Holographic charge density waves
Donos, Aristomenis
2013-01-01
We show that strongly coupled holographic matter at finite charge density can exhibit charge density wave phases which spontaneously break translation invariance while preserving time-reversal and parity invariance. We show that such phases are possible within Einstein-Maxwell-dilaton theory in general spacetime dimensions. We also discuss related spatially modulated phases when there is an additional coupling to a second vector field, possibly with non-zero mass. We discuss how these constructions, and others, should be associated with novel spatially modulated ground states.
Holographic charge density waves
Donos, Aristomenis; Gauntlett, Jerome P.
2013-06-01
We show that strongly coupled holographic matter at finite charge density can exhibit charge density wave phases which spontaneously break translation invariance while preserving time-reversal and parity invariance. We show that such phases are possible within Einstein-Maxwell-dilaton theory in general spacetime dimensions. We also discuss related spatially modulated phases when there is an additional coupling to a second vector field, possibly with nonzero mass. We discuss how these constructions, and others, should be associated with novel spatially modulated ground states.
Charge density waves in solids
Gor'kov, LP
2012-01-01
The latest addition to this series covers a field which is commonly referred to as charge density wave dynamics.The most thoroughly investigated materials are inorganic linear chain compounds with highly anisotropic electronic properties. The volume opens with an examination of their structural properties and the essential features which allow charge density waves to develop.The behaviour of the charge density waves, where interesting phenomena are observed, is treated both from a theoretical and an experimental standpoint. The role of impurities in statics and dynamics is considered and an
Microscopic Charge Density Wave Transport
Slot, Erwin
2005-01-01
This thesis describes the work performed on crystals with a phase transition to a Charge-Density Wave (CDW). The electrical transport properties change when crystal sizes are smaller than characteristic length scales for CDWs, typically 1 micrometer. In contrast to metals, semiconductors and superco
Thermoelectric studies of charge density wave dynamics.
McDonald, Ross; Harrison, Neil; Singleton, John
2008-03-01
The conventional pyroelectric effect is intimately connected to the symmetry, or rather lack of center of symmetry, of the material. Although the experiments we discuss involve studies of low symmetry materials, the pyroelectric currents observed are of an entirely new origin. Systems with broken-translational-symmetry phases that incorporate orbital quantization can exhibit significant departures from thermodynamic equilibrium due to a change in magnetic induction. For charge density wave systems, this metastable state consists of a balance between the density-wave pinning force and the Lorentz force on the extended currents due to the drift of cyclotron orbits. In this way the density wave pinning potential plays a similar role to the edge potential in a two-dimensional electron gas, leading to a large Hall angle and quantization of the Hall resistance. A thermal perturbation that reduces the pinning potential returns the system towards thermal equilibrium, via a phason avalanche orthogonal to the sample surface. The observation of this new form of pyroelectric effect in the high magnetic field phase (B > 30 T) of the organic charge transfer salt α-(BEDT-TTF)2KHg(SCN)4, thus provides a measure of the phason thermopower.
Competition between superconductivity and charge density waves
Kim, Ki-Seok
2007-02-01
We derive an effective field theory for the competition between superconductivity (SC) and charge density waves (CDWs) by employing the SO(3) pseudospin representation of the SC and CDW order parameters. One important feature in the effective nonlinear σ model is the emergence of a Berry phase even at half filling, originating from the competition between SC and CDWs, i.e., the pseudospin symmetry. A-well known conflict between the previous studies of Oshikawa [Phys. Rev. Lett. 84, 1535 (2000)] and Lee and Shankar [Phys. Rev. Lett. 65, 1490 (1990)] is resolved by the appearance of the Berry phase. The Berry phase contribution allows a deconfined quantum critical point of fractionalized charge excitations with e instead of 2e in the SC-CDW quantum transition at half filling. Furthermore, we investigate the stability of the deconfined quantum criticality against quenched randomness by performing a renormalization group analysis of an effective vortex action. We argue that, although randomness results in a weak disorder fixed point differing from the original deconfined quantum critical point, deconfinement of the fractionalized charge excitations still survives at the disorder fixed point owing to a nonzero fixed point value of the vortex charge.
Experimental Evidence for Static Charge Density Waves in Iron Oxypnictides
Martinelli, A.
2017-02-01
In this Letter we report high-resolution synchrotron x-ray powder diffraction and transmission electron microscope analysis of Mn-substituted LaFeAsO samples, demonstrating that a static incommensurate modulated structure develops across the low-temperature orthorhombic phase, whose modulation wave vector depends on the Mn content. The incommensurate structural distortion is likely originating from a charge-density-wave instability, a periodic modulation of the density of conduction electrons associated with a modulation of the atomic positions. Our results add a new component in the physics of Fe-based superconductors, indicating that the density wave ordering is charge driven.
Breathing Charge Density Waves in Intrinsic Josephson Junctions
Shukrinov, Yu M.; Abdelhafiz, H.
2013-01-01
We demonstrate the creation of a charge density wave (CDW) along a stack of coupled Josephson junctions in layered superconductors. Electric charge in each superconducting layer oscillates around some average value, forming a breathing CDW. We show the transformation of a longitudinal plasma wave to CDW in the state corresponding to the outermost branch. Transitions between different types of CDW's related to the inner branches of current voltage characteristics are demonstrated. The effect o...
Magnetothermopower and Nernst effect in unconventional charge density waves
Dóra, Balázs; Maki, Kazumi; Ványolos, András; Virosztek, Attila
2003-12-01
Recently we have shown that the striking angular dependent magnetoresistance in the low-temperature phase (LTP) of α-(BEDT-TTF)2KHg(SCN)4 is consistently described in terms of unconventional charge density wave (UCDW). Here we investigate theoretically the thermoelectric power and the Nernst effect in unconventional density wave (UDW). The present results account consistently for the recent data of magnetothermopower in α-(BEDT-TTF)2KHg(SCN)4 obtained by Choi et al. [Phys. Rev. B 65, 205119 (2002)]. This confirms further our identification of LTP in this salt as UCDW. We propose also that the Nernst effect provides a clear signature of UDW.
Thermal Rounding of the Charge Density Wave Depinning Transition
Middleton, A. Alan
1992-01-01
The rounding of the charge density wave depinning transition by thermal noise is examined. Hops by localized modes over small barriers trigger ``avalanches'', resulting in a creep velocity much larger than that expected from comparing thermal energies with typical barriers. For a field equal to the $T=0$ depinning field, the creep velocity is predicted to have a {\\em power-law} dependence on the temperature $T$; numerical computations confirm this result. The predicted order of magnitude of t...
Fast electronic resistance switching involving hidden charge density wave states
Vaskivskyi, I.; Mihailovic, I. A.; Brazovskii, S.; Gospodaric, J.; Mertelj, T.; Svetin, D.; Sutar, P.; Mihailovic, D.
2016-05-01
The functionality of computer memory elements is currently based on multi-stability, driven either by locally manipulating the density of electrons in transistors or by switching magnetic or ferroelectric order. Another possibility is switching between metallic and insulating phases by the motion of ions, but their speed is limited by slow nucleation and inhomogeneous percolative growth. Here we demonstrate fast resistance switching in a charge density wave system caused by pulsed current injection. As a charge pulse travels through the material, it converts a commensurately ordered polaronic Mott insulating state in 1T-TaS2 to a metastable electronic state with textured domain walls, accompanied with a conversion of polarons to band states, and concurrent rapid switching from an insulator to a metal. The large resistance change, high switching speed (30 ps) and ultralow energy per bit opens the way to new concepts in non-volatile memory devices manipulating all-electronic states.
Photoinduced Enhancement of the Charge Density Wave Amplitude
Singer, A.; Patel, S. K. K.; Kukreja, R.; Uhlíř, V.; Wingert, J.; Festersen, S.; Zhu, D.; Glownia, J. M.; Lemke, H. T.; Nelson, S.; Kozina, M.; Rossnagel, K.; Bauer, M.; Murphy, B. M.; Magnussen, O. M.; Fullerton, E. E.; Shpyrko, O. G.
2016-07-01
Symmetry breaking and the emergence of order is one of the most fascinating phenomena in condensed matter physics. It leads to a plethora of intriguing ground states found in antiferromagnets, Mott insulators, superconductors, and density-wave systems. Exploiting states of matter far from equilibrium can provide even more striking routes to symmetry-lowered, ordered states. Here, we demonstrate for the case of elemental chromium that moderate ultrafast photoexcitation can transiently enhance the charge-density-wave (CDW) amplitude by up to 30% above its equilibrium value, while strong excitations lead to an oscillating, large-amplitude CDW state that persists above the equilibrium transition temperature. Both effects result from dynamic electron-phonon interactions, providing an efficient mechanism to selectively transform a broad excitation of the electronic order into a well-defined, long-lived coherent lattice vibration. This mechanism may be exploited to transiently enhance order parameters in other systems with coupled degrees of freedom.
Photoemission spectra of charge density wave states in cuprates
Tu, Wei-Lin; Chen, Peng-Jen; Lee, Ting-Kuo
Angle-resolved photoemission spectroscopy(ARPES) experiments have reported many exotic properties of cuprates, such as Fermi arc at normal state, two gaps at superconducting state and particle-hole asymmetry at the antinodal direction. On the other hand, a number of inhomogeneous states or so-called charge density waves(CDW) states have also been discovered in cuprates by many experimental groups. The relation between these CDW states and ARPES spectra is unclear. With the help of Gutzwiller projected mean-field theory, we can reproduce the quasiparticle spectra in momentum space. The spectra show strong correspondence to the experimental data with afore-mentioned exotic features in it.
Charge-density waves physics revealed by photoconduction
Energy Technology Data Exchange (ETDEWEB)
Zaitsev-Zotov, S.V., E-mail: serzz@cplire.ru [Kotel' nikov Institute of Radio-engineering and Electronics of the RAS, 125009 Moscow (Russian Federation); Moscow Institute of Physics and Technology, 141700 Dolgoprudny (Russian Federation); Nasretdinova, V.F.; Minakova, V.E. [Kotel' nikov Institute of Radio-engineering and Electronics of the RAS, 125009 Moscow (Russian Federation)
2015-03-01
The results of photoconduction study of the Peierls conductors are reviewed. The studied materials are quasi-one-dimensional conductors with the charge-density wave: K{sub 0.3}MoO{sub 3}, both monoclinic and orthorhombic TaS{sub 3} and also a semiconducting phase of NbS{sub 3} (phase I). Experimental methods, relaxation times, effects of illumination on linear and nonlinear charge transport, the electric-field effect on photoconduction and results of the spectral studies are described. We demonstrate, in particular, that a simple model of modulated energy gap slightly smoothed by fluctuations fits the available spectral data fairly well. The level of the fluctuations is surprisingly small and does not exceed a few percent of the optical energy gap value.
Charge Order Induced in an Orbital Density-Wave State
Singh, Dheeraj Kumar; Takimoto, Tetsuya
2016-04-01
Motivated by recent angle resolved photoemission measurements [D. V. Evtushinsky et al., Phys. Rev. Lett. 105, 147201 (2010)] and evidence of the density-wave state for the charge and orbital ordering [J. García et al., Phys. Rev. Lett. 109, 107202 (2012)] in La0.5Sr1.5MnO4, the issue of charge and orbital ordering in a two-orbital tight-binding model for layered manganite near half doping is revisited. We find that the charge order with the ordering wavevector 2{Q} = (π ,π ) is induced by the orbital order of d-/d+-type having B1g representation with a different ordering wavevector Q, where the orbital order as the primary order results from the strong Fermi-surface nesting. It is shown that the induced charge order parameter develops according to TCO - T by decreasing the temperature below the orbital ordering temperature TCO, in addition to the usual mean-field behavior of the orbital order parameter. Moreover, the same orbital order is found to stabilize the CE-type spin arrangement observed experimentally below TCE < TCO.
Breathing charge density waves in intrinsic Josephson junctions
Shukrinov, Yu. M.; Abdelhafiz, H.
2014-01-01
We demonstrate the creation of a charge density wave (CDW) along a stack of coupled Josephson junctions (JJs) in layered superconductors. Electric charge in each superconducting layer oscillates around some average value, forming a breathing CDW. We show the transformation of a longitudinal plasma wave to CDW in the state corresponding to the outermost branch. Transition between different types of CDW's related to the inner branches of IV characteristic is demonstrated. The effect of the external electromagnetic radiation on the states corresponding to the inner branches differs crucially from the case of the single JJ. The Shapiro steps in the IV characteristics of the junctions in the stack do not correspond directly to the frequency of radiation ω. The system of JJs behaves like a single whole system: the Shapiro steps or their harmonics in the total IV characteristics appear at voltage , where V l is the voltage in the lth junction, N R is the number of JJs in the rotating state, and m and n are integers.
DEFF Research Database (Denmark)
Tanner, D. B.; Cummings, K. D.; Jacobsen, Claus Schelde
1981-01-01
Detailed far-infrared measurements at temperatures from 25 to 300 K provide strong support for a charge-density-wave mechanism for the dc conductivity and microwave dielectric constant of tetrathiafulvalene tetracyanoquinodimethane (TTF-TCNQ). At low temperatures the charge-density wave is pinned...
Deformations of charge-density wave crystals under electric field
Energy Technology Data Exchange (ETDEWEB)
Pokrovskii, V.Ya. [Kotel' nikov Institute of Radioengineering and Electronics of RAS, Mokhovaya 11, 125009 Moscow (Russian Federation)], E-mail: pok@cplire.ru; Zybtsev, S.G.; Loginov, V.B. [Kotel' nikov Institute of Radioengineering and Electronics of RAS, Mokhovaya 11, 125009 Moscow (Russian Federation); Timofeev, V.N. [Baikov Institute of Metallurgy of RAS, Leninsky prosp. 49, 119991 Moscow (Russian Federation); Kolesov, D.V.; Yaminsky, I.V. [Advanced Technologies Center, Department of Physics, Moscow State University, Leninskie Gori, 119991 Moscow (Russian Federation); Gorlova, I.G. [Kotel' nikov Institute of Radioengineering and Electronics of RAS, Mokhovaya 11, 125009 Moscow (Russian Federation)
2009-03-01
We report the effects of electric field induced deformations of quasi one-dimensional conductors with charge-density wave (CDW). The most pronounced sort of deformation is torsional strain (TS). The TS is found to comprise two contributions. The features of the 1st-the larger one-are threshold hysteretic dependence on electric field and high relaxation time {tau}: For o-TaS{sub 3}{tau}{approx}10{sup -2} s at T=80 K and falls as exp(900 K/T) with increasing T. The 2nd contribution is linear in electric field and does not drop with frequency increase. The amplitude of this contribution falls abruptly with T approaching the Peierls transition temperature T{sub P} from below. Similar features of TS are demonstrated for other CDW compounds: (TaSe{sub 4}){sub 2}I, K{sub 0.3}MoO{sub 3} and NbS{sub 3} type II, for which T{sub P}{approx}360 K. We attribute the 1st and the 2nd contributions to large (hysteretic) and small (near-equilibrium) CDW deformations, respectively, likely-shear at the surface. The TS is observed also above T{sub P}: For TaS{sub 3} and (TaSe{sub 4}){sub 2}I typical torsional amplitude is 10{sup -1} deg./V in the resonance regimes, corresponding to the piezomodulus {approx}10{sup -9} m/V. A separate study of TS was performed at room temperature with AFM technique. Apart from this ('intrinsic') effect, we observe electrostatic contribution to the TS. In contrast to the intrinsic response, the electrostatic one is proportional to the potential either over the sample, or over an additional electrode ('gate') placed nearby, but not to the difference of potentials between the sample ends. It is typically 2 orders of magnitude less. The intrinsic TS reveals a new electromechanical effect at room temperature, presumably associated with the excitations of the pinned mode of the CDW fluctuations. Its observation opens prospects for application of quasi one-dimensional conductors as micro- and nano-actuators. Basing on the electrostatic
Generation of localized magnetic moments in the charge-density-wave state
Akzyanov, R. S.; Rozhkov, A. V.
2014-01-01
We propose a mechanism explaining the generation of localized magnetic moments in charge-density-wave compounds. Our model Hamiltonian describes an Anderson impurity placed in a host material exhibiting the charge-density wave. There is a region of the model's parameter space, where even weak Coulomb repulsion on the impurity site is able to localize the magnetic moment on the impurity. The phase diagram of a single impurity at T=0 is mapped. To establish the connection with experiment thermo...
Orbital quantization in the high-magnetic-field state of a charge-density-wave system
Andres, D.; Kartsovnik, M. V.; Grigoriev, P. D.; Biberacher, W.; Müller, H.
2003-11-01
A superposition of the Pauli and orbital couplings of a high magnetic field to charge carriers in a charge-density-wave (CDW) system is proposed to give rise to transitions between subphases with quantized values of the CDW wave vector. By contrast to the purely orbital field-induced density-wave effects which require a strongly imperfect nesting of the Fermi surface, the new transitions can occur even if the Fermi surface is well nested at zero field. We suggest that such transitions are observed in the organic metal α-(BEDT-TTF)2KHg(SCN)4 under a strongly tilted magnetic field.
Directory of Open Access Journals (Sweden)
Alexander I. Voitenko
2011-10-01
Full Text Available A review of the theory describing the coexistence between d-wave superconductivity and s-wave charge-density-waves (CDWs is presented. The CDW gapping is identified with pseudogapping observed in high-Tc oxides. According to the cuprate specificity, the analysis is carried out for the two-dimensional geometry of the Fermi surface (FS. Phase diagrams on the σ0 − α plane—here, σ0 is the ratio between the energy gaps in the parent pure CDW and superconducting states, and the quantity 2α is connected with the degree of dielectric (CDW FS gapping—were obtained for various possible configurations of the order parameters in the momentum space. Relevant tunnel and photoemission experimental data for high-Tc oxides are compared with theoretical predictions. A brief review of the results obtained earlier for the coexistence between s-wave superconductivity and CDWs is also given.
Dimensionality-driven phonon softening and incipient charge density wave instability in TiS2
Dolui, Kapildeb; Sanvito, Stefano
2016-08-01
Density functional theory and density functional perturbation theory are used to investigate the electronic and vibrational properties of TiS2. Within the local density approximation the material is a semimetal both in the bulk and in the monolayer form. Most interestingly we observe a Kohn anomaly in the bulk phonon dispersion, which turns into a charge density wave instability when TiS2 is thinned to less than four monolayers. Such instability, however, disappears when one calculates the electronic structure with a functional, such as the LDA+U, which returns an insulating ground state. In this situation charge-doping or strain does not bring back the charge density wave instability, whereas the formation of the TiSSe alloy does.
Kartsovnik, Mark; Andres, Dieter; Grigoriev, Pavel; Biberacher, Werner; Müller, Harald
2004-04-01
The interlayer magnetoresistance of the low-dimensional organic metal α-(BEDT-TTF) 2KHg(SCN) 4 under pressure shows features which are likely associated with theoretically predicted field-induced charge-density-wave (FICDW) transitions. At ambient pressure, a magnetic field strongly tilted towards the conducting layers induces a series of hysteretic anomalies. We attribute these anomalies to a novel kind of FICDW originating from a superposition of the orbital quantization of the nesting vector and Pauli effect on the charge-density wave.
Energy Technology Data Exchange (ETDEWEB)
Kartsovnik, Mark; Andres, Dieter; Grigoriev, Pavel; Biberacher, Werner; Mueller, Harald
2004-04-30
The interlayer magnetoresistance of the low-dimensional organic metal {alpha}-(BEDT-TTF){sub 2}KHg(SCN){sub 4} under pressure shows features which are likely associated with theoretically predicted field-induced charge-density-wave (FICDW) transitions. At ambient pressure, a magnetic field strongly tilted towards the conducting layers induces a series of hysteretic anomalies. We attribute these anomalies to a novel kind of FICDW originating from a superposition of the orbital quantization of the nesting vector and Pauli effect on the charge-density wave.
Freericks, J. K.; Matveev, O. P.; Shen, Wen; Shvaika, A. M.; Devereaux, T. P.
2017-03-01
In this review, we develop the formalism employed to describe charge-density-wave insulators in pump/probe experiments that use ultrashort driving pulses of light. The theory emphasizes exact results in the simplest model for a charge-density-wave insulator (given by a noninteracting system with two bands and a gap) and employs nonequilibrium dynamical mean-field theory to solve the Falicov–Kimball model in its ordered phase. We show how to develop the formalism and how the solutions behave. Care is taken to describe the details behind these calculations and to show how to verify their accuracy via sum-rule constraints.
The angular magnetothermoelectric power of a charge density wave system
Krstovska, D.; Choi, E. S.; Steven, E.; Brooks, J. S.
2012-07-01
The angular dependence of the magnetothermopower of a charge transfer organic salt α-(ET)2KHg(SCN)4 below (4 K) and above (9 K) the phase transition temperature, Tp = 8 K, and under fields of 15 T and 25 T, below and above the ‘kinkfield’, has been studied. We find that for a longitudinal thermoelectric measurement both an interlayer thermopower (the Seebeck effect), Szz, and a transverse thermopower (the Nernst effect), Syz, exist in all three different B-T phases (the CDW 0, CDW x and metallic states) with large amplitude. Both thermoelectric effects display a resonant-like behavior without a sign reversal at the angles corresponding to angular magnetoresistance oscillation minima and maxima in this compound. The resonant behavior is most evident in the CDW0 state, indicating a mechanism involving the Fermi surface nesting. Angular dependences reveal different behaviors of the thermopower and Nernst effect in the high magnetic field (CDWx) state.
d-Density Wave Scenario Description of the New Hidden Charge Order in Cuprates
Makhfudz, Imam
2016-06-01
In this paper, we show that the theory of high Tc superconductivity based on a microscopic model with d-density wave (DDW) scenario in the pseudogap phase is able to reproduce some of the most important features of the recent experimentally discovered hidden charge order in several families of Cuprates. In particular, by computing and comparing energies of charge orders of different modulation directions derived from a full microscopic theory with d-density wave scenario, the axial charge order ϕX(Y) with wavevector Q = (Q0,0)((0,Q0)) is shown to be unambiguously energetically more favorable over the diagonal charge order ϕX±Y with wavevector Q = (Q0, ± Q0) at least in commensurate limit, to be expected also to hold even to more general incommensurate case, in agreement with experiment. The two types of axial charge order ϕX and ϕY are degenerate by symmetry. We find that within the superconducting background, biaxial (checkerboard) charge order is energetically more favorable than uniaxial (stripe) charge order, and therefore checkerboard axial charge order should be the one observed in experiments, assuming a single domain of charge ordered state on each CuO2 plane.
Resonant soft x-ray scattering and charge density waves in correlated systems
Rusydi, Andrivo
2006-01-01
Summary This work describes results obtained on the study of charge density waves (CDW) in strongly correlated systems with a new experimental method: resonant soft x-ray scattering (RSXS). The basic motivation is the 1986 discovery by Bednorz and Müler of a new type of superconductor, based on Cu a
THEORY OF THE THRESHOLD FIELD FOR THE DEPINNING TRANSITION OF A CHARGE-DENSITY WAVE
PIETRONERO, L; VERSTEEG, M
1991-01-01
The Hamiltonian of an elastic string pinned by random potentials is often used to describe the depinning transition of a charge density wave in the presence of impurity pinning. The properties of the pinned states show close analogies to those of glassy systems, while the depinning transition resemb
Direct Observation of Spin- and Charge-Density Waves in a Luttinger Liquid
Cao, Chenglin; Marcum, Andrew; Mawardi Ismail, Arif; Fonta, Francisco; O'Hara, Kenneth
2016-05-01
At low energy, interacting fermions in one dimension (e.g. electrons in quantum wires or fermionic atoms in 1D waveguides) should behave as Luttinger liquids. In stark contrast to Fermi liquids, the low-energy elementary excitations in Luttinger liquids are collective sound-like modes that propagate independently as spin-density and/or charge-density (i.e. particle-density) waves with generally unequal, and interaction-dependent, velocities. Here we aim to unambiguously confirm this hallmark feature of the Luttinger liquid - the phenomenon of spin-charge separation - by directly observing in real space the dynamics of spin-density and ``charge''-density waves excited in an ultracold gas of spin-1/2 fermions confined in an array of 1D optical waveguides. Starting from a two-component mixture of 6 Li atoms harmonically confined along each of the 1D waveguides, we excite low lying normal modes of the trapped system - namely the spin dipole and density dipole and quadrupole modes - and measure their frequency as a function of interaction strength. Luttinger liquid theory predicts that the spin dipole frequency is strongly dependent on interaction strength whereas the density dipole and quadrupole mode frequencies are relatively insensitive. We will also discuss extending our approach to exciting localized spin density and particle density wavepackets which should propagate at different velocities. Supported by AFOSR and NSF.
Generation of localized magnetic moments in the charge-density-wave state
Akzyanov, Ramil S.; Rozhkov, Alexander V.
2015-08-01
We propose a mechanism explaining the generation of localized magnetic moments in charge-density-wave compounds. Our model Hamiltonian describes an Anderson impurity placed in a host material exhibiting the charge-density wave. There is a region of the model's parameter space, where even weak Coulomb repulsion on the impurity site is able to localize the magnetic moment on the impurity. The phase diagram of a single impurity at T = 0 is mapped. To establish the connection with experiment, the thermodynamic properties of a random impurity ensemble is studied. Magnetic susceptibility of the ensemble diverges at low temperature; heat capacity as a function of the magnetic field demonstrates pronounced low field peak. Both features are consistent with experiments on orthorhombic TaS3 and blue bronze.
Universal Field-Induced Charge-Density-Wave Phase Diagram: Theory versus Experiment
Lebed, A. G.
2009-07-01
We suggest a theory of field-induced charge-density-wave phases, generated by high magnetic fields in quasi-low-dimensional conductors. We demonstrate that, in layered quasi-one-dimensional conductors, the corresponding critical magnetic field ratios are universal and do not depend on any fitting parameter. In particular, we find that H1/H0=0.73, H2/H0=0.59, H3/H0=0.49, and H4/H0=0.42, where Hn is a critical field of a phase transition between the field-induced charge-density-wave phases with numbers n and n+1. The suggested theory is in very good qualitative and quantitative agreement with the existing experimental data in α-(ET)2KHg(SCN)4 material.
Charge density waves in the graphene sheets of the superconductor CaC(6).
Rahnejat, K C; Howard, C A; Shuttleworth, N E; Schofield, S R; Iwaya, K; Hirjibehedin, C F; Renner, Ch; Aeppli, G; Ellerby, M
2011-11-29
Graphitic systems have an electronic structure that can be readily manipulated through electrostatic or chemical doping, resulting in a rich variety of electronic ground states. Here we report the first observation and characterization of electronic stripes in the highly electron-doped graphitic superconductor, CaC(6), by scanning tunnelling microscopy and spectroscopy. The stripes correspond to a charge density wave with a period three times that of the Ca superlattice. Although the positions of the Ca intercalants are modulated, no displacements of the carbon lattice are detected, indicating that the graphene sheets host the ideal charge density wave. This provides an exceptionally simple material-graphene-as a starting point for understanding the relation between stripes and superconductivity. Furthermore, our experiments suggest a strategy to search for superconductivity in graphene, namely in the vicinity of striped 'Wigner crystal' phases, where some of the electrons crystallize to form a superlattice.
Field-Induced Dynamic Diamagnetism in a Charge-Density-Wave System
Harrison, N.; Mielke, C. H.; Christianson, A. D.; Brooks, J. S.; Tokumoto, M.
2001-02-01
ac susceptibility measurements of the charge-density-wave (CDW) compound α-\\(BEDT-TTF\\)2-KHg\\(SCN\\)4 at magnetic fields, μ0H>23 T, above its Pauli paramagnetic limit, reveal unambiguously that the magnetic hysteresis observed previously within this CDW phase is diamagnetic and can only be explained by induced currents. It is argued that the ensemble of experimental techniques amounts to a strong case for dissipationless conductivity within this phase.
Time-domain pumping a quantum-critical charge density wave ordered material
Matveev, O. P.; Shvaika, A. M.; Devereaux, T. P.; Freericks, J. K.
2016-09-01
We determine the exact time-resolved photoemission spectroscopy for a nesting driven charge density wave (described by the spinless Falicov-Kimball model within dynamical mean-field theory). The pump-probe experiment involves two light pulses: the first is an ultrashort intense pump pulse that excites the system into nonequilibrium, and the second is a lower amplitude, higher frequency probe pulse that photoexcites electrons. We examine three different cases: the strongly correlated metal, the quantum-critical charge density wave, and the critical Mott insulator. Our results show that the quantum critical charge density wave has an ultraefficient relaxation channel that allows electrons to be de-excited during the pump pulse, resulting in little net excitation. In contrast, the metal and the Mott insulator show excitations that are closer to what one expects from these systems. In addition, the pump field produces spectral band narrowing, peak sharpening, and a spectral gap reduction, all of which rapidly return to their field free values after the pump is over.
Magnetic field dependence of the threshold electric field in unconventional charge density waves
Dóra, Balázs; Virosztek, Attila; Maki, Kazumi
2002-04-01
Many experiments suggest that the unidentified low-temperature phase of α-(BEDT-TTF)2KHg(SCN)4 is most likely unconventional charge density wave (UCDW). To further extend this identification we present our theoretical study of the threshold electric field of UCDW in a magnetic field. The magnetic field-temperature phase diagram is very similar to those in a d-wave superconductor. The optical conductivity shows clear features characteristic to both UDW and magnetic field. We find a rather strong field dependence of the threshold electric field, which shows qualitatively good agreement with the experimental data.
Extended phonon collapse in the charge-density-wave compound NbSe{sub 2}
Energy Technology Data Exchange (ETDEWEB)
Weber, Frank [Karlsruhe Institute of Technology, Institute of Solid State Physics, Karlsruhe (Germany); Materials Science Division, Argonne National Laboratory, Argonne, Illinois (United States); Rosenkranz, Stephan; Castellan, John-Paul; Osborn, Raymond [Materials Science Division, Argonne National Laboratory, Argonne, Illinois (United States); Hott, Roland; Heid, Rolf; Bohnen, Klaus-Peter [Karlsruhe Institute of Technology, Institute of Solid State Physics, Karlsruhe (Germany); Egami, Takeshi [Department of Materials Science and Engineering, University of Tennessee, Knoxville, Tennessee (United States); Said, Ayman [Advanced Photon Source, Argonne National Laboratory, Illinois (United States); Reznik, Dmitry [Karlsruhe Institute of Technology, Institute of Solid State Physics, Karlsruhe (Germany); Department of Physics, University of Colorado at Boulder, Boulder, Colorado (United States)
2011-07-01
We investigated the phonon softening in the charge density wave compound NbSe{sub 2} using the high-resolution hard inelastic X-ray scattering beamline 30-ID-C at the Advanced Photon Source, Argonne National Laboratory. The acoustic {sigma}{sub 1} phonon branch was measured from the zone center {gamma} to the M point at temperatures between 250 K and 8 K across the CDW transition at T{sub CDW}=33 K. Density functional theory calculations for the lattice dynamical properties which predict an extended phonon breakdown are used to analyze the detailed nature of the softening phonon branch.
Observation of a Charge Density Wave Incommensuration Near the Superconducting Dome in Cux TiSe2
Kogar, A.; de la Pena, G. A.; Lee, Sangjun; Fang, Y.; Sun, S. X.-L.; Lioi, D. B.; Karapetrov, G.; Finkelstein, K. D.; Ruff, J. P. C.; Abbamonte, P.; Rosenkranz, S.
2017-01-01
X-ray diffraction was employed to study the evolution of the charge density wave (CDW) in Cux TiSe2 as a function of copper intercalation in order to clarify the relationship between the CDW and superconductivity. The results show a CDW incommensuration arising at an intercalation value coincident with the onset of superconductivity at around x =0.055 (5 ) . Additionally, it was found that the charge density wave persists to higher intercalant concentrations than previously assumed, demonstrating that the CDW does not terminate inside the superconducting dome. A charge density wave peak was observed in samples up to x =0.091 (6 ), the highest copper concentration examined in this study. The phase diagram established in this work suggests that charge density wave incommensuration may play a role in the formation of the superconducting state.
Long-range charge-density-wave proximity effect at cuprate/manganate interfaces
Frano, A.; Blanco-Canosa, S.; Schierle, E.; Lu, Y.; Wu, M.; Bluschke, M.; Minola, M.; Christiani, G.; Habermeier, H. U.; Logvenov, G.; Wang, Y.; van Aken, P. A.; Benckiser, E.; Weschke, E.; Le Tacon, M.; Keimer, B.
2016-08-01
The interplay between charge density waves (CDWs) and high-temperature superconductivity is currently under intense investigation. Experimental research on this issue is difficult because CDW formation in bulk copper oxides is strongly influenced by random disorder, and a long-range-ordered CDW state in high magnetic fields is difficult to access with spectroscopic and diffraction probes. Here we use resonant X-ray scattering in zero magnetic field to show that interfaces with the metallic ferromagnet La2/3Ca1/3MnO3 greatly enhance CDW formation in the optimally doped high-temperature superconductor YBa2Cu3O6+δ (δ ~ 1), and that this effect persists over several tens of nanometres. The wavevector of the incommensurate CDW serves as an internal calibration standard of the charge carrier concentration, which allows us to rule out any significant influence of oxygen non-stoichiometry, and to attribute the observed phenomenon to a genuine electronic proximity effect. Long-range proximity effects induced by heterointerfaces thus offer a powerful method to stabilize the charge-density-wave state in the cuprates and, more generally, to manipulate the interplay between different collective phenomena in metal oxides.
Long-range charge-density-wave proximity effect at cuprate/manganate interfaces.
Frano, A; Blanco-Canosa, S; Schierle, E; Lu, Y; Wu, M; Bluschke, M; Minola, M; Christiani, G; Habermeier, H U; Logvenov, G; Wang, Y; van Aken, P A; Benckiser, E; Weschke, E; Le Tacon, M; Keimer, B
2016-08-01
The interplay between charge density waves (CDWs) and high-temperature superconductivity is currently under intense investigation. Experimental research on this issue is difficult because CDW formation in bulk copper oxides is strongly influenced by random disorder, and a long-range-ordered CDW state in high magnetic fields is difficult to access with spectroscopic and diffraction probes. Here we use resonant X-ray scattering in zero magnetic field to show that interfaces with the metallic ferromagnet La2/3Ca1/3MnO3 greatly enhance CDW formation in the optimally doped high-temperature superconductor YBa2Cu3O6+δ (δ ∼ 1), and that this effect persists over several tens of nanometres. The wavevector of the incommensurate CDW serves as an internal calibration standard of the charge carrier concentration, which allows us to rule out any significant influence of oxygen non-stoichiometry, and to attribute the observed phenomenon to a genuine electronic proximity effect. Long-range proximity effects induced by heterointerfaces thus offer a powerful method to stabilize the charge-density-wave state in the cuprates and, more generally, to manipulate the interplay between different collective phenomena in metal oxides.
Metal-charge density wave coexistence in TTF[Ni(dmit){sub 2}]{sub 2}
Energy Technology Data Exchange (ETDEWEB)
Kaddour, W. [Laboratoire de Physique des Solides, UMR 8502-CNRS, Univ. Paris-Sud, Orsay F-91405 (France); Laboratoire de Physique de la Matière Condensée, Campus Universitaire, Université de Tunis El-Manar, Tunis 2092 (Tunisia); Auban-Senzier, P.; Raffy, H.; Monteverde, M.; Pouget, J.-P. [Laboratoire de Physique des Solides, UMR 8502-CNRS, Univ. Paris-Sud, Orsay F-91405 (France); Pasquier, C.R., E-mail: pasquier@lps.u-psud.fr [Laboratoire de Physique des Solides, UMR 8502-CNRS, Univ. Paris-Sud, Orsay F-91405 (France); Alemany, P. [Departament de Química Física and Institut de Química Teòrica i Computacional (IQTCUB), Universitat de Barcelona, Martí i Franquès 1, 08028 Barcelona (Spain); Canadell, E. [Institut de Ciència de Materials de Barcelona (CSIC), Campus UAB, 08193 Bellaterra (Spain); Valade, L. [Laboratoire de Chimie de Coordination, Route de Narbonne F-31077 Toulouse (France)
2015-03-01
We have established a new pressure–temperature phase diagram of TTF[Ni(dmit){sub 2}]{sub 2} based on longitudinal and transverse resistivity measurements under pressure up to 30 kbar. We were able to identify three different charge density wave (CDW) states which all coexist with a metallic state in a wide temperature range and superconductivity at the lowest temperatures. At low pressure, two successive CDW transitions have been clearly identified. These two transitions merge into a single one at 12 kbar. A maximum of this unique CDW transition temperature is observed at 19 kbar.
Pressure Dependence of the Charge-Density-Wave Gap in Rare-Earth Tri-Tellurides
Energy Technology Data Exchange (ETDEWEB)
Sacchetti, A.; /Zurich, ETH; Arcangeletti, E.; Perucchi, A.; Baldassarre, L.; Postorino, P.; Lupi, S.; /Rome U.; Ru, N.; Fisher, I.R.; /Stanford U., Geballe Lab.; Degiorgi, L.; /Zurich, ETH
2009-12-14
We investigate the pressure dependence of the optical properties of CeTe{sub 3}, which exhibits an incommensurate charge-density-wave (CDW) state already at 300 K. Our data are collected in the mid-infrared spectral range at room temperature and at pressures between 0 and 9 GPa. The energy for the single particle excitation across the CDW gap decreases upon increasing the applied pressure, similarly to the chemical pressure by rare-earth substitution. The broadening of the bands upon lattice compression removes the perfect nesting condition of the Fermi surface and therefore diminishes the impact of the CDW transition on the electronic properties of RTe{sub 3}.
Optical properties of the Ce and La ditelluride charge density wave compounds
Energy Technology Data Exchange (ETDEWEB)
Lavagnini, M.; Sacchetti, A.; Degiorgi, L.; /Zurich, ETH; Shin, K.Y.; Fisher, I.R.; /Stanford U., Geballe Lab. /Stanford U., Appl. Phys. Dept.
2010-02-15
The La and Ce di-tellurides LaTe{sub 2} and CeTe{sub 2} are deep in the charge-density-wave (CDW) ground state even at 300 K. We have collected their electrodynamic response over a broad spectral range from the far infrared up to the ultraviolet. We establish the energy scale of the single particle excitation across the CDW gap. Moreover, we find that the CDW collective state gaps a very large portion of the Fermi surface. Similarly to the related rare earth tri-tellurides, we envisage that interactions and Umklapp processes play a role in the onset of the CDW broken symmetry ground state.
Origin of the charge density wave in 1T-TiSe2
Zhu, Zhiyong
2012-06-27
All-electron ab initio calculations are used to study the microscopic origin of the charge density wave (CDW) in 1T-TiSe2. A purely electronic picture is ruled out as a possible scenario, indicating that the CDW transition in the present system is merely a structural phase transition. The CDW instability is the result of a symmetry lowering by electron correlations occurring with electron localization. Suppression of the CDW in pressurized and in Cu-intercalated 1T-TiSe2 is explained by a delocalization of the electrons, which weakens the correlations and counteracts the symmetry lowering.
Near Gap Excitation of Collective Modes in a Charge Density Wave
Leuenberger, Dominik; Sobota, Jonathan; Yang, Shuolong; Kemper, Alexander; Giraldo, Paula; Moore, Rob; Fisher, Ian; Kirchmann, Patrick; Devereaux, Thomas; Shen, Zhi-Xun
2015-03-01
We present time- and angle-resolved photoemission spectroscopy (trARPES) measurements on the charge density wave system's (CDW) CeTe3. Optical excitation transiently populates the unoccupied band structure and reveals a CDW gap size of 2 Δ = 0 . 59 eV. In addition, the occupied Te- 5 p band dispersion is coherently modified by three collective modes. First, the spatial polarization of the modes is analyzed by fits of a transient model dispersion and DFT frozen phonon calculations. We thereby demonstrate how the rich information from trARPES allows identification of collective modes and their spatial polarization, which explains the mode-dependent coupling to charge order. Second, the exciting photon energy hν was gradually lowered towards 2 Δ , at constant optical excitation density. The coherent response of the amplitude mode deviates from the optical conductivity, which is dominated by direct interband transitions between the lower and upper CDW bands. The measured hν -dependence can be reproduced by a calculated joint density of states for optical transition between bands with different orbital character. This finding suggests, that the coherent response of the CDW amplitude mode is dominated by photo-doping of the charge ordering located in the Te-planes.
Superconductivity in the charge-density-wave state of the organic metal α- (BEDT-TTF)2 KHg (SCN)4
Andres, D.; Kartsovnik, M. V.; Biberacher, W.; Neumaier, K.; Schuberth, E.; Müller, H.
2005-11-01
The superconducting transition in the layered organic compound α-(BEDT-TTF)2KHg(SCN)4 has been studied in the two hydrostatic pressure regimes where a charge-density wave is either present or completely suppressed. Within the charge-density-wave state the experimental results reveal a network of weakly coupled superconducting regions. This is especially seen in a strong enhancement of the measured critical field and the corresponding positive curvature of its temperature dependence. Further, it is shown that on lowering the pressure into the density-wave state traces of a superconducting phase already start to appear at a much higher temperature.
Multiple charge density wave states at the surface of TbT e3
Fu, Ling; Kraft, Aaron M.; Sharma, Bishnu; Singh, Manoj; Walmsley, Philip; Fisher, Ian R.; Boyer, Michael C.
2016-11-01
We studied TbT e3 using scanning tunneling microscopy (STM) in the temperature range of 298-355 K. Our measurements detect a unidirectional charge density wave (CDW) state in the surface Te layer with a wave vector consistent with that of the bulk qCDW=0.30 ±0.01 c* . However, unlike previous STM measurements, and differing from measurements probing the bulk, we detect two perpendicular orientations for the unidirectional CDW with no directional preference for the in-plane crystal axes (a or c axis) and no noticeable difference in wave vector magnitude. In addition, we find regions in which the bidirectional CDW states coexist. We propose that observation of two unidirectional CDW states indicates a decoupling of the surface Te layer from the rare-earth block layer below, and that strain variations in the Te surface layer drive the local CDW direction to the specific unidirectional or, in rare occurrences, bidirectional CDW orders observed. This indicates that similar driving mechanisms for CDW formation in the bulk, where anisotropic lattice strain energy is important, are at play at the surface. Furthermore, the wave vectors for the bidirectional order we observe differ from those theoretically predicted for checkerboard order competing with stripe order in a Fermi-surface nesting scenario, suggesting that factors beyond Fermi-surface nesting drive CDW order in TbT e3 . Finally, our temperature-dependent measurements provide evidence for localized CDW formation above the bulk transition temperature TCDW.
Mean field theory of charge-density wave state in magnetic field
Grigoriev, Pavel; Lyubshin, Dmitrij
2005-03-01
We develop a mean field theory of charge-density wave (CDW) state in magnetic field and study properties of this state below the transition temperature. We show that the CDW state with shifted wave vector in high magnetic field (CDWx phase) has a double harmonic modulation on the most part of the phase diagram. At perfect nesting the single harmonic CDW state with shifted wave vector exists only in a very narrow region near the triple point. We show that the transition from CDW0 to CDWx state below the critical temperature is accompanied by a jump of the CDW order parameter and of the CDW wave vector rather than by their continuous increase. This implies a first order transition between these CDW states and explains a strong hysteresis accompanying this transition. The similarities between CDW in high magnetic field and nonuniform LOFF superconducting phase are pointed out. Our investigation provides a theoretical description for recent experiments on organic metal α-(BEDT-TTF)2KHg(SCN)4 and other compounds. In particular, we explain the higher value of the kink transition field and provide the calculation of the phase diagram in the case of perfect nesting.
The amplitudes and the structure of the charge density wave in YBCO
Kharkov, Y. A.; Sushkov, O. P.
2016-10-01
We find unknown s- and d-wave amplitudes of the recently discovered charge density wave (CDW) in underdoped cuprates. To do so we perform a combined analysis of experimental data for ortho-II YBa2Cu3Oy. The analysis includes data on nuclear magnetic resonance, resonant inelastic X-ray scattering, and hard X-ray diffraction. The amplitude of doping modulation found in our analysis is 3.5 · 10‑3 in a low magnetic field and T = 60 K, the amplitude is 6.5 · 10‑3 in a magnetic field of 30T and T = 1.3 K. The values are in units of elementary charge per unit cell of a CuO2 plane. We show that the data rule out a checkerboard pattern, and we also show that the data might rule out mechanisms of the CDW which do not include phonons.
Sun, Xu; Yao, Tao; Hu, Zhenpeng; Guo, Yuqiao; Liu, Qinghua; Wei, Shiqiang; Wu, Changzheng
2015-05-28
A deep understanding of the relationship between electronic and structure ordering across the charge-density-wave (CDW) transition is crucial for both fundamental study and technological applications. Herein, using in situ X-ray absorption fine structure (XAFS) spectroscopy coupled with high-resolution transmission electron microscopy (HRTEM), we have illustrated the atomic-level information on the local structural evolution across the CDW transition and its influence on the intrinsic electrical properties in VS2 system. The structure transformation, which is highlighted by the formation of vanadium trimers with derivation of V-V bond length (ΔR = 0.10 Å), was clearly observed across the CDW process. Moreover, the corresponding influence of lattice variation on the electronic behavior was clearly characterized by experimental results as well as theoretical analysis, which demonstrated that vanadium trimers drive the deformation of space charge density distribution into √3 ×√3 periodicity, with the conductivity of a1g band reducing by half. These observations directly unveiled the close connection between lattice evolution and electronic property variation, paving a new avenue for understanding the intrinsic nature of electron-lattice interactions in the VS2 system and other isostructural transition metal dichalcogenides across the CDW transition process.
Superconductivity and Charge Density Wave in ZrTe3-xSex.
Zhu, Xiangde; Ning, Wei; Li, Lijun; Ling, Langsheng; Zhang, Ranran; Zhang, Jinglei; Wang, Kefeng; Liu, Yu; Pi, Li; Ma, Yongchang; Du, Haifeng; Tian, Minglian; Sun, Yuping; Petrovic, Cedomir; Zhang, Yuheng
2016-06-02
Charge density wave (CDW), the periodic modulation of the electronic charge density, will open a gap on the Fermi surface that commonly leads to decreased or vanishing conductivity. On the other hand superconductivity, a commonly believed competing order, features a Fermi surface gap that results in infinite conductivity. Here we report that superconductivity emerges upon Se doping in CDW conductor ZrTe3 when the long range CDW order is gradually suppressed. Superconducting critical temperature Tc(x) in ZrTe3-xSex (0 ≤ x ≤ 0.1) increases up to 4 K plateau for 0.04 ≤ x ≤ 0.07. Further increase in Se content results in diminishing Tc and filametary superconductivity. The CDW modes from Raman spectra are observed in x = 0.04 and 0.1 crystals, where signature of ZrTe3 CDW order in resistivity vanishes. The electronic-scattering for high Tc crystals is dominated by local CDW fluctuations at high temperatures, the resistivity is linear up to highest measured T = 300 K and contributes to substantial in-plane anisotropy.
Possibility of charge density wave transition in a SrPt2Sb2 superconductor.
Ibuka, Soshi; Imai, Motoharu
2016-04-27
The first-order transition at T(0) = 270 K for the platinum-based SrPt2Sb2 superconductor was investigated using x-ray diffraction and magnetic susceptibility measurements. When polycrystalline SrPt2Sb2 was cooled down through T(0), the structure was transformed from monoclinic to a modulated orthorhombic structure, and no magnetic order was formed, which illustrates the possibility of a charge density wave (CDW) transition at T(0). SrPt2Sb2 can thus be a new example to examine the interplay of CDW and superconductivity in addition to SrPt2As2, BaPt2As2, and LaPt2Si2. It is unique that the average structure of the low-temperature phase has higher symmetry than that of the high-temperature phase.
Non-thermal separation of electronic and structural orders in a persisting charge density wave
Porer, M; Ménard, J -M; Dachraoui, H; Mouchliadis, L; Perakis, I E; Heinzmann, U; Demsar, J; Rossnagel, K; Huber, R
2016-01-01
The simultaneous ordering of different degrees of freedom in complex materials undergoing spontaneous symmetry-breaking transitions often involves intricate couplings that have remained elusive in phenomena as wide ranging as stripe formation, unconventional superconductivity or colossal magnetoresistance. Ultrafast optical, x-ray and electron pulses can elucidate the microscopic interplay between these orders by probing the electronic and lattice dynamics separately, but a simultaneous direct observation of multiple orders on the femtosecond scale has been challenging. Here we show that ultrabroadband terahertz pulses can simultaneously trace the ultrafast evolution of coexisting lattice and electronic orders. For the example of a charge-density-wave (CDW) in 1T-TiSe2, we demonstrate that two components of the CDW order parameter - excitonic correlations and a periodic lattice distortion (PLD) - respond very differently to 12-fs optical excitation. Even when the excitonic order of the CDW is quenched, the PL...
Thermodynamic and critical properties of the charge density wave system ErTe3
Saint-Paul, M.; Remenyi, G.; Guttin, C.; Lejay, P.; Monceau, P.
2017-01-01
We present specific heat and ultrasonic measurements on the rare earth tritelluride ErTe3 compound. Thermodynamic anomalies are observed at the upper charge density wave (CDW) phase transition TCDW1=265 K and the second one at TCDW2=155 K. Similar critical behaviors are found at both CDW phase transitions and that we tentatively described in terms of the 3D XY model. Different anisotropic stress dependences ∂TCDW1 / ∂σii and ∂TCDW2 / ∂σii are found at the two successive CDW phase transitions. Magnitude of the elastic constant anomalies at TCDW2 is ten times smaller than that at TCDW1. Anomalies in the elastic constants at the upper CDW TCDW1 exhibit two dimensional features in the layer planes while in contrast a three dimensional behavior is observed at TCDW2.
Finite-size effects in quasi-one-dimensional conductors with a charge-density wave
Energy Technology Data Exchange (ETDEWEB)
Zaitsev-Zotov, Sergei V [Institute of Radio Engineering and Electronics, Russian Academy of Sciences, Moscow (Russian Federation)
2004-06-30
Recent studies of finite-size effects in charge-density wave conductors are reviewed. Various manifestations of finite-size effects, including the transverse-size dependence of the nonlinear-conduction threshold field, the Peierls transition temperature, high-frequency conduction, and the relaxation rates of metastable states, are discussed. Resistivity jumps in thin samples, the smeared threshold field for nonlinear conduction, and threshold conduction above the Peierls transition temperature are considered, as are mesoscopic oscillations of the threshold field, one-dimensional conduction in thin crystals, absolute negative conductivity of quasi-one-dimensional conductors, the length dependence of the phase-slip voltage, and the Aharonov-Bohm oscillations in sliding CDWs. Problems yet to be solved are discussed. (reviews of topical problems)
Fermi Surface Evolution Across Multiple Charge Density Wave Transitions in ErTe3
Energy Technology Data Exchange (ETDEWEB)
Moore, R.G.; /SLAC, SSRL /Stanford U., Geballe Lab.; Brouet, V.; /Orsay, LPS; He, R.; /SLAC, SSRL /Stanford U., Geballe Lab.; Lu, D.H.; /SLAC, SSRL; Ru, N.; Chu, J.-H.; Fisher, I.R.; /Stanford U., Geballe Lab.; Shen, Z.-X.; /SLAC, SSRL /Stanford U., Geballe Lab.
2010-02-15
The Fermi surface (FS) of ErTe{sub 3} is investigated using angle-resolved photoemission spectroscopy (ARPES). Low temperature measurements reveal two incommensurate charge density wave (CDW) gaps created by perpendicular FS nesting vectors. A large {Delta}{sub 1} = 175 meV gap arising from a CDW with c* - q{sub CDW1} {approx} 0.70(0)c* is in good agreement with the expected value. A second, smaller {Delta}{sub 2} = 50 meV gap is due to a second CDW with a* - q{sub CDW2} {approx} 0.68(5)a*. The temperature dependence of the FS, the two gaps and possible interaction between the CDWs are examined.
Strain Tuning of the Charge Density Wave in Monolayer and Bilayer 1T-TaS2
Gan, Liyong
2015-12-07
By first-principles calculations, we investigate the strain effects on the charge density wave states of monolayer and bilayer 1T-TaS2. The modified stability of the charge density wave in the monolayer is understood in terms of the strain dependent electron localization, which determines the distortion amplitude. On the other hand, in the bilayer the effect of strain on the interlayer interaction is also crucial. The rich phase diagram under strain opens new venues for applications of 1T-TaS2. We interpret the experimentally observed insulating state of bulk 1T-TaS2 as inherited from the monolayer by effective interlayer decoupling.
Phase transitions to dipolar clusters and charge density waves in high Tc superconductors
Saarela, M.; Kusmartsev, F. V.
2017-02-01
We show that doping of hole charge carriers leads to formation of electric dipolar clusters in cuprates. They are created by many-body interactions between the dopant ion outside and holes inside the CuO planes. Because of the two-fold degeneracy holes in the CuO plane cluster into four-particles resonance valence bond plaquettes bound with dopant ions. Such dipoles may order into charge-density waves (CDW) or stripes or form a disordered state depending on doping and temperature. The lowest energy of the ordered system corresponds to a local anti-ferroelectric ordering. The mobility of individual disordered dipoles is very low at low temperatures and they prefer first to bind into dipole-dipole pairs. Electromagnetic radiation interacts strongly with electric dipoles and when the sample is subjected to it the mobility changes significantly. This leads to a fractal growth of dipolar clusters. The existence of electric dipoles and CDW induce two phase transitions with increasing temperature, melting of the ordered state and disappearance of the dipolar state. Ferroelectricity at low doping is a natural consequence of such dipole moments. We develop a theory based on two-level systems and dipole-dipole interaction to explain the behavior of the polarization as a function of temperature and electric field.
Poccia, Nicola; Ricci, Alessandro; Campi, Gaetano; Bianconi, Antonio
2017-03-01
Multiple functional ionic and electronic orders are observed in high temperature superconducting cuprates. The charge density wave order is one of them and it is spatially localized in different regions of the material. It is also known that the oxygen interstitials introduced by chemical intercalation self-organize in different oxygen rich regions corresponding with hole rich regions in the CuO2 layers left empty by the charge density wave order domains. However, what happens in between these two orders is not known, and neither there is a method to control this spatial separation. Here we demonstrate by using scanning nano x-ray diffraction, that dislocations or grain boundaries in the material can act as boundary between charge density wave and oxygen rich phases in a optimally doped {{La}}2{{CuO}}4+y high temperature superconductor. Dislocations can be used therefore to control the anti-correlation of the charge density wave order with the oxygen interstitials in specific portion of the material.
VANSMAALEN, S; DEBOER, JL; COPPENS, P
1993-01-01
Synchrotron radiation X-ray diffraction has been performed on niobium triselenide at 20K. The modulation parameters belonging to both Charge-Density-Waves (CDW's) have been determined. The high-temperature CDW is found to comprise of displacements on all atoms of column III, as well as on Se atoms o
Struzhkin, Viktor V.; Chen, Xiao-Jia
2016-10-01
The mechanism of high-temperature superconductivity of copper oxides (cuprates) remains unsolved puzzle in condensed matter physics. The cuprates represent extremely complicated system, showing fascinating variety of quantum phenomena and rich phase diagram as a function of doping. In the suggested "superconducting glue" mechanisms, phonon and spin excitations are invoked most frequently, and it appears that only spin excitations cover the energy scale required to justify very high transition temperature Tc ˜ 165 K (as in mercury-based triple layer cuprates compressed to 30 GPa). It appears that pressure is quite important variable helping to boost the Tc record by almost 30°. Pressure may be also considered as a clean tuning parameter, helping to understand the underlying balance of various energy scales and ordered states in cuprates. In this paper, a review of mostly our work on cuprates under pressure will be given, with the emphasis on the interactions between phonon and spin excitations. It appears that there is a strong coupling between superexchange interaction and stretching in-plane oxygen vibrations, which may give rise to a variety of complex phenomena, including the charge-density wave state intertwined with superconductivity and attracting a lot of interest recently.
Resonant Enhancement of Charge Density Wave Diffraction in the Rare-Earth Tri-Tellurides
Energy Technology Data Exchange (ETDEWEB)
Lee, W.S.; Sorini, A.P.; Yi, M.; Chuang, Y.D.; Moritz, B.; Yang, W.L.; Chu, J.-H.; Kuo, H.H.; Gonzalez, A.G.Cruz; Fisher, I.R.; Hussain, Z.; Devereau, T.P.; Shen, Z.X.
2012-05-15
We performed resonant soft X-ray diffraction on known charge density wave (CDW) compounds, rare earth tri-tellurides. Near the M{sub 5} (3d - 4f) absorption edge of rare earth ions, an intense diffraction peak is detected at a wavevector identical to that of CDW state hosted on Te{sub 2} planes, indicating a CDW-induced modulation on the rare earth ions. Surprisingly, the temperature dependence of the diffraction peak intensity demonstrates an exponential increase at low temperatures, vastly different than that of the CDW order parameter. Assuming 4f multiplet splitting due to the CDW states, we present a model to calculate X-ray absorption spectrum and resonant profile of the diffraction peak, agreeing well with experimental observations. Our results demonstrate a situation where the temperature dependence of resonant X-ray diffraction peak intensity is not directly related to the intrinsic behavior of the order parameter associated with the electronic order, but is dominated by the thermal occupancy of the valence states.
Magnetic field controlled charge density wave coupling in underdoped YBa2Cu3O6+x
Chang, J.; Blackburn, E.; Ivashko, O.; Holmes, A. T.; Christensen, N. B.; Hücker, M.; Liang, Ruixing; Bonn, D. A.; Hardy, W. N.; Rütt, U.; Zimmermann, M. V.; Forgan, E. M.; Hayden, S. M.
2016-05-01
The application of magnetic fields to layered cuprates suppresses their high-temperature superconducting behaviour and reveals competing ground states. In widely studied underdoped YBa2Cu3O6+x (YBCO), the microscopic nature of field-induced electronic and structural changes at low temperatures remains unclear. Here we report an X-ray study of the high-field charge density wave (CDW) in YBCO. For hole dopings ~0.123, we find that a field (B~10 T) induces additional CDW correlations along the CuO chain (b-direction) only, leading to a three-dimensional (3D) ordered state along this direction at B~15 T. The CDW signal along the a-direction is also enhanced by field, but does not develop an additional pattern of correlations. Magnetic field modifies the coupling between the CuO2 bilayers in the YBCO structure, and causes the sudden appearance of the 3D CDW order. The mirror symmetry of individual bilayers is broken by the CDW at low and high fields, allowing Fermi surface reconstruction, as recently suggested.
