WorldWideScience

Sample records for climate ambient air

  1. Ambient air pollution, climate change, and population health in China.

    Science.gov (United States)

    Kan, Haidong; Chen, Renjie; Tong, Shilu

    2012-07-01

    As the largest developing country, China has been changing rapidly over the last three decades and its economic expansion is largely driven by the use of fossil fuels, which leads to a dramatic increase in emissions of both ambient air pollutants and greenhouse gases (GHGs). China is now facing the worst air pollution problem in the world, and is also the largest emitter of carbon dioxide. A number of epidemiological studies on air pollution and population health have been conducted in China, using time-series, case-crossover, cross-sectional, cohort, panel or intervention designs. The increased health risks observed among Chinese population are somewhat lower in magnitude, per amount of pollution, than the risks found in developed countries. However, the importance of these increased health risks is greater than that in North America or Europe, because the levels of air pollution in China are very high in general and Chinese population accounts for more than one fourth of the world's totals. Meanwhile, evidence is mounting that climate change has already affected human health directly and indirectly in China, including mortality from extreme weather events; changes in air and water quality; and changes in the ecology of infectious diseases. If China acts to reduce the combustion of fossil fuels and the resultant air pollution, it will reap not only the health benefits associated with improvement of air quality but also the reduced GHG emissions. Consideration of the health impact of air pollution and climate change can help the Chinese government move forward towards sustainable development with appropriate urgency.

  2. Implications of Nitrogen-Climate Interactions for Ambient Air Pollution and Human Health

    Science.gov (United States)

    Haeuber, R.; Peel, J. L.; Garcia, V.; Neas, L.; Russell, A. G.

    2011-12-01

    Nitrogen oxides (NOX) are important components of ambient and indoor air pollution and are emitted from a range of combustion sources, including on-road mobile sources, electric power generators, and non-road mobile sources. While anthropogenic sources dominate, NOX is also formed by lightning and wildland fires and is emitted by soil. Reduced nitrogen (e.g., ammonia, NH3) is also emitted by various sources, including fertilizer application and animal waste decomposition. NOX, ozone and PM2.5 pollution related to atmospheric emissions of nitrogen and other pollutants can cause premature death and a variety of serious health effects. Climate change is expected to impact how nitrogen-related pollutants affect human health. For example, changes in temperature and precipitation patterns are projected to both lengthen the ozone season and intensify high ozone episodes in some areas. Other climate-related changes may increase the atmospheric release of nitrogen compounds through impacts on wildfire regimes, soil emissions, and biogenic emissions from terrestrial ecosystems. This session will examine the potential human health implications of climate change and nitrogen cycle interactions related to ambient air pollution.

  3. Environmental resources of selected areas of Hawaii: Climate, ambient air quality, and noise

    Energy Technology Data Exchange (ETDEWEB)

    Lombardi, D.A.; Blasing, T.J.; Easterly, C.E.; Reed, R.M. [Oak Ridge National Lab., TN (United States); Hamilton, C.B. [Univ. of Tennessee, Knoxville, TN (United States)

    1995-03-01

    This report has been prepared to make available and archive background scientific data and related information on climate, ambient air quality, and ambient noise levels collected during the preparation of the environmental impact statement (EIS) for Phases 3 and 4 of the Hawaii Geothermal Project (HGP) as defined by the state of Hawaii in its April 1989 proposal to Congress. The US Department of Energy (DOE) published a notice withdrawing its Notice of Intent to prepare the HGP-EIS. Since the state of Hawaii is no longer pursuing or planning to pursue the HGP, DOE considers the project to be terminated. The report presents a general description of the climate add air quality for the islands of Hawaii (henceforth referred to as Hawaii), Maui and Oahu. It also presents a literature review as baseline information on the health effects of sulfide. The scientific background data and related information is being made available for use by others in conducting future scientific research in these areas. This report describes the environmental resources present in the areas studied (i.e., the affected environment) and does not represent an assessment of environmental impacts.

  4. Environmental Resources of Selected Areas of Hawaii: Climate, Ambient Air Quality, and Noise (DRAFT)

    Energy Technology Data Exchange (ETDEWEB)

    Lombardi, D.A.; Blasing, T.J.; Easterly, C.E.; Hamilton, C.B.

    1994-06-01

    This report has been prepared to make available and archive background scientific data and related information on climate, ambient air quality, and ambient noise levels collected during the preparation of the environmental impact statement (EIS) for Phases 3 and 4 of the Hawaii Geothermal Project (HGP) as defined by the state of hawaii in its April 1989 proposal to Congress. The US Department of Energy (DOE) published a notice in the Federal Register on May 17, 1994 withdrawing its Notice of Intent of February 14, 1992, to prepare the HGP-EIS. Since the state of Hawaii is no longer pursuing or planning to pursue the HGP, DOE considers the project to be terminated. The report presents a general description of the climate and air quality for the islands of Hawaii (henceforth referred to as Hawaii), Maui, and Oahu. It also presents a literature review as baseline information on the health effects of hydrogen sulfide. the scientific background data and related information is being made available for use by others in conducting future scientific research in these areas. This report describes the environmental resources present in the areas studied (i.e., the affected environment) and does not represent an assessment of environmental impacts.

  5. Ambient Air Quality Data Inventory

    Data.gov (United States)

    U.S. Environmental Protection Agency — The Office of Air and Radiation??s (OAR) Ambient Air Quality Data (Current) contains ambient air pollution data collected by EPA, other federal agencies, as well as...

  6. Ambient Air Quality Data Inventory

    Data.gov (United States)

    U.S. Environmental Protection Agency — The Office of Air and Radiation's (OAR) Ambient Air Quality Data (Current) contains ambient air pollution data collected by EPA, other federal agencies, as well as...

  7. Historical Ambient Air Quality Data Inventory

    Data.gov (United States)

    U.S. Environmental Protection Agency — The Historical Ambient Air Quality Data Inventory contains measured and estimated data on ambient air pollution for use in assessing air quality, assisting in...

  8. Ambient air pollution and low birthweight

    DEFF Research Database (Denmark)

    Pedersen, Marie; Giorgis-Allemand, Lise; Bernard, Claire

    2013-01-01

    BACKGROUND: Ambient air pollution has been associated with restricted fetal growth, which is linked with adverse respiratory health in childhood. We assessed the effect of maternal exposure to low concentrations of ambient air pollution on birthweight. METHODS: We pooled data from 14 population...... air pollutants and traffic during pregnancy is associated with restricted fetal growth. A substantial proportion of cases of low birthweight at term could be prevented in Europe if urban air pollution was reduced. FUNDING: The European Union....

  9. 77 FR 12524 - Approval and Promulgation of Air Quality Implementation Plans; Indiana; Lead Ambient Air Quality...

    Science.gov (United States)

    2012-03-01

    ... Ambient Air Quality Standards AGENCY: Environmental Protection Agency (EPA). ACTION: Proposed rule...) under the Clean Air Act (CAA). This submittal incorporates the National Ambient Air Quality...

  10. 40 CFR 51.190 - Ambient air quality monitoring requirements.

    Science.gov (United States)

    2010-07-01

    ... 40 Protection of Environment 2 2010-07-01 2010-07-01 false Ambient air quality monitoring... PROGRAMS REQUIREMENTS FOR PREPARATION, ADOPTION, AND SUBMITTAL OF IMPLEMENTATION PLANS Ambient Air Quality Surveillance § 51.190 Ambient air quality monitoring requirements. The requirements for monitoring ambient...

  11. Wash-out of ambient air contaminations for breath measurements.

    Science.gov (United States)

    Maurer, F; Wolf, A; Fink, T; Rittershofer, B; Heim, N; Volk, T; Baumbach, J I; Kreuer, S

    2014-06-01

    In breath analysis, ambient air contaminations are ubiquitous and difficult to eliminate. This study was designed to investigate the reduction of ambient air background by a lung wash-out with synthetic air. The reduction of the initial ambient air volatile organic compound (VOC) intensity was investigated in the breath of 20 volunteers inhaling synthetic air via a sealed full face mask in comparison to inhaling ambient air. Over a period of 30 minutes, breath analysis was conducted using ion mobility spectrometry coupled to a multi-capillary column. A total of 68 VOCs were identified for inhaling ambient air or inhaling synthetic air. By treatment with synthetic air, 39 VOCs decreased in intensity, whereas 29 increased in comparison to inhaling ambient air. In total, seven VOCs were significantly reduced (P-value ambient air contaminations from the airways by a lung wash-out with synthetic air.

  12. Antimicrobial Applications of Ambient--Air Plasmas

    Science.gov (United States)

    Pavlovich, Matthew John

    The emerging field of plasma biotechology studies the applications of the plasma phase of matter to biological systems. "Ambient-condition" plasmas created at or near room temperature and atmospheric pressure are especially promising for biomedical applications because of their convenience, safety to patients, and compatibility with existing medical technology. Plasmas can be created from many different gases; plasma made from air contains a number of reactive oxygen and nitrogen species, or RONS, involved in various biological processes, including immune activity, signaling, and gene expression. Therefore, ambient-condition air plasma is of particular interest for biological applications. To understand and predict the effects of treating biological systems with ambient-air plasma, it is necessary to characterize and measure the chemical species that these plasmas produce. Understanding both gaseous chemistry and the chemistry in plasma-treated aqueous solution is important because many biological systems exist in aqueous media. Existing literature about ambient-air plasma hypothesizes the critical role of reactive oxygen and nitrogen species; a major aim of this dissertation is to better quantify RONS by produced ambient-air plasma and understand how RONS chemistry changes in response to different plasma processing conditions. Measurements imply that both gaseous and aqueous chemistry are highly sensitive to operating conditions. In particular, chemical species in air treated by plasma exist in either a low-power ozone-dominated mode or a high-power nitrogen oxide-dominated mode, with an unstable transition region at intermediate discharge power and treatment time. Ozone (O3) and nitrogen oxides (NO and NO2, or NOx) are mutually exclusive in this system and that the transition region corresponds to the transition from ozone- to nitrogen oxides-mode. Aqueous chemistry agrees well with to air plasma chemistry, and a similar transition in liquid-phase composition

  13. Assessment of SRS ambient air monitoring network

    Energy Technology Data Exchange (ETDEWEB)

    Abbott, K. [Savannah River Site (SRS), Aiken, SC (United States). Savannah River National Lab. (SRNL); Jannik, T. [Savannah River Site (SRS), Aiken, SC (United States). Savannah River National Lab. (SRNL)

    2016-08-03

    Three methodologies have been used to assess the effectiveness of the existing ambient air monitoring system in place at the Savannah River Site in Aiken, SC. Effectiveness was measured using two metrics that have been utilized in previous quantification of air-monitoring network performance; frequency of detection (a measurement of how frequently a minimum number of samplers within the network detect an event), and network intensity (a measurement of how consistent each sampler within the network is at detecting events). In addition to determining the effectiveness of the current system, the objective of performing this assessment was to determine what, if any, changes could make the system more effective. Methodologies included 1) the Waite method of determining sampler distribution, 2) the CAP88- PC annual dose model, and 3) a puff/plume transport model used to predict air concentrations at sampler locations. Data collected from air samplers at SRS in 2015 compared with predicted data resulting from the methodologies determined that the frequency of detection for the current system is 79.2% with sampler efficiencies ranging from 5% to 45%, and a mean network intensity of 21.5%. One of the air monitoring stations had an efficiency of less than 10%, and detected releases during just one sampling period of the entire year, adding little to the overall network intensity. By moving or removing this sampler, the mean network intensity increased to about 23%. Further work in increasing the network intensity and simulating accident scenarios to further test the ambient air system at SRS is planned

  14. Assessment of SRS ambient air monitoring network

    Energy Technology Data Exchange (ETDEWEB)

    Abbott, K. [Savannah River Site (SRS), Aiken, SC (United States). Savannah River National Lab. (SRNL); Jannik, T. [Savannah River Site (SRS), Aiken, SC (United States). Savannah River National Lab. (SRNL)

    2016-08-03

    Three methodologies have been used to assess the effectiveness of the existing ambient air monitoring system in place at the Savannah River Site in Aiken, SC. Effectiveness was measured using two metrics that have been utilized in previous quantification of air-monitoring network performance; frequency of detection (a measurement of how frequently a minimum number of samplers within the network detect an event), and network intensity (a measurement of how consistent each sampler within the network is at detecting events). In addition to determining the effectiveness of the current system, the objective of performing this assessment was to determine what, if any, changes could make the system more effective. Methodologies included 1) the Waite method of determining sampler distribution, 2) the CAP88- PC annual dose model, and 3) a puff/plume transport model used to predict air concentrations at sampler locations. Data collected from air samplers at SRS in 2015 compared with predicted data resulting from the methodologies determined that the frequency of detection for the current system is 79.2% with sampler efficiencies ranging from 5% to 45%, and a mean network intensity of 21.5%. One of the airmonitoring stations had an efficiency of less than 10%, and detected releases during just one sampling period of the entire year, adding little to the overall network intensity. By moving or removing this sampler, the mean network intensity increased to about 23%. Further work in increasing the network intensity and simulating accident scenarios to further test the ambient air system at SRS is planned

  15. Ambient particulate matter air pollution and cardiopulmonary diseases.

    Science.gov (United States)

    Thurston, George; Lippmann, Morton

    2015-06-01

    Population exposures to ambient outdoor particulate matter (PM) air pollution have been assessed to represent a major burden on global health. Ambient PM is a diverse class of air pollution, with characteristics and health implications that can vary depending on a host of factors, including a particle's original source of emission or formation. The penetration of inhaled particles into the thorax is dependent on their deposition in the upper respiratory tract during inspiration, which varies with particle size, flow rate and tidal volume, and in vivo airway dimensions. All of these factors can be quite variable from person to person, depending on age, transient illness, cigarette smoke and other short-term toxicant exposures that cause transient bronchoconstriction, and occupational history associated with loss of lung function or cumulative injury. The adverse effects of inhaled PM can result from both short-term (acute) and long-term (chronic) exposures to PM, and can range from relatively minor, such as increased symptoms, to very severe effects, including increased risk of premature mortality and decreased life expectancy from long-term exposure. Control of the most toxic PM components can therefore provide major health benefits, and can help guide the selection of the most human health optimal air quality control and climate change mitigation policy measures. As such, a continued improvement in our understanding of the nature and types of PM that are most dangerous to health, and the mechanism(s) of their respective health effects, is an important public health goal.

  16. Global air quality and climate.

    Science.gov (United States)

    Fiore, Arlene M; Naik, Vaishali; Spracklen, Dominick V; Steiner, Allison; Unger, Nadine; Prather, Michael; Bergmann, Dan; Cameron-Smith, Philip J; Cionni, Irene; Collins, William J; Dalsøren, Stig; Eyring, Veronika; Folberth, Gerd A; Ginoux, Paul; Horowitz, Larry W; Josse, Béatrice; Lamarque, Jean-François; MacKenzie, Ian A; Nagashima, Tatsuya; O'Connor, Fiona M; Righi, Mattia; Rumbold, Steven T; Shindell, Drew T; Skeie, Ragnhild B; Sudo, Kengo; Szopa, Sophie; Takemura, Toshihiko; Zeng, Guang

    2012-10-07

    Emissions of air pollutants and their precursors determine regional air quality and can alter climate. Climate change can perturb the long-range transport, chemical processing, and local meteorology that influence air pollution. We review the implications of projected changes in methane (CH(4)), ozone precursors (O(3)), and aerosols for climate (expressed in terms of the radiative forcing metric or changes in global surface temperature) and hemispheric-to-continental scale air quality. Reducing the O(3) precursor CH(4) would slow near-term warming by decreasing both CH(4) and tropospheric O(3). Uncertainty remains as to the net climate forcing from anthropogenic nitrogen oxide (NO(x)) emissions, which increase tropospheric O(3) (warming) but also increase aerosols and decrease CH(4) (both cooling). Anthropogenic emissions of carbon monoxide (CO) and non-CH(4) volatile organic compounds (NMVOC) warm by increasing both O(3) and CH(4). Radiative impacts from secondary organic aerosols (SOA) are poorly understood. Black carbon emission controls, by reducing the absorption of sunlight in the atmosphere and on snow and ice, have the potential to slow near-term warming, but uncertainties in coincident emissions of reflective (cooling) aerosols and poorly constrained cloud indirect effects confound robust estimates of net climate impacts. Reducing sulfate and nitrate aerosols would improve air quality and lessen interference with the hydrologic cycle, but lead to warming. A holistic and balanced view is thus needed to assess how air pollution controls influence climate; a first step towards this goal involves estimating net climate impacts from individual emission sectors. Modeling and observational analyses suggest a warming climate degrades air quality (increasing surface O(3) and particulate matter) in many populated regions, including during pollution episodes. Prior Intergovernmental Panel on Climate Change (IPCC) scenarios (SRES) allowed unconstrained growth, whereas

  17. Global Air Quality and Climate

    Science.gov (United States)

    Fiore, Arlene M.; Naik, Vaishali; Steiner, Allison; Unger, Nadine; Bergmann, Dan; Prather, Michael; Righi, Mattia; Rumbold, Steven T.; Shindell, Drew T.; Skeie, Ragnhild B.; Sudo, Kengo; Szopa, Sophie; Horowitz, Larry W.; Takemura, Toshihiko; Zeng, Guang; Cameron-Smith, Philip J.; Cionni, Irene; Collins, William J.; Dalsoren, Stig; Eyring, Veronika; Folberth, Gerd A.; Ginoux, Paul; Josse, Batrice; Lamarque, Jean-Francois; OConnor, Fiona M.; Mackenzie, Ian A.; Nagashima, Tatsuya; Shindell, Drew Todd; Spracklen, Dominick V.

    2012-01-01

    Emissions of air pollutants and their precursors determine regional air quality and can alter climate. Climate change can perturb the long-range transport, chemical processing, and local meteorology that influence air pollution. We review the implications of projected changes in methane (CH4), ozone precursors (O3), and aerosols for climate (expressed in terms of the radiative forcing metric or changes in global surface temperature) and hemispheric-to-continental scale air quality. Reducing the O3 precursor CH4 would slow near-term warming by decreasing both CH4 and tropospheric O3. Uncertainty remains as to the net climate forcing from anthropogenic nitrogen oxide (NOx) emissions, which increase tropospheric O3 (warming) but also increase aerosols and decrease CH4 (both cooling). Anthropogenic emissions of carbon monoxide (CO) and non-CH4 volatile organic compounds (NMVOC) warm by increasing both O3 and CH4. Radiative impacts from secondary organic aerosols (SOA) are poorly understood. Black carbon emission controls, by reducing the absorption of sunlight in the atmosphere and on snow and ice, have the potential to slow near-term warming, but uncertainties in coincident emissions of reflective (cooling) aerosols and poorly constrained cloud indirect effects confound robust estimates of net climate impacts. Reducing sulfate and nitrate aerosols would improve air quality and lessen interference with the hydrologic cycle, but lead to warming. A holistic and balanced view is thus needed to assess how air pollution controls influence climate; a first step towards this goal involves estimating net climate impacts from individual emission sectors. Modeling and observational analyses suggest a warming climate degrades air quality (increasing surface O3 and particulate matter) in many populated regions, including during pollution episodes. Prior Intergovernmental Panel on Climate Change (IPCC) scenarios (SRES) allowed unconstrained growth, whereas the Representative

  18. [Air quality and climate change].

    Science.gov (United States)

    Loft, Steffen

    2009-10-26

    Air quality, health and climate change are closely connected. Ozone depends on temperature and the greenhouse gas methane from cattle and biomass. Pollen presence depends on temperature and CO2. The effect of climate change on particulate air pollution is complex, but the likely net effect is greater health risks. Reduction of greenhouse-gas emissions by reduced livestock production and use of combustion for energy production, transport and heating will also improve air quality. Energy savings in buildings and use of CO2 neutral fuels should not deteriorate indoor and outdoor air quality.

  19. 77 FR 30087 - Air Quality Designations for the 2008 Ozone National Ambient Air Quality Standards

    Science.gov (United States)

    2012-05-21

    ... for the 2008 Ozone National Ambient Air Quality Standards; Implementation of the 2008 National Ambient Air Quality Standards for Ozone: Nonattainment Area Classifications Approach, Attainment Deadlines and... Quality Standards AGENCY: Environmental Protection Agency (EPA). ACTION: Final rule. SUMMARY: This...

  20. 78 FR 63878 - Approval and Promulgation of Air Quality Implementation Plans; Virginia; Revised Ambient Air...

    Science.gov (United States)

    2013-10-25

    ... Ambient Air Quality Standards for Fine Particulate Matter AGENCY: Environmental Protection Agency (EPA... Commonwealth of Virginia State Implementation Plan (SIP). The revisions add ambient air quality standards and... National Ambient Air Quality Standards (NAAQS) for PM 2.5 . EPA is approving these revisions in...

  1. 40 CFR 52.14 - State ambient air quality standards.

    Science.gov (United States)

    2010-07-01

    ... 40 Protection of Environment 3 2010-07-01 2010-07-01 false State ambient air quality standards. 52... quality standards. Any ambient air quality standard submitted with a plan which is less stringent than a national standard is not considered part of the plan....

  2. 78 FR 34177 - Implementation of the 2008 National Ambient Air Quality Standards for Ozone: State Implementation...

    Science.gov (United States)

    2013-06-06

    ... the 2008 National Ambient Air Quality Standards for Ozone: State Implementation Plan Requirements... Ambient Air Quality Standards for Ozone: State Implementation Plan Requirements AGENCY: Environmental... 2008 ozone national ambient air quality standards (NAAQS) (the ``2008 ozone NAAQS'') that...

  3. 77 FR 60985 - Ambient Air Monitoring Reference and Equivalent Methods: Designation of Three New Equivalent Methods

    Science.gov (United States)

    2012-10-05

    ... AGENCY Ambient Air Monitoring Reference and Equivalent Methods: Designation of Three New Equivalent... methods for monitoring ambient air quality. SUMMARY: Notice is hereby given that the Environmental... in the ambient air. FOR FURTHER INFORMATION CONTACT: Robert Vanderpool, Human Exposure...

  4. 78 FR 63933 - Approval and Promulgation of Air Quality Implementation Plans; Virginia; Revised Ambient Air...

    Science.gov (United States)

    2013-10-25

    ... Ambient Air Quality Standards for Fine Particulate Matter AGENCY: Environmental Protection Agency (EPA... submitted by the Commonwealth of Virginia adding ambient air quality standards and associated reference conditions for Fine Particulate Matter (PM 2.5 ) that are consistent with the 2013 National Ambient...

  5. 40 CFR 52.995 - Enhanced ambient air quality monitoring.

    Science.gov (United States)

    2010-07-01

    ... 40 Protection of Environment 3 2010-07-01 2010-07-01 false Enhanced ambient air quality monitoring. 52.995 Section 52.995 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) AIR... air quality monitoring. (a) The Governor of the State of Louisiana submitted the...

  6. 40 CFR Appendix C to Part 58 - Ambient Air Quality Monitoring Methodology

    Science.gov (United States)

    2010-07-01

    ... 40 Protection of Environment 5 2010-07-01 2010-07-01 false Ambient Air Quality Monitoring... PROGRAMS (CONTINUED) AMBIENT AIR QUALITY SURVEILLANCE Pt. 58, App. C Appendix C to Part 58—Ambient Air Quality Monitoring Methodology 1.0 Purpose 2.0 SLAMS Ambient Air Monitoring Stations 3.0 NCore Ambient...

  7. Survey of Ambient Air Pollution Health Risk Assessment Tools.

    Science.gov (United States)

    Anenberg, Susan C; Belova, Anna; Brandt, Jørgen; Fann, Neal; Greco, Sue; Guttikunda, Sarath; Heroux, Marie-Eve; Hurley, Fintan; Krzyzanowski, Michal; Medina, Sylvia; Miller, Brian; Pandey, Kiran; Roos, Joachim; Van Dingenen, Rita

    2016-09-01

    Designing air quality policies that improve public health can benefit from information about air pollution health risks and impacts, which include respiratory and cardiovascular diseases and premature death. Several computer-based tools help automate air pollution health impact assessments and are being used for a variety of contexts. Expanding information gathered for a May 2014 World Health Organization expert meeting, we survey 12 multinational air pollution health impact assessment tools, categorize them according to key technical and operational characteristics, and identify limitations and challenges. Key characteristics include spatial resolution, pollutants and health effect outcomes evaluated, and method for characterizing population exposure, as well as tool format, accessibility, complexity, and degree of peer review and application in policy contexts. While many of the tools use common data sources for concentration-response associations, population, and baseline mortality rates, they vary in the exposure information source, format, and degree of technical complexity. We find that there is an important tradeoff between technical refinement and accessibility for a broad range of applications. Analysts should apply tools that provide the appropriate geographic scope, resolution, and maximum degree of technical rigor for the intended assessment, within resources constraints. A systematic intercomparison of the tools' inputs, assumptions, calculations, and results would be helpful to determine the appropriateness of each for different types of assessment. Future work would benefit from accounting for multiple uncertainty sources and integrating ambient air pollution health impact assessment tools with those addressing other related health risks (e.g., smoking, indoor pollution, climate change, vehicle accidents, physical activity).

  8. [Ambient and enclosed space air sampling for determination of contaminants].

    Science.gov (United States)

    Dorogova, V B

    2010-01-01

    The paper touches upon the issues how to correctly and maximally take single and average daily samples of ambient, residential and public building, and enclosed space air for further tests for the content of hazardous substances. The paper is debated.

  9. 40 CFR 50.8 - National primary ambient air quality standards for carbon monoxide.

    Science.gov (United States)

    2010-07-01

    ... (CONTINUED) AIR PROGRAMS NATIONAL PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS § 50.8 National primary ambient air quality standards for carbon monoxide. (a) The national primary ambient air quality standards... 40 Protection of Environment 2 2010-07-01 2010-07-01 false National primary ambient air...

  10. Impact of fine particles in ambient air on lung cancer

    Institute of Scientific and Technical Information of China (English)

    Gerard Hoek; Ole Raaschou-Nielsen

    2014-01-01

    Recently, the International Agency for Research on Cancer (IARC) has classified outdoor air pol ution and the particulate matter component of outdoor air pollution as class I carcinogen. Air pollution is consistently associated with lung cancer in epidemiologic and experimental studies. The IARC assessment is specifical y designed as hazard identification, and it does not quantify the magnitude of the cancer risk. This article addresses the magnitude of the lung cancer risk in the population due to ambient air pol ution exposure.

  11. Biomarkers of ambient air pollution and lung cancer

    DEFF Research Database (Denmark)

    Demetriou, Christiana A; Raaschou-Nielsen, Ole; Loft, Steffen

    2012-01-01

    The association between ambient air pollution exposure and lung cancer risk has been investigated in prospective studies and the results are generally consistent, indicating that long-term exposure to air pollution may cause lung cancer. Despite the prospective nature and consistent findings...... the relationships between ambient air pollution and biological markers of dose and early response. The evidence for each marker was evaluated using assessment criteria which rate a group of studies from A (strong) to C (weak) on amount of evidence, replication of findings, and protection from bias. Biomarkers...

  12. Transportation, Air Pollution, and Climate Change

    Science.gov (United States)

    ... Share Facebook Twitter Google+ Pinterest Contact Us Transportation, Air Pollution, and Climate Change Accomplishments & Successes View successes from ... reduce carbon pollution. Carbon pollution from transportation Other Air Pollution Learn about smog, soot, ozone, and other air ...

  13. Air Pollution, Climate, and Heart Disease

    Science.gov (United States)

    ... of the American Heart Association Cardiology Patient Page Air Pollution, Climate, and Heart Disease Diane R. Gold , Jonathan ... http://www.epa.gov/greenheart/ . 7 What Is Air Pollution? Air pollution is a mixture of gases and ...

  14. 40 CFR 61.184 - Ambient air monitoring for inorganic arsenic.

    Science.gov (United States)

    2010-07-01

    ... 40 Protection of Environment 8 2010-07-01 2010-07-01 false Ambient air monitoring for inorganic....184 Ambient air monitoring for inorganic arsenic. (a) The owner or operator of each source to which... arsenic concentrations in the ambient air. (b) The ambient air monitors shall be located at sites...

  15. 77 FR 12482 - Approval and Promulgation of Air Quality Implementation Plans; Indiana; Lead Ambient Air Quality...

    Science.gov (United States)

    2012-03-01

    ... authority to address, as appropriate, disproportionate human health or environmental effects, using...).) List of Subjects in 40 CFR Part 52 Environmental protection, Air pollution control, Incorporation by... Ambient Air Quality Standards AGENCY: Environmental Protection Agency (EPA). ACTION: Direct final...

  16. 78 FR 19990 - Approval and Promulgation of Air Quality Implementation Plans; Ohio; Ohio Ambient Air Quality...

    Science.gov (United States)

    2013-04-03

    ... From the Federal Register Online via the Government Publishing Office ENVIRONMENTAL PROTECTION AGENCY 40 CFR Part 52 Approval and Promulgation of Air Quality Implementation Plans; Ohio; Ohio Ambient Air Quality Standards; Correction AGENCY: Environmental Protection Agency (EPA). ACTION: Final...

  17. Impacts of Climate Policy on Regional Air Quality, Health, and Air Quality Regulatory Procedures

    Science.gov (United States)

    Thompson, T. M.; Selin, N. E.

    2011-12-01

    Both the changing climate, and the policy implemented to address climate change can impact regional air quality. We evaluate the impacts of potential selected climate policies on modeled regional air quality with respect to national pollution standards, human health and the sensitivity of health uncertainty ranges. To assess changes in air quality due to climate policy, we couple output from a regional computable general equilibrium economic model (the US Regional Energy Policy [USREP] model), with a regional air quality model (the Comprehensive Air Quality Model with Extensions [CAMx]). USREP uses economic variables to determine how potential future U.S. climate policy would change emissions of regional pollutants (CO, VOC, NOx, SO2, NH3, black carbon, and organic carbon) from ten emissions-heavy sectors of the economy (electricity, coal, gas, crude oil, refined oil, energy intensive industry, other industry, service, agriculture, and transportation [light duty and heavy duty]). Changes in emissions are then modeled using CAMx to determine the impact on air quality in several cities in the Northeast US. We first calculate the impact of climate policy by using regulatory procedures used to show attainment with National Ambient Air Quality Standards (NAAQS) for ozone and particulate matter. Building on previous work, we compare those results with the calculated results and uncertainties associated with human health impacts due to climate policy. This work addresses a potential disconnect between NAAQS regulatory procedures and the cost/benefit analysis required for and by the Clean Air Act.

  18. 75 FR 65594 - Approval and Promulgation of Air Quality Implementation Plans; Ohio; Ohio Ambient Air Quality...

    Science.gov (United States)

    2010-10-26

    ... From the Federal Register Online via the Government Publishing Office ENVIRONMENTAL PROTECTION AGENCY 40 CFR Part 52 Approval and Promulgation of Air Quality Implementation Plans; Ohio; Ohio Ambient... consolidation of Ohio's Ambient Air Quality Standards (AAQS) into Ohio's State Implementation Plan (SIP)...

  19. Determination and evaluation of air quality control. Manual of ambient air quality control in Germany

    Energy Technology Data Exchange (ETDEWEB)

    Lahmann, E.

    1997-07-01

    Measurement of air pollution emissions and ambient air quality are essential instruments for air quality control. By undertaking such measurements, pollutants are registered both at their place of origin and at the place where they may have an effect on people or the environment. Both types of measurement complement each other and are essential for the implementation of air quality legislation, particularly, in compliance with emission and ambient air quality limit values. Presented here are similar accounts of measurement principles and also contains as an Appendix a list of suitability-tested measuring devices which is based on information provided by the manufacturers. In addition, the guide of ambient air quality control contains further information on discontinuous measurement methods, on measurement planning and on the assessment of ambient air quality data. (orig./SR)

  20. Ambient air pollution and pregnancy-induced hypertensive disorders

    DEFF Research Database (Denmark)

    Pedersen, Marie; Stayner, Leslie; Slama, Rémy

    2014-01-01

    to ambient air pollution and pregnancy-induced hypertensive disorders including gestational hypertension and preeclampsia. We searched electronic databases for English language studies reporting associations between ambient air pollution and pregnancy-induced hypertensive disorders published between December.......5), carbon monoxide (CO), ozone (O3), proximity to major roads, and traffic density met our inclusion criteria. Most studies reported that air pollution increased risk for pregnancy-induced hypertensive disorders. There was significant heterogeneity in meta-analysis, which included 16 studies reporting......-analysis combined odds ratio associated with a 5-μg/m3 increase in PM2.5 was 1.57 (95% confidence interval, 1.26-1.96) for combined pregnancy-induced hypertensive disorders and 1.31 (95%confidence interval, 1.14-1.50) for preeclampsia [corrected]. Our results suggest that exposure to air pollution increases...

  1. 77 FR 65310 - Additional Air Quality Designations for the 2006 24-Hour Fine Particle National Ambient Air...

    Science.gov (United States)

    2012-10-26

    ... Ambient Air Quality Standards AGENCY: Environmental Protection Agency (EPA). ACTION: Supplemental... particle (PM 2.5 ) national ambient air quality standards (NAAQS) air quality designations for the Ak-Chin... Federal Register NAAQS National Ambient Air Quality Standards NTTAA National Technology...

  2. Acute Impact of Hourly Ambient Air Pollution on Preterm Birth

    Science.gov (United States)

    Li, Shanshan; Guo, Yuming; Williams, Gail

    2016-01-01

    Background: Preterm birth is a major perinatal health problem, but factors leading to it are still not completely understood. Objectives: Our goal was to identify the relation between acute increase in ambient air pollution in a few hours before onset of labor and the risk of preterm birth. Methods: We collected registered birth outcome data and hourly ambient air pollution measurements during 2009‒2013 in Brisbane, Australia. Using a time-stratified case-crossover design and conditional logistic regression models with natural cubic splines, we assessed the shape of air pollution-preterm birth curve, after controlling for potential confounders. We also examined the effect modification of other factors. Results: The association between air pollution [nitrogen dioxide (NO2), sulfur dioxide (SO2), and carbon monoxide (CO)] and preterm birth was nonlinear. Threshold concentrations for the mean of 0‒24 hr NO2, 24‒48 hr SO2, and 24‒48 hr CO before onset of labor were 7.6 parts per billion (ppb), 3.8 ppb, and 162.5 ppb, respectively. Increases in air pollution concentrations above thresholds were associated with increased risks of preterm birth. The odds ratios of preterm birth at the 95th percentile of NO2, SO2, and CO against the thresholds were 1.17 (95% CI: 1.08, 1.27), 1.01 (95% CI: 0.99, 1.04), and 1.18 (95% CI: 1.06, 1.32), respectively. The associations were modified by demographic factors, such as maternal smoking and socioeconomic status. Conclusion: Acute increases in ambient air pollution concentrations above certain levels before onset of labor may stimulate preterm birth. Citation: Li S, Guo Y, Williams G. 2016. Acute impact of hourly ambient air pollution on preterm birth. Environ Health Perspect 124:1623–1629; http://dx.doi.org/10.1289/EHP200 PMID:27128028

  3. Application of amine-tethered solid sorbents for direct CO2 capture from the ambient air.

    Science.gov (United States)

    Choi, Sunho; Drese, Jeffrey H; Eisenberger, Peter M; Jones, Christopher W

    2011-03-15

    While current carbon capture and sequestration (CCS) technologies for large point sources can help address the impact of CO(2) buildup on global climate change, these technologies can at best slow the rate of increase of the atmospheric CO(2) concentration. In contrast, the direct CO(2) capture from ambient air offers the potential to be a truly carbon negative technology. We propose here that amine-based solid adsorbents have significant promise as key components of a hypothetical air capture process. Specifically, the CO(2) capture characteristics of hyperbranched aminosilica (HAS) materials are evaluated here using CO(2) mixtures that simulate ambient atmospheric concentrations (400 ppm CO(2) = "air capture") as well as more traditional conditions simulating flue gas (10% CO(2)). The air capture experiments demonstrate that the adsorption capacity of HAS adsorbents are only marginally influenced even with a significant dilution of the CO(2) concentration by a factor of 250, while capturing CO(2) reversibly without significant degradation of performance in multicyclic operation. These results suggest that solid amine-based air capture processes have the potential to be an effective approach to extracting CO(2) from the ambient air.

  4. 40 CFR 50.4 - National primary ambient air quality standards for sulfur oxides (sulfur dioxide).

    Science.gov (United States)

    2010-07-01

    ... PROTECTION AGENCY (CONTINUED) AIR PROGRAMS NATIONAL PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS § 50.4 National primary ambient air quality standards for sulfur oxides (sulfur dioxide). Link to an... applicable to all areas notwithstanding the promulgation of SO2 national ambient air quality standards...

  5. Colorado Air Quality Control Regulations and Ambient Air Quality Standards.

    Science.gov (United States)

    Colorado State Dept. of Health, Denver. Div. of Air Pollution Control.

    Regulations and standards relative to air quality control in Colorado are defined in this publication. Presented first are definitions of terms, a statement of intent, and general provisions applicable to all emission control regulations adopted by the Colorado Air Pollution Control Commission. Following this, three regulations are enumerated: (1)…

  6. Evaluation of ambient air quality in Guangzhou, China

    Institute of Scientific and Technical Information of China (English)

    ZHOU Kai; YE You-hua; LIU Qiang; LIU Ai-jun; PENG Shao-lin

    2007-01-01

    On the basis of the reported air quality index (API) and air pollutant monitoring data provided by the Guangzhou Environment Monitoring Stations over the last twenty-five years, the characteristics of air quality, prominent pollutants, and variation of the average annual concentrations of SO2, NO2, total suspended particulate(TSP), fine particulates (PM10), CO and dustfall in Guangzhou City were analyzed. Results showed that TSP was the prominent pollutant in the ambient air environment of Guangzhou City. Of the prominent pollutants, TSP accounted for nearly 62%, SO2 12.3%, and NOx 6.4%, respectively. The average API of Guangzhou over 6 years was higher than that of Beijing, Tianjin, Nanjing, Hangzhou, Suzhou and Shanghai, and lower than that of Shenzhen, Zhuhai and Shantou. Concentrations of air pollutants have shown an downward trend in recent years, but they are generally worse than ambient air quality standards for USA, Hong Kong and EU. SO2 and NOx pollution were still serious, impling that waste gas pollution from all kinds of vehicles had become a significant problem for environmental protection in Guangzhou. The possible causes of worsening air quality were also discussed in this paper.

  7. Air Quality System (AQS) ambient observations: 2007 PM2.5

    Data.gov (United States)

    U.S. Environmental Protection Agency — Ambient PM2.5 (particulate matter less than 2.5 microns) concentrations from the national ambient air quality monitoring networks stored in the Air Quality System...

  8. Air Quality System (AQS) ambient observations: 2008 PM2.5

    Data.gov (United States)

    U.S. Environmental Protection Agency — Ambient PM2.5 (particulate matter less than 2.5 microns) concentrations from the national ambient air quality monitoring networks stored in the Air Quality System...

  9. Ambient sesquiterpene concentration and its link to air ion measurements

    Directory of Open Access Journals (Sweden)

    B. Bonn

    2006-12-01

    Full Text Available Ambient air ion size distributions have been measured continuously at the Finnish boreal forest site in Hyytiälä since spring 2003. In general, these measurements show a maximum of air ions below 1.0 nm in diameter. But this physical characterization does not provide any information about the ion's chemical composition, which is one key question regarding the explanation of nucleation events observed. In this study we propose a link of the observed maximum of negative air ions between 0.56 and 0.75 nm to the so-called stabilised Criegee biradical, formed in the reaction of biogenic sesquiterpenes with ozone and predominantly destroyed by its reaction with ambient water vapour. Calculations of the electron and proton affinities of 120 kJ mol−1 (1.24 eV and of 960 kJ mol−1 support this link. Other possible candidates such as sulphuric acid derived clusters are unable to explain the observations made. By using this approach, we are able to calculate the ambient concentration of sesquiterpenes at the air ion instrument inlet with a high time resolution on the daily and seasonal scale. The estimated concentration is found to reveal the same seasonal pattern as emission measurements conducted at shoot level. As expected for biogenic VOCs, the concentration is obtained highest during summer (maximum values of about 100 pptv and smallest during winter (minimum less than 1 pptv. Because of the sesquiterpenes high reactivity and its low ambient concentrations, this approach can be a first step in understanding their emission and their impact on atmospheric chemistry in more detail. The findings presented are highly relevant for emission budgets too, since boreal forests are extended over large areas of the globe.

  10. Ambient sesquiterpene concentration and its link to air ion measurements

    Directory of Open Access Journals (Sweden)

    B. Bonn

    2007-06-01

    Full Text Available Ambient air ion size distributions have been measured continuously at the Finnish boreal forest site in Hyytiälä since spring 2003. In general, these measurements show a maximum of air ions below 1.0 nm in diameter. But this physical characterization does not provide any information about the ion's chemical composition, which is one key question regarding the explanation of nucleation events observed. In this study we propose a link of the observed maximum of negative air ions between 0.56 and 0.75 nm to the so-called stabilised Criegee biradical, formed in the reaction of biogenic sesquiterpenes with ozone and predominantly destroyed by its reaction with ambient water vapour. Calculations of the electron and proton affinities of 120 kJ mol−1 (1.24 eV and of 960 kJ mol−1 support this link. Other possible candidates such as sulphuric acid derived clusters are unable to explain the observations made. By using this approach, we are able to calculate the ambient concentration of sesquiterpenes at the air ion instrument inlet with a high time resolution on the daily and seasonal scale. The estimated concentration is found to reveal the same seasonal pattern as emission measurements conducted at shoot level. As expected for biogenic VOCs, the concentration is obtained highest during summer (maximum values of about 100 pptv and smallest during winter (minimum less than 1 pptv. Because of the sesquiterpenes high reactivity and its low ambient concentrations, this approach can be a first step in understanding their emission and their impact on atmospheric chemistry in more detail. The findings presented are highly relevant for emission budgets too, since boreal forests are extended over large areas of the globe.

  11. 78 FR 34964 - Implementation of the 2008 National Ambient Air Quality Standards for Ozone: State Implementation...

    Science.gov (United States)

    2013-06-11

    ... AGENCY 40 CFR Parts 50, 51, 70 and 71 Implementation of the 2008 National Ambient Air Quality Standards... proposed rule ``Implementation of the 2008 National Ambient Air Quality Standards for Ozone: State... proposed rulemaking proposes to implement the 2008 ozone national ambient air quality standards...

  12. 14 CFR 25.1527 - Ambient air temperature and operating altitude.

    Science.gov (United States)

    2010-01-01

    ... 14 Aeronautics and Space 1 2010-01-01 2010-01-01 false Ambient air temperature and operating... Information Operating Limitations § 25.1527 Ambient air temperature and operating altitude. The extremes of the ambient air temperature and operating altitude for which operation is allowed, as limited...

  13. 75 FR 2935 - Extension of Deadline for Promulgating Designations for the 2008 Ozone National Ambient Air...

    Science.gov (United States)

    2010-01-19

    ... Protection Agency 40 CFR Parts 50, 58 and 81 Ozone National Ambient Air Quality Standards; Final Rule and... Designations for the 2008 Ozone National Ambient Air Quality Standards AGENCY: Environmental Protection Agency... promulgating initial area designations for the ozone national ambient air quality standards (NAAQS) that...

  14. 76 FR 60020 - Agency Information Collection Activities: Proposed Collection; Comment Request; Ambient Air...

    Science.gov (United States)

    2011-09-28

    ... AGENCY Agency Information Collection Activities: Proposed Collection; Comment Request; Ambient Air... pollution control agencies, and tribal entities which collect and report ambient air quality data for the criteria pollutants to the EPA as well as other supporting measurements. Title: Ambient Air...

  15. 77 FR 55832 - Ambient Air Monitoring Reference and Equivalent Methods: Designation of a New Equivalent Method

    Science.gov (United States)

    2012-09-11

    ... AGENCY Ambient Air Monitoring Reference and Equivalent Methods: Designation of a New Equivalent Method... monitoring ambient air quality. SUMMARY: Notice is hereby given that the Environmental Protection Agency (EPA... concentrations of PM 2.5 in the ambient air. FOR FURTHER INFORMATION CONTACT: Robert Vanderpool, Human...

  16. 75 FR 81477 - Approval and Promulgation of Air Quality Implementation Plans; Virginia; Amendments to Ambient...

    Science.gov (United States)

    2010-12-28

    ... to Ambient Air Quality Standards for Particulate Matter AGENCY: Environmental Protection Agency (EPA... Commonwealth of Virginia. This revision consists of amendments to the Commonwealth of Virginia's ambient air... amendments to the Commonwealth's existing ambient air quality standards for particulate matter in...

  17. Effects of Ambient Air Pollution Exposure on Olfaction: A Review

    Science.gov (United States)

    Ajmani, Gaurav S.; Suh, Helen H.; Pinto, Jayant M.

    2016-01-01

    Background: Olfactory dysfunction affects millions of people worldwide. This sensory impairment is associated with neurodegenerative disease and significantly decreased quality of life. Exposure to airborne pollutants has been implicated in olfactory decline, likely due to the anatomic susceptibility of the olfactory nerve to the environment. Historically, studies have focused on occupational exposures, but more recent studies have considered effects from exposure to ambient air pollutants. Objectives: To examine all relevant human data evaluating a link between ambient pollution exposure and olfaction and to review supporting animal data in order to examine potential mechanisms for pollution-associated olfactory loss. Methods: We identified and reviewed relevant articles from 1950 to 2015 using PubMed and Web of Science and focusing on human epidemiologic and pathophysiologic studies. Animal studies were included only to support pertinent data on humans. We reviewed findings from these studies evaluating a relationship between environmental pollutant exposure and olfactory function. Results: We identified and reviewed 17 articles, with 1 additional article added from a bibliography search, for a total of 18 human studies. There is evidence in human epidemiologic and pathologic studies that increased exposure to ambient air pollutants is associated with olfactory dysfunction. However, most studies have used proxies for pollution exposure in small samples of convenience. Human pathologic studies, with supporting animal work, have also shown that air pollution can contact the olfactory epithelium, translocate to the olfactory bulb, and migrate to the olfactory cortex. Pollutants can deposit at each location, causing direct damage and disruption of tissue morphology or inducing local inflammation and cellular stress responses. Conclusions: Ambient air pollution may impact human olfactory function. Additional studies are needed to examine air pollution

  18. 76 FR 76048 - Air Quality Designations for the 2008 Lead (Pb) National Ambient Air Quality Standards

    Science.gov (United States)

    2011-12-06

    ... From the Federal Register Online via the Government Publishing Office ENVIRONMENTAL PROTECTION AGENCY 40 CFR Part 81 RIN 2060-AR17 Air Quality Designations for the 2008 Lead (Pb) National Ambient Air Quality Standards Correction In rule document 2011-29460 appearing on pages 72097-72120 in the issues...

  19. Ambient Air Sampling During Quantum-dot Spray Deposition

    Energy Technology Data Exchange (ETDEWEB)

    Jankovic, John Timothy [ORNL; Hollenbeck, Scott M [ORNL

    2010-01-01

    Ambient air sampling for nano-size particle emissions was performed during spot spray coating operations with a Sono-Tek Exactacoat Benchtop system (ECB). The ECB consisted of the application equipment contained within an exhaust enclosure. The enclosure contained numerous small access openings, including an exhaust hook-up. Door access comprised most of the width and height of the front. The door itself was of the swing-out type. Two types of nanomaterials, Cadmium selenide (Cd-Se) quantum-dots (QDs) and Gold (Au) QDs, nominally 3.3 and 5 nm in diameter respectively, were applied during the evaluation. Median spray drop size was in the 20 to 60 micrometer size range.1 Surface coating tests were of short duration, on the order of one-half second per spray and ten spray applications between door openings. The enclosure was ventilated by connection to a high efficiency particulate aerosol (HEPA) filtered house exhaust system. The exhaust rate was nominally 80 ft3 per minute producing about 5 air changes per minute. Real time air monitoring with a scanning mobility particle size analyzer (SMPS ) with a size detection limit of 7 nm indicated a significant increase in the ambient air concentration upon early door opening. A handheld condensation particle counter (CPC) with a lower size limit of 10 nm did not record changes in the ambient background. This increase in the ambient was not observed when door opening was delayed for 2 minutes (~10 air changes). The ventilated enclosure controlled emissions except for cases of rapid door opening before the overspray could be removed by the exhaust. A time delay sufficient to provide 10 enclosure air changes (a concentration reduction of more than 99.99 %) before door opening prevented the release of aerosol particles in any size.2 Scanning-transmission electron microscopy (STEM) and atomic force microscopy (AFM) demonstrated the presence of agglomerates in the surfaces of the spray applied deposition. A filtered air sample of

  20. Method for measurement of volatile oxygenated hydrocarbons in ambient air

    Science.gov (United States)

    Leibrock, E.; Slemr, J.

    An automated gas chromatographic method for the quantitative determination of oxygenated (C 2C 5 carbonyls and C 1C 2 alcohols) and some non-oxygenated (C 5C 8) hydrocarbons in ambient air has been developed. The analytical system consists of a gas chromatograph with a cryogenic sampling trap, a precolumn for the separation of water and other interfering compounds, a cryogenic focusing trap and two analytical columns connected in series. Substances are detected either by flame ionization or by a mass spectrometer. Ozone is removed by a potassium iodide scrubber placed upstream the sampling trap. External gas standards generated by a permeation device are used for calibration. The detection limits range between 0.03 and 0.08 ng (depending on the compound), equivalent to 5 to 56 ppt in 1 l of sampled air. The method was tested by an intercomparison with a different gas chromatographic technique for the determination of NMHC. The system has been applied since 1994 for measurements in ambient air. Data obtained during an intensive campaign in summer 1995 at the field station Wank (1778 m a.s.l.) near Garmisch-Partenkirchen, Germany, are reported and compared with NMHC mixing ratios measured simultaneously in the same air masses.

  1. Ocular surface adverse effects of ambient levels of air pollution

    Directory of Open Access Journals (Sweden)

    André Augusto Miranda Torricelli

    2011-10-01

    Full Text Available It is widely recognized today that outdoor air pollution can affect human health. Various chemical components that are present in ambient pollution may have an irritant effect on the mucous membranes of the body, particularly those of the respiratory tract. Much less attention has been focused on the adverse effect on the ocular surface, despite the fact that this structure is even more exposed to air pollution than the respiratory mucosa since only a very thin tear film separates the corneal and conjunctival epithelia from the air pollutants. So far, clinical data are the more widespread tools used by ophthalmologists for assessing possible aggression to the ocular surface; however, clinical findings alone appears not to correlate properly with the complaints presented by the patients pointing out the need for further clinical and laboratory studies on the subject. The purpose of this study is to review signs and symptoms associated with chronic long-term exposure to environmental air pollutants on the ocular structures currently defined as the ocular surface and to review clinical and laboratory tests used to investigate the adverse effects of air pollutants on such structures. We also review previous studies that investigated the adverse effects of air pollution on the ocular surface and discuss the need for further investigation on the subject.

  2. 40 CFR 50.16 - National primary and secondary ambient air quality standards for lead.

    Science.gov (United States)

    2010-07-01

    ... air quality standards for lead. 50.16 Section 50.16 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) AIR PROGRAMS NATIONAL PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS § 50.16 National primary and secondary ambient air quality standards for lead. (a) The national primary...

  3. 40 CFR 50.12 - National primary and secondary ambient air quality standards for lead.

    Science.gov (United States)

    2010-07-01

    ... air quality standards for lead. 50.12 Section 50.12 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) AIR PROGRAMS NATIONAL PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS § 50.12 National primary and secondary ambient air quality standards for lead. (a) National primary and...

  4. 40 CFR 50.6 - National primary and secondary ambient air quality standards for PM10.

    Science.gov (United States)

    2010-07-01

    ... air quality standards for PM10. 50.6 Section 50.6 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) AIR PROGRAMS NATIONAL PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS § 50.6 National primary and secondary ambient air quality standards for PM10. (a) The level of the...

  5. 40 CFR 50.15 - National primary and secondary ambient air quality standards for ozone.

    Science.gov (United States)

    2010-07-01

    ... air quality standards for ozone. 50.15 Section 50.15 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) AIR PROGRAMS NATIONAL PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS § 50.15 National primary and secondary ambient air quality standards for ozone. (a) The level of...

  6. Indoor Climate and Air Quality Problems

    DEFF Research Database (Denmark)

    Valbjørn, O.; Hagen, H.; Kukkonen, E.;

    This report presents a stepwise method for the investigation of and remedial actions for indoor climate and air quality problems. The report gives the basis for evaluation of the prevalence and causes of building related symptoms like mucosal irritation and headache. The report adresses members...... of occupational health and safety organisations, consulting engineers and architects, and also the people responsible for the operation of buildings and installations which is essential for the indoor climate and air quality....

  7. The TOMPs ambient air monitoring network - Continuous data on UK air quality for over 20 years.

    Science.gov (United States)

    Graf, Carola; Katsoyiannis, Athanasios; Jones, Kevin C; Sweetman, Andrew J

    2016-10-01

    Long-term air monitoring datasets are needed for persistent organic pollutants (POPs) to assess the effectiveness of source abatement measures and the factors controlling ambient levels. The Toxic Organic Micro Pollutants (TOMPs) Network, which has operated since 1991, collects ambient air samples at six sites across England and Scotland, using high-volume active air samplers. The network provides long-term ambient air trend data for a range of POPs at both urban and rural locations. Data from the network provides the UK Government, regulators and researchers with valuable information on emission/source controls and on the effectiveness of international chemicals regulation such as the Stockholm Convention and UN/ECE Protocol on POPs. The target chemicals of TOMPs have been polychlorinated biphenyls (PCBs), polycyclic aromatic hydrocarbons (PAHs), polychlorinated dibenzo-p-dioxins (PCDDs), polychlorinated dibenzofurans (PCDFs), and, since 2010, polybrominated diphenyl ethers (PBDEs). The continuous monitoring of these compounds demonstrates the constant decline in UK air concentrations over the last two decades, with average clearance rates for PCDD/Fs in urban locations of 5.1 years and for PCBs across all sites 6.6 years. No significant declines in rural locations for PCDD/Fs have been observed. There is a strong observable link between the declining ambient air concentrations and the emission reductions estimated in the annually produced National Atmospheric Emission Inventory (NAEI) dataset. These findings clearly demonstrate the unique strengths of long-term consistent datasets for the evaluation of the success of chemical regulation and control.

  8. Determination of beryllium concentrations in UK ambient air

    Science.gov (United States)

    Goddard, Sharon L.; Brown, Richard J. C.; Ghatora, Baljit K.

    2016-12-01

    Air quality monitoring of ambient air is essential to minimise the exposure of the general population to toxic substances such as heavy metals, and thus the health risks associated with them. In the UK, ambient air is already monitored under the UK Heavy Metals Monitoring Network for a number of heavy metals, including nickel (Ni), arsenic (As), cadmium (Cd) and lead (Pb) to ensure compliance with legislative limits. However, the UK Expert Panel on Air Quality Standards (EPAQS) has highlighted a need to limit concentrations of beryllium (Be) in air, which is not currently monitored, because of its toxicity. The aim of this work was to analyse airborne particulate matter (PM) sampled onto filter papers from the UK Heavy Metals Monitoring Network for quantitative, trace level beryllium determination and compare the results to the guideline concentration specified by EPAQS. Samples were prepared by microwave acid digestion in a matrix of 2% sulphuric acid and 14% nitric acid, verified by the use of Certified Reference Materials (CRMs). The digested samples were then analysed by Inductively Coupled Plasma Mass Spectrometry (ICP-MS). The filters from the UK Heavy Metals Monitoring Network were tested using this procedure and the average beryllium concentration across the network for the duration of the study period was 7.87 pg m-3. The highest site average concentration was 32.0 pg m-3 at Scunthorpe Low Santon, which is significantly lower than levels that are thought to cause harm. However the highest levels were observed at sites monitoring industrial point sources, indicating that beryllium is being used and emitted, albeit at very low levels, from these point sources. Comparison with other metals concentrations and data from the UK National Atmospheric Emissions Inventory suggests that current emissions of beryllium may be significantly overestimated.

  9. Characterization of ambient air pollution for stochastic health models

    Energy Technology Data Exchange (ETDEWEB)

    Batterman, S.A.

    1981-08-01

    This research is an analysis of various measures of ambient air pollution useful in cross-sectional epidemiological investigations and rick assessments. The Chestnut Ridge area health effects investigation, which includes a cross-sectional study of respiratory symptoms in young children, is used as a case study. Four large coal-fired electric generating power plants are the dominant pollution sources in this area of western Pennsylvania. The air pollution data base includes four years of sulfur dioxide and five years of total suspended particulate concentrations at seventeen monitors. Some 70 different characterizations of pollution are constructed and tested. These include pollutant concentrations at various percentiles and averaging times, exceedence measures which show the amount of time a specified threshold concentration is exceeded, and several dosage measures which transform non-linear dose-response relationships onto pollutant concentrations.

  10. The State of Ambient Air Quality of Jeddah, Saudi Arabia

    Science.gov (United States)

    Hussain, M. M.; Aburizaiza, O. S.; Khwaja, H. A.; Siddique, A.; Nayebare, S. R.; Zeb, J.; Blake, D. R.

    2014-12-01

    Ambient air pollution in major cities of Saudi Arabia is a substantial environmental and health concern. A study was undertaken to assess the air quality of Jeddah, Saudi Arabia by the analysis of respirable particulate matter (PM2.5), black carbon (BC), trace metals (Na, Mg, Al, Si, S, Cl, K, Ca, Ti, V, Cr, Mn, Fe, Ni, Cu, Zn, Br, Sr, Cd, Sb, and Pb), and water-soluble ions (F-, Cl-, NO3-, SO42-, C2O42-, and NH42+). Sulfur and BC mass concentration ranged 0.99 - 7.39 μg/m3 and 0.70 - 3.09 μg/m3, respectively, while the PM2.5 mass concentration ranged 23 - 186 μg/m3. Maximum BC contribution to PM2.5 was 5.6%. Atmospheric PM2.5 concentrations were well above the 24 h WHO guideline of 20 μg/m3. Air Quality Index (AQI) indicates that there were 8% days of moderate air quality, 28% days of unhealthy air quality for sensitive groups, 55% days of unhealthy air quality, and 9% days of very unhealthy air quality during the study period. Sulfate SO42- dominated the identifiable components. The major contributors to PM2.5 were soil and crustal material; vehicle emissions (black carbon factor); and fuel oil combustion in industries (sulfur factor), according to the Positive Matrix Factorization (PMF). This study highlights the importance of focusing control strategies not only on reducing PM concentration, but also on the reduction of toxic components of the PM, to most effectively protect human health and the environment.

  11. Utility of AIRS Retrievals for Climate Studies

    Science.gov (United States)

    Molnar, Guyla I.; Susskind, Joel

    2007-01-01

    Satellites provide an ideal platform to study the Earth-atmosphere system on practically all spatial and temporal scales. Thus, one may expect that their rapidly growing datasets could provide crucial insights not only for short-term weather processes/predictions but into ongoing and future climate change processes as well. Though Earth-observing satellites have been around for decades, extracting climatically reliable information from their widely varying datasets faces rather formidable challenges. AIRS/AMSU is a state of the art infrared/microwave sounding system that was launched on the EOS Aqua platform on May 4, 2002, and has been providing operational quality measurements since September 2002. In addition to temperature and atmospheric constituent profiles, outgoing longwave radiation and basic cloud parameters are also derived from the AIRS/AMSU observations. However, so far the AIRS products have not been rigorously evaluated and/or validated on a large scale. Here we present preliminary assessments of monthly and 8-day mean AIRS "Version 4.0" retrieved products (available to the public through the DAAC at NASA/GSFC) to assess their utility for climate studies. First we present "consistency checks" by evaluating the time series of means, and "anomalies" (relative to the first 4 full years' worth of AIRS "climate statistics") of several climatically important retrieved parameters. Finally, we also present preliminary results regarding interrelationships of some of these geophysical variables, to assess to what extent they are consistent with the known physics of climate variability/change. In particular, we find at least one observed relationship which contradicts current general circulation climate (GCM) model results: the global water vapor climate feedback which is expected to be strongly positive is deduced to be slightly negative (shades of the "Lindzen effect"?). Though the current AIRS climatology covers only -4.5 years, it will hopefully extend much

  12. Pure air-plasma bullets propagating inside microcapillaries and in ambient air

    KAUST Repository

    Lacoste, Deanna

    2014-11-04

    This paper reports on the characterization of air-plasma bullets in microcapillary tubes and in ambient air, obtained without the use of inert or noble gases. The bullets were produced by nanosecond repetitively pulsed discharges, applied in a dielectric barrier discharge configuration. The anode was a tungsten wire with a diameter of 50 μm, centered in the microcapillary, while the cathode was a silver ring, fixed on the outer surface of the fused silica tube. The effects of the applied voltage and the inner diameter of the microcapillary tube on the plasma behavior were investigated. Inside the tubes, while the topology of the bullets seems to be strongly dependent on the diameter, their velocity is only a function of the amplitude of the applied voltage. In ambient air, the propagation of air bullets with a velocity of about 1.25 ×105 m s-1 is observed.

  13. Pure air-plasma bullets propagating inside microcapillaries and in ambient air

    Science.gov (United States)

    Lacoste, Deanna A.; Bourdon, Anne; Kuribara, Koichi; Urabe, Keiichiro; Stauss, Sven; Terashima, Kazuo

    2014-12-01

    This paper reports on the characterization of air-plasma bullets in microcapillary tubes and in ambient air, obtained without the use of inert or noble gases. The bullets were produced by nanosecond repetitively pulsed discharges, applied in a dielectric barrier discharge configuration. The anode was a tungsten wire with a diameter of 50 µm, centered in the microcapillary, while the cathode was a silver ring, fixed on the outer surface of the fused silica tube. The effects of the applied voltage and the inner diameter of the microcapillary tube on the plasma behavior were investigated. Inside the tubes, while the topology of the bullets seems to be strongly dependent on the diameter, their velocity is only a function of the amplitude of the applied voltage. In ambient air, the propagation of air bullets with a velocity of about 1.25 × 105 m s-1 is observed.

  14. Impact of Climate Change on Ambient Ozone Level and Mortality in Southeastern United States

    Directory of Open Access Journals (Sweden)

    Montserrat Fuentes

    2010-07-01

    Full Text Available There is a growing interest in quantifying the health impacts of climate change. This paper examines the risks of future ozone levels on non-accidental mortality across 19 urban communities in Southeastern United States. We present a modeling framework that integrates data from climate model outputs, historical meteorology and ozone observations, and a health surveillance database. We first modeled present-day relationships between observed maximum daily 8-hour average ozone concentrations and meteorology measured during the year 2000. Future ozone concentrations for the period 2041 to 2050 were then projected using calibrated climate model output data from the North American Regional Climate Change Assessment Program. Daily community-level mortality counts for the period 1987 to 2000 were obtained from the National Mortality, Morbidity and Air Pollution Study. Controlling for temperature, dew-point temperature, and seasonality, relative risks associated with short-term exposure to ambient ozone during the summer months were estimated using a multi-site time series design. We estimated an increase of 0.43 ppb (95% PI: 0.14–0.75 in average ozone concentration during the 2040’s compared to 2000 due to climate change alone. This corresponds to a 0.01% increase in mortality rate and 45.2 (95% PI: 3.26–87.1 premature deaths in the study communities attributable to the increase in future ozone level.

  15. Impact of climate change on ambient ozone level and mortality in southeastern United States.

    Science.gov (United States)

    Chang, Howard H; Zhou, Jingwen; Fuentes, Montserrat

    2010-07-01

    There is a growing interest in quantifying the health impacts of climate change. This paper examines the risks of future ozone levels on non-accidental mortality across 19 urban communities in Southeastern United States. We present a modeling framework that integrates data from climate model outputs, historical meteorology and ozone observations, and a health surveillance database. We first modeled present-day relationships between observed maximum daily 8-hour average ozone concentrations and meteorology measured during the year 2000. Future ozone concentrations for the period 2041 to 2050 were then projected using calibrated climate model output data from the North American Regional Climate Change Assessment Program. Daily community-level mortality counts for the period 1987 to 2000 were obtained from the National Mortality, Morbidity and Air Pollution Study. Controlling for temperature, dew-point temperature, and seasonality, relative risks associated with short-term exposure to ambient ozone during the summer months were estimated using a multi-site time series design. We estimated an increase of 0.43 ppb (95% PI: 0.14-0.75) in average ozone concentration during the 2040's compared to 2000 due to climate change alone. This corresponds to a 0.01% increase in mortality rate and 45.2 (95% PI: 3.26-87.1) premature deaths in the study communities attributable to the increase in future ozone level.

  16. 76 FR 72097 - Air Quality Designations for the 2008 Lead (Pb) National Ambient Air Quality Standards

    Science.gov (United States)

    2011-11-22

    ... IQ Intelligence Quotient NAAQS National Ambient Air Quality Standards NTTAA National Technology... systems (including their brains) arising from Pb exposure may include intelligence quotient (IQ) loss... plants and animals, and neurological effects in vertebrates. V. What are the CAA requirements for...

  17. Amine-Oxide Hybrid Materials for CO2 Capture from Ambient Air.

    Science.gov (United States)

    Didas, Stephanie A; Choi, Sunho; Chaikittisilp, Watcharop; Jones, Christopher W

    2015-10-20

    Oxide supports functionalized with amine moieties have been used for decades as catalysts and chromatographic media. Owing to the recognized impact of atmospheric CO2 on global climate change, the study of the use of amine-oxide hybrid materials as CO2 sorbents has exploded in the past decade. While the majority of the work has concerned separation of CO2 from dilute mixtures such as flue gas from coal-fired power plants, it has been recognized by us and others that such supported amine materials are also perhaps uniquely suited to extract CO2 from ultradilute gas mixtures, such as ambient air. As unique, low temperature chemisorbents, they can operate under ambient conditions, spontaneously extracting CO2 from ambient air, while being regenerated under mild conditions using heat or the combination of heat and vacuum. This Account describes the evolution of our activities on the design of amine-functionalized silica materials for catalysis to the design, characterization, and utilization of these materials in CO2 separations. New materials developed in our laboratory, such as hyperbranched aminosilica materials, and previously known amine-oxide hybrid compositions, have been extensively studied for CO2 extraction from simulated ambient air (400 ppm of CO2). The role of amine type and structure (molecular, polymeric), support type and structure, the stability of the various compositions under simulated operating conditions, and the nature of the adsorbed CO2 have been investigated in detail. The requirements for an effective, practical air capture process have been outlined and the ability of amine-oxide hybrid materials to meet these needs has been discussed. Ultimately, the practicality of such a "direct air capture" process is predicated not only on the physicochemical properties of the sorbent, but also how the sorbent operates in a practical process that offers a scalable gas-solid contacting strategy. In this regard, the utility of low pressure drop monolith

  18. Interlaboratory study of toxaphene analysis in ambient air

    Science.gov (United States)

    Bidleman, Terry F.; Cussion, Sylvia; Jantunen, Liisa M.

    An interlaboratory study was conducted for total toxaphene and selected congeners in an extract of ambient air from the southern United States. All participating labs were experienced in toxaphene analysis and used GC-MS techniques. Ten labs reported the concentration of total toxaphene in a technical toxaphene solution, with a 113% average recovery of the target value and 40% relative standard deviation (RSD). Only six of the 10 labs fell within ±30% of the target value, a criterion recommended by good laboratory practice standards. The interlaboratory RSD was 65% for total toxaphene in the air sample extract (lowered to 43% when one outlying lab was omitted). Nine labs reported the concentrations of five toxaphene components (B8-1413, B8-1414+B8-1945, B8-806+B8-809, B8-2229 and B9-1679) with 33-47% RSD for the technical toxaphene unknown and 34-62% for the air sample. The precision was poorer for a sixth component, congener B9-1025, which has a very low response by electron capture negative ion mass spectrometry (ECNI): 59% RSD for the technical toxaphene unknown and 196% for the air sample. Factors contributing to the interlaboratory variability for total toxaphene and single components are discussed, and follow-up studies are required to identify and minimize the causes of variability. Based on the average analysis, B8-1413 was enriched and B8-806+B8-809 was depleted in the air sample relative to the technical toxaphene standard.

  19. Numerical Analysis of Exergy for Air-Conditioning Influenced by Ambient Temperature

    Directory of Open Access Journals (Sweden)

    Jing-Nang Lee

    2014-07-01

    Full Text Available The article presents numerical analysis of exergy for air-conditioning influenced by ambient temperature. The model of numerical simulation uses an integrated air conditioning system exposed in varied ambient temperature to observe change of the four main devices, the compressor, the condenser, the capillary, and the evaporator in correspondence to ambient temperature. The analysis devices of the four devices’s exergy influenced by the varied ambient temperature and found that the capillary has unusual increasing exergy loss vs. increasing ambient temperature in comparison to the other devices. The result shows that reducing exergy loss of the capillary influenced by the ambient temperature is the key for improving working efficiency of an air-conditioning system when influence of the ambient temperature is considered. The higher ambient temperature causes the larger pressure drop of capillary and more exergy loss.

  20. Joint Effects of Ambient Air Pollutants on Pediatric Asthma Emergency Department Visits in Atlanta, 1998–2004

    Science.gov (United States)

    Background: Because ambient air pollution exposure occurs in the form of mixtures, consideration of joint effects of multiple pollutants may advance our understanding of air pollution health effects. Methods: We assessed the joint effect of selected ambient air pollutant com...

  1. Carbon Dioxide Capture from Ambient Air Using Amine-Grafted Mesoporous Adsorbents

    Directory of Open Access Journals (Sweden)

    Annemarie Wagner

    2013-01-01

    Full Text Available Anthropogenic emissions of carbon dioxide (CO2 have been identified as a major contributor to climate change. An attractive approach to tackle the increasing levels of CO2 in the atmosphere is direct extraction via absorption of CO2 from ambient air, to be subsequently desorbed and processed under controlled conditions. The feasibility of this approach depends on the sorbent material that should combine a long lifetime with nontoxicity, high selectivity for CO2, and favorable thermodynamic cycling properties. Adsorbents based on pore-expanded mesoporous silica grafted with amines have previously been found to combine high CO2 adsorption capacity at low partial pressures with operational stability under highly defined laboratory conditions. Here we examine the real potential and functionality of these materials by using more realistic conditions using both pure CO2, synthetic air, and, most importantly, ambient air. Through a combination of thermogravimetric analysis and Fourier transform infrared (TGA-FTIR spectroscopy we address the primary functionality and by diffuse reflectance infrared Fourier transform (DRIFT spectroscopy the observed degradation of the material on a molecular level.

  2. Industrial CO2 Removal: CO2 Capture from Ambient Air and Geological Sequestration

    Energy Technology Data Exchange (ETDEWEB)

    Dooley, James J.

