted to the same thermal noise for several two dimensional models (Ising ferromagnet, symmetric spin glass, non symmetric spin glass). For all these models, we find a non zero critical temperature above which the two configurations always meet. Using finite size scaling ideas, we determine for these three models this dynamical phase transition and some of the critical exponents. For the ferromagnet, the transition T/sub c/ approx. = 2.25 coincides with the Curie temperature whereas for the two spin glass models +- J distribution of bonds) we obtain T/sub c/ approx. = 1.5-1.7.
Wal, Andrzej; Barnaś, Józef
2016-01-01
This book is a collection of lecture notes which were presented by invited speakers at the Eleventh School on Theoretical Physics "Symmetry and Structural Properties of Condensed Matter SSPCM 2014" in Rzeszów (Poland) in September 2014. The main challenge for the lecturers was the objective to present their subject as a review as well as in the form of introduction for beginners. Topics considered in the volume concentrate on: spin dynamics and spin transport in magnetic and non-magnetic structures, spin-orbit interaction in two-dimensional systems and graphene, and new mathematical method used in the condensed matter physics.
Electric probe for spin transition and fluctuation
Qiu, Zhiyong; Li, Jia; Hou, Dazhi; Arenholz, Elke; N'diaye, Alpha T.; Tan, Ali; Uchida, Ken-Ichi; Sato, Koji; Tserkovnyak, Yaroslov; Qiu, Z. Q.; Saitoh, Eiji
Spin fluctuation and transition have always been one of central topics of magnetism and condense matter science. To probe them, neutron scatterings have been used as powerful tools. A part of neutrons injected into a sample is scattered by spin fluctuation inside the sample. This process transcribes the spin fluctuation onto scattering intensity, which is commonly represented by dynamical magnetic susceptibility of the sample and is maximized at magnetic phase transitions. Importantly, a neutron carries spin without electric charge, and it thus can bring spin into a sample without being disturbed by electric energy: an advantage of neutrons, although large facilities such as a nuclear reactor is necessary. Here we show that spin pumping, frequently used in nanoscale spintronic devices, provides a desktop micro probe for spin fluctuation and transition; not only a neutron beam, spin current is also a flux of spin without an electric charge and its transport reflects spin fluctuation in a sample. We demonstrate detection of anti-ferromagnetic transition in ultra-thin CoO films via frequency dependent spin-current transmission measurements.
Dynamical passage to approximate equilibrium shapes for spinning, gravitating rubble asteroids
Sharma, Ishan; Jenkins, James T.; Burns, Joseph A.
2009-03-01
Many asteroids are thought to be particle aggregates held together principally by self-gravity. Here we study — for static and dynamical situations — the equilibrium shapes of spinning asteroids that are permitted for rubble piles. As in the case of spinning fluid masses, not all shapes are compatible with a granular rheology. We take the asteroid to always be an ellipsoid with an interior modeled as a rigid-plastic, cohesion-less material with a Drucker-Prager yield criterion. Using an approximate volume-averaged procedure, based on the classical method of moments, we investigate the dynamical process by which such objects may achieve equilibrium. We first collapse our dynamical approach to its statical limit to derive regions in spin-shape parameter space that allow equilibrium solutions to exist. At present, only a graphical illustration of these solutions for a prolate ellipsoid following the Drucker-Prager failure law is available [Sharma, I., Jenkins, J.T., Burns, J.A., 2005a. Bull. Am. Astron. Soc. 37, 643; Sharma, I., Jenkins, J.T., Burns, J.A., 2005b. Equilibrium shapes of ellipsoidal soil asteroids. In: García-Rojo, R., Hermann, H.J., McNamara, S. (Eds.), Proceedings of the 5th International Conference on Micromechanics of Granular Media, vol. 1. A.A. Balkema, UK; Holsapple, K.A., 2007. Icarus 187, 500-509]. Here, we obtain the equilibrium landscapes for general triaxial ellipsoids, as well as provide the requisite governing formulae. In addition, we demonstrate that it may be possible to better interpret the results of Richardson et al. [Richardson, D.C., Elankumaran, P., Sanderson, R.E., 2005. Icarus 173, 349-361] within the context of a Drucker-Prager material. The graphical result for prolate ellipsoids in the static limit is the same as those of Holsapple [Holsapple, K.A., 2007. Icarus 187, 500-509] because, when worked out, his final equations will match ours. This is because, though the formalisms to reach these expressions differ, in statics
Novotny, M.A.; Guerra, M.; Raedt, H. De; Michielsen, K.; Jin, F.
2012-01-01
An efficient algorithm for the computation of the real-time dependence of a single quantum spin-1/2 coupled to a specific set of quantum spin-1/2 baths is presented. The specific spin baths have couplings only with the spin operators Sx between bath spins and the central spin. We calculate spin expe
Jaris, M.; Yahagi, Y.; Mahato, B. K.; Dhuey, S.; Cabrini, S.; Nikitin, V.; Stout, J.; Hawkins, A. R.; Schmidt, H.
2016-11-01
We report the all-optical observation of intrinsic spin dynamics and extraction of magnetic material parameters from arrays of sub-100 nm spin-transfer torque magnetic random access memory (STT-MRAM) devices with a CoFeB/MgO interface. To this end, the interference of surface acoustic waves with time-resolved magneto-optic signals via magneto-elastic coupling was suppressed using a dielectric coating. The efficacy of this method is demonstrated experimentally and via modeling on a nickel nanomagnet array. The magnetization dynamics for both coated nickel and STT-MRAM arrays shows a restored field-dependent Kittel mode from which the effective damping can be extracted. We observe an increased low-field damping due to extrinsic contributions from magnetic inhomogeneities and variations in the nanomagnet shape, while the intrinsic Gilbert damping remains unaffected by patterning. The data are in excellent agreement with a local resonance model and have direct implications for the design of STT-MRAM devices as well as other nanoscale spintronic technologies.
Dynamic structure factor of the spin-1/2 XXZ chain in a transverse field
Bruognolo, Benedikt; Weichselbaum, Andreas; von Delft, Jan; Garst, Markus
2016-08-01
The spin-1/2 XXZ chain with easy-plane anisotropy in a transverse field describes well the thermodynamic properties of the material Cs2CoCl4 in a wide range of temperatures and fields including the region close to the spin-flop Ising quantum phase transition. For a comparison with prospective inelastic neutron scattering experiments on this compound, we present results of an extensive numerical study of its dynamic structure factor Sα β(k ,ω ) using matrix-product-state (MPS) techniques. Close to criticality, the dynamic part of the correlator Sx x longitudinal to the applied field is incoherent and possesses a small total weight as the ground state is already close to saturation. The transverse correlator Sz z, on the other hand, is dominated by a coherent single-particle excitation with additional spectral weight at higher energies that we tentatively attribute to a repulsively bound pair of particles. With increasing temperature, the latter quickly fades and spectral weight instead accumulates close to zero wave vector just above the single-particle energy. On a technical level, we compare the numerical efficiency of real-time evolution to an MPS-based Chebyshev expansion in the present context, finding that both methods yield results of similar quality at comparable numerical costs.
Larsen, DeLaine D; Choy, Regina Wai-Yan; Park, Minjong
2017-01-01
Synaptic activity is modulated by the activation of neuromodulator receptors present in dendrites of neurons. The majority of neuromodulator receptors are G protein coupled receptors (GPCRs), in which membrane trafficking regulates their activities. Membrane trafficking of neuromodulator receptors and their signaling occurs on a rapid time scale and emerging studies indicate that neuromodulator receptors function not just from the plasma membrane but also from the endocytic compartments. Here, we describe a live cell imaging approach using spinning disk confocal microscopy to investigate the effect of neuromodulator receptor activation on synaptic activity by measuring calcium dynamics in primary rat striatal neurons. The advantages of spinning disk confocal microscopy and recent improvements in the genetically encoded calcium sensor, GCaMP6, provide an imaging approach to image both the receptor membrane trafficking to endocytic compartments, and calcium dynamics at a high spatial and temporal resolution. We believe this approach of imaging both the neuromodulator receptor membrane trafficking and synaptic activity using GCaMP6 is a powerful tool to address many questions regarding possible roles of membrane trafficking of neuromodulator receptors in synaptic activity.
Acevedo, Óscar L.; Quiroga, Luis; Rodríguez, Ferney J.; Johnson, Neil F.
2014-03-01
Dynamical quantum phase crossings of spin networks have recently received increased attention thanks to their relation to adiabatic quantum computing, and their feasible realizations using ultra-cold atomic and molecular systems with a highly tunable degree of connectivity. Dynamical scaling of spatially distributed systems like Ising models have been widely studied, and successfully related to well-known theories like the Kibble-Zurek mechanism. The case of totally connected networks such as the Dicke Model and Lipkin-Meshkov-Glick Model, however, is known to exhibit a breakdown of these frameworks. Our analysis overcomes the lack of spatial correlation structure by developing a general approach which (i) is valid regardless the connectivity of the system, (ii) goes beyond critical exponents, and (iii) provides a time-resolved picture of dynamical scaling. By treating these models as a method for macroscopic quantum control of their subsystems, we have found microscopic signatures of the dynamical scaling as well as instances of dynamical enhancement of distinctive quantum properties such as entanglement and coherence. Our results yield novel prescriptions for the fields of quantum simulations and quantum control, and deepen our fundamental understanding of phase transitions.
Wencka, M.; Lijewski, S.; Hoffmann, S. K.
2008-06-01
ESR spectra were recorded in the X-band (9.6 GHz) and in the W-band (94 GHz) and electron spin relaxation was measured by electron spin echo (ESE) in the temperature range 4.2-300 K for radicals in natural calcite samples obtained from a cave stalactite and a dripstone layer. Four types of carbonate radical spectra and two sulfate radical spectra were identified and high accuracy g-factors were derived. Time and temperature behaviour of the spectra show that the dominating CO2- radicals are rigidly bonded or undergo free reorientations, whereas CO3-, SO2- and SO3- only undergo free reorientations. Below 200 K the free reorientations of CO2- are suppressed and a hindered rotation around single local axis appears. The ESE detected spectrum proves that the lines of free rotating radicals are homogeneously broadened, thus they cannot participate in electron spin echo formation. Spin-lattice relaxation data show that CO2- radicals are decoupled from lattice phonons and relax via local mode tunnelling motion between inequivalent oxygen positions of CO2- molecules. The tunnelling appears in two excited vibrational states of energy 71 and 138 cm-1. Librational motions of CO2- molecules were detected by electron spin echo decay (phase relaxation) with energy 153 cm-1. Two kinds of impurity hydrogen atoms were distinguished from ESEEM: in-water inclusions and water coordinated to the calcium ions.
Singularities of the dynamical structure factors of the spin-1/2 XXX chain at finite magnetic field
Carmelo, J. M. P.; Sacramento, P. D.; Machado, J. D. P.; Campbell, D. K.
2015-10-01
We study the longitudinal and transverse spin dynamical structure factors of the spin-1/2 XXX chain at finite magnetic field h, focusing in particular on the singularities at excitation energies in the vicinity of the lower thresholds. While the static properties of the model can be studied within a Fermi-liquid like description in terms of pseudoparticles, our derivation of the dynamical properties relies on the introduction of a form of the ‘pseudofermion dynamical theory’ (PDT) of the 1D Hubbard model suitably modified for the spin-only XXX chain and other models with two pseudoparticle Fermi points. Specifically, we derive the exact momentum and spin-density dependences of the exponents {{\\zeta}τ}(k) controlling the singularities for both the longitudinal ≤ft(τ =l\\right) and transverse ≤ft(τ =t\\right) dynamical structure factors for the whole momentum range k\\in ]0,π[ , in the thermodynamic limit. This requires the numerical solution of the integral equations that define the phase shifts in these exponents expressions. We discuss the relation to neutron scattering and suggest new experiments on spin-chain compounds using a carefully oriented crystal to test our predictions.
Energy Technology Data Exchange (ETDEWEB)
Guo, Y. J. [School of Physics and Electronic Engineering, Jiangsu Second Normal University, Nanjing 210013 (China); Laboratory of Solid State Microstructures, Nanjing University, Nanjing 210093 (China); Gao, Y. J.; Ge, C. N [School of Physics and Electronic Engineering, Jiangsu Second Normal University, Nanjing 210013 (China); Guo, Y. Y. [College of Electronic Science and Engineering, Nanjing University of Posts and Telecommunications, Nanjing 210003 (China); Yan, Z. B.; Liu, J.-M., E-mail: liujm@nju.edu.cn [Laboratory of Solid State Microstructures, Nanjing University, Nanjing 210093 (China)
2015-05-07
In this work, the dynamics of a diatomic chain is investigated with ↑↑↓↓ spin order in which the dispersion relation characterizes the effect of magnetic interactions on the lattice dynamics. The optical or acoustic mode softening in the center or boundary of the Brillouin zone can be observed, indicating the transitions of ferroelectric state, antiferromagnetic state, or ferroelastic state. The coexistence of the multiferroic orders related to the ↑↑↓↓ spin order represents a type of intrinsic multiferroic with strong ferroelectric order and different microscopic mechanisms.
Elasto-dynamic analysis of spinning nanodisks via a surface energy-based model
Kiani, Keivan
2016-07-01
Using the surface elasticity theory of Gurtin and Murdoch, in-plane vibrations of annular nanodisks due to their rotary motion are explored. By the imposition of non-classical boundary conditions on the innermost and outermost surfaces and employing Hamilton’s principle, the unknown elasto-dynamic fields of the bulk zone are determined via the finite element method. The roles of both nanodisk geometry and surface effect on the natural frequencies are addressed. Subsequently, forced vibrations of spinning nanodisks with fixed-free and free-free boundary conditions are comprehensively examined. The obtained results show that the maximum dynamic elastic fields grow in a parabolic manner as the steady angular velocity increases. By increasing the outermost radius, the maximum dynamic elastic field is magnified and the influence of the surface effect on the results reduced. This work can be considered as a pivotal step towards optimal design and dynamic analysis of nanorotors with disk-like parts, which are one of the basic building blocks of the upcoming advanced nanotechnologies.