Ideal charge-density-wave order in the high-field state of superconducting YBCO
Jang, H.; Lee, W.-S.; Nojiri, H.; Matsuzawa, S.; Yasumura, H.; Nie, L.; Maharaj, A. V.; Gerber, S.; Liu, Y.-J.; Mehta, A.; Bonn, D. A.; Liang, R.; Hardy, W. N.; Burns, C. A.; Islam, Z.; Song, S.; Hastings, J.; Devereaux, T. P.; Shen, Z.-X.; Kivelson, S. A.; Kao, C.-C.; Zhu, D.; Lee, J.-S.
2016-12-01
The existence of charge-density-wave (CDW) correlations in cuprate superconductors has now been established. However, the nature of the CDW ground state has remained uncertain because disorder and the presence of superconductivity typically limit the CDW correlation lengths to only a dozen unit cells or less. Here we explore the field-induced 3D CDW correlations in extremely pure detwinned crystals of YBa2Cu3O2 (YBCO) ortho-II and ortho-VIII at magnetic fields in excess of the resistive upper critical field (Hc2Hc2) where superconductivity is heavily suppressed. We observe that the 3D CDW is unidirectional and possesses a long in-plane correlation length as well as significant correlations between neighboring CuO2 planes. It is significant that we observe only a single sharply defined transition at a critical field proportional to Hc2Hc2, given that the field range used in this investigation overlaps with other high-field experiments including quantum oscillation measurements. The correlation volume is at least two to three orders of magnitude larger than that of the zero-field CDW. This is by far the largest CDW correlation volume observed in any cuprate crystal and so is presumably representative of the high-field ground state of an “ideal” disorder-free cuprate.
First-principles studies on the charge density wave in uranium
Qiu, Ruizhi; Lu, Haiyan; Ao, Bingyun; Tang, Tao; Chen, Piheng
2016-06-01
The charge density wave (CDW) state of α-U (called {α1} -U) was studied through a first-principles total-energy minimization using the conjugate gradient algorithm. The optimized crystal structure of {α1} -U was found to have the space group Pbnm, which was proposed in the earlier Landau-type theory and is isostructural with the α-Np structure. In particular, the changes in the lattice parameters of Pbnm-U with respect to α-U are consistent with the experimental observations. In addition, the energetic stability of Pbnm-U with respect to α-U was confirmed by enthalpy calculations, and the value of the critical pressure in the pressure-induced quantum transition from Pbnm-U to α-U is in good agreement with the experimental result. Moreover, the phonon calculation verified the dynamical instability of α-U and the stability of Pbnm-U. Finally, the calculated electronic structures exhibit features of the CDW state.
Novel charge density wave transition in crystals of R5Ir4Si10
Indian Academy of Sciences (India)
S Ramakrishnan
2002-05-01
We review the observation of novel charge density wave (CDW) transitions in ternary R5Ir4Si10 compounds. A high quality single crystal of Lu5Ir4Si10 shows the formation of a commensurate CDW along -axis below 80 K in the (ℎ, 0, ) plane that coexists with BCS type superconductivity below 3.9 K. However, in a single crystal of Er5Ir4Si10, one observes the development of a 1D-incommensurate CDW at 155 K, which then locks into a purely commensurate state below 55 K. The well-localized Er3 moments are antiferromagnetically ordered below 2.8 K which results in the coexistence of strongly coupled CDW with local moment antiferromagnetism in Er5Ir4Si10. Unlike conventional CDW systems, extremely sharp transition (width ∼ 1.5 K) in all bulk properties along with huge heat capacity anomalies in these compounds makes this CDW transition an interesting one.
Multiple charge density wave transitions in the antiferromagnets R NiC2 (R =Gd ,Tb)
Shimomura, S.; Hayashi, C.; Hanasaki, N.; Ohnuma, K.; Kobayashi, Y.; Nakao, H.; Mizumaki, M.; Onodera, H.
2016-04-01
X-ray scattering and electrical resistivity measurements were performed on GdNiC2 and TbNiC2. We found a set of satellite peaks characterized by q1=(0.5 ,η ,0 ) below T1, at which the resistivity shows a sharp inflection, suggesting the charge density wave (CDW) formation. The value of η decreases with decreasing temperature below T1, and then a transition to a commensurate phase with q1 C=(0.5 ,0.5 ,0 ) takes place. The diffuse scattering observed above T1 indicates the presence of soft phonon modes associated with CDW instabilities at q1 and q2=(0.5 ,0.5 ,0.5 ) . The long-range order given by q2 is developed in addition to that given by q1 C in TbNiC2, while the short-range correlation with q2 persists even at 6 K in GdNiC2. The amplitude of the q1 C lattice modulation is anomalously reduced below an antiferromagnetic transition temperature TN in GdNiC2. In contrast, the q2 order vanishes below TN in TbNiC2. We demonstrate that R NiC2 (R = rare earth) compounds exhibit similarities with respect to their CDW phenomena, and discuss the effects of magnetic transitions on CDWs. We offer a possible displacement pattern of the modulated structure characterized by q1 C and q2 in terms of frustration.
Spin polarization driven by a charge-density wave in monolayer 1T−TaS2
Zhang, Qingyun
2014-08-06
Using first-principles calculations, we investigate the electronic and vibrational properties of monolayer T-phase TaS2. We demonstrate that a charge-density wave is energetically favorable at low temperature, similar to bulk 1T-TaS2. Electron-phonon coupling is found to be essential for the lattice reconstruction. The charge-density wave results in a strong localization of the electronic states near the Fermi level and consequently in spin polarization, transforming the material into a magnetic semiconductor with enhanced electronic correlations. The combination of inherent spin polarization with a semiconducting nature distinguishes the monolayer fundamentally from the bulk compound as well as from other two-dimensional transition metal dichalcogenides. Monolayer T-phase TaS2 therefore has the potential to enable two-dimensional spintronics. © 2014 American Physical Society.
Unconventional charge density wave in the organic conductor alpha-(BEDT-TTF)_2KHg(SCN)_4
Maki, Kazumi; Dóra, Balázs; Kartsovnik, Mark; Virosztek, Attila; Korin-Hamzic, Bojana; Basletic, Mario
2002-01-01
The low temperature phase (LTP) of alpha-(BEDT-TTF)_2KHg(SCN)_4 salt is known for its surprising angular dependent magnetoresistance (ADMR), which has been studied intensively in the last decade. However, the nature of the LTP has not been understood until now. Here we analyse theoretically ADMR in unconventional (or nodal) charge density wave (UCDW). In magnetic field the quasiparticle spectrum in UCDW is quantized, which gives rise to spectacular ADMR. The present model accounts for many st...
De Haas-van Alphen oscillations in the charge-density wave compound lanthanum tritelluride (LaTe3)
Energy Technology Data Exchange (ETDEWEB)
Ru, N.; /Stanford U., Geballe Lab.; Borzi, R.A.; Rost, A.; Mackenzie, A.P.; /St. Andrews U., Phys. Astron.; Laverock, J.; Dugdale, S.B.; /Bristol U.; Fisher, I.R.; /Stanford U., Geballe Lab.
2009-12-14
De Haas-van Alphen oscillations were measured in lanthanum tritelluride (LaTe{sub 3}) to probe the partially gapped Fermi surface resulting from charge density wave (CDW) formation. Three distinct frequencies were observed, one of which can be correlated with a FS sheet that is unaltered by CDW formation. The other two frequencies arise from FS sheets that have been reconstructed in the CDW state.
Giant Nernst effect in the incommensurate charge density wave state of P4W12O44
Kolincio, Kamil K.; Daou, Ramzy; Pérez, Olivier; Guérin, Laurent; Fertey, Pierre; Pautrat, Alain
2016-12-01
We report the study of Nernst effect in quasi-low-dimensional tungsten bronze P4W12O44 showing a sequence of Peierls instabilities. We demonstrate that both condensation of the electronic carriers in the charge density wave state and the existence of high-mobility electrons and holes originating from the small pockets remaining in the incompletely nested Fermi surface give rise to a Nernst effect of a magnitude similar to that observed in heavy fermion compounds.
Pressure-induced quenching of the charge-density-wave state observed by x-ray diffraction
Energy Technology Data Exchange (ETDEWEB)
Sacchetti, A.
2010-05-03
We report an x-ray diffraction study on the charge-density-wave (CDW) LaTe{sub 3} and CeTe{sub 3} compounds as a function of pressure. We extract the lattice constants and the CDW modulation wave-vector, and provide direct evidence for a pressure-induced quenching of the CDW phase. We observe subtle differences between the chemical and mechanical compression of the lattice. We account for these with a scenario where the effective dimensionality in these CDW systems is dependent on the type of lattice compression and has a direct impact on the degree of Fermi surface nesting and on the strength of fluctuation effects.
Charge density wave order in 1D mirror twin boundaries of single-layer MoSe2
Barja, Sara; Wickenburg, Sebastian; Liu, Zhen-Fei; Zhang, Yi; Ryu, Hyejin; Ugeda, Miguel M.; Hussain, Zahid; Shen, Zhi-Xun; Mo, Sung-Kwan; Wong, Ed; Salmeron, Miquel B.; Wang, Feng; Crommie, Michael F.; Ogletree, D. Frank; Neaton, Jeffrey B.; Weber-Bargioni, Alexander
2016-08-01
We provide direct evidence for the existence of isolated, one-dimensional charge density waves at mirror twin boundaries (MTBs) of single-layer semiconducting MoSe2. Such MTBs have been previously observed by transmission electron microscopy and have been predicted to be metallic in MoSe2 and MoS2. Our low-temperature scanning tunnelling microscopy/spectroscopy measurements revealed a substantial bandgap of 100 meV opening at the Fermi energy in the otherwise metallic one-dimensional structures. We found a periodic modulation in the density of states along the MTB, with a wavelength of approximately three lattice constants. In addition to mapping the energy-dependent density of states, we determined the atomic structure and bonding of the MTB through simultaneous high-resolution non-contact atomic force microscopy. Density functional theory calculations based on the observed structure reproduced both the gap opening and the spatially resolved density of states.
Stripe and Short Range Order in the Charge Density Wave of 1 T -CuxTiSe2
Novello, A. M.; Spera, M.; Scarfato, A.; Ubaldini, A.; Giannini, E.; Bowler, D. R.; Renner, Ch.
2017-01-01
We study the impact of Cu intercalation on the charge density wave (CDW) in 1 T -CuxTiSe2 by scanning tunneling microscopy and spectroscopy. Cu atoms, identified through density functional theory modeling, are found to intercalate randomly on the octahedral site in the van der Waals gap and to dope delocalized electrons near the Fermi level. While the CDW modulation period does not depend on Cu content, we observe the formation of charge stripe domains at low Cu content (x domains at higher Cu content. The latter shrink with increasing Cu concentration and tend to be phase shifted. These findings invalidate a proposed excitonic pairing as the primary CDW formation mechanism in this material.
Remarkable Stability of Charge Density Wave Order in La1.875 Ba0.125 CuO4
Chen, X. M.; Thampy, V.; Mazzoli, C.; Barbour, A. M.; Miao, H.; Gu, G. D.; Cao, Y.; Tranquada, J. M.; Dean, M. P. M.; Wilkins, S. B.
2016-10-01
The occurrence of charge-density-wave (CDW) order in underdoped cuprates is now well established, although the precise nature of the CDW and its relationship with superconductivity is not. Theoretical proposals include contrasting ideas such as that pairing may be driven by CDW fluctuations or that static CDWs may intertwine with a spatially modulated superconducting wave function. We test the dynamics of CDW order in La1.825 Ba0.125 CuO4 by using x-ray photon correlation spectroscopy at the CDW wave vector, detected resonantly at the Cu L3 edge. We find that the CDW domains are strikingly static, with no evidence of significant fluctuations up to 2 ¾ h . We discuss the implications of these results for some of the competing theories.
Remarkable Stability of Charge Density Wave Order in La_{1.875}Ba_{0.125}CuO_{4}.
Chen, X M; Thampy, V; Mazzoli, C; Barbour, A M; Miao, H; Gu, G D; Cao, Y; Tranquada, J M; Dean, M P M; Wilkins, S B
2016-10-14
The occurrence of charge-density-wave (CDW) order in underdoped cuprates is now well established, although the precise nature of the CDW and its relationship with superconductivity is not. Theoretical proposals include contrasting ideas such as that pairing may be driven by CDW fluctuations or that static CDWs may intertwine with a spatially modulated superconducting wave function. We test the dynamics of CDW order in La_{1.825}Ba_{0.125}CuO_{4} by using x-ray photon correlation spectroscopy at the CDW wave vector, detected resonantly at the Cu L_{3} edge. We find that the CDW domains are strikingly static, with no evidence of significant fluctuations up to 2 ¾ h. We discuss the implications of these results for some of the competing theories.
Extended phonon collapse and the origin of the charge-density-wave in NbSe{sub 2}.
Energy Technology Data Exchange (ETDEWEB)
Weber, F.; Rosenkranz, S.; Castellan, J.-P.; Osborn, R.; Hott, R.; Heid, R.; Bohnen, K.-P.; Egami, T.; Said, A. H.; Reznik, D. (X-Ray Science Division); ( MSD); (Karlsruhe Inst. of Tech.); (Univ. of Tennessee); (Univ. of Colorado at Boulder)
2011-01-01
We report inelastic x-ray scattering measurements of the temperature dependence of phonon dispersion in the prototypical charge-density-wave (CDW) compound 2H-NbSe{sub 2}. Surprisingly, acoustic phonons soften to zero frequency and become overdamped over an extended region around the CDW wave vector. This extended phonon collapse is dramatically different from the sharp cusp in the phonon dispersion expected from Fermi surface nesting. Instead, our experiments, combined with ab initio calculations, show that it is the wave vector dependence of the electron-phonon coupling that drives the CDW formation in 2H-NbSe{sub 2} and determines its periodicity. This mechanism explains the so far enigmatic behavior of CDW in 2H-NbSe{sub 2} and may provide a new approach to other strongly correlated systems where electron-phonon coupling is important.
Unconventional Charge-Density Wave in the Organic Conductor α-(BEDT-TTF)2KHg(SCN)4
Maki, Kazumi; Dóra, Balázs; Kartsovnik, Mark; Virosztek, Attila; Korin-Hamzić, Bojana; Basletić, Mario
2003-06-01
The low temperature phase (LTP) of α-(BEDT-TTF)2KHg(SCN)4 salt is known for its surprising angular dependent magnetoresistance (ADMR), which has been studied intensively in the last decade. However, the nature of the LTP has not been understood until now. Here we analyze theoretically ADMR in unconventional (or nodal) charge-density wave (UCDW). In magnetic field the quasiparticle spectrum in UCDW is quantized, which gives rise to spectacular ADMR. The present model accounts for many striking features of ADMR data in α-(BEDT-TTF)2KHg(SCN)4.
The 181Ta Nuclear Quadrupole Interaction in the Charge Density Wave Phases of 1T-TaS2
Ganal, P.; Butz, T.; Lerf, A.; Naito, M.; Nishihara, H.
1990-04-01
With a high resolution time differential perturbed angular correlation spectrometer we investigated the nuclear quadrupole interaction of Ta in 1T-TaS2 . The results obtained for the commensurate charge density wave phase lead to a revised assignment of the previously observed 181Ta NQR resonances. Differences in the intracluster architecture of the 13-atom Star of David cluster between 1T-TaS2 and 1T-TaSe2 could be responsible for the metal to semiconductor transition which occurs in lT-TaS2 but not in lT-TaSe2 .
Optical Properties of the Charge-Density-Wave Polychalcogenide Compounds R2Te5 (R=Nd, Sm and Gd)
Energy Technology Data Exchange (ETDEWEB)
Pfuner, F.; Degiorgi, L.; /Zurich, ETH; Shin, K.Y.; Fisher, I.R.; /Stanford U., Geballe Lab.
2010-02-15
We investigate the rare-earth polychalcogenide R{sub 2}Te{sub 5} (R = Nd, Sm and Gd) charge-density-wave (CDW) compounds by optical methods. From the absorption spectrum we extract the excitation energy of the CDW gap and estimate the fraction of the Fermi surface which is gapped by the formation of the CDW condensate. In analogy to previous findings on the related RTe{sub n} (n = 2 and 3) families, we establish the progressive closing of the CDW gap and the moderate enhancement of the metallic component upon chemically compressing the lattice.
Magnetic field-induced charge-density-wave transitions: The role of the orbital and Pauli effects
Kartsovnik, M. V.; Andres, D.; Biberacher, W.; Müller, H.
2009-03-01
Due to a low transition temperature and, correspondingly, a small energy gap, the charge-density-wave (CDW) state of the layered organic metal α-(BEDT-TTF)2KHg(SCN)4 is very sensitive to pressure and magnetic field. The latter couples to the CDW via two competing mechanisms: Pauli paramagnetism and orbital motion of charge carriers in a magnetic field. We study the interplay between the Pauli and orbital effects under a pressure of 2.8 kbar, in the region of the field-induced CDW (FICDW) instability. We find that, in agreement with theoretical predictions, the FICDW state is enhanced when the Zeeman splitting becomes commensurate with the orbital quantization.
Magnetic field-induced charge-density-wave transitions: The role of the orbital and Pauli effects
Energy Technology Data Exchange (ETDEWEB)
Kartsovnik, M.V. [Walther-Meissner-Institut, Bayerische Akademie der Wissenschaften, 85748 Garching (Germany)], E-mail: mark.kartsovnik@wmi.badw.de; Andres, D.; Biberacher, W. [Walther-Meissner-Institut, Bayerische Akademie der Wissenschaften, 85748 Garching (Germany); Mueller, H. [European Synchrotron Radiation Facility, F-38043 Grenoble (France)
2009-03-01
Due to a low transition temperature and, correspondingly, a small energy gap, the charge-density-wave (CDW) state of the layered organic metal {alpha}-(BEDT-TTF){sub 2}KHg(SCN){sub 4} is very sensitive to pressure and magnetic field. The latter couples to the CDW via two competing mechanisms: Pauli paramagnetism and orbital motion of charge carriers in a magnetic field. We study the interplay between the Pauli and orbital effects under a pressure of 2.8 kbar, in the region of the field-induced CDW (FICDW) instability. We find that, in agreement with theoretical predictions, the FICDW state is enhanced when the Zeeman splitting becomes commensurate with the orbital quantization.
Zhou, Faran; Golubev, Timofey; Hwang, Bin; Ruan, Chong-Yu; Duxbury, Phil; Malliakas, Christos; Kanatzidis, Mercouri
2015-03-01
Electron-phonon interactions can give rise to various charge-ordered states, especially at low dimensions, where Fermi surface is more prone to form nesting. Rare earth tritellurides compound ErTe3 develops charge density waves (CDW) along two perpendicular directions at different temperatures. By directly probing the order parameters of the two CDWs using femtosecond electron crystallography under different temperatures and driving photonic energy, we investigated the emergences of competing CDW orders in a dynamical phase diagram. The anisotropic symmetry breaking and the role of electron-phonon coupling, and photo-doping effect are discussed in reference to other CDW systems. Our work is supported by Department of Energy under Grant No. DE-FG02-06ER46309.
Universal bulk charge-density-wave (CDW) correlations in the cuprate superconductors
Tabis, Wojciech
2014-03-01
The recent observation of bulk CDW order in YBa2Cu3O8+δ(YBCO) in competition with superconductivity is a significant development. Using Cu L-edge resonant X-ray scattering, we also observe bulk CDW order in HgBa2CuO4+δ(Hg1201 Tc = 72K). The correlations appear below TCDW ~ 200K, well below the pseudogap temperature T* ~ 320K associated with unusual magnetism, but coincident with the onset of Fermi-liquid-like charge transport. In contrast to YBCO, we observe no decrease of the CDW amplitude below Tc, and the correlation length is short and temperature independent. CDW correlations therefore are a universal property of underdoped cuprates, enhanced by low structural symmetry and a magnetic field, but fundamentally not in significant competition with superconductivity. We also discuss the relationship between the CDW modulation wave vector and the Fermi surface area extracted from QO experiments. Work supported by DOE-BES. In collaboration with Y. Li, M. Le Tacon, L. Braicovich, A. Kreyssig, M. Minola, G. Dellea, E. Weschke, M. Veit, A. Goldman, T. Schmitt, G. Ghiringhelli, N. Barisic, M.K. Chan, C. Dorow, G. Yu, X. Zhao, B. Keimer, M. Greven.
Magnetic-field-tuned charge density wave in SmNiC2 and NdNiC2
Lei, Hechang; Wang, Kefeng; Petrovic, C.
2017-02-01
We report magnetic field tuned competition between magnetic order and charge density wave (CDW) states in SmNiC2 and NdNiC2 polycrystals. The destruction of CDW can be observed not only in SmNiC2 below ferromagnetic (FM) but also in NdNiC2 below antiferromagnetic (AFM) transition temperature. Moreover, the CDW states near magnetic transition temperatures can be tuned by the magnetic field for both compounds. Magnetic-field induced FM state in NdNiC2 is more effective in weakening the CDW than the AFM state at temperatures near Neel temperature T N but both ordering states have the same effect on CDW below T N. The interplay between magnetic and CDW states in SmNiC2 and NdNiC2 may be different, suggesting that these materials are good models to study correlations between magnetic and CDW wave order.
Wave-vector-dependent electron-phonon coupling and the charge-density-wave transition in TbT e3
Maschek, M.; Rosenkranz, S.; Heid, R.; Said, A. H.; Giraldo-Gallo, P.; Fisher, I. R.; Weber, F.
2015-06-01
We present a high-energy-resolution inelastic x-ray scattering investigation of the soft phonon mode in the charge-density-wave (CDW) system TbT e3 . We analyze our data based on lattice dynamical calculations using density-functional-perturbation theory and find clear evidence that strongly momentum-dependent electron-phonon coupling defines the periodicity of the CDW superstructure: Our experiment reveals strong phonon softening and increased phonon linewidths over a large part in reciprocal space adjacent to the CDW ordering vector qCDW=(0 ,0 ,0.3 ) . Further, qCDW is clearly offset from the wave vector of (weak) Fermi surface nesting qFS=(0 ,0 ,0.25 ) , and our detailed analysis indicates that electron-phonon coupling is responsible for this shift. Hence, we can add TbT e3 , which was previously considered as a canonical CDW compound following the Peierls scenario, to the list of distinct charge-density-wave materials characterized by momentum-dependent electron-phonon coupling.
Scanning tunneling microscopy in TTF-TCNQ: Phase and amplitude modulated charge density waves
DEFF Research Database (Denmark)
Wang, Z.Z.; Gorard, J.C.; Pasquier, C.;
2003-01-01
phase transitions of TTF-TCNQ have been identified. The measurement of the modulation wave vector along the a direction provides evidence of the existence of domains comprising single plane wave modulated structures in the temperature regime where the transverse wave vector of the CDW is temperature...
Impact of quenched oxygen disorder on charge density wave order in YBa2Cu3O6+x.
Achkar, A J; Mao, X; McMahon, Christopher; Sutarto, R; He, F; Liang, Ruixing; Bonn, D A; Hardy, W N; Hawthorn, D G
2014-09-05
The competition between superconductivity and charge density wave (CDW) order in underdoped cuprates has now been widely reported, but the role of disorder in this competition has yet to be fully resolved. A central question is whether disorder sets the length scale of the CDW order, for instance by pinning charge density fluctuations or disrupting an otherwise long-range order. Using resonant soft x-ray scattering, we investigate the sensitivity of CDW order in YBa2Cu3O6+x (YBCO) to varying levels of oxygen disorder. We find that quench cooling YBCO6.67 (YBCO6.75) crystals to destroy their o-V and o-VIII (o-III) chains decreases the intensity of the CDW superlattice peak by a factor of 1.9 (1.3), but has little effect on the CDW correlation length, incommensurability, and temperature dependence. This reveals that while quenched oxygen disorder influences the CDW order parameter, the spatial extent of the CDW order is insensitive to the level of quenched oxygen disorder and may instead be a consequence of competition with superconductivity.
Energy Technology Data Exchange (ETDEWEB)
Yi, Y.; Bishop, A.R. [Theoretical Division and Center for Nonlinear Studies, Los Alamos National Laboratory, Los Alamos, New Mexico 87545 (United States)
1998-08-01
We study the spin-dependent geometric phase effect in mesoscopic rings of charge-density-wave (CDW) materials. When electron spin is explicitly taken into account, we show that the spin-dependent Aharonov-Casher phase can have pronounced frustration effects on such CDW materials with appropriate electron filling. We show that this frustration has observable consequences for transport experiments. We identify a phase transition from a Peierls insulator to metal, which is induced by spin-dependent phase interference effects. Mesoscopic CDW materials and spin-dependent geometric phase effects, and their interplay, are becoming attractive opportunities for exploitation with the rapid development of modern fabrication technology. {copyright} {ital 1998} {ital The American Physical Society}
Latyshev, Y I; Sinchenko, A A; Bulaevskii, L N; Monceau, P
2002-01-01
The peculiarities of the cross-sectional transport in the direction of the crystallographic axis alpha * in the conductor with the NbSe sub 3 wave charge density (WCD) are studied. The strong peak of dynamic conductivity is observed on the WCD of the layered structures and the NbSe sub 3 -NbSe sub 3 point contacts at low temperatures by the zero voltage shift. The identified behavior reminds in many respects the interlayer tunnel conductivity in the Bi-2212-type high-temperature layered conductors. The conductivity peak by the zero shift is explained in the model of the almost coherent interlayer tunneling of the carriers, noncondensed in the WCD
Three-Dimensional Charge Density Wave Order in YBa2Cu3O6.67 at High Magnetic Fields
Energy Technology Data Exchange (ETDEWEB)
Gerber, S.; Jang, H.; Nojiri, H.; Matsuzawa, S.; Yasumura, H.; Bonn, D. A.; Liang, R.; Hardy, W.; Islam, Z.; Lee, W. -S.; Zhu, D.; Lee, J. -S.
2015-11-20
Charge density wave (CDW) correlations have been shown to universally exist in cuprate superconductors. However, their nature at high fields inferred from nuclear magnetic resonance is distinct from that measured by x-ray scattering at zero and low fields. Here we combine a pulsed magnet with an x-ray free electron laser to characterize the CDW in YBa2Cu3O6.67 via x-ray scattering in fields up to 28 Tesla. While the zero-field CDW order, which develops below T ~ 150 K, is essentially two-dimensional, at lower temperature and beyond 15 Tesla, another three-dimensionally ordered CDW emerges. The field-induced CDW onsets around the zero-field superconducting transition temperature, yet the incommensurate inplane ordering vector is field-independent. This implies that the two forms of CDW and hightemperature superconductivity are intimately linked.
DEFF Research Database (Denmark)
Chang, J.; Blackburn, E.; Holmes, A. T.
2012-01-01
). This sample has a hole doping of 0.12 per copper and a well-ordered oxygen chain superstructure. Below Tc, the application of a magnetic field suppresses superconductivity and enhances the CDW. Hence, the CDW and superconductivity in this typical high-Tc material are competing orders with similar energy...... scales, and the high-Tc superconductivity forms from a pre-existing CDW environment. Our results provide a mechanism for the formation of small Fermi surface pockets, which explain the negative Hall and Seebeck effects and the ‘Tc plateau’ in this material when underdoped.......Superconductivity often emerges in the proximity of, or in competition with, symmetry-breaking ground states such as antiferromagnetism or charge density waves (CDW). A number of materials in the cuprate family, which includes the high transition-temperature (high-Tc) superconductors, show spin...
Institute of Scientific and Technical Information of China (English)
崔珊; 何兰坡; 洪晓晨; 朱相德; Cedomir Petrovic; 李世燕
2016-01-01
It was found that selenium doping can suppress the charge-density-wave (CDW) order and induce bulk supercon-ductivity in ZrTe3. The observed superconducting dome suggests the existence of a CDW quantum critical point (QCP) in ZrTe3−x Sex near x≈0.04. To elucidate the superconducting state near the CDW QCP, we measure the thermal conductivity of two ZrTe3−x Sex single crystals (x=0.044 and 0.051) down to 80 mK. For both samples, the residual linear termκ0/T at zero field is negligible, which is a clear evidence for nodeless superconducting gap. Furthermore, the field dependence ofκ0/T manifests a multigap behavior. These results demonstrate multiple nodeless superconducting gaps in ZrTe3−x Sex , which indicates conventional superconductivity despite of the existence of a CDW QCP.
Wang, H.-T.; Srivastava, M. K.; Wu, C.-C.; Hsieh, S.-H.; Wang, Y.-F.; Shao, Y.-C.; Liang, Y.-H.; Du, C.-H.; Chiou, J.-W.; Cheng, C.-M.; Chen, J.-L.; Pao, C.-W.; Lee, J.-F.; Kuo, C. N.; Lue, C. S.; Wu, M.-K.; Pong, W.-F.
2017-01-01
X-ray scattering (XRS), x-ray absorption near-edge structure (XANES) and extended x-ray absorption fine structure (EXAFS) spectroscopic techniques were used to study the electronic and atomic structures of the high-quality Sr3Ir4Sn13 (SIS) single crystal below and above the transition temperature (T* ≈ 147 K). The evolution of a series of modulated satellite peaks below the transition temperature in the XRS experiment indicated the formation of a possible charge density wave (CDW) in the (110) plane. The EXAFS phase derivative analysis supports the CDW-like formation by revealing different bond distances [Sn1(2)-Sn2] below and above T* in the (110) plane. XANES spectra at the Ir L3-edge and Sn K-edge demonstrated an increase (decrease) in the unoccupied (occupied) density of Ir 5d-derived states and a nearly constant density of Sn 5p-derived states at temperatures T atomic structures and the CDW-like phase in the SIS single crystal. PMID:28106144
Ekino, T.; Gabovich, A. M.; Li, Mai Suan; Szymczak, H.; Voitenko, A. I.
2016-11-01
The quasiparticle tunnel current J(V) between the superconducting ab-planes along the c-axis and the corresponding conductance G(V)=\\text{d}J/\\text{d}V were calculated for symmetric junctions composed of disordered d-wave layered superconductors partially gapped by charge density waves (CDWs). Here, V is the voltage. Both the checkerboard and unidirectional CDWs were considered. It was shown that the spatial spread of the CDW-pairing strength substantially smears the peculiarities of G(V) appropriate to uniform superconductors. The resulting curves G(V) become very similar to those observed for a number of cuprates in intrinsic junctions, e.g. mesas. In particular, the influence of CDWs may explain the peak-dip-hump structures frequently found for high-T c oxides.
Aspects of unconventional density waves
Maki, Kazumi; Dóra, Balázs; Virosztek, Attila
2003-12-01
Recently many people discuss unconventional density waves (i.e. unconventional charge density waves (UCDW) and unconventional spin density waves (USDW)). Unlike in conventional density waves, the quasiparticle spectrum in these systems is gapless. Also these systems remain metallic. Indeed it appears that there are many candidates for UDW. The low temperature phase of α-(BEDT-TTF)2KHg(SCN)4, the antiferromagnetic phase in URu2Si2, the CDW in transition metal dichalcogenite NbSe2, the pseudogap phase in high Tc cuprate superconductors, the glassy phase in organic superconductor κ-(BEDT-TTF)2Cu[N(CN)2]Br. After a brief introduction on UCDW and USDW, we shall discuss some of the above systems, where we believe we have evidence for unconventional density waves.
Pressure dependence of the optical properties of the charge-density-wave compound LaTe2
Energy Technology Data Exchange (ETDEWEB)
Lavagnini, M.; Sacchetti, A.; Degiorgi, L.; /Zurich, ETH; Arcangeletti, E.; Baldassarre, L.; Postorino, P.; Lupi, S.; /Rome U.; Perucchi, A.; /INFM, Trieste; Shin, K.Y.; Fisher, I.R.; /Stanford U., Geballe Lab.
2009-12-14
We report the pressure dependence of the optical response of LaTe{sub 2}, which is deep in the charge-density-wave (CDW) ground state even at 300 K. The reflectivity spectrum is collected in the mid-infrared spectral range at room temperature and at pressures between 0 and 7 GPa. We extract the energy scale due to the single particle excitation across the CDW gap and the Drude weight. We establish that the gap decreases upon compressing the lattice, while the Drude weight increases. This signals a reduction in the quality of nesting upon applying pressure, therefore inducing a lesser impact of the CDW condensate on the electronic properties of LaTe{sub 2}. The consequent suppression of the CDW gap leads to a release of additional charge carriers, manifested by the shift of weight from the gap feature into the metallic component of the optical response. On the contrary, the power-law behavior, seen in the optical conductivity at energies above the gap excitation and indicating a weakly interacting limit within the Tomonaga-Luttinger liquid scenario, seems to be only moderately dependent on pressure.
Splitting of the Ti-3d bands of TiSe2 in the charge-density wave phase
Ghafari, A.; Petaccia, L.; Janowitz, C.
2017-02-01
Very high resolution angular resolved photoemission (ARPES) spectra on TiSe2 in two distinct polarization geometries (vertical and horizontal) at temperatures between 300 K and 22 K enabled the observation of details of bands near the Fermi level not reported so far. Calculations of the electronic band structure based on density functional theory (DFT) using B3LYP hybrid functional and MBJ potential (with and without spin-orbit coupling) were performed to obtain the orbital symmetry and dispersion. Two degenerate conduction bands (CB's) were observed at the Γ-point, a weak CB- emission at the A-point, and two non degenerate CB's (i.e. splitting of CB) at the M/L-point of the Brillouin Zone (BZ). The splitting was detected at L for both polarizations, while at M remarkably only for horizontal polarization. These results cannot be fully accounted for by current theories for the charge density wave (CDW) and point to a reduced symmetry of the electronic states, possibly due to the chiral CDW.
Andres, D.; Kartsovnik, M. V.; Biberacher, W.; Neumaier, K.; Sheikin, I.; Müller, H.; Kushch, N. D.
2011-10-01
Successive magnetic-field-induced charge-density-wave transitions in the layered molecular conductor α-(BEDT-TTF)2KHg(SCN)4 are studied in a hydrostatic pressure regime in which the zero field charge-density- wave (CDW) state is completely suppressed. It is shown that the orbital effect of the magnetic field restores the density wave, while orbital quantization induces transitions between different CDW states as the field strength is varied. The latter show up as distinct anomalies in the magnetoresistance as a function of field. The interplay between the orbital and Pauli paramagnetic effects, which act, respectively, to enhance and to suppress the CDW instability, is particularly manifest in the angular dependence of the field-induced anomalies.
Energy Technology Data Exchange (ETDEWEB)
Creager, W.N.
1991-09-01
The far infrared reflectance and conductivity of (Ta{sub 1-x}Nb{sub x}Se{sub 4}){sub 2}I and TaS{sub 3} have been measured to determine the origin of a huge infrared resonance that dominates the charge density wave (CDW) dynamics along with the pinned acoustic phason mode in the related materials (TaSe{sub 4}){sub 2}I and K{sub 0. 3}MoO{sub 3}. The measurements cover frequencies from 3 to 700cm{sup {minus}1} and the temperature range from 15K to 300K. In the niobium-doped alloys (Ta{sub 1-x}Nb{sub x}Se{sub 4}){sub 2}I, the size and frequency of the giant infrared mode remain nearly constant as the impurity concentration x is increased. For TaS{sub 3}, the pinned acoustic phason near 0.5cm{sup {minus}1} dominates {var epsilon}({omega}) and an additional small mode lies near 9cm{sup {minus}1}. The latter mode is much smaller than the infrared mode in other CDW materials. These results rule out several models of a generic infrared mode'' in CDW excitations. They are compared in detail to the predictions of a recent theory attributing the infrared mode to a bound collective mode localized at impurity sites within the crystal. The transmittance of K{sub 0.3}MoO{sub 3} has been measured at 1.2K with a strong dc electric field applied across the crystal. Under these conditions, the charge density wave depins abruptly and carries large currents with near-zero differential resistance. For some samples, the low-frequency transmittance is enhanced slightly when the CDW depins. The magnitude of the oxygen isotope effect in the high-{Tc} superconductor YBa{sub 2}Cu{sub 3}O{sub 7} has been determined by substitution of {sup 18}O for {sup 16}O. A series of cross-exchanges was performed on high-quality polycrystalline specimens to eliminate uncertainties due to sample heat treatments and sample inhomogeneities.
Charge density wave and excitonic magnetic polarons in CeTe sub 2
Kasuya, T; Takabatake, T
2000-01-01
Mechanisms of anomalous magnetic and transport properties in CeTe sub 2 observed recently on single-crystal samples are studied by comparing with the nonmagnetic reference material LaTe sub 2 , as well as other typical low carrier-density systems such as Ce monopnictides, doped Eu chalcogenides and Yb sub 4 As sub 3. The present system is unique on the point of low-carrier semimetal due to CDW of near perfect nesting, which is shown to be nearly independent of the spin-orbit splitting. The large residual resistivity indicates the giant molecular scattering due to excitonic states forming the distorted Wigner crystal, similar to Yb sub 4 As sub 3. At low temperatures, induced magnetic polarons cause unusual novel transport properties with a sharp peak of resistivity without any anomaly on other physical properties. This is attributed to a sharp glassy transition from an antiferromagnetic short-range ordering to the ferromagnetic ordering of the magnetic polarons within each CeTe double layer sandwiching the mo...
Shao, D. F.; Xiao, R. C.; Lu, W. J.; Lv, H. Y.; Li, J. Y.; Zhu, X. B.; Sun, Y. P.
2016-09-01
The transition-metal dichalcogenide 1 T -TaS2 exhibits a rich set of charge-density-wave (CDW) orders. Recent investigations suggested that using light or an electric field can manipulate the commensurate CDW (CCDW) ground state. Such manipulations are considered to be determined by charge-carrier doping. Here we use first-principles calculations to simulate the carrier-doping effect on the CCDW in 1 T -TaS2 . We investigate the charge-doping effects on the electronic structures and phonon instabilities of the 1 T structure, and we analyze the doping-induced energy and distortion ratio variations in the CCDW structure. We found that both in bulk and monolayer 1 T -TaS2 , the CCDW is stable upon electron doping, while hole doping can significantly suppress the CCDW, implying different mechanisms of such reported manipulations. Light or positive perpendicular electric-field-induced hole doping increases the energy of the CCDW, so that the system transforms to a nearly commensurate CDW or a similar metastable state. On the other hand, even though the CCDW distortion is more stable upon in-plane electric-field-induced electron injection, some accompanied effects can drive the system to cross over the energy barrier from the CCDW to a nearly commensurate CDW or a similar metastable state. We also estimate that hole doping can introduce potential superconductivity with a Tc of 6-7 K. Controllable switching of different states such as a CCDW/Mott insulating state, a metallic state, and even a superconducting state can be realized in 1 T -TaS2 . As a result, this material may have very promising applications in future electronic devices.
Emergence of coherence in the charge-density wave state of 2H-NbSe2
Chatterjee, U.; Zhao, J.; Iavarone, M.; Di Capua, R.; Castellan, J. P.; Karapetrov, G.; Malliakas, C. D.; Kanatzidis, M. G.; Claus, H.; Ruff, J. P. C.; Weber, F.; van Wezel, J.; Campuzano, J. C.; Osborn, R.; Randeria, M.; Trivedi, N.; Norman, M. R.; Rosenkranz, S.
2015-01-01
A charge-density wave (CDW) state has a broken symmetry described by a complex order parameter with an amplitude and a phase. The conventional view, based on clean, weak-coupling systems, is that a finite amplitude and long-range phase coherence set in simultaneously at the CDW transition temperature Tcdw. Here we investigate, using photoemission, X-ray scattering and scanning tunnelling microscopy, the canonical CDW compound 2H-NbSe2 intercalated with Mn and Co, and show that the conventional view is untenable. We find that, either at high temperature or at large intercalation, CDW order becomes short-ranged with a well-defined amplitude, which has impacts on the electronic dispersion, giving rise to an energy gap. The phase transition at Tcdw marks the onset of long-range order with global phase coherence, leading to sharp electronic excitations. Our observations emphasize the importance of phase fluctuations in strongly coupled CDW systems and provide insights into the significance of phase incoherence in ‘pseudogap’ states. PMID:25687135
Charge density wave and superconductivity in 2H- and 4H-NbSe2: A revisit
Indian Academy of Sciences (India)
I Naik; A K Rastogi
2011-06-01
Good-quality hexagonal NbSe2 single crystals were prepared. In 2H-NbSe2, superconducting and charge density wave (CDW) transitions were found at = 7.4 K and = 35 K respectively as reported previously. We have noticed that these two transitions are changed to = 42 K and = 6.5 K, in 4H-NbSe2. Thermopower has shown clear anomaly at CDW transitions. The anisotropic upper critical ﬁeld was calculated as ∼ 3 and 6.3 for 2H- and 4H-single crystals around = 0.81, where = /, from resistivity and explained in terms of coherence length. From the relation, $H_{c2}() = H_{c2}(0)[1 − ^2]$, $H^l_{c2}(0)$ was calculated as ∼ 8.15 T and 16.98 T at = 0.84 in 2H-NbSe2 and 4H-NbSe2 respectively. However, $H^_{c2}(0) = 2.68$ T for both single crystals.
Mamun, A A; Shukla, P K
2009-09-01
Effects of the nonthermal distribution of electrons as well as the polarity of the net dust-charge number density on nonplanar (viz. cylindrical and spherical) dust-ion-acoustic solitary waves (DIASWs) are investigated by employing the reductive perturbation method. It is found that the basic features of the DIASWs are significantly modified by the effects of nonthermal electron distribution, polarity of net dust-charge number density, and nonplanar geometry. The implications of our results in some space and laboratory dusty plasma environments are briefly discussed.
Dóra, B.; Maki, K.; Virosztek, A.; Ványolos, A.
2004-04-01
We have investigated theoretically the thermoelectric power and the Nernst effect in unconventional density waves (UDW). Due to the presence of magnetic field, Landau levels are formed, and the low energy excitations change from gapless to gapped. The present results account consistently for the recent data of magnetothermopower in α-(BEDT-TTF)2KHg(SCN)4 obtained by Choi et al. (Phys. Rev. B, 65, 205119 (2002)). This confirms further our identification of low temperature phase (LTP) in this salt as UCDW. Key words. density waves, α-(BEDT-TTF)2KHg(SCN)4, thermoelectric power.
Suppression and inducement of the charge-density-wave state in Cr x TiSe2.
Selezneva, N V; Sherokalova, E M; Pleshchev, V G; Kazantsev, V A; Baranov, N V
2016-08-10
The x-ray diffraction, electrical resistivity and thermal expansion measurements have been employed to study how the intercalation of Cr atoms into TiSe2 matrix affects the crystal structure, formation of the charge density wave (CDW) and electrical properties. The intercalation of a small amount of Cr atoms (up to x ~ 0.03) is observed to suppress the CDW formation. The electrical resistivity of Cr x TiSe2 compounds with the Cr concentrations 0.03 ⩽ x ⩽ 0.20 shows a metallic-type behavior; while in the concentration range 0.25 ⩽ x ⩽ 0.5, the resistivity shows an anomalous behavior indicating the reappearance of the transition to a CDW-like state; further growth of the Cr content up to x = 0.6 again leads to the metallic-type resistivity. For the compound Cr0.25TiSe2, the phase transition below 160 K together with abnormal change in the electrical resistivity is found to be accompanied by anomalies in the lattice parameters and thermal expansion behavior; this transition is classified as first-order type. It has been found that despite the intercalation of Cr atoms some Ti-Se bonds in the Se-Ti-Se tri-layers of Cr x TiSe2 with x ⩽ 0.5 have nearly the same lengths as in the host lattice TiSe2, which apparently allows the transition to be returned to the CDW-like state.
DEFF Research Database (Denmark)
Blackburn, E.; Chang, J.; Hücker, M.;
2013-01-01
X-ray diffraction measurements show that the high-temperature superconductor YBa2Cu3O6.54, with ortho-II oxygen order, has charge-density-wave order in the absence of an applied magnetic field. The dominant wave vector of the charge density wave is qCDW=(0,0.328(2),0.5), with the in-plane compone...
Soto, F.; Berger, H.; Cabo, L.; Carballeira, C.; Mosqueira, J.; Pavuna, D.; Vidal, F.
2007-03-01
The fluctuation-diamagnetism (FD) above the superconducting transition was measured in 2H-NbSe2 single crystals. The moderate uniaxial anisotropy of this compound, and some experimental improvements, allowed us to measure the superconducting fluctuation effects in the two main crystallographic directions. These results reveal that the nonlocal electrodynamic effects on the FD are highly anisotropic, and they also discard a possible contribution to the FD coming from the charge-density waves (CDWs) appearing below TCDW>TC in 2H-NbSe2 , in agreement with a phenomenological estimate.
Energy Technology Data Exchange (ETDEWEB)
Kartsovnik, M.V., E-mail: mark.kartsovnik@wmi.badw.de [Walther-Meissner-Institut, Bayerische Akademie der Wissenschaften, 85748 Garching (Germany); Biberacher, W.; Andres, D.; Jakob, S.; Kunz, M.; Neumaier, K. [Walther-Meissner-Institut, Bayerische Akademie der Wissenschaften, 85748 Garching (Germany); Mueller, H. [European Synchrotron Radiation Facility, 38043 Grenoble (France); Kushch, N.D. [Institute of Problems of Chemical Physics, 142432 Chernogolovka (Russian Federation)
2012-06-01
Coupling of a magnetic field to the orbital and spin degrees of freedom of charge carriers is well known to cause suppression of superconductivity. While the orbital pair-breaking generally dominates in conventional superconductors, the Pauli paramagnetic effect may become important in some heavy fermion compounds or strongly anisotropic materials such as high-T{sub c} or organic superconductors. The same two mechanisms are predicted to be operative also in the case of charge-density-wave (CDW) ordering. However, now they lead to opposite effects: the paramagnetic coupling weakens the CDW interaction whereas the orbital coupling enhances it in a system with an imperfectly nested Fermi surface. Here we report on the experimental evidence of both kinds of magnetic field effects on the CDW and superconducting instabilities in the layered organic metal {alpha}-(BEDT-TTF){sub 2}KHg(SCN){sub 4} under quasihydrostatic pressure.
Kartsovnik, M. V.; Biberacher, W.; Andres, D.; Jakob, S.; Kunz, M.; Neumaier, K.; Müller, H.; Kushch, N. D.
2012-06-01
Coupling of a magnetic field to the orbital and spin degrees of freedom of charge carriers is well known to cause suppression of superconductivity. While the orbital pair-breaking generally dominates in conventional superconductors, the Pauli paramagnetic effect may become important in some heavy fermion compounds or strongly anisotropic materials such as high-Tc or organic superconductors. The same two mechanisms are predicted to be operative also in the case of charge-density-wave (CDW) ordering. However, now they lead to opposite effects: the paramagnetic coupling weakens the CDW interaction whereas the orbital coupling enhances it in a system with an imperfectly nested Fermi surface. Here we report on the experimental evidence of both kinds of magnetic field effects on the CDW and superconducting instabilities in the layered organic metal α-(BEDT-TTF)2KHg(SCN)4 under quasihydrostatic pressure.
Holographic Magnetisation Density Waves
Donos, Aristomenis
2016-01-01
We numerically construct asymptotically $AdS$ black brane solutions of $D=4$ Einstein theory coupled to a scalar and two $U(1)$ gauge fields. The solutions are holographically dual to $d=3$ CFTs in a constant external magnetic field along one of the $U(1)$'s. Below a critical temperature the system's magnetisation density becomes inhomogeneous, leading to spontaneous formation of current density waves. We find that the transition can be of second order and that the solutions which minimise the free energy locally in the parameter space of solutions have averaged stressed tensor of a perfect fluid.
Piel, Alexander; Arp, Oliver; Menzel, Kristoffer; Klindworth, Markus
2007-11-01
We report on experimental observations of dust density waves in a complex (dusty) plasma under microgravity. The plasma is produced in a radio-frequency parallel-plate discharge (argon, p=15Pa, U=65Vpp). Different sizes of dust particles were used (3.4 μm and 6.4μm diameter). The low-frequency (f 11Hz) dust density waves are naturally unstable modes, which are driven by the ion flow in the plasma. Surprisingly, the wave propagation direction is aligned with the ion flow direction in the bulk plasma but becomes oblique at the boundary of the dust cloud with an inclination of 60^o with respect to the plasma boundary. The experimental results are compared with a kinetic model in the electrostatic approximation [1] and a fluid model [2]. Moreover, the role of dust surface waves is discussed. [1] M. Rosenberg, J. Vac. Sci. Technol. A 14, 631 (1996) [2] A. Piel et al, Phys. Rev. Lett. 97, 205009 (2006)
X-ray study of femtosecond structural dynamics in the 2D charge density wave compound 1T-TaS{sub 2}
Energy Technology Data Exchange (ETDEWEB)
Laulhé, C., E-mail: laulhe@synchrotron-soleil.fr [Synchrotron SOLEIL, L' Orme des Merisiers, Saint Aubin - BP 48, F-91192 Gif-sur-Yvette (France); Université Paris-Sud, F-91405 Orsay Cedex (France); Cario, L.; Corraze, B.; Janod, E. [Institut des Matériaux Jean Rouxel - UMR 6502, Université de Nantes, 2 rue de la Houssinière, F-44322 Nantes (France); Huber, T. [Institute for Quantum Electronics, Physics Department, ETH Zurich, CH-8093 Zurich (Switzerland); Lantz, G. [Laboratoire de Physique des Solides, Université Paris-Sud, CNRS, UMR 8502, F-91405 Orsay (France); Boulfaat, S. [Synchrotron SOLEIL, L' Orme des Merisiers, Saint Aubin - BP 48, F-91192 Gif-sur-Yvette (France); Ferrer, A.; Mariager, S.O.; Johnson, J.A.; Grübel, S.; Lübcke, A.; Ingold, G.; Beaud, P. [Swiss Light Source, Paul Scherrer Institute, CH-5232, Villigen (Switzerland); Johnson, S.L. [Institute for Quantum Electronics, Physics Department, ETH Zurich, CH-8093 Zurich (Switzerland); Ravy, S. [Synchrotron SOLEIL, L' Orme des Merisiers, Saint Aubin - BP 48, F-91192 Gif-sur-Yvette (France)
2015-03-01
1T-TaS{sub 2} is a 2D metallic compound which undergoes a series of electronically driven phase transitions toward charge density wave and Mott phases. Its intricate electron–phonon interactions and electron–electron correlations have been promising peculiar out-of-equilibrium dynamics. In this paper, we provide the first direct information on the atomic structure response to an ultra-fast infrared laser pulse in the commensurate phase of 1T-TaS{sub 2}, by using femtosecond time-resolved X-ray diffraction. We show that ultra-fast excitation with near-infrared photons drives a displacive excitation of the amplitude mode of the commensurate charge density wave. About 3 ps after laser excitation, the system reaches a new, photo-induced state that is maintained for at least 10 ps. We give evidence that this long-lived state exhibits the same structural modulation as in the thermodynamically stable commensurate phase, with a large correlation length. Only the average amplitude of the modulation is found to decrease. We propose that the long-lived state is formed from the commensurate phase by reducing the modulation amplitude on few superlattice nodes. The underlying mechanism proposed is the annihilation of self-trapped polarons.
Kolincio, Kamil; Pérez, Olivier; Hébert, Sylvie; Fertey, Pierre; Pautrat, Alain
2016-06-01
Detailed structural and magnetotransport properties of monophosphate tungsten bronze Kx(PO2)4(WO3)8 single crystals are reported. Both galvanomagnetic and thermal properties are shown to be consistent with a charge density wave electronic transition due to hidden nesting of the quasi-1D portion of the Fermi surface. We also observe the enhancement of electronic anisotropy due to reconstruction of the Fermi surface at the Peierls transition. The resistivity presents a thermal hysteresis suggesting a first-order nature characteristic of a strong-coupling scenario. However, other measurements such as the change of carrier density demonstrate a second-order Peierls scenario with weak-coupling features. We suggest that the structural transition driven by the residual strain in the K-P-O environment is responsible for the resistivity hysteresis and modifies the Fermi surface which then helps the rise to the second-order Peierls instability.
Oberhofer, Harald; Blumberger, Jochen
2010-12-01
We present a plane wave basis set implementation for the calculation of electronic coupling matrix elements of electron transfer reactions within the framework of constrained density functional theory (CDFT). Following the work of Wu and Van Voorhis [J. Chem. Phys. 125, 164105 (2006)], the diabatic wavefunctions are approximated by the Kohn-Sham determinants obtained from CDFT calculations, and the coupling matrix element calculated by an efficient integration scheme. Our results for intermolecular electron transfer in small systems agree very well with high-level ab initio calculations based on generalized Mulliken-Hush theory, and with previous local basis set CDFT calculations. The effect of thermal fluctuations on the coupling matrix element is demonstrated for intramolecular electron transfer in the tetrathiafulvalene-diquinone (Q-TTF-Q-) anion. Sampling the electronic coupling along density functional based molecular dynamics trajectories, we find that thermal fluctuations, in particular the slow bending motion of the molecule, can lead to changes in the instantaneous electron transfer rate by more than an order of magnitude. The thermal average, ( { } )^{1/2} = 6.7 {mH}, is significantly higher than the value obtained for the minimum energy structure, | {H_ab } | = 3.8 {mH}. While CDFT in combination with generalized gradient approximation (GGA) functionals describes the intermolecular electron transfer in the studied systems well, exact exchange is required for Q-TTF-Q- in order to obtain coupling matrix elements in agreement with experiment (3.9 mH). The implementation presented opens up the possibility to compute electronic coupling matrix elements for extended systems where donor, acceptor, and the environment are treated at the quantum mechanical (QM) level.
Threshold electric field in unconventional density waves
Dóra, Balázs; Virosztek, Attila; Maki, Kazumi
2001-07-01
As it is well known most charge-density waves (CDW's) and spin-density waves exhibit nonlinear transport with well-defined threshold electric field ET. Here we study theoretically the threshold electric field of unconventional density waves. We find that the threshold field increases monotonically with temperature without divergent behavior at Tc, unlike the one in conventional CDW. The present result in the three-dimensional weak pinning limit appears to describe rather well the threshold electric field observed recently in the low-temperature phase of α-(BEDT-TTF)2KHg(SCN)4.
Energy Technology Data Exchange (ETDEWEB)
Croft, Thomas; Lester, Christopher; Hayden, Stephen [H.H. Wills Physics Laboratory, University of Bristol (United Kingdom); Bombardi, Alessandro; Senn, Mark [Diamond Light Source Ltd., Harwell Science and Innovation Campus, Didcot, Oxfordshire (United Kingdom)
2015-07-01
The recent observations of charge and stripe correlations in YBa{sub 2}Cu{sub 3}O{sub 6+x} and La{sub 2-x}Ba{sub x}CuO{sub 4} has reinvigorated interest in their role in influencing the superconductivity of the cuprates. However, structural complications of these systems makes it difficult to isolate the effect the lattice has in inducing the charge order. Here, we report hard X-ray diffraction measurements on three compositions (x=0.11,0.12,0.13) of the high-temperature superconductor La{sub 2-x}Sr{sub x}CuO{sub 4}, a canonical example of HTS with T{sub c} ∼ 35 K and a simple crystal structure. All samples show charge-density-wave (CDW) order with onset temperatures in the range 51-80 K and ordering wavevectors close to (0.23,0,0.5). We present a phase diagram of La{sub 2-x}Sr{sub x}CuO{sub 4} including the pseudogap phase, CDW and magnetic order.
Forgan, E. M.; Blackburn, E.; Holmes, A. T.; Briffa, A. K. R.; Chang, J.; Bouchenoire, L.; Brown, S. D.; Liang, Ruixing; Bonn, D.; Hardy, W. N.; Christensen, N. B.; Zimmermann, M. V.; Hücker, M.; Hayden, S. M.
2015-12-01
Charge density wave (CDW) order appears throughout the underdoped high-temperature cuprate superconductors, but the underlying symmetry breaking and the origin of the CDW remain unclear. We use X-ray diffraction to determine the microscopic structure of the CDWs in an archetypical cuprate YBa2Cu3O6.54 at its superconducting transition temperature ~60 K. We find that the CDWs in this material break the mirror symmetry of the CuO2 bilayers. The ionic displacements in the CDWs have two components, which are perpendicular and parallel to the CuO2 planes, and are out of phase with each other. The planar oxygen atoms have the largest displacements, perpendicular to the CuO2 planes. Our results allow many electronic properties of the underdoped cuprates to be understood. For instance, the CDWs will lead to local variations in the electronic structure, giving an explicit explanation of density-wave states with broken symmetry observed in scanning tunnelling microscopy and soft X-ray measurements.
Forgan, E M; Blackburn, E; Holmes, A T; Briffa, A K R; Chang, J; Bouchenoire, L; Brown, S D; Liang, Ruixing; Bonn, D; Hardy, W N; Christensen, N B; Zimmermann, M V; Hücker, M; Hayden, S M
2015-12-09
Charge density wave (CDW) order appears throughout the underdoped high-temperature cuprate superconductors, but the underlying symmetry breaking and the origin of the CDW remain unclear. We use X-ray diffraction to determine the microscopic structure of the CDWs in an archetypical cuprate YBa2Cu3O6.54 at its superconducting transition temperature ∼ 60 K. We find that the CDWs in this material break the mirror symmetry of the CuO2 bilayers. The ionic displacements in the CDWs have two components, which are perpendicular and parallel to the CuO2 planes, and are out of phase with each other. The planar oxygen atoms have the largest displacements, perpendicular to the CuO2 planes. Our results allow many electronic properties of the underdoped cuprates to be understood. For instance, the CDWs will lead to local variations in the electronic structure, giving an explicit explanation of density-wave states with broken symmetry observed in scanning tunnelling microscopy and soft X-ray measurements.
The Second Threshold Field of Charge-Density-Wave Conductor Rb0.3MoO3 in High Temperature Range
Institute of Scientific and Technical Information of China (English)
LI Da-Hua; XIONG Rui; WANG Jun-Feng; LI Chang-Zhen; YIN Di; YI Fan; TANG Wu-Feng; SHI Jing
2005-01-01
@@ The switching and threshold properties of quasi-one-dimensional charge-density-wave conductor rubidium blue bronze Rb0.3MoO3 single crystals are investigated in a comparative high and large temperature range. Beyond the limit temperature 50 K of Littlewood's theory, even up to about 100K, typical sharp switching to negative or zero differential resistance is observed in E-I characteristic curves. Correspondingly, an obvious switching between two conducting states, from a lowly conducting state to a highly conducting state, is observed in the I-E characteristic curves in the same temperature range. Temperature dependence of the second threshold field ET2 accompanied by this kind of high field switching behaviour is firstly obtained. These new observations are discussed in the mechanism of the current inhomogeneity and redistribution due to the existence of transverse energy barriers suggested by Zhang et al. [Solid State Commun. 85 (1993) 121
Argument for charge density wave sub-phases in the ground state of α-(BEDT-TTF) 2KHg(SCN) 4
Biskup, N.; Perenboom, J. A. A. J.; Brooks, J. S.; Qualls, J. S.