    2011-06-08

    This abstract and its accompanying presentation will provide an overview of two distinct industrial processes for removing carbon dioxide (CO2) from the atmosphere as a means of addressing anthropogenic climate change. The first of these is carbon dioxide capture and storage (CCS) coupled with large scale biomass production (hereafter referred to as bioCCS). The second is CO2 capture from ambient air via industrial systems (hereafter referred to as direct air capture (DAC)). In both systems, the captured CO2 would be injected into deep geologic formations so as to isolate it from the atmosphere. The technical literature is clear that both of these technologies are technically feasible as of today (IPCC, 2005; Keith, 2009; Lackner, 2009; Luckow et al., 2010; Ranjan and Herzog, 2011). What is uncertain is the relative cost of these industrial ambient-air CO2 removal systems when compared to other emissions mitigation measures, the ultimate timing and scale of their deployment, and the resolution of potential site specific constraints that would impact their ultimate commercial deployment.

  3. Thermal analysis of the ambient air around a particle detector

    CERN Document Server

    Gasser, D

    2003-01-01

    The ATLAS particle detector will be in operation at CERN in a few years. The so-called "end cap muon chambers", which form a sub-system of this detector, need to be aligned accurately by means of light rays. Despite the significant amount of heat released in the air by the detector, the rays must not be too much distorted by temperature difference. In order to predict ambient temperature gradient, a thermal analysis is done using a CFD (Computational Fluid Dynamics) model. Because of the complexity of ATLAS geometry, relevant assumptions need to be made in order to get a suitable model for numerical analysis and which give reliable results at the same time.

  4. Capture CO2 from Ambient Air Using Nanoconfined Ion Hydration.

    Science.gov (United States)

    Shi, Xiaoyang; Xiao, Hang; Lackner, Klaus S; Chen, Xi

    2016-03-14

    Water confined in nanoscopic pores is essential in determining the energetics of many physical and chemical systems. Herein, we report a recently discovered unconventional, reversible chemical reaction driven by water quantities in nanopores. The reduction of the number of water molecules present in the pore space promotes the hydrolysis of CO3(2-) to HCO3(-) and OH(-). This phenomenon led to a nano-structured CO2 sorbent that binds CO2 spontaneously in ambient air when the surrounding is dry, while releasing it when exposed to moisture. The underlying mechanism is elucidated theoretically by computational modeling and verified by experiments. The free energy of CO3 (2-) hydrolysis in nanopores reduces with a decrease of water availability. This promotes the formation of OH(-), which has a high affinity to CO2 . The effect is not limited to carbonate/bicarbonate, but is extendable to a series of ions. Humidity-driven sorption opens a new approach to gas separation technology.

  5. Direct Capture of CO2 from Ambient Air.

    Science.gov (United States)

    Sanz-Pérez, Eloy S; Murdock, Christopher R; Didas, Stephanie A; Jones, Christopher W

    2016-10-12

    The increase in the global atmospheric CO2 concentration resulting from over a century of combustion of fossil fuels has been associated with significant global climate change. With the global population increase driving continued increases in fossil fuel use, humanity's primary reliance on fossil energy for the next several decades is assured. Traditional modes of carbon capture such as precombustion and postcombustion CO2 capture from large point sources can help slow the rate of increase of the atmospheric CO2 concentration, but only the direct removal of CO2 from the air, or "direct air capture" (DAC), can actually reduce the global atmospheric CO2 concentration. The past decade has seen a steep rise in the use of chemical sorbents that are cycled through sorption and desorption cycles for CO2 removal from ultradilute gases such as air. This Review provides a historical overview of the field of DAC, along with an exhaustive description of the use of chemical sorbents targeted at this application. Solvents and solid sorbents that interact strongly with CO2 are described, including basic solvents, supported amine and ammonium materials, and metal-organic frameworks (MOFs), as the primary classes of chemical sorbents. Hypothetical processes for the deployment of such sorbents are discussed, as well as the limited array of technoeconomic analyses published on DAC. Overall, it is concluded that there are many new materials that could play a role in emerging DAC technologies. However, these materials need to be further investigated and developed with a practical sorbent-air contacting process in mind if society is to make rapid progress in deploying DAC as a means of mitigating climate change.

  6. Ambient air quality and the effects of air pollutants on otolaryngology in Beijing.

    Science.gov (United States)

    Zhang, Fengying; Xu, Jin; Zhang, Ziying; Meng, Haiying; Wang, Li; Lu, Jinmei; Wang, Wuyi; Krafft, Thomas

    2015-08-01

    To investigate temporal patterns, pollution concentrations and the health effects of air pollutants in Beijing we carried out time-series analyses on daily concentrations of ambient air pollutants and daily numbers of outpatient visits for otolaryngology over 2 years (2011-2012) to identify possible health effects of air pollutants. The results showed that PM10 was the major air pollutant in Beijing and that air quality was slightly better in 2012 than in 2011. Seasonal differences were apparent for SO2 and NO2. Both the background and urban areas of Beijing experienced particulate matter pollution in 2011. In addition to local air pollution, Beijing was also affected by pollutants transported from other regions, especially during heavy air pollution episodes. PM10, NO2, and SO2 concentrations showed positive associations with numbers of outpatient visits for otolaryngology during winter. NO2 and SO2 also had adverse ear, nose, and throat health effects outside of winter. The ear, nose, and throat health risks caused by air pollutants were higher during the winter than during the summer. NO2 had stronger influence on increased the likelihood of outpatient visits than SO2. The findings provide additional information about air quality and health effects of air pollution in Beijing.

  7. Air Quality of Beijing and Impacts of the New Ambient Air Quality Standard

    Directory of Open Access Journals (Sweden)

    Wei Chen

    2015-08-01

    Full Text Available Beijing has been publishing daily reports on its air quality since 2000, and while the air pollution index (API shows that the air quality has improved greatly since 2000, this is not the perception of Beijing’s residents. The new national ambient air quality standard (NAAQS-2012, which includes the monitoring of PM2.5, has posed stricter standards for evaluating air quality. With the new national standard, the air quality in Beijing is calculated using both NAAQS-2012 and the previous standard. The annual attainment rate has dropped from 75.5% to 50.7%. The spatial analysis of air quality shows that only a background station could attain the national standard, while urban and suburban stations exceed the national standard. Among the six pollutants included in the NAAQS-2012, PM2.5 is the major contributor to the air quality index (AQI comparing with the five other pollutants. The results indicate that under previous NAAQS without PM2.5 monitoring, the air quality has improved greatly in the past decade.  By considering PM2.5, the air quality attainment has dropped greatly. Furthermore, a great effort is needed for local government to bring down the PM2.5 concentration.

  8. 78 FR 12052 - Agency Information Collection Activities: Proposed Collection; Comment Request; Ambient Air...

    Science.gov (United States)

    2013-02-21

    ... AGENCY Agency Information Collection Activities: Proposed Collection; Comment Request; Ambient Air... were approved under separate rulemaking actions: ICR 2358 (OMB 2060-0638) Nitrogen Oxides Ambient Monitoring ] ICR 2370 (OMB 2060-0642) Sulfur Dioxides Ambient Monitoring ICR 0940 (OMB 2060-0084) PM...

  9. Heavy metal pollution of ambient air in Nagpur City.

    Science.gov (United States)

    Chaudhari, Pramod R; Gupta, Rakhi; Gajghate, Daulat Ghilagi; Wate, Satish R

    2012-04-01

    Heavy metals released from different sources in urban environment get adsorbed on respirable particulate matter less than 10 μm in size (PM(10)) and are important from public health point of view causing morbidity and mortality. Therefore, the ambient air quality monitoring was carried out to study the temporal and special pattern in the distribution of PM(10) and associated heavy metal content in the atmosphere of Nagpur, Maharashtra State, India during 2001 as well as in 2006. PM(10) fraction was observed to exceed the stipulated standards in both years. It was also observed that minimum range of PM(10) was observed to be increased in 2006 indicating increase in human activity during nighttime also. Six heavy metals were analyzed and were observed to occur in the order Zn > Fe > Pb > Ni > Cd > Cr in 2006, similar to the trend in other metro cities in India. Lead and Nickel were observed to be within the stipulated standards. Poor correlation coefficient (R(2)) between lead and PM(10) indicated that automobile exhaust is not the source of metals to air pollution. Commercial and industrial activity as well as geological composition may be the potential sources of heavy metal pollution. Total load of heavy metals was found to be increased in 2006 with prominent increase in zinc, lead, and nickel in the environment. Public health impacts of heavy metals as well as certain preventive measures to mitigate the impact of heavy metals on public health are also summarized.

  10. Air Entrainment in Dynamic Wetting: Knudsen Effects and the Influence of Ambient Air Pressure

    CERN Document Server

    Sprittles, James E

    2015-01-01

    Recent experiments on coating flows and liquid drop impact both demonstrate that wetting failures caused by air entrainment can be suppressed by reducing the ambient gas pressure. Here, it is shown that non-equilibrium effects in the gas can account for this behaviour, with ambient pressure reductions increasing the gas' mean free path and hence the Knudsen number $Kn$. These effects first manifest themselves through Maxwell slip at the gas' boundaries so that for sufficiently small $Kn$ they can be incorporated into a continuum model for dynamic wetting flows. The resulting mathematical model contains flow structures on the nano-, micro- and milli-metre scales and is implemented into a computational platform developed specifically for such multiscale phenomena. The coating flow geometry is used to show that for a fixed gas-liquid-solid system (a) the increased Maxwell slip at reduced pressures can substantially delay air entrainment, i.e. increase the `maximum speed of wetting', (b) unbounded maximum speeds ...

  11. Artificial intelligence modeling to evaluate field performance of photocatalytic asphalt pavement for ambient air purification.

    Science.gov (United States)

    Asadi, Somayeh; Hassan, Marwa; Nadiri, Ataallah; Dylla, Heather

    2014-01-01

    In recent years, the application of titanium dioxide (TiO₂) as a photocatalyst in asphalt pavement has received considerable attention for purifying ambient air from traffic-emitted pollutants via photocatalytic processes. In order to control the increasing deterioration of ambient air quality, urgent and proper risk assessment tools are deemed necessary. However, in practice, monitoring all process parameters for various operating conditions is difficult due to the complex and non-linear nature of air pollution-based problems. Therefore, the development of models to predict air pollutant concentrations is very useful because it can provide early warnings to the population and also reduce the number of measuring sites. This study used artificial neural network (ANN) and neuro-fuzzy (NF) models to predict NOx concentration in the air as a function of traffic count (Tr) and climatic conditions including humidity (H), temperature (T), solar radiation (S), and wind speed (W) before and after the application of TiO₂ on the pavement surface. These models are useful for modeling because of their ability to be trained using historical data and because of their capability for modeling highly non-linear relationships. To build these models, data were collected from a field study where an aqueous nano TiO₂ solution was sprayed on a 0.2-mile of asphalt pavement in Baton Rouge, LA. Results of this study showed that the NF model provided a better fitting to NOx measurements than the ANN model in the training, validation, and test steps. Results of a parametric study indicated that traffic level, relative humidity, and solar radiation had the most influence on photocatalytic efficiency.

  12. Measurements of volatile hydrocarbons in ambient air coking plant `Walbrzych`

    Energy Technology Data Exchange (ETDEWEB)

    Michalski, R.; Weglarz, A.; Skrok, R. [Polish Academy of Sciences, Zabrze (Poland). Inst. of Environmental Engineering

    1998-12-31

    The air is a matrix very difficult to handle. In addition, the pollutants are usually present at very low concentrations. Many techniques can be used to collect air samples. The simplest way is to use special containers, but this procedure is expensive and time-consuming. The adsorption of pollutants on adsorbents shows a growing interest, despite the difficulty to choose the appropriate support in order to obtain quantitative yields. To overcome this problem, two or three types of adsorbents may be used in series for collecting a wide range of analytes. In addition, the miniaturization of these techniques (i.e. microtraps and solid-phase microextraction) is also very promising: easy to handle, low cost, no solvent required, detection limits at ppt level when sensitive detectors are used. If we have no money for this modern equipment we must use traditional methods for compounds determination. This paper describes measurements of volatile hydrocarbons (such as benzene, toluene, ethylbenzene, xylene and phenol) in ambient air of coking plant `Walbrzych` Measuring points were at streets: Beethoven 4, Dworcowa 2, Kosteckiego 5 and Zamkowa 1. BTEX were collected on graphitized carbon and phenol on Chromosorb 102. After that samples were extracted by solvents (dichloromethane for BTEX or benzene for phenol). Next step was the analysis by gas chromatography with flame ionization detector without preconcentration. The lower limit of detection was circa 0.01 {mu}g/m{sup 3} for each of the determined compounds. These measurements of hydrocarbons in town of Walbrzych were performed for two years from 1996 to 1998. 2 tabs.

  13. 75 FR 22126 - Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods...

    Science.gov (United States)

    2010-04-27

    ... AGENCY Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods: Designation of One New Equivalent Method AGENCY: Environmental Protection Agency. ACTION: Notice of the designation of one new equivalent method for monitoring ambient air quality. SUMMARY: Notice is hereby...

  14. 76 FR 15974 - Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods...

    Science.gov (United States)

    2011-03-22

    ... AGENCY Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods: Designation of Four New Equivalent Methods AGENCY: Environmental Protection Agency. ACTION: Notice of the designation of four new equivalent methods for monitoring ambient air quality. SUMMARY: Notice is hereby...

  15. 75 FR 30022 - Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods...

    Science.gov (United States)

    2010-05-28

    ... AGENCY Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods: Designation of One New Equivalent Method AGENCY: Environmental Protection Agency. ACTION: Notice of the designation of one new equivalent method for monitoring ambient air quality. SUMMARY: Notice is hereby...

  16. 75 FR 51039 - Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods...

    Science.gov (United States)

    2010-08-18

    ... AGENCY Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods: Designation of Two New Equivalent Methods AGENCY: Environmental Protection Agency. ACTION: Notice of the designation of two new equivalent methods for monitoring ambient air quality. SUMMARY: Notice is hereby...

  17. 75 FR 45627 - Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods...

    Science.gov (United States)

    2010-08-03

    ... AGENCY Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods: Designation of One New Equivalent Method AGENCY: Environmental Protection Agency. ACTION: Notice of the designation of one new equivalent method for monitoring ambient air quality. SUMMARY: Notice is hereby...

  18. 78 FR 67360 - Ambient Air Monitoring Reference and Equivalent Methods: Designation of Five New Equivalent Methods

    Science.gov (United States)

    2013-11-12

    ... AGENCY Ambient Air Monitoring Reference and Equivalent Methods: Designation of Five New Equivalent... of the designation of five new equivalent methods for monitoring ambient air quality. SUMMARY: Notice... measuring concentrations of PM 10-2.5 , two for measuring PM 2.5, and one for measuring NO 2 in the...

  19. 76 FR 76972 - Release of Final Integrated Review Plan for the National Ambient Air Quality Standards for Lead

    Science.gov (United States)

    2011-12-09

    ... AGENCY Release of Final Integrated Review Plan for the National Ambient Air Quality Standards for Lead... the National Ambient Air Quality Standards for Lead. This document contains the plans for the review of the air quality criteria and national ambient air quality standards (NAAQS) for lead (Pb). The...

  20. 76 FR 20347 - Release of Draft Integrated Review Plan for the National Ambient Air Quality Standards for Lead

    Science.gov (United States)

    2011-04-12

    ... AGENCY Release of Draft Integrated Review Plan for the National Ambient Air Quality Standards for Lead... National Ambient Air Quality Standards for Lead (draft IRP). This document contains the plans for the review of the air quality criteria and national ambient air quality standards (NAAQS) for lead (Pb)....

  1. 40 CFR 50.10 - National 8-hour primary and secondary ambient air quality standards for ozone.

    Science.gov (United States)

    2010-07-01

    ... ambient air quality standards for ozone. 50.10 Section 50.10 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) AIR PROGRAMS NATIONAL PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS § 50.10 National 8-hour primary and secondary ambient air quality standards for ozone. (a) The level...

  2. 40 CFR 50.9 - National 1-hour primary and secondary ambient air quality standards for ozone.

    Science.gov (United States)

    2010-07-01

    ... ambient air quality standards for ozone. 50.9 Section 50.9 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) AIR PROGRAMS NATIONAL PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS § 50.9 National 1-hour primary and secondary ambient air quality standards for ozone. (a) The level...

  3. Ambient air cooling arrangement having a pre-swirler for gas turbine engine blade cooling

    Science.gov (United States)

    Lee, Ching-Pang; Tham, Kok-Mun; Schroeder, Eric; Meeroff, Jamie; Miller, Jr., Samuel R; Marra, John J

    2015-01-06

    A gas turbine engine including: an ambient-air cooling circuit (10) having a cooling channel (26) disposed in a turbine blade (22) and in fluid communication with a source (12) of ambient air: and an pre-swirler (18), the pre-swirler having: an inner shroud (38); an outer shroud (56); and a plurality of guide vanes (42), each spanning from the inner shroud to the outer shroud. Circumferentially adjacent guide vanes (46, 48) define respective nozzles (44) there between. Forces created by a rotation of the turbine blade motivate ambient air through the cooling circuit. The pre-swirler is configured to impart swirl to ambient air drawn through the nozzles and to direct the swirled ambient air toward a base of the turbine blade. The end walls (50, 54) of the pre-swirler may be contoured.

  4. Evaluation of Air Quality Zone Classification Methods Based on Ambient Air Concentration Exposure.

    Science.gov (United States)

    Freeman, Brian; McBean, Ed; Gharabaghi, Bahram; Thé, Jesse

    2016-12-14

    Air quality zones are used by regulatory authorities to implement ambient air standards in order to protect human health. Air quality measurements at discrete air monitoring stations are critical tools to determine whether an air quality zone complies with local air quality standards or is noncompliant. This study presents a novel approach for evaluation of air quality zone classification methods by breaking the concentration distribution of a pollutant measured at an air monitoring station into compliance and exceedance probability density functions (PDFs) and then using Monte Carlo analysis with the Central Limit Theorem to estimate long-term exposure. The purpose of this paper is to compare the risk associated with selecting one ambient air classification approach over another by testing the possible exposure an individual living within a zone may face. The chronic daily intake (CDI) is utilized to compare different pollutant exposures over the classification duration of 3 years between two classification methods. Historical data collected from air monitoring stations in Kuwait are used to build representative models of 1-hr NO2 and 8-hr O3 within a zone that meets the compliance requirements of each method. The first method, the "3 Strike" method, is a conservative approach based on a winner-take-all approach common with most compliance classification methods, while the second, the 99% Rule method, allows for more robust analyses and incorporates long-term trends. A Monte Carlo analysis is used to model the CDI for each pollutant and each method with the zone at a single station and with multiple stations. The model assumes that the zone is already in compliance with air quality standards over the 3 years under the different classification methodologies. The model shows that while the CDI of the two methods differs by 2.7% over the exposure period for the single station case, the large number of samples taken over the duration period impacts the sensitivity of

  5. 40 CFR Appendix D to Part 58 - Network Design Criteria for Ambient Air Quality Monitoring

    Science.gov (United States)

    2010-07-01

    ...—Network Design Criteria for Ambient Air Quality Monitoring 1. Monitoring Objectives and Spatial Scales 2... trends in air pollution abatement control measures' impact on improving air quality. In monitoring... required monitoring stations or sites must be sited to represent community-wide air quality. These...

  6. Ambient air pollution and the progression of atherosclerosis in adults.

    Directory of Open Access Journals (Sweden)

    Nino Künzli

    Full Text Available BACKGROUND: Cross-sectional studies suggest an association between exposure to ambient air pollution and atherosclerosis. We investigated the association between outdoor air quality and progression of subclinical atherosclerosis (common carotid artery intima-media thickness, CIMT. METHODOLOGY/PRINCIPAL FINDINGS: We examined data from five double-blind randomized trials that assessed effects of various treatments on the change in CIMT. The trials were conducted in the Los Angeles area. Spatial models and land-use data were used to estimate the home outdoor mean concentration of particulate matter up to 2.5 micrometer in diameter (PM2.5, and to classify residence by proximity to traffic-related pollution (within 100 m of highways. PM2.5 and traffic proximity were positively associated with CIMT progression. Adjusted coefficients were larger than crude associations, not sensitive to modelling specifications, and statistically significant for highway proximity while of borderline significance for PM2.5 (P = 0.08. Annual CIMT progression among those living within 100 m of a highway was accelerated (5.5 micrometers/yr [95%CI: 0.13-10.79; p = 0.04] or more than twice the population mean progression. For PM2.5, coefficients were positive as well, reaching statistical significance in the socially disadvantaged; in subjects reporting lipid lowering treatment at baseline; among participants receiving on-trial treatments; and among the pool of four out of the five trials. CONCLUSION: Consistent with cross-sectional findings and animal studies, this is the first study to report an association between exposure to air pollution and the progression of atherosclerosis--indicated with CIMT change--in humans. Ostensibly, our results suggest that air pollution may contribute to the acceleration of cardiovascular disease development--the main causes of morbidity and mortality in many countries. However, the heterogeneity of the volunteering populations across the

  7. Will the circle be unbroken: a history of the U.S. National Ambient Air Quality Standards.

    Science.gov (United States)

    Bachmann, John

    2007-06-01

    In celebration of the 100th anniversary of the Air & Waste Management Association, this review examines the history of air quality management (AQM) in the United States over the last century, with an emphasis on the ambient standards programs established by the landmark 1970 Clean Air Act (CAA) Amendments. The current CAA system is a hybrid of several distinct air pollution control philosophies, including the recursive or circular system driven by ambient standards. Although this evolving system has resulted in tremendous improvements in air quality, it has been far from perfect in terms of timeliness and effectiveness. The paper looks at several periods in the history of the U.S. program, including: (1) 1900-1970, spanning the early smoke abatement and smog control programs, the first federal involvement, and the development of a hybrid AQM approach in the 1970 CAA; (2) 1971-1976, when the first National Ambient Air Quality Standards (NAAQS) were set and implemented; (3) 1977-1993, a period of the first revisions to the standards, new CAA Amendments, delays in implementation and decision-making, and key science/policy/legislative developments that would alter both the focus and scale of air pollution programs and how they are implemented; and (4) 1993-2006, the second and third wave of NAAQS revisions and their implementation in the context of the 1990 CAA. This discussion examines where NAAQS have helped drive implementation programs and how improvements in both effects and air quality/control sciences influenced policy and legislation to enhance the effectiveness of the system over time. The review concludes with a look toward the future of AQM, emphasizing challenges and ways to meet them. The most significant of these is the need to make more efficient progress toward air quality goals, while adjusting the system to address the growing intersections between air quality management and climate change.

  8. Assessing environmental inequalities in ambient air pollution across urban Australia.

    Science.gov (United States)

    Knibbs, Luke D; Barnett, Adrian G

    2015-04-01

    Identifying inequalities in air pollution levels across population groups can help address environmental justice concerns. We were interested in assessing these inequalities across major urban areas in Australia. We used a land-use regression model to predict ambient nitrogen dioxide (NO2) levels and sought the best socio-economic and population predictor variables. We used a generalised least squares model that accounted for spatial correlation in NO2 levels to examine the associations between the variables. We found that the best model included the index of economic resources (IER) score as a non-linear variable and the percentage of non-Indigenous persons as a linear variable. NO2 levels decreased with increasing IER scores (higher scores indicate less disadvantage) in almost all major urban areas, and NO2 also decreased slightly as the percentage of non-Indigenous persons increased. However, the magnitude of differences in NO2 levels was small and may not translate into substantive differences in health.

  9. ISS Ambient Air Quality: Updated Inventory of Known Aerosol Sources

    Science.gov (United States)

    Meyer, Marit

    2014-01-01

    Spacecraft cabin air quality is of fundamental importance to crew health, with concerns encompassing both gaseous contaminants and particulate matter. Little opportunity exists for direct measurement of aerosol concentrations on the International Space Station (ISS), however, an aerosol source model was developed for the purpose of filtration and ventilation systems design. This model has successfully been applied, however, since the initial effort, an increase in the number of crewmembers from 3 to 6 and new processes on board the ISS necessitate an updated aerosol inventory to accurately reflect the current ambient aerosol conditions. Results from recent analyses of dust samples from ISS, combined with a literature review provide new predicted aerosol emission rates in terms of size-segregated mass and number concentration. Some new aerosol sources have been considered and added to the existing array of materials. The goal of this work is to provide updated filtration model inputs which can verify that the current ISS filtration system is adequate and filter lifetime targets are met. This inventory of aerosol sources is applicable to other spacecraft, and becomes more important as NASA considers future long term exploration missions, which will preclude the opportunity for resupply of filtration products.

  10. Synthesis of ammonia directly from air and water at ambient temperature and pressure.

    Science.gov (United States)

    Lan, Rong; Irvine, John T S; Tao, Shanwen

    2013-01-01

    The N≡N bond (225 kcal mol⁻¹) in dinitrogen is one of the strongest bonds in chemistry therefore artificial synthesis of ammonia under mild conditions is a significant challenge. Based on current knowledge, only bacteria and some plants can synthesise ammonia from air and water at ambient temperature and pressure. Here, for the first time, we report artificial ammonia synthesis bypassing N₂ separation and H₂ production stages. A maximum ammonia production rate of 1.14 × 10⁻⁵ mol m⁻² s⁻¹ has been achieved when a voltage of 1.6 V was applied. Potentially this can provide an alternative route for the mass production of the basic chemical ammonia under mild conditions. Considering climate change and the depletion of fossil fuels used for synthesis of ammonia by conventional methods, this is a renewable and sustainable chemical synthesis process for future.

  11. Impact of air traffic on the climate

    Energy Technology Data Exchange (ETDEWEB)

    Stief, G. [Florence Univ. (Italy). Ist. di Agrometeorologia

    1997-12-31

    Though emission from world-wide air traffic may seem to be relatively small in comparison to that from all other anthropogenic sources, the deleterious effect on the climate of the gases and particles emitted by planes is disproportionately large. It is thought that air traffic, working together with pollutants that have already accumulated at critical heights, and depending on humidity and temperature, plays a decisive role in helping to cause the changes, presented below, in global radiation, sunshine duration, rainfall and maximum and minimum temperatures which are taking place. (author) 7 refs.

  12. Experimental Investigation of the Effect of Change in Ambient Air Temperature on Power Consumption of Domestic Refrigerators

    Directory of Open Access Journals (Sweden)

    J. A. Olorunmaiye

    2012-12-01

    Full Text Available One of the manifestations of climate change is increase.in ambient air temperature usually referred to as global warming. For sustainable development in a country, there is need to identify impacts of climate change and the necessary adaptation and mitigation strategies to adopt. To simulate the effect of global warming on the power consumption of refrigerators, a (model No. 150 THERMOCOOL refrigerator filled with twenty-five 750cl packaged water bottleswas run in an air-conditioned room, in a room with the air-conditioner switched off and near an oven in a bakery. The electric power consumption of the refrigerator was measured using "Watts up?.net" Watt meter and the ambient temperature was measured using FLUKE temperature/humidity meter. The average hourly energy consumption of the refrigerator operating at mean ambient temperatures of 25.4°C, 30.7oC, 38.8°C were 93.844 Wh, 100.32 Wh and 105.08 Wh respectively. Some possible ways to reduce the increase in power consumption of refrigerators due to global warming include using compressors of higher efficiency and condensers of greater effectiveness.

  13. 40 CFR Appendix S to Part 50 - Interpretation of the Primary National Ambient Air Quality Standards for Oxides of Nitrogen...

    Science.gov (United States)

    2010-07-01

    ... Ambient Air Quality Standards for Oxides of Nitrogen (Nitrogen Dioxide) S Appendix S to Part 50 Protection... National Ambient Air Quality Standards for Oxides of Nitrogen (Nitrogen Dioxide) 1. General (a) This... national ambient air quality standards for oxides of nitrogen as measured by nitrogen dioxide (“NO2...

  14. 75 FR 1566 - Public Hearings for Reconsideration of the 2008 National Ambient Air Quality Standards for Ozone

    Science.gov (United States)

    2010-01-12

    ... Ambient Air Quality Standards for Ozone AGENCY: Environmental Protection Agency (EPA). ACTION... proposed rule, ``Reconsideration of the 2008 National Ambient Air Quality Standards for Ozone,'' which was... 2008 National Ambient Air Quality Standards for Ozone'' proposed rule should be addressed to Ms....

  15. 76 FR 48073 - Public Hearing for Secondary National Ambient Air Quality Standards for Oxides of Nitrogen and...

    Science.gov (United States)

    2011-08-08

    ... AGENCY 40 CFR Part 50 RIN 2060-AO72 Public Hearing for Secondary National Ambient Air Quality Standards... titled ``Secondary National Ambient Air Quality Standards for Oxides of Nitrogen and Sulfur'' which was... ``Secondary National Ambient Air Quality Standards for Oxides of Nitrogen and Sulfur'' proposed rule should...

  16. 75 FR 39253 - Release of Second Draft Document Related to the Review of the National Ambient Air Quality...

    Science.gov (United States)

    2010-07-08

    ... AGENCY Release of Second Draft Document Related to the Review of the National Ambient Air Quality... Assessment for the Review of the Particulate Matter National Ambient Air Quality Standards--Second External... revise the standards as part of the review of the national ambient air quality standards (NAAQS)...

  17. Influence of the ambient air temperature on the electrical contact reliability of electromagnetic relay

    Institute of Scientific and Technical Information of China (English)

    YAO Fang; ZHENG Jian-rong; HUANG Zhang-wu

    2007-01-01

    The dynamic contact resistances of HH52P electromagnetic relays are measured under different ambient air temperature. Their diagnostic parameters are extracted and determined. It is found that the ambient air temperature obviously influences some parameters. In order to research its influence on the electrical contact reliability of electromagnetic relay, the statistic analysis is applied to study the static contact resistance, the max of the dynamic contact resistance and the bounce time. It is found that the ambient air temperature regularly influences the three parameters. Thoroughly, the phenomenon is studied and analyzed in the point of material science so as to probe into the essential matter of it.

  18. 78 FR 44485 - Implementation of the 2008 National Ambient Air Quality Standards for Ozone: State Implementation...

    Science.gov (United States)

    2013-07-24

    ... AGENCY 40 CFR Parts 50, 51, 70 and 71 Implementation of the 2008 National Ambient Air Quality Standards... on this rulemaking, contact Dr. Karl Pepple, Office of Air Quality Planning and Standards, U.S... Stackhouse, Office of Air Quality Planning and Standards, U.S. Environmental Protection Agency, by phone...

  19. Coupling between air travel and climate

    Science.gov (United States)

    Karnauskas, Kristopher B.; Donnelly, Jeffrey P.; Barkley, Hannah C.; Martin, Jonathan E.

    2015-12-01

    The airline industry closely monitors the midlatitude jet stream for short-term planning of flight paths and arrival times. In addition to passenger safety and on-time metrics, this is due to the acute sensitivity of airline profits to fuel cost. US carriers spent US$47 billion on jet fuel in 2011, compared with a total industry operating revenue of US$192 billion. Beyond the timescale of synoptic weather, the El Niño/Southern Oscillation (ENSO), Arctic Oscillation (AO) and other modes of variability modulate the strength and position of the Aleutian low and Pacific high on interannual timescales, which influence the tendency of the exit region of the midlatitude Pacific jet stream to extend, retract and meander poleward and equatorward. The impact of global aviation on climate change has been studied for decades owing to the radiative forcing of emitted greenhouse gases, contrails and other effects. The impact of climate variability on air travel, however, has only recently come into focus, primarily in terms of turbulence. Shifting attention to flight durations, here we show that 88% of the interannual variance in domestic flight times between Hawaii and the continental US is explained by a linear combination of ENSO and the AO. Further, we extend our analysis to CMIP5 model projections to explore potential feedbacks between anthropogenic climate change and air travel.

  20. RELATIONSHIP BETWEEN AMBIENT AIR QUALITY AND SELECTED BIRTH DEFECTS, SEVEN COUNTY STUDY, TEXAS, 1997-2000

    Science.gov (United States)

    Background and Objectives: A number of epidemiologic investigations have shown adverse effects of ambient air pollution on reproductive outcomes including spontaneous abortion, fetal growth, preterm delivery, and infant mortality. A southern California, population-based, case-c...

  1. Single and double long pulse laser ablation of aluminum induced in air and water ambient

    Science.gov (United States)

    Akbari Jafarabadi, Marzieh; Mahdieh, Mohammad Hossein

    2017-02-01

    In this paper, single pulse and double pulse laser ablation of an aluminum target in two interaction ambient was investigated experimentally. The interaction was performed by nanosecond Nd:YAG laser beam in air and four depths (i.e. 9, 13, 17, and 21 mm) of distilled water ambient. The irradiation was carried out in single and collinear double pulse configurations in both air and liquid ambient. Crater geometry (depth and diameter) was measured by an optical microscope. The results indicated that the crater geometry strongly depends on both single pulse and double pulse configurations and interaction ambient. In single pulse regime, the crater diameter is higher for all water depths compared to that of air. However, the crater depth, depend on water depth, is higher or lower than the crater depth in air. In double pulse laser ablation, there are greater values for both crater diameters and crater depths in the water.

  2. Comparison of exposure estimation methods for air pollutants: ambient monitoring data and regional air quality simulation.

    Science.gov (United States)

    Bravo, Mercedes A; Fuentes, Montserrat; Zhang, Yang; Burr, Michael J; Bell, Michelle L

    2012-07-01

    Air quality modeling could potentially improve exposure estimates for use in epidemiological studies. We investigated this application of air quality modeling by estimating location-specific (point) and spatially-aggregated (county level) exposure concentrations of particulate matter with an aerodynamic diameter less than or equal to 2.5 μm (PM(2.5)) and ozone (O(3)) for the eastern U.S. in 2002 using the Community Multi-scale Air Quality (CMAQ) modeling system and a traditional approach using ambient monitors. The monitoring approach produced estimates for 370 and 454 counties for PM(2.5) and O(3), respectively. Modeled estimates included 1861 counties, covering 50% more population. The population uncovered by monitors differed from those near monitors (e.g., urbanicity, race, education, age, unemployment, income, modeled pollutant levels). CMAQ overestimated O(3) (annual normalized mean bias=4.30%), while modeled PM(2.5) had an annual normalized mean bias of -2.09%, although bias varied seasonally, from 32% in November to -27% in July. Epidemiology may benefit from air quality modeling, with improved spatial and temporal resolution and the ability to study populations far from monitors that may differ from those near monitors. However, model performance varied by measure of performance, season, and location. Thus, the appropriateness of using such modeled exposures in health studies depends on the pollutant and metric of concern, acceptable level of uncertainty, population of interest, study design, and other factors.

  3. Ambient air quality and asthma cases in Niğde, Turkey.

    Science.gov (United States)

    Kara, Ertan; Özdilek, Hasan Göksel; Kara, Emine Erman

    2013-06-01

    Urban air quality is one of the key factors affecting human health. Turkey has transformed itself into an urban society over the last 30 years. At the same time, air pollution has become a serious impairment to health in many urban areas in the country. This is due to many reasons. In this study, a nonparametric evaluation was conducted of health effects that are triggered by urban air pollution. Niğde, the city which is the administrative centre of Nigde province was chosen of the effects of air pollution since, like many central Turkish cities, it is situated on a valley where atmospheric inversion occurs. In this paper, the relationship between ambient urban air quality, namely PM10 and sulphur dioxide (SO2), and human health, specifically asthma, during the winter season is examined. Air pollution data and asthma cases from 2006 to 2010 are covered in this study. The results of our study indicate that total asthma cases reported in Nigde between 2008 and 2010 were highly dependent on ambient SO2 concentration. More asthma cases were recorded when 30 μg m(-3) or higher SO2 was present in the ambient air than those recorded under cleaner ambient air conditions. Moreover, it was determined that in Nigde in 2010, asthma cases reported in males aged between 45 and 64 were closely correlated with ambient SO2 (α=0.05).

  4. Testing of blowers and HVAC systems. Guide for energy optimization regarding ambient air ventilation systems. Pruefungen von Ventilatoren und Raumlufttechnischen Geraeten. Wegweiser zur Energieoptimierung bei RLT-Geraeten

    Energy Technology Data Exchange (ETDEWEB)

    Breit, O.

    1992-09-01

    Through a continuously increasing environmental consciousness and the increase of energy cost to be expected in the next years, ambient air ventilation systems with an optimized energy consumption are increasingly applied. For the determination of the energy consumption, special test rigs for the capacity are necessary. They consist of two climatic chambers arranged side by side, two measured sections and two speed controlled supporting fans. The tests carried out on the capacity and function of ambient air ventilation systems showed that the power consumption and thus, the energy consumption can be considerably reduced through constructional changes and an exact design of single components based on measured results. (BWI).

  5. Urban air pollution climates throughout the world

    DEFF Research Database (Denmark)

    Hertel, Ole; Goodsite, Michael Evan

    2009-01-01

    as well as the transport in and out of the city area. The building obstacles play a crucial role in causing generally high pollutant levels in the urban environment, especially inside street canyons where the canyon vortex flow governs the pollution distribution. Of the pollutants dominating urban air......The extent of the urban area, the local emission density, and the temporal pattern in the releases govern the local contribution to air pollution levels in urban environments. However, meteorological conditions also heavily affect the actual pollution levels as they govern the dispersion conditions...... pollution climates, particulate pollution in general together with gaseous and particulate polycyclic aromatic hydrocarbons (PAHs) and heavy metals are those where further field measurements, characterization and laboratory studies are urgently needed in order to fully assess the health impact on the urban...

  6. 40 CFR 50.7 - National primary and secondary ambient air quality standards for PM2.5.

    Science.gov (United States)

    2010-07-01

    ... air quality standards for PM2.5. 50.7 Section 50.7 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) AIR PROGRAMS NATIONAL PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS § 50.7 National primary and secondary ambient air quality standards for PM2.5. (a) The national primary...

  7. 40 CFR 50.13 - National primary and secondary ambient air quality standards for PM2.5.

    Science.gov (United States)

    2010-07-01

    ... air quality standards for PM2.5. 50.13 Section 50.13 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) AIR PROGRAMS NATIONAL PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS § 50.13 National primary and secondary ambient air quality standards for PM2.5. (a) The national...

  8. 40 CFR Appendix R to Part 50 - Interpretation of the National Ambient Air Quality Standards for Lead

    Science.gov (United States)

    2010-07-01

    ... Air Quality Standards for Lead R Appendix R to Part 50 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) AIR PROGRAMS NATIONAL PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS Pt. 50, App. R Appendix R to Part 50—Interpretation of the National Ambient Air Quality Standards...

  9. 40 CFR Appendix K to Part 50 - Interpretation of the National Ambient Air Quality Standards for Particulate Matter

    Science.gov (United States)

    2010-07-01

    ... Air Quality Standards for Particulate Matter K Appendix K to Part 50 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) AIR PROGRAMS NATIONAL PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS Pt. 50, App. K Appendix K to Part 50—Interpretation of the National Ambient Air Quality...

  10. The effect of future outdoor air pollution on human health and the contribution of climate change

    Science.gov (United States)

    Silva, R.; West, J. J.; Lamarque, J.; Shindell, D.; Collins, W.; Dalsoren, S. B.; Faluvegi, G. S.; Folberth, G.; Horowitz, L. W.; Nagashima, T.; Naik, V.; Rumbold, S.; Skeie, R.; Sudo, K.; Takemura, T.; Bergmann, D. J.; Cameron-Smith, P. J.; Cionni, I.; Doherty, R. M.; Eyring, V.; Josse, B.; MacKenzie, I. A.; Plummer, D.; Righi, M.; Stevenson, D. S.; Strode, S. A.; Szopa, S.; Zeng, G.

    2013-12-01

    At present, exposure to outdoor air pollution from ozone and fine particulate matter (PM2.5) causes over 2 million deaths per year, due to respiratory and cardiovascular diseases and lung cancer. Future ambient concentrations of ozone and PM2.5 will be affected by both air pollutant emissions and climate change. Here we estimate the potential impact of future outdoor air pollution on premature human mortality, and isolate the contribution of future climate change due to its effect on air quality. We use modeled present-day (2000) and future global ozone and PM2.5 concentrations from simulations with an ensemble of chemistry-climate models from the Atmospheric Chemistry and Climate Model Intercomparison Project (ACCMIP). Future air pollution was modeled for global greenhouse gas and air pollutant emissions in the four IPCC AR5 Representative Concentration Pathway (RCP) scenarios, for 2030, 2050 and 2100. All model outputs are regridded to a common 0.5°x0.5° horizontal resolution. Future premature mortality is estimated for each RCP scenario and year based on changes in concentrations of ozone and PM2.5 relative to 2000. Using a health impact function, changes in concentrations for each RCP scenario are combined with future population and cause-specific baseline mortality rates as projected by a single independent scenario in which the global incidence of cardiopulmonary diseases is expected to increase. The effect of climate change is isolated by considering the difference between air pollutant concentrations from simulations with 2000 emissions and a future year climate and simulations with 2000 emissions and climate. Uncertainties in the results reflect the uncertainty in the concentration-response function and that associated with variability among models. Few previous studies have quantified the effects of future climate change on global human health via changes in air quality, and this is the first such study to use an ensemble of global models.

  11. Impact of fine particles in ambient air on lung cancer

    NARCIS (Netherlands)

    Hoek, Gerard; Raaschou-Nielsen, Ole

    2014-01-01

    Recently, the International Agency for Research on Cancer (IARC) has classified outdoor air pollution and the particulate matter component of outdoor air pollution as class I carcinogen. Air pollution is consistently associated with lung cancer in epidemiologic and experimental studies. The IARC ass

  12. Exploring feedbacks between air pollution and climate policy

    OpenAIRE

    Chuwah, C.D.

    2015-01-01

    The climate of the Earth is changing in response to natural and anthropogenic forcing agents. Emissions of greenhouse gases and air pollutants have led to significant changes in the Earth’s climate systems and projections indicate that further extensive changes are likely. Increased scientific understanding into the processes responsible for climate change and the possible consequences of assumptions regarding future climate and air pollution policy is important to formulate effective r...

  13. Citizen participatory dioxin monitoring campaign by pine needles as biomonitor of ambient air dioxin pollution

    Energy Technology Data Exchange (ETDEWEB)

    Komichi, I.; Takatori, A. [Environmental Research Institute Inc., Tokyo (Japan); Aoyama, T. [Musashi Institute of Technology, Yokohama (Japan). Faculty of Environment and Informations; Vrzic, B. [Maxxam Analytics Inc. HRMS Laboratory, Waterloo, ON (Canada)

    2004-09-15

    The needle-type leaves of Japanese black pine trees (hereafter abbreviated as pine needles) have been used as an effective bio-monitor of ambient air pollution. Miyata Laboratory of Setsunan University has reported that the pine needles accumulate PCDDs and PCDFs (hereafter abbreviated as D/F) through photosynthesis and respiration during their lifetime. On the basis of this study, we have revealed the correlation between ambient air and pine needle concentrations to be estimated at or near 1:10 by analyzing long term continuous ambient dioxin monitoring data and that of pine needles sampled from the same area as ambient air in the Kanagawa Prefecture in 1999. Since then, the citizen groups of each local area all over Japan have started monitoring the ambient air dioxin concentration levels by using pine needles. Samples analyzed during these 5 years totaled more than 650 throughout Japan. The results of these citizen participatory environmental monitoring activities are the tremendous effects achieved in reducing the dioxin levels. This occurs through observation of the dioxin emission sources such as Municipal Solid Waste Incineration Plants as well as the Industrial Waste Incineration plants, which exist in numbers exceeding several thousands in Japan. This short paper will present the results of 56 municipalities of western Japan where ambient air dioxin levels have improved steadily against local averages during these 5 years.

  14. Comparison of stationary and personal air sampling with an air dispersion model for children's ambient exposure to manganese.

    Science.gov (United States)

    Fulk, Florence; Haynes, Erin N; Hilbert, Timothy J; Brown, David; Petersen, Dan; Reponen, Tiina

    2016-09-01

    Manganese (Mn) is ubiquitous in the environment and essential for normal growth and development, yet excessive exposure can lead to impairments in neurological function. This study modeled ambient Mn concentrations as an alternative to stationary and personal air sampling to assess exposure for children enrolled in the Communities Actively Researching Exposure Study in Marietta, OH. Ambient air Mn concentration values were modeled using US Environmental Protection Agency's Air Dispersion Model AERMOD based on emissions from the ferromanganese refinery located in Marietta. Modeled Mn concentrations were compared with Mn concentrations from a nearby stationary air monitor. The Index of Agreement for modeled versus monitored data was 0.34 (48 h levels) and 0.79 (monthly levels). Fractional bias was 0.026 for 48 h levels and -0.019 for monthly levels. The ratio of modeled ambient air Mn to measured ambient air Mn at the annual time scale was 0.94. Modeled values were also time matched to personal air samples for 19 children. The modeled values explained a greater degree of variability in personal exposures compared with time-weighted distance from the emission source. Based on these results modeled Mn concentrations provided a suitable approach for assessing airborne Mn exposure in this cohort.

  15. Biomarkers of ambient air pollution and lung cancer: a systematic review

    NARCIS (Netherlands)

    Demetriou, C.A.; Raaschou-Nielsen, O.; Loft, S.; Møller, P.; Vermeulen, R.; Palli, D.; Chadeau-Hyam, M.; Xun, W.W.; Vineis, P.

    2012-01-01

    The association between ambient air pollution exposure and lung cancer risk has been investigated in prospective studies and the results are generally consistent, indicating that long-term exposure to air pollution may cause lung cancer. Despite the prospective nature and consistent findings of thes

  16. A Passive Sampler for Determination of Nitrogen Dioxide in Ambient Air

    Science.gov (United States)

    Xiao, Dan; Lin, Lianzhi; Yuan, Hongyan; Choi, Martin M. F.; Chan, Winghong

    2005-08-01

    This article describes the use of a passive sampler for detecting and collecting nitrogen dioxide, NO 2 , in ambient air. This device is based on microporous PTFE membranes that allow air samples to diffuse through and subsequently react with an absorbing reagent solution. The absorbance value of this reagent is proportional to the NO 2 concentration in ambient air. It has been successfully applied to determine the NO 2 concentrations in various sampling sites. The sampler is simple, lightweight, and inexpensive. The experiments are suitable for college students in analytical chemistry and environmental studies.

  17. Ambient air pollution triggers wheezing symptoms in infants

    DEFF Research Database (Denmark)

    Andersen, Zorana Jovanovic; Loft, S; Ketzel, Matthias

    2008-01-01

    There is limited evidence for the role of air pollution in the development and triggering of wheezing symptoms in young children. A study was undertaken to examine the effect of exposure to air pollution on wheezing symptoms in children under the age of 3 years with genetic susceptibility to asthma....

  18. HYDROCARBON AND CARBONYL OZONE PRECURSORS IN MEXICO CITY AMBIENT AIR

    Science.gov (United States)

    Urban air pollution is an environmental problem in many cities around the world that has serious immediate and long-term implications to the health of the population and to the physical environment. Mexico City, in particular, faces a severe air pollution problem. The city is...

  19. Ambient air quality monitoring during the H1N1 influence period in Pune (India).

    Science.gov (United States)

    Pathak, M; Deshpande, A; Mirashe, P K; Sorte, R B; Ojha, A

    2010-10-01

    Ambient air quality in an urban area is directly linked with activity level in the city including transport, business and industrial activities. Maharashtra Pollution Control Board (MPCB) has established an ambient air quality network in the city including state-of-the-art continuous air quality monitoring stations which indicate short duration air quality variations for criteria and non-criteria pollutants. The influence of H1N1 outbreak in Pune hitting its worst pandemic condition, led the civic authorities to implement stringent isolation measures including closure of schools, colleges, business malls, cinema halls, etc. Additionally, the fear of such a pandemic brought the city to a stand still. It was therefore necessary to assess the impacts of such activity level on ambient air quality in the city. It has been observed that such events have positive impacts on air quality of the city. There was a decrease in PM concentration almost to the tune of 30 to 40% if the impacts of precipitation, i.e. seasonal variations, are taken into account. Similarly, the non criteria pollutants too showed a marked but unusual decrease in their concentrations in this ever growing city. The influence of these in turn led to lowered concentrations of secondary pollutants, i.e. O3. Overall, the ambient air quality of Pune was found to be improved during the study period.

  20. Ambient air temperature effects on the temperature of sewage sludge composting process

    Institute of Scientific and Technical Information of China (English)

    HUANG Qi-fei; CHEN Tong-bin; GAO Ding; HUANG Ze-chun

    2005-01-01

    Using data obtained with a full-scale sewage sludge composting facility, this paper studied the effects of ambient air temperature on the composting temperature with varying volume ratios of sewage sludge and recycled compost to bulking agent. Two volume ratios were examined experimentally, 1: 0: 1 and 3: 1: 2. The results show that composting temperature was influenced by ambient air temperature and the influence was more significant when composting was in the temperature rising process: composting temperature changed 2.4-6.5℃ when ambient air temperature changed 13℃. On the other hand, the influence was not significant when composting was in the high-temperature and/or temperature falling process: composting temperature changed 0.75-1.3℃ when ambient air temperature changed 8-15 ℃. Hysteresis effect was observed in composting temperature's responses to ambient air temperature. When the ventilation capability of pile was excellent(at a volume ratio of 1:0:1), the hysteresis time was short and ranging 1.1-1.2 h. On the contrary, when the proportion of added bulking agent was low, therefore less porosity in the substrate(at a volume ratio of 3:1:2), the hysteresis time was long and ranging 1.9-3.1 h.

  1. Cloud forming properties of ambient aerosol in the Netherlands and resultant shortwave radiative forcing of climate.

    NARCIS (Netherlands)

    Khlystov, A.

    1998-01-01

    This thesis discusses properties of ambient aerosols in the Netherlands which are controlling the magnitude of the local aerosol radiative forcing. Anthropogenic aerosols influence climate by changing the radiative transfer through the atmosphere via two effects, one is direct and a second is indire

  2. Ambient air pollution and allergic diseases in children

    Directory of Open Access Journals (Sweden)

    Byoung-Ju Kim

    2012-06-01

    Full Text Available The prevalence of allergic diseases has increased worldwide, a phenomenon that can be largely attributed to environmental effects. Among environmental factors, air pollution due to traffic is thought to be a major threat to childhood health. Residing near busy roadways is associated with increased asthma hospitalization, decreased lung function, and increased prevalence and severity of wheezing and allergic rhinitis. Recently, prospective cohort studies using more accurate measurements of individual exposure to air pollution have been conducted and have provided definitive evidence of the impact of air pollution on allergic diseases. Particulate matter and groundlevel ozone are the most frequent air pollutants that cause harmful effects, and the mechanisms underlying these effects may be related to oxidative stress. The reactive oxidative species produced in response to air pollutants can overwhelm the redox system and damage the cell wall, lipids, proteins, and DNA, leading to airway inflammation and hyper-reactivity. Pollutants may also cause harmful effects via epigenetic mechanisms, which control the expression of genes without changing the DNA sequence itself. These mechanisms are likely to be a target for the prevention of allergies. Further studies are necessary to identify children at risk and understand how these mechanisms regulate gene-environment interactions. This review provides an update of the current understanding on the impact of air pollution on allergic diseases in children and facilitates the integration of issues regarding air pollution and allergies into pediatric practices, with the goal of improving pediatric health.

  3. Satellite-based Estimates of Ambient Air Pollution and Global Variations in Childhood Asthma Prevalence

    Science.gov (United States)

    Anderson, H. Ross; Butland, Barbara K.; Donkelaar, Aaron Matthew Van; Brauer, Michael; Strachan, David P.; Clayton, Tadd; van Dingenen, Rita; Amann, Marcus; Brunekreef, Bert; Cohen, Aaron; Dentener, Frank; Lai, Christopher; Lamsal, Lok N.; Martin, Randall V.

    2012-01-01

    Background: The effect of ambient air pollution on global variations and trends in asthma prevalence is unclear. Objectives: Our goal was to investigate community-level associations between asthma prevalence data from the International Study of Asthma and Allergies in Childhood (ISAAC) and satellite-based estimates of particulate matter with aerodynamic diameter prevalence of severe asthma as the outcome and multilevel models to adjust for gross national income (GNI) and center- and country-level sex, climate, and population density. We examined associations (adjusting for GNI) between air pollution and asthma prevalence over time in centers with data from ISAAC Phase One (mid-1900s) and Phase Three (2001-2003). Results: For the 13- to 14-year age group (128 centers in 28 countries), the estimated average within-country change in center-level asthma prevalence per 100 children per 10% increase in center-level PM2.5 and NO2 was -0.043 [95% confidence interval (CI): -0.139, 0.053] and 0.017 (95% CI: -0.030, 0.064) respectively. For ozone the estimated change in prevalence per parts per billion by volume was -0.116 (95% CI: -0.234, 0.001). Equivalent results for the 6- to 7-year age group (83 centers in 20 countries), though slightly different, were not significantly positive. For the 13- to 14-year age group, change in center-level asthma prevalence over time per 100 children per 10% increase in PM2.5 from Phase One to Phase Three was -0.139 (95% CI: -0.347, 0.068). The corresponding association with ozone (per ppbV) was -0.171 (95% CI: -0.275, -0.067). Conclusion: In contrast to reports from within-community studies of individuals exposed to traffic pollution, we did not find evidence of a positive association between ambient air pollution and asthma prevalence as measured at the community level.

  4. 77 FR 51798 - First Draft Documents Related to the Review of the National Ambient Air Quality Standards for Ozone

    Science.gov (United States)

    2012-08-27

    ... AGENCY First Draft Documents Related to the Review of the National Ambient Air Quality Standards for... of the Ozone National Ambient Air Quality Standards: First External Review Draft. The Agency is...-001; July 2012), please contact Ms. Karen Wesson, Office of Air Quality Planning and Standards...

  5. 40 CFR 50.11 - National primary and secondary ambient air quality standards for oxides of nitrogen (with...

    Science.gov (United States)

    2010-07-01

    ... air quality standards for oxides of nitrogen (with nitrogen dioxide as the indicator). 50.11 Section... PRIMARY AND SECONDARY AMBIENT AIR QUALITY STANDARDS § 50.11 National primary and secondary ambient air quality standards for oxides of nitrogen (with nitrogen dioxide as the indicator). (a) The level of...

  6. Statistical Distributions of Ambient Air Pollutants in Shanghai,China

    Institute of Scientific and Technical Information of China (English)

    HAI-DONG KAN; BING-HENG CHEN

    2004-01-01

    To determine the best statistical distribution of concentration data of major air pollutants in Shanghai. Methods Four types of theoretic distributions (lognormal, gamma, Pearson V and extreme value) were chosen to fit daily average concentration data of PM10, SO2 and NO2 from June 1, 2000 to May 31, 2003 in Shanghai by using the maximum likelihood method. The fit results were evaluated by Chi-square test. Results The best-fit distributions for PM10, SO2 and NO2 concentrations in Shanghai were lognormal, Pearson V, and extreme value distributions, respectively. Conclusion The results can be further applied to local air pollution prediction and control, e.g., the probabilities exceeding the air quality standard and emission source reduction of air pollutant concentration to meet the standard.

  7. Ambient Air Pollution and Autism in Los Angeles County, California

    DEFF Research Database (Denmark)

    Becerra, Tracy Ann; Wilhelm, Michelle; Olsen, Jørn

    2013-01-01

    Background: The prevalence of Autistic Disorder (AD), a serious developmental condition, has risen dramatically over the past two decades but high-quality population-based research addressing etiology is limited. Objectives: We studied the influence of exposures to traffic-related air pollution d...... during pregnancy on the development of autism using data from air monitoring stations and a land use regression (LUR) model to estimate exposures....

  8. Exergy analysis of air cooling systems in buildings in hot humid climates

    Energy Technology Data Exchange (ETDEWEB)

    Alpuche, M.G. [UNAM, Temixco, Morelos (Mexico). Posgrado en Ingenieria; Heard, C. [Instituto Mexicano del Petroleo, Mexico DF (Mexico); Best, R.; Rojas, J. [UNAM, Temixco, Morelos (Mexico). Centro de Investigacion en Energia

    2005-03-01

    The purpose of this study is to analyze the influence of using air cooling desiccant systems on reaching thermal comfort conditions in the interior of a building, supposing this to be an open system. Exergy analysis has been carried out for the different design temperatures and relative humidity conditions within those established for ASHRAE summer thermal comfort conditions. The climatic conditions of a hot humid climate such as Villahermosa, Tabasco, Mexico, are used as an example. A novel reference state has been used for the exergy analysis, since this varies according to the fluctuation of the ambient temperature and humidity. (author)

  9. Application of grey weighted related degree to the ambient air quality assessment

    Institute of Scientific and Technical Information of China (English)

    MENG Xian-lin; SHEN Jin; SUN Li-xin; LV Xiao-ying

    2006-01-01

    It is difficult to establish the integrated method to assess the ambient air quality because the atmospheric environmental system is composed of several environmental elements, which contains many contamination factors. In view of the typical grey system character of the monitored data in the ambient air, this paper introduces the weighted value to obtain related degree during applying the method of grey related degree analysis to assess ambient air quality by each polluting factor producing different effects on the environment quality. This method could give more reasonable and reliable evaluating results. Taking the monitored data of Harbin, a provincial city of Heilongjiang, for example in this paper, the result of assessment by this method was coincident with the actual environmental quality of Harbin.

  10. Optimization of non-aqueous electrolytes for Primary lithium/air batteries operated in Ambient Enviroment

    Energy Technology Data Exchange (ETDEWEB)

    Xu, Wu; Xiao, Jie; Zhang, Jian; Wang, Deyu; Zhang, Jiguang

    2009-07-07

    The selection and optimization of non-aqueous electrolytes for ambient operations of lithium/air batteries has been studied. Organic solvents with low volatility and low moisture absorption are necessary to minimize the change of electrolyte compositions and the reaction between lithium anode and water during discharge process. It is critical to make the electrolytes with high polarity so that it can reduce wetting and flooding of carbon based air electrode and lead to improved battery performance. For ambient operations, the viscosity, ionic conductivity, and oxygen solubility of the electrolyte are less important than the polarity of organic solvents once the electrolyte has reasonable viscosity, conductivity, and oxygen solubility. It has been found that PC/EC mixture is the best solvent system and LiTFSI is the most feasible salt for ambient operations of Li/air batteries. Battery performance is not very sensitive to PC/EC ratio or salt concentration.

  11. Effects of respirator ambient air cooling on thermophysiological responses and comfort sensations.

    Science.gov (United States)

    Caretti, David M; Barker, Daniel J

    2014-01-01

    This investigation assessed the thermophysiological and subjective impacts of different respirator ambient air cooling options while wearing chemical and biological personal protective equipment in a warm environment (32.7 ± 0.4°C, 49.6 ± 6.5% RH). Ten volunteers participated in 90-min heat exposure trials with and without respirator (Control) wear and performed computer-generated tasks while seated. Ambient air cooling was provided to respirators modified to blow air to the forehead (FHC) or to the forehead and the breathing zone (BZC) of a full-facepiece air-purifying respirator using a low-flow (45 L·min(-1)) mini-blower. An unmodified respirator (APR) trial was also completed. The highest body temperatures (TTY) and least favorable comfort ratings were observed for the APR condition. With ambient cooling over the last 60 min of heat exposure, TTY averaged 37.4 ± 0.6°C for Control, 38.0 ± 0.4°C for APR, 37.8 ± 0.5°C for FHC, and 37.6 ± 0.7°C for BZC conditions independent of time. Both the FHC and BZC ambient air cooling conditions reduced facial skin temperatures, reduced the rise in body temperatures, and led to more favorable subjective comfort and thermal sensation ratings over time compared to the APR condition; however statistical differences among conditions were inconsistent. Independent of exposure time, average breathing apparatus comfort scores with BZC (7.2 ± 2.5) were significantly different from both Control (8.9 ± 1.4) and APR (6.5 ± 2.2) conditions when ambient cooling was activated. These findings suggest that low-flow ambient air cooling of the face under low work rate conditions and mild hyperthermia may be a practical method to minimize the thermophysiological strain and reduce perceived respirator discomfort.

  12. ambiental

    Directory of Open Access Journals (Sweden)

    Roque Leal Salcedo

    2008-01-01

    Full Text Available El derecho internacional ambiental es un conocimiento de carácter transversal, que entre otras consideraciones refleja las preocupaciones de la sociedad por la implementación de un modelo de desarrollo sustentable para el respeto a las reglas del medio natural que garantizan la integridad y renovación de los sistemas naturales. El presente artículo enfoca esta visión a través del análisis de material documental revisado, entre ellos tratados internacionales que permiten distinguir el desarrollo del derecho internacional ambiental y el papel de Organización de las Naciones Unidas (ONU, en el propósito común del derecho individual y colectivo de disfrutar de una vida, un ambiente seguro, sano y ecológicamente equilibrado. En función a estas disertaciones las consideraciones finales exponen parte de la visión que ha estructurado la ONU y que representan un aporte considerable en el fomento de la conciencia mundial sobre la necesidad de establecer vínculos entre las naciones para el continuo desarrollo de esta rama del derecho.

  13. Effects of ambient air temperature, humidity and rainfall on annual survival of adult little penguins Eudyptula minor in southeastern Australia

    Science.gov (United States)

    Ganendran, L. B.; Sidhu, L. A.; Catchpole, E. A.; Chambers, L. E.; Dann, P.

    2016-08-01

    Seabirds are subject to the influences of local climate variables during periods of land-based activities such as breeding and, for some species, moult; particularly if they undergo a catastrophic moult (complete simultaneous moult) as do penguins. We investigated potential relationships between adult penguin survival and land-based climate variables (ambient air temperature, humidity and rainfall) using 46 years of mark-recapture data of little penguins Eudyptula minor gathered at a breeding colony on Phillip Island in southeastern Australia. Our results showed that adult penguin survival had a stronger association with land-based climate variables during the moult period, when birds were unable to go to sea for up to 3 weeks, than during the breeding period, when birds could sacrifice breeding success in favour of survival. Annual adult survival probability was positively associated with humidity during moult and negatively associated with rainfall during moult. Prolonged heat during breeding and moult had a negative association with annual adult survival. Local climate projections suggest increasing days of high temperatures, fewer days of rainfall which will result in more droughts (and by implication, lower humidity) and more extreme rainfall events. All of these predicted climate changes are expected to have a negative impact on adult penguin survival.

  14. 75 FR 2938 - National Ambient Air Quality Standards for Ozone

    Science.gov (United States)

    2010-01-19

    ... their oral testimonies either electronically on computer disk, CD-ROM, or in paper copy. The hearing... Clean Air Scientific Advisory Committee (CASAC) of EPA's Science Advisory Board. B. Related Control... deterministic to a statistical form, which defined attainment of the standards as occurring when the...

  15. Comparison of stationary and personal air sampling with an air dispersion model for children’s ambient exposure to manganese

    Science.gov (United States)

    Manganese (Mn) is ubiquitous in the environment and essential for normal growth and development, yet excessive exposure can lead to impairments in neurological function. This study modeled ambient Mn concentrations as an alternative to stationary and personal air sampling to asse...

  16. Ambient air pollution and allergic diseases in children

    OpenAIRE

    Byoung-Ju Kim; Soo-Jong Hong

    2012-01-01

    The prevalence of allergic diseases has increased worldwide, a phenomenon that can be largely attributed to environmental effects. Among environmental factors, air pollution due to traffic is thought to be a major threat to childhood health. Residing near busy roadways is associated with increased asthma hospitalization, decreased lung function, and increased prevalence and severity of wheezing and allergic rhinitis. Recently, prospective cohort studies using more accurate measurements of ind...

  17. Megacities, air quality and climate: Seamless prediction approach

    Science.gov (United States)

    Baklanov, Alexander; Molina, Luisa T.; Gauss, Michael

    2016-04-01

    The rapid urbanization and growing number of megacities and urban complexes requires new types of research and services that make best use of science and available technology. With an increasing number of humans now living in urban sprawls, there are urgent needs of examining what the rising number of megacities means for air pollution, local climate and the effects these changes have on global climate. Such integrated studies and services should assist cities in facing hazards such as storm surge, flooding, heat waves, and air pollution episodes, especially in changing climates. While important advances have been made, new interdisciplinary research studies are needed to increase our understanding of the interactions between emissions, air quality, and regional and global climates. Studies need to address both basic and applied research and bridge the spatial and temporal scales connecting local emissions and air pollution and local weather, global atmospheric chemistry and climate. This paper reviews the current status of studies of the complex interactions between climate, air quality and megacities, and identifies the main gaps in our current knowledge as well as further research needs in this important field of research. Highlights • Climate, air quality and megacities interactions: gaps in knowledge, research needs. • Urban hazards: pollution episodes, storm surge, flooding, heat waves, public health. • Global climate change affects megacities' climate, environment and comfort. • Growing urbanization requires integrated weather, environment and climate monitoring systems. • New generation of multi-scale models and seamless integrated urban services are needed. Reference Baklanov, A., L.T. Molina, M. Gauss (2016) Megacities, air quality and climate. Atmospheric Environment, 126: 235-249. doi:10.1016/j.atmosenv.2015.11.059

  18. Impact of Ambient Air Pollution on Public Health under Various Traffic Policies in Shanghai,China

    Institute of Scientific and Technical Information of China (English)

    CHAN-GHONG CHEN; HAI-DONG KAN; CHENG HUANG; LI LI; YUN-HUI ZHANG; REN-JIE CHEN; BING-HENG CHEN

    2009-01-01

    Objective To investigate the potential impact of ambient air pollution on public health under various traffic policies in Shanghai. Methods The exposure level of Shanghai residents to air pollution under various planned traffic scenarios was estimated,and the public health impact was assessed using concentration-response functions derived from available epidemiological studies. Results Our results showed that ambient air pollution in relation to traffic scenarios had a significant impact on the future health status of Shanghai residents.Compared with the base case scenario,implementation of various traffic scenarios could prevent 759-1574,1885-2420,and 2277-2650 PM10-related avoidable deaths (mean-value) in 2010,2015,and 2020,respectively.It could also decrease the incidence of several relevant diseases. Conclusion Our findings emphasize the need to consider air pollution-related health effects as an important impact of traffic policy in Shanghai.

  19. Relationship between PAHs Concentrations in Ambient Air and Deposited on Pine Needles

    OpenAIRE

    Chun, Man Young

    2011-01-01

    Objectives This study was carried out to determine whether or not pine needles can be used as passive samplers of atmospheric polycyclic aromatic hydrocarbons (PAHs) using the correlation between accumulated PAH concentrations in air (Ca, ng/m3) and those deposited on pine needles (Cp, ng/g dry). Methods PAHs in ambient air was collected using low volume PUF sampler and pine needles was gathered at same place for 7 months. Results good correlation (R2=0.8582, p

  20. Ambient Air for Offshore Liquified Natural Gas Broadwater Project

    Science.gov (United States)

    This document may be of assistance in applying the New Source Review (NSR) air permitting regulations including the Prevention of Significant Deterioration (PSD) requirements. This document is part of the NSR Policy and Guidance Database. Some documents in the database are a scanned or retyped version of a paper photocopy of the original. Although we have taken considerable effort to quality assure the documents, some may contain typographical errors. Contact the office that issued the document if you need a copy of the original.

  1. 76 FR 62402 - Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods...

    Science.gov (United States)

    2011-10-07

    ... AGENCY Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods; Designation of One New Equivalent Method AGENCY: Environmental Protection Agency. ACTION: Notice of the..., Research Triangle Park, North Carolina 27711. Designation of this new equivalent method is intended...

  2. Report on sampling and analysis of ambient air at the central waste complex

    Energy Technology Data Exchange (ETDEWEB)

    Stauffer, M., Fluor Daniel Hanford

    1997-02-13

    Over 160 ambient indoor air samples were collected from warehouses at the Central Waste Complex used for the storage of low- level radioactive and mixed wastes. These grab (SUMMA) samples were analyzed by gas chromatography-mass spectrometry using a modified EPA TO-14 procedure. The data from this survey suggest that several buildings had elevated concentrations of volatile organic compounds.

  3. Comparison of the measurement techniques employed for evaluation of ambient air odor quality

    Science.gov (United States)

    Wojnowski, Wojciech; Majchrzak, Tomasz; Gebicki, Jacek; Dymerski, Tomasz; Namieśnik, Jacek

    2016-11-01

    The paper presents the results of investigation on ambient air odor quality in a vicinity of the industrial sewage treatment plant being a part of the crude oil processing plant. The investigation was performed during spring-winter season using a prototype of electronic nose and the Nasal Ranger field olfactometers. The prototype was equipped with a set of six semiconductor sensors by FIGARO Co. and one PID-type sensor. The field olfactometers were used to determine mean concentration of odorants, which amounted from 2.2 to 20.2 ou/m3 depending on the place of measurement. In case of the investigation with the electronic nose prototype a classification of the ambient air samples with respect to the place of sampling was performed utilizing the kNN (where k=3) algorithm supported with a cross-validation method. Correct classification of the ambient air samples was at the level of 47.9%. Performed investigation revealed that evaluation of the ambient air samples with respect to odor was possible using the electronic nose instrument.

  4. 75 FR 9894 - Office of Research and Development; Ambient Air Monitoring Reference and Equivalent Methods...

    Science.gov (United States)

    2010-03-04

    ... in Ambient Air TSP by Hot Plate Acid Extraction and ICP-MS Analysis.'' In this method, total...), extracted on a hot plate with 3M HNO 3 according to 40 CFR Appendix G to part 50, EPA Reference Method for... Inductively Coupled Plasma-Mass Spectrometry (ICP-MS) based on EPA SW-846 Method 6020A. The application for...

  5. Case report: Atrial fibrillation following exposure to ambient air pollution particles

    Science.gov (United States)

    CONTEXT: Exposure to air pollution can result in the onset of atrial fibrillation. CASE PRESENTATION: We present a case of a 58 year old woman who volunteered to participate in a controlled exposure to concentrated ambient particles (CAPs). Twenty minutes into the exposure, there...

  6. Characterization of ambient air quality during a rice straw burning episode.

    Science.gov (United States)

    Tai-Yi, Yu

    2012-03-01

    Spatiotemporal characteristics and impact of ambient air-quality attributed to open burning of rice straw were analyzed and estimated with measured data. Two multivariate analytic methods, factor analysis and cluster analysis, were adopted to analyze the temporal and spatial impact on ambient air-quality during the rice straw burning episode. Temporal features of three scenarios were cited to compare the concentrations for ambient air-quality between the rice straw burning episode and non-episodes over two typical stations by factor analysis. Factor analysis demonstrated that the first rotational component, identified as being highly correlated to the open burning of rice straw, accounts for about 40% of the concentration variance for ambient air-quality. In typical air-quality stations, the average hourly incremental concentrations between the episode and non-episodes were greater than 300 μg m(-3) for PM(10), 1.0 ppm for CO and 35 ppb for NO(2) during the impact of rice straw burning. Factor analysis presented that the first rotated component was highly correlated with several primary pollutants (NO(2), NMHC, PM(10) and CO) during the rice straw burning episode, while every component was only highly correlated with a unique air pollutant during non-episodes. The delineation isopleths indicated that factor analysis could serve as a better method than cluster analysis and provides cross-county cooperation for local governments located in the same separated district during the rice straw burning season. The results of factor analysis revealed that CO is the best index to demonstrate the impact of rice straw burning than the other six air pollutants measured during the episode. Backward trajectory analysis supplied a cause-effect relationship between measured stations and specific rice planted regions during the rice straw burning episode.