Boča, R.; Boča, M.; Ehrenberg, H.; Fuess, H.; Linert, W.; Renz, F.; Svoboda, I.
2003-09-01
The thermal expansion of the spin crossover system [Fe(pybzim) 3](ClO 4) 2 · H 2O (pybzim=2-(2 '-pyridyl)benzimidazole) has been determined from powder X-ray data between 50 and 250 K; the wavelength of the synchrotron source was 1.21888(1) Å. The unit cell parameters of the triclinic crystal system were a=12.091 Å, b=12.225 Å, c=14.083 Å, α=77.70°, β=80.35°, γ=74.35°, and V=1944.9 Å 3 at 250 K. In addition to the linear thermal expansion of the unit cell volume, an extra expansion due to the low-spin (LS) to high-spin (HS) transition is observed. The V( T) function shows a sudden increase comparable with the step in the effective magnetic moment at the transition region (140 K). A similar behavior is obtained on the basis of the infrared spectra. The absorption bands corresponding to the metal-ligand stretching modes change their intensities upon heating: the bands corresponding to the low-spin molecules (at ca. 409, 430, 443, and 460 cm -1) disappear in the gain of the high-spin bands (at 259 and 285 cm -1). The variable-temperature data obtained by different techniques (powder diffraction, EXAFS, IR spectra, Mössbauer spectra, magnetic susceptibility, DSC) have been transformed to a common basis - the temperature dependence of the high-spin mole fraction xHS( T). The application of the Ising-like (two-level) model of the spin crossover led to the thermodynamic data Δ H=2.6 kJ mol -1 and Δ S=19 J K -1 mol -1 as well as to the cooperativeness J/ k≈110 K (subtracted from the susceptibility data) that characterizes the abruptness of the spin crossover in the solid state.
Fisher, D S; Le Doussal, P; Monthus, C
2001-12-01
The nonequilibrium dynamics of classical random Ising spin chains with nonconserved magnetization are studied using an asymptotically exact real space renormalization group (RSRG). We focus on random field Ising model (RFIM) spin chains with and without a uniform applied field, as well as on Ising spin glass chains in an applied field. For the RFIM we consider a universal regime where the random field and the temperature are both much smaller than the exchange coupling. In this regime, the Imry-Ma length that sets the scale of the equilibrium correlations is large and the coarsening of domains from random initial conditions (e.g., a quench from high temperature) occurs over a wide range of length scales. The two types of domain walls that occur diffuse in opposite random potentials, of the form studied by Sinai, and domain walls annihilate when they meet. Using the RSRG we compute many universal asymptotic properties of both the nonequilibrium dynamics and the equilibrium limit. We find that the configurations of the domain walls converge rapidly toward a set of system-specific time-dependent positions that are independent of the initial conditions. Thus the behavior of this nonequilibrium system is pseudodeterministic at long times because of the broad distributions of barriers that occur on the long length scales involved. Specifically, we obtain the time dependence of the energy, the magnetization, and the distribution of domain sizes (found to be statistically independent). The equilibrium limits agree with known exact results. We obtain the exact scaling form of the two-point equal time correlation function and the two-time autocorrelations . We also compute the persistence properties of a single spin, of local magnetization, and of domains. The analogous quantities for the +/-J Ising spin glass in an applied field are obtained from the RFIM via a gauge transformation. In addition to these we compute the two-point two-time correlation function which can in
Digernes, Ingrid; Bjørnerud, Atle; Vatnehol, Svein Are S; Løvland, Grete; Courivaud, Frédéric; Vik-Mo, Einar; Meling, Torstein R; Emblem, Kyrre E
2017-06-01
Mapping the complex heterogeneity of vascular tissue in the brain is important for understanding cerebrovascular disease. In this translational study, we build on previous work using vessel architectural imaging (VAI) and present a theoretical framework for determining cerebral vascular function and heterogeneity from dynamic susceptibility contrast magnetic resonance imaging (MRI). Our tissue model covers realistic structural architectures for vessel branching and orientations, as well as a range of hemodynamic scenarios for blood flow, capillary transit times and oxygenation. In a typical image voxel, our findings show that the apparent MRI relaxation rates are independent of the mean vessel orientation and that the vortex area, a VAI-based parameter, is determined by the relative oxygen saturation level and the vessel branching of the tissue. Finally, in both simulated and patient data, we show that the relative distributions of the vortex area parameter as a function of capillary transit times show unique characteristics in normal-appearing white and gray matter tissue, whereas tumour-voxels in comparison display a heterogeneous distribution. Collectively, our study presents a comprehensive framework that may serve as a roadmap for in vivo and per-voxel determination of vascular status and heterogeneity in cerebral tissue.
Energy Technology Data Exchange (ETDEWEB)
Jabehdar Maralani, Pejman [University of Toronto, Department of Medical Imaging, Sunnybrook Health Sciences Center, Toronto, ON (Canada); Melhem, Elias R.; Herskovits, Edward H. [University of Maryland Medical Center, Department of Radiology, Baltimore, MD (United States); Wang, Sumei; Voluck, Matthew R.; Learned, Kim O.; Mohan, Suyash [Perelman School of Medicine at University of Pennsylvania, Department of Radiology, Division of Neuroradiology, Philadelphia, PA (United States); Kim, Sang Joon [University of Ulsan Asan Medical Center, Department of Radiology, Songpa-gu, Seoul (Korea, Republic of); O' Rourke, Donald M. [Perelman School of Medicine at University of Pennsylvania, Department of Surgery, Division of Neurosurgery, Philadelphia, PA (United States)
2015-09-15
We aimed to evaluate the prognostic value of dynamic susceptibility contrast (DSC) MR perfusion in elderly patients with glioblastomas (GBM). Thirty five patients aged ≥65 and 35 aged <65 years old, (referred to as elderly and younger, respectively) were included in this retrospective study. The median relative cerebral volume (rCBV) from the enhancing region (rCBV{sub ER-Med}) and immediate peritumoral region (rCBV{sub IPR-Med}) and maximum rCBV from the enhancing region of the tumor (rCBV{sub ER-Max}) were compared and correlated with survival data. Analysis was repeated after rCBVs were dichotomized into high and low values and after excluding elderly patients who did not receive postoperative chemoradiation (34.3 %). Kaplan-Meyer survival curves and parametric and semi-parametric regression tests were used for analysis. All rCBV parameters were higher in elderly compared to younger patients (p < 0.05). After adjustment for age, none were independently associated with shorter survival (p > 0.05). After rCBV dichotomization into high and low values, high rCBV in elderly was independently associated with shorter survival compared to low rCBV in elderly, or any rCBV in younger patients (p < 0.05). rCBV can be an imaging biomarker to identify a subgroup of GBM patients in the elderly with worse prognosis compared to others. (orig.)
Dynamic Susceptibility Contrast Magnetic Resonance Imaging Protocol of the Normal Canine Brain
Stadler, Krystina L.; Pease, Anthony P.; Ballegeer, Elizabeth A.
2017-01-01
Perfusion magnetic resonance imaging (MRI), specifically dynamic susceptibility MRI (DSC-MRI) is routinely performed as a supplement to conventional MRI in human medicine for patients with intracranial neoplasia and cerebrovascular events. There is minimal data on the use of DSC-MRI in veterinary patients and a DSC-MRI protocol in the veterinary patient has not been described. Sixteen normal dogs, 6 years or older were recruited for this study. The sample population included 11 large dogs (>11 kg) and 5 small dogs (11 kg, a useable AIF and perfusion map was generated. One dog less than 11 kg received the same contrast dose and rate. In this patient, the protocol did not generate a useable AIF. The remainder of the dogs less than 11 kg followed a protocol of 0.2 mmol/kg gadolinium-based contrast media at 1.5 ml/s with a 10 ml saline flush at 1.5 ml/s. A useable AIF and perfusion map was generated in the remaining dogs <11 kg using the higher contrast dose and slower rate protocol. This study establishes a contrast dose and administration rate for canine DSC-MRI imaging that is different in dogs greater than 11 kg compared to dogs less than 11 kg. These protocols may be used for future applications to evaluate hemodynamic disturbances in canine intracranial pathology.
Directory of Open Access Journals (Sweden)
Richard Leigh
Full Text Available PURPOSE: To determine if applying an arrival time correction (ATC to dynamic susceptibility contrast (DSC based permeability imaging will improve its ability to identify contrast leakage in stroke patients for whom the shape of the measured curve may be very different due to hypoperfusion. MATERIALS AND METHODS: A technique described in brain tumor patients was adapted to incorporate a correction for delayed contrast delivery due to perfusion deficits. This technique was applied to the MRIs of 9 stroke patients known to have blood-brain barrier (BBB disruption on T1 post contrast imaging. Regions of BBB damage were compared with normal tissue from the contralateral hemisphere. Receiver operating characteristic (ROC analysis was performed to compare the detection of BBB damage before and after ATC. RESULTS: ATC improved the area under the curve (AUC of the ROC from 0.53 to 0.70. The sensitivity improved from 0.51 to 0.67 and the specificity improved from 0.57 to 0.66. Visual inspection of the ROC curve revealed that the performance of the uncorrected analysis was worse than random guess at some thresholds. CONCLUSIONS: The ability of DSC permeability imaging to identify contrast enhancing tissue in stroke patients improved considerably when an ATC was applied. Using DSC permeability imaging in stroke patients without an ATC may lead to false identification of BBB disruption.
Mikolasek, Mirko; Félix, Gautier; Peng, Haonan; Rat, Sylvain; Terki, Férial; Chumakov, Aleksandr I.; Salmon, Lionel; Molnár, Gábor; Nicolazzi, William; Bousseksou, Azzedine
2017-07-01
We report the investigation of the size evolution of lattice dynamics in spin crossover coordination nanoparticles of [ Fe (pyrazine ) (Ni (CN) 4) ] through nuclear inelastic scattering (NIS) measurements. Vibrational properties in these bistable molecular materials are of paramount importance and NIS permits access to the partial vibrational density of states in both spin states [high spin (HS) and low spin (LS)] from which thermodynamical and mechanical properties can be extracted. We show that the size reduction leads to the presence of inactive metal centers with the coexistence of HS and LS vibrational modes. The confinement effect has only weak impact on the vibrational properties of nanoparticles, especially on the optical modes which remain almost unchanged. On the other hand, the acoustic modes are much more affected which results in the increase of the vibrational entropy and also the Debye sound velocity in the smallest particles (nanoparticles is also highlighted through the matrix dependence of the sound velocity.
High-energy spin dynamics in La1.69Sr0.31NiO4.
Bourges, P; Sidis, Y; Braden, M; Nakajima, K; Tranquada, J M
2003-04-11
To test the prediction that the dispersion of the magnetic resonance in superconducting YBa2Cu3O(6+x) is similar to magnons in an incommensurate antiferromagnet, we have mapped out the spin dynamics in a stripe-ordered nickelate, La(2-x)SrxNiO4, with x approximately equal to 0.31, using inelastic neutron scattering. We observe spin-wave excitations up to 80 meV emerging from the incommensurate magnetic peaks with a surprisingly large and almost isotropic spin velocity: variant Planck's over 2 pi c(s) approximately 0.32 eV A. A comparison indicates that the inferred spin-excitation spectrum is not, by itself, an adequate model for the magnetic resonance feature of the superconductor.
Incommensurability and spin dynamics in the low-temperature phases of Ni3V2O8
Ehlers, G.; Podlesnyak, A. A.; Hahn, S. E.; Fishman, R. S.; Zaharko, O.; Frontzek, M.; Kenzelmann, M.; Pushkarev, A. V.; Shiryaev, S. V.; Barilo, S.
2013-06-01
Magnetic order and low-energy spin dynamics in the zero field ground state of Ni3V2O8 are revealed in elastic and inelastic neutron scattering experiments. Neutron diffraction shows that below T=2.3 K the Ni2+ moments (spin S=1) order in a cycloid pattern with incommensurate wave vector kICM=(0,1,τ), where τ=0.4030±0.0004, which is superimposed on a commensurate antiferromagnetic spin arrangement with kCM=(0,0,0). Three spin wave modes are discerned below E˜3 meV in inelastic measurements and qualitatively described by a model Hamiltonian that involves near neighbor exchange, local anisotropy, and a small biquadratic coupling between the spine and cross-tie sites. Results from both elastic and inelastic scattering experiments suggest that the two sublattices on spine and cross-tie sites are largely decoupled.
Tuning the presence of dynamical phase transitions in a generalized X Y spin chain
Divakaran, Uma; Sharma, Shraddha; Dutta, Amit
2016-05-01
We study an integrable spin chain with three spin interactions and the staggered field (λ ) while the latter is quenched either slowly [in a linear fashion in time (t ) as t /τ , where t goes from a large negative value to a large positive value and τ is the inverse rate of quenching] or suddenly. In the process, the system crosses quantum critical points and gapless phases. We address the question whether there exist nonanalyticities [known as dynamical phase transitions (DPTs)] in the subsequent real-time evolution of the state (reached following the quench) governed by the final time-independent Hamiltonian. In the case of sufficiently slow quenching (when τ exceeds a critical value τ1), we show that DPTs, of the form similar to those occurring for quenching across an isolated critical point, can occur even when the system is slowly driven across more than one critical point and gapless phases. More interestingly, in the anisotropic situation we show that DPTs can completely disappear for some values of the anisotropy term (γ ) and τ , thereby establishing the existence of boundaries in the (γ -τ ) plane between the DPT and no-DPT regions in both isotropic and anisotropic cases. Our study therefore leads to a unique situation when DPTs may not occur even when an integrable model is slowly ramped across a QCP. On the other hand, considering sudden quenches from an initial value λi to a final value λf, we show that the condition for the presence of DPTs is governed by relations involving λi,λf, and γ , and the spin chain must be swept across λ =0 for DPTs to occur.