1998-07-01
A resistive anomaly at temperature Tp in the title compound is associated with a Fermi surface reconstruction from a metallic to a (spin or charge) density wave state. At high magnetic fields a corresponding feature in the magnetoresistance above a field BK indicates the breaking of this state. We argue that TP indicates a second order phase line identical to that measured by specific heat methods and show that it decreases monotonically up to 30T. We find that Pauli (rather than orbital) effects, dominate the reduction in Tp. We further argue that BK is a first-order transition between two subphases below Tp. We compare the phase diagram with recent theoretical models for CDW and SDW ground states in high magnetic fields.
DEFF Research Database (Denmark)
Forgan, E.M.; Blackburn, E.; Holmes, A.T.;
2015-01-01
Charge density wave (CDW) order appears throughout the underdoped high-temperature cuprate superconductors, but the underlying symmetry breaking and the origin of the CDW remain unclear. We use X-ray diffraction to determine the microscopic structure of the CDWs in an archetypical cuprate YBa2Cu3O6...... with broken symmetry observed in scanning tunnelling microscopy and soft X-ray measurements........54 at its superconducting transition temperature ∼60 K. We find that the CDWs in this material break the mirror symmetry of the CuO2 bilayers. The ionic displacements in the CDWs have two components, which are perpendicular and parallel to the CuO2 planes, and are out of phase with each other. The planar...
Chen, Runze; Gao, Chaojun; Bu, Kun; Hao, Xiaoyu; Wang, Zichen; Wen, Lianjun; Guo, Juan; Chao, Mingju; Liang, Erjun; Yang, Lihong; Dong, Cheng
2017-02-01
Potassium tungsten bronzes KxWO3 (x=0.20 and 0.22) with the coexistence of charge density wave (CDW) and superconductivity (SC) were prepared from K2WO4, WO3 and W powders using a hybrid microwave method. The structure refinement confirmed that all samples had a pure hexagonal phase with the space group of P63 /mcm. The distortion degree of W-O octahedron declines with x and is independent of synthesis condition for the same x (=0.20). The CDW transition is studied as a function of residual resistivity ratio. By increasing the crystallinity of sample, this transition can be suppressed, which is probably attributed to the interaction between CDW and defects in crystallites. The CDW transition temperature increases with x, which may be related to the decline of the distortion degree of W-O octahedron. The competition between CDW and SC is observed according to the resistivity and magnetization measurements.
Blackburn, E; Chang, J; Hücker, M; Holmes, A T; Christensen, N B; Liang, Ruixing; Bonn, D A; Hardy, W N; Rütt, U; Gutowski, O; von Zimmermann, M; Forgan, E M; Hayden, S M
2013-03-29
X-ray diffraction measurements show that the high-temperature superconductor YBa2Cu3O6.54, with ortho-II oxygen order, has charge-density-wave order in the absence of an applied magnetic field. The dominant wave vector of the charge density wave is q(CDW)=(0,0.328(2),0.5), with the in-plane component parallel to the b axis (chain direction). It has a similar incommensurability to that observed in ortho-VIII and ortho-III samples, which have different dopings and oxygen orderings. Our results for ortho-II contrast with recent high-field NMR measurements, which suggest a commensurate wave vector along the a axis. We discuss the relationship between spin and charge correlations in YBa2Cu3O(y) and recent high-field quantum oscillation, NMR, and ultrasound experiments.
Blackburn, E.; Chang, J.; Hücker, M.; Holmes, A. T.; Christensen, N. B.; Liang, Ruixing; Bonn, D. A.; Hardy, W. N.; Rütt, U.; Gutowski, O.; Zimmermann, M. v.; Forgan, E. M.; Hayden, S. M.
2013-03-01
X-ray diffraction measurements show that the high-temperature superconductor YBa2Cu3O6.54, with ortho-II oxygen order, has charge-density-wave order in the absence of an applied magnetic field. The dominant wave vector of the charge density wave is qCDW=(0,0.328(2),0.5), with the in-plane component parallel to the b axis (chain direction). It has a similar incommensurability to that observed in ortho-VIII and ortho-III samples, which have different dopings and oxygen orderings. Our results for ortho-II contrast with recent high-field NMR measurements, which suggest a commensurate wave vector along the a axis. We discuss the relationship between spin and charge correlations in YBa2Cu3Oy and recent high-field quantum oscillation, NMR, and ultrasound experiments.
Relationship between hole density and charge-ordering wave vector in Sr14-xCaxCu24O41
Rusydi, A.; Berciu, M.; Abbamonte, P.; Smadici, S.; Eisaki, H.; Fujimaki, Y.; Uchida, S.; Ruebhausen, M.; Sawatzky, G. A.
2007-01-01
The distribution of holes in Sr14-xCaxCu24O41 is revisited with semiempirical reanalysis of the x-ray absorption data and exact diagonalization cluster calculations. Another interpretation of the XAS data leads to much larger ladder hole densities than previously suggested. These new hole densities
Krstovska, Danica
2017-02-01
Magnetic field dependence of the thermopower and Nernst effect of the multiband organic conductor α - (BEDT - TTF)2KHg(SCN)4 is theoretically studied at low temperatures in the charge density wave (CDW) state, to fields of 30 T and several field directions. A theoretical model of quantum interlayer tunneling for the q1D charge carriers is used to probe the thermoelectric effects in the CDW state. The contribution from the q2D carriers is calculated by using the Boltzmann transport theory. The background components of the thermopower and Nernst effect as well as the quantum oscillations that originate from the closed Fermi surface orbits are analyzed. The model implies that in the CDW state, the properties of α - (BEDT - TTF)2KHg(SCN)4 are determined mostly by the orbits on the new open Fermi sheets. This is in accord with the previously reported CDW scenario of the low temperature state of α - (BEDT - TTF)2KHg(SCN)4 with imperfect nesting of the open Fermi surface sections.
Kawasaki, Shinji; Tani, Yoshihiko; Mabuchi, Tomosuke; Kudo, Kazutaka; Nishikubo, Yoshihiro; Mitsuoka, Daisuke; Nohara, Minoru; Zheng, Guo-qing
2015-02-01
The relationship between charge-density wave (CDW) orders and superconductivity in arsenide superconductor SrPt2As2 with Tc=5.2 K which crystallizes in the CaBe2Ge2 -type structure was studied by 75As nuclear magnetic resonance (NMR) measurements up to 520 K, and 75As nuclear quadrupole resonance (NQR) and 195Pt-NMR measurements down to 1.5 K. At high temperature, 75As-NMR spectrum and nuclear-spin-relaxation rate (1 /T1) have revealed two distinct CDW orders, one realized in the As-Pt-As layer below TCDWAs (1 )=410 K and the other in the Pt-As-Pt layer below TCDWAs (2 )=255 K . The 1 /T1 measured by 75As-NQR shows a clear Hebel-Slichter peak just below Tc and decreases exponentially well below Tc. Concomitantly, 195Pt Knight shift decreases below Tc. Our results indicate that superconductivity in SrPt2As2 is in the spin-singlet state with an s -wave gap and is robust under the two distinct CDW orders in different layers.
Gabovich, Alexander M.; Voitenko, Alexander I.
2016-10-01
The state of the art concerning tunnel measurements of energy gaps in cuprate oxides has been analyzed. A detailed review of the relevant literature is made, and original results calculated for the quasiparticle tunnel current J(V) between a metallic tip and a disordered d-wave superconductor partially gapped by charge density waves (CDWs) are reported, because it is this model of high-temperature superconductors that becomes popular owing to recent experiments in which CDWs were observed directly. The current was calculated suggesting the scatter of both the superconducting and CDW order parameters due to the samples' intrinsic inhomogeneity. It was shown that peculiarities in the current-voltage characteristics inherent to the case of homogeneous superconducting material are severely smeared, and the CDW-related features transform into experimentally observed peak-dip-hump structures. Theoretical results were used to fit data measured for YBa2Cu3O7-δ and Bi2Sr2CaCu2O8+δ. The fitting demonstrated a good qualitative agreement between the experiment and model calculations. The analysis of the energy gaps in high-Tc superconductors is important both per se and as a tool to uncover the nature of superconductivity in cuprates not elucidated so far despite of much theoretical effort and experimental progress.
Energy Technology Data Exchange (ETDEWEB)
Brouet, V.; Yang, W.L.; Zhou, X.J.; Hussain, Z.; Moore, R.G.; He, R.; Lu, D.H.; Shen, Z.X.; Laverock, J.; Dugdale, S.; Ru, N.; Fisher, I.R.
2010-02-15
We present a detailed ARPES investigation of the RTe{sub 3} family, which sets this system as an ideal 'textbook' example for the formation of a nesting driven Charge Density Wave (CDW). This family indeed exhibits the full range of phenomena that can be associated to CDW instabilities, from the opening of large gaps on the best nested parts of Fermi Surface (FS) (up to 0.4eV), to the existence of residual metallic pockets. ARPES is the best suited technique to characterize these features, thanks to its unique ability to resolve the electronic structure in k-space. An additional advantage of RTe{sub 3} is that the band structure can be very accurately described by a simple 2D tight-binding (TB) model, which allows one to understand and easily reproduce many characteristics of the CDW. In this paper, we first establish the main features of the electronic structure, by comparing our ARPES measurements with Linear Muffin-Tin Orbital band calculations. We use this to define the validity and limits of the TB model. We then present a complete description of the CDW properties and, for the first time, of their strong evolution as a function of R. Using simple models, we are able to reproduce perfectly the evolution of gaps in k-space, the evolution of the CDW wave vector with R and the shape of the residual metallic pockets. Finally, we give an estimation of the CDW interaction parameters and find that the change in the electronic density of states n(Ef), due to lattice expansion when different R ions are inserted, has the correct order of magnitude to explain the evolution of the CDW properties.
Hydrodynamic waves in an anomalous charged fluid
Abbasi, Navid; Davody, Ali; Hejazi, Kasra; Rezaei, Zahra
2016-11-01
We study the collective excitations in a relativistic fluid with an anomalous U (1) current. In 3 + 1 dimensions at zero chemical potential, in addition to ordinary sound modes we find two propagating modes in presence of an external magnetic field. The first one which is a transverse degenerate mode, propagates with a velocity proportional to the coefficient of gravitational anomaly; this is in fact the Chiral Alfvén wave recently found in [1]. Another one is a wave of density perturbation, namely a chiral magnetic wave (CMW). The velocity dependence of CMW on the chiral anomaly coefficient is well known. We compute the dependence of CMW's velocity on the coefficient of gravitational anomaly as well. We also show that the dissipation splits the degeneracy of CAW. At finite chiral charge density we show that in general there may exist five chiral hydrodynamic waves. Of these five waves, one is the CMW while the other four are mixed Modified Sound-Alfvén waves. It turns out that in propagation transverse to the magnetic field no anomaly effect appears while in parallel to the magnetic field we find sound waves become dispersive due to anomaly.
Vucic, Z; Gladic, J; Haas, C; DeBoer, JL
1996-01-01
An X-ray study of the quasi-one-dimensional charge density wave (CDW) system (NbSe4)(10)I-3 as a function of temperature from room temperature down to 130 K has been performed by taking oscillation and zeroth level Weissenberg photographs. A reversible transformation of the room temperature tetragon
Magnetic field controlled charge density wave coupling in underdoped YBa_{2}Cu_{3}O_{6+x}
DEFF Research Database (Denmark)
Chang, J.; Blackburn, E.; Ivashko, O.;
2016-01-01
The application of magnetic fields to layered cuprates suppresses their high-temperature superconducting behaviour and reveals competing ground states. In widely studied underdoped YBa2Cu3O6+x (YBCO), the microscopic nature of field-induced electronic and structural changes at low temperatures...... remains unclear. Here we report an X-ray study of the high-field charge density wave (CDW) in YBCO. For hole dopings ∼ 0.123, we find that a field (B∼10 T) induces additional CDW correlations along the CuO chain (b-direction) only, leading to a three-dimensional (3D) ordered state along this direction...... at B∼15 T. The CDW signal along the a-direction is also enhanced by field, but does not develop an additional pattern of correlations. Magnetic field modifies the coupling between the CuO2 bilayers in the YBCO structure, and causes the sudden appearance of the 3D CDW order. The mirror symmetry...
Hsieh, S H; Solanki, R S; Wang, Y F; Shao, Y C; Lee, S H; Yao, C H; Du, C H; Wang, H T; Chiou, J W; Chin, Y Y; Tsai, H M; Chen, J-L; Pao, C W; Cheng, C-M; Chen, W-C; Lin, H J; Lee, J F; Chou, F C; Pong, W F
2017-12-01
The local electronic and atomic structures of the high-quality single crystal of SrFeO3-δ (δ~0.19) were studied using temperature-dependent x-ray absorption and valence-band photoemission spectroscopy (VB-PES) to investigate the origin of anisotropic resistivity in the ab-plane and along the c-axis close to the region of thermal hysteresis (near temperature for susceptibility maximum, Tm~78 K). All experiments herein were conducted during warming and cooling processes. The Fe L 3,2-edge X-ray linear dichroism results show that during cooling from room temperature to below the transition temperature, the unoccupied Fe 3d e g states remain in persistently out-of-plane 3d 3z(2)-r(2) orbitals. In contrast, in the warming process below the transition temperature, they change from 3d 3z(2)-r(2) to in-plane 3d x(2)-y(2) orbitals. The nearest-neighbor (NN) Fe-O bond lengths also exhibit anisotropic behavior in the ab-plane and along the c-axis below Tm. The anisotropic NN Fe-O bond lengths and Debye-Waller factors stabilize the in-plane Fe 3d x(2)-y(2) and out-of-plane 3d 3z(2)-r(2) orbitals during warming and cooling, respectively. Additionally, a VB-PES study further confirms that a relative band gap opens at low temperature in both the ab-plane and along the c-axis, providing the clear evidence of the charge-density-wave nature of SrFeO3-δ (δ~0.19) single crystal.
Imperfect nesting in unconventional density waves
Dóra, Balázs; Virosztek, Attila; Maki, Kazumi
2002-03-01
Recently, we have shown that unconventional charge density wave (UCDW) is the most likely candidate for the unidentified low-temperature phase (LTP) in α-(ET)2 salts. In particular, UCDW describes reasonably well the temperature dependence of the threshold electric field of LTP in α-(ET)2KHg(SCN)4. Here, we shall show that the imperfect nesting in UCDW is crucial to further improve the theoretical description of the threshold electric field.
Quantum crystallographic charge density of urea
Wall, Michael E.
2015-01-01
Standard X-ray crystallography methods use free-atom models to calculate mean unit-cell charge densities. Real molecules, however, have shared charge that is not captured accurately using free-atom models. To address this limitation, a charge density model of crystalline urea was calculated using high-level quantum theory and was refined against publicly available ultra-high-resolution experimental Bragg data, including the effects of atomic displacement parameters. The resulting quantum crys...
Kang, W.; Osada, T.; Konoike, T.; Uchida, K.
2013-11-01
The stereoscopic angle-dependent magnetoresistance oscillations (AMRO) in an organic conductor α-(BEDT-TTF)2KHg(SCN)4 were measured across the temperature-pressure boundary that separates the charge-density-wave state from the metallic state. The gnomonic projections of the data clearly resolved the contributions from different parts of the Fermi surfaces. The temperature and pressure dependencies of the AMRO results revealed the progressive formation of a quasi-one-dimensional orbit in the charge-density-wave state. The AMRO measurements at ambient pressures and at low temperatures revealed the presence of two sets of quasi-one-dimensional Fermi surfaces. Additional evidence for multiple quasi-one-dimensional orbits was obtained from the data collected in conjunction with the in-plane field rotations.
Charge density fluctuation of low frequency in a dusty plasma
Institute of Scientific and Technical Information of China (English)
李芳; 吕保维; O.Havnes
1997-01-01
The charge density fluctuation of low frequency in a dusty plasma, which is derived from the longitudinal dielectric permittivity of the dusty plasma, has been studied by kinetic theory. The results show that the P value, which describes the relative charge density on the dust in the plasma, and the charging frequency of a dust particle Ωc, which describes the ratio of charge changing of the dust particles, determine the character of the charge density fluctuation of low frequency. For a dusty plasma of P<<1, when the charging frequency Ωc is much smaller than the dusty plasma frequency wd, there is a strong charge density fluctuation which is of character of dust acoustic eigen wave. For a dusty plasma of P>>1, when the frequency Ωc, is much larger than wd there are weaker fluctuations with a wide spectrum. The results have been applied to the ionosphere and the range of radius and density of dust particles is found, where a strong charge density fluctuation of low frequency should exist.
Self-excitation of space charge waves
DEFF Research Database (Denmark)
Lyuksyutov, Sergei; Buchhave, Preben; Vasnetsov, Mikhail
1997-01-01
We report a direct observation of space charge waves in photorefractive crystals with point group 23 (sillenites) based on their penetration into an area with uniform light illumination. It is shown experimentally that the quality factor of the waves increases substantially with respect to what c...... current theory predicts [B. Sturman el al., Appl. Phys. A 55, 235 (1992)]. This results in the appearance of strong spontaneous beams caused by space charge wave self-excitation....
Bonding charge density from atomic perturbations.
Wang, Yi; Wang, William Yi; Chen, Long-Qing; Liu, Zi-Kui
2015-05-15
Charge transfer among individual atoms is the key concept in modern electronic theory of chemical bonding. In this work, we present a first-principles approach to calculating the charge transfer. Based on the effects of perturbations of an individual atom or a group of atoms on the electron charge density, we determine unambiguously the amount of electron charge associated with a particular atom or a group of atoms. We computed the topological electron loss versus gain using ethylene, graphene, MgO, and SrTiO3 as examples. Our results verify the nature of chemical bonds in these materials at the atomic level.
Hydrodynamic Waves in an Anomalous Charged Fluid
Abbasi, Navid; Rezaei, Zahra
2015-01-01
We study the collective excitations in a relativistic fluid with an anomalous conserved charge. In $3+1$ dimensions, in addition to two ordinary sound modes we find two propagating modes in presence of an external magnetic field: one with a velocity proportional to the coefficient of gauge-gravitational anomaly coefficient and the other with a velocity which depends on both chiral anomaly and the gauge gravitational anomaly coefficients. While the former is the Chiral Alfv\\'en wave recently found in arXiv:1505.05444, the latter is a new type of collective excitations originated from the density fluctuations. We refer to these modes as the Type-M and Type-D chiral Alfv\\'en waves respectively. We show that the Type-M Chiral Alfv\\'en mode is split into two chiral Alfv\\'en modes when taking into account the effect of dissipation processes in the fluid. In 1+1 dimensions we find only one propagating mode associated with the anomalous effects. We explicitly compute the velocity of this wave and show that in contras...
Density waves in the organic metal α-(BEDT-TTF) 2KHg(SCN) 4
Kato, Masaru
2003-05-01
We have investigated possible spin and charge density waves in the organic metal α-(BEDT-TTF) 2KHg(SCN) 4. This system shows density wave like transition at T=8 K, and the nature of the density wave is not clarified up to now. Using a realistic tight binding model and an inhomogeneous mean-field theory, we obtained several stable density wave states. Especially, spin density wave states (SDW) are stable only for large on-site Coulomb interaction U⩾400 meV. Their spin moments are tiny and inhomogeneous even in the unit cell. Also charge density wave appears simultaneously with the SDW.
Charge densities and charge noise in mesoscopic conductors
Indian Academy of Sciences (India)
M Büttiker
2002-02-01
We introduce a hierarchy of density of states to characterize the charge distribution in a mesoscopic conductor. At the bottom of this hierarchy are the partial density of states which represent the contribution to the local density of states if both the incident and the out-going scattering channel is prescribed. The partial density of states play a prominent role in measurements with a scanning tunneling microscope on multiprobe conductors in the presence of current ﬂow. The partial density of states determine the degree of dephasing generated by a weakly coupled voltage probe. In addition the partial density of states determine the frequency-dependent response of mesoscopic conductors in the presence of slowly oscillating voltages applied to the contacts of the sample. The partial density of states permit the formulation of a Friedel sum rule which can be applied locally. We introduce the off-diagonal elements of the partial density of states matrix to describe charge ﬂuctuation processes. This generalization leads to a local Wigner–Smith life-time matrix.
Quantum crystallographic charge density of urea.
Wall, Michael E
2016-07-01
Standard X-ray crystallography methods use free-atom models to calculate mean unit-cell charge densities. Real molecules, however, have shared charge that is not captured accurately using free-atom models. To address this limitation, a charge density model of crystalline urea was calculated using high-level quantum theory and was refined against publicly available ultra-high-resolution experimental Bragg data, including the effects of atomic displacement parameters. The resulting quantum crystallographic model was compared with models obtained using spherical atom or multipole methods. Despite using only the same number of free parameters as the spherical atom model, the agreement of the quantum model with the data is comparable to the multipole model. The static, theoretical crystalline charge density of the quantum model is distinct from the multipole model, indicating the quantum model provides substantially new information. Hydrogen thermal ellipsoids in the quantum model were very similar to those obtained using neutron crystallography, indicating that quantum crystallography can increase the accuracy of the X-ray crystallographic atomic displacement parameters. The results demonstrate the feasibility and benefits of integrating fully periodic quantum charge density calculations into ultra-high-resolution X-ray crystallographic model building and refinement.
Quantum crystallographic charge density of urea
Wall, Michael E.
2016-01-01
Standard X-ray crystallography methods use free-atom models to calculate mean unit-cell charge densities. Real molecules, however, have shared charge that is not captured accurately using free-atom models. To address this limitation, a charge density model of crystalline urea was calculated using high-level quantum theory and was refined against publicly available ultra-high-resolution experimental Bragg data, including the effects of atomic displacement parameters. The resulting quantum crystallographic model was compared with models obtained using spherical atom or multipole methods. Despite using only the same number of free parameters as the spherical atom model, the agreement of the quantum model with the data is comparable to the multipole model. The static, theoretical crystalline charge density of the quantum model is distinct from the multipole model, indicating the quantum model provides substantially new information. Hydrogen thermal ellipsoids in the quantum model were very similar to those obtained using neutron crystallography, indicating that quantum crystallography can increase the accuracy of the X-ray crystallographic atomic displacement parameters. The results demonstrate the feasibility and benefits of integrating fully periodic quantum charge density calculations into ultra-high-resolution X-ray crystallographic model building and refinement. PMID:27437111
Quantum crystallographic charge density of urea
Directory of Open Access Journals (Sweden)
Michael E. Wall
2016-07-01
Full Text Available Standard X-ray crystallography methods use free-atom models to calculate mean unit-cell charge densities. Real molecules, however, have shared charge that is not captured accurately using free-atom models. To address this limitation, a charge density model of crystalline urea was calculated using high-level quantum theory and was refined against publicly available ultra-high-resolution experimental Bragg data, including the effects of atomic displacement parameters. The resulting quantum crystallographic model was compared with models obtained using spherical atom or multipole methods. Despite using only the same number of free parameters as the spherical atom model, the agreement of the quantum model with the data is comparable to the multipole model. The static, theoretical crystalline charge density of the quantum model is distinct from the multipole model, indicating the quantum model provides substantially new information. Hydrogen thermal ellipsoids in the quantum model were very similar to those obtained using neutron crystallography, indicating that quantum crystallography can increase the accuracy of the X-ray crystallographic atomic displacement parameters. The results demonstrate the feasibility and benefits of integrating fully periodic quantum charge density calculations into ultra-high-resolution X-ray crystallographic model building and refinement.
Institute of Scientific and Technical Information of China (English)
Wang Hong-Tao; Li Lin-Jun; Ye De-shu; Cheng Xin-Hong; Xu Zhu-An
2007-01-01
Single crystals of Te-doped dichalcogenides 2H-NbSe2-χTeχ(χ=0,0.10,0.20)were grown by vapour transport method.The effect of Te doping on the superconducting and charge-density wave(CDW)transitions has been investigated.The sharp decrease of residual resistance ratio,RRR=R(300K)/R(8K),with increasing Te content was observed,indicating that the disorder in the conducting plane is induced by Te doping.Meanwhile the superconducting transition temperature,Tc,decreases monotonically with Te content.However,the CDW transition temperature,TCDW,shown by a small jump in the temperature dependence of the resistivity near 30 K,increases slightly.The results show that the suppression of superconductivity might be caused by the enhancement of CDW ordering.The disorder has little influence on the CDW ordering.
ULF Waves and Diffusive Radial Transport of Charged Particles
Ali, Ashar Fawad
The Van Allen radiation belts contain highly energetic particles which interact with a variety of plasma and magnetohydrodynamic (MHD) waves. Waves in the ultra low-frequency (ULF) range play an important role in the loss and acceleration of energetic particles. Considering the geometry of the geomagnetic field, charged particles trapped in the inner magnetosphere undergo three distinct types of periodic motions; an adiabatic invariant is associated with each type of motion. The evolution of the phase space density of charged particles in the magnetosphere in the coordinate space of the three adiabatic invariants is modeled by the Fokker-Planck equation. If we assume that the first two adiabatic invariants are conserved while the third invariant is violated, then the general Fokker-Planck equation reduces to a radial diffusion equation with the radial diffusion coefficient quantifying the rate of the radial diffusion of charged particles, including contributions from perturbations in both the magnetic and the electric fields. This thesis investigates two unanswered questions about ULF wave-driven radial transport of charged particles. First, how important are the ULF fluctuations in the magnetic field compared with the ULF fluctuations in the electric field in driving the radial diffusion of charged particles in the Earth's inner magnetosphere? It has generally been accepted that magnetic field perturbations dominate over electric field perturbations, but several recently published studies suggest otherwise. Second, what is the distribution of ULF wave power in azimuth, and how does ULF wave power depend upon radial distance and the level of geomagnetic activity? Analytic treatments of the diffusion coefficients generally assume uniform distribution of power in azimuth, but in situ measurements suggest that this may not be the case. We used the magnetic field data from the Combined Release and Radiation Effects Satellite (CRRES) and the electric and the magnetic
Density waves in the organic metal {alpha}-(BEDT-TTF){sub 2}KHg(SCN){sub 4}
Energy Technology Data Exchange (ETDEWEB)
Kato, Masaru
2003-05-01
We have investigated possible spin and charge density waves in the organic metal {alpha}-(BEDT-TTF){sub 2}KHg(SCN){sub 4}. This system shows density wave like transition at T=8 K, and the nature of the density wave is not clarified up to now. Using a realistic tight binding model and an inhomogeneous mean-field theory, we obtained several stable density wave states. Especially, spin density wave states (SDW) are stable only for large on-site Coulomb interaction U{>=}400 meV. Their spin moments are tiny and inhomogeneous even in the unit cell. Also charge density wave appears simultaneously with the SDW.
An experimental charge density of HEPES.
Sledź, Paweł; Kamiński, Radosław; Chruszcz, Maksymilian; Zimmerman, Matthew D; Minor, Wladek; Woźniak, Krzysztof
2010-08-01
We report the experimental charge density of HEPES [4-(2-hydroxyethyl)-1-piperazineethanesulfonic acid], which is a common buffering agent. The structure was refined using the Hansen-Coppens formalism. The ability of the HEPES molecule to form stable intermolecular interactions and intermolecular hydrogen bonds in the crystal structure is discussed in terms of its buffering properties. The protonation mode observed in the crystal structure is different from that expected in solution, suggesting that additional factors must be taken into consideration in order to explain the solution properties of the compound. As ordered HEPES molecules are found in the active sites of proteins in several protein crystal structures, our results will allow for quantitative analysis of the electrostatic potential of the interacting surfaces of those proteins.
Charge Exchange Effect on Space-Charge-Limited Current Densities in Ion Diode
Institute of Scientific and Technical Information of China (English)
石磊
2002-01-01
The article theoretically studied the charge-exchange effects on space charge limited electron and ion current densities of non-relativistic one-dimensional slab ion diode, and compared with those of without charge exchange.
Density shock waves in confined microswimmers
Tsang, Alan Cheng Hou
2015-01-01
Motile and driven particles confined in microfluidic channels exhibit interesting emergent behavior from propagating density bands to density shock waves. A deeper understanding of the physical mechanisms responsible for these emergent structures is relevant to a number of physical and biomedical applications. Here, we study the formation of density shock waves in the context of an idealized model of microswimmers confined in a narrow channel and subject to a uniform external flow. Interestingly, these density shock waves exhibit a transition from `subsonic' with compression at the back to `supersonic' with compression at the front of the population as the intensity of the external flow increases. This behavior is the result of a non-trivial interplay between hydrodynamic interactions and geometric confinement, and is confirmed by a novel quasilinear wave model that properly captures the dependence of the shock formation on the external flow. These findings can be used to guide the development of novel mechan...
Schaper, Danielle; McElroy, Kyle; Calleja, Eduardo; Dai, Jixia; Li, Lijun; Lu, Wenjian; Sun, Yuping; Zhu, Xiangde
2014-03-01
Charged ordered states are becoming a common feature in the phase diagrams of correlated materials. In many cased there are indications that doping controlled quantum critical points between the CO state and others are related to interesting properties including superconductivity. An interesting test case is the ordered 2D CDW found in the transition metal dichalcogenides. We performed an analytical study on the dichalcogenides tantalum disulfide (TaS2) and tantalum diselenide (TaSe2) to observe how CDWs present in the material can be melted as disorder is introduced into the system via copper doping. Data was taken using a scanning tunneling microscope (STM) below the transition to the CDW state, both with and without copper dopants added. The resulting topographs were then analyzed to investigate the relationship between the phase and the amplitude of the disordered CDW. We found that the copper doping caused disorder in the CDW state characterized by phase wanderings and 2 π phase winding ``point defects'' in the CDW not present in the undoped parent compound. The locations of these point defects and windings were, in turn, found to have the characteristics of topological defects. Implications for studies of other disordered CO states seen in STM will be discussed.
Institute of Scientific and Technical Information of China (English)
董宇兵; 王翼展
2011-01-01
The transverse charge density of pions is calculated based on relativistic quantum mechanics, where the pion is regarded as a quark-antiquark bound state. Corrections from the two spin-1/2 constituents and from the wave function of a quark and antiquark i
Orbital symmetry of charge-density-wave order in La1.875Ba0.125CuO4 and YBa2Cu3O6.67
Achkar, A. J.; He, F.; Sutarto, R.; McMahon, Christopher; Zwiebler, M.; Hücker, M.; Gu, G. D.; Liang, Ruixing; Bonn, D. A.; Hardy, W. N.; Geck, J.; Hawthorn, D. G.
2016-06-01
Recent theories of charge-density-wave (CDW) order in high-temperature superconductors have predicted a primarily d CDW orbital symmetry. Here, we report on the orbital symmetry of CDW order in the canonical cuprate superconductors La1.875Ba0.125CuO4 (LBCO) and YBa2Cu3O6.67 (YBCO), using resonant soft X-ray scattering and a model mapped to the CDW orbital symmetry. From measurements sensitive to the O sublattice, we conclude that LBCO has predominantly s' CDW orbital symmetry, in contrast to the d orbital symmetry recently reported in other cuprates. Furthermore, we show for YBCO that the CDW orbital symmetry differs along the a and b crystal axes and that these both differ from LBCO. This work highlights CDW orbital symmetry as an additional key property that distinguishes the different cuprate families. We discuss how the CDW symmetry may be related to the `1/8-anomaly’ and to static spin ordering.
He, Xiao; Ryu, Shinsei; Hirata, So
2014-01-14
Finite-temperature extensions of ab initio Gaussian-basis-set spin-restricted Hartree-Fock (HF) and second-order many-body perturbation (MP2) theories are implemented for infinitely extended, periodic, one-dimensional solids and applied to the Peierls and charge-density-wave (CDW) transitions in polyyne and all-trans polyacetylene. The HF theory predicts insulating CDW ground states for both systems in their equidistant structures at low temperatures. In the same structures, they turn metallic at high temperatures. Starting from the "dimerized" low-temperature equilibrium structures, the systems need even higher temperatures to undergo a Peierls transition, which is accompanied by geometric as well as electronic distortions from dimerized to non-dimerized forms. The conventional finite-temperature MP2 theory shows a sign of divergence in any phase at any nonzero temperature and is useless. The renormalized finite-temperature MP2 (MP2R) theory is divergent only near metallic electronic structures, but is well behaved elsewhere. MP2R also predicts CDW and Peierls transitions occurring at two different temperatures. The effect of electron correlation is primarily to lower the Peierls transition temperature.
Quantum coherent switch utilizing commensurate nanoelectrode and charge density periodicities
Harrison, Neil; Singleton, John; Migliori, Albert
2008-08-05
A quantum coherent switch having a substrate formed from a density wave (DW) material capable of having a periodic electron density modulation or spin density modulation, a dielectric layer formed onto a surface of the substrate that is orthogonal to an intrinsic wave vector of the DW material; and structure for applying an external spatially periodic electrostatic potential over the dielectric layer.
Unconventional Density Waves in Organic Conductors and in Superconductors
Maki, K.; Dóra, B.; Virosztek, A.
Unconventional density waves (UDW) are one of the ground states in metallic crystalline solids and have been speculated already in 1968. However, more focused studies on UDWstarted only recently, perhaps after the identification of the low temperature phase in α-(BEDT-TTF)2KHg(SCN)4 as unconventional charge density wave (UCDW) in 2002. More recently, the metallic phase of Bechgaard salts (TMTSF)2X with X=PF6 and ReO4 under both pressure and magnetic field appears to be unconventional spin density wave (USDW). The pseudogap regime of high T c superconductors LSCO, YBCO, Bi2212 and the one in CeCoIn5 belong to d-wave density waves (d-DW). In these identifications, the angular dependent magnetoresistance and the giant Nernst effect have played the crucial role. These are the simplest manifestations of the Landau quantization of quasiparticle energy in UDW in the presence of magnetic field (the Nersesyan effect). Also we speculate that UDW will be most likely found in α-(BEDT-TTF)2I3, α-(BEDT-TTF)2I2Br, κ-(BEDT-TTF)2Cu(NCS)2, κ-(BEDT-TTF)2Cu(CN)2Br, γ-(BEDT)2GaCl4 and in many other organic compounds.
Charge-Confining Gravitational Electrovacuum Shock Wave
Guendelman, Eduardo; Pacheva, Svetlana
2013-01-01
In previous publications we have extensively studied spherically symmetric solutions of gravity coupled to a non-standard type of non-linear electrodynamics containing a square root of the ordinary Maxwell Lagrangian (the latter is known to yield QCD-like confinement in flat space-time). A class of these solutions describe non-standard black holes of Reissner-Nordstroem-(anti-)-de-Sitter type with an additional constant radial vacuum electric field, in particular, a non-asymptotically flat Reissner-Nordstroem-type black hole. Here we study the ultra-relativistic boost (Aichelburg-Sexl-type) limit of the latter and show that, unlike the ordinary Reissner-Nordstroem case, we obtain a gravitational electrovacuum shock wave as a result of the persistence of the gauge field due to the "square-root" Maxwell Lagrangian term. Next, we show that this gravitational electrovacuum shock wave confines charged test particles (both massive and massless) within a finite distance from its front.
Wave Beam Propagation Through Density Fluctuations
Balakin, A. A.; Bertelli, N.; Westerhof, E.
2011-01-01
Perturbations induced by edge density fluctuations on electron cyclotron wave beams propagating in fusion plasmas are studied by means of a quasi-optical code. The effects of such fluctuations are illustrated here by showing the beam propagation in the case of single harmonic perturbations to the wa
Fluxon density waves in long Josephson junctions
DEFF Research Database (Denmark)
Olsen, O. H.; Ustinov, A. V.; Pedersen, Niels Falsig
1993-01-01
Numerical simulations of the multiple fluxon dynamics stimulated by an external oscillating force applied at a boundary of a long Josephson junction are presented. The calculated IV characteristics agree well with a recent experimental observation of rf-induced satellite flux-flow steps. The volt...... density waves....
Oblique interactions of dust density waves
Energy Technology Data Exchange (ETDEWEB)
Wang, Zhelchui [Los Alamos National Laboratory; Li, Yang - Fang [MAX-PLANCK INSTITUTE; Hou, Lujing [MAX-PLANCK INSTITUTE; Jiang, Ke [MAX-PLANCK INSTITUTE; Wu, De - Jin [CHINA; Thomas, Hubertus M [MAX-PLANCK INSTITUTE; Morfill, Gregor E [MAX-PLANCK INSTITUTE
2010-01-01
Self-excited dust density waves (DDWs) are studied in a striped electrode device. In addition to the usual perpendicularly (with respect to the electrode) propagating DDWs, which have been frequently observed in dusty plasma experiments on the ground, a low-frequency oblique mode is also observed. This low-frequency oblique DDW has a frequency much lower than the dust plasma frequency and its spontaneous excitation is observed even with a very low dust density. It is found that the low-frequency oblique mode can exist either separately or together with the usual perpendicular mode. In the latter case, a new mode arises as a result of the interactions between the perpendicular and the oblique modes. The experiments show that these three modes satisfy the wave coupling conditions in both the frequencies and the wave-vectors.
Drozdova, Olga; Yakushi, Kyuya; Yamamoto, Kaoru; Ota, Akira; Yamochi, Hideki; Saito, Gunzi; Tashiro, Hidenori; Tanner, David B.
2004-08-01
We present the electronic and vibrational spectra of quasi-one-dimensional (3)/(4) -filled (EDO-TTF)2X ( EDO-TTF=ethylenedioxy-tetrathiafulvalene , X=PF6 and AsF6 ) above and below the metal-insulator phase transition ( TMI=280K for the PF6 salt and 268K for the AsF6 salt). For the low-temperature insulating phase, the pattern of both bond and charge order was identified. Almost all charge density is localized on the strongly bound central pair of 0110 tetramer giving rise to a characteristic spectrum of electronic excitations. Infrared spectra along the stacking axis show evidence of strong electron-molecular vibration coupling between the charge transfer band within the pair and some specific intramolecular vibrations. This charge order is assisted by a molecular deformation.
Space-Charge Waves and Instabilities in Intense Beams
Wang, J. G.
1997-11-01
Advancced accelerator applications, such as drivers for heavy ion inertial fusion, high-intensity synchrotrons for spallation neutron sources, high energy boosters, free electron lasers, high-power microwave generators, etc., require ever-increasing beam intensity. An important beam dynamics issue in such beams is the collective behavior of charged particles due to their space charge effects. This includes the phenomena of space-charge waves and instabilities excited on beams by external perturbations. It is very crucial to fully understand these phenomena in order to develop advanced accelerators for various applications. At the University of Maryland we have been conducting experimental programs to study space-charge waves and longitudinal instabilities by employing low-energy, high-current, space-charge dominated electron beams. Localized perturbations on the beams are generated from a gridded electron gun. In a conducting transport channel focused by short solenoids, these perturbations evolve into space-charge waves propagating on the beams. The wave speed is measured and many beam parameters are determined with this technique. The reflection of space-charge waves at the shoulder of an initially rectangular beam bunch is also observed. In a resistive-wall channel focused by a uniform long solenoid, the space-charge waves suffer longitudinal instability. The properties of the instabilities are studied in detail in the long wavelength range. In this talk we review our experimental results on the waves and instabilities and compare with theory.
Fast magnetohydrodynamic density waves in spiral galaxies
Lou, Yu-Qing; Han, J. L.; Fan, Zuhui
1999-09-01
The newly observed large-scale structures of a southern grand-design spiral galaxy NGC 2997 in total and polarized radio-continuum emission together with their overall correlations with the known optical spiral structure are physically interpreted in terms of fast magnetohydrodynamic (MHD) density waves in contrast to slow MHD density waves in NGC 6946. The global spiral pattern of such fast MHD density waves extends from the very centre, where the disc rotates almost rigidly within ~0.5arcmin, all the way to the outer disc with a more or less flat rotation curve. To strengthen the case, several known features of spiral galaxies M51 and IC 342 are referred to and their pattern identifications discussed. It is emphasized that the nature of a magnetized spiral galaxy would be much better appreciated by examining large-scale structures in optical, atomic hydrogen Hi, total and polarized radio-continuum and infrared emission together. As various star-formation processes occur concurrently and/or sequentially in spiral arms of high gas concentration, relatively broad and fuzzy Hi arms, roughly coincident with optical arms in the inner disc, are expected to extend from the extremities of fading optical arms further into the outer gas disc. We predict that the south-east `magnetic arm', apparently isolated from any optical features, in total and polarized radio-continuum intensity maps of NGC 2997 should be associated with an Hi gas arm yet to be detected in 21-cm line emission.
Dust charge fluctuation effects on Langmuir waves with kappa distributed electrons
Jamshidi, M.; Rouhani, M. R.; Hakimi Pajouh, H.
2016-03-01
Using a kinetic description, dust charge fluctuations due to the inelastic collisions between dust particles and plasma particles are studied in unmagnetized dusty plasmas. Most astrophysical and space plasmas are observed to have non-Maxwellian high energy tail. Therefore, a kappa distribution for electrons in the equilibrium is assumed. The dispersion relation and damping rates for Langmuir waves are obtained. Considering the dust charge fluctuations increases the damping rate of Langmuir waves. It is shown that the damping rate of Langmuir waves depends on the spectral index and the dust density parameter.
WSN-Based Space Charge Density Measurement System.
Deng, Dawei; Yuan, Haiwen; Lv, Jianxun; Ju, Yong
2017-01-01
It is generally acknowledged that high voltage direct current (HVDC) transmission line endures the drawback of large area, because of which the utilization of cable for space charge density monitoring system is of inconvenience. Compared with the traditional communication network, wireless sensor network (WSN) shows advantages in small volume, high flexibility and strong self-organization, thereby presenting great potential in solving the problem. Additionally, WSN is more suitable for the construction of distributed space charge density monitoring system as it has longer distance and higher mobility. A distributed wireless system is designed for collecting and monitoring the space charge density under HVDC transmission lines, which has been widely applied in both Chinese state grid HVDC test base and power transmission projects. Experimental results of the measuring system demonstrated its adaptability in the complex electromagnetic environment under the transmission lines and the ability in realizing accurate, flexible, and stable demands for the measurement of space charge density.
Wave induced density modification in RF sheaths and close to wave launchers
Van Eester, D.; Crombé, K.; Lu, Ling-Feng
2015-12-01
With the return to full metal walls - a necessary step towards viable fusion machines - and due to the high power densities of current-day ICRH (Ion Cyclotron Resonance Heating) or RF (radio frequency) antennas, there is ample renewed interest in exploring the reasons for wave-induced sputtering and formation of hot spots. Moreover, there is experimental evidence on various machines that RF waves influence the density profile close to the wave launchers so that waves indirectly influence their own coupling efficiency. The present study presents a return to first principles and describes the wave-particle interaction using a 2-time scale model involving the equation of motion, the continuity equation and the wave equation on each of the time scales. Through the changing density pattern, the fast time scale dynamics is affected by the slow time scale events. In turn, the slow time scale density and flows are modified by the presence of the RF waves through quasilinear terms. Although finite zero order flows are identified, the usual cold plasma dielectric tensor - ignoring such flows - is adopted as a first approximation to describe the wave response to the RF driver. The resulting set of equations is composed of linear and nonlinear equations and is tackled in 1D in the present paper. Whereas the former can be solved using standard numerical techniques, the latter require special handling. At the price of multiple iterations, a simple 'derivative switch-on' procedure allows to reformulate the nonlinear problem as a sequence of linear problems. Analytical expressions allow a first crude assessment - revealing that the ponderomotive potential plays a role similar to that of the electrostatic potential arising from charge separation - but numerical implementation is required to get a feeling of the full dynamics. A few tentative examples are provided to illustrate the phenomena involved.
Wave induced density modification in RF sheaths and close to wave launchers
Energy Technology Data Exchange (ETDEWEB)
Van Eester, D., E-mail: d.van.eester@fz-juelich.de [Laboratory for Plasma Physics, ERM/KMS, EUROfusion Consortium Member, Brussels (Belgium); Crombé, K. [Laboratory for Plasma Physics, ERM/KMS, EUROfusion Consortium Member, Brussels (Belgium); Department of Applied Physics, Ghent University, Ghent (Belgium); Lu, Ling-Feng [CEA, IRFM, F-13108 Saint-Paul-Lez-Durance (France)
2015-12-10
With the return to full metal walls - a necessary step towards viable fusion machines - and due to the high power densities of current-day ICRH (Ion Cyclotron Resonance Heating) or RF (radio frequency) antennas, there is ample renewed interest in exploring the reasons for wave-induced sputtering and formation of hot spots. Moreover, there is experimental evidence on various machines that RF waves influence the density profile close to the wave launchers so that waves indirectly influence their own coupling efficiency. The present study presents a return to first principles and describes the wave-particle interaction using a 2-time scale model involving the equation of motion, the continuity equation and the wave equation on each of the time scales. Through the changing density pattern, the fast time scale dynamics is affected by the slow time scale events. In turn, the slow time scale density and flows are modified by the presence of the RF waves through quasilinear terms. Although finite zero order flows are identified, the usual cold plasma dielectric tensor - ignoring such flows - is adopted as a first approximation to describe the wave response to the RF driver. The resulting set of equations is composed of linear and nonlinear equations and is tackled in 1D in the present paper. Whereas the former can be solved using standard numerical techniques, the latter require special handling. At the price of multiple iterations, a simple ’derivative switch-on’ procedure allows to reformulate the nonlinear problem as a sequence of linear problems. Analytical expressions allow a first crude assessment - revealing that the ponderomotive potential plays a role similar to that of the electrostatic potential arising from charge separation - but numerical implementation is required to get a feeling of the full dynamics. A few tentative examples are provided to illustrate the phenomena involved.
Six Decades of Spiral Density Wave Theory
Shu, Frank H.
2016-09-01
The theory of spiral density waves had its origin approximately six decades ago in an attempt to reconcile the winding dilemma of material spiral arms in flattened disk galaxies. We begin with the earliest calculations of linear and nonlinear spiral density waves in disk galaxies, in which the hypothesis of quasi-stationary spiral structure (QSSS) plays a central role. The earliest success was the prediction of the nonlinear compression of the interstellar medium and its embedded magnetic field; the earliest failure, seemingly, was not detecting color gradients associated with the migration of OB stars whose formation is triggered downstream from the spiral shock front. We give the reasons for this apparent failure with an update on the current status of the problem of OB star formation, including its relationship to the feathering substructure of galactic spiral arms. Infrared images can show two-armed, grand design spirals, even when the optical and UV images show flocculent structures. We suggest how the nonlinear response of the interstellar gas, coupled with overlapping subharmonic resonances, might introduce chaotic behavior in the dynamics of the interstellar medium and Population I objects, even though the underlying forces to which they are subject are regular. We then move to a discussion of resonantly forced spiral density waves in a planetary ring and their relationship to the ideas of disk truncation, and the shepherding of narrow rings by satellites orbiting nearby. The back reaction of the rings on the satellites led to the prediction of planet migration in protoplanetary disks, which has had widespread application in the exploding data sets concerning hot Jupiters and extrasolar planetary systems. We then return to the issue of global normal modes in the stellar disk of spiral galaxies and its relationship to the QSSS hypothesis, where the central theoretical concepts involve waves with negative and positive surface densities of energy and angular
Superconducting pairing and density-wave instabilities in quasi-one-dimensional conductors
Nickel, J. C.; Duprat, R.; Bourbonnais, C.; Dupuis, N.
2006-04-01
Using a renormalization group approach, we determine the phase diagram of an extended quasi-one-dimensional electron gas model that includes interchain hopping, nesting deviations, and both intrachain and interchain repulsive interactions. d -wave superconductivity, which dominates over the spin-density-wave (SDW) phase at large nesting deviations, becomes unstable to the benefit of a triplet f -wave phase for a weak repulsive interchain backscattering term g1⊥>0 , despite the persistence of dominant SDW correlations in the normal state. Antiferromagnetism becomes unstable against the formation of a charge-density-wave state when g1⊥ exceeds some critical value. While these features persist when both Umklapp processes and interchain forward scattering (g2⊥) are taken into account, the effect of g2⊥ alone is found to frustrate nearest-neighbor interchain d - and f -wave pairing and instead favor next-nearest-neighbor interchain singlet or triplet pairing. We argue that the close proximity of SDW and charge-density-wave phases, singlet d -wave, and triplet f -wave superconducting phases in the theoretical phase diagram provides a possible explanation for recent puzzling experimental findings in the Bechgaard salts, including the coexistence of SDW and charge-density-wave phases and the possibility of a triplet pairing in the superconducting phase.
Observational Confirmations of Spiral Density Wave Theory
Kennefick, Julia D.; Kennefick, Daniel; Shameer Abdeen, Mohamed; Berrier, Joel; Davis, Benjamin; Fusco, Michael; Pour Imani, Hamed; Shields, Doug; DMS, SINGS
2017-01-01
Using two techniques to reliably and accurately measure the pitch angles of spiral arms in late-type galaxies, we have compared pitch angles to directly measured black hole masses in local galaxies and demonstrated a strong correlation between them. Using the relation thus established we have developed a pitch angle distribution function of a statistically complete volume limited sample of nearby galaxies and developed a central black hole mass function for nearby spiral galaxies.We have further shown that density wave theory leads us to a three-way correlation between bulge mass, pitch angle, and disk gas density, and have used data from the Galaxy Disk Mass Survey to confirm this possible fundamental plane. Density wave theory also predicts that the pitch angle of spiral arms should change with observed waveband as each waveband is sampling a different stage in stellar population formation and evolution. We present evidence that this is indeed the case using a sample of galaxies from the Spitzer Infrared Nearby Galaxy Survey. Furthermore, the evolved spiral arms cross at the galaxy co-rotation radius. This gives a new method for determining the co-rotation radius of spiral galaxies that is found to agree with those found using previous methods.
Charge and spin fluctuations in the density functional theory
Energy Technology Data Exchange (ETDEWEB)
Gyoerffy, B.L.; Barbieri, A. (Bristol Univ. (UK). H.H. Wills Physics Lab.); Staunton, J.B. (Warwick Univ., Coventry (UK). Dept. of Physics); Shelton, W.A.; Stocks, G.M. (Oak Ridge National Lab., TN (USA))
1990-01-01
We introduce a conceptual framework which allow us to treat charge and spin fluctuations about the Local density Approximation (LDA) to the Density Functional Theory (DFT). We illustrate the approach by explicit study of the Disordered Local Moment (DLM) state in Fe above the Curie Temperature {Tc} and the Mott insulating state in MnO. 27 refs., 6 figs.
Do plasma proteins distinguish between liposomes of varying charge density?
Capriotti, Anna Laura
2012-03-01
Cationic liposomes (CLs) are one of the most employed nonviral nanovector systems in gene therapy. However, their transfection efficiency is strongly affected by interactions with plasma components, that lead to the formation of a "protein corona" onto CL surface. The interactions between nanoparticles entering the body and biomolecules have an essential role for their biodistribution. Because the knowledge of proteins adsorbed onto vector surface could be useful in the screening of new, more efficient and more biocompatible liposomal formulations, the behavior of three CLs with different membrane charge densities was investigated. The proteins of the three coronas were identified by nano-liquid chromatography-tandem mass spectrometry, and quantified with label-free spectral counting strategy. Fibrinogen displayed higher association with CLs with high membrane charge density, while apolipoproteins and C4b-binding protein with CLs with low membrane charge density. These results are discussed in terms of the different lipid compositions of CLs and may have a deep biological impact for in vivo applications. Surface charge of nanoparticles is emerging as a relevant factor determining the corona composition after interaction with plasma proteins. Remarkably, it is also shown that the charge of the protein corona formed around CLs is strongly related to their membrane charge density. © 2012 Elsevier B.V.
The effect of polymer charge density and charge distribution on the formation of multilayers
Voigt, U; Tauer, K; Hahn, M; Jäger, W; Klitzing, K V
2003-01-01
Polyelectrolyte multilayers which are built up by alternating adsorption of polyanions and polycations from aqueous solutions at a solid interface are investigated by reflectometry and ellipsometry. Below a degree of charge of about 70% the adsorption stops after a certain number of dipping cycles and no multilayer formation occurs. This indicates an electrostatically driven adsorption process. Below a charge density of 70% an adsorption can take place if the charged segments are combined as a block of the polymer.
Investigation of microalgae with photon density waves
Frankovitch, Christine; Reich, Oliver; Löhmannsröben, Hans-Gerd
2007-09-01
Phototropic microalgae have a large potential for producing valuable substances for the feed, food, cosmetics, pigment, bioremediation, and pharmacy industries as well as for biotechnological processes. Today it is estimated that the microalgal aquaculture worldwide production is 5000 tons of dry matter per year (not taking into account processed products) making it an approximately $1.25 billion U.S. per year industry. For effective observation of the photosynthetic growth processes, fast on-line sensor systems that analyze the relevant biological and technical process parameters are preferred. The optical properties of the microalgae culture influence the transport of light in the photobioreactor and can be used to extract relevant information for efficient cultivation practices. Microalgae cultivation media show a combination of light absorption and scattering, which are influenced by the concentrations and the physical and chemical properties of the different absorbing and scattering species (e.g. pigments, cell components, etc.). Investigations with frequency domain photon density waves (PDW) allow for the examination of absorption and scattering properties of turbid media, namely the absorption and reduced scattering coefficient. The reduced scattering coefficient can be used to characterize physical and morphological properties of the medium, including the cell concentration, whereas the absorption coefficient correlates with the pigment content. Nannochloropsis oculata, a single-cell species of microalgae, were examined in a nutrient solution with photon density waves. The absorption and reduced scattering coefficients were experimentally determined throughout the cultivation process, and applied to gain information about the cell concentration and average cell radius.
Stopping power of charged particles due to ion wave excitations
Nitta, H.; Muroki, C.; Nambu, M.
2002-08-01
Stopping power due to ion wave excitations is derived for a charged particle moving in a two-component plasma. Unlike previous theories based on ion-acoustic-wave approximation (IAWA), the excitation of short-wavelength ion waves is taken into account. The obtained stopping power has a magnitude larger than that of IAWA. Stopping power at subsonic velocities, where stopping power in IAWA disappears, is even larger than that of supersonic velocities.
Stopping power of charged particles due to ion wave excitations.
Nitta, H; Muroki, C; Nambu, M
2002-08-01
Stopping power due to ion wave excitations is derived for a charged particle moving in a two-component plasma. Unlike previous theories based on ion-acoustic-wave approximation (IAWA), the excitation of short-wavelength ion waves is taken into account. The obtained stopping power has a magnitude larger than that of IAWA. Stopping power at subsonic velocities, where stopping power in IAWA disappears, is even larger than that of supersonic velocities.
Nuclear charge radii: Density functional theory meets Bayesian neural networks
Utama, Raditya; Piekarewicz, Jorge
2016-01-01
The distribution of electric charge in atomic nuclei is fundamental to our understanding of the complex nuclear dynamics and a quintessential observable to validate nuclear structure models. We explore a novel approach that combines sophisticated models of nuclear structure with Bayesian neural networks (BNN) to generate predictions for the charge radii of thousands of nuclei throughout the nuclear chart. A class of relativistic energy density functionals is used to provide robust predictions for nuclear charge radii. In turn, these predictions are refined through Bayesian learning for a neural network that is trained using residuals between theoretical predictions and the experimental data. Although predictions obtained with density functional theory provide a fairly good description of experiment, our results show significant improvement (better than 40%) after BNN refinement. Moreover, these improved results for nuclear charge radii are supplemented with theoretical error bars. We have successfully demonst...
Contributions of charge-density research to medicinal chemistry
Directory of Open Access Journals (Sweden)
Birger Dittrich
2014-11-01
Full Text Available This article reviews efforts in accurate experimental charge-density studies with relevance to medicinal chemistry. Initially, classical charge-density studies that measure electron density distribution via least-squares refinement of aspherical-atom population parameters are summarized. Next, interaction density is discussed as an idealized situation resembling drug–receptor interactions. Scattering-factor databases play an increasing role in charge-density research, and they can be applied both to small-molecule and macromolecular structures in refinement and analysis; software development facilitates their use. Therefore combining both of these complementary branches of X-ray crystallography is recommended, and examples are given where such a combination already proved useful. On the side of the experiment, new pixel detectors are allowing rapid measurements, thereby enabling both high-throughput small-molecule studies and macromolecular structure determination to higher resolutions. Currently, the most ambitious studies compute intermolecular interaction energies of drug–receptor complexes, and it is recommended that future studies benefit from recent method developments. Selected new developments in theoretical charge-density studies are discussed with emphasis on its symbiotic relation to crystallography.
Indian Academy of Sciences (India)
K B Joshi; Nishant N Patel
2008-02-01
Charge density calculations and electronic band structures for GaAl1- = 1.0, 0.5 and 0.0 are presented in this work. The calculations are performed using the empirical pseudopotential method. The charge density is computed for a number of planes, i.e. = 0:0, 0.125 and 0.25 0 by generating the potential through a number of potential parameters available in the literature. The virtual crystal approximation was applied for the semiconducting alloy. The characteristics of the band structure and charge density are observed to be affected by the potential parameters. Calculated band gaps and the nature of gaps are in good agreement with the experimental data reported. The ionicity is also reasonably in good agreement with other scales proposed in the literature; however the formulation needs to be improved. The present work also demands indirect experimental band gap for the alloy.
Millimeter Wave Scattering from Neutral and Charged Water Droplets
Heifetz, Alexander; Liao, Shaolin; Gopalsami, N Sami; Raptis, A C Paul
2010-01-01
We investigated 94GHz millimeter wave (MMW) scattering from neutral and charged water mist produced in the laboratory with an ultrasonic atomizer. Diffusion charging of the mist was accomplished with a negative ion generator (NIG). We observed increased forward and backscattering of MMW from charged mist, as compared to MMW scattering from an uncharged mist. In order to interpret the experimental results, we developed a model based on classical electrodynamics theory of scattering from a dielectric sphere with diffusion-deposited mobile surface charge. In this approach, scattering and extinction cross-sections are calculated for a charged Rayleigh particle with effective dielectric constant consisting of the volume dielectric function of the neutral sphere and surface dielectric function due to the oscillation of the surface charge in the presence of applied electric field. For small droplets with (radius smaller than 100nm), this model predicts increased MMW scattering from charged mist, which is qualitative...
Institute of Scientific and Technical Information of China (English)
LIU Jian; CHU Yan-Yun; REN Zhong-Zhou; WANG Zai-Jun
2012-01-01
The charge form factors of elastic electron scattering for isotones with N =20 and N =28 are calculated using the phase-shift analysis method,with corresponding charge density distributions from relativistic mean-field theory.The results show that there are sharp variations at the inner parts of charge distributions with the proton number decreasing.The corresponding charge form factors are divided into two groups because of the unique properties of the s-states wave functions,though the proton numbers change uniformly in two isotonic chains.Meanwhile,the shift regularities of the minima are also discussed,and we give a clear relation between the minima of the charge form factors and the corresponding charge radii.This relation is caused by the diffraction effect of the electron.Under this conclusion,we calculate the charge density distributions and the charge form factors of the A =44 nuclei chain.The results are also useful for studying the central depression in light exotic nuclei.