  7. Depreciation in Ambient Air Quality in Iron Ore Mining Region of Goa

    Directory of Open Access Journals (Sweden)

    Gurdeep Singh

    2015-04-01

    Full Text Available Goa is one of the most famous international tourist destinations of the world. Export of Iron ore extracted from the midland of Goa is a major economic activity. However, there is a serious concern of air pollution due to iron ore mining activities. In order to assess the impact of mining activities on the environmental regime, the air quality depreciation index was adopted for this study due to its realistic and meaningful presentation of deterioration in ambient air quality. The index had been applied to the ambient air quality monitoring results of thirty four locations in the iron ore mining region of Goa. To envisage upon the deterioration in air quality due to various activities, eight stations were selected around mines, twelve in the buffer zone (within 4 Km radius of the core mining activities and fourteen along the ore transportation routes for monitoring of SPM, PM10, SO2 and NOX. The deterioration of air quality in the iron ore mining region of Goa is clearly apparent as the depreciation in air quality was found < -1 from the most desired value of 0 at all the stations. In general, the air quality was found most depreciated along the ore transportation routes, which is also evidenced by a considerable load of particulate matters observed. This infers that ore transportation is the most devastating activity in the iron ore mining region of Goa and accordingly mitigation plan should be adopted.

  8. Ambient air quality levels in Tehran, Iran, from 1988 to 1993

    Energy Technology Data Exchange (ETDEWEB)

    Shirazi, M.A.; Harding, A.K. [Oregon State Univ., Dept. of Public Health, Corvallis, OR (United States)

    2001-07-01

    The objectives of this study were to describe trends in ambient air quality in Tehran between 1988 and 1993, to determine if these levels exceeded the World Health Organisation (WHO) guidelines, and to discuss possible health effects related to exposure for these particular pollutants. Data were acquired from Iran's Environmental Protection Agency (IEPA) and the Ministry of Health (MH). These agencies operate five automated ambient air monitoring stations located in areas with heavy traffic. Daily samples of SO{sub 2}, NO{sub 2}, CO, total suspended particulate matter (TSM), and hydrocarbons (HC) were collected to provide 24 hour averages for each pollutant. Every three months, mean concentrations were reported to IEPA. Composite samples from all five stations were stored in a databank operated by IEPA. The ambient air quality guidelines were obtained from WHO reports. Statistical analysis was carried out using a regression model, which was designed to fit the air pollution data and take into account missing data. The results showed that there was a statistically significant upward trend in air pollution levels for all of the measured pollutants, except NO{sub 2}, during the years 1988 to 1993. WHO guidelines were routinely and substantially exceeded by all pollutants except TSM. These findings suggest that as the population continues to grow, and increasing numbers of motor vehicles are driven in Tehran, there is concern for the health effects that may result from exposure to these pollutants. (Author)

  9. Ambient air pollution and congenital heart defects in Lanzhou, China

    Science.gov (United States)

    Jin, Lan; Qiu, Jie; Zhang, Yaqun; Qiu, Weitao; He, Xiaochun; Wang, Yixuan; Sun, Qingmei; Li, Min; Zhao, Nan; Cui, Hongmei; Liu, Sufen; Tang, Zhongfeng; Chen, Ya; Yue, Li; Da, Zhenqiang; Xu, Xiaoying; Huang, Huang; Liu, Qing; Bell, Michelle L.; Zhang, Yawei

    2015-07-01

    Congenital heart defects are the most prevalent type of birth defects. The association of air pollution with congenital heart defects is not well understood. We investigated a cohort of 8969 singleton live births in Lanzhou, China during 2010-2012. Using inverse distance weighting, maternal exposures to particulate matter with diameters ≤10 μm (PM10), nitrogen dioxide (NO2), and sulfur dioxide (SO2) were estimated as a combination of monitoring station levels for time spent at home and in a work location. We used logistic regression to estimate the associations, adjusting for maternal age, education, income, BMI, disease, folic acid intake and therapeutic drug use, and smoking; season of conception, fuel used for cooking and temperature. We found significant positive associations of Patent Ductus Arteriosus (PDA) with PM10 during the 1st trimester, 2nd trimester and the entire pregnancy (OR 1st trimester = 3.96, 95% confidence interval (CI): 1.36, 11.53; OR 2nd trimester = 3.59, 95% CI: 1.57, 8.22; OR entire pregnancy = 2.09, 95% CI: 1.21, 3.62, per interquartile range (IQR) increment for PM10 (IQR = 71.2, 61.6, and 27.4 μg m-3, respectively)), and associations with NO2 during 2nd trimester and the entire pregnancy (OR 2nd trimester = 1.92, 95% CI: 1.11, 3.34; OR entire pregnancy = 2.32, 95% Cl: 1.14, 4.71, per IQR increment for NO2 (IQR = 13.4 and 10.9 μg m-3, respectively)). The associations for congenital malformations of the great arteries and pooled cases showed consistent patterns. We also found positive associations for congenital malformations of cardiac septa with PM10 exposures in the 2nd trimester and the entire pregnancy, and SO2 exposures in the entire pregnancy. Results indicate a health burden from maternal exposures to air pollution, with increased risk of congenital heart defects.

  10. Ambient air pollution and primary liver cancer incidence in four European cohorts within the ESCAPE project

    DEFF Research Database (Denmark)

    Pedersen, Marie; Andersen, Zorana J.; Stafoggia, Massimo

    2017-01-01

    Background: Tobacco smoke exposure increases the risk of cancer in the liver, but little is known about the possible risk associated with exposure to ambient air pollution. Objectives: We evaluated the association between residential exposure to air pollution and primary liver cancer incidence...... in PM2.5. Conclusions: The results provide suggestive evidence that ambient air pollution may increase the risk of liver cancer. Confidence intervals for associations with NO2 and NOX were narrower than for the other exposures.......) at baseline home addresses were estimated using land-use regression models from the ESCAPE project. We also investigated traffic density on the nearest road. We used Cox proportional-hazards models with adjustment for potential confounders for cohort-specific analyses and random-effects meta...

  11. Effects of Ambient Air Particulate Exposure on Blood-Gas Barrier Permeability and Lung Function

    DEFF Research Database (Denmark)

    Bräuner, Elvira Vaclavik; Mortensen, Jann; Møller, Peter

    2009-01-01

    Particulate air pollution is associated with increased risk of pulmonary diseases and detrimental outcomes related to the cardiovascular system, including altered vessel functions. This study's objective was too evaluate the effects of ambient particle exposure on the blood-gas permeability, lung.......5-15.8 microg/m(3) PM(10-2.5)) or filtered (91-542 particles/cm(3)) air collected above a busy street. The clearance rate of aerosolized (99m)Tc-labeled diethylenetriamine pentaacetic acid ((99m)Tc-DTPA) was measured as an index for the alveolar epithelial membrane integrity and permeability of the lung blood...... on the concentration of CC16 in plasma and urine or on the static and dynamic volumes or ventilation distribution of the lungs. The study thus demonstrates increased permeability of the alveolar blood-gas barrier following moderate exercise, whereas exposure to ambient levels of urban air particles has no detectable...

  12. Relationship Between Ambient Air Pollution and Daily Mortality of SARS in Beijing

    Institute of Scientific and Technical Information of China (English)

    HAI-DONG KAN; BING-HENG CHEN; CHAO-WEI FU; SHUN-ZHANG YU; LI-NA MU

    2005-01-01

    Objective To study the relationship between ambient air pollution and daily mortality of SARS in Beijing. Methods The approach of time-series Poisson regression was used to assess the relationship between daily SARS mortality, ambient air pollution, and other factors from April 25 to May 31, 2003 in Beijing. Results An increase of each 10 μμg/m3 over a 5-day moving average of PM10, SO2 and NO2 corresponded to 1.06 (1.00-1.12), 0.74 (0.48-1.13) and 1.22 (1.01-1.48) relative risks (RRs) of daily SARS mortality, respectively. The relative risks (RRs) values depended largely on the selection of lag days. Conclusion The daily mortality of SARS might be associated with certain air pollutants in Beijing.

  13. Environmental dust effects on aluminum surfaces in humid air ambient

    Science.gov (United States)

    Yilbas, Bekir Sami; Hassan, Ghassan; Ali, Haider; Al-Aqeeli, Nasser

    2017-01-01

    Environmental dusts settle on surfaces and influence the performance of concentrated solar energy harvesting devices, such as aluminum troughs. The characteristics of environmental dust and the effects of mud formed from the dust particles as a result of water condensing in humid air conditions on an aluminum wafer surface are examined. The dissolution of alkaline and alkaline earth compounds in water condensate form a chemically active mud liquid with pH 8.2. Due to gravity, the mud liquid settles at the interface of the mud and the aluminum surface while forming locally scattered patches of liquid films. Once the mud liquid dries, adhesion work to remove the dry mud increases significantly. The mud liquid gives rise to the formation of pinholes and local pit sites on the aluminum surface. Morphological changes due to pit sites and residues of the dry mud on the aluminum surface lower the surface reflection after the removal of the dry mud from the surface. The characteristics of the aluminum surface can address the dust/mud-related limitations of reflective surfaces and may have implications for the reductions in the efficiencies of solar concentrated power systems. PMID:28378798

  14. Determination of Sulphur Dioxide Concentrations in Ambient Air of Some Selected Traffic Areas in Kaduna Metropolis

    Directory of Open Access Journals (Sweden)

    Y. Mohammed

    2013-09-01

    Full Text Available This research study was aimed at determining concentrations of sulphurdioxide in ambient air of some selected areas viz: industrial area (Kakuri, high vehicler traffic/commercial area (Leventis Roundabout, traveling route (Kawo overhead bridge, Low vehicler traffic area (Tafawa Balewa Roundabout, residential area (Kawo New Extension and a control site (NFA base in Kaduna metropolis Nigeria. Air sample was collected at each sampling site by passing ambient air through an impinger bottle containing hydrogen peroxide (absorbent, at a flow-rate of 10 L/min for 30 min using air vacuum pump. The concentration of SO2 in the resultant solution (absorbent was determined by titrating against 0.005 moL/dm3 NaOH solutions. The average SO2 concentrations in the six sampling stations were within the range 0.16-0.75 ppm, with the highest values of 0.75 and 0.70 ppm at highly industrialized area (Kakuri and a high traffic area (Leventis roundabout respectively. The ambient air concentrations of SO2 depict the pattern; Industrial area (Kakuri >High vehicler traffic/commercial area (Leventis roundabout >Traveling route (Kawo overhead bridge >Low traffic area (Tafawa Balewa roundabout >Residential area (Kawo New Extension >Remote area (NAF Base Mando. Except for highly industrial area (Kakuri and the high traffic area (Leventis, The ambient air SO2 concentration are within the acceptable limits of United States Environmental Protection Agency (EPA and Nigeria’s Federal Environmental Protection Agency (FEPA standard limit which is 0.5 ppm for 30 min exposure time.

  15. The Comparative Reactivity Method ─ a new tool to measure total OH Reactivity in ambient air

    Directory of Open Access Journals (Sweden)

    J. Lelieveld

    2008-04-01

    Full Text Available Hydroxyl (OH radicals play a vital role in maintaining the oxidizing capacity of the atmosphere. To understand variations in OH radicals both source and sink terms must be understood. Currently the overall sink term, or the total atmospheric reactivity to OH, is poorly constrained. Here, we present a new on-line method to directly measure the total OH reactivity (i.e.~total loss rate of OH radicals in a sampled air mass. In this method, a reactive molecule (X, not normally present in air, is passed through a glass reactor and its concentration is monitored with a suitable detector. OH radicals are then introduced in the glass reactor at a constant rate to react with X, first in the presence of zero air and then in the presence of ambient air containing VOCs and other OH reactive species. Comparing the amount of X exiting the reactor with and without the ambient air allows the air reactivity to be determined. In our existing set up, X is pyrrole and the detector used is a proton transfer reaction mass spectrometer. The present dynamic range for ambient air reactivity is about 6 to 300 s−1, with an overall maximum uncertainty of 25% above 8 s−1 and up to 50% between 6–8 s−1. The system has been tested and calibrated with different single and mixed hydrocarbon standards showing excellent linearity and accountability with the reactivity of the standards. Potential interferences such as high NO in ambient air, varying relative humidity and photolysis of pyrrole within the setup have also been investigated. While interferences due changing humidity and photolysis of pyrrole are easily overcome by ensuring that humidity in the set up does not change drastically and the photolytic loss of pyrrole is measured and taken into account, respectively, NO>10 ppb in ambient air remains a significant interference for the current configuration of the instrument. Field tests in the tropical rainforest of Suriname (~53 s and the urban atmosphere of Mainz

  16. Exploring Air-Climate-Energy Impacts with GCAM-USA

    Science.gov (United States)

    The Global Climate Assessment Model (GCAM) is a global integrated assessment model used for exploring future scenarios and examining strategies that address air pollution, climate change and energy (ACE) goals. My research focuseson integration of impact factors in GCAM-USA and a...

  17. Air flow assisted ionization for remote sampling of ambient mass spectrometry and its application.

    Science.gov (United States)

    He, Jiuming; Tang, Fei; Luo, Zhigang; Chen, Yi; Xu, Jing; Zhang, Ruiping; Wang, Xiaohao; Abliz, Zeper

    2011-04-15

    Ambient ionization methods are an important research area in mass spectrometry (MS) analysis. Under ambient conditions, the gas flow and atmospheric pressure significantly affect the transfer and focusing of ions. The design and implementation of air flow assisted ionization (AFAI) as a novel and effective, remote sampling method for ambient mass spectrometry are described herein. AFAI benefits from a high extracting air flow rate. A systematic investigation of the extracting air flow in the AFAI system has been carried out, and it has been demonstrated not only that it plays a role in the effective capture and remote transport of charged droplets, but also that it promotes desolvation and ion formation, and even prevents ion fragmentation during the ionization process. Moreover, the sensitivity of remote sampling ambient MS analysis was improved significantly by the AFAI method. Highly polar and nonpolar molecules, including dyes, pharmaceutical samples, explosives, drugs of abuse, protein and volatile compounds, have been successfully analyzed using AFAI-MS. The successful application of the technique to residue detection on fingers, large object analysis and remote monitoring in real time indicates its potential for the analysis of a variety of samples, especially large objects. The ability to couple this technique with most commercially available MS instruments with an API interface further enhances its broad applicability.

  18. The discharge of fine silica sand in a silo under different ambient air pressures

    Science.gov (United States)

    Hsiau, Shu-San; Liao, Chun-Chung; Lee, Jie-Hsien

    2012-04-01

    Silos are widely used for the industrial scale handling and transportation of powdered and granular materials. The process of discharging powder in a silo involves the flow of both solid particles and an interstitial fluid, usually air. In this study, we experimentally investigate the effects of particle size and ambient pressure on the discharge process in open- and closed-top silos. The discharge rate, pressure drop, and pressure recovery rate are measured and discussed. The results show that the particle size, the diameter of the orifice, and the ambient pressure significantly influence the process of discharge. The effect of air flow is stronger on fine-powdered flow in a closed-top silo. The results indicate that the effects of air flow could be reduced by lowering the ambient pressure. In addition, a normalized critical pressure can be defined beyond which the discharge rate increases dramatically. With reduced ambient pressure, this normalized critical pressure decreases with increasing particle size. Finally, the experimental results are compared with results calculated using the Beverloo equation and Darcy's law.

  19. Effects of Using Wind Guiding Nets to Improve Prevailing Ambient Wind on Direct Air-cooled Condensers

    Institute of Scientific and Technical Information of China (English)

    YANG Jianguo; LIU Da; ZHANG Zhaoying; JU Xiaoli

    2012-01-01

    Prevailing ambient wind is the main reason that causes inlet flow rate (air mass flow rate) decreasing and air flowing backward to the air-cooled condenser fans upward to the wind, hence a set of wind guiding nets is designed to improve the detrimental effect. Fig. 1 shows four typical units of a 1000MW direct air-cooled condenser (DACC) and a set of wind guiding nets installed under its edge upward to the ambient wind. As shown in Fig. 2, the fan inlet flow rate decreases as the prevailing ambient wind velocity increasing, especially for the first two units upward to the wind.

  20. Quantile-based Bayesian maximum entropy approach for spatiotemporal modeling of ambient air quality levels.

    Science.gov (United States)

    Yu, Hwa-Lung; Wang, Chih-Hsin

    2013-02-05

    Understanding the daily changes in ambient air quality concentrations is important to the assessing human exposure and environmental health. However, the fine temporal scales (e.g., hourly) involved in this assessment often lead to high variability in air quality concentrations. This is because of the complex short-term physical and chemical mechanisms among the pollutants. Consequently, high heterogeneity is usually present in not only the averaged pollution levels, but also the intraday variance levels of the daily observations of ambient concentration across space and time. This characteristic decreases the estimation performance of common techniques. This study proposes a novel quantile-based Bayesian maximum entropy (QBME) method to account for the nonstationary and nonhomogeneous characteristics of ambient air pollution dynamics. The QBME method characterizes the spatiotemporal dependence among the ambient air quality levels based on their location-specific quantiles and accounts for spatiotemporal variations using a local weighted smoothing technique. The epistemic framework of the QBME method can allow researchers to further consider the uncertainty of space-time observations. This study presents the spatiotemporal modeling of daily CO and PM10 concentrations across Taiwan from 1998 to 2009 using the QBME method. Results show that the QBME method can effectively improve estimation accuracy in terms of lower mean absolute errors and standard deviations over space and time, especially for pollutants with strong nonhomogeneous variances across space. In addition, the epistemic framework can allow researchers to assimilate the site-specific secondary information where the observations are absent because of the common preferential sampling issues of environmental data. The proposed QBME method provides a practical and powerful framework for the spatiotemporal modeling of ambient pollutants.

  1. The effect of future ambient air pollution on human premature mortality to 2100 using output from the ACCMIP model ensemble

    Science.gov (United States)

    Silva, Raquel A.; West, J. Jason; Lamarque, Jean-François; Shindell, Drew T.; Collins, William J.; Dalsoren, Stig; Faluvegi, Greg; Folberth, Gerd; Horowitz, Larry W.; Nagashima, Tatsuya; Naik, Vaishali; Rumbold, Steven T.; Sudo, Kengo; Takemura, Toshihiko; Bergmann, Daniel; Cameron-Smith, Philip; Cionni, Irene; Doherty, Ruth M.; Eyring, Veronika; Josse, Beatrice; MacKenzie, Ian A.; Plummer, David; Righi, Mattia; Stevenson, David S.; Strode, Sarah; Szopa, Sophie; Zengast, Guang

    2016-08-01

    Ambient air pollution from ground-level ozone and fine particulate matter (PM2.5) is associated with premature mortality. Future concentrations of these air pollutants will be driven by natural and anthropogenic emissions and by climate change. Using anthropogenic and biomass burning emissions projected in the four Representative Concentration Pathway scenarios (RCPs), the ACCMIP ensemble of chemistry-climate models simulated future concentrations of ozone and PM2.5 at selected decades between 2000 and 2100. We use output from the ACCMIP ensemble, together with projections of future population and baseline mortality rates, to quantify the human premature mortality impacts of future ambient air pollution. Future air-pollution-related premature mortality in 2030, 2050 and 2100 is estimated for each scenario and for each model using a health impact function based on changes in concentrations of ozone and PM2.5 relative to 2000 and projected future population and baseline mortality rates. Additionally, the global mortality burden of ozone and PM2.5 in 2000 and each future period is estimated relative to 1850 concentrations, using present-day and future population and baseline mortality rates. The change in future ozone concentrations relative to 2000 is associated with excess global premature mortality in some scenarios/periods, particularly in RCP8.5 in 2100 (316 thousand deaths year-1), likely driven by the large increase in methane emissions and by the net effect of climate change projected in this scenario, but it leads to considerable avoided premature mortality for the three other RCPs. However, the global mortality burden of ozone markedly increases from 382 000 (121 000 to 728 000) deaths year-1 in 2000 to between 1.09 and 2.36 million deaths year-1 in 2100, across RCPs, mostly due to the effect of increases in population and baseline mortality rates. PM2.5 concentrations decrease relative to 2000 in all scenarios, due to projected reductions in emissions, and

  2. 75 FR 71033 - Air Quality Designations for the 2008 Lead (Pb) National Ambient Air Quality Standards

    Science.gov (United States)

    2010-11-22

    ... Agency FR Federal Register FRM Federal Reference Method IQ Intelligence Quotient NAAQS National Ambient... plants and animals, and neurological effects in vertebrates. V. What are the CAA requirements for...

  3. CO2 Capture from Ambient Air by Crystallization with a Guanidine Sorbent.

    Science.gov (United States)

    Seipp, Charles A; Williams, Neil J; Kidder, Michelle K; Custelcean, Radu

    2017-01-19

    Carbon capture and storage is an important strategy for stabilizing the increasing concentration of atmospheric CO2 and the global temperature. A possible approach toward reversing this trend and decreasing the atmospheric CO2 concentration is to remove the CO2 directly from air (direct air capture). Herein we report a simple aqueous guanidine sorbent that captures CO2 from ambient air and binds it as a crystalline carbonate salt by guanidinium hydrogen bonding. The resulting solid has very low aqueous solubility (Ksp =1.0(4)×10(-8) ), which facilitates its separation from solution by filtration. The bound CO2 can be released by relatively mild heating of the crystals at 80-120 °C, which regenerates the guanidine sorbent quantitatively. Thus, this crystallization-based approach to CO2 separation from air requires minimal energy and chemical input, and offers the prospect for low-cost direct air capture technologies.

  4. Addition of PM 2.5 into the national ambient air quality standards of China and the contribution to air pollution control: the case study of Wuhan, China.

    Science.gov (United States)

    You, Mingqing

    2014-01-01

    PM2.5 has gradually become a major environmental problem of China with its rapid economic development, urbanization, and increasing of motor vehicles. Findings and awareness of serious PM2.5 pollution make the PM2.5 a new criterion pollutant of the Chinese National Ambient Air Quality Standard (NAAQS) revised in 2012. The 2012 NAAQS sets the PM2.5 concentrate limitation with the 24-hour average value and the annual mean value. Wuhan is quite typical among central and southern China in climate, economy, development level, and energy consumption. The data are cited from the official website of Wuhan Environmental Protection Bureau and cover the period from 1 January to 30 June 2013. The data definitely confirm the existence of serious PM2.5 pollution in Wuhan and indicate that the addition of PM2.5 as a criterion pollutant significantly brings down the attainment rate of air quality. The example of Wuhan reveals that local governments should take measures to reduce the emission of PM2.5 if it affects the attainment rate and the performance evaluation value of air quality. The main contribution of 2012 NAAQS is that it brings down the attainment rate of the air quality and forces local governmental officials to take the measures accordingly.

  5. Addition of PM2.5 into the National Ambient Air Quality Standards of China and the Contribution to Air Pollution Control: The Case Study of Wuhan, China

    Directory of Open Access Journals (Sweden)

    Mingqing You

    2014-01-01

    Full Text Available PM2.5 has gradually become a major environmental problem of China with its rapid economic development, urbanization, and increasing of motor vehicles. Findings and awareness of serious PM2.5 pollution make the PM2.5 a new criterion pollutant of the Chinese National Ambient Air Quality Standard (NAAQS revised in 2012. The 2012 NAAQS sets the PM2.5 concentrate limitation with the 24-hour average value and the annual mean value. Wuhan is quite typical among central and southern China in climate, economy, development level, and energy consumption. The data are cited from the official website of Wuhan Environmental Protection Bureau and cover the period from 1 January to 30 June 2013. The data definitely confirm the existence of serious PM2.5 pollution in Wuhan and indicate that the addition of PM2.5 as a criterion pollutant significantly brings down the attainment rate of air quality. The example of Wuhan reveals that local governments should take measures to reduce the emission of PM2.5 if it affects the attainment rate and the performance evaluation value of air quality. The main contribution of 2012 NAAQS is that it brings down the attainment rate of the air quality and forces local governmental officials to take the measures accordingly.

  6. Ambient particulate air pollution from vehicles promotes lipid peroxidation and inflammatory responses in rat lung

    Directory of Open Access Journals (Sweden)

    C.E.L. Pereira

    2007-10-01

    Full Text Available Oxidative stress plays a major role in the pathogenesis of particle-dependent lung injury. Ambient particle levels from vehicles have not been previously shown to cause oxidative stress to the lungs. The present study was conducted to a determine whether short-term exposure to ambient levels of particulate air pollution from vehicles elicits inflammatory responses and lipid peroxidation in rat lungs, and b determine if intermittent short-term exposures (every 4 days induce some degree of tolerance. Three-month-old male Wistar rats were exposed to ambient particulate matter (PM from vehicles (N = 30 for 6 or 20 continuous hours, or for intermittent (5 h periods during 20 h for 4 consecutive days or to filtered air (PM <10 µm; N = 30. Rats continuously breathing polluted air for 20 h (P-20 showed a significant increase in the total number of leukocytes in bronchoalveolar lavage compared to control (C-20: 2.61 x 105 ± 0.51;P-20: 5.01 x 105 ± 0.81; P < 0.05 and in lipid peroxidation ([MDA] nmol/mg protein: C-20: 0.148 ± 0.01; P-20: 0.226 ± 0.02; P < 0.05. Shorter exposure (6 h and intermittent 5-h exposures over a period of 4 days did not cause significant changes in leukocytes. Lipid damage resulting from 20-h exposure to particulate air pollution did not cause a significant increase in lung water content. These data suggest oxidative stress as one of the mechanisms responsible for the acute adverse respiratory effects of particles, and suggest that short-term inhalation of ambient particulate air pollution from street with high automobile traffic represents a biological hazard.

  7. Estimating the effects of ambient conditions on the performance of UVGI air cleaners

    Energy Technology Data Exchange (ETDEWEB)

    Lau, Josephine; Bahnfleth, William; Freihaut, James [Indoor Environment Center, Department of Architectural Engineering, The Pennsylvania State University, University Park, PA (United States)

    2009-07-15

    Ultraviolet germicidal irradiation (UVGI) uses UVC radiation produced by low pressure mercury vapor lamps to control biological air contaminants. Ambient air velocity and temperature have a strong effect on lamp output by influencing the lamp surface cold spot temperature. In-duct UVGI systems are particularly susceptible to ambient effects due to the range of velocity and temperature conditions they may experience. An analytical model of the effect of ambient conditions on lamp surface temperature was developed for three common lamp types in cross flow from a convective-radiative energy balance assuming constant surface temperature. For one lamp type, a single tube standard output lamp, UVC output and cold spot temperature data were obtained under typical in-duct operating conditions. Over an ambient temperature range of 10-32.2 C and an air velocity range of 0-3.25 m/s, measured cold spot temperature varied from 12.7 to 41.9 C and measured lamp output varied by 68% of maximum. Surface temperatures predicted by the heat transfer model were 6-17 C higher than corresponding measured cold spot temperatures, but were found to correlate well with cold spot temperature via a two-variable linear regression. When corrected using this relationship, the simple model predicted the cold spot temperature within 1 C and lamp UVC output within {+-}5%. To illustrate its practical use, the calibrated lamp model was employed in a simulation of the control of a contaminant in a single-zone ventilation system by an in-duct UVGI device. In this example, failure to account for the impact of ambient condition effects resulted in under-prediction of average space concentration by approximately 20% relative to a constant output system operating at maximum UVC output. (author)

  8. 75 FR 65572 - Approval and Promulgation of Air Quality Implementation Plans; Ohio; Ohio Ambient Air Quality...

    Science.gov (United States)

    2010-10-26

    ... authority to address, as appropriate, disproportionate human health or environmental effects, using...).) List of Subjects in 40 CFR Part 52 Environmental protection, Air pollution control, Carbon monoxide... Air Quality Standards AGENCY: Environmental Protection Agency (EPA). ACTION: Direct final...

  9. Mixed uncertainty analysis of polycyclic aromatic hydrocarbon inhalation and risk assessment in ambient air of Beijing

    Institute of Scientific and Technical Information of China (English)

    YU Yajuan; GUO Huaicheng; LIU Yong; HUANG Kai; WANG Zhen; ZHAN Xinye

    2008-01-01

    This article presents the application of an integrated method that estimates the dispersion of polycyclic aromatic hydrocarbons (PAHs) in air, and assesses the human health risk associated with PAHs inhalation. An uncertainty analysis method consisting of three components were applied in this study, where the three components include a bootstrapping method for analyzing the whole process associated uncertainty, an inhalation rate (IR) representation for evaluating the total PAH inhalation risk for human health, and a normally distributed absorption fraction (AF) ranging from 0% to 100% to represent the absorption capability of PAHs in human body. Using this method, an integrated process was employed to assess the health risk of the residents in Beijing, China, from inhaling PAHs in the air. The results indicate that the ambient air PAHs in Beijing is an important contributor to human health impairment, although over 68% of residents seem to be safe from daily PAH carcinogenic inhalation. In general, the accumulated daily inhalation amount is relatively higher for male and children at 10 years old of age than for female and children at 6 years old. In 1997, about 1.73% cancer sufferers in Beijing were more or less related to ambient air PAHs inhalation. At 95% confidence interval, approximately 272-309 individual cancer incidences can be attributed to PAHs pollution in the air. The probability of greater than 500 cancer occurrence is 15.3%. While the inhalation of ambient air PAHs was shown to be an important factor responsible for higher cancer occurrence in Beijing, while the contribution might not be the most significant one.

  10. A multi-model assessment of the co-benefits of climate mitigation for global air quality

    Energy Technology Data Exchange (ETDEWEB)

    Rao, Shilpa; Klimont, Zbigniew; Leitao, Joana; Riahi, Keywan; van Dingenen, Rita; Reis, Lara Aleluia; Calvin, Katherine; Dentener, Frank; Drouet, Laurent; Fujimori, Shinichiro; Harmsen, Mathijs; Luderer, Gunnar; Heyes, Chris; Strefler, Jessica; Tavoni, Massimo; van Vuuren, Detlef P.

    2016-12-01

    The recent International Panel on Climate change (IPCC) report identifies significant co-benefits from climate policies on near-term ambient air pollution and related human health outcomes [1]. This is increasingly relevant for policy making as the health impacts of air pollution are a major global concern- the Global Burden of Disease (GBD) study identifies outdoor air pollution as the sixth major cause of death globally [2]. Integrated assessment models (IAMs) are an effective tool to evaluate future air pollution outcomes across a wide range of assumptions on socio-economic development and policy regimes. The Representative Concentration Pathways (RCPs) [3] were the first set of long-term global scenarios developed across multiple integrated assessment models that provided detailed estimates of a number of air pollutants until 2100. However these scenarios were primarily designed to cover a defined range of radiative forcing outcomes and thus did not specifically focus on the interactions of long-term climate goals on near-term air pollution impacts. More recently, [4] used the RCP4.5 scenario to evaluate the co-benefits of global GHG reductions on air quality and human health in 2030. [5-7] have further examined the interactions of more diverse pollution control regimes with climate policies. This paper extends the listed studies in a number of ways. Firstly it uses multiple IAMs to look into the co-benefits of a global climate policy for ambient air pollution under harmonized assumptions on near-term air pollution control. Multi-model frameworks have been extensively used in the analysis of climate change mitigation pathways, and the structural uncertainties regarding the underlying mechanisms (see for example [8-10]. This is to our knowledge the first time that a multi-model evaluation has been specifically designed and applied to analyze the co-benefits of climate change policy on ambient air quality, thus enabling a better understanding of at a detailed

  11. Ambient air monitoring plan for Ciudad Acuna and Piedra Negras, Coahuila, Mexico. Final report

    Energy Technology Data Exchange (ETDEWEB)

    Winberry, J.; Henning, L.; Crume, R.

    1998-01-01

    The Cities of Ciudad Acuna and Piedras Negras and the State of Coahuila in Mexico are interested in improving ambient air quality monitoring capabilities in the two cities through the establishment of a network of ambient air monitors. The purpose of the network is to characterize population exposure to potentially harmful air contaminants, possibly including sulfur dioxide (SO{sub 2}), nitrogen oxides (NO{sub x}), ozone (O{sub 3}), carbon monoxide (CO), total suspended particulate matter (TSP), particulate matter with aerodynamic diameter less than 100 micrometers PM-10, and lead. This report presents the results of an evaluation of existing air quality monitoring equipment and facilities in Ciudad Acuna and Piedras Negras. Additionally, the report presents recommendations for developing an air quality monitoring network for PM-10, SO{sub 2}, lead, and ozone in these cities, using a combination of both new and existing equipment. The human resources currently available and ultimately needed to operate and maintain the network are also discussed.

  12. Single-step ambient-air synthesis of graphene from renewable precursors as electrochemical genosensor

    Science.gov (United States)

    Seo, Dong Han; Pineda, Shafique; Fang, Jinghua; Gozukara, Yesim; Yick, Samuel; Bendavid, Avi; Lam, Simon Kwai Hung; Murdock, Adrian T.; Murphy, Anthony B.; Han, Zhao Jun; Ostrikov, Kostya (Ken)

    2017-01-01

    Thermal chemical vapour deposition techniques for graphene fabrication, while promising, are thus far limited by resource-consuming and energy-intensive principles. In particular, purified gases and extensive vacuum processing are necessary for creating a highly controlled environment, isolated from ambient air, to enable the growth of graphene films. Here we exploit the ambient-air environment to enable the growth of graphene films, without the need for compressed gases. A renewable natural precursor, soybean oil, is transformed into continuous graphene films, composed of single-to-few layers, in a single step. The enabling parameters for controlled synthesis and tailored properties of the graphene film are discussed, and a mechanism for the ambient-air growth is proposed. Furthermore, the functionality of the graphene is demonstrated through direct utilization as an electrode to realize an effective electrochemical genosensor. Our method is applicable to other types of renewable precursors and may open a new avenue for low-cost synthesis of graphene films.

  13. Single-step ambient-air synthesis of graphene from renewable precursors as electrochemical genosensor

    Science.gov (United States)

    Seo, Dong Han; Pineda, Shafique; Fang, Jinghua; Gozukara, Yesim; Yick, Samuel; Bendavid, Avi; Lam, Simon Kwai Hung; Murdock, Adrian T.; Murphy, Anthony B.; Han, Zhao Jun; Ostrikov, Kostya (Ken)

    2017-01-01

    Thermal chemical vapour deposition techniques for graphene fabrication, while promising, are thus far limited by resource-consuming and energy-intensive principles. In particular, purified gases and extensive vacuum processing are necessary for creating a highly controlled environment, isolated from ambient air, to enable the growth of graphene films. Here we exploit the ambient-air environment to enable the growth of graphene films, without the need for compressed gases. A renewable natural precursor, soybean oil, is transformed into continuous graphene films, composed of single-to-few layers, in a single step. The enabling parameters for controlled synthesis and tailored properties of the graphene film are discussed, and a mechanism for the ambient-air growth is proposed. Furthermore, the functionality of the graphene is demonstrated through direct utilization as an electrode to realize an effective electrochemical genosensor. Our method is applicable to other types of renewable precursors and may open a new avenue for low-cost synthesis of graphene films. PMID:28134336

  14. Laser-induced fluorescence from N2(+) ions generated by a corona discharge in ambient air.

    Science.gov (United States)

    Konthasinghe, Kumarasiri; Fitzmorris, Kristin; Peiris, Manoj; Hopkins, Adam J; Petrak, Benjamin; Killinger, Dennis K; Muller, Andreas

    2015-09-01

    In this work, we present the measurement of laser-induced fluorescence from N2(+) ions via the B(2)Σu(+)-X(2)Σg(+) band system in the near-ultraviolet. The ions were generated continuously by a plasma glow discharge in low pressure N2 and by a corona discharge in ambient air. The fluorescence decay time was found to rapidly decrease with increasing pressure leading to an extrapolated decay rate of ≍10(10) s(-1) at atmospheric pressure. In spite of this quenching, we were able to observe laser induced fluorescence in ambient air by means of a time-gated spectral measurement. In the process of comparing the emission signal with that of N2 spontaneous Raman scattering, ion concentrations in ambient air of order 10(8-)10(10) cm(-3) were determined. With moderate increases in laser power and collection efficiency, ion concentrations of less than 10(6) cm(-3) may be measurable, potentially enabling applications in atmospheric standoff detection of ionizing radiation from hazardous radioactive sources.

  15. Air quality and climate--synergies and trade-offs.

    Science.gov (United States)

    von Schneidemesser, Erika; Monks, Paul S

    2013-07-01

    Air quality and climate are often treated as separate science and policy areas. Air quality encompasses the here-and-now of pollutant emissions, atmospheric transformations and their direct effect on human and ecosystem health. Climate change deals with the drivers leading to a warmer world and the consequences of that. These two science and policy issues are inexorably linked via common pollutants, such as ozone (methane) and black carbon. This short review looks at the new scientific evidence around so-called "short-lived climate forcers" and the growing realisation that a way to meet short-term climate change targets may be through the control of "air quality" pollutants. None of the options discussed here can replace reduction of long-lived greenhouse gases, such as CO2, which is required for any long-term climate change mitigation strategy. An overview is given of the underlying science, remaining uncertainties, and some of the synergies and trade-offs for addressing air quality and climate in the science and policy context.

  16. Secondary organic aerosol formation from photo-oxidation of toluene with NOx and SO2: Chamber simulation with purified air versus urban ambient air as matrix

    Science.gov (United States)

    Deng, Wei; Liu, Tengyu; Zhang, Yanli; Situ, Shuping; Hu, Qihou; He, Quanfu; Zhang, Zhou; Lü, Sujun; Bi, Xinhui; Wang, Xuemei; Boreave, Antoinette; George, Christian; Ding, Xiang; Wang, Xinming

    2017-02-01

    Chamber studies on the formation of secondary aerosols are mostly performed with purified air as matrix, it is of wide concern in what extent they might be different from the situations in ambient air, where a variety of gaseous and particulate components preexist. Here we compared the photo-oxidation of "toluene + NOx + SO2" combinations in a smog chamber in real urban ambient air matrix with that in purified air matrix. The secondary organic aerosols (SOA) mass concentrations and yields from toluene in the ambient air matrix, after subtracted ambient air background primary and secondary organic aerosols, were 9.0-34.0 and 5.6-12.9 times, respectively, greater than those in purified air matrix. Both homogeneous and heterogeneous oxidation of SO2 were enhanced in ambient air matrix experiments with observed 2.0-7.5 times higher SO2 degradation rates and 2.6-6.8 times faster sulfate formation than that in purified air matrix, resulting in higher in-situ particle acidity and consequently promoting acid-catalyzed SOA formation. In the ambient air experiments although averaged OH radical levels were elevated probably due to heterogeneous formation of OH on particle surface and/or ozonolysis of alkenes, non-OH oxidation pathways of SO2 became even more dominating. Under the same organic aerosol mass concentration, the SOA yields of toluene in purified air matrix experiments matched very well with the two-product model curve by Ng et al. (2007), yet the yields in ambient air on average was over two times larger. The results however were much near the best fit curve by Hildebrandt et al. (2009) with the volatility basis set (VBS) approach.

  17. Multi-Gas analysis of ambient air using FTIR spectroscopy over Mexico City

    Energy Technology Data Exchange (ETDEWEB)

    Grutter, Michel [Centro de Ciencias de la Atmosfera, Universidad Nacional Autonoma de Mexico (UNAM), Mexico, D.F. (Mexico)

    2003-01-01

    A Fourier Transform Infrared (FTIR) spectrometer was used to analyze the composition of ambient air at a specific site in Mexico City metropolitan area. A continuous flow of air was passed through a multi-pass cell and the absorption spectra were collected over a period of two weeks. Quantitative analysis was performed by means of the classical-least square (CLS) method using synthetically generated spectra as references and calibration sources. Ambient levels of CO, CO{sup 2}, CH{sub 4} and N{sub 2}O are reported with a time resolution of five minutes for September 2001, showing interesting results in their diurnal patterns. Comments on the precision, detection limits and signal to noise of the instrument are included for the evaluation of this technique. Water concentrations were estimated and compared with those obtained with a relative humidity sensor. The technique of extractive FTIR for ambient trace gas monitoring was utilized in Mexico for the fist time and some potential applications are given. [Spanish] Se utilizo un espectrometro en el infrarrojo por transformadas de Fourier (FTIR) para analizar la composicion de aire ambiente en un sitio de la zona metropolitana de la Ciudad de Mexico. Para ello se introdujo un flujo constante de aire a una celda de gases de paso multiple y se colectaron los espectros durante un periodo de dos semanas. Para el analisis cuantitativo, se aplico el metodo clasico de minimos cuadrados (CLS) utilizando espectros sinteticos como referencias y fuentes de calibracion. Se observaron patrones interesantes en los niveles ambientales de CO, CO{sup 2}, CH{sub 4} y N{sub 2}O, los cuales son reportados con una resolucion temporal de cinco minutos para el mes de septiembre del 2001. En la evaluacion de esta tecnica se incluyen comentarios sobre la precision, los limites de deteccion, asi como de la relacion senal/ruido del instrumento. Se estimaron concentraciones de vapor de agua a traves de sus absorciones en el infrarrojo y se

  18. Climate Strategy with CO2 Capture from the Air

    Energy Technology Data Exchange (ETDEWEB)

    Keith, D.W. [Department of Chemical and Petroleum Engineering, University of Calgary, 2500 University Drive NW, Calgary, AB (Canada); Ha-Duong, M. [CNRS-CIRED, Campus du Jardin Tropical, 45 bis, av. de la Belle Gabrielle, 94736 Nogent sur Marne CEDEX (France); Stolaroff, J.K. [Department of Engineering and Public Policy, Carnegie Mellon University, 5000 Forbes Ave, Pittsburgh, PA 15213 (United States)

    2006-01-15

    It is physically possible to capture CO2 directly from the air and immobilize it in geological structures. Air capture differs from conventional mitigation in three key aspects. First, it removes emissions from any part of the economy with equal ease or difficulty, so its cost provides an absolute cap on the cost of mitigation. Second, it permits reduction in concentrations faster than the natural carbon cycle: the effects of irreversibility are thus partly alleviated. Third, because it is weakly coupled to existing energy infrastructure, air capture may offer stronger economies of scale and smaller adjustment costs than the more conventional mitigation technologies. We assess the ultimate physical limits on the amount of energy and land required for air capture and describe two systems that might achieve air capture at prices under 200 and 500 $/tC using current technology. Like geoengineering, air capture limits the cost of a worst-case climate scenario. In an optimal sequential decision framework with uncertainty, existence of air capture decreases the need for near-term precautionary abatement. The long-term effect is the opposite; assuming that marginal costs of mitigation decrease with time while marginal climate change damages increase, then air capture increases long-run abatement. Air capture produces an environmental Kuznets curve, in which concentrations are returned to preindustrial levels.

  19. The association of ambient air pollution and physical inactivity in the United States.

    Directory of Open Access Journals (Sweden)

    Jennifer D Roberts

    Full Text Available BACKGROUND: Physical inactivity, ambient air pollution and obesity are modifiable risk factors for non-communicable diseases, with the first accounting for 10% of premature deaths worldwide. Although community level interventions may target each simultaneously, research on the relationship between these risk factors is lacking. OBJECTIVES: After comparing spatial interpolation methods to determine the best predictor for particulate matter (PM2.5; PM10 and ozone (O3 exposures throughout the U.S., we evaluated the cross-sectional association of ambient air pollution with leisure-time physical inactivity among adults. METHODS: In this cross-sectional study, we assessed leisure-time physical inactivity using individual self-reported survey data from the Centers for Disease Control and Prevention's 2011 Behavioral Risk Factor Surveillance System. These data were combined with county-level U.S. Environmental Protection Agency air pollution exposure estimates using two interpolation methods (Inverse Distance Weighting and Empirical Bayesian Kriging. Finally, we evaluated whether those exposed to higher levels of air pollution were less active by performing logistic regression, adjusting for demographic and behavioral risk factors, and after stratifying by body weight category. RESULTS: With Empirical Bayesian Kriging air pollution values, we estimated a statistically significant 16-35% relative increase in the odds of leisure-time physical inactivity per exposure class increase of PM2.5 in the fully adjusted model across the normal weight respondents (p-value<0.0001. Evidence suggested a relationship between the increasing dose of PM2.5 exposure and the increasing odds of physical inactivity. CONCLUSIONS: In a nationally representative, cross-sectional sample, increased community level air pollution is associated with reduced leisure-time physical activity particularly among the normal weight. Although our design precludes a causal inference, these

  20. Trends of chlordane and toxaphene in ambient air of Columbia, South Carolina

    Science.gov (United States)

    Bidleman, T. F.; Alegria, H.; Ngabe, B.; Green, C.

    A long-term record of chlordane and toxaphene (chlorobornanes, CHBs) measurements in Columbia, South Carolina is presented. Chlordane was used as a termiticide in the city and toxaphene was applied to cotton, soybeans and other crops in the region. Ratios among chlordane compounds in ambient air agreed well with those in technical chlordane when weighted for differences in volatility. Atmospheric concentrations ( Ca, pg m -3) in pre-ban years (1988 for chlordane, 1986 for toxaphene) are compared to those made more recently by normalizing concentrations for the effect of varying ambient temperature. Plots of log C a vs 1/ T suggest that chlordane concentrations at 20°C declined by about 40% between pre-ban years and 1994-1995, but no change is apparent at 5°C. Recent concentrations of CHBs are lower than those measured when toxaphene was in use. Temperature slopes are flatter in post-ban years, possibly because of retarded evaporation of old residues as compared to freshly applied pesticide. The 1994-1995 concentrations of chlordanes and CHBs in Columbia air were several times higher than those found in the Great Lakes region. No distinct trend in CHB levels with air transport direction was noted, suggesting that volatilization from local or regional soils is supplying CHBs to Columbia air.

  1. Air Pollution and Preterm Birth in the U.S. State of Georgia (2002–2006): Associations with Concentrations of 11 Ambient Air Pollutants Estimated by Combining Community Multiscale Air Quality Model (CMAQ) Simulations with Stationary Monitor Measurements

    Science.gov (United States)

    Hao, Hua; Chang, Howard H.; Holmes, Heather A.; Mulholland, James A.; Klein, Mitch; Darrow, Lyndsey A.; Strickland, Matthew J.

    2015-01-01

    Background: Previous epidemiologic studies suggest associations between preterm birth and ambient air pollution. Objective: We investigated associations between 11 ambient air pollutants, estimated by combining Community Multiscale Air Quality model (CMAQ) simulations with measurements from stationary monitors, and risk of preterm birth (Darrow LA, Strickland MJ. 2016. Air pollution and preterm birth in the U.S. state of Georgia (2002–2006): associations with concentrations of 11 ambient air pollutants estimated by combining Community Multiscale Air Quality Model (CMAQ) simulations with stationary monitor measurements. Environ Health Perspect 124:875–880; http://dx.doi.org/10.1289/ehp.1409651 PMID:26485731

  2. Designations in US EPA Region 9 for the 1997 8-hour ozone (O3) national ambient air quality standards

    Data.gov (United States)

    U.S. Environmental Protection Agency — Polygon Esri shapefile of designated areas for 8-hour ozone, for the revoked primary and secondary 1997 National Ambient Air Quality Standards (NAAQS). Nonattainment...

  3. Effects of ambient air pollution on upper and lower respiratory symptoms and peak expiratory flow in children

    NARCIS (Netherlands)

    Boezen, H M; van der Zee, S C; Postma, D S; Vonk, J M; Gerritsen, J; Hoek, G; Brunekreef, B; Rijcken, B; Schouten, J P

    1999-01-01

    BACKGROUND: Previous epidemiological studies have shown acute effects of increased amounts of ambient air pollution on the prevalence of respiratory symptoms in children with respiratory disorders. We investigated whether children with bronchial hyperresponsiveness (BHR) and relatively high serum co

  4. Proposed Pathophysiologic Framework to Explain Some Excess Cardiovascular Death Associated with Ambient Air Particle Pollution: Insights for Public Health Translation

    Science.gov (United States)

    The paper proposes a pathophysiologic framework to explain the well-established epidemiological association between exposure to ambient air particle pollution and premature cardiovascular mortality, and offers insights into public health solutions that extend beyond regularory en...

  5. Ambient Air Quality Assessment with Particular Reference to Particulates in Jharia Coalfield, Eastern India.

    Science.gov (United States)

    Singh, Gurdeep; Roy, Debananda; Sinha, Sweta

    2014-01-01

    Jharia Coalfield is the critically polluted area with the intense mining and associated industrial activities. There has been widespread concern of particulate pollution with the alarming levels of Suspended Particulate Matter (SPM) and Respirable Particulate Matter (PM10 & PM2.5). Coke oven plants, coal washing, thermal power stations and associated activities coupled with the transportation activities, give rise to critical air pollution levels in the region. This study envisages the assessment of air pollution of the region with particular reference to SPM, PM10 and PM2.5. Eighteen monitoring stations were selected considering various sources of pollution such as mining, industrial, commercial and residential areas apart from siting criteria as per IS: 5182 Part XIV. Air quality monitoring was carried out following standard methodologies and protocols as per Central Pollution Control Board (CPCB)/ National Ambient Air Quality Standard (NAAQS) norms using Respirable Dust Samplers (RDS) and Fine Particulate Samplers (PM2.5 Samplers). This study reveals considerable load of particulates (SPM, PM10, PM 2.5) which exceed not only the NAAQS but also the coal mining areas standards of Jharia coalfield, thus falling under the category of critically polluted area. Air Quality Indexing has also been developed which provides a clear map of the deterioration of air quality and also presenting comparative ranking of all the monitoring locations with respect to air quality status in the study area.

  6. Removal of polycyclic aromatic hydrocarbons (PAHs) from industrial sludges in the ambient air conditions: automotive industry.

    Science.gov (United States)

    Karaca, Gizem; Tasdemir, Yucel

    2013-01-01

    Removal of polycyclic aromatic hydrocarbons (PAHs) existed in automotive industry treatment sludge was examined by considering the effects of temperature, UV, titanium dioxide (TiO2) and diethyl amine (DEA) in different dosages (i.e., 5% and 20%) in this study. Application of TiO2 and DEA to the sludge samples in ambient environment was studied. Ten PAH (Σ10 PAH) compounds were targeted and their average value in the sludge was found to be 4480 ± 1450 ng/g dry matter (DM). Total PAH content of the sludge was reduced by 25% in the ambient air environment. Meteorological conditions, atmospheric deposition, evaporation and sunlight irradiation played an effective role in the variations in PAH levels during the tests carried out in ambient air environment. Moreover, it was observed that when the ring numbers of PAHs increased, their removal rates also increased. Total PAH level did not change with the addition of 5% DEA and only 10% decreased with 5% TiO2 addition. PAH removal ratios were 8% and 32% when DEA (20%) and TiO2 (20%) were added, respectively. It was concluded that DEA was a weak photo-sensitizer yet TiO2 was effective only at 20% dosage.

  7. A metrological approach to improve accuracy and reliability of ammonia measurements in ambient air

    Science.gov (United States)

    Pogány, Andrea; Balslev-Harder, David; Braban, Christine F.; Cassidy, Nathan; Ebert, Volker; Ferracci, Valerio; Hieta, Tuomas; Leuenberger, Daiana; Martin, Nicholas A.; Pascale, Céline; Peltola, Jari; Persijn, Stefan; Tiebe, Carlo; Twigg, Marsailidh M.; Vaittinen, Olavi; van Wijk, Janneke; Wirtz, Klaus; Niederhauser, Bernhard

    2016-11-01

    The environmental impacts of ammonia (NH3) in ambient air have become more evident in the recent decades, leading to intensifying research in this field. A number of novel analytical techniques and monitoring instruments have been developed, and the quality and availability of reference gas mixtures used for the calibration of measuring instruments has also increased significantly. However, recent inter-comparison measurements show significant discrepancies, indicating that the majority of the newly developed devices and reference materials require further thorough validation. There is a clear need for more intensive metrological research focusing on quality assurance, intercomparability and validations. MetNH3 (Metrology for ammonia in ambient air) is a three-year project within the framework of the European Metrology Research Programme (EMRP), which aims to bring metrological traceability to ambient ammonia measurements in the 0.5-500 nmol mol-1 amount fraction range. This is addressed by working in three areas: (1) improving accuracy and stability of static and dynamic reference gas mixtures, (2) developing an optical transfer standard and (3) establishing the link between high-accuracy metrological standards and field measurements. In this article we describe the concept, aims and first results of the project.

  8. Co-benefits of air quality and climate change policies on air quality of the Mediterranean

    Science.gov (United States)

    Pozzoli, Luca; Mert Gokturk, Ozan; Unal, Alper; Kindap, Tayfun; Janssens-Maenhout, Greet

    2015-04-01

    The Mediterranean basin is one of the regions of the world where significant impacts due to climate changes are predicted to occur in the future. Observations and model simulations are used to provide to the policy makers scientifically based estimates of the necessity to adjust national emission reductions needed to achieve air quality objectives in the context of a changing climate, which is not only driven by GHGs, but also by short lived climate pollutants, such as tropospheric ozone and aerosols. There is an increasing interest and need to design cost-benefit emission reduction strategies, which could improve both regional air quality and global climate change. In this study we used the WRF-CMAQ air quality modelling system to quantify the contribution of anthropogenic emissions to ozone and particulate matter concentrations in Europe and the Eastern Mediterranean and to understand how this contribution could change in different future scenarios. We have investigated four different future scenarios for year 2050 defined during the European Project CIRCE: a "business as usual" scenario (BAU) where no or just actual measures are taken into account; an "air quality" scenario (BAP) which implements the National Emission Ceiling directive 2001/81/EC member states of the European Union (EU-27); a "climate change" scenario (CC) which implements global climate policies decoupled from air pollution policies; and an "integrated air quality and climate policy" scenario (CAP) which explores the co-benefit of global climate and EU-27 air pollution policies. The BAP scenario largely decreases summer ozone concentrations over almost the entire continent, while the CC and CAP scenarios similarly determine lower decreases in summer ozone but extending all over the Mediterranean, the Middle East countries and Russia. Similar patterns are found for winter PM concentrations; BAP scenario improves pollution levels only in the Western EU countries, and the CAP scenario determines

  9. Seasonal Variability of Concentration and Air Quality of Ambient Particulate Matter in Sosnowiec City

    Directory of Open Access Journals (Sweden)

    Jolanta Cembrzyńska

    2015-12-01

    Full Text Available Introduction: Exposing the population to more than standard concentration of particulate matter (PM is a crucial factor shaping the public health on urbanized areas both in Europe and Poland. In most cases, exceeded air quality standards relate to the winter period, in which there has been the greatest amount. Many studies have indicated, that exposure to PM can cause adverse health effects. Human exposure especially to fine particles (with an aerodynamic diameter less than 2.5 µm, causes risk of cardiovascular and respiratory diseases, due to daily mortality and hospital admissions. Various types of epidemiological studies have indicated, that ambient air pollution is responsible for increasing risk of lung cancer. For this reason, in 2013 The International Agency for Research on Cancer (IARC classified outdoor air pollution and particulate matter as carcinogenic to humans (Group 1.

  10. Quantification Method for Electrolytic Sensors in Long-Term Monitoring of Ambient Air Quality.

    Science.gov (United States)

    Masson, Nicholas; Piedrahita, Ricardo; Hannigan, Michael

    2015-10-27

    Traditional air quality monitoring relies on point measurements from a small number of high-end devices. The recent growth in low-cost air sensing technology stands to revolutionize the way in which air quality data are collected and utilized. While several technologies have emerged in the field of low-cost monitoring, all suffer from similar challenges in data quality. One technology that shows particular promise is that of electrolytic (also known as amperometric) sensors. These sensors produce an electric current in response to target pollutants. This work addresses the development of practical models for understanding and quantifying the signal response of electrolytic sensors. Such models compensate for confounding effects on the sensor response, such as ambient temperature and humidity, and address other issues that affect the usability of low-cost sensors, such as sensor drift and inter-sensor variability.

  11. Influence of chemical and physical forms of ambient air acids on airway doses

    Energy Technology Data Exchange (ETDEWEB)

    Larson, T.V.

    1989-02-01

    The effects of ambient relative humidity and particle size on acid deposition within the airways have been examined with a computer model. For H/sub 2/SO/sub 4/ particles initially at 90% relative humidity in ambient air that are inhaled via the nose or mouth, there is significant deposition of acid in the airways even in the presence of typical values of respiratory NH/sub 3/. When these same particles are found in a fog at 100.015% relative humidity, there is significant deposition of acid in the nasal region during nose breathing but insignificant deposition to the deep lung for either nose or mouth breathing. The factors governing the partitioning of labile acid gases in the gas and liquid phases prior to inhalation are also discussed.

  12. Ambient air pollution exposure and the incidence of related health effects among racial/ethnic minorities

    Energy Technology Data Exchange (ETDEWEB)

    Nieves, L.A.; Wernette, D.R.

    1997-02-01

    Differences among racial and ethnic groups in morbidity and mortality rates for diseases, including diseases with environmental causes, have been extensively documented. However, documenting the linkages between environmental contaminants, individual exposures, and disease incidence has been hindered by difficulties in measuring exposure for the population in general and for minority populations in particular. After briefly discussing research findings on associations of common air pollutants with disease incidence, the authors summarize recent studies of radial/ethnic subgroup differences in incidence of these diseases in the US. They then present evidence of both historic and current patterns of disproportionate minority group exposure to air pollution as measured by residence in areas where ambient air quality standards are violated. The current indications of disproportionate potential exposures of minority and low-income populations to air pollutants represent the continuation of a historical trend. The evidence of linkage between disproportionate exposure to air pollution of racial/ethnic minorities and low-income groups and their higher rates of some air pollution-related diseases is largely circumstantial. Differences in disease incidence and mortality rates among racial/ethnic groups are discussed for respiratory diseases, cancers, and lead poisoning. Pollutants of concern include CO, Pb, SO{sub 2}, O{sub 3}, and particulates.

  13. Low Energy Air Conditioning for Hot Climates

    OpenAIRE

    Almutairi, Hamad Hhn

    2012-01-01

    Fossil fuels are the major sources of electrical power generation in the world. Among all fossil fuels, oil is considered as the most sought-after fuel. The burden on countries that provide subsidized electricity produced from oil-fired power plants is noteworthy. Kuwait is a notable example of these countries. Electricity in Kuwait is heavily consumed by residential air conditioning, which comprises 60% of the total electricity generated at peak times on a hot summer day. From this perspecti...

  14. Innovative Air Conditioning and Climate Control

    Science.gov (United States)

    Graf, John

    2015-01-01

    NASA needed to develop a desiccant wheel based humidity removal system to enable the long term testing of the Orion CO2 scrubber on the International Space Station. In the course of developing that system, we learned three things that are relevant to energy efficient air conditioning of office towers. NASA developed a conceptual design for a humidity removal system for an office tower environment. We are looking for interested partners to prototype and field test this concept.

  15. Ambient air pollution and risk of birth defects in Southern California.

    Science.gov (United States)

    Ritz, Beate; Yu, Fei; Fruin, Scott; Chapa, Guadalupe; Shaw, Gary M; Harris, John A

    2002-01-01

    The authors evaluated the effect of air pollution on the occurrence of birth defects ascertained by the California Birth Defects Monitoring Program in neonates and fetuses delivered in southern California in 1987-1993. By using measurements from ambient monitoring stations of carbon monoxide (CO), nitrogen dioxide, ozone, and particulate matter <10 microm in aerodynamic diameter, they calculated average monthly exposure estimates for each pregnancy. Conventional, polytomous, and hierarchical logistic regression was used to estimate odds ratios for subgroups of cardiac and orofacial defects. Odds ratios for cardiac ventricular septal defects increased in a dose-response fashion with increasing second-month CO exposure (odds ratio (OR)(2nd quartile) CO = 1.62, 95% confidence interval (CI): 1.05, 2.48; OR(3rd quartile) CO = 2.09, 95% CI: 1.19, 3.67; OR(4th quartile) CO = 2.95, 95% CI: 1.44, 6.05). Similarly, risks for aortic artery and valve defects, pulmonary artery and valve anomalies, and conotruncal defects increased with second-month ozone exposure. The study was inconclusive for other air pollutants. The authors' results are supported by the specificity of the timing of the effect and some evidence from animal data; however, this is the first known study to link ambient air pollution during a vulnerable window of development to human malformations. Confirmation by further studies is needed.

  16. Sources of Particular Pollutants in Ambient Air at a Petrochemical Enterprise

    Institute of Scientific and Technical Information of China (English)

    Xue Jianliang; Zhao Dongfeng; ChengJianguang; Chen Lu; Liu Wei

    2013-01-01

    The study on source apportionment of particular pollutants in ambient air at a petrochemical enterprise is the ba-sis of the control over air pollution. Through analyzing particular pollutants in the samples collected from one petrochemi-cal enterprise in northwestern China, the sources of particular pollutants were discussed. The test results showed that con-centrations of particular pollutants in different sites were remarkably different. Results showed that the sampling sites with higher concentrations of particular pollutants, including toluene, xylenes, NH3 and H2S, were located at the boundary of the petrochemical enterprise. Instead, the concentrations of NMHC in the ambient air sampling sites were higher than those at the boundary of the petrochemical enterprise. The sampling sites with higher concentrations of particular pollutants were located in the area that was close to the petrochemical enterprise. The results obtained from the Pearson correlation co-efifcients analyses, the factor analyses, andχ2-tests of the particular pollutants had revealed that NH3, H2S, toluene and xylenes at all sampling sites came from the same source, while NMHC might come from some other sources besides the petrochemical enterprise.

  17. Particle-bound Dechlorane Plus and polybrominated diphenyl ethers in ambient air around Shanghai, China

    Energy Technology Data Exchange (ETDEWEB)

    Yu Zhiqiang [State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environment and Resources, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640 (China); Liao Ru' e [State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environment and Resources, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640 (China); Graduate School of the Chinese Academy of Sciences, Beijing 100039 (China); Li Huiru, E-mail: huiruli@gig.ac.cn [State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environment and Resources, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640 (China); Mo Ligui [State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environment and Resources, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640 (China); Graduate School of the Chinese Academy of Sciences, Beijing 100039 (China); Zeng Xiangying; Sheng Guoying; Fu Jiamo [State Key Laboratory of Organic Geochemistry, Guangdong Key Laboratory of Environment and Resources, Guangzhou Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640 (China)

    2011-10-15

    In present study, atmospheric particles from Shanghai, the biggest city and the most important industrial base in China, were analyzed for polybrominated diphenyl ethers (PBDEs) and Dechlorane Plus (DP). Concentrations of {Sigma}{sub 20}PBDEs and DP both exhibited the changing trend of industrial area > urban areas. Jiading District had the highest levels of particulate PBDEs and DP with values of 744 {+-} 152 pg/m{sup 3} and 5.48 {+-} 1.28 pg/m{sup 3}, respectively. Compared with similar data in other areas of the world, PBDEs in Shanghai were at medium pollution level, while DP was at lower level, which reflected their different production and use in Shanghai. The results from multiple linear regression analysis suggested that deca-BDE mixture was the most important contributor of particulate PBDEs in Shanghai. The fractions of anti-DP showed no significant differences to those of the technical mixtures (p > 0.05), which suggested that no obviously stereoselective process occurred in ambient air around Shanghai. - Highlights: > Atmospheric PBDEs of Shanghai were at moderate levels and dominated by BDE-209. > Particulate DP was low even Shanghai is not far from the DP manufacturing factory. > DP showed no obviously stereoselective process in air particles from Shanghai. > Significant positive correlation was found between particulate PBDEs and PBDD/Fs. - The moderate PBDEs levels with deca-BDE being the most important contributor and low DP levels in ambient air around Shanghai reflected their different usage in this area.

  18. Mass spectrometry of solid samples in open air using combined laser ionization and ambient metastable ionization

    Science.gov (United States)

    He, X. N.; Xie, Z. Q.; Gao, Y.; Hu, W.; Guo, L. B.; Jiang, L.; Lu, Y. F.

    2012-01-01

    Mass spectrometry of solid samples in open air was carried out using combined laser ionization and metastable ionization time-of-flight mass spectrometry (LI-MI-TOFMS) in ambient environment for qualitative and semiquantitative (relative analyte information, not absolute information) analysis. Ambient metastable ionization using a direct analysis in realtime (DART) ion source was combined with laser ionization time-of-flight mass spectrometry (LI-TOFMS) to study the effects of combining metastable and laser ionization. A series of metallic samples from the National Institute of Standards and Technology (NIST 494, 495, 498, 499, and 500) and a pure carbon target were characterized using LI-TOFMS in open air. LI-MI-TOFMS was found to be superior to laser-induced breakdown spectroscopy (LIBS). Laser pulse energies between 10 and 200 mJ at the second harmonic (532 nm) of an Nd:YAG laser were applied in the experiment to obtain a high degree of ionization in plasmas. Higher laser pulse energy improves signal intensities of trace elements (such as Fe, Cr, Mn, Ni, Ca, Al, and Ag). Data were analyzed by numerically calculating relative sensitivity coefficients (RSCs) and limit of detections (LODs) from mass spectrometry (MS) and LIBS spectra. Different parameters, such as boiling point, ionization potential, RSC, LOD, and atomic weight, were shown to analyze the ionization and MS detection processes in open air.

  19. Ambient air pollution and lung disease in China: health effects, study design approaches and future research.

    Science.gov (United States)

    Mandel, Jeffrey H; Wendt, Christine; Lo, Charles; Zhou, Guangbiao; Hertz, Marshall; Ramachandran, Gurumurthy

    2015-09-01

    Ambient air pollution in China has worsened following dramatic increases in industrialization, automobile use and energy consumption. Particularly bothersome is the increase in the PM2.5 fraction of pollutants. This fraction has been associated with increasing rates of cardio-respiratory disease in China and elsewhere. Ambient pollutant levels have been described in many of China's cities and are comparable to previous levels in southern California. Lung cancer mortality in China has increased since the 1970s and has been higher in men and in urban areas, the exact explanation for which has not been determined. The estimation of individual risk for Chinese citizens living in areas of air pollution will require further research. Occupational cohort and case-control designs each have unique attributes that could make them helpful to use in this setting. Other important future research considerations include detailed exposure assessment and the possible use of biomarkers as a means to better understand and manage the threat posed by air pollution in China.

  20. Impact of a new gasoline benzene regulation on ambient air pollutants in Anchorage, Alaska

    Science.gov (United States)

    Yano, Yuriko; Morris, Stephen S.; Salerno, Christopher; Schlapia, Anne M.; Stichick, Mathew

    2016-05-01

    The purpose of this study was to quantify the impact of a new U.S. Environmental Protection Agency (EPA) standard that limits the amount of benzene allowed in gasoline on ambient benzene concentrations. This new standard, together with two companion regulations that limit cold-temperature automotive emissions and the permeability of portable fuel containers, was expected to lower the levels of ambient benzene and other volatile organic compounds (VOCs) nationwide. In this study the impact of the gasoline benzene standard was evaluated in Anchorage, Alaska in a two-phase ambient air monitoring study conducted before and after the new gasoline standard was implemented. Gasoline sold by Anchorage retailers was also evaluated in each phase to determine the content of benzene and other gasoline components. The average benzene content in Anchorage gasoline was reduced by 70%, from 5.05% (w/w) to 1.53% (w/w) following the implementation of the standard. The annual mean ambient benzene concentration fell by 51%, from 0.99 ppbv in Phase 1 to 0.49 ppbv in Phase 2. Analysis suggests the change in gasoline benzene content alone reduced benzene emissions by 46%. The changes in toluene, ethylbenzene, and xylene content in gasoline between Phase 1 and 2 were relatively small and the differences in the mean ambient concentrations of these compounds between phases were modest. Our results suggest that cold winter communities in high latitude and mountainous regions may benefit more from the gasoline benzene standard because of high benzene emissions resulting from vehicle cold start and a tendency to develop atmospheric stagnation conditions in the winter.

  1. Linking Urban Air Pollution to Global Tropospheric Chemistry and Climate

    Science.gov (United States)

    Wang, Chien

    2005-01-01

    The two major tasks of this project are to study: (a) the impact of urban nonlinear chemistry on chemical budgets of key pollutants in non-urban areas; and (b) the influence of air pollution control strategies in selected metropolitan areas, particularly of emerging economies in East and South Asia, on tropospheric chemistry and hence on regional and global climate.

  2. In situ secondary organic aerosol formation from ambient pine forest air using an oxidation flow reactor

    Directory of Open Access Journals (Sweden)

    B. B. Palm

    2015-11-01

    Full Text Available Ambient air was oxidized by OH radicals in an oxidation flow reactor (OFR located in a montane pine forest during the BEACHON-RoMBAS campaign to study biogenic secondary organic aerosol (SOA formation and aging. High OH concentrations and short residence times allowed for semi-continuous cycling through a large range of OH exposures ranging from hours to weeks of equivalent (eq. atmospheric aging. A simple model is derived and used to account for the relative time scales of condensation of low volatility organic compounds (LVOCs onto particles, condensational loss to the walls, and further reaction to produce volatile, non-condensing fragmentation products. More SOA production was observed in the OFR at nighttime (average 4 μg m-3 when LVOC fate corrected compared to daytime (average 1 μg m-3 when LVOC fate corrected, with maximum formation observed at 0.4–1.5 eq. days of photochemical aging. SOA formation followed a similar diurnal pattern to monoterpenes, sesquiterpenes, and toluene + p-cymene concentrations, including a substantial increase just after sunrise at 07:00 LT. Higher photochemical aging (> 10 eq. days led to a decrease in new SOA formation and a loss of preexisting OA due to heterogeneous oxidation followed by fragmentation and volatilization. When comparing two different commonly used methods of OH production in OFRs (OFR185 and OFR254, similar amounts of SOA formation were observed. We recommend the OFR185 mode for future forest studies. Concurrent gas-phase measurements of air after OH oxidation illustrate the decay of primary VOCs, production of small oxidized organic compounds, and net production at lower ages followed by net consumption of terpenoid oxidation products as photochemical age increased. New particle formation was observed in the reactor after oxidation, especially during times when precursor gas concentrations and SOA formation were largest. Approximately 6 times more SOA was formed in the reactor from OH

  3. European air pollution in 2050, a regional air quality and climate perspective under CMIP5 scenarios

    Science.gov (United States)

    Colette, A.; Bessagnet, B.; Vautard, R.; Szopa, S.; Rao, S.; Schucht, S.; Klimont, Z.; Holland, M.; Menut, L.; Meleux, F.; Rouïl, L.