Charge and spin dynamics driven by ultrashort extreme broadband pulses: A theory perspective
Moskalenko, Andrey S.; Zhu, Zhen-Gang; Berakdar, Jamal
2017-02-01
This article gives an overview on recent theoretical progress in controlling the charge and spin dynamics in low-dimensional electronic systems by means of ultrashort and ultrabroadband electromagnetic pulses. A particular focus is put on sub-cycle and single-cycle pulses and their utilization for coherent control. The discussion is mostly limited to cases where the pulse duration is shorter than the characteristic time scales associated with the involved spectral features of the excitations. The relevant current theoretical knowledge is presented in a coherent, pedagogic manner. We work out that the pulse action amounts in essence to a quantum map between the quantum states of the system at an appropriately chosen time moment during the pulse. The influence of a particular pulse shape on the post-pulse dynamics is reduced to several integral parameters entering the expression for the quantum map. The validity range of this reduction scheme for different strengths of the driving fields is established and discussed for particular nanostructures. Acting with a periodic pulse sequence, it is shown how the system can be steered to and largely maintained in predefined states. The conditions for this nonequilibrium sustainability are worked out by means of geometric phases, which are identified as the appropriate quantities to indicate quasistationarity of periodically driven quantum systems. Demonstrations are presented for the control of the charge, spin, and valley degrees of freedom in nanostructures on picosecond and subpicosecond time scales. The theory is illustrated with several applications to one-dimensional semiconductor quantum wires and superlattices, double quantum dots, semiconductor and graphene quantum rings. In the case of a periodic pulsed driving the influence of the relaxation and decoherence processes is included by utilizing the density matrix approach. The integrated and time-dependent spectra of the light emitted from the driven system deliver
Ando, Shinji; Harris, Robin K.; Reinsberg, Stefan A.
1999-11-01
The phenomenological theory of spin thermodynamics based on the spin temperature hypothesis was employed to describe the cross-polarization (CP) dynamics between two abundant nuclei, 19F and 1H, when the number of fluorine atoms is not substantially less than the number of hydrogens. The influence of T1ρ's of both nuclei and the relative magnitude (heat capacity) of the two spin baths must be incorporated explicitly into the analysis in order to derive values for the parameters involved in the CP dynamics. Numerical calculations were performed to clarify the difference in the evolution of magnetization in variable contact time CP experiments between the 1H → 13C and 1H → 19F cases. A new type of CP-drain experiment was developed for observing the residual 1H magnetization after 1H → 19F CP. 19F direct polarization magic-angle spinning (MAS), 1H → 19F CP, and 1H → 19F CP-drain MAS NMR spectra have been measured for a fluorinated polyimide, 6FDA/ODA. The CP dynamics between 1H and 19F for the polyimide were analyzed on the basis of the spin thermodynamics theory. The constant for polarization transfer (THF) was determined by the analysis using the effective CP parameters, which were directly obtained from the CP and CP-drain experiments, together with independently measured values of TH1ρ and TF1ρ.
Temperature effects on the dynamics of the 1-D transverse Ising model with four-spin interactions
Florencio, J.; de Alcantara Bonfim, O. F.
2004-12-01
The dynamics of one-dimensional quantum spin systems has been a long standing theoretical and experimental problem. Among them, the transverse Ising model with multi-spin interactions, regarded as one of the simplest with non-trivial dynamics, has attracted considerable interest in recent years. We investigate the temperature effects on the dynamics of the transverse Ising model with four-spin interactions. The model is relevant to the physics of poly(vinylidene fluoride-trifluoroethylene)[P(VDF-TrFE)] copolymers. We determine the time-dependent correlation function and spectral density for all temperatures for cases where the transverse field B is less, equal or greater than the four-spin coupling J. Our calculations were done with rings of up to 11 spins. However the results presented are also valid in the thermodynamic limit. We find that the time-dependent correlation function in general has oscillatory behavior when the transverse field is stronger than the coupling energy. On the other hand, when the field is weaker the real part of the time-dependent correlation function decreases monotonically at high enough temperatures. The temperature effects are best seen from the spectral density: at zero temperature the system can only absorb energy and, as the temperature is raised, the correlation functions keep memory of the zero-temperature quantum phases. Such feature persists up to the infinite temperature limit.
Longitudinal Susceptibility of S = 1/2 Low-Dimensional Heisenberg Ferromagnet in a Magnetic Field
Institute of Scientific and Technical Information of China (English)
CHEN Yuan; XIANG Ying; HU Ai-Yuan
2008-01-01
Longitudinal susceptibility of the spin-1/2 low-dimensional Heisenberg ferromagnet in a magnetic field, is studied by the Green's function method within the random phase approximation. The static and dynamic longitudinal susceptibilities are calculated in the low- and high-field regions. Power laws for the position and height of the static susceptibility maximum are shown not to support the predictions of Landau theory.
Energy Technology Data Exchange (ETDEWEB)
Rojas, D.P., E-mail: d.rojas@upm.es [Departamento de Fisica e Instalaciones-ETSAM, Universidad Politecnica de Madrid, Av. Juan Herrera, 4. 28040 Madrid (Spain); Fernandez Barquin, L.; Gonzalez Legarreta, L. [CITIMAC and MAGMA, Unidad Asociada-CSIC, Facultad de Ciencias, Universidad de Cantabria, Av. de los Castros s/n.39005 Santander (Spain); Chaboy, J.; Piquer, C. [ICMA and Departamento de Fisica de la Materia Condensada, CSIC-Universidad de Zaragoza, 50009 Zaragoza (Spain); Pedro, I. de; Rodriguez Fernandez, J. [CITIMAC and MAGMA, Unidad Asociada-CSIC, Facultad de Ciencias, Universidad de Cantabria, Av. de los Castros s/n.39005 Santander (Spain)
2013-01-15
The static and dynamic magnetic macroscopic properties of bulk and nanocrystalline TbAl{sub 1.5}Fe{sub 0.5} alloys have been investigated. In bulk state, this alloy is understood as a reentrant ferromagnet. This is characterized by a ferromagnetic Curie transition at 114 K, as deduced from magnetization including Arrott plots, higher than that of TbAl{sub 2}. The reentrance is found at lower temperatures, below 66 K, with a cluster glass behavior setting in, deduced from the magnetization irreversibility. This is accompanied by an abrupt increase in the coercivity from 0.08 kOe to 15 kOe at 5 K, with respect to the TbAl{sub 2} alloy. Room temperature Moessbauer spectroscopy confirms the paramagnetic state of such a bulk alloy. The spin dynamics within the disordered magnetic state is described by the AC-susceptibility which shows a Vogel-Fulcher law for the slowing down process. This is caused by a random anisotropy affecting the existing clusters. The production of milled TbAl{sub 1.5}Fe{sub 0.5} alloys enhances the presence of magnetic disorder and results in the particle downsizing toward the nanocrystalline state (close to 10 nm). In this case, two frequency-dependent contributions exist, with different activation energies, one of them cannot be described by ideal spin glass nor blocking/unblocking (nanoparticle) processes. In addition, the coercivity reduces to 1 kOe with the decrease in the size as a consequence of the existence of single domain particles. The results are explained by the intricate interplay between exchange interactions and magnetocrystalline anisotropy with disorder and size effects. - Highlights: Black-Right-Pointing-Pointer Bulk and nanocrystalline TbAl{sub 1.5}Fe{sub 0.5} alloys. Black-Right-Pointing-Pointer Enhancement of the magnetic properties when Fe substitutes Al in bulk TbAl{sub 2}, with a glassy behavior below 54 K. Black-Right-Pointing-Pointer AC susceptibility of nanocrystalline TbAl{sub 1.5}Fe{sub 0.5} alloys shows atypical
Control Study for Five-axis Dynamic Spin Rig Using Magnetic Bearings
Choi, Benjamin; Johnson, Dexter; Provenza, Andrew; Morrison, Carlos; Montague, Gerald
2003-01-01
The NASA Glenn Research Center (GRC) has developed a magnetic bearing system for the Dynamic Spin Rig (DSR) with a fully suspended shaft that is used to perform vibration tests of turbomachinery blades and components under spinning conditions in a vacuum. Two heteropolar radial magnetic bearings and a thrust magnetic bearing and the associated control system were integrated into the DSR to provide magnetic excitation as well as non-contact mag- netic suspension of a 15.88 kg (35 lb) vertical rotor with blades to induce turbomachinery blade vibration. For rotor levitation, a proportional-integral-derivative (PID) controller with a special feature for multidirectional radial excitation worked well to both support and shake the shaft with blades. However, more advanced controllers were developed and successfully tested to determine the optimal controller in terms of sensor and processing noise reduction, smaller rotor orbits, more blade vibration amplitude, and energy savings for the system. The test results of a variety of controllers that were demonstrated up to 10.000 rpm are shown. Furthermore, rotor excitation operation and conceptual study of active blade vibration control are addressed.
Slow spin dynamics between ferromagnetic chains in a pure-inorganic framework.
David, Rénald; Kabbour, Houria; Colis, Silviu; Mentré, Olivier
2013-12-02
The crystal structure of the new phase BaCo(II)2(As(III)3O6)2·2(H2O) is built from the stacking of infinite [BaCo2(As3O6)2·H2O] sheets containing ∞[Co(II)O4](6-) chains interconnected by perpendicular ∞[As(III)O2](-) chains. It shows a metamagnetic transition below ∼9 K at a critical field of ∼0.11 T, leading to a moment value of 70% of the expected saturation, related to the spin flip between individual robust canted ferromagnetic chains. We propose a field-dependent scenario with magnetic moments lying in the Co(II)O6 octahedral basal planes, fully compatible with our experimental results. Magnetic measurements under ac-field show slow spin dynamics with an intrinsic single-chain magnet (SCM)-like component slightly modified in the field-aligned regime. The characteristic relaxation time and energy barrier are about τo = 5.1 × 10(-10) s and Δτ = 35.3 K at H(dc) = 0, respectively, which falls close to values found for other (but organometallic) SCM Co(II) chains. This magnetic behavior is unique in the field of pure-inorganic compounds.
Spin S = 1 centers: a universal type of paramagnetic defects in nanodiamonds of dynamic synthesis
Shames, A. I.; Osipov, V. Yu; von Bardeleben, H. J.; Vul', A. Ya
2012-06-01
Intrinsic paramagnetic defects in ˜5 nm sized nanodiamonds, produced by various dynamic synthesis (DySND) techniques (detonation, shock-wave, pulsed laser ablation of solid carbon containing targets), have been studied by multi-frequency electron paramagnetic resonance (EPR). X-band (9-10 GHz) EPR spectra of DySND, in addition to the main intensive singlet Lorentzian-like EPR signal, reveal a low intensity doublet pattern within the half-field (HF) region (g ˜ 4). On transferring spectra to the Q-band (34 GHz) the shape of the HF pattern changes and splitting between doublet components is reduced from 10.4 to 2.6 mT. The HF patterns observed are attributed to the ‘forbidden’ ΔMS = 2 transitions between the Zeeman levels of some spin-triplet (S = 1) centers. The model of two triplet centers with g ˜ 2.003 and zero-field splitting parameters D1 = 0.095 cm-1 (TR1) and D2 = 0.030 cm-1 (TR2) satisfactorily describes experimental results at both microwave frequencies. The spin-triplet-type defects are observed in a wide variety of DySND samples irrespective of industrial supplier, cooling and carbon soot refinement methods, initial purity, disintegration, or subsequent targeted chemical modification. This indicates that the intrinsic defects with S = 1 in DySND systems are of universal origin.
Lattice and spin dynamics in a low-symmetry antiferromagnet NiWO4
Prosnikov, M. A.; Davydov, V. Yu.; Smirnov, A. N.; Volkov, M. P.; Pisarev, R. V.; Becker, P.; Bohatý, L.
2017-07-01
Lattice and magnetic dynamics of NiWO4 single crystals were studied with the use of polarized Raman spectroscopy in a wide temperature range of 10-300 K including the antiferromagnetic ordering temperature TN=62 K. Static magnetic measurements were used for characterizing the single crystals. All Raman-active phonons predicted by the group theory were observed and characterized. Magnetic symmetry analysis was used to determine possible magnetic space groups for NiWO4 which can be also applied to any other isostructural crystal with the same magnetic propagation vector k =(1 /2 ,0 ,0 ) . Although the magnetic structure of NiWO4 is relatively simple, a rich set of narrow and broad magnetic excitations with different polarization properties and temperature behavior in the very broad frequency range of 10-200 cm-1 was observed, with some modes surviving at temperatures much higher than TN up to 220 K. Part of the magnetic excitations were identified as acoustic and optical spin-wave branches which allowed us to construct exchange structure and estimate exchange and anisotropy constants with the use of linear spin-wave theory.
Switching dynamics of the spin density wave in superconducting CeCoIn5
Kim, Duk Y.; Lin, Shi-Zeng; Bauer, Eric D.; Ronning, Filip; Thompson, J. D.; Movshovich, Roman
2017-06-01
The ordering wave vector Q of a spin density wave (SDW), stabilized within the superconducting state of CeCoIn5 in a high magnetic field, has been shown to be hypersensitive to the direction of the field. Q can be switched from a nodal direction of the d -wave superconducting order parameter to a perpendicular node by rotating the in-plane magnetic field through the antinodal direction within a fraction of a degree. Here, we address the dynamics of the switching of Q . We use a free-energy functional based on the magnetization density, which describes the condensation of magnetic fluctuations of nodal quasiparticles, and show that the switching process includes closing of the SDW gap at one Q and then reopening the SDW gap at another Q perpendicular to the first one. The magnetic field couples to Q through the spin-orbit interaction. Our calculations show that the width of the hysteretic region of switching depends linearly on the deviation of magnetic field from the critical field associated with the SDW transition, consistent with our thermal conductivity measurements. The agreement between theory and experiment supports our scenario of the hypersensitivity of the Q phase on the direction of magnetic field, as well as the magnon condensation as the origin of the SDW phase in CeCoIn5.