Johansson, Mikael P; Sundholm, Dage
2004-02-15
We recently performed detailed analyses of the electronic structure of low-spin iron porphyrins using density-functional theory (DFT). Both the spin-density distributions of the oxidized, ferric forms, as well as the changes in total charge density upon reduction to the ferrous forms have been explored. Here, we compare the DFT results with wave-function theory, more specifically, with the approximate singles and doubles coupled-cluster method (CC2). Different spin states are considered by studying representative models of low spin, intermediate spin, and high spin species. The CC2 calculations corroborate the DFT results; the spin density exhibits the same amount of molecular spin polarization, and the charge delocalization is of comparable magnitude. Slight differences in the descriptions are noted and discussed.
Nuclear charge radii: density functional theory meets Bayesian neural networks
Utama, R.; Chen, Wei-Chia; Piekarewicz, J.
2016-11-01
The distribution of electric charge in atomic nuclei is fundamental to our understanding of the complex nuclear dynamics and a quintessential observable to validate nuclear structure models. The aim of this study is to explore a novel approach that combines sophisticated models of nuclear structure with Bayesian neural networks (BNN) to generate predictions for the charge radii of thousands of nuclei throughout the nuclear chart. A class of relativistic energy density functionals is used to provide robust predictions for nuclear charge radii. In turn, these predictions are refined through Bayesian learning for a neural network that is trained using residuals between theoretical predictions and the experimental data. Although predictions obtained with density functional theory provide a fairly good description of experiment, our results show significant improvement (better than 40%) after BNN refinement. Moreover, these improved results for nuclear charge radii are supplemented with theoretical error bars. We have successfully demonstrated the ability of the BNN approach to significantly increase the accuracy of nuclear models in the predictions of nuclear charge radii. However, as many before us, we failed to uncover the underlying physics behind the intriguing behavior of charge radii along the calcium isotopic chain.
Charge density asymmetry of heavy-ion fusion reactions
Energy Technology Data Exchange (ETDEWEB)
Poenaru, N.D.; Ivascu, M.; Mazilu, D.; Sandulescu, A. (Institutul de Fizica si Inginerie Nucleara, Bucharest (Romania))
1980-01-01
The generalized liquid-drop model replacing surface energy by double folded Yukawa-plus-exponential function is extended for fusion of heavy ions with different charge densities. Calculated interaction barriers for some 58 pairs of nuclei are in good agreement with experimental ones, within -10% and +7%. For even-even beta-stable nuclei with Z =4-104 the general trend of variation of interaction barriers and fusion Q-values show the regions where the charge density asymmetry cannot be neglected. PES for the entrance channel of the reactions /sup 109/Ag + /sup 40/Ar, /sup 138/Ce + /sup 57/Fe, /sup 144/Nd + /sup 84/Kr and the corresponding charge-equilibrated system have been computed.
Nonextensive dust acoustic waves in a charge varying dusty plasma
Bacha, Mustapha; Tribeche, Mouloud
2012-01-01
Our recent analysis on nonlinear nonextensive dust-acoustic waves (DA) [Amour and Tribeche in Phys. Plasmas 17:063702, 2010] is extended to include self-consistent nonadiabatic grain charge fluctuation. The appropriate nonextensive electron charging current is rederived based on the orbit-limited motion theory. Our results reveal that the amplitude, strength and nature of the nonlinear DA waves (solitons and shocks) are extremely sensitive to the degree of ion nonextensivity. Stronger is the electron correlation, more important is the charge variation induced nonlinear wave damping. The anomalous dissipation effects may prevail over that dispersion as the electrons evolve far away from their Maxwellian equilibrium. Our investigation may be of wide relevance to astronomers and space scientists working on interstellar dusty plasmas where nonthermal distributions are turning out to be a very common and characteristic feature.
Diffuse Waves and Energy Densities Near Boundaries
Sanchez-Sesma, F. J.; Rodriguez-Castellanos, A.; Campillo, M.; Perton, M.; Luzon, F.; Perez-Ruiz, J. A.
2007-12-01
Green function can be retrieved from averaging cross correlations of motions within a diffuse field. In fact, it has been shown that for an elastic inhomogeneous, anisotropic medium under equipartitioned, isotropic illumination, the average cross correlations are proportional to the imaginary part of Green function. For instance coda waves are due to multiple scattering and their intensities follow diffusive regimes. Coda waves and the noise sample the medium and effectively carry information along their paths. In this work we explore the consequences of assuming both source and receiver at the same point. From the observable side, the autocorrelation is proportional to the energy density at a given point. On the other hand, the imaginary part of the Green function at the source itself is finite because the singularity of Green function is restricted to the real part. The energy density at a point is proportional with the trace of the imaginary part of Green function tensor at the source itself. The Green function availability may allow establishing the theoretical energy density of a seismic diffuse field generated by a background equipartitioned excitation. We study an elastic layer with free surface and overlaying a half space and compute the imaginary part of the Green function for various depths. We show that the resulting spectrum is indeed closely related to the layer dynamic response and the corresponding resonant frequencies are revealed. One implication of present findings lies in the fact that spatial variations may be useful in detecting the presence of a target by its signature in the distribution of diffuse energy. These results may be useful in assessing the seismic response of a given site if strong ground motions are scarce. It suffices having a reasonable illumination from micro earthquakes and noise. We consider that the imaginary part of Green function at the source is a spectral signature of the site. The relative importance of the peaks of
Waves in relativistic electron beam in low-density plasma
Sheinman, I.; Sheinman (Chernenco, J.
2016-11-01
Waves in electron beam in low-density plasma are analyzed. The analysis is based on complete electrodynamics consideration. Dependencies of dispersion laws from system parameters are investigated. It is shown that when relativistic electron beam is passed through low-density plasma surface waves of two types may exist. The first type is a high frequency wave on a boundary between the beam and neutralization area and the second type wave is on the boundary between neutralization area and stationary plasma.
C library for topological study of the electronic charge density.
Vega, David; Aray, Yosslen; Rodríguez, Jesús
2012-12-05
The topological study of the electronic charge density is useful to obtain information about the kinds of bonds (ionic or covalent) and the atom charges on a molecule or crystal. For this study, it is necessary to calculate, at every space point, the electronic density and its electronic density derivatives values up to second order. In this work, a grid-based method for these calculations is described. The library, implemented for three dimensions, is based on a multidimensional Lagrange interpolation in a regular grid; by differentiating the resulting polynomial, the gradient vector, the Hessian matrix and the Laplacian formulas were obtained for every space point. More complex functions such as the Newton-Raphson method (to find the critical points, where the gradient is null) and the Cash-Karp Runge-Kutta method (used to make the gradient paths) were programmed. As in some crystals, the unit cell has angles different from 90°, the described library includes linear transformations to correct the gradient and Hessian when the grid is distorted (inclined). Functions were also developed to handle grid containing files (grd from DMol® program, CUBE from Gaussian® program and CHGCAR from VASP® program). Each one of these files contains the data for a molecular or crystal electronic property (such as charge density, spin density, electrostatic potential, and others) in a three-dimensional (3D) grid. The library can be adapted to make the topological study in any regular 3D grid by modifying the code of these functions.
Institute of Scientific and Technical Information of China (English)
XueJu-Kui; LangHe
2003-01-01
The effect of dust charge variation on the dust-acoustic solitary structures is investigated in a warm magnetized two-ion-temperature dusty plasma consisting of a negatively and variably charged extremely massive dust fluid and ions of two different temperatures. It is shown that the dust charge variation as well as the presence of a second component of ions would modify the properties of the dust-acoustic solitary structures and may exite both dust-acoustic solitary holes (soliton waves with a density dip) and positive solitons (soliton waves with a density hump).
Institute of Scientific and Technical Information of China (English)
薛具奎; 郎和
2003-01-01
The effect of dust charge variation on the dust-acoustic solitary structures is investigated in a warm magnetized two-ion-temperature dusty plasma consisting of a negatively and variably charged extremely massive dust fluid and ions of two different temperatures. It is shown that the dust charge variation as well as the presence of a second component of ions would modify the properties of the dust-acoustic solitary structures and may excite both dust-acoustic solitary holes (soliton waves with a density dip) and positive solitons (soliton waves with a density hump).
Emergent loop current order from pair density wave superconductivity
Kashyap, Manoj; Melchert, Drew; Agterberg, Daniel
2015-03-01
In addition to charge density wave (CDW) order, there is evidence that the pseudogap phase in the cuprates breaks time reversal symmetry. Here we show that pair density wave (PDW) states give rise to a translational invariant non-superconducting order parameter that breaks time reversal and parity symmetries, but preserves their product. This secondary order parameter has a different origin, but shares the same symmetry properties as a magnetoelectric loop current order that has been proposed earlier in the context of the cuprates to explain the appearance of intra-cell magnetic order. We further show that, due to fluctuations, this secondary loop current order, which represents the breaking of discrete symmetries, can preempt PDW order, which breaks both continuous and discrete symmetries. In such a phase, the emergent loop current order coexists with spatial short range CDW and short range superconducting order. Finally, we propose a PDW phase that accounts for intra-cell magnetic order and the Kerr effect, has CDW order consistent with x-ray scattering and nuclear magnetic resonance observations, and quasi-particle properties consistent with angle resolved photoemission scattering. We acknowledge support from NSF Grant No. DMR-1335215
Determination of Transverse Charge Density from Kaon Form Factor Data
Mejia-Ott, Johann; Horn, Tanja; Pegg, Ian; Mecholski, Nicholas; Carmignotto, Marco; Ali, Salina
2016-09-01
At the level of nucleons making up atomic nuclei, among subatomic particles made up of quarks, K-mesons or kaons represent the most simple hadronic system including the heavier strange quark, having a relatively elementary bound state of a quark and an anti-quark as its valence structure. Its electromagnetic structure is then parametrized by a single, dimensionless quantity known as the form factor, the two-dimensional Fourier transform of which yields the quantity of transverse charge density. Transverse charge density, in turn, provides a needed framework for the interpretation of form factors in terms of physical charge and magnetization, both with respect to the propagation of a fast-moving nucleon. To this is added the value of strange quarks in ultimately presenting a universal, process-independent description of nucleons, further augmenting the importance of studying the kaon's internal structure. The pressing character of such research questions directs the present paper, describing the first extraction of transverse charge density from electromagnetic kaon form factor data. The extraction is notably extended to form factor data at recently acquired higher energy levels, whose evaluation could permit more complete phenomenological models for kaon behavior to be proposed. This work was supported in part by NSF Grant PHY-1306227.
Theoretical study of pair density wave superconductors
Zheng, Zhichao
In conventional superconductors, the Cooper pairs are formed from quasiparticles. We explore another type of superconducting state, a pair density wave (PDW) order, which spontaneously breaks some of the translational and point group symmetries. In a PDW superconductor, the order parameter is a periodic function of the center-of-mass coordinate, and the spatial average value of the superconducting order parameter vanishes. In the early 1960s, following the success of the BCS theory of superconductivity, Fulde and Ferrell and Larkin and Ovchinnikov (FFLO) developed theories of inhomogeneous superconducting states. Because of this Zeeman splitting in a magnetic field, the Cooper pairs having a nonzero center-of-mass momentum are more stable than the normal pairing, leading to the FFLO state. Experiments suggest possible occurrence of the FFLO state in the heavy-fermion compound CeCoIn5, and in quasi-low-dimensional organic superconductors. FFLO phases have also been argued to be of importance in understanding ultracold atomic Fermi gases and in the formation of color superconductivity in high density quark matter. In all Fermi superfluids known at the present time, Cooper pairs are composed of particles with spin 1/2. The spin component of a pair wave function can be characterized by its total spin S = 0 (singlet) and S = 1 (triplet). In the discovered broken inversion superconductors CePt3Si, Li2Pt3B, and Li2Pd3B, the magnetic field leads to novel inhomogeneous superconducting states, namely the helical phase and the multiple-q phase. Its order parameter exhibits periodicity similar to FFLO phase, and the consequences of both phases are same: the enhancement of transition temperature as a function of magnetic field. We have studied the PDW phases in broken parity superconductors with vortices included. By studying PDW vortex states, we find the usual Abrikosov vortex solution is unstable against a new solution with fractional vortex pairs. We have also studied the
Survival of charged rho condensation at high temperature and density
Liu, Hao; Huang, Mei
2015-01-01
The charged vector $\\rho$ mesons in the presence of external magnetic fields at finite temperature $T$ and chemical potential $\\mu$ have been investigated in the framework of the Nambu--Jona-Lasinio model. We compute the masses of charged $\\rho$ mesons numerically as a function of the magnetic field for different values of temperature and chemical potential. The self-energy of the $\\rho$ meson contains the quark-loop contribution, i.e. the leading order contribution in $1/N_c$ expansion. The charged $\\rho$ meson mass decreases with the magnetic field and drops to zero at a critical magnetic field $eB_c$, which means that the charged vector meson condensation, i.e. the electromagnetic superconductor can be induced above the critical magnetic field. Surprisingly, it is found that the charged $\\rho$ condensation can even survive at high temperature and density. At zero temperature, the critical magnetic field just increases slightly with the chemical potential, which indicates that the charged $\\rho$ condensatio...
Damping of Resonantly Forced Density Waves in Dense Planetary Rings
Lehmann, Marius; Schmidt, Jürgen; Salo, Heikki
2016-10-01
We address the stability of resonantly forced density waves in dense planetary rings.Already by Goldreich and Tremaine (1978) it has been argued that density waves might be unstable, depending on the relationship between the ring's viscosity and the surface mass density. In the recent paper (Schmidt et al. 2016) we have pointed out that when - within a fluid description of the ring dynamics - the criterion for viscous overstability is satisfied, forced spiral density waves become unstable as well. In this case, linear theory fails to describe the damping.We apply the multiple scale formalism to derive a weakly nonlinear damping relation from a hydrodynamical model.This relation describes the resonant excitation and nonlinear viscous damping of spiral density waves in a vertically integrated fluid disk with density dependent transport coefficients. The model consistently predicts linear instability of density waves in a ring region where the conditions for viscous overstability are met. In this case, sufficiently far away from the Lindblad resonance, the surface mass density perturbation is predicted to saturate to a constant value due to nonlinear viscous damping. In general the model wave damping lengths depend on a set of input parameters, such as the distance to the threshold for viscous overstability and the ground state surface mass density.Our new model compares reasonably well with the streamline model for nonlinear density waves of Borderies et al. 1986.Deviations become substantial in the highly nonlinear regime, corresponding to strong satellite forcing.Nevertheless, we generally observe good or at least qualitative agreement between the wave amplitude profiles of both models. The streamline approach is superior at matching the total wave profile of waves observed in Saturn's rings, while our new damping relation is a comparably handy tool to gain insight in the evolution of the wave amplitude with distance from resonance, and the different regimes of
Ghosh, Soumen; Sonnenberger, Andrew L; Hoyer, Chad E; Truhlar, Donald G; Gagliardi, Laura
2015-08-11
The correct description of charge transfer in ground and excited states is very important for molecular interactions, photochemistry, electrochemistry, and charge transport, but it is very challenging for Kohn-Sham (KS) density functional theory (DFT). KS-DFT exchange-correlation functionals without nonlocal exchange fail to describe both ground- and excited-state charge transfer properly. We have recently proposed a theory called multiconfiguration pair-density functional theory (MC-PDFT), which is based on a combination of multiconfiguration wave function theory with a new type of density functional called an on-top density functional. Here we have used MC-PDFT to study challenging ground- and excited-state charge-transfer processes by using on-top density functionals obtained by translating KS exchange-correlation functionals. For ground-state charge transfer, MC-PDFT performs better than either the PBE exchange-correlation functional or CASPT2 wave function theory. For excited-state charge transfer, MC-PDFT (unlike KS-DFT) shows qualitatively correct behavior at long-range with great improvement in predicted excitation energies.
Close-in Blast Waves from Spherical Charges*
Howard, William; Kuhl, Allen
2011-06-01
We study the close-in blast waves created by the detonation of spherical high explosives (HE) charges, via numerical simulations with our Arbitrary-Lagrange-Eulerian (ALE3D) code. We used a finely-resolved, fixed Eulerian 2-D mesh (200 μm per cell) to capture the detonation of the charge, the blast wave propagation in air, and the reflection of the blast wave from an ideal surface. The thermodynamic properties of the detonation products and air were specified by the Cheetah code. A programmed-burn model was used to detonate the charge at a rate based on measured detonation velocities. The results were analyzed to evaluate the: (i) free air pressure-range curves: Δps (R) , (ii) free air impulse curves, (iii) reflected pressure-range curves, and (iv) reflected impulse-range curves. A variety of explosives were studied. Conclusions are: (i) close-in (R Heat of Detonation'' of the explosive (because close-in, there is not enough time to fully couple the chemical energy to the air via piston work); (iii) instead they are related to the detonation conditions inside the charge. Scaling laws will be proposed for such close-in blast waves.
Geometric interpretation of density displacements and charge sensitivities
Indian Academy of Sciences (India)
Roman F Nalewajski
2005-09-01
The ``geometric” interpretation of the electronic density displacements in the Hilbert space is given and the associated projection-operator partitioning of the hardness and softness operators (kernels) is developed. The eigenvectors |á 〉 = \\{| 〉 \\} of the hardness operator define the complete (identity) projector $\\hat{P}$ = | 〉 〈 = 1 for general density displacements, including the charge-transfer (CT) component, while the eigenvectors | i 〉 = { | 〉} of the linear response operator determine the polarizational -projector, $\\hat{P}$ = | 〉 〈 |. Their difference thus defines the complementary CT-projector: $\\hat{P}$ = 1 - $\\hat{P}$. The complete vector space for density displacements can be also spanned by supplementing the -modes with the homogeneous CT-mode. These subspaces separate the integral (normalization) and local aspects of density shifts in molecular systems.
Simulation of the Reflected Blast Wave froma C-4 Charge
Energy Technology Data Exchange (ETDEWEB)
Howard, W M; Kuhl, A L; Tringe, J W
2011-08-01
The reflection of a blast wave from a C4 charge detonated above a planar surface is simulated with our ALE3D code. We used a finely-resolved, fixed Eulerian 2-D mesh (167 {micro}m per cell) to capture the detonation of the charge, the blast wave propagation in nitrogen, and its reflection from the surface. The thermodynamic properties of the detonation products and nitrogen were specified by the Cheetah code. A programmed-burn model was used to detonate the charge at a rate based on measured detonation velocities. Computed pressure histories are compared with pressures measured by Kistler 603B piezoelectric gauges at 8 ranges (GR = 0, 2, 4, 8, 10, and 12 inches) along the reflecting surface. Computed and measured waveforms and positive-phase impulses were similar, except at close-in ranges (GR < 2 inches), which were dominated by jetting effects.
Charge Management for Gravitational Wave Observatories using UV LEDs
Pollack, S E; Schlamminger, S; Hagedorn, C A; Gundlach, J H
2009-01-01
Accumulation of electrical charge on the end mirrors of gravitational wave observatories, such as the space-based LISA mission and ground-based LIGO detectors, can become a source of noise limiting the sensitivity of such detectors through electronic couplings to nearby surfaces. Torsion balances provide an ideal means for testing gravitational wave technologies due to their high sensitivity to small forces. Our torsion pendulum apparatus consists of a movable Au-coated Cu plate brought near a Au-coated Si plate pendulum suspended from a non-conducting quartz fiber. A UV LED located near the pendulum photoejects electrons from the surface, and a UV LED driven electron gun directs photoelectrons towards the pendulum surface. We have demonstrated both charging and discharging of the pendulum with equivalent charging rates of $\\sim
Charge density study of two FeS2 polymorphs
DEFF Research Database (Denmark)
Schmøkel, Mette Stokkebro; Jørgensen, Mads Ry Vogel; Bjerg, Lasse
experimental electron density studies of an inorganic solid containing a transition metal was presented by Stevens et al. [2] who investigated the effect of crystal-field splitting of the partially filled iron d-orbitals in the pyrite structure of FeS2. Other studies of various FeS2 structures, including......-temperature single crystal diffraction data were collected with synchrotron radiation on both compounds at the ChemMatCARS beamline at the Advanced Photon Source. Extinction and absorption effects were minimized using small crystals (10 μm) and high-energy (28 keV) radiation. The experimental charge density has...
Scattered surface charge density: A tool for surface characterization
Naydenov, Borislav
2011-11-28
We demonstrate the use of nonlocal scanning tunneling spectroscopic measurements to characterize the local structure of adspecies in their states where they are significantly less perturbed by the probe, which is accomplished by mapping the amplitude and phase of the scattered surface charge density. As an example, we study single-H-atom adsorption on the n-type Si(100)-(4 × 2) surface, and demonstrate the existence of two different configurations that are distinguishable using the nonlocal approach and successfully corroborated by density functional theory. © 2011 American Physical Society.
Charge, density and electron temperature in a molecular ultracold plasma
Rennick, C J; Ortega-Arroyo, J; Godin, P J; Grant, E R
2009-01-01
A Rydberg gas of NO entrained in a supersonic molecular beam releases electrons as it evolves to form an ultracold plasma. The size of this signal, compared with that extracted by the subsequent application of a pulsed electric field, determines the absolute magnitude of the plasma charge. This information, combined with the number density of ions, supports a simple thermochemical model that explains the evolution of the plasma to an ultracold electron temperature.
Topics in the Dynamics of Charge-Density
Ramakrishna, Sathyanarayan (Satish).
This dissertation is an investigation into some interesting transport properties of charge-density-waves (CDWs). The field of CDW dynamics is an arena for the battle between mathematical analysis and random disorder. It is a very difficult physical situation to analyze. The theoretical study of CDW dynamics dates to the prescient suggestion of John Bardeen (in the 70s) that the nonlinear I-V characteristic of the quasi one-dimensional material TTF-TCNQ was a consequence of collective transport of condensate resulting from a Peierls instability. This instability, described first by Peierls, is studied in Chapter 1. Once the underlying physics of the instability was understood, the effects of coupling the CDW to impurities and to electric and magnetic fields were studied. The most striking effect of impurities is to produce CDW pinning, so that collective-mode transport ceases to occur if the applied electric field is smaller than a threshold field. Intensive research led to the Fukuyama-Lee-Rice model of CDW pinning. Experiments in the field are complicated by the difficulty in preparing well characterized samples of the relevant materials, among which are the trichalco-genides NbSe_3, TaS_3, the dichalcogenides (TaSe_4)_2I, TaS_2, NbSe_2 and blue bronze K_{0.3}MoO _3. Over the last decade, growth techniques have been perfected and intensive comparison between the various theoretical models and experiment is feasible. An outline of the dissertation is as follows. First, we review the theoretical ideas that underlie the subject. Then we discuss each new piece of work separately. First, this thesis presents one important theoretical approach to the study of CDW dynamics. The approach builds upon previous work on the microscopic theory of superconductors and results in a new formulation of the problem that seems likely to lend itself to non-perturbative approaches. The perturbative approach cannot provide answers to the question of what happens near the depinning
Spiral density wave generation by vortices in Keplerian flows
Bodo, G; Murante, G; Tevzadze, A; Rossi, P; Ferrari, A
2005-01-01
We perform a detailed analytical and numerical study of the dynamics of perturbations (vortex/aperiodic mode, Rossby and spiral-density waves) in 2D compressible disks with a Keplerian law of rotation. We draw attention to the process of spiral-density wave generation from vortices, discussing, in particular, the initial, most peculiar stages of wave emission. We show that the linear phenomenon of wave generation by vortices in smooth (without inflection points) shear flows found by using the so-called non-modal approach, is directly applicable to the present case. After an analytical non-modal description of the physics and characteristics of the spiral-density wave generation/propagation in the local shearing-sheet model, we follow the process of wave generation by small amplitude coherent circular vortex structures, by direct global numerical simulation, describing the main features of the generated waves.
Kato, Shinichi; Harada, Hiroyuki; Hotchi, Hideaki; Okabe, Kota; Yamamoto, Kazami; Kinsho, Michikazu
For high intensity proton accelerators, one of the beam loss sources is the incoherent tune spread caused by the space charge force. In the 3 GeV rapid cycling synchrotron of the Japan Proton Accelerator Research Complex, beams are injected sequentially and shifted slightly from the central orbit in order to increase the beam size intentionally and suppress the charge density and incoherent tune spread. This injection method has been adopted and suppressed the beam loss. However, simulations clarified that beams did not spread as much as expected because of the space charge effect in the high current case. As simulation results of the optimized beam shift pattern when the space charge effect is considered, it was obtained that the incoherent tune spread could be suppressed to an extent that has not been achieved previously.
The influence of oxidation on space charge formation in gamma-irradiated low-density polyethylene
Chen, G; Xie, H K; Banford, H M; Davies, A E
2003-01-01
The research presented in this paper investigates the role of oxidation in the formation of space charge in gamma-irradiated low-density polyethylene after being electrically stressed under dc voltage. Polyethylene plaques both with and without antioxidant were irradiated up to 500 kGy using a sup 6 sup 0 Co gamma source and space charge distributions were measured using the piezoelectric induced pressure wave propagation method. It has been found that a large amount of positive charge evolved adjacent to the cathode in the sample without antioxidant and was clearly associated with oxidation of the surface. The amount of charge formed for a given applied stress increased with the dose absorbed by the material. A model has been proposed to explain the formation of space charge and its profile. The charge decay after the removal of the external applied stress is dominated by a process being controlled by the cathode interfacial stress (charge injection) rather than a conventional RC circuit model. On the other ...
Realizing vector meson dominance with transverse charge densities
Miller, G A; Weiss, C
2011-01-01
The transverse charge density in a fast-moving nucleon is represented as a dispersion integral of the imaginary part of the Dirac form factor in the timelike region (spectral function). At a given transverse distance b the integration effectively extends over energies in a range sqrt{t} ~< 1/b, with exponential suppression of larger values. The transverse charge density at peripheral distances thus acts as a low-pass filter for the spectral function and allows one to select energy regions dominated by specific t-channel states, corresponding to definite exchange mechanisms in the spacelike form factor. We show that distances b ~ 0.5 - 1.5 fm in the isovector density are maximally sensitive to the rho meson region, with only a ~10% contribution from higher-mass states. Soft-pion exchange governed by chiral dynamics becomes relevant only at larger distances. In the isoscalar density higher-mass states beyond the omega are comparatively more important. The dispersion approach suggests that the positive transv...
Density Waves in the Flows of Granular Media
1993-01-01
We study density waves in the flows of granular particles through vertical tubes and hoppers using both analytic methods and molecular dynamics (MD) simulations. We construct equations of motion for quasi one-dimensional systems. The equations, combined with the Bagnold's law for friction, are used to describe the time evolutions of the density and the velocity fields for narrow tubes and hoppers. The solutions of the equations can have two types of density waves, kinetic and dynamic. For tub...
RAYLEIGH WAVE STUDIES OF CATHODIC H-CHARGING OF Fe
Lunarska, E.; Fiore, N.
1981-01-01
The attenuation of 2-6 MHz Rayleigh waves /RW/ was measured in sheet samples of Fe which were undergoing electrolytic charging with H. The cathodic polarization and As2O3 addition into electrolyte were found to effect the attenuation and velocity of the surface waves. The attenuation changes were retarded by the deposition of a thin /2µm/ layer of Cu on the Fe surface, with the Cu acting as a H-permeation barrier. The decrease in attenuation was caused by the entry of H into solid solution at...
The thermal-wave model: A Schroedinger-like equation for charged particle beam dynamics
Fedele, Renato; Miele, G.
1994-01-01
We review some results on longitudinal beam dynamics obtained in the framework of the Thermal Wave Model (TWM). In this model, which has recently shown the capability to describe both longitudinal and transverse dynamics of charged particle beams, the beam dynamics is ruled by Schroedinger-like equations for the beam wave functions, whose squared modulus is proportional to the beam density profile. Remarkably, the role of the Planck constant is played by a diffractive constant epsilon, the emittance, which has a thermal nature.
Surface modification for polystyrene colloidal particles with controlled charge densities.
Lee, Jongman; Kwon, Oh-Sun; Shin, Kwanwoo; Song, Ju-Myung; Kim, Joon-Seop; Seo, Young-Soo; Tael, Giyoong; Jon, Sangyong
2007-11-01
A significant amount of polystyrene sulfonated acid (PSSA) and poly(styrene-ran-acrylic acid) (PSAA) random copolymer can be adsorbed by dispersion of PS particles via a swelling-quenching process. A THF-water mixed solvent was used in the swelling process and a large amount of pure water was used, to give a low concentration of THF% in quenching process. Our results showed that functional PSSA groups were randomly and tightly adsorbed to the PS particles. When the mol.% of charged segments was increased, the progressive adsorption of PSSA chains to the PS particles leads to an increase in the electrophoretic mobility and zeta-potential of aqueous dispersions. Thus, we were able to obtain well-distributed surface charge density on the PS particles.
Effects of Charge in Heavy Ions on Solitary Kinetic Alfvén Waves in Double-Ion Plasmas
Institute of Scientific and Technical Information of China (English)
YANG Lei; WU De-Jin
2006-01-01
@@ After the charge of heavy ions is considered, a Sagdeev equation is obtained for the solitary kinetic Alfvén waves (SKAWs) in a low-β(me/mp＜＜β＜＜1 or mp/me＞＞α＞＞1), three-component (electrons, protons, and highly charged heavy ions) plasma. Numerical results show that the charge number q of heavy ions can cause the width of the solitary structure to decrease, but increase for the maximum of electron density nem≤1.2 and the initial abundance of heavy ions Cb0 ≤ 0.1. The parallel phase speed of the waves increases with larger q.
3D High Density Wave Interconnects Project
National Aeronautics and Space Administration — Nuvotronics has developed and optimized the PolyStrataTM process for the fabrication of intricate microwave and millimeter-wave devices. These devices have primarily...
Probing density waves in fluidized granular media with diffusing-wave spectroscopy
Born, Philip; Reinhold, Steffen; Sperl, Matthias
2016-09-01
Density waves are characteristic for fluidized beds and affect measurements on liquidlike dynamics in fluidized granular media. Here the intensity autocorrelation function as obtainable with diffusing-wave spectroscopy is derived in the presence of density waves. The predictions by the derived form of the intensity autocorrelation function match experimental observations from a gas-fluidized bed. The model suggests separability of the contribution from density waves from the contribution by microscopic scatterer displacement to the decay of correlation and thus paves the way for characterizing microscopic particle motions using diffusing-wave spectroscopy as well as heterogeneities in fluidized granular media.
Continuous Dependence on the Density for Stratified Steady Water Waves
Chen, Robin Ming; Walsh, Samuel
2016-02-01
There are two distinct regimes commonly used to model traveling waves in stratified water: continuous stratification, where the density is smooth throughout the fluid, and layer-wise continuous stratification, where the fluid consists of multiple immiscible strata. The former is the more physically accurate description, but the latter is frequently more amenable to analysis and computation. By the conservation of mass, the density is constant along the streamlines of the flow; the stratification can therefore be specified by prescribing the value of the density on each streamline. We call this the streamline density function. Our main result states that, for every smoothly stratified periodic traveling wave in a certain small-amplitude regime, there is an L ∞ neighborhood of its streamline density function such that, for any piecewise smooth streamline density function in that neighborhood, there is a corresponding traveling wave solution. Moreover, the mapping from streamline density function to wave is Lipschitz continuous in a certain function space framework. As this neighborhood includes piecewise smooth densities with arbitrarily many jump discontinues, this theorem provides a rigorous justification for the ubiquitous practice of approximating a smoothly stratified wave by a layered one. We also discuss some applications of this result to the study of the qualitative features of such waves.
Shells of charge: a density functional theory for charged hard spheres.
Roth, Roland; Gillespie, Dirk
2016-06-22
A functional for the electrostatic excess free-energy for charged, hard sphere fluids is proposed. The functional is derived from two complementary, but equivalent, interpretations of the mean spherical approximation (MSA). The first combines fundamental measure theory (FMT) from hard-core interactions with the idea that MSA can be interpreted in terms of the interaction spherical shells of charge. This formulation gives the free-energy density as a function of weighted densities. When all the ions have the same size, the functional adopts an FMT-like form. The second in effect 'functionalizes' the derivation of MSA; that is, it generalizes the MSA as a functional-based version of MSA (fMSA). This formulation defines the free-energy density as a function of a position-dependent MSA screening parameter and the weighted densities of the FMT approach. This FMT/fMSA functional is shown to give accurate density profiles, as compared to Monte Carlo simulations, under a wide range of ion concentrations, size asymmetries, and valences.
Shells of charge: a density functional theory for charged hard spheres
Roth, Roland; Gillespie, Dirk
2016-06-01
A functional for the electrostatic excess free-energy for charged, hard sphere fluids is proposed. The functional is derived from two complementary, but equivalent, interpretations of the mean spherical approximation (MSA). The first combines fundamental measure theory (FMT) from hard-core interactions with the idea that MSA can be interpreted in terms of the interaction spherical shells of charge. This formulation gives the free-energy density as a function of weighted densities. When all the ions have the same size, the functional adopts an FMT-like form. The second in effect ‘functionalizes’ the derivation of MSA; that is, it generalizes the MSA as a functional-based version of MSA (fMSA). This formulation defines the free-energy density as a function of a position-dependent MSA screening parameter and the weighted densities of the FMT approach. This FMT/fMSA functional is shown to give accurate density profiles, as compared to Monte Carlo simulations, under a wide range of ion concentrations, size asymmetries, and valences.
Impact of density information on Rayleigh surface wave inversion results
Ivanov, Julian; Tsoflias, Georgios; Miller, Richard D.; Peterie, Shelby; Morton, Sarah; Xia, Jianghai
2016-12-01
We assessed the impact of density on the estimation of inverted shear-wave velocity (Vs) using the multi-channel analysis of surface waves (MASW) method. We considered the forward modeling theory, evaluated model sensitivity, and tested the effect of density information on the inversion of seismic data acquired in the Arctic. Theoretical review, numerical modeling and inversion of modeled and real data indicated that the density ratios between layers, not the actual density values, impact the determination of surface-wave phase velocities. Application on real data compared surface-wave inversion results using: a) constant density, the most common approach in practice, b) indirect density estimates derived from refraction compressional-wave velocity observations, and c) from direct density measurements in a borehole. The use of indirect density estimates reduced the final shear-wave velocity (Vs) results typically by 6-7% and the use of densities from a borehole reduced the final Vs estimates by 10-11% compared to those from assumed constant density. In addition to the improved absolute Vs accuracy, the resulting overall Vs changes were unevenly distributed laterally when viewed on a 2-D section leading to an overall Vs model structure that was more representative of the subsurface environment. It was observed that the use of constant density instead of increasing density with depth not only can lead to Vs overestimation but it can also create inaccurate model structures, such as a low-velocity layer. Thus, optimal Vs estimations can be best achieved using field estimates of subsurface density ratios.
Charge carrier density in Li-intercalated graphene
Kaloni, Thaneshwor P.
2012-05-01
The electronic structures of bulk C 6Li, Li-intercalated free-standing bilayer graphene, and Li-intercalated bilayer and trilayer graphene on SiC(0 0 0 1) are studied using density functional theory. Our estimate of Young\\'s modulus suggests that Li-intercalation increases the intrinsic stiffness. For decreasing Li-C interaction, the Dirac point shifts to the Fermi level and the associated band splitting vanishes. For Li-intercalated bilayer graphene on SiC(0 0 0 1) the splitting at the Dirac point is tiny. It is also very small at the two Dirac points of Li-intercalated trilayer graphene on SiC(0 0 0 1). For all the systems under study, a large enhancement of the charge carrier density is achieved by Li intercalation. © 2012 Elsevier B.V. All rights reserved.
A study of transverse charge density of pions in relativistic quantum mechanics
Institute of Scientific and Technical Information of China (English)
DONG Yu-Bing; WANG Yi-Zhan
2011-01-01
The transverse charge density of pions is calculated based on relativistic quantum mechanics,where the pion is regarded as a quark-antiquark bound state. Corrections from the two spin-1/2 constituents and from the wave function of a quark and antiquark inside the bound system are discussed. The calculated results are compared to the results with a realistic effective Lagrangian approach as well as to that with a simple covariant model where the pion is regarded as a composite system with two scalar particles.
Enhancement of electric and magnetic wave fields at density gradients
Directory of Open Access Journals (Sweden)
A. Reiniusson
2006-03-01
Full Text Available We use Freja satellite data to investigate irregular small-scale density variations. The observations are made in the auroral region at about 1000-1700 km. The density variations are a few percent, and the structures are found to be spatial down to a scale length of a few ion gyroradii. Irregular density variations are often found in an environment of whistler mode/lower hybrid waves and we show that at the density gradients both the electric and magnetic wave fields are enhanced.
Cassini RSS occultation observations of density waves in Saturn's rings
McGhee, C. A.; French, R. G.; Marouf, E. A.; Rappaport, N. J.; Schinder, P. J.; Anabtawi, A.; Asmar, S.; Barbinis, E.; Fleischman, D.; Goltz, G.; Johnston, D.; Rochblatt, D.
2005-08-01
On May 3, 2005, the first of a series of eight nearly diametric occultations by Saturn's rings and atmosphere took place, observed by the Cassini Radio Science (RSS) team. Simultaneous high SNR measurements at the Deep Space Network (DSN) at S, X, and Ka bands (λ = 13, 3.6, and 0.9 cm) have provided a remarkably detailed look at the radial structure and particle scattering behavior of the rings. By virtue of the relatively large ring opening angle (B=-23.6o), the slant path optical depth of the rings was much lower than during the Voyager epoch (B=5.9o), making it possible to detect many density waves and other ring features in the Cassini RSS data that were lost in the noise in the Voyager RSS experiment. Ultimately, diffraction correction of the ring optical depth profiles will yield radial resolution as small as tens of meters for the highest SNR data. At Ka band, the Fresnel scale is only 1--1.5 km, and thus even without diffraction correction, the ring profiles show a stunning array of density waves. The A ring is replete with dozens of Pandora and Prometheus inner Lindblad resonance features, and the Janus 2:1 density wave in the B ring is revealed with exceptional clarity for the first time at radio wavelengths. Weaker waves are abundant as well, and multiple occultation chords sample a variety of wave phases. We estimate the surface mass density of the rings from linear density wave models of the weaker waves. For stronger waves, non-linear models are required, providing more accurate estimates of the wave dispersion relation, the ring surface mass density, and the angular momentum exchange between the rings and satellite. We thank the DSN staff for their superb support of these complex observations.
Obliquely propagating large amplitude solitary waves in charge neutral plasmas
Directory of Open Access Journals (Sweden)
F. Verheest
2007-01-01
Full Text Available This paper deals in a consistent way with the implications, for the existence of large amplitude stationary structures in general plasmas, of assuming strict charge neutrality between electrons and ions. With the limit of pair plasmas in mind, electron inertia is retained. Combining in a fluid dynamic treatment the conservation of mass, momentum and energy with strict charge neutrality has indicated that nonlinear solitary waves (as e.g. oscillitons cannot exist in electron-ion plasmas, at no angle of propagation with respect to the static magnetic field. Specifically for oblique propagation, the proof has turned out to be more involved than for parallel or perpendicular modes. The only exception is pair plasmas that are able to support large charge neutral solitons, owing to the high degree of symmetry naturally inherent in such plasmas. The nonexistence, in particular, of oscillitons is attributed to the breakdown of the plasma approximation in dealing with Poisson's law, rather than to relativistic effects. It is hoped that future space observations will allow to discriminate between oscillitons and large wave packets, by focusing on the time variability (or not of the phase, since the amplitude or envelope graphs look very similar.
Merlon-type density waves in a compartmentalized conveyor system
Kanellopoulos, G.; van derWeele, K.
2016-09-01
Multi-particle flow through a cyclic array of K connected compartments with a preferential direction is known to be able to organize itself in the form of density waves [Kanellopoulos, Van der Meer, and Van der Weele, Phys. Rev. E 92, 022205 (2015)]. In this brief note we focus on the intriguing shape these waves take when K is even, in which case they travel through alternatingly dense and diluted compartments. We call them "merlon waves", since the sequence of high and low densities is reminiscent of the merlons and crenels on the battlements of medieval castles.
Analysis of the stability and density waves for traffic flow
Institute of Scientific and Technical Information of China (English)
薛郁
2002-01-01
In this paper, the optimal velocity model of traffic is extended to take into account the relative velocity. Thestability and density waves for traffic flow are investigated analytically with the perturbation method. The stabilitycriterion is derived by the linear stability analysis. It is shown that the triangular shock wave, soliton wave and kinkwave appear respectively in our model for density waves in the three regions: stable, metastable and unstable regions.These correspond to the solutions of the Burgers equation, Kortewegg-de Vries equation and modified Korteweg-de Vriesequation.The analytical results are confirmed to be in good agreement with those of numerical simulation. All theresults indicate that the interaction of a car with relative velocity can affect the stability of the traffic flow and raisecritical density.
Pair density wave superconducting states and statistical mechanics of dimers
Soto Garrido, Rodrigo Andres
3 we show that the pair-density-wave superconducting state emergent in extended Heisenberg-Hubbard models in two-leg ladders is topological in the presence of an Ising spin symmetry and supports a Majorana zero mode (MZM) at an open boundary and at a junction with a uniform d-wave one-dimensional superconductor. Similarly to a conventional finite-momentum paired state, the order parameter of the PDW state is a charge-2e field with finite momentum. However, the order parameter here is a quartic electron operator and conventional mean-field theory cannot be applied to study this state. We use bosonization to show that the 1D PDW state has a MZM at a boundary. This superconducting state is an exotic topological phase supporting Majorana fermions with finite-momentum pairing fields and charge-4e superconductivity. In chapter 4 we provide a quasi-one-dimensional model which can support a PDW state. The model consists of an array of strongly-interacting one-dimensional systems, where the one-dimensional systems are coupled to each other by local interactions.Within the interchain mean-field theory (MFT), we find several SC states from the model, including a conventional uniform SC state, PDW SC state, and a coexisting phase of the uniform SC and PDW states. In this quasi-1D regime we can treat the strong correlation physics essentially exactly using bosonization methods and the crossover to the 2D system by means of interchain MFT. The resulting critical temperatures of the SC phases generically exhibit a power-law scaling with the coupling constants of the array, instead of the essential singularity found in weak-coupling BCS-type theories. Electronic excitations with an open Fermi surface, which emerge from the electronic Luttinger liquid systems below their crossover temperature to the Fermi liquid, are then coupled to the SC order parameters via the proximity effect. From the Fermi surface thus coupled to the SC order parameters, we calculate the quasiparticle
Institute of Scientific and Technical Information of China (English)
Li Cheng-Bin; Li Ming-Kai; Yin Dong; Liu Fu-Qing; Fan Xiang-Jun
2005-01-01
A first principles study of the electronic properties and bulk modulus (B0) of the fcc and bcc transition metals,transition metal carbides and nitrides is presented. The calculations were performed by plane-wave pseudopotential method in the framework of the density functional theory with local density approximation. The density of states and the valence charge densities of these solids are plotted. The results show that B0 does not vary monotonically when the number of the valence d electrons increases. B0 reaches a maximum and then decreases for each of the four sorts of solids. It is related to the occupation of the bonding and anti-bonding states in the solid. The value of the valence charge density at the midpoint between the two nearest metal atoms tends to be proportional to B0.
Effects of dispersive wave modes on charged particles transport
Schreiner, Cedric
2015-01-01
The transport of charged particles in the heliosphere and the interstellar medium is governed by the interaction of particles and magnetic irregularities. For the transport of protons a rather simple model using a linear Alfv\\'en wave spectrum which follows the Kolmogorov distribution usually yields good results. Even magnetostatic spectra may be used. For the case of electron transport, particles will resonate with the high-k end of the spectrum. Here the magnetic fluctuations do not follow the linear dispersion relation, but the kinetic regime kicks in. We will discuss the interaction of fluctuations of dispersive waves in the kinetic regime using a particle-in-cell code. Especially the scattering of particles following the idea of Lange et al. (2013) and its application to PiC codes will be discussed. The effect of the dispersive regime on the electron transport will be discussed in detail.
Motion of a charge in a superstrong electromagnetic standing wave
Esirkepov, Timur Z.; Bulanov, Stepan S.; Koga, James K.; Kando, Masaki; Kondo, Kiminori; Rosanov, Nikolay N.; Korn, Georg; Bulanov, Sergei V.
2015-05-01
Radiation reaction radically influences the electron motion in an electromagnetic standing wave formed by two super-intense colliding laser pulses. Depending on the laser intensity and wavelength, the quantum corrections to the electron motion and the radiation reaction force can be independently small or large, thus dividing the parameter space into 4 regions. When radiation reaction dominates, the electron motion evolves to limit cycles and strange attractors. This creates a new framework for high energy physics experiments on the interaction of energetic charged particle beams and colliding super-intense laser pulses.
Spiral density waves in M81. I. Stellar spiral density waves
Energy Technology Data Exchange (ETDEWEB)
Feng, Chien-Chang; Lin, Lien-Hsuan; Wang, Hsiang-Hsu; Taam, Ronald E., E-mail: hhwang@asiaa.sinica.edu.tw [Institute of Astronomy and Astrophysics, Academia Sinica, P.O. Box 23-141, Taipei 10617, Taiwan, R.O.C (China)
2014-04-20
Aside from the grand-design stellar spirals appearing in the disk of M81, a pair of stellar spiral arms situated well inside the bright bulge of M81 has been recently discovered by Kendall et al. The seemingly unrelated pairs of spirals pose a challenge to the theory of spiral density waves. To address this problem, we have constructed a three-component model for M81, including the contributions from a stellar disk, a bulge, and a dark matter halo subject to observational constraints. Given this basic state for M81, a modal approach is applied to search for the discrete unstable spiral modes that may provide an understanding for the existence of both spiral arms. It is found that the apparently separated inner and outer spirals can be interpreted as a single trailing spiral mode. In particular, these spirals share the same pattern speed 25.5 km s{sup –1} kpc{sup –1} with a corotation radius of 9.03 kpc. In addition to the good agreement between the calculated and the observed spiral pattern, the variation of the spiral amplitude can also be naturally reproduced.
Dust acoustic shock wave generation due to dust charge variation in a dusty plasma
Indian Academy of Sciences (India)
M R Gupta; S Sarkar; M Khan; Samiran Ghosh
2003-12-01
In a dusty plasma, the non-adiabaticity of the charge variation on a dust grain surface results in an anomalous dissipation. Analytical investigation shows that this results in a small but ﬁnite amplitude dust acoustic (DA) wave propagation which is described by the Korteweg–de Vries–Burger equation. Results of the numerical investigation of the propagation of large-amplitude dust acoustic stationary shock wave are presented here using the complete set of non-linear dust ﬂuid equations coupled with the dust charging equation and Poisson equation. The DA waves are of compressional type showing considerable increase of dust density, which is of signiﬁcant importance in astrophysical context as it leads to enhanced gravitational attraction considered as a viable process for star formation. The DA shock transition to its far downstream amplitude is oscillatory in nature due to dust charge ﬂuctuations, the oscillation amplitude and shock width depending on the ratio pd/ch and other plasma parameters.
Mixed density wave state in quasi-2D organic conductor
Energy Technology Data Exchange (ETDEWEB)
Katono, K., E-mail: k_katono@eng.hokudai.ac.jp [Department of Applied Physics, Hokkaido University, Sapporo 060-8628 (Japan); Ichimura, K. [Department of Applied Physics, Hokkaido University, Sapporo 060-8628 (Japan); Center of Education and Research for Topological Science and Technology, Hokkaido University, Sapporo 060-8628 (Japan); Kawashima, Y.; Yamaya, K. [Department of Applied Physics, Hokkaido University, Sapporo 060-8628 (Japan); Tanda, S. [Department of Applied Physics, Hokkaido University, Sapporo 060-8628 (Japan); Center of Education and Research for Topological Science and Technology, Hokkaido University, Sapporo 060-8628 (Japan)
2012-06-01
The density wave phase of {alpha}-(BEDT-TTF){sub 2}KHg(SCN){sub 4} was investigated by transport properties and magnetic susceptibility. The density wave transition was observed as a broad increase at T{sub DW}=9 K by resistance measurement. Temperature dependence of the static magnetic susceptibility {chi} shows a large Curie tail below 100 K. By subtracting the Curie component, we found that the magnetic susceptibility increases like weak ferromagnetism with decreasing temperature below 7.4 K. The gradual increase of {chi} below T{sub DW} is not expected in simple CDW or SDW, where the magnetic susceptibility decreases with decreasing temperature due to the reduction of Pauli paramagnetic component. To explain the weak ferromagnetic behavior, we consider the coexistence of CDW and SDW. We propose a model of the mixed density wave, where CDW exists with antiferromagnetically coupled canting spins.
Mixed density wave state in quasi-2D organic conductor
Katono, K.; Ichimura, K.; Kawashima, Y.; Yamaya, K.; Tanda, S.
2012-06-01
The density wave phase of α-(BEDT-TTF)2KHg(SCN)4 was investigated by transport properties and magnetic susceptibility. The density wave transition was observed as a broad increase at TDW=9 K by resistance measurement. Temperature dependence of the static magnetic susceptibility χ shows a large Curie tail below 100 K. By subtracting the Curie component, we found that the magnetic susceptibility increases like weak ferromagnetism with decreasing temperature below 7.4 K. The gradual increase of χ below TDW is not expected in simple CDW or SDW, where the magnetic susceptibility decreases with decreasing temperature due to the reduction of Pauli paramagnetic component. To explain the weak ferromagnetic behavior, we consider the coexistence of CDW and SDW. We propose a model of the mixed density wave, where CDW exists with antiferromagnetically coupled canting spins.
Enhanced propagation of photon density waves in random amplifying media
Renthlei, Lalruatfela; Ramakrishna, S A
2013-01-01
We demonstrate enhanced wave-like character of diffuse photon density waves (DPDW) in an amplifying random medium. The amplifying nature makes it contingent to choose the wave solution that grows inside the amplifying medium, and has a propagation vector pointing opposite to the growth direction. This results in negative refraction of the DPDW at an absorbing-amplifying random medium interface as well as the possibility of supporting "anti"-surface-like modes at the interface. A slab of amplifying random medium sandwiched between two absorbing random media supports waveguide resonances that can be utilized to extend the imaging capabilities of DPDW.
Energy density and energy flow of magnetoplasmonic waves on graphene
Moradi, Afshin
2017-03-01
By means the linearized magnetohydrodynamic theory, expressions for energy density and energy flow are derived for the p-polarized surface magnetoplasmon polaritons on graphene in the Voigt configuration, where a static magnetic field is normal to the graphene surface. Numerical results show that the external magnetic field has significant impact on the energy density and energy transport velocity of magnetoplasmon waves in the long-wavelength region, while total power flow vary only weakly with magnetostatic field. The velocity of energy propagation is proved to be identical with group velocity of the surface waves.
Luther-Emery Phase and Atomic-Density Waves in a Trapped Fermion Gas
Xianlong, Gao; Rizzi, M.; Polini, Marco; Fazio, Rosario; Tosi, M. P.; Campo, V. L., Jr.; Capelle, K.
2007-01-01
The Luther-Emery liquid is a state of matter that is predicted to occur in one-dimensional systems of interacting fermions and is characterized by a gapless charge spectrum and a gapped spin spectrum. In this Letter we discuss a realization of the Luther-Emery phase in a trapped cold-atom gas. We study by means of the density-matrix renormalization-group technique a two-component atomic Fermi gas with attractive interactions subject to parabolic trapping inside an optical lattice. We demonstrate how this system exhibits compound phases characterized by the coexistence of spin pairing and atomic-density waves. A smooth crossover occurs with increasing magnitude of the atom-atom attraction to a state in which tightly bound spin-singlet dimers occupy the center of the trap. The existence of atomic-density waves could be detected in the elastic contribution to the light-scattering diffraction pattern.
Plane density of induced vacuum charge in a supercritical Coulomb potential
Khalilov, V R
2016-01-01
An expression for the density of a planar induced vacuum charge is obtained in a strong Coulomb potential in coordinate space. Treatment is based on a self-adjoint extension approach for constructing of the Green's function of a charged fermion in this potential. Induced vacuum charge density is calculated and analyzed at the subcritical and supercritical Coulomb potentials for massless and massive fermions. The behavior of the obtained vacuum charge density is investigated at long and short distances from the Coulomb center. The induced vacuum charge has a screening sign. Screening of a Coulomb impurity in graphene is briefly discussed. We calculate the real vacuum polarization charge density that acquires the quantum electrodynamics vacuum in the supercritical Coulomb potential due to the so-called real vacuum polarization. It is shown that the vacuum charge densities essentially differ in massive and massless cases. We expect that our results can, as a matter of principle, be tested in graphene with a supe...
Response of Charged Particles in a Storage Ring to Gravitational Waves
Institute of Scientific and Technical Information of China (English)
DONG Dong; HUANG Chao-Guang
2003-01-01
The influence of gravitational waves on the charged particles in a storage ring is studied. It shows thatthe gravitational waves might be directly detected by monitoring the motion of charged particles in a storage ring. Theangular velocity of the charged particles is continually adjustable by changing the initial energy of particles and thestrength of the magnetic field. This feature is very useful for finding the gravitational waves with different frequencies.
Response of Charged Particles in a Storage Ring to Gravitational Waves
Institute of Scientific and Technical Information of China (English)
DONGDong; HUANGChao-Guang
2003-01-01
The influence of gravitational waves on the charged particles in a storage ring is studied. It shows that the gravitational waves might be directly detected by monitoring the motion of charged particles in a storage ring. The angular velocity of the charged particles is continually adjustable by changing the initial energy of particles and the strength of the magnetic field. This feature is very useful for finding the gravitational waves with different frequencies.
Application of singular perturbation method in analyzing traffic density waves
Institute of Scientific and Technical Information of China (English)
SHEN Fei-ying; GE Hong-xia; LEI Li
2009-01-01
Car following model is one of microscopic models for describing traffic flow. Through linear stability analysis, the neutral stability lines and the critical points are obtained for the different types of car following models and two modified models. The singular perturbation method has been used to derive various nonlinear wave equations, such as the Korteweg-de-Vries (KdV) equation and the modified Korteweg-de-Vries (mKdV) equation, which could describe different density waves occurring in traffic flows under certain conditions. These density waves are mainly employed to depict the formation of traffic jams in the congested traffic flow. The general soliton solutions are given for the different types of car following models, and the results have been used to the modified models efficiently.
Spiral Density Waves in a Young Protoplanetary Disk
Pérez, Laura M; Andrews, Sean M; Ricci, Luca; Isella, Andrea; Linz, Hendrik; Sargent, Anneila I; Wilner, David J; Henning, Thomas; Deller, Adam T; Chandler, Claire J; Dullemond, Cornelis P; Lazio, Joseph; Menten, Karl M; Corder, Stuartt A; Storm, Shaye; Testi, Leonardo; Tazzari, Marco; Kwon, Woojin; Calvet, Nuria; Greaves, Jane S; Harris, Robert J; Mundy, Lee G
2016-01-01
Gravitational forces are expected to excite spiral density waves in protoplanetary disks, disks of gas and dust orbiting young stars. However, previous observations that showed spiral structure were not able to probe disk midplanes, where most of the mass is concentrated and where planet formation takes place. Using the Atacama Large Millimeter/submillimeter Array we detected a pair of trailing symmetric spiral arms in the protoplanetary disk surrounding the young star Elias 2-27. The arms extend to the disk outer regions and can be traced down to the midplane. These millimeter-wave observations also reveal an emission gap closer to the star than the spiral arms. We argue that the observed spirals trace shocks of spiral density waves in the midplane of this young disk.
Coexistence of superconductivity and density waves in quasi-two-dimensional metals
Energy Technology Data Exchange (ETDEWEB)
Ismer, Jan-Peter
2011-06-03
This dissertation deals with the high-temperature superconductivity in the hole- and electron-doped copper superconductors. In the first part, superconducting phases are investigated on a background of different types of density waves. Singlet superconductivity is studied with s- and d-wave symmetry on a background of spin, charge or D-density waves with respect to stability as well as phase structure and impulse dependence of the gap function. In the second part, the dynamic spin susceptibility for different phases is calculated and compared with experimental data extracted from results of inelastic neutron scattering experiments. The observed phases are d-wave superconductivity, D-density wave, and coexistence of the two. For d-wave superconductivity, the influence of a magnetic field parallel to the copper oxide layer and the temperature development of the susceptibility when for T >> T{sub c} a spin density wave phase is present are investigated. [German] Diese Dissertation beschaeftigt sich mit der Hochtemperatursupraleitung in den loch- und elektron-dotierten Kuprat-Supraleitern. Im ersten Teil der Arbeit werden supraleitende Phasen auf einem Hintergrund verschiedener Typen von Dichtewellen untersucht. Es wird Singlett-Supraleitung mit s- und d-Wellen-Symmetrie auf einem Hintergrund von Spin-, Ladungs- oder D-Dichtewelle hinsichtlich Stabilitaet sowie Phasenstruktur und Impulsabhaengigkeit der Gapfunktion untersucht. Im zweiten Teil wird die dynamische Spinsuszeptibilitaet fuer verschiedene Phasen berechnet und mit experimentellen Daten verglichen, die aus Ergebnissen von Inelastischen Neutronenstreuungsexperimenten extrahiert wurden. Die betrachteten Phasen sind d-Wellen-Supraleitung, D-Dichtewelle und Koexistenz der beiden. Fuer d-Wellen-Supraleitung werden der Einfluss eines Magnetfelds parallel zur Kupferoxidschicht und die Temperaturentwicklung der Suszeptibilitaet, wenn fuer T >> T{sub c} eine Spin-Dichtewelle-Phase vorliegt, untersucht.
Propagation of waves in a multicomponent plasma having charged dust particles
Indian Academy of Sciences (India)
Sukanya Burman; A Roy Chowdhury; S N Paul
2001-06-01
Propagation of both low and high frequency waves in a plasma consisting of electrons, ions, positrons and charged dust particles have been theoretically studied. The characteristics of dust acoustic wave propagating through the plasma has been analysed and the dispersion relation deduced is a generalization of that obtained by previous authors. It is found that nonlinear localization of high frequency electromagnetic ﬁeld in such a plasma generates magnetic ﬁeld. This magnetic ﬁeld is seen to depend on the temperatures of electrons and positrons and also on their equilibrium density ratio. It is suggested that the present model would be applicable to ﬁnd the magnetic ﬁeld generation in space plasma.