    2013-12-01

    Air pollution and climate change are closely related. They share both driving geophysical processes and mitigation strategies. Increased temperature, changes in weather regimes and precipitation patterns will alter the formation of pollution episodes. At the same time curbing greenhouse gases emission will also induce indirect co-benefits for air pollutant emissions. As a consequence, understanding the long-term efficiency of air pollution mitigation strategies requires the integrated implementation of comprehensive geophysical and economical models. Coupling air pollution and climate models for long term projections raise a number of scientific and technical issues. Global scale circulation outputs must be downscaled in order to provide high resolution three dimensional meteorological fields at high temporal frequency to the chemistry transport model. The computational cost of the air quality model is comparable to the cost of the regional climate model. So that the computing demand and storage call for an efficient design of a complex modelling suite. Moreover the cost of the project prohibits the implementation of large ensemble of model, thereby raising concerns on the treatment of uncertainty analyses of the projections. We present an integrated assessment of future air quality that relies on up-to-date emission scenarios and full-frame geophysical models of climate and atmospheric chemistry which are themselves embedded in monetised economical models to propose a cost-benefit assessment. Emissions: For long lived trace species, we use the Representative Concentrations Pathways (RCP) produced for the Fifth Assessment Report (AR5) of IPCC whereas regional air quality modelling is based on the updated emissions scenarios produced in the framework of the Global Energy Assessment (GEA) that offer an explicit representation of air quality policies. Climate and chemistry models: We use the latest sources of recent coordinated model intercomparison projects, each

  4. Global Air Quality and Climate Impacts of Mitigating Short-lived Climate Pollution in China

    Science.gov (United States)

    Harper, K.; Unger, N.; Heyes, C.; Kiesewetter, G.; Klimont, Z.; Schoepp, W.; Wagner, F.

    2014-12-01

    China is a major emitter of harmful air pollutants, including the short-lived climate pollutants (SLCPs) and their precursors. Implementation of pollution control technologies provides a mechanism for simultaneously protecting human and ecosystem health and achieving near-term climate co-benefits; however, predicting the outcomes of technical and policy interventions is challenging because the SLCPs participate in both climate warming and cooling and share many common emission sources. Here, we present the results of a combined regional integrated assessment and global climate modeling study aimed at quantifying the near-term climate and air quality co-benefits of selective control of Chinese air pollution emissions. Results from IIASA's Greenhouse Gas - Air Pollution Interactions and Synergies (GAINS) integrated assessment model indicate that methane emission reductions make up > 75% of possible CO2-equivalent emission reductions of the SLCPs and their precursors in China in 2030. A multi-pollutant emission reduction scenario incorporating the 2030 Chinese pollution control measures with the highest potential for future climate impact is applied to the NASA ModelE2 - Yale Interactive Terrestrial Biosphere (NASA ModelE2-YIBs) global carbon - chemistry - climate model to assess the regional and long-range impacts of Chinese SLCP mitigation measures. Using model simulations that incorporate dynamic methane emissions and photosynthesis-dependent isoprene emissions, we quantify the impacts of Chinese reductions of the short-lived air pollutants on radiative forcing and on surface ozone and particulate air pollution. Present-day modeled methane mole fractions are evaluated against SCIAMACHY methane columns and NOAA ESRL/GMD surface flask measurements.

  5. Recent climate and air pollution impacts on Indian agriculture.

    Science.gov (United States)

    Burney, Jennifer; Ramanathan, V

    2014-11-18

    Recent research on the agricultural impacts of climate change has primarily focused on the roles of temperature and precipitation. These studies show that India has already been negatively affected by recent climate trends. However, anthropogenic climate changes are a result of both global emissions of long-lived greenhouse gases (LLGHGs) and other short-lived climate pollutants (SLCPs). Two potent SLCPs, tropospheric ozone and black carbon, have direct effects on crop yields beyond their indirect effects through climate; emissions of black carbon and ozone precursors have risen dramatically in India over the past three decades. Here, to our knowledge for the first time, we present results of the combined effects of climate change and the direct effects of SLCPs on wheat and rice yields in India from 1980 to 2010. Our statistical model suggests that, averaged over India, yields in 2010 were up to 36% lower for wheat than they otherwise would have been, absent climate and pollutant emissions trends, with some densely populated states experiencing 50% relative yield losses. [Our point estimates for rice (-20%) are similarly large, but not statistically significant.] Upper-bound estimates suggest that an overwhelming fraction (90%) of these losses is due to the direct effects of SLCPs. Gains from addressing regional air pollution could thus counter expected future yield losses resulting from direct climate change effects of LLGHGs.

  6. Ambient air pollution exposure and full-term birth weight in California

    Directory of Open Access Journals (Sweden)

    Sadd James L

    2010-07-01

    Full Text Available Abstract Background Studies have identified relationships between air pollution and birth weight, but have been inconsistent in identifying individual pollutants inversely associated with birth weight or elucidating susceptibility of the fetus by trimester of exposure. We examined effects of prenatal ambient pollution exposure on average birth weight and risk of low birth weight in full-term births. Methods We estimated average ambient air pollutant concentrations throughout pregnancy in the neighborhoods of women who delivered term singleton live births between 1996 and 2006 in California. We adjusted effect estimates of air pollutants on birth weight for infant characteristics, maternal characteristics, neighborhood socioeconomic factors, and year and season of birth. Results 3,545,177 singleton births had monitoring for at least one air pollutant within a 10 km radius of the tract or ZIP Code of the mother's residence. In multivariate models, pollutants were associated with decreased birth weight; -5.4 grams (95% confidence interval -6.8 g, -4.1 g per ppm carbon monoxide, -9.0 g (-9.6 g, -8.4 g per pphm nitrogen dioxide, -5.7 g (-6.6 g, -4.9 g per pphm ozone, -7.7 g (-7.9 g, -6.6 g per 10 μg/m3 particulate matter under 10 μm, -12.8 g (-14.3 g, -11.3 g per 10 μg/m3 particulate matter under 2.5 μm, and -9.3 g (-10.7 g, -7.9 g per 10 μg/m3 of coarse particulate matter. With the exception of carbon monoxide, estimates were largely unchanged after controlling for co-pollutants. Effect estimates for the third trimester largely reflect the results seen from full pregnancy exposure estimates; greater variation in results is seen in effect estimates specific to the first and second trimesters. Conclusions This study indicates that maternal exposure to ambient air pollution results in modestly lower infant birth weight. A small decline in birth weight is unlikely to have clinical relevance for individual infants, and there is debate about whether

  7. Ambient air quality trends and driving factor analysis in Beijing, 1983-2007

    Institute of Scientific and Technical Information of China (English)

    Ju Zhang; Zhiyun Ouyang; Hong Miao; Xiaoke Wang

    2011-01-01

    The rapid development in Beijing,the capital of China,has resulted in serious air pollution problems.Meanwhile great efforts have been made to improve the air quality,especially since 1998.The variation in air quality under the interaction of pollution and control in this mega city has attracted much attention.We analyzed the changes in ambient air quality in Beijing since the 1980's using the Daniel trend test based on data from long-term monitoring stations.The results showed that different pollutants displayed three trends:a decreasing trend,an increasing trend and a fiat trend.SO2,dustfall,B[a]P,NO2 and PM10 fit decreasing trend pattern,while NOx showed an increasing trend,and CO,ozone pollution,total suspended particulate (TSP),as well as Pb fit the flat trend.The cause of the general air pollution in Beijing has changed from being predominantly related to coal burning to mixed traffic exhaust and coal burning related pollution.Seasonally,the pollution level is typically higher during the heating season from November to the following March.The interaction between pollution sources change and implementation of air pollution control measures was the main driving factor that caused the variation in air quality.Changes of industrial structure and improved energy efficiency,the use of clean energy and preferred use of clean coal,reduction in pollution sources,and implementation of advanced environmental standards have all contributed to the reduction in air pollution,particularly since 1998.

  8. Climate Change and Air Pollution: Effects on Respiratory Allergy.

    Science.gov (United States)

    D'Amato, Gennaro; Pawankar, Ruby; Vitale, Carolina; Lanza, Maurizia; Molino, Antonio; Stanziola, Anna; Sanduzzi, Alessandro; Vatrella, Alessandro; D'Amato, Maria

    2016-09-01

    A body of evidence suggests that major changes involving the atmosphere and the climate, including global warming induced by anthropogenic factors, have impact on the biosphere and human environment. Studies on the effects of climate change on respiratory allergy are still lacking and current knowledge is provided by epidemiological and experimental studies on the relationship between allergic respiratory diseases, asthma and environmental factors, such as meteorological variables, airborne allergens, and air pollution. Urbanization with its high levels of vehicle emissions, and a westernized lifestyle are linked to the rising frequency of respiratory allergic diseases and bronchial asthma observed over recent decades in most industrialized countries. However, it is not easy to evaluate the impact of climate changes and air pollution on the prevalence of asthma in the general population and on the timing of asthma exacerbations, although the global rise in asthma prevalence and severity could also be an effect of air pollution and climate change. Since airborne allergens and air pollutants are frequently increased contemporaneously in the atmosphere, an enhanced IgE-mediated response to aeroallergens and enhanced airway inflammation could account for the increasing frequency of respiratory allergy and asthma in atopic subjects in the last 5 decades. Pollen allergy is frequently used to study the relationship between air pollution and respiratory allergic diseases, such as rhinitis and bronchial asthma. Epidemiologic studies have demonstrated that urbanization, high levels of vehicle emissions, and westernized lifestyle are correlated with an increased frequency of respiratory allergy prevalently in people who live in urban areas in comparison with people living in rural areas. Climatic factors (temperature, wind speed, humidity, thunderstorms, etc.) can affect both components (biological and chemical) of this interaction.

  9. Spatially differentiated and source-specific population exposure to ambient urban air pollution

    Science.gov (United States)

    Zou, Bin; Wilson, J. Gaines; Zhan, F. Benjamin; Zeng, Yongnian

    Models assessing exposure to air pollution often focus on macro-scale estimates of exposure to all types of sources for a particular pollutant across an urban study area. While results based on these models may aid policy makers in identifying larger areas of elevated exposure risk, they often do not differentiate the proportion of population exposure attributable to different polluting sources (e.g. traffic or industrial). In this paper, we introduce a population exposure modeling system that integrates air dispersion modeling, Geographic Information Systems (GIS), and population exposure techniques to spatially characterize a source-specific exposure to ambient air pollution for an entire urban population at a fine geographical scale. By area, total population exposure in Dallas County in 2000 was more attributable to vehicle polluting sources than industrial polluting sources at all levels of exposure. Population exposure was moderately correlated with vehicle sources ( r = 0.440, p air quality assessments must incorporate more than industrial or vehicle polluting sources-based population exposure values alone, but should consider multiple sources. The population exposure modeling system proposed in this study shows promise for use by municipal authorities, policy makers, and epidemiologists in evaluating and controlling the quality of the air in the process of urban planning and mitigation measures.

  10. Energy and material balance of CO2 capture from ambient air.

    Science.gov (United States)

    Zeman, Frank

    2007-11-01

    Current Carbon Capture and Storage (CCS) technologies focus on large, stationary sources that produce approximately 50% of global CO2 emissions. We propose an industrial technology that captures CO2 directly from ambient air to target the remaining emissions. First, a wet scrubbing technique absorbs CO2 into a sodium hydroxide solution. The resultant carbonate is transferred from sodium ions to calcium ions via causticization. The captured CO2 is released from the calcium carbonate through thermal calcination in a modified kiln. The energy consumption is calculated as 350 kJ/mol of CO2 captured. It is dominated by the thermal energy demand of the kiln and the mechanical power required for air movement. The low concentration of CO2 in air requires a throughput of 3 million cubic meters of air per ton of CO2 removed, which could result in significant water losses. Electricity consumption in the process results in CO2 emissions and the use of coal power would significantly reduce to net amount captured. The thermodynamic efficiency of this process is low but comparable to other "end of pipe" capture technologies. As another carbon mitigation technology, air capture could allow for the continued use of liquid hydrocarbon fuels in the transportation sector.

  11. A statistical modeling framework for projecting future ambient ozone and its health impact due to climate change

    Science.gov (United States)

    Chang, Howard H.; Hao, Hua; Sarnat, Stefanie Ebelt

    2014-06-01

    The adverse health effects of ambient ozone are well established. Given the high sensitivity of ambient ozone concentrations to meteorological conditions, the impacts of future climate change on ozone concentrations and its associated health effects are of concern. We describe a statistical modeling framework for projecting future ozone levels and its health impacts under a changing climate. This is motivated by the continual effort to evaluate projection uncertainties to inform public health risk assessment. The proposed approach was applied to the 20-county Atlanta metropolitan area using regional climate model (RCM) simulations from the North American Regional Climate Change Assessment Program. Future ozone levels and ozone-related excesses in asthma emergency department (ED) visits were examined for the period 2041-2070. The computationally efficient approach allowed us to consider 8 sets of climate model outputs based on different combinations of 4 RCMs and 4 general circulation models. Compared to the historical period of 1999-2004, we found consistent projections across climate models of an average 11.5% higher ozone levels (range: 4.8%, 16.2%), and an average 8.3% (range: -7%-24%) higher number of ozone exceedance days. Assuming no change in the at-risk population, this corresponds to excess ozone-related ED visits ranging from 267 to 466 visits per year. Health impact projection uncertainty was driven predominantly by uncertainty in the health effect association and climate model variability. Calibrating climate simulations with historical observations reduced differences in projections across climate models.

  12. Assessment of selected metals in the ambient air PM10 in urban sites of Bangkok (Thailand).

    Science.gov (United States)

    Pongpiachan, Siwatt; Iijima, Akihiro

    2016-02-01

    Estimating the atmospheric concentrations of PM10-bounded selected metals in urban air is crucial for evaluating adverse health impacts. In the current study, a combination of measurements and multivariate statistical tools was used to investigate the influence of anthropogenic activities on variations in the contents of 18 metals (i.e., Al, Sc, V, Cr, Mn, Fe, Co, Ni, Cu, Zn, As, Se, Cd, Sb, Ba, La, Ce and Pb) in ambient air. The concentrations of PM10-bounded metals were measured simultaneously at eight air quality observatory sites during a half-year period at heavily trafficked roads and in urban residential zones in Bangkok, Thailand. Although the daily average concentrations of Al, V, Cr, Mn and Fe were almost equivalent to those of other urban cities around the world, the contents of the majority of the selected metals were much lower than the existing ambient air quality guidelines and standard limit values. The sequence of average values of selected metals followed the order of Al > Fe > Zn > Cu > Pb > Mn > Ba > V > Sb > Ni > As > Cr > Cd > Se > Ce > La > Co > Sc. The probability distribution function (PDF) plots showed sharp symmetrical bell-shaped curves in V and Cr, indicating that crustal emissions are the predominant sources of these two elements in PM10. The comparatively low coefficients of divergence (COD) that were found in the majority of samples highlight that site-specific effects are of minor importance. A principal component analysis (PCA) revealed that 37.74, 13.51 and 11.32 % of the total variances represent crustal emissions, vehicular exhausts and the wear and tear of brakes and tires, respectively.

  13. Ambient Air Quality Assessment With Particular Reference to Particulates in Western Part of Jharia Coalfield, India

    Directory of Open Access Journals (Sweden)

    Gurdeep Singh

    2015-08-01

    Full Text Available India is in the list of fastest growing countries of the world. India's energy needs are also increasing due to population and industrial growth for improving quality of living style. In India, coal is major input infrastructure industries for example Power plants, Steel plants and Cement industries. India’s 52% of primary energy is coal dependent1. 66% of India's power generation depends upon coal production1. Jharia Coalfield (JCF is falling in the Lower Gondwana Coalfields of India. The area of the JCF is about 450 km2. It is important for the major supply of precious coking coal required for steel plants in India. It is located in Dhanbad district of Jharkhand state of India, The latitude is 23° 39' to 23° 48' N and longitude is 86° 11' to 86° 27' E for the Jharia coalfield. Based on environmental parameters, all the 103 mines of BCCL have been grouped under 17 Clusters. A cluster consists of a group of mines with mine lease boundary lying in close vicinity and includes-Operating mines, Abandoned/ closed mines and proposed projects.The focused study area is in the western part of the Jharia coalfield is named as Cluster XV group of mines of BCCL consists of four mines, Kharkharee Colliery (UG, Dharmaband Colliery (UG, Madhuband Colliery (UG and Phularitand Colliery (UG .The present study was carried out with the objective to measure the ambient air quality of the study area with reference to particulate matter (SPM, PM10 & PM2.5. Ambient air monitoring results have shown that the observe air quality were found within the limit prescribed by MoEF / CPCB. It may due to Underground mines as there are pollution causing lesser activities involved in the UG mining process compared to opencast mining. Implementation of Master plan for Jharia coalfields for environmental management has also improve the air quality in the area10,11.

  14. A proposed methodology for the assessment of arsenic, nickel, cadmium and lead levels in ambient air

    Energy Technology Data Exchange (ETDEWEB)

    Santos, Germán, E-mail: santosg@unican.es; Fernández-Olmo, Ignacio

    2016-06-01

    Air quality assessment, required by the European Union (EU) Air Quality Directive, Directive 2008/50/EC, is part of the functions attributed to Environmental Management authorities. Based on the cost and time consumption associated with the experimental works required for the air quality assessment in relation to the EU-regulated metal and metalloids, other methods such as modelling or objective estimation arise as competitive alternatives when, in accordance with the Air Quality Directive, the levels of pollutants permit their use at a specific location. This work investigates the possibility of using statistical models based on Partial Least Squares Regression (PLSR) and Artificial Neural Networks (ANNs) to estimate the levels of arsenic (As), cadmium (Cd), nickel (Ni) and lead (Pb) in ambient air and their application for policy purposes. A methodology comprising the main steps that should be taken into consideration to prepare the input database, develop the model and evaluate their performance is proposed and applied to a case of study in Santander (Spain). It was observed that even though these approaches present some difficulties in estimating the individual sample concentrations, having an equivalent performance they can be considered valid for the estimation of the mean values – those to be compared with the limit/target values – fulfilling the uncertainty requirements in the context of the Air Quality Directive. Additionally, the influence of the consideration of input variables related to atmospheric stability on the performance of the studied statistical models has been determined. Although the consideration of these variables as additional inputs had no effect on As and Cd models, they did yield an improvement for Pb and Ni, especially with regard to ANN models. - Highlights: • EU encourages modelling techniques over measurements for air quality assessment. • A methodology for minor pollutants assessment by statistical modelling is presented.

  15. CARBONIZED FIBROUS RESIN AS A NEW SORBENT FOR SAMPLING POLYCYCLIC AROMATIC HYDROCARBONS (PAHS) IN AMBIENT AIR

    Institute of Scientific and Technical Information of China (English)

    2002-01-01

    A new sampling method of ambient air analysis using carbonized fibrous resin as asorbent for polycyclic aromatic hydrocarbons (PAHs) was reported.The physical and chemical properties of the carbonized fibrous resins were measured. Thesample pretreatment with ultrasonic extraction and subsequent clean-up ehition through a silica gelcolumn was optimized. The suitable ultrasonic extraction conditions were selected as follows: resinweight was 1.5 g, ultrasonic extraction time 20 min, volume of extraction solvent 100 mi andextraction operation times 2~3. The concentrated extractable organic matter was submitted to nextstep of clean-up procedure of adsorption chromatography on silica gel column/n-hexane and amixture of dichloromethene:n-hexane solution 2:3 (v/v). The PAHs fractions in the real samplesfrom Changzhou, China were particularly analyzed using GC-MS data system and the data of massspectra, retention times and scan numbers of the real samples were compared with that of thestandards of 16 PAHs listed by the US EPA as "priority pollutants" of the environment. Theanalysis of the real samples indicates that the carbonized fibrous resin is a good sorbent. Thepretreatment of samples of ambient air with carbonized fibrous resin as a sorbent for P,AHs isproved to be reliable and might be used for the procedure of the determination of PAHs inatmospheric environment.

  16. An isotopic dilution approach for 1,3-butadiene tailpipe emissions and ambient air monitoring.

    Science.gov (United States)

    Riservato, Manuela; Rolla, Antonio; Davoli, Enrico

    2004-01-01

    An isotopic dilution approach for 1,3-butadiene analysis in gaseous samples is presented. The methodology is based on active sampling on sorbent tubes and subsequent analysis by thermal desorption into a gas chromatography/mass spectrometry system. By adding a perdeuterated internal standard onto the sorbent tubes before sampling, and using mass spectrometric detection, the methodology gives high accuracy for this unstable analyte. The method has been used to monitor 1,3-butadiene ambient air concentrations in a residential area in proximity to a heavy-traffic roadway over a one-week period, for comparison with other traffic-related pollutants analysed by standard procedures. It has also been used to determine tailpipe emissions of two vehicles by standard emission testing procedures in a dynamometer. These vehicles were chosen as examples of low- and high-end emission rate vehicles, i.e., an old no-catalytic converter Otto engine and a new direct-injection diesel engine with catalytic converter. Exhaust gas emissions were 0.052 and 35.85 mg/km, reflecting differences in fuel, engine design, age, and presence (or not) of a catalytic abatement system. The ambient air results showed a weekly average concentration of 1,3-butadiene of 0.53 microg/m(3).

  17. Biofilm Formation Derived from Ambient Air and the Characteristics of Apparatus

    Science.gov (United States)

    Kanematsu, H.; Kougo, H.; Kuroda, D.; Itho, H.; Ogino, Y.; Yamamoto, Y.

    2013-04-01

    Biofilm is a kind of thin film on solidified matters, being derived from bacteria. Generally, planktonic bacteria float in aqueous environments, soil or air, most of which can be regarded as oligotrophic environments. Since they have to survive by instinct, they seek for nutrients that would exist on materials surfaces as organic matters. Therefore, bacteria attach materials surfaces reversibly. The attachment and detachment repeat for a while and finally, they attach on them irreversibly and the number of bacteria on them increases. At a threshold number, bacteria produce polymeric matters at the same time by quorum sensing mechanism and the biofilm produces on material surfaces. The biofilm produced in that way generally contains water (more than 80%), EPS (Exopolymeric Substance) and bacteria themselves. And they might bring about many industrial problems, fouling, corrosion etc. Therefore, it is very important for us to control and prevent the biofilm formation properly. However, it is generally very hard to produce biofilm experimentally and constantly in ambient atmosphere on labo scale. The authors invented an apparatus where biofilm could form on specimen's surfaces from house germs in the ambient air. In this experiment, we investigated the basic characteristics of the apparatus, reproducibility, the change of biofilm with experimental time, the quality change of water for biofilm formation and their significance for biofilm research.

  18. Risk of leukemia in relation to exposure to ambient air toxics in pregnancy and early childhood.

    Science.gov (United States)

    Heck, Julia E; Park, Andrew S; Qiu, Jiaheng; Cockburn, Myles; Ritz, Beate

    2014-07-01

    There are few established causes of leukemia, the most common type of cancer in children. Studies in adults suggest a role for specific environmental agents, but little is known about any effect from exposures in pregnancy to toxics in ambient air. In our case-control study, we ascertained 69 cases of acute lymphoblastic leukemia (ALL) and 46 cases of acute myeloid leukemia (AML) from California Cancer Registry records of children leukemia associated with one interquartile range increase in air toxic exposure. Risk of ALL was elevated with 3(rd) trimester exposure to polycyclic aromatic hydrocarbons (OR=1.16, 95% CI 1.04, 1.29), arsenic (OR=1.33, 95% CI 1.02, 1.73), benzene (OR=1.50, 95% CI 1.08, 2.09), and three other toxics related to fuel combustion. Risk of AML was increased with 3rd trimester exposure to chloroform (OR=1.30, 95% CI 1.00, 1.69), benzene (1.75, 95% CI 1.04, 2.93), and two other traffic-related toxics. During the child's first year, exposure to butadiene, ortho-xylene, and toluene increased risk for AML and exposure to selenium increased risk for ALL. Benzene is an established cause of leukemia in adults; this study supports that ambient exposures to this and other chemicals in pregnancy and early life may also increase leukemia risk in children.

  19. Quantitative and enantioselective analysis of monoterpenes from plant chambers and in ambient air using SPME

    Directory of Open Access Journals (Sweden)

    N. Yassaa

    2010-08-01

    Full Text Available A solid-phase microextraction (HS-SPME and gas chromatography/mass spectrometry (GC/MS system has been developed for quantifying enantiomeric and nonenantiomeric monoterpenes in plant chamber studies and ambient air. Performance of this system was checked using a capillary diffusion system to produce monoterpene standards. The adsorption efficiency, competitive adsorption and chromatographic peak resolution of monoterpene enantiomer pairs were compared for three SPME fibre coatings: 75 μm Carboxen-PDMS (CAR-PDMS, 50/30 μm, divinylbenzene-carboxen-polydimethylsiloxane (DVB-CAR-PDMS and 65 μm divinylbenzene-polydimethyl-siloxane (DVB-PDMS. Key parameters such as the linearity and reproducibility of the SPME system have been investigated in this work. The best compromise between the enantiomeric separation of monoterpenes and competitive adsorption of the isoprenoids on the solid SPME fibre coating was found for DVB-PDMS fibres. The optimum conditions using DVB-PDMS fibres were applied to measure the exchange rates of monoterpenes in the emission of Quercus ilex using a laboratory whole plant enclosure under light and dark conditions, as well as in ambient air. With 592 and 223 ng m−2 s−1, respectively, β-myrcene and limonene were the predominant monoterpenes in the emission of Q. ilex. These values were closely comparable to those obtained using a zNose and cartridge GC-FID systems.

  20. Assessment of reduced sulfur compounds in ambient air as malodor components in an urban area

    Science.gov (United States)

    Susaya, Janice; Kim, Ki-Hyun; Phan, Nhu-Thuc; Kim, Jo-Chun

    2011-07-01

    Long-term monitoring of reduced sulfur compounds (RSCs: hydrogen sulfide (H 2S), methanethiol (CH 3SH), dimethyl sulfide (DMS), and dimethyl disulfide (DMDS)) in ambient air was made using an on-line GC system at an odor monitoring station in the city of Ansan, South Korea (August 2005-December 2007). The results were examined to assess the status of RSC pollution, its relative contribution to malodor, and the controlling factors of its occurrence. H 2S (mean of 0.27 ppb) was eminent in terms of both magnitude and occurrence frequency, while others were not with mean values of 0.11 (DMDS), 0.10 (DMS), and 0.07 ppb (CH 3SH). Unlike others, the temporal trends of H 2S were best represented by the combined effects of its source processes and meteorological conditions. The results of correlation analysis indicate strong correlations between RSCs and water-related parameters (e.g., rainfall, dew point, and relative humidity). The role of RSCs as malodor component appears to be pronounced during nighttime, especially in summer. If the relative contribution of RSCs to malodor is assessed by means of the sum of odor intensity (SOI), its impact is relatively low, with an SOI value of 1.22 (weak odor strength). Consequently, a more deliberate approach may be needed to effectively assess odor occurrence patterns in ambient air.

  1. Quantitative and enantioselective analysis of monoterpenes from plant chambers and in ambient air using SPME

    Directory of Open Access Journals (Sweden)

    N. Yassaa

    2010-11-01

    Full Text Available A headspace solid-phase microextraction (HS-SPME and gas chromatography/mass spectrometry (GC/MS system has been developed for quantifying enantiomeric and nonenantiomeric monoterpenes in plant chamber studies and ambient air. Performance of this system was checked using a capillary diffusion system to produce monoterpene standards. The adsorption efficiency, competitive adsorption and chromatographic peak resolution of monoterpene enantiomer pairs were compared for three SPME fibre coatings: 75 μm Carboxen-PDMS (CAR-PDMS, 50/30 μm divinylbenzene-carboxen-polydimethylsiloxane (DVB-CAR-PDMS and 65 μm divinylbenzene-polydimethylsiloxane (DVB-PDMS. Key parameters such as the linearity and reproducibility of the SPME system have been investigated in this work. The best compromise between the enantiomeric separation of monoterpenes and competitive adsorption of the isoprenoids on the solid SPME fibre coating was found for DVB-PDMS fibres. The optimum conditions using DVB-PDMS fibres were applied to measure the exchange rates of monoterpenes in the emission of Quercus ilex using a laboratory whole plant enclosure under light and dark conditions, as well as in ambient air. With 592 and 223 ng m−2 s−1 respectively, β-myrcene and limonene were the predominant monoterpenes in the emission of Q. ilex. These values were closely comparable to those obtained using a zNose and cartridge GC-FID systems.

  2. Proceedings of the clean air and climate change summit

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    2010-07-01

    The Clean Air Partnership was established in the Greater Toronto Area (GTA) over 10 years ago to work on issues related to air pollution and climate change. This summit presented details of the partnership's municipal activities and provided an outline of various projects conducted to reduce air pollution, increase the use of green energy, and encourage residents to reduce their ecological footprint. Climate change was discussed in relation to the recent economic crisis and recently discovered problems related to ocean acidification. The International Energy Agency (IEA) annual report was discussed in relation to peak oil and future economic crises. Advancements in green energy policy in Ontario were outlined. Sustainable housing and renewable energy projects in Germany were presented along with successful urban designs in Melbourne, New York City, and Denver. The GTA-CAC inter-governmental declaration on clean air was discussed, and an interim progress report was presented. The summit concluded with a video presentation of a collaborative artistic piece about climate change and the Arctic. 11 figs.

  3. Application of DALYs in Measuring Health Effect of Ambient Air Pollution: A Case Study in Shanghai, China

    Institute of Scientific and Technical Information of China (English)

    YUN-HUI ZHANG; CHANG-HONG CHEN; GUO-HAI CHEN; GUI-XIANG SONG; BING-HENG CHEN; QING-YAN FU; HAI-DONG KAN

    2006-01-01

    To investigate the effect of ambient air pollution on human health and the subsequent disability-adjusted life years (DALYs) lost in Shanghai. Methods We used epidemiology-based exposure-response functions to calculate the attributable number of cases due to air pollution in Shanghai in 2000, and then we estimated the corresponding DALYs lost in Shanghai based on unit DALYs values of the health consequences. Results Ambient air pollution caused 103 064 DALYs lost in Shanghai in 2000. Among all the health endpoints, premature deaths and chronic bronchitis predominated in the value of total DALYs lost. Conclusion The air pollution levels have an adverse effect on the general population health and strengthen the rationale for limiting the levels of air pollution in outdoor air in Shanghai.

  4. The cardiopulmonary effects of ambient air pollution and mechanistic pathways: a comparative hierarchical pathway analysis.

    Directory of Open Access Journals (Sweden)

    Ananya Roy

    Full Text Available Previous studies have investigated the associations between exposure to ambient air pollution and biomarkers of physiological pathways, yet little has been done on the comparison across biomarkers of different pathways to establish the temporal pattern of biological response. In the current study, we aim to compare the relative temporal patterns in responses of candidate pathways to different pollutants. Four biomarkers of pulmonary inflammation and oxidative stress, five biomarkers of systemic inflammation and oxidative stress, ten parameters of autonomic function, and three biomarkers of hemostasis were repeatedly measured in 125 young adults, along with daily concentrations of ambient CO, PM2.5, NO2, SO2, EC, OC, and sulfate, before, during, and after the Beijing Olympics. We used a two-stage modeling approach, including Stage I models to estimate the association between each biomarker and pollutant over each of 7 lags, and Stage II mixed-effect models to describe temporal patterns in the associations when grouping the biomarkers into the four physiological pathways. Our results show that candidate pathway groupings of biomarkers explained a significant amount of variation in the associations for each pollutant, and the temporal patterns of the biomarker-pollutant-lag associations varied across candidate pathways (p<0.0001 and were not linear (from lag 0 to lag 3: p = 0.0629, from lag 3 to lag 6: p = 0.0005. These findings suggest that, among this healthy young adult population, the pulmonary inflammation and oxidative stress pathway is the first to respond to ambient air pollution exposure (within 24 hours and the hemostasis pathway responds gradually over a 2-3 day period. The initial pulmonary response may contribute to the more gradual systemic changes that likely ultimately involve the cardiovascular system.

  5. Study of Ambient and Indoor Air Quality in the Building Built on the Former Landfill

    Directory of Open Access Journals (Sweden)

    Anuar Ithnin

    2012-01-01

    Full Text Available Problem statement: The air quality study of PPR Taman Wahyu II, Selayang, Selangor was a residential project that was built on the former landfill site. The landfill site will produce landfill gases which can influence the air quality level in and outside the building. Approach: This air quality study also involving PPR Intan Baiduri, Batu Caves, Selangor as a control building. The air quality parameters chosen were physical, chemical and biological. Instruments used were HVS, Biogas Analyzer, Aeroqual, MultiRAE, ICP-MS, NMAM 7303 and gravimetric method. Gilian High Volume Air Sampler was used to measure heavy metal parameters that were conducted for 8 h, Personal Sampling Pump to measure total suspended particulates for 8 h, MultiRAE for H2S and CH4 gas, Aeroqual for CO2 gas, Multilog for CO gas and a Tedlar bag for O2 gas. For biological parameters, settle plate method was used and conducted for 20 min. Veloci CALC and wind probe were used to measure physical parameters. Results: In the ambient air, the mean concentration of Total Suspended Particulate (TSP, lead and cadmium were higher at an exposed location compared to the control with a reading of 0.325±0.29, 0.108±0.050 and 0.06±0.045 ng m-3 respectively. The reason was that the exposed location was a former landfill site and there were several co-founding factors. Mean concentration for chemical parameters were higher at the exposed location and all the chemical parameters were not exceeding the EPA Protocol Gas for Single Component. The mean concentration of oxygen is 20.95±0.005%, carbon dioxide 669.25±84.109 ppm and carbon monoxide 1.8±0.957 ppm. For biological parameters, mean for the colony total count also higher at the exposed location compared to control location where the mean for bacterial was 17.75±4.573cfu while for fungal, the mean is 8.0±2.828 cfu. Indoor air quality results showed that concentration means of CO2 was 877.8±59.40 ppm, CO was 5.0

  6. A Review of Epidemiological Research on Adverse Neurological Effects of Exposure to Ambient Air Pollution.

    Science.gov (United States)

    Xu, Xiaohui; Ha, Sandie Uyen; Basnet, Rakshya

    2016-01-01

    There is a growing body of epidemiological research reporting the neurological effects of ambient air pollution. We examined current evidence, identified the strengths and weaknesses of published epidemiological studies, and suggest future directions for research in this area. Studies were identified through a systematic search of online scientific databases, in addition to a manual search of the reference lists from the identified papers. Despite being a relatively new area of investigation, overall, there is mounting evidence implicating adverse effects of air pollution on neurobehavioral function in both adults and children. Further research is needed to expand our understanding of these relationships, including improvement in the accuracy of exposure assessments; focusing on specific toxicants and their relationships to specific health endpoints, such as neurodevelopmental disorders and neurodegenerative diseases; investigating the combined neurological effects of multiple air pollutants; and further exploration of genetic susceptibility for neurotoxicity of air pollution. In order to achieve these goals collaborative efforts are needed from multidisciplinary teams, including experts in toxicology, biostatistics, geographical science, epidemiology, and neurology.

  7. Ambient air pollution, temperature and out-of-hospital coronary deaths in Shanghai, China.

    Science.gov (United States)

    Dai, Jinping; Chen, Renjie; Meng, Xia; Yang, Changyuan; Zhao, Zhuohui; Kan, Haidong

    2015-08-01

    Few studies have evaluated the effects of ambient air pollution and temperature in triggering out-of-hospital coronary deaths (OHCDs) in China. We evaluated the associations of air pollution and temperature with daily OHCDs in Shanghai, China from 2006 to 2011. We applied an over-dispersed generalized additive model and a distributed lag nonlinear model to analyze the effects of air pollution and temperature, respectively. A 10 μg/m(3) increase in the present-day PM10, PM2.5, SO2, NO2 and CO were associated with increases in OHCD mortality of 0.49%, 0.68%, 0.88%, 1.60% and 0.08%, respectively. A 1 °C decrease below the minimum-mortality temperature corresponded to a 3.81% increase in OHCD mortality on lags days 0-21, and a 1 °C increase above minimum-mortality temperature corresponded to a 4.61% increase over lag days 0-3. No effects were found for in-hospital coronary deaths. This analysis suggests that air pollution, low temperature and high temperature may increase the risk of OHCDs.

  8. Health Impacts of Air Pollution Under a Changing Climate

    Science.gov (United States)

    Kinney, P. L.; Knowlton, K.; Rosenthal, J.; Hogrefe, C.; Rosenzweig, C.; Solecki, W.

    2003-12-01

    Outdoor air pollution remains a serious public health problem in cities throughout the world. In the US, despite considerable progress in reducing emissions over the past 30 years, as many as 50,000 premature deaths each year have been attributed to airborne particulate matter alone. Tropospheric ozone has been associated with increased daily mortality and hospitalization rates, and with a variety of related respiratory problems. Weather plays an important role in the transport and transformation of air pollution. In particular, a warming climate is likely to promote the atmospheric reactions that are responsible for ozone and secondary aerosol production, as well as increasing emissions of many of their volatile precursors. Increasingly, efforts to address urban air pollution problems throughout the world will be complicated by trends and variability in climate. The New York Climate and Health Project (NYCHP) is developing and applying tools for integrated assessment of health impacts from air pollution and heat associated with climate and land-use changes in the New York City metropolitan region. Global climate change is modeled over the 21st century based on the Intergovernmental Panel on Climate Change (IPCC) A2 greenhouse gas emissions scenario using the Goddard Institute for Space Studies (GISS) Global Atmosphere-Ocean Model (GCM). Meteorological fields are downscaled to a 36 km grid over the eastern US using the Penn State/NCAR MM5 mesoscale meteorological model. MM5 results are then used as input to the Community Multiscale Air Quality (CMAQ) model for simulating air quality, with emissions based on the Sparse Matrix Operator Kernel Emissions Modeling System (SMOKE). To date, simulations have been performed for five summer seasons each during the 1990s and the 2050s. An evaluation of the present-day climate and air quality predictions indicates that the modeling system largely captures the observed climate-ozone system. Analysis of future-year predictions

  9. 40 CFR Appendix T to Part 50 - Interpretation of the Primary National Ambient Air Quality Standards for Oxides of Sulfur (Sulfur...

    Science.gov (United States)

    2010-07-01

    ... Ambient Air Quality Standards for Oxides of Sulfur (Sulfur Dioxide) T Appendix T to Part 50 Protection of... AIR QUALITY STANDARDS Pt. 50, App. T Appendix T to Part 50—Interpretation of the Primary National Ambient Air Quality Standards for Oxides of Sulfur (Sulfur Dioxide) 1. General (a) This appendix...

  10. 40 CFR Appendix H to Part 50 - Interpretation of the 1-Hour Primary and Secondary National Ambient Air Quality Standards for Ozone

    Science.gov (United States)

    2010-07-01

    ... and Secondary National Ambient Air Quality Standards for Ozone H Appendix H to Part 50 Protection of... AIR QUALITY STANDARDS Pt. 50, App. H Appendix H to Part 50—Interpretation of the 1-Hour Primary and Secondary National Ambient Air Quality Standards for Ozone 1. General This appendix explains how...

  11. The deployment of carbon monoxide wireless sensor network (CO-WSN) for ambient air monitoring.

    Science.gov (United States)

    Chaiwatpongsakorn, Chaichana; Lu, Mingming; Keener, Tim C; Khang, Soon-Jai

    2014-06-16

    Wireless sensor networks are becoming increasingly important as an alternative solution for environment monitoring because they can reduce cost and complexity. Also, they can improve reliability and data availability in places where traditional monitoring methods are difficult to site. In this study, a carbon monoxide wireless sensor network (CO-WSN) was developed to measure carbon monoxide concentrations at a major traffic intersection near the University of Cincinnati main campus. The system has been deployed over two weeks during Fall 2010, and Summer 2011-2012, traffic data was also recorded by using a manual traffic counter and a video camcorder to characterize vehicles at the intersection 24 h, particularly, during the morning and evening peak hour periods. According to the field test results, the 1 hr-average CO concentrations were found to range from 0.1-1.0 ppm which is lower than the National Ambient Air Quality Standards (NAAQS) 35 ppm on a one-hour averaging period. During rush hour periods, the traffic volume at the intersection varied from 2,067 to 3,076 vehicles per hour with 97% being passenger vehicles. Furthermore, the traffic volume based on a 1-h average showed good correlation (R2 = 0.87) with the 1-h average CO-WSN concentrations for morning and evening peak time periods whereas CO-WSN results provided a moderate correlation (R2 = 0.42) with 24 hours traffic volume due to fluctuated changes of meteorological conditions. It is concluded that the performance and the reliability of wireless ambient air monitoring networks can be used as an alternative method for real time air monitoring.

  12. Oxidative potential and inflammatory impacts of source apportioned ambient air pollution in Beijing.

    Science.gov (United States)

    Liu, Qingyang; Baumgartner, Jill; Zhang, Yuanxun; Liu, Yanju; Sun, Yongjun; Zhang, Meigen

    2014-11-01

    Air pollution exposure is associated with a range of adverse health impacts. Knowledge of the chemical components and sources of air pollution most responsible for these health effects could lead to an improved understanding of the mechanisms of such effects and more targeted risk reduction strategies. We measured daily ambient fine particulate matter (Beijing, and assessed the contribution of its chemical components to the oxidative potential of ambient air pollution using the dithiothreitol (DTT) assay. The composition data were applied to a multivariate source apportionment model to determine the PM contributions of six sources or factors: a zinc factor, an aluminum factor, a lead point factor, a secondary source (e.g., SO4(2-), NO3(2-)), an iron source, and a soil dust source. Finally, we assessed the relationship between reactive oxygen species (ROS) activity-related PM sources and inflammatory responses in human bronchial epithelial cells. In peri-urban Beijing, the soil dust source accounted for the largest fraction (47%) of measured ROS variability. In central Beijing, a secondary source explained the greatest fraction (29%) of measured ROS variability. The ROS activities of PM collected in central Beijing were exponentially associated with in vivo inflammatory responses in epithelial cells (R2=0.65-0.89). We also observed a high correlation between three ROS-related PM sources (a lead point factor, a zinc factor, and a secondary source) and expression of an inflammatory marker (r=0.45-0.80). Our results suggest large differences in the contribution of different PM sources to ROS variability at the central versus peri-urban study sites in Beijing and that secondary sources may play an important role in PM2.5-related oxidative potential and inflammatory health impacts.

  13. Alternative Refrigerant Evaluation for High-Ambient-Temperature Environments: R-22 and R-410A Alternatives for Rooftop Air Conditioners

    Energy Technology Data Exchange (ETDEWEB)

    Abdelaziz, Omar [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Shrestha, Som S. [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Shen, Bo [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Linkous, Randall Lee [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Goetzler, William [Navigant Consulting Inc., Burlington, MA (United States); Guernsey, Matt [Navigant Consulting Inc., Burlington, MA (United States); Bargach, Youssef [Navigant Consulting Inc., Burlington, MA (United States)

    2016-09-01

    The Oak Ridge National Laboratory (ORNL) High-Ambient-Temperature Evaluation Program for Low-Global Warming Potential (Low-GWP) Refrigerants aims to develop an understanding of the performance of low-GWP alternative refrigerants relative to hydrochlorofluorocarbon (HCFC) and hydrofluorocarbon (HFC) refrigerants in packaged or Rooftop Unit (RTU) air conditioners under high-ambient-temperature conditions. This final report describes the parties involved, the alternative refrigerants selection process, the test procedures, and the final results.

  14. Monofractal nature of air temperature signals reveals their climate variability

    OpenAIRE

    Deliège, Adrien; Nicolay, Samuel

    2014-01-01

    We use the discrete "wavelet transform microscope" to show that the surface air temperature signals of weather stations selected in Europe are monofractal. This study reveals that the information obtained in this way are richer than previous works studying long range correlations in meteorological stations. The approach presented here allows to bind the H\\"older exponents with the climate variability. We also establish that such a link does not exist with methods previously carried out.

  15. Potential impact of a US climate policy and air quality regulations on future air quality and climate change

    Science.gov (United States)

    Lee, Yunha; Shindell, Drew T.; Faluvegi, Greg; Pinder, Rob W.

    2016-04-01

    We have investigated how future air quality and climate change are influenced by the US air quality regulations that existed or were proposed in 2013 and a hypothetical climate mitigation policy that aims to reduce 2050 CO2 emissions to be 50 % below 2005 emissions. Using the NASA GISS ModelE2 general circulation model, we look at the impacts for year 2030 and 2055. The US energy-sector emissions are from the GLIMPSE project (GEOS-Chem LIDORT Integrated with MARKAL (MARKet ALlocation) for the Purpose of Scenario Exploration), and other US emissions data sets and the rest of the world emissions data sets are based on the RCP4.5 scenario. The US air quality regulations are projected to have a strong beneficial impact on US air quality and public health in year 2030 and 2055 but result in positive radiative forcing. Under this scenario, no more emission constraints are added after 2020, and the impacts on air quality and climate change are similar between year 2030 and 2055. Surface particulate matter with a diameter smaller than 2.5 µm (PM2.5) is reduced by ˜ 2 µg m-3 on average over the USA, and surface ozone by ˜ 8 ppbv. The improved air quality prevents about 91 400 premature deaths in the USA, mainly due to the PM2.5 reduction (˜ 74 200 lives saved). The air quality regulations reduce the light-reflecting aerosols (i.e., sulfate and organic matter) more than the light-absorbing species (i.e., black carbon and ozone), leading to a strong positive radiative forcing (RF) over the USA by both aerosols' direct and indirect forcing: the total RF is ˜ 0.04 W m-2 over the globe, and ˜ 0.8 W m-2 over the USA. Under the hypothetical climate policy, a future CO2 emissions cut is achieved in part by relying less on coal, and thus SO2 emissions are noticeably reduced. This provides air quality co-benefits, but it could lead to potential climate disbenefits over the USA. In 2055, the US mean total RF is +0.22 W m-2 due to positive aerosol direct and indirect forcing

  16. Potential Impact of a US Climate Policy and Air Quality Regulations on Future Air Quality and Climate Change

    Science.gov (United States)

    Lee, Y. H.; Faluvegi, Gregory S.

    2016-01-01

    We have investigated how future air quality and climate change are influenced by the US air quality regulations that existed or were proposed in 2013 and a hypothetical climate mitigation policy that aims to reduce 2050 CO2 emissions to be 50% below 2005 emissions. Using the NASA GISS ModelE2 general circulation model, we look at the impacts for year 2030 and 2055. The US energy-sector emissions are from the GLIMPSE project (GEOS-Chem LIDORT Integrated with MARKAL (MARKet ALlocation) for the Purpose of Scenario Exploration), and other US emissions data sets and the rest of the world emissions data sets are based on the RCP4.5 scenario. The US air quality regulations are projected to have a strong beneficial impact on US air quality and public health in year 2030 and 2055 but result in positive radiative forcing. Under this scenario, no more emission constraints are added after 2020, and the impacts on air quality and climate change are similar between year 2030 and 2055. Surface particulate matter with a diameter smaller than 2.5 micron PM(sub 2:5) is reduced by 2 approximately µg/m(sup -3) on average over the USA, and surface ozone by approximately 8 ppbv. The improved air quality prevents about 91 400 premature deaths in the USA, mainly due to the PM(sub 2:5) reduction approximately (74 200 lives saved). The air quality regulations reduce the light-reflecting aerosols (i.e., sulfate and organic matter) more than the light-absorbing species (i.e., black carbon and ozone), leading to a strong positive radiative forcing (RF) over the USA by both aerosols' direct and indirect forcing: the total RF is approximately 0.04 W m(sup -2) over the globe, and approximately 0.8 W m(sup -2) over the USA. Under the hypothetical climate policy, a future CO2 emissions cut is achieved in part by relying less on coal, and thus SO2 emissions are noticeably reduced. This provides air quality co-benefits, but it could lead to potential climate disbenefits over the USA. In 2055, the US

  17. An evaluation of public health impact of ambient air pollution under various energy scenarios in Shanghai, China

    Energy Technology Data Exchange (ETDEWEB)

    Haidong Kan; Bingheng Chen [Fudan Univ., Dept. of Environmental Health, Shanghai (China); Changhong Chen; Qingyan Fu; Minghua Chen [Shanghai Academy of Environmental Sciences, Shanghai (China)

    2004-01-01

    To investigate the potential public health impact of ambient air pollution under various energy scenarios in Shanghai, we estimated the air pollution exposure level of the general population under various planned energy scenarios, and assessed the potential public health impact using the concentration-response functions derived from available epidemiologic studies. The results show that ambient air pollution in relation to various energy scenarios could have significant impact on the health status of Shanghai residents. Compared with base case scenario, implementation of various energy scenarios could prevent 608-5144 and 1189-10,462 PM{sub 10}-related avoidable deaths (mid-value) in 2010 and 2020, respectively; and it could also decrease substantial cases of relevant diseases. These findings illustrate that an effective energy and environmental policy will play an active role in reduction of air pollutant emissions, improvement of air quality, and public health. (Author)

  18. The effect of ambient air pollution on respiratory health of school children: a panel study

    Directory of Open Access Journals (Sweden)

    McLeod Susan

    2008-05-01

    Full Text Available Abstract Background Adverse respiratory effects of particulate air pollution have been identified by epidemiological studies. We aimed to examine the health effects of ambient particulate air pollution from wood burning on school-age students in Christchurch, New Zealand, and to explore the utility of urine and exhaled breath condensate biomarkers of exposure in this population. Methods A panel study of 93 male students (26 with asthma living in the boarding house of a metropolitan school was undertaken in the winter of 2004. Indoor and outdoor pollution data was continuously monitored. Longitudinal assessment of lung function (FEV1 and peak flow and symptoms were undertaken, with event studies of high pollution on biomarkers of exposure (urinary 1-hydroxypyrene and effect (exhaled breath condensate (EBC pH and hydrogen peroxide concentration. Results Peak levels of air pollution were associated with small but statistically significant effects on lung function in the asthmatic students, but not healthy students. No significant effect of pollution could be seen either on airway inflammation and oxidative stress either in healthy students or students with asthma. Minor increases in respiratory symptoms were associated with high pollution exposure. Urinary 1-hydroxypyrene levels were raised in association with pollution events by comparison with low pollution control days. Conclusion There is no significant effect of ambient wood-smoke particulate air pollution on lung function of healthy school-aged students, but a small effect on respiratory symptoms. Asthmatic students show small effects of peak pollution levels on lung function. Urinary 1-hydroxypyrene shows potential as a biomarker of exposure to wood smoke in this population; however measurement of EBC pH and hydrogen peroxide appears not to be useful for assessment of population health effects of air pollution. Some of the data presented in this paper has previously been published in Kingham

  19. Polyfluorinated compounds in ambient air from ship- and land-based measurements in northern Germany

    Science.gov (United States)

    Dreyer, Annekatrin; Ebinghaus, Ralf

    Neutral volatile and semi-volatile polyfluorinated organic compounds (PFC) and ionic perfluorinated compounds were determined in air samples collected at two sites in the vicinity of Hamburg, Germany, and onboard the German research vessel Atair during a cruise in the German Bight, North Sea, in early November 2007. PUF/XAD-2/PUF cartridges and glass fiber filters as sampling media were applied to collect several fluorotelomer alcohols (FTOH), fluorotelomer acrylates (FTA), perfluoroalkyl sulfonamides (FASA), and perfluoroalkyl sulfonamido ethanols (FASE) in the gas- and particle-phase as well as a set of perfluorinated carboxylates (PFCA) and sulfonates (PFSA) in the particle-phase. This study presents the distribution of PFC in ambient air of the German North Sea and in the vicinity of Hamburg for the first time. Average total PFC concentrations in and around Hamburg (180 pg m -3) were higher than those observed in the German Bight (80 pg m -3). In the German Bight, minimum-maximum gas-phase concentrations of 17-82 pg m -3 for ΣFTOH, 2.6-10 pg m -3 for ΣFTA, 10-15 pg m -3 for ΣFASA, and 2-4.4 pg m -3 for ΣFASE were determined. In the vicinity of Hamburg, minimum-maximum gas-phase concentrations of 32-204 pg m -3 for ΣFTOH, 3-26 pg m -3 for ΣFTA, 3-18 pg m -3 for ΣFASA, and 2-15 pg m -3 for ΣFASE were detected. Concentrations of perfluorinated acids were in the range of 1-11 pg m -3. FTOH clearly dominated the substance spectrum; 8:2 FTOH occurred in maximum proportions. Air mass back trajectories, cluster, and correlation analyses revealed that the air mass origin and thus medium to long range atmospheric transport was the governing parameter for the amount of PFC in ambient air. Southwesterly located source regions seemed to be responsible for elevated PFC concentrations, local sources appeared to be of minor importance.

  20. Landfills as sources of polyfluorinated compounds, polybrominated diphenyl ethers and musk fragrances to ambient air

    Science.gov (United States)

    Weinberg, Ingo; Dreyer, Annekatrin; Ebinghaus, Ralf

    2011-02-01

    In order to investigate landfills as sources of polyfluorinated compounds (PFCs), polybrominated diphenyl ethers (PBDEs) and synthetic musk fragrances to the atmosphere, air samples were simultaneously taken at two landfills (one active and one closed) and two reference sites using high volume air samplers. Contaminants were accumulated on glass fiber filters (particle phase) and PUF/XAD-2/PUF cartridges (gas phase), extracted by methyl-tert butyl ether/acetone (neutral PFCs), methanol (ionic PFCs) or hexane/acetone (PBDEs, musk fragrances), and detected by GC-MS (neutral PFCs, PBDEs, musk fragrances) or HPLC-MS/MS (ionic PFCs). Total concentrations ranged from 84 to 706 pg m -3 (volatile PFCs, gas phase), from ambient air.

  1. Ambient air sampling for radioactive air contaminants at Los Alamos National Laboratory: A large research and development facility

    Energy Technology Data Exchange (ETDEWEB)

    Eberhart, C.F.

    1998-09-01

    This paper describes the ambient air sampling program for collection, analysis, and reporting of radioactive air contaminants in and around Los Alamos National Laboratory (LANL). Particulate matter and water vapor are sampled continuously at more than 50 sites. These samples are collected every two weeks and then analyzed for tritium, and gross alpha, gross beta, and gamma ray radiation. The alpha, beta, and gamma measurements are used to detect unexpected radionuclide releases. Quarterly composites are analyzed for isotopes of uranium ({sup 234}U, {sup 235}U, {sup 238}U), plutonium ({sup 238}Pu, {sup 239/249}Pu), and americium ({sup 241}Am). All of the data is stored in a relational database with hard copies as the official records. Data used to determine environmental concentrations are validated and verified before being used in any calculations. This evaluation demonstrates that the sampling and analysis process can detect tritium, uranium, plutonium, and americium at levels much less than one percent of the public dose limit of 10 millirems. The isotopic results also indicate that, except for tritium, off-site concentrations of radionuclides potentially released from LANL are similar to typical background measurements.

  2. Ambient Air Pollution and Cardiovascular Malformations in Atlanta, Georgia, 1986–2003

    Science.gov (United States)

    Klein, Mitchel; Correa, Adolfo; Reller, Mark D.; Mahle, William T.; Riehle-Colarusso, Tiffany J.; Botto, Lorenzo D.; Flanders, W. Dana; Mulholland, James A.; Siffel, Csaba; Marcus, Michele; Tolbert, Paige E.

    2009-01-01

    Associations between ambient air pollution levels during weeks 3–7 of pregnancy and risks of cardiovascular malformations were investigated among the cohort of pregnancies reaching at least 20 weeks’ gestation that were conceived during January 1, 1986–March 12, 2003, in Atlanta, Georgia. Surveillance records obtained from the Metropolitan Atlanta Congenital Defects Program, which conducts active, population-based surveillance on this cohort, were reviewed to classify cardiovascular malformations. Ambient 8-hour maximum ozone and 24-hour average carbon monoxide, nitrogen dioxide, particulate matter with an average aerodynamic diameter of <10 μm (PM10), and sulfur dioxide measurements were obtained from centrally located stationary monitors. Temporal associations between these pollutants and daily risks of secundum atrial septal defect, aortic coarctation, hypoplastic left heart syndrome, patent ductus arteriosus, valvar pulmonary stenosis, tetralogy of Fallot, transposition of the great arteries, muscular ventricular septal defect, perimembranous ventricular septal defect, conotruncal defects, left ventricular outflow tract defect, and right ventricular outflow defect were modeled by using Poisson generalized linear models. A statistically significant association was observed between PM10 and patent ductus arteriosus (for an interquartile range increase in PM10 levels, risk ratio = 1.60, 95% confidence interval: 1.11, 2.31). Of the 60 associations examined in the primary analysis, no other significant associations were observed. PMID:19258486

  3. Detection of Coxiella burnetii in Ambient Air after a Large Q Fever Outbreak.

    Directory of Open Access Journals (Sweden)

    Myrna M T de Rooij

    Full Text Available One of the largest Q fever outbreaks ever occurred in the Netherlands from 2007-2010, with 25 fatalities among 4,026 notified cases. Airborne dispersion of Coxiella burnetii was suspected but not studied extensively at the time. We investigated temporal and spatial variation of Coxiella burnetii in ambient air at residential locations in the most affected area in the Netherlands (the South-East, in the year immediately following the outbreak. One-week average ambient particulate matter < 10 μm samples were collected at eight locations from March till September 2011. Presence of Coxiella burnetii DNA was determined by quantitative polymerase chain reaction. Associations with various spatial and temporal characteristics were analyzed by mixed logistic regression. Coxiella burnetii DNA was detected in 56 out of 202 samples (28%. Airborne Coxiella burnetii presence showed a clear seasonal pattern coinciding with goat kidding. The spatial variation was significantly associated with number of goats on the nearest goat farm weighted by the distance to the farm (OR per IQR: 1.89, CI: 1.31-2.76. We conclude that in the year after a large Q fever outbreak, temporal variation of airborne Coxiella burnetii is suggestive to be associated with goat kidding, and spatial variation with distance to and size of goat farms. Aerosol measurements show to have potential for source identification and attribution of an airborne pathogen, which may also be applicable in early stages of an outbreak.

  4. Phytotoxic risk assessment of ambient air pollution on agricultural crops in Selangor State, Malaysia.

    Science.gov (United States)

    Ishii, S; Bell, J N B; Marshall, F M

    2007-11-01

    The phytotoxic risk of ambient air pollution to local vegetation was assessed in Selangor State, Malaysia. The AOT40 value was calculated by means of the continuously monitored daily maximum concentration and the local diurnal pattern of O3. Together with minor risks associated with the levels of NO2 and SO2, the study found that the monthly AOT40 values in these peri-urban sites were consistently over 1.0 ppm.h, which is well in exceedance of the given European critical level. Linking the O3 level to actual agricultural crop production in Selangor State also indicated that the extent of yield losses could have ranged from 1.6 to 5.0% (by weight) in 2000. Despite a number of uncertainties, the study showed a simple but useful methodological framework for phytotoxic risk assessment with a limited data set, which could contribute to appropriate policy discussion and countermeasures in countries under similar conditions.

  5. Pollution characteristic of VOCs of ambient air in winter and spring in Shijiazhuang City

    Directory of Open Access Journals (Sweden)

    Qing CHANG

    2015-06-01

    Full Text Available In order to further explore the pollution characteristics of volatile organic compounds in ambient air in winter and spring in Shijiazhuang City, the pollution characteristics of 62 volatile organic compounds (VOCs, monthly and quarterly variation, the correlation between VOCs and PM2.5, and the main sources of VOCs are investigated by using EPA TO-15 method. It shows that 40 organic compounds of the 64 VOCs have been quantitatively determined in winter and spring in the city, which are mainly acetone, benzene, carbon tetrachloride, dichloromethane, toluene, ethyl acetate, etc.. In the no-quantitatively determined components, higher ethanol, butyl acetate, butane etc. are detected. The VOCs concentration has positive correlation with the PM2.5 concentration during haze days.

  6. Assessing the impact of the forthcoming decrease in diesel exhaust particulate matter emissions on air quality: implications for black carbon concentrations in ambient air

    Science.gov (United States)

    González, Y.; Rodríguez, S.; Cuevas, E.; Ramos, R.; Abreu-Afonso, J.; Baldasano, J. M.

    2009-04-01

    Forthcoming regulations (e.g. EURO 5 and EURO 6) are planned to reduce particulate matter emissions (PM) in the exhaust of forthcoming vehicles. In this study we assess the impact of such reduction in the diesel PM exhaust emissions on the urban ambient air PM concentrations. This has been done by studying the relationship between black carbon (BC) and carbon monoxide (CO) in urban ambient air and in the exhaust of current and forthcoming vehicles. The slope of the BC-vs-CO linear relationship is mainly affected by the percentage (%) of diesel automobiles in the urban vehicles fleet. This slope is a better indicator of the diesel PM emissions than bulk BC concentrations in urban ambient air. BC-vs-CO slopes within the range 1-3 and 7-14 ngBC/µgCO are typically observed in urban areas with low (fuel consumption for on road transportation, respectively. The entry into force of forthcoming regulations will decrease the BC-vs-CO slope in urban ambient air from about 10 to 5 ngBC/µgCO in the next decade, according to calculations based on the current data on diesel vehicles in urban fleets in Spanish cities. However, this will not necessary prompt a significant decrease in the urban BC concentrations if road traffic volume follows the increasing trend of the last decade. The results of this study shows that the analysis of the BC-vs-CO slope trend in ambient air is an useful tool for understanding the involvement "of the changes in the vehicle exhaust emissions rates" and "of the changes in the road traffic volume" in the BC and PMx trends in urban ambient air.

  7. Modification of the effect of ambient air pollution on pediatric asthma emergency visits: susceptible subpopulations

    Science.gov (United States)

    Strickland, Matthew J; Klein, Mitchel; Flanders, W Dana; Chang, Howard H; Mulholland, James A; Tolbert, Paige E; Darrow, Lyndsey A

    2016-01-01

    Background Children may have differing susceptibility to ambient air pollution concentrations depending on various background characteristics of the children. Methods Using emergency department (ED) data linked with birth records from Atlanta, Georgia, we identified ED visits for asthma or wheeze among children aged 2–16 years from 1 January 2002 through 30 June 2010 (n=109,758). We stratified by preterm delivery, term low birth weight, maternal race, Medicaid status, maternal education, maternal smoking, delivery method, and history of a bronchiolitis ED visit. Population-weighted daily average concentrations were calculated for 1-hour maximum carbon monoxide and nitrogen dioxide; 8-hour maximum ozone; and 24-hour average particulate matter less than 10 microns in diameter, particulate matter less than 2.5 microns in diameter (PM2.5), and the PM2.5 components sulfate, nitrate, ammonium, elemental carbon, and organic carbon, using measurements from stationary monitors. Poisson time-series models were used to estimate rate ratios for associations between three-day moving average pollutant concentrations and daily ED visit counts and to investigate effect-measure modification by the stratification factors. Results Associations between pollutant concentrations and asthma exacerbations were larger among children born preterm and among children born to African American mothers. Stratification by race and preterm status together suggested that both factors affected susceptibility. The largest estimated effect size (for an interquartile-range increase in pollution) was observed for ozone among preterm births to African American mothers: rate ratio=1.138 (95% confidence interval=1.077–1.203). In contrast, the rate ration for the ozone association among full-term births to mothers of other races was 1.025 (0.970–1.083). Conclusions Results support the hypothesis that children vary in their susceptibility to ambient air pollutants. PMID:25192402

  8. Ambient air quality and the frequency of physician visits by preschool children

    Directory of Open Access Journals (Sweden)

    Durmišević Smajil

    2007-01-01

    Full Text Available Introduction. Ambient air pollution in the town of Kakanj, mostly of industrial origin, has become a major reason for increased use of health care services by children under the age of six years. The aim of this study was to examine the correlation between ambient concentrations of sulphur dioxide (SO2, suspended particles and nitrogenoxides (NOx, and the frequency/number of visits to health care institutions by children under the age of six years. Material and methods. The investigation was carried out in the period from January to December 2003, in the area of Kakanj and Brnjic. We examined the average number of monthly visits to health care institutions and concentrations of sulphur dioxide, suspended particles and nitrogen oxides in the town of Kakanj. Results. The investigation shows that there is a linear increase of visits to health care institutions in relation to linear increase of concetrations of sulphur dioxide, suspended particles and nitrogen oxides (Oair. .

  9. Benzene toxicity of the occurrence of benzene in the ambient air of the Houston area

    Energy Technology Data Exchange (ETDEWEB)

    Lin, Y.C.

    1980-01-01

    This study was conducted by either literature review or actual field survey. Results are summarized as follows: (1) long-term occupational exposure of workers to benzene vapor at levels of 3 to 7 ppM, 2 to 3 ppM and 1.6 ppM may result in a decreased level of leucocyte alkaline phosphates, an increased incidence of chromosome aberrations and an increased level of ALA in erythrocytes, respectively; (2) benzene is capable of causing fetotoxic effects in animals at levels as low as 10 ppM by volume; (3) exposure of animals to or less than 1 ppM benzene vapor may result in leucopenia, an inverse ratio of muscle antagonist chronaxy and a decreased level of ascorbic acid in fetus's and mother's liver as well as whole embryo; (4) benzene is causally associated with the increased incidence of pancytopenia, including unicytopenia, bicytopenia and aplastic anemia, and chromosome aberrations in occupational exposure population, and at best benzene must also be considered as a leukemogen; (5) since it can be emitted into the atmosphere from both man-made and natural sources, benzene in some concentrations is presented everywhere in the various compartments of the environment; (6) the findings of the emission of benzene from certain natural sources indicate that reducing benzene to a zero-level of exposure is theoretically impossible; (7) the annual average of benzene concentration detected in the Houston ambient air is 2.50 ppB, which is about 2.4 times higher than the nation-wide annual average exposure level and may have some health implications to the general public; and (8) in the Houston area, stationary sources are more important than mobile sources in contributing to benzene in the ambient air.

  10. Aircraft engine exhaust emissions and other airport-related contributions to ambient air pollution: A review

    Science.gov (United States)

    Masiol, Mauro; Harrison, Roy M.

    2014-10-01

    Civil aviation is fast-growing (about +5% every year), mainly driven by the developing economies and globalisation. Its impact on the environment is heavily debated, particularly in relation to climate forcing attributed to emissions at cruising altitudes and the noise and the deterioration of air quality at ground-level due to airport operations. This latter environmental issue is of particular interest to the scientific community and policymakers, especially in relation to the breach of limit and target values for many air pollutants, mainly nitrogen oxides and particulate matter, near the busiest airports and the resulting consequences for public health. Despite the increased attention given to aircraft emissions at ground-level and air pollution in the vicinity of airports, many research gaps remain. Sources relevant to air quality include not only engine exhaust and non-exhaust emissions from aircraft, but also emissions from the units providing power to the aircraft on the ground, the traffic due to the airport ground service, maintenance work, heating facilities, fugitive vapours from refuelling operations, kitchens and restaurants for passengers and operators, intermodal transportation systems, and road traffic for transporting people and goods in and out to the airport. Many of these sources have received inadequate attention, despite their high potential for impact on air quality. This review aims to summarise the state-of-the-art research on aircraft and airport emissions and attempts to synthesise the results of studies that have addressed this issue. It also aims to describe the key characteristics of pollution, the impacts upon global and local air quality and to address the future potential of research by highlighting research needs.

  11. Ambient air pollution and hypertensive disorders of pregnancy: A systematic review and meta-analysis

    Science.gov (United States)

    Hu, Hui; Ha, Sandie; Roth, Jeffrey; Kearney, Greg; Talbott, Evelyn O.; Xu, Xiaohui

    2014-11-01

    Hypertensive disorders of pregnancy (HDP, including gestational hypertension, preeclampsia, and eclampsia) have a substantial public health impact. Maternal exposure to high levels of air pollution may trigger HDP, but this association remains unclear. The objective of our report is to assess and quantify the association between maternal exposures to criteria air pollutants (ozone, carbon monoxide, nitrogen dioxide, sulfur dioxide, and particulate matter ≤10, 2.5 μm) on HDP risk. PubMed, EMBASE, MEDLINE, Current Contents, Global Health, and Cochrane were searched (last search: September, 2013). After a detailed screening of 270 studies, 10 studies were extracted. We conducted meta-analyses if a pollutant in a specific exposure window was reported by at least four studies. Using fixed- and random-effects models, odds ratios (ORs) and 95% CIs were calculated for each pollutant with specific increment of concentration. Increases in risks of HDP (OR per 10 ppb = 1.16; 95% CI, 1.03-1.30) and preeclampsia (OR per 10 ppb = 1.10; 95% CI, 1.03-1.17) were observed to be associated with exposure to NO2 during the entire pregnancy, and significant associations between HDP and exposure to CO (OR per 1 ppm = 1.79; 95% CI, 1.31-2.45) and O3 (OR per 10 ppb = 1.09; 95% CI, 1.05-1.13) during the first trimester were also observed. Our review suggests an association between ambient air pollution and HDP risk. Although the ORs were relatively low, the population-attributable fractions were not negligible given the ubiquitous nature of air pollution.

  12. Ambient Fine Particulate (PM2.5) Air Pollution Attributable to Household Cooking Fuel in Asia

    Science.gov (United States)

    Chafe, Z.; Mehta, S.; Smith, K. R.

    2011-12-01

    Using the Greenhouse Gas and Air Pollution Interactions and Synergies (GAINS) model, hosted by the International Institute for Applied Systems Analysis (IIASA), we estimate the proportion of fine particulate ambient air pollution (PM2.5) attributable to household fuel use for cooking in Asia. This analysis considers primary anthropogenic PM2.5 emissions in two years: 1990 and 2005. Only emissions from household cooking fuels-not heating or lighting-are considered. Due to data availability, this analysis focuses solely on Asian countries, notably India and China which are home to about half of the households using solid fuel use worldwide. Forest and grassland fires, dust, and other "natural" particle sources were omitted from this analysis. The impact of emission sources on secondary particles from aerosol precursors was not determined. In China, the proportion of total primary anthropogenic PM2.5 attributable to household cooking decreased from 44% to 31% between 1990 and 2005. In India, the percent of primary anthropogenic PM2.5 emissions attributable to household cooking decreased from 55% to 49% between 1990 and 2005. Total mass change in primary anthropogenic PM2.5 emissions was much more variable by state in India, between 1990 and 2005, than by province in China (where there was a general downward trend in the total mass emitted). Similarly, growth in industrial emissions was much more variable at the sub-national level, between 1990 and 2005, in India than in China. Energy production played a more prominent role in the growth of primary anthropogenic PM2.5 emissions in India than it did in China. Forward-looking GAINS scenarios show that the contribution of household cooking to total primary anthropogenic PM2.5 emissions is much greater than that from on-road transport in India and China between 1990 and 2030. On-road cars, trucks, and other transport vehicles are, however, the cause of important pollutants other than PM2.5 (as are as cooking stoves that do

  13. Industry, air and climate control; Industrie, protection de l'air et du climat

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    2001-11-01

    Facing the fight against the climatic changes, the industry invests in processes to control the greenhouse effect gazes. This colloquium proposes to insist on the dialog between the public policy and the manufacturers, to make the state of the art on the performances evolution and the agreements and to present the financial and energetic cost of the pollution control. (A.L.B.)