Finite-temperature dynamics of the spin- (1)/(2) bond alternating Heisenberg antiferromagnetic chain
Mikeska, H. J.; Luckmann, C.
2006-05-01
We present results for the dynamic structure factor of the S=1/2 bond alternating Heisenberg chain over a large range of frequencies and temperatures. Data are obtained from a numerical evaluation of thermal averages based on the calculation of all eigenvalues and eigenfunctions for chains of up to 20 spins. Interpretation is guided by the exact temperature dependence in the noninteracting dimer limit which remains qualitatively valid up to an interdimer exchange λ≈0.5 . The temperature induced central peak around zero frequency is clearly identified and aspects of the crossover to spin diffusion in its variation from low to high temperatures are discussed. The one-magnon peak acquires an asymmetric shape with increasing temperature. The two-magnon peak is dominated by the S=1 bound state which remains well defined up to temperatures of the order of J . The variation with temperature and wave vector of the integrated intensity for one-magnon and two-magnon scattering and of the central peak are discussed.
Chiral fermion dynamics in 2d magnetic vortices: Manifestation of momentum-spin-locking
Pötz, W.; Hammer, René
2016-11-01
The electronic surface-states of a topological insulator in the presence of an in-plane magnetization vortex M (ϕ)=M (cos(Φ+νϕ), sin(Φ+νϕ)) are investigated theoretically. For a general angle of magnetization Φ∈[0 ,2 π) and topological charge ν = 1, the modifications to the zero-mass single Dirac cone dispersion are treated exactly and the spectrum of bound eigenstates which forms in the energy window ±M cos(Φ) is derived. The space-time resolved dynamics of Dirac fermions in the presence of such vortices is studied numerically using a single-cone (2 + 1)D finite-difference scheme. In the continuous spectral region, Φ-dependent scattering of Dirac fermions at the vortex is observed. Depending on the type of vortex ( Φ, ν) and the impact parameter, the propagation direction of the Dirac fermion is changed: the magnetization of the vortex exerts a torque onto the fermion spin which, by momentum-spin locking associated with the helical Dirac states, results in an in-plane rotation of the propagation direction of the scattered Dirac fermion. In head-on collisions of a Gaussian wave-packet with ν = 1 vortices a Φ-dependent lensing effect is seen in our simulations. Depending on the direction of incidence, the vortex Φ=-π/2 , ν = 2 is identified as a coherent particle-beam splitter or "condenser" in head-on collisions.
Energy Technology Data Exchange (ETDEWEB)
Furtner, J., E-mail: julia.furtner@meduniwien.ac.at [Department of Biomedical Imaging und Image-guided Therapy, Medical University of Vienna (Austria); Comprehensive Cancer Center-Central Nervous System Tumors Unit (CCC-CNS), Medical University of Vienna (Austria); Schöpf, V., E-mail: veronika.schoepf@meduniwien.ac.at [Department of Biomedical Imaging und Image-guided Therapy, Medical University of Vienna (Austria); Preusser, M., E-mail: matthias.preusser@meduniwien.ac.at [Department of Medicine I, Division of Oncology, Medical University of Vienna (Austria); Comprehensive Cancer Center-Central Nervous System Tumors Unit (CCC-CNS), Medical University of Vienna (Austria); Asenbaum, U., E-mail: ulrika.asenbaum@meduniwien.ac.at [Department of Biomedical Imaging und Image-guided Therapy, Medical University of Vienna (Austria); Woitek, R., E-mail: ramona.woitek@meduniwien.ac.at [Department of Biomedical Imaging und Image-guided Therapy, Medical University of Vienna (Austria); Wöhrer, A., E-mail: adelheid.woehrer@meduniwien.ac.at [Institute of Neurology, Medical University of Vienna (Austria); Comprehensive Cancer Center-Central Nervous System Tumors Unit (CCC-CNS), Medical University of Vienna (Austria); Hainfellner, J.A., E-mail: johannes.hainfellner@meduniwien.ac.at [Institute of Neurology, Medical University of Vienna (Austria); Comprehensive Cancer Center-Central Nervous System Tumors Unit (CCC-CNS), Medical University of Vienna (Austria); Wolfsberger, S., E-mail: stefan.wolfsberger@meduniwien.ac.at [Department of Neurosurgery, Medical University of Vienna (Austria); Comprehensive Cancer Center-Central Nervous System Tumors Unit (CCC-CNS), Medical University of Vienna (Austria); Prayer, D., E-mail: daniela.prayer@meduniwien.ac.at [Department of Biomedical Imaging und Image-guided Therapy, Medical University of Vienna (Austria); Comprehensive Cancer Center-Central Nervous System Tumors Unit (CCC-CNS), Medical University of Vienna (Austria)
2014-05-15
Using conventional MRI methods, the differentiation of primary cerebral lymphomas (PCNSL) and other primary brain tumors, such as glioblastomas, is difficult due to overlapping imaging characteristics. This study was designed to discriminate tumor entities using normalized vascular intratumoral signal intensity values (nVITS) obtained from pulsed arterial spin labeling (PASL), combined with intratumoral susceptibility signals (ITSS) from susceptibility-weighted imaging (SWI). Thirty consecutive patients with glioblastoma (n = 22) and PCNSL (n = 8), histologically classified according to the WHO brain tumor classification, were included. MRIs were acquired on a 3 T scanner, and included PASL and SWI sequences. nVITS was defined by the signal intensity ratio between the tumor and the contralateral normal brain tissue, as obtained by PASL images. ITSS was determined as intratumoral low signal intensity structures detected on SWI sequences and were divided into four different grades. Potential differences in the nVITS and ITSS between glioblastomas and PCNSLs were revealed using statistical testing. To determine sensitivity, specificity, and diagnostic accuracy, as well as an optimum cut-off value for the differentiation of PCNSL and glioblastoma, a receiver operating characteristic analysis was used. We found that nVITS (p = 0.011) and ITSS (p = 0.001) values were significantly higher in glioblastoma than in PCNSL. The optimal cut-off value for nVITS was 1.41 and 1.5 for ITSS, with a sensitivity, specificity, and accuracy of more than 95%. These findings indicate that nVITS values have a comparable diagnostic accuracy to ITSS values in differentiating glioblastoma and PCNSL, offering a completely non-invasive and fast assessment of tumoral vascularity in a clinical setting.
Spin dynamics modeling in the AGS based on a stepwise ray-tracing method
Energy Technology Data Exchange (ETDEWEB)
Dutheil, Yann [Univ. of Grenoble (France)
2006-08-07
The AGS provides a polarized proton beam to RHIC. The beam is accelerated in the AGS from Gγ= 4.5 to Gγ = 45.5 and the polarization transmission is critical to the RHIC spin program. In the recent years, various systems were implemented to improve the AGS polarization transmission. These upgrades include the double partial snakes configuration and the tune jumps system. However, 100% polarization transmission through the AGS acceleration cycle is not yet reached. The current efficiency of the polarization transmission is estimated to be around 85% in typical running conditions. Understanding the sources of depolarization in the AGS is critical to improve the AGS polarized proton performances. The complexity of beam and spin dynamics, which is in part due to the specialized Siberian snake magnets, drove a strong interest for original methods of simulations. For that, the Zgoubi code, capable of direct particle and spin tracking through field maps, was here used to model the AGS. A model of the AGS using the Zgoubi code was developed and interfaced with the current system through a simple command: the AgsFromSnapRampCmd. Interfacing with the machine control system allows for fast modelization using actual machine parameters. Those developments allowed the model to realistically reproduce the optics of the AGS along the acceleration ramp. Additional developments on the Zgoubi code, as well as on post-processing and pre-processing tools, granted long term multiturn beam tracking capabilities: the tracking of realistic beams along the complete AGS acceleration cycle. Beam multiturn tracking simulations in the AGS, using realistic beam and machine parameters, provided a unique insight into the mechanisms behind the evolution of the beam emittance and polarization during the acceleration cycle. Post-processing softwares were developed to allow the representation of the relevant quantities from the Zgoubi simulations data. The Zgoubi simulations proved particularly
Magnetic Order and Spin Dynamics in a Hexagonal Rare Earth Manganite
Helton, J. S.; Singh, D. K.; Elizabeth, S.; Harikrishnan, S.; Lynn, J. W.
2011-03-01
Hexagonal rare earth manganites, RMn O3 R = Dy, Ho, Er, Tm, Yb, Lu, Y, or Sc), have attracted a great deal of recent attention as magnetoelectric multiferroics as most of these systems are ferroelectric at room temperature and display magnetic order below TN ~ 100 K. This magnetic order can be quite complex, as both the R and Mn ions lie on geometrically frustrated triangular lattices. DyMn O3 is typically orthorhombic, but can also be grown in the hexagonal phase; Dy 0.5 Y0.5 Mn O3 displays the hexagonal phase and is magnetically diluted at the rare earth site. We have used neutron scattering experiments to explore the magnetic structure and spin dynamics of Dy 0.5 Y0.5 Mn O3 .
Equilibrium and Nonequilibrium Dynamics of the Sub-Ohmic Spin-Boson Model
Anders, Frithjof B.; Bulla, Ralf; Vojta, Matthias
2007-05-01
Employing the nonperturbative numerical renormalization group method, we study the dynamics of the spin-boson model, which describes a two-level system coupled to a bosonic bath with a spectral density J(ω)∝ωs. We show that, in contrast with the case of Ohmic damping, the delocalized phase of the sub-Ohmic model cannot be characterized by a single energy scale only, due to the presence of a nontrivial quantum phase transition. In the strongly sub-Ohmic regime, s≪1, weakly damped coherent oscillations on short time scales are possible even in the localized phase—this is of crucial relevance, e.g., for qubits subject to electromagnetic noise.
A Study of Particle Beam Spin Dynamics for High Precision Experiments
Energy Technology Data Exchange (ETDEWEB)
Fiedler, Andrew J. [Northern Illinois Univ., DeKalb, IL (United States)
2017-05-01
In the search for physics beyond the Standard Model, high precision experiments to measure fundamental properties of particles are an important frontier. One group of such measurements involves magnetic dipole moment (MDM) values as well as searching for an electric dipole moment (EDM), both of which could provide insights about how particles interact with their environment at the quantum level and if there are undiscovered new particles. For these types of high precision experiments, minimizing statistical uncertainties in the measurements plays a critical role. \\\\ \\indent This work leverages computer simulations to quantify the effects of statistical uncertainty for experiments investigating spin dynamics. In it, analysis of beam properties and lattice design effects on the polarization of the beam is performed. As a case study, the beam lines that will provide polarized muon beams to the Fermilab Muon \\emph{g}-2 experiment are analyzed to determine the effects of correlations between the phase space variables and the overall polarization of the muon beam.
Vortex-induced dynamic loads on a non-spinning volleyball
Qing-ding, Wei; Rong-sheng, Lin; Zhi-jie, Liu
1988-09-01
An experiment on vortex-induced dynamic loads on a non-spinning Volleyball was conducted in a wind tunnel. The flow past the Volleyball was visualized, and the aerodynamic load was measured by use of a strain gauge balance. The separation on the Volleyball was measured with hot-film. The experimental results suggest that under the action of an unstable tail vortex system the separation region is changeable, and that the fluctuation of drag and lateral forces is the same order of magnitude as the mean drag, no matter whether the seam of the Volleyball is symmetric or asymmetric, with regard to the flow. Based on the experimental data a numerical simulation of Volleyball swerve motion was made.
Electron dynamics in the carbon atom induced by spin-orbit interaction
Rey, H F
2014-01-01
We use R-Matrix theory with Time dependence (RMT) to investigate multiphoton ionization of ground-state atomic carbon with initial orbital magnetic quantum number $M_L$=0 and $M_L$=1 at a laser wavelength of 390 nm and peak intensity of 10$^{14}$ W cm$^{-2}$. Significant differences in ionization yield and ejected-electron momentum distribution are observed between the two values for $M_L$. We use our theoretical results to model how the spin-orbit interaction affects electron emission along the laser polarization axis. Under the assumption that an initial C atom is prepared at zero time delay with $M_L=0$, the dynamics with respect to time delay of an ionizing probe pulse modelled using RMT theory is found to be in good agreement with available experimental data.
Rey, H. F.; van der Hart, H. W.
2014-09-01
We use R-matrix theory with time dependence (RMT) to investigate multiphoton ionization of ground-state atomic carbon with initial orbital magnetic quantum number ML=0 and ML=1 at a laser wavelength of 390 nm and peak intensity of 1014W/cm2. Significant differences in ionization yield and ejected-electron momentum distribution are observed between the two values for ML. We use our theoretical results to model how the spin-orbit interaction affects electron emission along the laser polarization axis. Under the assumption that an initial C atom is prepared at zero time delay with ML=0, the dynamics with respect to time delay of an ionizing probe pulse modeled by using RMT theory is found to be in good agreement with available experimental data.
Energy Technology Data Exchange (ETDEWEB)
Fernández-Pacheco, A., E-mail: af457@cam.ac.uk; Mansell, R.; Petit, D.; Lee, J. H.; Cowburn, R. P. [Cavendish Laboratory, University of Cambridge, J. J. Thomson Avenue, Cambridge CB3 0HE (United Kingdom); Ummelen, F. C.; Swagten, H. J. M. [Department of Applied Physics, Center for NanoMaterials, Eindhoven University of Technology, P.O. Box 513, 5600 MB Eindhoven (Netherlands)
2014-09-01
We have designed a bilayer synthetic antiferromagnet where the order of layer reversal can be selected by varying the sweep rate of the applied magnetic field. The system is formed by two ultra-thin ferromagnetic layers with different proximities to the spin reorientation transition, coupled antiferromagnetically using Ruderman-Kittel-Kasuya-Yosida interactions. The different dynamic magnetic reversal behavior of both layers produces a crossover in their switching fields for field rates in the kOe/s range. This effect is due to the different effective anisotropy of both layers, added to an appropriate asymmetric antiferromagnetic coupling between them. Field-rate controlled selective switching of perpendicular magnetic anisotropy layers as shown here can be exploited in sensing and memory applications.