Numerical Study of Stratified Charge Combustion in Wave Rotors
Nalim, M. Razi
1997-01-01
A wave rotor may be used as a pressure-gain combustor effecting non-steady flow, and intermittent, confined combustion to enhance gas turbine engine performance. It will be more compact and probably lighter than an equivalent pressure-exchange wave rotor, yet will have similar thermodynamic and mechanical characteristics. Because the allowable turbine blade temperature limits overall fuel/air ratio to sub-flammable values, premixed stratification techniques are necessary to burn hydrocarbon fuels in small engines with compressor discharge temperature well below autoignition conditions. One-dimensional, unsteady numerical simulations of stratified-charge combustion are performed using an eddy-diffusivity turbulence model and a simple reaction model incorporating a flammability limit temperature. For good combustion efficiency, a stratification strategy is developed which concentrates fuel at the leading and trailing edges of the inlet port. Rotor and exhaust temperature profiles and performance predictions are presented at three representative operating conditions of the engine: full design load, 40% load, and idle. The results indicate that peak local gas temperatures will result in excessive temperatures within the rotor housing unless additional cooling methods are used. The rotor itself will have acceptable temperatures, but the pattern factor presented to the turbine may be of concern, depending on exhaust duct design and duct-rotor interaction.
Characteristics and mechanisms of strain waves generated in rock by cylindrical explosive charges
Institute of Scientific and Technical Information of China (English)
刘科伟; 李萧翰; 李夕兵; 姚志华; 舒宗宪; 袁明华
2016-01-01
A superposing principle, by suitably adding the strain waves from a number of concentrated explosive charges to approximate the waves generated by a cylindrical charge based on the strain wave of a point or small spherical explosive charge generated in rock, is used to further study the triggering time of strain gauges installed in radial direction at same distances but different positions surrounding a cylindrical explosive charge in rock. The duration of the first compression phase and peak value of strain wave, and furthermore, their differences are analyzed and some explanations are given. Besides that, the gauge orientation in which the maximum peak value occurs is also discussed. At last, the effect of velocity of detonation (V.O.D.) of a cylindrical explosive charge on the strain waves generated in the surrounding rock is taken as key research and the pattern of peak amplitude of a strain wave varies with the V.O.D. is likely to have been found.
Charge Fluctuation of Dust Grain and Its Impact on Dusty-Acoustic Wave Damping
Atamaniuk, B
2007-01-01
We consider the influence of dust charge fluctuations on damping of the dust-ion-acoustic waves. It is assumed that all grains have equal masses but charges are not constant in time - they may fluctuate in time. The dust charges are not really independent of the variations in the plasma potentials. All modes will influence the charging mechanism, and feedback will lead to several new interesting and unexpected phenomena. The charging of the grains depends on local plasma characteristics. If the waves disturb these characteristic, then charging of the grains is affected and the grain charge is modified, with a resulting feedback on the wave mode. In the case considered here, when the temperature of electrons is much greater than the temperature of the ions and the temperature of electrons is not great enough for further ionization of the ions, we show that attenuation of the acoustic wave depends only on one phenomenological coefficient
Experimental surface charge density of the Si (100)-2x1H surface
DEFF Research Database (Denmark)
Ciston, J.; Marks, L.D.; Feidenhans'l, R.;
2006-01-01
We report a three-dimensional charge density refinement from x-ray diffraction intensities of the Si (100) 2x1H surface. By paying careful attention to parameterizing the bulk Si bonding, we are able to locate the hydrogen atoms at the surface, which could not be done previously. In addition, we...... are able to partially refine the local charge density at the surface. We find experimentally an increased, slightly localized bond density of approximately 0.31 electrons between each Si atom pair at the surface. Both the atomic positions and the charge density are in remarkably good agreement with density...
Waves in cell monolayer without proliferation: density determines cell velocity and wave celerity
Tlili, S; Li, B; Cardoso, O; Ladoux, B; Delanoë-Ayari, H; Graner, F
2016-01-01
Collective cell migration contributes to morphogenesis, wound healing or tumor metastasis. Culturing epithelial monolayers on a substrate is an in vitro configuration suitable to quantitatively characterize such tissue migration by measuring cell velocity, density and cell-substrate interaction force. Inhibiting cell division, we limit cell density increase and favor steady cell migration, while by using long narrow strips we stabilise the migrating front shape, so that we observe migration over a day or more. In the monolayer bulk, the cell velocity is a function of the cell density, namely it increases as a linear function of the cell radius. At least ten periods of propagating velocity waves are detected with a high signal-to-noise ratio, enabling for their quantitative spatio-temporal analysis. Cell density displays waves, in phase opposition with the velocity, as predicted by mass conservation; similarly, cell-substrate force appear to display small amplitude waves, in phase quadrature with respect to ve...
The B-ring's surface mass density from hidden density waves: Less than meets the eye?
Hedman, M M
2016-01-01
Saturn's B ring is the most opaque ring in our solar system, but many of its fundamental parameters, including its total mass, are not well constrained. Spiral density waves generated by mean-motion resonances with Saturn's moons provide some of the best constraints on the rings' mass density, but detecting and quantifying such waves in the B ring has been challenging because of this ring's high opacity and abundant fine-scale structure. Using a wavelet-based analyses of 17 occultations of the star gamma Crucis observed by the Visual and Infrared Mapping Spectrometer (VIMS) onboard the Cassini spacecraft, we are able to examine five density waves in the B ring. Two of these waves are generated by the Janus 2:1 and Mimas 5:2 Inner Lindblad Resonances at 96,427 km and 101,311 km from Saturn's center, respectively. Both of these waves can be detected in individual occultation profiles, but the multi-profile wavelet analysis reveals unexpected variations in the pattern speed of the Janus 2:1 wave that might arise...
The density stratification and amplitude dispersion of internal waves
Makarenko, N.; Ulanova, E.
2012-04-01
We consider the theoretical model of large amplitude internal solitary waves propagating in a weakly stratified fluid under gravity. It is well known that steady 2D Euler equations of non-homogeneous fluid reduce in this case to the second-order quasi-linear equation for a stream function (the Dubreil-Jacotin-Long equation). Subsequently, the shape of traveling solitary wave can be determined in the long-wave scaling limit by solving the dispersive KdV-type model equation. The non-linear terms of this equation depend considerably on the instantaneous fine-scale density profile formed over background linear- or exponential stratification (Benney&Ko, 1978; Borisov&Derzho 1990; Derzho&Grimshaw 1997; Makarenko, 1999; Makarenko, Maltseva and Kazakov, 2009). Now we derive and analyze Fredholm-type integral equations coupling immediately the fluid density coefficient with the dispersion function for internal solitary waves. The inverse problem which means to find the fine-scale density by known curve of the amplitude dispersion is discussed in more details.
Density-Wave Spiral Theories in the 1960s. I
Pasha, I I
2004-01-01
With the arrival of computers, plasma physics and several fresh investigators by the early 1960s, understanding the spiral structure of galaxies entered a new stage of unusually vigorous activity broadly grouped under the umbrella marked "density-wave theory". Paper I starts with acknowledging B. Lindblad, rightly regarded the main father of this whole subject, and then describes the early contributions by Lynden-Bell, Toomre, Hunter and Kalnajs, who had formulated and applied such notions as the stability of flat galaxies, the regenerative spiral phenomenon, the shearing density waves and the global spiral modes. But the foremost enthusiast and proponent of the density-wave picture was undoubtedly C.C. Lin whose 1964 and 1966 papers with Shu, written in support of his working hypothesis of the quasi-stationary wave-mode spiral structure, had a big and immediate impact upon astronomers, at least as a welcome sign that genuine understanding of the spiral phenomenon seemed in some sense to be just around the co...
Observations of ULF wave related equatorial electrojet and density fluctuations
Yizengaw, E.; Zesta, E.; Biouele, C. M.; Moldwin, M. B.; Boudouridis, A.; Damtie, B.; Mebrahtu, A.; Anad, F.; Pfaff, R. F.; Hartinger, M.
2013-10-01
We report on Pc5 wave related electric field and vertical drift velocity oscillations at the equator as observed by ground magnetometers for an extended period on 9 August 2008. We show that the magnetometer-estimated equatorial E×B drift oscillates with the same frequency as ULF Pc5 waves, creating significant ionospheric density fluctuations. We also show ionospheric density fluctuations during the period when we observed ULF wave activity. At the same time, we detect the ULF activity on the ground using ground-based magnetometer data from the African Meridian B-field Education and Research (AMBER) and the South American Meridional B-field Array (SAMBA). From space, we use magnetic field observations from the GOES 12 and the Communication/Navigation Outage and Forecast System (C/NOFS) satellites. Upstream solar wind conditions are provided by the ACE spacecraft. We find that the wave power observed on the ground also occurs in the upstream solar wind and in the magnetosphere. All these observations demonstrate that Pc5 waves with a likely driver in the solar wind can penetrate to the equatorial ionosphere and modulate the equatorial electrodynamics. While no direct drift measurements from equatorial radars exist for the 9 August 2008 event, we used JULIA 150 km radar drift velocities observed on 2 May 2010 and found similar fluctuations with the period of 5-8 min, as a means of an independent confirmation of our magnetometer derived drift dynamics.
Rendering high charge density of states in ionic liquid-gated MoS 2 transistors
Lee, Y.; Lee, J.; Kim, S.; Park, H.S.
2014-01-01
We investigated high charge density of states (DOS) in the bandgap of MoS2 nanosheets with variable temperature measurements on ionic liquid-gated MoS2 transistors. The thermally activated charge transport indicates that the electrical current in the two-dimensional MoS 2 nanosheets under high charg
Directory of Open Access Journals (Sweden)
D. K. Narvilkar
1979-07-01
Full Text Available In the present paper, the equations of internal ballistics of composite charge consisting of N component charge with quadratic form are solved. Largange density approximation and hydrodynamic flow behaviour, have been assumed and the solutions are obtained for the composite charge for these assumptions.
Ultrafast Spin Density Wave Transition in Chromium Governed by Thermalized Electron Gas
Nicholson, C. W.; Monney, C.; Carley, R.; Frietsch, B.; Bowlan, J.; Weinelt, M.; Wolf, M.
2016-09-01
The energy and momentum selectivity of time- and angle-resolved photoemission spectroscopy is exploited to address the ultrafast dynamics of the antiferromagnetic spin density wave (SDW) transition photoexcited in epitaxial thin films of chromium. We are able to quantitatively extract the evolution of the SDW order parameter Δ through the ultrafast phase transition and show that Δ is governed by the transient temperature of the thermalized electron gas, in a mean field description. The complete destruction of SDW order on a sub-100 fs time scale is observed, much faster than for conventional charge density wave materials. Our results reveal that equilibrium concepts for phase transitions such as the order parameter may be utilized even in the strongly nonadiabatic regime of ultrafast photoexcitation.
Enhanced propagation of photon density waves in random amplifying media
Renthlei, Lalruatfela; Wanare, Harshawardhan; Ramakrishna, S. Anantha
2015-04-01
We demonstrate enhanced wavelike character of diffuse photon density waves (DPDW) in an amplifying random medium. The amplifying nature makes it necessary to choose the wave solution that grows inside the amplifying medium, and has a propagation vector pointing opposite to the growth direction. This results in negative refraction of the DPDW at an absorbing-amplifying random medium interface as well as the possibility of supporting "anti"-surface-like modes at the interface. A slab of an amplifying random medium sandwiched between two absorbing random media supports waveguide resonances that can be utilized to extend the imaging capabilities of DPDW.
A gravitational test of wave reinforcement versus fluid density models
Johnson, Jacqueline Umstead
1990-10-01
Spermatozoa, protozoa, and algae form macroscopic patterns somewhat analogous to thermally driven convection cells. These bioconvective patterns have attracted interest in the fluid dynamics community, but whether in all cases these waves were gravity driven was unknown. There are two conflicting theories, one gravity dependent (fluid density model), the other gravity independent (wave reinforcement theory). The primary objectives of the summer faculty fellows were to: (1) assist in sample collection (spermatozoa) and preparation for the KC-135 research airplane experiment; and (2) to collaborate on ground testing of bioconvective variables such as motility, concentration, morphology, etc., in relation to their macroscopic patterns. Results are very briefly given.
Farris, Stefano; Mora, Luigi; Capretti, Giorgio; Piergiovanni, Luciano
2012-01-01
An easy analytical method for determination of the charge density of polyelectrolytes, including polysaccharides and other biopolymers, is presented. The basic principles of conductometric titration, which is used in the pulp and paper industry as well as in colloid and interface science, were adapted to quantify the charge densities of a…
Frequency clusters in self-excited dust density waves
Menzel, Kristoffer O.; Arp, Oliver; Piel, Alexander
2010-11-01
Self-excited dust density waves were studied under microgravity conditions. Their non-sinusoidal shape and high degrees of modulation suggests that nonlinear effects play an important role in their spatio-temporal dynamics. The resulting complex wave pattern is analyzed in great detail by means of the Hilbert transform, which provides instantaneous wave attributes, such as the phase and the frequency. Our analysis showed that the spatial frequency distribution of the DDWs is usually not constant over the dust cloud. In contrast, the wave field is divided into regions of different but almost constant frequencies [1]. The boundaries of these so-called frequency clusters coincide with the locations of phase defects in the wave field. It is found that the size of the clusters depends on the strength of spatial gradients in the plasma parameters. We attribute the formation of frequency clusters to synchronization phenomena as a consequence of the nonlinear character of the wave.[1] K. O. Menzel, O. Arp, A.Piel, Phys. Rev. Lett. 104, 235002 (2010)
Empirical transverse charge densities in the nucleon and the nucleon-to-Delta transition
Energy Technology Data Exchange (ETDEWEB)
Carl Carlson; Marc Vanderhaeghen
2008-01-01
Using only the current empirical information on the nucleon electromagnetic form factors we map out the transverse charge density in proton and neutron as viewed from a light front moving towards a transversely polarized nucleon. These charge densities are characterized by a dipole pattern, in addition to the monopole field corresponding with the unpolarized density. Furthermore, we use the latest empirical information on the $N \\to \\Delta$ transition form factors to map out the transition charge density which induces the $N \\to \\Delta$ excitation. This transition charge density in a transversely polarized $N$ and $\\Delta$ contains both monopole, dipole and quadrupole patterns, the latter corresponding with a deformation of the hadron's charge distribution.
Linear density response function in the projector augmented wave method
DEFF Research Database (Denmark)
Yan, Jun; Mortensen, Jens Jørgen; Jacobsen, Karsten Wedel;
2011-01-01
We present an implementation of the linear density response function within the projector-augmented wave method with applications to the linear optical and dielectric properties of both solids, surfaces, and interfaces. The response function is represented in plane waves while the single......-particle eigenstates can be expanded on a real space grid or in atomic-orbital basis for increased efficiency. The exchange-correlation kernel is treated at the level of the adiabatic local density approximation (ALDA) and crystal local field effects are included. The calculated static and dynamical dielectric...... functions of Si, C, SiC, AlP, and GaAs compare well with previous calculations. While optical properties of semiconductors, in particular excitonic effects, are generally not well described by ALDA, we obtain excellent agreement with experiments for the surface loss function of graphene and the Mg(0001...
Spin density wave order, topological order, and Fermi surface reconstruction
Sachdev, Subir; Chatterjee, Shubhayu; Schattner, Yoni
2016-01-01
In the conventional theory of density wave ordering in metals, the onset of spin density wave (SDW) order co-incides with the reconstruction of the Fermi surfaces into small 'pockets'. We present models which display this transition, while also displaying an alternative route between these phases via an intermediate phase with topological order, no broken symmetry, and pocket Fermi surfaces. The models involve coupling emergent gauge fields to a fractionalized SDW order, but retain the canonical electron operator in the underlying Hamiltonian. We establish an intimate connection between the suppression of certain defects in the SDW order, and the presence of Fermi surface sizes distinct from the Luttinger value in Fermi liquids. We discuss the relevance of such models to the physics of the hole-doped cuprates near optimal doping.
Effects of charged sand on electromagnetic wave propagation and its scattering field
Institute of Scientific and Technical Information of China (English)
HE; Qinshu; ZHOU; Youhe; ZHENG; Xiaojing
2006-01-01
Based on the Rayleigh's scattering theory, the effects of sandstorms on the propagation of electromagnetic wave with different visibilities are presented by solving the scattering field of charged sand particles. Because of the electric charges on the sand surface, the theoretical attenuation will be large enough to match the measured value under certain conditions. And the results show that the effect of sand with electric charges all over its surface on electromagnetic wave attenuation is the same as that of sand without charge, which proves that electric charges distribute on partial surface of the sand in fact.
From super-charged nuclei to massive nuclear density cores
Popov, Vladimir
2010-01-01
Due to $e^+e^-$-pair production in the field of supercritical $(Z \\gg Z_{cr}\\approx 170 $) nucleus an electron shell, created out of the vacuum, is formed. The distribution of the vacuum charge in this shell has been determined for super-charged nuclei $Ze^3 \\ga 1$ within the framework of the Thomas-Fermi equation generalized to the relativistic case. For $Ze^3 \\gg 1$ the electron shell penetrates inside the nucleus and almost completely screens its charge. Inside such nucleus the potential takes a constant value equal to $V_0=-(3\\pi^2 n_p)^{1/3} \\sim -2m_{\\pi}c^2$, and super-charged nucleus represents an electrically neutral plasma consisting of $e,p$ and $n$. Near the edge of the nucleus a transition layer exists with a width $\\lambda \\approx \\alpha^{-1/2} \\hbar/m_{\\pi} c\\sim 15$ fm, which is independent of $Z~~ (\\hbar/m_{\\pi} c \\ll \\lambda \\ll \\hbar/m_e c)$. The electric field and surface charge are concentrated in this layer. These results, obtained earlier for hypothetical superheavy nuclei with $Z \\sim ...
Spin density waves predicted in zigzag puckered phosphorene, arsenene and antimonene nanoribbons
Wu, Xiaohua; Zhang, Xiaoli; Wang, Xianlong; Zeng, Zhi
2016-04-01
The pursuit of controlled magnetism in semiconductors has been a persisting goal in condensed matter physics. Recently, Vene (phosphorene, arsenene and antimonene) has been predicted as a new class of 2D-semiconductor with suitable band gap and high carrier mobility. In this work, we investigate the edge magnetism in zigzag puckered Vene nanoribbons (ZVNRs) based on the density functional theory. The band structures of ZVNRs show half-filled bands crossing the Fermi level at the midpoint of reciprocal lattice vectors, indicating a strong Peierls instability. To remove this instability, we consider two different mechanisms, namely, spin density wave (SDW) caused by electron-electron interaction and charge density wave (CDW) caused by electron-phonon coupling. We have found that an antiferromagnetic Mott-insulating state defined by SDW is the ground state of ZVNRs. In particular, SDW in ZVNRs displays several surprising characteristics:1) comparing with other nanoribbon systems, their magnetic moments are antiparallelly arranged at each zigzag edge and almost independent on the width of nanoribbons; 2) comparing with other SDW systems, its magnetic moments and band gap of SDW are unexpectedly large, indicating a higher SDW transition temperature in ZVNRs; 3) SDW can be effectively modified by strains and charge doping, which indicates that ZVNRs have bright prospects in nanoelectronic device.
Modulated spin and charge densities in cuprate superconductors
Tranquada, J. M.
1997-01-01
Neutron scattering experiments have played a crucial role in characterizing the spin and charge correlations in copper-oxide superconductors. While the data are often interpreted with respect to specific theories of the cuprates, an attempt is made here to distinguish those facts that can be extracted empirically, and the connections that can be made with minimal assumptions.
The density wave in a new anisotropic continuum model
Institute of Scientific and Technical Information of China (English)
Ge Hong-Xia; Dai Shi-Qiang; Dong Li-Yun
2008-01-01
In this paper the new continuum traffic flow model proposed by Jiang et al is developed based on an improved car-following model,in which the speed gradient term replaces the density gradient term in the equation of motion.It overcomes the wrong-way travel which exists in many high-order continuum models.Based on the continuum version of car-following model,the condition for stable traffic flow is derived.Nonlinear analysis shows that the density fluctuation in traffic flow induces a variety of density waves.Near the onset of instability,a small disturbance could lead to solitons determined by the Korteweg-de-Vries (KdV) equation,and the soliton solution is derived.
Molecular Weight and Charge Density Asymmetry in Polyelectrolyte Complexation
Audus, Debra; Fredrickson, Glenn; Duechs, Dominik
2009-03-01
We investigate the phase diagram of oppositely charged polymers in a good solvent using a field-theoretic model. Mean-field solutions fail to predict the experimentally observed macroscopic phase separation into a solvent-rich phase and a dense liquid aggregate of polymers - a ``complex coacervate.'' We therefore study the model within a one-loop approximation, which accounts for Gaussian fluctuations in electrostatic and chemical potentials. Our particular focus is the effect of molecular weight, ionic strength, and charge asymmetry on the phase envelope. A set of dimensionless parameters is identified that dictate the size and shape of the two-phase region. Our results should be helpful in guiding experimental studies of coacervation.
Influence of electric charge and modified gravity on density irregularities
Energy Technology Data Exchange (ETDEWEB)
Bhatti, M.Z. Ul Haq; Yousaf, Z. [University of the Punjab, Department of Mathematics, Lahore (Pakistan)
2016-04-15
This work aims to identify some inhomogeneity factors for a plane symmetric topology with anisotropic and dissipative fluid under the effects of both electromagnetic field as well as Palatini f(R) gravity. We construct the modified field equations, kinematical quantities, and mass function to continue our analysis. We have explored the dynamical quantities, conservation equations and modified Ellis equations with the help of a viable f(R) model. Some particular cases are discussed with and without dissipation to investigate the corresponding inhomogeneity factors. For a non-radiating scenario, we examine such factors as dust, and isotropic and anisotropic matter in the presence of charge. For a dissipative fluid, we investigate the inhomogeneity factor with a charged dust cloud. We conclude that the electromagnetic field increases the inhomogeneity in matter while the extra curvature terms make the system more homogeneous with the evolution of time. (orig.)
Influence of Electric Charge and Modified Gravity on Density Irregularities
Bhatti, M Zaeem Ul Haq
2016-01-01
This work aims to identify some inhomogeneity factors for plane symmetric topology with anisotropic and dissipative fluid under the effects of both electromagnetic field as well as Palatini $f(R)$ gravity. We construct the modified field equations, kinematical quantities and mass function to continue our analysis. We have explored the dynamical quantities, conservation equations and modified Ellis equations with the help of a viable $f(R)$ model. Some particular cases are discussed with and without dissipation to investigate the corresponding inhomogeneity factors. For non-radiating scenario, we examine such factors with dust, isotropic and anisotropic matter in the presence of charge. For dissipative fluid, we investigate the inhomogeneity factor with charged dust cloud. We conclude that electromagnetic field increases the inhomogeneity in matter while the extra curvature terms make the system more homogeneous with the evolution of time.
Peltier effect in multilayered nanopillars under high density charge current
Gravier, L.; Fukushima, A.; Kubota, H.; Yamamoto, A.; Yuasa, S.
2006-12-01
From the basic equations of thermoelectricity, we model the thermal regimes that develop in multilayered nanopillar elements experiencing continuous charge currents. The energy conservation principle was applied to all layer-layer and layer-electrode junctions. The obtained set of equations was solved to derive the temperature of each junction. The contribution of the Peltier effect is included in an effective resistance. This model gives satisfactory fits to experimental data obtained on a series of reference nanopillar elements.
Peltier effect in multilayered nanopillars under high density charge current
Energy Technology Data Exchange (ETDEWEB)
Gravier, L [Institut de Physique des Nanostructures, Ecole Polytechnique Federale de Lausanne (EPFL), EPFL-SB-IPN station 3, 1015 Lausanne (Switzerland); Fukushima, A [National Institute of Advances Industrial Science and Technology (AIST) 1-1-1 Umezono, Tsukuba, Ibaraki 305-8568 (Japan); Kubota, H [National Institute of Advances Industrial Science and Technology (AIST) 1-1-1 Umezono, Tsukuba, Ibaraki 305-8568 (Japan); Yamamoto, A [National Institute of Advances Industrial Science and Technology (AIST) 1-1-1 Umezono, Tsukuba, Ibaraki 305-8568 (Japan); Yuasa, S [National Institute of Advances Industrial Science and Technology (AIST) 1-1-1 Umezono, Tsukuba, Ibaraki 305-8568 (Japan)
2006-12-21
From the basic equations of thermoelectricity, we model the thermal regimes that develop in multilayered nanopillar elements experiencing continuous charge currents. The energy conservation principle was applied to all layer-layer and layer-electrode junctions. The obtained set of equations was solved to derive the temperature of each junction. The contribution of the Peltier effect is included in an effective resistance. This model gives satisfactory fits to experimental data obtained on a series of reference nanopillar elements.
Melting Point Of Metals In Relation Io Electron Charge Density
Directory of Open Access Journals (Sweden)
Boczkal G.
2015-09-01
Full Text Available The concept of spatial criterion of the electron charge concentration is applied to determine the metal melting point. Based on the model proposed for bcc metals, a model for hcp metals and general form for others has been developed. To calculate the melting point, only structural data and atomic number are required. The obtained results show good consistency with the experimental data for metals with atomic number Z < 70.
Supersonic Propagation of Heat Waves in Low Density Heavy Material
Institute of Scientific and Technical Information of China (English)
Jiang Shaoen; Zhang Wenhai; Yi Rongqing; Cui Yanli; Chen Jiusen; Xu Yan; Ding Yongkun; Lai Dongxian; Zheng Zhijian; Huang Yikiang; Li Jinghong; Sun Kexu; Hu Xin
2005-01-01
The propagation of a supersonic heat-wave through copper-doped foam with a density of 50 mg/cm3 was experimentally investigated. The wave is driven by 140 eV Holhraum radiations generated in a cylindrical gold cavity heated by a 2 k J, 1ns laser pulse (0.35 μm). The delayed breakout time of the radiation waves from the rear side of the foam is measured by a threechromatic streaked x-ray spectrometer (TCS) consisting of a set of three-imaging pinholes and an array of three transmission gratings coupled with an x-ray streak camera (XSC). With one shot,simultaneous measurements of the delays of the drive source and the radiation with two different energies (210 eV, 840 eV) through the foam have been made for the first time. The experimental results indicate that the time delays vary with photon energies. The radiation with an energy of 210 eV propagates at a lower velocity. The radiating heat wave propagates with a velocity that is larger than the sound speed. Using TGS, the transmitting spectrum was measured, and then lower limit of the optical depth which is more than 1, was obtained. The experimental data were in agreement with numerical simulations.
Charge-density analysis of 1-nitroindoline: refinement quality using free R factors and restraints.
Zarychta, Bartosz; Zaleski, Jacek; Kyzioł, Janusz; Daszkiewicz, Zdzisław; Jelsch, Christian
2011-06-01
Nitramines and related N-nitro compounds have attracted significant attention owing to their use in rocket fuel and as explosives. The charge density of 1-nitroindoline was determined experimentally and from theoretical calculations. Electron-density refinements were performed using the multipolar atom formalism. In order to design the ideal restraint strategy for the charge-density parameters, R-free analyses were performed involving a series of comprehensive refinements. Different weights were applied to the charge-density restraints, namely the similarity between chemically equivalent atoms and local symmetry. Additionally, isotropic thermal motion and an anisotropic model calculated by rigid-body analysis were tested on H atoms. The restraint weights which resulted in the lowest values of the averaged R-free factors and the anisotropic H-atom model were considered to yield the best charge density and were used in the final refinement. The derived experimental charge density along with intra- and intermolecular interactions was analysed and compared with theoretical calculations, notably with respect to the symmetry of multipole parameters. A comparison of different refinements suggests that the appropriate weighting scheme applied to charge-density restraints can reduce the observed artefacts. The topological bond orders of the molecule were calculated.
Imperfect nesting and transport properties in unconventional density waves
Dóra, Balázs; Maki, Kazumi; Virosztek, Attila
2002-10-01
We consider the effect of imperfect nesting in quasi-one-dimensional unconventional density waves (DW's). The phase diagram is very close to those in a conventional DW's. The linear and non-linear aspects of the electric conductivity are discussed. At T=0 the frequency dependent electric conductivity develops a small dip at low frequencies. The threshold electric field depends strongly on the imperfect nesting parameter, allowing us to describe very well the measured threshold electric field in the low temperature phase of the quasi-two-dimensional organic conductor, α-(BEDT-TTF)2KHg(SCN)4.
Wave Localization and Density Bunching in Pair Ion Plasmas
Mahajan, Swadesh M
2008-01-01
By investigating the nonlinear propagation of high intensity electromagnetic (EM) waves in a pair ion plasma, whose symmetry is broken via contamination by a small fraction of high mass immobile ions, it is shown that this new and interesting state of (laboratory created) matter is capable of supporting structures that strongly localize and bunch the EM radiation with density excess in the region of localization. Testing of this prediction in controlled laboratory experiments can lend credence, inter alia, to conjectures on structure formation (via the same mechanism) in the MEV era of the early universe.
Superlattice origin of incommensurable density waves in $La__{2-x}Ae_xCuO4$ (Ae = Ba, Sr)
Bucher, Manfred
2013-01-01
In line with the Coulomb-oscillator model of superconductivity, loop currents of excited 3s electrons from O^2- ions, passing in the CuO2 plane through nuclei of nearest-neighbor oxygen quartets, create the antiferromagnetic phase of undoped copper oxides. Holes, introduced by alkaline-earth doping of La2CuO4, destroy the loop currents, thereby weakening antiferromagnetism until it disappears at doping x = 0.02. Further doping of La_2-xAe_xCuO4 gives rise to incommensurate free-hole density waves whose wavelength is determined by the spacing of a doping superlattice. Modulating the ordering of the ions' magnetic moments, the charge-density wave, of incommensurability 2 delta, causes a magnetic density wave of incommensurability delta. The formula derived for delta(x) is in excellent agreement with data from X-ray diffraction and neutron scattering.
Mapping surface charge density of lipid bilayers by quantitative surface conductivity microscopy
Klausen, Lasse Hyldgaard; Fuhs, Thomas; Dong, Mingdong
2016-08-01
Local surface charge density of lipid membranes influences membrane-protein interactions leading to distinct functions in all living cells, and it is a vital parameter in understanding membrane-binding mechanisms, liposome design and drug delivery. Despite the significance, no method has so far been capable of mapping surface charge densities under physiologically relevant conditions. Here, we use a scanning nanopipette setup (scanning ion-conductance microscope) combined with a novel algorithm to investigate the surface conductivity near supported lipid bilayers, and we present a new approach, quantitative surface conductivity microscopy (QSCM), capable of mapping surface charge density with high-quantitative precision and nanoscale resolution. The method is validated through an extensive theoretical analysis of the ionic current at the nanopipette tip, and we demonstrate the capacity of QSCM by mapping the surface charge density of model cationic, anionic and zwitterionic lipids with results accurately matching theoretical values.
Determination of charge carrier mobility in doped low density polyethylene using DC transients
DEFF Research Database (Denmark)
Khalil, M.Salah; Henk, Peter O; Henriksen, Mogens
1989-01-01
Charge carrier mobility was determined for plain and doped low-density polyethylene (LDPE) using DC transient currents. Barium titanate was used as a strongly polar dopant and titanium dioxide as a semiconductor dopant. The values of the mobility obtained were on the order of 10-10 cm2 v-1 s-1...... by a factor of five. Charge trapping and space charge formation were modified by the introduction of titanium dioxide...
Indian Academy of Sciences (India)
Sourabh Bal; M Bose
2009-10-01
We have investigated analytically the stimulated Brillouin scattering (SBS) of an electromagnetic wave in non-dissipative weakly magnetized plasma in the presence of dust particles with variable charge.
A topological analysis of charge densities in diamond, silicon and germanium crystals
Energy Technology Data Exchange (ETDEWEB)
Abramov, Yu.A. [National Inst. for Research in Inorganic Materials, Tsukuba, Ibaraki (Japan); Okamura, F.P. [National Inst. for Research in Inorganic Materials, Tsukuba, Ibaraki (Japan)
1997-03-01
The Hansen-Coppens multipole model of charge density has been fitted to highly accurate published experimental and theoretical structure factors for diamond, silicon and germanium crystals. Analysis of both model experimental and theoretical charge densities using the resulting model parameters was performed in terms of Bader`s topological theory. The general topology of the charge density appeared to be identical for all crystals, containing the four possible types of critical points of rank three, and no non-nuclear attractors between neighboring atoms were found within achieved accuracy. Theoretical and experimental values of charge density and its Laplacian show quantitative and semiquantitative agreement, respectively, at the critical points of model charge densities. For Ge crystals, such agreement is worse at the ring critical point. These results suggest the possibility of semiquantitative (within 10-30%) study of the topological characteristics of highly accurate X-ray charge densities of crystals displaying shared interatomic interactions. Comparative topological analysis of the chemical bond in this series of crystals is discussed in terms of the quantum topological theory. (orig.).
Directory of Open Access Journals (Sweden)
Yongjun Ahn
Full Text Available The charging infrastructure location problem is becoming more significant due to the extensive adoption of electric vehicles. Efficient charging station planning can solve deeply rooted problems, such as driving-range anxiety and the stagnation of new electric vehicle consumers. In the initial stage of introducing electric vehicles, the allocation of charging stations is difficult to determine due to the uncertainty of candidate sites and unidentified charging demands, which are determined by diverse variables. This paper introduces the Estimating the Required Density of EV Charging (ERDEC stations model, which is an analytical approach to estimating the optimal density of charging stations for certain urban areas, which are subsequently aggregated to city level planning. The optimal charging station's density is derived to minimize the total cost. A numerical study is conducted to obtain the correlations among the various parameters in the proposed model, such as regional parameters, technological parameters and coefficient factors. To investigate the effect of technological advances, the corresponding changes in the optimal density and total cost are also examined by various combinations of technological parameters. Daejeon city in South Korea is selected for the case study to examine the applicability of the model to real-world problems. With real taxi trajectory data, the optimal density map of charging stations is generated. These results can provide the optimal number of chargers for driving without driving-range anxiety. In the initial planning phase of installing charging infrastructure, the proposed model can be applied to a relatively extensive area to encourage the usage of electric vehicles, especially areas that lack information, such as exact candidate sites for charging stations and other data related with electric vehicles. The methods and results of this paper can serve as a planning guideline to facilitate the extensive
Ahn, Yongjun; Yeo, Hwasoo
2015-01-01
The charging infrastructure location problem is becoming more significant due to the extensive adoption of electric vehicles. Efficient charging station planning can solve deeply rooted problems, such as driving-range anxiety and the stagnation of new electric vehicle consumers. In the initial stage of introducing electric vehicles, the allocation of charging stations is difficult to determine due to the uncertainty of candidate sites and unidentified charging demands, which are determined by diverse variables. This paper introduces the Estimating the Required Density of EV Charging (ERDEC) stations model, which is an analytical approach to estimating the optimal density of charging stations for certain urban areas, which are subsequently aggregated to city level planning. The optimal charging station's density is derived to minimize the total cost. A numerical study is conducted to obtain the correlations among the various parameters in the proposed model, such as regional parameters, technological parameters and coefficient factors. To investigate the effect of technological advances, the corresponding changes in the optimal density and total cost are also examined by various combinations of technological parameters. Daejeon city in South Korea is selected for the case study to examine the applicability of the model to real-world problems. With real taxi trajectory data, the optimal density map of charging stations is generated. These results can provide the optimal number of chargers for driving without driving-range anxiety. In the initial planning phase of installing charging infrastructure, the proposed model can be applied to a relatively extensive area to encourage the usage of electric vehicles, especially areas that lack information, such as exact candidate sites for charging stations and other data related with electric vehicles. The methods and results of this paper can serve as a planning guideline to facilitate the extensive adoption of electric
Dust-Acoustic Waves in Strongly Coupled Dusty Plasmas Containing Variable-Charge Impurities
Institute of Scientific and Technical Information of China (English)
XIE Bai-Song; HE Kai-Fen; M. Y. Yu
2000-01-01
A relatively self-consistent theory of dust-acoustic waves in the strongly coupled dusty plasmas containing variable charge impurities is given. Relevant physical processes such as dust elastic relaxation and dust charge relaxation are taken into account. It is shown that the negative dispersion of dust-acoustic waves due to the strong correlation of dusts is enhanced in the presence of dust-neutral collisions.
The KP and ZK equations for electrostatic waves with grain charge fluctuation
Institute of Scientific and Technical Information of China (English)
Xue Ju-Kui; Lang He
2004-01-01
@@ The propagation of three-dimensional nonlinear dust-acoustic and dust-Coulomb waves in unmagnetized/magnetized dusty plasmas consisting of electrons, ions, and charged dust particles is investigated. The grain charge fluctuation effect is also incorporated through the current balance equation. By using the perturbation method,a Kadomtsev-Petviashvili equation and a Zakharov-Kuznetsov equation governing the nonlinear waves in the unmagnetized and magnetized systems are obtained respectively. It has been shown that with the combined effects of grain charge fluctuation, the transverse perturbation, and the external magnetic field would modify the wave structures.Waves in those systems are unstable to the high-order long-wave perturbations.
DEFF Research Database (Denmark)
Benavente, J.; Silva, V.; Pradanos, P.;
2010-01-01
by impedance spectroscopy, and the electric potential drop during retention experiments has also been measured. These experimental data on conductivity and electric potential are analyzed, by using the thermodynamics of irreversible processes and the space charge model, to obtain the pore charge density......A version of the Donnan steric-partitioning pore model with dielectrical exclusion (DSPM-DE) has been used to get information on the pore size and charge density of a commercial membrane, NF45 from FilmTec, from its retention of KCl solutions. The conductivity inside the pores has been measured...
A relativistic non-relativistic Goldstone theorem: gapped Goldstones at finite charge density
Nicolis, Alberto
2012-01-01
We adapt the Goldstone theorem to study spontaneous symmetry breaking in relativistic theories at finite charge density. It is customary to treat systems at finite density via non-relativistic Hamiltonians. Here we highlight the importance of the underlying relativistic dynamics. This leads to seemingly new results whenever the charge in question is spontaneously broken and does not commute with other broken charges. These would normally be associated with gapless Goldstone excitations. We find that, in fact, their currents interpolate gapped excitations. We derive exact non-perturbative expressions for their gaps, in terms of the chemical potential and of the symmetry algebra.
Propagation of dust-acoustic waves in weakly ionized plasmas with dust-charge fluctuation
Indian Academy of Sciences (India)
K K Mondal
2004-11-01
For an unmagnetized partially ionized dusty plasma containing electrons, singly charged positive ions, micron-sized massive negatively charged dust grains and a fraction of neutral atoms, dispersion relations for both the dust-ion-acoustic and the dust-acoustic waves have been derived, incorporating dust charge fluctuation. The dispersion relations, under various conditions, have been exhaustively analysed. The explicit expressions for the growth rates have also been derived.
Institute of Scientific and Technical Information of China (English)
Duan Wen-Shan
2004-01-01
The effect of dust charging and the influence of its adiabatic variation on dust acoustic waves is investigated. By employing the reductive perturbation technique we derived a Zakharov-Kuznetsov (ZK) equation for small amplitude dust acoustic waves. We have analytically verified that there are only rarefactive solitary waves for this system. The instability region for one-dimensional solitary wave under transverse perturbations has also been obtained. The obliquely propagating solitary waves to the z-direction for the ZK equation are given in this paper as well.
Regnier, D; Schunck, N; Verriere, M
2016-01-01
Accurate knowledge of fission fragment yields is an essential ingredient of numerous applications ranging from the formation of elements in the r-process to fuel cycle optimization for nuclear energy. The need for a predictive theory applicable where no data is available is an incentive to develop a fully microscopic approach to fission dynamics. In this work, we calculate the pre-neutron emission charge and mass distributions of the fission fragments formed in the neutron-induced fission of 239Pu using a microscopic method based on nuclear energy density functional (EDF) method, where large amplitude collective motion is treated adiabatically using the time dependent generator coordinate method (TDGCM) under the Gaussian overlap approximation (GOA). Fission fragment distributions are extracted from the flux of the collective wave packet through the scission line. We find that the main characteristics of the fission charge and mass distributions can be well reproduced by existing energy functionals even in tw...
Indian Academy of Sciences (India)
S Haddad
2010-09-01
The influence of the isovector coupling channel on the central depression parameter and the central value of the charge density distribution in heavy spherical nuclei was studied. The isovector coupling channel leads to about 50% increase of the central depression parameter, and weakens the dependency of both central depression parameter and central density on the asymmetry, impressively contributing to the semibubble form of the charge density distribution in heavy nuclei, and increasing the probability of larger nuclei with higher proton numbers and higher neutron-to-proton ratios stable.
Density Functional Theory Approach for Charged Hard Sphere Fluids Confined in Spherical Micro-Cavity
Institute of Scientific and Technical Information of China (English)
KANG Yan-Shuang; WANG Hai-Jun
2009-01-01
Within the framework of the density functional theory for classical fluids,the equilibrium density profiles of charged hard sphere fluid confined in micro-cavity are studied by means of the modified fundamental measure theory.The dimension of micro-cavity,the charge of hard sphere and the applied electric field are found to have significant effects on the density profiles.In particular,it is shown that Coulomb interaction,excluded volume interaction and applied electric Geld play the central role in controlling the aggregated structure of the system.
DEFF Research Database (Denmark)
Bambery, K.R.; Fleming, R.J.; Holbøll, Joachim
2001-01-01
Laser induced pressure pulse space charge measurements were made on 1.5 mm thick plaques of high purity low density polyethylene equipped with vacuum-evaporated aluminium electrodes. Temperature differences up to 20 °C were maintained across the samples, which were subjected to dc fields up to 1.......5×107 V m-1. Current density was also measured as a function of temperature and field. Space charge due exclusively to the temperature gradient was detected, with density of order 0.01 C m-3. The activation energy associated with the transport of electrons through the bulk was calculated as 0.09 e...
Collisionless damping of dust-acoustic waves in a charge varying dusty plasma with nonextensive ions
Energy Technology Data Exchange (ETDEWEB)
Amour, Rabia; Tribeche, Mouloud [Faculty of Physics, Theoretical Physics Laboratory (TPL), Plasma Physics Group (PPG), University of Bab-Ezzouar, USTHB, B.P. 32, El Alia, Algiers 16111 (Algeria)
2014-12-15
The charge variation induced nonlinear dust-acoustic wave damping in a charge varying dusty plasma with nonextensive ions is considered. It is shown that the collisionless damping due to dust charge fluctuation causes the nonlinear dust acoustic wave propagation to be described by a damped Korteweg-de Vries (dK-dV) equation the coefficients of which depend sensitively on the nonextensive parameter q. The damping term, solely due to the dust charge variation, is affected by the ion nonextensivity. For the sake of completeness, the possible effects of nonextensivity and collisionless damping on weakly nonlinear wave packets described by the dK-dV equation are succinctly outlined by deriving a nonlinear Schrödinger-like equation with a complex nonlinear coefficient.
A numerical study on charged-particle scattering and radiography of a steep density gradient
Shao, Guangchao; Wang, Xiaofang
2016-09-01
Electron and proton radiography of polystyrene planar targets with different density gradients is studied by Monte Carlo simulations in a regime that the incident charged-particle's kinetic energy is much higher than its energy loss in the targets. It is shown that by scattering of the electrons or protons, the density gradient causes modulations of the charged-particle beam transmitted from the target and the modulation contrast is sensitive only to a steep gradient, which suggests a novel diagnostic method wherein a steep density gradient could be distinguished from the scattering of a charged-particle beam in radiography. By using a 100-MeV charged-particle beam, it is found that the modulation is evident for a steep density gradient of width smaller than 1 μm for electron radiography and 0.6 μm for proton radiography, respectively, but almost negligible when the density gradient width is greater than 1 μm. The feasibility of diagnosing the steep density gradients in compressed matter is confirmed by the simulations of radiographing a laser-ablated planar foil. Simulations also show that it is possible to diagnose the density gradients inside a multilayered spherical capsule.
Cozma, M. D.
2017-01-01
The charged pion multiplicity ratio in intermediate-energy heavy-ion collisions, a probe of the density dependence of symmetry energy above the saturation point, has been proven in a previous study to be extremely sensitive to the strength of the isovector Δ (1232 ) potential in nuclear matter. As there is no knowledge, either from theory or experiment, about the magnitude of this quantity, the extraction of constraints on the slope of the symmetry energy at saturation by using exclusively the mentioned observable is hindered at present. It is shown that, by including the ratio of average pT of charged pions / in the list of fitted observables, the noted problem can be circumvented. A realistic description of this observable requires accounting for the interaction of pions with the dense nuclear matter environment by the incorporation of the so-called S -wave and P -wave pion optical potentials. This is performed within the framework of a quantum molecular dynamics transport model that enforces the conservation of the total energy of the system. It is shown that constraints on the slope of the symmetry energy at saturation density and the strength of the Δ (1232) potential can be simultaneously extracted. A symmetry energy with a value of the slope parameter L >50 MeV is favored, at 1 σ confidence level, from a comparison with published FOPI experimental data. A precise constraint will require experimental data more accurate than presently available, particularly for the charged pion multiplicity ratio, and better knowledge of the density and momentum dependence of the pion potential for the whole range of these two variables probed in intermediate-energy heavy-ion collisions.
Wave theories of non-laminar charged particle beams: from quantum to thermal regime
Fedele, Renato; Tanjia, Fatema; Jovanović, Dusan; de Nicola, Sergio; Ronsivalle, Concetta; Ronsivalle
2014-04-01
The standard classical description of non-laminar charged particle beams in paraxial approximation is extended to the context of two wave theories. The first theory that we discuss (Fedele R. and Shukla, P. K. 1992 Phys. Rev. A 45, 4045. Tanjia, F. et al. 2011 Proceedings of the 38th EPS Conference on Plasma Physics, Vol. 35G. Strasbourg, France: European Physical Society) is based on the Thermal Wave Model (TWM) (Fedele, R. and Miele, G. 1991 Nuovo Cim. D 13, 1527.) that interprets the paraxial thermal spreading of beam particles as the analog of quantum diffraction. The other theory is based on a recently developed model (Fedele, R. et al. 2012a Phys. Plasmas 19, 102106; Fedele, R. et al. 2012b AIP Conf. Proc. 1421, 212), hereafter called Quantum Wave Model (QWM), that takes into account the individual quantum nature of single beam particle (uncertainty principle and spin) and provides collective description of beam transport in the presence of quantum paraxial diffraction. Both in quantum and quantum-like regimes, the beam transport is governed by a 2D non-local Schrödinger equation, with self-interaction coming from the nonlinear charge- and current-densities. An envelope equation of the Ermakov-Pinney type, which includes collective effects, is derived for both TWM and QWM regimes. In TWM, such description recovers the well-known Sacherer's equation (Sacherer, F. J. 1971 IEEE Trans. Nucl. Sci. NS-18, 1105). Conversely, in the quantum regime and in Hartree's mean field approximation, one recovers the evolution equation for a single-particle spot size, i.e. for a single quantum ray spot in the transverse plane (Compton regime). We demonstrate that such quantum evolution equation contains the same information as the evolution equation for the beam spot size that describes the beam as a whole. This is done heuristically by defining the lowest QWM state accessible by a system of non-overlapping fermions. The latter are associated with temperature values that are
Generation of ramp waves using variable areal density flyers
Winter, R. E.; Cotton, M.; Harris, E. J.; Chapman, D. J.; Eakins, D.
2016-07-01
Ramp loading using graded density impactors as flyers in gas-gun-driven plate impact experiments can yield new and useful information about the equation of state and the strength properties of the loaded material. Selective Laser Melting, an additive manufacturing technique, was used to manufacture a graded density flyer, termed the "bed-of-nails" (BON). A 2.5-mm-thick × 99.4-mm-diameter solid disc of stainless steel formed a base for an array of tapered spikes of length 5.5 mm and spaced 1 mm apart. The two experiments to test the concept were performed at impact velocities of 900 and 1100 m/s using the 100-mm gas gun at the Institute of Shock Physics at Imperial College London. In each experiment, a BON flyer was impacted onto a copper buffer plate which helped to smooth out perturbations in the wave profile. The ramp delivered to the copper buffer was in turn transmitted to three tantalum targets of thicknesses 3, 5 and 7 mm, which were mounted in contact with the back face of the copper. Heterodyne velocimetry (Het-V) was used to measure the velocity-time history, at the back faces of the tantalum discs. The wave profiles display a smooth increase in velocity over a period of ˜ 2.5 μs, with no indication of a shock jump. The measured profiles have been analysed to generate a stress vs. volume curve for tantalum. The results have been compared with the predictions of the Sandia National Laboratories hydrocode, CTH.
Low Density Phases in a Uniformly Charged Liquid
Knüpfer, Hans; Muratov, Cyrill B.; Novaga, Matteo
2016-07-01
This paper is concerned with the macroscopic behavior of global energy minimizers in the three-dimensional sharp interface unscreened Ohta-Kawasaki model of diblock copolymer melts. This model is also referred to as the nuclear liquid drop model in the studies of the structure of highly compressed nuclear matter found in the crust of neutron stars, and, more broadly, is a paradigm for energy-driven pattern forming systems in which spatial order arises as a result of the competition of short-range attractive and long-range repulsive forces. Here we investigate the large volume behavior of minimizers in the low volume fraction regime, in which one expects the formation of a periodic lattice of small droplets of the minority phase in a sea of the majority phase. Under periodic boundary conditions, we prove that the considered energy {Γ}-converges to an energy functional of the limit "homogenized" measure associated with the minority phase consisting of a local linear term and a non-local quadratic term mediated by the Coulomb kernel. As a consequence, asymptotically the mass of the minority phase in a minimizer spreads uniformly across the domain. Similarly, the energy spreads uniformly across the domain as well, with the limit energy density minimizing the energy of a single droplet per unit volume. Finally, we prove that in the macroscopic limit the connected components of the minimizers have volumes and diameters that are bounded above and below by universal constants, and that most of them converge to the minimizers of the energy divided by volume for the whole space problem.
Institute of Scientific and Technical Information of China (English)
CHEN Jian-Hong; WEI Nan-Xia
2009-01-01
Taking into account the combined effects of the external magnetic field, adiabatic dust charge fluctuation and collisions occurring between the charged dust gains and neutral gas particles (dust-neutral collisions), the dust-acoustic solitary waves in three-dimensional uniform dusty plasmas are investigated analytically. By using the reductive perturbation method, the Korteweg-de Vries (KdV) equation governing the dust-acoustic solitary waves is obtained. The present analytical results show that only rarefactive solitary waves exist in this system. It is also found that the effects of the wave vector along the z-direction, dust charge variation, collisional frequency, the plasma density, and temperature ratio can significantly influence the characteristics of low-frequency wave modes. Moreover, for the collisional dusty plasmas, there is a certain critical value μc of the plasma density ratio #, if μ < μc, the width of the waves increases with μ, otherwise the width of waves decreases with μ.
Energy Technology Data Exchange (ETDEWEB)
Hoeng, Fanny; Denneulin, Aurore [Université Grenoble Alpes, LGP2 (France); Neuman, Charles [Poly-Ink (France); Bras, Julien, E-mail: julien.bras@grenoble-inp.fr [Université Grenoble Alpes, LGP2 (France)
2015-06-15
Synthesis of silver nanoparticles using cellulose nanocrystals (CNC) has been found to be a great method for producing metallic particles in a sustainable way. In this work, we propose to evaluate the influence of the charge density of 2,2,6,6-tetramethyl-1-piperidinyloxy (TEMPO)-oxidized CNC on the morphology and the stability of synthetized silver nanoparticles. Silver nanoparticles were obtained by sol–gel reaction using borohydride reduction, and charge density of TEMPO-oxidized CNC was tuned by an amine grafting. The grafting was performed at room temperature and neutral pH. Crystallinity and morphology were kept intact during the peptidic reaction on CNC allowing knowing the exact impact of the charge density. Charge density has been found to have a strong impact on shape, organization, and suspension stability of resulting silver particles. Results show an easy way to tune the charge density of CNC and propose a sustainable way to control the morphology and stability of silver nanoparticles in aqueous suspension.
Shock wave velocity and shock pressure for low density powders : A novel approach
Dijken, D.K.; Hosson, J.Th.M. De
1994-01-01
A novel approach is presented to predict the shock wave velocity as well as the shock wave pressure in powder materials. It is shown that the influence of the specific volume behind the shock wave on shock wave velocity and shock pressure decreases with decreasing initial powder density. The new mod
SHOCK-WAVE VELOCITY AND SHOCK PRESSURE FOR LOW-DENSITY POWDERS - A NOVEL-APPROACH
DIJKEN, DK; DEHOSSON, JTM
1994-01-01
A novel approach is presented to predict the shock wave velocity as well as the shock wave pressure in powder materials. It is shown that the influence of the specific volume behind the shock wave on shock wave velocity and shock pressure decreases with decreasing initial powder density. The new mod
High charge carrier density at the NaTaO3/SrTiO3 hetero-interface
Nazir, Safdar
2011-08-05
The formation of a (quasi) two-dimensional electron gas between the band insulators NaTaO3 and SrTiO3 is studied by means of the full-potential linearized augmented plane-wave method of density functional theory. Optimization of the atomic positions points to only small changes in the chemical bonding at the interface. Both the p-type (NaO)−/(TiO2)0 and n-type (TaO2)+/(SrO)0 interfaces are found to be metallic with high charge carrier densities. The effects of O vacancies are discussed. Spin-polarized calculations point to the formation of isolated O 2pmagnetic moments, located in the metallic region of the p-type interface.
The c-axis charge traveling wave in a coupled system of Josephson junctions
Shukrinov, Yu. M.; Hamdipour, M.
2012-05-01
We demonstrate a manifestation of the charge traveling wave along the c axis (TW) in current voltage characteristics of coupled Josephson junctions in high- T c superconductors. The branches related to the TW with different wavelengths are found for the stacks with different number of Josephson junctions at different values of system's parameters. Transitions between the TW branches and the outermost branch are observed. The electric charge in the superconducting layers and charge-charge correlation functions for TW and outermost branches show different behavior with bias current. We propose an experimental testing of the TW branching by microwave irradiation.
Vortex Dynamics in Selfdual Maxwell-Higgs Systems with Uniform Background Electric Charge Density
Lee, K M
1994-01-01
We introduce selfdual Maxwell-Higgs systems with uniform background electric charge density and show that the selfdual equations satisfied by topological vortices can be reduced to the original Bogomol'nyi equations without any background. These vortices are shown to carry no spin but to feel the Magnus force due to the shielding charge carried by the Higgs field. We also study the dynamics of slowly moving vortices and show that the spin-statistics theorem holds to our vortices.
Charge carrier density dependence of the hole mobility in poly(p-phenylene vinylene)
Tanase, C; Blom, PWM; De Leeuw, DM; de Meijer, EJ
2004-01-01
The hole transport in various poly(p-phenylene vinylene) (PPV) derivatives has been investigated in field-effect transistors (FETs) and light-emitting diodes (LEDs) as a function of temperature and applied bias. The discrepancy between the experimental hole mobilities extracted from FETs and LEDs based on a single disordered polymeric semiconductor originates from the strong dependence of the hole mobility on the charge carrier density. The microscopic charge transport parameters are directly...
Effects of charge density and hydrophobicity of poly(amido amine)s for non-viral gene delivery
Piest, Martin; Engbersen, Johan F.J.
2010-01-01
High cationic charge densities in polymeric vectors result in tight DNA condensation, leading to small highly positively charged polyplexes which show generally high cellular uptake in vitro. However, high cationic charge densities also introduce membrane-disruptive properties to the polymers, there
Zhou Dai Mei; Sá Ben-Hao; Li Zhong Dao
2002-01-01
Using a hadron and string cascade model, JPCIAE, and the corresponding Monte Carlo events generator, the energy and centrality dependences of charged particle pseudorapidity density in relativistic nuclear collisions were studied. Within the framework of this model, both the relativistic p anti p experimental data and the PHOBOS and PHENIX Au + Au data could be reproduced fairly well without retuning the model parameters. The author shows that since is not a well defined physical variable both experimentally and theoretically, the charged particle pseudorapidity density per participant pair can increase and also can decrease with increasing of , so it may be hard to use charged particle pseudorapidity density per participant pair as a function of to distinguish various theoretical models for particle production
Trapped charge densities in Al2O3-based silicon surface passivation layers
Jordan, Paul M.; Simon, Daniel K.; Mikolajick, Thomas; Dirnstorfer, Ingo
2016-06-01
In Al2O3-based passivation layers, the formation of fixed charges and trap sites can be strongly influenced by small modifications in the stack layout. Fixed and trapped charge densities are characterized with capacitance voltage profiling and trap spectroscopy by charge injection and sensing, respectively. Al2O3 layers are grown by atomic layer deposition with very thin (˜1 nm) SiO2 or HfO2 interlayers or interface layers. In SiO2/Al2O3 and HfO2/Al2O3 stacks, both fixed charges and trap sites are reduced by at least a factor of 5 compared with the value measured in pure Al2O3. In Al2O3/SiO2/Al2O3 or Al2O3/HfO2/Al2O3 stacks, very high total charge densities of up to 9 × 1012 cm-2 are achieved. These charge densities are described as functions of electrical stress voltage, time, and the Al2O3 layer thickness between silicon and the HfO2 or the SiO2 interlayer. Despite the strong variation of trap sites, all stacks reach very good effective carrier lifetimes of up to 8 and 20 ms on p- and n-type silicon substrates, respectively. Controlling the trap sites in Al2O3 layers opens the possibility to engineer the field-effect passivation in the solar cells.
Correlation between the extent of catalytic activity and charge density of montmorillonites.
Ertem, Gözen; Steudel, Annett; Emmerich, Katja; Lagaly, Gerhard; Schuhmann, Rainer
2010-09-01
The clay mineral montmorillonite is a member of the phyllosilicate group of minerals, which has been detected on martian soil. Montmorillonite catalyzes the condensation of activated monomers to form RNA-like oligomers. Extent of catalysis, that is, the yield of oligomers, and the length of the longest oligomer formed in these reactions widely varies with the source of montmorillonite (i.e., the locality where the mineral is mined). This study was undertaken to establish whether there exists a correlation between the extent of catalytic property and the charge density of montmorillonites. Charge density was determined by saturating the montmorillonites with alkyl ammonium cations that contained increasing lengths of alkyl chains, [CH₃-(CH₂)(n)-NH₃](+), where n = 3-16 and 18, and then measuring d(₀₀₁), interlayer spacing of the resulting montmorillonite-alkyl ammonium-montmorillonite complex by X-ray diffractometry (XRD). Results demonstrate that catalytic activity of montmorillonites with lower charge density is superior to that of higher charge density montmorillonite. They produce longer oligomers that contain 9 to 10 monomer units, while montmorillonite with high charge density catalyzes the formation of oligomers that contain only 4 monomer units. The charge density of montmorillonites can also be calculated from the chemical composition if elemental analysis data of the pure mineral are available. In the next mission to Mars, CheMin (Chemistry and Mineralogy), a combined X-ray diffraction/X-ray fluorescence instrument, will provide information on the mineralogical and elemental analysis of the samples. Possible significance of these results for planning the future missions to Mars for the search of organic compounds and extinct or extant life is discussed.