  14. Air-quality and Climatic Consequences of Bioenergy Crop Cultivation

    Science.gov (United States)

    Porter, William Christian

    Bioenergy is expected to play an increasingly significant role in the global energy budget. In addition to the use of liquid energy forms such as ethanol and biodiesel, electricity generation using processed energy crops as a partial or full coal alternative is expected to increase, requiring large-scale conversions of land for the cultivation of bioenergy feedstocks such as cane, grasses, or short rotation coppice. With land-use change identified as a major contributor to changes in the emission of biogenic volatile organic compounds (BVOCs), many of which are known contributors to the pollutants ozone (O 3) and fine particulate matter (PM2.5), careful review of crop emission profiles and local atmospheric chemistry will be necessary to mitigate any unintended air-quality consequences. In this work, the atmospheric consequences of bioenergy crop replacement are examined using both the high-resolution regional chemical transport model WRF/Chem (Weather Research and Forecasting with Chemistry) and the global climate model CESM (Community Earth System Model). Regional sensitivities to several representative crop types are analyzed, and the impacts of each crop on air quality and climate are compared. Overall, the high emitting crops (eucalyptus and giant reed) were found to produce climate and human health costs totaling up to 40% of the value of CO 2 emissions prevented, while the related costs of the lowest-emitting crop (switchgrass) were negligible.

  15. Fish oil and olive oil supplements attenuate the adverse cardiovascular effects of concentrated ambient air pollution particles exposure in healthy middle-aged adult human volunteers

    Science.gov (United States)

    Exposure to ambient levels of air pollution increases cardiovascular morbidity and mortality. Advanced age is among the factors associated with susceptibility to the adverse effects of air pollution. Dietary fatty acid supplementation has been shown to decrease cardiovascular ris...

  16. Particulate matter concentration in ambient air and its effects on lung functions among residents in the National Capital Region, India.

    Science.gov (United States)

    Kesavachandran, C; Pangtey, B S; Bihari, V; Fareed, M; Pathak, M K; Srivastava, A K; Mathur, N

    2013-02-01

    The World Health Organization has estimated that air pollution is responsible for 1.4 % of all deaths and 0.8 % of disability-adjusted life years. NOIDA, located at the National Capital Region, India, was declared as one of the critically air-polluted areas by the Central Pollution Control Board of the Government of India. Studies on the relationship of reduction in lung functions of residents living in areas with higher concentrations of particulate matter (PM) in ambient air were inconclusive since the subjects of most of the studies are hospital admission cases. Very few studies, including one from India, have shown the relationship of PM concentration and its effects of lung functions in the same location. Hence, a cross-sectional study was undertaken to study the effect of particulate matter concentration in ambient air on the lung functions of residents living in a critically air-polluted area in India. PM concentrations in ambient air (PM(1,) PM(2.5)) were monitored at residential locations and identified locations with higher (NOIDA) and lower concentrations (Gurgaon). Lung function tests (FEV(1), PEFR) were conducted using a spirometer in 757 residents. Both air monitoring and lung function tests were conducted on the same day. Significant negative linear relationship exists between higher concentrations of PM(1) with reduced FEV(1) and increased concentrations of PM(2.5) with reduced PEFR and FEV(1). The study shows that reductions in lung functions (PEFR and FEV(1)) can be attributed to higher particulate matter concentrations in ambient air. Decline in airflow obstruction in subjects exposed to high PM concentrations can be attributed to the fibrogenic response and associated airway wall remodeling. The study suggests the intervention of policy makers and stake holders to take necessary steps to reduce the emissions of PM concentrations, especially PM(1,) PM(2.5), which can lead to serious respiratory health concerns in residents.

  17. Future research needs associated with the assessment of potential human health risks from exposure to toxic ambient air pollutants

    DEFF Research Database (Denmark)

    Möller, Lennart; Schuetzle, Dennis; Autrup, Herman

    1994-01-01

    This paper presents key conclusions and future research needs from a Workshop on the Risk Assessment of Urban Air, Emissions, Exposure, Risk Identification, and Quantification, which was held in Stockholm during June 1992 by 41 participants from 13 countries. Research is recommended in the areas...... of identification and quantification of toxics in source emissions and ambient air, atmospheric transport and chemistry, exposure level assessment, the development of improved in vitro bioassays, biomarker development, the development of more accurate epidemiological methodologies, and risk quantification...

  18. Effect of poverty on the relationship between personal exposures and ambient concentrations of air pollutants in Ho Chi Minh City

    Science.gov (United States)

    Mehta, Sumi; Sbihi, Hind; Dinh, Tuan Nguyen; Xuan, Dan Vu; Le Thi Thanh, Loan; Thanh, Canh Truong; Le Truong, Giang; Cohen, Aaron; Brauer, Michael

    2014-10-01

    Socioeconomic factors often affect the distribution of exposure to air pollution. The relationships between health, air pollution, and poverty potentially have important public health and policy implications, especially in areas of Asia where air pollution levels are high and income disparity is large. The objective of the study was to characterize the levels, determinants of exposure, and relationships between children personal exposures and ambient concentrations of multiple air pollutants amongst different socioeconomic segments of the population of Ho Chi Minh City, Vietnam. Using repeated (N = 9) measures personal exposure monitoring and determinants of exposure modeling, we compared daily average PM2.5, PM10, PM2.5 absorbance and NO2 concentrations measured at ambient monitoring sites to measures of personal exposures for (N = 64) caregivers of young children from high and low socioeconomic groups in two districts (urban and peri-urban), across two seasons. Personal exposures for both PM sizes were significantly higher among the poor compared to non-poor participants in each district. Absolute levels of personal exposures were under-represented by ambient monitors with median individual longitudinal correlations between personal exposures and ambient concentrations of 0.4 for NO2, 0.6 for PM2.5 and PM10 and 0.7 for absorbance. Exposures of the non-poor were more highly correlated with ambient concentrations for both PM size fractions and absorbance while those for NO2 were not significantly affected by socioeconomic position. Determinants of exposure modeling indicated the importance of ventilation quality, time spent in the kitchen, air conditioner use and season as important determinant of exposure that are not fully captured by the differences in socioeconomic position. Our results underscore the need to evaluate how socioeconomic position affects exposure to air pollution. Here, differential exposure to major sources of pollution, further influenced by

  19. Air Gaps, Size Effect, and Corner-Turning in Ambient LX-17

    Energy Technology Data Exchange (ETDEWEB)

    Souers, P C; Hernandez, A; Cabacungan, C; Fried, L; Garza, R; Glaesemann, K; Lauderbach, L; Liao, S; Vitello, P

    2008-02-05

    Various ambient measurements are presented for LX-17. The size (diameter) effect has been measured with copper and Lucite confinement, where the failure radii are 4.0 and 6.5 mm, respectively. The air well corner-turn has been measured with an LX-07 booster, and the dead-zone results are comparable to the previous TATB-boosted work. Four double cylinders have been fired, and dead zones appear in all cases. The steel-backed samples are faster than the Lucite-backed samples by 0.6 {micro}s. Bare LX-07 and LX-17 of 12.7 mm-radius were fired with air gaps. Long acceptor regions were used to truly determine if detonation occurred or not. The LX-07 crossed at 10 mm with a slight time delay. Steady state LX-17 crossed at 3.5 mm gap but failed to cross at 4.0 mm. LX-17 with a 12.7 mm run after the booster crossed a 1.5 mm gap but failed to cross 2.5 mm. Timing delays were measured where the detonation crossed the gaps. The Tarantula model is introduced as embedded in 0 reactive flow JWL++ and Linked Cheetah V4, mostly at 4 zones/mm. Tarantula has four pressure regions: off, initiation, failure and detonation. The physical basis of the input parameters is considered.

  20. Pulmonary function and respiratory symptoms of school children exposed to ambient air pollution

    Energy Technology Data Exchange (ETDEWEB)

    Kim, Yoon Shin; Ko, Ung Ring [Hanyang Univ., Seoul (Korea, Republic of)

    1996-12-31

    This study was undertaken to evaluate the health effect of air pollution on pulmonary function and respiratory symptoms of Korean school children between 7 and 10 years of age during November 1995-January 1996. A standard respiratory symptom questionnaire was administered and spirometry was performed to examine pulmonary function of 121 children in an urban polluted area, Seoul, and of 119 children in non-polluted area, Sokcho, respectively. There was significant difference in the level of pulmonary function [forced expiratory volume in second (FEV{sub 1.0}) and forced vital capacity (FVC)] between exposed groups to polluted area and non-polluted area. Parental smoking was significantly related to respiratory symptoms of cough, phlegm, and the level of pulmonary function. The observed changes in FEV{sub 1.0} and FVC seemed to relate to home cooking fuel, not to respiratory symptoms. The additional longitudinal work that carefully monitors ambient and indoor air pollution and health effects data should be conducted to confirm these results.

  1. The effect of humidity on ionic wind velocity in ambient air

    Science.gov (United States)

    Chen, She; Nobelen, J. C. P. Y.; Nijdam, S.

    2016-09-01

    Due to the evolution of portable electronics and LED lightning system, advances in air cooling technologies must also keep pace. Active cooling by ionic wind, which is usually generated by corona discharge, can greatly reduce the noise and lifetime issues compared to the mechanical fans. The wind is induced when a gas discharge is formed, and neutral molecules gain their energy by the momentum transfer of ion-neutral collisions. However, there is few discussion about the effect of gas composition such as humidity on the wind generation and the physical mechanism is not clear. In the experiment, a positive 5-20 kV DC voltage is applied to the needle-cylinder electrodes with separation of 20 mm. The ionic wind velocity is measured by hot wire anemometry. As the relative humidity (RH) in the ambient air increases, the velocity is found to be severely inhibited. The current is also measured between the cylinder electrode and earth. The results show that the DC component of corona current decreases when RH increases. Since both the discharge current and the ion mobility are reduced when RH increases, their combined effects determine the ionic wind velocity. This work is supported by STW project 13651.

  2. Concentration and Size Distribution of Particulate Matter in a Broiler House Ambient Air

    Directory of Open Access Journals (Sweden)

    Ismael Rodrigues Amador

    2016-07-01

    Full Text Available Atmospheric particulate matter (PM is an important constituent of ambient air. The determination of its concentration and size distribution in different environments is essential because of its ability to penetrate deeply into animal and human respiratory tract. In this study, air sampling was performed in a broiler house to estimate the concentration and size distribution of PM emitted along with its activities. Low-vol impactor (< 10 mm, cyclones (< 2.5 e < 1.0 mm, and Sioutas cascade impactor (> 2.5; 1.0 – 2.5; 0.50 – 1.0; 0.25 – 0.50; < 0.25 mm connected with membrane pumps were used. PM10 showed high concentration (209 - 533 mg m-3. PM2.5 and PM1.0 initially showed relatively low concentration (20.8 and 16.0 mg m-3 respectively with significantly increasing levels (412.9 and 344.8 mg m-3 respectively during the samplings. It was also possible to observe the contribution of fine particles. This was evidenced by the high correlation between PM2.5 and PM1.0 and by the profile of particle distribution in the Sioutas sampler. PM concentration levels are considered excessively high, with great potential to affect animal and human health. DOI: http://dx.doi.org/10.17807/orbital.v8i3.847 

  3. Impact of road traffic emissions on ambient air quality in an industrialized area.

    Science.gov (United States)

    Garcia, Sílvia M; Domingues, Gonçalo; Gomes, Carla; Silva, Alexandra V; Almeida, S Marta

    2013-01-01

    Several epidemiological studies showed a correlation between airborne particulate matter(PM) and the incidence of several diseases in exposed populations. Consequently, the European Commission reinforced the need and obligation of member-states to monitor exposure levels of PM and adopt measures to reduce this exposure. However, in order to plan appropriate actions, it is necessary to understand the main sources of air pollution and their relative contributions to the formation of the ambient aerosol. The aim of this study was to develop a methodology to assess the contribution of vehicles to the atmospheric aerosol,which may constitute a useful tool to assess the effectiveness of planned mitigation actions.This methodology is based on three main steps: (1) estimation of traffic emissions provided from the vehicles exhaust and resuspension; (2) use of the dispersion model TAPM (“The Air Pollution Model”) to estimate the contribution of traffic for the atmospheric aerosol; and(3) use of geographic information system (GIS) tools to map the PM10 concentrations provided from traffic in the surroundings of a target area. The methodology was applied to an industrial area, and results showed that the highest contribution of traffic for the PM10 concentrations resulted from dust resuspension and that heavy vehicles were the type that most contributed to the PM10 concentration.

  4. 77 FR 39205 - Public Hearings for Proposed Rules-National Ambient Air Quality Standards for Particulate Matter

    Science.gov (United States)

    2012-07-02

    ... slide presentations unless we receive special requests in advance. Commenters should notify Mr. Rush if... data handling conventions for PM and ambient air monitoring, reporting, and network design requirements... questions during the oral presentations, but will not respond to the presentations at that time....

  5. 40 CFR Appendix P to Part 50 - Interpretation of the Primary and Secondary National Ambient Air Quality Standards for Ozone

    Science.gov (United States)

    2010-07-01

    ... 40 Protection of Environment 2 2010-07-01 2010-07-01 false Interpretation of the Primary and Secondary National Ambient Air Quality Standards for Ozone P Appendix P to Part 50 Protection of Environment... STANDARDS Pt. 50, App. P Appendix P to Part 50—Interpretation of the Primary and Secondary National...

  6. The Association between Ambient Air Pollution and Allergic Rhinitis: Further Epidemiological Evidence from Changchun, Northeastern China

    Science.gov (United States)

    Teng, Bo; Zhang, Xuelei; Yi, Chunhui; Zhang, Yan; Ye, Shufeng; Wang, Yafang; Tong, Daniel Q.; Lu, Binfeng

    2017-01-01

    With the continuous rapid urbanization process over the last three decades, outdoors air pollution has become a progressively more serious public health hazard in China. To investigate the possible associations, lag effects and seasonal differences of urban air quality on respiratory health (allergic rhinitis) in Changchun, a city in Northeastern China, we carried out a time-series analysis of the incidents of allergic rhinitis (AR) from 2013 to 2015. Environmental monitoring showed that PM2.5 and PM10 were the major air pollutants in Changchun, followed by SO2, NO2 and O3. The results also demonstrated that the daily concentrations of air pollutants had obvious seasonal differences. PM10 had higher daily mean concentrations in spring (May, dust storms), autumn (October, straw burning) and winter (November to April, coal burning). The mean daily number of outpatient AR visits in the warm season was higher than in the cold season. The prevalence of allergic rhinitis was significantly associated with PM2.5, PM10, SO2 and NO2, and the increased mobility was 10.2% (95% CI, 5.5%–15.1%), 4.9% (95% CI, 0.8%–9.2%), 8.5% (95% CI, −1.8%–19.8%) and 11.1% (95% CI, 5.8%–16.5%) for exposure to each 1-Standard Deviation (1-SD) increase of pollutant, respectively. Weakly or no significant associations were observed for CO and O3. As for lag effects, the highest Relative Risks (RRs) of AR from SO2, NO2, PM10 and PM2.5 were on the same day, and the highest RR from CO was on day 4 (L4). The results also indicated that the concentration of air pollutants might contribute to the development of AR. To summarize, this study provides further evidence of the significant association between ambient particulate pollutants (PM2.5 and PM10, which are usually present in high concentrations) and the prevalence of respiratory effects (allergic rhinitis) in the city of Changchun, located in Northeastern China. Environmental control and public health strategies should be enforced to

  7. Impact of Asian Dust on Climate and Air Quality

    Science.gov (United States)

    Chin, Mian; Tan, Qian; Diehl, Thomas; Yu, Hongbin

    2010-01-01

    Dust generated from Asian permanent desert and desertification areas can be efficiently transported around the globe, making significant radiative impact through their absorbing and scattering solar radiation and through their deposition on snow and ice to modify the surface albedo. Asian dust is also a major concern of surface air quality not only in the source and immediate downwind regions but also areas thousands of miles away across the Pacific. We present here a global model, GOCART, analysis of data from satellite remote sensing instrument (MODIS, MISR, CALIPSO, OMI) and other observations on Asian dust sources, transport, and deposition, and use the model to assess the Asian dust impact on global climate and air quality.

  8. Iatrogenic Complications in Five Patients with Upper Gastrointestinal Bleeding due to Ambient Air: Case Series and Literature Review

    Directory of Open Access Journals (Sweden)

    Christine N. Manser

    2012-04-01

    Full Text Available Despite the increasing use of carbon dioxide for endoscopies during the last years, ambient air is still used. The amount of air depends on several factors such as examination time, presumable diameter of the endoscope channel and of course active use of air by the operator. Although endoscopic complications due to ambient air in the gastrointestinal (GI tract are a rare observation and mostly described in the colon, we report five cases in the upper GI tract due to insufflating large amounts of air through the endoscopes. All 5 patients needed an emergency upper endoscopy for acute presumed upper GI bleeding. In two cases both esophageal variceal bleeding and ulcer bleeding were detected; the fifth case presented with a bleeding due to gastric cancer. Due to insufflation of inadequate amounts of air through the endoscope channel, all patients deteriorated in circulation and ventilation. Two rumenocenteses and consecutively three laparotomies had to be performed in three patients. In the other two, gastroscopies had to be stopped for an emergency computed tomography. All critical incidents were believed to be a consequence of a long-lasting examination with use of too much air. Therefore in emergency situations, endoscopies should be performed with either submersion, low air flow pumps or even better by the use of carbon dioxide.

  9. Identification of the Products of Oxidation of Quercetin by Air Oxygenat Ambient Temperature

    Directory of Open Access Journals (Sweden)

    Viktor A Utsal

    2007-03-01

    Full Text Available Oxidation of quercetin by air oxygen takes place in water and aqueous ethanol solutions under mild conditions, namely in moderately-basic media (pH ∼ 8-10 at ambient temperature and in the absence of any radical initiators, without enzymatic catalysis or irradiation of the reaction media by light. The principal reaction products are typical of other oxidative degradation processes of quercetin, namely 3,4-dihydroxy-benzoic (proto-catechuic and 2,4,6-trihydroxybenzoic (phloroglucinic acids, as well as the decarboxylation product of the latter – 1,3,5-trihydroxybenzene (phloroglucinol. In accordance with the literature data, this process involves the cleavage of the γ-pyrone fragment (ring C of the quercetin molecule by oxygen, with primary formation of 4,6-dihydroxy-2-(3,4-dihydroxybenzoyloxybenzoic acid (depside. However under such mild conditions the accepted mechanism of this reaction (oxidative decarbonylation with formation of carbon monoxide, CO should be reconsidered as preferably an oxidative decarboxylation with formation of carbon dioxide, CO2. Direct head-space analysis of the gaseous components formed during quercetin oxidation in aqueous solution at ambient temperature indicates that the ratio of carbon dioxide/carbon monoxide in the gas phase after acidification of the reaction media is ca. 96:4 %. Oxidation under these mild conditions is typical for other flavonols having OH groups at C3 (e.g., kaempferol, but it is completely suppressed if this hydroxyl group is substituted by a glycoside fragment (as in rutin, or a methyl substituent. An alternative oxidation mechanism involving the direct cleavage of the C2-C3 bond in the diketo-tautomer of quercetin is proposed.

  10. Association of ambient air quality with children`s lung function in urban and rural Iran

    Energy Technology Data Exchange (ETDEWEB)

    Asgari, M.M.; Dubois, A.; Beckett, W.S. [Yale Univ. School of Medicine, New Haven, CT (United States); Asgari, M. [Shaheed Beheshti Univ., Tehran (Iran, Islamic Republic of); Gent, J. [John B. Pierce Lab., New Haven, CT (United States)

    1998-05-01

    During the summer of 1994, a cross-sectional epidemiological study, in which the pulmonary function of children in Tehran was compared with pulmonary function in children in a rural town in Iran, was conducted. Four hundred children aged 5--11 y were studied. Daytime ambient nitrogen dioxide, sulfur dioxide, and particulate matter were measured with portable devices, which were placed in the children`s neighborhoods on the days of study. Levels of these ambient substances were markedly higher in urban Tehran than in rural areas. Children`s parents were questioned about home environmental exposures (including heating source and environmental tobacco smoke) and the children`s respiratory symptoms. Pulmonary function was assessed, both by spirometry and peak expiratory flow meter. Forced expiratory volume in 1 s and forced vital capacity--as a percentage of predicted for age, sex and height--were significantly lower in urban children than in rural children. Both measurements evidenced significant reverse correlations with levels of sulfur dioxide, nitrogen dioxide, and particulate matter. Differences in spirometric lung function were not explained by nutritional status, as assessed by height and weight for age, or by home environmental exposures. Reported airway symptoms were higher among rural children, whereas reported physician diagnosis of bronchitis and asthma were higher among urban children. The association between higher pollutant concentrations and reduced pulmonary function in this urban-rural comparison suggests that there is an effect of urban air pollution on short-term lung function and/or lung growth and development during the preadolescent years.

  11. Evaluation of ambient air concentrations of polycyclic aromatic hydrocarbons in Germany from 1990 to 1998.

    Science.gov (United States)

    Fertmann, Regina; Tesseraux, Irene; Schümann, Michael; Neus, Hermann

    2002-03-01

    All available polycyclic aromatic hydrocarbon (PAH) concentration data in ambient air obtained over the past 10 years in Germany were evaluated to clarify whether it is justified to use benzo(a)pyrene (BaP) as a marker compound for the total PAH exposure. The data basis comprises annual mean concentrations from 1990 to 1998 supplied by the emission protection authorities of the federal states with additional information on the region, year and site of measurement. The data are very heterogeneous with respect to sample size, the number of individual PAHs analyzed, place of origin and year. Nine of 25 individual compounds with sufficient sample size (74German reunion and time characterize the distributive patterns, e.g., from 1991 to 1997, a significant decrease in BaP could be determined based on the data from North Rhine-Westphalia (1991, N=51, median 1.6 ng/m(3); 1997, N=45, median 0.7 ng/m(3); Pambient air.

  12. Study on an air quality evaluation model for Beijing City under haze-fog pollution based on new ambient air quality standards.

    Science.gov (United States)

    Li, Li; Liu, Dong-Jun

    2014-08-28

    Since 2012, China has been facing haze-fog weather conditions, and haze-fog pollution and PM2.5 have become hot topics. It is very necessary to evaluate and analyze the ecological status of the air environment of China, which is of great significance for environmental protection measures. In this study the current situation of haze-fog pollution in China was analyzed first, and the new Ambient Air Quality Standards were introduced. For the issue of air quality evaluation, a comprehensive evaluation model based on an entropy weighting method and nearest neighbor method was developed. The entropy weighting method was used to determine the weights of indicators, and the nearest neighbor method was utilized to evaluate the air quality levels. Then the comprehensive evaluation model was applied into the practical evaluation problems of air quality in Beijing to analyze the haze-fog pollution. Two simulation experiments were implemented in this study. One experiment included the indicator of PM2.5 and was carried out based on the new Ambient Air Quality Standards (GB 3095-2012); the other experiment excluded PM2.5 and was carried out based on the old Ambient Air Quality Standards (GB 3095-1996). Their results were compared, and the simulation results showed that PM2.5 was an important indicator for air quality and the evaluation results of the new Air Quality Standards were more scientific than the old ones. The haze-fog pollution situation in Beijing City was also analyzed based on these results, and the corresponding management measures were suggested.

  13. Fire Influences on Atmospheric Composition, Air Quality, and Climate

    Science.gov (United States)

    Voulgarakis, Apostolos; Field, Robert D.

    2015-01-01

    Fires impact atmospheric composition through their emissions, which range from long-lived gases to short-lived gases and aerosols. Effects are typically larger in the tropics and boreal regions but can also be substantial in highly populated areas in the northern mid-latitudes. In all regions, fire can impact air quality and health. Similarly, its effect on large-scale atmospheric processes, including regional and global atmospheric chemistry and climate forcing, can be substantial, but this remains largely unexplored. The impacts are primarily realised in the boundary layer and lower free troposphere but can also be noticeable in upper troposphere/lower stratosphere (UT/LS) region, for the most intense fires. In this review, we summarise the recent literature on findings related to fire impact on atmospheric composition, air quality and climate. We explore both observational and modelling approaches and present information on key regions and on the globe as a whole. We also discuss the current and future directions in this area of research, focusing on the major advances in emission estimates, the emerging efforts to include fire as a component in Earth system modelling and the use of modelling to assess health impacts of fire emissions.

  14. Polar Air Quality and Climate from a Molniya Orbit

    Science.gov (United States)

    O'Neill, N.; McConnell, J. C.; Mullins, M.; Chesser, H.; Solheim, B.; Kaminski, J.; Strong, K.; Jones, D.; Drummond, J.; Martin, R.; McElroy, C. T.; Evans, W. F.; Giroux, J. G.; Soucy, M. A.; Buijs, H. L.; Moreau, L. M.; Buttner, G.; Rahnama, P.; Rowlands, N.; Hackett, J.; Bell, A.

    2008-05-01

    The Arctic is a region of rapid climate change with warming temperatures and depleting summer ice which may be exacerbated by transport of soot and other anthropogenic material from mid-latitudes. It is also the source of winter storms delivering cold air to lower latitudes. Currently data is available for these areas from polar orbiting satellites, but only intermittently at a given location as the satellites pass overhead. Data from geostationary satellites, useful at lower latitudes, is not available for the Arctic because viewing angles to high latitude locations from geostationary orbit are poor. We are proposing the use of a satellite in a Molniya orbit for the acquisition of data for high latitudes which is a quasi-stationary orbit close to apogee. This talk will describe a proposal to the Canadian Space Agency for a mission aimed at the acquisition of air quality and climate data in boreal polar regions and mid-latitudes. Molniya orbits (named after the Russian communications satellite series that first used them) are highly elliptical orbits with an inclination of approximately 63°. At this inclination, the Earth oblateness perturbation does not cause any change to the orbit's argument of perigee. Further, if the orbit semi-major axis is chosen appropriately, the orbit can be timed to have a period of half a day (typical Molniya orbits have an apogee altitude of about 39750 km and a perigee altitude of about 600 km). The result of these two constraints is that the satellite is at apogee over the same high latitude location on the Earth every two orbits. At the alternate apogees, it is over a location at the same latitude but 180° away in longitude. Either location provides viewing coverage of the entire Earth above 60°N, and reasonable viewing down to 50°N. Further, because the satellite is travelling slowly at apogee, the viewing geometry is maintained for approximately 2/3 of the orbit (8 hr out of every 12). The suite of instruments we are

  15. A CFD analysis on the effect of ambient conditions on the hygro-thermal stresses distribution in a planar ambient air-breathing PEM fuel cell

    Directory of Open Access Journals (Sweden)

    Maher A.R. Sadiq Al-Baghdadi

    2011-07-01

    Full Text Available The need for improved lifetime of air-breathing proton exchange membrane (PEM fuel cells for portable applications necessitates that the failure mechanisms be clearly understood and life prediction models be developed, so that new designs can be introduced to improve long-term performance. An operating air-breathing PEM fuel cell has varying local conditions of temperature and humidity. As a result of in the changes in temperature and moisture, the membrane, GDL and bipolar plates will all experience expansion and contraction. Because of the different thermal expansion and swelling coefficients between these materials, hygro-thermal stresses are introduced into the unit cell during operation. In addition, the non-uniform current and reactant flow distributions in the cell result in non-uniform temperature and moisture content of the cell which could in turn, potentially causing localized increases in the stress magnitudes, and this leads to mechanical damage, which can appear as through-the-thickness flaws or pinholes in the membrane, or delaminating between the polymer membrane and gas diffusion layers. Therefore, in order to acquire a complete understanding of these damage mechanisms in the membranes and gas diffusion layers, mechanical response under steady-state hygro-thermal stresses should be studied under real cell operation conditions. A three-dimensional, multi–phase, non-isothermal computational fluid dynamics model of a planar ambient air-breathing, proton exchange membrane fuel cell has been developed and used to study the effects of ambient conditions on the temperature distribution, displacement, deformation, and stresses inside the cell. The behaviour of the fuel cell during operation has been studied and investigated under real cell operating conditions. A unique feature of the present model is to incorporate the effect of mechanical, hygro and thermal stresses into actual three-dimensional fuel cell model. The results show

  16. The Use of Lichens as Indicators of Ambient Air Quality in Southern Ontario

    Science.gov (United States)

    Tulumello, Patricia M.

    The inverse relationship between arboreal lichen species richness and sulphur dioxide in ambient air has been thoroughly documented in the literature. Previous work in southern Ontario has shown that lichen bioindication can identify areas of potential concern regarding air quality. The EMAN suite of lichens was applied in the City of Sarnia by surveying 458 Sugar Maple trees, in order to test the applicability of lichen bioindication under conditions of high mean SO2 levels and high species richness values. The results of the survey were explored using Geographic Information Systems. A spatial relationship between lichen community variables, the Bluewater Bridge and the highway was identified. Lichen species richness, lichen percent cover and Index of Atmospheric Purity values were higher along the bridge and highway. No strong gradients were found between other known pollution sources and no lichen deserts were identified. The most common community grouping consisted of Physcia millegrana Degel, Candelaria concolor (Dicks) B. Stein, Physcia aipolia (Ehrh ex Humb.) Furnrohr; all of which are known nitrophytes. The relationship between substrate pH and lichen species richness was examined. Sites with a known source of anthropogenic chemical contamination were found to have a correlation of r2=o.8 between lichen species richness and pH. The inverse was found for sites with no known source of contamination with a correlation of r2=-0.72. The findings suggest that species richness may be influenced by altering substrate pH which promotes the growth of nitrophytic species capable of tolerating high SO2 levels.

  17. Air Gaps, Size Effect, and Corner-Turning in Ambient LX-17

    Energy Technology Data Exchange (ETDEWEB)

    Souers, P C; Hernandez, A; Cabacungen, C; Fried, L; Garza, R; Glaesemann, K; Lauderbach, L; Liao, S; Vitello, P

    2007-05-30

    Various ambient measurements are presented for LX-17. The size (diameter) effect has been measured with copper and Lucite confinement, where the failure radii are 4.0 and 6.5 mm, respectively. The air well corner-turn has been measured with an LX-07 booster, and the dead-zone results are comparable to the previous TATB-boosted work. Four double cylinders have been fired, and dead zones appear in all cases. The steel-backed samples are faster than the Lucite-backed samples by 0.6 {micro}s. Bare LX-07 and LX-17 of 12.7 mm-radius were fired with air gaps. Long acceptor regions were used to truly determine if detonation occurred or not. The LX-07 crossed at 10 mm with a slight time delay. Steady state LX-17 crossed at 3.5 mm gap but failed to cross at 4.0 mm. LX-17 with a 12.7 mm run after the booster crossed a 1.5 mm gap but failed to cross 2.5 mm. Timing delays were measured where the detonation crossed the gaps. The Tarantula model is introduced as embedded in the Linked Cheetah V4.0 reactive flow code at 4 zones/mm. Tarantula has four pressure regions: off, initiation, failure and detonation. A report card of 25 tests run with the same settings on LX-17 is shown, possibly the most extensive simultaneous calibration yet tried with an explosive. The physical basis of some of the input parameters is considered.

  18. Chemo-Mechanical Characteristics of Mud Formed from Environmental Dust Particles in Humid Ambient Air

    Science.gov (United States)

    Hassan, Ghassan; Yilbas, B. S.; Said, Syed A. M.; Al-Aqeeli, N.; Matin, Asif

    2016-07-01

    Mud formed from environmental dust particles in humid ambient air significantly influences the performance of solar harvesting devices. This study examines the characterization of environmental dust particles and the chemo-mechanics of dry mud formed from dust particles. Analytical tools, including scanning electron microscopy, atomic force microscopy, energy dispersive spectroscopy, particle sizing, and X-ray diffraction, are used to characterize dry mud and dust particles. A micro/nano tribometer is used to measure the tangential force and friction coefficient while tensile tests are carried out to assess the binding forces of dry mud pellets. After dry mud is removed, mud residuals on the glass surface are examined and the optical transmittance of the glass is measured. Dust particles include alkaline compounds, which dissolve in water condensate and form a mud solution with high pH (pH = 7.5). The mud solution forms a thin liquid film at the interface of dust particles and surface. Crystals form as the mud solution dries, thus, increasing the adhesion work required to remove dry mud from the surface. Optical transmittance of the glass is reduced after dry mud is removed due to the dry mud residue on the surface.

  19. Antioxidants keep the potentially probiotic but highly oxygen-sensitive human gut bacterium Faecalibacterium prausnitzii alive at ambient air.

    Directory of Open Access Journals (Sweden)

    M Tanweer Khan

    Full Text Available The beneficial human gut microbe Faecalibacterium prausnitzii is a 'probiotic of the future' since it produces high amounts of butyrate and anti-inflammatory compounds. However, this bacterium is highly oxygen-senstive, making it notoriously difficult to cultivate and preserve. This has so far precluded its clinical application in the treatment of patients with inflammatory bowel diseases. The present studies were therefore aimed at developing a strategy to keep F. prausnitzii alive at ambient air. Our previous research showed that F. prausnitzii can survive in moderately oxygenized environments like the gut mucosa by transfer of electrons to oxygen. For this purpose, the bacterium exploits extracellular antioxidants, such as riboflavin and cysteine, that are abundantly present in the gut. We therefore tested to what extent these antioxidants can sustain the viability of F. prausnitzii at ambient air. The present results show that cysteine can facilitate the survival of F. prausnitzii upon exposure to air, and that this effect is significantly enhanced the by addition of riboflavin and the cryoprotectant inulin. The highly oxygen-sensitive gut bacterium F. prausnitzii can be kept alive at ambient air for 24 h when formulated with the antioxidants cysteine and riboflavin plus the cryoprotectant inulin. Improved formulations were obtained by addition of the bulking agents corn starch and wheat bran. Our present findings pave the way towards the biomedical exploitation of F. prausnitzii in redox-based therapeutics for treatment of dysbiosis-related inflammatory disorders of the human gut.

  20. Online hourly determination of 62 VOCs in ambient air: system evaluation and comparison with another two analytical techniques.

    Science.gov (United States)

    Durana, Nieves; Navazo, Marino; Alonso, Luclo; García, José A; Ilardia, Juan L; Gómez, M Carmen; Gangoiti, Gotzon

    2002-10-01

    This paper presents results of the processing and validation of data collected by an automatic gas chromatograph (AGC). This system was used to monitor 62 volatile organic compounds (VOCs) in urban air in the Basque Country, Spain. The nonpolar compounds (C2-C10) identified-paraffins, olefins, aromatics, and chlorinated compounds-accounted for 88% of the mass of total non-methane hydrocarbons (TNMHCs) in ambient air. The evaluation of linearity, precision, detection limits (DLs), and stability of retention times (RTs) indicates that the equipment is suitable for measuring ambient air automatically for prolonged periods (6 months). The calibration of the equipment using response factors calculated on the basis of the effective carbon number (ECN) showed variations of over 10% for acetylene, isoprene, and n-hexane. The results provided by the automatic chromatograph correlated significantly with simultaneous results from other widely used techniques for determining VOCs in ambient air: (1) portable GC, equipped with photoionization detector (PID), and (2) active adsorption on Tenax-TA followed by thermal desorption and chromatographic analysis.

  1. Occurrence and Concentrations of Toxic VOCs in the Ambient Air of Gumi, an Electronics-Industrial City in Korea

    Directory of Open Access Journals (Sweden)

    Sung-Ok Baek

    2015-08-01

    Full Text Available This study was carried out to characterize the occurrence and concentrations of a variety of volatile organic compounds (VOCs including aliphatic, aromatic, halogenated, nitrogenous, and carbonyl compounds, in the ambient air of Gumi City, where a large number of electronics industries are found. Two field monitoring campaigns were conducted for a one year period in 2003/2004 and 2010/2011 at several sampling sites in the city, representing industrial, residential and commercial areas. More than 80 individual compounds were determined in this study, and important compounds were then identified according to their abundance, ubiquity and toxicity. The monitoring data revealed toluene, trichloroethylene and acetaldehyde to be the most significant air toxics in the city, and their major sources were mainly industrial activities. On the other hand, there was no clear evidence of an industrial impact on the concentrations of benzene and formaldehyde in the ambient air of the city. Overall, seasonal variations were not as distinct as locational variations in the VOCs concentrations, whereas the within-day variations showed a typical pattern of urban air pollution, i.e., increase in the morning, decrease in the afternoon, and an increase again in the evening. Considerable decreases in the concentrations of VOCs from 2003 to 2011 were observed. The reductions in the ambient concentrations were confirmed further by the Korean PRTR data in industrial emissions within the city. Significant decreases in the concentrations of benzene and acetaldehyde were also noted, whereas formaldehyde appeared to be almost constant between the both campaigns. The decreased trends in the ambient levels were attributed not only to the stricter regulations for VOCs in Korea, but also to the voluntary agreement of major companies to reduce the use of organic solvents. In addition, a site planning project for an eco-friendly industrial complex is believed to play a contributory

  2. Quantitative sampling and analysis of trace elements in ambient air: impactor characterization and Synchrotron-XRF mass calibration

    Directory of Open Access Journals (Sweden)

    A. Richard

    2010-06-01

    Full Text Available Identification of trace elements in ambient air can add substantial information to pollution source apportionment studies, although they do not contribute significantly to emissions in terms of mass. A method for quantitative size and time-resolved trace element evaluation in ambient aerosols with a rotating drum impactor and synchrotron radiation based X-ray fluorescence is presented. The impactor collection efficiency curves and size segregation characteristics were investigated in an experiment with oil and salt particles. Cutoff diameters were determined through the ratio of size distributions measured with two particles sizers. Furthermore, an external calibration technique to empirically link fluorescence intensities to ambient concentrations was developed. Solutions of elemental standards were applied with an ink-jet printer on thin films and area concentrations were subsequently evaluated with external wet chemical methods. These customized and reusable reference standards enable quantification of different data sets analyzed under varying experimental conditions.

  3. Real-time measurements of secondary organic aerosol formation and aging from ambient air in an oxidation flow reactor in the Los Angeles area

    Science.gov (United States)

    Ortega, Amber M.; Hayes, Patrick L.; Peng, Zhe; Palm, Brett B.; Hu, Weiwei; Day, Douglas A.; Li, Rui; Cubison, Michael J.; Brune, William H.; Graus, Martin; Warneke, Carsten; Gilman, Jessica B.; Kuster, William C.; de Gouw, Joost; Gutiérrez-Montes, Cándido; Jimenez, Jose L.

    2016-06-01

    Field studies in polluted areas over the last decade have observed large formation of secondary organic aerosol (SOA) that is often poorly captured by models. The study of SOA formation using ambient data is often confounded by the effects of advection, vertical mixing, emissions, and variable degrees of photochemical aging. An oxidation flow reactor (OFR) was deployed to study SOA formation in real-time during the California Research at the Nexus of Air Quality and Climate Change (CalNex) campaign in Pasadena, CA, in 2010. A high-resolution aerosol mass spectrometer (AMS) and a scanning mobility particle sizer (SMPS) alternated sampling ambient and reactor-aged air. The reactor produced OH concentrations up to 4 orders of magnitude higher than in ambient air. OH radical concentration was continuously stepped, achieving equivalent atmospheric aging of 0.8 days-6.4 weeks in 3 min of processing every 2 h. Enhancement of organic aerosol (OA) from aging showed a maximum net SOA production between 0.8-6 days of aging with net OA mass loss beyond 2 weeks. Reactor SOA mass peaked at night, in the absence of ambient photochemistry and correlated with trimethylbenzene concentrations. Reactor SOA formation was inversely correlated with ambient SOA and Ox, which along with the short-lived volatile organic compound correlation, indicates the importance of very reactive (τOH ˜ 0.3 day) SOA precursors (most likely semivolatile and intermediate volatility species, S/IVOCs) in the Greater Los Angeles Area. Evolution of the elemental composition in the reactor was similar to trends observed in the atmosphere (O : C vs. H : C slope ˜ -0.65). Oxidation state of carbon (OSc) in reactor SOA increased steeply with age and remained elevated (OSC ˜ 2) at the highest photochemical ages probed. The ratio of OA in the reactor output to excess CO (ΔCO, ambient CO above regional background) vs. photochemical age is similar to previous studies at low to moderate ages and also extends to

  4. Development of ambient air quality population-weighted metrics for use in time-series health studies.

    Science.gov (United States)

    Ivy, Diane; Mulholland, James A; Russell, Armistead G

    2008-05-01

    A robust methodology was developed to compute population-weighted daily measures of ambient air pollution for use in time-series studies of acute health effects. Ambient data, including criteria pollutants and four fine particulate matter (PM) components, from monitors located in the 20-county metropolitan Atlanta area over the time period of 1999-2004 were normalized, spatially resolved using inverse distance-square weighting to Census tracts, denormalized using descriptive spatial models, and population-weighted. Error associated with applying this procedure with fewer than the maximum number of observations was also calculated. In addition to providing more representative measures of ambient air pollution for the health study population than provided by a central monitor alone and dampening effects of measurement error and local source impacts, results were used to evaluate spatial variability and to identify air pollutants for which ambient concentrations are poorly characterized. The decrease in correlation of daily monitor observations with daily population-weighted average values with increasing distance of the monitor from the urban center was much greater for primary pollutants than for secondary pollutants. Of the criteria pollutant gases, sulfur dioxide observations were least representative because of the failure of ambient networks to capture the spatial variability of this pollutant for which concentrations are dominated by point source impacts. Daily fluctuations in PM of particles less than 10 microm in aerodynamic diameter (PM10) mass were less well characterized than PM of particles less than 2.5 microm in aerodynamic diameter (PM2.5) mass because of a smaller number of PM10 monitors with daily observations. Of the PM2.5 components, the carbon fractions were less well spatially characterized than sulfate and nitrate both because of primary emissions of elemental and organic carbon and because of differences in measurement techniques used to assess

  5. Comparison of Ambient Radon Concentrations in Air in the Northern Mojave Desert from Continuous and Integrating Instruments

    Energy Technology Data Exchange (ETDEWEB)

    David S. Shafer; David McGraw; Lynn H. Karr; Greg McCurdy; Tammy L. Kluesner; Karen J. Gray; Jeffrey Tappen

    2010-05-18

    As part of a program to characterize and baseline environmental parameters, ambient radon-222 (Rn) monitoring was conducted in the rural community of Amargosa Valley, NV, the closest community to Yucca Mountain. Passive integrating and continuous Rn monitoring instruments were deployed adjacent to the Community Environmental Monitoring Program (CEMP) station in Amargosa Valley. The CEMP station provided real-time ambient gamma exposure and meteorological data used to correct the integrated Rn measurements, verified the meteorological data collected by the continuous Rn monitoring instrument, and for provided instrumentation for evaluating the relationships between meteorological conditions and Rn concentrations. Hourly Rn concentrations in air measured by the continuous Rn monitoring instrument (AlphaGUARD®) were compared to the average hourly values for the integrating Rn measurements (E-PERM®) by dividing the total Rn measurements by the number of hours the instruments were deployed. The results of the comparison indicated that average hourly ambient Rn concentrations as measured by both methods ranged from 0.2 to 0.4 pico-curies per liter of air. Ambient Rn values for the AlphaGUARD exhibited diurnal variations. When Rn concentrations were compared with measurements of temperature (T), barometric pressure, and relative humidity, the correlation (inversely) was highest with T, albeit weakly.

  6. The value of health benefits from ambient air quality improvements in Central and Eastern Europe. An exercise in benefits transfer

    Energy Technology Data Exchange (ETDEWEB)

    Krupnick, A.; Harrison, K.; Nickell, E.; Toman, M. [Resources for the Future, Washington, DC (United States)

    1996-06-01

    The study on the title subject is an initial effort to estimate the effects of air pollution on human health in Bulgaria, Hungary, Poland and Ukraine. The estimates are derived from data on ambient air quality in those countries, together with a model that links these ambient conditions to physical impacts on health and attaches economic values (dollars) to these impacts. The focus is on particulates, SO{sub 2} and Pb. Dose response functions, taken from the clinical and epidemiological literature in the USA, Canada, and Western Europe are used to generate estimates of the change in physical effects. These effects then are given an economic value by applying two approaches for scaling unit valuation figures, applicable to the USA. A Monte Carlo model is constructed to propagate the uncertainties of the dose-response functions and unit values to obtain confidence intervals on the total benefits from pollutant reductions in each country. Scenarios are examined where the above-mentioned countries improve ambient conditions for the pollutants in question to meet the European Community standards and then compare these scenarios to ones involving uniform percentage ambient reductions across locations in each country. 3 figs., 9 tabs., 33 refs.

  7. Technical comments on EPA`s proposed revisions to the National Ambient Air Quality Standard for particulate matter

    Energy Technology Data Exchange (ETDEWEB)

    Lipfert, F.W.

    1997-03-01

    The US Environmental Protection Agency (EPA) has proposed new ambient air quality standards specifically for fine particulate matter, regulating concentrations of particles with median aerodynamic diameters less than 2.5 {mu}m (PM{sub 2.5}). Two new standards have been proposed: a maximum 24-hr concentration that is intended to protect against acute health effects, and an annual concentration limit that is intended to protect against longer-term health effects. EPA has also proposed a slight relaxation of the 24-hr standard for inhalable particles (PM{sub 10}), by allowing additional exceedances each year. Fine particles are currently being indirectly controlled by means of regulations for PM{sub 10} and TSP, under the Clean Air Act of 1970 and subsequent amendments. Although routine monitoring of PM{sub 2.5} is rare and data are sparse, the available data indicate that ambient concentrations have been declining at about 6% per year under existing regulations.

  8. Impact of emissions from natural gas production facilities on ambient air quality in the Barnett Shale area: a pilot study.

    Science.gov (United States)

    Zielinska, Barbara; Campbell, Dave; Samburova, Vera

    2014-12-01

    Rapid and extensive development of shale gas resources in the Barnett Shale region of Texas in recent years has created concerns about potential environmental impacts on water and air quality. The purpose of this study was to provide a better understanding of the potential contributions of emissions from gas production operations to population exposure to air toxics in the Barnett Shale region. This goal was approached using a combination of chemical characterization of the volatile organic compound (VOC) emissions from active wells, saturation monitoring for gaseous and particulate pollutants in a residential community located near active gas/oil extraction and processing facilities, source apportionment of VOCs measured in the community using the Chemical Mass Balance (CMB) receptor model, and direct measurements of the pollutant gradient downwind of a gas well with high VOC emissions. Overall, the study results indicate that air quality impacts due to individual gas wells and compressor stations are not likely to be discernible beyond a distance of approximately 100 m in the downwind direction. However, source apportionment results indicate a significant contribution to regional VOCs from gas production sources, particularly for lower-molecular-weight alkanes (gas production. Implications: Rapid and extensive development of shale gas resources in recent years has created concerns about potential environmental impacts on water and air quality. This study focused on directly measuring the ambient air pollutant levels occurring at residential properties located near natural gas extraction and processing facilities, and estimating the relative contributions from gas production and motor vehicle emissions to ambient VOC concentrations. Although only a small-scale case study, the results may be useful for guidance in planning future ambient air quality studies and human exposure estimates in areas of intensive shale gas production.

  9. The nationwide survey of the level of PCDD/Fs in ambient air in Taiwan between 2002 and 2003

    Energy Technology Data Exchange (ETDEWEB)

    Lee Tzu-Yi; Yuan-Wu Chen; Ying-Ming Weng [EAL, EPA, TW (China)

    2004-09-15

    Taiwan is a solitary island on the western edge of the Pacific Ocean. Incineration is the major way for waste treatment in Taiwan. EPA of the ROC government has planed to build 30 municipal solid waste incinerators MSWIs. Currently, there are 19 MSWIs in operation with a daily treatment capacity of 21,000 tons. The emission of PCDD/Fs from MSWIs has been of great concern from the public. Therefore, large-scale surveys over the PCDD/Fs in ambient air were focused largely on the vicinity of MSWIs in the last three years2. There were only several small-scale projects for ordinary areas were implemented in northern and southern Taiwan. The EPA started to set up the Taiwan Air Quality Monitoring Network TAQMN in 1990. For now, there are 72 air quality monitoring stations, including 58 ordinary ambient air stations, 5 traffic pattern stations, 4 background pattern stations, 3 industrial pattern stations and 2 national park pattern stations. The priority pollutants being monitored in TAQMN include PM10, sulfur dioxides, nitrogen oxides, carbon monoxide, ozone, and hydrocarbons. Besides, it also records several meteorological conditions. These stations were set up after proper evaluation and can well represent the air quality in the vicinity areas. The most recent data for the concentration of PCDD/Fs in ambient air have shown a trend of deceasing level in many areas, but have not been reported in Taiwan. Therefore, in this study, EAL selected 16 TAQMN monitoring stations as sampling sites and launched this nationwide survey from 2002 to 2003.

  10. The impact of European measures to reduce air pollutants on air quality, human health and climate

    Science.gov (United States)

    Turnock, S.; Butt, E. W.; Richardson, T.; Mann, G.; Forster, P.; Haywood, J. M.; Crippa, M.; Janssens-Maenhout, G. G. A.; Johnson, C.; Bellouin, N.; Spracklen, D. V.; Carslaw, K. S.; Reddington, C.

    2015-12-01

    European air quality legislation has reduced emissions of air pollutants across Europe since the 1970s, resulting in improved air quality and benefits to human health but also an unintended impact on regional climate. Here we used a coupled chemistry-climate model and a new policy relevant emission scenario to determine the impact of air pollutant emission reductions over Europe. The emission scenario shows that a combination of technological improvements and end-of-pipe abatement measures in the energy, industrial and road transport sectors reduced European emissions of sulphur dioxide, black carbon and organic carbon by 53%, 59% and 32% respectively. We estimate that these emission reductions decreased European annual mean concentrations of fine particulate matter (PM2.5) by 35%, sulphate by 44%, black carbon (BC) by 56% and particulate organic matter (POM) by 23%. The reduction in PM2.5 concentrations is calculated to have prevented 107,000 (40,000-172,000, 5-95% confidence intervals) premature deaths annually from cardiopulmonary disease and lung cancer across the EU member states. The decrease in aerosol concentrations caused a positive all-sky aerosol radiative forcing at the top of atmosphere over Europe of 2.3±0.06 W m-2 and a positive clear-sky forcing of 1.7±0.05 W m-2. Additionally, the amount of solar radiation incident at the surface over Europe increased by 3.3±0.07 W m-2 under all-sky and by 2.7±0.05 W m-2 under clear-sky conditions. Reductions in BC concentrations caused a 1 Wm-2 reduction in atmospheric absorption. We use an energy budget approximation to show that the aerosol induced radiative changes caused both temperature and precipitation to increase globally and over Europe. Our results show that the implementation of European legislation to reduce the emission of air pollutants has improved air quality and human health over Europe, as well as altered the regional radiative balance and climate.

  11. Exposure to genotoxins present in ambient air in Bangkok, Thailand - particle associated polycyclic aromatic hydrocarbons and biomarkers

    DEFF Research Database (Denmark)

    Ruchirawat, Mathuros; Mahidol, Chulabhorn; Tangjarukij, Chanthana

    2002-01-01

    Exposure to genotoxic compounds in ambient air has been studied in Bangkok, Thailand, by analysis of polycyclic aromatic hydrocarbons (PAHs) associated with particles and using different biomarkers of exposure. Eighty-nine male, non-smoking Royal Thai police officers were investigated. The police...... of individual PAHs or total PAH. Our data show, that people in Bangkok, who spend most of the day outside air-conditioned offices, are exposed to high levels of genotoxic PAHs. However, for people who spend their working day in offices, the exposure is similar to people living in other metropolitan areas....

  12. The association between low level exposures to ambient air pollution and term low birth weight: a retrospective cohort study

    Directory of Open Access Journals (Sweden)

    Stieb David

    2006-02-01

    Full Text Available Abstract Background Studies in areas with relatively high levels of air pollution have found some positive associations between exposures to ambient levels of air pollution and several birth outcomes including low birth weight (LBW. The purpose of this study was to examine the association between LBW among term infants and ambient air pollution, by trimester of exposure, in a region of lower level exposures. Methods The relationship between LBW and ambient levels of particulate matter up to 10 um in diameter (PM10, sulfur dioxide (SO2 and ground-level ozone (O3 was evaluated using the Nova Scotia Atlee Perinatal Database and ambient air monitoring data from the Environment Canada National Air Pollution Surveillance Network and the Nova Scotia Department of Environment. The cohort consisted of live singleton births (≥37 weeks of gestation between January1,1988 and December31,2000. Maternal exposures to air pollution were assigned to women living within 25 km of a monitoring station at the time of birth. Air pollution was evaluated as a continuous and categorical variable (using quartile exposures for each trimester and relative risks were estimated from logistic regression, adjusted for confounding variables. Results There were 74,284 women with a term, singleton birth during the study period and with exposure data. In the analyses unadjusted for year of birth, first trimester exposures in the highest quartile for SO2 and PM10suggested an increased risk of delivering a LBW infant (relative risk = 1.36, 95% confidence interval = 1.04 to 1.78 for SO2 exposure and relative risk = 1.33, 95% confidence interval = 1.02 to 1.74 for PM10. After adjustment for birth year, the relative risks were attenuated somewhat and not statistically significant. A dose-response relationship for SO2 was noted with increasing levels of exposure. No statistically significant effects were noted for ozone. Conclusion Our results suggest that exposure during the first

  13. Development of open air silicon deposition technology by silane-free atmospheric pressure plasma enhanced chemical transport under local ambient gas control

    Science.gov (United States)

    Naito, Teruki; Konno, Nobuaki; Yoshida, Yukihisa

    2016-07-01

    Open air silicon deposition was performed by combining silane-free atmospheric pressure plasma-enhanced chemical transport and a newly developed local ambient gas control technology. The effect of air contamination on silicon deposition was investigated using a vacuum chamber, and the allowable air contamination level was confirmed to be 3 ppm. The capability of the local ambient gas control head was investigated numerically and experimentally. A safe and clean process environment with air contamination less than 1 ppm was achieved. Combining these technologies, a microcrystalline silicon film was deposited in open air, the properties of which were comparable to those of silicon films deposited in a vacuum chamber.

  14. EMRP JRP MetNH3: Towards a Consistent Metrological Infrastructure for Ammonia Measurements in Ambient Air

    Science.gov (United States)

    Leuenberger, Daiana; Balslev-Harder, David; Braban, Christine F.; Ebert, Volker; Ferracci, Valerio; Gieseking, Bjoern; Hieta, Tuomas; Martin, Nicholas A.; Pascale, Céline; Pogány, Andrea; Tiebe, Carlo; Twigg, Marsailidh M.; Vaittinen, Olavi; van Wijk, Janneke; Wirtz, Klaus; Niederhauser, Bernhard

    2016-04-01

    Measuring ammonia in ambient air is a sensitive and priority issue due to its harmful effects on human health and ecosystems. In addition to its acidifying effect on natural waters and soils and to the additional nitrogen input to ecosystems, ammonia is an important precursor for secondary aerosol formation in the atmosphere. The European Directive 2001/81/EC on "National Emission Ceilings for Certain Atmospheric Pollutants (NEC)" regulates ammonia emissions in the member states. However, there is a lack of regulation regarding certified reference material (CRM), applicable analytical methods, measurement uncertainty, quality assurance and quality control (QC/QA) procedures as well as in the infrastructure to attain metrological traceability. As shown in a key comparison in 2007, there are even discrepancies between reference materials provided by European National Metrology Institutes (NMIs) at amount fraction levels up to three orders of magnitude higher than ambient air levels. MetNH3 (Metrology for ammonia in ambient air), a three-year project that started in June 2014 in the framework of the European Metrology Research Programme (EMRP), aims to reduce the gap between requirements set by the European emission regulations and state-of-the-art of analytical methods and reference materials. The overarching objective of the JRP is to achieve metrological traceability for ammonia measurements in ambient air from primary certified reference material CRM and instrumental standards to the field level. This requires the successful completion of the three main goals, which have been assigned to three technical work packages: To develop improved reference gas mixtures by static and dynamic gravimetric generation methods Realisation and characterisation of traceable preparative calibration standards (in pressurised cylinders as well as mobile generators) of ammonia amount fractions similar to those in ambient air based on existing methods for other reactive analytes. The

  15. Secondary Organic Aerosol Formation from Ambient Air in an Oxidation Flow Reactor at GoAmazon2014/5

    Science.gov (United States)

    Palm, Brett B.; de Sa, Suzane S.; Campuzano-Jost, Pedro; Day, Douglas A.; Hu, Weiwei; Seco, Roger; Park, Jeong-Hoo; Guenther, Alex; Kim, Saewung; Brito, Joel; Wurm, Florian; Artaxo, Paulo; Yee, Lindsay; Isaacman-VanWertz, Gabrial; Goldstein, Allen; Newburn, Matt K.; Lizabeth Alexander, M.; Martin, Scot T.; Brune, William H.; Jimenez, Jose L.

    2016-04-01

    During GoAmazon2014/5, ambient air was exposed to controlled concentrations of OH or O3 in situ using an oxidation flow reactor (OFR). Oxidation ranged from hours-several weeks of aging. Oxidized air was sampled by several instruments (e.g., HR-AMS, ACSM, PTR-TOF-MS, SMPS, CCN) at both the T3 site (IOP1: Feb 1-Mar 31, 2014, and IOP2: Aug 15-Oct 15, 2014) and T2 site (between IOPs and into 2nd IOP). The oxidation of ambient air in the OFR led to substantial and variable secondary organic aerosol (SOA) formation from any SOA-precursor gases, known and unknown, that entered the OFR. In general, more SOA was produced during the nighttime than daytime, suggesting that SOA-precursor gases were found in relatively higher concentrations at night. Similarly, more SOA was formed in the dry season (IOP2) than wet season (IOP1). The maximum amount of SOA produced during nighttime from OH oxidation ranged from less than 1 μg/m3 on some nights to greater than 10 μg/m3 on other nights. O3 oxidation of ambient air also led to SOA formation, although several times less than from OH oxidation. The amount of SOA formation sometimes, but not always, correlated with measured gas-phase biogenic and/or anthropogenic SOA precursors (e.g., SV-TAG sesquiterpenes, PTR-TOFMS aromatics, isoprene, and monoterpenes). The SOA mass formed in the OFR from OH oxidation was up to an order of magnitude larger than could be explained from aerosol yields of measured primary VOCs. This along with measurements from previous campaigns suggests that most SOA was formed from intermediate S/IVOC sources (e.g., VOC oxidation products, evaporated POA, or direct emissions). To verify the SOA yields of VOCs under OFR experimental conditions, atmospherically-relevant concentrations of several VOCs were added individually into ambient air in the OFR and oxidized by OH or O3. SOA yields in the OFR were similar to published chamber yields. Preliminary PMF factor analysis showed production of secondary factors in

  16. Transcriptome Profiling of the Lungs Reveals Molecular Clock Genes Expression Changes after Chronic Exposure to Ambient Air Particles

    Science.gov (United States)

    Song, Pengcheng; Li, Zhigang; Li, Xiaoqian; Yang, Lixin; Zhang, Lulu; Li, Nannan; Guo, Chen; Lu, Shuyu; Wei, Yongjie

    2017-01-01

    The symptoms of asthma, breathlessness, insomnia, etc. all have relevance to pulmonary rhythmic disturbances. Epidemiology and toxicology studies have demonstrated that exposure to ambient air particles can result in pulmonary dysfunction. However, there are no data directly supporting a link between air pollution and circadian rhythm disorder. In the present study, we found that breathing highly polluted air resulted in changes of the molecular clock genes expression in lung by transcriptome profiling analyses in a rodent model. Compared to those exposed to filtered air, in both pregnant and offspring rats in the unfiltered group, key clock genes (Per1, Per2, Per3, Rev-erbα and Dbp) expression level decreased and Bmal1 expression level increased. In both rat dams and their offspring, after continuous exposure to unfiltered air, we observed significant histologic evidence for both perivascular and peribronchial inflammation, increased tissue and systemic oxidative stress in the lungs. Our results suggest that chronic exposure to particulate matter can induce alterations of clock genes expression, which could be another important pathway for explaining the feedbacks of ambient particle exposure in addition to oxidative stress and inflammation. PMID:28106813

  17. Low-carbon energy policy and ambient air pollution in Shanghai, China. A health-based economic assessment

    Energy Technology Data Exchange (ETDEWEB)

    Chen, Changhong; Wang, Bingyan [Shanghai Academy of Environmental Sciences, Shanghai 200233 (China); Chen, Bingheng; Kan, Haidong [Department of Environmental Health, School of Public Health, Fudan University, Shanghai 200032 (China); Huang, Cheng; Zhao, Jing; Dai, Yi [East China University of Science and Technology, Shanghai 200237 (China)

    2007-02-01

    Energy and related health issues are of growing concern worldwide today. To investigate the potential public health and economic impact of ambient air pollution under various low-carbon energy scenarios in Shanghai, we estimated the exposure level of Shanghai residents to air pollution under various planned scenarios, and assessed the public health impact using concentration-response functions derived from available epidemiologic studies. We then estimated the corresponding economic values of the health effects based on unit values for each health outcome. Our results show that ambient air pollution in relation to low-carbon energy scenarios could have a significant impact on the future health status of Shanghai residents, both in physical and monetary terms. Compared with the base case scenario, implementation of various low-carbon energy scenarios could prevent 2804-8249 and 9870-23,100 PM{sub 10}-related avoidable deaths (mid-value) in 2010 and 2020, respectively. It could also decrease incidence of several relevant diseases. The corresponding economic benefits could reach 507.31-1492.33 and 2642.45-6192.11 million U.S. dollars (mid-value) in 2010 and 2020, respectively. These findings illustrate that a low-carbon energy policy will not only decrease the emission of greenhouse gases, but also play an active role in the reduction of air pollutant emissions, improvement of air quality, and promotion of public health. Our estimates can provide useful information to local decision-makers for further cost-benefit analysis. (author)

  18. Low-carbon energy policy and ambient air pollution in Shanghai, China: A health-based economic assessment

    Energy Technology Data Exchange (ETDEWEB)

    Chen Changhong [Shanghai Academy of Environmental Sciences, Shanghai 200233 (China); Chen Bingheng [Department of Environmental Health, School of Public Health, Fudan University, Shanghai 200032 (China); Wang Bingyan [Shanghai Academy of Environmental Sciences, Shanghai 200233 (China); Huang Cheng [East China University of Science and Technology, Shanghai 200237 (China); Zhao Jing [East China University of Science and Technology, Shanghai 200237 (China); Dai Yi [East China University of Science and Technology, Shanghai 200237 (China); Kan Haidong [Department of Environmental Health, School of Public Health, Fudan University, Shanghai 200032 (China)]. E-mail: haidongkan@gmail.com

    2007-02-01

    Energy and related health issues are of growing concern worldwide today. To investigate the potential public health and economic impact of ambient air pollution under various low-carbon energy scenarios in Shanghai, we estimated the exposure level of Shanghai residents to air pollution under various planned scenarios, and assessed the public health impact using concentration-response functions derived from available epidemiologic studies. We then estimated the corresponding economic values of the health effects based on unit values for each health outcome. Our results show that ambient air pollution in relation to low-carbon energy scenarios could have a significant impact on the future health status of Shanghai residents, both in physical and monetary terms. Compared with the base case scenario, implementation of various low-carbon energy scenarios could prevent 2804-8249 and 9870-23,100 PM{sub 10}-related avoidable deaths (mid-value) in 2010 and 2020, respectively. It could also decrease incidence of several relevant diseases. The corresponding economic benefits could reach 507.31-1492.33 and 2642.45-6192.11 million U.S. dollars (mid-value) in 2010 and 2020, respectively. These findings illustrate that a low-carbon energy policy will not only decrease the emission of greenhouse gases, but also play an active role in the reduction of air pollutant emissions, improvement of air quality, and promotion of public health. Our estimates can provide useful information to local decision-makers for further cost-benefit analysis.

  19. Influence of ambient air on the flowing afterglow of an atmospheric pressure Ar/O2 radiofrequency plasma

    CERN Document Server

    Duluard, C Y; Hubert, J; Reniers, F

    2016-01-01

    The influence of ambient air on the flowing afterglow of an atmospheric pressure Ar/O2 radiofrequency plasma has been investigated experimentally. Spatially resolved mass spectrometry and laser induced fluorescence on OH radicals were used to estimate the intrusion of air in between the plasma torch and the substrate as a function of the torch-to-substrate separation distance. No air is detected, within the limits of measurement uncertainties, for separation distances smaller than 5 mm. For larger distances, the effect of ambient air can no longer be neglected, and radial gradients in the concentrations of species appear. The Ar 4p population, determined through absolute optical emission spectroscopy, is seen to decrease with separation distance, whereas a rise in emission from the N2(C--B) system is measured. The observed decay in Ar 4p and N2(C) populations for separation distances greater than 9mm is partly assigned to the increasing collisional quenching rate by N2 and O2 molecules from the entrained air....

  20. Low-carbon energy policy and ambient air pollution in Shanghai, China: a health-based economic assessment.

    Science.gov (United States)

    Chen, Changhong; Chen, Bingheng; Wang, Bingyan; Huang, Cheng; Zhao, Jing; Dai, Yi; Kan, Haidong

    2007-02-01

    Energy and related health issues are of growing concern worldwide today. To investigate the potential public health and economic impact of ambient air pollution under various low-carbon energy scenarios in Shanghai, we estimated the exposure level of Shanghai residents to air pollution under various planned scenarios, and assessed the public health impact using concentration-response functions derived from available epidemiologic studies. We then estimated the corresponding economic values of the health effects based on unit values for each health outcome. Our results show that ambient air pollution in relation to low-carbon energy scenarios could have a significant impact on the future health status of Shanghai residents, both in physical and monetary terms. Compared with the base case scenario, implementation of various low-carbon energy scenarios could prevent 2804-8249 and 9870-23,100 PM10-related avoidable deaths (mid-value) in 2010 and 2020, respectively. It could also decrease incidence of several relevant diseases. The corresponding economic benefits could reach 507.31-1492.33 and 2642.45-6192.11 million U.S. dollars (mid-value) in 2010 and 2020, respectively. These findings illustrate that a low-carbon energy policy will not only decrease the emission of greenhouse gases, but also play an active role in the reduction of air pollutant emissions, improvement of air quality, and promotion of public health. Our estimates can provide useful information to local decision-makers for further cost-benefit analysis.

  1. Transcriptome Profiling of the Lungs Reveals Molecular Clock Genes Expression Changes after Chronic Exposure to Ambient Air Particles

    Directory of Open Access Journals (Sweden)

    Pengcheng Song

    2017-01-01

    Full Text Available The symptoms of asthma, breathlessness, insomnia, etc. all have relevance to pulmonary rhythmic disturbances. Epidemiology and toxicology studies have demonstrated that exposure to ambient air particles can result in pulmonary dysfunction. However, there are no data directly supporting a link between air pollution and circadian rhythm disorder. In the present study, we found that breathing highly polluted air resulted in changes of the molecular clock genes expression in lung by transcriptome profiling analyses in a rodent model. Compared to those exposed to filtered air, in both pregnant and offspring rats in the unfiltered group, key clock genes (Per1, Per2, Per3, Rev-erbα and Dbp expression level decreased and Bmal1 expression level increased. In both rat dams and their offspring, after continuous exposure to unfiltered air, we observed significant histologic evidence for both perivascular and peribronchial inflammation, increased tissue and systemic oxidative stress in the lungs. Our results suggest that chronic exposure to particulate matter can induce alterations of clock genes expression, which could be another important pathway for explaining the feedbacks of ambient particle exposure in addition to oxidative stress and inflammation.

  2. Ambient Air Pollution Exposure and Respiratory, Cardiovascular and Cerebrovascular Mortality in Cape Town, South Africa: 2001–2006

    Directory of Open Access Journals (Sweden)

    Kuku Voyi

    2012-11-01

    Full Text Available Little evidence is available on the strength of the association between ambient air pollution exposure and health effects in developing countries such as South Africa. The association between the 24-h average ambient PM10, SO2 and NO2 levels and daily respiratory (RD, cardiovascular (CVD and cerebrovascular (CBD mortality in Cape Town (2001–2006 was investigated with a case-crossover design. For models that included entire year data, an inter-quartile range (IQR increase in PM10 (12 mg/m3 and NO2 (12 mg/m3 significantly increased CBD mortality by 4% and 8%, respectively. A significant increase of 3% in CVD mortality was observed per IQR increase in NO2 and SO2 (8 mg/m3. In the warm period, PM10 was significantly associated with RD and CVD mortality. NO2 had significant associations with CBD, RD and CVD mortality, whilst SO2 was associated with CVD mortality. None of the pollutants were associated with any of the three outcomes in the cold period. Susceptible groups depended on the cause-specific mortality and air pollutant. There is significant RD, CVD and CBD mortality risk associated with ambient air pollution exposure in South Africa, higher than reported in developed countries.

  3. Energy requirements for CO2 capture from ambient air (DAC) competitive with capture from flue-gas (PCC)

    Science.gov (United States)

    Meinrenken, Christoph

    2015-03-01

    Capture of CO2, whether from a flue gas source (PCC) or from distributed sources via ambient air (DAC), is a key enabling technology to provide carbon for sustainable synthetic energy carriers such as solar fuels. Based on thermodynamic minimum considerations, DAC is often expected to require about 3 times more energy (per ton CO2 captured) than PCC because CO2 in ambient air is more dilute. Here, we calculate the energy required for a humidity swing-based DAC installation that uses an anionic exchange resin as sorbent. The calculation uses recently measured equilibrium CO2 loadings of the sorbent as function of partial CO2 pressure, temperature, and humidity. We calculate the installation's electricity consumption to be about 45 kJ per mole of pure CO2 at 1 bar (scenario-dependent). Furthermore, we estimate the amount of heat provided by ambient air and thus provide context of the overall energy and entropy balance and thermodynamic minimum views. The electricity consumption is competitive with typical parasitic loads of PCC-equipped coal-fired power plants (40-50 kJ per mole at same pressure) and significantly lower than predicted for other DAC installations such as Na(OH) sorbent-based systems. Our analyses elucidate why DAC is not always more energy-intensive that PCC, thus alleviating often cited concerns of significant cost impediments. Financial support by ABB for research presented herein is gratefully acknowledged.

  4. U.S. Air Quality and Health Benefits from Avoided Climate Change under Greenhouse Gas Mitigation.

    Science.gov (United States)

    Garcia-Menendez, Fernando; Saari, Rebecca K; Monier, Erwan; Selin, Noelle E

    2015-07-07

    We evaluate the impact of climate change on U.S. air quality and health in 2050 and 2100 using a global modeling framework and integrated economic, climate, and air pollution projections. Three internally consistent socioeconomic scenarios are used to value health benefits of greenhouse gas mitigation policies specifically derived from slowing climate change. Our projections suggest that climate change, exclusive of changes in air pollutant emissions, can significantly impact ozone (O3) and fine particulate matter (PM2.5) pollution across the U.S. and increase associated health effects. Climate policy can substantially reduce these impacts, and climate-related air pollution health benefits alone can offset a significant fraction of mitigation costs. We find that in contrast to cobenefits from reductions to coemitted pollutants, the climate-induced air quality benefits of policy increase with time and are largest between 2050 and 2100. Our projections also suggest that increasing climate policy stringency beyond a certain degree may lead to diminishing returns relative to its cost. However, our results indicate that the air quality impacts of climate change are substantial and should be considered by cost-benefit climate policy analyses.