Directory of Open Access Journals (Sweden)
Lisa Teich
2015-11-01
Full Text Available The development of magnetoresistive sensors based on magnetic nanoparticles which are immersed in conductive gel matrices requires detailed information about the corresponding magnetoresistive properties in order to obtain optimal sensor sensitivities. Here, crucial parameters are the particle concentration, the viscosity of the gel matrix and the particle structure. Experimentally, it is not possible to obtain detailed information about the magnetic microstructure, i.e., orientations of the magnetic moments of the particles that define the magnetoresistive properties, however, by using numerical simulations one can study the magnetic microstructure theoretically, although this requires performing classical spin dynamics and molecular dynamics simulations simultaneously. Here, we present such an approach which allows us to calculate the orientation and the trajectory of every single magnetic nanoparticle. This enables us to study not only the static magnetic microstructure, but also the dynamics of the structuring process in the gel matrix itself. With our hybrid approach, arbitrary sensor configurations can be investigated and their magnetoresistive properties can be optimized.
Pathak, Anand; Sinha, Sitabhra
2015-09-01
Many complex systems can be represented as networks of dynamical elements whose states evolve in response to interactions with neighboring elements, noise and external stimuli. The collective behavior of such systems can exhibit remarkable ordering phenomena such as chimera order corresponding to coexistence of ordered and disordered regions. Often, the interactions in such systems can also evolve over time responding to changes in the dynamical states of the elements. Link adaptation inspired by Hebbian learning, the dominant paradigm for neuronal plasticity, has been earlier shown to result in structural balance by removing any initial frustration in a system that arises through conflicting interactions. Here we show that the rate of the adaptive dynamics for the interactions is crucial in deciding the emergence of different ordering behavior (including chimera) and frustration in networks of Ising spins. In particular, we observe that small changes in the link adaptation rate about a critical value result in the system exhibiting radically different energy landscapes, viz., smooth landscape corresponding to balanced systems seen for fast learning, and rugged landscapes corresponding to frustrated systems seen for slow learning.
Fully Suspended, Five-Axis, Three-Magnetic-Bearing Dynamic Spin Rig With Forced Excitation
Morrison, Carlos R.; Provenza, Andrew; Kurkov, Anatole; Montague, Gerald; Duffy, Kirsten; Mehmed, Oral; Johnson, Dexter; Jansen, Ralph
2004-01-01
The Five-Axis, Three-Magnetic-Bearing Dynamic Spin Rig, a significant advancement in the Dynamic Spin Rig (DSR), is used to perform vibration tests of turbomachinery blades and components under rotating and nonrotating conditions in a vacuum. The rig has as its critical components three magnetic bearings: two heteropolar radial active magnetic bearings and a magnetic thrust bearing. The bearing configuration allows full vertical rotor magnetic suspension along with a feed-forward control feature, which will enable the excitation of various natural blade modes in bladed disk test articles. The theoretical, mechanical, electrical, and electronic aspects of the rig are discussed. Also presented are the forced-excitation results of a fully levitated, rotating and nonrotating, unbladed rotor and a fully levitated, rotating and nonrotating, bladed rotor in which a pair of blades was arranged 180 degrees apart from each other. These tests include the bounce mode excitation of the rotor in which the rotor was excited at the blade natural frequency of 144 Hz. The rotor natural mode frequency of 355 Hz was discerned from the plot of acceleration versus frequency. For nonrotating blades, a blade-tip excitation amplitude of approximately 100 g/A was achieved at the first-bending critical (approximately 144 Hz) and at the first-torsional and second-bending blade modes. A blade-tip displacement of 70 mils was achieved at the first-bending critical by exciting the blades at a forced-excitation phase angle of 908 relative to the vertical plane containing the blades while simultaneously rotating the shaft at 3000 rpm.
Segmental dynamics of polyethylene-alt-propylene studied by NMR spin echo techniques
Lozovoi, A.; Mattea, C.; Hofmann, M.; Saalwaechter, K.; Fatkullin, N.; Stapf, S.
2017-06-01
Segmental dynamics of a highly entangled melt of linear polyethylene-alt-propylene with a molecular weight of 200 kDa was studied with a novel proton nuclear magnetic resonance (NMR) approach based upon 1H → 2H isotope dilution as applied to a solid-echo build-up function ISE(t), which is constructed from the NMR spin echo signals arising from the Hahn echo (HE) and two variations of the solid-echo pulse sequence. The isotope dilution enables the separation of inter- and intramolecular contributions to this function and allows one to extract the segmental mean-squared displacements in the millisecond time range, which is hardly accessible by other experimental methods. The proposed technique in combination with time-temperature superposition yields information about segmental translation in polyethylene-alt-propylene over 6 decades in time from 10-6 s up to 1 s. The time dependence of the mean-squared displacement obtained in this time range clearly shows three regimes of power law with exponents, which are in good agreement with the tube-reptation model predictions for the Rouse model, incoherent reptation and coherent reptation regimes. The results at short times coincide with the fast-field cycling relaxometry and neutron spin echo data, yet, significantly extending the probed time range. Furthermore, the obtained data are verified as well by the use of the dipolar-correlation effect on the Hahn echo, which was developed before by the co-authors. At the same time, the amplitude ratio of the intermolecular part of the proton dynamic dipole-dipole correlation function over the intramolecular part obtained from the experimental data is not in agreement with the predictions of the tube-reptation model for the regimes of incoherent and coherent reptation.
Engle, Jonathan
2013-01-01
The spin foam framework provides a way to define the dynamics of canonical loop quantum gravity in a spacetime covariant way, by using a path integral over histories of quantum states which can be interpreted as `quantum space-times'. This chapter provides a basic introduction to spin foams aimed principally at beginning graduate students and, where possible, at broader audiences.
Memory-keeping effects and forgetfulness in the dynamics of a qubit coupled to a spin chain
Apollaro, T J G; Plastina, F; Paternostro, M
2010-01-01
Using recently proposed measures for non-Markovianity [H. P. Breuer, E. M. Laine, and J. Piilo, Phys. Rev. Lett. {\\bf 103}, 210401 (2009)], we study the dynamics of a qubit coupled to a spin environment via an energy-exchange mechanism. We show the existence of a point, in the parameter space of the system, where the qubit dynamics is effectively Markovian and that such a point separates two regions with completely different dynamical behaviors. Indeed, our study demonstrates that the qubit evolution can in principle be tuned from a perfectly forgetful one to a deep non-Markovian regime where the qubit is strongly affected by the dynamical back-action of the environmental spins. By means of quantum process tomography, we provide a complete and intuitive characterization of the qubit channel.
Wei, Hongjiang; Dibb, Russell; Zhou, Yan; Sun, Yawen; Xu, Jianrong; Wang, Nian; Liu, Chunlei
2015-01-01
Quantitative susceptibility mapping (QSM) is a novel MRI technique for measuring tissue magnetic susceptibility in 3D. While there are numerous algorithms developed to solve this ill-posed inverse problem, estimating susceptibility maps with a wide range of values is still problematic. In cases such as large veins, contrast agent uptake, and intracranial hemorrhages, extreme susceptibility values in focal areas cause severe streaking artifacts. To enable the reduction of these artifacts while preserving subtle susceptibility contrast, a two-level QSM reconstruction algorithm (STAR-QSM) was developed in this study by tuning a regularization parameter to automatically reconstruct both large and small susceptibility values. Compared to current state-of-the-art QSM methods such as iLSQR, STAR-QSM significantly reduced streaking artifacts while preserving sharp boundaries for blood vessels of mouse brains in vivo and fine anatomical details of high resolution mouse brains ex vivo. Brain image data from patients with cerebral hematoma and multiple sclerosis further illustrated the superiority of this method in reducing streaking artifacts caused by large susceptibility sources while maintaining sharp anatomical details. STAR-QSM is implemented in STI Suite, a comprehensive shareware for susceptibility imaging and quantification. PMID:26313885
Energy Technology Data Exchange (ETDEWEB)
Kostylev, M. [School of Physics, M013, University of Western Australia, Crawley, Perth 6009, Western Australia (Australia)
2014-06-21
In this work, we derive the interface exchange boundary conditions for the classical linear dynamics of magnetization in ferromagnetic layers with the interface Dzyaloshinskii-Moriya interaction (IDMI). We show that IDMI leads to pinning of dynamic magnetization at the interface. An unusual peculiarity of the IDMI-based pinning is that its scales as the spin-wave wave number. We incorporate these boundary conditions into an existing numerical model for the dynamics of the Damon-Eshbach spin wave in ferromagnetic films. IDMI affects the dispersion and the frequency non-reciprocity of the travelling Damon-Eshbach spin wave. For a broad range of film thicknesses L and wave numbers, the results of the numerical simulations of the spin wave dispersion are in a good agreement with a simple analytical expression, which shows that the contribution of IDMI to the dispersion scales as 1/L, similarly to the effect of other types of interfacial anisotropy. Suggestions to experimentalists how to detect the presence of IDMI in a spin wave experiment are given.
Coherent spin dynamics of an interwell excitonic gas in GaAs/AlGaAs coupled quantum wells
DEFF Research Database (Denmark)
Larionov, A. V.; Bisti, V. E.; Bayer, M.;
2006-01-01
The spin dynamics of an interwell exciton gas has been investigated in n-i-n GaAs/AlGaAs coupled quantum wells. The time evolution kinetics of the interwell exciton photoluminescence has been measured under resonant excitation of the 1s heavy-hole intrawell exciton, using a pulsed tunable laser...
Fuson, Michael M.
2017-01-01
Laboratories studying the anisotropic rotational diffusion of bromobenzene using nuclear spin relaxation and molecular dynamics simulations are described. For many undergraduates, visualizing molecular motion is challenging. Undergraduates rarely encounter laboratories that directly assess molecular motion, and so the concept remains an…
Spin-flip dynamics of the Curie-Weiss model : Loss of Gibbsianness with possibly broken symmetry
Kulske, Christof; Le Ny, Arnaud
2007-01-01
We study the conditional probabilities of the Curie-Weiss Ising model in vanishing external field under a symmetric independent stochastic spin-flip dynamics and discuss their set of points of discontinuity (bad points). We exhibit a complete analysis of the transition between Gibbsian and non-Gibbs
Energy Technology Data Exchange (ETDEWEB)
Boukheddaden, Kamel, E-mail: kbo@physique.uvsq.fr [GEMaC, Université de Versailles St-Quentin, 45 Avenue des Etats Unis, 78035 Versailles (France); Sy, Mouhamadou; Paez-Espejo, Miguel [GEMaC, Université de Versailles St-Quentin, 45 Avenue des Etats Unis, 78035 Versailles (France); Slimani, Ahmed [Laboratoire des matériaux ferroélectriques, Département de Physique, Faculté des Sciences de Sfax, Route de la Soukra km 3.5 BP 1171, 3018 Sfax (Tunisia); Varret, François [GEMaC, Université de Versailles St-Quentin, 45 Avenue des Etats Unis, 78035 Versailles (France)
2016-04-01
We have succeeded to achieve experimentally, using an adapted optical microscopy setup, the reversible control of the front transformation between the low-spin (LS)–high-spin (HS) interface in the spin-crossover (SC) single crystal [{Fe(NCSe)(py)_2}{sub 2}(m-bpypz)] undergoing a first-order transition at 112 K with a 7 K hysteresis width. For that, we first generate a phase separation state (a HS/LS interface at equilibrium) inside the hysteresis loop by tuning the light intensity of the microscope. In the second step, this intensity is monitored in such a way to drive, through a photo-heating process, the interface motion. This photo-control is found to be reversible, accurate and requiring a very small amount of energy. In addition the integrity of the crystal is maintained even after a large number of cycling. The experimental observations, are well described as a reaction diffusion process accounting for the front propagation and the photo-heating effects.
The dynamic compensation temperature in a kinetic spin-5/2 Ising model on a hexagonal lattice
Institute of Scientific and Technical Information of China (English)
(U)müt Temizer; Ay(s)egül (O)zkili(c)
2013-01-01
We present a study of the dynamic behavior of a two-sublattice spin-5/2 Ising model with bilinear and crystal-field interactions in the presence of a time-dependent oscillating external magnetic field on alternating layers of a hexagonal lattice by using the Glauber-type stochastic dynamics.The lattice is formed by alternate layers of spins σ =5/2 and S =5/2.We employ the Glauber transition rates to construct the mean-field dynamic equations.First,we investigate the time variations of the average sublattice magnetizations to find the phases in the system and then the thermal behavior of the dynamic sublattice magnetizations to characterize the nature (first-or second-order) of the phase transitions and to obtain the dynamic phase transition (DPT) points.We also study the thermal behavior of the dynamic total magnetization to find the dynamic compensation temperature and to determine the type of the dynamic compensation behavior.We present the dynamic phase diagrams,including the dynamic compensation temperatures,in nine different planes.The phase diagrams contain seven different fundamental phases,thirteen different mixed phases,in which the binary and ternary combination of fundamental phases and the compensation temperature or the L-type behavior strongly depend on the interaction parameters.
Cichy, K; Garcia-Ramos, E; Jansen, K
2011-01-01
We study the 'spectral projector' method for the computation of the chiral condensate and the topological susceptibility, using $N_f=2+1+1$ dynamical flavors of maximally twisted mass Wilson fermions. In particular, we perform a study of the quark mass dependence of the chiral condensate $\\Sigma$ and topological susceptibility $\\chi_{top}$ in the range $270 MeV < m_{\\pi} < 500 MeV$ and compare our data with analytical predictions. In addition, we compute $\\chi_{top} in the quenched approximation where we match the lattice spacing to the $N_f=2+1+1$ dynamical simulations. Using the Kaon, $\\eta$ and $\\eta^{\\prime}$ meson masses computed on the $N_f=2+1+1$ ensembles, we then perform a preliminary test of the Witten-Veneziano relation.