A Composite Fermion Hofstadter Problem: Partially Polarized Density Wave States in the FQHE
Murthy, Ganpathy
2000-03-01
It is well known that the 2/5 FQH state can have two translationally invariant ground states, one of which is a singlet and the other fully polarized. A quantum phase transition occurs between these two as a function of the Zeeman field. This can be simply explained in terms of the crossing of Composite Fermion Landau levels. However, recently Kukushkin et al (PRL 82, 3665 (99)) have seen plateaus of half the maximal polarization in the 2/5 fraction at intermediate Zeeman fields. Similar plateaus, which are not allowed for translationally invariant CF states, are seen in other fractions as well. I propose a class of novel partially polarized spin/charge density wave states which display the co-existence of density wave and quantum Hall order (the Hall crystal state). The physical properties of the states, including gaps and collective excitations are computed using the formalism for the FQHE developed recently by Shankar and myself (for details see Murthy and Shankar in "Composite Fermions", Olle Heinonen, Editor).
Mapping surface charge density of lipid bilayers by quantitative surface conductivity microscopy
DEFF Research Database (Denmark)
Klausen, Lasse Hyldgaard; Fuhs, Thomas; Dong, Mingdong
2016-01-01
Local surface charge density of lipid membranes influences membrane-protein interactions leading to distinct functions in all living cells, and it is a vital parameter in understanding membrane-binding mechanisms, liposome design and drug delivery. Despite the significance, no method has so far...... approach, quantitative surface conductivity microscopy (QSCM), capable of mapping surface charge density with high-quantitative precision and nanoscale resolution. The method is validated through an extensive theoretical analysis of the ionic current at the nanopipette tip, and we demonstrate the capacity...
Energy Technology Data Exchange (ETDEWEB)
Clarke, Tracey M.; Shoaee, Safa; Soon, Ying W.; Durrant, James R. [Centre for Plastic Electronics, Department of Chemistry, Imperial College London, Exhibition Road, London SW7 2AZ (United Kingdom); Ballantyne, Amy; Nelson, Jenny [Centre for Plastic Electronics, Department of Physics, Imperial College London, Exhibition Road, London SW7 2AZ (United Kingdom); Duffy, Warren; Heeney, Martin; McCulloch, Iain [Centre for Plastic Electronics, Department of Chemistry, Imperial College London, Exhibition Road, London SW7 2AZ (United Kingdom); Merck Chemicals, Chilworth Science Park, Southampton SO16 7QD (United Kingdom)
2010-12-07
Charge photogeneration: The correlation between the efficiency of photogeneration of dissociated polarons and photocurrent densities for organic solar cells based on polymer:fullerene blend films is investigated. Optical assays of polaron yield measured in films without electrodes show a remarkably clear correlation with short circuit density and quantum yield measured in complete devices. For the blend films studied herein, the primary determinant of photocurrent generation is the efficiency of dissociation of photogenerated charges away from the polymer/fullerene interface and the primary loss pathway is geminate recombination. (Copyright copyright 2010 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)
Yang, Weitao; Mori-Sánchez, Paula; Cohen, Aron J
2013-09-14
The exact conditions for density functionals and density matrix functionals in terms of fractional charges and fractional spins are known, and their violation in commonly used functionals has been shown to be the root of many major failures in practical applications. However, approximate functionals are designed for physical systems with integer charges and spins, not in terms of the fractional variables. Here we develop a general framework for extending approximate density functionals and many-electron theory to fractional-charge and fractional-spin systems. Our development allows for the fractional extension of any approximate theory that is a functional of G(0), the one-electron Green's function of the non-interacting reference system. The extension to fractional charge and fractional spin systems is based on the ensemble average of the basic variable, G(0). We demonstrate the fractional extension for the following theories: (1) any explicit functional of the one-electron density, such as the local density approximation and generalized gradient approximations; (2) any explicit functional of the one-electron density matrix of the non-interacting reference system, such as the exact exchange functional (or Hartree-Fock theory) and hybrid functionals; (3) many-body perturbation theory; and (4) random-phase approximations. A general rule for such an extension has also been derived through scaling the orbitals and should be useful for functionals where the link to the Green's function is not obvious. The development thus enables the examination of approximate theories against known exact conditions on the fractional variables and the analysis of their failures in chemical and physical applications in terms of violations of exact conditions of the energy functionals. The present work should facilitate the calculation of chemical potentials and fundamental bandgaps with approximate functionals and many-electron theories through the energy derivatives with respect to the
Spatially separated charge densities of electrons and holes in organic-inorganic halide perovskites
Energy Technology Data Exchange (ETDEWEB)
Li, Dan; Liang, Chunjun, E-mail: chjliang@bjtu.edu.cn, E-mail: zhqhe@bjtu.edu.cn; Zhang, Huimin; You, Fangtian; He, Zhiqun, E-mail: chjliang@bjtu.edu.cn, E-mail: zhqhe@bjtu.edu.cn [Key Laboratory of Luminescence and Optical Information, Ministry of Education, School of Science, Beijing Jiaotong University, Beijing 100044 (China); Zhang, Chunxiu [Information Recording Materials Lab, Beijing Institute of Graphic Communication, Beijing 102600 (China)
2015-02-21
Solution-processable methylammonium lead trihalide perovskites exhibit remarkable high-absorption and low-loss properties for solar energy conversion. Calculation from density functional theory indicates the presence of non-equivalent halogen atoms in the unit cell because of the specific orientation of the organic cation. Considering the 〈100〉 orientation as an example, I{sub 1}, one of the halogen atoms, differs from the other iodine atoms (I{sub 2} and I{sub 3}) in terms of its interaction with the organic cation. The valance-band-maximum (VBM) and conduction-band-minimum (CBM) states are derived mainly from 5p orbital of I{sub 1} atom and 6p orbital of Pb atom, respectively. The spatially separated charge densities of the electrons and holes justify the low recombination rate of the pure iodide perovskite. Chlorine substitution further strengthens the unique position of the I{sub 1} atom, leading to more localized charge density around the I{sub 1} atom and less charge density around the other atoms at the VBM state. The less overlap of charge densities between the VBM and CBM states explains the relatively lower carrier recombination rate of the iodine-chlorine mixed perovskite. Chlorine substitution significantly reduces the effective mass at a direction perpendicular to the Pb-Cl bond and organic axis, enhancing the carrier transport property of the mixed perovskite in this direction.
Spatially separated charge densities of electrons and holes in organic-inorganic halide perovskites
Li, Dan; Liang, Chunjun; Zhang, Huimin; Zhang, Chunxiu; You, Fangtian; He, Zhiqun
2015-02-01
Solution-processable methylammonium lead trihalide perovskites exhibit remarkable high-absorption and low-loss properties for solar energy conversion. Calculation from density functional theory indicates the presence of non-equivalent halogen atoms in the unit cell because of the specific orientation of the organic cation. Considering the orientation as an example, I1, one of the halogen atoms, differs from the other iodine atoms (I2 and I3) in terms of its interaction with the organic cation. The valance-band-maximum (VBM) and conduction-band-minimum (CBM) states are derived mainly from 5p orbital of I1 atom and 6p orbital of Pb atom, respectively. The spatially separated charge densities of the electrons and holes justify the low recombination rate of the pure iodide perovskite. Chlorine substitution further strengthens the unique position of the I1 atom, leading to more localized charge density around the I1 atom and less charge density around the other atoms at the VBM state. The less overlap of charge densities between the VBM and CBM states explains the relatively lower carrier recombination rate of the iodine-chlorine mixed perovskite. Chlorine substitution significantly reduces the effective mass at a direction perpendicular to the Pb-Cl bond and organic axis, enhancing the carrier transport property of the mixed perovskite in this direction.
Induced fermionic charge and current densities in two-dimensional rings
Bellucci, S; Grigoryan, A Kh
2016-01-01
For a massive quantum fermionic field, we investigate the vacuum expectation values (VEVs) of the charge and current densities induced by an external magnetic flux in a two-dimensional circular ring. Both the irreducible representations of the Clifford algebra are considered. On the ring edges the bag (infinite mass) boundary conditions are imposed for the field operator. This leads to the Casimir type effect on the vacuum characteristics. The radial current vanishes. The charge and the azimuthal current are decomposed into the boundary-free and boundary-induced contributions. Both these contributions are odd periodic functions of the magnetic flux with the period equal to the flux quantum. An important feature that distinguishes the VEVs of the charge and current densities from the VEV of the energy density, is their finiteness on the ring edges. The current density is equal to the charge density for the outer edge and has the opposite sign on the inner edge. The VEVs are peaked near the inner edge and, as f...
Bifurcation of space-charge wave in a plasma waveguide including the wake potential effect
Lee, Myoung-Jae; Jung, Young-Dae
2016-09-01
The wake potential effects on the propagation of the space-charge dust ion-acoustic wave are investigated in a cylindrically bounded dusty plasma with the ion flow. The results show that the wake potential would generate the double frequency modes in a cylindrically bounded dusty plasma. It is found that the upper mode of the wave frequency with the root of higher-order is smaller than that with the root of lower-order in intermediate wave number domains. However, the lower mode of the scaled wave frequency with the root of higher-order is found to be greater than that with the root of lower-order. It is found that the influence in the order of the root of the Bessel function on the wave frequency of the space-charge dust-ion-acoustic wave in a cylindrically confined dusty plasma decreases with an increase in the propagation wave number. It is also found that the double frequency modes increase with increasing Mach number due to the ion flow in a cylindrical dusty plasma. In addition, it is found that the upper mode of the group velocity decreases with an increase in the scaled radius of the plasma cylinder. However, it is shown that the lower mode of the scaled group velocity of the space-charge dust ion acoustic wave increases with an increase in the radius of the plasma cylinder. The variation of the space-charge dust-ion-acoustic wave due to the wake potential and geometric effects is also discussed.
Density decrease in vanadium-base alloys irradiated in the dynamic helium charging experiment
Energy Technology Data Exchange (ETDEWEB)
Chung, H.M.; Galvin, T.M.; Smith, D.L. [Argonne National Laboratory, Chicago, IL (United States)
1996-04-01
Combined effects of dynamically charged helium and neutron damage on density decrease (swelling) of V-4Cr-4Ti, V-5Ti, V-3Ti-1Si, and V-8Cr-6Ti alloys have been determined after irradiation to 18-31 dpa at 425-600{degrees}C in the Dynamic helium Charging Experiment (DHCE). To ensure better accuracy in density measurement, broken pieces of tensile specimens {approx} 10 times heavier than a transmission electron microscopy (TEM) disk were used. Density increases of the four alloys irradiated in the DHCE were <0.5%. This small change seems to be consistent with the negligible number density of microcavities characterized by TEM. Most of the dynamically produced helium atoms seem to have been trapped in the grain matrix without significant cavity nucleation or growth.
Bellucci, S; Bragança, E; Saharian, A A
2016-01-01
We evaluate the fermion condensate and the expectation values of the charge and current densities for a massive fermionic field in (2+1)-dimensional conical spacetime with a magnetic flux located at the cone apex. The consideration is done for both irreducible representations of the Clifford algebra. The expectation values are decomposed into the vacuum expectation values and contributions coming from particles and antiparticles. All these contributions are periodic functions of the magnetic flux with the period equal to the flux quantum. Related to the non-invariance of the model under the parity and time-reversal transformations, the fermion condensate and the charge density have indefinite parity with respect to the change of the signs of the magnetic flux and chemical potential. The expectation value of the radial current density vanishes. The azimuthal current density is the same for both the irreducible representations of the Clifford algebra. It is an odd function of the magnetic flux and an even funct...
Sarma, S. Das; Hwang, E. H.
1998-01-01
We calculate within the Boltzmann equation approach the charged impurity scattering limited low temperature electronic resistivity of low density $n$-type inversion layers in Si MOSFET structures. We find a rather sharp quantum to classical crossover in the transport behavior in the $0 - 5$K temperature range, with the low density, low temperature mobility showing a strikingly strong non-monotonic temperature dependence, which may qualitatively explain the recently observed anomalously strong...
Energy Technology Data Exchange (ETDEWEB)
Bellucci, S. [INFN, Laboratori Nazionali di Frascati, Frascati (Italy); Bezerra de Mello, E.R. [Universidade Federal da Parai ba, Departamento de Fisica, 58.059-970, Joao Pessoa, PB (Brazil); Braganca, E. [INFN, Laboratori Nazionali di Frascati, Frascati (Italy); Universidade Federal da Parai ba, Departamento de Fisica, 58.059-970, Joao Pessoa, PB (Brazil); Saharian, A.A. [Yerevan State University, Department of Physics, Yerevan (Armenia)
2016-06-15
We evaluate the fermion condensate and the expectation values of the charge and current densities for a massive fermionic field in (2+1)-dimensional conical spacetime with a magnetic flux located at the cone apex. The consideration is done for both irreducible representations of the Clifford algebra. The expectation values are decomposed into the vacuum expectation values and contributions coming from particles and antiparticles. All these contributions are periodic functions of the magnetic flux with the period equal to the flux quantum. Related to the non-invariance of the model under the parity and time-reversal transformations, the fermion condensate and the charge density have indefinite parity with respect to the change of the signs of the magnetic flux and chemical potential. The expectation value of the radial current density vanishes. The azimuthal current density is the same for both the irreducible representations of the Clifford algebra. It is an odd function of the magnetic flux and an even function of the chemical potential. The behavior of the expectation values in various asymptotic regions of the parameters are discussed in detail. In particular, we show that for points near the cone apex the vacuum parts dominate. For a massless field with zero chemical potential the fermion condensate and charge density vanish. Simple expressions are derived for the part in the total charge induced by the planar angle deficit and magnetic flux. Combining the results for separate irreducible representations, we also consider the fermion condensate, charge and current densities in parity and time-reversal symmetric models. Possible applications to graphitic nanocones are discussed. (orig.)
Two-Dimensional Wave Motion on the Charged Surface of a Viscous Liquid
Institute of Scientific and Technical Information of China (English)
LI Fang; YIN Xie-Yuan; YIN Xie-Zhen
2008-01-01
The wave motion on the charged surface of a viscous Newtonian liquid is solved as an initial-value problem. Both the leaky dielectric and perfect dielectric cases are considered. The amplitude of wave is assumed to be small. The electric field induced by surface charge is shown to have a generally destabilizing effect on surface wave. The neutral stability curve is drawn in the (G, N,e) plane (G: the gravitational bond number; Ne: the electrical Bond number). The Ohnesorge number, Taylor-Melcher number and permittivity ratio have little influence on the neutral stability curve. It is testified that the classical normal mode method cannot predict wave behaviour at small times.
The c-axis charge traveling wave in coupled system of Josephson junctions
Shukrinov, Yu M.; Hamdipour, M.
2011-01-01
We demonstrate a manifestation of the charge traveling wave along the c-axis (TW) in current voltage characteristics of coupled Josephson junctions in high-$T_c$ superconductors. The branches related to the TW with different wavelengths are found for the stacks with different number of Josephson junctions at different values of system's parameters. Transitions between the TW branches and the outermost branch are observed. Time dependence of the electric charge in the superconducting layers an...
Charge and spin currents in normal metal sandwiched by tow p-wave
Directory of Open Access Journals (Sweden)
Y Rahnavard
2010-09-01
Full Text Available Charge and spin transport properties of a clean $SNS$ Josephson junction (triplet superconductor-normal metal-triplet superconductor are studied using the quasiclassical Eilenberger equation of Green’s function. Our system consists of two p-wave superconducting crystals separated by a Copper nano layer. Effects of thickness of normal layer between superconductors on the spin and charge currents are investigated. Also misorientation between triplet superconductors which creates the spin current is another subject of this paper.
Dust-acoustic solitary waves in dusty plasma with variable dust charge
Forozani, Gh
2011-01-01
In this article we are going to consider dust acoustic wave in dusty plasma whose constituents are inertial negative charged dust particles, Boltzmann distributed electrons and non-thermal distributed ions with variable dust charge. Using reductive perturbation method, we have obtained Korteweg-de Veries (kdv) and modified kdv(mkdv) equations. A Sagdeev potential for the system and stability conditions for solitonic solution are also derived.
Yao, Yanyan; Jiang, Tao; Zhang, Limin; Chen, Xiangyu; Gao, Zhenliang; Wang, Zhong Lin
2016-08-24
Ocean waves are one of the most promising renewable energy sources for large-scope applications due to the abundant water resources on the earth. Triboelectric nanogenerator (TENG) technology could provide a new strategy for water wave energy harvesting. In this work, we investigated the charging characteristics of utilizing a wavy-structured TENG to charge a capacitor under direct water wave impact and under enclosed ball collision, by combination of theoretical calculations and experimental studies. The analytical equations of the charging characteristics were theoretically derived for the two cases, and they were calculated for various load capacitances, cycle numbers, and structural parameters such as compression deformation depth and ball size or mass. Under the direct water wave impact, the stored energy and maximum energy storage efficiency were found to be controlled by deformation depth, while the stored energy and maximum efficiency can be optimized by the ball size under the enclosed ball collision. Finally, the theoretical results were well verified by the experimental tests. The present work could provide strategies for improving the charging performance of TENGs toward effective water wave energy harvesting and storage.
Accretion Discs with an Inner Spiral Density Wave
Montgomery, M M
2010-01-01
In Montgomery (2009a), we show that accretion discs in binary systems could retrogradely precess by tidal torques like the Moon and the Sun on a tilted, spinning, non-spherical Earth. In addition, we show that the state of matter and the geometrical shape of the celestial object could significantly affect the precessional value. For example, a Cataclysmic Variable (CV) Dwarf Novae (DN) non-magnetic system that shows negative superhumps in its light curve can be described by a retrogradely precessing, differentially rotating, tilted disc. Because the disc is a fluid and because the gas stream overflows the tilted disc and particles can migrate into inner disc annuli, coupled to the disc could be a retrogradely precessing inner ring that is located near the innermost annuli of the disc. However, numerical simulations by Bisikalo et al. (2003, 2004) and this work show that an inner spiral density wave can be generated instead of an inner ring. Therefore, we show that retrograde precession in non-magnetic, spinni...
The energy density of a Landau damped plasma wave
Best, R. W. B.
1999-01-01
In this paper some theories about the energy of a Landau damped plasma wave are discussed and new initial conditions are proposed. Analysis of a wave packet, rather than an infinite wave, gives a clear picture of the energy transport from field to particles. Initial conditions are found which excite
Cozma, M D
2016-01-01
The charged pion multiplicity ratio in intermediate energy heavy-ion collisions, a probe of the density dependence of symmetry energy above the saturation point, has been proven in a previous study to be extremely sensitive to the strength of the isovector $\\Delta$(1232) potential in nuclear matter. As there is no current knowledge, either from theory or experiment, about the magnitude of this quantity, the extraction of constraints for the slope of the symmetry energy at saturation by using exclusively the mentioned observable is hindered at present. It is shown that, by including the ratio of average $p_T$ of charged pions $\\langle p_T^{(\\pi^+)}\\rangle/\\langle p_T^{(\\pi^-)}\\rangle$ in the list of fitted observables, the noted problem can be circumvented. A realistic description of this observable requires the accounting for the interaction of pions with the dense nuclear matter environment by the incorporation of the so called S-wave and P-wave pion optical potentials. This is performed within the framework...
Lester, Jacob; Chandler, Timothy; Gemene, Kebede L
2015-11-17
We present a simple, rapid, and inexpensive electrochemical sensor based on a reversible pulsed chronopotentiometric polyanion-selective membrane electrode for the detection and quantification of oversulfated chondroitin sulfate (OSCS) and other high charge-density polyanions that could potentially be used to adulterate heparin. The membrane is free of ion exchanger and is formulated with plasticized poly(vinyl chloride) (PVC) and an inert lipophilic salt, tridodecylmethylammonium-dinonylnaphthaline sulfonate (TDMA-DNNS). The neutral salt is used to reduce membrane resistance and to ensure reversibility of the sensor. More importantly, TDMA(+) is used as the recognition element for the polyanions. Here an anodic galvanostatic current pulse is applied across the membrane to cause the extraction of the polyanions from the sample into the membrane and potential is measured at the sample-membrane interface. The measured electromotive force (emf) is proportional to the concentration and the charge density of the polyanions. High charge-density polyanion contaminants and impurities in heparin can be detected using this method since the overall equilibrium potential response of polyions increases with increasing charge density of the polyions. Here, first the potential response of pure heparin is measured at a saturation concentration, the concentration beyond which further addition of heparin does not produce a change in potential response. Then the potential response of heparin tainted with different quantities of the high charge-density contaminant is measured at a fixed total polyion concentration (heparin concentration + contaminant concentration). The latter gives a greater negative potential response due to the presence of the high charge-density contaminant. The increase in the negative potential response can be used for detection and quantification of high charge-density contaminants in heparin. We demonstrate here that 0.3% (w/w) OSCS as well as 0.1% (w
Institute of Scientific and Technical Information of China (English)
无
2000-01-01
Based on the density functional theory and the atom-bond electronegativity equalization model (ABEEM), a method is proposed to construct the softness matrix and to obtain the electron population normal modes (PNMs) for a closed system. Using this method the information about the bond charge polarization in a molecule can be obtained easily. The test calculation shows that the PNM obtained by this method includes all the modes about the bond charge polarization explicitly. And the bond charge polarization mode characterized by the biggest eigenvalue, which is the softest one of all modes related with chemical bonds, can describe the charge polarization process in a molecule as exquisitely as the corresponding ab initio method.
Johnson, Erin R; Salamone, Michela; Bietti, Massimo; DiLabio, Gino A
2013-02-07
Conventional density-functional theory (DFT) has the potential to overbind radical-molecule complexes because of erroneous charge transfer. We examined this behavior by exploring the ability of various DFT approximations to predict fractional charge transfer and by quantifying the overbinding in a series of complexes. It is demonstrated that too much charge is transferred from molecules to radicals when the radical singly unoccupied molecular orbitals are predicted to be erroneously too low in energy relative to the molecule highest occupied molecular orbitals, leading to excessive Coulombic attraction. In this respect, DFT methods formulated with little or no Hartree-Fock exchange perform most poorly. The present results illustrate that the charge-transfer problem is much broader than may have been previously expected and is not limited to conventional (i.e., molecule-molecule) donor-acceptor complexes.
Quantifying the nucleon’s pion cloud with transverse charge densities
Energy Technology Data Exchange (ETDEWEB)
Strikman, M.; Weiss, C.
2010-10-01
The transverse densities in a fast-moving nucleon offer a model-independent framework for analyzing the spatial structure of the pion cloud and its role in current matrix elements. We calculate the chiral large-distance component of the charge density in a dispersion representation of the form factor and discuss its partonic interpretation. It dominates over the nonchiral density only at surprisingly large distances above ~2 fm. The chiral component can be probed in precision low-Q^2 elastic eN scattering or in peripheral deep-inelastic processes that resolve its quark/gluon content.
Electrostatic force density for a scanned probe above a charged surface
Energy Technology Data Exchange (ETDEWEB)
Passian, A.; Wig, A.; Meriaudeau, F.; Buncick, M.; Thundat, T.; Ferrell, T. L.
2001-07-15
The Coulomb interaction of a dielectric probe tip with a uniform field existing above a semi-infinite, homogeneous dielectric substrate is studied. The induced polarization surface charge density and the field distribution at the bounding surface of the dielectric medium with the geometry of half of a two sheeted hyperboloid of revolution located above the dielectric half space interfaced with a uniform surface charge density is calculated. The force density on the hyperboloidal probe medium is calculated as a function of the probe tip shape. The calculation is based on solving Laplace's equation and employing a newly derived integral expansion for the vanishing dielectric limit of the potential. The involved numerical simulations comprise the evaluation of infinite double integrals involving conical functions.
Electrostatic force density for a scanned probe above a charged surface
Passian, A.; Wig, A.; Meriaudeau, F.; Buncick, M.; Thundat, T.; Ferrell, T. L.
2001-07-01
The Coulomb interaction of a dielectric probe tip with a uniform field existing above a semi-infinite, homogeneous dielectric substrate is studied. The induced polarization surface charge density and the field distribution at the bounding surface of the dielectric medium with the geometry of half of a two sheeted hyperboloid of revolution located above the dielectric half space interfaced with a uniform surface charge density is calculated. The force density on the hyperboloidal probe medium is calculated as a function of the probe tip shape. The calculation is based on solving Laplace's equation and employing a newly derived integral expansion for the vanishing dielectric limit of the potential. The involved numerical simulations comprise the evaluation of infinite double integrals involving conical functions.
The motion of charged particles in strong plane waves including radiation reaction
Leinemann, R.; Herold, H.; Ruder, H.; Kegel, W. H.
The Lorentz-Dirac equation in the Landau approximation is used to study the motion of charged particles in strong plane vacuum waves. It is shown that integration for circularly polarized waves can be used to determine analytically the curves of the particle trajectories. The solution is used to investigate the particle trajectories and energy evolution for various strong waves. The initial conditions for the motion are chosen so that the particles start from a radiation-free path and the growing effect of the radiation reaction on the particle trajectory is highlighted.
Energy Technology Data Exchange (ETDEWEB)
Arregui, I.; Asensio Ramos, A. [Instituto de Astrofisica de Canarias, Via Lactea s/n, E-38205 La Laguna, Tenerife (Spain); Pascoe, D. J., E-mail: iarregui@iac.es [School of Mathematics and Statistics, University of St. Andrews, St. Andrews KY16 9SS (United Kingdom)
2013-06-01
We present a Bayesian seismology inversion technique for propagating magnetohydrodynamic transverse waves observed in coronal waveguides. The technique uses theoretical predictions for the spatial damping of propagating kink waves in transversely inhomogeneous coronal waveguides. It combines wave amplitude damping length scales along the waveguide with theoretical results for resonantly damped propagating kink waves to infer the plasma density variation across the oscillating structures. Provided that the spatial dependence of the velocity amplitude along the propagation direction is measured and the existence of two different damping regimes is identified, the technique would enable us to fully constrain the transverse density structuring, providing estimates for the density contrast and its transverse inhomogeneity length scale.
Determination of Transverse Density Structuring from Propagating MHD Waves in the Solar Atmosphere
Arregui, I; Pascoe, D J
2013-01-01
We present a Bayesian seismology inversion technique for propagating magnetohydrodynamic (MHD) transverse waves observed in coronal waveguides. The technique uses theoretical predictions for the spatial damping of propagating kink waves in transversely inhomogeneous coronal waveguides. It combines wave amplitude damping length scales along the waveguide with theoretical results for resonantly damped propagating kink waves to infer the plasma density variation across the oscillating structures. Provided the spatial dependence of the velocity amplitude along the propagation direction is measured and the existence of two different damping regimes is identified, the technique would enable us to fully constrain the transverse density structuring, providing estimates for the density contrast and its transverse inhomogeneity length scale.
Geometrical optics response tensors and the transport of the wave energy density
Energy Technology Data Exchange (ETDEWEB)
Bornatici, M [INFM, Physics Department ' A. Volta' , University of Pavia, I-27100 Pavia (Italy); Maj, O [INFM, Physics Department, University of Milan, I-20133 Milan (Italy)
2003-08-01
Two forms of the transport equation for the wave energy density inherent in two (apparently diverse) formulations of geometrical optics (GO) are discussed on the basis of the relationships among the plane-wave dielectric tensor, the effective dielectric tensor and the effective conductivity tensor. For a generic space- and time-varying medium, a novel relationship between the dielectric tensor and the conductivity tensor is obtained whereupon the equivalence of the two GO formulations is established. The conditions for which either the wave action density or the wave energy density is conserved are discussed.
A perturbative analysis of Quasi-Radial density waves in galactic disks
Hernandez, X
2011-01-01
The theoretical understanding of density waves in disk galaxies starts from the classical WKB perturbative analysis of tight-winding perturbations, the key assumption being that the potential due to the density wave is approximately radial. The above has served as a valuable guide in aiding the understanding of both simulated and observed galaxies, in spite of a number of caveats being present. The observed spiral or bar patterns in real galaxies are frequently only marginally consistent with the tight-winding assumption, often in fact, outright inconsistent. Here we derive a complementary formulation to the problem, by treating quasi-radial density waves under simplified assumptions in the linear regime. We assume that the potential due to the density wave is approximately tangential, and derive the corresponding dispersion relation of the problem. We obtain an instability criterion for the onset of quasi-radial density waves, which allows a clear understanding of the increased stability of the higher order ...
Moon, Jong Kyun; Song, Myung Won; Pak, Hyuk Kyu
2015-05-20
A solid surface in contact with water or aqueous solution usually carries specific electric charges. These surface charges attract counter ions from the liquid side. Since the geometry of opposite charge distribution parallel to the solid-liquid interface is similar to that of a capacitor, it is called an electrical double layer capacitor (EDLC). Therefore, there is an electrical potential difference across an EDLC in equilibrium. When a liquid bridge is formed between two conducting plates, the system behaves as two serially connected EDLCs. In this work, we propose a new method for investigating the surface charge density on solid-liquid interfaces. By mechanically modulating the electrical double layers and simultaneously applying a dc bias voltage across the plates, an ac electric current can be generated. By measuring the voltage drop across a load resistor as a function of bias voltage, we can study the surface charge density on solid-liquid interfaces. Our experimental results agree very well with the simple equivalent electrical circuit model proposed here. Furthermore, using this method, one can determine the polarity of the adsorbed state on the solid surface depending on the material used. We expect this method to aid in the study of electrical phenomena on solid-liquid interfaces.
Cotaescu, Ion I; Sporea, Ciprian
2016-01-01
The asymptotic form of the Dirac spinors in the field of the Reissner-Nordstrom black hole are derived for the scattering states (with $E>mc^2$) obtaining the phase shifts of the partial wave analysis of the Dirac fermions scattered from charged black holes. The elastic scattering and the absorption are studied giving analytic formulas for the partial amplitudes and cross sections.
Dust acoustic and drift waves in a non-Maxwellian dusty plasma with dust charge fluctuation
Zakir, U.; Haque, Q.; Imtiaz, N.; Qamar, A.
2015-12-01
> ) on the wave dispersion and instability are presented. It is found that the presence of the non-thermal electron and ion populations reduce the growth rate of the instability which arises due to the dust charging effect. In addition, the nonlinear vortex solutions are also obtained. For illustration, the results are analysed by using the dusty plasma parameters of Saturn's magnetosphere.
Charge transport in the normal metal/diffusive ferromagnet/s-wave superconductor junctions
Yokoyama, Takehito; Tanaka, Yukio; Golubov, Alexander; Inoue, Jun-ichiro; Asano, Yasuhiro
2005-01-01
Charge transport in the normal metal/insulator/diffusive ferromagnet/insulator/s-wave superconductor (N/I/DF/I/S) junctions is studied for various situations solving the Usadel equation under the Nazarov's generalized boundary condition. Conductance of the junction is calculated by changing the magn
Charge transfer polarisation wave in high Tc oxides and superconductive pairing
Chakraverty, B. K.
1991-01-01
A general formalism of quantized charge transfer polarization waves was developed. The nature of possible superconductive pairing between oxygen holes is discussed. Unlike optical phonons, these polarization fields will give rise to dielectric bipolarons or bipolaron bubbles. In the weak coupling limit, a new class of superconductivity is to be expected.
Fractional-charge and fractional-spin errors in range-separated density-functional theory
Mussard, Bastien
2016-01-01
We investigate fractional-charge and fractional-spin errors in range-separated density-functional theory. Specifically, we consider the range-separated hybrid (RSH) method which combines long-range Hartree-Fock (HF) exchange with a short-range semilocal exchange-correlation density functional, and the RSH+MP2 method which adds long-range second-order M{{\\o}}ller-Plesset (MP2) correlation. Results on atoms and molecules show that the fractional-charge errors obtained in RSH are much smaller than in the standard Kohn-Sham (KS) scheme applied with semilocal or hybrid approximations, and also generally smaller than in the standard HF method. The RSH+MP2 method tends to have smaller fractional-charge errors than standard MP2 for the most diffuse systems, but larger fractional-charge errors for the more compact systems. Even though the individual contributions to the fractional-spin errors in the H atom coming from the short-range exchange and correlation density-functional approximations are smaller than the corre...
Inferring Magnetospheric Heavy Ion Density using EMIC Waves
Energy Technology Data Exchange (ETDEWEB)
Kim, Eun-Hwa; Johnson, Jay R.; Kim, Hyomin; Lee, Dong-Hun
2014-05-01
We present a method to infer heavy ion concentration ratios from EMIC wave observations that result from ionion hybrid (IIH) resonance. A key feature of the ion-ion hybrid resonance is the concentration of wave energy in a field-aligned resonant mode that exhibits linear polarization. This mode converted wave is localized at the location where the frequency of a compressional wave driver matches the IIH resonance condition, which depends sensitively on the heavy ion concentration. This dependence makes it possible to estimate the heavy ion concentration ratio. In this letter, we evaluate the absorption coefficients at the IIH resonance at Earth's geosynchronous orbit for variable concentrations of He+ and field-aligned wave numbers using a dipole magnetic field. Although wave absorption occurs for a wide range of heavy ion concentrations, it only occurs for a limited range of field-aligned wave numbers such that the IIH resonance frequency is close to, but not exactly the same as the crossover frequency. Using the wave absorption and observed EMIC waves from GOES-12 satellite, we demonstrate how this technique can be used to estimate that the He+ concentration is around 4% near L = 6.6.
The generalization of charged AdS black hole specific volume and number density
Wang, Zi-Liang; He, Miao; Fang, Chao; Sun, Dao-Quan; Deng, Jian-Bo
2017-04-01
In this paper, by proposing a generalized specific volume, we restudy the P- V criticality of charged AdS black holes in the extended phase space. The results show that most of the previous conclusions can be generalized without change, but the ratio {\\tilde{ρ }}_c should be 3 {\\tilde{α }}/16 in general case. Further research on the thermodynamical phase transition of black hole leads us to a natural interpretation of our assumption, and more black hole properties can be generalized. Finally, we study the number density for charged AdS black hole in higher dimensions, the results show the necessity of our assumption.
Simulation of the reflected blast wave from a C-4 charge
Howard, W. Michael; Kuhl, Allen L.; Tringe, Joseph
2012-03-01
The reflection of a blast wave from a C4 charge detonated above a planar surface is simulated with our ALE3D code. We used a finely-resolved, fixed Eulerian 2-D mesh (167 μm per cell) to capture the detonation of the charge, the blast wave propagation in nitrogen, and its reflection from the surface. The thermodynamic properties of the detonation products and nitrogen were specified by the Cheetah code. A programmed-burn model was used to detonate the charge at a rate based on measured detonation velocities. Computed pressure histories are compared with pressures measured by Kistler 603B piezoelectric gauges at 7 ranges (GR = 0, 5.08, 10.16, 15.24, 20.32, 25.4, and 30.48 cm) along the reflecting surface. Computed and measured waveforms and positive-phase impulses were similar, except at close-in ranges (GR < 5 cm), which were dominated by jetting effects.
Numerical simulation of amplification of space charge waves in n-InP films
Energy Technology Data Exchange (ETDEWEB)
Garcia-Barrientos, Abel, E-mail: abel@upp.edu.mx [Department of Mechatronics, Polytechnic University of Pachuca (UPP), Km. 20 Carretera Pachuca-Cd.Sahagun, Ex-Hacienda de Santa Barbara, 43830 Pachuca, Hidalgo (Mexico); Advanced Materials and Device Analysis Group, Inst. for Microelectronics, TU Wien, Gusshausstr. 27-29, 1040 Vienna (Austria); Palankovski, Vassil, E-mail: palankovski@iue.tuwien.ac.at [Advanced Materials and Device Analysis Group, Inst. for Microelectronics, TU Wien, Gusshausstr. 27-29, 1040 Vienna (Austria)
2011-10-25
The non-linear interaction of space charge waves including the amplification in microwave and millimeter wave range in n-InP films, possessing the negative differential conductance phenomenon, is investigated theoretically. Both the amplified signal and the generation of harmonics of the input signal are demonstrated, which are due to non-linear effect of the negative differential resistance. It is possible to observe an amplification of the space charge waves in n-InP films of submicron thicknesses at essentially higher frequencies f <70 GHz, when compared with n-GaAs films f < 44 GHz. The increment observed in the gain is due to the larger dynamic range in n-InP than in n-GaAs films.
Charge Density Analysis and Transport Properties of TTF Based Molecular Nanowires: A DFT Approach
Directory of Open Access Journals (Sweden)
Karuppannan Selvaraju
2015-01-01
Full Text Available The present study has been performed to understand the charge density distribution and the electrical characteristics of Au and thiol substituted tetrathiafulvalene (TTF based molecular nanowire. A quantum chemical calculation has been carried out using DFT method (B3LYP with the LANL2DZ basis set under various applied electric fields (EFs. The bond topological analysis characterizes the terminal Au–S and S–C bonds as well as all the bonds of central TTF unit of the molecule. The variation of electron density and Laplacian of electron density at the bond critical point of bonds for zero and different applied fields reveal the electron density distribution of the molecule. The molecular conformation, the variation of atomic charges and energy density distribution of the molecule have been analyzed for the various levels of applied EFs. The HOMO-LUMO gap calculated from quantum chemical calculations has been compared with the value calculated from the density of states. The variation of dipole moment due to the polarization effect and the I-V characteristics of the molecule for the various applied EFs have been well discussed.
Static and Dynamical Valence-Charge-Density Properties of GaAs
Pietsch, Ullrich
1993-02-01
Owing to the close neighbourhood of Ga and As in Mendeleev's table, GaAs shows two fundamental classes of X-ray structure amplitudes distinguished by their extremely different scattering power. They are differently sensitive to the valence electron density (VED) redistribution caused by the chemical bond and must be measured by different experimental methods. Using such data, both the VED and the difference electron densities (DED) are calculated here. Comparison with theoret-ical densities shows that the VED is characterized by covalent, ionic and metallic contributions. The DED constructed from GaAs and Ge data demonstrates the electronic response caused by a "protonic" charge transfer between both f.c.c. sublattices as well as the transition from a purely covalent to a mixed covalent-ionic bond. Especially the charge-density accumulation between nearest neighbours (bond charge (BC)) depends on the distance between the bonding atoms and changes under the influence of any lattice deformation. This phenomenon is described by a BC-transfer model. Its direct experimental proof is given by measuring the variation of the scattering power of weak reflections under the influence of an external electric field. This experiment demonstrates that the ionicity of the bond changes in addition to the BC variation.
Charge transfer to a dielectric target by guided ionization waves using electric field measurements
Slikboer, Elmar; Garcia-Caurel, Enric; Guaitella, Olivier; Sobota, Ana
2017-03-01
A kHz-operated atmospheric pressure plasma jet is investigated by measuring charge transferred to a dielectric electro-optic surface (BSO crystal) allowing for the measurement of electric field by exploiting the Pockels effect. The electric field values, distribution of the surface discharge and amount of deposited charge are obtained for various parameters, including gas flow, applied voltage, target distance and the length of the capillary from ground to the end. A newly formed surface discharge emerges at the target when enough charge is deposited at the impact point and electric fields are high enough, i.e. 200 pC and 9 ± 2 kV cm‑1. The maximum amount of charge transferred by a single ionization wave (‘plasma bullet’) is 350 ± 40 pC. Due to the emerging new surface discharge behind the impact point, the total charge deposited on the surface of the dielectric target can increase up to 950 pC. The shape of the secondary discharge on the target is found to be mainly driven by gas flow, while the applied voltage allows us to utilize longer distances within the boundaries set by this gas mixing. Finally the ionization wave is found to lose charge along its propagation on the inner walls of the capillary. The loss is estimated to be approximately 7.5 pC mm‑1 of travel distance inside the capillary.
Nassour, Ayoub; Kubicki, Maciej; Wright, Jonathan; Borowiak, Teresa; Dutkiewicz, Grzegorz; Lecomte, Claude; Jelsch, Christian
2014-04-01
The experimental charge-density distribution in 2-methyl-1,3-cyclopentanedione in the crystal state was analyzed by synchrotron X-ray diffraction data collection at 0.33 Å resolution. The molecule in the crystal is in the enol form. The experimental electron density was refined using the Hansen-Coppens multipolar model and an alternative modeling, based on spherical atoms and additional charges on the covalent bonds and electron lone-pair sites. The crystallographic refinements, charge-density distributions, molecular electrostatic potentials, dipole moments and intermolecular interaction energies obtained from the different charge-density models were compared. The experimental results are also compared with the theoretical charge densities using theoretical structure factors obtained from periodic quantum calculations at the B3LYP/6-31G** level. A strong intermolecular O-H···O hydrogen bond connects molecules along the [001] direction. The deformation density maps show the resonance within the O=C-C=C-OH fragment and merged lone pair lobes on the hydroxyl O atom. This resonance is further confirmed by the analysis of charges and topology of the electron density.
Charge carrier density at the (Na/K)TaO{sub 3}/SrTiO{sub 3} interfaces
Energy Technology Data Exchange (ETDEWEB)
Schwingenschloegl, Udo; Nazir, Safdar [KAUST, PSE Division, Thuwal 23955-6900, Kingdom of Saudi Arabia (Saudi Arabia)
2012-07-01
The formation of a quasi two-dimensional electron gas between the band insulators NaTaO{sub 3} and SrTiO{sub 3} as well as KTaO{sub 3} and SrTiO{sub 3} is studied by means of the full-potential linearized augmented plane-wave method of density functional theory. Optimization of the atomic positions points to only small changes in the chemical bonding at the interface. The creation of metallic interface states thus is not affected by structural relaxation but can be explained by charge transfer between transition metal and oxygen atoms. It is to be expected that a charge transfer is likewise important for related interfaces such as LaAlO{sub 3}/SrTiO{sub 3}. Both the p-type (NaO){sup -}/(TiO{sub 2}){sup 0} and n-type (TaO{sub 2}){sup +}/(SrO){sup 0} interfaces in NaTaO{sub 3}/SrTiO{sub 3} are found to be metallic with strongly enhanced charge carrier densities as compared to the respective interfaces in KTaO{sub 3}/SrTiO{sub 3}. The effects of O vacancies are discussed. Spin-polarized calculations point to the formation of isolated O 2p magnetic moments, located in the metallic region of the p-type interface. The systems under investigation are suitable for disentangling the complex behavior of metallic interface states, since the structural relaxation is small.
A Weakly Nonlinear Model for the Damping of Resonantly Forced Density Waves in Dense Planetary Rings
Lehmann, Marius; Schmidt, Jürgen; Salo, Heikki
2016-10-01
In this paper, we address the stability of resonantly forced density waves in dense planetary rings. Goldreich & Tremaine have already argued that density waves might be unstable, depending on the relationship between the ring’s viscosity and the surface mass density. In the recent paper Schmidt et al., we have pointed out that when—within a fluid description of the ring dynamics—the criterion for viscous overstability is satisfied, forced spiral density waves become unstable as well. In this case, linear theory fails to describe the damping, but nonlinearity of the underlying equations guarantees a finite amplitude and eventually a damping of the wave. We apply the multiple scale formalism to derive a weakly nonlinear damping relation from a hydrodynamical model. This relation describes the resonant excitation and nonlinear viscous damping of spiral density waves in a vertically integrated fluid disk with density dependent transport coefficients. The model consistently predicts density waves to be (linearly) unstable in a ring region where the conditions for viscous overstability are met. Sufficiently far away from the Lindblad resonance, the surface mass density perturbation is predicted to saturate to a constant value due to nonlinear viscous damping. The wave’s damping lengths of the model depend on certain input parameters, such as the distance to the threshold for viscous overstability in parameter space and the ground state surface mass density.
Sanderson, Brian A; Sowersby, Drew S; Crosby, Sergio; Goss, Marcus; Lewis, L Kevin; Beall, Gary W
2013-12-01
Hydrotalcite (HT) and other layered double metal hydroxides are of great interest as gene delivery and timed release drug delivery systems and as enteric vehicles for biologically active molecules that are sensitive to gastric fluids. HT is a naturally occurring double metal hydroxide that can be synthesized as a nanomaterial consisting of a brucite structure with isomorphous substitution of aluminum ions. These positively charged nanoparticles exhibit plate-like morphology with very high aspect ratios. Biomolecules such as nucleic acids and proteins form strong associations with HT because they can associate with the positively charged layers. The binding of nucleic acids with HT and other nanomaterials is currently being investigated for potential use in gene therapy; however, the binding of specific nucleic acid forms, such as single- and double-stranded DNA, has been little explored. In addition, the effects of charge density and particle size on DNA adsorption has not been studied. In this paper, the binding of different forms of DNA to a series of HTs prepared at different temperatures and with different anion exchange capacities has been investigated. Experiments demonstrated that HTs synthesized at higher temperatures associate with both single- and double-stranded oligomers and circular plasmid DNA more tightly than HTs synthesized at room temperature, likely due to the hydrothermal conditions promoting larger particle sizes. HT with an anion exchange capacity of 300 meq/100 g demonstrated the highest binding of DNA, likely due to the closer match of charge densities between the HT and DNA. The details of the interaction of various forms of DNA with HT as a function of charge density, particle size, and concentration are discussed.
Institute of Scientific and Technical Information of China (English)
华建军; 刘金远; 马腾才
2002-01-01
The effect of the charge fluctuation of dust particles on ion acoustic wave (IAW) excited through ionization instability was investigated. The hydrodynamic equations and linear time-dependent perturbation theory served as the starting point of theory, by which the dispersion relation and growth rate of the IAW were given. By comparing the results with the case of constant dust charges, it was found that the charge fluctuation of dust particles reduces the instability of the wave mode.
Sperber, Bram L. H. M.; Schols, Henk A.; Stuart, Martien A. Cohen; Norde, Willem; Voragen, Alphons G. J.
2009-01-01
The complex formation between beta-lactoglobulin (beta-lg) and pectin is studied using pectins with different physicochemical characteristics. Pectin allows for the control of both the overall charge by degree of methyl-esterification as well as local charge density by the degree of blockiness. Vary
Charge transfer polarisation wave and carrier pairing in the high T(sub c) copper oxides
Chakraverty, B. K.
1990-01-01
The High T(sub c) oxides are highly polarizable materials and are charge transfer insulators. The charge transfer polarization wave formalism is developed in these oxides. The dispersion relationships due to long range dipole-dipole interaction of a charge transfer dipole lattice are obtained in 3-D and 2-D. These are high frequency bosons and their coupling with carriers is weak and antiadiabatic in nature. As a result, the mass renormalization of the carriers is negligible in complete contrast to conventional electron-phonon interaction, that give polarons and bipolarons. Both bound and superconducting pairing is discussed for a model Hamiltonian valid in the antiadiabatic regime, both in 3-D and 2-D. The stability of the charge transfer dipole lattice has interesting consequences that are discussed.
Charged Multiplicity Density and Number of Participant Nucleons in Relativistic Nuclear Collisions
Institute of Scientific and Technical Information of China (English)
SA Ben-Hao; CAI Xu; ZHOU Dai-Mei
2003-01-01
The energy and centrality dependencies of charged particle pseudorapidity density in relativistic nuclearcollisions were studied using a hadron and string cascade model, JPCIAE. Both the relativistic p+p experimental dataand the PHOBOS and PHENIX Au+Au data at RHIC energy could be fairly reproduced within the framework ofJPCIAE model and without retuning the model parameters. The predictions for Pb + Pb collisions at the LHC energywere also given. We computed the participant nucleon distributions using different methods. It was found that thenumber of participant nucleons is not a well defined variable both experimentally and theoretically. Thus it may beinappropriate to use the charged particle pseudorapidity density per participant pair .as a function of the number ofparticipant nucleons for distinguishing various theoretical models.
Local distortion in Co-doped LSMO from entropy-maximized charge density distribution
Energy Technology Data Exchange (ETDEWEB)
Syed Ali, K.S. [Department of Physics, The Madura College, Madurai 625011 (India); Saravanan, R., E-mail: saragow@dataone.i [Department of Physics, The Madura College, Madurai 625011 (India); Pashchenko, A.V.; Pashchenko, V.P. [Galkin Donetsk Institute of Physics and Technology, National Academy of Sciences of Ukraine, Donetsk 83114 (Ukraine)
2010-07-09
Perovskite structure manganites La{sub 0.67}Sr{sub 0.22}Mn{sub 1.11-x}Co{sub x}O{sub 3} were prepared by the solid state reaction method. An X-ray analysis of the structure was undertaken using the Rietveld technique on the experimental powder X-ray diffraction data and, then, a charge density distribution study was undertaken, using the maximum entropy method (MEM). The charge density in the unit cell was reconstructed and the effect of Co{sup 3+} doping in the Mn-O matrix was studied. Local distortions due to Co doping were analyzed and the results are now discussed.
Bond length and charge density variations within extended arm chair defects in graphene.
Warner, Jamie H; Lee, Gun-Do; He, Kuang; Robertson, Alex W; Yoon, Euijoon; Kirkland, Angus I
2013-11-26
Extended linear arm chair defects are intentionally fabricated in suspended monolayer graphene using controlled focused electron beam irradiation. The atomic structure is accurately determined using aberration-corrected transmission electron microscopy with monochromation of the electron source to achieve ∼80 pm spatial resolution at an accelerating voltage of 80 kV. We show that the introduction of atomic vacancies in graphene disrupts the uniformity of C-C bond lengths immediately surrounding linear arm chair defects in graphene. The measured changes in C-C bond lengths are related to density functional theory (DFT) calculations of charge density variation and corresponding DFT calculated structural models. We show good correlation between the DFT predicted localized charge depletion and structural models with HRTEM measured bond elongation within the carbon tetragon structure of graphene. Further evidence of bond elongation within graphene defects is obtained from imaging a pair of 5-8-5 divacancies.
Semilocal and Hybrid Density Embedding Calculations of Ground-State Charge-Transfer Complexes
Laricchia, S; Della Sala, F; 10.1063/1.4795825
2013-01-01
We apply the frozen density embedding method, using a full relaxation of embedded densities through a freeze-and-thaw procedure, to study the electronic structure of several benchmark ground-state charge-transfer complexes, in order to assess the merits and limitations of the approach for this class of systems. The calculations are performed using both semilocal and hybrid exchange-correlation (XC) functionals. The results show that embedding calculations using semilocal XC functionals yield rather large deviations with respect to the corresponding supermolecular calculations. Due to a large error cancellation effect, however, they can often provide a relatively good description of the electronic structure of charge-transfer complexes, in contrast to supermolecular calculations performed at the same level of theory. On the contrary, when hybrid XC functionals are employed, both embedding and supermolecular calculations agree very well with each other and with the reference benchmark results. In conclusion, fo...
Exploring effective interactions through transition charge density study of 70,72,74,76Ge nuclei
Indian Academy of Sciences (India)
A Shukla; P K Raina; P K Rath
2005-02-01
Transition charge densities (TCD) for $0^{+} → 2_{1}^{+}$ excitation have been calculated for 70, 72, 74, 76Ge nuclei within microscopic variational framework employing 23/2, 15/2, 21/2 and 19/2 valence space. The calculated TCDs for different monopole variants of Kuo interaction are compared with available experimental results. Other systematics like reduced transition probabilities (2) and static quadrupole moments (2) are also presented. It is observed that the transition density study acts as a sensitive probe for discriminating the response of different parts of effective interactions.
Institute of Scientific and Technical Information of China (English)
LIN Chang; ZHANG Xiu-Lian
2005-01-01
The nonlinear dust acoustic waves in two-dimensional dust plasma with dust charge variation is analytically investigated by using the formally variable separation approach. New analytical solutions for the governing equation of this system have been obtained for dust acoustic waves in a dust plasma for the first time. We derive exact analytical expressions for the general case of the nonlinear dust acoustic waves in two-dimensional dust plasma with dust charge variation.
The scaling dimension of low lying Dirac eigenmodes and of the topological charge density
Energy Technology Data Exchange (ETDEWEB)
Aubin, C. [Department of Physics, Washington University, St. Louis, MO 63130 (United States); Bernard, C. [Department of Physics, Washington University, St. Louis, MO 63130 (United States); Gottlieb, Steven [Department of Physics, Indiana Univerity, Bloomington, IN 47405 (United States); Gregory, E.B. [Department of Physics, University of Arizona, Tucson, AZ 85721 (United States); Heller, Urs M. [American Physical Society, One Research Road, Box 9000, Ridge, NY 11961 (United States); Hetrick, J.E. [Physics Department, University of the Pacific, Stockton, CA 95211 (United States); Osborn, J.; Sugar, R. [Department of Physics, University of California, Santa Barbara, CA 93106 (United States); Forcrand, Ph. de [Institute for Theoretical Physics, ETH Zuerich, CH-8093 Zurich (Switzerland); CERN, Theory Division, CH-1211 Geneva 23 (Switzerland); Jahn, O. [Center for Theoretical Physics, MIT, Cambridge, MA 02139 (United States)
2005-03-15
As a quantitative measure of localization, the inverse participation ratio of low lying Dirac eigenmodes and topological charge density is calculated on quenched lattices over a wide range of lattice spacings and volumes. Since different topological objects (instantons, vortices, monopoles, and artifacts) have different co-dimension, scaling analysis provides information on the amount of each present and their correlation with the localization of low lying eigenmodes.
Energy Technology Data Exchange (ETDEWEB)
Reshak, A.H. [New Technologies-Research Center, University of West Bohemia, Univerzitni 8, 306 14 Pilsen (Czech Republic); Center of Excellence Geopolymer and Green Technology, School of Material Engineering, University Malaysia Perlis, 01007 Kangar, Perlis (Malaysia); Khan, Wilayat, E-mail: walayat76@gmail.com [New Technologies-Research Center, University of West Bohemia, Univerzitni 8, 306 14 Pilsen (Czech Republic)
2014-04-01
Highlights: • FP-LAPW technique is used for calculating the electronic structure. • The band structure shows that the calculated compound is semiconductor. • The complex dielectric function has been calculated. • Nonlinear optical properties has also been calculated. • This compound can be used for molecular engineering of the crystals. - Abstract: Self-consistent calculations is performed using the full potential linear augmented plane wave (FP-LAPW) technique based on density functional theory (DFT) to investigate the electronic band structure, density of states, electronic charge density, linear and non-linear optical properties of α-LiAlTe{sub 2} compound having tetragonal symmetry with space group I4{sup ¯}2d. The electronic structure are calculated using the Ceperley Alder local density approach (CA-LDA), Perdew Burke and Ernzerhof generalize gradient approach (PBE-GGA), Engel–Vosko generalize gradient approach (EVGGA) and modified Becke Johnson approach (mBJ). Band structure calculations of (α-LiAlTe{sub 2}) depict semiconducting nature with direct band gap of 2.35 eV (LDA), 2.48 eV (GGA), 3.05 eV (EVGGA) and 3.13 eV (mBJ), which is comparable to experimental value. The calculated electronic charge density show ionic interaction between Te and Li atoms and polar covalent interaction between Al and Te atoms. Some optical susceptibilities like dielectric constants, refractive index, extension co-efficient, reflectivity and energy loss function have been calculated and analyzed on the basis of electronic structure. The compound α-LiAlTe{sub 2} provides a considerable negative value of birefringence of −0.01. Any anisotropy observed in the linear optical properties which are in favor to enhance the nonlinear optical properties. The symbol χ{sub abc}{sup (2)}(ω) represents the second order nonlinear optical susceptibilities, possess six non-zero components in this symmetry (tetragonal), called: 1 2 3, 2 1 3, 2 3 1, 1 3 2, 3 1 2 and 3 2 1
3D High Density mmWave Interconnects Project
National Aeronautics and Space Administration — Nuvotronics has developed and optimized the PolyStrataTM process for the fabrication of intricate microwave and millimeter-wave devices. These devices have primarily...
Winters, Caroline; Petrishchev, Vitaly; Yin, Zhiyao; Lempert, Walter R.; Adamovich, Igor V.
2015-10-01
The present work provides insight into surface charge dynamics and kinetics of radical species reactions in nanosecond pulse discharges sustained at a liquid-vapor interface, above a distilled water surface. The near-surface plasma is sustained using two different discharge configurations, a surface ionization wave discharge between two exposed metal electrodes and a double dielectric barrier discharge. At low discharge pulse repetition rates (~100 Hz), residual surface charge deposition after the discharge pulse is a minor effect. At high pulse repetition rates (~10 kHz), significant negative surface charge accumulation over multiple discharge pulses is detected, both during alternating polarity and negative polarity pulse trains. Laser induced fluorescence (LIF) and two-photon absorption LIF (TALIF) line imaging are used for in situ measurements of spatial distributions of absolute OH and H atom number densities in near-surface, repetitive nanosecond pulse discharge plasmas. Both in a surface ionization wave discharge and in a double dielectric barrier discharge, peak measured H atom number density, [H] is much higher compared to peak OH number density, due to more rapid OH decay in the afterglow between the discharge pulses. Higher OH number density was measured near the regions with higher plasma emission intensity. Both OH and especially H atoms diffuse out of the surface ionization wave plasma volume, up to several mm from the liquid surface. Kinetic modeling calculations using a quasi-zero-dimensional H2O vapor / Ar plasma model are in qualitative agreement with the experimental data. The results demonstrate the experimental capability of in situ radical species number density distribution measurements in liquid-vapor interface plasmas, in a simple canonical geometry that lends itself to the validation of kinetic models.
Rajalakshmi, Gnanasekaran; Hathwar, Venkatesha R; Kumaradhas, Poomani
2014-06-01
An experimental charge-density analysis of pyrazinamide (a first line antitubercular drug) was performed using high-resolution X-ray diffraction data [(sin θ/λ)max = 1.1 Å(-1)] measured at 100 (2) K. The structure was solved by direct methods using SHELXS97 and refined by SHELXL97. The total electron density of the pyrazinamide molecule was modeled using the Hansen-Coppens multipole formalism implemented in the XD software. The topological properties of electron density determined from the experiment were compared with the theoretical results obtained from CRYSTAL09 at the B3LYP/6-31G** level of theory. The crystal structure was stabilized by N-H...N and N-H...O hydrogen bonds, in which the N3-H3B...N1 and N3-H3A...O1 interactions form two types of dimers in the crystal. Hirshfeld surface analysis was carried out to analyze the intermolecular interactions. The fingerprint plot reveals that the N...H and O...H hydrogen-bonding interactions contribute 26.1 and 18.4%, respectively, of the total Hirshfeld surface. The lattice energy of the molecule was calculated using density functional theory (B3LYP) methods with the 6-31G** basis set. The molecular electrostatic potential of the pyrazinamide molecule exhibits extended electronegative regions around O1, N1 and N2. The existence of a negative electrostatic potential (ESP) region just above the upper and lower surfaces of the pyrazine ring confirm the π-electron cloud.