  5. Severe and Moderate Asthma Exacerbations in Asthmatic Children and Exposure to Ambient Air Pollutants

    Science.gov (United States)

    Tétreault, Louis-Francois; Doucet, Marieve; Gamache, Philippe; Fournier, Michel; Brand, Allan; Kosatsky, Tom; Smargiassi, Audrey

    2016-01-01

    Background: It is well established that short-term exposure to ambient air pollutants can exacerbate asthma, the role of early life or long-term exposure is less clear. We assessed the association between severe asthma exacerbations with both birth and annual exposure to outdoor air pollutants with a population-based cohort of asthmatic children in the province of Quebec (Canada). Method: Exacerbations of asthma occurring between 1 April 1996 and 31 March 2011 were defined as one hospitalization or emergency room visit with a diagnosis of asthma for children (<13 years old) already diagnosed with asthma. Annual daily average concentrations of ozone (O3) and nitrogen dioxide (NO2) were estimated at the child’s residential postal code. Satellite based levels of fine particulate (PM2.5) estimated for a grid of 10 km by 10 km were also assigned to postal codes of residence for the whole province. Hazard ratios (HRs) were estimated from Cox models with a gap time approach for both birth and time-dependant exposure. Results: Of the 162,752 asthmatic children followed (1,020,280 person-years), 35,229 had at least one asthma exacerbation. The HRs stratified by age groups and adjusted for the year of birth, the ordinal number of exacerbations, sex, as well as material and social deprivation, showed an interquartile range increase in the time-dependant exposure to NO2 (4.95 ppb), O3 (3.85 ppb), and PM2.5 (1.82 μg/m3) of 1.095 (95% CI 1.058–1.131), 1.052 (95% CI 1.037–1.066) and 1.025 (95% CI 1.017–1.031), respectively. While a positive association was found to PM2.5, no associations were found between exposure at birth to NO2 or O3. Conclusions: Our results support the conclusion, within the limitation of this study, that asthma exacerbations in asthmatic children are mainly associated with time dependent residential exposures less with exposure at birth. PMID:27490556

  6. Estimating Personal Exposures from Ambient Air Pollution Measures - Using Meta-Analysis to Assess Measurement Error

    Science.gov (United States)

    Although ambient concentrations of particulate matter ≤ 10μm (PM10) are often used as proxies for total personal exposure, correlation (r) between ambient and personal PM10 concentrations varies. Factors underlying this variation and its effect on he...

  7. Air pollution-related health and climate benefits of clean cookstove programs in Mozambique

    Science.gov (United States)

    Anenberg, Susan C.; Henze, Daven K.; Lacey, Forrest; Irfan, Ans; Kinney, Patrick; Kleiman, Gary; Pillarisetti, Ajay

    2017-02-01

    Approximately 95% of households in Mozambique burn solid fuels for cooking, contributing to elevated indoor and outdoor fine particulate matter (PM2.5) concentrations and subsequent health and climate impacts. Little is known about the potential health and climate benefits of various approaches for expanding the use of cleaner stoves and fuels in Mozambique. We use state-of-the-science methods to provide a first-order estimation of potential air pollution-related health and climate benefits of four illustrative scenarios in which traditional cooking fires and stoves are displaced by cleaner and more efficient technologies. For rural areas, we find that a 10% increase in the number of households using forced draft wood-burning stoves could achieve >2.5 times more health benefits from reduced PM2.5 exposure (200 avoided premature deaths and 14 000 avoided disability adjusted life years, DALYs, over a three-year project lifetime) compared to natural draft stoves in the same households, assuming 70% of households use the new technology for both cases. Expanding use of LPG stoves to 10% of households in five major cities is estimated to avoid 160 premature deaths and 11 000 DALYs from reduced PM2.5 exposure for a three-year intervention, assuming 60% of households use the new stove. Advanced charcoal stoves would achieve ∽80% of the PM2.5-related health benefits of LPG stoves. Approximately 2%–5% additional health benefits would result from reduced ambient PM2.5, depending on the scenario. Although climate impacts are uncertain, we estimate that all scenarios would reduce expected climate change-related temperature increases from continued solid fuel use by 4%–6% over the next century. All results are based on an assumed adjustment factor of 0.8 to convert from laboratory-based emission reduction measurements to exposure reductions, which could be optimistic in reality given potential for continued use of the traditional stove. We conclude that cleaner cooking

  8. Controlled environment laboratory for the energy certification of refrigeration and air conditioning systems; Laboratorio de ambiente controlado para la certificacion energetica de sistemas de refrigeracion y aire acondicionado

    Energy Technology Data Exchange (ETDEWEB)

    Ambriz, Juan Jose; Romero Paredes, Hernando; Dorantes, Ruben [Universidad Autonoma Metropolitana, Mexico, D.F. (Mexico)

    1999-07-01

    In this paper the general characteristics of the Controlled Environment Laboratory (CELAB) are described and some of the possible tests that could be performed in this device to evaluate the energy efficiency in air conditioning systems, domestic refrigeration and industrial refrigeration, as well as tests to evaluate the hydrothermal comfort in national populations, are presented. [Spanish] En este trabajo se describen las caracteristicas generales del Laboratorio de Ambiente Controlado (LAB), y se presentan algunas de las posibles pruebas que podran ser desarrolladas en este dispositivo para evaluar la eficiencia energetica en sistemas de aire acondicionado, refrigeracion domestica y refrigeracion industrial, asi como para pruebas para evaluar el confort hidrotermico en poblaciones nacionales.

  9. Integrated effects of air pollution and climate change on forests: a northern hemisphere perspective.

    Science.gov (United States)

    Bytnerowicz, Andrzej; Omasa, Kenji; Paoletti, Elena

    2007-06-01

    Many air pollutants and greenhouse gases have common sources, contribute to radiative balance, interact in the atmosphere, and affect ecosystems. The impacts on forest ecosystems have been traditionally treated separately for air pollution and climate change. However, the combined effects may significantly differ from a sum of separate effects. We review the links between air pollution and climate change and their interactive effects on northern hemisphere forests. A simultaneous addressing of the air pollution and climate change effects on forests may result in more effective research, management and monitoring as well as better integration of local, national and global environmental policies.

  10. Impact of Climate Change on Air Quality and Public Health in Urban Areas.

    Science.gov (United States)

    Hassan, Noor Artika; Hashim, Zailina; Hashim, Jamal Hisham

    2016-03-01

    This review discusses how climate undergo changes and the effect of climate change on air quality as well as public health. It also covers the inter relationship between climate and air quality. The air quality discussed here are in relation to the 5 criteria pollutants; ozone (O3), carbon dioxide (CO2), nitrogen dioxide (NO2), sulfur dioxide (SO2), and particulate matter (PM). Urban air pollution is the main concern due to higher anthropogenic activities in urban areas. The implications on health are also discussed. Mitigating measures are presented with the final conclusion.

  11. State of the Climate Monthly Overview - Upper Air

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — The State of the Climate is a collection of periodic summaries recapping climate-related occurrences on both a global and national scale. The State of the Climate...

  12. Energy efficient air-conditioning technology for a healthier climate; Energieeffiziente Klimatechnik fuer ein gesundes Raumklima

    Energy Technology Data Exchange (ETDEWEB)

    Hartl, Thorsten [ebm-papst Motoren und Ventilatoren GmbH, St. Florian (Austria)

    2011-07-01

    Since climate and indoor air quality have a great impact on concentration, health and well being, it is important to provide good indoor air for example in classrooms. The use of air conditioning equipment enables an optimal air-conditioning, whether in new buildings or building alterations or renovations. Energy-saving EC fans in these air conditioning systems provide an efficient and quiet ventilation meeting the requirements. Thus, the contribution under consideration reports on centrifugal fans.

  13. Association between exposure to ambient air pollution before conception date and likelihood of giving birth to girls in Guangzhou, China

    Science.gov (United States)

    Lin, Hualiang; Liang, Zhijiang; Liu, Tao; Di, Qian; Qian, Zhengmin; Zeng, Weilin; Xiao, Jianpeng; Li, Xing; Guo, Lingchuan; Ma, Wenjun; Zhao, Qingguo

    2015-12-01

    A few studies have linked ambient air pollution with sex ratio at birth. Most of these studies examined the long-term effects using spatial or temporal comparison approaches. This study aimed to investigate whether parental exposure to air pollution before conception date could affect the likelihood of the offspring being male or female. We used the information collected in a major maternal hospital in Guangzhou, China. The parental exposure to air pollution was assessed using the air pollution concentration before the conception date. Logistic regression models were used to assess the association between air pollution exposure and birth sex with adjustment for potential confounding factors, such as maternal age, parental education levels, long-term trend, season, and weather condition (mean temperature and relative humidity). The analysis revealed that higher air pollution was associated with higher probability of female newborns, with the effective exposure around one week prior to conception date. In the one-pollutant models, PM10, SO2 and NO2 had significant effects. For example, the excess risk was 0.61% (95% confidence interval (95% CI): 0.36%, 0.86%) for a 10 ug/m3 increase in lag 2 day's PM10, 0.42% (95% CI: 0.21%, 0.64%) for lag 3 day's SO2 and 0.97% (95% CI: 0.44%, 1.50%) for lag 3 day's NO2; and in two-pollutant models, PM10 remained statistically significant. These results suggest that parental exposure to ambient air pollution a few days prior to conception might be a contributing factor to higher probability of giving birth to female offspring in Guangzhou.

  14. An integrated assessment of regional air pollution and climate change in Europe: findings of the AIR-CLIM project

    NARCIS (Netherlands)

    Alcamo, J.; Mayerhofer, P.; Guardans, R.; Harmelen, T. van; Minnen, J. van; Onigkeit, J.; Posch, M.; Vries, B. de

    2002-01-01

    This paper presents results of an assessment of the linkages between regional air pollution and climate change in Europe (the AIR-CLIM Project). The main research tool was an integrated modeling framework and the main product was a consistent set of long-term scenarios covering Europe between 1995 a

  15. Do US Ambient Air Lead Levels Have a Significant Impact on Childhood Blood Lead Levels: Results of a National Study

    Directory of Open Access Journals (Sweden)

    LuAnn L. Brink

    2013-01-01

    Full Text Available Introduction. Although lead paint and leaded gasoline have not been used in the US for thirty years, thousands of US children continue to have blood lead levels (BLLs of concern. Methods. We investigated the potential association of modeled air lead levels and BLLs ≥ 10 μg/dL using a large CDC database with BLLs on children aged 0–3 years. Percent of children with BLLs ≥ 10 μg/dL (2000–2007 by county and proportion of pre-50 housing and SES variables were merged with the US EPA's National Air Toxics Assessment (NATA modeled air lead data. Results. The proportion with BLL ≥ 10 μg/dL was 1.24% in the highest air lead counties, and the proportion with BLL ≥ 10 μg/dL was 0.36% in the lowest air lead counties, resulting in a crude prevalence ratio of 3.4. Further analysis using multivariate negative binomial regression revealed that NATA lead was a significant predictor of % BLL ≥ 10 μg/dL after controlling for percent pre-l950 housing, percent rural, and percent black. A geospatial regression revealed that air lead, percent older housing, and poverty were all significant predictors of % BLL ≥ 10 μg/dL. Conclusions. More emphasis should be given to potential sources of ambient air lead near residential areas.

  16. Health effects of tropospheric ozone: Review of recent research findings and their implications to ambient air quality standards

    Energy Technology Data Exchange (ETDEWEB)

    Lippmann, M. (New York Univ. Medical Center, Tuxedo (United States))

    1993-01-01

    The US Environmental Protection Agency (EPA) Administrator proposed (on August 3, 1992) to retain the current National Ambient Air Quality Standard (NAAQS) for ozone (O3) on the basis of data assembled in a draft Criteria Document (1986) and its Addendum (1988) which, together with a draft Staff Paper (1988), received public comment and review comments by the EPA's Clean Air Scientific Advisory Committee (CASAC). This paper summarizes and discusses research findings presented since 1988 which, based on the author's experience as a Chairman of CASAC, are most relevant to the promulgation of a primary (health based) NAAQS for O3. These newer findings include substantial evidence from controlled chamber exposure studies and field studies in natural settings that the current NAAQS contains no margin of safety against short-term effects that the EPA has considered to be adverse. They also include evidence from epidemiologic studies that current ambient exposures are associated with reduced baseline lung function, exacerbation of asthma and premature mortality, as well as evidence from chronic animal exposure studies at concentrations within current ambient peak levels that indicate progressive and persistent lung function and structural abnormalities. The current NAAQS, if retained, may therefore also be inadequate to protect the public from effects resulting from chronic exposure to O3. 96 refs.

  17. Indicative levels of PM in the ambient air in the surrounding villages of the copper smelter complex Bor, Serbia

    Directory of Open Access Journals (Sweden)

    Tasić Viša

    2012-01-01

    Full Text Available While information on air pollution in the form of particulate matter (PM has been monitored for longer period for EU countries, availability of PM data sets in the Western Balkan countries including the Republic of Serbia are still limited. Studies, related to the particulate pollution research, have been only carried out in the past several years. The main objective of this paper is to present PM levels measured in the ambient air in the surrounding settlements of the Copper Smelter Complex Bor. Also, one of the goals is a comparison of PM levels in the surrounding settlements with those measured in Bor town. The ambient levels of PM particles (PM10, PM2.5 were measured by automatic PM monitors at 4 nearby settlements: Slatina, Oštrelj, Krivelj and Brezonik in the time interval from 2005 to 2010. According to the measurement results, PM10 and PM2.5 levels in the ambient air were higher in the cold, heating, (October-March than in the warm no heating period (April-September. The exceeding of the daily limit of PM10 and PM2.5 mass concentration levels was observed at all measuring points. A higher number of exceedances were detected in the cold period. The results indicate that there is a significant seasonal change in the level of fine particles at all measuring places in surroundings. In addition, the PM levels in Bor town are more influenced by the air pollution from the Copper Smelter Complex than settlements in the vicinity, where the PM concentrations were greatly influenced by the presence of domestic heating in the cold period. [Projekat Ministarstva nauka Republike Srbije, br. III42008: Evaluation of Energy Performances and Indoor Environment Quality of Educational Buildings in Serbia with Impact to Health i br. III41028: “An Integral Study to Identify the Regional Genetic and Environmental Risk Factors for the Common Noncommunicable Diseases in the Human Population of Serbia

  18. Exposure to ambient concentrations of particulate air pollution does not influence vascular function or inflammatory pathways in young healthy individuals

    DEFF Research Database (Denmark)

    Bräuner, E. V.; Møller, P.; Barregård, L.;

    2008-01-01

    : 11600 +/- 5600 per cm(3), mass concentrations: 13.8 +/- 7.4 mu g/m(3) and 10.5 +/- 4.8 mu g/m(3) for PM10-2.5 and PM2.5, respectively) or particle filtered (NC: 555 +/- 1053 per cm(3)) air collected above a busy street. Microvascular function was assessed non-invasively by measuring digital peripheral......Background: Particulate air pollution is associated with increased risk of cardiovascular events although the involved mechanisms are poorly understood. The objective of the present study was to investigate the effects of controlled exposure to ambient air fine and ultrafine particles...... on microvascular function and biomarkers related to inflammation, haemostasis and lipid and protein oxidation. Methods: Twenty-nine subjects participated in a randomized, two-factor crossover study with or without biking exercise for 180 minutes and with 24 hour exposure to particle rich (number concentrations, NC...

  19. Ambient air/near-field measurements of methane and Volatile Organic Compounds (VOCs) from a natural gas facility in Northern Europe

    Science.gov (United States)

    Baudic, Alexia; Gros, Valérie; Bonsang, Bernard; Baisnee, Dominique; Vogel, Félix; Yver Kwok, Camille; Ars, Sébastien; Finlayson, Andrew; Innocenti, Fabrizio; Robinson, Rod

    2015-04-01

    Since the 1970's, the natural gas consumption saw a rapid growth in large urban centers, thus becoming an important energy resource to meet continuous needs of factories and inhabitants. Nevertheless, it can be a substantial source of methane (CH4) and pollutants in urban areas. For instance, we have determined that about 20% of Volatile Organic Compounds (VOCs) in downtown Paris are originating from this emission source (Baudic, Gros et al., in preparation). Within the framework of the "Fugitive Methane Emissions" (FuME) project (Climate-KIC, EIT); 2-weeks gas measurements were conducted at a gas compressor station in Northern Europe. Continuous ambient air measurements of methane and VOCs concentrations were performed using a cavity ring-down spectrometer (model G2201, Picarro Inc., Santa Clara, USA) and two portable GC-FID (Chromatotec, Saint-Antoine, France), respectively. On-site near-field samplings were also carried out at the source of two pipelines using stainless steel flasks (later analyzed with a laboratory GC-FID). The objective of this study aims to use VOCs as additional tracers in order to better characterize the fugitive methane emissions in a complex environment, which can be affected by several urban sources (road-traffic, others industries, etc.). Moreover, these measurements have allowed determining the chemical composition of this specific source. Our results revealed that the variability of methane and some VOCs was (rather) well correlated, especially for alkanes (ethane, propane, etc.). An analysis of selected events with strong concentrations enhancement was performed using ambient air measurements; thus allowing the preliminary identification of different emission sources. In addition, some flasks were also sampled in Paris to determine the local natural gas composition. A comparison between both was then performed. Preliminary results from these experiments will be presented here.

  20. European atmosphere in 2050, a regional air quality and climate perspective under CMIP5 scenarios

    Directory of Open Access Journals (Sweden)

    A. Colette

    2013-03-01

    Full Text Available To quantify changes in air pollution in Europe at the 2050 horizon, we designed a comprehensive modelling system that captures the external factors considered to be most relevant and relies on up-to-date and consistent sets of air pollution and climate policy scenarios. Global and regional climate as well as global chemistry simulations are based on the recent Representative Concentrations Pathways (RCP produced for the Fifth Assessment Report (AR5 of IPCC whereas regional air quality modelling is based on the updated emissions scenarios produced in the framework of the Global Energy Assessment. We explored two diverse scenarios: a reference scenario where climate policies are absent and a mitigation scenario which limits global temperature rise to within 2 °C by the end of this century. This first assessment of projected air quality and climate at the regional scale based on CMIP5 (5th Climate Model Intercomparison Project climate simulations is in line with the existing literature using CMIP3. The discrepancy between air quality simulations obtained with a climate model or with meteorological reanalyses is pointed out. Sensitivity simulations show that the main factor driving future air quality projections is air pollutant emissions, rather than climate change or long range transport. Whereas the well documented "climate penalty" bearing upon ozone over Europe is confirmed, other features appear less robust compared to the literature: such as the impact of climate on PM2.5. The quantitative disentangling of each contributing factor shows that the magnitude of the ozone climate penalty has been overstated in the past while on the contrary the contribution of the global ozone burden is overlooked in the literature.

  1. European atmosphere in 2050, a regional air quality and climate perspective under CMIP5 scenarios

    Directory of Open Access Journals (Sweden)

    A. Colette

    2013-08-01

    Full Text Available To quantify changes in air pollution over Europe at the 2050 horizon, we designed a comprehensive modelling system that captures the external factors considered to be most relevant, and that relies on up-to-date and consistent sets of air pollution and climate policy scenarios. Global and regional climate as well as global chemistry simulations are based on the recent representative concentration pathways (RCP produced for the Fifth Assessment Report (AR5 of the IPCC (Intergovernmental Panel on Climate Change whereas regional air quality modelling is based on the updated emissions scenarios produced in the framework of the Global Energy Assessment. We explored two diverse scenarios: a reference scenario where climate policies are absent and a mitigation scenario which limits global temperature rise to within 2 °C by the end of this century. This first assessment of projected air quality and climate at the regional scale based on CMIP5 (5th Coupled Model Intercomparison Project climate simulations is in line with the existing literature using CMIP3. The discrepancy between air quality simulations obtained with a climate model or with meteorological reanalyses is pointed out. Sensitivity simulations show that the main factor driving future air quality projections is air pollutant emissions, rather than climate change or intercontinental transport of pollution. Whereas the well documented "climate penalty" that weights upon ozone (increase of ozone pollution with global warming over Europe is confirmed, other features appear less robust compared to the literature, such as the impact of climate on PM2.5. The quantitative disentangling of external factors shows that, while several published studies focused on the climate penalty bearing upon ozone, the contribution of the global ozone burden is somewhat overlooked in the literature.

  2. Long-term ambient air pollution exposure and risk of high blood pressure among citizens in Nis, Serbia.

    Science.gov (United States)

    Stanković, Aleksandra; Nikolić, Maja

    2016-01-01

    Epidemiological studies suggest that long-term exposure to air pollution increases the risk for high blood pressure (BP). The aim of our study is to evaluate any effects in BP in citizens exposed to long-term ambient air pollution. The subjects are 1136 citizens, aged 18-70 years, living for more than 5 years in the same home in the areas with a different level of air pollution. The air concentrations of black smoke and sulfur dioxide were determined in the period from 2001 to 2011. We measured systolic and diastolic BP and heart rate. Multivariate methods were used in the analysis. Alcohol consumption had the greatest influence on the incidence of hypertension as a risk factor (RR: 3.461; 95% CI: 1.72-6.93) and age had the least (RR: 1.23; 95% CI: 1.183-1.92). Exposure to air pollution increases risk for developing hypertension 2.5 times (95% CI: 1.46-4.49). Physical activity has proved to be statistically significant protective factor for the development of hypertension. Long-term exposure to low levels of main air pollutants is significantly associated with elevated risk of hypertension.

  3. Urban Climate Effects on Air Pollution and Atmospheric Chemistry

    Science.gov (United States)

    Rasoul, Tara; Bloss, William; Pope, Francis

    2016-04-01

    Tropospheric ozone, adversely affects the environment and human health. The presence of chlorine nitrate (ClNO2) in the troposphere can enhance ozone (O3) formation as it undergoes photolysis, releasing chlorine reactive atoms (Cl) and nitrogen dioxide (NO2), both of which enhance tropospheric ozone formation. The importance of new sources of tropospheric ClNO2 via heterogeneous processes has recently been highlighted. This study employed a box model, using the Master Chemical Mechanism (MCM version 3.2) to assess the effect of ClNO2 on air quality in urban areas within the UK. The model updated to include ClNO2 production, photolysis, a comprehensive parameterisation of dinitrogen pentoxide (N2O5) uptake, and ClNO2 production calculated from bulk aerosol composition. The model simulation revealed the presence of ClNO2 enhances the formation of NO2, organic peroxy radical (CH3O2), O3, and hydroxyl radicals (OH) when compared with simulations excluding ClNO2. In addition, the study examined the effect of temperature variation upon ClNO2 formation. The response of ClNO2 to temperature was analysed to identify the underlying drivers, of particular importance when assessing the response of atmospheric chemistry processes under potential future climates.

  4. Tackling air pollution and extreme climate changes in China: Implementing the Paris climate change agreement.

    Science.gov (United States)

    Tambo, Ernest; Duo-Quan, Wang; Zhou, Xiao-Nong

    2016-10-01

    China still depends on coal for more than 60% of its power despite big investments in the process of shifting to nuclear, solar and wind power renewable energy resources alignment with Paris climate change agreement (Paris CCA). Chinese government through the Communist Party Central Committee (CPCC) ascribes great importance and commitment to Paris CCA legacy and history landmark implementation at all levels. As the world's biggest carbon dioxide emitter, China has embarked on "SMART" pollution and climate changes programs and measures to reduce coal-fired power plants to less than 50% in the next five years include: new China model of energy policies commitment on CO2 and greenhouse gas emissions reductions to less than 20% non-fossil energy use by 2030 without undermining their economic growth, newly introduced electric vehicles transportation benefits, interactive and sustained air quality index (AQI) monitoring systems, decreasing reliance on fossil fuel economic activities, revision of energy price reforms and renewable energy to less energy efficient technologies development. Furthermore, ongoing CPCC improved environmental initiatives, implemented strict regulations and penalties on local companies and firms' pollution production management, massive infrastructures such as highways to reduce CO2 expansion of seven regional emissions trading markets and programs for CO2 emissions and other pollutants are being documented. Maximizing on the centralized nature of the China's government, implemented Chinese pollution, climate changes mitigation and adaptation initiatives, "SMART" strategies and credible measures are promising. A good and practical example is the interactive and dynamic website and database covering 367 Chinese cities and providing real time information on environmental and pollution emissions AQI. Also, water quality index (WQI), radiation and nuclear safety monitoring and management systems over time and space. These are ongoing Chinese

  5. Impacts of Ozone-vegetation Interactions and Biogeochemical Feedbacks on Atmospheric Composition and Air Quality Under Climate Change

    Science.gov (United States)

    Sadeke, M.; Tai, A. P. K.; Lombardozzi, D.; Val Martin, M.

    2015-12-01

    Surface ozone pollution is one of the major environmental concerns due to its damaging effects on human and vegetation. One of the largest uncertainties of future surface ozone prediction comes from its interaction with vegetation under a changing climate. Ozone can be modulated by vegetation through, e.g., biogenic emissions, dry deposition and transpiration. These processes are in turn affected by chronic exposure to ozone via lowered photosynthesis rate and stomatal conductance. Both ozone and vegetation growth are expected to be altered by climate change. To better understand these climate-ozone-vegetation interactions and possible feedbacks on ozone itself via vegetation, we implement an online ozone-vegetation scheme [Lombardozzi et al., 2015] into the Community Earth System Model (CESM) with active atmospheric chemistry, climate and land surface components. Previous overestimation of surface ozone in eastern US, Canada and Europe is shown to be reduced by >8 ppb, reflecting improved model-observation comparison. Simulated surface ozone is lower by 3.7 ppb on average globally. Such reductions (and improvements) in simulated ozone are caused mainly by lower isoprene emission arising from reduced leaf area index in response to chronic ozone exposure. Effects via transpiration are also potentially significant but require better characterization. Such findings suggest that ozone-vegetation interaction may substantially alter future ozone simulations, especially under changing climate and ambient CO2 levels, which would further modulate ozone-vegetation interactions. Inclusion of such interactions in Earth system models is thus necessary to give more realistic estimation and prediction of surface ozone. This is crucial for better policy formulation regarding air quality, land use and climate change mitigation. Reference list: Lombardozzi, D., et al. "The Influence of Chronic Ozone Exposure on Global Carbon and Water Cycles." Journal of Climate 28.1 (2015): 292-305.

  6. Potential Alternative Lower Global Warming Refrigerants for Air Conditioning in Hot Climates

    Energy Technology Data Exchange (ETDEWEB)

    Abdelaziz, Omar [ORNL; Shrestha, Som S [ORNL; Shen, Bo [ORNL

    2017-01-01

    The earth continues to see record increase in temperatures and extreme weather conditions that is largely driven by anthropogenic emissions of warming gases such as carbon dioxide and other more potent greenhouse gases such as refrigerants. The cooperation of 188 countries in the Conference of the Parties in Paris 2015 (COP21) resulted in an agreement aimed to achieve a legally binding and universal agreement on climate, with the aim of keeping global warming below 2 C. A global phasedown of hydrofluorocarbons (HFCs) can prevent 0.5 C of warming by 2100. However, most of the countries in hot climates are considered as developing countries and as such are still using R-22 (a Hydrochlorofluorocarbon (HCFC)) as the baseline refrigerant and are currently undergoing a phase-out of R-22 which is controlled by current Montreal Protocol to R-410A and other HFC based refrigerants. These HFCs have significantly high Global Warming Potential (GWP) and might not perform as well as R-22 at high ambient temperature conditions. In this paper we present recent results on evaluating the performance of alternative lower GWP refrigerants for R-22 and R-410A for small residential mini-split air conditioners and large commercial packaged units. Results showed that several of the alternatives would provide adequate replacement for R-22 with minor system modification. For the R-410A system, results showed that some of the alternatives were almost drop-in ready with benefit in efficiency and/or capacity. One of the most promising alternatives for R-22 mini-split unit is propane (R-290) as it offers higher efficiency; however it requires compressor and some other minor system modification to maintain capacity and minimize flammability risk. Between the R-410A alternatives, R-32 appears to have a competitive advantage; however at the cost of higher compressor discharge temperature. With respect to the hydrofluoroolefin (HFO) blends, there existed a tradeoff in performance and system design

  7. The Relationship between Odour Annoyance Scores and Modelled Ambient Air Pollution in Sarnia, “Chemical Valley”, Ontario

    Directory of Open Access Journals (Sweden)

    Dominic Odwa Atari

    2009-10-01

    Full Text Available This study aimed at establishing the relationship between annoyance scores and modelled air pollution in “Chemical Valley”, Sarnia, Ontario (Canada. Annoyance scores were taken from a community health survey (N = 774; and respondents’ exposure to nitrogen dioxide (NO2 and sulphur dioxide (SO2 were estimated using land use regression (LUR models. The associations were examined by univariate analysis while multivariate logistic regression was used to examine the determinants of odour annoyance. The results showed that odour annoyance was significantly correlated to modelled pollutants at the individual (NO2, r = 0.15; SO2, r = 0.13 and census tract (NO2, r = 0.56; SO2, r = 0.67 levels. The exposure-response relationships show that residents of Sarnia react to very low pollution concentrations levels even if they are within the Ontario ambient air quality criteria. The study found that exposure to high NO2 and SO2 concentrations, gender, and perception of health effects were significant determinants of individual odour annoyance reporting. The observed association between odour annoyance and modelled ambient pollution suggest that individual and census tract level annoyance scores may serve as proxies for air quality in exposed communities because they capture the within area spatial variability of pollution. However, questionnaire-based odour annoyance scores need to be validated longitudinally and across different scales if they are to be adopted for use at the national level.

  8. ASSESSMENT OF SO2 CONCENTRATION IN AMBIENT AIR AND ITS IMPACT ON HUMAN HEALTH IN THE CITY OF GWALIOR, INDIA

    Directory of Open Access Journals (Sweden)

    Ishfaq Ahmad

    2014-09-01

    Full Text Available Gwalior is a historical and major city in the Indian state of Madhya Pradesh. It is located south of Delhi the capital city of India, and 423 kilometers north of Bhopal, the state capital. Gwalior is being called as The Heart of Incredible India. Gwalior is surrounded by industrial and commercial zones of neighboring districts (Malanpur – Bhind, Banmor – Morena on all three main directions. Rapid increase in urbanization with vehicle congestion has increased enormously on the roads of Gwalior city. As a result of this, gaseous pollutants (SOx, NOx and Respirable and suspended particulate matter pollutants are continuously increasing in the ambient air of Gwalior city. Levels of SO2 were monitored at 4 locations of Gwalior city by using high volume air sampler (Envirotech APM 415 and 411. The average ambient air concentration of SO2 was found below the permissible limits of NAAQS of CPCB at all the sites. Comparatively somewhat higher concentration of SO2 was observed during these months. A health survey was also carried out which demonstrated that symptoms were developed such as sneezing, sore throat, shortness of breath, wheezing, chest tightness, skin irritation, nausea etc. In this study, an exposure–response assessment (aged 10 to 60 years was carried out related to health problems due to vehicular pollution between the months of November-2013 to May-2014 (winter. The main objectives of this study are to investigate the state of vehicular emission in Gwalior and to investigate the impact of vehicular emission on people.

  9. Impact of Climate Change on Ambient Ozone Level and Mortality in Southeastern United States

    OpenAIRE

    Montserrat Fuentes; Chang, Howard H.; Jingwen Zhou

    2010-01-01

    There is a growing interest in quantifying the health impacts of climate change. This paper examines the risks of future ozone levels on non-accidental mortality across 19 urban communities in Southeastern United States. We present a modeling framework that integrates data from climate model outputs, historical meteorology and ozone observations, and a health surveillance database. We first modeled present-day relationships between observed maximum daily 8-hour average ozone concentrations an...

  10. Impacts of Air Pollution and Climate Change on Forest Ecosystems — Emerging Research Needs

    Directory of Open Access Journals (Sweden)

    Elena Paoletti

    2007-01-01

    Full Text Available Outcomes from the 22nd meeting for Specialists in Air Pollution Effects on Forest Ecosystems “Forests under Anthropogenic Pressure Effects of Air Pollution, Climate Change and Urban Development”, September 1016, 2006, Riverside, CA, are summarized. Tropospheric or ground-level ozone (O3 is still the phytotoxic air pollutant of major interest. Challenging issues are how to make O3 standards or critical levels more biologically based and at the same time practical for wide use; quantification of plant detoxification processes in flux modeling; inclusion of multiple environmental stresses in critical load determinations; new concept development for nitrogen saturation; interactions between air pollution, climate, and forest pests; effects of forest fire on air quality; the capacity of forests to sequester carbon under changing climatic conditions and coexposure to elevated levels of air pollutants; enhanced linkage between molecular biology, biochemistry, physiology, and morphological traits.

  11. The use of alternative pollutant metrics in time-series studies of ambient air pollution and respiratory emergency department visits.

    Science.gov (United States)

    Darrow, Lyndsey A; Klein, Mitchel; Sarnat, Jeremy A; Mulholland, James A; Strickland, Matthew J; Sarnat, Stefanie E; Russell, Armistead G; Tolbert, Paige E

    2011-01-01

    Various temporal metrics of daily pollution levels have been used to examine the relationships between air pollutants and acute health outcomes. However, daily metrics of the same pollutant have rarely been systematically compared within a study. In this analysis, we describe the variability of effect estimates attributable to the use of different temporal metrics of daily pollution levels. We obtained hourly measurements of ambient particulate matter (PM₂.₅), carbon monoxide (CO), nitrogen dioxide (NO₂), and ozone (O₃) from air monitoring networks in 20-county Atlanta for the time period 1993-2004. For each pollutant, we created (1) a daily 1-h maximum; (2) a 24-h average; (3) a commute average; (4) a daytime average; (5) a nighttime average; and (6) a daily 8-h maximum (only for O₃). Using Poisson generalized linear models, we examined associations between daily counts of respiratory emergency department visits and the previous day's pollutant metrics. Variability was greatest across O₃ metrics, with the 8-h maximum, 1-h maximum, and daytime metrics yielding strong positive associations and the nighttime O₃ metric yielding a negative association (likely reflecting confounding by air pollutants oxidized by O₃). With the exception of daytime metric, all of the CO and NO₂ metrics were positively associated with respiratory emergency department visits. Differences in observed associations with respiratory emergency room visits among temporal metrics of the same pollutant were influenced by the diurnal patterns of the pollutant, spatial representativeness of the metrics, and correlation between each metric and copollutant concentrations. Overall, the use of metrics based on the US National Ambient Air Quality Standards (for example, the use of a daily 8-h maximum O₃ as opposed to a 24-h average metric) was supported by this analysis. Comparative analysis of temporal metrics also provided insight into underlying relationships between specific air

  12. Effects of ambient air pollution on functional status in patients with chronic congestive heart failure: a repeated-measures study

    Directory of Open Access Journals (Sweden)

    Phillips Russell S

    2007-09-01

    Full Text Available Abstract Background Studies using administrative data report a positive association between ambient air pollution and the risk of hospitalization for congestive heart failure (HF. Circulating levels of B-type natriuretic peptide (BNP are directly associated with cardiac hemodynamics and symptom severity in patients with HF and, therefore, serves as a marker of functional status. We tested the hypothesis that BNP levels would be positively associated with short-term changes in ambient pollution levels among 28 patients with chronic stable HF and impaired systolic function. Methods BNP was measured in whole blood at 0, 6, and 12 weeks. We used linear mixed models to evaluate the association between fine particulate matter (PM2.5, carbon monoxide, sulfur dioxide, nitrogen dioxide, ozone, and black carbon and log(BNP. Lags of 0 to 3 days were considered in separate models. We calculated the intraclass correlation coefficient and within-subject coefficient of variation as measures of reproducibility. Results We found no association between any pollutant and measures of BNP at any lag. For example, a 10 μg/m3 increase in PM2.5 was associated with a 0.8% (95% CI: -16.4, 21.5; p = 0.94 increase in BNP on the same day. The within-subject coefficient of variation was 45% on the natural scale and 9% on the log scale. Conclusion These results suggest that serial BNP measurements are unlikely to be useful in a longitudinal study of air pollution-related acute health effects. The magnitude of expected ambient air pollution health effects appears small in relation to the considerable within-person variability in BNP levels in this population.

  13. Health effects of ambient air pollution – recent research development and contemporary methodological challenges

    Directory of Open Access Journals (Sweden)

    Ren Cizao

    2008-11-01

    Full Text Available Abstract Exposure to high levels of air pollution can cause a variety of adverse health outcomes. Air quality in developed countries has been generally improved over the last three decades. However, many recent epidemiological studies have consistently shown positive associations between low-level exposure to air pollution and health outcomes. Thus, adverse health effects of air pollution, even at relatively low levels, remain a public concern. This paper aims to provide an overview of recent research development and contemporary methodological challenges in this field and to identify future research directions for air pollution epidemiological studies.

  14. Ambient air pollution and years of life lost in Ningbo, China.

    Science.gov (United States)

    He, Tianfeng; Yang, Zuyao; Liu, Tao; Shen, Yueping; Fu, Xiaohong; Qian, Xujun; Zhang, Yuelun; Wang, Yong; Xu, Zhiwei; Zhu, Shankuan; Mao, Chen; Xu, Guozhang; Tang, Jinling

    2016-03-01

    To evaluate the burden of air pollution on years of life lost (YLL) in addition to mortality, we conducted a time series analysis based on the data on air pollution, meteorological conditions and 163,704 non-accidental deaths of Ningbo, China, 2009-2013. The mean concentrations of particulate matter with aerodynamic diameter air pollution lasted for four days (lag 0-3), and were more significant in the elderly than in the young population for both outcomes. These findings clarify the burden of air pollution on YLL and highlight the importance and urgency of air pollution control in China.

  15. The Effects of Urban Form on Ambient Air Pollution and Public Health Risk: A Case Study in Raleigh, North Carolina.

    Science.gov (United States)

    Mansfield, Theodore J; Rodriguez, Daniel A; Huegy, Joseph; Gibson, Jacqueline MacDonald

    2015-05-01

    Since motor vehicles are a major air pollution source, urban designs that decrease private automobile use could improve air quality and decrease air pollution health risks. Yet, the relationships among urban form, air quality, and health are complex and not fully understood. To explore these relationships, we model the effects of three alternative development scenarios on annual average fine particulate matter (PM2.5 ) concentrations in ambient air and associated health risks from PM2.5 exposure in North Carolina's Raleigh-Durham-Chapel Hill area. We integrate transportation demand, land-use regression, and health risk assessment models to predict air quality and health impacts for three development scenarios: current conditions, compact development, and sprawling development. Compact development slightly decreases (-0.2%) point estimates of regional annual average PM2.5 concentrations, while sprawling development slightly increases (+1%) concentrations. However, point estimates of health impacts are in opposite directions: compact development increases (+39%) and sprawling development decreases (-33%) PM2.5-attributable mortality. Furthermore, compactness increases local variation in PM2.5 concentrations and increases the severity of local air pollution hotspots. Hence, this research suggests that while compact development may improve air quality from a regional perspective, it may also increase the concentration of PM2.5 in local hotspots and increase population exposure to PM2.5 . Health effects may be magnified if compact neighborhoods and PM2.5 hotspots are spatially co-located. We conclude that compactness alone is an insufficient means of reducing the public health impacts of transportation emissions in automobile-dependent regions. Rather, additional measures are needed to decrease automobile dependence and the health risks of transportation emissions.

  16. A review of scientifc linkages and interactions between climate change and air quality, with implications for air quality management in South Africa

    Directory of Open Access Journals (Sweden)

    Tirusha Thambiran

    2010-04-01

    Full Text Available In recent years there has been considerable advancement in our scientifc understanding of the linkages and interactions between climate change and air quality. A warmer, evolving climate is likely to have severe consequences for air quality due to impacts on pollution sources and meteorology. Climate-induced changes to sources of tropospheric ozone precursor gases and to atmospheric circulation are likely to lead to changes in both the concentration and dispersion of near-surface ozone that could act to offset improvements in air quality. The control of air pollutants through air quality management is also likely to impact on climate change, with reductions in ozone, particulate matter and sulphur dioxide being of particular interest. The improved understanding of the relationship between air quality and climate change provides a scientific basis for policy interventions. After a review of the scientific linkages, the potential to include climate change considerations in air quality management planning processes in South Africa was examined.

  17. Understanding urban vehicular pollution problem vis-a-vis ambient air quality--case study of a megacity (Delhi, India).

    Science.gov (United States)

    Goyal, S K; Ghatge, S V; Nema, P; M Tamhane, S

    2006-08-01

    Air pollution has become a growing problem in megacities and large urban areas through out the globe, and transportation is recognized as the major source of air pollution in many cities, especially in developing countries. Contribution of automobiles is reported in the range of 40 to 80% of the total air pollution. The challenge facing megacities is how to reduce the adverse environmental impacts and other negative effects of transportation without giving up the benefits of mobility. The dilemma becomes most pressing under conditions of rapid urban growth, which is likely to increase travel demand significantly. The paper is aimed at understanding the problem of vehicular pollution vis-a-vis ambient air quality for a highly traffic affected megacity, Delhi, wherein, the contribution of transport sector was estimated to be as high as 72%. An effort has been made to review and evaluate the benefits (in terms of improved air quality) of the technological interventions/policies adopted for vehicular pollution control in Delhi. It also highlights the outcome of the efforts and suggests further improvements thereon. The importance of public participation and awareness are also discussed. The paper focuses on deriving the benefits of the implementation of management strategies, supported by scientific and technical data/interpretation, so that the people can realize and participate in the government's endeavor for clean city drive in a more effective manner.

  18. 40 CFR 86.161-00 - Air conditioning environmental test facility ambient requirements.

    Science.gov (United States)

    2010-07-01

    ... heat loading. (1)(i) Acceptable types of radiant energy emitters that may be used for simulating solar heat load are: (A) Metal halide; (B) Quartz halogen with dichroic mirrors; and (C) Sodium iodide. (ii... to simulate the impact of an ambient heat load on the power requirements of the vehicle's...

  19. 40 CFR Appendix I to Part 50 - Interpretation of the 8-Hour Primary and Secondary National Ambient Air Quality Standards for Ozone

    Science.gov (United States)

    2010-07-01

    ... and Secondary National Ambient Air Quality Standards for Ozone I Appendix I to Part 50 Protection of... AIR QUALITY STANDARDS Pt. 50, App. I Appendix I to Part 50—Interpretation of the 8-Hour Primary and... valid day if valid 8-hour averages are available for at least 75% of possible hours in the day (i.e.,...

  20. Combined effects of road traffic noise and ambient air pollution in relation to risk for stroke?

    DEFF Research Database (Denmark)

    Sørensen, Mette; Lühdorf, Pernille; Ketzel, Matthias

    2014-01-01

    Exposure to road traffic noise and air pollution have both been associated with risk for stroke. The few studies including both exposures show inconsistent results. We aimed to investigate potential mutual confounding and combined effects between road traffic noise and air pollution in association...... to 2009 were identified in national registers and road traffic noise and air pollution were modeled for all addresses. Analyses were done using Cox regression. A higher mean annual exposure at time of diagnosis of 10µg/m(3) nitrogen dioxide (NO2) and 10dB road traffic noise at the residential address...... was found for combination of high noise and high NO2 (IRR=1.28; 95% CI=1.09-1.52). Fatal stroke was positively associated with air pollution and not with traffic noise. In conclusion, in mutually adjusted models road traffic noise and not air pollution was associated ischemic stroke, while only air...

  1. A system for the determination of trace-level polar and non-polar toxic organic compounds in ambient air

    Energy Technology Data Exchange (ETDEWEB)

    Tipler, A.; Dang, R.; Hoberecht, H. [Perkin Elmer Corp., Norwalk, CT (United States). Fresh Aire Lab.

    1994-12-31

    A gas chromatographic system is described for the determination of toxic organic compounds in ambient air. These compounds include all those specified within the US EPA Compendium Method TO14 and some polar additional analytes under consideration for the proposed TO15 Method. The system supports both on-line and off-line (passivated canisters and adsorption tubes) methods for sampling air--providing a fully automated analysis. A key feature of the system is that liquid cryogen is not required for either the analyte preconcentration or the subsequent chromatographic separation. Water management is achieved by dry-purging an adsorbent trap upon which the sample analytes have been retained. The performance of the system is demonstrated with conventional detection systems (electron capture and flame ionization) and with a mass spectrometer.

  2. Ozone deposition to an oat crop ( Avena sativa L.) grown in open-top chambers and in the ambient air

    Science.gov (United States)

    Pleijel, H.; Wallin, G.; Karlsson, P. E.; Skarby, L.; Sellden, G.

    Fluxes and deposition velocities for ozone were determined for open-top chambers with and without an oat crop, and for the adjacent field, using a resistance analogue model and the aerodynamic wind-profile method, respectively. During a period when the canopy was green and the ambient wind speeds modest, the fluxes and deposition velocities were higher in the chamber with plants than in the field crop. The deposition to chamber walls and soil in the chamber only accounted for part of that difference. The deposition velocity for ozone to the crop was light-dependent both in the chamber with plants and in the ambient air. With increasing plant senescence, the deposition velocity declined and the light dependence disappeared. Fluctuations in deposition velocity superimposed on the overall declining trend followed the same temporal pattern in the chambers with and without plants. These fluctuations in deposition velocity may partly be explained by variations in surface wetness. Differences in boundary layer conductance between chamber and ambient, which under certain conditions may significantly influence the validity of the chamber as a test system, were observed.

  3. Pediatric emergency department visits and ambient Air pollution in the U.S. State of Georgia: a case-crossover study

    OpenAIRE

    Xiao, Qingyang; Liu, Yang; Mulholland, James A.; Russell, Armistead G.; Darrow, Lyndsey A.; Tolbert, Paige E.; Strickland, Matthew J.

    2016-01-01

    Background Estimating the health effects of ambient air pollutant mixtures is necessary to understand the risk of real-life air pollution exposures. Methods Pediatric Emergency Department (ED) visit records for asthma or wheeze (n = 148,256), bronchitis (n = 84,597), pneumonia (n = 90,063), otitis media (n = 422,268) and upper respiratory tract infection (URI) (n = 744,942) were obtained from Georgia hospitals during 2002–2008. Spatially-contiguous daily concentrations of 11 ambient air pollu...

  4. Polycyclic aromatic hydrocarbons in ambient air in the Philippines derived from passive sampler with polyurethane foam disk

    Science.gov (United States)

    Santiago, Evangeline C.; Cayetano, Mylene G.

    Passive samplers with polyurethane disks (PUF) were applied in the determination of the concentration of polycyclic aromatic hydrocarbons (PAHs) in ambient air in six residential areas in the Philippines during four simultaneous sampling periods. The uptake profiles of PAHs were determined at one site during one sampling period. Most of the PAHs that were detected in air at concentrations that were significantly higher than their analytical detection limits exhibited a linear uptake trend on the PUF disk. The linear uptake profiles of some high molecular weight (HMW) PAHs were not established and this is attributed to the low concentration of the compounds in air in the gaseous phase. The retention concentrations of phenanthrene-d-10 were determined after depuration in four sampling sites during two sampling periods. The sampling rate for phenanthrene-d-10 was calculated at the linear phase of the uptake using the kA derived from depuration experiments and the relationship of kA and sampling rate which was established in a previous passive sampling study. The average sampling rate obtained for phenanthrene d-10 (2.94±0.69 m 3 d -1) was applied for derivation of the concentrations of the PAHs in the field samples. The passive sampler with PUF disk and short integration time of 42-56 days is applicable for the derivation of the concentrations of PAHs in ambient air in the Philippines. The concentrations of the organic pollutants derived from the passive sampler showed variability for the six residential areas; reflecting the influence of possible sources of emission of the pollutants at the sites at the different sampling periods. The weather conditions, including the occurrence of a tropical cyclone, increased rainfall and high-relative humidity during the rainy season, had an influence on the concentrations of PAHs derived by the passive sampler.

  5. Climate change and air pollution jointly creating nightmare for tourism industry.

    Science.gov (United States)

    Sajjad, Faiza; Noreen, Umara; Zaman, Khalid

    2014-11-01

    The objective of the study is to examine the long-run and causal relationship between climate change (i.e., greenhouse gas emissions, hydrofluorocarbons, per fluorocarbons, and sulfur hexafluoride), air pollution (i.e., methane emissions, nitrous oxide emissions, and carbon dioxide emissions), and tourism development indicators (i.e., international tourism receipts, international tourism expenditures, natural resource depletion, and net forest depletion) in the World's largest regions. The aggregate data is used for robust analysis in the South Asia, the Middle East and North Africa, sub-Saharan Africa, and East Asia and the Pacific regions, over a period of 1975-2012. The results show that climatic factors and air pollution have a negative impact on tourism indicators in the form of deforestation and natural resource depletion. The impact is evident, as we have seen the systematic eroding of tourism industry, due to severe changes in climate and increasing strain of air pollution. There are several channels of cause-effect relationship between the climatic factors, air pollution, and tourism indicators in the World's region. The study confirms the unidirectional, bidirectional, and causality independent relationship between climatic factors, air pollution, and tourism indicators in the World. It is conclusive that tourism industry is facing all time bigger challenges of reduce investment, less resources, and minor importance from the government agencies because of the two broad challenges, i.e., climate change and air pollution, putting them in a dismal state.

  6. Alfalfa nutritive quality for ruminant livestock as influenced by ambient air quality in west-central Alberta

    Energy Technology Data Exchange (ETDEWEB)

    Lin, J.C. [Department of Animal Sciences, Auburn University, Auburn, AL 36849 (United States); Nosal, M. [Department of Mathematics and Statistics, University of Calgary, Calgary, AB T2N 1N4 (Canada); Muntifering, R.B. [Department of Animal Sciences, Auburn University, Auburn, AL 36849 (United States)]. E-mail: muntirb@auburn.edu; Krupa, S.V. [Department of Plant Pathology, University of Minnesota, St. Paul, MN 55108 (United States)

    2007-09-15

    Alfalfa (Medicago sativa) nutritive quality response to ambient ozone (O{sub 3}), sulfur dioxide (SO{sub 2}) and oxides of nitrogen (NO {sub x} ) were assessed at three locations in west-central Alberta, Canada (1998-2002). Yield data were segregated into high and low relative to overall median yield. Ozone concentrations (hourly median and 95th-percentile) and precipitation (P) contributed 69 and 29%, respectively, to the variability in crude protein (CP) concentration in low-yielding alfalfa, whereas mean temperature (T) and relative humidity (RH) collectively influenced 98% of the variation in CP in high-yielding alfalfa. Three-fourths of the accounted variation in relative feed value (RFV) of low-yielding alfalfa was attributable to P, T and RH, whereas median and 95th-percentile hourly O{sub 3} concentrations and SO{sub 2} and NO {sub x} exposure integrals contributed 25%. In contrast, air quality, (mainly O{sub 3}) influenced 86% of the accounted variation in RFV of high-yielding alfalfa, and T and P collectively contributed 14%. - Exposure to ambient concentrations of phytotoxic air pollutants affected nutritive quality of alfalfa for ruminant livestock in a yield-dependent manner.

  7. Fast oxidation processes from emission to ambient air introduction of aerosol emitted by residential log wood stoves

    Science.gov (United States)

    Nalin, Federica; Golly, Benjamin; Besombes, Jean-Luc; Pelletier, Charles; Aujay-Plouzeau, Robin; Verlhac, Stéphane; Dermigny, Adrien; Fievet, Amandine; Karoski, Nicolas; Dubois, Pascal; Collet, Serge; Favez, Olivier; Albinet, Alexandre

    2016-10-01

    Little is known about the impact of post-combustion processes, condensation and dilution, on the aerosol concentration and chemical composition from residential wood combustion. The evolution of aerosol emitted by two different residential log wood stoves (old and modern technologies) from emission until it is introduced into ambient air was studied under controlled "real" conditions. The first objective of this research was to evaluate the emission factors (EF) of polycyclic aromatic hydrocarbons (PAH) and their nitrated and oxygenated derivatives from wood combustion. These toxic substances are poorly documented in the literature. A second objective was to evaluate the oxidation state of the wood combustion effluent by studying these primary/secondary compounds. EFs of Σ37PAHs and Σ27Oxy-PAHs were in the same range and similar to those reported in literature (4-240 mg kg-1). Σ31Nitro-PAH EFs were 2-4 orders of magnitude lower (3.10-2-8.10-2 mg kg-1) due to the low temperature and low emission of NO2 from wood combustion processes. An increase of equivalent EF of PAH derivatives was observed suggesting that the oxidation state of the wood combustion effluent from the emission point until its introduction in ambient air changed in a few seconds. These results were confirmed by the study of both, typical compounds of SOA formation from PAH oxidation and, PAH ratio-ratio plots commonly used for source evaluation.

  8. Community Air Sensor Network (CAIRSENSE) Project: Lower Cost, Continuous Ambient Monitoring Methods

    Science.gov (United States)

    Advances in air pollution sensor technology have enabled the development of small and low cost systems to measure outdoor air pollution. The deployment of numerous sensors across a small geographic area would have potential benefits to supplement existing monitoring networks and ...

  9. Is There an Association Between Ambient Air Pollution and Bladder Cancer Incidence?

    DEFF Research Database (Denmark)

    Pedersen, Marie; Stafoggia, Massimo; Weinmayr, Gudrun

    2016-01-01

    of information about lifetime exposure. Conclusions: There was no evidence of an association between exposure to outdoor air pollution levels at place of residence and risk of BC. Patient summary: We assessed the link between outdoor air pollution at place of residence and bladder cancer using the largest study...

  10. Temporal variations of atmospheric carbonyls in urban ambient air and street canyons of a Mountainous city in Southwest China

    Science.gov (United States)

    Pang, Xiaobing; Lee, Xinqing

    2010-06-01

    Carbonyl compounds in urban ambient air and street canyons were measured from December 2008 to August 2009 in a mountainous city in southwest China (Guiyang). The formaldehyde yield from the photo-oxidation of isoprene emitted by vegetation was estimated to be in the range of 0.63-3.62 μg m -3 from May to August, which accounted for 28.8-33.4% of ambient formaldehyde. Based on the calculation of photolysis rates and rates of reaction with the OH radical, it was found that photolysis was the predominant sink for formaldehyde and acetone in both summer and winter. For acetaldehyde, photo-oxidation by OH radicals and photolysis were the major sinks in summer while photo-oxidation by OH radicals was the dominant sink in winter. Wet precipitation was found to be an important removal process for the atmospheric carbonyls. In the urban ambient air, the average concentrations of formaldehyde, acetaldehyde, acetone and all carbonyls were 4.8 ± 2.1, 5.7 ± 3.3, 5.1 ± 2.5, and 25.1 ± 9.2 μg m -3 ( n = 139), respectively. The average concentrations of these species in street canyons were 18.8 ± 6.5, 9.4 ± 3.2, 10.9 ± 2.1, and 64.1 ± 16.3 μg m -3 ( n = 62), respectively. The significantly higher carbonyl levels on weekdays (compared to weekends) highlight the contribution of vehicle emissions to carbonyls in the street canyons.

  11. Long-Term Exposure to Ambient Air Pollution and Incidence of Cerebrovascular Events

    DEFF Research Database (Denmark)

    Stafoggia, Massimo; Cesaroni, Giulia; Peters, Annette

    2014-01-01

    BACKGROUND: Few studies have investigated effects of air pollution on the incidence of cerebrovascular events. OBJECTIVES: We assessed the association between long-term exposure to multiple air pollutants and the incidence of stroke in European cohorts. METHODS: Data from 11 cohorts were collected...... and occurrence of a first stroke was evaluated. Individual air pollution exposures were predicted from land-use regression models developed within the "European Study of Cohorts for Air Pollution Effects" (ESCAPE). The exposures were: PM2.5 (particulate matter [PM] below 2.5 µm in diameter), coarse PM (PM...... found suggestive evidence of an association between fine particles and incidence of cerebrovascular events in Europe, even at lower concentrations than set by the current air quality limit value....

  12. Environmental impact of the programs of substitution of room type air conditioning equipment; Impacto ambiental de los programas de sustitucion de equipos de aire tipo cuarto

    Energy Technology Data Exchange (ETDEWEB)

    Alarcon Aleman, Jose Mauricio [OLADE, Quito (Ecuador)

    2002-09-01

    The present article approaches in a general way the relation that exists between the environment and the saving of electrical energy, especially in the Programs of Demand Side Management (DSM). In particular form the potential environmental impacts are described, derived of the use and the discard of the room type air conditioning equipment, goes deep into the characteristics of their cooling fluids, as well as in the relation that these keep with the protocols of Montreal and Kyoto. Finally, this article comments the incidence which have, the manufacturers as the institutions that implement DSM programs, on the environmental part of the programs of substitution of room type air conditioning equipment. In addition it is briefly described, the pilot program developed by Fideicomiso para el Ahorro de Energia Electrica (FIDE) as a successful case. [Spanish] En forma general, el presente articulo aborda la relacion que existe entre el medio ambiente y el ahorro de energia electrica, especialmente en los Programas de Administracion por el Lado de la Demanda (ALD). En forma particular se describen los impactos ambientales potenciales, derivados del uso y desecho de los equipos de aire acondicionado tipo cuarto, se ahonda en las caracteristicas de sus refrigerantes, asi como en la relacion que estos guardan con los protocolos de Montreal y Kioto. Finalmente, se comenta la incidencia que tienen, tanto los fabricantes como las instituciones que implementan programas de ALD, sobre la parte ambiental de los programas de sustitucion de equipos de aire acondicionado tipo cuarto. Ademas se describe brevemente, el programa piloto desarrollado por el Fideicomiso para el Ahorro de Energia Electrica (FIDE) como un caso exitoso.

  13. Biochemical and cellular effects of electrophiles present in ambient air samples

    Science.gov (United States)

    Iwamoto, Noriko; Nishiyama, Akira; Eiguren-Fernandez, Arantzazu; Hinds, William; Kumagai, Yoshito; Froines, John R.; Cho, Arthur K.; Shinyashiki, Masaru

    2010-04-01

    Ambient vapor-phase samples collected in Riverside, California had shown that both redox and electrophilic activity were present, with the vapor phase containing higher levels of electrophiles than the particle phase. In this study, the biochemical effects of the vapor-phase electrophiles were examined using the purified thiol proteins, glyceraldehyde-3-phosphate dehydrogenase (GAPDH), protein tyrosine phosphatase 1B (PTP1B) and KELCH-1 like ECH-associated protein 1 (Keap1). The results demonstrated that the thiol proteins were inactivated by the vapor-phase samples through covalent modifications. Next, two cellular responses, epidermal growth factor receptor (EGFR)/mitogen-activated protein (MAP) kinase and NF-E2-related factor 2 (Nrf2), to the ambient vapor-phase samples were assessed in A549 and RAW 264.7 cell lines, respectively. The vapor-phase samples, at non-oxidative concentrations, increased phosphorylation of EGFR, which is negatively regulated by PTP1B, and its downstream MAP kinase, extracellular signal-regulated kinase (ERK)1/2. Activation of Nrf2, which requires Keap1 alkylation, and expression of its downstream proteins were also observed. The electrophilic compounds present in ambient vapor-phase were shown to modify cellular proteins through covalent modification and to activate diverse cellular responses that can lead to inflammatory and adaptive responses.

  14. The burden of COPD mortality due to ambient air pollution in Guangzhou, China

    Science.gov (United States)

    Li, Li; Yang, Jun; Song, Yun-Feng; Chen, Ping-Yan; Ou, Chun-Quan

    2016-05-01

    Few studies have investigated the chronic obstructive pulmonary disease (COPD) mortality fraction attributable to air pollution and modification by individual characteristics of air pollution effects. We applied distributed lag non-linear models to assess the associations between air pollution and COPD mortality in 2007–2011 in Guangzhou, China, and the total COPD mortality fraction attributable to air pollution was calculated as well. We found that an increase of 10 μg/m3 in particulate matter with an aerodynamic diameter of 10 μm or less (PM10), sulfur dioxide (SO2) and nitrogen dioxide (NO2) was associated with a 1.58% (95% confidence interval (CI): 0.12–3.06%), 3.45% (95% CI: 1.30–5.66%) and 2.35% (95% CI: 0.42–4.32%) increase of COPD mortality over a lag of 0–15 days, respectively. Greater air pollution effects were observed in the elderly, males and residents with low educational attainment. The results showed 10.91% (95% CI: 1.02–9.58%), 12.71% (95% CI: 5.03–19.85%) and 13.38% (95% CI: 2.67–22.84%) COPD mortality was attributable to current PM10, SO2 and NO2 exposure, respectively. In conclusion, the associations between air pollution and COPD mortality differed by individual characteristics. There were remarkable COPD mortality burdens attributable to air pollution in Guangzhou.

  15. The burden of COPD mortality due to ambient air pollution in Guangzhou, China.

    Science.gov (United States)

    Li, Li; Yang, Jun; Song, Yun-Feng; Chen, Ping-Yan; Ou, Chun-Quan

    2016-05-19

    Few studies have investigated the chronic obstructive pulmonary disease (COPD) mortality fraction attributable to air pollution and modification by individual characteristics of air pollution effects. We applied distributed lag non-linear models to assess the associations between air pollution and COPD mortality in 2007-2011 in Guangzhou, China, and the total COPD mortality fraction attributable to air pollution was calculated as well. We found that an increase of 10 μg/m(3) in particulate matter with an aerodynamic diameter of 10 μm or less (PM10), sulfur dioxide (SO2) and nitrogen dioxide (NO2) was associated with a 1.58% (95% confidence interval (CI): 0.12-3.06%), 3.45% (95% CI: 1.30-5.66%) and 2.35% (95% CI: 0.42-4.32%) increase of COPD mortality over a lag of 0-15 days, respectively. Greater air pollution effects were observed in the elderly, males and residents with low educational attainment. The results showed 10.91% (95% CI: 1.02-9.58%), 12.71% (95% CI: 5.03-19.85%) and 13.38% (95% CI: 2.67-22.84%) COPD mortality was attributable to current PM10, SO2 and NO2 exposure, respectively. In conclusion, the associations between air pollution and COPD mortality differed by individual characteristics. There were remarkable COPD mortality burdens attributable to air pollution in Guangzhou.

  16. Weekday/Weekend differences in ambient air pollutant concentrations in atlanta and the southeastern United States.

    Science.gov (United States)

    Blanchard, Charles L; Tanenbaum, Shelley

    2006-03-01

    The authors quantified changes between mean weekday and weekend ambient concentrations of ozone (O3) precursors (volatile organic compounds [VOC], carbon monoxide [CO], nitric oxide, and oxides of nitrogen [NOx]) in Atlanta and surrounding areas to observe how weekend precursor emission levels influenced ambient O3 levels. The authors analyzed CO, nitric oxide (NO), and NO, measurements from 1998 to 2002 and speciated VOC from 1996 to 2003. They observed a strong weekend effect in the Atlanta region, with median daytime (6:00 a.m. to 3:00 p.m. Eastern Standard Time) decreases of 62%, 57%, and 31%, respectively, in the ambient levels of NO, NOx, and CO from Wednesdays to Sundays, during the ozone season (March to October). They also observed significant decreases in ambient VOC levels between Wednesdays and Sundays, with decreases of 28% for the sum of aromatic compounds and 19% for the sum of Photochemical Assessment Monitoring Stations target compounds. Despite large reductions in O3 precursor levels on weekends, day-of-week differences in O3 mixing ratios in and near Atlanta were much smaller. Averaging overall O3-season days, the 1-hr and 8-hr mean peak daily O3 maxima on Sundays were 4.5% and 2.3% lower, respectively, than their mean levels on Wednesdays (median of 14 site differences), with no sites showing statistically significant Wednesday-to-Sunday differences. When restricted to high-O3 days (highest 3 peak O3 days per day of week per site per year), the 1-hr and 8-hr Sunday O3 mixing ratios were 11% and 10% lower, respectively, than their mean peak levels on Wednesdays (median of 14 site differences), with 6 of 14 sites showing statistically significant Wednesday-to-Sunday differences. The analyses of weekday/weekend differences in O3 precursor concentrations show that different emission reductions than normally take place each weekend will be required to achieve major reductions in ambient ozone levels in the Atlanta area.

  17. Community Air Sensor Network (CAIRSENSE) Project: Lower Cost, Continuous Ambient Monitoring Methods

    Science.gov (United States)

    CAIRSENSE Project presentation was given at the 108th Annual Meeting of the Air & Waste Management Associate in June 2015. The presentation provides an overview of the CAIRSENSE Project and general info about the sensors used in the CAIRSENSE Project.

  18. Ambient Air Quality and Human Health: Current Concepts—Part 1

    Directory of Open Access Journals (Sweden)

    Tee L Guidotti

    1995-01-01

    the control of which invites interest in second-order determinants of health. This article attempts to provide a framework for understanding air quality issues that pertain to human health. The objective is to provide the specialist in respiratory medicine with an overview that will assist in educating patients and in responding to their inquiries, and to equip the physician to respond to requests for assistance or interpretation when called upon to comment on public policy issues involving air pollution. The implications of setting air quality standards or objectives to meet arbitrary levels of risk of health effects are examined. The current state of the art does not support risk-based air quality standards. A policy of continuous improvement is most protective of both human health and the environment.

  19. Design and laboratory testing of a new flow-through directional passive air sampler for ambient particulate matter.

    Science.gov (United States)

    Lin, Chun; Solera Garcia, Maria Angeles; Timmis, Roger; Jones, Kevin C

    2011-03-01

    A new type of directional passive air sampler (DPAS) is described for collecting particulate matter (PM) in ambient air. The prototype sampler has a non-rotating circular sampling tray that is divided into covered angular channels, whose ends are open to winds from sectors covering the surrounding 360°. Wind-blown PM from different directions enters relevant wind-facing channels, and is retained there in collecting pools containing various sampling media. Information on source direction and type can be obtained by examining the distribution of PM between channels. Wind tunnel tests show that external wind velocities are at least halved over an extended area of the collecting pools, encouraging PM to settle from the air stream. Internal and external wind velocities are well-correlated over an external velocity range of 2.0-10.0 m s⁻¹, which suggests it may be possible to relate collected amounts of PM simply to ambient concentrations and wind velocities. Measurements of internal wind velocities in different channels show that velocities decrease from the upwind channel round to the downwind channel, so that the sampler effectively resolves wind directions. Computational fluid dynamics (CFD) analyses were performed on a computer-generated model of the sampler for a range of external wind velocities; the results of these analyses were consistent with those from the wind tunnel. Further wind tunnel tests were undertaken using different artificial particulates in order to assess the collection performance of the sampler in practice. These tests confirmed that the sampler can resolve the directions of sources, by collecting particulates preferentially in source-facing channels.

  20. Ambient particulate air pollution induces oxidative stress and alterations of mitochondria and gene expression in brown and white adipose tissues

    Directory of Open Access Journals (Sweden)

    Harkema Jack R

    2011-07-01

    Full Text Available Abstract Background Prior studies have demonstrated a link between air pollution and metabolic diseases such as type II diabetes. Changes in adipose tissue and its mitochondrial content/function are closely associated with the development of insulin resistance and attendant metabolic complications. We investigated changes in adipose tissue structure and function in brown and white adipose depots in response to chronic ambient air pollutant exposure in a rodent model. Methods Male ApoE knockout (ApoE-/- mice inhaled concentrated fine ambient PM (PM 2.5 or filtered air (FA for 6 hours/day, 5 days/week, for 2 months. We examined superoxide production by dihydroethidium staining; inflammatory responses by immunohistochemistry; and changes in white and brown adipocyte-specific gene profiles by real-time PCR and mitochondria by transmission electron microscopy in response to PM2.5 exposure in different adipose depots of ApoE-/- mice to understand responses to chronic inhalational stimuli. Results Exposure to PM2.5 induced an increase in the production of reactive oxygen species (ROS in brown adipose depots. Additionally, exposure to PM2.5 decreased expression of uncoupling protein 1 in brown adipose tissue as measured by immunohistochemistry and Western blot. Mitochondrial number was significantly reduced in white (WAT and brown adipose tissues (BAT, while mitochondrial size was also reduced in BAT. In BAT, PM2.5 exposure down-regulated brown adipocyte-specific genes, while white adipocyte-specific genes were differentially up-regulated. Conclusions PM2.5 exposure triggers oxidative stress in BAT, and results in key alterations in mitochondrial gene expression and mitochondrial alterations that are pronounced in BAT. We postulate that exposure to PM2.5 may induce imbalance between white and brown adipose tissue functionality and thereby predispose to metabolic dysfunction.

  1. Effect of Revised "Ambient Air Quality Standards" on Assessing Results of the Ambient Air Quality in the Cities of Sichuan Province%修订《环境空气质量标准》对四川省城市环境空气质量评价结果的影响

    Institute of Scientific and Technical Information of China (English)

    全利; 余恒; 王晓波

    2012-01-01

    In this paper, according to the monitoring data of ambient air quality in provincially administered municipalities during the "llth Five Year Plan", and based on the comparison of difference between the new Ambient Air Quality Standards and the old, the effects of revised "Ambient Air Quality Standards" on assessing results of the ambient air quality in the cities of Sichuan province were analyzed.%根据“十一五”期间和2011年四川省省控城市环境空气质量监测数据,在比较新、旧环境空气质量标准不同的基础上,本文分析了修订后的《环境空气质量标准》对四川省城市环境空气质量评价结果的影响。

  2. Long term exposure to ambient air pollution and incidence of acute coronary events

    DEFF Research Database (Denmark)

    Cesaroni, Giulia; Forastiere, Francesco; Stafoggia, Massimo

    2014-01-01

    To study the effect of long term exposure to airborne pollutants on the incidence of acute coronary events in 11 cohorts participating in the European Study of Cohorts for Air Pollution Effects (ESCAPE).......To study the effect of long term exposure to airborne pollutants on the incidence of acute coronary events in 11 cohorts participating in the European Study of Cohorts for Air Pollution Effects (ESCAPE)....

  3. Sources and perceptions of indoor and ambient air pollution in rural Alaska.

    Science.gov (United States)

    Ware, Desirae; Lewis, Johnnye; Hopkins, Scarlett; Boyer, Bert; Noonan, Curtis; Ward, Tony

    2013-08-01

    Even though Alaska is the largest state in the United States, much of the population resides in rural and underserved areas with documented disparities in respiratory health. This is especially true in the Yukon-Kuskokwim (southwest) and Ahtna (southcentral) Regions of Alaska. In working with community members, the goal of this study was to identify the air pollution issues (both indoors and outdoors) of concern within these two regions. Over a two-year period, 328 air quality surveys were disseminated within seven communities in rural Alaska. The surveys focused on understanding the demographics, home heating practices, indoor activities, community/outdoor activities, and air quality perceptions within each community. Results from these surveys showed that there is elevated potential for PM10/PM2.5 exposures in rural Alaska communities. Top indoor air quality concerns included mold, lack of ventilation or fresh air, and dust. Top outdoor air pollution concerns identified were open burning/smoke, road dust, and vehicle exhaust (e.g., snow machines, ATVs, etc.). These data can now be used to seek additional funding for interventions, implementing long-term, sustainable solutions to the identified problems. Further research is needed to assess exposures to PM10/PM2.5 and the associated impacts on respiratory health, particularly among susceptible populations such as young children.