Energy Technology Data Exchange (ETDEWEB)
Radu, I.E.
2006-03-15
This thesis presents the femtosecond laser-induced electron, lattice and spin dynamics on two representative rare-earth systems: The ferromagnetic gadolinium Gd(0001) and the paramagnetic yttrium Y(0001) metals. The employed investigation tools are the time-resolved linear reflectivity and second-harmonic generation, which provide complementary information about the bulk and surface/interface dynamics, respectively. The femtosecond laser excitation of the exchange-split surface state of Gd(0001) triggers simultaneously the coherent vibrational dynamics of the lattice and spin subsystems in the surface region at a frequency of 3 THz. The coherent optical phonon corresponds to the vibration of the topmost atomic layer against the underlying bulk along the normal direction to the surface. The coupling mechanism between phonons and magnons is attributed to the modulation of the exchange interaction J between neighbour atoms due to the coherent lattice vibration. This leads to an oscillatory motion of the magnetic moments having the same frequency as the lattice vibration. Thus these results reveal a new type of phonon-magnon coupling mediated by the modulation of the exchange interaction and not by the conventional spin-orbit interaction. Moreover, we show that coherent spin dynamics in the THz frequency domain is achievable, which is at least one order of magnitude faster than previously reported. The laser-induced (de)magnetization dynamics of the ferromagnetic Gd(0001) thin films have been studied. Upon photo-excitation, the nonlinear magneto-optics measurements performed in this work show a sudden drop in the spin polarization of the surface state by more than 50% in a <100 fs time interval. Under comparable experimental conditions, the time-resolved photoemission studies reveal a constant exchange splitting of the surface state. The ultrafast decrease of spin polarization can be explained by the quasi-elastic spin-flip scattering of the hot electrons among spin
Energy Technology Data Exchange (ETDEWEB)
Griesbeck, Michael
2012-11-22
Since many years there has been great effort to explore the spin dynamics in low-dimensional electron systems embedded in GaAs/AlGaAs based heterostructures for the purpose of quantum computation and spintronics applications. Advances in technology allow for the design of high quality and well-defined two-dimensional electron systems (2DES), which are perfectly suited for the study of the underlying physics that govern the dynamics of the electron spin system. In this work, spin dynamics in high-mobility 2DES is studied by means of the all-optical time-resolved Kerr/Faraday rotation technique. In (001)-grown 2DES, a strong in-plane spin dephasing anisotropy is studied, resulting from the interference of comparable Rashba and Dresselhaus contributions to the spin-orbit field (SOF). The dependence of this anisotropy on parameters like the confinement length of the 2DES, the sample temperature, as well as the electron density is demonstrated. Furthermore, coherent spin dynamics of an ensemble of ballistically moving electrons is studied without and within an applied weak magnetic field perpendicular to the sample plane, which forces the electrons to move on cyclotron orbits. Finally, strongly anisotropic spin dynamics is investigated in symmetric (110)-grown 2DES, using the resonant spin amplification method. Here, extremely long out-of-plane spin dephasing times can be achieved, in consequence of the special symmetry of the Dresselhaus SOF.
Tanamoto, Tetsufumi; Ono, Keiji; Liu, Yu-xi; Nori, Franco
2015-06-17
Hamiltonian engineering is an important approach for quantum information processing, when appropriate materials do not exist in nature or are unstable. So far there is no stable material for the Kitaev spin Hamiltonian with anisotropic interactions on a honeycomb lattice, which plays a crucial role in the realization of both Abelian and non-Abelian anyons. Here, we show two methods to dynamically realize the Kitaev spin Hamiltonian from the conventional Heisenberg spin Hamiltonian using pulse-control techniques based on the Baker-Campbell-Hausdorff (BCH) formula. In the first method, the Heisenberg interaction is changed into Ising interactions in the first process of the pulse sequence. In the next process of the first method, we transform them to a desirable anisotropic Kitaev spin Hamiltonian. In the second more efficient method, we show that if we carefully design two-dimensional pulses that vary depending on the qubit location, we can obtain the desired Hamiltonian in only one step of applying the BCH formula. As an example, we apply our methods to spin qubits based on quantum dots, in which the effects of both the spin-orbit interaction and the hyperfine interaction are estimated.
Tsuchimoto, Masashi; Tanimura, Yoshitaka
2015-08-11
A system with many energy states coupled to a harmonic oscillator bath is considered. To study quantum non-Markovian system-bath dynamics numerically rigorously and nonperturbatively, we developed a computer code for the reduced hierarchy equations of motion (HEOM) for a graphics processor unit (GPU) that can treat the system as large as 4096 energy states. The code employs a Padé spectrum decomposition (PSD) for a construction of HEOM and the exponential integrators. Dynamics of a quantum spin glass system are studied by calculating the free induction decay signal for the cases of 3 × 2 to 3 × 4 triangular lattices with antiferromagnetic interactions. We found that spins relax faster at lower temperature due to transitions through a quantum coherent state, as represented by the off-diagonal elements of the reduced density matrix, while it has been known that the spins relax slower due to suppression of thermal activation in a classical case. The decay of the spins are qualitatively similar regardless of the lattice sizes. The pathway of spin relaxation is analyzed under a sudden temperature drop condition. The Compute Unified Device Architecture (CUDA) based source code used in the present calculations is provided as Supporting Information .
Energy Technology Data Exchange (ETDEWEB)
Friemel, Gerd
2014-05-26
This thesis contains a comprehensive study of the spin excitations by inelastic neutron scattering (INS) in two different correlated electron systems: the alkali-metal iron selenide superconductors (FeSe122) A{sub x}Fe{sub 2-y}Se{sub 2} (A=K, Rb, Cs) and the heavy-fermion antiferromagnet CeB6. Both systems exhibit intense modes in their spin-fluctuation spectrum below their respective transition temperatures that can be derived from the spin dynamics of the itinerant quasiparticles. However, the implications of these observations, presented here, are different for each particular compound. The A{sub x}Fe{sub 2-y}Se{sub 2} superconductors, with a uniform T{sub c} of 32 K, belong to a qualitative new family of superconductors. They possess a distinctly different Fermi surface compared to the iron-arsenide-based analogues XFe{sub 2}As{sub 2} (X=Ca, Sr, Ba). Instead of the central hole pockets at Γ and the electron pockets at X((1)/(2) 0), which are nested by the Q{sub AFM} = ((1)/(2) 0) vector, there exist only large electron pockets at the X point. Therefore, the magnetic instability along Q{sub AFM} that presumably provides the pairing glue for the superconductivity in the shape of spin fluctuations is absent in the FeSe122. The search for spin fluctuations by INS was motivated by a theoretical analysis that predicted their presence at an incommensurate wave vector near Q = (0.5 δ), δ = 0.3125 which results from a quasinesting by Q between the flat parts of the electron pockets. Two samples, namely Rb{sub 0.8}Fe{sub 1.6}Se{sub 2} and K{sub 0.77}Fe{sub 1.85}Se{sub 2}, were prepared and both showed a sizable anisotropic magnetic response at Q{sub sf} = ((1)/(2) (1)/(4)) in the normal state. Furthermore, upon entering the superconducting (SC) state a strong excitation appears at ℎω{sub res} = 14 meV in the spectrum at Q{sub sf}, which is referred to as magnetic resonant mode. This mode is interpreted as a bound spin-1 exciton below the SC charge gap. Its presence
Energy Technology Data Exchange (ETDEWEB)
Bourges, Ph
2003-07-01
This work is dedicated to the detailed investigations of the magnetic resonance peak in the superconducting state of cuprates. The existence of such a peak could be the signature of a mechanism linked to magnetism that could explain high critical temperature superconductivity. Inelastic neutron scattering is an adequate tool for the understanding of cuprate properties because it reveals magnetic fluctuations whose behaviour and variety depend strongly on temperature and on the level of doping. The last part of this work is dedicated to the study of spin dynamics in YBa{sub 2}Cu{sub 3}O{sub 6+x} system.
Keatley, Paul Steven; Redjai Sani, Sohrab; Hrkac, Gino; Majid Mohseni, Seyed; Dürrenfeld, Philipp; Åkerman, Johan; Hicken, Robert James
2017-04-01
Nano-contact spin-torque vortex oscillators (STVOs) are anticipated to find application as nanoscale sources of microwave emission in future technological applications. Presently the output power and phase stability of individual STVOs are not competitive with existing oscillator technologies. Synchronisation of multiple nano-contact STVOs via magnetisation dynamics has been proposed to enhance the microwave emission. The control of device-to-device variations, such as mode splitting of the microwave emission, is essential if multiple STVOs are to be successfully synchronised. In this work a combination of electrical measurements and time-resolved scanning Kerr microscopy (TRSKM) was used to demonstrate how mode splitting in the microwave emission of STVOs was related to the magnetisation dynamics that are generated. The free-running STVO response to a DC current only was used to identify devices and bias magnetic field configurations for which single and multiple modes of microwave emission were observed. Stroboscopic Kerr images were acquired by injecting a small amplitude RF current to phase lock the free-running STVO response. The images showed that the magnetisation dynamics of a multimode device with moderate splitting could be controlled by the injected RF current so that they exhibit similar spatial character to that of a single mode. Significant splitting was found to result from a complicated equilibrium magnetic state that was observed in Kerr images as irregular spatial characteristics of the magnetisation dynamics. Such dynamics were observed far from the nano-contact and so their presence cannot be detected in electrical measurements. This work demonstrates that TRSKM is a powerful tool for the direct observation of the magnetisation dynamics generated by STVOs that exhibit complicated microwave emission. Characterisation of such dynamics outside the nano-contact perimeter permits a deeper insight into the requirements for optimal phase-locking of
Spin dynamics of complex oxides, bismuth-antimony alloys, and bismuth chalcogenides
Sahin, Cuneyt
The emerging field of spintronics relies on the manipulation of electron spin in order to use it in spin-based electronics. Such a paradigm change has to tackle several challenges including finding materials with sufficiently long spin lifetimes and materials which are efficient in generating pure spin currents. This thesis predicts that two types of material families could be a solution to the aforementioned challenges: complex oxides and bismuth based materials. We derived a general approach for constructing an effective spin-orbit Hamiltonian which is applicable to all nonmagnetic materials. This formalism is useful for calculating spin-dependent properties near an arbitrary point in momentum space. We also verified this formalism through comparisons with other approaches for III-V semiconductors, and its general applicability is illustrated by deriving the spin-orbit interaction and predicting spin lifetimes for strained strontium titanate (STO) and a two-dimensional electron gas in STO (such as at the LAO/STO interface). Our results suggest robust spin coherence and spin transport properties in STO related materials even at room temperature. In the second part of the study we calculated intrinsic spin Hall conductivities for bismuth-antimony (BISb) semimetals with strong spin-orbit couplings, from the Kubo formula and using Berry curvatures evaluated throughout the Brillouin zone from a tight-binding Hamiltonian. Nearly crossing bands with strong spin-orbit interaction generate giant spin Hall conductivities in these materials, ranging from 474 ((h/e)O--1cm--1) for bismuth to 96((h/e)O--1cm --1) for antimony; the value for bismuth is more than twice that of platinum. The large spin Hall conductivities persist for alloy compositions corresponding to a three-dimensional topological insulator state, such as Bi0.83Sb0.17. The spin Hall conductivity could be changed by a factor of 5 for doped Bi, or for Bi0.83Sb0.17, by changing the chemical potential by 0.5 e
Mook, Alexander; Henk, Jürgen; Mertig, Ingrid
2016-11-01
We demonstrate theoretically that atomistic spin dynamics simulations of topological magnon insulators (TMIs) provide access to the magnon-mediated transport of both spin and heat. The TMIs, modeled by kagome ferromagnets with Dzyaloshinskii-Moriya interaction, exhibit nonzero transverse-current correlation functions from which conductivities are derived for the entire family of magnon Hall effects. Both longitudinal and transverse conductivities are studied in dependence on temperature and on an external magnetic field. A comparison between theoretical and experimental results for Cu(1,3-benzenedicarboxylate), a recently discovered TMI, is drawn.
Oganesyan, Vasily S.; Chami, Fatima; White, Gaye F.; Thomson, Andrew J.
2017-01-01
EPR studies combined with fully atomistic Molecular Dynamics (MD) simulations and an MD-EPR simulation method provide evidence for intrinsic low rotameric mobility of a nitroxyl spin label, Rn, compared to the more widely employed label MTSL (R1). Both experimental and modelling results using two structurally different sites of attachment to Myoglobin show that the EPR spectra of Rn are more sensitive to the local protein environment than that of MTSL. This study reveals the potential of using the Rn spin label as a reporter of protein motions.
Spin-lattice coupling induced weak dynamical magnetism in EuTiO3 at high temperatures
Guguchia, Z.; Keller, H.; Kremer, R. K.; Köhler, J.; Luetkens, H.; Goko, T.; Amato, A.; Bussmann-Holder, A.
2014-08-01
EuTiO3, which is a G-type antiferromagnet below TN=5.5 K, has some fascinating properties at high temperatures, suggesting that macroscopically hidden dynamically fluctuating weak magnetism exists at high temperatures. This conjecture is substantiated by magnetic field dependent magnetization measurements, which exhibit pronounced anomalies below 200 K becoming more distinctive with increasing magnetic field strength. Additional results from muon spin rotation experiments provide evidence for weak fluctuating bulk magnetism induced by spin-lattice coupling which is strongly supported in increasing magnetic field.