Fluctuations around Periodic BPS-Density Waves in the Calogero Model
Bardek, V; Meljanac, S
2010-01-01
The collective field formulation of the Calogero model supports periodic density waves. An important set of such density waves is a two-parameter family of BPS solutions of the equations of motion of the collective field theory. One of these parameters is essentially the average particle density, which determines the period, while the other parameter determines the amplitude. These BPS solutions are sometimes referred to as "small amplitude waves" since they undulate around their mean density, but never vanish. We present complete analysis of quadratic fluctuations around these BPS solutions. The corresponding fluctuation hamiltonian (i.e., the stability operator) is diagonalized in terms of bosonic creation and annihilation operators which correspond to the complete orthogonal set of Bloch-Floquet eigenstates of a related periodic Schr\\"odinger hamiltonian, which we derive explicitly. Remarkably, the fluctuation spectrum is independent of the parameter which determines the density wave's amplitude. As a cons...
Energy Technology Data Exchange (ETDEWEB)
Balsa Terzic, Gabriele Bassi
2011-07-01
In this paper we discuss representations of charge particle densities in particle-in-cell (PIC) simulations, analyze the sources and profiles of the intrinsic numerical noise, and present efficient methods for their removal. We devise two alternative estimation methods for charged particle distribution which represent significant improvement over the Monte Carlo cosine expansion used in the 2d code of Bassi, designed to simulate coherent synchrotron radiation (CSR) in charged particle beams. The improvement is achieved by employing an alternative beam density estimation to the Monte Carlo cosine expansion. The representation is first binned onto a finite grid, after which two grid-based methods are employed to approximate particle distributions: (i) truncated fast cosine transform (TFCT); and (ii) thresholded wavelet transform (TWT). We demonstrate that these alternative methods represent a staggering upgrade over the original Monte Carlo cosine expansion in terms of efficiency, while the TWT approximation also provides an appreciable improvement in accuracy. The improvement in accuracy comes from a judicious removal of the numerical noise enabled by the wavelet formulation. The TWT method is then integrated into Bassi's CSR code, and benchmarked against the original version. We show that the new density estimation method provides a superior performance in terms of efficiency and spatial resolution, thus enabling high-fidelity simulations of CSR effects, including microbunching instability.
Energy Technology Data Exchange (ETDEWEB)
Campsie, P; Cunningham, L; Hendry, M; Hough, J; Reid, S; Rowan, S; Hammond, G D, E-mail: p.campsie@physics.gla.ac.uk [SUPA , Institute for Gravitational Research, School of Physics and Astronomy, University of Glasgow, Glasgow, G12 8QQ (United Kingdom)
2011-11-07
Charging of silica test masses in gravitational wave detectors could potentially become a significant low-frequency noise source for advanced detectors. Charging noise has already been observed and confirmed in the GEO600 detector and is thought to have been observed in one of the LIGO detectors. In this paper, two charge mitigation techniques using glow and corona discharges were investigated to create repeatable and robust procedures. The glow discharge procedure was used to mitigate charge under vacuum and would be intended to be used in the instance where an optic has become charged while the detector is in operation. The corona discharge procedure was used to discharge samples at atmospheric pressure and would be intended to be used to discharge the detector optics during the cleaning of the optics. Both techniques were shown to reduce both polarities of surface charge on fused silica to a level that would not limit advanced LIGO. Measurements of the transmission of samples that had undergone the charge mitigation procedures showed no significant variation in transmission, at a sensitivity of {approx} 200 ppm, in TiO{sub 2}-doped Ta{sub 2}O{sub 5}/SiO{sub 2} multi-layer coated fused silica.
Dong, Xiao-Yan; Chen, Ran; Yang, Chun-Yan; Sun, Yan
2014-06-20
We have previously found that addition of like-charged media in a refolding solution can greatly enhance the refolding of pure proteins by suppressing protein aggregation. Herein, negatively charged mono-sized microspheres with sulfonic groups were fabricated to explore the facilitating effect of like-charged media on the refolding of enhanced green fluorescent protein (EGFP) expressed as inclusion bodies (IBs). A sequential polymer-tentacle grafting and sulfonate modification strategy was developed to increase the charge density of mono-sized poly(glycidyl methacrylate) (pGMA) beads (2.4μm). Namely, GMA was first grafted onto the beads by grafting polymerization to form poly(GMA) tentacles on the pGMA beads, and then the epoxy groups on the tentacles were converted into sulfonic groups by modification with sodium sulfite. By this fabrication strategy, the charge density of the beads reached 793μmol/g, about 2.8 times higher than that modified without prior grafting of the pGMA beads (285μmol/g). The negatively charged beads of different charge densities were used for facilitating the refolding of like-charged EGFP from IBs. The refolding yield as well as refolding rate increased with increasing charge density. The anti-aggregation effects of urea and like-charged microspheres were synergetic. In addition, partial purification of EGFP was achieved because the ion-exchange adsorption led to 52% removal of positively charged contaminant proteins in the refolded solution. Finally, reusability of the tentacle beads was demonstrated by repetitive EGFP refolding and recovery cycles.
GyPSuM: A Detailed Tomographic Model of Mantle Density and Seismic Wave Speeds
Energy Technology Data Exchange (ETDEWEB)
Simmons, N A; Forte, A M; Boschi, L; Grand, S P
2010-03-30
GyPSuM is a tomographic model fo mantle seismic shear wave (S) speeds, compressional wave (P) speeds and detailed density anomalies that drive mantle flow. the model is developed through simultaneous inversion of seismic body wave travel times (P and S) and geodynamic observations while considering realistic mineral physics parameters linking the relative behavior of mantle properties (wave speeds and density). Geodynamic observations include the (up to degree 16) global free-air gravity field, divergence of the tectonic plates, dynamic topography of the free surface, and the flow-induced excess ellipticity of the core-mantle boundary. GyPSuM is built with the philosophy that heterogeneity that most closely resembles thermal variations is the simplest possible solution. Models of the density field from Earth's free oscillations have provided great insight into the density configuration of the mantle; but are limited to very long-wavelength solutions. Alternatively, simply scaling higher resolution seismic images to density anomalies generates density fields that do not satisfy geodynamic observations. The current study provides detailed density structures in the mantle while directly satisfying geodynamic observations through a joint seismic-geodynamic inversion process. Notable density field observations include high-density piles at the base of the superplume structures, supporting the fundamental results of past normal mode studies. However, these features are more localized and lower amplitude than past studies would suggest. When we consider all seismic anomalies in GyPSuM, we find that P and S-wave speeds are strongly correlated throughout the mantle. However, correlations between the high-velocity S zones in the deep mantle ({approx} 2000 km depth) and corresponding P-wave anomalies are very low suggesting a systematic divergence from simplified thermal effects in ancient subducted slab anomalies. Nevertheless, they argue that temperature variations are
Equivalence theorem for the spectral density of light waves on weak scattering.
Wang, Tao; Ji, Xiaoling; Zhao, Daomu
2014-07-01
The Equivalence theorem for the spectral density of light waves on weak scattering is discussed. It is shown that when a spatially coherent plane light wave is scattered from two entirely different media, the far-zone spectral density may have identical distribution provided the low-frequency antidiagonal spatial Fourier components of the correlation function of the media are the same. An example of light waves on scattering from a Gaussian Schell model medium is discussed, and the condition on which two different media may produce identical spectral densities is presented.
Semi-analytic variable charge solitary waves involving dust phase-space vortices (holes)
Energy Technology Data Exchange (ETDEWEB)
Tribeche, Mouloud; Younsi, Smain; Amour, Rabia; Aoutou, Kamel [Plasma Physics Group, Faculty of Sciences-Physics, Theoretical Physics Laboratory, University of Bab-Ezzouar, USTHB BP 32, El Alia, Algiers 16111 (Algeria)], E-mail: mtribeche@usthb.dz
2009-09-15
A semi-analytic model for highly nonlinear solitary waves involving dust phase-space vortices (holes) is outlined. The variable dust charge is expressed in terms of the Lambert function and we take advantage of this transcendental function to investigate the localized structures that may occur in a dusty plasma with variable charge trapped dust particles. Our results which complement the previously published work on this problem (Schamel et al 2001 Phys. Plasmas 8 671) should be of basic interest for experiments that involve the trapping of dust particles in ultra-low-frequency dust acoustic modes.
Dust ion-acoustic shock waves due to dust charge fluctuation in a superthermal dusty plasma
Energy Technology Data Exchange (ETDEWEB)
Alinejad, H., E-mail: alinejad@nit.ac.ir [Department of Physics, Faculty of Basic Science, Babol University of Technology, Babol 47148-71167 (Iran, Islamic Republic of); Research Institute for Fundamental Sciences (RIFS), University of Tabriz, 51664, Tabriz (Iran, Islamic Republic of); Tribeche, M. [Plasma Physics Group, Faculty of Sciences – Physics, University of Bab-Ezzouar (Algeria); Mohammadi, M.A. [Research Institute for Fundamental Sciences (RIFS), University of Tabriz, 51664, Tabriz (Iran, Islamic Republic of); Department of Atomic and Molecular Physics, Faculty of Physics, University of Tabriz, Tabriz (Iran, Islamic Republic of)
2011-11-14
The nonlinear propagation of dust ion-acoustic (DIA) shock waves is studied in a charge varying dusty plasma with electrons having kappa velocity distribution. We use hot ions with equilibrium streaming speed and a fast superthermal electron charging current derived from orbit limited motion (OLM) theory. It is found that the presence of superthermal electrons does not only significantly modify the basic properties of shock waves, but also causes the existence of shock profile with only positive potential in such plasma with parameter ranges corresponding to Saturn's rings. It is also shown that the strength and steepness of the shock waves decrease with increase of the size of dust grains and ion temperature. -- Highlights: ► The presence of superthermal electrons causes the existence of shock waves with only positive potential. ► The strength and steepness of the shock waves decrease with increase of the size of dust grains and ion temperature. ► As the electrons evolve toward their thermodynamic equilibrium, the shock structures are found with smaller amplitude.
Optimization design of a Lamb wave device for density sensing of nonviscous liquid.
Chen, Zhijun; Li, Lianger; Shi, Wenkang; Guo, Huawei
2007-10-01
A Lamb wave device composed of a piezoelectric plate loaded with a nonviscous liquid layer is presented. The relation between the Lamb wave phase velocity and the liquid density can be used for liquid density sensing. In this paper, utilizing the partial wave theory, the concept of effective permittivity is introduced to analyze the Lamb wave's excitation and the phase velocity calculation under a certain liquid density. The interface between the Lamb wave device and the liquid layer is metallized to eliminate the influence of liquid electrical properties when sensing liquid density. Based on the theory model, the phase difference measurement method is adopted to study the device's sensitivity to liquid density. In order to achieve high sensitivity to liquid density with sufficient excitation efficiency of Lamb wave, the optimal parameters of the Lamb wave device including plate thickness and cut orientation are obtained by numerical calculation. The experimental results are found to be in agreement with the theoretical simulations, verifying the validity of the theory model and the practicability of the optimization design.
Interaction of solitary waves in magnetized warm dusty plasmas with dust charging effects
Institute of Scientific and Technical Information of China (English)
Xue Ju-Kui
2006-01-01
In consideration of adiabatic dust charge variation, the combined effect of the external magnetized field and the dust temperature on head-on collision of the three-dimensional dust acoustic solitary waves is investigated. By using the extended Poincaré-Lighthill-Kuo method, the phase shifts and the trajectories of two solitons after the collision are obtained. The effects of the magnitude and the obliqueness of the external magnetic field and the dust temperature on the solitary wave collisions are discussed in detail.
Lee, Louis P; Limas, Nidia Gabaldon; Cole, Daniel J; Payne, Mike C; Skylaris, Chris-Kriton; Manz, Thomas A
2014-12-01
The density derived electrostatic and chemical (DDEC/c3) method is implemented into the onetep program to compute net atomic charges (NACs), as well as higher-order atomic multipole moments, of molecules, dense solids, nanoclusters, liquids, and biomolecules using linear-scaling density functional theory (DFT) in a distributed memory parallel computing environment. For a >1000 atom model of the oxygenated myoglobin protein, the DDEC/c3 net charge of the adsorbed oxygen molecule is approximately -1e (in agreement with the Weiss model) using a dynamical mean field theory treatment of the iron atom, but much smaller in magnitude when using the generalized gradient approximation. For GaAs semiconducting nanorods, the system dipole moment using the DDEC/c3 NACs is about 5% higher in magnitude than the dipole computed directly from the quantum mechanical electron density distribution, and the DDEC/c3 NACs reproduce the electrostatic potential to within approximately 0.1 V on the nanorod's solvent-accessible surface. As examples of conducting materials, we study (i) a 55-atom Pt cluster with an adsorbed CO molecule and (ii) the dense solids Mo2C and Pd3V. Our results for solid Mo2C and Pd3V confirm the necessity of a constraint enforcing exponentially decaying electron density in the tails of buried atoms.
Charge creation and nucleation of longitudinal plasma wave in coupled Josephson junctions
Shukrinov, Yu M.; Hamdipour, M.
2009-01-01
We study the phase dynamics in coupled Josephson junctions describing by system of nonlinear differential equations. Results of detailed numerical simulations of charge creation in the superconducting layers and the longitudinal plasma wave (LPW) nucleation are presented. We demonstrate the different time stages in the development of the LPW and present results of FFT analysis at different values of bias current. The correspondence between the breakpoint position on the outermost branch of cu...
Phase modulation spectroscopy of space-charge wave resonances in Bi12SiO20
DEFF Research Database (Denmark)
Vasnetsov, M.; Buchhave, Preben; Lyuksyutov, S.
1997-01-01
A new experimental method for the study of resonance effects and space-charge wave excitation in photorefractive Bi12SiO20 crystals by using a combination of frequency detuning and phase modulation technique has been developed. The accuracy of the method allows a detection of resonance peaks...... and revealed its resonance dependence. A minimum of electric current through the sample corresponds to the main resonance detected by phase modulation technique....
Bachelard, R; Chandre, C; Vittot, M
2008-09-01
The Hamiltonian description of the self-consistent interaction between an electromagnetic plane wave and a copropagating beam of charged particles is considered. We show how the motion can be reduced to a one-dimensional Hamiltonian model (in a canonical setting) from the Vlasov-Maxwell Poisson brackets. The reduction to this paradigmatic Hamiltonian model is performed using a Lie algebraic formalism which allows us to preserve the Hamiltonian character at each step of the derivation.
Bachelard, Romain; Vittot, Michel
2008-01-01
The Hamiltonian description of the self-consistent interaction between an electromagnetic plane-wave and a co-propagating beam of charged particles is considered. We show how the motion can be reduced to a one-dimensional Hamiltonian model (in a canonical setting) from the Vlasov-Maxwell Poisson brackets. The reduction to this paradigmatic Hamiltonian model is performed using a Lie algebraic formalism which allows us to remain Hamiltonian at each step of the derivation.
Haldrup, Sofie; Catalano, Jacopo; Hinge, Mogens; Jensen, Grethe V; Pedersen, Jan S; Bentien, Anders
2016-02-23
The electrokinetic energy conversion (EKEC) of hydraulic work directly into electrical energy has been investigated in charged polymeric membranes with different pore charge densities and characteristic diameters of the nanoporous network. The membranes were synthesized from blends of nitrocellulose and sulfonated polystyrene (SPS) and were comprehensively characterized with respect to structure, composition, and transport properties. It is shown that the SPS can be used as a sacrificial pore generation medium to tune the pore size and membrane porosity, which in turn highly affects the transport properties of the membranes. Furthermore, it is shown that very high EKEC efficiencies (>35%) are encountered in a rather narrow window of the properties of the nanoporous membrane network, that is, with pore diameters of ca. 10 nm and pore charge densities of 4.6 × 10(2) to 1.5 × 10(3) mol SO3(-) m(-3) for dilute solutions (0.03 M LiCl). The high absolute value of the efficiency combined with the determination of the optimal membrane morphology makes membrane-based EKEC devices a step closer to practical applications and high-performance membrane design less empirical.
Shock-associated MHD waves - A model for interstellar density fluctuations
Spangler, Steven R.
1988-01-01
The possibility that the density fluctuations responsible for radio scintillations could be due to ion-beam-generated MHD waves near interstellar shock waves is discussed. This suggestion is inspired by spacecraft observations which reveal these phenomena near shocks in the solar system. The model quite naturally accounts for the scale on which these fluctuations occur; it is dictated by the wavelength of the unstable waves.
Damping-Growth Transition for Ion-Acoustic Waves in a Density Gradient
DEFF Research Database (Denmark)
D'Angelo, N.; Michelsen, Poul; Pécseli, Hans
1975-01-01
A damping-growth transition for ion-acoustic waves propagating in a nonuniform plasma (e-folding length for the density ln) is observed at a wavelength λ∼2πln. This result supports calculations performed in connection with the problem of heating of the solar corona by ion-acoustic waves generated...
Charge creation and nucleation of the longitudinal plasma wave in coupled Josephson junctions
Shukrinov, Yu. M.; Hamdipour, M.
2010-11-01
We study the phase dynamics in coupled Josephson junctions described by a system of nonlinear differential equations. Results of detailed numerical simulations of charge creation in the superconducting layers and the longitudinal plasma wave (LPW) nucleation are presented. We demonstrate the different time stages in the development of the LPW and present the results of FFT analysis at different values of bias current. The correspondence between the breakpoint position on the outermost branch of current voltage characteristics (CVC) and the growing region in time dependence of the electric charge in the superconducting layer is established. The effects of noise in the bias current and the external microwave radiation on the charge dynamics of the coupled Josephson junctions are found. These effects introduce a way to regulate the process of LPW nucleation in the stack of IJJ.
Fujita, Toshiyuki; Sasaki, Takahiko; Yoneyama, Naoki; Kobayashi, Norio
2004-06-01
Current-voltage characteristics are measured in the quasi-two dimensional organic conductor α-(BEDT-TTF)2KHg(SCN)4 at temperatures down to 0.5 K and in the magnetic field up to 25 T. The non-linear conduction with a threshold electric field is found in the density wave state. The features of threshold electric field obtained in the low magnetic field region are explained by the unconventional charge density wave model. In the high magnetic field region, where the Shubnikov-de Haas oscillations appear, the current-voltage characteristics reveal that the density wave state synchronizes with the filling of the electron on the Landau level and continues even above a kink field 23 T.
Foury-Leylekian, Pascale; Pouget, Jean-Paul; Lee, Young-Joo; Nieminen, Risto M.; Ordejón, Pablo; Canadell, Enric
2010-10-01
α-(BEDT-TTF)2KHg(SCN)4 develops a density wave ground state below 8 K whose origin is still debated. Here we report a combined x-ray diffuse scattering and first-principles density functional theory study supporting the charge density wave (CDW) scenario. In particular, we observe a triply incommensurate anharmonic lattice modulation with intralayer wave vector components which coincide within experimental errors to the maximum of the calculated Lindhard response function. A detailed study of the structural aspects of the modulation shows that the CDW instability in α-(BEDT-TTF)2KHg(SCN)4 is considerably more involved than those following a standard Peierls mechanism. We thus propose a microscopic mechanism where the CDW instability of the BEDT-TTF layer is triggered by the anion sublattice. Our mechanism also emphasizes the key role of the coupling of the BEDT-TTF and anion layers via the hydrogen bond network to set the global modulation.
(2 kF , 2 kF) density-wave orders of interacting p-orbital fermions in square optical lattice
Zhang, Zixu; Liu, W. Vincent
2011-03-01
We study instabilities of spinless fermionic atoms in the p- orbital bands in two dimensional optical lattices at non- integer filling against interactions. Stripe charge-density- wave or orbital-density-wave orders are found for attractive and repulsive interactions, respectively. A surprising result is that the superfluid phase, usually expected of attractively interacting fermions, is less energetically favored. Nesting quasi-one-dimensional Fermi surfaces in such systems are independent of filling, which ensures that the stripe density- wave orders occur in a large parameter regime. This work is supported by ARO (W911NF-07-1-0293) and ARO-DARPA-OLE (W911NF-07-1-0464). We also thank the KITP at UCSB for its hospitality where this research is supported in part by NSF Grant No. PHY05-51164.
Li, Xiao; Roy, Bitan; Das Sarma, S.
2016-11-01
We theoretically address the effects of strong magnetic fields in three-dimensional Weyl semimetals (WSMs) built out of Weyl nodes with a monopole charge n . For n =1 , 2, and 3 we realize single, double, and triple WSM, respectively, and the monopole charge n determines the integer topological invariant of the WSM. Within the linearized continuum description, the quasiparticle spectrum is then composed of Landau levels (LLs), containing exactly n number of chiral zeroth Landau levels (ZLLs), irrespective of the orientation of the magnetic field. In the presence of strong backscattering, for example (due to quenched disorder associated with random impurities), these systems generically give rise to longitudinal magnetotransport. Restricting ourselves to the quantum limit (and assuming only the subspace of the ZLLs to be partially filled) and mainly accounting for Gaussian impurities, we show that the longitudinal magnetoconductivity (LMC) in all members of the Weyl family displays a positive linear-B scaling when the field is applied along the axis that separates the Weyl nodes. But, in double and triple WSM, LMC displays a smooth crossover to a nonlinear B dependence as the field is tilted away from such a high-symmetry direction. In addition, due to the enhanced density of states, the LL quantization can trigger instabilities toward the formation of translational symmetry-breaking density-wave orderings for sufficiently weak interaction (BCS instability), which gaps out the ZLLs. Concomitantly as the temperature (magnetic field) is gradually decreased (increased) the LMC becomes negative. Thus WSMs with arbitrary monopole charge (n ) can host an intriguing interplay of LL quantization, longitudinal magnetotransport (a possible manifestation of one-dimensional chiral or axial anomaly), and density-wave ordering, when placed in a strong magnetic field.
Naik, Hemantkumar G; Yeniad, Bahar; Koning, Cor E; Heise, Andreas
2012-07-01
In an effort to study the effect of substituent groups of the substrate on the alcohol dehydrogenase (ADH) reductions of aryl-alkyl ketones, several derivatives of acetophenone have been evaluated against ADHs from Lactobacillus brevis (LB) and Thermoanaerobacter sp. (T). Interestingly, ketones with non-demanding (neutral) para-substituents were reduced to secondary alcohols by these enzymes in enantiomerically pure form whereas those with demanding (ionizable) substituents could not be reduced. The effect of substrate size, their solubility in the reaction medium, electron donating and withdrawing properties of the ligand and also the electronic charge density distribution on the substrate molecules have been studied and discussed in detail. From the results, it is observed that the electronic charge distribution in the substrate molecules is influencing the orientation of the substrate in the active site of the enzyme and hence the ability to reduce the substrate.
Dispersive MHD waves and alfvenons in charge non-neutral plasmas
Directory of Open Access Journals (Sweden)
K. Stasiewicz
2008-08-01
Full Text Available Dispersive properties of linear and nonlinear MHD waves, including shear, kinetic, electron inertial Alfvén, and slow and fast magnetosonic waves are analyzed using both analytical expansions and a novel technique of dispersion diagrams. The analysis is extended to explicitly include space charge effects in non-neutral plasmas. Nonlinear soliton solutions, here called alfvenons, are found to represent either convergent or divergent electric field structures with electric potentials and spatial dimensions similar to those observed by satellites in auroral regions. Similar solitary structures are postulated to be created in the solar corona, where fast alfvenons can provide acceleration of electrons to hundreds of keV during flares. Slow alfvenons driven by chromospheric convection produce positive potentials that can account for the acceleration of solar wind ions to 300–800 km/s. New results are discussed in the context of observations and other theoretical models for nonlinear Alfvén waves in space plasmas.
Unconventional Density Wave and Superfluidity in Cold Atom Systems
2014-06-01
fillings between quarter and half, with on-site and 16 30 nearest-neighbor repulsion [26]. Its application to the coupled quarter-filled ladders with...result that Majorana fermions can be generated as a zero-energy mode in the excitation spectrum of a half-quantum vortex in a (p + ip)-wave superconductor ...spin populations have been studied in electronic mate- rials, such as magnetic-field-induced organic superconductors [63, 64]. Mixtures of different
Commensurate and incommensurate spin-density waves in heavy electron systems
Directory of Open Access Journals (Sweden)
P. Schlottmann
2016-05-01
Full Text Available The nesting of the Fermi surfaces of an electron and a hole pocket separated by a nesting vector Q and the interaction between electrons gives rise to itinerant antiferromagnetism. The order can gradually be suppressed by mismatching the nesting and a quantum critical point (QCP is obtained as the Néel temperature tends to zero. The transfer of pairs of electrons between the pockets can lead to a superconducting dome above the QCP (if Q is commensurate with the lattice, i.e. equal to G/2. If the vector Q is not commensurate with the lattice there are eight possible phases: commensurate and incommensurate spin and charge density waves and four superconductivity phases, two of them with modulated order parameter of the FFLO type. The renormalization group equations are studied and numerically integrated. A re-entrant SDW phase (either commensurate or incommensurate is obtained as a function of the mismatch of the Fermi surfaces and the magnitude of |Q − G/2|.
Energy Flux and Density of Nonuniform Electromagnetic Waves with Total Reflection
Petrov, N. S.
2014-07-01
Analytic expressions are obtained for the energy flux and density of refracted nonuniform waves produced during total reflection at the boundary between two isotropic media for the general case of elliptically polarized incident light. The average values are determined as functions of the parameters of the adjoining media and the angle of incidence. The cases of linearly and circularly polarized incident waves are examined in detail. An explicit general expression relating the energy fl ux and density of these waves for arbitrarily polarized incident light is obtained.
Calculation of the Nuclear Transition Charge Density in a Microscopic sdgIBM-1
Institute of Scientific and Technical Information of China (English)
ZHANG Zhan-Jun; SANG Jian-ping; LIU Yong
2000-01-01
Formulae of proton and neutron boson structure functions (BSF's) are deduced in terms of a microscopic approach of sdgIBM (namely, microscopic sdgIBM). For the nucleus 190Os, the value of BSF's is worked out. Due to the high similarity, the maximum F-spin truncation is made under the full-symmetry approximation. Thereafter, calculations of E2 and E4 transition charge densities (TCD's) are performed in the sdgIBM-1. It is found that the E2 and E4 TCD's can be reproduced quite satisfactorily in the uniform frame of microscopic sdgIBM-1.
Effect of the surface charge density on the creep of copper
Zhmakin, Yu. D.; Rybyanets, V. A.; Nevskii, S. A.; Gromov, V. E.
2015-01-01
The creep of polycrystalline copper under the action of high and low electric potentials is studied. At potentials of ±4 kV and ±5 V, the steady-state creep rate decreases, and the effect in the former case is weaker than in the latter by a factor of 2.5. This difference is caused by the fact that the charge density in the sample-capacitor bank system at the high electric potentials is lower than at the low potentials.
Mitri, F G
2016-09-01
Energy and angular momentum flux density characteristics of an optical nondiffracting nonparaxial vector Bessel vortex beam of fractional order are examined based on the dual-field method for the generation of symmetric electric and magnetic fields. Should some conditions determined by the polarization state, the half-cone angle as well as the beam-order (or topological charge) be met, the axial energy and angular momentum flux densities vanish (representing Poynting singularities), before they become negative. These negative counterintuitive properties suggest retrograde (negative) propagation as well as a rotation reversal of the angular momentum with respect to the beam handedness. These characteristics of nondiffracting nonparaxial Bessel fractional vortex beams of progressive waves open new capabilities in optical tractor beam tweezers, optical spanners, invisibility cloaks, optically engineered metamaterials, and other applications.
Tracking the density evolution in counter-propagating shock waves using imaging X-ray scattering
Zastrau, U.; Gamboa, E. J.; Kraus, D.; Benage, J. F.; Drake, R. P.; Efthimion, P.; Falk, K.; Falcone, R. W.; Fletcher, L. B.; Galtier, E.; Gauthier, M.; Granados, E.; Hastings, J. B.; Heimann, P.; Hill, K.; Keiter, P. A.; Lu, J.; MacDonald, M. J.; Montgomery, D. S.; Nagler, B.; Pablant, N.; Schropp, A.; Tobias, B.; Gericke, D. O.; Glenzer, S. H.; Lee, H. J.
2016-07-01
We present results from time-resolved X-ray imaging and inelastic scattering on collective excitations. These data are then employed to infer the mass density evolution within laser-driven shock waves. In our experiments, thin carbon foils are first strongly compressed and then driven into a dense state by counter-propagating shock waves. The different measurements agree that the graphite sample is about twofold compressed when the shock waves collide, and a sharp increase in forward scattering indicates disassembly of the sample 1 ns thereafter. We can benchmark hydrodynamics simulations of colliding shock waves by the X-ray scattering methods employed.
Electronic properties and charge density of BeZn1−Te alloys
Indian Academy of Sciences (India)
C B Swarnkar; U Paliwal; N N Patel; K B Joshi
2011-06-01
Electronic band structure calculations are performed for the BeZn1−Te (0 ≤ ≤ 1 in steps of 0.2) alloys following the empirical pseudopotential method. The alloying effects are modelled through the modified virtual crystal approximation. Throughout the composition, valence band maximum resides at the point. The conduction band minimum, however, shifts from to point of symmetry when = 0.27. The observed crossover from direct to indirect bandgap is well in accordance with the experimental observations. Effect of alloying on the density of states is also discussed. The charge density distribution along a few major planes is computed and discussed. The electronic band structure related parameters like bandwidths, bandgaps and ionicity are reported and compared with experimental data wherever available. We also give estimates of cohesive energy and bulk modulus for the alloys.
Energy Technology Data Exchange (ETDEWEB)
Gillet, Natacha; Berstis, Laura; Wu, Xiaojing; Gajdos, Fruzsina; Heck, Alexander; de la Lande, Aurelien; Blumberger, Jochen; Elstner, Marcus
2016-10-11
In this article, four methods to calculate charge transfer integrals in the context of bridge-mediated electron transfer are tested. These methods are based on density functional theory (DFT). We consider two perturbative Green's function effective Hamiltonian methods (first, at the DFT level of theory, using localized molecular orbitals; second, applying a tight-binding DFT approach, using fragment orbitals) and two constrained DFT implementations with either plane-wave or local basis sets. To assess the performance of the methods for through-bond (TB)-dominated or through-space (TS)-dominated transfer, different sets of molecules are considered. For through-bond electron transfer (ET), several molecules that were originally synthesized by Paddon-Row and co-workers for the deduction of electronic coupling values from photoemission and electron transmission spectroscopies, are analyzed. The tested methodologies prove to be successful in reproducing experimental data, the exponential distance decay constant and the superbridge effects arising from interference among ET pathways. For through-space ET, dedicated p-stacked systems with heterocyclopentadiene molecules were created and analyzed on the basis of electronic coupling dependence on donor-acceptor distance, structure of the bridge, and ET barrier height. The inexpensive fragment-orbital density functional tight binding (FODFTB) method gives similar results to constrained density functional theory (CDFT) and both reproduce the expected exponential decay of the coupling with donor-acceptor distances and the number of bridging units. These four approaches appear to give reliable results for both TB and TS ET and present a good alternative to expensive ab initio methodologies for large systems involving long-range charge transfers.
Gillet, Natacha; Berstis, Laura; Wu, Xiaojing; Gajdos, Fruzsina; Heck, Alexander; de la Lande, Aurélien; Blumberger, Jochen; Elstner, Marcus
2016-10-11
In this article, four methods to calculate charge transfer integrals in the context of bridge-mediated electron transfer are tested. These methods are based on density functional theory (DFT). We consider two perturbative Green's function effective Hamiltonian methods (first, at the DFT level of theory, using localized molecular orbitals; second, applying a tight-binding DFT approach, using fragment orbitals) and two constrained DFT implementations with either plane-wave or local basis sets. To assess the performance of the methods for through-bond (TB)-dominated or through-space (TS)-dominated transfer, different sets of molecules are considered. For through-bond electron transfer (ET), several molecules that were originally synthesized by Paddon-Row and co-workers for the deduction of electronic coupling values from photoemission and electron transmission spectroscopies, are analyzed. The tested methodologies prove to be successful in reproducing experimental data, the exponential distance decay constant and the superbridge effects arising from interference among ET pathways. For through-space ET, dedicated π-stacked systems with heterocyclopentadiene molecules were created and analyzed on the basis of electronic coupling dependence on donor-acceptor distance, structure of the bridge, and ET barrier height. The inexpensive fragment-orbital density functional tight binding (FODFTB) method gives similar results to constrained density functional theory (CDFT) and both reproduce the expected exponential decay of the coupling with donor-acceptor distances and the number of bridging units. These four approaches appear to give reliable results for both TB and TS ET and present a good alternative to expensive ab initio methodologies for large systems involving long-range charge transfers.
Lauben, D.; Cohen, M.; Inan, U.
2012-12-01
We deduce the 3d intra-plasmaspheric distribution of VLF wave power between conjugate regions of strong VLF wave amplitudes as measured by DEMETER for high-power terrestrial VLF transmitters during its ~6-yr lifetime. We employ a mixed WKB/full-wave technique to solve for the primary and secondary electromagnetic and electrostatic waves which are transmitted and reflected from strong cold-plasma density gradients and posited irregularities, in order to match the respective end-point measured amplitude distributions. Energy arriving in the conjugate region and also escaping to other regions of the magnetosphere is note. The resulting 3d distribution allows improved estimates for the long-term average particle scattering induced by terrestrial VLF transmitters.
Regnier, D.; Dubray, N.; Schunck, N.; Verrière, M.
2016-05-01
Background: Accurate knowledge of fission fragment yields is an essential ingredient of numerous applications ranging from the formation of elements in the r process to fuel cycle optimization for nuclear energy. The need for a predictive theory applicable where no data are available, together with the variety of potential applications, is an incentive to develop a fully microscopic approach to fission dynamics. Purpose: In this work, we calculate the pre-neutron emission charge and mass distributions of the fission fragments formed in the neutron-induced fission of 239Pu using a microscopic method based on nuclear density functional theory (DFT). Methods: Our theoretical framework is the nuclear energy density functional (EDF) method, where large-amplitude collective motion is treated adiabatically by using the time-dependent generator coordinate method (TDGCM) under the Gaussian overlap approximation (GOA). In practice, the TDGCM is implemented in two steps. First, a series of constrained EDF calculations map the configuration and potential-energy landscape of the fissioning system for a small set of collective variables (in this work, the axial quadrupole and octupole moments of the nucleus). Then, nuclear dynamics is modeled by propagating a collective wave packet on the potential-energy surface. Fission fragment distributions are extracted from the flux of the collective wave packet through the scission line. Results: We find that the main characteristics of the fission charge and mass distributions can be well reproduced by existing energy functionals even in two-dimensional collective spaces. Theory and experiment agree typically within two mass units for the position of the asymmetric peak. As expected, calculations are sensitive to the structure of the initial state and the prescription for the collective inertia. We emphasize that results are also sensitive to the continuity of the collective landscape near scission. Conclusions: Our analysis confirms
Density functional theory for the description of charge-transfer processes at TTF/TCNQ interfaces
Van Regemorter, Tanguy
2012-09-15
In the field of organic electronics, a central issue is to assess how the frontier electronic levels of two adjacent organic layers align with respect to one another at the interface. This alignment can be driven by the presence of a partial charge transfer and the formation of an interface dipole; it plays a key role for instance in determining the rates of exciton dissociation or exciton formation in organic solar cells or light-emitting diodes, respectively. Reliably modeling the processes taking place at these interfaces remains a challenge for the computational chemistry community. Here, we review our recent theoretical work on the influence of the choice of density functional theory (DFT) methodology on the description of the charge-transfer character in the ground state of TTF/ TCNQ model complexes and interfaces. Starting with the electronic properties of the isolated TTF and TCNQ molecules and then considering the charge transfer and resulting interface dipole in TTF/TCNQ donor-acceptor stacks and bilayers, we examine the impact of the choice of DFT functional in describing the interfacial electronic structure. Finally, we employ computations based on periodic boundary conditions to highlight the impact of depolarization effects on the interfacial dipole moment. © Springer-Verlag 2012.
Gavrilov, A. A.; Chertovich, A. V.; Kramarenko, E. Yu.
2016-11-01
In this work, we study the question of how to introduce electrostatic interactions in dissipative particle dynamics (DPD) method in order to correctly reproduce the properties of systems with high density of charges, including those with inhomogeneous charge distribution. To this end, we formulate general requirements for the electrostatic force in DPD and propose a new functional form of the force which suits better for satisfying these requirements than the previously used ones. In order to verify the proposed model, we study the problem of a single polyelectrolyte chain collapse and compare the results with molecular dynamics (MD) simulations in which the exact Coulomb force is used. We show that an excellent quantitative agreement between MD and DPD models is observed if the length parameter D of the proposed electrostatic force is chosen properly; the recommendations concerning the choice of this parameter value are given based on the analysis of a polyelectrolyte chain collapse behavior. Finally, we demonstrate the applicability of DPD with the proposed electrostatic force to studying microphase separation phenomenon in polyelectrolyte melts and show that the same values of D as in the case of single chain collapse should be used, thus indicating universality of the model. Due to the charge correlation attraction, a long-range order in such melts can be observed even at zero Flory-Huggins parameter.
Charged-particle rapidity density in Au+Au collisions in a quark combination model
Shao, Feng-Lan; Yao, Tao; Xie, Qu-Bing
2007-03-01
Rapidity/pseudorapidity densities for charged particles and their centrality, rapidity, and energy dependence in Au+Au collisions at the Relativistic Heavy Ion Collider are studied in a quark combination model. Using a Gaussian-type rapidity distribution for constituent quarks as a result of Landau hydrodynamic evolution, the data at sNN=130,200 GeV at various centralities in full pseudorapidity range are well described, and the charged-particle multiplicities are reproduced as functions of the number of participants. The energy dependence of the shape of the dNch/dη distribution is also described at various collision energies sNN=200,130,62.4 GeV in central collisions with same value of parameters except 19.6 GeV. The calculated rapidity distributions and yields for the charged pions and kaons in central Au+Au collisions at sNN=200 GeV are compared with experimental data of the BRAHMS Collaboration.
Liu, Yanju; Naidu, Ravendra; Ming, Hui
2013-03-15
The surface electrochemical properties of red mud (bauxite residue) from different alumina refineries in Australia and China were studied by electrophoresis and measuring surface charge density obtained from acid/base potentiometric titrations. The electrophoretic properties were measured from zeta potentials obtained in the presence of 0.01 and 0.001 M KNO(3) over a wide pH range (3.5-10) by titration. The isoelectric point (IEP) values were found to vary from 6.35 to 8.70 for the red mud samples. Further investigation into the surface charge density of one sample (RRM) by acid/base potentiometric titration showed similar results for pH(PZC) with pH(IEP) obtained from electrokinetic measurements. The pH(IEP) determined from zeta potential measurements can be used as a characteristic property of red mud. The minerals contained in red mud contributed to the different values of pH(IEP) of samples obtained from different refineries. Different relationships of pH(IEP) with Al/Fe and Al/Si ratios (molar basis) were also found for different red mud samples.
Directory of Open Access Journals (Sweden)
Petri Tanska
2013-01-01
Full Text Available The aim of this study was to investigate if the experimentally detected altered chondrocyte volumetric behavior in early osteoarthritis can be explained by changes in the extracellular and pericellular matrix properties of cartilage. Based on our own experimental tests and the literature, the structural and mechanical parameters for normal and osteoarthritic cartilage were implemented into a multiscale fibril-reinforced poroelastic swelling model. Model simulations were compared with experimentally observed cell volume changes in mechanically loaded cartilage, obtained from anterior cruciate ligament transected rabbit knees. We found that the cell volume increased by 7% in the osteoarthritic cartilage model following mechanical loading of the tissue. In contrast, the cell volume decreased by 4% in normal cartilage model. These findings were consistent with the experimental results. Increased local transversal tissue strain due to the reduced collagen fibril stiffness accompanied with the reduced fixed charge density of the pericellular matrix could increase the cell volume up to 12%. These findings suggest that the increase in the cell volume in mechanically loaded osteoarthritic cartilage is primarily explained by the reduction in the pericellular fixed charge density, while the superficial collagen fibril stiffness is suggested to contribute secondarily to the cell volume behavior.
Density waves in traffic flow of two kinds of vehicles.
Liu, Z Z; Zhou, X J; Liu, X M; Luo, J
2003-01-01
Through the car-following model, the traffic flow of two types of vehicles (cars and trucks) on a single-lane flow is studied, in which drivers on different vehicles have different sensitivities and the safety distance is assumed to be the same for all vehicles. The linear analysis is carried out to determine the condition of critical stability. With the nonlinear analysis, it proves that the small fluctuation of the vehicle density near the critical stable state satisfies the Korteweg-deVries equation and different sensitivities affect only the soliton evolution. When the headway in the critical state is more than the safety distance, the density around the soliton peak exceeds the density of the critical stable state, which can be explained as the formation of traffic jam. Contrarily, when the headway state is less than the safety distance, drivers will increase the headway to avoid the jam. The direct approach of the soliton perturbation shows that drivers' sensitivity will increase the soliton's amplitude continuously. Moreover, the increase of the number of trucks in the traffic flow will slow down the evolution of the amplitude.
Internal wave pressure, velocity, and energy flux from density perturbations
Allshouse, Michael R; Morrison, Philip J; Swinney, Harry L
2016-01-01
Determination of energy transport is crucial for understanding the energy budget and fluid circulation in density varying fluids such as the ocean and the atmosphere. However, it is rarely possible to determine the energy flux field $\\mathbf{J} = p \\mathbf{u}$, which requires simultaneous measurements of the pressure and velocity perturbation fields, $p$ and $\\mathbf{u}$. We present a method for obtaining the instantaneous $\\mathbf{J}(x,z,t)$ from density perturbations alone: a Green's function-based calculation yields $p$, and $\\mathbf{u}$ is obtained by integrating the continuity equation and the incompressibility condition. We validate our method with results from Navier-Stokes simulations: the Green's function method is applied to the density perturbation field from the simulations, and the result for $\\mathbf{J}$ is found to agree typically to within $1\\%$ with $\\mathbf{J}$ computed directly using $p$ and $ \\mathbf{u}$ from the Navier-Stokes simulation. We also apply the Green's function method to densit...
Spectral power density of the random excitation for the photoacoustic wave equation
Directory of Open Access Journals (Sweden)
Hakan Erkol
2014-09-01
Full Text Available The superposition of the Green's function and its time reversal can be extracted from the photoacoustic point sources applying the representation theorems of the convolution and correlation type. It is shown that photoacoustic pressure waves at locations of random point sources can be calculated with the solution of the photoacoustic wave equation and utilization of the continuity and the discontinuity conditions of the pressure waves in the frequency domain although the pressure waves cannot be measured at these locations directly. Therefore, with the calculated pressure waves at the positions of the sources, the spectral power density can be obtained for any system consisting of two random point sources. The methodology presented here can also be generalized to any finite number of point like sources. The physical application of this study includes the utilization of the cross-correlation of photoacoustic waves to extract functional information associated with the flow dynamics inside the tissue.
Correlation of densities with shear wave velocities and SPT N values
Anbazhagan, P.; Uday, Anjali; Moustafa, Sayed S. R.; Al-Arifi, Nassir S. N.
2016-06-01
Site effects primarily depend on the shear modulus of subsurface layers, and this is generally estimated from the measured shear wave velocity (V s) and assumed density. Very rarely, densities are measured for amplification estimation because drilling and sampling processes are time consuming and expensive. In this study, an attempt has been made to derive the correlation between the density (dry and wet density) and V s/SPT (standard penetration test) N values using measured data. A total of 354 measured V s and density data sets and 364 SPT N value and density data sets from 23 boreholes have been used in the study. Separate relations have been developed for all soil types as well as fine-grained and coarse-grained soil types. The correlations developed for bulk density were compared with the available data and it was found that the proposed relation matched well with the existing data. A graphical comparison and validation based on the consistency ratio and cumulative frequency curves was performed and the newly developed relations were found to demonstrate good prediction performance. An attempt has also been made to propose a relation between the bulk density and shear wave velocity applicable for a wide range of soil and rock by considering data from this study as well as that of previous studies. These correlations will be useful for predicting the density (bulk and dry) of sites having measured the shear wave velocity and SPT N values.
Directory of Open Access Journals (Sweden)
Raicharan Denra
2016-12-01
Full Text Available In this paper, characteristics of small amplitude nonlinear dust acoustic wave have been investigated in a unmagnetized, collisionless, Lorentzian dusty plasma where electrons and ions are inertialess and modeled by generalized Lorentzian Kappa distribution. Dust grains are inertial and equilibrium dust charge is negative. Both adiabatic and nonadiabatic fluctuation of charges on dust grains have been taken under consideration. For adiabatic dust charge variation reductive perturbation analysis gives rise to a KdV equation that governs the nonlinear propagation of dust acoustic waves having soliton solutions. For nonadiabatic dust charge variation nonlinear propagation of dust acoustic wave obeys KdV-Burger equation and gives rise to dust acoustic shock waves. Numerical estimation for adiabatic grain charge variation shows the existence of rarefied soliton whose amplitude and width varies with grain charges. Amplitude and width of the soliton have been plotted for different electron Kappa indices keeping ion velocity distribution Maxwellian. For non adiabatic dust charge variation, ratio of the coefficients of Burger term and dispersion term have been plotted against charge fluctuation for different kappa indices. All these results approach to the results of Maxwellian plasma if both electron and ion kappa tends to infinity.
Denra, Raicharan; Paul, Samit; Sarkar, Susmita
2016-12-01
In this paper, characteristics of small amplitude nonlinear dust acoustic wave have been investigated in a unmagnetized, collisionless, Lorentzian dusty plasma where electrons and ions are inertialess and modeled by generalized Lorentzian Kappa distribution. Dust grains are inertial and equilibrium dust charge is negative. Both adiabatic and nonadiabatic fluctuation of charges on dust grains have been taken under consideration. For adiabatic dust charge variation reductive perturbation analysis gives rise to a KdV equation that governs the nonlinear propagation of dust acoustic waves having soliton solutions. For nonadiabatic dust charge variation nonlinear propagation of dust acoustic wave obeys KdV-Burger equation and gives rise to dust acoustic shock waves. Numerical estimation for adiabatic grain charge variation shows the existence of rarefied soliton whose amplitude and width varies with grain charges. Amplitude and width of the soliton have been plotted for different electron Kappa indices keeping ion velocity distribution Maxwellian. For non adiabatic dust charge variation, ratio of the coefficients of Burger term and dispersion term have been plotted against charge fluctuation for different kappa indices. All these results approach to the results of Maxwellian plasma if both electron and ion kappa tends to infinity.
Kurniawan, Andi; Tsuchiya, Yuki; Eda, Shima; Morisaki, Hisao
2015-12-01
Biofilm polymers contain both electrically positively and negatively charged sites. These charged sites enable the biofilm to trap and retain ions leading to an important role of biofilm such as nutrient recycling and pollutant purification. Much work has focused on the ion-exchange capacity of biofilms, and they are known to adsorb ions through an exchange mechanism between the ions in solution and the ions adsorbed to the charged sites on the biofilm polymer. However, recent studies suggest that the adsorption/desorption behavior of ions in a biofilm cannot be explained solely by this ion exchange mechanism. To examine the possibility that a substantial amount of ions are held in the interstitial region of the biofilm polymer by an electrostatic interaction, intact biofilms formed in a natural environment were immersed in distilled water and ion desorption was investigated. All of the detected ion species were released from the biofilms over a short period of time, and very few ions were subsequently released over more time, indicating that the interstitial region of biofilm polymers is another ion reserve. The extent of ion retention in the interstitial region of biofilms for each ion can be determined largely by charge density, |Z|/r, where |Z| is the ion valence as absolute value and r is the ion radius. The higher |Z|/r value an ion has, the stronger it is retained in the interstitial region of biofilms. Ion shape is also a key determinant of ion retention. Spherical and non-spherical ions have different correlations between the condensation ratio and |Z|/r. The generality of these findings were assured by various biofilm samples. Thus, the internal regions of biofilms exchange ions dynamically with the outside environment.
Energy Technology Data Exchange (ETDEWEB)
Migunov, V., E-mail: v.migunov@fz-juelich.de; Dunin-Borkowski, R. E. [Ernst Ruska-Centre for Microscopy and Spectroscopy with Electrons (ER-C) and Peter Grünberg Institute (PGI), Forschungszentrum Jülich, D-52425 Jülich (Germany); London, A. [Department of Materials, University of Oxford, Parks Road, Oxford OX1 3PH (United Kingdom); Farle, M. [Fakultät für Physik and Center of Nanointegration (CeNIDE), Universität Duisburg-Essen, D-47048 Duisburg (Germany)
2015-04-07
The one-dimensional charge density distribution along an electrically biased Fe atom probe needle is measured using a model-independent approach based on off-axis electron holography in the transmission electron microscope. Both the mean inner potential and the magnetic contribution to the phase shift are subtracted by taking differences between electron-optical phase images recorded with different voltages applied to the needle. The measured one-dimensional charge density distribution along the needle is compared with a similar result obtained using model-based fitting of the phase shift surrounding the needle. On the assumption of cylindrical symmetry, it is then used to infer the three-dimensional electric field and electrostatic potential around the needle with ∼10 nm spatial resolution, without needing to consider either the influence of the perturbed reference wave or the extension of the projected potential outside the field of view of the electron hologram. The present study illustrates how a model-independent approach can be used to measure local variations in charge density in a material using electron holography in the presence of additional contributions to the phase, such as those arising from changes in mean inner potential and specimen thickness.
Dutta, Tirthankar; Ramasesha, S.
2012-01-01
In this paper we investigate the effect of terminal substituents on the dynamics of spin and charge transport in donor-acceptor substituted polyenes [D-(CH)x-A] chains, also known as push-pull polyenes. We employ a long-range correlated model Hamiltonian for the D-(CH)x-A system, and time-dependent density matrix renormalization group technique for time propagating the wave packet obtained by injecting a hole at a terminal site, in the ground state of the system. Our studies reveal that the end groups do not affect spin and charge velocities in any significant way, but change the amount of charge transported. We have compared these push-pull systems with donor-acceptor substituted polymethine imine (PMI), D-(CHN)x-A, systems in which besides electron affinities, the nature of pz orbitals in conjugation also alternate from site to site. We note that spin and charge dynamics in the PMIs are very different from that observed in the case of push-pull polyenes, and within the time scale of our studies, transport of spin and charge leads to the formation of a “quasi-static” state.
Millimeter-wave Line Ratios and Sub-beam Volume Density Distributions
Leroy, Adam K.; Usero, Antonio; Schruba, Andreas; Bigiel, Frank; Kruijssen, J. M. Diederik; Kepley, Amanda; Blanc, Guillermo A.; Bolatto, Alberto D.; Cormier, Diane; Gallagher, Molly; Hughes, Annie; Jiménez-Donaire, Maria J.; Rosolowsky, Erik; Schinnerer, Eva
2017-02-01
We explore the use of mm-wave emission line ratios to trace molecular gas density when observations integrate over a wide range of volume densities within a single telescope beam. For observations targeting external galaxies, this case is unavoidable. Using a framework similar to that of Krumholz & Thompson, we model emission for a set of common extragalactic lines from lognormal and power law density distributions. We consider the median density of gas that produces emission and the ability to predict density variations from observed line ratios. We emphasize line ratio variations because these do not require us to know the absolute abundance of our tracers. Patterns of line ratio variations have the potential to illuminate the high-end shape of the density distribution, and to capture changes in the dense gas fraction and median volume density. Our results with and without a high-density power law tail differ appreciably; we highlight better knowledge of the probability density function (PDF) shape as an important area. We also show the implications of sub-beam density distributions for isotopologue studies targeting dense gas tracers. Differential excitation often implies a significant correction to the naive case. We provide tabulated versions of many of our results, which can be used to interpret changes in mm-wave line ratios in terms of adjustments to the underlying density distributions.
Quantum Larmor radiation from a moving charge in an electromagnetic plane wave background
Nakamura, Gen; 10.1142/S0217751X12501424
2012-01-01
We extend our previous work [Phys. Rev. D83 045030 (2011)], which investigated the first-order quantum effect in the Larmor radiation from a moving charge in a spatially homogeneous time-dependent electric field. Specifically, we investigate the quantum Larmor radiation from a moving charge in a monochromatic electromagnetic plane wave background based on the scalar quantum electrodynamics at the lowest order of the perturbation theory. Using the in-in formalism, we derive the theoretical formula of the total radiation energy from a charged particle in the initial states being at rest and being in a relativistic motion. Expanding the theoretical formula in terms of the Planck constant \\hbar, we obtain the first-order quantum effect on the Larmor radiation. The quantum effect generally suppresses the total radiation energy compared with the prediction of the classical Larmor formula, which is a contrast to the previous work. The reason is explained by the fact that the radiation from a moving charge in a monoc...
Kim, SeongMin; Ha, Jaewook; Kim, Jin-Baek
2016-11-01
We analytically calculated polarization and bound charge density inside the dielectric material in metal-to-dielectric-mode triboelectric nanogenerators (TENG) where the transferred charges are collected on the bottom metal via electrostatic induction from the triboelectric charges that are generated by frictional contact. This bound charge density is associated with the surface density of states (DOS), overline{Ns(E)}. Two cases are considered here: i) for overline{Ns(E)} ≫ 1, it is calculated that the bound charge density is proportional to the dielectric constant and the work function difference between the two materials, but inversely proportional to the thickness of the dielectric material (ɛ0(ɛ2-1) (E0-W)/e \\cdot d2); ii) for overline{Ns(E)} ≪ 1 with constant overline{Ns(E)}, the bound charge density is mostly proportional to the work function difference between the materials, and inversely proportional to the thickness of the dielectric material ((ɛ2-1)x/d_{2+\\varepsilon2\\cdot x} \\cdot Ns(E)\\cdot e\\cdot (E0-W)).
Density-Wave Spiral Theories in the 1960s. II
Pasha, I I
2004-01-01
By the 1970s the spiral subject was in considerable disarray. The semiempirical theory by Lin and Shu was confronted with serious problems. They were put on the defensive over their tightly wrapped steady modes on two principal fronts: from the radial propagation at the group velocity that would tend to wind them almost at the material rate, and from the tendencies of galaxy disks toward a strong global instability that appeared likely to overwhelm them. Of course, one might claim that such threats were imaginary and only of academic interest, on the ground that nature itself had overcome them. One might also be confident that the QSSS hypothesis must be correct as illuminated by the everlasting truth of Hubble's classification. One might even take pride in the fact that a very promising concept developed, although not connected to the wave steadiness, on spiral shocks in interstellar gas and their induced star formation. But such a heuristic approach did not stimulate very strong progress in understanding dy...
Wave theories of non-laminar charged particle beams: from quantum to thermal regime
Fedele, Renato; Jovanovic, Dusan; De Nicola, Sergio; Ronsivalle, Concetta
2013-01-01
The standard classical description of non-laminar charge particle beams in paraxial approximation is extended to the context of two wave theories. The first theory is the so-called Thermal Wave Model (TWM) that interprets the paraxial thermal spreading of the beam particles as the analog of the quantum diffraction. The other theory, hereafter called Quantum Wave Model (QWM), that takes into account the individual quantum nature of the single beam particle (uncertainty principle and spin) and provides the collective description of the beam transport in the presence of the quantum paraxial diffraction. QWM can be applied to beams that are sufficiently cold to allow the particles to manifest their individual quantum nature but sufficiently warm to make overlapping-less the single-particle wave functions. In both theories, the propagation of the beam transport in plasmas or in vacuo is provided by fully similar set of nonlinear and nonlocal governing equations, where in the case of TWM the Compton wavelength (fun...
Carnal, Fabrice; Stoll, Serge
2011-10-27
Complex formation between a weak flexible polyelectrolyte chain and one positively charged nanoparticle in presence of explicit counterions and salt particles is investigated using Monte Carlo simulations. The influence of parameters such as the nanoparticle surface charge density, salt valency, and solution property such as the pH on the chain protonation/deprotonation process and monomer adsorption at the nanoparticle surface are systematically investigated. It is shown that the nanoparticle presence significantly modifies chain acid/base and polyelectrolyte conformational properties. The importance of the attractive electrostatic interactions between the chain and the nanoparticle clearly promotes the chain deprotonation leading, at high pH and nanoparticle charge density, to fully wrapped polyelectrolyte at the nanoparticle surface. When the nanoparticle bare charge is overcompensated by the polyelectrolyte charges, counterions and salt particles condense at the surface of the polyelectrolyte-nanoparticle complex to compensate for the excess of charges providing from the adsorbed polyelectrolyte chain. It is also shown that the complex formation is significantly affected by the salt valency. Indeed, with the presence of trivalent salt cations, competition is observed between the nanoparticle and the trivalent cations. As a result, the amount of adsorbed monomers is less important than in the monovalent and divalent case and chain conformations are different due to the collapse of polyelectrolyte segments around trivalent cations out of the nanoparticle adsorption layer.
Directory of Open Access Journals (Sweden)
Kaihan Fakhar
Full Text Available OBJECTIVE: We aimed in this investigation to study deep brain stimulation (DBS battery drain with special attention directed toward patient symptoms prior to and following battery replacement. BACKGROUND: Previously our group developed web-based calculators and smart phone applications to estimate DBS battery life (http://mdc.mbi.ufl.edu/surgery/dbs-battery-estimator. METHODS: A cohort of 320 patients undergoing DBS battery replacement from 2002-2012 were included in an IRB approved study. Statistical analysis was performed using SPSS 20.0 (IBM, Armonk, NY. RESULTS: The mean charge density for treatment of Parkinson's disease was 7.2 µC/cm(2/phase (SD = 3.82, for dystonia was 17.5 µC/cm(2/phase (SD = 8.53, for essential tremor was 8.3 µC/cm(2/phase (SD = 4.85, and for OCD was 18.0 µC/cm(2/phase (SD = 4.35. There was a significant relationship between charge density and battery life (r = -.59, p<.001, as well as total power and battery life (r = -.64, p<.001. The UF estimator (r = .67, p<.001 and the Medtronic helpline (r = .74, p<.001 predictions of battery life were significantly positively associated with actual battery life. Battery status indicators on Soletra and Kinetra were poor predictors of battery life. In 38 cases, the symptoms improved following a battery change, suggesting that the neurostimulator was likely responsible for symptom worsening. For these cases, both the UF estimator and the Medtronic helpline were significantly correlated with battery life (r = .65 and r = .70, respectively, both p<.001. CONCLUSIONS: Battery estimations, charge density, total power and clinical symptoms were important factors. The observation of clinical worsening that was rescued following neurostimulator replacement reinforces the notion that changes in clinical symptoms can be associated with battery drain.
On the Control of the Fixed Charge Densities in Al2O3-Based Silicon Surface Passivation Schemes.