  4. Association between Ambient Air Pollution and Outpatient Visits for Acute Bronchitis in a Chinese City

    Institute of Scientific and Technical Information of China (English)

    GUO Li Juan; ZHAO Ang; CHEN Ren Jie; KAN Hai Dong; KUANG Xing Ya

    2014-01-01

    Objective To investigate the short-term association between outdoor air pollution and outpatient visits for acute bronchitis, which is a rare subject of research in the mainland of China. Methods A time-series analysis was conducted to examine the association of outdoor air pollutants with hospital outpatient visits in Shanghai by using two-year daily data (2010-2011). Results Outdoor air pollution was found to be associated with an increased risk of outpatient visits for acute bronchitis in Shanghai. The effect estimates of air pollutants varied with the lag structures of the concentrations of the pollutants. For lag06, a 10μg/m3 increase in the concentrations of PM10, SO2, and NO2 corresponded to 0.94%(95%CI:0.83%, 1.05%), 11.12%(95%CI:10.76%, 11.48%), and 4.84%(95%CI: 4.49%, 5.18%) increases in hospital visits for acute bronchitis, respectively. These associations appeared to be stronger in females (P Conclusion Our analyses have provided the first evidence that the current air pollution level in China has an effect on acute bronchitis and that the rationale for further limiting air pollution levels in Shanghai should be strengthened.

  5. Alternative Refrigerant Evaluation for High-Ambient-Temperature Environments: R-22 and R-410A Alternatives for Mini-Split Air Conditioners

    Energy Technology Data Exchange (ETDEWEB)

    Abdelaziz, Omar [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Shrestha, Som S. [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Munk, Jeffrey D. [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Linkous, Randall Lee [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Goetzler, William [Navigant Consulting Inc., Burlington, MA (United States); Guernsey, Matt [Navigant Consulting Inc., Burlington, MA (United States); Kassuga, Theo [Navigant Consulting Inc., Burlington, MA (United States)

    2015-10-01

    The Oak Ridge National Laboratory (ORNL) High-Ambient-Temperature Evaluation Program for low– global warming potential (Low-GWP) Refrigerants aims to develop an understanding of the performance of low-GWP alternative refrigerants to hydrochlorofluorocarbon (HCFC) and hydrofluorocarbon (HFC) refrigerants in mini-split air conditioners under high-ambient-temperature conditions. This final report describes the parties involved, the alternative refrigerant selection process, the test procedures, and the final results.

  6. Alternative Refrigerant Evaluation for High-Ambient Temperature Environments: R-22 and R-410A Alternatives for Mini-Split Air Conditioners

    Energy Technology Data Exchange (ETDEWEB)

    Abdelaziz, Omar [ORNL; Munk, Jeffrey D [ORNL; Shrestha, Som S [ORNL; Linkous, Randall Lee [ORNL; Goetzler, William [Navigant Consulting Inc.; Guernsey, Matt [Navigant Consulting Inc.; Kassuga, Theo [Navigant Consulting Inc.

    2015-08-01

    The Oak Ridge National Laboratory (ORNL) High-Ambient Temperature Testing Program for Low-GWP Refrigerants aims to develop an understanding of the performance of low-Global Warming Potential (low-GWP) alternatives to Hydrochlorofluorocarbon (HCFC) and Hydrofluorocarbon (HFC) refrigerants in mini-split air conditioners under high ambient temperature conditions. This interim working paper describes the parties involved, the alternative refrigerants selection process, the test procedures, and the preliminary results.

  7. Climate change, extreme weather events, air pollution and respiratory health in Europe.

    Science.gov (United States)

    De Sario, M; Katsouyanni, K; Michelozzi, P

    2013-09-01

    Due to climate change and other factors, air pollution patterns are changing in several urbanised areas of the world, with a significant effect on respiratory health both independently and synergistically with weather conditions; climate scenarios show Europe as one of the most vulnerable regions. European studies on heatwave episodes have consistently shown a synergistic effect of air pollution and high temperatures, while the potential weather-air pollution interaction during wildfires and dust storms is unknown. Allergen patterns are also changing in response to climate change, and air pollution can modify the allergenic potential of pollens, especially in the presence of specific weather conditions. The underlying mechanisms of all these interactions are not well known; the health consequences vary from decreases in lung function to allergic diseases, new onset of diseases, exacerbation of chronic respiratory diseases, and premature death. These multidimensional climate-pollution-allergen effects need to be taken into account in estimating both climate and air pollution-related respiratory effects, in order to set up adequate policy and public health actions to face both the current and future climate and pollution challenges.

  8. Recent advances in improvement of forecast skill and understanding climate processes using AIRS Version-5 products

    Science.gov (United States)

    Susskind, Joel; Molnar, Gyula; Iredell, Lena; Rosenberg, Robert

    2012-10-01

    The NASA Goddard Earth Sciences (GES) Data and Information Services Center (DISC) generates products derived from AIRS/AMSU-A observations, starting from September 2002 when the AIRS instrument became stable, using the AIRS Science Team Version-5 retrieval algorithm. This paper shows results of some of our research using Version-5 products from the points of view of improving forecast skill as well as aiding in the understanding of climate processes.

  9. The impact of international shipping on European air quality and climate forcing

    Energy Technology Data Exchange (ETDEWEB)

    van Aardenne, J. [European Environment Agency (EEA), Copenhagen (Denmark); Colette, A. [INERIS (France); Degraeuwe, B.; de Vlieger, I. [VITO (Belgium); Hammingh, P. [PBL Netherlands Environmental Assessment Agency (Netherlands); Viana, M. [CSIC (Spain)

    2013-03-15

    This EEA Technical report provides an overview on the state of knowledge on the impact of international shipping in European waters to air quality and climate change. Based on literature review and model assessment studies information is provided on past and future emissions of air pollutants and greenhouse gases, monitoring of ship emissions, emission mitigation policies and impact on European air quality and radiative forcing. (Author)

  10. An Evaluation of Uncertainty Associated to Analytical Measurements of Selected Polycyclic Aromatic Compounds in Ambient Air; Estudio sobre las Incertidumbres Asociadas al Metodo de Determinacion de PAC's Seleccionados en Muestras de Aire Ambiente

    Energy Technology Data Exchange (ETDEWEB)

    Barrado, A. I.; Garcia, S.; Perez, R. M.

    2013-06-01

    This paper presents an evaluation of uncertainty associated to analytical measurement of eighteen polycyclic aromatic compounds (PACs) in ambient air by liquid chromatography with fluorescence detection (HPLC/FD). The study was focused on analyses of PM{sub 1}0, PM{sub 2}.5 and gas phase fractions. Main analytical uncertainty was estimated for eleven polycyclic aromatic hydrocarbons (PAHs), four nitro polycyclic aromatic hydrocarbons (nitro-PAHs) and two hydroxy polycyclic aromatic hydrocarbons (OH-PAHs) based on the analytical determination, reference material analysis and extraction step. Main contributions reached 15-30% and came from extraction process of real ambient samples, being those for nitro- PAHs the highest (20-30%). Range and mean concentration of PAC mass concentrations measured in gas phase and PM{sub 1}0/PM{sub 2}.5 particle fractions during a full year are also presented. Concentrations of OH-PAHs were about 2-4 orders of magnitude lower than their parent PAHs and comparable to those sparsely reported in literature. (Author) 7 refs.

  11. Downscaling a Global Climate Model to Simulate Climate Change Impacts on U.S. Regional and Urban Air Quality

    Science.gov (United States)

    Trail, M.; Tsimpidi, A. P.; Liu, P.; Tsigaridis, K.; Hu, Y.; Nenes, A.; Russell, A. G.

    2013-01-01

    Climate change can exacerbate future regional air pollution events by making conditions more favorable to form high levels of ozone. In this study, we use spectral nudging with WRF to downscale NASA earth system GISS modelE2 results during the years 2006 to 2010 and 2048 to 2052 over the continental United States in order to compare the resulting meteorological fields from the air quality perspective during the four seasons of five-year historic and future climatological periods. GISS results are used as initial and boundary conditions by the WRF RCM to produce hourly meteorological fields. The downscaling technique and choice of physics parameterizations used are evaluated by comparing them with in situ observations. This study investigates changes of similar regional climate conditions down to a 12km by 12km resolution, as well as the effect of evolving climate conditions on the air quality at major U.S. cities. The high resolution simulations produce somewhat different results than the coarse resolution simulations in some regions. Also, through the analysis of the meteorological variables that most strongly influence air quality, we find consistent changes in regional climate that would enhance ozone levels in four regions of the U.S. during fall (Western U.S., Texas, Northeastern, and Southeastern U.S), one region during summer (Texas), and one region where changes potentially would lead to better air quality during spring (Northeast). We also find that daily peak temperatures tend to increase in most major cities in the U.S. which would increase the risk of health problems associated with heat stress. Future work will address a more comprehensive assessment of emissions and chemistry involved in the formation and removal of air pollutants.

  12. Natural variation of ambient dose rate in the air of Izu-Oshima Island after the Fukushima Daiichi Nuclear Power Plant accident.

    Science.gov (United States)

    Maedera, Fumihiko; Inoue, Kazumasa; Sugino, Masato; Sano, Ryosuke; Furue, Mai; Shimizu, Hideo; Tsuruoka, Hiroshi; Le Van, Tan; Fukushi, Masahiro

    2016-03-01

    The ambient dose rate in air and radioactivity concentration in soil samples collected on Izu-Oshima Island were observed in 2012, 2013 and 2014, i.e. 1, 2 and 3 years after the severe accident at the Fukushima Daiichi Nuclear Power Plant. A car-borne survey for the ambient dose rate in air was carried out for the entire island. Soil samples were collected for the radioactivity concentration measurements from 22 points. The ambient dose rates in air were 36 nGy h(-1) in 2012, 34 nGy h(-1) in 2013 and 29 nGy h(-1) in 2014. The corresponding radioactivity concentrations in those years for (134)Cs were 53, 39 and 29 Bq kg(-1) and for (137)Cs, 87, 73 and 75 Bq kg(-1). All the values have decreased every year.

  13. Analysis of Ambient Air Quality in Shouyang County%寿阳县城环境空气质量分析

    Institute of Scientific and Technical Information of China (English)

    贾怡平

    2015-01-01

    通过对2014年10月至2015年5月山西省寿阳县城环境空气质量监测数据进行分析,反映了目前的县城环境空气质量,重点分析了臭氧污染,提出了一些建议,以便能改善县城的环境空气质量。%Through the analysis of ambient air quality monitoring data from October 2014 to May 2015 in Shouyang County ,Shanxi Province ,the results reflect the current ambient air quality of the county .The article focuses on the analysis of ozone pollution and puts forward some pieces of advices for improving ambient air quality of the county .

  14. 76 FR 6056 - Additional Air Quality Designations for the 2006 24-Hour Fine Particle National Ambient Air...

    Science.gov (United States)

    2011-02-03

    ...-5432 or by e-mail at: palma.elizabeth@epa.gov or Carla Oldham, Office of Air Quality Planning and... number (919) 541-3347 or by e-mail at: oldham.carla@epa.gov . Regional Office Contacts Region 4--Steve... open from 8:30 a.m. to 4:30 p.m. Monday through Friday, excluding legal holidays. The telephone...

  15. Exposure to ambient concentrations of particulate air pollution does not influence vascular function or inflammatory pathways in young healthy individuals

    Directory of Open Access Journals (Sweden)

    Vinzents Peter

    2008-10-01

    Full Text Available Abstract Background Particulate air pollution is associated with increased risk of cardiovascular events although the involved mechanisms are poorly understood. The objective of the present study was to investigate the effects of controlled exposure to ambient air fine and ultrafine particles on microvascular function and biomarkers related to inflammation, haemostasis and lipid and protein oxidation. Methods Twenty-nine subjects participated in a randomized, two-factor crossover study with or without biking exercise for 180 minutes and with 24 hour exposure to particle rich (number concentrations, NC: 11600 ± 5600 per cm3, mass concentrations: 13.8 ± 7.4 μg/m3 and 10.5 ± 4.8 μg/m3 for PM10-2.5 and PM2.5, respectively or particle filtered (NC: 555 ± 1053 per cm3 air collected above a busy street. Microvascular function was assessed non-invasively by measuring digital peripheral artery tone following arm ischemia. Biomarkers included haemoglobin, red blood cells, platelet count, coagulation factors, C-reactive protein, fibrinogen, interleukin-6, tumour necrosis factor α, lag time to copper-induced oxidation of plasma lipids and protein oxidation measured as 2-aminoadipic semialdehyde in plasma. Results No statistically significant differences were observed on microvascular function or the biomarkers after exposure to particle rich or particle filtered air. Conclusion This study indicates that exposure to air pollution particles at outdoor concentrations is not associated with detectable systemic inflammation, lipid or protein oxidation, altered haemostasis or microvascular function in young healthy participants.

  16. Retrospective screening of pesticide metabolites in ambient air using liquid chromatography coupled to high-resolution mass spectrometry.

    Science.gov (United States)

    López, Antonio; Yusà, Vicent; Millet, Maurice; Coscollà, Clara

    2016-04-01

    A new methodology for the retrospective screening of pesticide metabolites in ambient air was developed, using liquid chromatography coupled to Orbitrap high-resolution mass spectrometry (UHPLC-HRMS), including two systematic workflows (i) post-run target screening (suspect screening) and (ii) non-target screening. An accurate-mass database was built and used for the post-run screening analysis. The database contained 240 pesticide metabolites found in different matrixes such as air, soil, water, plants, animals and humans. For non-target analysis, a "fragmentation-degradation" relationship strategy was selected. The proposed methodology was applied to 31 air samples (PM10) collected in the Valencian Region (Spain). In the post-target analysis 34 metabolites were identified, of which 11 (3-ketocarburan, carbofuran-7-phenol, carbendazim, desmethylisoproturon, ethiofencarb-sulfoxide, malaoxon, methiocarb-sulfoxide, N-(2-ethyl-6-methylphenyl)-L-alanine, omethoate, 2-hydroxy-terbuthylazine, and THPAM) were confirmed using analytical standards. The semiquantitative estimated concentration ranged between 6.78 and 198.31 pg m(-3). Likewise, two unknown degradation products of malaoxon and fenhexamid were elucidated in the non-target screening.

  17. Ambient particulate air pollution and circulating antioxidant enzymes: A repeated-measure study in healthy adults in Beijing, China.

    Science.gov (United States)

    Wu, Shaowei; Wang, Bin; Yang, Di; Wei, Hongying; Li, Hongyu; Pan, Lu; Huang, Jing; Wang, Xin; Qin, Yu; Zheng, Chanjuan; Shima, Masayuki; Deng, Furong; Guo, Xinbiao

    2016-01-01

    The association of systemic antioxidant activity with ambient air pollution has been unclear. A panel of 40 healthy college students underwent repeated blood collection for 12 occasions under three exposure scenarios before and after relocating from a suburban area to an urban area in Beijing, China in 2010-2011. We measured various air pollutants including fine particles (PM2.5) and determined circulating levels of antioxidant enzymes extracellular superoxide dismutase (EC-SOD) and glutathione peroxidase 1 (GPX1) in the laboratory. An interquartile range increase of 63.4 μg/m(3) at 3-d PM2.5 moving average was associated with a 6.3% (95% CI: 0.6, 12.4) increase in EC-SOD and a 5.5% (95% CI: 1.3, 9.8) increase in GPX1. Several PM2.5 chemical constituents, including negative ions (nitrate and chloride) and metals (e.g., iron and strontium), were consistently associated with increases in EC-SOD and GPX1. Our results support activation of circulating antioxidant enzymes following exposure to particulate air pollution.

  18. Monoaromatic compounds in ambient air of various cities: a focus on correlations between the xylenes and ethylbenzene

    Science.gov (United States)

    Monod, Anne; Sive, Barkley C.; Avino, Pasquale; Chen, Tai; Blake, Donald R.; Sherwood Rowland, F.

    Speciation of o-xylene, m-xylene, p-xylene and ethylbenzene was performed by gas chromatography from ambient air and liquid fuel samples collected at various locations in 19 cities in Europe, Asia and South America. The xylene's mixing ratios were compared to each other from the various locations, which included urban air, traffic air and liquid fuel. For all samples, the xylenes exhibited robust correlations, and the slopes remained constant. The m-xylene/ p-xylene ratio was found to be 2.33±0.30, and the m-xylene/ o-xylene ratio was found to be 1.84±0.25. These ratios remain persistent even in biomass combustion experiments (in South America and South Africa). Comparing the xylenes to toluene and benzene indicate that combustion, but not fuel evaporation, is the major common source of the xylenes in areas dominated by automotive emissions. Although a wide range of combustion types and combustion efficiencies were encountered throughout all the locations investigated, xylenes and ethylbenzene ratios remained persistent. We discuss the implications of the constancies in the xylenes and ethylbenzene ratios on atmospheric chemistry.

  19. Determination of phase-distributed PAH in Rome ambient air by denuder/GC-MS method

    Science.gov (United States)

    Possanzini, Massimiliano; Di Palo, Vincenzo; Gigliucci, Pierfrancesco; Scianò, Maria Concetta Tomasi; Cecinato, Angelo

    An annular denuder—filter sampler has been tested for determination of both gaseous and particulate polycyclic aromatic hydrocarbons (PAH) in air. Collection efficiency and capacity over 6-h sampling at an air flow rate of 6 l min -1 were assessed. Concentrations were measured and phase distributions of the most important 2-6 ring PAH in air samples collected in downtown Rome during November 2002 to April 2003 were determined. The 2- and 3-ring PAH were found for more than 90% in the gas phase, whilst congeners with more than 4 rings were present almost entirely in the particle phase. Comparison with a high-volume filter—PUF sampler showed that similar results for total PAH contents (gas + particle) were observed only for congeners with molecular mass higher than 178 (phenanthrene and anthracene).

  20. Combined effects of road traffic noise and ambient air pollution in relation to risk for stroke?

    Science.gov (United States)

    Sørensen, Mette; Lühdorf, Pernille; Ketzel, Matthias; Andersen, Zorana J; Tjønneland, Anne; Overvad, Kim; Raaschou-Nielsen, Ole

    2014-08-01

    Exposure to road traffic noise and air pollution have both been associated with risk for stroke. The few studies including both exposures show inconsistent results. We aimed to investigate potential mutual confounding and combined effects between road traffic noise and air pollution in association with risk for stroke. In a population-based cohort of 57,053 people aged 50-64 years at enrollment, we identified 1999 incident stroke cases in national registries, followed by validation through medical records. Mean follow-up time was 11.2 years. Present and historical residential addresses from 1987 to 2009 were identified in national registers and road traffic noise and air pollution were modeled for all addresses. Analyses were done using Cox regression. A higher mean annual exposure at time of diagnosis of 10 µg/m(3) nitrogen dioxide (NO2) and 10 dB road traffic noise at the residential address was associated with ischemic stroke with incidence rate ratios (IRR) of 1.11 (95% CI: 1.03, 1.20) and 1.16 (95% CI: 1.07, 1.24), respectively, in single exposure models. In two-exposure models road traffic noise (IRR: 1.15) and not NO2 (IRR: 1.02) was associated with ischemic stroke. The strongest association was found for combination of high noise and high NO2 (IRR=1.28; 95% CI=1.09-1.52). Fatal stroke was positively associated with air pollution and not with traffic noise. In conclusion, in mutually adjusted models road traffic noise and not air pollution was associated ischemic stroke, while only air pollution affected risk for fatal strokes. There were indications of combined effects.

  1. Measurements and source apportionment of particle-associated polycyclic aromatic hydrocarbons in ambient air in Riyadh, Saudi Arabia

    Science.gov (United States)

    Bian, Qijing; Alharbi, Badr; Collett, Jeffrey; Kreidenweis, Sonia; Pasha, Mohammad J.

    2016-07-01

    Ambient air samples were obtained in Riyadh, the capital and largest city of Saudi Arabia, during two measurement campaigns spanning September 2011 to September 2012. Sixteen particle-phase polycyclic aromatic hydrocarbons (PAH) were quantified in 167 samples. Pyrene and fluoranthene were the most abundant PAH, with average of 3.37 ± 14.01 ng m-3 and 8.00 ± 44.09 ng m-3, respectively. A dominant contribution from low molecular weight (LMW) PAH (MW < 228) suggested a large influence of industrial emissions on PAH concentrations. Monte Carlo source apportionment using diagnostic ratios showed that 80 ± 10% of the average LMW PAH concentrations were contributed by petroleum vapor emissions, while 53 ± 19% of high molecular weight (HMW) PAH were from solid fuel combustion emissions. The positive matrix factorization model estimated that oil combustion emissions dominated total PAH concentrations, accounting for on average 96%, likely due to widespread use of oil fuels in energy production (power plants and industries). Our results demonstrate the significant influence of petroleum product production and consumption on particulate-phase PAH concentrations in Riyadh, but also point to the importance of traffic and solid fuel burning, including coke burning and seasonal biomass burning, especially as they contribute to the ambient levels of HMW PAH.

  2. Evaluation of the use of bioethanol fuelled buses based on ambient air pollution screening and on-road measurements.

    Science.gov (United States)

    López-Aparicio, S; Hak, C

    2013-05-01

    Mitigation measures to reduce greenhouse gas emissions may have adverse effects on urban air quality and human exposure to harmful pollutants. The use of bioethanol fuelled vehicles is increasing worldwide and may create new undesired pollution effects. Different measurement campaigns were performed in a pilot study to contribute to the understanding of the consequences associated with the use of bioethanol blended fuel (E95) on a series of pollutants. Ambient screening measurements of NO2, O3, acetic acid, formaldehyde and acetaldehyde were performed at different urban locations, exposed and not exposed to the circulation of bioethanol buses. In addition, volatile organic compounds were measured at the exhaust pipe of a bioethanol fuelled bus, both under idling conditions (carbonyls; DNPH cartridge) and under on-road driving conditions applying online monitoring (PTR-TOF). Higher ambient acetaldehyde values were measured at locations exposed to bioethanol fuelled buses than at locations not exposed, and very high acetaldehyde and acetic acid values were measured from the exhaust pipe during driving conditions (acetaldehyde>150 ppm; acetic acid ≈ 20-30 ppm) and modelled at close distance to the bioethanol bus. Human exposure to high concentration of acetaldehyde is expected, and it may involve a significantly increased chance in developing cancer. The high concentration of acetic acid will involve odour annoyance and significant material degradation or corrosion.

  3. Preliminary assessment of BTEX concentrations in indoor air of residential buildings and atmospheric ambient air in Ardabil, Iran

    Science.gov (United States)

    Hazrati, Sadegh; Rostami, Roohollah; Farjaminezhad, Manoochehr; Fazlzadeh, Mehdi

    2016-05-01

    BTEX concentrations in indoor and outdoor air of 50 homes were studied in Ardabil city and their influencing parameters including; heating system, using gas stove and samovar, tobacco smoking, the floors in which the monitored homes were located, and kitchen plan were considered in the study. Risk assessment analysis was carried out with the obtained concentrations based on EPA IRIS reference doses. BTEX compounds were sampled by charcoal tubes and the samples were analyzed by a GC-FID. Concentrations of benzene (15.18 μg/m3 vs. 8.65 μg/m3), toluene (69.70 μg/m3 vs. 40.56 μg/m3), ethylbenzene (12.07 μg/m3 vs. 4.92 μg/m3) and xylene (48.08 μg/m3 vs. 7.44 μg/m3) in indoor air were significantly (p < 0.05) higher than the levels quantified for outdoor air. The obtained concentrations of benzene were considerably higher than the recommended value of 5 μg/m3 established by Iran environmental protection organization. Among the BTEX compounds, benzene (HQ = 0.51) and xylene (HQ = 0.47) had notable hazard quotient and were the main pollutants responsible for high hazard index in the monitored homes (HI = 1.003). The results showed considerably high cancer risk for lifetime exposure to the indoor (125 × 10-6) and outdoor (71 × 10-6) benzene. Indoor benzene concentrations in homes were significantly influenced by type of heating system, story, and natural gas appliances.

  4. Volatile organic compounds in urban atmospheres: Long-term measurements of ambient air concentrations in differently loaded regions of Leipzig

    Energy Technology Data Exchange (ETDEWEB)

    Knobloch, T.; Asperger, A.; Engewald, W. [University of Leipzig, Institute of Analytical Chemistry, Leipzig (Germany)

    1997-09-01

    For the comprehensive characterization of ambient air concentrations of a broad spectrum of volatile organic compounds (VOCs) an analytical method is described, consisting of adsorptive enrichment, thermal desorption without cryofocusing, and capillary gas chromatographic separation. The method was applied during two-week measuring campaigns in winter and summer 1995, and in the winter of 1996. Long-term sampling was carried out at sampling points in residential areas in the suburbs and near the city center of Leipzig. About 70 VOCs - mainly hydrocarbons from propene to hexadecane - were identified both by GC-MS and chromatographic retention data and quantified after external calibration. Mean values of VOC concentrations obtained during the sampling periods are reported and discussed with regard to the topographical location of the sampling points in the Leipzig area, seasonal variations, and possible emission sources. (orig.) With 7 figs., 3 tabs., 18 refs.

  5. Splashing phenomena of room temperature liquid metal droplet striking on the pool of the same liquid under ambient air environment

    CERN Document Server

    Li, Haiyan; Wang, Lei; Gao, Yunxia; Liu, Jing

    2013-01-01

    In this article, the fluid dynamics of room temperature liquid metal (RTLM) droplet impacting onto a pool of the same liquid in ambient air was investigated. A series of experiments were conducted in order to disclose the influence of the oxidation effect on the impact dynamics. The droplet shape and impact phenomenology were recorded with the aid of a high-speed digital camera. The impact energy stored in the splash structures was estimated via a theoretical model and several morphological parameters obtained from instantaneous images of the splash. It was observed that the droplet shape and the splashing morphology of RTLM were drastically different from those of water, so was the impact dynamics between room temperature LM pool and high temperature LM pool. The energy analysis disclosed that the height of the jet is highly sensitive to the viscosity of the fluid, which is subjected to the oxidation effect and temperature effect simultaneously, and thus perfectly explained the phenomena. These basic finding...

  6. Research Update: Direct conversion of h-BN into pure c-BN at ambient temperatures and pressures in air

    Directory of Open Access Journals (Sweden)

    Jagdish Narayan

    2016-02-01

    Full Text Available We report a direct conversion of hexagonal boron nitride (h-BN into pure cubic boron nitride (c-BN by nanosecond laser melting at ambient temperatures and atmospheric pressure in air. According to the phase diagram, the transformation from h-BN into c-BN can occur only at high temperatures and pressures, as the hBN-cBN-Liquid triple point is at 3500 K/9.5 GPa. Using nanosecond laser melting, we have created super undercooled state and shifted this triple point to as low as 2800 K and atmospheric pressure. The rapid quenching from super undercooled state leads to formation of super undercooled BN (Q-BN. The c-BN phase is nucleated from Q-BN depending upon the time allowed for nucleation and growth.

  7. Dose-response-relation between croup syndrome/obstructive bronchitis and ambient air pollution in Baden-Wuerttemberg

    Energy Technology Data Exchange (ETDEWEB)

    Wichmann, H.E.; Beckmann, M.; Huebner, H.R.; Malin, E.M.; Rebmann, H.; Pizard-Weyrich, M.; Hippke, G.; Doeller, G.; Herrmann, S.; Horsch, F.; Filby, W.G.; Fund, N.; Gross, S.; Hanisch, B.; Kilz, E.; Seidel, A. (comps.)

    1988-04-01

    The data collection for the epidemiologic study which started in January 1986 has been completed. In Stuttgart, Tuebingen/Reutlingen/Rottenburg and Freudenstadt 188 physicians and 3 hospitals participated in the longitudinal study and more than 3000 cases of croup syndrome or obstructive bronchitis were reported. In the cross-sectional study the parents of more than 8000 children filled in a questionnaire, which corresponds to a response rate of about 90%. Of the positive virologic isolations approximately 50% were RS-viruses, 25% parainfluenza-viruses and 16% influenze-viruses. Parainfluenza viruses had their maximum during fall as croup syndrome had. In contrast RS-viruses were isolated more frequently in spring where also an increase of obstructive bronchitis was reported. During the winter of 1986 an epidemics of influenza B coincided with elevated numbers for both deseases. Statistical analysis of the data with respect to ambient air pollution is in process.

  8. Speciated mercury measurements in ambient air from 2009 to 2011 at a Central European rural background monitoring site

    Directory of Open Access Journals (Sweden)

    Weigelt A.

    2013-04-01

    Full Text Available Since January 2009 highly time-resolved mercury speciation measurements in ambient air are carried out at the Central European German EMEP monitoring station and measurement site of the German Federal Environment Agency “Waldhof“, providing the longest Central European dataset for mercury species. First statistical analyses do not indicate long term trends for the concentrations of gaseous elemental mercury (GEM and particle bound mercury (TPM. A potential increasing trend for reactive gaseous mercury (RGM will have to be verified in the coming years and should be regarded as indicative only at present. A seasonal cycle for TPM could be observed with higher concentrations during winter time. Furthermore a diurnal cycle for RGM is apparent with highest concentrations in the early afternoon.

  9. Research Update: Direct conversion of h-BN into pure c-BN at ambient temperatures and pressures in air

    Energy Technology Data Exchange (ETDEWEB)

    Narayan, Jagdish, E-mail: narayan@ncsu.edu; Bhaumik, Anagh [Department of Materials Science and Engineering, Centennial Campus, North Carolina State University, Raleigh, North Carolina 27695-7907 (United States)

    2016-02-01

    We report a direct conversion of hexagonal boron nitride (h-BN) into pure cubic boron nitride (c-BN) by nanosecond laser melting at ambient temperatures and atmospheric pressure in air. According to the phase diagram, the transformation from h-BN into c-BN can occur only at high temperatures and pressures, as the hBN-cBN-Liquid triple point is at 3500 K/9.5 GPa. Using nanosecond laser melting, we have created super undercooled state and shifted this triple point to as low as 2800 K and atmospheric pressure. The rapid quenching from super undercooled state leads to formation of super undercooled BN (Q-BN). The c-BN phase is nucleated from Q-BN depending upon the time allowed for nucleation and growth.

  10. Enhanced photovoltaic performance of planar perovskite solar cells fabricated in ambient air by solvent annealing treatment method

    Science.gov (United States)

    Obiozo Eze, Vincent; Mori, Tatsuo

    2016-12-01

    In this paper, we report on planar perovskite solar cells (PSCs) fabricated by a simple one-step solution process and an antisolvent bath (ASB) method in ambient air. The ASB method enabled the efficient extraction of the precursor solvent and induced the swift crystallization of uniform and highly smooth perovskite films with an average grain size of about 0.34 µm. The morphology and grain growth of the resultant perovskite film were further improved by solvent annealing (SA) under dimethyl sulfoxide (DMSO) vapor atmosphere at 150 °C for 10 min and thus an average power conversion efficiency (PCE) of 15.20% and a maximum efficiency of 16.77% were achieved. This work highlights the importance of solvent annealing for perovskite prepared by a one-step solution process and an ASB method, and offers a facile and attractive way to fabricate high-performance perovskite solar cells.

  11. 76 FR 8157 - National Ambient Air Quality Standards for Carbon Monoxide

    Science.gov (United States)

    2011-02-11

    ... consumption conditions make boiler combustion highly efficient. In contrast, internal combustion engines used..., exercise (which increases the amount of air removed and replaced per unit of time for gas exchange), the... performed for previous reviews have included modeling simulations both without and with indoor sources...

  12. Acute effects of ambient air pollution episodes on respiratory health of children.

    NARCIS (Netherlands)

    Hoek, G.

    1992-01-01

    In this thesis the acute effects of air pollution episodes on respiratory health of seven to eleven year old children living in non-urban communities in the Netherlands are discussed. Repeated measurements of pulmonary function (spirometry) and the occurrence of acute respiratory symptoms using a da

  13. Vascular Effects of a Subchronic Inhalation Exposure to Concentrated Ambient Air Particles in Atherosclerosis Susceptible Mice

    Science.gov (United States)

    Numerous studies have reported the adverse effects of particulate air pollution on cardiovascular function and disease. The causal physiochemical properties of particles and their mechanisms of action/injury remain unknown. This study examined the vascular effects in 15 wk old ma...

  14. Concentrations in ambient air and emissions of cyclic volatile methylsiloxanes in Zurich, Switzerland.

    Science.gov (United States)

    Buser, Andreas M; Kierkegaard, Amelie; Bogdal, Christian; MacLeod, Matthew; Scheringer, Martin; Hungerbühler, Konrad

    2013-07-02

    Tens of thousands of tonnes of cyclic volatile methylsiloxanes (cVMS) are used each year globally, which leads to high and continuous cVMS emissions to air. However, field measurements of cVMS in air and empirical information about emission rates to air are still limited. Here we present measurements of decamethylcyclopentasiloxane (D5) and dodecamethylcyclohexasiloxane (D6) in air for Zurich, Switzerland. The measurements were performed in January and February 2011 over a period of eight days and at two sites (city center and background) with a temporal resolution of 6-12 h. Concentrations of D5 and D6 are higher in the center of Zurich and range from 100 to 650 ng m(-3) and from 10 to 79 ng m(-3), respectively. These values are among the highest levels of D5 and D6 reported in the literature. In a second step, we used a multimedia environmental fate model parametrized for the region of Zurich to interpret the levels and time trends in the cVMS concentrations and to back-calculate the emission rates of D5 and D6 from the city of Zurich. The average emission rates obtained for D5 and D6 are 120 kg d(-1) and 14 kg d(-1), respectively, which corresponds to per-capita emissions of 310 mg capita(-1) d(-1) for D5 and 36 mg capita(-1) d(-1) for D6.

  15. Emission of linalool from Valencia orange blossoms and its observation in ambient air

    Science.gov (United States)

    Arey, Janet; Corchnoy, Stephanie B.; Atkinson, Roger

    Emission measurements made over a 5-month period of a Valencia orange tree showed the significant emission of the terpenoid linalool (C 10H 18O) from Valencia orange blossoms. The average annual emission rate of this Olinda Valencia orange, derived from emission measurements which include the blossoming season, is a factor of ˜10 higher than the average annual emission rate derived from measurements taken outside of the blossom season. Ambient monoterpene and linalool concentrations were measured in Riverside, California, in the spring and supported the chamber plant emissions data, with linalool concentrations as high as 17 μg m -3 being observed in an orange grove. These results show that current biogenic emission inventories which are formulated from limited survey data, generally not including seasonal variations in the vegetative emissions, can be subject to large uncertainties.

  16. Measurement of polycyclic aromatic hydrocarbons in ambient air by fluorescence spectroscopic techniques

    OpenAIRE

    Elcoroaristizabal Martin, Saioa

    2015-01-01

    250 p. + anexos Este proyecto de Tesis Doctoral se inició en marzo de 2011 gracias a la becapredoctoral otorgada por la Universidad del País Vasco (UPV/EHU), a través delprograma de ¿Formación de Personal Investigador¿, para trabajar en el Grupo deInvestigación Atmosférica (GIA) del Departamento de Ingeniería Química y del MedioAmbiente de la Escuela Técnica Superior de Ingeniería de Bilbao (Universidad delPaís Vasco, UPV/EHU). Asimismo, parte de este trabajo de investigación se hadesarrol...

  17. Calculating Air Quality and Climate Co-Benefits Metrics from Adjoint Elasticities in Chemistry-Climate Models

    Science.gov (United States)

    Spak, S.; Henze, D. K.; Carmichael, G. R.

    2013-12-01

    The science and policy communities both need common metrics that clearly, comprehensively, and intuitively communicate the relative sensitivities of air quality and climate to emissions control strategies, include emissions and process uncertainties, and minimize the range of error that is transferred to the metric. This is particularly important because most emissions control policies impact multiple short-lived climate forcing agents, and non-linear climate and health responses in space and time limit the accuracy and policy value of simple emissions-based calculations. Here we describe and apply new second-order elasticity metrics to support the direct comparison of emissions control policies for air quality and health co-benefits analyses using adjoint chemical transport and chemistry-climate models. Borrowing an econometric concept, the simplest elasticities in the atmospheric system are the percentage changes in concentrations due to a percentage change in the emissions. We propose a second-order elasticity metric, the Emissions Reduction Efficiency, which supports comparison across compounds, to long-lived climate forcing agents like CO2, and to other air quality impacts, at any temporal or spatial scale. These adjoint-based metrics (1) possess a single uncertainty range; (2) allow for the inclusion of related health and other impacts effects within the same framework; (3) take advantage of adjoint and forward sensitivity models; and (4) are easily understood. Using global simulations with the adjoint of GEOS-Chem, we apply these metrics to identify spatial and sectoral variability in the climate and health co-benefits of sectoral emissions controls on black carbon, sulfur dioxide, and PM2.5. We find spatial gradients in optimal control strategies on every continent, along with differences among megacities.

  18. Nonradioactive Ambient Air Monitoring at Los Alamos National Laboratory 2001--2002

    Energy Technology Data Exchange (ETDEWEB)

    E. Gladney; J.Dewart, C.Eberhart; J.Lochamy

    2004-09-01

    During the spring of 2000, the Cerro Grande forest fire reached Los Alamos National Laboratory (LANL) and ignited both above-ground vegetation and disposed materials in several landfills. During and after the fire, there was concern about the potential human health impacts from chemicals emitted by the combustion of these Laboratory materials. Consequently, short-term, intensive air-monitoring studies were performed during and shortly after the fire. Unlike the radiological data from many years of AIRNET sampling, LANL did not have an adequate database of nonradiological species under baseline conditions with which to compare data collected during the fire. Therefore, during 2001 the Meteorology and Air Quality Group designed and implemented a new air-monitoring program, entitled NonRadNET, to provide nonradiological background data under normal conditions. The objectives of NonRadNET were to: (1) develop the capability for collecting nonradiological air-monitoring data, (2) conduct monitoring to develop a database of typical background levels of selected nonradiological species in the communities nearest the Laboratory, and (3) determine LANL's potential contribution to nonradiological air pollution in the surrounding communities. NonRadNET ended in late December 2002 with five quarters of data. The purpose of this paper is to organize and describe the NonRadNET data collected over 2001-2002 to use as baseline data, either for monitoring during a fire, some other abnormal event, or routine use. To achieve that purpose, in this paper we will: (1) document the NonRadNET program procedures, methods, and quality management, (2) describe the usual origins and uses of the species measured, (3) compare the species measured to LANL and other area emissions, (4) present the five quarters of data, (5) compare the data to known typical environmental values, and (6) evaluate the data against exposure standards.

  19. The application of an improved gas and aerosol collector for ambient air pollutants in China

    Science.gov (United States)

    Dong, Huabin; Zeng, Limin; Zhang, Yuanhang; Hu, Min; Wu, Yusheng

    2016-04-01

    An improved Gas and Aerosol Collector (GAC) equipped with a newly designed aerosol collector and a set of dull-polished wet annular denuder (WAD) was developed by Peking University based on a Steam Jet Aerosol Collector (SJAC) sampler. Combined with Ion Chromatography (IC) the new sampler performed well in laboratory tests with high collection efficiencies for SO2 (above 98 %) and particulate sulfate (as high as 99.5 %). An inter-comparison between the GAC-IC system and the filter-pack method was performed and the results indicated that the GAC-IC system could supply reliable particulate sulfate, nitrate, chloride, and ammonium data in field measurement with a much wider range of ambient concentrations. From 2008 to 2015, dozens of big field campaigns (rural and coastal sites) were executed in different parts of China, the GAC-IC system took the chance having its field measurement performance checked repeatedly and provided high quality data in ambient conditions either under high loadings of pollutants or background area. Its measurements were highly correlated with data by other commercial instruments such as the SO2 analyzer, the HONO analyzer, a filter sampler, Aerosol Mass Spectrometer (AMS), etc. over a wide range of concentrations and proved particularly useful in future intensive campaigns or long-term monitoring stations to study various environmental issues such as secondary aerosol and haze formation. During these years of applications of GAC-IC in those field campaigns, we found some problems of several instruments running under field environment and some interesting results could also be drew from the large amount of data measured in near 20 provinces of China. Detail results will be demonstrated on the poster afterwards.

  20. Fundamental Study of Nano-Scale Adhesion and Friction Properties of Graphene in Ambient Air and Liquid Environments

    Science.gov (United States)

    Ramayanam, Sai Suvineeth

    The aim of this study is to understand the fundamental tribological interactions of model contacts developed between a 'single' asperity silicon tip and a few layer graphene surface in ambient air, ionic liquid, and lubricating oil environments. The motivation to investigate such fundamental interactions stems from the need to gain an understanding of the tribological properties, morphology and defects of few layer graphene with respect to different synthesis methods including both bottom-up and top-down approaches. In particular, the surface properties of atomically thin sheets of graphene synthesized by three methods; (i) liquid phase exfoliation of graphene, (ii) chemical reduction of exfoliated graphene oxide, on a silicon oxide substrate, and (iii) graphene synthesis by halogen based plasma etching on a silicon carbide substrate are studied using atomic force microscopy, lateral force microscopy and x-ray photoelectron spectroscopy. Friction of Si 'single' asperities sliding against a few layer graphene surface in ambient air, ionic liquid, and lubricating oil environments is reported. It is found that oxygen based defects play a major role in controlling the friction and adhesion properties of few layer graphene surfaces. The role of substrate and its bonding with the few layer graphene is also an important parameter. In liquids, we report a newly observed Stribeck like behavior in the nanoscale. This work can lead to important device applications with reduced friction such as contact-based microelectromechanical systems. It also sheds light on liquid-graphene interfacial characteristics which can be proved vital in applications spanning from electrochemical energy devices to nanolubricants.

  1. Climate change and pollutant emissions impacts on air quality in 2050 over Portugal

    Science.gov (United States)

    Sá, E.; Martins, H.; Ferreira, J.; Marta-Almeida, M.; Rocha, A.; Carvalho, A.; Freitas, S.; Borrego, C.

    2016-04-01

    Changes in climate and air pollutant emissions will affect future air quality from global to urban scale. In this study, regional air quality simulations for historical and future periods are conducted, with CAMx version 6.0, to investigate the impacts of future climate and anthropogenic emission projections on air quality over Portugal and the Porto metropolitan area in 2050. The climate and the emission projections were derived from the Representative Concentrations Pathways (RCP8.5) scenario. Modelling results show that climate change will impact NO2, PM10 and O3 concentrations over Portugal. The NO2 and PM10 annual means will increase in Portugal and in the Porto municipality, and the maximum 8-hr daily O3 value will increase in the Porto suburban areas (approximately 5%) and decrease in the urban area (approximately 2%). When considering climate change and projected anthropogenic emissions, the NO2 annual mean decreases (approximately 50%); PM10 annual mean will increase in Portugal and decrease in Porto municipality (approximately 13%); however PM10 and O3 levels increase and extremes occur more often, surpassing the currently legislated annual limits and displaying a higher frequency of daily exceedances. This air quality degradation is likely to be related with the trends found for the 2046-2065 climate, which implies warmer and dryer conditions, and with the increase of background concentrations of ozone and particulate matter. The results demonstrate the need for Portuguese authorities and policy-makers to design and implement air quality management strategies that take climate change impacts into account.

  2. Some reflections on researches of Future Earth changes in air quality and climate

    Institute of Scientific and Technical Information of China (English)

    ZHANG; Xiao-Ye

    2015-01-01

    Within the context of our current research and understanding of climate change,decisionmakers are particularly concerned with the extent of future climate change,its comprehensive impact,and the types of socioeconomic pathways available with respect to mitigation and adaptation.Among the factors contributing to these important issues,the role of air pollution in global and regional climate warming remains as one of the largest uncertainties.On the basis of understanding of the IPCC Fifth Assessment Report,specifically,in the role of air pollution in climate change,scenarios establishment,and relationship between the Shared Socioeconomic Pathways(SSPs) and Representative Concentration Pathways(RCPs).Weaknesses and reflections were discussed here especially in strengthening impact,adaptation and mitigation research that related with changes in air pollution and climate.In the future,there are needs to in-depth understand how and why the air pollution in China is so serious and changing; to understand the likely future changes in air pollution and climate; to strengthen comprehensive impact research and selective reduction strategies related to changes in air pollution and climate.Furthermore,this study outlines the needs to develop strategies to close the loop of differential impacts and costs; to establish co-benefits and sustainable development goals,to identify the crucial risks and options for synergies/trade-offs; to integrate sector-specific details with macro-economics,and to integrate the assessments of the various policy instruments.All these focus areas will help to facilitate the transition of economic development patterns towards green and low-carbon development.

  3. Some reflections on researches of Future Earth changes in air quality and climate

    Directory of Open Access Journals (Sweden)

    Xiao-Ye Zhang

    2015-06-01

    Full Text Available Within the context of our current research and understanding of climate change, decisionmakers are particularly concerned with the extent of future climate change, its comprehensive impact, and the types of socioeconomic pathways available with respect to mitigation and adaptation. Among the factors contributing to these important issues, the role of air pollution in global and regional climate warming remains as one of the largest uncertainties. On the basis of understanding of the IPCC Fifth Assessment Report, specifically, in the role of air pollution in climate change, scenarios establishment, and relationship between the Shared Socioeconomic Pathways (SSPs and Representative Concentration Pathways (RCPs. Weaknesses and reflections were discussed here especially in strengthening impact, adaptation and mitigation research that related with changes in air pollution and climate. In the future, there are needs to in-depth understand how and why the air pollution in China is so serious and changing; to understand the likely future changes in air pollution and climate; to strengthen comprehensive impact research and selective reduction strategies related to changes in air pollution and climate. Furthermore, this study outlines the needs to develop strategies to close the loop of differential impacts and costs; to establish co-benefits and sustainable development goals, to identify the crucial risks and options for synergies/trade-offs; to integrate sector-specific details with macro-economics, and to integrate the assessments of the various policy instruments. All these focus areas will help to facilitate the transition of economic development patterns towards green and low-carbon development.

  4. Impacts of household coal and biomass combustion on indoor and ambient air quality in China: Current status and implication.

    Science.gov (United States)

    Li, Qing; Jiang, Jingkun; Wang, Shuxiao; Rumchev, Krassi; Mead-Hunter, Ryan; Morawska, Lidia; Hao, Jiming

    2017-01-15

    This review briefly introduces current status of indoor and ambient air pollution originating from household coal and biomass combustion in mainland China. Owing to low combustion efficiency, emissions of CO, PM2.5, black carbon (BC), and polycyclic aromatic hydrocarbons have significant adverse consequences for indoor and ambient air qualities, resulting in relative contributions of more than one-third in all anthropogenic emissions. Their contributions are higher in less economically developed regions, such as Guizhou (61% PM2.5, 80% BC), than that in more developed regions, such as Shanghai (4% PM2.5, 17% BC). Chimneys can reduce ~80% indoor PM2.5 level when burning dirty solid fuels, such as plant materials. Due to spending more time near stoves, housewives suffer much more (~2 times) PM2.5 than the adult men, especially in winter in northern China (~4 times). Improvement of stove combustion/thermal efficiencies and solid fuel quality are the two essential methods to reduce pollutant emissions. PM2.5 and BC emission factors (EFs) have been identified to increase with volatile matter content in traditional stove combustion. EFs of dirty fuels are two orders higher than that of clean ones. Switching to clean ones, such as semi-coke briquette, was identified to be a feasible path for reducing >90% PM2.5 and BC emissions. Otherwise, improvement of thermal and combustion efficiencies by using under-fire technology can reduce ~50% CO2, 87% NH3, and 80% PM2.5 and BC emissions regardless of volatile matter content in solid fuel. However, there are still some knowledge gaps, such as, inventory for the temporal impact of household combustion on air quality, statistic data for deployed clean solid fuels and advanced stoves, and the effect of socioeconomic development. Additionally, further technology research for reducing air pollution emissions is urgently needed, especially low cost and clean stove when burning any type of solid fuel. Furthermore, emission

  5. The Impact of Individual Anthropogenic Emissions Sectors on the Global Burden of Human Mortality due to Ambient Air Pollution

    Science.gov (United States)

    Silva, Raquel A.; Adelman, Zachariah; Fry, Meridith M.; West, J. Jason

    2016-01-01

    Background: Exposure to ozone and fine particulate matter (PM2.5) can cause adverse health effects, including premature mortality due to cardiopulmonary diseases and lung cancer. Recent studies quantify global air pollution mortality but not the contribution of different emissions sectors, or they focus on a specific sector. Objectives: We estimated the global mortality burden of anthropogenic ozone and PM2.5, and the impact of five emissions sectors, using a global chemical transport model at a finer horizontal resolution (0.67° × 0.5°) than previous studies. Methods: We performed simulations for 2005 using the Model for Ozone and Related Chemical Tracers, version 4 (MOZART-4), zeroing out all anthropogenic emissions and emissions from specific sectors (All Transportation, Land Transportation, Energy, Industry, and Residential and Commercial). We estimated premature mortality using a log-linear concentration–response function for ozone and an integrated exposure–response model for PM2.5. Results: We estimated 2.23 (95% CI: 1.04, 3.33) million deaths/year related to anthropogenic PM2.5, with the highest mortality in East Asia (48%). The Residential and Commercial sector had the greatest impact globally—675 (95% CI: 428, 899) thousand deaths/year—and in most regions. Land Transportation dominated in North America (32% of total anthropogenic PM2.5 mortality), and it had nearly the same impact (24%) as Residential and Commercial (27%) in Europe. Anthropogenic ozone was associated with 493 (95% CI: 122, 989) thousand deaths/year, with the Land Transportation sector having the greatest impact globally (16%). Conclusions: The contributions of emissions sectors to ambient air pollution–related mortality differ among regions, suggesting region-specific air pollution control strategies. Global sector-specific actions targeting Land Transportation (ozone) and Residential and Commercial (PM2.5) sectors would particularly benefit human health. Citation: Silva RA

  6. A two-time-period comparison of the effects of ambient air pollution on outpatient visits for acute respiratory illnesses.

    Science.gov (United States)

    Sinclair, Amber Hughes; Edgerton, Eric S; Wyzga, Ron; Tolsma, Dennis

    2010-02-01

    Concentrations of numerous ambient air pollutants have declined in recent years across the United States. Although it can be expected that reductions in air pollutants are associated with reductions in health effects, it is unclear whether this is actually the case. The purpose of this analysis was to compare the levels of and relationships between air pollutants and acute respiratory outpatient visits for two consecutive time periods totaling 53 mo. Air pollution data were collected at a centrally located monitor in Atlanta, GA, and include 24-hr averages of particulate matter (PM) less than 2.5 microm in aerodynamic diameter (PM2.5) and its components; coarse PM (PM10-2.5); PM less than 10 microm in aerodynamic diameter (PM10); oxygenated volatile organic compounds (OVOCs); 8-hr maximum ozone (O3); and 1-hr maximum nitrogen dioxide (NO2), carbon monoxide (CO), and sulfur dioxide (SO2). In addition, several metals and fractions of elemental carbon (EC) and organic carbon (OC) were investigated. Daily outpatient visit data were obtained from the electronic data warehouse of the Atlanta-based region of a nonprofit managed care organization. Poisson general linear modeling determined associations between daily levels of acute visits for four diagnosis groups (adult and child asthma, upper and lower respiratory infection) and air pollution measurements. Overall declining trends were observed in air pollutants and acute visits over the study period. Childhood asthma had the greatest number of significant associations with air pollutants, namely zinc and EC. The significant lag time between pollutant measurement and visit occurrence changed from 3-5 days in the first time period to 6-8 days in the later time period, but there was general consistency in several childhood asthma and pollutant associations over both time periods. The greatest evidence for a reduction in pollution being associated with an improvement in health response was for lower respiratory disease

  7. Comparison of road traffic emission factors and testing by comparison of modelled and measured ambient air quality data.

    Science.gov (United States)

    Peace, H; Owen, B; Raper, D W

    2004-12-01

    This paper describes a comparison of three different sets of road traffic emission factors released by the UK government for use in air quality review and assessment. The air quality management process of review and assessment began in 1997 in the UK. During this period of ongoing review and assessment, a number of changes have been made to the emission factors provided by the government. The use of different sets of emission factors during the assessment process has lead to some inconsistencies between results from neighbouring local authorities and also between different modelling exercises undertaken by the same local authorities. One purpose of this study has been to compare three different sets of emission factors, including the most recent set, and to some degree highlight the uncertainty associated with the use of factors, such as the shift of emphasis in terms of emissions from cars to heavy goods vehicles. The most recently released emission factors are the most comprehensive to date, and theoretically more accurate than previous sets due to the larger database of emission measurements that they have been based on. Therefore, the most recent set of emission factors have been additionally used in a validation exercise between modelled and monitored data. Comparison has been undertaken with monitoring data at a variety of urban background, urban centre and roadside sites. This work has shown some differences between the predicted trends in emission factors and measured trends in ambient air pollution levels, especially at roadside sites, indicating an under-prediction of the air pollution contribution from road traffic.

  8. Exposure to Ultrafine Particles from Ambient Air and Oxidative Stress-Induced DNA Damage

    DEFF Research Database (Denmark)

    Bräuner, Elvira Vaclavik; Forchhammer, Lykke; Møller, Peter

    2007-01-01

    BACKGROUND: Particulate matter, especially ultrafine particles (UFPs), may cause health effects through generation of oxidative stress, with resulting damage to DNA and other macromolecules. OBJECTIVE: We investigated oxidative damage to DNA and related repair capacity in peripheral blood...... mononuclear cells (PBMCs) during controlled exposure to urban air particles with assignment of number concentration (NC) to four size modes with average diameters of 12, 23, 57, and 212 nm. DESIGN. Twenty-nine healthy adults participated in a randomized, two-factor cross-over study with or without biking...... exercise for 180 min and with exposure to particles (NC 6169-15362/cm3) or filtered air (NC 91-542/cm3) for 24 hr. METHODS: The levels of DNA strand breaks (SBs), oxidized purines as formamidopyrimidine DNA glycolase (FPG) sites, and activity of 7,8-dihydro-8-oxoguanine-DNA glycosylase (OGG1) in PBMCs were...

  9. Pollution Response Score of Tree Species in Relation to Ambient Air Quality in an Urban Area.

    Science.gov (United States)

    Mukherjee, Arideep; Agrawal, Madhoolika

    2016-02-01

    Multivariate statistical techniques were employed on twelve leaf traits in four selected common tree species (Mangifera indica L., Polyalthia longifolia Sonn., Ficus benghalensis L. and Psidium guajava L.) to evaluate their responses with respect to major air pollutants in an urban area. Discriminant analysis (DA) identified chlorophyll/carotenoid ratio, leaf dry matter content, carotenoids, net water content and ascorbic acid as the major discriminating leaf traits, which varied maximally with respect to the pollution status. Pollution response score (PRS), calculated on the basis of discriminate functional coefficient values, increased with an increase in air pollution variables for all the tested species, with the highest increase in P. longifolia and the lowest in F. benghalensis. The study highlights the usefulness of DA for evaluation of plant specific traits and PRS for selection of tolerant species.

  10. Summer concentrations of NMHCs in ambient air of the Arctic and Antarctic

    Energy Technology Data Exchange (ETDEWEB)

    Hellen, H.; Paatero, J.; Hakola, H.; Virkkula, A. [Finnish Meteorological Inst., Helsinki (Finland); Leck, C. [Stockholm Univ. (Sweden). Dept. of Meteorology

    2012-11-01

    Summer concentrations of C{sub 2}-C{sub 6} non-methane hydrocarbons (NMHCs) were measured in Antarctica and in the Arctic in 2008. The results show that NMHC concentrations are on average five times higher in the Arctic than in Antarctica. In Antarctica, there were few concentration peaks, but during most of the remaining time concentrations were below or close to the detection limits. Over the Arctic pack ice area north of 80 deg, concentrations of most of the measured NMHCs were always above the detection limits. No differences based on air-mass origin were detected in Antarctica, but samples collected over the central Arctic Ocean showed higher concentrations in air masses being advected from the Kara Sea and the western-central Arctic Ocean. The relatively higher NMHC-to-ethyne molar ratios calculated for samples collected over the central Arctic Ocean suggest additional alkane sources in the region. (orig.)

  11. Urban air pollution, climate and its impact on asthma morbidity

    Institute of Scientific and Technical Information of China (English)

    Lyudmila Vasilievna Veremchuk; Vera Innokentievna Yankova; Tatyana Isaakovna Vitkina; Anna Vladimirovna Nazarenko; Kirill Sergeevich Golokhvast

    2016-01-01

    Objective: To study the mechanism of formation of air quality and to determine the impact of the studied factors on asthma morbidity in Vladivostok. Methods: The evaluation of air pollution in Vladivostok was done using long-term (2008–2012) monitoring data (temperature, humidity, atmospheric pressure, wind speed, etc.). The levels of suspended particulate matter, nitrogen and sulfur dioxide, carbon monoxide, ammonia, formaldehyde (mg/m3) in six stationary observation posts were assessed. We studied the aerosol suspensions of solid particles, which were collected during snowfall from precipitation (snow) and air in 14 districts with different levels of anthropogenic impact. Melted snow was analyzed on laser granulometry. The impact of air pollution on the distribution of asthma morbidity was evaluated in various age groups by data of federal statistical observation obtained from 8 adults and 7 children municipal clinics in Vladivostok (2008–2012). Results: The content of suspended particulate components of pollution remained more stable, due to the features of atmospheric circulation, rugged terrain and residential development. The nano- and micro-sized particles (0–50 mm), which can absorb highly toxic metals, prevail in dust aerosols. These respirable fractions of particles, even in small doses, can contribute to the increase in asthma morbidity in the city. Conclusions: We determined that asthma morbidity depends from general air pollution (in the range of 18.3%). It was detected that the highest age-specific dependence is associated with the content of particulate matter, carbon monoxide and nitrogen dioxide in air.

  12. Salt Survey Comparison of Pressurized vs Ambient Deck Air Intakes on JEFF (B) Hovercraft

    Science.gov (United States)

    1981-02-02

    10 Vegetation Collected on Lift Fan Screen 21 Figure 11 Paint Stripping in Lift Fan Shows Dirty vs Clean Air 22 APPENDIX FIGURES Figure A-l Nuclepore...terms of the readings on deck and that ingested in No. 6 engine. Although one single reading is insufficient to draw any fir * conclusions, these data, on...salt above 0.14 PPM, correlates with AVCO experimental data (TF-35 engine). 11. The pressurized engine data demonstrated that the effectof leakage

  13. Air pollutant emissions from Chinese households: A major and underappreciated ambient pollution source.

    Science.gov (United States)

    Liu, Jun; Mauzerall, Denise L; Chen, Qi; Zhang, Qiang; Song, Yu; Peng, Wei; Klimont, Zbigniew; Qiu, Xinghua; Zhang, Shiqiu; Hu, Min; Lin, Weili; Smith, Kirk R; Zhu, Tong

    2016-07-12

    As part of the 12th Five-Year Plan, the Chinese government has developed air pollution prevention and control plans for key regions with a focus on the power, transport, and industrial sectors. Here, we investigate the contribution of residential emissions to regional air pollution in highly polluted eastern China during the heating season, and find that dramatic improvements in air quality would also result from reduction in residential emissions. We use the Weather Research and Forecasting model coupled with Chemistry to evaluate potential residential emission controls in Beijing and in the Beijing, Tianjin, and Hebei (BTH) region. In January and February 2010, relative to the base case, eliminating residential emissions in Beijing reduced daily average surface PM2.5 (particulate mater with aerodynamic diameter equal or smaller than 2.5 micrometer) concentrations by 14 ± 7 μg⋅m(-3) (22 ± 6% of a baseline concentration of 67 ± 41 μg⋅m(-3); mean ± SD). Eliminating residential emissions in the BTH region reduced concentrations by 28 ± 19 μg⋅m(-3) (40 ± 9% of 67 ± 41 μg⋅m(-3)), 44 ± 27 μg⋅m(-3) (43 ± 10% of 99 ± 54 μg⋅m(-3)), and 25 ± 14 μg⋅m(-3) (35 ± 8% of 70 ± 35 μg⋅m(-3)) in Beijing, Tianjin, and Hebei provinces, respectively. Annually, elimination of residential sources in the BTH region reduced emissions of primary PM2.5 by 32%, compared with 5%, 6%, and 58% achieved by eliminating emissions from the transportation, power, and industry sectors, respectively. We also find air quality in Beijing would benefit substantially from reductions in residential emissions from regional controls in Tianjin and Hebei, indicating the value of policies at the regional level.

  14. Estimation of the effects of ambient air pollution on life expectancy of urban residents in China

    Science.gov (United States)

    Wang, Cuicui; Zhou, Xiaodan; Chen, Renjie; Duan, Xiaoli; Kuang, Xingya; Kan, Haidong

    2013-12-01

    The air quality in China's cities has improved in recent years, but its impact on public health has rarely been investigated. This study was aimed at estimating the potential effects of air quality on life expectancy between 2003 and 2010 in China. We collected annual average concentrations of particulate matter less than 10 microns in aerodynamic diameter (PM10) in 113 key cities, covering all provinces in China, along with the national average age-specific mortality from 2003 to 2010. We constructed a cause-eliminated life table after excluding premature deaths attributable to PM10. The annual average PM10 levels in these cities decreased from 125.3 μg m-3 in 2003 to 88.3 μg m-3 in 2010. As the result, life expectancy loss due to PM10 decreased from 2.13 years in 2003 to 1.30 years in 2010. The estimated life expectancy increase due to PM10 mitigation accounted for 34% of the total increase in life expectancy in the same period. Our results suggested that air quality might have contributed substantially to life expectancy in China.

  15. Geología ambiental de la laguna de las Perdices, Monte, Buenos Aires, Argentina

    Directory of Open Access Journals (Sweden)

    Nauris Dangavs

    2010-09-01

    Full Text Available El estudio de la laguna de las Perdices abarca tres aspectos: el geolimnológico, el geoambiental y el de remediación. El primero ha consistido en caracterizar el medio físico de un ambiente léntico típico de la Pampasia meridional prácticamente desconocido. El segundo, la evaluación del grado de deterioro natural y la contaminación físico-química y bacteriológica. El tercero propicia las medidas para su recuperación, máxime teniendo en cuenta que el Municipio de Monte pretende transformarla en Reserva Natural. Esta laguna de 11.50 km2, situada en el noreste bonaerense, pertenece a la cuenca de las Lagunas Encadenadas de Monte y fue evaluada con metodología geolimnológica, en base a cartografía, fotografía aérea e imágenes satelitales, nivelaciones, batimetría, freatimetría, perforaciones, muestreo de sedimentos, suelos y aguas. A tal efecto se caracterizaron los aspectos fisiográficos, geomorfológicos, geológicos e hidrológicos de la región y de la laguna. En la cubeta lagunar se estudiaron los depósitos colmatantes, integrados por siete unidades estratigráficas, de las cuales la de mayor interés corresponde a los depósitos actuales, indicadores directos del estado de degradación del ambiente. El régimen hidrológico de la laguna se estableció caracterizando las precipitaciones sobre la superficie lagunar, la evaporación, el escurrimiento superficial y freático, la freatimetría, la interrelación del cuerpo de agua con el agua subterránea, el balance hídrico anual y la dinámica acuática. Las aguas fueron evaluadas en los aspectos físico-químicos, estableciéndose su composición iónica y tipificación química según Maucha y la clasificación limnológica del ambiente acuático. Las determinaciones en agua y sedimentos confirmaron la severa contaminación físico-química y bacteriológica, incompatible con la vida acuática y el uso recreativo, de acuerdo a la normativa vigente. Dicha contaminaci

  16. Extension of the PMV model to non-air-conditioned building in warm climates

    DEFF Research Database (Denmark)

    Fanger, Povl Ole; Toftum, Jørn

    2002-01-01

    The PMV model agrees well with high-quality field studies in buildings with HVAC systems, situated in cold, temperate and warm climates, studied during both summer and winter. In non-air-conditioned buildings in warm climates, occupants may sense the warmth as being less severe than the PMV...... predicts. The main reason is low expectations, but a metabolic rate that is estimated too high can also contribute to explaining the difference. An extension of the PMV model that includes an expectancy factor is introduced for use in non-air-conditioned buildings in warm climates. The extended PMV model...... agrees well with quality field studies in non-air-conditioned buildings of three continents....

  17. Prediction of thermal sensation in non-air-conditioned buildings in warm climates

    DEFF Research Database (Denmark)

    Fanger, Povl Ole; Toftum, Jørn

    2002-01-01

    The PMV model agrees well with high-quality field studies in buildings with HVAC systems, situated in cold, temperate and warm climates, studied during both summer and winter. In non-air-conditioned buildings in warm climates, occupants may sense the warmth as being less severe than the PMV...... predicts. The main reason is low expectations, but a metabolic rate that is estimated too high can also contribute to explaining the difference. An extension of the PMV model that includes an expectancy factor is introduced for use in non-air-conditioned buildings in warm climates. The extended PMV model...... agrees well with quality field studies in non-air-conditioned buildings of three continents....

  18. Forests under climate change and air pollution: Gaps in understanding and future directions for research

    DEFF Research Database (Denmark)

    Matyssek, R.; Wieser, G.; Calfapietra, C.

    2012-01-01

    Forests in Europe face significant changes in climate, which in interaction with air quality changes, may significantly affect forest productivity, stand composition and carbon sequestration in both vegetation and soils. Identified knowledge gaps and research needs include: (i) interaction between...... for synthesis. This position paper highlights the above focuses, including the global dimension of air pollution as part of climate change and the need for knowledge transfer to enable reliable risk assessment. A new type of research site in forest ecosystems (“supersites”) will be conducive to addressing...... changes in air quality (trace gas concentrations), climate and other site factors on forest ecosystem response, (ii) significance of biotic processes in system response, (iii) tools for mechanistic and diagnostic understanding and upscaling, and (iv) the need for unifying modelling and empirical research...

  19. Superhydrophilicity to superhydrophobicity transition of picosecond laser microstructured aluminum in ambient air.

    Science.gov (United States)

    Long, Jiangyou; Zhong, Minlin; Zhang, Hongjun; Fan, Peixun

    2015-03-01

    Studies regarding the wettability transition of micro- and nano-structured metal surfaces over time are frequently reported, but there seems to be no generally accepted theory that explains this phenomenon. In this paper, we aim to clarify the mechanism underlying the transition of picosecond laser microstructured aluminum surfaces from a superhydrophilic nature to a superhydrophobic one under ambient conditions. The aluminum surface studied exhibited superhydrophilicity immediately after being irradiated by a picosecond laser. However, the contact angles on the surface increased over time, eventually becoming large enough to classify the surface as superhydrophobic. The storage conditions significantly affected this process. When the samples were stored in CO2, O2 and N2 atmospheres, the wettability transition was restrained. However, the transition was accelerated in atmosphere that was rich with organic compounds. Moreover, the superhydrophobic surface could recover their original superhydrophilicity by low temperature annealing. A detailed XPS analysis indicated that this wettability transition process was mainly caused by the adsorption of organic compounds from the surrounding atmosphere onto the oxide surface.

  20. Detection of biological particles in ambient air using Bio-Aerosol Mass Spectrometry

    Energy Technology Data Exchange (ETDEWEB)

    McJimpsey, E L; Steele, P T; Coffee, K R; Fergenson, D P; Riot, V J; Woods, B W; Gard, E E; Frank, M; Tobias, H J; Lebrilla, C

    2006-03-16

    The Bio-Aerosol Mass Spectrometry (BAMS) system is an instrument used for the real time detection and identification of biological aerosols. Particles are drawn from the atmosphere directly into vacuum and tracked as they scatter light from several continuous wave lasers. After tracking, the fluorescence of individual particles is excited by a pulsed 266nm or 355nm laser. Molecules from those particles with appropriate fluorescence properties are subsequently desorbed and ionized using a pulsed 266nm laser. Resulting ions are analyzed in a dual polarity mass spectrometer. During two field deployments at the San Francisco International Airport, millions of ambient particles were analyzed and a small but significant fraction were found to have fluorescent properties similar to Bacillus spores and vegetative cells. Further separation of non-biological background particles from potential biological particles was accomplished using laser desorption/ionization mass spectrometry. This has been shown to enable some level of species differentiation in specific cases, but the creation and observation of higher mass ions is needed to enable a higher level of specificity across more species. A soft ionization technique, matrix-assisted laser desorption/ionization (MALDI) is being investigated for this purpose. MALDI is particularly well suited for mass analysis of biomolecules since it allows for the generation of molecular ions from large mass compounds that would fragment under normal irradiation. Some of the initial results from a modified BAMS system utilizing this technique are described.

  1. Seasonal behavior of carbonyls and source characterization of formaldehyde (HCHO) in ambient air

    Science.gov (United States)

    Lui, K. H.; Ho, Steven Sai Hang; Louie, Peter K. K.; Chan, C. S.; Lee, S. C.; Hu, Di; Chan, P. W.; Lee, Jeffrey Chi Wai; Ho, K. F.

    2017-03-01

    Gas-phase formaldehyde (HCHO) is an intermediate and a sensitive indicator for volatile organic compounds (VOCs) oxidation, which drives tropospheric ozone production. Effective photochemical pollution control strategies demand a thorough understanding of photochemical oxidation precursors, making differentiation between sources of primary and secondary generated HCHO inevitable. Spatial and seasonal variations of airborne carbonyls based on two years of measurements (2012-2013), coupled with a correlation-based HCHO source apportionment analysis, were determined for three sampling locations in Hong Kong (denoted HT, TC, and YL). Formaldehyde and acetaldehyde were the two most abundant compounds of the total quantified carbonyls. Pearson's correlation analysis (r > 0.7) implies that formaldehyde and acetaldehyde possibly share similar sources. The total carbonyl concentration trends (HT urban > rural). A regression analysis further quantifies the relative primary HCHO source contributions at HT (∼13%), TC (∼21%), and YL (∼40%), showing more direct vehicular emissions in urban than rural areas. Relative secondary source contributions at YL (∼36%) and TC (∼31%) resemble each other, implying similar urban source contributions. Relative background source contributions at TC could be due to a closed structure microenvironment that favors the trapping of HCHO. Comparable seasonal differences are observed at all stations. The results of this study will aid in the development of a new regional ozone (O3) control policy, as ambient HCHO can enhance O3 production and also be produced from atmospheric VOCs oxidation (secondary HCHO).

  2. Air pollution and survival within the Washington University-EPRI veterans cohort: risks based on modeled estimates of ambient levels of hazardous and criteria air pollutants.