High dynamic range magnetometry with a single nuclear spin in diamond
Energy Technology Data Exchange (ETDEWEB)
Waldherr, Gerald; Beck, Johannes; Neumann, Philipp; Nitsche, Matthias; Wrachtrup, Joerg [3. Physikalisches Institut, Universitaet Stuttgart, 70569 Stuttgart (Germany); Said, Ressa S. [Institut fuer Quanten-Informationsverarbeitung, Universitaet Ulm, 89081 Ulm (Germany); Twamley, Jason [Centre for Engineered Quantum Systems, Faculty of Science, Macquarie University, Sydney (Australia); Jelezko, Fedor [Institut fuer Quantenoptik, Universitaet Ulm, 89073 Ulm (Germany)
2012-07-01
Sensors based on the nitrogen-vacancy (NV) defect in diamond are being developed to measure weak magnetic and electric fields at nanoscale. However, such sensors rely on measurements of a shift in the Lamor frequency of the defect, so an accumulation of quantum phase causes the measurement signal to exhibit a periodic modulation. This means that the measurement time is either restricted to half of one oscillation period, which limits accuracy, or that the magnetic field range must be known in advance. Moreover, the precision increases only slowly, as T{sup -0.5}, with the measurement time T. We implement a quantum phase estimation algorithm on a single nuclear spin in diamond to combine both high sensitivity and high dynamic range. By achieving a scaling of the precision with time to T{sup -0.85}, we improve the sensitivity by a factor of 7.4, for an accessible field range of 16 mT, or alternatively, we improve the dynamic range by a factor of 130 for a sensitivity of 2.5 {mu}T/Hz{sup 0.5}. These methods are applicable to a variety of field detection schemes, and do not require entanglement.
Energy Technology Data Exchange (ETDEWEB)
Ma, Q. L., E-mail: maqinli@gmail.com, E-mail: mizukami@wpi-aimr.tohoku.ac.jp; Miyazaki, T.; Mizukami, S., E-mail: maqinli@gmail.com, E-mail: mizukami@wpi-aimr.tohoku.ac.jp [WPI Advanced Institute for Materials Research, Tohoku University, 2-1-1, Katahira, 980-8577 Sendai (Japan); Iihama, S. [Department of Applied Physics, Tohoku University, 6-6-05 Aza-Aoba, Aramaki, Aoba-ku, Sendai 980-8579 (Japan); Zhang, X. M. [Key Laboratory for Anisotropy and Texture of Materials, Ministry of Education, Northeastern University, Shenyang 110819 (China)
2015-11-30
The laser-induced spin dynamics of FeCo in perpendicularly magnetized L1{sub 0}-MnGa/FeCo bilayers with ferromagnetic and antiferromagnetic interfacial exchange coupling (IEC) are examined using the time-resolved magneto-optical Kerr effect. We found a precessional phase reversal of the FeCo layer as the IEC changes from ferromagnetic to antiferromagnetic. Moreover, a precession-suspension window was observed when the magnetic field was applied in a certain direction for the bilayer with ferromagnetic IEC. Our observations reveal that the spin dynamics modulation is strongly dependent on the IEC type within the Landau-Lifshitz-Gilbert depiction. The IEC dependence of the precessional phase and amplitude suggests the interesting method for magnetization dynamics modulation.
Liu, Ho-Ling; Chang, Ting-Ting; Yan, Feng-Xian; Li, Cheng-He; Lin, Yu-Shi; Wong, Alex M
2015-06-01
The forward volumetric transfer constant (K(trans)), a physiological parameter extracted from dynamic contrast-enhanced (DCE) MRI, is weighted by vessel permeability and tissue blood flow. The permeability × surface area product per unit mass of tissue (PS) in brain tumors was estimated in this study by combining the blood flow obtained through pseudo-continuous arterial spin labeling (PCASL) and K(trans) obtained through DCE MRI. An analytical analysis and a numerical simulation were conducted to understand how errors in the flow and K(trans) estimates would propagate to the resulting PS. Fourteen pediatric patients with brain tumors were scanned on a clinical 3-T MRI scanner. PCASL perfusion imaging was performed using a three-dimensional (3D) fast-spin-echo readout module to determine blood flow. DCE imaging was performed using a 3D spoiled gradient-echo sequence, and the K(trans) map was obtained with the extended Tofts model. The numerical analysis demonstrated that the uncertainty of PS was predominantly dependent on that of K(trans) and was relatively insensitive to the flow. The average PS values of the whole tumors ranged from 0.006 to 0.217 min(-1), with a mean of 0.050 min(-1) among the patients. The mean K(trans) value was 18% lower than the PS value, with a maximum discrepancy of 25%. When the parametric maps were compared on a voxel-by-voxel basis, the discrepancies between PS and K(trans) appeared to be heterogeneous within the tumors. The PS values could be more than two-fold higher than the K(trans) values for voxels with high K(trans) levels. This study proposes a method that is easy to implement in clinical practice and has the potential to improve the quantification of the microvascular properties of brain tumors.
Spin reorientation transition process in single crystal NdFeO3
Song, Gaibei; Jiang, Junjie; Kang, Baojuan; Zhang, Jincang; Cheng, Zhenxiang; Ma, Guohong; Cao, Shixun
2015-06-01
The spin reorientation transition in single crystal NdFeO3 is studied using AC magnetic susceptibility, hysteresis loops, and polarized terahertz (THz) time domain spectroscopy measurements. Different frequency dependence behaviors of AC susceptibility reflect that the dynamic response of magnetization inside the spin reorientation region differs from the phase outside the transition region. The magnetization hysteresis loops at different temperatures reveal that domains formed during the spin reorientation process, which coincides with the abrupt increase of AC magnetic susceptibility during the transition. In addition, temperature dependent THz wave excitation of quasi-antiferromagnetic mode indicates the process of spin reorientation as a continuous rotation of Fe3+ spins rather than a mixed phase of Γ4 and Γ2.
Quantum spin dynamics with pairwise-tunable, long-range interactions
Hung, C.-L.; González-Tudela, Alejandro; Cirac, J. Ignacio; Kimble, H. J.
2016-08-01
We present a platform for the simulation of quantum magnetism with full control of interactions between pairs of spins at arbitrary distances in 1D and 2D lattices. In our scheme, two internal atomic states represent a pseudospin for atoms trapped within a photonic crystal waveguide (PCW). With the atomic transition frequency aligned inside a band gap of the PCW, virtual photons mediate coherent spin-spin interactions between lattice sites. To obtain full control of interaction coefficients at arbitrary atom-atom separations, ground-state energy shifts are introduced as a function of distance across the PCW. In conjunction with auxiliary pump fields, spin-exchange versus atom-atom separation can be engineered with arbitrary magnitude and phase, and arranged to introduce nontrivial Berry phases in the spin lattice, thus opening new avenues for realizing topological spin models. We illustrate the broad applicability of our scheme by explicit construction for several well-known spin models.
Henriet, Loïc; Sclocchi, Antonio; Orth, Peter P.; Le Hur, Karyn
2017-02-01
We analyze the topological deformations of the ground state manifold of a quantum spin-1/2 in a magnetic field H =H (sinθ cosϕ ,sinθ sinϕ ,cosθ ) induced by a coupling to an ohmic quantum dissipative environment at zero temperature. From Bethe ansatz results and a variational approach, we confirm that the Chern number associated with the geometry of the reduced spin ground state manifold is preserved in the delocalized phase for α <1 . We report a divergence of the Berry curvature at αc=1 for magnetic fields aligned along the equator θ =π /2 . This divergence is caused by the complete quenching of the transverse magnetic field by the bath associated with a gap closing that occurs at the localization Kosterlitz-Thouless quantum phase transition in this model. Recent experiments in quantum circuits have engineered nonequilibrium protocols to access topological properties from a measurement of a dynamical Chern number defined via the out-of-equilibrium spin expectation values. Applying a numerically exact stochastic Schrödinger approach we find that, for a fixed field sweep velocity θ (t )=v t , the bath induces a crossover from (quasi)adiabatic to nonadiabatic dynamical behavior when the spin bath coupling α increases. We also investigate the particular regime H /ωc≪v /H ≪1 with large bath cutoff frequency ωc, where the dynamical Chern number vanishes already at α =1 /2 . In this regime, the mapping to an interacting resonance level model enables us to analytically describe the behavior of the dynamical Chern number in the vicinity of α =1 /2 . We further provide an intuitive physical explanation of the bath-induced breakdown of adiabaticity in analogy to the Faraday effect in electromagnetism. We demonstrate that the driving of the spin leads to the production of a large number of bosonic excitations in the bath, which strongly affect the spin dynamics. Finally, we quantify the spin-bath entanglement and formulate an analogy with an effective
Thurber, Kent R; Tycko, Robert
2012-08-28
We present theoretical calculations of dynamic nuclear polarization (DNP) due to the cross effect in nuclear magnetic resonance under magic-angle spinning (MAS). Using a three-spin model (two electrons and one nucleus), cross effect DNP with MAS for electron spins with a large g-anisotropy can be seen as a series of spin transitions at avoided crossings of the energy levels, with varying degrees of adiabaticity. If the electron spin-lattice relaxation time T(1e) is large relative to the MAS rotation period, the cross effect can happen as two separate events: (i) partial saturation of one electron spin by the applied microwaves as one electron spin resonance (ESR) frequency crosses the microwave frequency and (ii) flip of all three spins, when the difference of the two ESR frequencies crosses the nuclear frequency, which transfers polarization to the nuclear spin if the two electron spins have different polarizations. In addition, adiabatic level crossings at which the two ESR frequencies become equal serve to maintain non-uniform saturation across the ESR line. We present analytical results based on the Landau-Zener theory of adiabatic transitions, as well as numerical quantum mechanical calculations for the evolution of the time-dependent three-spin system. These calculations provide insight into the dependence of cross effect DNP on various experimental parameters, including MAS frequency, microwave field strength, spin relaxation rates, hyperfine and electron-electron dipole coupling strengths, and the nature of the biradical dopants.
Solvent effect on librational dynamics of spin-labelled haemoglobin by ED- and CW-EPR.
Scarpelli, Francesco; Bartucci, Rosa; Sportelli, Luigi; Guzzi, Rita
2011-03-01
Two-pulse, echo-detected electron paramagnetic resonance (ED-EPR) spectra and continuous-wave EPR (CW-EPR) spectra were used to investigate the solvent effect on the librational motion of human haemoglobin spin-labelled on cysteine β93 with the nitroxide derivative of maleimide, 6-MSL. Protein samples fully hydrated in phosphate buffer solution (PBS), in a 60% v/v glycerol/water mixture and in the lyophilized form were measured at cryogenic temperature in the frozen state. The protein librational motion was characterized by the amplitude-correlation time product, τ(c), deduced from the ED-EPR spectra. The librational amplitude, τ(c), was determined independently, from the motionally averaged hyperfine splitting in the CW-EPR spectra, and the librational correlation time, τ(c), was derived from the combination of the pulsed and conventional EPR data. Rapid librational motion of small amplitude was detected in all samples. In each case, the librational dynamics was restricted up to 180 K, beyond which it increased steeply for the hydrated protein in PBS and in the presence of glycerol. In contrast, in the dehydrated protein, the librational dynamics was hindered and less dependent on temperature up to ~240 K. In all samples, deviated from small values only for T > 200 K, where a rapid increase of was evident for the hydrated samples, whereas limited temperature variation was shown in the lyophilized samples. The librational correlation time was in the sub-nanosecond regime and weakly dependent on temperature. The results evidence that solvent favours protein dynamics.
Independent freezing of charge and spin dynamics in La1.5Sr0.5CoO4
Zaliznyak; Hill; Tranquada; Erwin; Moritomo
2000-11-13
We present elastic and quasielastic neutron scattering measurements characterizing peculiar short-range charge-orbital and spin order in the layered perovskite material La1.5Sr0.5CoO4. We find that below T(c) approximately 750 K holes introduced by Sr doping lose mobility and enter a statically ordered charge glass phase with loosely correlated checkerboard arrangement of empty and occupied d(3z(2)-r(2)) orbitals ( Co3+ and Co2+). The dynamics of the resultant mixed spin system is governed by the anisotropic nature of the crystal-field Hamiltonian and the peculiar exchange pattern produced by the orbital order. It undergoes a spin freezing transition at a much lower temperature, T(s) less, similar30 K.
Directory of Open Access Journals (Sweden)
Alex Förster
Full Text Available PURPOSE: Crossed cerebellar diaschisis (CCD is a state of neural depression caused by loss of connections to injured neural structures remote from the cerebellum usually evaluated by positron emission tomography. Recently it has been shown that dynamic susceptibility contrast perfusion weighted MRI (PWI may also be feasible to detect the phenomenon. In this study we aimed to assess the frequency of CCD on PWI in patients with acute thalamic infarction. METHODS: From a MRI report database we identified patients with acute isolated thalamic infarction. Contralateral cerebellar hypoperfusion was identified by inspection of time to peak (TTP maps and evaluated quantitatively on TTP, mean transit time (MTT, cerebral blood flow and volume (CBF, CBV maps. A competing cerebellar pathology or an underlying vascular pathology were excluded. RESULTS: A total of 39 patients was included. Common symptoms were hemiparesis (53.8%, hemihypaesthesia (38.5%, dysarthria (30.8%, aphasia (17.9%, and ataxia (15.4%. In 9 patients (23.1% PWI showed hypoperfusion in the contralateral cerebellar hemisphere. All of these had lesions in the territory of the tuberothalamic, paramedian, or inferolateral arteries. Dysarthria was observed more frequently in patients with CCD (6/9 vs. 6/30; OR 8.00; 95%CI 1.54-41.64, p = 0.01. In patients with CCD, the median ischemic lesion volume on DWI (0.91 cm³, IQR 0.49-1.54 cm³ was larger compared to patients with unremarkable PWI (0.51 cm³, IQR 0.32-0.74, p = 0.05. The most pronounced changes were found in CBF (0.94±0.11 and MTT (1.06±0.13 signal ratios, followed by TTP (1.05±0.02. CONCLUSIONS: Multimodal MRI demonstrates CCD in about 20% of acute isolated thalamic infarction patients. Lesion size seems to be a relevant factor in its pathophysiology.