Simon, Daniel K; Jordan, Paul M; Mikolajick, Thomas; Dirnstorfer, Ingo
2015-12-30
A controlled field-effect passivation by a well-defined density of fixed charges is crucial for modern solar cell surface passivation schemes. Al2O3 nanolayers grown by atomic layer deposition contain negative fixed charges. Electrical measurements on slant-etched layers reveal that these charges are located within a 1 nm distance to the interface with the Si substrate. When inserting additional interface layers, the fixed charge density can be continuously adjusted from 3.5 × 10(12) cm(-2) (negative polarity) to 0.0 and up to 4.0 × 10(12) cm(-2) (positive polarity). A HfO2 interface layer of one or more monolayers reduces the negative fixed charges in Al2O3 to zero. The role of HfO2 is described as an inert spacer controlling the distance between Al2O3 and the Si substrate. It is suggested that this spacer alters the nonstoichiometric initial Al2O3 growth regime, which is responsible for the charge formation. On the basis of this charge-free HfO2/Al2O3 stack, negative or positive fixed charges can be formed by introducing additional thin Al2O3 or SiO2 layers between the Si substrate and this HfO2/Al2O3 capping layer. All stacks provide very good passivation of the silicon surface. The measured effective carrier lifetimes are between 1 and 30 ms. This charge control in Al2O3 nanolayers allows the construction of zero-fixed-charge passivation layers as well as layers with tailored fixed charge densities for future solar cell concepts and other field-effect based devices.
Estimation of Plasma Density by Surface Plasmons for Surface-Wave Plasmas
Institute of Scientific and Technical Information of China (English)
CHEN Zhao-Quan; LIU Ming-Hai; LAN Chao-Hui; CHEN Wei; LUO Zhi-Qing; HU Xi-Wei
2008-01-01
@@ An estimation method of plasma density based on surface plasmons theory for surface-wave plasmas is proposed. The number of standing-wave is obtained directly from the discharge image, and the propagation constant is calculated with the trim size of the apparatus in this method, then plasma density can be determined with the value of 9.1 × 1017 m-3. Plasma density is measured using a Langmuir probe, the value is 8.1 × 1017 m-3 which is very close to the predicted value of surface plasmons theory. Numerical simulation is used to check the number of standing-wave by the finite-difference time-domain (FDTD) method also. All results are compatible both of theoretical analysis and experimental measurement.
Energy flow, energy density of Timoshenko beam and wave mode incoherence
Zhou, Jun; Rao, Zhushi; Ta, Na
2015-10-01
Time-averaged energy flow and energy density are of significance in vibration analysis. The wave decomposition method is more fruitful and global in physical sense than the state variables depicted point by point. By wave approach, the Timoshenko beam vibration field is decomposed into two distinct modes: travelling and evanescent waves. Consequently, the power and energy functions defined on these waves' amplitude and phase need to be established. However, such formulas on Timoshenko beam are hardly found in literatures. Furthermore, the incoherence between these two modes is of theoretical and practical significance. This characteristic guarantees that the resultant power or energy of a superposed wave field is equal to the sum of the power or energy that each wave mode would generate individually. Unlike Euler-Bernoulli beam, such incoherence in the Timoshenko beam case has not been theoretically proved so far. Initially, the power and energy formulas based on wave approach and the corresponding incoherence proof are achieved by present work, both in theoretical and numerical ways. Fortunately, the theoretical and numerical results show that the travelling and evanescent wave modes are incoherent with each other both on power and energy functions. Notably, the energy function is unconventional and self-defined in order to obtain the incoherence. Some remarkable power transmission characteristics of the evanescent wave are also illustrated meanwhile.
A procedure to analyze nonlinear density waves in Saturn's rings using several occultation profiles
Rappaport, N J; French, R G; Marouf, E A; McGhee, C A
2010-01-01
Cassini radio science experiments have provided multiple occultation optical depth profiles of Saturn's rings that can be used in combination to analyze density waves. This paper establishes an accurate procedure of inversion of the wave profiles to reconstruct the wave kinematic parameters as a function of semi-major axis, in the nonlinear regime. This procedure is achieved from simulated data in the presence of realistic noise perturbations, to control the reconstruction error. By way of illustration we have applied our procedure to the Mimas 5:3 density wave. We were able to recover precisely the kinematic parameters from the radio experiment occultation data in most of the propagation region; a preliminary analysis of the pressure-corrected dispersion allowed us to determine new but still uncertain values for the opacity ($K\\simeq 0.02$ cm$^2$/g) and velocity dispersion of ($c_o\\simeq 0.6$ cm/s) in the wave region. Our procedure constitutes the first step in our planned analysis of the density waves of Sa...
A Study of Saturn's Normal Mode Oscillations and Their Forcing of Density Waves in the Rings
Friedson, Andrew James; Cao, Lyra
2016-10-01
Analysis of Cassini Visual and Infrared Mapping Spectrometer (VIMS) ring occultation profiles has revealed the presence of spiral density waves in Saturn's C ring that are consistent with being driven by gravitational perturbations associated with normal-mode oscillations of the planet [1]. These waves allow the C ring to serve as a sort of seismometer, since their pattern speeds (i.e., azimuthal phase speeds) can in principle be mapped onto the frequencies of the predominant normal oscillations of the planet. The resonant mode frequencies in turn are sensitive to Saturn's internal structure and rotational state. Characterization of the normal modes responsible for the forcing holds the potential to supply important new constraints on Saturn's internal structure and rotation. We perform numerical calculations to determine the resonant frequencies of the normal modes of a uniformly rotating planet for various assumptions regarding its internal stratification and compare the implied pattern speeds to those of density waves observed in the C ring. A question of particular interest that we address is whether quasi-toroidal modes are responsible for exciting a mysterious class of slowly propagating density waves in the ring. We also explore the implications of avoided crossings between modes for explaining observed fine splitting in the pattern speeds of spiral density waves having the same number of spiral arms, and weigh the role that convective overstability may play in exciting large-scale quasi-toroidal modes in Saturn. [1] Hedman, M.M. and Nicholson, P.D. 2014. MNRAS 444, 1369.
Constraining the gravitational wave energy density of the Universe using Earth's ring
Coughlin, Michael
2014-01-01
The search for gravitational waves is one of today's major scientific endeavors. A gravitational wave can interact with matter by exciting vibrations of elastic bodies. Earth itself is a large elastic body whose so-called normal-mode oscillations ring up when a gravitational wave passes. Therefore, precise measurement of vibration amplitudes can be used to search for the elusive gravitational-wave signals. Earth's free oscillations that can be observed after high-magnitude earthquakes have been studied extensively with gravimeters and low-frequency seismometers over many decades leading to invaluable insight into Earth's structure. Making use of our detailed understanding of Earth's normal modes, numerical models are employed for the first time to accurately calculate Earth's gravitational-wave response, and thereby turn a network of sensors that so far has served to improve our understanding of Earth, into an astrophysical observatory exploring our Universe. In this article, we constrain the energy density o...
First measurements of charge carrier density and mobility of in-situ enriched 28Si
Ramanayaka, A. N.; Dwyer, K. J.; Kim, Hyun-Soo; Stewart, M. D., Jr.; Pomeroy, J. M.
Magnetotransport in top gated Hall bar devices is investigated to characterize the electrical properties of in-situ enriched 28Si. Isotopically enriched 28Si is an ideal candidate for quantum information processing devices as the elimination of unpaired nuclear spins improves the fidelity of the quantum information. Using mass filtered ion beam deposition we, in-situ, enrich and deposit epitaxial 28Si, achieving several orders of magnitude better enrichment compared to other techniques. In order to explore the electrical properties and optimize the growth conditions of in-situ enriched 28Si we perform magnetotransport measurements on top gated Hall bar devices at temperatures ranging from 300 K to cryogenic temperatures and at moderate magnetic fields. Here, we report on the charge carrier density and mobility extracted from such experiments, and will be compared among different growth conditions of in-situ enriched 28Si.
$\\eta^\\prime$ meson mass from topological charge density correlator in QCD
Fukaya, H; Cossu, G; Hashimoto, S; Kaneko, T; Noaki, J
2015-01-01
The flavor-singlet component of the eta prime meson is related to the topological structure of the SU(3) gauge field through the chiral anomaly. We perform a 2+1-flavor lattice QCD calculation and demonstrate that the two-point function of a gluonically defined topological charge density after a short Yang-Mills gradient flow contains the propagation of the eta prime meson, by showing that its mass in the chiral and continuum limit is consistent with the experimental value. The gluonic correlator does not suffer from the contamination of the pion contribution, and the clean signal is obtained at significantly lower numerical cost compared to the conventional method with the quark bilinear operators.
Spin-charge and spin-orbital separations in density-functional theory
Vieira, Daniel
2012-01-01
It is known that the separation of electrons into spinons and chargons, the spin-charge separation, plays a decisive role when describing strongly correlated one-dimensional (1D) Friedel oscillations. Here, we extend the investigation by considering a third electron fractionalization: the separation into spinons and orbitons. Specifically, we deal with two exact constraints of exchange-correlation (XC) density-functionals: (i) The constancy of the highest occupied Kohn-Sham eigenvalues upon fractional electron numbers, and (ii) their discontinuities at integers. By means of 1D Hubbard chains, we show that spin-orbital separation can be decisive when dealing with derivative discontinuities of XC potentials, especially at strong correlations.
Brophy, Thomas G.; Rosen, Paul A.
1992-01-01
A parallel examination is conducted of Voyager radio and photopolarimeter occultation observations of the Saturn A ring's density waves. The radio instrument waves exhibit an average -90 deg offset from the dynamical phase. A warping height of about 100-m amplitude can qualtitatively reproduce this phase shift, while preserving the overall model wave shape. These results may be profoundly relevant for satellite-ring torque calculations in Saturn's rings, given the deposition of all of the net torque of the standard model in the first wavelength.
Atamaniuk, B; Atamaniuk, Barbara; Zuchowski, Krzysztof
2007-01-01
There is a quickly increasing wealth of experimental data on so-called dusty plasmas i. e. ionized gases or usual plasmas that contain micron sized charged particles. Interest in these structures is driven both by their importance in many astrophysical as well as commercial situations. Among them are linear and nonlinear wave phenomena. We consider the influence of dust charge fluctuations on stability of the ion-acoustic waves when the stream of particles is present. It is assumed that all grains of dust have equal masses but charges are not constant in time-they may fluctuate in time. The dust charges are not really independent of the variations of the plasma potentials. All modes will influence the charging mechanism, and feedback will lead to several new interesting and unexpected phenomena. The charging of the grains depends on local plasma characteristics. If the waves disturb these characteristic, then charging of the grains is affected and the grain charge is modified, with a resulting feedback on the...
Grigoriev, P. D.; Kostenko, S. S.
2015-03-01
Superconductivity or metallic state may coexist with density wave ordering at imperfect nesting of the Fermi surface. In addition to the macroscopic spatial phase separation, there are, at least, two possible microscopic structures of such coexistence: (i) the soliton-wall phase and (ii) the ungapped Fermi-surface pockets. We show that the conductivity anisotropy allows us to distinguish these two microscopic density-wave structures. The results obtained may help to analyze the experimental observations in layered organic metals (TMTSF)2PF6, (TMTSF)2ClO4, α-(BEDT-TTF)2KHg(SCN)4 and in other compounds.
Energy Technology Data Exchange (ETDEWEB)
Grigoriev, P.D., E-mail: grigorev@itp.ac.ru [L.D. Landau Institute for Theoretical Physics, Chernogolovka 142432 (Russian Federation); Institut Laue-Langevin, Grenoble (France); Kostenko, S.S. [Institute of Problems of Chemical Physics, 142432 Chernogolovka (Russian Federation)
2015-03-01
Superconductivity or metallic state may coexist with density wave ordering at imperfect nesting of the Fermi surface. In addition to the macroscopic spatial phase separation, there are, at least, two possible microscopic structures of such coexistence: (i) the soliton-wall phase and (ii) the ungapped Fermi-surface pockets. We show that the conductivity anisotropy allows us to distinguish these two microscopic density-wave structures. The results obtained may help to analyze the experimental observations in layered organic metals (TMTSF){sub 2}PF{sub 6}, (TMTSF){sub 2}ClO{sub 4}, α-(BEDT-TTF){sub 2}KHg(SCN){sub 4} and in other compounds.
Central depressions in the charge density profiles of the nuclei around $^{46}$Ar
Song, Jun Ling; Long, Wen Hui
2015-01-01
The occurrence of the proton bubble-like structure has been studied within the relativistic Hartree-Fock-Bogoliubov (RHFB) and relativistic Hartree-Bogoliubov (RHB) theories by exploring the bulk properties, the charge density profiles and single proton spectra of argon isotopes and $N = 28$ isotones. It is found that the RHFB calculations with PKA1 effective interaction, which can properly reproduce the charge radii of argon isotopes and the $Z=16$ proton shell nearby, do not support the occurrence of the proton bubble-like structure in argon isotopes due to the prediction of deeper bound proton orbit $\\pi2s_{1/2}$ than $\\pi1d_{3/2}$. For $N = 28$ isotones, $^{42}$Si and $^{40}$Mg are predicted by both RHFB and RHB models to have the proton bubble-like structure, owing to the large gap between the proton $\\pi2s_{1/2}$ and $\\pi1d_{5/2}$ orbits, namely the $Z=14$ proton shell. Therefore, $^{42}$Si is proposed as the potential candidate of proton bubble nucleus, which has longer life-time than $^{40}$Mg.
High-resolution synchrotron data collection for charge-density work at 100 and 20 K.
Luger, Peter; Messerschmidt, Marc; Scheins, Stephan; Wagner, Armin
2004-09-01
For the measurement of very accurate high-resolution X-ray data for charge-density work, synchrotron beamlines provide a bright radiation source of outstanding properties. Most important are the very high primary intensity and the possibility of choosing hard radiation with lambda approximately 0.5 A or even shorter. This together with area detection and a stable low-temperature device means that accurate and large data sets can be measured in a short time. A number of data collections are reported, which were carried out at the beamlines F1 and D3 of Hasylab (DESY, Hamburg) first at 100 K and later at 15-20 K, demonstrating the quality of the measured intensities. A low temperature of around 20 K was obtained at beamline D3 with a double-stage closed-cycle helium cryostat where the standard beryllium cylinder of the vacuum chamber was replaced by a 0.1 mm Kapton film. Comparison of different data sets measured for a strychnine crystal demonstrated how I/sigma ratios favorably improve if synchrotron radiation at a low temperature of 15 K was used. Synchrotron-based studies on several biologically active compounds are briefly summarized and a synchrotron experiment of an otherwise not sufficiently diffracting crystal of a tetraphenyl barbaralane derivative is described in detail. Atomic volumes and charges of a highly substituted C(60) fullerene are reported derived from a synchrotron data set of more than 350000 reflections.
Bai, Yang; Liu, Shouping; Jiang, Ping; Zhou, Lei; Li, Jing; Tang, Charles; Verma, Chandra; Mu, Yuguang; Beuerman, Roger W; Pervushin, Konstantin
2009-08-01
Defensins are small (3-5 kDa) cysteine-rich cationic proteins found in both vertebrates and invertebrates constituting the front line of host innate immunity. Despite intensive research, bactericidal and cytotoxic mechanisms of defensins are still largely unknown. Moreover, we recently demonstrated that small peptides derived from defensins are even more potent bactericidal agents with less toxicity toward host cells. In this paper, structures of three C-terminal (R36-K45) analogues of human beta-defensin-3 were studied by 1H NMR spectroscopy and extensive molecular dynamics simulations. Because of indications that these peptides might target the inner bacterial membrane, they were reconstituted in dodecylphosphocholine or dodecylphosphocholine/1-palmitoyl-2-oleoyl-sn-glycero-3-[phospho-rac-(1-glycerol)] mixed micelles, and lipid bicelles mimicking the phospholipid-constituted bilayer membrane of mammalian and bacterial cells. The results show that the binding affinity and partitioning into the lipid phase and the ability to dimerize and accrete well-defined structures upon interactions with lipid membranes contribute to compactization of positive charges within peptide oligomers. The peptide charge density, mediated by corresponding three-dimensional structures, was found to directly correlate with the antimicrobial activity. These novel observations may provide a new rationale for the design of improved antimicrobial agents.
Rauhalahti, Markus; Taubert, Stefan; Sundholm, Dage; Liégeois, Vincent
2017-03-08
Magnetically induced current density susceptibilities and ring-current strengths have been calculated for neutral and doubly charged persubstituted benzenes C6X6 and C6X6(2+) with X = F, Cl, Br, I, At, SeH, SeMe, TeH, TeMe, and SbH2. The current densities have been calculated using the gauge-including magnetically induced current (GIMIC) method, which has been interfaced to the Gaussian electronic structure code rendering current density calculations using effective core potentials (ECP) feasible. Relativistic effects on the ring-current strengths have been assessed by employing ECP calculations of the current densities. Comparison of the ring-current strengths obtained in calculations on C6At6 and C6At6(2+) using relativistic and non-relativistic ECPs show that scalar relativistic effects have only a small influence on the ring-current strengths. Comparisons of the ring-current strengths and ring-current profiles show that the C6I6(2+), C6At6(2+), C6(SeH)6(2+), C6(SeMe)6(2+), C6(TeH)6(2+), C6(TeMe)6(2+), and C6(SbH2)6(2+) dications are doubly aromatic sustaining spatially separated ring currents in the carbon ring and in the exterior of the molecule. The C6I6(+) radical cation is also found to be doubly aromatic with a weaker ring current than obtained for the dication.
Monodisperse TiO2 Spheres with High Charge Density and Their Self-Assembly.
Xia, Hongbo; Wu, Suli; Su, Xin; Zhang, Shufen
2017-01-03
Titanium dioxide (TiO2 ) spheres are potential candidates to fabricate three-dimensional (3D) photonic crystals owing to their high refractive index and low absorption in the visible and near-infrared regions. Here, TiO2 spheres with both high surface charge density and uniform size, which are necessary for the self-assembly of TiO2 spheres, have been prepared by means of sol-gel methods in ethanol in the presence of thioglycolic acid as ligand. Thioglycolic acid, which contains two functional groups, not only acts as coordinating ligand for stabilizing and controlling the growth of TiO2 spheres but also endows the resulting TiO2 spheres with high charge density as based on ζ-potential analysis when the pH of the TiO2 aqueous dispersion was 6.5 or higher. The SEM images illustrate that the diameter of the prepared TiO2 spheres can be tuned from 100 to 300 nm by simply controlling the concentration of H2 O. FTIR spectra confirm that thioglycolic acid bonded to the surface of TiO2 spheres through carboxylic groups. As anticipated, the obtained TiO2 spheres could self-assemble to form a 3D opal photonic crystal structure by means of a simple gravity sedimentation method. Then the TiO2 spheres in the 3D opal photonic crystal structure were able to transform into a pure anatase phase by annealing at different temperatures.
Time-dependent quantum wave packet dynamics to study charge transfer in heavy particle collisions
Zhang, Song Bin; Wu, Yong; Wang, Jian Guo
2016-12-01
The method of time-dependent quantum wave packet dynamics has been successfully extended to study the charge transfer/exchange process in low energy two-body heavy particle collisions. The collision process is described by coupled-channel equations with diabatic potentials and (radial and rotational) couplings. The time-dependent coupled equations are propagated with the multiconfiguration time-dependent Hartree method and the modulo squares of S-matrix is extracted from the wave packet by the flux operator with complex absorbing potential (FCAP) method. The calculations of the charge transfer process 12Σ+ H-(1s2) +Li(1 s22 s ) →22Σ+ /32 Σ+ /12 Π H(1 s ) +Li-(1s 22 s 2 l ) (l =s ,p ) at the incident energy of about [0.3, 1.3] eV are illustrated as an example. It shows that the calculated reaction probabilities by the present FCAP reproduce that of quantum-mechanical molecular-orbital close-coupling very well, including the peak structures contributed by the resonances. Since time-dependent external interactions can be directly included in the present FCAP calculations, the successful implementation of FCAP provides us a powerful potential tool to study the quantum control of heavy particle collisions by lasers in the near future.
GRB Afterglow Blast Wave Encountering Sudden Circumburst Density Change Produces No Flares
Gat, Ilana; MacFadyen, Andrew
2013-01-01
Afterglows of gamma-ray bursts are observed to produce light curves with the flux following power law evolution in time. However, recent observations reveal bright flares at times on the order of minutes to days. One proposed explanation for these flares is the interaction of a relativistic blast wave with a circumburst density transition. In this paper, we model this type of interaction computationally in one and two dimensions, using a relativistic hydrodynamics code with adaptive mesh refinement called ram, and analytically in one dimension. We simulate a blast wave traveling in a stellar wind environment that encounters a sudden change in density, followed by a homogeneous medium, and compute the observed radiation using a synchrotron model. We show that flares are not observable for an encounter with a sudden density increase, such as a wind termination shock, nor for an encounter with a sudden density decrease. Furthermore, by extending our analysis to two dimensions, we are able to resolve the spreadin...
No flares from GRB afterglow blast waves encountering sudden circumburst density change
Gat, Ilana; MacFadyen, Andrew
2013-01-01
Afterglows of gamma-ray bursts are observed to produce light curves with the flux following power law evolution in time. However, recent observations reveal bright flares at times on the order of minutes to days. One proposed explanation for these flares is the interaction of a relativistic blast wave with a circumburst density transition. In this paper, we model this type of interaction computationally in one and two dimensions, using a relativistic hydrodynamics code with adaptive mesh refinement called RAM, and analytically in one dimension. We simulate a blast wave traveling in a stellar wind environment that encounters a sudden change in density, followed by a homogeneous medium, and compute the observed radiation using a synchrotron model. We show that flares are not observable for an encounter with a sudden density increase, such as a wind termination shock, nor for an encounter with a sudden density decrease. Furthermore, by extending our analysis to two dimensions, we are able to resolve the spreadin...
Nonlinear waves in electron–positron–ion plasmas including charge separation
Indian Academy of Sciences (India)
A MUGEMANA; S MOOLLA; I J LAZARUS
2017-02-01
Nonlinear low-frequency electrostatic waves in a magnetized, three-component plasma consisting of hot electrons, hot positrons and warm ions have been investigated. The electrons and positrons are assumed to have Boltzmann density distributions while the motion of the ions are governed by fluid equations. The system is closed with the Poisson equation. This set of equations is numerically solved for the electric field. The effects of the driving electric field, ion temperature, positron density, ion drift, Mach number and propagation angle are investigated. It is shown that depending on the driving electric field, ion temperature, positron density, ion drift, Mach number and propagation angle, the numerical solutions exhibit waveforms that are sinusoidal, sawtooth andspiky. The introduction of the Poisson equation increased the Mach number required to generate the waveforms but the driving electric field E0 was reduced. The results are compared with satellite observations.
Energy Technology Data Exchange (ETDEWEB)
Es’kin, V. A.; Zaboronkova, T. M.; Kudrin, A. V., E-mail: kud@rf.unn.ru; Ostafiychuk, O. M. [Lobachevskii State University of Nizhni Novgorod (Russian Federation)
2015-03-15
Guidance of azimuthally symmetric waves by cylindrical density ducts in magnetoplasma in the nonresonant region of the whistler frequency range is investigated. It is demonstrated that eigenmodes existing at the studied frequencies in ducts with enhanced plasma density allow simplified description that makes analysis of the features of their guided propagation much easier. The results of calculation of the dispersion characteristics and field structure of the whistler modes supported by such ducts are presented.
Magnetohydrodynamic Density Waves in a Galactic Disk System of Stars and Gas
Institute of Scientific and Technical Information of China (English)
YuqingLOU; ZuhuiFAN
1997-01-01
We study galactic magnetohydrodynamic(MHD) density waves in a composite system consisting of a stellar disk and a magnetized thermal gaseous disk.Perturbations in the two disks are conpled through gravitational interaction.In the tight-winding regime,Dispersion relations for MHD density wvaes are derived under two different approximations for the stellar disk.This investigation clarifies the interrelation between spiral structures in the stellar disk and spiral synchrotron radio structures in the magnetized thermal gaseous disk.
Murthy, Ganpathy
2000-01-01
It is well known that the ν = 2/5 state is unpolarized at zero Zeeman energy, while it is fully polarized at large Zeeman energies. A novel state with a charge/spin density wave order for composite fermions is proposed to exist at intermediate values of the Zeeman coupling for ν = 2/5. This state has half the maximum possible polarization, and can be extended to other incompressible fractions. A Hartree-Fock calculation based on the new approach for all fractional quantum Hall states developed by R. Shankar and the author is used to demonstrate the stability of this state to single-particle excitations and to compute gaps. A very recent experiment shows direct evidence for this state.
Murthy
2000-01-10
It is well known that the nu = 2/5 state is unpolarized at zero Zeeman energy, while it is fully polarized at large Zeeman energies. A novel state with a charge/spin density wave order for composite fermions is proposed to exist at intermediate values of the Zeeman coupling for nu = 2/5. This state has half the maximum possible polarization, and can be extended to other incompressible fractions. A Hartree-Fock calculation based on the new approach for all fractional quantum Hall states developed by R. Shankar and the author is used to demonstrate the stability of this state to single-particle excitations and to compute gaps. A very recent experiment shows direct evidence for this state.
Charge-Density-Excitation Spectrum in the t-t'-J-V Model
Greco, Andrés; Yamase, Hiroyuki; Bejas, Matías
2017-03-01
We study the density-density correlation function in a large-N scheme of the t-t'-J-V model. When the nearest-neighbor Coulomb interaction V is zero, our model exhibits phase separation in a wide doping region and we obtain large spectral weight near momentum q = (0,0) at low energy, which originates from the proximity to phase separation. These features are much stronger for electron doping than for hole doping. However, once phase separation is suppressed by including a finite V, the low-energy spectral weight around q = (0,0) is substantially suppressed. Instead a sharp zero-sound mode is stabilized above the particle-hole continuum. We discuss that the presence of a moderate value of V, which is frequently neglected in the t-J model, is important to understand low-energy charge excitations especially close to q = (0,0) for electron doping. This insight should be taken into account in a future study of x-ray scattering measurements.
Large amplitude solitary waves in ion-beam plasmas with charged dust impurities
Misra, A P
2011-01-01
The nonlinear propagation of large amplitude dust ion-acoustic (DIA) solitary waves (SWs) in an ion-beam plasma with stationary charged dusts is investigated. For typical plasma parameters relevant for experiments [J. Plasma Phys. \\textbf{60}, 69 (1998)], when the beam speed is larger than the DIA speed ($v_{b0}\\gtrsim1.7c_s$), three stable waves, namely the "fast" and "slow" ion-beam modes and the plasma DIA wave are shown to exist. These modes can propagate as SWs in the beam plasmas. However, in the other regime ($c_s0)$ is found to be limited by a critical value which typically depends on $M$, $v_{b0}$ as well as the ion/beam temperature. The conditions for the existence of DIA solitons are obtained and their properties are analyzed numerically in terms of the system parameters. While the system supports both the compressive and rarefactive large amplitude SWs, the small amplitude solitons exist only of the compressive type. The theoretical results may be useful for observation of soliton excitations in l...
Van Aggelen, Helen; Bultinck, Patrick; Verstichel, Brecht; Van Neck, Dimitri; Ayers, Paul W
2009-07-21
The behaviour of diatomic molecules is examined using the variational second-order density matrix method under the P, Q and G conditions. It is found that the method describes the dissociation limit incorrectly, with fractional charges on the well-separated atoms. This can be traced back to the behaviour of the energy versus the number of electrons for the isolated atoms. It is shown that the energies for fractional charges are much too low.
Thidé, B; Then, H; Tamburini, F
2010-01-01
Starting from Stratton-Panofsky-Phillips-Jefimenko equations for the electric and magnetic fields generated by completely arbitrary charge and current density distributions at rest, we derive far-zone approximations for the fields, containing all components, dominant as well as sub-dominant. Using these approximate formulas, we derive general formulas for the total electromagnetic linear momentum and angular momentum, valid at large distances from arbitrary, non-moving charge and current sources.
Coexistence of density wave and superfluid order in a dipolar Fermi gas
DEFF Research Database (Denmark)
Wu, Zhigang; Block, Jens Kusk; Bruun, Georg M.
2015-01-01
We analyse the coexistence of superfluid and density wave (stripe) order in a quasi-two-dimensional gas of dipolar fermions aligned by an external field. Remarkably, the anisotropic nature of the dipolar interaction allows for such a coexistence in a large region of the zero temperature phase dia...
The Potential Energy Density in Transverse String Waves Depends Critically on Longitudinal Motion
Rowland, David R.
2011-01-01
The question of the correct formula for the potential energy density in transverse waves on a taut string continues to attract attention (e.g. Burko 2010 "Eur. J. Phys." 31 L71), and at least three different formulae can be found in the literature, with the classic text by Morse and Feshbach ("Methods of Theoretical Physics" pp 126-127) stating…
Time-dependent density-functional theory in the projector augmented-wave method
DEFF Research Database (Denmark)
Walter, Michael; Häkkinen, Hannu; Lehtovaara, Lauri
2008-01-01
We present the implementation of the time-dependent density-functional theory both in linear-response and in time-propagation formalisms using the projector augmented-wave method in real-space grids. The two technically very different methods are compared in the linear-response regime where we...
Orthogonality of embedded wave functions for different states in frozen-density embedding theory
Energy Technology Data Exchange (ETDEWEB)
Zech, Alexander; Wesolowski, Tomasz A. [Département de Chimie Physique, Université de Genève, 30 quai Ernest-Ansermet, CH-1211 Genève 4 (Switzerland); Aquilante, Francesco [Dipartimento di Chimica “G. Ciamician,” Università di Bologna, Via Selmi 2, IT-40126 Bologna (Italy)
2015-10-28
Other than lowest-energy stationary embedded wave functions obtained in Frozen-Density Embedding Theory (FDET) [T. A. Wesolowski, Phys. Rev. A 77, 012504 (2008)] can be associated with electronic excited states but they can be mutually non-orthogonal. Although this does not violate any physical principles — embedded wave functions are only auxiliary objects used to obtain stationary densities — working with orthogonal functions has many practical advantages. In the present work, we show numerically that excitation energies obtained using conventional FDET calculations (allowing for non-orthogonality) can be obtained using embedded wave functions which are strictly orthogonal. The used method preserves the mathematical structure of FDET and self-consistency between energy, embedded wave function, and the embedding potential (they are connected through the Euler-Lagrange equations). The orthogonality is built-in through the linearization in the embedded density of the relevant components of the total energy functional. Moreover, we show formally that the differences between the expectation values of the embedded Hamiltonian are equal to the excitation energies, which is the exact result within linearized FDET. Linearized FDET is shown to be a robust approximation for a large class of reference densities.
Chang, Lei; Li, Qingchong; Zhang, Huijie; Li, Yinghong; Wu, Yun; Zhang, Bailing; Zhuang, Zhong
2016-08-01
The effect of the radial density configuration in terms of width, edge gradient and volume gradient on the wave field and energy flow in an axially uniform helicon plasma is studied in detail. A three-parameter function is employed to describe the density, covering uniform, parabolic, linear and Gaussian profiles. It finds that the fraction of power deposition near the plasma edge increases with density width and edge gradient, and decays in exponential and “bump-on-tail” profiles, respectively, away from the surface. The existence of a positive second-order derivative in the volume density configuration promotes the power deposition near the plasma core, which to our best knowledge has not been pointed out before. The transverse structures of wave field and current density remain almost the same during the variation of density width and gradient, confirming the robustness of the m=1 mode observed previously. However, the structure of the electric wave field changes significantly from a uniform density configuration, for which the coupling between the Trivelpiece-Gould (TG) mode and the helicon mode is very strong, to non-uniform ones. The energy flow in the cross section of helicon plasma is presented for the first time, and behaves sensitive to the density width and edge gradient but insensitive to the volume gradient. Interestingly, the radial distribution of power deposition resembles the radial profile of the axial component of current density, suggesting the control of the power deposition profile in the experiment by particularly designing the antenna geometry to excite a required axial current distribution. supported by National Natural Science Foundation of China (No. 11405271)
Imteyaz, Shahla; Rafiuddin
2016-11-01
Polystyrene (PS) dispersed tin molybdate (TM) composite was prepared by sol-gel method. The membrane was characterized for its thermal stability by TG-DTA. SEM reveals the formation of composite material with uniform surface morphology. Crystallinity and phosphorylation of the membrane was confirmed by X-RD and FT-IR. Membrane potential of different monovalent electrolytes with varying concentration followed the order LiCl > NaCl > NH4Cl > KCl. Membrane potential increases with dilution of electrolytes confirming it to be cation selective in nature. The theoretical value of fixed charge density for the membrane was also evaluated from membrane potential using different approaches proposed by (a) Teorell-Meyer-Sievers (b) Kobatake and (c) Nagasawa, which are comparable with the experimental values. Fixed charge density examined for the electrolytes follows the order LiCl > NaCl > NH4Cl > KCl. Li+ ion shows highest value of fixed charge density in all the methods as the Donnan exclusion is highest for the electrolyte of smaller cation size. Transport number and mobility ratio for ion selectivity also increases with dilution. Membrane shows the lowest permselectivity for K+ while highest for Li+. The strong binding affinity of K+ counter-ion with fixed charge groups on the polymer decreases the membrane charge density and permselectivity. Thus, the membrane shows its applicability in various electro-membrane processes.
Probability Density Function for Waves Propagating in a Straight PEC Rough Wall Tunnel
Energy Technology Data Exchange (ETDEWEB)
Pao, H
2004-11-08
The probability density function for wave propagating in a straight perfect electrical conductor (PEC) rough wall tunnel is deduced from the mathematical models of the random electromagnetic fields. The field propagating in caves or tunnels is a complex-valued Gaussian random processing by the Central Limit Theorem. The probability density function for single modal field amplitude in such structure is Ricean. Since both expected value and standard deviation of this field depend only on radial position, the probability density function, which gives what is the power distribution, is a radially dependent function. The radio channel places fundamental limitations on the performance of wireless communication systems in tunnels and caves. The transmission path between the transmitter and receiver can vary from a simple direct line of sight to one that is severely obstructed by rough walls and corners. Unlike wired channels that are stationary and predictable, radio channels can be extremely random and difficult to analyze. In fact, modeling the radio channel has historically been one of the more challenging parts of any radio system design; this is often done using statistical methods. In this contribution, we present the most important statistic property, the field probability density function, of wave propagating in a straight PEC rough wall tunnel. This work only studies the simplest case--PEC boundary which is not the real world but the methods and conclusions developed herein are applicable to real world problems which the boundary is dielectric. The mechanisms behind electromagnetic wave propagation in caves or tunnels are diverse, but can generally be attributed to reflection, diffraction, and scattering. Because of the multiple reflections from rough walls, the electromagnetic waves travel along different paths of varying lengths. The interactions between these waves cause multipath fading at any location, and the strengths of the waves decrease as the distance
Energy Technology Data Exchange (ETDEWEB)
Chung, H.M.; Nowicki, L.; Gazda, J. [Argonne National Lab., Chicago, IL (United States)] [and others
1995-04-01
The objective of this work is to determine void structure, distribution, and density changes of several promising vanadium-base alloys irradiated in the Dynamic Helium Charging Experiment (DHCE). Combined effects of dynamically charged helium and neutron damage on density change, void distribution, and microstructural evolution of V-4Cr-4Ti alloy have been determined after irradiation to 18-31 dpa at 425-600{degree}C in the DHCE, and the results compared with those from a non-DHCE in which helium generation was negligible.
Step density waves on growing vicinal crystal surfaces - Theory and experiment
Ranguelov, Bogdan; Müller, Pierre; Metois, Jean-Jacques; Stoyanov, Stoyan
2017-01-01
The Burton, Cabrera and Frank (BCF) theory plays a key conceptual role in understanding and modeling the crystal growth of vicinal surfaces. In BCF theory the adatom concentration on a vicinal surface obeys to a diffusion equation, generally solved within quasi-static approximation where the adatom concentration at a given distance x from a step has a steady state value n (x) . Recently, we show that going beyond this approximation (Ranguelov and Stoyanov, 2007) [6], for fast surface diffusion and slow attachment/detachment kinetics of adatoms at the steps, a train of fast-moving steps is unstable against the formation of steps density waves. More precisely, the step density waves are generated if the step velocity exceeds a critical value related to the strength of the step-step repulsion. This theoretical treatment corresponds to the case when the time to reach a steady state concentration of adatoms on a given terrace is comparable to the time for a non-negligible change of the step configuration leading to a terrace adatom concentration n (x , t) that depends not only on the terrace width, but also on its "past width". This formation of step density waves originates from the high velocity of step motion and has nothing to do with usual kinetic instabilities of step bunching induced by Ehrlich-Schwoebel effect, surface electromigration and/or the impact of impurities on the step rate. The so-predicted formation of step density waves is illustrated by numerical integration of the equations for step motion. In order to complete our previous theoretical treatment of the non-stationary BCF problem, we perform an in-situ reflection electron microscopy experiment at specific temperature interval and direction of the heating current, in which, for the first time, the step density waves instability is evidenced on Si(111) surface during highest possible Si adatoms deposition rates.
The imprint of crustal density heterogeneities on regional seismic wave propagation
Płonka, Agnieszka; Blom, Nienke; Fichtner, Andreas
2016-11-01
Density heterogeneities are the source of mass transport in the Earth. However, the 3-D density structure remains poorly constrained because travel times of seismic waves are only weakly sensitive to density. Inspired by recent developments in seismic waveform tomography, we investigate whether the visibility of 3-D density heterogeneities may be improved by inverting not only travel times of specific seismic phases but complete seismograms.As a first step in this direction, we perform numerical experiments to estimate the effect of 3-D crustal density heterogeneities on regional seismic wave propagation. While a finite number of numerical experiments may not capture the full range of possible scenarios, our results still indicate that realistic crustal density variations may lead to travel-time shifts of up to ˜ 1 s and amplitude variations of several tens of percent over propagation distances of ˜ 1000 km. Both amplitude and travel-time variations increase with increasing epicentral distance and increasing medium complexity, i.e. decreasing correlation length of the heterogeneities. They are practically negligible when the correlation length of the heterogeneities is much larger than the wavelength. However, when the correlation length approaches the wavelength, density-induced waveform perturbations become prominent. Recent regional-scale full-waveform inversions that resolve structure at the scale of a wavelength already reach this regime.Our numerical experiments suggest that waveform perturbations induced by realistic crustal density variations can be observed in high-quality regional seismic data. While density-induced travel-time differences will often be small, amplitude variations exceeding ±10 % are comparable to those induced by 3-D velocity structure and attenuation. While these results certainly encourage more research on the development of 3-D density tomography, they also suggest that current full-waveform inversions that use amplitude
Li, Yonghui; Ullrich, Carsten
2013-03-01
The time-dependent transition density matrix (TDM) is a useful tool to visualize and interpret the induced charges and electron-hole coherences of excitonic processes in large molecules. Combined with time-dependent density functional theory on a real-space grid (as implemented in the octopus code), the TDM is a computationally viable visualization tool for optical excitation processes in molecules. It provides real-time maps of particles and holes which gives information on excitations, in particular those that have charge-transfer character, that cannot be obtained from the density alone. Some illustration of the TDM and comparison with standard density difference plots will be shown for photoexcited organic donor-acceptor molecules. This work is supported by NSF Grant DMR-1005651
Kappatou, A.; Jaspers, R. J. E.; Delabie, E.; Marchuk, O.; Biel, W.; Jakobs, M. A.
2012-10-01
Investigation of impurity transport properties in tokamak plasmas is essential and a diagnostic that can provide information on the impurity content is required. Combining charge exchange recombination spectroscopy (CXRS) and beam emission spectroscopy (BES), absolute radial profiles of impurity densities can be obtained from the CXRS and BES intensities, electron density and CXRS and BES emission rates, without requiring any absolute calibration of the spectra. The technique is demonstrated here with absolute impurity density radial profiles obtained in TEXTOR plasmas, using a high efficiency charge exchange spectrometer with high etendue, that measures the CXRS and BES spectra along the same lines-of-sight, offering an additional advantage for the determination of absolute impurity densities.
Energy Technology Data Exchange (ETDEWEB)
Kappatou, A.; Delabie, E. [FOM Institute DIFFER - Dutch Institute for Fundamental Energy Research, Association EURATOM-FOM, 3430 BE Nieuwegein (Netherlands); Jaspers, R. J. E.; Jakobs, M. A. [Science and Technology of Nuclear Fusion, Eindhoven University of Technology, 5600 MB Eindhoven (Netherlands); Marchuk, O.; Biel, W. [Institute for Energy and Climate Research, Forschungszentrum Julich GmbH, Trilateral Euregio Cluster, 52425 Julich (Germany)
2012-10-15
Investigation of impurity transport properties in tokamak plasmas is essential and a diagnostic that can provide information on the impurity content is required. Combining charge exchange recombination spectroscopy (CXRS) and beam emission spectroscopy (BES), absolute radial profiles of impurity densities can be obtained from the CXRS and BES intensities, electron density and CXRS and BES emission rates, without requiring any absolute calibration of the spectra. The technique is demonstrated here with absolute impurity density radial profiles obtained in TEXTOR plasmas, using a high efficiency charge exchange spectrometer with high etendue, that measures the CXRS and BES spectra along the same lines-of-sight, offering an additional advantage for the determination of absolute impurity densities.
Gangopadhyay, Sunandan; Saha, Swarup
2014-01-01
Interaction of a charged particle in a static magnetic background, i.e., a Landau system with circularly polarised gravitational wave (GW) is studied quantum mechanically in the long wavelength and low velocity limit. We quantize the classical Hamiltonian following \\cite{speli}. The rotating polarization vectors of the circularly polarized GW are employed to form a unique directional triad which served as the coordinate axes. The Schrodinger equations for the system are cast in the form of a set of coupled linear differential equations. This system is solved by iterative technique. We compute the time-evolution of the position and momentum expectation values of the particle. The results show that the resonance behaviour obtained earlier\\cite{emgw_classical} by classical treatements of the system has a quantum analogue not only for the linearly polarized GW \\cite{emgw_1_lin}, but for circularly polarized GW as well.
Modulation of waves due to charge-exchange collisions in magnetized partially ionized space plasma
Shaikh, Dastgeer
2010-01-01
A nonlinear time dependent fluid simulation model is developed that describes the evolution of magnetohydrodynamic waves in the presence of collisional and charge exchange interactions of a partially ionized plasma. The partially ionized plasma consists of electrons, ions and a significant number of neutral atoms. In our model, the electrons and ions are described by a single fluid compressible magnetohydrodynamic (MHD) model and are coupled self-consistently to the neutral gas, described by the compressible hydrodynamic equations. Both the plasma and neutral fluids are treated with different energy equations that describe thermal energy exchange processes between them. Based on our self-consistent model, we find that propagating Alfv\\'enic and fast/slow modes grow and damp alternately through a nonlinear modulation process. The modulation appears to be robust and survives strong damping by the neutral component.
Modulation of waves due to charge-exchange collisions in magnetized partially ionized space plasma
Energy Technology Data Exchange (ETDEWEB)
Shaikh, Dastgeer, E-mail: dastgeer.shaikh@uah.ed [Department of Physics and Center for Space Plasma and Aeronomy Research, University of Alabama in Huntsville, Huntsville, AL 35899 (United States); Zank, G.P. [Department of Physics and Center for Space Plasma and Aeronomy Research, University of Alabama in Huntsville, Huntsville, AL 35899 (United States)
2010-10-04
A nonlinear time dependent fluid simulation model is developed that describes the evolution of magnetohydrodynamic waves in the presence of collisional and charge exchange interactions of a partially ionized plasma. The partially ionized plasma consists of electrons, ions and a significant number of neutral atoms. In our model, the electrons and ions are described by a single fluid compressible magnetohydrodynamic (MHD) model and are coupled self-consistently to the neutral gas, described by the compressible hydrodynamic equations. Both the plasma and neutral fluids are treated with different energy equations that describe thermal energy exchange processes between them. Based on our self-consistent model, we find that propagating Alfvenic and fast/slow modes grow and damp alternately through a nonlinear modulation process. The modulation appears to be robust and survives strong damping by the neutral component.
Energy Technology Data Exchange (ETDEWEB)
Mayout, Saliha; Tribeche, Mouloud, E-mail: mouloudtribeche@yahoo.fr [Plasma Physics Group (PPG), Theoretical Physics Laboratory (TPL), Faculty of Sciences- Physics, University of Bab-Ezzouar, U.S.T.H.B, B.P. 32, El Alia, Algiers 16111 (Algeria); Sahu, Biswajit [Department of Mathematics, West Bengal State University, Barasat, Kolkata-700126 (India)
2015-12-15
A theoretical study on the nonlinear propagation of nonplanar (cylindrical and spherical) dust ion-acoustic solitary waves (DIASW) is carried out in a dusty plasma, whose constituents are inertial ions, superthermal electrons, and charge fluctuating stationary dust particles. Using the reductive perturbation theory, a modified Korteweg-de Vries equation is derived. It is shown that the propagation characteristics of the cylindrical and spherical DIA solitary waves significantly differ from those of their one-dimensional counterpart.
Shekhar, Himanshu; Tzabari, Lior; Solomeshch, Olga; Tessler, Nir
2016-10-01
We have investigated the influence of the active layer thickness on the balance of the internal mechanisms affecting the efficiency of copper phthalocyanine - fullerene (C60) based vacuum deposited bulk heterojunction organic photocell. We fabricated a range of devices for which we varied the thickness of the active layer from 40 to 120 nm and assessed their performance using optical and electrical characterization techniques. As reported previously for phthalocyanine:C60, the performance of the device is highly dependent on the active layer thickness and of all the thicknesses we tried, the 40 nm thin active layer device showed the best solar cell characteristic parameters. Using the transfer matrix based optical model, which includes interference effects, we calculated the optical power absorbed in the active layers for the entire absorption band, and we found that this cannot explain the trend with thickness. Measurement of the cell quantum efficiency as a function of light intensity showed that the relative weight of the device internal processes changes when going from 40 nm to 120 nm thick active layer. Electrical modeling of the device, which takes different internal processes into account, allowed to quantify the changes in the processes affecting the generation - recombination balance. Sub gap external quantum efficiency and morphological analysis of the surface of the films agree with the model's result. We found that as the thickness grows the density of charge transfer states and of dark carriers goes up and the uniformity in the vertical direction is reduced.
Maity, N. P.; Thakur, R. R.; Maity, Reshmi; Thapa, R. K.; Baishya, S.
2016-10-01
In this paper, the interface charge densities (Dit) are studied and analyzed for ultra thin dielectric metal oxide semiconductor (MOS) devices using different high-k dielectric materials such as Al2O3, ZrO2 and HfO2. The Dit have been calculated by a new approach using conductance method and it indicates that by reducing the thickness of the oxide, the Dit increases and similar increase is also found by replacing SiO2 with high-k. For the same oxide thickness, SiO2 has the lowest Dit and found to be the order of 1011cm-2eV-1. Linear increase in Dit has been observed as the dielectric constant of the oxide increases. The Dit is found to be in good agreement with published fabrication results at p-type doping level of 1×1017cm-3. Numerical calculations and solutions are performed by MATLAB and device simulation is done by ATLAS.
Scivetti, Iván; Persson, Mats
2013-09-01
As a first step to meet the challenge to calculate the electronic structure and total energy of charged states of atoms and molecules adsorbed on ultrathin insulating films supported by a metallic substrate using density functional theory (DFT), we have developed a simplified new DFT scheme that only describes the electrostatic interaction of an external charged system with a metal surface. This purely electrostatic interaction is obtained from the assumption that the electron densities of the two fragments (charged system and metal surface) are non-overlapping and by neglecting non-local exchange-correlation effects such as the van der Waals interactions between the two fragments. In addition, the response of the metal surface to the electrostatic potential from the charged system is treated to linear order, whereas the charged system is treated fully within DFT. In particular, we consider the classical perfect conductor model for the metal response, although our formalism is not limited to this approximation. To test the computational implementation of this new scheme, we have considered the case of a Na+ cation interacting with a perfect conductor. The application of this new methodology to realistic problems involving charged systems adsorbed on insulating films supported by a metal surface are deferred to a separate following publication.
Density bump formation in a collisionless electrostatic shock wave in a laser-ablated plasma
Garasev, M A; Kocharovsky, V V; Malkov, Yu A; Murzanev, A A; Nechaev, A A; Stepanov, A N
2016-01-01
The emergence of a density bump at the front of a collisionless electrostatic shock wave have been observed experimentally during the ablation of an aluminium foil by a femtosecond laser pulse. We have performed numerical simulations of the dynamics of this phenomena developing alongside the generation of a package of ion-acoustic waves, exposed to a continual flow of energetic electrons, in a collisionless plasma. We present the physical interpretation of the observed effects and show that the bump consists of transit particles, namely, the accelerated ions from the dense plasma layer, and the ions from the diluted background plasma, formed by a nanosecond laser prepulse during the ablation.
Solitary Density Waves for Improved Traffic Flow Model with Variable Brake Distances
Institute of Scientific and Technical Information of China (English)
朱文兴; 丁瑞玲
2012-01-01
Traffic flow model is improved by introducing variable brake distances with varying slopes. Stability of the traffic flow on a gradient is analyzed and the neutral stability condition is obtained. The KdV （Korteweg-de Vries） equation is derived the use of nonlinear analysis and soliton solution is obtained in the meta-stable region. Solitary density waves are reproduced in the numerical simulations. It is found that as uniform headway is less than the safety distance solitary wave exhibits upward form, otherwise it exhibits downward form. In general the numerical results are in good agreement with the analytical results.
Yin, W.-L.
1984-04-01
It is shown that, in the case of non-zero charge density, the class of steady, plane, incompressible, aligned-fluid magnetofluiddynamic flows contains no rotational motions. Therefore, this class of flows is exhausted by the irrotational solutions of Kingston and Power.
Charge and current density profiles of a degenerate magnetized free-electron gas near a hard wall
M.M. Kettenis; L.G. Suttorp
1998-01-01
The charge and current densities of a completely degenerate free-electron gas in a uniform magnetic field are found to have a damped oscillatory spatial dependence near a wall that is parallel to the magnetic field. For large distances from the wall the behaviour of the associated profile functions
Kronoseismology: Using density waves in Saturn's C ring to probe the planet's interior
Hedman, M M
2013-01-01
Saturn's C ring contains multiple spiral patterns that appear to be density waves driven by periodic gravitational perturbations. In other parts of Saturn's rings, such waves are generated by Lindblad resonances with Saturn's various moons, but most of the wave-like C-ring features are not situated near any strong resonance with any known moon. Using stellar occultation data obtained by the Visual and Infrared Mapping Spectrometer (VIMS) onboard the Cassini spacecraft, we investigate the origin of six unidentified C-ring waves located between 80,900 and 87,200 km from Saturn's center. By measuring differences in the waves' phases among the different occultations, we are able to determine both the number of arms in each spiral pattern and the speeds at which these patterns rotate around the planet. We find that all six of these waves have between 2 and 4 arms and pattern speeds between 1660 degrees/day and 1861 degrees/day. These speeds are too large to be attributed to any satellite resonance. Instead they ar...
Institute of Scientific and Technical Information of China (English)
杨忠志; 王长生
2000-01-01
Based on the density functional theory and the atom-bond electronegativity equalization model (ABEEM), a method is proposed to construct the softness matrix and to obtain the electron population normal modes (PNMs) for a closed system. Using this method the information about the bond charge polarization in a molecule can be obtained easily. The test calculation shows that the PNM obtained by this method includes all the modes about the bond charge polarization explicitly. And the bond charge polarization mode characterized by the biggest eigenvalue, which is the softest one of all modes related with chemical bonds, can describe the charge polarization process in a molecule as exquisitely as the corresponding ab initio method.
Origin of charge density at LaAlO3-on-SrTiO3 heterointerfacespossibility of intrinsic doping
Energy Technology Data Exchange (ETDEWEB)
Siemons, W.
2010-04-29
As discovered by Ohtomo et al., a large sheet charge density with high mobility exists at the interface between SrTiO{sub 3} and LaAlO{sub 3}. Based on transport, spectroscopic and oxygen-annealing experiments, we conclude that extrinsic defects in the form of oxygen vacancies introduced by the pulsed laser deposition process used by all researchers to date to make these samples is the source of the large carrier densities. Annealing experiments show a limiting carrier density. We also present a model that explains the high mobility based on carrier redistribution due to an increased dielectric constant.
Density dependence of the /s-wave repulsion in pionic atoms
Friedman, E.
2002-11-01
Several mechanisms of density dependence of the s-wave repulsion in pionic atoms, beyond the conventional model, are tested by parameter fits to a large (106 points) set of data from 16O to 238U, including 'deeply bound' states in 205Pb. Special attention is paid to the proper choice of nuclear density distributions. A density-dependent isovector scattering amplitude suggested recently by Weise to result from a density dependence of the pion decay constant is introduced and found to account for most of the so-called anomalous repulsion. The presence of such an effect might indicate partial chiral symmetry restoration in dense matter. The anomalous repulsion is fully accounted for when an additional relativistic impulse approximation term is included in the potential.
Millimeter-Wave Line Ratios and Sub-beam Volume Density Distributions
Leroy, Adam K; Schruba, Andreas; Bigiel, Frank; Kruijssen, J M Diederik; Kepley, Amanda; Blanc, Guillermo A; Bolatto, Alberto D; Cormier, Diane; Gallagher, Molly; Hughes, Annie; Jimenez-Donaire, Maria J; Rosolowsky, Erik; Schinnerer, Eva
2016-01-01
We explore the use of mm-wave emission line ratios to trace molecular gas density when observations integrate over a wide range of volume densities within a single telescope beam. For observations targeting external galaxies, this case is unavoidable. Using a framework similar to that of Krumholz and Thompson (2007), we model emission for a set of common extragalactic lines from lognormal and power law density distributions. We consider the median density of gas producing emission and the ability to predict density variations from observed line ratios. We emphasize line ratio variations, because these do not require knowing the absolute abundance of our tracers. Patterns of line ratio variations have the prospect to illuminate the high-end shape of the density distribution, and to capture changes in the dense gas fraction and median volume density. Our results with and without a high density power law tail differ appreciably; we highlight better knowledge of the PDF shape as an important area. We also show th...
Incommensurate spin density wave in metallic V2-yO3
Bao, Wei; Broholm, C.; Carter, S. A.; Rosenbaum, T. F.; Aeppli, G.; Trevino, S. F.; Metcalf, P.; Honig, J. M.; Spalek, J.
1993-08-01
We show by neutron diffraction that metallic V2-7O3 develops a spin density wave below TN~=9 K with incommensurate wave vector q~=1.7c* and an ordered moment of 0.15μB. The weak ordering phenomenon is accompanied by strong, nonresonant spin fluctuations with a velocity c=67(4) meV Å. The spin correlations of the metal are very different from those of the insulator and place V2-yO3 in a distinct class of Motte-Hubbard systems where the wave vector for magnetic order in the metal is far from a high symmetry commensurate reciprocal lattice point.
Linear-scaling density functional theory using the projector augmented wave method
Hine, Nicholas D. M.
2017-01-01
Quantum mechanical simulation of realistic models of nanostructured systems, such as nanocrystals and crystalline interfaces, demands computational methods combining high-accuracy with low-order scaling with system size. Blöchl’s projector augmented wave (PAW) approach enables all-electron (AE) calculations with the efficiency and systematic accuracy of plane-wave pseudopotential calculations. Meanwhile, linear-scaling (LS) approaches to density functional theory (DFT) allow for simulation of thousands of atoms in feasible computational effort. This article describes an adaptation of PAW for use in the LS-DFT framework provided by the ONETEP LS-DFT package. ONETEP uses optimisation of the density matrix through in situ-optimised local orbitals rather than the direct calculation of eigenstates as in traditional PAW approaches. The method is shown to be comparably accurate to both PAW and AE approaches and to exhibit improved convergence properties compared to norm-conserving pseudopotential methods.
Protoplanetary Disk Heating and Evolution Driven by the Spiral Density Waves
Rafikov, Roman R
2016-01-01
High-resolution imaging of some protoplanetary disks in scattered light reveals presence of the global spiral arms of significant amplitude, likely excited by massive planets or stellar companions. Assuming that these arms are density waves, evolving into spiral shocks, we assess their effect on the thermodynamics, accretion, and global evolution of the disk. We derive analytical expressions for the direct (irreversible) heating, angular momentum transport, and mass accretion rate induced by the disk shocks of arbitrary strength. We find these processes to be very sensitive to the shock amplitude. Focusing on the waves of moderate strength (density jump at the shock $\\Delta\\Sigma/\\Sigma\\sim 1$) we show the associated disk heating to be negligible (contributing at $\\sim 1\\%$ level to the energy budget) in passive, irradiated protoplanetary disks on $\\sim 100$ AU scales, but becoming important within several AU from the star. At the same time, shock heating can be a significant (or even dominant) energy source ...
Chiral density wave versus pion condensation in the 1+1 dimensional NJL model
Adhikari, Prabal
2016-01-01
In this paper, we study the possibility of an inhomogeneous quark condensate in the 1+1 dimensional Nambu-Jona-Lasinio model in the large-$N_c$ limit at finite temperature $T$ and quark chemical potential $\\mu$ using dimensional regularization. The phase diagram in the $\\mu$--$T$ plane is mapped out. At zero temperature, an inhomogeneous phase with a chiral-density wave exists for all values of $\\mu>\\mu_c$. Performing a Ginzburg-Landau analysis, we show that in the chiral limit, the critical point and the Lifschitz point coincide. We also consider the competition between a chiral-density wave and a constant pion condensate at finite isospin chemical potential $\\mu_I$. The phase diagram in the $\\mu_I$--$\\mu$ plane is mapped out and shows a rich phase structure.
Testing Density Wave Theory with Resolved Stellar Populations around Spiral Arms in M81
Choi, Yumi; Williams, Benjamin F; Weisz, Daniel R; Skillman, Evan D; Fouesneau, Morgan; Dolphin, Andrew E
2015-01-01
Stationary density waves rotating at a constant pattern speed $\\Omega_{\\rm P}$ would produce age gradients across spiral arms. We test whether such age gradients are present in M81 by deriving the recent star formation histories (SFHs) of 20 regions around one of M81's grand-design spiral arms. For each region, we use resolved stellar populations to determine the SFH by modeling the observed color-magnitude diagram (CMD) constructed from archival Hubble Space Telescope (HST) F435W and F606W imaging. Although we should be able to detect systematic time delays in our spatially-resolved SFHs, we find no evidence of star formation propagation across the spiral arm. Our data therefore provide no convincing evidence for a stationary density wave with a single pattern speed in M81, and instead favor the scenario of kinematic spiral patterns that are likely driven by tidal interactions with the companion galaxies M82 and NGC 3077.