    Science.gov (United States)

    Lipfert, Frederick W; Wyzga, Ronald E; Baty, Jack D; Miller, J Philip

    2009-04-01

    For this paper, we considered relationships between mortality, vehicular traffic density, and ambient levels of 12 hazardous air pollutants, elemental carbon (EC), oxides of nitrogen (NOx), sulfur dioxide (SO2), and sulfate (SO4(2-)). These pollutant species were selected as markers for specific types of emission sources, including vehicular traffic, coal combustion, smelters, and metal-working industries. Pollutant exposures were estimated using emissions inventories and atmospheric dispersion models. We analyzed associations between county ambient levels of these pollutants and survival patterns among approximately 70,000 U.S. male veterans by mortality period (1976-2001 and subsets), type of exposure model, and traffic density level. We found significant associations between all-cause mortality and traffic-related air quality indicators and with traffic density per se, with stronger associations for benzene, formaldehyde, diesel particulate, NOx, and EC. The maximum effect on mortality for all cohort subjects during the 26-yr follow-up period is approximately 10%, but most of the pollution-related deaths in this cohort occurred in the higher-traffic counties, where excess risks approach 20%. However, mortality associations with diesel particulates are similar in high- and low-traffic counties. Sensitivity analyses show risks decreasing slightly over time and minor differences between linear and logarithmic exposure models. Two-pollutant models show stronger risks associated with specific traffic-related pollutants than with traffic density per se, although traffic density retains statistical significance in most cases. We conclude that tailpipe emissions of both gases and particles are among the most significant and robust predictors of mortality in this cohort and that most of those associations have weakened over time. However, we have not evaluated possible contributions from road dust or traffic noise. Stratification by traffic density level suggests the

  3. Air flow-assisted ionization imaging mass spectrometry method for easy whole-body molecular imaging under ambient conditions.

    Science.gov (United States)

    Luo, Zhigang; He, Jiuming; Chen, Yi; He, Jingjing; Gong, Tao; Tang, Fei; Wang, Xiaohao; Zhang, Ruiping; Huang, Lan; Zhang, Lianfeng; Lv, Haining; Ma, Shuanggang; Fu, Zhaodi; Chen, Xiaoguang; Yu, Shishan; Abliz, Zeper

    2013-03-01

    Whole-body molecular imaging is able to directly map spatial distribution of molecules and monitor its biotransformation in intact biological tissue sections. Imaging mass spectrometry (IMS), a label-free molecular imaging method, can be used to image multiple molecules in a single measurement with high specificity. Herein, a novel easy-to-implement, whole-body IMS method was developed with air flow-assisted ionization in a desorption electrospray ionization mode. The developed IMS method can effectively image molecules in a large whole-body section in open air without sample pretreatment, such as chemical labeling, section division, or matrix deposition. Moreover, the signal levels were improved, and the spatial assignment errors were eliminated; thus, high-quality whole-body images were obtained. With this novel IMS method, in situ mapping analysis of molecules was performed in adult rat sections with picomolar sensitivity under ambient conditions, and the dynamic information of molecule distribution and its biotransformation was provided to uncover molecular events at the whole-animal level. A global view of the differential distribution of an anticancer agent and its metabolites was simultaneously acquired in whole-body rat and model mouse bearing neuroglioma along the administration time. The obtained drug distribution provided rich information for identifying the targeted organs and predicting possible tumor spectrum, pharmacological activity, and potential toxicity of drug candidates.

  4. On the system of monitoring ambient air quality in relation to the health of the population of the Czech Republic

    Energy Technology Data Exchange (ETDEWEB)

    Kazmarova, H. [National Inst. of Public Health, Prague (Czech Republic)

    1995-12-31

    In 1991 the Government of the Czech republic in Ruling No 369 approved a draft of a system for monitoring the health of the population in relation to the environment on the basis of a need to obtain purposefully targeted information for an appropriate policy for the protection of health and the environment. The aim of monitoring does not and cannot consist of determining the cause and effect relationship between the health status and pollutants. The system of monitoring is an open and comprehensive system of the continual collection, processing and evaluation of data concerned with the load on the organism and damage to human health in relation to environmental pollution. Air pollution and health are one of the six subsystems realised in the whole system (beside drinking water, noise, food, biomarkers, and demographic and health statistics). The aim of the monitoring is to obtain a data base that shall serve three main purposes: (1) Description of the status of health of the population and characteristics of the ambient air, (2) Evaluation of the trend of each index, (3) Assessment and evaluation of the risk to health of the parameters under study. Thirty cities and towns were selected in the Czech Republic for the realisation of the monitoring system. (author)

  5. 环境空气质量监测系统探讨%Discussion on Ambient Air Quality Monitoring System

    Institute of Scientific and Technical Information of China (English)

    罗鸿初

    2014-01-01

    Air quality monitoring is an important part of national environmental monitoring and management, and sustainable development of urban ecological environment system has a major impact. Combined with years of practical experience, the material from the gas monitoring and surveillance of both solid particles departure, focuses on the comparison of ambient air quality monitoring system, and make relevant comments, for practical reference.%空气质量监测是国家环境监测管理的重要组成部分,对城市生态环境系统的可持续发展有着重大的影响。结合多年的实践经验,从气体物质监测和固体颗粒物监测两方面出发,重点探讨了环境空气质量监测系统的比较,并提出相关意见,以供实践参考。

  6. Quantitative Assessment of Detection Frequency for the INL Ambient Air Monitoring Network

    Energy Technology Data Exchange (ETDEWEB)

    Sondrup, A. Jeffrey [Idaho National Lab. (INL), Idaho Falls, ID (United States); Rood, Arthur S. [Idaho National Lab. (INL), Idaho Falls, ID (United States)

    2014-11-01

    A quantitative assessment of the Idaho National Laboratory (INL) air monitoring network was performed using frequency of detection as the performance metric. The INL air monitoring network consists of 37 low-volume air samplers in 31 different locations. Twenty of the samplers are located on INL (onsite) and 17 are located off INL (offsite). Detection frequencies were calculated using both BEA and ESER laboratory minimum detectable activity (MDA) levels. The CALPUFF Lagrangian puff dispersion model, coupled with 1 year of meteorological data, was used to calculate time-integrated concentrations at sampler locations for a 1-hour release of unit activity (1 Ci) for every hour of the year. The unit-activity time-integrated concentration (TICu) values were calculated at all samplers for releases from eight INL facilities. The TICu values were then scaled and integrated for a given release quantity and release duration. All facilities modeled a ground-level release emanating either from the center of the facility or at a point where significant emissions are possible. In addition to ground-level releases, three existing stacks at the Advanced Test Reactor Complex, Idaho Nuclear Technology and Engineering Center, and Material and Fuels Complex were also modeled. Meteorological data from the 35 stations comprising the INL Mesonet network, data from the Idaho Falls Regional airport, upper air data from the Boise airport, and three-dimensional gridded data from the weather research forecasting model were used for modeling. Three representative radionuclides identified as key radionuclides in INL’s annual National Emission Standards for Hazardous Air Pollutants evaluations were considered for the frequency of detection analysis: Cs-137 (beta-gamma emitter), Pu-239 (alpha emitter), and Sr-90 (beta emitter). Source-specific release quantities were calculated for each radionuclide, such that the maximum inhalation dose at any publicly accessible sampler or the National

  7. Ambient concentrations of aldehydes in relation to Beijing Olympic air pollution control measures

    Directory of Open Access Journals (Sweden)

    J. C. Gong

    2010-08-01

    Full Text Available Aldehydes are ubiquitous constituents of the atmosphere. Their concentrations are elevated in polluted urban atmospheres. The present study was carried out to characterize three aldehydes of most health concern (formaldehyde, acetaldehyde, and acrolein in a central Beijing site in the summer and early fall of 2008 (from June to October. Measurements were made before, during, and after the Beijing Olympics to examine whether the air pollution control measures implemented to improve Beijing's air quality during the Olympics had any impact on concentrations of the three aldehydes. Average concentrations of formaldehyde, acetaldehyde and acrolein were 29.34 ± 15.12 μg/m3, 27.09 ± 15.74 μg/m3 and 2.32 ± 0.95 μg/m3, respectively, for the entire period of measurements, all being the highest among the levels measured in cities around the world in photochemical smog seasons. Among the three measured aldehydes, only acetaldehyde had a substantially reduced mean concentration during the Olympic air pollution control period compared to the pre-Olympic period. Formaldehyde and acrolein followed the changing pattern of temperature and were each significantly correlated with ozone (a secondary product of photochemical reactions. In contrast, acetaldehyde was significantly correlated with several pollutants emitted mainly from local emission sources (e.g., NO2, CO, and PM2.5. These findings suggest that local direct emissions had a larger impact on acetaldehyde than formaldehyde and acrolein.

  8. Impurity intrusion in radio-frequency micro-plasma jets operated in ambient air

    CERN Document Server

    Niermann, B; Böke, M; Winter, J

    2011-01-01

    Space and time resolved concentrations of helium metastable atoms in an atmospheric pressure radio-frequency micro-plasma jet were measured using tunable diode laser absorption spectroscopy. Spatial profiles as well as lifetime measurements show significant influences of air entering the discharge from the front nozzle and of impurities originating from the gas supply system. Quenching of metastables was used to deduce quantitative concentrations of intruding impurities. The impurity profile along the jet axis was determined from optical emission spectroscopy as well as their dependance on the feed gas flow through the jet.

  9. Prototype development and test results of a continuous ambient air monitoring system for hydrazine at the 10 ppb level

    Science.gov (United States)

    Meneghelli, Barry; Parrish, Clyde; Barile, Ron; Lueck, Dale E.

    1995-01-01

    A Hydrazine Vapor Area Monitor (HVAM) system is currently being field tested as a detector for the presence of hydrazine in ambient air. The MDA/Polymetron Hydrazine Analyzer has been incorporated within the HVAM system as the core detector. This analyzer is a three-electrode liquid analyzer typically used in boiler feed water applications. The HVAM system incorporates a dual-phase sample collection/transport method which simultaneously pulls ambient air samples containing hydrazine and a very dilute sulfuric acid solution (0.0001 M) down a length of 1/4 inch outside diameter (OD) tubing from a remote site to the analyzer. The hydrazine-laden dilute acid stream is separated from the air and the pH is adjusted by addition of a dilute caustic solution to a pH greater than 10.2 prior to analysis. Both the dilute acid and caustic used by the HVAM are continuously generated during system operation on an "as needed" basis by mixing a metered amount of concentrated acid/base with dilution water. All of the waste water generated by the analyzer is purified for reuse by Barnstead ion-exchange cartridges so that the entire system minimizes the generation of waste materials. The pumping of all liquid streams and mixing of the caustic solution and dilution water with the incoming sample are done by a single pump motor fitted with the appropriate mix of peristaltic pump heads. The signal to noise (S/N) ratio of the analyzer has been enhanced by adding a stirrer in the MDA liquid cell to provide mixing normally generated by the high liquid flow rate designed by the manufacturer. An onboard microprocessor continuously monitors liquid levels, sample vacuum, and liquid leak sensors, as well as handles communications and other system functions (such as shut down should system malfunctions or errors occur). The overall system response of the HVAM can be automatically checked at regular intervals by measuring the analyzer response to a metered amount of calibration standard injected

  10. Respiratory diseases in preschool children in the city of Niš exposed to suspended particulates and carbon monoxide from ambient air

    Directory of Open Access Journals (Sweden)

    Đorđević Amelija

    2016-01-01

    Full Text Available Background/Aim. Analysis of air quality in Serbia indicates that the city of Niš belongs to a group of cities characterized by the third category of air quality (excessive air pollution. The aim of the study was to analyze the degree of causality between ambient air quality affected by particulate matter of 10 μm (PM10 and carbon monoxide (CO and the incidence of respiratory diseases in preschool children in the city of Niš. Methods. We quantified the influence of higher PM10 concentrations and carbon monoxide comprising motor vehicle exhausts in the city of Niš on the occurrence of unwanted health effects in preschool children by means of the hazard quotient (HQ, individual health risk (Ri, and the probability of cancer (ICR. The methodology used was according to the US Environmental Protection Agency (EPA, and it included basic scientific statistical methods, compilation methods, and the relevant mathematical methods for assessing air pollution health risk, based on the use of attribute equations. Results. Measurement of ambient air pollutant concentrations in the analyzed territory for the entire monitoring duration revealed that PM10 concentrations were significantly above the allowed limits during 80% of the days. The maximum measured PM10 concentration was 191.6 μg/m3, and carbon monoxide 5.415 mg/m3. The incidence of respiratory diseases in the experimental group, with a prominent impact of polluted air was 57.17%, whereas the incidence in the control group was considerably lower, 41.10 %. There were also significant differences in the distribution of certain respiratory diseases. Conclusion. In order to perform good causal analysis of air quality and health risk, it is very important to establish and develop a system for long-term monitoring, control, assessment, and prediction of air pollution. We identified the suspended PM10 and CO as ambient air pollutants causing negative health effects in the exposed preschool children

  11. Apply Woods Model in the Predictions of Ambient Air Particles and Metallic Elements (Mn, Fe, Zn, Cr, and Cu at Industrial, Suburban/Coastal, and Residential Sampling Sites

    Directory of Open Access Journals (Sweden)

    Guor-Cheng Fang

    2012-01-01

    Full Text Available The main purpose for this study was to monitor ambient air particles and metallic elements (Mn, Fe, Zn, Cr, and Cu in total suspended particulates (TSPs concentration, dry deposition at three characteristic sampling sites of central Taiwan. Additionally, the calculated/measured dry deposition flux ratios of ambient air particles and metallic elements were calculated with Woods models at these three characteristic sampling sites during years of 2009-2010. As for ambient air particles, the results indicated that the Woods model generated the most accurate dry deposition prediction results when particle size was 18 μm in this study. The results also indicated that the Woods model exhibited better dry deposition prediction performance when the particle size was greater than 10 μm for the ambient air metallic elements in this study. Finally, as for Quan-xing sampling site, the main sources were many industrial factories under process around these regions and were severely polluted areas. In addition, the highest average dry deposition for Mn, Fe, Zn, and Cu species occurred at Bei-shi sampling site, and the main sources were the nearby science park, fossil fuel combustion, and Taichung thermal power plant (TTPP. Additionally, as for He-mei sampling site, the main sources were subjected to traffic mobile emissions.

  12. Online Automatic Monitoring of Ambient Air Quality Control Technology Research%环境空气自动监测在线质控技术研究

    Institute of Scientific and Technical Information of China (English)

    陈国伟

    2014-01-01

    The automatic monitoring system for ambient air monitoring, to ensure the accuracy and reliability of the monitoring data. Online quality control technology innovation automatic detection system, which can maximize their potential in the monitoring of ambient air. This paper analyzes the necessity of quality control techniques and management methods automatic ambient air monitoring; quality control methods discussed online automatic monitoring of ambient air.%利用自动监测系统对环境空气进行监测,可保证监测数据的准确性和可靠性。利用在线质控技术不断革新自动检测系统,可使其在监测环境空气时发挥最大功效。分析了质控技术对环境空气自动监测的必要性和管理方法,探讨了环境空气自动监测的在线质控方式。

  13. Biomarkers for Exposure to Ambient Air Pollution - Comparison of Carcinogen-DNA Adduct Levels with Other Exposure Markers and Markers for Oxidative Stress

    DEFF Research Database (Denmark)

    Autrup, Herman; Daneshvar, Bahram; Dragsted, Lars Ove;

    1999-01-01

    Human exposure to genotoxic compounds present in ambient air has been studied using selected biomarkers in nonsmoking Danish bus drivers and postal workers. A large interindividual variation in biomarker levels was observed. Significantly higher levels of bulky carcinogen-DNA adducts (75.42 adduc...

  14. Evergreen or deciduous trees for capturing PAHs from ambient air? A case study.

    Science.gov (United States)

    De Nicola, Flavia; Concha Graña, Estefanía; López Mahía, Purificación; Muniategui Lorenzo, Soledad; Prada Rodríguez, Darío; Retuerto, Rubén; Carballeira, Alejo; Aboal, Jesús R; Fernández, J Ángel

    2017-02-01

    Tree canopies play a key role in the cycling of polycyclic aromatic hydrocarbons (PAHs) in terrestrial ecosystems, as leaves can capture PAHs from the air. In this study, accumulation of PAHs was compared in an evergreen species, P. pinaster, and in a deciduous species, Q. robur, in relation to some physio-morphological characteristics. For this purpose, pine needles and oak leaves collected from different sites across Galicia (NW Spain) were analysed to determine PAH contents, specific leaf area, stomatal density and conductance. Leaves and needles contained similar total amounts of PAHs. The major contribution of particle-bound PAHs in oak (the concentrations of 4- and 5-ring PAHs were two times higher, and those of 6-ring PAHs five times higher in oak than in pine) may be related to the higher specific leaf area (13 and 4 cm(2) g(-1) dry mass in respectively oak and pine). However, the major contribution of vapor-phase PAHs in pines may be affected by the stomatal conductance (two times higher in pine than in oak). Moreover, an increase in the diameter at breast height of trees led to an increase in accumulation of PAHs, with pine capturing higher amounts of low and medium molecular weight PAHs. The study findings underline the potential role of trees in improving air quality, taking into account the canopy biomass and life cycle.

  15. Impact of natural gas extraction on Pah levels in ambient air

    Science.gov (United States)

    Paulik, L. Blair; Donald, Carey E.; Smith, Brian W.; Tidwell, Lane G.; Hobbie, Kevin A.; Kincl, Laurel; Haynes, Erin N.; Anderson, Kim A.

    2015-01-01

    Natural gas extraction, often referred to as “fracking,” has increased rapidly in the U.S. in recent years. To address potential health impacts, passive air samplers were deployed in a rural community heavily affected by the natural gas boom. Samplers were analyzed for 62 polycyclic aromatic hydrocarbons (PAHs). Results were grouped based on distance from each sampler to the nearest active well. PAH levels were highest when samplers were closest to active wells. Additionally, PAH levels closest to natural gas activity were an order of magnitude higher than levels previously reported in rural areas. Sourcing ratios indicate that PAHs were predominantly petrogenic, suggesting that elevated PAH levels were influenced by direct releases from the earth. Quantitative human health risk assessment estimated the excess lifetime cancer risks associated with exposure to the measured PAHs. Closest to active wells, the risk estimated for maximum residential exposure was 2.9 in 10,000, which is above the U.S. EPA's acceptable risk level. Overall, risk estimates decreased 30% when comparing results from samplers closest to active wells to those farthest. This work suggests that natural gas extraction may be contributing significantly to PAHs in air, at levels that are relevant to human health. PMID:25810398

  16. THE QUALITY OF AIR IN HOSPITAL ENVIRONMENTS CLIMATIZED AND ITS INFLUENCE IN THE OCCURRENCE OF INFECTIONS

    Directory of Open Access Journals (Sweden)

    Patrícia Staciarini Anders

    2004-08-01

    Full Text Available Climatized environment is defined as the environment where temperature and humidity are controlled.We have made a review of literature, from 1990 to 2001, through data base MEDLINE, LILACS and Ministry ofHealth – Brazil. The aim of this study was to analyze the air quality in climatized environment and the last as a riskfactor for hospital infection – HI. Twenty-three articles where analyzed and gathered by the focused theme;patterns and principles for maintaining the air quality; air quality and isolation of microorganism; air quality andoccurrence of infection. The standard of quality quotes: ventilation, maintenance and cleanness of climatizationsystems. Aspergillus, Legionella, Acinetobacter, Clostridium, Nocardia, among others where found in airconditioned devices and the first three ones being responsable for booms of HI.

  17. Characterization of Carbonyl Compounds in the Ambient Air of an Industrial City in Korea

    Directory of Open Access Journals (Sweden)

    Sung-Ok Baek

    2011-01-01

    Full Text Available The purpose of this study was to characterize spatial and temporal variations of carbonyl compounds in Gumi city, where a number of large electronic-industrial complexes are located. Carbonyl samples were collected at five sites in the Gumi area: three industrial, one commercial, and one residential area. Sampling was carried out throughout a year from December 2003 to November 2004. At one industrial site, samples were taken every six days, while those of the other sites were for seven consecutive days in every season. Each sample was collected for 150 minutes and at intervals of three times a day (morning, afternoon, and evening. A total of 476 samples were analyzed to determine 15 carbonyl compounds by the USEPA TO-11A (DNPH-cartridge/HPLC method. In general, acetaldehyde appeared to be the most abundant compound, followed by formaldehyde, and acetone+acrolein. Mean concentrations of acetaldehyde were two to three times higher in the industrial sites than in the other sites, with its maximum of 77.7 ppb. In contrast, ambient levels of formaldehyde did not show any significant difference between the industrial and non-industrial groups. Its concentrations peaked in summer probably due to the enhanced volatilization and photochemical reactivity. These results indicate significant emission sources of acetaldehyde in the Gumi industrial complexes. Mean concentrations of organic solvents (such as acetone+acrolein and methyl ethyl ketone were also significantly high in industrial areas. In conclusion, major sources of carbonyl compounds, including acetaldehyde, are strongly associated with industrial activities in the Gumi city area.

  18. Removal of mercury vapor from ambient air of dental clinics using an air cleaning system based on silver nanoparticles

    Directory of Open Access Journals (Sweden)

    Chiman Saeidi

    2015-06-01

    Full Text Available Background & objective: Mercury is a toxic and bio-accumulative pollutant that has adverse effects on environmental and human health. There have been a number of attempts to regulate mercury emissions tothe atmosphere. Silver nanoparticles are a number of materials that have highly potential to absorb mercury and formation of mercury amalgam.The aim of this study is removal of mercury vapors in the dental clinic using a n a ir cleaning system based on silver nanoparticles. Methods: In this study, silver nanoparticles coated on the bed of foam and chemical and structural properties were determined using a number of methods such as UV-VIS-NIR spectroscopy and Scanning Electron Microscope (SEM connected the X-ray Emission Spectroscopy Energy (EDS. The a ir cleaning system efficiency to remove of the mercury vapor in simulated conditions in the laboratory and real conditions in the dental clinicwere measured by Cold Vapor Atomic Absorption Spectroscopy (CVAAS. Results: The images of SEM, showed that average sizeof silver nanoparticles in colloidal solution was ∼ 30nm and distribution of silver nanoparticles coated on foam was good. EDS spectrum confirmed associated the presence of silver nanoparticles coated on foam. The significantly difference observed between the concentration of mercury vapor in the off state (9.43 ± 0.342 μg.m-3 and on state (0.51 ± 0.031μg.m-3 of the a ir cleaning system. The mercury vapor removal efficiencyof the a ir cleaning system was calculated 95%. Conclusion : The air cleaning system based on foam coated by silver nanoparticles, undertaken to provide the advantages such as use facilitating, highly efficient operational capacity and cost effective, have highly sufficiency to remove mercury vapor from dental clinics.

  19. Hot air : meeting Canada's climate change challenge

    Energy Technology Data Exchange (ETDEWEB)

    Simpson, J.; Jaccard, M.; Rivers, N.

    2007-07-01

    As a large northern country, Canada will change significantly as a result of climate change. Global warming is expected to cause diminutions of snow and ice changes in the Arctic, as well as changes to glaciers, and the mountain snowpacks that feed rivers, and provide sources of fresh water. This book argued that the effects of global warming have been apparent in Canada for many years. Water levels in lakes and rivers have been falling, and a thawing permafrost has led to difficulties in building and maintaining winter roads in the far north. Disturbances such as the mountain pine beetle (MPB) infestation in British Columbia have also been attributed to global warming, the beetles are only killed by cold weather. The book also considered Canada's current climate change policies, and discussed attempts to arrive at meaningful and effective strategies. 30 refs.

  20. Atmospheric chemistry and physics from air pollution to climate change

    CERN Document Server

    Seinfeld, John H

    2016-01-01

    Expanded and updated with new findings and new features Since the second edition of Seinfeld and Pandis’ classic textbook, significant progress has taken place in the field of atmospheric chemistry and physics, particularly in the areas of tropospheric chemistry, aerosols, and the science of climate change. A new edition of this comprehensive work has been developed by the renowned author team. Atmospheric Chemistry and Physics, 3rd Edition, as the previous two editions have done, provides a rigorous and comprehensive treatment of the chemistry and physics of the atmosphere – including the chemistry of the stratosphere and troposphere, aerosol physics and chemistry, atmospheric new particle formation, physical meteorology, cloud physics, global climate, statistical analysis of data, and mathematical chemical/transport models of the atmosphere. Each of these topics is covered in detail and in each area the central results are developed from first principles. In this way the reader gains a significant un...

  1. Retrofitting Air Conditioning and Duct Systems in Hot, Dry Climates

    Energy Technology Data Exchange (ETDEWEB)

    Shapiro, C.; Aldrich, R.; Arena, L.

    2012-07-01

    This technical report describes CARB's work with Clark County Community Resources Division in Las Vegas, Nevada, to optimize procedures for upgrading cooling systems on existing homes in the area to implement health, safety, and energy improvements. Detailed monitoring of five AC systems showed that three of the five systems met or exceeded air flow rate goals.

  2. Climate Prediction Center (CPC) Global Land Surface Air Temperature Analysis

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — A station observation-based global land monthly mean surface air temperature dataset at 0.5 0.5 latitude-longitude resolution for the period from 1948 to the present...

  3. Benefits of European Climate Policies for Mercury Air Pollution

    Directory of Open Access Journals (Sweden)

    Peter Rafaj

    2014-01-01

    Full Text Available This paper presents the methodology and results of impact assessment of renewable energy policies on atmospheric emissions of mercury in Europe. The modeling exercise described here involves an interaction of several models. First, a set of energy scenarios has been developed with the REMix (Renewable Energy Mix model that simulates different levels of penetration of renewable energies in the European power sector. The energy scenarios were input to the GAINS (Greenhouse Gas and Air Pollution Interactions and Synergies model, which prepared projections of mercury releases to the atmosphere through 2050, based on the current air pollution control policies in each country. Data on mercury emissions from individual sectors were subsequently disaggregated to a fine spatial resolution using various proxy parameters. Finally, the dispersion of mercury in the atmosphere was computed by the chemistry transport model, implemented to the air quality system, Polyphemus. The simulations provided information on changes in concentrations and depositions of various forms of mercury over Europe. Scenarios that simulate a substantial expansion of renewable energies within the power sector indicate extensive co-benefits for mercury abatement, due to the restructuring of the energy system and changes in the fuel mix. The potential for mercury reductions in Europe depends on the rate of fuel switches and renewable technology deployment, but is also influenced by the stringency and timing of the air quality measures. The overall scope for co-benefits is therefore higher in regions relying on coal combustion as a major energy source.

  4. Climate Prediction Center (CPC) Global Land Surface Air Temperature Analysis

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — A station observation-based global land monthly mean surface air temperature dataset at 0.5 x 0.5 latitude-longitude resolution for the period from 1948 to the...

  5. A strategy for climate evaluation of aircraft technology: an efficient climate impact assessment tool – AirClim

    Directory of Open Access Journals (Sweden)

    A. Stenke

    2007-08-01

    Full Text Available Climate change is a challenge to society and to cope with requires assessment tools which are suitable to evaluate new technology options with respect to their impact on climate. Here we present AirClim, a model which comprises a linearisation of the processes occurring from the emission to an estimate in near surface temperature change, which is presumed to be a reasonable indicator for climate change. The model is designed to be applicable to aircraft technology, i.e.~the climate agents CO2, H2O, CH4 and O3 (latter two resulting from NOx-emissions and contrails are taken into account. It employs a number of precalculated atmospheric data and combines them with aircraft emission data to obtain the temporal evolution of atmospheric concentration changes, radiative forcing and temperature changes. The linearisation is based on precalculated data derived from 25 steady-state simulations of the state-of-the-art climate-chemistry model E39/C, which include sustained normalised emissions at various atmospheric regions. The results show that strongest climate impacts from ozone changes occur for emissions in the tropical upper troposphere (60 mW/m²; 80 mK for 1 TgN emitted, whereas from methane in the middle tropical troposphere (–2.7% change in methane lifetime; –30 mK per TgN. The estimate of the temperature changes caused by the individual climate agents takes into account a perturbation lifetime, related to the region of emission. A comparison of this approach with results from the TRADEOFF and SCENIC projects shows reasonable agreement with respect to concentration changes, radiative forcing, and temperature changes. The total impact of a supersonic fleet on radiative forcing (mainly water vapour is reproduced within 5%. For subsonic air traffic (sustained emissions after 2050 results show that although ozone-radiative forcing is much less important than that from CO2 for the year 2100. However the impact on temperature is of comparable size

  6. Ultimate detectability of volatile organic compounds: how much further can we reduce their ambient air sample volumes for analysis?

    Science.gov (United States)

    Kim, Yong-Hyun; Kim, Ki-Hyun

    2012-10-02

    To understand the ultimately lowest detection range of volatile organic compounds (VOCs) in air, application of a high sensitivity analytical system was investigated by coupling thermal desorption (TD) technique with gas chromatography (GC) and time-of-flight (TOF) mass spectrometry (MS). The performance of the TD-GC/TOF MS system was evaluated using liquid standards of 19 target VOCs prepared in the range of 35 pg to 2.79 ng per μL. Studies were carried out using both total ion chromatogram (TIC) and extracted ion chromatogram (EIC) mode. EIC mode was used for calibration to reduce background and to improve signal-to-noise. The detectability of 19 target VOCs, if assessed in terms of method detection limit (MDL, per US EPA definition) and limit of detection (LOD), averaged 5.90 pg and 0.122 pg, respectively, with the mean coefficient of correlation (R(2)) of 0.9975. The minimum quantifiable mass of target analytes, when determined using real air samples by the TD-GC/TOF MS, is highly comparable to the detection limits determined experimentally by standard. In fact, volumes for the actual detection of the major aromatic VOCs like benzene, toluene, and xylene (BTX) in ambient air samples were as low as 1.0 mL in the 0.11-2.25 ppb range. It was thus possible to demonstrate that most target compounds including those in low abundance could be reliably quantified at concentrations down to 0.1 ppb at sample volumes of less than 10 mL. The unique sensitivity of this advanced analytical system can ultimately lead to a shift in field sampling strategy with smaller air sample volumes facilitating faster, simpler air sampling (e.g., use of gas syringes rather than the relative complexity of pumps or bags/canisters), with greatly reduced risk of analyte breakthrough and minimal interference, e.g., from atmospheric humidity. The improved detection limits offered by this system can also enhance accuracy and measurement precision.

  7. Lasing of ambient air with microjoule pulse energy pumped by a multi terawatt IR femtosecond laser

    CERN Document Server

    Point, Guillaume; Brelet, Yohann; Mitryukovskiy, Sergey; Ding, Pengji; Houard, Aurélien; Mysyrowicz, André

    2014-01-01

    We report on the lasing action of atmospheric air pumped by an 800 nm femtosecond laser pulse with peak power up to 4 TW. Lasing emission at 428 nm increases rapidly over a small range of pump laser power, followed by saturation above ~ 1.5 TW. The maximum lasing pulse energy is measured to be 2.6 uJ corresponding to an emission power in the MW range, while a maximum conversion efficiency of is measured at moderate pump pulse energy. The optical gain inside the filament plasma is estimated to be excess of 0.7/cm. The lasing emission shows a doughnut profile, reflecting the spatial distribution of the pump-generated white-light continuum that acts as a seed for the lasing. We attribute the pronounced saturation to the defocusing of the seed in the plasma amplifying region and to the saturation of the seed intensity.

  8. An Ambient Air Quality Model for Assessment of U.S. Naval Aviation Emittants

    Science.gov (United States)

    1976-09-01

    Laboratory at Kirkland AFBf New Mexico , the Naval Air Propulsion Test Center (NAPTC) at Trenton, New Jersey, and the Naval Post- graduate School...w« I t^ I MMtv I turn« I turn« i «ma> i »«nir» i vino i ««e I i>iinw> i «wm i v~*o I xeir I w I «<r» I um<u i ain« i r-irnu i uiw<r> i tvou« I mom I...r 1 vino i «’wir | u> ui«<o i wm«D i r-««o i MWO o • e 1 VI 1 w 1 u 1 u- 1 3 1 u 1 VI 11- t t- 1 "B t K 1 u i a. I ** I m 1 X 1 o

  9. Particulate matter in ambient air - Assessment of health risks. Partiklar i omgivningsluften - en bedoemning av haelsorisker

    Energy Technology Data Exchange (ETDEWEB)

    Camner, P.

    1986-07-01

    An investigation, based on literature data and research at SML, was made on deposition of particulate matter in lungs. The importance of mouth and nose breathing respectively is illustrated. By nose breathing only substances <10 micrometers reach the lung as compared to mouth breathing where substances >10 micrometers may deposit in the lung. Swedish limit values of total suspended particulate matter (TSP) of 50 micrograms/cubic meter are recommended as a 6 month mean value and 150 micrograms/cubic meter as a day mean value. For the PM/sub 10/ fraction, which is a measure of the mass fraction of particulate matter in the air that is deposited in the lung by mouth breathing, it is not possible to give a corresponding recommendation. Epidemiological data are lacking and the proposed method of measuring the PM/sub 10/ fraction would underestimate the importance of particles larger than 10 micrometers. (O.S.).

  10. Ion chemistry for the detection of isoprene and other volatile organic compounds in ambient air

    Science.gov (United States)

    Leibrock, Edeltraud; Huey, L. Gregory

    2000-06-01

    A chemical ionization mass spectrometer (CIMS) and a flowing afterglow apparatus were used to study reactions of benzene cations (C6H6+ and (C6H6)2+) with a series of volatile organic compounds (VOCs). Both cations react at the collision rate with compounds of lower ionization potential than benzene, such as isoprene (C5H8), other conjugated dienes, and aromatics. These ions are generally unreactive with substances of higher ionization potential such as alkanes, simple alcohols, simple carbonyls, etc. The results demonstrate that C6H6+ and (C6H6)2+ are excellent reagent ions for the sensitive detection of isoprene in air with a CIMS. However, 2-methyl-3-buten-2-ol (MBO) and C5H8 conjugated dienes were identified as potential interferences to this technique. This indicates that the selectivity of the CIMS isoprene measurement must be tested by intercomparison with well-established methods, e.g. gas chromatography techniques.

  11. Analyzing x-ray emissions from meter-scale negative discharges in ambient air

    DEFF Research Database (Denmark)

    Kochkin, Pavlo; Köhn, Christoph; Ebert, Ute

    2016-01-01

    When voltage pulses of 1 MV drive meter long air discharges, short and intense bursts of x-rays are measured. Here we develop a model for electron acceleration and subsequent photon generation within this discharge to understand these bursts. We start from the observation that the encounter of two...... streamers of opposite polarity launches the electrons, that they are further accelerated in the discharge field and then lose their energy, e.g., by photon emission through Bremsstrahlung. We model electron and photon dynamics in space and energy with a Monte Carlo model. Also the detector response...... to incoming photons is modelled in detail. The model justifies the approximation that the x-ray bursts are isotropic in space; this assumption is used to conclude that x-ray bursts near the high-voltage electrode with 6x 104 photons and characteristic energies of 160 keV closely reproduce the measured spectra...

  12. Evaluation of co-benefits from combined climate change and air pollution reduction strategies

    Science.gov (United States)

    Leitao, Joana; Van Dingenen, Rita; Dentener, Frank; Rao, Shilpa

    2014-05-01

    The connection of climate change and air pollution is becoming more relevant in the process of policy making and implementation of emission control strategies because of resulting co-benefits and trade-offs. Some sectors, such as fossil fuel combustion, are sources of both pollutants (NOx and PM) as well as greenhouse gas (CO2). Additionally, the use of wood burning as biofuel to reduce climate impact may in fact deteriorate air quality. Furthermore, several air pollutants are important radiative forcers and regulating their emissions impacts on climate. It is evident that both problems need to be undertaken with a common strategy and the existence of cross-policy with co-benefits may encourage their implementation. The LIMITS FP7 project (http://www.feem-project.net/limits/index.html) was designed with the main goal of assessing strategies for reduction of GHG emissions so that the 2°C target can be achieved. The work developed focus on the evaluation of the implementation of strategies analysing several aspects of different scenarios, namely: the feasibility of low carbon scenarios in terms of available technologies and infrastructure, the required financial mechanisms, and also the co-benefits regarding energy security, economic development and air pollution. For the latter, five integrated assessment models (IAMs) provided greenhouse gases and pollutant emission values for several scenarios. These were based on air pollution scenarios defined according to stringency and implementation of future global legislation. They which were also combined with 2 climate policy scenarios (no climate policy and 2.8 W/m2 target). The former are mostly focused on non-climate policies and technical control measures for emissions of air pollutants, such as PM2.5, NOx and SO2, with their emission factors harmonized between the IAMs. With the global air quality source-receptor model TM5-FASST the impact of the resulting emissions was analysed and the co-benefits of combined

  13. Trace Elements in Ambient Air at Porto Metropolitan Area-Checking for Compliance with New European Union (EU) Air Quality Standards.

    Science.gov (United States)

    Pinto, Edgar; Soares, Carlos; Couto, Cristina M C M; Almeida, Agostinho

    2015-01-01

    Because of the scientific evidence showing that arsenic (As), cadmium (Cd), and nickel (Ni) are human genotoxic carcinogens, the European Union (EU) recently set target values for metal concentration in ambient air (As: 6 ng/m(3), Cd: 5 ng/m(3), Ni: 20 ng/m(3)). The aim of our study was to determine the concentration levels of these trace elements in Porto Metropolitan Area (PMA) in order to assess whether compliance was occurring with these new EU air quality standards. Fine (PM2.5) and inhalable (PM10) air particles were collected from October 2011 to July 2012 at two different (urban and suburban) locations in PMA. Samples were analyzed for trace elements content by inductively coupled plasma-mass spectrometry (ICP-MS). The study focused on determination of differences in trace elements concentration between the two sites, and between PM2.5 and PM10, in order to gather information regarding emission sources. Except for chromium (Cr), the concentration of all trace elements was higher at the urban site. However, results for As, Cd, Ni, and lead (Pb) were well below the EU limit/target values (As: 1.49 ± 0.71 ng/m(3); Cd: 1.67 ± 0.92 ng/m(3); Ni: 3.43 ± 3.23 ng/m(3); Pb: 17.1 ± 10.1 ng/m(3)) in the worst-case scenario. Arsenic, Cd, Ni, Pb, antimony (Sb), selenium (Se), vanadium (V), and zinc (Zn) were predominantly associated to PM2.5, indicating that anthropogenic sources such as industry and road traffic are the main source of these elements. High enrichment factors (EF > 100) were obtained for As, Cd, Pb, Sb, Se, and Zn, further confirming their anthropogenic origin.

  14. Air conditioning according to Earth, Wind and Fire. Climate cascade is effective and energy efficient; Airconditioning volgens Earth, Wind and Fire. Klimaatcascade is effectief en energievriendelijk

    Energy Technology Data Exchange (ETDEWEB)

    Bronsema, B. [Sectie klimaatontwerp en Duurzaamheid, Afdeling Architectural Engineering and Technology, Technische Universiteit Delft, Delft (Netherlands)

    2012-06-15

    In a collaboration project of the Technical University in Delft, the Technical University of Delft and VVKH Architects, a project was started in 2007 to examine whether gravitation and the ambient energy of earth mass, wind and solar can be deployed for a natural climate control in buildings. The climate cascade, a promising sub concept, is a gravity-driven construction component for conditioning ventilation air. [Dutch] In een samenwerkingsproject van de TU Delft, de TU Eindhoven en VVKH Architecten is in 2007 een project gestart om te onderzoeken of zwaartekracht en de omgevingsenergie van aardmassa, wind en zon kunnen worden ingezet voor een natuurlijke klimaatregeling van gebouwen. De klimaatcascade, een veelbelovend subconcept, is een door zwaartekracht gedreven bouwdeel voor conditionering van ventilatielucht.

  15. Investigation of levels in ambient air near sources of Polychlorinated Biphenyls (PCBs) in Kanpur, India, and risk assessment due to inhalation.

    Science.gov (United States)

    Goel, Anubha; Upadhyay, Kritika; Chakraborty, Mrinmoy

    2016-05-01

    Polychlorinated biphenyls (PCBs) are a class of organic compounds listed as persistent organic pollutant and have been banned for use under Stockholm Convention (1972). They were used primarily in transformers and capacitors, paint, flame retardants, plasticizers, and lubricants. PCBs can be emitted through the primary and secondary sources into the atmosphere, undergo long-range atmospheric transport, and hence have been detected worldwide. Reported levels in ambient air are generally higher in urban areas. Active sampling of ambient air was conducted in Kanpur, a densely populated and industrialized city in the Indo-Gangetic Plain, for detection of 32 priority PCBs, with the aim to determine the concentration in gas/particle phase and assess exposure risk. More than 50 % of PCBs were detected in air. Occurrence in particles was dominated by heavier congeners, and levels in gas phase were below detection. Levels determined in this study are lower than the levels in Coastal areas of India but are at par with other Asian countries where majority of sites chosen for sampling were urban industrial areas. Human health risk estimates through air inhalation pathway were made in terms of lifetime average daily dose (LADD) and incremental lifetime cancer risks (ILCR). The study found lower concentrations of PCBs than guideline values and low health risk estimates through inhalation within acceptable levels, indicating a minimum risk to the adults due to exposure to PCBs present in ambient air in Kanpur.

  16. Exposure to ambient air pollution in Canada and the risk of adult leukemia.

    Science.gov (United States)

    Winters, Nicholas; Goldberg, Mark S; Hystad, Perry; Villeneuve, Paul J; Johnson, Kenneth C

    2015-09-01

    There is a paucity of studies investigating adult leukemia and air pollution. To address this gap, we analyzed data from a Canadian population-based case-control study conducted in 1994-1997. Cases were 1064 adults with incident leukemia and controls were 5039 healthy adults. We used data from satellites and fixed-site monitoring stations to estimate residential concentrations of NO2 and fine particulate matter (PM2.5) for the period prior to diagnosis, starting in 1975 and ending in 1994. We modeled the average annual exposure of each subject. Odds ratios (OR) and their 95% confidence intervals (CI) were estimated using logistic regression, adjusted for age, gender, province, smoking, education, body mass index, income, and self-reported exposures to ionizing radiation and benzene. We found an 'n-shaped' response function between exposure to NO2 and all forms of leukemia: from the tenth percentile to the median (4.51 to 14.66 ppb), the OR was 1.20; 95% CI: 0.97-1.48 and from the 75th percentile to the 90th (22.75 to 29.7 ppb), the OR was 0.79; 95% CI 0.68-0.93. For PM2.5 we found a response function consistent with a linear model, with an OR per 10 μg/m(3) of 0.97 (95% CI 0.75-1.26). For chronic lymphocytic leukemia we found response functions that were consistent with a simple linear model, with an OR per 5 ppb of NO2 of 0.93 (95% CI 0.86-1.00) and an OR per 10 μg/m(3) of PM2.5 of 0.62 (95% CI 0.42-0.93). In summary, for chronic lymphocytic leukemia we found no evidence of an association with air pollution and with all forms of leukemia we found weak evidence of an association only at low concentrations of NO2. It is possible that these inconsistent results may have arisen because of unaccounted urban/rural differences or possibly from a selection effect, especially among controls.

  17. A reactive and sensitive diffusion sampler for the determination of aldehydes and ketones in ambient air

    Science.gov (United States)

    Uchiyama, Shigehisa; Hasegawa, Shuji

    We developed a diffusive sampling device (DSD-carbonyl) for organic carbonyl compounds (aldehydes and ketones) which is suitable for collection and analysis of low concentration levels. This sampling device is composed of three parts, an exposure part made of a porous polytetrafluoroethylene (PPTFE) tube, an analysis part made of polypropylene (PP) tubing and an absorbent part made of 2,4-dinitrophenylhydrazine (DNPH) coated silica gel (DNPH-silica). Aldehydes and ketones diffuse to the DSD-carbonyl through PPTFE-tube by the mechanism of molecular diffusion and react specifically with DNPH to form a stable DNPH-derivatives. Collection is controlled by moving the absorbent from the exposure part to the analysis part by changing the posture of the DSD-carbonyl. DNPH-derivatives were eluted from an analysis part of DSD-carbonyl with acetonitrile directly and analyzed by high performance liquid chromatography (HPLC). The advantages of the DSD-carbonyl are the following: (1) The DSD-carbonyl can be used in a wide range of concentration of aldehydes and ketones in atmosphere, as the DSD-carbonyl exposure part has a variable diffusion area, (2) DNPH-derivatives are eluted from DNPH-silica without contamination of air. (3) The sampler can be applied to active sampling by connecting it with a pump. The limit of detection (LOD) for concentrations of major aldehydes and ketones ranged from 0.072 to 0.13 ppb, and the limit of quantitation (LOQ) ranged from 0.24 to 0.42 ppb. The coefficient variation (CV) for concentrations of major aldehydes and ketones ranged from 2.5 to 3.0% in laboratory air. The DSD-carbonyl method and active sampling method (US EPA method IP-6A) showed a good correlation (formaldehyde, r2=0.995). The uptake rates for formaldehyde, acetaldehyde, and acetone were estimated as 0.078, 0.062 and 0.079 nmol ppb -1 h -1, respectively. It is possible to estimate atmospheric aldehydes and ketones at parts per billion (ppb), with high sensitivity and precision, by

  18. Exposure to ambient air pollution in Canada and the risk of adult leukemia

    Energy Technology Data Exchange (ETDEWEB)

    Winters, Nicholas [Department of Medicine, McGill University, Montreal, Quebec (Canada); Goldberg, Mark S., E-mail: mark.goldberg@mcgill.ca [Department of Medicine, McGill University, Montreal, Quebec (Canada); Division of Clinical Epidemiology, McGill University Health Centre, 687 Pine Ave. W., R4.29, Montreal, Quebec H3A 1A1 (Canada); Hystad, Perry [College of Public Health and Human Sciences, Oregon State University, Corvallis, OR (United States); Villeneuve, Paul J. [Department of Health Sciences, Carleton University, Ottawa, Ontario (Canada); Johnson, Kenneth C. [Science Integration Division, Centre for Chronic Disease Prevention and Control, Public Health Agency of Canada, Ottawa, Ontario (Canada)

    2015-09-01

    There is a paucity of studies investigating adult leukemia and air pollution. To address this gap, we analyzed data from a Canadian population-based case–control study conducted in 1994–1997. Cases were 1064 adults with incident leukemia and controls were 5039 healthy adults. We used data from satellites and fixed-site monitoring stations to estimate residential concentrations of NO{sub 2} and fine particulate matter (PM{sub 2.5}) for the period prior to diagnosis, starting in 1975 and ending in 1994. We modeled the average annual exposure of each subject. Odds ratios (OR) and their 95% confidence intervals (CI) were estimated using logistic regression, adjusted for age, gender, province, smoking, education, body mass index, income, and self-reported exposures to ionizing radiation and benzene. We found an ‘n-shaped’ response function between exposure to NO{sub 2} and all forms of leukemia: from the tenth percentile to the median (4.51 to 14.66 ppb), the OR was 1.20; 95% CI: 0.97–1.48 and from the 75th percentile to the 90th (22.75 to 29.7 ppb), the OR was 0.79; 95% CI 0.68–0.93. For PM{sub 2.5} we found a response function consistent with a linear model, with an OR per 10 μg/m{sup 3} of 0.97 (95% CI 0.75–1.26). For chronic lymphocytic leukemia we found response functions that were consistent with a simple linear model, with an OR per 5 ppb of NO{sub 2} of 0.93 (95% CI 0.86–1.00) and an OR per 10 μg/m{sup 3} of PM{sub 2.5} of 0.62 (95% CI 0.42–0.93). In summary, for chronic lymphocytic leukemia we found no evidence of an association with air pollution and with all forms of leukemia we found weak evidence of an association only at low concentrations of NO{sub 2}. It is possible that these inconsistent results may have arisen because of unaccounted urban/rural differences or possibly from a selection effect, especially among controls. - Highlights: • Analyzed associations between incidence of adult leukemia and PM • We used 20-year residential

  19. Potential Industrial Applications of the One Atmosphere Uniform Glow Discharge Plasma (OAUGDP) Operating in Ambient Air

    Science.gov (United States)

    Reece Roth, J.

    2004-11-01

    The majority of industrial plasma processing with glow discharges has been conducted at pressures below 10 torr. This tends to limit applications to high value workpieces as a result of the high capital cost of vacuum systems and the production constraints of batch processing. It has long been recognized that glow discharge plasmas would play a much larger industrial role if they could be generated at one atmosphere. The One Atmosphere Uniform Glow Discharge Plasma (OAUGDP), developed at the University of Tennessee's Plasma Sciences Laboratory, is a non-thermal RF plasma operating on displacement currents with the time-resolved characteristics of a classical low pressure DC normal glow discharge. As a glow discharge, the OAUGDP operates with maximum electrical efficiency at the Stoletow point, where the energy input per ion-electron pair is a minimum [1, 2]. Several interdisciplinary teams have investigated potential applications of the OAUGDP. These teams included collaborators from the UTK Textiles and Nonwovens Development Center (TANDEC), and the Departments of Electrical and Computer Engineering, Microbiology, and Food Science and Technology, as well as the NASA Langley Research Center. The potential applications of the OAUGDP have all been at one atmosphere and room temperature, using air as the working gas. These applications include sterilizing medical and dental equipment; sterilizable air filters to deal with the "sick building syndrome"; removal of soot from Diesel engine exhaust; subsonic plasma aerodynamic effects, including flow re-attachment to airfoils and boundary layer modification; electrohydrodynamic (EDH) flow control of working gases; increasing the surface energy of materials; improving the adhesion of paints and electroplated layers: improving the wettability and wickability of fabrics; stripping of photoresist; and plasma deposition and directional etching of potential microelectronic relevance. [1] J. R. Roth, Industrial Plasma Engineering

  20. Long-Term Exposure to Ambient Air Pollution and Metabolic Syndrome in Adults.

    Directory of Open Access Journals (Sweden)

    Ikenna C Eze

    Full Text Available Air pollutants (AP play a role in subclinical inflammation, and are associated with cardiovascular morbidity and mortality. Metabolic syndrome (MetS is inflammatory and precedes cardiovascular morbidity and type 2 diabetes. Thus, a positive association between AP and MetS may be hypothesized. We explored this association, (taking into account, pathway-specific MetS definitions, and its potential modifiers in Swiss adults. We studied 3769 participants of the Swiss Cohort Study on Air Pollution and Lung and Heart Diseases in Adults, reporting at least four-hour fasting time before venepuncture. AP exposures were 10-year mean residential PM10 (particulate matter <10μm in diameter and NO2 (nitrogen dioxide. Outcomes included MetS defined by World Health Organization (MetS-W, International Diabetes Federation (MetS-I and Adult Treatment Panel-III (MetS-A using four- and eight-hour fasting time limits. We also explored associations with individual components of MetS. We applied mixed logistic regression models to explore these associations. The prevalence of MetS-W, MetS-I and MetS-A were 10%, 22% and 18% respectively. Odds of MetS-W, MetS-I and MetS-A increased by 72% (51-102%, 31% (11-54% and 18% (4-34% per 10μg/m3 increase in 10-year mean PM10. We observed weaker associations with NO2. Associations were stronger among physically-active, ever-smokers and non-diabetic participants especially with PM10 (p<0.05. Associations remained robust across various sensitivity analyses including ten imputations of missing observations and exclusion of diabetes cases. The observed associations between AP exposure and MetS were sensitive to MetS definitions. Regarding the MetS components, we observed strongest associations with impaired fasting glycemia, and positive but weaker associations with hypertension and waist-circumference-based obesity. Cardio-metabolic effects of AP may be majorly driven by impairment of glucose homeostasis, and to a less

  1. Benefits of European climate policies for mercury air pollution

    OpenAIRE

    2014-01-01

    This paper presents the methodology and results of impact assessment of renewable energy policies on atmospheric emissions of mercury in Europe. The modeling exercise described here involves an interaction of several models. First, a set of energy scenarios has been developed with the REMix (Renewable Energy Mix) model that simulates different levels of penetration of renewable energies in the European power sector. The energy scenarios were input to the GAINS (Greenhouse Gas and Air Polluti...

  2. Evaluación de la contaminación atmosférica en el aire ambiente de Manizales por COPs y PM10

    OpenAIRE

    Cortés Araújo, Johana De La Paz

    2013-01-01

    Este trabajo presenta un estudio de la calidad del aire realizado en cuatro puntos de la ciudad de Manizales, en el cual se analizó la dinámica de dispersión de las dioxinas (PCDD), furanos (PCDFs), dioxin-like PCBs (dl-PCBs) y el Material Particulado inferior a 10 micrómetros de diámetro (PM10) en el aire ambiente de la ciudad. Las PCDD/PCDFs fueron evaluadas en la fase gaseosa y en la fase particulada, utilizando equipos de monitoreo de aire pasivo (PAS) y equipos de alto volumen (HiVol), r...

  3. The potential effect of differential ambient and deployment chamber temperatures on PRC derived sampling rates with polyurethane foam (PUF) passive air samplers

    Energy Technology Data Exchange (ETDEWEB)

    Kennedy, Karen, E-mail: k.kennedy@uq.edu.a [University of Queensland, EnTox (National Research Centre for Environmental Toxicology), 39 Kessels Rd., Coopers Plains QLD 4108 (Australia); Hawker, Darryl W. [Griffith University, School of Environment, Nathan QLD 4111 (Australia); Bartkow, Michael E. [University of Queensland, EnTox (National Research Centre for Environmental Toxicology), 39 Kessels Rd., Coopers Plains QLD 4108 (Australia); Carter, Steve [Queensland Health Forensic and Scientific Services, Coopers Plains QLD 4108 (Australia); Ishikawa, Yukari; Mueller, Jochen F. [University of Queensland, EnTox (National Research Centre for Environmental Toxicology), 39 Kessels Rd., Coopers Plains QLD 4108 (Australia)

    2010-01-15

    Performance reference compound (PRC) derived sampling rates were determined for polyurethane foam (PUF) passive air samplers in both sub-tropical and temperate locations across Australia. These estimates were on average a factor of 2.7 times higher in summer than winter. The known effects of wind speed and temperature on mass transfer coefficients could not account for this observation. Sampling rates are often derived using ambient temperatures, not the actual temperatures within deployment chambers. If deployment chamber temperatures are in fact higher than ambient temperatures, estimated sampler-air partition coefficients would be greater than actual partition coefficients resulting in an overestimation of PRC derived sampling rates. Sampling rates determined under measured ambient temperatures and estimated deployment chamber temperatures in summer ranged from 7.1 to 10 m{sup 3} day{sup -1} and 2.2-6.8 m{sup 3} day{sup -1} respectively. These results suggest that potential differences between ambient and deployment chamber temperatures should be considered when deriving PRC-based sampling rates. - Internal deployment chamber temperatures rather than ambient temperatures may be required to accurately estimate PRC-based sampling rates.

  4. Embryotoxicity of organic extracts from airborne particulates in ambient air in the chicken embryo

    Energy Technology Data Exchange (ETDEWEB)

    Matsumoto, H.; Kashimoto, T.

    1986-07-01

    A fraction containing polycyclic aromatic hydrocarbons (PAHs), prepared from an organic extract of airborne particulate matter, was separated into nine subfractions by high pressure liquid chromatography (HPLC). The embryotoxicity of each of these fractions was investigated and analysis for PAHs by capillary gas chromatography-mass spectrometry (GC-MS) was performed. The ninth subfraction, with coronene as its main component, had the strongest toxic effects on chicken embryos per m/sup 3/ of air. Of the remaining eight subfractions, three had the greatest toxicity: the second fraction with benzofluoranthenes and benzo(e)pyrene as the main components, the fourth fraction having PAH-estimated compounds in small amounts, and the fifth fraction with indeno(1,2,3-cd)pyrene and benzo(ghi)perylene as the main ingredients had the greatest toxicity. These findings indicate PAHs to be responsible for embryotoxicity but the total amounts were not necessarily proportional to it. For further characterization of toxicity, the effects of each PAH and/or quantification of other embryotoxic compounds possibly present in small amounts should be investigated.

  5. Particle size distributions of currently used pesticides in ambient air of an agricultural Mediterranean area

    Science.gov (United States)

    Coscollà, Clara; Muñoz, Amalia; Borrás, Esther; Vera, Teresa; Ródenas, Milagros; Yusà, Vicent

    2014-10-01

    This work presents first data on the particle size distribution of 16 pesticides currently used in Mediterranean agriculture in the atmosphere. Particulate matter air samples were collected using a cascade impactor distributed into four size fractions in a rural site of Valencia Region, during July to September in 2012 and from May to July in 2013. A total of 16 pesticides were detected, including six fungicides, seven insecticides and three herbicides. The total concentrations in the particulate phase (TSP: Total Suspended Particulate) ranged from 3.5 to 383.1 pg m-3. Most of the pesticides (such as carbendazim, tebuconazole, chlorpyrifos-ethyl and chlorpyrifos-methyl) were accumulated in the ultrafine-fine (<1 μm) and coarse (2.5-10 μm) particle size fractions. Others like omethoate, dimethoate and malathion were presented only in the ultrafine-fine size fraction (<1 μm). Finally, diuron, diphenylamine and terbuthylazine-desethyl-2-OH also show a bimodal distribution but mainly in the coarse size fractions.

  6. Nonattainment of national ambient air quality standards: implications for energy policy

    Energy Technology Data Exchange (ETDEWEB)

    Garvey, D.B.; Streets, D.G.; Kotecki, R.; Senew, M.

    1979-10-01

    In accordance with the 1977 Clean Air Act Amendments, EPA established regulations governing new and existing sources of emissions in areas where the NAAQS are being exceeded. These requirements may constrain the implementation of a national energy policy to increase the use of coal in utilities and industries. The states designated the nonattainment areas and prepared State Implementation Plans, outlining strategies for attaining the standards by the deadline of December 31, 1982. This report contains maps of nonattainment areas for all pollutants and summaries of the attainment strategies for those pollutants most likely to affect fossil-fueled energy development - SO/sub 2/, TSP, and NO/sub x/. The review of SIPs indicates that attainment of SO/sub 2/ standards should be relatively easy. Attainment of TSP standards may be more difficult since point sources are already well controlled and further reductions in emissions will require controls on fugitive sources. NO/sub x/ nonattainment is currently limited to three small areas. The report also contains an examination of emission limitations in nonattainment areas and a national assessment of the potential constraints of nonattainment on energy development in 1985 to 1990. The assessment concludes that constraints on projected new coal-fired utilities should not be significant. Constraints on expanded industrial coal use from TSP nonattainment may be significant but the effects of SO/sub 2/ nonattainment should be limited.

  7. Gas phase formation of extremely oxidized pinene reaction products in chamber and ambient air

    Directory of Open Access Journals (Sweden)

    M. Ehn

    2012-06-01

    Full Text Available High molecular weight (300–650 Da naturally charged negative ions have previously been observed at a boreal forest site in Hyytiälä, Finland. The long-term measurements conducted in this work showed that these ions are observed practically every night between spring and autumn in Hyytiälä. The ambient mass spectral patterns could be reproduced in striking detail during additional measurements of α-pinene (C10H16 oxidation at low-OH conditions in the Jülich Plant Atmosphere Chamber (JPAC. The ions were identified as clusters of the nitrate ion (NO3 and α-pinene oxidation products reaching oxygen to carbon ratios of 0.7–1.3, while retaining most of the initial ten carbon atoms. Attributing the ions to clusters instead of single molecules was based on additional observations of the same extremely oxidized organics in clusters with HSO4 (Hyytiälä and C3F5O2 (JPAC. The most abundant products in the ion spectra were identified as C10H14O7, C10H14O9, C10H16O9, and C10H14O11. The mechanism responsible for forming these molecules is still not clear, but the initial reaction is most likely ozone attack at the double bond, as the ions are mainly observed under dark conditions. β-pinene also formed highly oxidized products under the same conditions, but less efficiently, and mainly C9 compounds which were not observed in Hyytiälä, where β-pinene on average is 4–5 times less abundant than α-pinene. Further, to explain the high O/C together with the relatively high H/C, we propose that geminal diols and/or hydroperoxide groups may be important. We estimate that the night-time concentration of the sum of the neutral extremely oxidized products is on the order of 0.1–1 ppt (~10

  8. Gas phase formation of extremely oxidized pinene reaction products in chamber and ambient air

    Directory of Open Access Journals (Sweden)

    M. Ehn

    2012-02-01

    Full Text Available High molecular weight (300–650 Da naturally charged negative ions have previously been observed at a boreal forest site in Hyytiälä, Finland. The long-term measurements conducted in this work showed that these ions are observed practically every night during spring and summer in Hyytiälä. The ambient mass spectral patterns could be reproduced in striking detail during additional measurements of α-pinene (C10H16 oxidation at low-OH conditions in the Jülich Plant Atmosphere Chamber (JPAC. The ions were identified as clusters of the nitrate ion (NO3 and α-pinene oxidation products reaching oxygen to carbon ratios of 0.7–1.3, while retaining most of the initial ten carbon atoms. Attributing the ions to clusters instead of single molecules was based on additional observations of the same extremely oxidized organics in clusters with HSO4 (Hyytiälä and C3F5O2 (JPAC. The most abundant products in the ion spectra were identified as C105H14O7, C10H14O9, C10H16O9, and C10H14O11. The mechanism responsible for forming these molecules is still not clear, but the initial reaction is most likely ozone attack at the double bond, as the ions are mainly observed under dark conditions. β-pinene also formed highly oxidized products under the same conditions, but less efficiently, and mainly C9 compounds which were not observed in Hyytiälä, where β-pinene on average is 4–5 times less abundant than α-pinene. Further, to explain the high O/C together with the relatively high H/C, we propose that geminal diols and/or hydroperoxide groups may be important. We estimate that the night-time concentration of the sum of the neutral extremely oxidized products is on the order of 0.1–1 ppt (~10

  9. VARIATIONAL ITERATION SOLVING METHOD FOR SEA-AIR OSCILLATOR MODEL OF INTERDECADAL CLIMATE FLUCTUATIONS

    Institute of Scientific and Technical Information of China (English)

    MO Jia-qi; LIN Yi-hua; WANG Hui

    2005-01-01

    Atmospheric physics is a very complicated natural phenomenon and needs to simplify its basic models for the sea-air oscillator. And it is solved by using the approximate method. The variational iteration method is a simple and valid method. In this paper the coupled system for a sea-air oscillator model of interdecadal climate fluctuations is considered. Firstly, through introducing a set of functions, and computing the variations, the Lagrange multipliers are obtained. And then, the generalized expressions of variational iteration are constructed. Finally, through selecting appropriate initial iteration from the iteration expressions, the approximations of solution for the sea-air oscillator model are solved successively.

  10. Key Technologies of Using Renewable Energy to Capture Carbon from Ambient Air Directly%新能源驱动的从空气中直接捕碳的关键技术

    Institute of Scientific and Technical Information of China (English)

    黎灿兵; 王煌; 耿英会; 孙良; 曹一家; 石海清

    2014-01-01

    Reducing the content of carbon dioxide in air is the key to addressing climate change.Carbon capture and storage is an important measure to reduce carbon dioxide emission.Capturing carbon from ambient air directly needs large amounts of energy.The loads on carbon capture devices are flexible,which to some extent can be driven by intermittent energy. Renewable energy such as wind power and solar energy has great potential for development,which has the characteristics of fluctuation.Using renewable energy to capture carbon from ambient air directly can reduce the concentration of carbon dioxide in the atmosphere.It is a promising way to address global climate change.This paper analyzes the potential of using renewable energy to capture carbon from ambient air directly,and proposes the key technologies of using renewable energy to capture carbon.The planning of using renewable energy to capture carbon is preliminarily studied,and the development trend of carbon capture driven by renewable energy is discussed.%降低空气中二氧化碳的含量是应对气候变化的关键。碳捕集与封存是减少二氧化碳排放量的重要措施。从空气中直接捕碳需要消耗大量能源。捕碳装置负荷是柔性负荷,可以在一定程度上接受波动性能源驱动。风能、太阳能等新能源开发潜力巨大,具有波动性的特点。利用其驱动捕碳装置从空气中直接捕碳,可以降低大气中二氧化碳的浓度,可望成为解决全球气候变化问题的关键途径。文中分析了利用新能源驱动的从空气中直接捕碳的潜力,提出了新能源捕碳的关键技术。对新能源捕碳的规划进行了初步研究,并对利用新能源捕碳的发展趋势进行了展望。

  11. Indoor air quality of a museum in a subtropical climate: the Oscar Niemeyer museum in Curitiba, Brazil.

    Science.gov (United States)

    Godoi, Ricardo H M; Carneiro, Barbara H B; Paralovo, Sarah L; Campos, Vania P; Tavares, Tania M; Evangelista, Heitor; Van Grieken, Rene; Godoi, Ana F L

    2013-05-01

    The assessment of damage to indoor cultural heritage, in particular by pollutants, is nowadays a major and growing concern for curators and conservators. Nevertheless, although many museums have been widely investigated in Europe, the effects of particulate matter and gaseous pollutants in museums under tropical and subtropical climates and with different economic realities are still unclear. An important portion of the world's cultural heritage is currently in tropical countries where both human and financial resources for preserving museum collections are limited. Hence, our aim is to assess the damage that can be caused to the artwork by pollution in hot and humid environments, where air quality and microclimatic condition differences can cause deterioration. As a case study, particulate matter as well as gases were collected at the Oscar Niemeyer Museum (MON) in Curitiba, Brazil, where large modern and contemporary works of art are displayed. NO2, SO2, O3, Acetic Acid, Formic Acids and BTEX, in the ambient air, were sampled by means of passive diffusive sampling and their concentrations were determined by IC or GC-MS. The particulate matter was collected in bulk form and analyzed with the use of energy dispersive X-ray fluorescence and aethalometer. The chemical compositions of individual particles were quantitatively elucidated, including low-Z components like C, N and O, as well as higher-Z elements, using automated electron probe microanalysis. The gaseous and particulate matter levels were then compared with the concentrations obtained for the same pollutants in other museums, located in places with different climates, and with some reference values provided by international cultural heritage conservation centers. Results are interpreted separately and as a whole with the specific aim of identifying compounds that could contribute to the chemical reactions taking place on the surfaces of artifacts and which could potentially cause irreversible damage to the

  12. Air traffic simulation in chemistry-climate model EMAC 2.41: AirTraf 1.0

    Science.gov (United States)

    Yamashita, Hiroshi; Grewe, Volker; Jöckel, Patrick; Linke, Florian; Schaefer, Martin; Sasaki, Daisuke

    2016-09-01

    Mobility is becoming more and more important to society and hence air transportation is expected to grow further over the next decades. Reducing anthropogenic climate impact from aviation emissions and building a climate-friendly air transportation system are required for a sustainable development of commercial aviation. A climate optimized routing, which avoids climate-sensitive regions by re-routing horizontally and vertically, is an important measure for climate impact reduction. The idea includes a number of different routing strategies (routing options) and shows a great potential for the reduction. To evaluate this, the impact of not only CO2 but also non-CO2 emissions must be considered. CO2 is a long-lived gas, while non-CO2 emissions are short-lived and are inhomogeneously distributed. This study introduces AirTraf (version 1.0) that performs global air traffic simulations, including effects of local weather conditions on the emissions. AirTraf was developed as a new submodel of the ECHAM5/MESSy Atmospheric Chemistry (EMAC) model. Air traffic information comprises Eurocontrol's Base of Aircraft Data (BADA Revision 3.9) and International Civil Aviation Organization (ICAO) engine performance data. Fuel use and emissions are calculated by the total energy model based on the BADA methodology and Deutsches Zentrum für Luft- und Raumfahrt (DLR) fuel flow method. The flight trajectory optimization is performed by a genetic algorithm (GA) with respect to a selected routing option. In the model development phase, benchmark tests were performed for the great circle and flight time routing options. The first test showed that the great circle calculations were accurate to -0.004 %, compared to those calculated by the Movable Type script. The second test showed that the optimal solution found by the algorithm sufficiently converged to the theoretical true-optimal solution. The difference in flight time between the two solutions is less than 0.01 %. The dependence of

  13. Adaptation of forest ecosystems to air pollution and climate change: a global assessment on research priorities

    Directory of Open Access Journals (Sweden)

    Serengil Y

    2011-04-01

    Full Text Available Climate change and air pollution are two of the anthropogenic stressors that require international collaboration. Influence mechanisms and combating strategies towards them have similarities to some extent. Impacts of air pollution and climate change have long been studied under IUFRO Research Group 7.01 and state of the art findings are presented at biannual meetings. Monitoring, modelling, assessment of multiple stressors, ecophysiology, and nutrient cycles have been thoroughly studied aspects of climate change and air pollution research for a long time under the umbrella of IUFRO RG 7.01. Recently, social and economic issues together with water relations are gaining more attention in parallel with science requirements on adaptation. In this paper, we summarise the main research needs emphasized at the recent 24th IUFRO RG 7.01 Conference titled “Adaptation of Forest Ecosystems to Air Pollution and Climate Change”. One important conclusion of the conference was the need for information on nutritional status of forest stands for sustainable forest management. It has been suggested to maintain long-term monitoring programs and to account for the effects of extreme years, and past and present management practices. Long-term monitoring can also help to understand the effects of forestry treatments on the nutrient and water budgets of the ecosystems which may enable to improve management practices like water saving silviculture.

  14. Aerosols: connection between regional climatic change and air quality (Iupac Technical Report)

    NARCIS (Netherlands)

    Slanina, J.; Zhang, Y.H.

    2004-01-01

    yAerosols play an important role in all problems connected with air pollution, ranging from very local effects and human health problems to regional problems such as acid deposition and eutrophication up to continental and global questions such as stratospheric ozone loss and climatic change. In thi

  15. A Literature Review on Heating of Ventilation Air with Large Diameter Earth Tubes in Cold Climates

    Directory of Open Access Journals (Sweden)

    Lili Tan

    2013-07-01

    Full Text Available Earth-air heat exchange (EAHE systems offer the possibility of reducing use of nonrenewable energy for heating ventilation air in cold climates. The number of installations of large diameter (greater than 900 mm EAHE systems reported for cold climates is small. Even less has been reported on their heating performance, but the available information suggests that further rigorous assessment is warranted to determine whether the reported better than expected temperature rise is supported and, if so, the reasons for this. Another concern is the possibility of long-term heat depletion in the surrounding soil, which would affect performance. Only a couple of short-term experimental studies of ground temperature effects of heating with EAHE were found for cool climates. Four articles that addressed ground temperature effects with horizontal ground source heat pump exchangers had conflicting findings regarding heat depletion in the soil.

  16. Social Justice Is in the Air: Teaching Climate Change and Air Pollution with Scientific and Social Inquiry

    Science.gov (United States)

    Hahnenberger, M.

    2014-12-01

    The intersection of environmental with social problems is a growing area of concern for scientists, policy makers, and citizens. Climate change and air pollution are two current environmental issues holding the public's attention which require collaboration of all stakeholders to create meaningful solutions. General education science co