Application of dynamic susceptibility contrast-enhanced perfusion in temporal lobe epilepsy
Energy Technology Data Exchange (ETDEWEB)
Xing, Wu; Wang, Xiaoyi; Xie, Fangfang; Liao, Weihua [Dept. of Radiology, Xiangya Hospital of Central South Univ., Changsha (China)], e-mail: doctoring@sina.com
2013-02-15
Background: Accurately locatithe epileptogenic focus in temporal lobe epilepsy (TLE) is important in clinical practice. Single-photon emission computed tomography (SPECT) and positron-emission tomography (PET) have been widely used in the lateralization of TLE, but both have limitations. Magnetic resonance perfusion imaging can accurately and reliably reflect differences in cerebral blood flow and volume. Purpose: To investigate the diagnostic value of dynamic susceptibility contrast-enhanced (DSC) perfusion magnetic resonance imaging (MRI) in the lateralization of the epileptogenic focus in TLE. Material and Methods: Conventional MRI and DSC-MRI scanning was performed in 20 interictal cases of TLE and 20 healthy volunteers. The relative cerebral blood volume (rCBV) and relative cerebral blood flow (rCBF) of the bilateral mesial temporal lobes of the TLE cases and healthy control groups were calculated. The differences in the perfusion asymmetry indices (AIs), derived from the rCBV and rCBF of the bilateral mesial temporal lobes, were pared between the two groups. Results: In the control group, there were no statistically significant differences between the left and right sides in terms of rCBV (left 1.55 {+-} 0.32, right 1.57 {+-} 0.28) or rCBF (left 99.00 {+-} 24.61, right 100.38 {+-} 23.46) of the bilateral mesial temporal lobes. However, in the case group the ipsilateral rCBV and rCBF values (1.75 {+-} 0.64 and 96.35 {+-} 22.63, respectively) were markedly lower than those of the contralateral side (2.01 {+-} 0.79 and 108.56 {+-} 26.92; P < 0.05). Both the AI of the rCBV (AIrCBV; 13.03 {+-} 10.33) and the AI of the rCBF (AIrCBF; 11.24 {+-} 8.70) of the case group were significantly higher than that of the control group (AIrCBV 5.55 {+-} 3.74, AIrCBF 5.12 {+-} 3.48; P < 0.05). The epileptogenic foci of nine patients were correctly lateralized using the 95th percentile of the AIrCBV and AIrCBF of the control group as the normal upper limits. Conclusion: In
Kim, Jinsuh; Leira, Enrique C; Callison, Richard C; Ludwig, Bryan; Moritani, Toshio; Magnotta, Vincent A; Madsen, Mark T
2010-05-01
We developed fully automated software for dynamic susceptibility contrast (DSC) MR perfusion-weighted imaging (PWI) to efficiently and reliably derive critical hemodynamic information for acute stroke treatment decisions. Brain MR PWI was performed in 80 consecutive patients with acute nonlacunar ischemic stroke within 24h after onset of symptom from January 2008 to August 2009. These studies were automatically processed to generate hemodynamic parameters that included cerebral blood flow and cerebral blood volume, and the mean transit time (MTT). To develop reliable software for PWI analysis, we used computationally robust algorithms including the piecewise continuous regression method to determine bolus arrival time (BAT), log-linear curve fitting, arrival time independent deconvolution method and sophisticated motion correction methods. An optimal arterial input function (AIF) search algorithm using a new artery-likelihood metric was also developed. Anatomical locations of the automatically determined AIF were reviewed and validated. The automatically computed BAT values were statistically compared with estimated BAT by a single observer. In addition, gamma-variate curve-fitting errors of AIF and inter-subject variability of AIFs were analyzed. Lastly, two observes independently assessed the quality and area of hypoperfusion mismatched with restricted diffusion area from motion corrected MTT maps and compared that with time-to-peak (TTP) maps using the standard approach. The AIF was identified within an arterial branch and enhanced areas of perfusion deficit were visualized in all evaluated cases. Total processing time was 10.9+/-2.5s (mean+/-s.d.) without motion correction and 267+/-80s (mean+/-s.d.) with motion correction on a standard personal computer. The MTT map produced with our software adequately estimated brain areas with perfusion deficit and was significantly less affected by random noise of the PWI when compared with the TTP map. Results of image
DEFF Research Database (Denmark)
Falk, Anna; Fahlström, Markus; Rostrup, Egill;
2014-01-01
INTRODUCTION: Perfusion magnetic resonance imaging (MRI) can be used in the pre-operative assessment of brain tumours. The aim of this prospective study was to identify the perfusion parameters from dynamic contrast-enhanced (DCE) and dynamic susceptibility contrast (DSC) perfusion imaging...... that could best discriminate between grade II and III gliomas. METHODS: MRI (3 T) including morphological ((T2 fluid attenuated inversion recovery (FLAIR) and T1-weighted (T1W)+Gd)) and perfusion (DCE and DSC) sequences was performed in 39 patients with newly diagnosed suspected low-grade glioma after...
Wieser, Robert
2015-03-01
The classical Landau-Lifshitz equation has been derived from quantum mechanics. Starting point is the assumption of a non-Hermitian Hamilton operator to take the energy dissipation into account. The corresponding quantum mechanical spin dynamics along with the time dependent Schrödinger, Liouville and Heisenberg equation has been described and the similarities and differences between classical and quantum mechanical spin dynamics have been discussed. Furthermore, a time dependent Schrödinger equation corresponding to the classical Landau-Lifshitz-Gilbert equation and two ways to include temperature into the quantum mechanical spin dynamics have been proposed.
Romera, M.; Lacoste, B.; Ebels, U.; Buda-Prejbeanu, L. D.
2016-09-01
The general concepts of spin wave theory are adapted to the spin torque driven dynamics of a self-polarized system based on two layers coupled via interlayer exchange (conservative coupling) and mutual spin torque (dissipative coupling). An analytical description of the nonlinear dynamics is proposed and validated through numerical simulations. In contrast to the single layer model, the phase equation of the coupled system has a contribution coming from the dissipative part of the LLGS equation. It is shown that this is a major contribution to the frequency mandatory to describe well the most basic features of the dynamics of this coupled system. Using the proposed model a specific feature of coupled dynamics is addressed: the redshift to blueshift transition observed in the frequency current dependence of this kind of exchange coupled systems upon increasing the applied field. It is found that the blueshift regime can only occur in a region of field where the two linear eigenmodes contribute equally to the steady state mode (i.e., high mode hybridization). Finally, a general perturbed Hamiltonian equation for the coupled system is proposed.
Institute of Scientific and Technical Information of China (English)
Shao Yuan-Zhi; Zhong Wei-Rong; Lin Guang-Ming; Li Jian-Can
2005-01-01
The dynamic response and stochastic resonance of a kinetic Ising spin system (ISS) subject to the joint action of an external field of weak sinusoidal modulation and stochastic white-noise are studied by solving the mean-field equation of motion based on Glauber dynamics. The periodically driven stochastic ISS shows that the characteristic stochastic resonance as well as nonequilibrium dynamic phase transition (NDPT) occurs when the frequency ω and amplitude h0 of driving field, the temperature t of the system and noise intensity D are all specifically in accordance with each other in quantity. There exist in the system two typical dynamic phases, referred to as dynamic disordered paramagnetic and ordered ferromagnetic phases respectively, corresponding to a zero- and a unit-dynamic order parameter. The NDPT boundary surface of the system which separates the dynamic paramagnetic phase from the dynamic ferromagnetic phase in the 3D parameter space of h0-t-D is also investigated. An interesting dynamical ferromagnetic phase with an intermediate order parameter of 0.66 is revealed for the first time in the ISS subject to the perturbation of a joint determinant and stochastic field. The intermediate order dynamical ferromagnetic phase is dynamically metastable in nature and owns a peculiar characteristic in its stability as well as the response to external driving field as compared with a fully order dynamic ferromagnetic phase.
Balakin, Alexander B.; Popov, Vladimir A.
2017-04-01
In the framework of the Einstein-aether theory we consider a cosmological model, which describes the evolution of the unit dynamic vector field with activated rotational degree of freedom. We discuss exact solutions of the Einstein-aether theory, for which the space-time is of the Gödel-type, the velocity four-vector of the aether motion is characterized by a non-vanishing vorticity, thus the rotational vectorial modes can be associated with the source of the universe rotation. The main goal of our paper is to study the motion of test relativistic particles with a vectorial internal degree of freedom (spin or polarization), which is coupled to the unit dynamic vector field. The particles are considered as the test ones in the given space-time background of the Gödel-type the spin (polarization) coupling to the unit dynamic vector field is modeled using exact solutions of three types. The first exact solution describes the aether with arbitrary Jacobson's coupling constants; the second one relates to the case, when the Jacobson's constant responsible for the vorticity is vanishing; the third exact solution is obtained using three constraints for the coupling constants. The analysis of the exact expressions, which are obtained for the particle momentum and for the spin (polarization) four-vector components, shows that the interaction of the spin (polarization) with the unit vector field induces a rotation, which is additional to the geodesic precession of the spin (polarization) associated with the universe rotation as a whole.
Dynamical properties of the sine-Gordon quantum spin magnet Cu-PM at zero and finite temperature
Tiegel, Alexander C.; Honecker, Andreas; Pruschke, Thomas; Ponomaryov, Alexey; Zvyagin, Sergei A.; Feyerherm, Ralf; Manmana, Salvatore R.
2016-03-01
The material copper pyrimidine dinitrate (Cu-PM) is a quasi-one-dimensional spin system described by the spin-1/2 X X Z Heisenberg antiferromagnet with Dzyaloshinskii-Moriya interactions. Based on numerical results obtained by the density-matrix renormalization group, exact diagonalization, and accompanying electron spin resonance (ESR) experiments we revisit the spin dynamics of this compound in an applied magnetic field. Our calculations for momentum and frequency-resolved dynamical quantities give direct access to the intensity of the elementary excitations at both zero and finite temperature. This allows us to study the system beyond the low-energy description by the quantum sine-Gordon model. We find a deviation from the Lorentz invariant dispersion for the single-soliton resonance. Furthermore, our calculations only confirm the presence of the strongest boundary bound state previously derived from a boundary sine-Gordon field theory, while composite boundary-bulk excitations have too low intensities to be observable. Upon increasing the temperature, we find a temperature-induced crossover of the soliton and the emergence of new features, such as interbreather transitions. The latter observation is confirmed by our ESR experiments on Cu-PM over a wide range of the applied field.
Jang, Kyeong-Jin; Lim, Jongseok; Ahn, Jaewook; Kim, Ji-Hee; Yee, Ki-Ju; Ahn, Jai Seok; Cheong, Sang-Wook
2010-02-01
The concurrent existence of ferroelectricity and magnetism within a single crystalline system characterizes the multiferroic materials discovered in recent years. To understand and develop the multiferroic phenomenon, we need to investigate the unusual coupling between spin and lattice degrees of freedom. Spins in multiferroics are expected to be elastically coupled to phonons. Therefore, the time-dependent study can be a crucial factor in understanding the coupled dynamics. Here, we report the observations of strong dynamic spin-lattice coupling in multiferroic LuMnO3. A coherent optical phonon of 3.6 THz and its temperature dependence is measured for the first time from our femtosecond IR pump and probe spectroscopy. Also, we observed a coherent acoustic phonon of 47 GHz similar to a previous report (Lim et al 2003 Appl. Phys. Lett. 83 4800). Temperature-dependent measurements show that both optical and acoustic phonons become significantly underdamped as temperature decreases to TN, and they disappear below TN. These observations reveal that phonons are coupled to spins by magneto-elastic coupling, and the disappearance of phonon modes at TN is consistent with the isostructural coupling scheme suggested by Lee et al (2008 Nature 451 805).
Energy Technology Data Exchange (ETDEWEB)
Classen, Aimee T [ORNL; Chapman, Samantha K. [Smithsonian Environmental Research Center, Edgewater, MD; Whitham, Thomas G [Northern Arizona University; Hart, Stephen C [Northern Arizona University; Koch, George W [Northern Arizona University
2007-01-01
It is generally assumed that leaf and root litter decomposition have similar drivers and that nutrient release from these substrates is synchronized. Few studies have examined these assumptions, and none has examined how plant genetics (i.e., plant susceptibility to herbivory) could affect these relationships. Here we examine the effects of herbivore susceptibility and resistance on needle and fine root litter decomposition of pi on pine, Pinus edulis. The study population consists of individual trees that are either susceptible or resistant to herbivory by the pi on needle scale, Matsucoccus acalyptus, or the stem-boring moth, Dioryctria albovittella. Genetic analyses and experimental removals and additions of these insects have identified trees that are naturally resistant and susceptible to these insects. These herbivores increase the chemical quality of litter inputs and alter soil microclimate, both of which are important decomposition drivers. Our research leads to four major conclusions: Herbivore susceptibility and resistance effects on 1) needle litter mass loss and phosphorus (P) retention in moth susceptible and resistant litter are governed by microclimate, 2) root litter nitrogen (N) and P retention, and needle litter N retention are governed by litter chemical quality, 3) net nutrient release from litter can reverse over time, 4) root and needle litter mass loss and nutrient release are determined by location (above- vs. belowground), suggesting that the regulators of needle and root decomposition differ at the local scale. Understanding of decomposition and nutrient retention in ecosystems requires consideration of herbivore effects on above- and belowground processes and how these effects may be governed by plant genotype. Because an underlying genetic component to herbivory is common to most ecosystems of the world and herbivory may increase in climatic change scenarios, it is important to evaluate the role of plant genetics in affecting carbon and